FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Wang, H Whittaker-Brooks, L Fleming, GR AF Wang, He Whittaker-Brooks, Luisa Fleming, Graham R. TI Exciton and Free Charge Dynamics of Methylammonium Lead Iodide Perovskites Are Different in the Tetragonal and Orthorhombic Phases SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLAR-CELLS; CARRIER MOBILITY; EFFICIENCY; CH3NH3PBI3; SEMICONDUCTORS; RECOMBINATION; TEMPERATURE; LENGTHS; FILMS; BR AB The small exciton binding energy of perovskite suggests that the long-lived photoluminescence and slow recovery of the ground state bleaching of the tetragonal phase at room temperature results primarily from the decay of free charges rather than the decay of the initially created excitons. Here we demonstrate the ground state bleaching recovery of the orthorhombic phase of methylammonium lead iodide (CH3NH3PbI3) is much faster than that of the tetragonal phase using temperature dependent transient absorption spectroscopy. The distribution in orientation of the methylammonium group which is disordered in the tetragonal phase and ordered in the orthorhombic phase results in smaller dielectric constant and larger exciton binding energy in the latter phase. We observe the recovery of the ground state bleaching in the orthorhombic phase to be comprised of decays of both excitons and free charges. Our findings suggest CH3NH3PbI3 behaves like a nonexcitonic semiconductor in the tetragonal phase and an excitonic semiconductor in the orthorhombic phase. C1 [Wang, He; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Wang, He; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Wang, He; Fleming, Graham R.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Wang, He; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Whittaker-Brooks, Luisa] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM fleming@cchem.berkeley.edu FU National Science Foundation (NSF) [CHE-1012168, CHE-1362830] FX This work was supported by the National Science Foundation (NSF) under Awards CHE-1012168 and CHE-1362830. NR 32 TC 19 Z9 19 U1 2 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 27 PY 2015 VL 119 IS 34 BP 19590 EP 19595 DI 10.1021/acs.jpcc.5b04403 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CQ2FP UT WOS:000360415700003 ER PT J AU Hopper, EM Perret, E Ingram, BJ You, H Chang, KC Baldo, PM Fuoss, PH Eastman, JA AF Hopper, E. Mitchell Perret, Edith Ingram, Brian J. You, Hoydoo Chang, Kee-Chul Baldo, Peter M. Fuoss, Paul H. Eastman, Jeffrey A. TI Oxygen Exchange in La0.6Sr0.4Co0.2Fe0.8O3-delta Thin-Film Heterostructures under Applied Electric Potential SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOPED CERIUM OXIDE; DOUBLE-LAYER CATHODES; SURFACE EXCHANGE; CGO ELECTROLYTES; PART I; REDUCTION; DIFFUSION; KINETICS; MODEL; LSCF AB In situ synchrotron X-ray diffraction was used to investigate oxygen surface exchange behavior in La0.6Sr0.4Co0.2Fe0.8O3-delta/Gd2O3-doped CeO2/Y2O3-stabilized ZrO2 (LSCF/GDC/YSZ) epitaxial thin-film heterostructures. Applying electrical potentials across the heterostructure under high temperature and controlled oxygen partial pressure conditions resulted in significant changes in oxygen vacancy concentrations due to differing rates of oxygen transport across the LSCF/air surface and LSCF/GDC buried interface. These changes in stoichiometry were correlated with time-dependent out-of-plane LSCF lattice parameter changes. An electrochemical reaction rate analysis was used to determine that the rate constant associated with oxygen exchange at the LSCF/air surface dominates the behavior of the sample as a whole and that the rate of oxygen transport across the LSCF/air surface is smaller than or equal to the rate of oxygen transport across the buried LSCF/GDC interface. C1 [Hopper, E. Mitchell; Perret, Edith; You, Hoydoo; Chang, Kee-Chul; Baldo, Peter M.; Fuoss, Paul H.; Eastman, Jeffrey A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Ingram, Brian J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Ingram, BJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ingram@anl.gov RI You, Hoydoo/A-6201-2011 OI You, Hoydoo/0000-0003-2996-9483 FU Solid State Energy Conversion Alliance (SECA) program; Fossil Energy Program of the U.S. Department of Energy; Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy; DOE Office of Science [DE-AC02-06CH11357] FX This work was supported by the Solid State Energy Conversion Alliance (SECA) program and Fossil Energy Program of the U.S. Department of Energy (E.M.H., K-C.C., B.J.I.), as well as by Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy (P.M.B., E.P., J.A.E., P.H.F., H.Y.). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 30 TC 1 Z9 1 U1 5 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 27 PY 2015 VL 119 IS 34 BP 19915 EP 19921 DI 10.1021/acs.jpcc.5b05505 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CQ2FP UT WOS:000360415700041 ER PT J AU Henderson, MA AF Henderson, Michael A. TI Photochemical Outcomes of Adsorbed Oxygen: Desorption, Dissociation, and Passivation by Coadsorbed Water SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; RUTILE TIO2(110); O-2 PHOTODESORPTION; LEED CRYSTALLOGRAPHY; SURFACE-STRUCTURE; TITANIUM-DIOXIDE; OXIDE SURFACES; ADSORPTION; FE3O4(111); OXIDATION AB A mixed Fe + Cr oxide surface was used to explore the photochemical fate of adsorbed O-2 under ultra-high-vacuum conditions. The mixed oxide surface possessed a magnetite-like (111) structure based on low-energy electron diffraction, with its chemical behavior resembling that of Fe3O4(111). Oxygen adsorption at 40 K resulted in two chemisorption states, a strongly bound form desorbing in temperature-programmed desorption (TPD) at 230 K and a weakly bound form evolving at 100 K. The former was assigned to charge transfer adsorption at Fe2+ sites and the latter to electrostatic binding at Fe" sites. A minority state was also detected at similar to 160 K and tentatively assigned to adsorption at Cr3+ sites. The 230 K O-2 state was the focus of photochemical studies employing four wavelengths of light from the red to the UV. Irrespective of wavelength, O-2 molecules in the 230 K state preferentially photodesorbed when irradiated, with comparable rates across the visible and an order of magnitude higher in the UV. Approximately 10% of adsorbed O-2 irreversibly photodissociated, irrespective of wavelength, with the resulting fragments blocking access to both Fe3+ and Fe2+ sites for subsequent O-2 adsorption. Preadsorbed water also blocked O-2 adsorption, but postadsorbed water stabilized O-2 at Fe2+ sites in TPD to 285 K. The water-stabilized O-2 molecules were insensitive to photodesorption. O-2 photodissociation and photopassivation both represent potentially adverse outcomes in the release of O-2 during the heterogeneous water photooxidation reaction. C1 Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Henderson, MA (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-87, Richland, WA 99352 USA. EM ma.henderson@pnnl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research FX The author thanks Drs. Sara Chamberlin and Scott Chambers for supplying the film used in this work. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for the DOE by Battelle. The research reported here was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 67 TC 4 Z9 4 U1 4 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 27 PY 2015 VL 119 IS 34 BP 19976 EP 19986 DI 10.1021/acs.jpcc.5b05972 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CQ2FP UT WOS:000360415700049 ER PT J AU Bottoni, S Leoni, S Fornal, B Raabe, R Rusek, K Benzoni, G Bracco, A Crespi, FCL Morales, AI Bednarczyk, P Cieplicka-Orynczak, N Krolas, W Maj, A Szpak, B Callens, M Bouma, J Elseviers, J De Witte, H Flavigny, F Orlandi, R Reiter, P Seidlitz, M Warr, N Siebeck, B Hellgartner, S Mucher, D Pakarinen, J Vermeulen, M Bauer, C Georgiev, G Janssens, RVF Balabanski, D Sferrazza, M Kowalska, M Rapisarda, E Voulot, D Benito, ML Wenander, F AF Bottoni, S. Leoni, S. Fornal, B. Raabe, R. Rusek, K. Benzoni, G. Bracco, A. Crespi, F. C. L. Morales, A. I. Bednarczyk, P. Cieplicka-Orynczak, N. Krolas, W. Maj, A. Szpak, B. Callens, M. Bouma, J. Elseviers, J. De Witte, H. Flavigny, F. Orlandi, R. Reiter, P. Seidlitz, M. Warr, N. Siebeck, B. Hellgartner, S. Muecher, D. Pakarinen, J. Vermeulen, M. Bauer, C. Georgiev, G. Janssens, R. V. F. Balabanski, D. Sferrazza, M. Kowalska, M. Rapisarda, E. Voulot, D. Benito, M. Lozano Wenander, F. TI Cluster-transfer reactions with radioactive beams: A spectroscopic tool for neutron-rich nuclei SO PHYSICAL REVIEW C LA English DT Article ID REX-ISOLDE; FUSION; LI-6,LI-7; BREAKUP AB An exploratory experiment performed at REX-ISOLDE to investigate cluster-transfer reactions with radioactive beams in inverse kinematics is presented. The aim of the experiment was to test the potential of cluster-transfer reactions at the Coulomb barrier as a mechanism to explore the structure of exotic neutron-rich nuclei. The reactions Li-7(Rb-98, alpha xn) and Li-7(Rb-98, txn) were studied through particle-gamma coincidence measurements, and the results are presented in terms of the observed excitation energies and spins. Moreover, the reaction mechanism is qualitatively discussed as a transfer of a clusterlike particle within a distorted-wave Born approximation framework. The results indicate that cluster-transfer reactions can be described well as a direct process and that they can be an efficient method to investigate the structure of neutron-rich nuclei at medium-high excitation energies and spins. C1 [Bottoni, S.; Leoni, S.; Bracco, A.; Crespi, F. C. L.] Univ Milan, I-20133 Milan, Italy. [Bottoni, S.; Leoni, S.; Benzoni, G.; Bracco, A.; Crespi, F. C. L.; Morales, A. I.; Cieplicka-Orynczak, N.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Bottoni, S.; Raabe, R.; Callens, M.; Bouma, J.; Elseviers, J.; De Witte, H.; Flavigny, F.; Orlandi, R.] Katholieke Univ Leuven, Inst Kern Stralingsfys, B-3001 Leuven, Belgium. [Fornal, B.; Bednarczyk, P.; Cieplicka-Orynczak, N.; Krolas, W.; Maj, A.; Szpak, B.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Rusek, K.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Flavigny, F.] Univ Paris 11, Inst Phys Nucl Orsay, CNRS, IN2P3, F-91406 Orsay, France. [Orlandi, R.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Reiter, P.; Seidlitz, M.; Warr, N.; Siebeck, B.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Hellgartner, S.; Muecher, D.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Pakarinen, J.] Univ Jyvaskyla, FIN-40014 Jyvaskyla, Finland. [Vermeulen, M.] Univ York, Dept Phys, Nucl Phys Grp, York YO10 5DD, N Yorkshire, England. [Bauer, C.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. [Georgiev, G.] Univ Paris 11, CSNSM, IN2P3, CNRS,UMR8609, F-91405 Orsay, France. [Janssens, R. V. F.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Balabanski, D.] Hora Hulubei Natl Inst Phys & Nucl Engn, ELI NP, Magurele 077125, Romania. [Sferrazza, M.] Univ Libre Bruxelles, Dept Phys, B-1050 Brussels, Belgium. [Kowalska, M.; Rapisarda, E.; Voulot, D.; Benito, M. Lozano; Wenander, F.] CERN, CH-1211 Geneva 23, Switzerland. RP Leoni, S (reprint author), Univ Milan, I-20133 Milan, Italy. EM silvia.leoni@mi.infn.it RI Morales Lopez, Ana Isabel/A-2445-2017; Georgiev, Georgi/C-5110-2008 OI Morales Lopez, Ana Isabel/0000-0002-6665-0925; benzoni, giovanna/0000-0002-7938-0338; Pakarinen, Janne/0000-0001-8944-8757; Georgiev, Georgi/0000-0003-1467-1764 FU Istituto Nazionale di Fisica Nucleare (INFN-Italy); FWO-Vlaanderen (Belgium); BOF KU Leuven [GOA/2010/010]; Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office [P7/12]; Polish Ministry of Science and Higher Education [N-N202-263238]; European Commission [RII3-CT-2010-262010]; German BMBF [06K-167, 06KY205I, 05P09PKCI5, 05P12PKFNE]; US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; European Commission through the Marie Curie Actions [PIEFGA-2011-30096] FX This work was funded by Istituto Nazionale di Fisica Nucleare (INFN-Italy), by FWO-Vlaanderen (Belgium), by Grant No. GOA/2010/010 (BOF KU Leuven), by the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), by the Polish Ministry of Science and Higher Education under Contract No. N-N202-263238, by the European Commission within the Seventh Framework Programme through I3-ENSAR (Contract No. RII3-CT-2010-262010), by the German BMBF (Contracts No. 06K-167, No. 06KY205I, No. 05P09PKCI5, and No. 05P12PKFNE), by the US Department of Energy, Office of Science, Office of Nuclear Physics under Contract No. DE-AC02-06CH11357, and by the European Commission through the Marie Curie Actions Contract No. PIEFGA-2011-30096. NR 45 TC 1 Z9 1 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 27 PY 2015 VL 92 IS 2 AR 024322 DI 10.1103/PhysRevC.92.024322 PG 8 WC Physics, Nuclear SC Physics GA CP8EA UT WOS:000360123600001 ER PT J AU Wang, BS Norman, EB Scielzo, ND Smith, AR Thomas, KJ Wender, SA AF Wang, B. S. Norman, E. B. Scielzo, N. D. Smith, A. R. Thomas, K. J. Wender, S. A. TI Cosmogenic-neutron activation of TeO2 and implications for neutrinoless double-beta decay experiments SO PHYSICAL REVIEW C LA English DT Article ID PARTIAL CROSS-SECTIONS; ENERGY NUCLEAR-REACTIONS; RAY INDUCED NEUTRONS; ASTROPHYSICAL APPLICATIONS; GERMANIUM DETECTOR; SPECTRUM; SIMULATION; TELLURIUM; TARGETS; YIELDS AB Flux-averaged cross sections for cosmogenic-neutron activation of natural tellurium were measured using a neutron beam containing neutrons of kinetic energies up to similar to 800 MeV and having an energy spectrum similar to that of cosmic-ray neutrons at sea level. Analysis of the radioisotopes produced reveals that Ag-110m will be a dominant contributor to the cosmogenic-activation background in experiments searching for neutrinoless double-beta decay of Te-130, such as the Cryogenic Underground Observatory for Rare Events (CUORE) and the Sudbury Neutrino Observatory Plus (SNO+). An estimate of the cosmogenic-activation background in the CUORE experiment has been obtained using the results of this measurement and cross-section measurements of proton activation of tellurium. Additionally, the measured cross sections in this work are also compared with results from semiempirical cross-section calculations. C1 [Wang, B. S.; Norman, E. B.; Thomas, K. J.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Norman, E. B.; Scielzo, N. D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Smith, A. R.; Thomas, K. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Wender, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Wang, BS (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. OI Wender, Stephen/0000-0002-2446-5115 FU Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC52- 06NA25396]; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U.S. Department of Energy Office of Defense Nuclear Nonproliferation [NA-22]; U.S. Department of Energy National Nuclear Security Administration [DE-NA0000979]; Nuclear Forensics Graduate Fellowship from the U.S. Department of Homeland Security [2012-DN-130-NF0001-02] FX We gratefully acknowledge the many valuable discussions with Maura Pavan and Silvia Capelli from the CUORE Collaboration. This work was supported by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, Los Alamos National Laboratory under Contract No. DE-AC52- 06NA25396, Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, the U.S. Department of Energy Office of Defense Nuclear Nonproliferation (NA-22), the U.S. Department of Energy National Nuclear Security Administration under Award No. DE-NA0000979, and the Nuclear Forensics Graduate Fellowship from the U.S. Department of Homeland Security under Grant Award No. 2012-DN-130-NF0001-02. The views and conclusions contained in this document are those of the authors and should not be interpreted as necessarily representing the official policies, either expressed or implied, of the U.S. Department of Homeland Security. NR 42 TC 3 Z9 3 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 27 PY 2015 VL 92 IS 2 AR 024620 DI 10.1103/PhysRevC.92.024620 PG 11 WC Physics, Nuclear SC Physics GA CP8EA UT WOS:000360123600004 ER PT J AU Song, YS Taruya, A Linder, E Koyama, K Sabiu, CG Zhao, GB Bernardeau, F Nishimichi, T Okumura, T AF Song, Yong-Seon Taruya, Atsushi Linder, Eric Koyama, Kazuya Sabiu, Cristiano G. Zhao, Gong-Bo Bernardeau, Francis Nishimichi, Takahiro Okumura, Teppei TI Consistent modified gravity analysis of anisotropic galaxy clustering using BOSS DR11 SO PHYSICAL REVIEW D LA English DT Article ID OSCILLATION SPECTROSCOPIC SURVEY; DIGITAL SKY SURVEY; REDSHIFT-SPACE DISTORTIONS; SDSS-III; GROWTH; EXPANSION; UNIVERSE; SAMPLE; BIAS AB We analyze the clustering of a cosmic large scale structure using a consistent modified gravity perturbation theory, accounting for anisotropic effects along and transverse to the line of sight. The growth factor has a particular scale dependence in f(R) gravity and we fit for the shape parameter f(R0) simultaneously with the distance and the large scale (general relativity) limit of the growth function. Using more than 690,000 galaxies in the baryon oscillation spectroscopy survey data release 11, we find no evidence for extra scale dependence, with the 95% confidence upper limit vertical bar f(R0)vertical bar < 8 x 10(-4). Future clustering data, such as from the dark energy spectroscopic instrument, can use this consistent methodology to impose tighter constraints. C1 [Song, Yong-Seon; Sabiu, Cristiano G.] Korea Astron & Space Sci Inst, Taejon 305348, South Korea. [Taruya, Atsushi] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Taruya, Atsushi; Bernardeau, Francis; Nishimichi, Takahiro; Okumura, Teppei] Univ Tokyo, Univ Tokyo Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Taruya, Atsushi; Bernardeau, Francis; Nishimichi, Takahiro; Okumura, Teppei] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math, Kashiwa, Chiba 2778583, Japan. [Linder, Eric] Univ Calif Berkeley, Berkeley Lab, Berkeley, CA 94720 USA. [Linder, Eric] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Koyama, Kazuya; Zhao, Gong-Bo] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Zhao, Gong-Bo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. [Bernardeau, Francis; Nishimichi, Takahiro] CNRS, F-75014 Paris, France. [Bernardeau, Francis; Nishimichi, Takahiro] UPMC, UMR 7095, Inst Astrophys Paris, F-75014 Paris, France. [Nishimichi, Takahiro] JST, CREST, Kawaguchi, Saitama 3320012, Japan. RP Song, YS (reprint author), Korea Astron & Space Sci Inst, Taejon 305348, South Korea. EM ysong@kasi.re.kr FU U.S. DOE [DE-SC-0007867, DE-AC02-05CH11231]; Science and Technology Facilities Council [K00090X/1]; Japan Society for the Promotion of Science (JSPS) [26887012]; Strategic Priority Research Program "The Emergence of Cosmological Structures" of the Chinese Academy of Sciences [XDB09000000]; University of Portsmouth; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science FX Numerical calculations were performed by using a high performance computing cluster in the Korea Astronomy and Space Science Institute. E. L. was supported in part by U.S. DOE Grants No. DE-SC-0007867 and No. DE-AC02-05CH11231. K. K. is supported by the Science and Technology Facilities Council (Grant No. K00090X/1). T. N. was supported by JSPS Postdoctoral Fellowships for Research Abroad. T. O. was supported by Grant-in-Aid for Young Scientists (Start-up) from the Japan Society for the Promotion of Science (JSPS) (No. 26887012). G. B. Z. is supported by the Strategic Priority Research Program "The Emergence of Cosmological Structures" of the Chinese Academy of Sciences Grant No. XDB09000000, and by University of Portsmouth. We thank Marc Manera for providing the mock simulations. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. NR 59 TC 9 Z9 9 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 27 PY 2015 VL 92 IS 4 AR 043522 DI 10.1103/PhysRevD.92.043522 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CP8EY UT WOS:000360126200001 ER PT J AU Bragg, AD Ireland, PJ Collins, LR AF Bragg, Andrew D. Ireland, Peter J. Collins, Lance R. TI Mechanisms for the clustering of inertial particles in the inertial range of isotropic turbulence SO PHYSICAL REVIEW E LA English DT Article ID HOMOGENEOUS TURBULENCE; PLANETESIMAL FORMATION; AEROSOL-PARTICLES; HEAVY-PARTICLES; STATISTICS; VELOCITY; COLLISION; FLOW AB In this paper, we consider the physical mechanism for the clustering of inertial particles in the inertial range of isotropic turbulence. We analyze the exact, but unclosed, equation governing the radial distribution function (RDF) and compare the mechanisms it describes for clustering in the dissipation and inertial ranges. We demonstrate that in the limit St(r) << 1, where St(r) is the Stokes number based on the eddy turnover time scale at separation r, the clustering in the inertial range can be understood to be due to the preferential sampling of the coarse-grained fluid velocity gradient tensor at that scale. When St(r) greater than or similar to O(1) this mechanism gives way to a nonlocal clustering mechanism. These findings reveal that the clustering mechanisms in the inertial range are analogous to the mechanisms that we identified for the dissipation regime [see New J. Phys. 16, 055013 (2014)]. Further, we discuss the similarities and differences between the clustering mechanisms we identify in the inertial range and the "sweep-stick" mechanism developed by Coleman and Vassilicos [Phys. Fluids 21, 113301 (2009)]. We show that the idea that initial particles are swept along with acceleration stagnation points is only approximately true because there always exists a finite difference between the velocity of the acceleration stagnation points and the local fluid velocity. This relative velocity is sufficient to allow particles to traverse the average distance between the stagnation points within the correlation time scale of the acceleration field. We also show that the stick part of the mechanism is only valid for St(r) << 1 in the inertial range. We emphasize that our clustering mechanism provides the more fundamental explanation since it, unlike the sweep-stick mechanism, is able to explain clustering in arbitrary spatially correlated velocity fields. We then consider the closed, model equation for the RDF given in Zaichik and Alipchenkov [Phys. Fluids 19, 113308 (2007)] and use this, together with the results from our analysis, to predict the analytic form of the RDF in the inertial range for St(r) << 1, which, unlike that in the dissipation range, is not scale invariant. The results are in good agreement with direct numerical simulations, provided the separations are well within the inertial range. C1 [Bragg, Andrew D.; Ireland, Peter J.; Collins, Lance R.] Cornell Univ, Sibley Sch Mech & Aerosp Engn, Ithaca, NY 14853 USA. RP Bragg, AD (reprint author), Los Alamos Natl Lab, Appl Math & Plasma Phys Grp, POB 1663, Los Alamos, NM 87545 USA. EM adbragg265@gmail.com RI Bragg, Andrew/K-6099-2015 OI Bragg, Andrew/0000-0001-7068-8048 FU National Science Foundation [CBET-0967349]; National Science Foundation FX The authors acknowledge financial support from the National Science Foundation through Grant No. CBET-0967349 and through the Graduate Research Fellowship awarded to P.J.I. Computational simulations were performed on Yellow-stone [41] (ark:/85065/d7wd3xhc) at the US National Center for Atmospheric Research through its Computational and Information Systems Laboratory (sponsored by the National Science Foundation). NR 41 TC 4 Z9 4 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD AUG 27 PY 2015 VL 92 IS 2 AR 023029 DI 10.1103/PhysRevE.92.023029 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CP8FI UT WOS:000360127200007 PM 26382525 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A 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CA ATLAS Collaboration TI Measurements of the Total and Differential Higgs Boson Production Cross Sections Combining the H -> gamma gamma and H -> ZZ* -> 4l Decay Channels at root s=8 TeV with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTON DISTRIBUTIONS; GLUON-FUSION; LHC; QUARK AB Measurements of the total and differential cross sections of Higgs boson production are performed using 20.3 fb(-1) of pp collisions produced by the Large Hadron Collider at a center-of-mass energy of root s = 8 TeV and recorded by the ATLAS detector. Cross sections are obtained from measured H -> gamma gamma and H -> ZZ*. 4l event yields, which are combined accounting for detector efficiencies, fiducial acceptances, and branching fractions. Differential cross sections are reported as a function of Higgs boson transverse momentum, Higgs boson rapidity, number of jets in the event, and transverse momentum of the leading jet. 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J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Phys Dept, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.; Robson, A.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys 4, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, Inst Tech Informat, ZITI, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Fullana Torregrosa, E.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. 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P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bagiacchi, P.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Brau, J. E.; Brost, E.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hopkins, W. H.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Majewski, S.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Potter, C. T.; Ptacek, E.; Puzo, P.; Radloff, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Shamim, M.; Simion, S.; Sinev, N. B.; Strom, D. M.; Tanaka, R.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Haney, B.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrument & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Carvalho, J.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Benchekroun, D.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lanon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, IRFU, DSM, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Israel Inst Technol, Dept Phys, Tech, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Giordani, M. P.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; van der Geer, R.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; van der Geer, R.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; van der Geer, R.; Vos, M.] Univ Valencia, Dept Ingn Elect & Inst Microelect Barcelona IMB C, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; van der Geer, R.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maetttig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Stroehmer, R.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ, Dept Phys, Fresno, CA USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Taipei, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Mitsou, Vasiliki/D-1967-2009; Di Domenico, Antonio/G-6301-2011; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Boldyrev, Alexey/M-9684-2015; Nechaeva, Polina/N-1148-2015; Tikhomirov, Vladimir/M-6194-2015; Negrini, Matteo/C-8906-2014; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Livan, Michele/D-7531-2012 OI Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Mitsou, Vasiliki/0000-0002-1533-8886; Di Domenico, Antonio/0000-0001-8078-2759; Tikhomirov, Vladimir/0000-0002-9634-0581; Negrini, Matteo/0000-0003-0101-6963; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Livan, Michele/0000-0002-5877-0062 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 56 TC 8 Z9 8 U1 11 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 27 PY 2015 VL 115 IS 9 AR 091801 DI 10.1103/PhysRevLett.115.091801 PG 19 WC Physics, Multidisciplinary SC Physics GA CP8HP UT WOS:000360134200005 ER PT J AU Zeng, YN Zhao, S Wei, H Tucker, MP Himmel, ME Mosier, NS Meilan, R Ding, SY AF Zeng, Yining Zhao, Shuai Wei, Hui Tucker, Melvin P. Himmel, Michael E. Mosier, Nathan S. Meilan, Richard Ding, Shi-You TI In situ micro-spectroscopic investigation of lignin in poplar cell walls pretreated by maleic acid SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Lignin autofluorescence; Fluorescence lifetime imaging microscopy; Stimulated Raman scattering imaging; Lignin-carbohydrate complexes droplets ID LIFETIME IMAGING MICROSCOPY; EXTRACTED AUTOHYDROLYSIS LIGNIN; POPULUS-TREMULOIDES LIGNINS; RAMAN-SCATTERING MICROSCOPY; CORN STOVER; HEMICELLULOSE HYDROLYSIS; BIOCHEMICAL PROCESSES; LABEL-FREE; WOOD; BIOMASS AB Background: In higher plant cells, lignin provides necessary physical support for plant growth and resistance to attack by microorganisms. For the same reason, lignin is considered to be a major impediment to the process of deconstructing biomass to simple sugars by hydrolytic enzymes. The in situ variation of lignin in plant cell walls is important for better understanding of the roles lignin play in biomass recalcitrance. Results: A micro-spectroscopic approach combining stimulated Raman scattering microscopy and fluorescence lifetime imaging microscopy was employed to probe the physiochemical structure of lignin in poplar tracheid cell walls. Two forms of lignins were identified: loosely packed lignin, which had a long (4 ns) fluorescence lifetime and existed primarily in the secondary wall layers; and dense lignin, which had a short (0.5-1 ns) fluorescence lifetime and was present in all wall layers, including the cell corners, compound middle lamellae, and secondary wall. At low maleic acid concentration (0.025 and 0.05 M) pretreatment conditions, some of the dense lignin was modified to become more loosely packed. High acid concentration removed both dense and loosely packed lignins. These modified lignins reformed to make lignin-carbohydrate complex droplets containing either dense or loosely packed lignin (mostly from secondary walls) and were commonly observed on the cell wall surface. Conclusions: We have identified dense and loosely packed lignins in plant cell walls. During maleic acid pretreatment, both dense lignin droplets and loosely packed lignin droplets were formed. Maleic acid pretreatment more effectively removes loosely packed lignin in secondary walls which increases enzyme accessibility for digestion. C1 [Zeng, Yining; Zhao, Shuai; Wei, Hui; Himmel, Michael E.; Ding, Shi-You] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Tucker, Melvin P.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Mosier, Nathan S.] Purdue Univ, Dept Agr & Biol Engn, W Lafayette, IN 47907 USA. [Meilan, Richard] Purdue Univ, Dept Forestry & Nat Resources, W Lafayette, IN 47907 USA. RP Zeng, YN (reprint author), Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. EM yining.zeng@nrel.gov; sding@msu.edu FU Center for Direct Catalytic Conversion of Biomass to Biofuels, an Energy Frontier Research Center - US Department of Energy, Office of Science, Basic Energy Sciences (BES) [DE-SC0000997]; BioEnergy Science Center (BESC) - Office of Biological and Environmental Research (BER) in the DOE Office of Science; DOE Bioenergy Research Center - Office of Biological and Environmental Research (BER) in the DOE Office of Science; Genomic Science Program - Office of Biological and Environmental Research (BER) in the DOE Office of Science [ER181000] FX We thank Kathryn Ruckman for manuscript editing. The authors acknowledge research support from the Center for Direct Catalytic Conversion of Biomass to Biofuels, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences (BES) under Award # DE-SC0000997 for maleic acid pretreatment methodologies applied to biomass. Development of the micro-spectroscopy SRS method was supported by the BioEnergy Science Center (BESC), a DOE Bioenergy Research Center, and development of the FLIM method was supported by the Genomic Science Program (ER181000), both funded by the Office of Biological and Environmental Research (BER) in the DOE Office of Science. NR 60 TC 3 Z9 3 U1 9 U2 45 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 27 PY 2015 VL 8 AR 126 DI 10.1186/s13068-015-0312-1 PG 11 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CP8AP UT WOS:000360113000001 PM 26312066 ER PT J AU Piot, P AF Piot, Philippe TI PARTICLE PHYSICS Positrons ride the wave SO NATURE LA English DT Editorial Material ID PLASMA; ELECTRONS; ACCELERATION C1 [Piot, Philippe] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Piot, Philippe] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Piot, P (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. EM ppiot@niu.edu NR 6 TC 1 Z9 1 U1 2 U2 6 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 27 PY 2015 VL 524 IS 7566 BP 422 EP 423 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP7LN UT WOS:000360069300026 PM 26310761 ER PT J AU Young, L AF Young, Linda TI PHOTONICS A stable narrow-band X-ray laser SO NATURE LA English DT Editorial Material ID FREE-ELECTRON LASER; OPERATION C1 Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Young, L (reprint author), Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM young@anl.gov NR 16 TC 0 Z9 0 U1 4 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 27 PY 2015 VL 524 IS 7566 BP 424 EP 425 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP7LN UT WOS:000360069300028 PM 26310762 ER PT J AU Li, DH Lv, CX Liu, L Xia, YZ She, XL Guo, SJ Yang, DJ AF Li, Daohao Lv, Chunxiao Liu, Long Xia, Yanzhi She, Xilin Guo, Shaojun Yang, Dongjiang TI Egg-Box Structure in Cobalt Alginate: A New Approach to Multifunctional Hierarchical Mesoporous N-Doped Carbon Nanofibers for Efficient Catalysis and Energy Storage SO ACS CENTRAL SCIENCE LA English DT Article ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIALS; OXYGEN REDUCTION; BACTERIAL CELLULOSE; ELECTRODE MATERIAL; SUPERCAPACITORS; GRAPHENE; ELECTROCATALYST; NANOCOMPOSITE; CONVERSION AB Carbon nanomaterials with both doped heteroatom and porous structure represent a new class of carbon nanostructures for boosting electrochemical application, particularly sustainable electrochemical energy conversion and storage applications. We herein demonstrate a unique large-scale sustainable biomass conversion strategy for the synthesis of earth-abundant multifunctional carbon nanomaterials with well-defined doped heteroatom level and multimodal pores through pyrolyzing electrospinning renewable natural alginate. The key part for our chemical synthesis is that we found that the egg-box structure in cobalt alginate nanofiber can offer new opportunity to create large mesopores (similar to 10-40 nm) on the surface of nitrogen-doped carbon nanofibers. The as-prepared hierarchical carbon nanofibers with three-dimensional pathway for electron and ion transport are conceptually new as high-performance multifunctional electrochemical materials for boosting the performance of oxygen reduction reaction (ORR), lithium ion batteries (LIBs), and supercapacitors (SCs). In particular, they show amazingly the same ORR activity as commercial Pt/C catalyst and much better long-term stability and methanol tolerance for ORR than Pt/C via a four-electron pathway in alkaline electrolyte. They also exhibit a large reversible capacity of 625 mAh g(-1) at 1 A g(-1), good rate capability, and excellent cycling performance for LIBs, making them among the best in all the reported carbon nanomaterials. They also represent highly efficient carbon nanomaterials for SCs with excellent capacitive behavior of 197 F g(-1) at 1 A g(-1) and superior stability. The present work highlights the importance of biomass-derived multifunctional mesoporous carbon nanomaterials in enhancing electrochemical catalysis and energy storage. C1 [Li, Daohao; Lv, Chunxiao; Liu, Long; Xia, Yanzhi; She, Xilin; Yang, Dongjiang] Qingdao Univ, Collaborat Innovat Ctr Marine Biomass Fibers Mat, Coll Chem & Environm Engn, Qingdao 266071, Peoples R China. [Guo, Shaojun] Los Alamos Natl Lab, Phys Chem & Appl Spect, Los Alamos, NM 87545 USA. [Yang, Dongjiang] Griffith Univ, QMNC, Brisbane, Qld 4111, Australia. RP Yang, DJ (reprint author), Qingdao Univ, Collaborat Innovat Ctr Marine Biomass Fibers Mat, Coll Chem & Environm Engn, Qingdao 266071, Peoples R China. EM xiayzh@qdu.edu.cn; sguo@lanl.gov; d.yang@griffith.edu.au RI Guo, Shaojun/A-8449-2011; Griffith University, QMNC/I-5498-2013 OI Guo, Shaojun/0000-0002-5941-414X; NR 47 TC 28 Z9 28 U1 64 U2 107 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD AUG 26 PY 2015 VL 1 IS 5 BP 261 EP 269 DI 10.1021/acscentsci.5b00191 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CX8QN UT WOS:000365968800009 PM 27162980 ER PT J AU Gliga, S Kakay, A Heyderman, LJ Hertel, R Heinonen, OG AF Gliga, Sebastian Kakay, Attila Heyderman, Laura J. Hertel, Riccardo Heinonen, Olle G. TI Broken vertex symmetry and finite zero-point entropy in the artificial square ice ground state SO PHYSICAL REVIEW B LA English DT Article ID SPIN-ICE AB We study degeneracy and entropy in the ground state of artificial square ice. In theoretical models, individual nanomagnets are typically treated as single spins with only two degrees of freedom, leading to a twofold degenerate ground state with intensive entropy and thus no zero-point entropy. Here, we show that the internal degrees of freedom of the nanostructures can result, through edge bending of the magnetization and breaking of local magnetic symmetry at the vertices, in a transition to a highly degenerate ground state with finite zero-point entropy, similar to that of the pyrochlore spin ices. We find that these additional degrees of freedom have observable consequences in the resonant spectrum of the lattice, and predict the occurrence of edge "melting" above a critical temperature at which the magnetic symmetry is restored. C1 [Gliga, Sebastian; Heyderman, Laura J.] Swiss Fed Inst Technol, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland. [Gliga, Sebastian; Heyderman, Laura J.] Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland. [Kakay, Attila] Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, D-01328 Dresden, Germany. [Hertel, Riccardo] Univ Strasbourg, CNRS UMR 7504, Inst Phys & Chim Mat Strasbourg, F-67034 Strasbourg, France. [Heinonen, Olle G.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Heinonen, Olle G.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Gliga, S (reprint author), Swiss Fed Inst Technol, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland. EM sebastian.gliga@psi.ch RI Heyderman, Laura/E-7959-2015; Hertel, Riccardo/H-9964-2016; Hertel, Riccardo/P-5806-2016; OI Hertel, Riccardo/0000-0002-0646-838X; Hertel, Riccardo/0000-0002-0646-838X; Heinonen, Olle/0000-0002-3618-6092 FU Department of Energy, Office of Science, Materials Science and Engineering Division FX S.G. wishes to thank Armin Kleibert for fruitful discussions about the experimental implications of this work and Gino Hrkac for helpful suggestions. The work by O.G.H. was supported by the Department of Energy, Office of Science, Materials Science and Engineering Division. We gratefully acknowledge the computing resources provided on Blues and Fusion, high-performance computing clusters operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 23 TC 4 Z9 4 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 26 PY 2015 VL 92 IS 6 AR 060413 DI 10.1103/PhysRevB.92.060413 PG 5 WC Physics, Condensed Matter SC Physics GA CS6OU UT WOS:000362200700002 ER PT J AU Green, J Meinel, S Engelhardt, M Krieg, S Laeuchli, J Negele, J Orginos, K Pochinsky, A Syritsyn, S AF Green, Jeremy Meinel, Stefan Engelhardt, Michael Krieg, Stefan Laeuchli, Jesse Negele, John Orginos, Kostas Pochinsky, Andrew Syritsyn, Sergey TI High-precision calculation of the strange nucleon electromagnetic form factors SO PHYSICAL REVIEW D LA English DT Article ID LATTICE QCD; MAGNETIC-MOMENT; PROTON AB We report a direct lattice QCD calculation of the strange nucleon electromagnetic form factors G(E)(s) and G(M)(s) in the kinematic range 0 <= Q(2) less than or similar to 1.2 GeV2. For the first time, both G(E)(s) and G(M)(s) are shown to be nonzero with high significance. This work uses closer to physical lattice parameters than previous calculations, and achieves an unprecedented statistical precision by implementing a recently proposed variance reduction technique called hierarchical probing. We perform model-independent fits of the form factor shapes using the z-expansion and determine the strange electric and magnetic radii and magnetic moment. We compare our results to parity-violating electron-proton scattering data and to other theoretical studies. C1 [Green, Jeremy] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Meinel, Stefan] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Meinel, Stefan; Syritsyn, Sergey] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Engelhardt, Michael] New Mexico State Univ, Dept Phys, Las Cruces, NM 88003 USA. [Krieg, Stefan] Berg Univ Wuppertal, D-42119 Wuppertal, Germany. [Krieg, Stefan] Forschungszentrum Julich, IAS, Julich Supercomp Ctr, D-52425 Julich, Germany. [Laeuchli, Jesse] Coll William & Mary, Dept Comp Sci, Williamsburg, VA 23187 USA. [Negele, John; Pochinsky, Andrew] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. [Orginos, Kostas] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Orginos, Kostas] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Green, J (reprint author), Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. EM green@kph.uni-mainz.de; smeinel@email.arizona.edu OI Krieg, Stefan/0000-0002-8417-9823 FU Office of Science of the U.S. Department of Energy (DOE); National Science Foundation [ACI-1053575]; U.S. Department of Energy Office of Nuclear Physics [DE-FG02-94ER40818]; DOE Award [DE-FG02-96ER40965, DE-FC02-12ER41890, DE-FG02-04ER41302, DE-AC05-06OR23177, DE-AC02-05CH11231]; NSF [CCF-121834]; RIKEN Foreign Postdoctoral Researcher Program; Deutsche Forschungsgemeinschaft [SFB-TRR 55]; PRISMA Cluster of Excellence at the University of Mainz; RIKEN BNL Research Center FX Computations for this work were carried out on facilities of the USQCD Collaboration, which are funded by the Office of Science of the U.S. Department of Energy (DOE), and on facilities provided by XSEDE, funded by the National Science Foundation Grant No. ACI-1053575. During this research J. G., S. M., J. N., and A. P. were supported in part by the U.S. Department of Energy Office of Nuclear Physics under Award No. DE-FG02-94ER40818; M. E. was supported in part by DOE Award No. DE-FG02-96ER40965; J. L. was supported in part by DOE Award No. DE-FC02-12ER41890 and NSF Grant No. CCF-121834; K. O. was supported in part by DOE Award No. DE-FG02-04ER41302 and also DOE Award No. DE-AC05-06OR23177, under which JSA operates the Thomas Jefferson National Accelerator Facility; S. S. was supported in part by DOE Award No. DE-AC02-05CH11231 and the RIKEN Foreign Postdoctoral Researcher Program; and S. K. was supported in part by Deutsche Forschungsgemeinschaft through Grant No. SFB-TRR 55. J. G. was also supported in part by the PRISMA Cluster of Excellence at the University of Mainz, and S. M. was also supported in part by the RHIC Physics Fellow Program of the RIKEN BNL Research Center. Calculations were performed with the Chroma software suite [54], using QUDA [55] with multi-GPU support [56]. NR 56 TC 12 Z9 12 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 26 PY 2015 VL 92 IS 3 AR 031501 DI 10.1103/PhysRevD.92.031501 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CS6UI UT WOS:000362218000001 ER PT J AU Wetzel, DJ Malone, MA Haasch, RT Meng, YF Vieker, H Hahn, NT Golzhauser, A Zuo, JM Zavadil, KR Gewirth, AA Nuzzo, RG AF Wetzel, David J. Malone, Marvin A. Haasch, Richard T. Meng, Yifei Vieker, Henning Hahn, Nathan T. Goelzhaeuser, Armin Zuo, Jian-Min Zavadil, Kevin R. Gewirth, Andrew A. Nuzzo, Ralph G. TI Passivation Dynamics in the Anisotropic Deposition and Stripping of Bulk Magnesium Electrodes During Electrochemical Cycling SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE rechargeable magnesium battery; magnesium anode; passivation; corrosion; columnar growth ID RECHARGEABLE MG BATTERIES; LITHIUM DENDRITE GROWTH; CRYSTALLOGRAPHIC ORIENTATION; PHOTOELECTRON-SPECTRA; CURRENT COLLECTORS; PITTING CORROSION; AQUEOUS-SOLUTION; SINGLE-CRYSTALS; ELECTROLYTES; SPECTROSCOPY AB Although rechargeable magnesium (Mg) batteries show promise for use as a next generation technology for high-density energy storage, little is known about the Mg anode solid electrolyte interphase and its implications for the performance and durability of a Mg-based battery. We explore in this report passivation effects engendered during the electrochemical cycling of a bulk Mg anode, characterizing their influences during metal deposition and dissolution in a simple, nonaqueous, Grignard electrolyte solution (ethylmagnesium bromide, EtMgBr, in tetrahydrofuran). Scanning electron microscopy images of Mg foil working electrodes after electrochemical polarization to dissolution potentials show the formation of corrosion pits. The pit densities so evidenced are markedly potential-dependent. When the Mg working electrode is cycled both potentiostatically and galvanostatically in EtMgBr these pits, formed due to passive layer breakdown, act as the foci for subsequent electrochemical activity. Detailed microscopy, diffraction, and spectroscopic data show that further passivation and corrosion results in the anisotropic stripping of the Mg {0001} plane, leaving thin oxide-comprising passivated side wall structures that demark the {0001} fiber texture of the etched Mg grains. Upon long-term cycling, oxide side walls formed due to the pronounced crystallographic anisotropy of the anodic stripping processes, leading to complex overlay anisotropic, columnar structures, exceeding 50 mu m in height. The passive responses mediating the growth of these structures appear to be an intrinsic feature of the electrochemical growth and dissolution of Mg using this electrolyte. C1 [Wetzel, David J.; Malone, Marvin A.; Gewirth, Andrew A.; Nuzzo, Ralph G.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Haasch, Richard T.; Meng, Yifei; Zuo, Jian-Min] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Meng, Yifei; Zuo, Jian-Min] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Vieker, Henning; Goelzhaeuser, Armin] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany. [Hahn, Nathan T.; Zavadil, Kevin R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Nuzzo, RG (reprint author), Univ Illinois, Dept Chem, 1209 W Calif St, Urbana, IL 61801 USA. EM r-nuzzo@illinois.edu RI Golzhauser, Armin/I-1270-2016 OI Golzhauser, Armin/0000-0002-0838-9028 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. This work was carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois at Urbana-Champaign and in the Department of Physics, Bielefeld University. NR 44 TC 6 Z9 6 U1 11 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 26 PY 2015 VL 7 IS 33 BP 18406 EP 18414 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CQ0XN UT WOS:000360322000028 PM 26258957 ER PT J AU Song, J Lim, J Lee, D Thambidurai, M Kim, JY Park, M Song, HJ Lee, S Char, K Lee, C AF Song, Jiyun Lim, Jaehoon Lee, Donggu Thambidurai, M. Kim, Jun Young Park, Myeongjin Song, Hyung-Jun Lee, Seonghoon Char, Kookheon Lee, Changhee TI Nanostructured Electron-Selective Interlayer for Efficient Inverted Organic Solar Cells SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE nanostructured extraction layer; electron-selective interlayer; electron buffer layer; organic-inorganic hybrid solar cells; CdSe tetrapods; bulkheterojunction ID POWER CONVERSION EFFICIENCY; OPTICAL SPACER; ZNO; GROWTH; RECOMBINATION; OXIDE AB We report a unique nanostmctured electron-selective interlayer comprising of In-doped ZnO (ZnO:In) and vertically aligned CdSe tetrapods (TPs) for inverted polymer:fullerene bulkheterojunction (BHP solar cells. With dimension-controlled CdSe TPs, the direct inorganic electron transport pathway is provided, resulting in the improvement of the short circuit current and fill factor of devices. We demonstrate that the enhancement is attributed to the roles of CdSe TPs that reduce the recombination losses between the active layer and buffer layer, improve the hole-blocking as well as electron-transporting properties, and simultaneously improve charge collection characteristics. As a result, the power conversion efficiency of PTB7:PC70BM based solar cell with nanostructured CdSe TPs increases to 7.55%. We expect this approach can be extended to a general platform for improving charge extraction in organic solar cells. C1 [Song, Jiyun; Lee, Donggu; Thambidurai, M.; Kim, Jun Young; Park, Myeongjin; Song, Hyung-Jun; Lee, Changhee] Seoul Natl Univ, Interuniv Semicond Res Ctr, Dept Elect & Comp Engn, Seoul 151744, South Korea. [Lim, Jaehoon; Char, Kookheon] Seoul Natl Univ, WCU Program Chem Convergence Energy & Environm, Sch Chem & Biol Engn, Natl Creat Res Initiat Ctr Intelligent Hybrids, Seoul 151744, South Korea. [Lim, Jaehoon; Song, Hyung-Jun] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Lee, Seonghoon] Seoul Natl Univ, Sch Chem, Seoul 151747, South Korea. RP Char, K (reprint author), Seoul Natl Univ, WCU Program Chem Convergence Energy & Environm, Sch Chem & Biol Engn, Natl Creat Res Initiat Ctr Intelligent Hybrids, 1 Gwanak Ro, Seoul 151744, South Korea. EM khchar@plaza.snu.ac.kr; chlee7@snu.ac.kr RI Lee, Changhee/A-2471-2009; Song, Hyung-Jun/J-8091-2016 OI Lee, Changhee/0000-0003-2800-8250; FU Human Resources Development program of Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant - Korea government Ministry of Trade, Industry, and Energy [20124010203170]; National Research Foundation of Korea (NRF) grant - Korea government Ministry of Science, ICT & Future Planning (MSIP): the National Creative Research Initiative Center for Intelligent Hybrids [2010-0018290]; WCU Program of C2E2 [R31-10013]; Technology Development Program [NRF-2009-0093304, NRF-2014R1A2A1A11054246, NRF-2009-0093319]; Global Frontier R&D Program on Center for Multiscale Energy System [2011-0031567]; Brain Korea 21 Plus Project FX This work was supported by the Human Resources Development program (No. 20124010203170) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Trade, Industry, and Energy. This work was also financially supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government Ministry of Science, ICT & Future Planning (MSIP): the National Creative Research Initiative Center for Intelligent Hybrids (No. 2010-0018290), the WCU Program of C2E2 (R31-10013), the Technology Development Program to Solve Climate Changes (NRF-2009-0093304, NRF-2014R1A2A1A11054246, and NRF-2009-0093319), the Global Frontier R&D Program on Center for Multiscale Energy System (2011-0031567), and the Brain Korea 21 Plus Project in 2015. NR 27 TC 0 Z9 0 U1 2 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 26 PY 2015 VL 7 IS 33 BP 18460 EP 18466 DI 10.1021/acsami.5b04624 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CQ0XN UT WOS:000360322000035 PM 26238224 ER PT J AU Shewmon, NT Watkins, DL Galindo, JF Zerdan, RB Chen, JH Keum, J Roitberg, AE Xue, JG Castellano, RK AF Shewmon, Nathan T. Watkins, Davita L. Galindo, Johan F. Zerdan, Raghida Bou Chen, Jihua Keum, Jong Roitberg, Adrian E. Xue, Jiangeng Castellano, Ronald K. TI Enhancement in Organic Photovoltaic Efficiency through the Synergistic Interplay of Molecular Donor Hydrogen Bonding and pi-Stacking SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE bulk heterojunctions; hydrogen bonding; organic photovoltaics; self-assembly; supramolecular chemistry ID HETEROJUNCTION SOLAR-CELLS; FIELD-EFFECT TRANSISTORS; OPEN-CIRCUIT VOLTAGE; SUPRAMOLECULAR CHEMISTRY; OLIGOTHIOPHENE NANORODS; FLUORINE SUBSTITUENTS; SELF-ORGANIZATION; CHARGE-TRANSPORT; PERFORMANCE; POLYMER AB For organic photovoltaic (OPV) cells based on the bulk heterojunction (BHJ) structure, it remains challenging to rationally control the degree of phase separation and percolation within blends of donors and acceptors to secure optimal charge separation and transport. Reported is a bottom-up, supramolecular approach to BHJ OPVs wherein tailored hydrogen bonding (H-bonding) interactions between -conjugated electron donor molecules encourage formation of vertically aligned donor -stacks while simultaneously suppressing lateral aggregation; the programmed arrangement facilitates fine mixing with fullerene acceptors and efficient charge transport. The approach is illustrated using conventional linear or branched quaterthiophene donor chromophores outfitted with terminal functional groups that are either capable or incapable of self-complementary H-bonding. When applied to OPVs, the H-bond capable donors yield a twofold enhancement in power conversion efficiency relative to the comparator systems, with a maximum external quantum efficiency of 64%. H-bond promoted assembly results in redshifted absorption (in neat films and donor:C-60 blends) and enhanced charge collection efficiency despite disparate donor chromophore structure. Both features positively impact photocurrent and fill factor in OPV devices. Film structural characterization by atomic force microscopy, transmission electron microscopy, and grazing incidence wide angle X-ray scattering reveals a synergistic interplay of lateral H-bonding interactions and vertical -stacking for directing the favorable morphology of the BHJ. C1 [Shewmon, Nathan T.; Xue, Jiangeng] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Watkins, Davita L.; Galindo, Johan F.; Zerdan, Raghida Bou; Roitberg, Adrian E.; Castellano, Ronald K.] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Chen, Jihua; Keum, Jong] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Shewmon, NT (reprint author), Univ Florida, Dept Mat Sci & Engn, POB 116400, Gainesville, FL 32611 USA. EM jxue@mse.ufl.edu; castellano@chem.ufl.edu RI Chen, Jihua/F-1417-2011; Keum, Jong/N-4412-2015 OI Chen, Jihua/0000-0001-6879-5936; Keum, Jong/0000-0002-5529-1373 FU National Science Foundation [CHE-1057411]; Research Corporation for Science Advancement (Scialog Award) [20316]; University of Florida Office of Research; DOE Office of Science User Facility [CNMS2014-286] FX R.K.C. acknowledges financial support from the National Science Foundation (CHE-1057411). J.X. and R.K.C. also acknowledge partial financial support from the Research Corporation for Science Advancement (Scialog Award No. 20316) and the University of Florida Office of Research. The authors thank University of Florida Research Computing for providing computational resources and support that have contributed to the research results are reported in this paper. The authors are also grateful to Prof. Kirk Schanze for providing access to the AFM instrumentation, and to Danielle Fagnani for assistance with the synthesis. TEM (J.C.) and GIWAXS (J.K.) experiments were conducted at the Center for Nanophase Materials Sciences (user project CNMS2014-286) at the Oak Ridge National Laboratory, which is a DOE Office of Science User Facility. NR 76 TC 4 Z9 4 U1 12 U2 92 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 26 PY 2015 VL 25 IS 32 BP 5166 EP 5177 DI 10.1002/adfm.201501815 PG 12 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP9NX UT WOS:000360222400010 ER PT J AU Fu, Q Yang, L Wang, WH Han, A Huang, J Du, PW Fan, ZY Zhang, JY Xiang, B AF Fu, Qi Yang, Lei Wang, Wenhui Han, Ali Huang, Jian Du, Pingwu Fan, Zhiyong Zhang, Jingyu Xiang, Bin TI Synthesis and Enhanced Electrochemical Catalytic Performance of Monolayer WS2(1-x)Se2x with a Tunable Band Gap SO ADVANCED MATERIALS LA English DT Article DE WS2(1-x)Se2x; tunable band gap; photoluminescence; catalytic activity; hydrogen evolution reactions ID HYDROGEN EVOLUTION REACTION; TRANSITION-METAL DICHALCOGENIDES; MOLYBDENUM-DISULFIDE; RAMAN-SPECTROSCOPY; SINGLE-LAYER; MOS2; WS2; NANOSHEETS; PHOTOLUMINESCENCE; GROWTH C1 [Fu, Qi; Yang, Lei; Wang, Wenhui; Han, Ali; Huang, Jian; Du, Pingwu; Xiang, Bin] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China. [Fan, Zhiyong] Hong Kong Univ Sci & Technol, Dept Elect & Comp Engn, Hong Kong 8523, Hong Kong, Peoples R China. [Zhang, Jingyu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Xiang, Bin] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. RP Xiang, B (reprint author), Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China. EM binxiang@ustc.edu.cn RI Fan, Zhiyong/C-4970-2012; Xiang, Bin/C-9192-2012; OI Fan, Zhiyong/0000-0002-5397-0129 FU National Science Foundation of China [21373196, 11434009]; National Program for Thousand Young Talents of China; Fundamental Research Funds for the Central Universities [WK2060140014, WK2340000050] FX This work was supported by the National Science Foundation of China (21373196 and 11434009), the National Program for Thousand Young Talents of China, and the Fundamental Research Funds for the Central Universities (WK2060140014 and WK2340000050). NR 46 TC 22 Z9 22 U1 28 U2 177 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 26 PY 2015 VL 27 IS 32 BP 4732 EP 4738 DI 10.1002/adma.201500368 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP9PW UT WOS:000360227800010 PM 26153276 ER PT J AU Qu, J Barnhill, WC Luo, HM Meyer, HM Leonard, DN Landauer, AK Kheireddin, B Gao, H Papke, BL Dai, S AF Qu, Jun Barnhill, William C. Luo, Huimin Meyer, Harry M., III Leonard, Donovan N. Landauer, Alexander K. Kheireddin, Bassem Gao, Hong Papke, Brian L. Dai, Sheng TI Synergistic Effects Between Phosphonium-Alkylphosphate Ionic Liquids and Zinc Dialkyldithiophosphate (ZDDP) as Lubricant Additives SO ADVANCED MATERIALS LA English DT Article DE ionic liquids; ZDDP; lubricant additives; synergistic effects; friction and wear reductions ID ANTIWEAR PERFORMANCE; NEAT LUBRICANTS; BASE OILS; STEEL; ACID; ORGANOPHOSPHATE; TEMPERATURE; EXTRACTION; MECHANISM; ALUMINUM C1 [Qu, Jun; Barnhill, William C.; Meyer, Harry M., III; Leonard, Donovan N.; Landauer, Alexander K.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Luo, Huimin] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Kheireddin, Bassem; Gao, Hong; Papke, Brian L.] Shell Global Solut, Technol Ctr Houston, Houston, TX 77082 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Qu, J (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008,MS 6063, Oak Ridge, TN 37831 USA. EM qujn@ornl.gov RI Dai, Sheng/K-8411-2015; OI Dai, Sheng/0000-0002-8046-3931; Qu, Jun/0000-0001-9466-3179 FU Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, US Department of Energy (DOE); Scientific User Facilities Division, Office of DOE-BES; DOE Science Undergraduate Laboratory Internships program; U.S. Department of Energy [DE-AC05-00OR22725] FX The authors thank Dr. J. Dyck from Cytec Industries Inc. for providing phosphonium cation feedstocks, D. W. Coffey from ORNL for TEM sample preparation, and A. E. Marquez Rossy from ORNL for assist in nanoindentation, respectively. This research was sponsored by the Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, US Department of Energy (DOE). Electron microscopy characterization was performed at ORNL's Center for Nanophase Materials Sciences, sponsored by the Scientific User Facilities Division, Office of DOE-BES. A. K. Landauer was supported by the DOE Science Undergraduate Laboratory Internships program.; Notice: This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 35 TC 15 Z9 15 U1 12 U2 51 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 26 PY 2015 VL 27 IS 32 BP 4767 EP 4774 DI 10.1002/adma.201502037 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP9PW UT WOS:000360227800015 PM 26173561 ER PT J AU Nanayakkara, SU van de Lagemaat, J Luther, JM AF Nanayakkara, Sanjini U. van de Lagemaat, Jao Luther, Joseph M. TI Scanning Probe Characterization of Heterostructured Colloidal Nanomaterials SO CHEMICAL REVIEWS LA English DT Review ID NANOCRYSTAL QUANTUM DOTS; ATOMIC-FORCE MICROSCOPY; MULTIPLE EXCITON GENERATION; LIGHT-EMITTING TRANSISTOR; ASSEMBLED MOLECULAR NANOSTRUCTURE; CDSE/CDS CORE/SHELL NANOCRYSTALS; ELECTRON CHARGING ENERGIES; FIELD-EFFECT TRANSISTORS; CORE-SHELL NANOCRYSTALS; PERMANENT DIPOLE-MOMENT C1 [Nanayakkara, Sanjini U.; van de Lagemaat, Jao; Luther, Joseph M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Nanayakkara, SU (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Sanjini.Nanayakkara@nrel.gov; Joey.Luther@nrel.gov RI van de Lagemaat, Jao/J-9431-2012 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences; DOE [DE-AC36-08G028308]; solar photochemistry program FX We thanks Ryan Crisp and Al Hicks for help with the figures and Mathew Beard for helpful discussions. S.U.N. and J.M.L acknowledge the Energy Frontier Research Centers program within the Center for Advanced Solar Photophysics supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences. J.V.D.L. acknowledges support from the solar photochemistry program. DOE funding was provided to NREL through contract DE-AC36-08G028308. NR 257 TC 8 Z9 8 U1 6 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD AUG 26 PY 2015 VL 115 IS 16 BP 8157 EP 8181 DI 10.1021/cr500280t PG 25 WC Chemistry, Multidisciplinary SC Chemistry GA CQ0XH UT WOS:000360321300001 PM 26196958 ER PT J AU Zhu, CZ Du, D Eychmuller, A Lin, YH AF Zhu, Chengzhou Du, Dan Eychmueller, Alexander Lin, Yuehe TI Engineering Ordered and Nonordered Porous Noble Metal Nanostructures: Synthesis, Assembly, and Their Applications in Electrochemistry SO CHEMICAL REVIEWS LA English DT Review ID OXYGEN-REDUCTION REACTION; ENHANCED ELECTROCATALYTIC ACTIVITY; FORMIC-ACID OXIDATION; ONE-POT SYNTHESIS; GALVANIC REPLACEMENT REACTION; HIGH-SURFACE-AREA; PT-RU ALLOY; CORE-SHELL NANOPARTICLES; AU-AT-PD; MESOPOROUS PLATINUM NANOPARTICLES C1 [Zhu, Chengzhou; Du, Dan; Lin, Yuehe] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Du, Dan] Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China. [Eychmueller, Alexander] Tech Univ Dresden, Phys Chem, D-01062 Dresden, Germany. [Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Lin, YH (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. EM Yuehe.lin@wsu.edu RI Lin, Yuehe/D-9762-2011; Zhu, Chengzhou/M-3566-2014; OI Lin, Yuehe/0000-0003-3791-7587; Zhu, Chengzhou/0000-0003-0679-7965 FU WSU; Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL); US-DOE [DE-AC05-76RL01830]; National Natural Science Foundation of China [21275062]; Program for New Century Excellent Talents in University [NCET-12-0871] FX This work was supported by a start-up grant from WSU and a Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for US-DOE under Contract DE-AC05-76RL01830. C.Z. and A.E. also acknowledge the Alexander von Humboldt Foundation. D.D. acknowledges the financial support of the National Natural Science Foundation of China (21275062) and the Program for New Century Excellent Talents in University (NCET-12-0871). NR 487 TC 96 Z9 96 U1 98 U2 400 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD AUG 26 PY 2015 VL 115 IS 16 BP 8896 EP 8943 DI 10.1021/acs.chemrev.5b00255 PG 48 WC Chemistry, Multidisciplinary SC Chemistry GA CQ0XH UT WOS:000360321300016 PM 26181885 ER PT J AU Meng, LZ Gruszkiewicz, MS Deng, TL Guo, YF Li, D AF Meng, Lingzong Gruszkiewicz, Miroslaw S. Deng, Tianlong Guo, Yafei Li, Dan TI Isothermal Evaporation Process Simulation Using the Pitzer Model for the Quinary System LiCl NaCl KCl SrCl2 H2O at 298.15 K SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID THERMODYNAMIC PROPERTIES; ISOPIESTIC MOLALITIES; ACTIVITY-COEFFICIENTS; STRONTIUM CHLORIDE; AQUEOUS-SOLUTIONS; PHASE-EQUILIBRIA; 25-DEGREES-C; ELECTROLYTES; TEMPERATURES; SOLUBILITY AB The Pitzer thermodynamic model for liquid solid equilibrium in the quinary system LiCl-NaCl-KCl-SrCl2 H2O at 298.15 K was constructed by selecting the proper parameters and standard chemical potential. The solubility data and water activity data of the systems SrCl2-H2O, NaCl-SrCl2-H2O, KCl-SrCl2-H2O, LiCl-SrCl2-H2O, and NaCl-KCl-SrCl2-H2O were used to evaluate the model. Good agreement between the calculated and experimental solubility data indicates that the model is reliable. The Pitzer model for the above system at 298.15 K was then used to calculate the component solubilities and conduct computer simulation of isothermal evaporation of the mother liquor for the oilfield brine in Nanyishan region of Qaidam Basin (China). The evaporation-crystallization route and order of salt precipitation, changes in concentration and precipitation of lithium, sodium, potassium, and strontium, and water activities during the evaporation process were demonstrated. The salts crystallized from the brine in the order: KCl, NaCl, SrCl2 center dot 6H(2)O, SrCl2 center dot 2H(2)O, and LiCl center dot H2O. The entire evaporation crystallization process may consist of six stages. In each stage, the variation trends for the relationships between ion concentrations or water activities and the evaporation ratio are different. This result of the simulation of brines can be used as a theoretical reference for comprehensive exploitation and utilization of this type of brine resources. C1 [Meng, Lingzong; Li, Dan] Linyi Univ, Sch Chem & Chem Engn, Linyi 276000, Peoples R China. [Meng, Lingzong; Gruszkiewicz, Miroslaw S.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Deng, Tianlong; Guo, Yafei] Tianjin Univ Sci & Technol, Tianjin Key Lab Marine Resources & Chem, Tianjin 300457, Peoples R China. RP Meng, LZ (reprint author), Linyi Univ, Sch Chem & Chem Engn, Linyi 276000, Peoples R China. EM menglingzong@lyu.edu.cn RI Gruszkiewicz, Miroslaw/L-2389-2016 OI Gruszkiewicz, Miroslaw/0000-0002-6551-6724 FU NNSFC [21406104, 21276194, 21306136, U1406113]; Key Laboratory of Salt Lake Resources and Chemistry, Qinghai Institute of Salt Lake, Chinese Academy of Sciences [KLSLRC-KF-13-HX-4]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Bioscience; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the NNSFC (Nos. 21406104, 21276194, 21306136, and U1406113), and the Key Laboratory of Salt Lake Resources and Chemistry, Qinghai Institute of Salt Lake, Chinese Academy of Sciences (KLSLRC-KF-13-HX-4). Efforts by M.S.G. in this work were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 26 TC 1 Z9 1 U1 4 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD AUG 26 PY 2015 VL 54 IS 33 BP 8311 EP 8318 DI 10.1021/acs.iecr.5b01897 PG 8 WC Engineering, Chemical SC Engineering GA CQ0XR UT WOS:000360322400035 ER PT J AU Matheu, R Ertem, MZ Benet-Buchholz, J Coronado, E Batista, VS Sala, X Llobet, A AF Matheu, Roc Ertem, Mehmed Z. Benet-Buchholz, Jordi Coronado, Eugenio Batista, Victor S. Sala, Xavier Llobet, Antoni TI Intramolecular Proton Transfer Boosts Water Oxidation Catalyzed by a Ru Complex SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MONONUCLEAR RUTHENIUM COMPLEXES; CYCLIC VOLTAMMETRY; OXYGEN EVOLUTION; HIGHLY EFFICIENT; ONE-SITE; ELECTROCATALYSTS; LIGAND; MECHANISMS; DIOXYGEN; KINETICS AB We introduce a new family of complexes with the general formula [Ru-n(tda)(py)(2)](m+) (n = 2, m = 0, 1; n = 3, m = 1, 2(+); n = 4, m = 2, 3(2+)), with tda(2-) being [2,2':6',2"-terpyridine]-6,6"-dicarboxylate, including complex [Ru-IV(OH)(tda-kappa-(NO)-O-3)(py)(2)](+), 4H(+), which we find to be an impressive water oxidation catalyst, formed by hydroxo coordination to 3(2+) under basic conditions. The complexes are synthesized, isolated, and thoroughly characterized by analytical, spectroscopic (UV-vis, nuclear magnetic resonance, electron paramagnetic resonance), computational, and electrochemical techniques (cyclic voltammetry, differential pulse voltammetry, coulometry), including solid-state monocrystal X-ray diffraction analysis. In oxidation state IV, the Ru center is seven-coordinated and diamagnetic, whereas in oxidation state II, the complex has an unbonded dangling carboxylate and is six-coordinated while still diamagnetic. With oxidation state III, the coordination number is halfway between the coordination of oxidation states II and IV. Species generated in situ have also been characterized by spectroscopic, computational, and electrochemical techniques, together with the related species derived from a different degree of protonation and oxidation states. 4H(+) can be generated potentiometrically, or voltammetrically, from 3(2+), and both coexist in solution. While complex 3(2+) is not catalytically active, the catalytic performance of complex 4H(+) is characterized by the foot of the wave analysis, giving an impressive turnover frequency record of 8000 s(-1) at pH 7.0 and 50 000 s(-1) at pH 10.0. Density functional theory calculations provide a complete description of the water oxidation catalytic cycle of 4H(+), manifesting the key functional role of the dangling carboxylate in lowering the activation free energies that lead to O-O bond formation. C1 [Matheu, Roc; Benet-Buchholz, Jordi; Llobet, Antoni] Inst Chem Res Catalonia ICIQ, Tarragona 43007, Spain. [Ertem, Mehmed Z.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Coronado, Eugenio] Univ Valencia, Inst Ciencia Mol ICMol, Paterna 46980, Spain. [Batista, Victor S.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Sala, Xavier; Llobet, Antoni] Univ Autonoma Barcelona, Dept Quim, E-08193 Barcelona, Spain. RP Batista, VS (reprint author), Yale Univ, Dept Chem, POB 208107, New Haven, CT 06520 USA. EM victor.batista@yale.edu; xavier.sala@uab.cat; allobet@iciq.cat RI Sala, Xavier/N-7363-2013; Coronado, Eugenio/E-8960-2014; Llobet, Antoni/C-3296-2016; OI Sala, Xavier/0000-0002-7779-6313; Llobet, Antoni/0000-0002-6176-5272; Matheu, Roc/0000-0001-8601-5219 FU "La Caixa" foundation; Argonne-Northwestern Solar Energy 524 Research (ANSER) Center; Energy Frontier Research Center - U.S. Department of Energy, Office of 526 Science, Office of Basic Energy Sciences [527 DE-SC0001059]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC00112704] FX R.M. thanks "La Caixa" foundation for a Ph.D. grant. A.L. thanks MINECO (CTQ-2013-49075-R, SEV-2013-0319; CTQ-2014-52974-REDC) and "La Caixa" foundation for financial support. COST actions, CM1202, and CM1205 from the EU are also gratefully acknowledged. V.S.B. acknowledges supercomputer time from NERSC and financial support as part of the Argonne-Northwestern Solar Energy 524 Research (ANSER) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of 526 Science, Office of Basic Energy Sciences under Award Number 527 DE-SC0001059. The work at BNL (M.Z.E.) was carried out under contract DE-SC00112704 with the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. We thank J.M. Martinez-Agudo from the Universidad de Valencia for his assistance with the EPR measurements. NR 57 TC 21 Z9 21 U1 13 U2 85 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 26 PY 2015 VL 137 IS 33 BP 10786 EP 10795 DI 10.1021/jacs.5b06541 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CQ0XF UT WOS:000360321100052 PM 26226390 ER PT J AU Hulvey, Z Vlaisavljevich, B Mason, JA Tsivion, E Dougherty, TP Bloch, ED Head-Gordon, M Smit, B Long, JR Brown, CM AF Hulvey, Zeric Vlaisavljevich, Bess Mason, Jarad A. Tsivion, Ehud Dougherty, Timothy P. Bloch, Eric D. Head-Gordon, Martin Smit, Berend Long, Jeffrey R. Brown, Craig M. TI Critical Factors Driving the High Volumetric Uptake of Methane in Cu-3(btc)(2) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; TOTAL-ENERGY CALCULATIONS; SITU NEUTRON-DIFFRACTION; NANOPOROUS MATERIALS; POROUS MATERIALS; HYDROGEN ADSORPTION; COORDINATION SITES; GAS-STORAGE; SEPARATION; DESIGN AB A thorough experimental and computational study has been carried out to elucidate the mechanistic reasons for the high volumetric uptake of methane in the metal-organic framework Cu-3(btc)(2) (btc(3-) = 1,3,5-benzenetricarboxylate; HKUST-1). Methane adsorption data measured at several temperatures for Cu-3(btc)(2), and its isostructural analogue Cr-3(btc)(2), show that there is little difference in volumetric adsorption capacity when the metal center is changed. In situ neutron powder diffraction data obtained for both materials were used to locate four CD4 adsorption sites that fill sequentially. This data unequivocally shows that primary adsorption sites around, and within, the small octahedral cage in the structure are favored over the exposed Cu2+ or Cr2+ cations. These results are supported by an exhaustive parallel computational study, and contradict results recently reported using a time-resolved diffraction structure envelope (TRDSE) method. Moreover, the computational study reveals that strong methane binding at the open metal sites is largely due to methane-methane interactions with adjacent molecules adsorbed at the primary sites instead of an electronic interaction with the metal center. Simulated methane adsorption isotherms for Cu-3(btc)(2) are shown to exhibit excellent agreement with experimental isotherms, allowing for additional simulations that show that modifications to the metal center, ligand, or even tuning the overall binding enthalpy would not improve the working capacity for methane storage over that measured for Cu-3(btc)(2) itself. C1 [Hulvey, Zeric; Dougherty, Timothy P.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Hulvey, Zeric] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Vlaisavljevich, Bess; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Mason, Jarad A.; Tsivion, Ehud; Bloch, Eric D.; Head-Gordon, Martin; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Tsivion, Ehud; Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Dougherty, Timothy P.] Georgetown Univ, Dept Chem, Washington, DC 20057 USA. [Smit, Berend] Ecole Polytech Fed Lausanne, Inst Sci & Ingn Chim, CH-1015 Lausanne, Switzerland. [Brown, Craig M.] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. RP Hulvey, Z (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM zeric.hulvey@nist.gov; craig.brown@nist.gov RI Brown, Craig/B-5430-2009; Smit, Berend/B-7580-2009; Vlaisavljevich, Bess/Q-9737-2016 OI Brown, Craig/0000-0002-9637-9355; Smit, Berend/0000-0003-4653-8562; Vlaisavljevich, Bess/0000-0001-6065-0732 FU Nanoporous Materials Genome Center - U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-12ER16362]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; NIST/NSF REU Summer Undergraduate Research Fellowship (SURF) - Center for High Resolution Neutron Scattering (CHRNS) [DMR-09414772]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Prof. Efrain Rodriguez for assistance with the synthesis of Cr3(btc)2 and Dr. Matthew Hudson for assistance with neutron powder diffraction experiments. Gas adsorption measurements were supported by the Nanoporous Materials Genome Center, which is funded by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Award DE-FG02-12ER16362. Computational efforts were supported by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001015. T.P.D. was supported through the NIST/NSF REU Summer Undergraduate Research Fellowship (SURF) funded through the Center for High Resolution Neutron Scattering (CHRNS) DMR-09414772. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 10 Z9 10 U1 10 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 26 PY 2015 VL 137 IS 33 BP 10816 EP 10825 DI 10.1021/jacs.5b06657 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CQ0XF UT WOS:000360321100055 PM 26263038 ER PT J AU Motruk, J Grushin, AG de Juan, F Pollmann, F AF Motruk, Johannes Grushin, Adolfo G. de Juan, Fernando Pollmann, Frank TI Interaction-driven phases in the half-filled honeycomb lattice: An infinite density matrix renormalization group study SO PHYSICAL REVIEW B LA English DT Article ID TOPOLOGICAL INSULATORS; GRAPHENE; MATTER AB The emergence of the Haldane Chern insulator state due to strong short-range repulsive interactions in the half-filled fermionic spinless honeycomb lattice model has been proposed and challenged with different methods and yet it still remains controversial. In this work we revisit the problem using the infinite density matrix renormalization group method and report numerical evidence supporting (i) the absence of the Chern insulator state, (ii) two previously unnoticed charge ordered phases, and (iii) the existence and stability of all the nontopological competing orders that were found previously within mean field. In addition, we discuss the nature of the corresponding phase transitions based on our numerical data. Our work establishes the phase diagram of the half-filled honeycomb lattice model, tilting the balance towards the absence of a Chern insulator phase for this model. C1 [Motruk, Johannes; Grushin, Adolfo G.; Pollmann, Frank] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [de Juan, Fernando] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [de Juan, Fernando] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Motruk, J (reprint author), Max Planck Inst Phys Komplexer Syst, Nothnitzer Str 38, D-01187 Dresden, Germany. RI Grushin, Adolfo G./A-5704-2011; de Juan, Fernando/B-9392-2008; Pollmann, Frank/L-5378-2013 OI Grushin, Adolfo G./0000-0001-7678-7100; de Juan, Fernando/0000-0001-6852-1484; NR 48 TC 19 Z9 19 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 26 PY 2015 VL 92 IS 8 AR 085147 DI 10.1103/PhysRevB.92.085147 PG 11 WC Physics, Condensed Matter SC Physics GA CP7JW UT WOS:000360064300003 ER PT J AU Refaely-Abramson, S Jain, M Sharifzadeh, S Neaton, JB Kronik, L AF Refaely-Abramson, Sivan Jain, Manish Sharifzadeh, Sahar Neaton, Jeffrey B. Kronik, Leeor TI Solid-state optical absorption from optimally tuned time-dependent range-separated hybrid density functional theory SO PHYSICAL REVIEW B LA English DT Article ID ELECTRON-HOLE EXCITATIONS; SHAM ORBITAL ENERGIES; AB-INITIO CALCULATION; BAND-GAP PROBLEM; GREENS-FUNCTION; QUASI-PARTICLE; SEMICONDUCTORS; EXCHANGE; SPECTRA; DESIGN AB We present a framework for obtaining reliable solid-state charge and optical excitations and spectra from optimally tuned range-separated hybrid density functional theory. The approach, which is fully couched within the formal framework of generalized Kohn-Sham theory, allows for the accurate prediction of exciton binding energies. We demonstrate our approach through first principles calculations of one- and two-particle excitations in pentacene, a molecular semiconducting crystal, where our work is in excellent agreement with experiments and prior computations. We further show that with one adjustable parameter, set to produce the known band gap, this method accurately predicts band structures and optical spectra of silicon and lithium fluoride, prototypical covalent and ionic solids. Our findings indicate that for a broad range of extended bulk systems, this method may provide a computationally inexpensive alternative to many-body perturbation theory, opening the door to studies of materials of increasing size and complexity. C1 [Refaely-Abramson, Sivan; Kronik, Leeor] Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. [Jain, Manish] Indian Inst Sci, Dept Phys, Bangalore 560012, Karnataka, India. [Sharifzadeh, Sahar] Boston Univ, Div Mat Sci & Engn, Dept Elect & Comp Engn & Phys, Boston, MA 02215 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Refaely-Abramson, S (reprint author), Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. RI Jain, Manish/A-8303-2010; Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; Sharifzadeh, Sahar/P-4881-2016 OI Jain, Manish/0000-0001-9329-6434; Neaton, Jeffrey/0000-0001-7585-6135; Sharifzadeh, Sahar/0000-0003-4215-4668 FU European Research Council; Israel Science Foundation; United States - Israel Binational Science Foundation; Helmsley Foundation; Wolfson Foundation; Adams fellowship of the Israel Academy of Sciences and Humanities; Scientific Discovery through Advanced Computing (SciDAC) Partnership program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences FX Work at the Weizmann Institute was supported by the European Research Council, the Israel Science Foundation, the United States - Israel Binational Science Foundation, the Helmsley Foundation, and the Wolfson Foundation. S.R.A. was supported by an Adams fellowship of the Israel Academy of Sciences and Humanities. S.S. and J.B.N were supported by the Scientific Discovery through Advanced Computing (SciDAC) Partnership program funded by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences. We thank the National Energy Research Scientific Computing center for computational resources. NR 74 TC 18 Z9 18 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 26 PY 2015 VL 92 IS 8 AR 081204 DI 10.1103/PhysRevB.92.081204 PG 6 WC Physics, Condensed Matter SC Physics GA CP7JW UT WOS:000360064300001 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Contin, G Cramer, JG Crawford, HJ Cudd, AB Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, F Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Eyser, O Fatemi, R Fazio, S Fedorisin, J Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hamed, A Han, LX Haque, R Harris, JW Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huang, X Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olvitt, DL Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Pujahari, PR Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM Szelezniak, MA Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G Van Nieuwenhuizen, G Vandenbroucke, M Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Vossen, A Wada, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, J Xu, N Xu, QH Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, JL Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bueltmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Campbell, J. M. Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Contin, G. Cramer, J. G. Crawford, H. J. Cudd, A. B. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. de Souza, R. Derradi Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huang, X. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olvitt, D. L., Jr. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szelezniak, M. A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. Van Nieuwenhuizen, G. Vandenbroucke, M. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Vossen, A. Wada, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, J. Xu, N. Xu, Q. H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Yu, N. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, J. L. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Precision Measurement of the Longitudinal Double-Spin Asymmetry for Inclusive Jet Production in Polarized Proton Collisions at root s=200 GeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTON DISTRIBUTIONS; UNCERTAINTIES AB We report a new measurement of the midrapidity inclusive jet longitudinal double-spin asymmetry, A(LL), in polarized pp collisions at center-of-mass energy root s = 200 GeV. The STAR data place stringent constraints on polarized parton distribution functions extracted at next-to-leading order from global analyses of inclusive deep-inelastic scattering (DIS), semi-inclusive DIS, and RHIC pp data. The measured asymmetries provide evidence at the 3 sigma level for positive gluon polarization in the Bjorken-x region x > 0.05. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. 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K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; Kycia, Radoslaw/J-4397-2015; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Fazio, Salvatore /G-5156-2010; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Chaloupka, Petr/E-5965-2012; Takahashi, Jun/B-2946-2012; Huang, Bingchu/H-6343-2015; Derradi de Souza, Rafael/M-4791-2013; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016 OI Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Ke, Hongwei/0000-0003-1463-7291; Kycia, Radoslaw/0000-0002-6390-4627; Alekseev, Igor/0000-0003-3358-9635; Sumbera, Michal/0000-0002-0639-7323; Takahashi, Jun/0000-0002-4091-1779; Huang, Bingchu/0000-0002-3253-3210; Derradi de Souza, Rafael/0000-0002-2084-7001; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657 FU RHIC Operations Group and RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium; Offices of NP and HEP within the U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We would like to thank J. Blumlein, H. Bottcher, E. Leader, E. Nocera, D. B. Stamenov, M. Stratmann, and W. Vogelsang for information regarding their respective polarized PDF sets and their uncertainties. We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, the National Science Centre of Poland, the National Research Foundation (NRF-2012004024), the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 33 TC 16 Z9 16 U1 2 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 26 PY 2015 VL 115 IS 9 AR 092002 DI 10.1103/PhysRevLett.115.092002 PG 7 WC Physics, Multidisciplinary SC Physics GA CP7KJ UT WOS:000360065900003 PM 26371644 ER PT J AU Kim, SW Liu, C Kim, HJ Lee, JH Yao, YX Ho, KM Cho, JH AF Kim, Sun-Woo Liu, Chen Kim, Hyun-Jung Lee, Jun-Ho Yao, Yongxin Ho, Kai-Ming Cho, Jun-Hyung TI Nature of the Insulating Ground State of the 5d Postperovskite CaIrO3 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SR2IRO4; PHASE AB The insulating ground state of the 5d transition metal oxide CaIrO3 has been classified as a Mott-type insulator. Based on a systematic density functional theory (DFT) study with local, semilocal, and hybrid exchange-correlation functionals, we reveal that the Ir t(2g) states exhibit large splittings and one-dimensional electronic states along the c axis due to a tetragonal crystal field. Our hybrid DFT calculation adequately describes the antiferromagnetic (AFM) order along the c direction via a superexchange interaction between Ir4+ spins. Furthermore, the spin-orbit coupling (SOC) hybridizes the t(2g) states to open an insulating gap. These results indicate that CaIrO3 can be represented as a spin-orbit Slater insulator, driven by the interplay between a long-range AFM order and the SOC. Such a Slater mechanism for the gap formation is also demonstrated by the DFT + dynamical mean field theory calculation, where the metal-insulator transition and the paramagnetic to AFM phase transition are concomitant with each other. C1 [Kim, Sun-Woo; Kim, Hyun-Jung; Lee, Jun-Ho; Cho, Jun-Hyung] Hanyang Univ, Dept Phys, Seoul 133791, South Korea. [Kim, Sun-Woo; Kim, Hyun-Jung; Lee, Jun-Ho; Cho, Jun-Hyung] Hanyang Univ, Res Inst Nat Sci, Seoul 133791, South Korea. [Liu, Chen; Yao, Yongxin; Ho, Kai-Ming] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Liu, Chen; Yao, Yongxin; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Kim, Hyun-Jung; Ho, Kai-Ming; Cho, Jun-Hyung] Univ Sci & Technol China, HFNL, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China. [Lee, Jun-Ho] Korea Inst Adv Study, Seoul 130722, South Korea. RP Kim, SW (reprint author), Hanyang Univ, Dept Phys, 17 Haengdang Dong, Seoul 133791, South Korea. EM ykent@iastate.edu; chojh@hanyang.ac.kr RI Hyun-Jung, Kim/E-8074-2011; Cho, Jun-Hyung/R-7256-2016 OI Hyun-Jung, Kim/0000-0002-5602-1404; Cho, Jun-Hyung/0000-0002-1785-1835 FU National Research Foundation of Korea (NRF) grant - Korea Government [2015R1A2A2A01003248]; Program of Introducing Talents of Discipline to Universities of Ministry of Education (MOE); State Administration of Foreign Experts Affairs of the People's Republic of China (SAFEA); NSFC [61434002]; KISTI supercomputing center [KSC-2014-C3-011]; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Iowa State University [DE-AC02-07CH11358] FX This work was supported in part by National Research Foundation of Korea (NRF) grant funded by the Korea Government (2015R1A2A2A01003248), by Program of Introducing Talents of Discipline to Universities of Ministry of Education (MOE) & the State Administration of Foreign Experts Affairs of the People's Republic of China (SAFEA), and by NSFC (Grant No. 61434002). The calculations were performed by KISTI supercomputing center through the strategic support program (KSC-2014-C3-011) for the supercomputing application research. Research at Ames Laboratory was supported by the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 41 TC 4 Z9 4 U1 11 U2 65 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 26 PY 2015 VL 115 IS 9 AR 096401 DI 10.1103/PhysRevLett.115.096401 PG 5 WC Physics, Multidisciplinary SC Physics GA CP7KJ UT WOS:000360065900011 PM 26371665 ER PT J AU Wagner, SR Huang, B Park, C Feng, JG Yoon, M Zhang, PP AF Wagner, Sean R. Huang, Bing Park, Changwon Feng, Jiagui Yoon, Mina Zhang, Pengpeng TI Growth of Metal Phthalocyanine on Deactivated Semiconducting Surfaces Steered by Selective Orbital Coupling SO PHYSICAL REVIEW LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; PHOTOELECTRON-SPECTROSCOPY; THIN-FILMS; COBALT-PHTHALOCYANINE; EPITAXIAL GRAPHENE; ELECTRONIC STATES; ORIENTATION; ADSORPTION; MOLECULES; AG(111) AB Using scanning tunneling microscopy and density functional theory, we show that the molecular ordering and orientation of metal phthalocyanine molecules on the deactivated Si surface display a strong dependency on the central transition-metal ion, driven by the degree of orbital hybridization at the heterointerface via selective p -d orbital coupling. This Letter identifies a selective mechanism for modifying the molecule-substrate interaction which impacts the growth behavior of transitionmetal- incorporated organic molecules on a technologically relevant substrate for silicon-based devices. C1 [Wagner, Sean R.; Feng, Jiagui; Zhang, Pengpeng] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Huang, Bing; Park, Changwon; Yoon, Mina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wagner, SR (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM myoon@ornl.gov; zhang@pa.msu.edu RI Yoon, Mina/A-1965-2016; Park, Changwon/B-3417-2016; Huang, Bing/D-8941-2011 OI Yoon, Mina/0000-0002-1317-3301; Park, Changwon/0000-0002-1788-045X; Huang, Bing/0000-0001-6735-4637 FU U.S. Department of Energy Office of Science Early Career Research Program through the Office of Basic Energy Sciences [DE-SC0006400]; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Materials Sciences and Engineering Divisions, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Experiment work was supported by the U.S. Department of Energy Office of Science Early Career Research Program (Grant No. DE-SC0006400) through the Office of Basic Energy Sciences. Theory work (C.P. and M.Y.) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy and partly (B. H.) supported by the Materials Sciences and Engineering Divisions, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank R. R. Lunt and C. J. Traverse for aiding in the molecular purification process. NR 60 TC 5 Z9 5 U1 6 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 26 PY 2015 VL 115 IS 9 AR 096101 DI 10.1103/PhysRevLett.115.096101 PG 6 WC Physics, Multidisciplinary SC Physics GA CP7KJ UT WOS:000360065900010 PM 26371664 ER PT J AU Morgan, TJ Turn, SQ George, A AF Morgan, Trevor James Turn, Scott Q. George, Anthe TI Fast Pyrolysis Behavior of Banagrass as a Function of Temperature and Volatiles Residence Time in a Fluidized Bed Reactor SO PLOS ONE LA English DT Article ID FLASH PYROLYSIS; ELEPHANT GRASS; BIO-OIL; SECONDARY REACTIONS; BIOMASS; PRODUCTS; WOOD; GASIFICATION; FEATURES; CHARCOAL AB A reactor was designed and commissioned to study the fast pyrolysis behavior of banagrass as a function of temperature and volatiles residence time. Four temperatures between 400 and 600 degrees C were examined as well as four residence times between similar to 1.0 and 10 seconds. Pyrolysis product distributions of bio-oil, char and permanent gases were determined at each reaction condition. The elemental composition of the bio-oils and chars was also assessed. The greatest bio-oil yield was recorded when working at 450 degrees C with a volatiles residence time of 1.4 s, similar to 37 wt% relative to the dry ash free feedstock (excluding pyrolysis water). The amounts of char (organic fraction) and permanent gases under these conditions are similar to 4 wt% and 8 wt% respectively. The bio-oil yield stated above is for 'dry' bio-oil after rotary evaporation to remove solvent, which results in volatiles and pyrolysis water being removed from the bio-oil. The material removed during drying accounts for the remainder of the pyrolysis products. The 'dry' bio-oil produced under these conditions contains similar to 56 wt% carbon which is similar to 40 wt% of the carbon present in the feedstock. The oxygen content of the 450 degrees C, 1.4 s 'dry' bio-oil is similar to 38 wt%, which accounts for similar to 33 wt% of the oxygen in the feedstock. At higher temperature or longer residence time less bio-oil and char is recovered and more gas and light volatiles are produced. Increasing the temperature has a more significant effect on product yields and composition than increasing the volatiles residence time. At 600 degrees C and a volatiles residence time of 1.2 seconds the bio-oil yield is similar to 21 wt% of the daf feedstock, with a carbon content of 64 wt% of the bio-oil. The bio-oil yield from banagrass is significantly lower than from woody biomass or grasses such as switchgrass or miscanthus, but is similar to barley straw. The reason for the low bio-oil yield from banagrass is thought to be related to its high ash content (8.5 wt% dry basis) and high concentration of alkali and alkali earth metals (totaling similar to 2.8 wt% relative to the dry feedstock) which are catalytic and increase cracking reactions during pyrolysis. C1 [Morgan, Trevor James; Turn, Scott Q.] Univ Hawaii Manoa, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. [George, Anthe] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. RP Morgan, TJ (reprint author), Univ Hawaii Manoa, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. EM morgatr@gmail.com OI Aburto, Jorge/0000-0002-8282-6046 FU U.S. Department of Energy (Cooperative Agreement) [DE-EE0003507] FX This work was conducted under the Hawai'i Energy Sustainability Program with funding from the U.S. Department of Energy (Cooperative Agreement #DE-EE0003507). The funding was received by SQT. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 45 TC 2 Z9 2 U1 3 U2 17 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 26 PY 2015 VL 10 IS 8 AR e0136511 DI 10.1371/journal.pone.0136511 PG 28 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP7LO UT WOS:000360069400131 PM 26308860 ER PT J AU Choudhury, S Aguiar, JA Fluss, MJ Hsiung, LL Misra, A Uberuaga, BP AF Choudhury, Samrat Aguiar, Jeffery A. Fluss, Michael J. Hsiung, Luke L. Misra, Amit Uberuaga, Blas P. TI Non-uniform Solute Segregation at Semi-Coherent Metal/Oxide Interfaces SO SCIENTIFIC REPORTS LA English DT Article ID METAL-CERAMIC INTERFACES; HETEROPHASE INTERFACES; ADHESION; ENERGY; SUBNANOSCALE; RESOLUTION; NANOSCALE; STABILITY; EVOLUTION; MISFIT AB The properties and performance of metal/oxide nanocomposites are governed by the structure and chemistry of the metal/oxide interfaces. Here we report an integrated theoretical and experimental study examining the role of interfacial structure, particularly misfit dislocations, on solute segregation at a metal/oxide interface. We find that the local oxygen environment, which varies significantly between the misfit dislocations and the coherent terraces, dictates the segregation tendency of solutes to the interface. Depending on the nature of the solute and local oxygen content, segregation to misfit dislocations can change from attraction to repulsion, revealing the complex interplay between chemistry and structure at metal/oxide interfaces. These findings indicate that the solute chemistry at misfit dislocations is controlled by the dislocation density and oxygen content. Fundamental thermodynamic concepts - the Hume-Rothery rules and the Ellingham diagram - qualitatively predict the segregation behavior of solutes to such interfaces, providing design rules for novel interfacial chemistries. C1 [Choudhury, Samrat; Aguiar, Jeffery A.; Misra, Amit; Uberuaga, Blas P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fluss, Michael J.; Hsiung, Luke L.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Choudhury, S (reprint author), Univ Idaho, Moscow, ID 83844 USA. EM metsam4@yahoo.com RI Choudhury, Samrat/B-4115-2009; OI Aguiar, Jeffery/0000-0001-6101-4762 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; Laboratory Directed Research and Development program at Los Alamos National Laboratory (LANL) [20130118DR]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396] FX The authors acknowledge the Center for Materials at Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026 for supporting the calculations of interfacial structure and Cr segregation and funding from the Laboratory Directed Research and Development program at Los Alamos National Laboratory (LANL) under project number 20130118DR for supporting the segregation calculations of the other solutes. Experimental microscopy was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. JAA further acknowledges the Lawrence Livermore National Laboratory graduate scholar program. One of the authors (SC) would like to thank Dr. Christopher Taylor from Ohio State University for helpful discussions. This research used resources provided by the LANL Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. NR 42 TC 4 Z9 4 U1 2 U2 19 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 26 PY 2015 VL 5 AR 13086 DI 10.1038/srep13086 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP7ED UT WOS:000360049100001 PM 26306812 ER PT J AU Ciovati, G Dhakal, P Matalevich, J Myneni, G Schmidt, A Iversen, J Matheisen, A Singer, W AF Ciovati, G. Dhakal, P. Matalevich, J. Myneni, G. Schmidt, A. Iversen, J. Matheisen, A. Singer, W. TI Mechanical properties of niobium radio-frequency cavities SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Strain measurement; Mechanical properties; Niobium ID HIGH RRR NIOBIUM; SRF CAVITIES; TEXTURE AB Radio-frequency cavities made of bulk niobium are one of the components used in modern particle accelerators. The mechanical stability is an important aspect of cavity design, which typically relies on finite-element analysis simulations using material properties from tensile tests on sample. This contribution presents the results of strain and resonant frequency measurements as a function of a uniform pressure up to 620 kPa, applied to single-cell niobium cavities with different crystallographic structure, purity and treatments. In addition, burst tests of high-purity multi-cell cavities with different crystallographic structures have been conducted up to the tensile strength of the material. Finite-element analysis of the single-cell cavity geometry is in good agreement with the observed behavior in the elastic regime assuming a Young's modulus value of 88.5 GPa and a Poisson's ratio of 0.4, regardless of crystallographic structure, purity or treatment. However, the measured yield strength and tensile strength depend on crystallographic structure, material purity and treatment. In particular, the results from this study show that the mechanical properties of niobium cavities made from ingot material with large crystals are comparable to those of cavities made of fine-grain niobium. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ciovati, G.; Dhakal, P.; Matalevich, J.; Myneni, G.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Schmidt, A.; Iversen, J.; Matheisen, A.; Singer, W.] DESY, D-22607 Hamburg, Germany. RP Ciovati, G (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM gciovati@jlab.org FU Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX We would like to acknowledge our colleagues from Jefferson Lab: B. Carpenter, J. Henry, P. Kneisel, J. Mammosser, S. Yang and S. Dutton for helping with the work on single-cell cavities and J. Spradlin for the RRR measurements. We would also like to thank H. Roy of Micro-Measurements for many suggestions related to strain gage installation. This manuscript has been authored by Jefferson Science Associates, LLC under U.S. DOE Contract no. DE-AC05-06OR23177. The U.S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce this manuscript for U.S. Government purposes. NR 41 TC 3 Z9 3 U1 2 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD AUG 26 PY 2015 VL 642 BP 117 EP 127 DI 10.1016/j.msea.2015.06.095 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CO4YR UT WOS:000359167300015 ER PT J AU Bud'ko, SL Kong, T Ma, XM Canfield, PC AF Bud'ko, Sergey L. Kong, Tai Ma, Xiaoming Canfield, Paul C. TI Study of Fe-57 Mossbauer effect in RFe2Zn20 (R = Lu, Yb, Gd) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE Mossbauer effect; hyperfine parameters; ferromagnetism; RFe2Zn20 ID CO AB We report measurements of Fe-57 Mossbauer spectra for RFe2Zn20 (R = Lu, Yb, Gd) from similar to 4.5 K to room temperature. The obtained isomer shift values are very similar for all three compounds, their temperature dependence was analyzed within the Debye model and resulted in an estimate of the Debye temperatures of 450-500 K. The values of quadrupole splitting at room temperature change with the cubic lattice constant a in a linear fashion. For GdFe2Zn20, ferromagnetic order is seen as an appearance of a sextet in the spectra. The Fe-57 site hyperfine field for T -> 0 was evaluated to be similar to 2.4 T. C1 [Bud'ko, Sergey L.; Kong, Tai; Ma, Xiaoming; Canfield, Paul C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Bud'ko, Sergey L.; Kong, Tai; Ma, Xiaoming; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ma, Xiaoming] Lanzhou Univ, Key Lab Magnetism & Magnet Mat, Minist Educ, Inst Appl Magnet, Lanzhou 730000, Gansu, Peoples R China. RP Bud'ko, SL (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM budko@ameslab.gov OI Kong, Tai/0000-0002-5064-3464 FU US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; China Scholarship Council FX We are very grateful to D Ryan, for the critical reading of the manuscript and many useful suggestions. We thank S Jua for synthesis of some early samples of RFe2Zn20 and Udhara Kaluarachchi for help in preparation of the figure 1. Work at the Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. XM was supported in part by the China Scholarship Council. NR 15 TC 3 Z9 3 U1 1 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 26 PY 2015 VL 27 IS 33 AR 336003 DI 10.1088/0953-8984/27/33/336003 PG 6 WC Physics, Condensed Matter SC Physics GA CO3SQ UT WOS:000359080100016 PM 26241786 ER PT J AU Nakashima, K Stoller, RE Xu, HX AF Nakashima, Kenichi Stoller, Roger E. Xu, Haixuan TI Recombination radius of a Frenkel pair and capture radius of a self-interstitial atom by vacancy clusters in bcc Fe SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE point defect recombination; bcc iron; reaction radius; kinetic Monte Carlo ID DAMAGE EVOLUTION; RADIATION-DAMAGE; ALPHA-IRON; SIMULATION; TEMPERATURE AB The recombination radius of a Frenkel pair is a fundamental parameter for the object kinetic Monte Carlo (OKMC) and mean field rate theory (RT) methods that are used to investigate irradiation damage accumulation in irradiated materials. The recombination radius in bcc Fe has been studied both experimentally and numerically, however there is no general consensus about its value. The detailed atomistic processes of recombination also remain uncertain. Values from 1.0a(0) to 3.3a(0) have been employed as a recombination radius in previous studies using OKMC and RT. The recombination process of a Frenkel pair is investigated at the atomic level using the self-evolved atomistic kinetic Monte Carlo (SEAKMC) method in this paper. SEAKMC calculations reveal that a self-interstitial atom recombines with a vacancy in a spontaneous reaction from several nearby sites following characteristic pathways. The recombination radius of a Frenkel pair is estimated to be 2.26a(0) by taking the average of the recombination distances from 80 simulation cases. In addition, we apply these procedures to the capture radius of a self-interstitial atom by a vacancy cluster. The capture radius is found to gradually increase with the size of the vacancy cluster. The fitting curve for the capture radius is obtained as a function of the number of vacancies in the cluster. C1 [Nakashima, Kenichi; Stoller, Roger E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Nakashima, Kenichi] Cent Res Inst Elect Power Ind, Mat Sci Res Lab, Komae, Tokyo 2018511, Japan. [Xu, Haixuan] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Nakashima, K (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM ken-ichi@criepi.denken.or.jp RI Xu, Haixuan/C-9841-2009 FU Center for Defect Physics, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences; Central Research Institute of Electric Power Industry FX Research at the Oak Ridge National Laboratory was supported as part of the Center for Defect Physics, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. KN was supported at ORNL by the Central Research Institute of Electric Power Industry. NR 20 TC 2 Z9 2 U1 5 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 26 PY 2015 VL 27 IS 33 AR 335401 DI 10.1088/0953-8984/27/33/335401 PG 7 WC Physics, Condensed Matter SC Physics GA CO3SQ UT WOS:000359080100004 PM 26241190 ER PT J AU Oh, HJ Coh, S Cohen, ML AF Oh, Hyungju Coh, Sinisa Cohen, Marvin L. TI Calculation of the specific heat of optimally K-doped BaFe2As2 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE optimally K-doped BaFe2As2; specific heat; semi-empirical density functional theory ID ELECTRONIC-STRUCTURE; IRON; SUPERCONDUCTIVITY; SYSTEMS; MAGNETISM; STATES AB The calculated specific heat of optimally K-doped BaFe2As2 in density functional theory is about five times smaller than that found in the experiment. We report that by adjusting the potential on the iron atom to be slightly more repulsive for electrons improves the calculated heat capacity as well as the electronic band structure of Ba0.6K0.4Fe2As2. In addition, structural and magnetic properties are moved in the direction of experimental values. Applying the same correction to the antiferromagnetic state, we find that the electron-phonon coupling is strongly enhanced. C1 [Oh, Hyungju] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Oh, HJ (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM xtom97@civet.berkeley.edu FU National Science Foundation (electronic and magnetic structure calculation) [DMR10-1006184]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy (electron-phonon calculation) [DE-AC02-05CH11231] FX We thank Profs N E Phillips and R J Birgeneau for useful discussions. This work was supported by National Science Foundation Grant No. DMR10-1006184 (electronic and magnetic structure calculation) and by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231 (electron-phonon calculation). Computational resources have been provided by the DOE at Lawrence Berkeley National Laboratory's NERSC facility. NR 38 TC 0 Z9 0 U1 4 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 26 PY 2015 VL 27 IS 33 AR 335504 DI 10.1088/0953-8984/27/33/335504 PG 6 WC Physics, Condensed Matter SC Physics GA CO3SQ UT WOS:000359080100008 PM 26241358 ER PT J AU Ruotsalainen, KO Sahle, CJ Ritschel, T Geck, J Hosoda, M Bell, C Hikita, Y Hwang, HY Fister, TT Gordon, RA Hamalainen, K Hakala, M Huotari, S AF Ruotsalainen, Kari O. Sahle, Christoph J. Ritschel, Tobias Geck, Jochen Hosoda, Masayuki Bell, Christopher Hikita, Yasuyuki Hwang, Harold Y. Fister, Tim T. Gordon, Robert A. Hamalainen, Keijo Hakala, Mikko Huotari, Simo TI Inelastic x-ray scattering in heterostructures: electronic excitations in LaAlO3/SrTiO3 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE inelastic x-ray scattering; heterostructures; electronic structure ID ENERGY-LOSS SPECTROSCOPY; SEMICONDUCTING SRTIO3; SUPERCONDUCTIVITY; FERROMAGNETISM; INTERFACES; COEXISTENCE; DEPENDENCE; VALENCE; STATE AB We present an investigation of the valence-electron excitation spectra including the collective plasmon modes of SrTiO3, LaAlO3 and their heterostructures with non-resonant inelastic x-ray scattering. We analyse the spectra using calculations based on first principles and atomic multiplet models. We demonstrate the feasibility of performing valence IXS experiments in a total reflection geometry. Surprisingly, we find that the plasmon, interband and semicore excitations in multilayers are well described as a superposition of bulk-compound spectra even in a superstructure composing of layers of only one atomic layer thickness. C1 [Ruotsalainen, Kari O.; Sahle, Christoph J.; Hamalainen, Keijo; Hakala, Mikko; Huotari, Simo] Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland. [Sahle, Christoph J.] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France. [Ritschel, Tobias; Geck, Jochen] Leibniz Inst Solid State & Mat Res IFW Dresden, D-01069 Dresden, Germany. [Hosoda, Masayuki; Bell, Christopher; Hikita, Yasuyuki; Hwang, Harold Y.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Hosoda, Masayuki] Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan. [Hwang, Harold Y.] Stanford Univ, Dept Appl Phys, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Fister, Tim T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Gordon, Robert A.] PNCSRF CLS, Argonne, IL USA. RP Ruotsalainen, KO (reprint author), Univ Helsinki, Dept Phys, POB 64, FI-00014 Helsinki, Finland. EM kari.ruotsalainen@helsinki.fi RI Hamalainen, Keijo/A-3986-2010; Bell, Christopher/B-8785-2009; Yambo, MBPT Code/O-4564-2015; Hikita, Yasuyuki/F-5600-2011 OI Hamalainen, Keijo/0000-0002-9234-9810; Bell, Christopher/0000-0003-4732-0354; Hikita, Yasuyuki/0000-0002-7748-8329 FU Academy of Finland [1260204, 1256211, 1127462, 1259526, 1254065]; University of Helsinki Research Funds; Department of Energy's Office of Science [DE-AC02-06CH11]; US Department of Energy-Basic Energy Sciences; Canadian Light Source and its funding partners; University of Washington; Advanced Photon Source; US DOE [DE-AC02-06CH11357]; Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515]; German Research Foundation through the Emmy Noether Program [GE-1647/2-1]; Research Training Group [DFG-GRK 1621] FX We thank M Aramini and T Talka for assistance in sample characterization. Computational resources were provided by CSC-Centre for Scientific Computation Espoo, Finland. Funding was provided by the Academy of Finland (Grants 1260204, 1256211, 1127462, 1259526 and 1254065) and University of Helsinki Research Funds. T Fister was supported by the Department of Energy's Office of Science under contract award number DE-AC02-06CH11. PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy-Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. MH, CB, YH and HYH acknowledge support from the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract DE-AC02-76SF00515. J Geck and T Ritschel gratefully acknowledge the support by the German Research Foundation through the Emmy Noether Program (Grant GE-1647/2-1) and the Research Training Group DFG-GRK 1621. NR 64 TC 1 Z9 1 U1 3 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 26 PY 2015 VL 27 IS 33 AR 335501 DI 10.1088/0953-8984/27/33/335501 PG 10 WC Physics, Condensed Matter SC Physics GA CO3SQ UT WOS:000359080100005 PM 26221981 ER PT J AU Glatz, A Galda, A Varlamov, AA AF Glatz, A. Galda, A. Varlamov, A. A. TI Effect of fluctuations on the NMR relaxation beyond the Abrikosov vortex state SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; MAGNETIC-FIELD; SPIN SUSCEPTIBILITY; YBA2CU3O7-DELTA AB The effect of fluctuations on the nuclear magnetic resonance (NMR) relaxation rate W = T-1(-1) is studied in a complete phase diagram of a two-dimensional superconductor above the upper critical field line H-c2(T). In the region of relatively high temperatures and low magnetic fields, the relaxation rate W is determined by two competing effects. The first one is its decrease in the result of suppression of the quasiparticle density of states (DOS) due to formation of fluctuation Cooper pairs (FCPs). The second one is a specific, purely quantum relaxation process of the Maki-Thompson (MT) type, which for low field leads to an increase of the relaxation rate. The latter describes particular fluctuation processes involving self-pairing of a single electron on self-intersecting trajectories of a size up to phase-breaking length l(phi) which becomes possible due to an electron spin-flip scattering event at a nucleus. As a result, different scenarios with either growth or decrease of the NMR relaxation rate are possible upon approaching the normal-metal-type-II superconductor transition. The character of fluctuations changes along the line H-c2(T) from the thermal long-wavelength type in weak magnetic fields to the clusters of rotating FCPs in fields comparable to H-c2(0). We find that below the well-defined temperature T-0(*) approximate to 0.6T(c0), the MT process becomes ineffective even in the absence of intrinsic pair breaking. The small scale of the FCP rotations xi(xy) in such high fields impedes formation of long (less than or similar to l(phi)) self-intersecting trajectories, causing the corresponding relaxation mechanism to lose its efficiency. This reduces the effect of superconducting fluctuations in the domain of high fields and low temperatures to just the suppression of quasiparticle DOS, analogous to the Abrikosov vortex phase below the H-c2(T) line. C1 [Glatz, A.; Galda, A.; Varlamov, A. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60639 USA. [Glatz, A.] Univ Illinois, Dept Phys, De Kalb, IL 60115 USA. [Varlamov, A. A.] CNR SPIN, I-00133 Rome, Italy. RP Glatz, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 South Cass Ave, Argonne, IL 60639 USA. FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences FX We express our deep gratitude to A. Rigamonti and A. Lasciafari for attracting our attention to their experiments and numerous elucidating discussions. This work was partially supported by the Scientific Discovery through Advanced Computing (SciDAC) program funded by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences. NR 25 TC 0 Z9 0 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 25 PY 2015 VL 92 IS 5 AR 054513 DI 10.1103/PhysRevB.92.054513 PG 10 WC Physics, Condensed Matter SC Physics GA CS6QT UT WOS:000362206700004 ER PT J AU Chen, Y Rangasamy, E Lang, CD An, K AF Chen, Yan Rangasamy, Ezhiylmurugan Lang, Chengdu An, Ke TI Origin of High Li+ Conduction in Doped Li7La3Zr2O12 Garnets SO CHEMISTRY OF MATERIALS LA English DT Article ID ION CONDUCTORS; SOLID ELECTROLYTES; CUBIC LI7LA3ZR2O12; LITHIUM GARNET; AL; TRANSPORT; BATTERY C1 [Chen, Yan; An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Rangasamy, Ezhiylmurugan; Lang, Chengdu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP An, K (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM kean@ornl.gov RI An, Ke/G-5226-2011; Chen, Yan/H-4913-2014 OI An, Ke/0000-0002-6093-429X; Chen, Yan/0000-0001-6095-1754 FU Division of Materials Sciences and Engineering, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); Scientific User Facilities Division, BES, DOE FX This work was supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). Neutron work at ORNL's Spa Ration Neutron Source was sponsored by the Scientific User Facilities Division, BES, DOE. The authors thank Mrs. R. Mills, Mr. M. Frost, and Mr. H. Skorpenske from SNS for their technical support. The authors thank Mrs. G. Zhu for the technical support. NR 31 TC 7 Z9 7 U1 9 U2 61 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5491 EP 5494 DI 10.1021/acs.chemmater.5b02521 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700007 ER PT J AU Schroder, K Avarado, J Yersak, TA Li, JC Dudney, N Webb, LJ Meng, YS Stevenson, KJ AF Schroder, Kjell Avarado, Judith Yersak, Thomas A. Li, Juchuan Dudney, Nancy Webb, Lauren J. Meng, Ying Shirley Stevenson, Keith J. TI The Effect of Fluoroethylene Carbonate as an Additive on the Solid Electrolyte Interphase on Silicon Lithium-Ion Electrodes SO CHEMISTRY OF MATERIALS LA English DT Article ID FREE GRAPHITE-ELECTRODES; BATTERY ANODES; SURFACE-CHEMISTRY; VINYLENE CARBONATE; THERMAL-STABILITY; TOF-SIMS; ELECTROCHEMICAL PERFORMANCE; PHOTOELECTRON-SPECTROSCOPY; REDUCTION-MECHANISMS; LAYER DEPOSITION AB Fluoroethylene carbonate (FEC) has become a standard electrolyte additive for use with silicon negative electrodes, but how FEC affects solid electrolyte interphase (SET) formation on the silicon anode's surface is still not well understood. Herein, SET formed from LiPF6-based carbonate electrolytes, with and without FEC, were investigated on 50 nm thick amorphous silicon thin film electrodes to understand the role of FEC on silicon electrode surface reactions. In contrast to previous work, anhydrous and anoxic techniques were used to prevent air and moisture contamination of prepared SET films. This allowed for accurate characterization of the SEI structure and composition by X-ray photoelectron spectroscopy and time-of-flight secondary ion mass spectrometry depth profiling. These results show that FEC reduction leads to fluoride ion and LiF formation, consistent with previous computational and experimental results. Surprisingly, we also find that these species decrease lithium-ion solubility and increase the reactivity of the silicon surface. We conclude that the effectiveness of FEC at improving the Coulombic efficiency and capacity retention is due to fluoride ion formation from reduction of the electrolyte, which leads to the chemical attack of any silicon-oxide surface passivation layers and the formation of a kinetically stable SET comprising predominately lithium fluoride and lithium oxide. C1 [Schroder, Kjell; Webb, Lauren J.; Stevenson, Keith J.] Univ Texas Austin, Mat Sci & Engn Program, Texas Mat Inst, Austin, TX 78712 USA. [Schroder, Kjell; Webb, Lauren J.; Stevenson, Keith J.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Avarado, Judith; Yersak, Thomas A.; Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Li, Juchuan; Dudney, Nancy] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37830 USA. RP Webb, LJ (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Texas Mat Inst, Austin, TX 78712 USA. EM lwebb@cm.utexas.edu; shmeng@ucsd.edu; stevenson@cm.utexas.edu RI Li, Juchuan/A-2992-2009; Alvarado, Judith/K-6108-2016 OI Li, Juchuan/0000-0002-6587-5591; FU program "Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)", an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001091]; Office of Vehicle Technologies, U.S. Department of Energy [DE-AC02-05CH11231]; Advanced Battery Materials Research (BMR) Program [7073923]; California Institute for Energy and Environment (CIEE) Subaward from the Multiple Campus Award program of the California Energy Commission [PODR05-S16] FX This material is based on work supported as part of the program "Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)", an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001091. Y.S.M. and J.A. would like to acknowledge the support from the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 7073923 under the Advanced Battery Materials Research (BMR) Program and a California Institute for Energy and Environment (CIEE) Subaward No. PODR05-S16 from the Multiple Campus Award program of the California Energy Commission. NR 76 TC 31 Z9 31 U1 30 U2 174 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5531 EP 5542 DI 10.1021/acs.chemmater.5b01627 PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700012 ER PT J AU Tsai, HH Nie, WY Cheruku, P Mack, NH Xu, P Gupta, G Mohite, AD Wang, HL AF Tsai, Hsinhan Nie, Wanyi Cheruku, Pradeep Mack, Nathan H. Xu, Ping Gupta, Gautam Mohite, Aditya D. Wang, Hsing-Lin TI Optimizing Composition and Morphology for Large-Grain Perovskite Solar Cells via Chemical Control SO CHEMISTRY OF MATERIALS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITES; SOLUTION-PROCESSED PEROVSKITE; TRIHALIDE PEROVSKITES; HIGH-PERFORMANCE; LEAD TRIHALIDE; EFFICIENT; CHLORIDE; CH3NH3PBI3; DEPOSITION; CRYSTALLIZATION AB We report solid iodine as a precursor additive for achieving purified organometallic perovskite crystals. By adding iodine, we found that the reaction can be pushed toward pure iodine phase rather than the kinetically favored chlorine phase. This approach can be applied in large crystalline perovskite solar cells and improved the average efficiency from 9.83% to 15.58%. C1 [Tsai, Hsinhan; Cheruku, Pradeep; Mack, Nathan H.; Xu, Ping; Wang, Hsing-Lin] Los Alamos Natl Lab, PCS, Div Chem, Los Alamos, NM 87545 USA. [Nie, Wanyi; Gupta, Gautam; Mohite, Aditya D.] Los Alamos Natl Lab, Mat Phys & Applicat Div, MPA 11, Los Alamos, NM 87545 USA. RP Mohite, AD (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, MPA 11, POB 1663, Los Alamos, NM 87545 USA. EM amohite@lanl.gov; hwang@lanl.gov FU Laboratory Directed Research and Development (LDRD) program under Department of Energy (DOE); Basic Energy Science (BES), Biomaterials program, Materials Sciences and Engineering Division; Los Alamos Director Funded Postdoctoral Fellowship FX This research is supported by the Laboratory Directed Research and Development (LDRD) program, under the auspices of Department of Energy (DOE). H.T. is partially supported by Basic Energy Science (BES), Biomaterials program, Materials Sciences and Engineering Division. W.N., P.C., and P.X. are supported by Los Alamos Director Funded Postdoctoral Fellowship. NR 39 TC 19 Z9 19 U1 15 U2 108 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5570 EP 5576 DI 10.1021/acs.chemmater.5b02378 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700016 ER PT J AU Han, F Wang, D Malliakas, CD Sturza, M Chung, DY Wan, XG Kanatzidis, MG AF Han, Fei Wang, Di Malliakas, Christos D. Sturza, Mihai Chung, Duck Young Wan, Xiangang Kanatzidis, Mercouri G. TI (CaO)(FeSe): A Layered Wide-Gap Oxychalcogenide Semiconductor SO CHEMISTRY OF MATERIALS LA English DT Article ID MAGNETIC-PROPERTIES; 43 K; SUPERCONDUCTIVITY; COMPOUND; FESE; SR; BA; SE AB A new iron-oxychalcogenide (CaO)(FeSe) was obtained which crystallizes in the orthorhombic space group Pnma (No. 62) with a = 5.9180(12) angstrom, b = 3.8802(8) angstrom, c = 13.193(3) angstrom. The unique structure of (CaO)(FeSe) is built up of a quasi-two-dimensional network of corrugated infinite layers of corner-shared FeSe2O2 tetrahedra that extend in the ab plane. The corrugated layers composed of corner-shared FeSe2O2 tetrahedra stack along the c axis with Ca2+ cations sandwiched between the layers. Optical spectroscopy and resistivity measurements reveal semiconducting behavior with an indirect optical band gap of around 1.8 eV and an activation energy of 0.19(1) eV. Electronic band structure calculations at the density function level predict a magnetic configuration as ground state and confirm the presence of an indirect wide gap in (CaO)(FeSe). C1 [Han, Fei; Malliakas, Christos D.; Sturza, Mihai; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Wang, Di; Wan, Xiangang] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Sch Phys, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013 OI Han, Fei/0000-0001-7782-2713 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF of China [11374137, 91122035, 11174124] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Use of the Center for Nanoscale Materials, including resources in the Electron Microscopy Center, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Work done at Nanjing University (by D.W. and X.W.) was supported by the NSF of China (Grant Nos. 11374137, 91122035, and 11174124). NR 42 TC 3 Z9 3 U1 19 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5695 EP 5701 DI 10.1021/acs.chemmater.5b02164 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700030 ER PT J AU Wang, LP Bai, JM Gao, P Wang, XY Looney, JP Wang, F AF Wang, Liping Bai, Jianming Gao, Peng Wang, Xiaoya Looney, J. Patrick Wang, Feng TI Structure Tracking Aided Design and Synthesis of Li3V2(PO4)(3) Nanocrystals as High-Power Cathodes for Lithium Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID ELECTROCHEMICAL PROPERTIES; ROOM-TEMPERATURE; CAPACITY; PERFORMANCE; COMPOSITES; NANOCOMPOSITE; PHASE; OXIDE AB Preparing new electrode materials with synthetic control of phases and electrochemical properties is desirable for battery applications but hardly achievable without knowing how the synthesis reaction proceeds. Herein, we report on structure tracking-aided design and synthesis of single-crystalline Li3V2(PO4)(3) (LVP) nanoparticles with extremely high rate capability. A comprehensive investigation was made to the local structural orderings of the involved phases and their evolution toward forming LVP phase using in situ/ex situ synchrotron X-ray and electron-beam diffraction, spectroscopy, and imaging techniques. The results shed light on the thermodynamics and kinetics of synthesis reactions and enabled the design of a cost-efficient synthesis protocol to make nanocrystalline LVP, wherein solvothermal treatment is a crucial step leading to an amorphous intermediate with local structural ordering resembling that of LVP, which, upon calcination at moderate temperatures, rapidly transforms into the desired LVP phase. The obtained LVP particles are about 50 nm, coated with a thin layer of amorphous carbon and featured with excellent cycling stability and rate capability - 95% capacity retention after 200 cycles and 66% theoretical capacity even at a current rate of 10 C. The structure tracking based method we developed in this work offers a new way of designing battery electrodes with synthetic control of material phases and properties. C1 [Wang, Liping; Gao, Peng; Wang, Xiaoya; Looney, J. Patrick; Wang, Feng] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Bai, Jianming] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Wang, Liping] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Sch Microelect & Solid State Elect, Chengdu 610054, Sichuan, Peoples R China. [Wang, Xiaoya] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11790 USA. RP Wang, F (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. EM fwang@bnl.gov RI Gao, Peng/B-4675-2012; Bai, Jianming/O-5005-2015; Wang, Feng/C-1443-2016; Wang, Xiaoya/F-9394-2015 OI Wang, Feng/0000-0003-4068-9212; FU U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy [DE-SC0012704]; Laboratory Directed Research and Development (LDRD) program at Brookhaven National Laboratory [13-022]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX We thank John Johnson, Steven Ehrlich, and Lihua Zhang for technical support and thank Tiffany Bowman for graphic design. This work is supported by the U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy under the Advanced Battery Materials Research (BMR) program, Contract No. DE-SC0012704. P.G. was supported by the Laboratory Directed Research and Development (LDRD) program at Brookhaven National Laboratory, under Award No. 13-022. Research carried out at the Center for Functional Nanomaterials and the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 27 TC 9 Z9 9 U1 16 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5712 EP 5718 DI 10.1021/acs.chemmater.5b02236 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700032 ER PT J AU Tian, ZQ Dai, S Jiang, DE AF Tian, Ziqi Dai, Sheng Jiang, De-en TI Stability and Core-Level Signature of Nitrogen Dopants in Carbonaceous Materials SO CHEMISTRY OF MATERIALS LA English DT Article ID ORDERED MESOPOROUS CARBONS; OXYGEN REDUCTION REACTION; CARBIDE-DERIVED CARBON; LITHIUM-ION BATTERIES; X-RAY-ABSORPTION; DOPED GRAPHENE; POLYPYRROLE NANOSPHERES; NANOPOROUS CARBON; ANODE MATERIALS; CO2 ADSORPTION AB Nitrogen doping is an important strategy in tuning the properties and functions of carbonaceous materials. But the chemical speciation of the nitrogen groups in the sp(2)-carbon framework has not been firmly established. Here we address two important questions in nitrogen doping of carbonaceous materials from a computational approach: the relative stability of different nitrogen groups and their X-ray photoelectron spectrum (XPS) signatures of the core-level (N 1s) electron binding energies. Four types of nitrogen groups (graphitic, pyrrolic, aza-pyrrolic, and pyrichnic) in 69 model compounds have been examined. Computed formation energies indicate that pyrrolic and pyridinic nitrogens are significantly more stable (by about 110 kJ/mol) than graphitic and aza-pyrrolic nitrogens. This stability trend can be understood from the Clar's sextet rule. Predicted N is binding energies show relatively high consistency among each dopant type, thereby offering a guide to identify nitrogen groups. The relative stability coupled with predicted N is binding energies can explain the temperature-dependent change in the experimental XPS spectra. The present work therefore provides fundamental insights into nitrogen dopants in carbonaceous materials, which will be useful in understanding the applications of nitrogen-doped carbons in electric energy storage, electrocatalysis, and carbon capture. C1 [Tian, Ziqi; Jiang, De-en] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Jiang, DE (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. EM de-en.jiang@ucr.edu RI Dai, Sheng/K-8411-2015; Jiang, De-en/D-9529-2011 OI Dai, Sheng/0000-0002-8046-3931; Jiang, De-en/0000-0001-5167-0731 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05-CH11231] FX This work was supported by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05-CH11231. NR 54 TC 6 Z9 6 U1 10 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 25 PY 2015 VL 27 IS 16 BP 5775 EP 5781 DI 10.1021/acs.chemmater.5b02370 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0YE UT WOS:000360323700039 ER PT J AU Chen, XC Kortright, JB Balsara, NP AF Chen, X. Chelsea Kortright, Jeffrey B. Balsara, Nitash P. TI Water Uptake and Proton Conductivity in Porous Block Copolymer Electrolyte Membranes SO MACROMOLECULES LA English DT Article ID X-RAY-SCATTERING; TRANSPORT-PROPERTIES; TRIBLOCK COPOLYMERS; HOMOPOLYMER BLENDS; PHASE-EQUILIBRIA; MORPHOLOGY; MICROEMULSIONS; MIXTURES; CHANNELS; BEHAVIOR AB We demonstrate that the water uptake and conductivity of proton-conducting block copolymer electrolyte membranes can be controlled systematically by the introduction of pores in the conducting domains. We start with a membrane comprising a mixture of homopolymer polystyrene (hPS) and a polystyrene-b-polyethylene-b-polystyrene (SES) copolymer. Rinsing the membranes in tetrahydrofuran and methanol results in the dissolution of hPS, leaving behind a porous membrane. The polystyrene domains in the porous SES membranes are then sulfonated to give a porous membrane with hydrophilic and hydrophobic domains. The porosity is controlled by controlling phi(v), the volume fraction of hPS in the blended membrane. The morphology of the membranes before and after sulfonation was studied by scanning transmission electron microscopy (STEM), electron tomography, and resonance soft X-ray scattering (RSoXS). The porous structures before and after sulfonation are qualitatively different. Water uptake of the sulfonated membranes increased with increasing phi(v). Proton conductivity is a nonmonotonic function of phi(v) with a maximum at phi(v) = 0.1. The introduction of microscopic pores in the conducting domain provides an additional handle for tuning water uptake and ion transport in proton-conducting membranes. C1 [Chen, X. Chelsea; Kortright, Jeffrey B.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Soft Matter Electron Microscopy Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX Primary funding for the work was provided by the Soft Matter Electron Microscopy Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract DE-AC02-05CH11231. RSoXS experiments were performed at the Advanced Light Source (ALS), Beam line 11.0.1.2. The STEM and STEM tomography experiments were performed as user projects at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory. ALS and NCEM are DOE national user facilities and are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under the same contract. We thank Anthony Young for help with RSoXS experiments, Karen Bustillo and Peter Ercius for their help with STEM tomography experiments, and Nicolas Young for help with additional flux measurements on the membranes. NR 37 TC 7 Z9 7 U1 9 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 25 PY 2015 VL 48 IS 16 BP 5648 EP 5655 DI 10.1021/acs.macromol.5b00950 PG 8 WC Polymer Science SC Polymer Science GA CQ0YL UT WOS:000360324400025 ER PT J AU Nagayama, T Mancini, RC Mayes, D Tommasini, R Florido, R AF Nagayama, T. Mancini, R. C. Mayes, D. Tommasini, R. Florido, R. TI An important criterion for reliable multi-monochromatic x-ray imager diagnostics and its impact on the reconstructed images SO HIGH POWER LASER SCIENCE AND ENGINEERING LA English DT Article DE high power laser; inertial confinement fusion; monochromatic imager; x-ray diagnostics ID PLASMAS AB Temperature and density asymmetry diagnosis is critical to advance inertial confinement fusion (ICF) science. A multi-monochromatic x-ray imager, MMI, records the spectral signature from an ICF implosion core with time resolution, 2D spatial resolution and spectral resolution. While narrow-band images and 2D space-resolved spectra from the MMI data constrain the temperature and the density spatial structure of the core, the accuracy of the images and the spectra highly depends on the quality of the MMI data and the processing tools. Here, we synthetically investigate the criterion for reliable MMI diagnostics and its effects on the accuracy of the reconstructed images. The pinhole array tilt determines the object spatial sampling efficiency and the minimum reconstruction width, w. When the spectral width associated with w is significantly narrower than the spectral linewidth, the line images reconstructed from the MMI data become reliable. The MMI setup has to be optimized for every application to meet this criterion for reliable ICF diagnostics. C1 [Nagayama, T.; Mancini, R. C.; Mayes, D.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. [Tommasini, R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Florido, R.] Univ Las Palmas Gran Canaria, Dept Fis, Las Palmas Gran Canaria 35017, Spain. RP Nagayama, T (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tnnagay@sandia.gov RI Florido, Ricardo/H-5513-2015; Tommasini, Riccardo/A-8214-2009 OI Florido, Ricardo/0000-0001-7428-6273; Tommasini, Riccardo/0000-0002-1070-3565 NR 19 TC 2 Z9 2 U1 1 U2 4 PU CAMBRIDGE UNIV PRESS PI CAMBRIDGE PA EDINBURGH BLDG, SHAFTESBURY RD, CB2 8RU CAMBRIDGE, ENGLAND SN 2095-4719 EI 2052-3289 J9 HIGH POWER LASER SCI JI High Power Laser Sci. Eng. PD AUG 25 PY 2015 VL 3 AR e23 DI 10.1017/hpl.2015.25 PG 7 WC Optics SC Optics GA CQ0HS UT WOS:000360276700001 ER PT J AU Chang, FJ Riera, A Evrin, C Sun, JC Li, HL Speck, C Weinreich, M AF Chang, FuJung Riera, Alberto Evrin, Cecile Sun, Jingchuan Li, Huilin Speck, Christian Weinreich, Michael TI Cdc6 ATPase activity disengages Cdc6 from the pre-replicative complex to promote DNA replication SO ELIFE LA English DT Article ID SACCHAROMYCES-CEREVISIAE; BUDDING YEAST; ORIGIN DNA; STRUCTURAL BASIS; MCM2-7 HELICASE; INITIATION; BINDING; PROTEIN; HYDROLYSIS; ACTIVATION AB To initiate DNA replication, cells first load an MCM helicase double hexamer at origins in a reaction requiring ORC, Cdc6, and Cdt1, also called pre-replicative complex (pre-RC) assembly. The essential mechanistic role of Cdc6 ATP hydrolysis in this reaction is still incompletely understood. Here, we show that although Cdc6 ATP hydrolysis is essential to initiate DNA replication, it is not essential for MCM loading. Using purified proteins, an ATPase-defective Cdc6 mutant 'Cdc6-E224Q' promoted MCM loading on DNA. Cdc6-E224Q also promoted MCM binding at origins in vivo but cells remained blocked in G1-phase. If after loading MCM, Cdc6-E224Q was degraded, cells entered an apparently normal S-phase and replicated DNA, a phenotype seen with two additional Cdc6 ATPase-defective mutants. Cdc6 ATP hydrolysis is therefore required for Cdc6 disengagement from the pre-RC after helicase loading to advance subsequent steps in helicase activation in vivo. C1 [Chang, FuJung; Weinreich, Michael] Van Andel Res Inst, Grand Rapids, MI 49503 USA. [Riera, Alberto; Evrin, Cecile; Speck, Christian] Univ London Imperial Coll Sci Technol & Med, Fac Med, London, England. [Sun, Jingchuan; Li, Huilin] Brookhaven Natl Lab, Dept Biosci, New York, NY USA. [Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY USA. RP Weinreich, M (reprint author), Van Andel Res Inst, Grand Rapids, MI 49503 USA. EM chris.speck@imperial.ac.uk; michael.weinreich@vai.org RI 7aVqn2, 7aVqn2/L-5089-2015; Speck, Christian/G-2882-2011 OI Speck, Christian/0000-0001-6646-1692 FU National Institutes of Health (NIH) [R01-GM74985]; National Science Foundation (NSF) [MCB-0950464]; Medical Research Council (MRC) FX National Institutes of Health (NIH) R01-GM74985 Huilin Li; National Science Foundation (NSF) MCB-0950464 Michael Weinreich; Medical Research Council (MRC) Christian Speck NR 42 TC 6 Z9 6 U1 1 U2 11 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 25 PY 2015 VL 4 AR e05795 DI 10.7554/eLife.05795 PG 14 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CQ0JE UT WOS:000360280500001 ER PT J AU Liddick, SN Walters, WB Chiara, CJ Janssens, RVF Abromeit, B Ayres, A Bey, A Bingham, CR Carpenter, MP Cartegni, L Chen, J Crawford, HL Darby, IG Grzywacz, R Harker, J Hoffman, CR Ilyushkin, S Kondev, FG Larson, N Madurga, M Miller, D Padgett, S Paulauskas, SV Rajabali, MM Rykaczewski, K Seweryniak, D Suchyta, S Zhu, S AF Liddick, S. N. Walters, W. B. Chiara, C. J. Janssens, R. V. F. Abromeit, B. Ayres, A. Bey, A. Bingham, C. R. Carpenter, M. P. Cartegni, L. Chen, J. Crawford, H. L. Darby, I. G. Grzywacz, R. Harker, J. Hoffman, C. R. Ilyushkin, S. Kondev, F. G. Larson, N. Madurga, M. Miller, D. Padgett, S. Paulauskas, S. V. Rajabali, M. M. Rykaczewski, K. Seweryniak, D. Suchyta, S. Zhu, S. TI Analogous intruder behavior near Ni, Sn, and Pb isotopes SO PHYSICAL REVIEW C LA English DT Article ID ATOMIC-NUCLEI; SHELL-MODEL; MASS NUCLEI; HALF-LIVES; STATES; ODD; COEXISTENCE; CU-69; NI-68; DECAY AB Near shell closures, the presence of unexpected states at lowenergies provides a critical test of our understanding of the atomic nucleus. New measurements for the N = 42 isotones Co-69(27) and Cu-71(29), along with recent data and calculations in the Ni isotopes, establish a full set of complementary, deformed, intruder states astride the closed-shell Ni-28 isotopes. Nuclei with a one-proton hole or one-proton particle adjacent to Z = 28 were populated in beta-decay experiments and in multinucleon transfer reactions. A beta-decaying isomer, with a 750(250)-ms half-life, has been identified in Co-69(27)42. It likely has low spin and accompanies the previously established 7/2(-) state. Complementary data for the levels of isotonic Cu-71(29)42 support the presence of a deformed, Delta J = 1 band built on the proton intruder 7/2(-) level at 981 keV. These data, together with recent studies of lower-mass Co and Cu isotopes and extensive work near Ni-68, support the view that intruder states based on particle-hole excitations accompany all closed proton shells with Z >= 28. C1 [Liddick, S. N.; Abromeit, B.; Larson, N.; Suchyta, S.] Michigan State Univ, NSCL, E Lansing, MI 48824 USA. [Liddick, S. N.; Larson, N.; Suchyta, S.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Walters, W. B.; Chiara, C. J.; Harker, J.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Chiara, C. J.; Janssens, R. V. F.; Carpenter, M. P.; Hoffman, C. R.; Seweryniak, D.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Ayres, A.; Bey, A.; Bingham, C. R.; Cartegni, L.; Grzywacz, R.; Madurga, M.; Miller, D.; Padgett, S.; Paulauskas, S. V.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Chen, J.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Crawford, H. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Nucl Sci Div, Berkeley, CA 94720 USA. [Darby, I. G.; Rajabali, M. M.] Katholieke Univ Leuven, Inst Kern & Stralingsfys, B-3001 Leuven, Belgium. [Ilyushkin, S.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Rykaczewski, K.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Liddick, SN (reprint author), Michigan State Univ, NSCL, E Lansing, MI 48824 USA. RI Carpenter, Michael/E-4287-2015; Miller, David/B-5372-2012; Hoffman, Calem/H-4325-2016; Larson, Nicole/S-5997-2016 OI Bey, Anissa/0000-0002-8035-6853; Carpenter, Michael/0000-0002-3237-5734; Miller, David/0000-0002-0426-974X; Chen, Jun/0000-0003-0447-7466; Paulauskas, Stanley/0000-0002-6479-4626; Hoffman, Calem/0000-0001-7141-9827; Larson, Nicole/0000-0003-0292-957X FU National Science Foundation [NSF-06067007]; US Department of Energy, National Nuclear Security Administration [DE-FC03-03NA00143, DE-NA0000979]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics, (Maryland) [DE-FG02-94ER40834, DE-AC05-060R23100, DE-AC02-06CH11357, DE-AC05-00OR22725] FX This material is based upon work supported by the National Science Foundation under Contract No. NSF-06067007 (NSCL), the US Department of Energy, National Nuclear Security Administration under Grant No. DE-FC03-03NA00143, and Award No. DE-NA0000979, the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Grants No. DE-FG02-94ER40834 (Maryland), No. DE-FG02-96ER40983 (UT), No. DE-AC05-060R23100 (ORAU), and under Contracts No. DE-AC02-06CH11357 (ANL) and No. DE-AC05-00OR22725 (ORNL). This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 51 TC 4 Z9 4 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 25 PY 2015 VL 92 IS 2 AR 024319 DI 10.1103/PhysRevC.92.024319 PG 7 WC Physics, Nuclear SC Physics GA CP6GZ UT WOS:000359985300001 ER PT J AU Willias, SP Chauhan, S Lo, CC Chain, PSG Motin, VL AF Willias, Stephan P. Chauhan, Sadhana Lo, Chien-Chi Chain, Patrick S. G. Motin, Vladimir L. TI CRP-Mediated Carbon Catabolite Regulation of Yersinia pestis Biofilm Formation Is Enhanced by the Carbon Storage Regulator Protein, CsrA SO PLOS ONE LA English DT Article ID ESCHERICHIA-COLI; GLYCOGEN BIOSYNTHESIS; HMS(+) PHENOTYPE; GLOBAL REGULATOR; PLAGUE; EXPRESSION; GENE; RNA; TRANSMISSION; TRANSLATION AB The natural transmission of Yersinia pestis is reliant upon biofilm blockage of the flea vector. However, the environmentally-responsive adaptive regulators which facilitate Y. pestis biofilm production in accordance with the flea midgut milieu are not well understood. We seek to establish the impact of available carbon source metabolism and storage upon Y. pestis biofilm production. Our findings demonstrate that Y. pestis biofilm production is subject to carbon catabolite regulation in which the presence of glucose impairs biofilm production; whereas, the sole metabolism of alternate carbon sources promotes robust biofilm formation. This observation is facilitated by the cAMP receptor protein, CRP. In accordance with a stark growth defect, deletion of crp in both CO92 and KIM6+ Y. pestis strains significantly impaired biofilm production when solely utilizing alternate carbon sources. Media supplementation with cAMP, a small-molecule activator of CRP, did not significantly alter Y. pestis biofilm production. Furthermore, CRP did not alter mRNA abundance of previously-characterized hms biofilm synthesis and regulation factors. Therefore, our findings indicate CRP does not confer a direct stimulatory effect, but may indirectly promote Y. pestis biofilm production by facilitating the alternate carbon source expression profile. Additionally, we assessed the impact of the carbon storage regulator protein, CsrA, upon Y. pestis biofilm production. Contrary to what has been described for E. coli, Y. pestis biofilm formation was found to be enhanced by CsrA. Regardless of media composition and available carbon source, deletion of csrA significantly impaired Y. pestis biofilm production. CsrA was found to promote Y. pestis biofilm production independent of glycogen regulation. Loss of csrA did not significantly alter relative hmsH, hmsP, or hmsT mRNA abundance. However, deletion of hmsP in the csrA-deficient mutant enabled excessive biofilm production, suggesting CsrA enables potent Y. pestis biofilm production through cyclic diguanylate regulation. C1 [Willias, Stephan P.; Motin, Vladimir L.] Univ Texas Med Branch, Dept Pathol, Galveston, TX 77555 USA. [Chauhan, Sadhana; Motin, Vladimir L.] Univ Texas Med Branch, Dept Microbiol & Immunol, Galveston, TX 77555 USA. [Lo, Chien-Chi; Chain, Patrick S. G.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. RP Motin, VL (reprint author), Univ Texas Med Branch, Dept Pathol, Galveston, TX 77555 USA. EM vlmotin@utmb.edu RI Motin, Vladimir/O-1535-2013; OI Chain, Patrick/0000-0003-3949-3634 FU NIH/NIAID [Y01 AI008401, T32 AI007526]; UTMB McLaughlin pre-doctoral fellowship FX This work was supported by NIH/NIAID, Y01 AI008401; NIH/NIAID, T32 AI007526; and UTMB McLaughlin pre-doctoral fellowship to SPW, http://www.utmb.edu/mclaughlin/predoctoral.shtml. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 48 TC 4 Z9 4 U1 0 U2 5 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 25 PY 2015 VL 10 IS 8 AR e0135481 DI 10.1371/journal.pone.0135481 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6KK UT WOS:000359995500023 PM 26305456 ER PT J AU Shui, JL Chen, C Grabstanowicz, L Zhao, D Liu, DJ AF Shui, Jianglan Chen, Chen Grabstanowicz, Lauren Zhao, Dan Liu, Di-Jia TI Highly efficient nonprecious metal catalyst prepared with metal-organic framework in a continuous carbon nanofibrous network SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE nanofibrous; nonprecious metal catalyst; metal-organic framework; fuel cell; oxygen reduction ID OXYGEN REDUCTION REACTION; PEM FUEL-CELLS; ZEOLITIC IMIDAZOLATE FRAMEWORKS; HIGH ELECTROCATALYTIC ACTIVITY; CATHODE CATALYST; FE/N/C CATALYSTS; HEAT-TREATMENT; IRON; PRECURSOR; BLACKS AB Fuel cell vehicles, the only all-electric technology with a demonstrated >300 miles per fill travel range, use Pt as the electrode catalyst. The high price of Pt creates a major cost barrier for large-scale implementation of polymer electrolyte membrane fuel cells. Nonprecious metal catalysts (NPMCs) represent attractive low-cost alternatives. However, a significantly lower turnover frequency at the individual catalytic site renders the traditional carbon-supported NPMCs inadequate in reaching the desired performance afforded by Pt. Unconventional catalyst design aiming at maximizing the active site density at much improved mass and charge transports is essential for the next-generation NPMC. We report here a method of preparing highly efficient, nanofibrous NPMC for cathodic oxygen reduction reaction by electro-spinning a polymer solution containing ferrous organometallics and zeolitic imidazolate framework followed by thermal activation. The catalyst offers a carbon nanonetwork architecture made of microporous nanofibers decorated by uniformly distributed high-density active sites. In a single-cell test, the membrane electrode containing such a catalyst delivered unprecedented volumetric activities of 3.3 A.cm(-3) at 0.9 V or 450 A.cm(-3) extrapolated at 0.8 V, representing the highest reported value in the literature. Improved fuel cell durability was also observed. C1 [Shui, Jianglan; Chen, Chen; Grabstanowicz, Lauren; Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Shui, Jianglan] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Grabstanowicz, Lauren] Alcoa Tech Ctr, New Kensington, PA 15068 USA. [Zhao, Dan] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117576, Singapore. RP Liu, DJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM djliu@anl.gov RI Zhao, Dan/D-5975-2011 OI Zhao, Dan/0000-0002-4427-2150 FU US Department of Energy's Office of Science; Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office FX We thank Dr. Deborah J. Myers, Dr. Magali Ferrandon, Heather Barkholtz, and Zachary Kaiser for their assistance in fuel cell performance tests and material characterizations. This work was supported by the US Department of Energy's Office of Science and the Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office. NR 34 TC 49 Z9 49 U1 26 U2 105 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 25 PY 2015 VL 112 IS 34 BP 10629 EP 10634 DI 10.1073/pnas.1507159112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6NZ UT WOS:000360005600041 PM 26261338 ER PT J AU Hejazi, MI Voisin, N Liu, L Bramer, LM Fortin, DC Hathaway, JE Huang, M Kyle, P Leung, LR Li, HY Liu, Y Patel, PL Pulsipher, TC Rice, JS Tesfa, TK Vernon, CR Zhou, YY AF Hejazi, Mohamad I. Voisin, Nathalie Liu, Lu Bramer, Lisa M. Fortin, Daniel C. Hathaway, John E. Huang, Maoyi Kyle, Page Leung, L. Ruby Li, Hong-Yi Liu, Ying Patel, Pralit L. Pulsipher, Trenton C. Rice, Jennie S. Tesfa, Teklu K. Vernon, Chris R. Zhou, Yuyu TI 21st century United States emissions mitigation could increase water stress more than the climate change it is mitigating SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE climate change; mitigation; water deficit; Earth system model; integrated assessment ID EARTH SYSTEM MODELS; INTEGRATED ASSESSMENT; HIGH-RESOLUTION; LAND-SURFACE; RESOURCES; STABILIZATION; PATHWAYS; AVAILABILITY; MANAGEMENT; BIOENERGY AB There is evidence that warming leads to greater evapotranspiration and surface drying, thus contributing to increasing intensity and duration of drought and implying that mitigation would reduce water stresses. However, understanding the overall impact of climate change mitigation on water resources requires accounting for the second part of the equation, i.e., the impact of mitigation-induced changes in water demands from human activities. By using integrated, high-resolution models of human and natural system processes to understand potential synergies and/or constraints within the climate-energy-water nexus, we show that in the United States, over the course of the 21st century and under one set of consistent socioeconomics, the reductions in water stress from slower rates of climate change resulting from emission mitigation are overwhelmed by the increased water stress from the emissions mitigation itself. The finding that the human dimension outpaces the benefits from mitigating climate change is contradictory to the general perception that climate change mitigation improves water conditions. This research shows the potential for unintended and negative consequences of climate change mitigation. C1 [Hejazi, Mohamad I.; Liu, Lu; Kyle, Page; Patel, Pralit L.; Zhou, Yuyu] Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Voisin, Nathalie; Bramer, Lisa M.; Fortin, Daniel C.; Hathaway, John E.; Huang, Maoyi; Leung, L. Ruby; Li, Hong-Yi; Liu, Ying; Pulsipher, Trenton C.; Rice, Jennie S.; Tesfa, Teklu K.; Vernon, Chris R.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hejazi, MI (reprint author), Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM mohamad.hejazi@pnnl.gov RI Li, Hong-Yi/C-9143-2014; Bramer, Lisa/L-9184-2016; Huang, Maoyi/I-8599-2012; OI Li, Hong-Yi/0000-0001-5690-3610; Bramer, Lisa/0000-0002-8384-1926; Huang, Maoyi/0000-0001-9154-9485; Voisin, Nathalie/0000-0002-6848-449X FU US Department of Energy [DE-AC05-76RL01830]; US Department of Energy, Office of Science, Biological and Environmental Research as part of the Integrated Assessment Research and Earth System Modeling programs FX This research is part of the Platform for Regional Integrated Modeling and Analysis (PRIMA) Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the US Department of Energy under Contract DE-AC05-76RL01830. This research also leveraged capabilities that were funded by the US Department of Energy, Office of Science, Biological and Environmental Research as part of the Integrated Assessment Research and Earth System Modeling programs. NR 41 TC 10 Z9 10 U1 9 U2 31 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 25 PY 2015 VL 112 IS 34 BP 10635 EP 10640 DI 10.1073/pnas.1421675112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6NZ UT WOS:000360005600042 PM 26240363 ER PT J AU Weber, CA Suzuki, R Schaller, V Aranson, IS Bausch, AR Frey, E AF Weber, Christoph A. Suzuki, Ryo Schaller, Volker Aranson, Igor S. Bausch, Andreas R. Frey, Erwin TI Random bursts determine dynamics of active filaments SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE active filaments; nonthermal statistics; molecular motors; gliding assay; kinetic model ID MYOSIN STEP-SIZE; SEMIFLEXIBLE POLYMERS; XENOPUS MELANOPHORES; ASSAY; MOVEMENT; INVITRO; MOTION; HYDRODYNAMICS; FLUCTUATIONS; MICROTUBULES AB Constituents of living or synthetic active matter have access to a local energy supply that serves to keep the system out of thermal equilibrium. The statistical properties of such fluctuating active systems differ from those of their equilibrium counterparts. Using the actin filament gliding assay as a model, we studied how nonthermal distributions emerge in active matter. We found that the basic mechanism involves the interplay between local and random injection of energy, acting as an analog of a thermal heat bath, and nonequilibrium energy dissipation processes associated with sudden jump-like changes in the system's dynamic variables. We show here how such a mechanism leads to a nonthermal distribution of filament curvatures with a non-Gaussian shape. The experimental curvature statistics and filament relaxation dynamics are reproduced quantitatively by stochastic computer simulations and a simple kinetic model. C1 [Weber, Christoph A.; Frey, Erwin] Univ Munich, Arnold Sommerfeld Ctr Theoret Phys, D-80333 Munich, Germany. [Weber, Christoph A.; Frey, Erwin] Univ Munich, Dept Phys, Ctr NanoSci, D-80333 Munich, Germany. [Weber, Christoph A.] Max Planck Inst Phys Komplexer Syst, Dept Biol Phys, D-01187 Dresden, Germany. [Suzuki, Ryo; Schaller, Volker; Bausch, Andreas R.] Tech Univ Munich, Lehrstuhl Biophys E27, D-85748 Garching, Germany. [Aranson, Igor S.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Bausch, AR (reprint author), Tech Univ Munich, Lehrstuhl Biophys E27, D-85748 Garching, Germany. EM abausch@mytum.de; frey@lmu.de FU Deutsche Forschungsgemeinschaft [SFB 863]; German Excellence Initiative via the program "NanoSystems Initiative Munich"; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering FX We thank Frank Julicher for fruitful and stimulating discussions. This project was supported by the Deutsche Forschungsgemeinschaft in the framework of the SFB 863 "Forces in Biomolecular Systems" (Projects B1 and B2) and the German Excellence Initiative via the program "NanoSystems Initiative Munich". The work of I. S. A. was also supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering. NR 53 TC 5 Z9 5 U1 7 U2 27 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 25 PY 2015 VL 112 IS 34 BP 10703 EP 10707 DI 10.1073/pnas.1421322112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6NZ UT WOS:000360005600054 PM 26261319 ER PT J AU Balachandran, PV Theiler, J Rondinelli, JM Lookman, T AF Balachandran, Prasanna V. Theiler, James Rondinelli, James M. Lookman, Turab TI Materials Prediction via Classification Learning SO SCIENTIFIC REPORTS LA English DT Article ID ORBITAL-RADII; STRUCTURAL STABILITY; CRYSTAL-CHEMISTRY; BINARY COMPOUNDS; SUPPORT; SOLIDS; PSEUDOPOTENTIALS; SEMICONDUCTORS; ENERGIES; DIAGRAMS AB In the paradigm of materials informatics for accelerated materials discovery, the choice of feature set (i.e. attributes that capture aspects of structure, chemistry and/or bonding) is critical. Ideally, the feature sets should provide a simple physical basis for extracting major structural and chemical trends and furthermore, enable rapid predictions of new material chemistries. Orbital radii calculated from model pseudopotential fits to spectroscopic data are potential candidates to satisfy these conditions. Although these radii (and their linear combinations) have been utilized in the past, their functional forms are largely justified with heuristic arguments. Here we show that machine learning methods naturally uncover the functional forms that mimic most frequently used features in the literature, thereby providing a mathematical basis for feature set construction without a priori assumptions. We apply these principles to study two broad materials classes: (i) wide band gap AB compounds and (ii) rare earth-main group RM intermetallics. The AB compounds serve as a prototypical example to demonstrate our approach, whereas the RM intermetallics show how these concepts can be used to rapidly design new ductile materials. Our predictive models indicate that ScCo, ScIr, and YCd should be ductile, whereas each was previously proposed to be brittle. C1 [Balachandran, Prasanna V.; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Theiler, James] Los Alamos Natl Lab, Intelligence & Space Res, Los Alamos, NM 87545 USA. [Rondinelli, James M.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. RP Lookman, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM txl@lanl.gov RI Rondinelli, James/A-2071-2009 OI Rondinelli, James/0000-0003-0508-2175 FU Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR on Materials Informatics [20140013DR]; NSF-DMR [1454688] FX P.V.B., T.L. and J.T. acknowledge funding support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR (#20140013DR) on Materials Informatics. J.M.R. acknowledges support from NSF-DMR 1454688. P.V.B. thanks J. Hogden for comments on the paper. P.V.B. thanks M. Sanati for bringing the RM intermetallics problem to our attention and M. Topsakal for assistance with the Dy-pseudopotentials. P.V.B. also thanks J. Gubernatis and G. Pilania for insightful discussions. DFT calculations were performed using the Institutional Computing (IC) resources at LANL. NR 60 TC 12 Z9 12 U1 11 U2 49 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 25 PY 2015 VL 5 AR 13285 DI 10.1038/srep13285 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6UH UT WOS:000360023200001 PM 26304800 ER PT J AU Tan, XD Rajguru, S Young, H Xia, N Stock, SR Xiao, XH Richter, CP AF Tan, Xiaodong Rajguru, Suhrud Young, Hunter Xia, Nan Stock, Stuart R. Xiao, Xianghui Richter, Claus-Peter TI Radiant energy required for infrared neural stimulation SO SCIENTIFIC REPORTS LA English DT Article ID LASER STIMULATION; OPTICAL STIMULATION; NERVE-STIMULATION; PERIPHERAL-NERVE; CAVERNOUS NERVES; IN-VIVO; NEURONS; ACTIVATION; MECHANISMS; THRESHOLD AB Infrared neural stimulation (INS) has been proposed as an alternative method to electrical stimulation because of its spatial selective stimulation. Independent of the mechanism for INS, to translate the method into a device it is important to determine the energy for stimulation required at the target structure. Custom-designed, flat and angle polished fibers, were used to deliver the photons. By rotating the angle polished fibers, the orientation of the radiation beam in the cochlea could be changed. INS-evoked compound action potentials and single unit responses in the central nucleus of the inferior colliculus (ICC) were recorded. X-ray computed tomography was used to determine the orientation of the optical fiber. Maximum responses were observed when the radiation beam was directed towards the spiral ganglion neurons (SGNs), whereas little responses were seen when the beam was directed towards the basilar membrane. The radiant exposure required at the SGNs to evoke compound action potentials (CAPs) or ICC responses was on average 18.9 +/- 12.2 or 10.3 +/- 4.9 mJ/cm(2), respectively. For cochlear INS it has been debated whether the radiation directly stimulates the SGNs or evokes a photoacoustic effect. The results support the view that a direct interaction between neurons and radiation dominates the response to INS. C1 [Tan, Xiaodong; Young, Hunter; Xia, Nan; Richter, Claus-Peter] Northwestern Univ, Dept Otolaryngol, Chicago, IL 60611 USA. [Rajguru, Suhrud] Univ Miami, Dept Biomed Engn, Miami, FL 33146 USA. [Rajguru, Suhrud] Univ Miami, Dept Otolaryngol, Miami, FL 33136 USA. [Xia, Nan] Chongqing Univ, Bioengn Coll, Key Lab Biorheol Sci & Technol, Chongqing 400044, Peoples R China. [Stock, Stuart R.] Northwestern Univ Feinberg Sch Med, Dept Cell & Mol Biol, Chicago, IL 60611 USA. [Xiao, Xianghui] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Richter, Claus-Peter] Northwestern Univ, Dept Biomed Engn, Evanston, IL 60208 USA. [Richter, Claus-Peter] Northwestern Univ, Dept Commun Sci & Disorders, Hugh Knowles Ctr, Evanston, IL 60208 USA. RP Richter, CP (reprint author), Northwestern Univ, Dept Otolaryngol, 303 E Chicago Ave,Searle 12-561, Chicago, IL 60611 USA. EM cri529@northwestern.edu FU National Institute on Deafness and Other Communication Disorders, National Institutes of Health [R01 DC011855]; Lockheed Martin Aculight FX This project has been funded with federal funds from the National Institute on Deafness and Other Communication Disorders, National Institutes of Health, grant R01 DC011855, and by Lockheed Martin Aculight. NR 46 TC 6 Z9 7 U1 8 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 25 PY 2015 VL 5 AR 13273 DI 10.1038/srep13273 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP6TZ UT WOS:000360022400001 PM 26305106 ER PT J AU Dennis, BS Czaplewski, DA Haftel, MI Lopez, D Blumberg, G Aksyuk, V AF Dennis, Brian S. Czaplewski, David A. Haftel, Michael I. Lopez, Daniel Blumberg, Girsh Aksyuk, Vladimir TI Diffraction limited focusing and routing of gap plasmons by a metal-dielectric-metal lens SO OPTICS EXPRESS LA English DT Article ID SURFACE-PLASMONS; WAVE-GUIDES; PHASE MODULATORS; POLARITONS; OPTICS AB Passive optical elements can play key roles in photonic applications such as plasmonic integrated circuits. Here we experimentally demonstrate passive gap-plasmon focusing and routing in two-dimensions. This is accomplished using a high numerical-aperture metal-dielectric-metal lens incorporated into a planar-waveguide device. Fabrication via metal sputtering, oxide deposition, electron-and focused-ion-beam lithography, and argon ion-milling is reported on in detail. Diffraction-limited focusing is optically characterized by sampling out-coupled light with a microscope. The measured focal distance and full-width-half-maximum spot size agree well with the calculated lens performance. The surface plasmon polariton propagation length is measured by sampling light from multiple out-coupler slits. (C) 2015 Optical Society of America C1 [Dennis, Brian S.; Blumberg, Girsh] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Czaplewski, David A.; Lopez, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Haftel, Michael I.] Univ Colorado, Dept Phys, Colorado Springs, CO 80918 USA. [Aksyuk, Vladimir] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. RP Aksyuk, V (reprint author), NIST, Ctr Nanoscale Sci & Technol, 100 Bur Dr, Gaithersburg, MD 20899 USA. EM vladimir.aksyuk@nist.gov FU Measurement Science and Engineering Research Grant Program of the National Institute of Standards and Technology [70NANB14H259, 70NANB14H030]; National Science Foundation [DMR-1104884]; Air Force Office of Scientific Research [FA9550-09-1-0698]; Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX This work has been supported by the Measurement Science and Engineering Research Grant Program of the National Institute of Standards and Technology (award nos. 70NANB14H259 and 70NANB14H030), the National Science Foundation DMR-1104884, and the Air Force Office of Scientific Research (grant no. FA9550-09-1-0698). Computational support from the Department of Defense High Performance Computation Modernization project is acknowledged. This work was performed, in part, at the Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility (contract no. DE-AC02-06CH11357). NR 36 TC 1 Z9 1 U1 7 U2 35 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD AUG 24 PY 2015 VL 23 IS 17 BP 21899 EP 21908 DI 10.1364/OE.23.021899 PG 10 WC Optics SC Optics GA CS9NR UT WOS:000362418300032 PM 26368166 ER PT J AU Farfurnik, D Jarmola, A Pham, LM Wang, ZH Dobrovitski, VV Walsworth, RL Budker, D Bar-Gill, N AF Farfurnik, D. Jarmola, A. Pham, L. M. Wang, Z. H. Dobrovitski, V. V. Walsworth, R. L. Budker, D. Bar-Gill, N. TI Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond SO PHYSICAL REVIEW B LA English DT Article ID COHERENCE TIME; RESOLUTION; SEQUENCES; CENTERS; BATH; NMR AB We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T-1 effects and DD microwave pulses are used to increase the transverse coherence time T-2 from similar to 0.7 ms up to similar to 30 ms. We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states. C1 [Farfurnik, D.; Bar-Gill, N.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-9190401 Jerusalem, Israel. [Farfurnik, D.; Bar-Gill, N.] Hebrew Univ Jerusalem, Ctr Nanosci & Nanotechnol, IL-9190401 Jerusalem, Israel. [Jarmola, A.; Budker, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Pham, L. M.; Walsworth, R. L.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Wang, Z. H.] Univ So Calif, Dept Chem, Los Angeles, CA 90089 USA. [Dobrovitski, V. V.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Walsworth, R. L.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Budker, D.] Johannes Gutenberg Univ Mainz, Helmholtz Inst, D-55099 Mainz, Germany. [Bar-Gill, N.] Hebrew Univ Jerusalem, Dept Appl Phys, Rachel & Selim Sch Engn, IL-9190401 Jerusalem, Israel. RP Farfurnik, D (reprint author), Hebrew Univ Jerusalem, Racah Inst Phys, IL-9190401 Jerusalem, Israel. RI Budker, Dmitry/F-7580-2016 OI Budker, Dmitry/0000-0002-7356-4814 FU EU CIG; Minerva ARCHES award; Israel Science Foundation [750/14]; Ministry of Science and Technology, Israel; German-Israeli Project Cooperation (DIP) program; NSF [ECCS-1202258]; AFOSR/DARPA QuASAR program; U.S. Department of Energy-Basic Energy Sciences [DE-AC02-07CH11358]; CAMBR fellowship for Nanoscience and Nanotechnology; Binational Science Foundation Rahamimoff travel grant FX We thank Gonzalo A. Alvarez for fruitful discussions. This work has been supported in part by the EU CIG, the Minerva ARCHES award, the Israel Science Foundation (Grant No. 750/14), and the Ministry of Science and Technology, Israel. Additional support was provided by the German-Israeli Project Cooperation (DIP) program, the NSF through Grant No. ECCS-1202258, and the AFOSR/DARPA QuASAR program. Work at Ames Laboratory was supported by the U.S. Department of Energy-Basic Energy Sciences under Contract No. DE-AC02-07CH11358. D.F. was partially supported by the CAMBR fellowship for Nanoscience and Nanotechnology, and the Binational Science Foundation Rahamimoff travel grant. NR 39 TC 12 Z9 12 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 24 PY 2015 VL 92 IS 6 AR 060301 DI 10.1103/PhysRevB.92.060301 PG 5 WC Physics, Condensed Matter SC Physics GA CS6SO UT WOS:000362212200002 ER PT J AU MacLaughlin, DE Bernal, OO Shu, L Ishikawa, J Matsumoto, Y Wen, JJ Mourigal, M Stock, C Ehlers, G Broholm, CL Machida, Y Kimura, K Nakatsuji, S Shimura, Y Sakakibara, T AF MacLaughlin, D. E. Bernal, O. O. Shu, Lei Ishikawa, Jun Matsumoto, Yosuke Wen, J. -J. Mourigal, M. Stock, C. Ehlers, G. Broholm, C. L. Machida, Yo Kimura, Kenta Nakatsuji, Satoru Shimura, Yasuyuki Sakakibara, Toshiro TI Unstable spin-ice order in the stuffed metallic pyrochlore Pr2+xIr2-xO7-delta SO PHYSICAL REVIEW B LA English DT Article ID MU-SR; FIELD; LIQUID; FLUCTUATIONS; TEMPERATURE; RELAXATION; MAGNETISM; PR2IR2O7; SYSTEMS; MODEL AB Specific heat, elastic neutron scattering, and muon spin rotation (mu SR) experiments have been carried out on a well-characterized sample of "stuffed" (Pr-rich) Pr2+xIr2-xO7-delta. Elastic neutron scattering shows the onset of long-range spin-ice "2-in/2-out" magnetic order at T-M = 0.93 K, with an ordered moment of 1.7(1)mu(B)/Pr ion at low temperatures. Approximate lower bounds on the correlation length and correlation time in the ordered state are 170 angstrom and 0.7 ns, respectively. mu SR experiments yield an upper bound 2.6(7) mT on the local field B-loc(4f) at the muon site, which is nearly two orders of magnitude smaller than the expected dipolar field for long-range spin-ice ordering of 1.7 mu(B) moments (120-270 mT, depending on muon site). This shortfall is due in part to splitting of the non-Kramers crystal-field ground-state doublets of near-neighbor Pr3+ ions by the mu(+)-induced lattice distortion. For this to be the only effect, however, similar to 160 Pr moments out to a distance of similar to 14 angstrom must be suppressed. An alternative scenario, which is consistent with the observed reduced nuclear hyperfine Schottky anomaly in the specific heat, invokes slow correlated Pr-moment fluctuations in the ordered state that average B-loc(4f) on the mu SR time scale (similar to 10(-7) s), but are static on the time scale of the elastic neutron scattering experiments (similar to 10(-9) s). In this picture, the dynamic muon relaxation suggests a Pr3+ 4f correlation time of a few nanoseconds, which should be observable in a neutron spin echo experiment. C1 [MacLaughlin, D. E.; Shu, Lei] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. [MacLaughlin, D. E.; Ishikawa, Jun; Matsumoto, Yosuke; Machida, Yo; Kimura, Kenta; Nakatsuji, Satoru; Shimura, Yasuyuki; Sakakibara, Toshiro] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Bernal, O. O.] Calif State Univ Los Angeles, Dept Phys & Astron, Los Angeles, CA 90032 USA. [Shu, Lei] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Shu, Lei] Fudan Univ, Collaborat Innovat Ctr Adv Microstruct, Shanghai 200433, Peoples R China. [Wen, J. -J.; Mourigal, M.; Stock, C.; Broholm, C. L.] Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. [Wen, J. -J.; Mourigal, M.; Stock, C.; Broholm, C. L.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Stock, C.; Broholm, C. L.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Ehlers, G.; Broholm, C. L.] Oak Ridge Natl Lab, Neutron Sci Directorate, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Broholm, C. L.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. [Nakatsuji, Satoru] Japan Sci & Technol Agcy JST, PRESTO, Kawaguchi, Saitama 3320012, Japan. RP MacLaughlin, DE (reprint author), Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. EM macl@physics.ucr.edu; satoru@issp.u-tokyo.ac.jp RI Ehlers, Georg/B-5412-2008; Instrument, CNCS/B-4599-2012; Mourigal, Martin/F-4495-2010; Kimura, Kenta/F-4267-2017 OI Ehlers, Georg/0000-0003-3513-508X; Mourigal, Martin/0000-0003-2772-8440; FU U.S. NSF (Riverside) [0422671, 0801407]; U.S. NSF (Los Angeles) [1105380]; Japanese Society for the Promotion of Science (JSPS) [21684019]; Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan [17071003, 19052003]; National Natural Science Foundation of China [11474060]; STCSM of China [15XD1500200]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX C.L.B. and S.N. thank the Aspen Center for Physics, where progress was made on this project, for their hospitality during the summer of 2014. D.E.M. wishes to thank the Institute for Solid State Physics, Tokyo University, for their hospitality during his stays there. We are grateful for technical assistance from the TRIUMF Centre for Molecular and Materials Science, where the mu SR experiments were carried out. We thank E. J. Ansaldo, J. M. Mackie, K. Onuma, and S. Zhao for assistance with the experiments, and R. F. Kiefl and G. M. Luke for useful discussions. We are grateful to S. Koohpayeh for performing powder x-ray diffraction at IQM. This work was partially supported by U.S. NSF Grant Nos. 0422671, 0801407 (Riverside), and 1105380 (Los Angeles), by a Grant-in-Aid (No. 21684019) from the Japanese Society for the Promotion of Science (JSPS), by Grants-in-Aid for Scientific Research on Priority Areas (Nos. 17071003 and 19052003) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan, by the National Natural Science Foundation of China (No. 11474060), and STCSM of China (No. 15XD1500200). The work at IQM was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering under grant DE-FG02-08ER46544. The research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 53 TC 4 Z9 4 U1 8 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 24 PY 2015 VL 92 IS 5 AR 054432 DI 10.1103/PhysRevB.92.054432 PG 12 WC Physics, Condensed Matter SC Physics GA CS6RZ UT WOS:000362210600006 ER PT J AU Mkhitaryan, VV Dobrovitski, VV AF Mkhitaryan, V. V. Dobrovitski, V. V. TI Hyperfine-induced spin relaxation of a diffusively moving carrier in low dimensions: Implications for spin transport in organic semiconductors SO PHYSICAL REVIEW B LA English DT Article ID MONTE-CARLO-SIMULATION; CHARGE-TRANSPORT; ROOM-TEMPERATURE; RANDOM-WALKS; INJECTION; MAGNETORESISTANCE; DEPOLARIZATION; LATTICES; SOLIDS; VALVE AB The hyperfine coupling between the spin of a charge carrier and the nuclear spin bath is a predominant channel for the carrier spin relaxation in many organic semiconductors. We theoretically investigate the hyperfine-induced spin relaxation of a carrier performing a random walk on a d-dimensional regular lattice, in a transport regime typical for organic semiconductors. We show that in d = 1 and 2, the time dependence of the space-integrated spin polarization P(t) is dominated by a superexponential decay, crossing over to a stretched-exponential tail at long times. The faster decay is attributed to multiple self-intersections (returns) of the random-walk trajectories, which occur more often in lower dimensions. We also show, analytically and numerically, that the returns lead to sensitivity of P(t) to external electric and magnetic fields, and this sensitivity strongly depends on dimensionality of the system (d = 1 versus d = 3). Furthermore, we investigate in detail the coordinate dependence of the time-integrated spin polarization sigma(r), which can be probed in the spin-transport experiments with spin-polarized electrodes. We demonstrate that, while sigma(r) is essentially exponential, the effect of multiple self-intersections can be identified in transport measurements from the strong dependence of the spin-decay length on the external magnetic and electric fields. C1 [Mkhitaryan, V. V.; Dobrovitski, V. V.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Mkhitaryan, VV (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. FU US Department of Energy, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We thank J. Shinar and M. E. Raikh for many useful discussions. Work at the Ames Laboratory was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering. The Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 48 TC 3 Z9 3 U1 3 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 24 PY 2015 VL 92 IS 5 AR 054204 DI 10.1103/PhysRevB.92.054204 PG 14 WC Physics, Condensed Matter SC Physics GA CS6RZ UT WOS:000362210600002 ER PT J AU Highland, MJ Fong, DD Ju, GX Thompson, C Baldo, PM Fuoss, PH Eastman, JA AF Highland, Matthew J. Fong, Dillon D. Ju, Guangxu Thompson, Carol Baldo, Peter M. Fuoss, Paul H. Eastman, Jeffrey A. TI In-situ x-ray studies of compositional control during synthesis of LaGaO3 by radio frequency-magnetron sputtering SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; LA2O3-GA2O3 SYSTEM AB In-situ synchrotron x-ray scattering has been used to monitor and control the synthesis of LaGaO3 epitaxial thin films by 90 degrees off-axis RF-magnetron sputtering. Films deposited from a single LaGaO3 source were compared with those prepared by alternating deposition from separate La2O3 and Ga2O3 sources. The conditions for growth of stoichiometric films were determined by real-time monitoring of secondary phase formation as well as from features in the diffuse scatter from island formation during synthesis. These results provide atomic-scale insight into the mechanisms taking place during reactive epitaxial growth and demonstrate how in-situ techniques can be utilized to achieve stoichiometric control in ultrathin films. (C) 2015 AIP Publishing LLC. C1 [Highland, Matthew J.; Fong, Dillon D.; Ju, Guangxu; Baldo, Peter M.; Fuoss, Paul H.; Eastman, Jeffrey A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Thompson, Carol] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Highland, MJ (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mhighland@anl.gov FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering; DOE-BES [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering. Use of the Advanced Photon Source was supported by DOE-BES, under Contract No. DE-AC02-06CH11357. We thank Brad Stumphy and Tim Spila for conducting and analyzing the RBS measurements, which were carried out in the Frederick Seitz Materials Research Laboratory at the University of Illinois at Urbana-Champaign. NR 19 TC 1 Z9 1 U1 2 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 24 PY 2015 VL 107 IS 8 AR 081606 DI 10.1063/1.4929753 PG 5 WC Physics, Applied SC Physics GA CQ4SC UT WOS:000360593900019 ER PT J AU Jalarvo, N Pramanick, A Do, C Diallo, SO AF Jalarvo, N. Pramanick, A. Do, C. Diallo, S. O. TI Effects of configurational changes on molecular dynamics in polyvinylidene fluoride and poly(vinylidene fluoride-trifluoroethylene) ferroelectric polymers SO APPLIED PHYSICS LETTERS LA English DT Article ID INCOHERENT NEUTRON-SCATTERING; VINYLIDENE FLUORIDE; COPOLYMER FILMS; PHASE-TRANSITION; TRIFLUOROETHYLENE; DIFFUSION; BEHAVIOR; PIEZOELECTRICITY; SPECTRA; DENSITY AB We present a comparative study of proton dynamics in unpoled non-ferroelectric polymer polyvinylidene fluoride (PVDF) and in its trifluoroethylene containing ferroelectric copolymer (with 70/30 molar proportion), using quasi-elastic neutron scattering. The neutron data reveal the existence of two distinct types of molecular motions in the temperature range investigated. The slower motion, which is characterized in details here, is ascribed to protons jump diffusion along the polymeric carbon chains, while the faster motion could be attributed to localized rotational motion of methylene groups. At temperatures below the Curie point (T-c similar to 385 K) of the composite polymer, the slower diffusive mode experiences longer relaxation times in the ferroelectric blend than in the bare PVDF, although the net corresponding diffusion coefficient remains comparatively the same in both polymers with characteristic activation energy of E-A approximate to 27-33 kJ/mol. This arises because of a temperature dependent jump length r(0), which we observe to be effectively longer in the copolymer, possibly due to the formation of ordered ferroelectric domains below Tc. Above Tc, there is no appreciable difference in r(0) between the two systems. This observation directly relates the known dependence of Tc on molar ratio to changes in r(0), providing fundamental insight into the ferroelectric properties of PVDF-based copolymers. (C) 2015 AIP Publishing LLC. C1 [Jalarvo, N.] Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52428 Julich, Germany. [Jalarvo, N.; Diallo, S. O.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Pramanick, A.] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. [Do, C.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Jalarvo, N (reprint author), Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52428 Julich, Germany. EM jalarvonh@ornl.gov; abhijit.pramanick@gmail.com; omardiallos@ornl.gov RI Diallo, Souleymane/B-3111-2016; Jalarvo, Niina/Q-1320-2015; Pramanick, Abhijit/D-9578-2011; Do, Changwoo/A-9670-2011 OI Diallo, Souleymane/0000-0002-3369-8391; Jalarvo, Niina/0000-0003-0644-6866; Pramanick, Abhijit/0000-0003-0687-4967; Do, Changwoo/0000-0001-8358-8417 FU City University of Hong Kong; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors would like to thank R. Goyette and R. Mills for their excellent technical support during the neutron measurements. AP acknowledges funding support from City University of Hong Kong. Work at ORNL's Spallation Neutron Source is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 36 TC 0 Z9 0 U1 6 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 24 PY 2015 VL 107 IS 8 AR 082907 DI 10.1063/1.4929693 PG 5 WC Physics, Applied SC Physics GA CQ4SC UT WOS:000360593900057 ER PT J AU Macrander, AT Kubec, A Conley, R Bouet, N Zhou, J Wojcik, M Maser, J AF Macrander, Albert T. Kubec, Adam Conley, Raymond Bouet, Nathalie Zhou, Juan Wojcik, Michael Maser, Jorg TI Efficiency of a multilayer-Laue-lens with a 102 mu m aperture SO APPLIED PHYSICS LETTERS LA English DT Article ID X-RAY OPTICS; PERFORMANCE AB A multilayer-Laue-lens (MLL) comprised of WSi2/Al layers stacked to a full thickness of 102 mu m was characterized for its diffraction efficiency and dynamical diffraction properties by x-ray measurements made in the far field. The achieved aperture roughly doubles the previous maximum reported aperture for an MLL, thereby doubling the working distance. Negative and positive first orders were found to have 14.2% and 13.0% efficiencies, respectively. A section thickness of 9.6 mu m was determined from Laue-case thickness fringes in the diffraction data. A background gas consisting of 90% Ar and 10% N-2 was used for sputtering. This material system was chosen to reduce grown-in stress as the multilayer is deposited. Although some regions of the full MLL exhibited defects, the presently reported results were obtained for a region devoid of defects. The data compare well to dynamical diffraction calculations with Coupled Wave Theory (CWT) which provided confirmation of the optical constants and densities assumed for the CWT calculations. (C) 2015 AIP Publishing LLC. C1 [Macrander, Albert T.; Kubec, Adam; Conley, Raymond; Wojcik, Michael; Maser, Jorg] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Kubec, Adam] Fraunhofer IWS Dresden, D-01277 Dresden, Germany. [Conley, Raymond; Bouet, Nathalie; Zhou, Juan] Brookhaven Natl Lab, NSLS 2, Upton, NY 11973 USA. RP Macrander, AT (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM atm@anl.gov OI Bouet, Nathalie/0000-0002-5816-9429 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC-02-06CH11357]; U.S. Department of Energy, Office Basic Energy Sciences [DE-SC00112704]; European Union (ERDF); Free State of Saxony via the ESF Project [100087859] FX We acknowledge Dr. N. Kujala for assistance in the early phases of this work, and we thank H. Yan for commenting on the manuscript. We are grateful to the X-ray Science Division of the Advanced Photon Source for support. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC-02-06CH11357. Work carried out at National Synchrotron Light Source II and the Center for Functional Nanomaterials at Brookhaven was supported by the U.S. Department of Energy, Office Basic Energy Sciences under Contract No. DE-SC00112704. Work at Fraunhofer IWS was partly funded by the European Union (ERDF) and the Free State of Saxony via the ESF Project No. 100087859 (ENano). NR 24 TC 4 Z9 4 U1 1 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 24 PY 2015 VL 107 IS 8 AR 081904 DI 10.1063/1.4929505 PG 3 WC Physics, Applied SC Physics GA CQ4SC UT WOS:000360593900025 ER PT J AU Warren, EL Kibbler, AE France, RM Norman, AG Stradins, P McMahon, WE AF Warren, Emily L. Kibbler, Alan E. France, Ryan M. Norman, Andrew G. Stradins, Paul McMahon, William E. TI Growth of antiphase-domain-free GaP on Si substrates by metalorganic chemical vapor deposition using an in situ AsH3 surface preparation SO APPLIED PHYSICS LETTERS LA English DT Article ID SI(100) SURFACES; SPECTROSCOPY; GAAS; RDS AB Antiphase-domain (APD) free GaP films were grown on Si(100) substrates prepared by annealing under dilute AsH3 in situ in an MOCVD reactor. LEED and AES surface analysis of Si(100) surfaces prepared by this treatment show that AsH3 etching quickly removes O and C contaminants at a relatively low temperature (690-740 degrees C), and creates a single-domain "A-type" As/Si surface reconstruction. The resulting GaP epilayers grown at the same temperature are APD-free, and could thereby serve as templates for direct growth of III-V semiconductors on Si. This single chamber process has a low thermal budget, and can enable heteroepitaxial integration of III-Vs and Si at an industrial scale. (C) 2015 AIP Publishing LLC. C1 [Warren, Emily L.; Kibbler, Alan E.; France, Ryan M.; Norman, Andrew G.; Stradins, Paul; McMahon, William E.] Natl Ctr Photovolta, Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Warren, EL (reprint author), Natl Ctr Photovolta, Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM emily.warren@nrel.gov RI Norman, Andrew/F-1859-2010; OI Norman, Andrew/0000-0001-6368-521X; Warren, Emily/0000-0001-8568-7881 FU DOE EERE SETP [DE- EE00025783] FX This work was supported by DOE EERE SETP under DE- EE00025783. We thank Sanjini Nanayakkara, Bobby To, and Adele Tamboli for sample characterization and helpful discussions. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 22 TC 2 Z9 2 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 24 PY 2015 VL 107 IS 8 AR 082109 DI 10.1063/1.4929714 PG 4 WC Physics, Applied SC Physics GA CQ4SC UT WOS:000360593900037 ER PT J AU Bailey, WD Luconi, L Rossin, A Yakhvarov, D Flowers, SE Kaminsky, W Kemp, RA Giambastiani, G Goldberg, KI AF Bailey, Wilson D. Luconi, Lapo Rossin, Andrea Yakhvarov, Dmitry Flowers, Sarah E. Kaminsky, Werner Kemp, Richard A. Giambastiani, Giuliano Goldberg, Karen I. TI Pyrazole-Based PCN Pincer Complexes of Palladium(II): Mono- and Dinuclear Hydroxide Complexes and Ligand Rollover C-H Activation SO ORGANOMETALLICS LA English DT Article ID INTRAMOLECULAR HYDROAMINATION REACTIONS; UNEXPECTED REACTIVITY PATHS; CRYSTAL-STRUCTURE; TRANSITION-ELEMENTS; BOND ACTIVATION; CYCLOMETALATED COMPOUNDS; REDUCTIVE ELIMINATION; STRUCTURAL-ANALYSIS; CATALYTIC-ACTIVITY; PLATINUM AB Palladium complexes of the novel unsymmetrical phosphine pyrazole-containing pincer ligands PCNH (PCNH = 1-[3- [(di-tert-butylphosphino)methyl]pheny1]-1H-pyrazole) and PCNMe (PCNMe = 1-[3-(di-tert-butylphosphino)methyl]pheny1]-5-methyl-1H-pyrazole) have been prepared and characterized through single-crystal X-ray diffraction and multinudear H-1, C-13{H-1}, and P-31{H-1} NMR spectroscopy. In preparations of the monomeric hydroxide species (PCNH)Pd(OH), an unexpected N detachment followed by C-H activation on the heterocycle 5-position took place resulting in conversion of the monoanionic {P,C-,N} framework into a dianionic {P,C-,C-} ligand set. The dinuclear hydroxide-bridged species (PCNH)Pd(mu-OH)Pd(PCC) was the final product obtained under ambient conditions. The "rollover" activation was followed via P-31{H-1} NMR spectroscopy, and dinuclear cationic mu-OH and monomeric Pd-II hydroxide intermediates were identified. DFT computational analysis of the process (M06//6-31G*, THF) showed that the energy barriers for the pyrazolyl rollover and for C-H activation through a sigma-bond metathesis reaction are low enough to be overcome under ambient-temperature conditions, in line with the experimental findings. In contrast to the PCNH system, no "rollover" reactivity was observed in the PCNMe system, and the terminal hydroxide complex (PCNMe)Pd(OH) could be readily isolated and fully characterized. C1 [Bailey, Wilson D.; Flowers, Sarah E.; Kaminsky, Werner; Goldberg, Karen I.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Luconi, Lapo; Rossin, Andrea; Giambastiani, Giuliano] CNR, Inst Chem Organomet Cpds ICCOM, I-50019 Sesto Fno Florence, Italy. [Luconi, Lapo; Rossin, Andrea; Giambastiani, Giuliano] CNR, Consorzio INSTM, I-50019 Sesto Fno Florence, Italy. [Yakhvarov, Dmitry; Giambastiani, Giuliano] Kazan Fed Univ, Kazan 420008, Russia. [Kemp, Richard A.] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. [Kemp, Richard A.] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. RP Kemp, RA (reprint author), Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. EM rakemp@unm.edu; giuliano.giambastiani@iccom.cnr.it; goldberg@chem.washington.edu RI Rossin, Andrea/P-6379-2015; Giambastiani, Giuliano/E-3255-2016 OI Rossin, Andrea/0000-0002-1283-2803; Giambastiani, Giuliano/0000-0002-0315-3286 FU Fondazione Cariplo ("Crystalline Elastomers"); Groupe de Recherche International (GDRI) "Homogeneous Catalysis for Sustainable Development"; COST action: "EUFEN: European F-Element Network" [CM1006]; [DE-FG02-06ER15765] FX L.L., A.R., and G.G. thank the Fondazione Cariplo ("Crystalline Elastomers" project), the Groupe de Recherche International (GDRI) "Homogeneous Catalysis for Sustainable Development", and the COST action CM1006: "EUFEN: European F-Element Network" for supporting this work. CREA (Centro Ricerche Energia e Ambiente) in Colle Val d'Elsa (Siena, Italy) is also acknowledged for computational resources. The work done at the University of Washington and the University of New Mexico was supported by the Department of Energy (DE-FG02-06ER15765). NR 100 TC 5 Z9 5 U1 7 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD AUG 24 PY 2015 VL 34 IS 16 BP 3998 EP 4010 DI 10.1021/acs.organomet.5b00355 PG 13 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA CQ0XS UT WOS:000360322500011 ER PT J AU Alvarado, SR Shortt, IA Fan, HJ Vela, J AF Alvarado, Samuel R. Shortt, Ian A. Fan, Hua-Jun Vela, Javier TI Assessing Phosphine-Chalcogen Bond Energetics from Calculations SO ORGANOMETALLICS LA English DT Article ID ELECTRONIC POPULATION ANALYSIS; MOLECULAR WAVE FUNCTIONS; SULFUR ATOM-TRANSFER; NMR CHEMICAL-SHIFTS; SEMICONDUCTOR NANOCRYSTAL SYNTHESIS; NUCLEAR-MAGNETIC-RESONANCE; PERTURBATION-THEORY; EXCHANGE-REACTIONS; LCAO; MECHANISM AB Phosphine chalcogenides are useful reagents in chalcogen atom transfer reactions and nanocrystal syntheses. Understanding the strength and electronic structure of these bonds is key to optimizing their use, but a limited number of experimental and computational studies probe these issues. Using density functional theory (DFT), we computationally screen multiple series of trisubstituted phosphine chalcogenide molecules with a variety of phosphorus substituents and examine how these affect the strength of the phosphorus-chalcogen bond. DFT provides valuable data on these compounds including PE bond dissociation energies, P-E bond order, Lowdin charge on phosphorus and chalcogen atoms, and molecular geometries. Experimentally monitoring the P-31 and Se-77 NMR chemical shifts and published Hammett constants provides good estimates and confirmation of the relative magnitude of electronic shielding around these nuclei and confirms the predictive value of the computational results. C1 [Alvarado, Samuel R.; Vela, Javier] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Alvarado, Samuel R.; Vela, Javier] Ames Lab, Ames, IA 50011 USA. [Shortt, Ian A.; Fan, Hua-Jun] Prairie View A&M Univ, Dept Chem, Prairie View, TX 77446 USA. RP Fan, HJ (reprint author), Prairie View A&M Univ, Dept Chem, Prairie View, TX 77446 USA. EM hjfan@pvamu.edu; vela@iastate.edu RI Vela, Javier/I-4724-2014 OI Vela, Javier/0000-0001-5124-6893 FU National Science Foundation through Division of Materials Research, Solid State and Materials Chemistry program [NSF-DMR-1309510]; Department of Chemistry at Prairie View AM University [115103-00011]; U.S. Department of Energy, National Nuclear Security Administration [DE-NA 0001861] FX J.V. gratefully acknowledges the National Science Foundation for funding of this work through the Division of Materials Research, Solid State and Materials Chemistry program (NSF-DMR-1309510). H.-J.F. thanks the Department of Chemistry at Prairie View A&M University for release time and a 2014 Summer Research mini-grant (115103-00011), and the U.S. Department of Energy, National Nuclear Security Administration, for support (DE-NA 0001861). S.R.A. thanks Stephen Todey for assistance with NMR experiments. The authors would like to dedicate this work to Prof. John Verkade for his six decades of research excellence and thank him, Pat Holland, Gordie Miller, and Arthur Winter for comments. NR 67 TC 6 Z9 6 U1 3 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD AUG 24 PY 2015 VL 34 IS 16 BP 4023 EP 4031 DI 10.1021/acs.organomet.5b00428 PG 9 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA CQ0XS UT WOS:000360322500014 ER PT J AU Efremenko, I Fish, RH AF Efremenko, Irena Fish, Richard H. TI Quantum Chemical and Molecular Docking Studies of [(eta(6)-Cp*Rh-Tyr(1))-Leu-enkephalin](2+) to G-Protein-Coupled mu-, partial derivative- and kappa-Opioid Receptors and Comparisons to the Neuropeptide [Tyr(1)]-Leu-enkephalin: Conformations, Noncovalent Amino Acid Binding Sites, Binding Energies, Electronic Factors, and Receptor Distortion Forces SO ORGANOMETALLICS LA English DT Article ID BIOORGANOMETALLIC CHEMISTRY; BASIS-SETS; COMPLEXES; DFT; STABILITY; CANCER AB Recently reported studies by Kobilka et al. (Nature 2012, 485, 321, 400) and Stevens et al. (Nature 2012, 485, 327) have characterized the structures of the G-protein-coupled mu-, partial derivative-, and kappa-opioid receptors (GPCORs) via X-ray crystallography, including the use of guest, morphinan antagonist, drug analogues. These GPCORs have been shown to control the physiological functions of pain and, therefore, have been designated as a prime target for new, nonaddictive, pain drug discoveries. Moreover, Fish et al. (J. Am. Chem. Soc. 2012, 134, 10321) have recently reported on a chemoselective reaction of GPCR tyrosine-containing peptides with [Cp*Rh(H2O3)](OTf)(2) to provide [(eta(6)-Cp*Rh-Tyr(#))-GPCR-peptide] (OTf)(2) complexes. For example, the agonist, endogenous neuropeptide [Tyr(1)]-Leu-enkephalin, 1 (Tyr(1)-Gly-Gly-Phe-Leu), upon reaction with the Cp*Rh tris aqua complex, at pH 5-6, gave the [(eta(6)-Cp*Rh-Tyr(1))-Leu-enkephalin](OTf)(2) complex 2, also an agonist, which was found to bind to individual and coexpressed mu- and partial derivative-opioid receptor cells. Therefore, we present, in this contribution, the first comprehensive quantum chemical and molecular docking studies of an organometallic neuropeptide complex, 2, to structurally characterized mu-, partial derivative-, and kappa-GPCORs. We found that the docked conformations of dication 2 at the three opioid receptors were in similar receptor locations to the natural neuropeptide 1, as well as the morphinan drug derivatives, all antagonists, used in the X-ray structures of the mu-, partial derivative-, and kappa-opioid receptors, but, importantly, had distinctly different noncovalent H-bonding, pi-pi and CH-pi interactions with the nearby transmembrane receptor amino acids compared to 1, with only H-bonding interactions. Therefore, quantum chemical calculations showed this was due to four critical factors: (a) Dication 2 was found to be a non-zwitterion versus 1 being a zwitterion; (b) significant differences in the electron density and hydrophobic effects of the (eta(6)-Cp*Rh-Tyr(1))(2+) versus the (Tyr(1)) moieties on the message paradigm for receptor molecular recognition; (c) binding energies of 2 in comparison to 1, for the opioid receptors; and (d) receptor distortion forces that could possibly hinder binding regimes of 1 and 2, especially to the kappa-opioid receptor. Furthermore, we have attempted to understand how these factors might possibly be related to the previously reported EC50 receptor binding values (nM) of agonists 1 and 2 at the mu-, partial derivative-, and kappa-opioid receptors. C1 [Efremenko, Irena] Weizmann Inst Sci, Dept Organ Chem, IL-76100 Rehovot, Israel. [Fish, Richard H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Efremenko, I (reprint author), Weizmann Inst Sci, Dept Organ Chem, IL-76100 Rehovot, Israel. EM irena.efremenko@weizmann.ac.il; rhfish@lbl.gov FU Helen and Martin Kimmel Center for Molecular Design; Minerva Foundation; Lise Meitner-Minerva Center; Weizmann Institute of Science; Israel Science Foundation [709/05]; [DE AC02-05CH11231] FX I.E. gratefully acknowledges the financial support at the Weizmann Institute of Science, by the Helen and Martin Kimmel Center for Molecular Design, the Israel Science Foundation (grant 709/05), the Minerva Foundation, and the Lise Meitner-Minerva Center for Computational Quantum Chemistry. R.H.F. thanks Dr. H. Bauke Albada, formerly of the Department of Bioinorganic Chemistry, Ruhr University, Bochum, and now of the Department of Organic Chemistry, Hebrew University, Jerusalem, for collaboration on the synthesis and purification of peptide 1 and complex 2 (ref 6). We also thank Dr. Jennifer Whistler, Department of Neurology, University of California, San Francisco, for critical discussions on the biological aspects. R.H.F. also gratefully acknowledges support by the Department of Energy under Contract No. DE AC02-05CH11231. NR 39 TC 3 Z9 3 U1 2 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD AUG 24 PY 2015 VL 34 IS 16 BP 4117 EP 4126 DI 10.1021/acs.organomet.5b00542 PG 10 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA CQ0XS UT WOS:000360322500026 ER PT J AU Chikara, S Haskel, D Sim, JH Kim, HS Chen, CC Fabbris, G Veiga, LSI Souza-Neto, NM Terzic, J Butrouna, K Cao, G Han, MJ van Veenendaal, M AF Chikara, Shalinee Haskel, Daniel Sim, Jae-Hoon Kim, Heung-Sik Chen, Cheng-Chien Fabbris, G. Veiga, L. S. I. Souza-Neto, N. M. Terzic, J. Butrouna, K. Cao, G. Han, Myung Joon van Veenendaal, Michel TI Sr2Ir1-xRhxO4(x < 0.5): An inhomogeneous j(eff)=1/2 Hubbard system SO PHYSICAL REVIEW B LA English DT Article AB In a combined experimental and theoretical study, we investigate the properties of Sr2Ir1-xRhxO4. From the branching ratios of the L-edge isotropic x-ray absorption spectra, we determine that the spin-orbit coupling is remarkably independent of x for both iridium and rhodium sites. DFT + U calculations show that the doping is close to isoelectronic and introduces impurity bands of predominantly rhodium character close to the lower Hubbard band. Overlap of these two bands leads to metallic behavior. Since the low-energy states for x < 0.5 have predominantly j(eff) = 1/2 character, we suggest that the electronic properties of this material can be described by an inhomogeneous Hubbard model, where the on-site energies change due to local variations in the spin-orbit interaction strength combined with additional changes in binding energy. C1 [Chikara, Shalinee; Haskel, Daniel; Chen, Cheng-Chien; Fabbris, G.; Veiga, L. S. I.; van Veenendaal, Michel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sim, Jae-Hoon; Kim, Heung-Sik; Han, Myung Joon] Korea Adv Inst Sci & Technol, Dept Phys, Taejon 305701, South Korea. [Fabbris, G.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Veiga, L. S. I.; Souza-Neto, N. M.] LNLS, BR-13083970 Campinas, SP, Brazil. [Veiga, L. S. I.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. [Terzic, J.; Butrouna, K.; Cao, G.] Univ Kentucky, Ctr Adv Mat, Lexington, KY 40506 USA. [Terzic, J.; Butrouna, K.; Cao, G.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [van Veenendaal, Michel] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Chikara, S (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RI Fabbris, Gilberto/F-3244-2011; Han, Myung Joon/H-7104-2012; Souza-Neto, Narcizo/G-1303-2010; Inst. of Physics, Gleb Wataghin/A-9780-2017; Chikara, Shalinee/E-4654-2017 OI Fabbris, Gilberto/0000-0001-8278-4985; Han, Myung Joon/0000-0002-8089-7991; Souza-Neto, Narcizo/0000-0002-7474-8017; FU US DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-03ER46097]; NIU's Institute for Nanoscience, Engineering, and Technology; US DOE [DE-AC02-05CH11231]; National Institute of Supercomputing and Networking/Korea Institute of Science and Technology Information [KSC-2013-C2-23]; Basic Science Research Program through NRF [2014R1A1A2057202]; Samsung Advanced Institute of Technology (SAIT); Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [2013R1A6A3A01064947]; NSF [DMR1265162] FX Work at Argonne National Laboratory was supported by the US DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. M.v.V. was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-03ER46097 and NIU's Institute for Nanoscience, Engineering, and Technology. The computational work was partially performed at NERSC, which is supported by the US DOE Contract No. DE-AC02-05CH11231. Computational resources were partly supported by the National Institute of Supercomputing and Networking/Korea Institute of Science and Technology Information with supercomputing resources including technical support (Grant No. KSC-2013-C2-23). J.H.S. and M.J.H were supported by Basic Science Research Program through NRF (2014R1A1A2057202) and by Samsung Advanced Institute of Technology (SAIT). H.-S.K. was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education (Grant No. 2013R1A6A3A01064947). The work at the University of Kentucky was supported by NSF via Grant No. DMR1265162. NR 20 TC 6 Z9 6 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 24 PY 2015 VL 92 IS 8 AR 081114 DI 10.1103/PhysRevB.92.081114 PG 5 WC Physics, Condensed Matter SC Physics GA CP5SD UT WOS:000359943400002 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Bouchet, J Brandin, AV Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Cervantes, MC Chakaberia, I Chaloupka, P Chang, Z Chattopadhyay, S Chen, JH Chen, X Cheng, J Cherney, M Christie, W Contin, G Crawford, HJ Das, S De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA di Ruzza, B Didenko, L Dilks, C Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Eppley, G Esha, R Evdokimov, O Eyser, O Fatemi, R Fazio, S Federic, P Fedorisin, J Feng, Z Filip, P Fisyak, Y Flores, CE Fulek, L Gagliardi, CA Garand, D Geurts, F Gibson, A Girard, M Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, S Gupta, A Guryn, W Hamad, A Hamed, A Haque, R Harris, JW He, L Heppelmann, S Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, X Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Jiang, K Judd, EG Jung, K Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Kochenda, L Koetke, DD Kollegger, T Kosarzewski, LK Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Li, X Li, C Li, W Li, ZM Li, Y Li, X Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, YG Ma, GL Ma, L Ma, R Magdy, N Majka, R Manion, A Margetis, S Markert, C Masui, H Matis, HS McDonald, D Meehan, K Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, D Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Okorokov, V Olvitt, D Page, BS Pak, R Pan, YX Pandit, Y Panebratsev, Y Pawlik, B Pei, H Perkins, C Peterson, A Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Posik, M Poskanzer, AM Pruthi, NK Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandweiss, J Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, MK Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Sikora, R Simko, M Skoby, MJ Smirnov, D Smirnov, N Song, L Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stepanov, M Stock, R Strikhanov, M Stringfellow, B Sumbera, M Summa, B Sun, X Sun, Z Sun, XM Sun, Y Surrow, B Svirida, N Szelezniak, MA Tang, AH Tang, Z Tarnowsky, T Tawfik, AN Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Tripathy, SK Trzeciak, BA Tsai, OD Ullrich, T Underwood, DG Upsal, I Van Buren, G van Nieuwenhuizen, G Vandenbroucke, M Varma, R Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Voloshin, SA Vossen, A Wang, G Wang, Y Wang, F Wang, Y Wang, H Wang, JS Webb, JC Webb, G Wen, L Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, ZG Xie, W Xin, K Xu, QH Xu, Z Xu, H Xu, N Xu, YF Yang, Q Yang, Y Yang, S Yang, Y Yang, C Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zbroszczyk, H Zha, W Zhang, XP Zhang, J Zhang, Y Zhang, J Zhang, JB Zhang, S Zhang, Z Zhao, J Zhong, C Zhou, L Zhu, X Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Bouchet, J. Brandin, A. V. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Campbell, J. M. Cebra, D. Cervantes, M. C. Chakaberia, I. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, J. H. Chen, X. Cheng, J. Cherney, M. Christie, W. Contin, G. Crawford, H. J. Das, S. De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. di Ruzza, B. Didenko, L. Dilks, C. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Eppley, G. Esha, R. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Federic, P. Fedorisin, J. Feng, Z. Filip, P. Fisyak, Y. Flores, C. E. Fulek, L. Gagliardi, C. A. Garand, D. Geurts, F. Gibson, A. Girard, M. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, S. Gupta, A. Guryn, W. Hamad, A. Hamed, A. Haque, R. Harris, J. W. He, L. Heppelmann, S. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, X. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Jiang, K. Judd, E. G. Jung, K. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Kochenda, L. Koetke, D. D. Kollegger, T. Kosarzewski, L. K. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Li, X. Li, C. Li, W. Li, Z. M. Li, Y. Li, X. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, Y. G. Ma, G. L. Ma, L. Ma, R. Magdy, N. Majka, R. Manion, A. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. Meehan, K. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Okorokov, V. Olvitt, D., Jr. Page, B. S. Pak, R. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlik, B. Pei, H. Perkins, C. Peterson, A. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Posik, M. Poskanzer, A. M. Pruthi, N. K. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandweiss, J. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, M. K. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Sikora, R. Simko, M. Skoby, M. J. Smirnov, D. Smirnov, N. Song, L. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stepanov, M. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Summa, B. Sun, X. Sun, Z. Sun, X. M. Sun, Y. Surrow, B. Svirida, N. Szelezniak, M. A. Tang, A. H. Tang, Z. Tarnowsky, T. Tawfik, A. N. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Tripathy, S. K. Trzeciak, B. A. Tsai, O. D. Ullrich, T. Underwood, D. G. Upsal, I. Van Buren, G. van Nieuwenhuizen, G. Vandenbroucke, M. Varma, R. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Vossen, A. Wang, G. Wang, Y. Wang, F. Wang, Y. Wang, H. Wang, J. S. Webb, J. C. Webb, G. Wen, L. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. G. Xie, W. Xin, K. Xu, Q. H. Xu, Z. Xu, H. Xu, N. Xu, Y. F. Yang, Q. Yang, Y. Yang, S. Yang, Y. Yang, C. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I. -K. Yu, N. Zbroszczyk, H. Zha, W. Zhang, X. P. Zhang, J. Zhang, Y. Zhang, J. Zhang, J. B. Zhang, S. Zhang, Z. Zhao, J. Zhong, C. Zhou, L. Zhu, X. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Measurements of dielectron production in Au plus Au collisions at root s(NN)=200 GeV from the STAR experiment SO PHYSICAL REVIEW C LA English DT Article ID RELATIVISTIC NUCLEAR COLLISIONS; SUPER-PROTON SYNCHROTRON; HEAVY-ION COLLISIONS; DILEPTON PRODUCTION; CHIRAL RESTORATION; TRANSPORT APPROACH; SPS ENERGIES; CERN-SPS; MULTIPLICITY; FLOW AB We report on measurements of dielectron (e(+) e(-)) production in Au + Au collisions at a center-of-mass energy of 200 GeV per nucleon-nucleon pair using the STAR detector at BNL Relativistic Heavy Ion Collider. Systematic measurements of the dielectron yield as a function of transverse momentum (p(T)) and collision centrality show an enhancement compared to a cocktail simulation of hadronic sources in the low invariant-mass region (M-ee < 1 GeV / c(2)). This enhancement cannot be reproduced by the rho-meson vacuum spectral function. In minimum-bias collisions, in the invariant-mass range of 0.30-0.76 GeV / c(2), integrated over the full pT acceptance, the enhancement factor is 1.76 +/- 0.06 (stat.) +/- 0.26 (sys.) +/- 0.29 (cocktail). The enhancement factor exhibits weak centrality and pT dependence in STAR's accessible kinematic regions, while the excess yield in this invariant-mass region as a function of the number of participating nucleons follows a power-law shape with a power of 1.44 +/- 0.10. Models that assume an in-medium broadening of the rho-meson spectral function consistently describe the observed excess in these measurements. Additionally, we report on measurements of omega-and phi-meson production through their e+ e(-) decay channel. These measurements show good agreement with Tsallis blast-wave model predictions, as well as, in the case of the phi meson, results through its K+ K- decay channel. In the intermediate invariant-mass region (1.1 < Mee < 3 GeV / c(2)), we investigate the spectral shapes from different collision centralities. Physics implications for possible in-medium modification of charmed hadron production and other physics sources are discussed. C1 [Adamczyk, L.; Fulek, L.; Sikora, R.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Arkhipkin, D.; Aschenauer, E. C.; Bland, L. C.; Burton, T. P.; Chakaberia, I.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Heppelmann, S.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; Li, X.; Ljubicic, T.; Longacre, R. S.; Ma, R.; Ogawa, A.; Page, B. S.; Pak, R.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; van Nieuwenhuizen, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Webb, G.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Sanchez, M. Calderon de la Barca; Cebra, D.; Draper, J. E.; Flores, C. E.; Meehan, K.; Romero, J. L.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Esha, R.; Huang, H. Z.; Igo, G.; Landry, K. D.; Nasim, Md.; Pan, Y. X.; Trentalange, S.; Tsai, O. D.; Wang, G.; Wen, L.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Feng, Z.; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Shi, S. S.; Sun, X. M.; Wang, Y.; Wu, Y. F.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Huang, B.; Khan, Z. H.; Pandit, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Cherney, M.; De Silva, L. C.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Rusnakova, O.; Trzeciak, B. A.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Bielcikova, J.; Federic, P.; Rusnak, J.; Simko, M.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] Frankfurt Inst Adv Studies FIAS, D-60438 Frankfurt, Germany. [Das, S.; Sahu, P. K.; Tripathy, S. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Jacobs, W. W.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bhasin, A.; Gupta, S.; Gupta, A.; Sharma, M. K.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Hamad, A.; Kabana, S.; Keane, D.; Lomnitz, M.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Ramachandran, S.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Taejon 305701, South Korea. [Chen, X.; Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.; Zhang, J.] Inst Modern Phys, Lanzhou 730000, Peoples R China. [Contin, G.; Dong, X.; Greiner, L.; Manion, A.; Masui, H.; Matis, H. S.; Mustafa, M. K.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Sichtermann, E. P.; Sun, X.; Szelezniak, M. A.; Thomas, J. H.; Wieman, H.; Xu, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kochenda, L.; Kravtsov, P.; Nigmatkulov, G.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Mohanty, B.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Campbell, J. M.; Humanic, T. J.; Lisa, M. A.; Peterson, A.; Upsal, I.] Ohio State Univ, Columbus, OH 43210 USA. [Kycia, R. A.; Pawlik, B.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Dilks, C.; Heppelmann, S.; Summa, B.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Garand, D.; He, L.; Hirsch, A.; Jung, K.; Scharenberg, R. P.; Srivastava, B.; Stepanov, M.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Guo, Y.; Jiang, K.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Yang, Q.; Yang, S.; Yang, C.; Zha, W.; Zhang, Y.; Zhou, L.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.; Zhang, J.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Li, W.; Ma, Y. G.; Ma, G. L.; Ma, L.; Shah, N.; Shen, W. Q.; Shou, Q. Y.; Xu, Y. F.; Zhang, S.; Zhang, Z.; Zhong, C.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D., Jr.; Posik, M.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Hoffmann, G. W.; Markert, C.; Ray, R. L.; Schambach, J.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Song, L.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z. G.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Roy, A.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pluta, J.; Poniatowska, K.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Kauder, K.; Llope, W. J.; Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Magdy, N.; Tawfik, A. N.] WLCAPP, Cairo 11571, Egypt. [Caines, H.; Harris, J. W.; Horvat, S.; Majka, R.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; Kycia, Radoslaw/J-4397-2015; Fazio, Salvatore /G-5156-2010; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Tawfik, Abdel Nasser/M-6220-2013; Okorokov, Vitaly/C-4800-2017 OI Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Kycia, Radoslaw/0000-0002-6390-4627; Sumbera, Michal/0000-0002-0639-7323; Huang, Bingchu/0000-0002-3253-3210; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Tawfik, Abdel Nasser/0000-0002-1679-0225; Okorokov, Vitaly/0000-0002-7162-5345 FU RHIC Operations Group; RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium; Office of Nuclear Physics within the U.S. DOE Office of Science; U.S. NSF [CNRS/IN2P3]; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; MoST of China (973 Program) [2014CB845400, 2015CB856900]; MoE of China; CAS; Korean Research Foundation; GA of the Czech Republic; MSMT of the Czech Republic; FIAS of Germany; DAE of India; DST of India; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank Prof. Ralf Rapp for discussions and clarifications on model calculations. We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported, in part, by the Office of Nuclear Physics within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3; FAPESP CNPq of Brazil; the Ministry of Education and Science of the Russian Federation; the NNSFC, the MoST of China (973 Program No. 2014CB845400, 2015CB856900), CAS, the MoE of China; the Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE, DST, and CSIR of India; the National Science Centre of Poland; National Research Foundation (Grant No. NRF-2012004024); the Ministry of Science, Education and Sports of the Republic of Croatia; and RosAtom of Russia. NR 74 TC 15 Z9 15 U1 6 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 24 PY 2015 VL 92 IS 2 AR 024912 DI 10.1103/PhysRevC.92.024912 PG 35 WC Physics, Nuclear SC Physics GA CP5SK UT WOS:000359944200007 ER PT J AU Mahmoud, ME Yakout, AA El Aziz, MTA Osman, MM Abdel-Fattah, TM AF Mahmoud, Mohamed E. Yakout, Amr A. El Aziz, Marwa T. Abed Osman, Maher M. Abdel-Fattah, Tarek M. TI A novel cellulose-dioctyl phthate-baker's yeast biosorbent for removal of Co(II), Cu(II), Cd(II), Hg(II) and Pb(II) SO JOURNAL OF ENVIRONMENTAL SCIENCE AND HEALTH PART A-TOXIC/HAZARDOUS SUBSTANCES & ENVIRONMENTAL ENGINEERING LA English DT Article DE Adsorption; Baker's yeast; bioremediation; cellulose; environmental bioengineering; waste treatment ID SOLID-PHASE EXTRACTION; WATER-TREATMENT; ADSORPTIVE REMOVAL; AQUEOUS-SOLUTIONS; HEAVY-METALS; SORBENTS; IONS; LEAD; ADSORBENT; CADMIUM AB In this work, dioctyl phthalate (Dop) was used as a highly plasticizing material to coat and link the surface of basic cellulose (Cel) with baker's yeast for the formation of a novel modified cellulose biosorbent (Cel-Dop-Yst). Characterization was accomplished by Fourier Transform Infrared Spectroscopy (FT-IR), Thermogravimetric analysis (TGA) and Scanning Electron Microscope (SEM) measurements. The feasibility of using Cel-Dop-Yst biosorbent as an efficient material for removal of Co(II), Cu(II), Cd(II), Hg(II) and Pb(II) ions was explored using the batch equilibrium technique along with various experimental controlling parameters. The optimum pH values for removal of these metal ions were characterized in the range of 5.0-7.0. Cel-Dop-Yst was identified as a highly selective biosorbent for removal of the selected divalent metal ions. The Cel-Dop-Yst biosorbent was successfully implemented in treatment and removal of these divalent metal ions from industrial wastewater, sea water and drinking water samples using a multistage microcolumn technique. C1 [Mahmoud, Mohamed E.; Yakout, Amr A.; El Aziz, Marwa T. Abed; Osman, Maher M.] Univ Alexandria, Fac Sci, Dept Chem, Alexandria, Egypt. [Yakout, Amr A.] Jeddah Univ, Dept Chem, Fac Sci, Jeddah, Saudi Arabia. [Abdel-Fattah, Tarek M.] Christopher Newport Univ, Appl Res Ctr, Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Abdel-Fattah, Tarek M.] Christopher Newport Univ, Dept Mol Biol & Chem, Newport News, VA 23606 USA. RP Abdel-Fattah, TM (reprint author), Christopher Newport Univ, Appl Res Ctr, 1 Univ Pl, Newport News, VA 23606 USA. EM fattah@cnu.edu NR 38 TC 0 Z9 0 U1 0 U2 25 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1093-4529 EI 1532-4117 J9 J ENVIRON SCI HEAL A JI J. Environ. Sci. Health Part A-Toxic/Hazard. Subst. Environ. Eng. PD AUG 24 PY 2015 VL 50 IS 10 BP 1072 EP 1081 DI 10.1080/10934529.2015.1038184 PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CL5QW UT WOS:000357016000009 PM 26121022 ER PT J AU Bertram, E Glover, SCO Clark, PC Klessen, RS AF Bertram, Erik Glover, Simon C. O. Clark, Paul C. Klessen, Ralf S. TI Star formation efficiencies of molecular clouds in a galactic centre environment SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE stars: formation; ISM: clouds; Galaxy: centre; galaxies: ISM ID CENTER DUST RIDGE; GRAVITATIONAL COLLAPSE; MILKY-WAY; INTERSTELLAR TURBULENCE; SUPERSONIC TURBULENCE; INITIAL CONDITIONS; MOVING MESH; GAS; GALAXIES; DENSITY AB We use the arepo moving mesh code to simulate the evolution of molecular clouds exposed to a harsh environment similar to that found in the galactic centre (GC), in an effort to understand why the star formation efficiency (SFE) of clouds in this environment is so small. Our simulations include a simplified treatment of time-dependent chemistry and account for the highly non-isothermal nature of the gas and the dust. We model clouds with a total mass of 1.3 x 10(5) M-aS (TM) and explore the effects of varying the mean cloud density and the virial parameter, alpha = E-kin/ vertical bar E-pot vertical bar. We vary the latter from alpha = 0.5 to 8.0, and so many of the clouds that we simulate are gravitationally unbound. We expose our model clouds to an interstellar radiation field (ISRF) and cosmic ray flux (CRF) that are both a factor of 1000 higher than the values found in the solar neighbourhood. As a reference, we also run simulations with local solar neighbourhood values of the ISRF and the CRF in order to better constrain the effects of the extreme conditions in the GC on the SFE. Despite the harsh environment and the large turbulent velocity dispersions adopted, we find that all of the simulated clouds form stars within less than a gravitational free-fall time. Increasing the virial parameter from alpha = 0.5 to 8.0 decreases the SFE by a factor of similar to 4-10, while increasing the ISRF/CRF by a factor of 1000 decreases the SFE again by a factor of similar to 2-6. However, even in our most unbound clouds, the SFE remains higher than that inferred for real GC clouds. We therefore conclude that high levels of turbulence and strong external heating are not enough by themselves to lead to a persistently low SFE at the centre of the Galaxy. C1 [Bertram, Erik; Glover, Simon C. O.; Clark, Paul C.; Klessen, Ralf S.] Heidelberg Univ, Inst Theoret Astrophys, Zentrum Astron, D-69120 Heidelberg, Germany. [Clark, Paul C.] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3AA, S Glam, Wales. [Klessen, Ralf S.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Klessen, Ralf S.] Stanford Univ, SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. RP Bertram, E (reprint author), Heidelberg Univ, Inst Theoret Astrophys, Zentrum Astron, Albert Ueberle Str 2, D-69120 Heidelberg, Germany. EM bertram@zah.uni-heidelberg.de FU Deutsche Forschungsgemeinschaft (DFG) [SFB 881, SPP 1573]; Konrad-Adenauer-Stiftung (KAS) via their 'Promotionsforderung'; DFG via Emmy-Noether grant - German Excellence Initiative [BA 3706]; DFG via Frontier grant of Heidelberg University - German Excellence Initiative; Baden-Wurttemberg Foundation; European Research Council under the European Community [339177] FX We thank J. M. Diederik Kruijssen, Katharine Johnston, Rowan Smith. Christian Baczynski, Mark Krumholz and Javier Ballesteros Paredes for informative discussions about the project. We also thank the referee for a timely and very constructive report, which helped to improve the paper a lot. EB, SCOG and RSK acknowledge support from the Deutsche Forschungsgemeinschaft (DFG) via the SFB 881 (sub projects B1, B2, B5 and B8) The Milky Way System' and the SPP (priority programme) 1573, 'Physics of the ISM'. Furthermore, EB acknowledges financial support from the Konrad-Adenauer-Stiftung (KAS) via their 'Promotionsforderung'. The simulations presented in this paper were performed on the Milkyway supercomputer at the Julich Forschungszentrum, funded via SFB 881. Additional simulations were performed on the kolob cluster at the University of Heidelberg, which is funded in part by the DFG via Emmy-Noether grant BA 3706, and via a Frontier grant of Heidelberg University, sponsored by the German Excellence Initiative as well as the Baden-Wurttemberg Foundation. RSK acknowledges support from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013) via the ERC Advanced Grant 'STARLIGHT: Formation of the First Stars' (project number 339177). NR 68 TC 4 Z9 4 U1 0 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2015 VL 451 IS 4 BP 3679 EP 3692 DI 10.1093/mnras/stv1239 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ8HA UT WOS:000360846400025 ER PT J AU Balke, N Jesse, S Li, Q Maksymovych, P Okatan, MB Strelcov, E Tselev, A Kalinin, SV AF Balke, Nina Jesse, Stephen Li, Qian Maksymovych, Petro Okatan, M. Baris Strelcov, Evgheni Tselev, Alexander Kalinin, Sergei V. TI Current and surface charge modified hysteresis loops in ferroelectric thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PIEZORESPONSE FORCE MICROSCOPY; SCANNING PROBE MICROSCOPY; NANOSCALE; SPECTROSCOPY AB Polarization domains in ferroelectric materials and the ability to orient them with an external electric field lead to the development of a variety of applications from information storage to actuation. The development of piezoresponse force microscopy (PFM) has enabled researchers to investigate ferroelectric domains and ferroelectric domain switching on the nanoscale, which offers a pathway to study structure-function relationships in this important material class. Due to its commercial availability and ease of use, PFM has become a widely used research tool. However, measurement artifacts, i.e., alternative signal origins besides the piezoelectric effect are barely discussed or considered. This becomes especially important for materials with a small piezoelectric coefficient or materials with unknown ferroelectric properties, including non-ferroelectric materials. Here, the role of surface charges and current flow during PFM measurements on classical ferroelectrics are discussed and it will be shown how they alter the PFM hysteresis loop shape. This will help to better address alternative signal origins in PFM-type experiments and offer a pathway to study additional phenomena besides ferroelectricity. (C) 2015 AIP Publishing LLC. C1 [Balke, Nina; Jesse, Stephen; Li, Qian; Maksymovych, Petro; Okatan, M. Baris; Strelcov, Evgheni; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Balke, N (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM balken@ornl.gov RI Tselev, Alexander/L-8579-2015; Balke, Nina/Q-2505-2015; Kalinin, Sergei/I-9096-2012; Maksymovych, Petro/C-3922-2016; Jesse, Stephen/D-3975-2016; Okatan, M. Baris/E-1913-2016 OI Tselev, Alexander/0000-0002-0098-6696; Balke, Nina/0000-0001-5865-5892; Kalinin, Sergei/0000-0001-5354-6152; Maksymovych, Petro/0000-0003-0822-8459; Jesse, Stephen/0000-0002-1168-8483; Okatan, M. Baris/0000-0002-9421-7846 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Personal support was provided by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (N.B., Q.L.). The experiments were performed at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy which also provided additional personal support (S.J., E.S., P.M., A.T., M.B.O., S.V.K.). The authors gratefully acknowledge the samples provided by P. Yu. NR 35 TC 5 Z9 5 U1 7 U2 41 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072013 DI 10.1063/1.4927811 PG 8 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900014 ER PT J AU Balke, N Bassiri-Gharb, N Lichtensteiger, C AF Balke, Nina Bassiri-Gharb, Nazanin Lichtensteiger, Celine TI Preface to Special Topic: Piezoresponse Force Microscopy SO JOURNAL OF APPLIED PHYSICS LA English DT Editorial Material C1 [Balke, Nina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Bassiri-Gharb, Nazanin] Georgia Inst Technol, Sch Mat Sci & Engn, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Lichtensteiger, Celine] Univ Geneva, DQMP, CH-1211 Geneva 4, Switzerland. RP Bassiri-Gharb, N (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. EM nazanin.bassirigharb@me.gatech.edu RI Bassiri-Gharb, Nazanin/F-1783-2011; Balke, Nina/Q-2505-2015 OI Bassiri-Gharb, Nazanin/0000-0002-0183-5160; Balke, Nina/0000-0001-5865-5892 NR 5 TC 0 Z9 0 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 071901 DI 10.1063/1.4927818 PG 3 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900001 ER PT J AU Borovikov, VA Kalinin, SV Khavin, Y Mirman, B Karapetian, E AF Borovikov, V. A. Kalinin, S. V. Khavin, Yu. Mirman, B. Karapetian, E. TI Point force and point electric charge applied to the boundary of three-dimensional anisotropic piezoelectric solid SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INHOMOGENEITY PROBLEMS; INCLUSION; INFINITE AB The Green's functions for a three-dimensional semi-infinite fully anisotropic piezoelectric material are derived using the plane wave theory method. The solution gives the complete set of electromechanical fields due to an arbitrarily oriented point force and a point electric charge applied to the boundary of the half-space. The solution constitutes generalization of Boussinesq's and Cerruti's problems of elastic isotropy for the anisotropic piezoelectric materials. On the example of piezoceramics PZT-6B, the present results are compared with the previously obtained solution for the special case of transversely isotropic piezoelectric solid subjected to the same boundary condition. (C) 2015 AIP Publishing LLC. C1 [Borovikov, V. A.] Russian Acad Sci, Inst Mech, Moscow, Russia. [Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Khavin, Yu.] Janis Res Co Inc, Woburn, MA 01801 USA. [Mirman, B.; Karapetian, E.] Suffolk Univ, Dept Math & Comp Sci, Boston, MA 02114 USA. RP Kalinin, SV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM sergei2@ornl.gov; ekarapetian@suffolk.edu RI Kalinin, Sergei/I-9096-2012 OI Kalinin, Sergei/0000-0001-5354-6152 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX The work was supported in part (S.V.K.) by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. With great sadness, we acknowledge the passing of the first author. This article is his last contribution to the advancement of science, and we dedicate this work to the memory of a great applied mathematician Vladimir Borovikov. NR 22 TC 1 Z9 1 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072009 DI 10.1063/1.4927808 PG 8 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900010 ER PT J AU Kolasinski, RD Shimada, M Oya, Y Buchenauer, DA Chikada, T Cowgill, DF Donovan, DC Friddle, RW Michibayashi, K Sato, M AF Kolasinski, R. D. Shimada, M. Oya, Y. Buchenauer, D. A. Chikada, T. Cowgill, D. F. Donovan, D. C. Friddle, R. W. Michibayashi, K. Sato, M. TI A multi-technique analysis of deuterium trapping and near-surface precipitate growth in plasma-exposed tungsten SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID EQUATION-OF-STATE; HELIUM BUBBLES; HYDROGEN; RETENTION; IMPURITIES; METALS; TDS AB In this work, we examine how deuterium becomes trapped in plasma-exposed tungsten and forms near-surface platelet-shaped precipitates. How these bubbles nucleate and grow, as well as the amount of deuterium trapped within, is crucial for interpreting the experimental database. Here, we use a combined experimental/theoretical approach to provide further insight into the underlying physics. With the Tritium Plasma Experiment, we exposed a series of ITER-grade tungsten samples to high flux D plasmas (up to 1.5 x 10(22) m(-2) s(-1)) at temperatures ranging between 103 and 554 degrees C. Retention of deuterium trapped in the bulk, assessed through thermal desorption spectrometry, reached a maximum at 230 degrees C and diminished rapidly thereafter for T>300 degrees C. Post-mortem examination of the surfaces revealed non-uniform growth of bubbles ranging in diameter between 1 and 10 mu m over the surface with a clear correlation with grain boundaries. Electron back-scattering diffraction maps over a large area of the surface confirmed this dependence; grains containing bubbles were aligned with a preferred slip vector along the < 111 > directions. Focused ion beam profiles suggest that these bubbles nucleated as platelets at depths of 200 nm-1 mu m beneath the surface and grew as a result of expansion of sub-surface cracks. To estimate the amount of deuterium trapped in these defects relative to other sites within the material, we applied a continuum-scale treatment of hydrogen isotope precipitation. In addition, we propose a straightforward model of near-surface platelet expansion that reproduces bubble sizes consistent with our measurements. For the tungsten microstructure considered here, we find that bubbles would only weakly affect migration of D into the material, perhaps explaining why deep trapping was observed in prior studies with plasma-exposed neutron-irradiated specimens. We foresee no insurmountable issues that would prevent the theoretical framework developed here from being extended to a broader range of systems where precipitation of insoluble gases in ion beam or plasma-exposed metals is of interest. (C) 2015 AIP Publishing LLC. C1 [Kolasinski, R. D.; Buchenauer, D. A.; Cowgill, D. F.; Donovan, D. C.] Sandia Natl Labs, Hydrogen & Combust Technol Dept, Livermore, CA 94551 USA. [Shimada, M.] Idaho Natl Lab, Fus Safety Program, Idaho Falls, ID 83415 USA. [Oya, Y.; Chikada, T.; Sato, M.] Shizuoka Univ, Grad Sch Sci, Dept Chem, Shizuoka 4228529, Japan. [Friddle, R. W.] Sandia Natl Labs, Energy Nanomat Dept, Livermore, CA 94551 USA. [Michibayashi, K.] Shizuoka Univ, Inst Geosci, Shizuoka 4228529, Japan. RP Kolasinski, RD (reprint author), Sandia Natl Labs, Hydrogen & Combust Technol Dept, Livermore, CA 94551 USA. EM rkolasi@sandia.gov OI Shimada, Masashi/0000-0002-1592-843X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; DOE Idaho Field Office [DE-AC07-05ID14517] FX It is a pleasure to thank Michael Rye (Sandia) for performing the FIB profiling, as well as Robert Pawelko (INL), Josh Whaley (Sandia), and L. Shayne Loftus (INL) for their technical support of the experiments. Our colleague Christopher San Marchi (Sandia) provided valuable guidance on equation of state models, as did Brian Somerday (Sandia) on crack propagation. In addition, we express our appreciation to Norman Bartelt (Sandia) for helpful comments regarding the manuscript. This work was performed under the U.S.-Japan collaborative research project, PHENIX. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was prepared for the U.S. Department of Energy, the Office of Fusion Energy Sciences, under the DOE Idaho Field Office Contract No. DE-AC07-05ID14517. NR 47 TC 2 Z9 2 U1 4 U2 27 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 073301 DI 10.1063/1.4928184 PG 13 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900025 ER PT J AU Pannala, S Turner, JA Allu, S Elwasif, WR Kalnaus, S Simunovic, S Kumar, A Billings, JJ Wang, H Nanda, J AF Pannala, S. Turner, J. A. Allu, S. Elwasif, W. R. Kalnaus, S. Simunovic, S. Kumar, A. Billings, J. J. Wang, H. Nanda, J. TI Multiscale modeling and characterization for performance and safety of lithium-ion batteries SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID RUNAWAY RISK-EVALUATION; INTERNAL SHORT-CIRCUIT; LI-ION; CAPACITY FADE; FUEL-CELLS; MECHANICAL-PROPERTIES; RAMAN MICROSCOPY; ENERGY-STORAGE; INSERTION CELL; THERMAL-MODEL AB Lithium-ion batteries are highly complex electrochemical systems whose performance and safety are governed by coupled nonlinear electrochemical-electrical-thermal-mechanical processes over a range of spatiotemporal scales. Gaining an understanding of the role of these processes as well as development of predictive capabilities for design of better performing batteries requires synergy between theory, modeling, and simulation, and fundamental experimental work to support the models. This paper presents the overview of the work performed by the authors aligned with both experimental and computational efforts. In this paper, we describe a new, open source computational environment for battery simulations with an initial focus on lithium-ion systems but designed to support a variety of model types and formulations. This system has been used to create a three-dimensional cell and battery pack models that explicitly simulate all the battery components (current collectors, electrodes, and separator). The models are used to predict battery performance under normal operations and to study thermal and mechanical safety aspects under adverse conditions. This paper also provides an overview of the experimental techniques to obtain crucial validation data to benchmark the simulations at various scales for performance as well as abuse. We detail some initial validation using characterization experiments such as infrared and neutron imaging and micro-Raman mapping. In addition, we identify opportunities for future integration of theory, modeling, and experiments. (C) 2015 AIP Publishing LLC. C1 [Pannala, S.; Turner, J. A.; Allu, S.; Elwasif, W. R.; Kalnaus, S.; Simunovic, S.; Kumar, A.; Billings, J. J.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Wang, H.; Nanda, J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Pannala, S (reprint author), SABIC 14100 Southwest Freeway,Suite 600, Sugar Land, TX 77478 USA. EM spannala@sabic.com RI Wang, Hsin/A-1942-2013; OI Turner, John/0000-0003-2521-4091; allu, srikanth/0000-0003-2841-4398; Wang, Hsin/0000-0003-2426-9867; Kalnaus, Sergiy/0000-0002-7465-3034; Billings, Jay/0000-0001-8811-2688; Elwasif, Wael/0000-0003-0554-1036 FU U.S. Department of Energy [DE-AC05-00OR22725]; Vehicle Technologies Program in the Office of Energy Efficiency and Renewable Energy; Advanced Research Projects Agency-Energy (ARPA-E); National Highway Transportation Safety Agency (NHTSA) of the U.S. Department of Transportation; ORNL Laboratory Directed Research and Development (LDRD) program FX The research was performed using the resources at Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. The authors acknowledge the support of the Vehicle Technologies Program in the Office of Energy Efficiency and Renewable Energy, the Advanced Research Projects Agency-Energy (ARPA-E), the National Highway Transportation Safety Agency (NHTSA) of the U.S. Department of Transportation, and the ORNL Laboratory Directed Research and Development (LDRD) program. NR 76 TC 4 Z9 4 U1 10 U2 79 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072017 DI 10.1063/1.4927817 PG 14 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900018 ER PT J AU Seol, D Seo, H Jesse, S Kim, Y AF Seol, Daehee Seo, Hosung Jesse, Stephen Kim, Yunseok TI Nanoscale mapping of electromechanical response in ionic conductive ceramics with piezoelectric inclusions SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ATOMIC-FORCE MICROSCOPY; IN-SITU AFM; FERROELECTRIC CAPACITORS; SWITCHING DYNAMICS; GLASS-CERAMICS; THIN-FILMS; LITHIUM; BATTERY; SURFACE; LI AB Electromechanical (EM) response in ion conductive ceramics with piezoelectric inclusions was spatially explored using strain-based atomic force microscopy. Since the sample is composed of two dominant phases of ionic and piezoelectric phases, it allows us to explore two different EM responses of electrically induced ionic response and piezoresponse over the same surface. Furthermore, EM response of the ionic phase, i.e., electrochemical strain, was quantitatively investigated from the comparison with that of the piezoelectric phase, i.e., piezoresponse. These results could provide additional information on the EM properties, including the electrochemical strain at nanoscale. (C) 2015 AIP Publishing LLC. C1 [Seol, Daehee; Seo, Hosung; Kim, Yunseok] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea. [Jesse, Stephen] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Kim, Y (reprint author), Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea. EM yunseokkim@skku.edu RI Jesse, Stephen/D-3975-2016 OI Jesse, Stephen/0000-0002-1168-8483 FU Basic Science Research Program through National Research Foundation of Korea (NRF) - Ministry of Science, ICT and Future Planning [NRF-2014R1A1A1008061]; Center for Nanophase Materials Sciences - Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science, ICT and Future Planning (NRF-2014R1A1A1008061) (D.S. and Y.K.). A portion of this research was supported by the Center for Nanophase Materials Sciences (S.J.), which is sponsored at the Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors gratefully acknowledge multiple discussions with S. V. Kalinin (Oak Ridge National Laboratory). NR 36 TC 4 Z9 4 U1 4 U2 27 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072014 DI 10.1063/1.4927813 PG 7 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900015 ER PT J AU Varenyk, OV Silibin, MV Kiselev, DA Eliseev, EA Kalinin, SV Morozovska, AN AF Varenyk, O. V. Silibin, M. V. Kiselev, D. A. Eliseev, E. A. Kalinin, S. V. Morozovska, A. N. TI Self-consistent modelling of electrochemical strain microscopy in mixed ionic-electronic conductors: Nonlinear and dynamic regimes SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SCANNING FORCE MICROSCOPY; FERROELECTRIC THIN-FILMS; DOMAIN-STRUCTURE; BATTERY CATHODE; NANOMETER-SCALE; NANOSCALE; ELECTROMECHANICS; TRANSPORT; BEHAVIOR AB The frequency dependent Electrochemical Strain Microscopy (ESM) response of mixed ionic-electronic conductors is analyzed within the framework of Fermi-Dirac statistics and the Vegard law, accounting for steric effects from mobile donors. The emergence of dynamic charge waves and nonlinear deformation of the surface in response to bias applied to the tip-surface junction is numerically explored. The 2D maps of the strain and concentration distributions across the mixed ionic-electronic conductor and bias-induced surface displacements are calculated. The obtained numerical results can be applied to quantify the ESM response of Li-based solid electrolytes, materials with resistive switching, and electroactive ferroelectric polymers, which are of potential interest for flexible and high-density non-volatile memory devices. (C) 2015 AIP Publishing LLC. C1 [Varenyk, O. V.; Morozovska, A. N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Silibin, M. V.] Natl Res Univ Elect Technol MIET, Moscow 124498, Russia. [Kiselev, D. A.] Natl Univ Sci & Technol MISiS, Moscow 119049, Russia. [Eliseev, E. A.] NAS Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Kalinin, SV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM sergei2@ornl.gov; anna.n.morozovska@gmail.com RI Kalinin, Sergei/I-9096-2012; Silibin, Maxim/J-6227-2014; OI Kalinin, Sergei/0000-0001-5354-6152; Kiselev, Dmitry/0000-0003-1047-3007 FU Russian Federation [14.Y30.15.2883-MK]; Center for Nanophase Materials Sciences [CNMS 2013-293, CNMS 2014-270]; National Academy of Sciences of Ukraine [35-02-14]; [11.2551.2014/K] FX M.V.S. acknowledges the grant of the President of the Russian Federation for state support of young Russian scientists-PhD (No. 14.Y30.15.2883-MK) and the project part of the State tasks in the field of scientific activity No. 11.2551.2014/K. O.V.V., E.A.E., and A.N.M. acknowledge Center for Nanophase Materials Sciences, user projects CNMS 2013-293, CNMS 2014-270, and National Academy of Sciences of Ukraine (Grant No. 35-02-14). The authors are very grateful to Dr. Rama K. Vasudevan and Lisa A. Goins for their help in the manuscript preparation. NR 39 TC 2 Z9 2 U1 1 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072015 DI 10.1063/1.4927815 PG 7 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900016 ER PT J AU Vasudevan, RK Zhang, SJ Okatan, MB Jesse, S Kalinin, SV Bassiri-Gharb, N AF Vasudevan, Rama K. Zhang, Shujun Okatan, M. Baris Jesse, Stephen Kalinin, Sergei V. Bassiri-Gharb, Nazanin TI Multidimensional dynamic piezoresponse measurements: Unraveling local relaxation behavior in relaxor-ferroelectrics via big data SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LEAD MAGNESIUM NIOBATE; FORCE MICROSCOPY; SINGLE-CRYSTALS; POLARIZATION AB Compositional and charge disorder in ferroelectric relaxors lies at the heart of the unusual properties of these systems, such as aging and non-ergodicity, polarization rotations, and a host of temperature and field-driven phase transitions. However, much information about the field-dynamics of the polarization in the prototypical ferroelectric relaxor (1 - x) Pb(Mg1/3Nb2/3)O-3-xPbTiO(3) (PMN-xPT) remains unprobed at the mesoscopic level. Here, we use a piezoresponse force microscopy-based dynamic multimodal relaxation spectroscopy technique, enabling the study of ferroelectric switching and polarization relaxation at mesoscopic length scales, and carry out measurements on a PMN-0.28PT sample with minimal polishing. Results indicate that beyond a threshold DC bias the average relaxation increases as the system attempts to relax to the previous state. Phenomenological fitting reveals the presence of mesoscale heterogeneity in relaxation amplitudes and clearly suggests the presence of two distinct amplitudes. Independent component analysis reveals the presence of a disorder component of the relaxation, which is found to be strongly anti-correlated with the maximum piezoresponse at that location, suggesting smaller disorder effects where the polarization reversal is large and vice versa. The disorder in the relaxation amplitudes is postulated to arise from rhombohedral and field-induced tetragonal phase in the crystal, with each phase associated with its own relaxation amplitude. These studies highlight the crucial importance of the mixture of ferroelectric phases in the compositions in proximity of the morphotropic phase boundary in governing the local response and further highlight the ability of PFM voltage and time spectroscopies, in conjunction with big-data multivariate analyses, to locally map disorder and correlate it with parameters governing the dynamic behavior. (C) 2015 AIP Publishing LLC. C1 [Vasudevan, Rama K.; Okatan, M. Baris; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Vasudevan, Rama K.; Okatan, M. Baris; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Zhang, Shujun] Penn State Univ, Mat Res Inst, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Bassiri-Gharb, Nazanin] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Bassiri-Gharb, Nazanin] Georgia Inst Technol, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. RP Bassiri-Gharb, N (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. EM nazanin.bassirigharb@me.gatech.edu RI Bassiri-Gharb, Nazanin/F-1783-2011; Vasudevan, Rama/Q-2530-2015; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Okatan, M. Baris/E-1913-2016 OI Bassiri-Gharb, Nazanin/0000-0002-0183-5160; Vasudevan, Rama/0000-0003-4692-8579; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Okatan, M. Baris/0000-0002-9421-7846 FU Division of Materials Sciences and Engineering, BES, DOE; Center for Nanophase Materials Sciences; U.S. National Science Foundation [DMR-1255379] FX This research was sponsored by the Division of Materials Sciences and Engineering, BES, DOE (R.K.V. and S.V.K.). A portion of this research was conducted at and partially supported by (S.J. and M.B.O.) the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. N.B.-G. acknowledges funding from the U.S. National Science Foundation through Grant No. DMR-1255379. NR 39 TC 3 Z9 3 U1 3 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2015 VL 118 IS 7 AR 072003 DI 10.1063/1.4927803 PG 10 WC Physics, Applied SC Physics GA CQ2OX UT WOS:000360441900004 ER PT J AU Huang, C Perez, D Voter, AF AF Huang, Chen Perez, Danny Voter, Arthur F. TI Hyperdynamics boost factor achievable with an ideal bias potential SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ACCELERATED MOLECULAR-DYNAMICS; TRANSITION-STATE THEORY; INFREQUENT EVENTS; CHEMICAL-REACTIONS; SELF-DIFFUSION; TIME-SCALE; SIMULATION; SURFACE; TEMPERATURE; SYSTEMS AB Hyperdynamics is a powerful method to significantly extend the time scales amenable to molecular dynamics simulation of infrequent events. One outstanding challenge, however, is the development of the so-called bias potential required by the method. In this work, we design a bias potential using information about all minimum energy pathways (MEPs) out of the current state. While this approach is not suitable for use in an actual hyperdynamics simulation, because the pathways are generally not known in advance, it allows us to show that it is possible to come very close to the theoretical boost limit of hyperdynamics while maintaining high accuracy. We demonstrate this by applying this MEP-based hyperdynamics (MEP-HD) to metallic surface diffusion systems. In most cases, MEP-HD gives boost factors that are orders of magnitude larger than the best existing bias potential, indicating that further development of hyperdynamics bias potentials could have a significant payoff. Finally, we discuss potential practical uses of MEP-HD, including the possibility of developing MEP-HD into a true hyperdynamics. (C) 2015 AIP Publishing LLC. C1 [Huang, Chen; Perez, Danny; Voter, Arthur F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Huang, C (reprint author), Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. EM chuang3@fsu.edu; afv@lanl.gov OI Voter, Arthur/0000-0001-9788-7194 FU United States Department of Energy (U.S. DOE) Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; National Nuclear Security administration of the U.S. DOE [DE-AC52-06NA25396] FX This work was supported by the United States Department of Energy (U.S. DOE) Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security administration of the U.S. DOE under Contract No. DE-AC52-06NA25396. NR 35 TC 2 Z9 2 U1 2 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2015 VL 143 IS 7 AR 074113 DI 10.1063/1.4928636 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ2OJ UT WOS:000360440400016 PM 26298121 ER PT J AU Steeves, AH Park, GB Bechtel, HA Baraban, JH Field, RW AF Steeves, Adam H. Park, G. Barratt Bechtel, Hans A. Baraban, Joshua H. Field, Robert W. TI Communication: Observation of local-bender eigenstates in acetylene SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID BENDING DYNAMICS; (A)OVER-TILDE(1)A(U) STATE; VIBRATIONAL LEVELS; MODES; FLUORESCENCE; INTENSITIES; SIGNATURES; SPECTRA; QUANTUM; C2H2 AB We report the observation of eigenstates that embody large-amplitude, local-bending vibrational motion in acetylene by stimulated emission pumping spectroscopy via vibrational levels of the S-1 state involving excitation in the non-totally symmetric bending modes. The N-b = 14 level, lying at 8971.69 cm(-1) (J = 0), is assigned on the basis of degeneracy due to dynamical symmetry breaking in the local-mode limit. The level pattern for the N-b = 16 level, lying at 10218.9 cm(-1), is consistent with expectations for increased separation of l = 0 and 2 vibrational angular momentum components. Increasingly poor agreement between our observations and the predicted positions of these levels highlights the failure of currently available normal mode effective Hamiltonian models to extrapolate to regions of the potential energy surface involving large-amplitude displacement along the acetylene reversible arrow vinylidene isomerization coordinate. (C) 2015 AIP Publishing LLC. C1 [Steeves, Adam H.; Park, G. Barratt; Bechtel, Hans A.; Baraban, Joshua H.; Field, Robert W.] MIT, Dept Chem, Cambridge, MA 02139 USA. [Steeves, Adam H.] Ithaca Coll, Dept Chem & Biochem, Ithaca, NY 14850 USA. [Park, G. Barratt] Max Planck Inst Biophys Chem, Gottingen, Germany. [Bechtel, Hans A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Baraban, Joshua H.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Steeves, AH (reprint author), MIT, Dept Chem, Cambridge, MA 02139 USA. EM rwfield@mit.edu OI Steeves, Adam/0000-0001-5813-4659; Park, Barratt/0000-0002-8716-220X; Field, Robert/0000-0002-7609-4205 FU U.S. Department of Energy, Office of Science, Chemical Sciences Geosciences and Biosciences Division of the Basic Energy Sciences Office [DE-FG0287ER13671] FX We are grateful to Annelise Beck for her assistance. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Chemical Sciences Geosciences and Biosciences Division of the Basic Energy Sciences Office, under Award No. DE-FG0287ER13671. NR 33 TC 1 Z9 1 U1 1 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2015 VL 143 IS 7 AR 071101 DI 10.1063/1.4928638 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ2OJ UT WOS:000360440400001 PM 26298106 ER PT J AU White, AF McCurdy, CW Head-Gordon, M AF White, Alec F. McCurdy, C. William Head-Gordon, Martin TI Restricted and unrestricted non-Hermitian Hartree-Fock: Theory, practical considerations, and applications to metastable molecular anions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SELF-CONSISTENT-FIELD; ELECTRON TRANSMISSION SPECTROSCOPY; STATIC-EXCHANGE APPROXIMATION; SHAPE RESONANCE; CONFIGURATION-INTERACTION; CROSS-SECTIONS; CONVERGENCE ACCELERATION; FORMALDEHYDE SCATTERING; VIBRATIONAL-EXCITATION; POLYATOMIC-MOLECULES AB This work describes the implementation and applications of non-Hermitian self-consistent field (NH-SCF) theory with complex basis functions for the ab initio computation of positions and widths of shape resonances in molecules. We utilize both the restricted open-shell and the previously unexplored spin-unrestricted variants to compute Siegert energies of several anionic shape resonances in small diatomic and polyatomic molecules including carbon tetrafluoride which has been the subject of several recent experimental studies. The computation of general molecular properties from a non-Hermitian wavefunction is discussed, and a density-based analysis is applied to the B-2(1) shape resonance in formaldehyde. Spin-unrestricted NH-SCF is used to compute a complex potential energy surface for the carbon monoxide anion which correctly describes dissociation. (C) 2015 AIP Publishing LLC. C1 [White, Alec F.] Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Dept Chem, Berkeley, CA 94720 USA. [White, Alec F.; McCurdy, C. William; Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [McCurdy, C. William] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA. [McCurdy, C. William] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP White, AF (reprint author), Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Dept Chem, Berkeley, CA 94720 USA. FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research, and Basic Energy Sciences FX Support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research, and Basic Energy Sciences. The authors thank Satoshi Yabushita for providing valuable computational benchmarks using an independent complex Gaussian implementation based on the COLUMBUS quantum chemistry codes. The authors thank Paul Horn for invaluable advice on the implementation of nonlinear solvers. NR 84 TC 6 Z9 6 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2015 VL 143 IS 7 AR 074103 DI 10.1063/1.4928529 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ2OJ UT WOS:000360440400006 PM 26298111 ER PT J AU Boughezal, R Caola, F Melnikov, K Petriello, F Schulze, M AF Boughezal, Radja Caola, Fabrizio Melnikov, Kirill Petriello, Frank Schulze, Markus TI Higgs Boson Production in Association with a Jet at Next-to-Next-to-Leading Order SO PHYSICAL REVIEW LETTERS LA English DT Article ID DOUBLE-REAL RADIATION; PARTON DISTRIBUTIONS; SECTOR DECOMPOSITION; NUMERICAL EVALUATION; SUBTRACTION SCHEME; NNLO QCD; LHC; AMPLITUDES; FACTORIZATION; INTEGRALS AB We present precise predictions for Higgs boson production in association with a jet. We work in the Higgs effective field theory framework and compute next-to-next-to-leading order QCD corrections to the gluon-gluon and quark-gluon channels, which is sufficient for reliable LHC phenomenology. We present fully differential results as well as total cross sections for the LHC. Our next-to-next-to-leading order predictions reduce the unphysical scale dependence by more than a factor of 2 and enhance the total rate by about twenty percent compared to next-to-leading order QCD predictions. Our results demonstrate for the first time satisfactory convergence of the perturbative series. C1 [Boughezal, Radja; Petriello, Frank] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Caola, Fabrizio; Schulze, Markus] CERN, Div Theory, CH-1211 Geneva 23, Switzerland. [Melnikov, Kirill] KIT, Inst Theoret Particle Phys, D-76128 Karlsruhe, Germany. [Petriello, Frank] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Boughezal, R (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. EM rboughezal@anl.gov; fabrizio.caola@cern.ch; kirill.melnikov@kit.edu; f-petriello@northwestern.edu; markus.schulze@cern.ch OI Caola, Fabrizio/0000-0003-4739-9285 FU DOE [DE-AC02-06CH11357, DE-FG02-91ER40684]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank T. Becher, J. Campbell, T. Gehrmann, and M. Jaquier for helpful communications. We are grateful to S. Badger for making his results for tree-level amplitudes available to us. F. C. would like to thank the Institute for Theoretical Particle Physics of KIT and the Physics and Astronomy Department of Northwestern University for hospitality at various stages of this project. R. B. is supported by the DOE under Contract No. DE-AC02-06CH11357. F. P. is supported by the DOE Grants No. DE-FG02-91ER40684 and No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 62 TC 33 Z9 33 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 21 PY 2015 VL 115 IS 8 AR 082003 DI 10.1103/PhysRevLett.115.082003 PG 6 WC Physics, Multidisciplinary SC Physics GA CP4SM UT WOS:000359872900005 PM 26340184 ER PT J AU Echevarria, D Gutfraind, A Boodram, B Major, M Del Valle, S Cotler, SJ Dahari, H AF Echevarria, Desarae Gutfraind, Alexander Boodram, Basmattee Major, Marian Del Valle, Sara Cotler, Scott J. Dahari, Harel TI Mathematical Modeling of Hepatitis C Prevalence Reduction with Antiviral Treatment Scale-Up in Persons Who Inject Drugs in Metropolitan Chicago SO PLOS ONE LA English DT Article ID HIV-ASSOCIATED BEHAVIORS; DIRECT-ACTING ANTIVIRALS; VIRUS-INFECTION; UNITED-STATES; RISK BEHAVIORS; YOUNG-ADULTS; USERS; METAANALYSIS; REINFECTION; PEOPLE AB Background/Aim New direct-acting antivirals (DAAs) provide an opportunity to combat hepatitis C virus (HCV) infection in persons who inject drugs (PWID). Here we use a mathematical model to predict the impact of a DAA-treatment scale-up on HCV prevalence among PWID and the estimated cost in metropolitan Chicago. Methods To estimate the HCV antibody and HCV-RNA (chronic infection) prevalence among the metropolitan Chicago PWID population, we used empirical data from three large epidemiological studies. Cost of DAAs is assumed $50,000 per person. Results Approximately 32,000 PWID reside in metropolitan Chicago with an estimated HCV-RNA prevalence of 47% or 15,040 cases. Approximately 22,000 PWID (69% of the total PWID population) attend harm reduction (HR) programs, such as syringe exchange programs, and have an estimated HCV-RNA prevalence of 30%. There are about 11,000 young PWID (<30 years old) with an estimated HCV-RNA prevalence of 10% (PWID in these two subpopulations overlap). The model suggests that the following treatment scale-up is needed to reduce the baseline HCV-RNA prevalence by one-half over 10 years of treatment [cost per year, min-max in millions]: 35 per 1,000 [$50-$77] in the overall PWID population, 19 per 1,000 [$20-$26] for persons in HR programs, and 5 per 1,000 [$3-$4] for young PWID. Conclusions Treatment scale-up could dramatically reduce the prevalence of chronic HCV infection among PWID in Chicago, who are the main reservoir for on-going HCV transmission. Focusing treatment on PWID attending HR programs and/or young PWID could have a significant impact on HCV prevalence in these subpopulations at an attainable cost. C1 [Echevarria, Desarae; Gutfraind, Alexander; Cotler, Scott J.; Dahari, Harel] Loyola Univ Chicago, Med Ctr, Program Expt & Theoret Modeling, Div Hepatol,Dept Med, Maywood, IL 60526 USA. [Gutfraind, Alexander; Boodram, Basmattee] Univ Illinois, Sch Publ Hlth, Div Epidemiol & Biostat, Chicago, IL USA. [Major, Marian] US FDA, Div Viral Prod, Ctr Biol Evaluat & Res, Silver Spring, MD USA. [Del Valle, Sara] Los Alamos Natl Lab, Energy & Infrastruct Anal Grp, Los Alamos, NM USA. [Dahari, Harel] Los Alamos Natl Lab, Theoret & Biophys Grp, Los Alamos, NM USA. RP Dahari, H (reprint author), Loyola Univ Chicago, Med Ctr, Program Expt & Theoret Modeling, Div Hepatol,Dept Med, Maywood, IL 60526 USA. EM hdahari@lumc.edu FU NIH [P20-GM103452, R01-AI078881]; U.S. Department of Energy [DE-AC52-06NA25396]; UIC Award of Excellence FX This study was supported by NIH grants P20-GM103452 and R01-AI078881, the U.S. Department of Energy contract DE-AC52-06NA25396 and UIC Award of Excellence. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 54 TC 0 Z9 0 U1 1 U2 8 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 21 PY 2015 VL 10 IS 8 AR e0135901 DI 10.1371/journal.pone.0135901 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP5MR UT WOS:000359926900048 PM 26295805 ER PT J AU Hamilton, P Jaffe, M Haslinger, P Simmons, Q Muller, H Khoury, J AF Hamilton, P. Jaffe, M. Haslinger, P. Simmons, Q. Mueller, H. Khoury, J. TI Atom-interferometry constraints on dark energy SO SCIENCE LA English DT Article ID COSMOLOGICAL CONSTANT AB If dark energy, which drives the accelerated expansion of the universe, consists of a light scalar field, it might be detectable as a "fifth force" between normal-matter objects, in potential conflict with precision tests of gravity. Chameleon fields and other theories with screening mechanisms, however, can evade these tests by suppressing the forces in regions of high density, such as the laboratory. Using a cesium matter-wave interferometer near a spherical mass in an ultrahigh-vacuum chamber, we reduced the screening mechanism by probing the field with individual atoms rather than with bulk matter. We thereby constrained a wide class of dark energy theories, including a range of chameleon and other theories that reproduce the observed cosmic acceleration. C1 [Hamilton, P.; Jaffe, M.; Haslinger, P.; Simmons, Q.; Mueller, H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mueller, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Khoury, J.] Univ Penn, Dept Phys & Astron, Ctr Particle Cosmol, Philadelphia, PA 19104 USA. RP Muller, H (reprint author), Univ Calif Berkeley, Dept Phys, 366 Le Conte Hall MS 7300, Berkeley, CA 94720 USA. EM hm@berkeley.edu OI Hamilton, Paul/0000-0001-6080-632X FU David and Lucile Packard Foundation; Defense Advanced Research Projects Agency [N66001-12-1-4232]; NSF [PHY-1404566, PHY-1145525]; NASA [NNH13ZTT002N, NNH11ZTT001N]; Austrian Science Fund [J3680]; NASA Astrophysics Theory Program [NNX11AI95G] FX We acknowledge important discussions with D. Budker, C. Burrage, A. Charman, Y. Nomura, S. Perlmutter, S. Rajendran, and P. Steinhardt. This work was supported by the David and Lucile Packard Foundation; a Defense Advanced Research Projects Agency Young Faculty Award (no. N66001-12-1-4232); NSF grant PHY-1404566; and NASA grants NNH13ZTT002N, NNH13ZTT002N, and NNH11ZTT001N. P. Has. thanks the Austrian Science Fund (grant J3680). The work of J.K. is supported by the NSF Faculty Early Career Development Program (award PHY-1145525) and the NASA Astrophysics Theory Program (grant NNX11AI95G). NR 27 TC 34 Z9 35 U1 1 U2 10 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 21 PY 2015 VL 349 IS 6250 BP 849 EP 851 DI 10.1126/science.aaa8883 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP4DR UT WOS:000359832700044 PM 26293958 ER PT J AU Lebeis, SL Paredes, SH Lundberg, DS Breakfield, N Gehring, J McDonald, M Malfatti, S del Rio, TG Jones, CD Tringe, SG Dangl, JL AF Lebeis, Sarah L. Paredes, Sur Herrera Lundberg, Derek S. Breakfield, Natalie Gehring, Jase McDonald, Meredith Malfatti, Stephanie del Rio, Tijana Glavina Jones, Corbin D. Tringe, Susannah G. Dangl, Jeffery L. TI Salicylic acid modulates colonization of the root microbiome by specific bacterial taxa SO SCIENCE LA English DT Article ID PLANT IMMUNE-SYSTEM; ARABIDOPSIS-THALIANA; DEFENSE AB Immune systems distinguish "self" from "nonself" to maintain homeostasis and must differentially gate access to allow colonization by potentially beneficial, nonpathogenic microbes. Plant roots grow within extremely diverse soil microbial communities but assemble a taxonomically limited root-associated microbiome. We grew isogenic Arabidopsis thaliana mutants with altered immune systems in a wild soil and also in recolonization experiments with a synthetic bacterial community. We established that biosynthesis of, and signaling dependent on, the foliar defense phytohormone salicylic acid is required to assemble a normal root microbiome. Salicylic acid modulates colonization of the root by specific bacterial families. Thus, plant immune signaling drives selection from the available microbial communities to sculpt the root microbiome. C1 [Lebeis, Sarah L.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Lebeis, Sarah L.; Paredes, Sur Herrera; Lundberg, Derek S.; Breakfield, Natalie; Gehring, Jase; McDonald, Meredith; Jones, Corbin D.; Dangl, Jeffery L.] Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. [Paredes, Sur Herrera; Dangl, Jeffery L.] Univ N Carolina, Howard Hughes Med Inst, Chapel Hill, NC 27599 USA. [Paredes, Sur Herrera; Jones, Corbin D.; Dangl, Jeffery L.] Univ N Carolina, Curriculum Bioinformat & Computat Biol, Chapel Hill, NC 27599 USA. [Lundberg, Derek S.; Jones, Corbin D.; Dangl, Jeffery L.] Univ N Carolina, Curriculum Genet & Mol Biol, Chapel Hill, NC 27599 USA. [Malfatti, Stephanie; del Rio, Tijana Glavina; Tringe, Susannah G.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Jones, Corbin D.; Dangl, Jeffery L.] Univ N Carolina, Carolina Ctr Genome Sci, Chapel Hill, NC 27599 USA. [Dangl, Jeffery L.] Univ N Carolina, Dept Microbiol & Immunol, Chapel Hill, NC 27599 USA. RP Lebeis, SL (reprint author), Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. EM slebeis@utk.edu; dangl@email.unc.edu OI Breakfield, Natalie/0000-0001-8517-885X; Herrera Paredes, Sur/0000-0001-9246-8337 FU NSF Microbial Systems Biology [IOS-0958245]; NSF INSPIRE [IOS-1343020]; NIH [T32 GM067553-06, T32 GM07092-34]; HHMI; Gordon and Betty Moore Foundation [GBMF3030]; NIH Minority Opportunities in Research division of the National Institute of General Medical Sciences (NIGMS) [K12GM000678]; NIH Dr. Ruth L. Kirschstein National Research Service Award Fellowship [F32-GM103156]; Office of Science of the DOE [DE-AC02-05CH11231]; DOE-JGI Director's Discretionary Grand Challenge Program FX This work was supported by NSF Microbial Systems Biology grant IOS-0958245 and NSF INSPIRE grant IOS-1343020 to J.L.D. S.H.P. was supported by NIH Training Grant T32 GM067553-06 and is a Howard Hughes Medical Institute (HHMI) International Student Research Fellow. D.S.L. was supported by NIH Training Grant T32 GM07092-34. J.L.D. is an Investigator of HHMI, supported by HHMI and the Gordon and Betty Moore Foundation (GBMF3030). S.L.L. was supported by the NIH Minority Opportunities in Research division of the National Institute of General Medical Sciences (NIGMS) grant K12GM000678. N.B. was supported by NIH Dr. Ruth L. Kirschstein National Research Service Award Fellowship F32-GM103156. The work conducted by the U.S. Department of Energy (DOE) Joint Genome Institute (JGI), a DOE Office of Science User Facility, is supported by the Office of Science of the DOE under contract DE-AC02-05CH11231. This work was also funded by the DOE-JGI Director's Discretionary Grand Challenge Program. We thank the Dangl laboratory microbiome group for useful discussions and S. Grant, S. Y. He, P. Hugenholtz, J. Kremer, and D. Weigel for critical comments on the manuscript. The supplementary materials contain additional data. J.L.D. is a cofounder, shareholder, and chair of the Scientific Advisory Board of AgBiome, a corporation whose goal is to use plant-associated microbes to improve plant productivity. Raw sequence data are available at the Short Read Archive accessions ERP010780 and ERP010863 and at the JGI portal http://genome.jgi.doe.gov/Immunesamples/Immunesamples.info.html, which requires registration to access. NR 16 TC 68 Z9 68 U1 33 U2 187 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 21 PY 2015 VL 349 IS 6250 BP 860 EP 864 DI 10.1126/science.aaa8764 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP4DR UT WOS:000359832700048 PM 26184915 ER PT J AU Chien, TY He, XB Mo, SK Hashimoto, M Hussain, Z Shen, ZX Plummer, EW AF Chien, TeYu He, Xiaobo Mo, Sung-Kwan Hashimoto, Makoto Hussain, Zahid Shen, Zhi-Xun Plummer, E. W. TI Electron-phonon coupling in a system with broken symmetry: Surface of Be(0001) SO PHYSICAL REVIEW B LA English DT Article ID PHOTOEMISSION SPECTRA; METAL-SURFACES; BI2SR2CACU2O8+DELTA; SUPERCONDUCTIVITY; DISPERSION; BERYLLIUM; ENERGY AB The momentum-resolved Eliashberg function (ELF) alpha(2) F(omega, k) for the Be(0001) zone-center surface state was extracted from the high-quality angle-resolved photoemission spectroscopy (ARPES) data at the Fermi energy in the (Gamma) over bar -> (M) over bar direction, displaying ten peaks. A comparison of the peaks in the ELF to the bulk phonon density of states (DOS) and the bulk and surface phonon dispersion allows for an identification of the origin of all but two of the peaks. The five high energy peaks (> 52 meV) are associated with the coupling of the surface state to bulk phonon modes. The peaks at 44.5 and at 49.0 meV have contributions from both the bulk and surface phonons. The most intense peak at 37.5 meV is evidently having a contribution from electron-phonon coupling (EPC) of the surface state to the surface Rayleigh phonon mode. Surprisingly, the two lowest energy modes, which must be associated with surface Rayleigh phonon, cannot be attributed to a high phonon DOS at the surface nor to any Fermi surface nesting. After detail analysis, the three lowest energy peaks are associated with momentum dependence in the EPC matrix, reflected in the phonon linewidth changes. As a result of the broken symmetry at the surface, coupling of the initial surface state due to the presence of the surface phonons contributes similar to 48.5 +/- 12.5% of the spectral weight in the ELF and similar to 66.5 +/- 10.5% to the mass enhancement (lambda). C1 [Chien, TeYu] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [He, Xiaobo; Plummer, E. W.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Mo, Sung-Kwan; Hussain, Zahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Hashimoto, Makoto] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Shen, Zhi-Xun] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Shen, Zhi-Xun] Stanford Univ, Dept Phys, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Shen, Zhi-Xun] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. RP Chien, TY (reprint author), Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. EM tchien@uwyo.edu RI Mo, Sung-Kwan/F-3489-2013 OI Mo, Sung-Kwan/0000-0003-0711-8514 FU National Science Foundation [DMR-0451163, DMR-1504226]; Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation, TYC by DMR-0451163; and EWP by DMR-1504226. The ALS is supported by the Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 44 TC 1 Z9 1 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 21 PY 2015 VL 92 IS 7 AR 075133 DI 10.1103/PhysRevB.92.075133 PG 10 WC Physics, Condensed Matter SC Physics GA CP4NX UT WOS:000359860100002 ER PT J AU Gharbharan, D Britsch, D Soto, G Weed, AMK Svec, F Zajickova, Z AF Gharbharan, Deepa Britsch, Denae Soto, Gabriela Weed, Anna-Marie Karen Svec, Frantisek Zajickova, Zuzana TI Tuning preparation conditions towards optimized separation performance of thermally polymerized organo-silica monolithic columns in capillary liquid chromatography SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Organo-silica; Hybrid; Monolith; Sol-gel; Photo-polymerization; Thermal polymerization ID SOL-GEL MONOLITHS; HIGH-EFFICIENCY; ELECTROCHROMATOGRAPHY; HPLC; PHASE; METHACRYLATE; BEHAVIOR AB Tuning of preparation conditions, such as variations in the amount of a porogen, concentration of an aqueous acid catalyst, and adjustment in polymerization temperature and time, towards optimized chromatographic performance of thermally polymerized monolithic capillaries prepared from 3-(methacryloyloxy)propyltrimethoxysilane has been carried out. Performance of capillary columns in reversed-phase liquid chromatography was assessed utilizing various sets of solutes. Results describing hydrophobicity, steric selectivity, and extent of hydrogen bonding enabled comparison of performance of hybrid monolithic columns prepared under thermal (TSG) and photopolymerized (PSG) conditions. Reduced amounts of porogen in the polymerization mixture, and prolonged reaction times were necessary for the preparation of monolithic columns with enhanced retention and column efficiency that reached to 111,000 plates/m for alkylbenzenes with shorter alkyl chains. Both increased concentration of catalyst and higher temperature resulted in faster polymerization but inevitably in insufficient time for pore formation. Thermally polymerized monoliths produced surfaces, which were slightly more hydrophobic (a methylene selectivity of 1.28 +/- 10.002 TSG vs 1.20 +/- 0.002 PSG), with reduced number of residual silanols (a caffeine/phenol selectivity of 0.13 +/- 10.001 TSG vs 0.17 +/- 0.003 PSG). However, steric selectivity of 1.70 +/- 1 0.01 was the same for both types of columns. The batch-to-batch repeatability was better using thermal initiation compared to monolithic columns prepared under photopolymerized conditions. RSD for retention factor of benzene was 3.7% for TSG capillaries (n = 42) vs. 6.6% for PSG capillaries (n = 18). A similar trend was observed for columns prepared within the same batch. (C) 2015 Elsevier B.V. All rights reserved. C1 [Gharbharan, Deepa; Britsch, Denae; Soto, Gabriela; Weed, Anna-Marie Karen; Zajickova, Zuzana] Barry Univ, Dept Phys Sci, Miami Shores, FL 33161 USA. [Svec, Frantisek] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Zajickova, Z (reprint author), Barry Univ, Dept Phys Sci, Miami Shores, FL 33161 USA. EM ZZajickova@barry.edu FU National Science Foundation [CBET-1066113]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX Financial support of this project by the National Science Foundation (CBET-1066113) is gratefully acknowledged. Experimental work carried out at the Molecular Foundry, Lawrence Berkeley National Laboratory and F.S. were supported by the Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 23 TC 3 Z9 3 U1 2 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD AUG 21 PY 2015 VL 1408 BP 101 EP 107 DI 10.1016/j.chroma.2015.06.069 PG 7 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA CO7GH UT WOS:000359327100013 PM 26169907 ER PT J AU Polyanskiy, MN Babzien, M Pogorelsky, IV AF Polyanskiy, Mikhail N. Babzien, Marcus Pogorelsky, Igor V. TI Chirped-pulse amplification in a CO2 laser SO OPTICA LA English DT Article ID PICOSECOND 10-MU-M PULSES; COMPRESSION; ABSORPTION; DISPERSION; REFRACTION; RADIATION; GERMANIUM; CARRIERS AB Chirped-pulse amplification (CPA) is an integral part of present-day ultra-intense laser systems that normally employ near-infrared (similar to 1 mu m) solid-state lasers. The recently revived interest in expanding the reach of strong-field laser physics into the mid-infrared (mid-IR) spectral domain directs our attention to 9-11 mu m carbon-dioxide (CO2) lasers for which progress to reaching high peak intensities has been limited so far. We propose that employing the CPA technique will allow us to realize a new breakthrough toward multiterawatt, ultrafast mid-IR lasers; here we report, to our knowledge, the first implementation of this method for a CO2 laser. Our stretching of a 1 ps, 9 mu m pulse to 80 ps improved energy extraction from a regenerative CO2 laser amplifier by 1 order of magnitude. We explain this accomplishment by the reduction in nonlinear absorption and refraction on the amplifier's optical elements. We consider these findings as being a pivotal step toward establishing next-generation ultra-intense CO2 CPA laser systems for strong-field mid-IR research and its applications. (C) 2015 Optical Society of America C1 [Polyanskiy, Mikhail N.; Babzien, Marcus; Pogorelsky, Igor V.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Polyanskiy, MN (reprint author), Brookhaven Natl Lab, Bldg 820M, Upton, NY 11973 USA. EM polyanskiy@bnl.gov RI Polyanskiy, Mikhail/E-8406-2010 FU U.S. Department of Energy (DOE) [DE-AC02-98CH10886] FX U.S. Department of Energy (DOE) (DE-AC02-98CH10886). NR 18 TC 6 Z9 6 U1 4 U2 6 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2334-2536 J9 OPTICA JI Optica PD AUG 20 PY 2015 VL 2 IS 8 BP 675 EP 681 PG 7 WC Optics SC Optics GA CV7VV UT WOS:000364484600003 ER PT J AU Demos, SG Negres, RA Raman, RN Feit, MD Manes, KR Rubenchik, AM AF Demos, Stavros G. Negres, Raluca A. Raman, Rajesh N. Feit, Michael D. Manes, Kenneth R. Rubenchik, Alexander M. TI Relaxation dynamics of nanosecond laser superheated material in dielectrics SO OPTICA LA English DT Article ID FUSED-SILICA; PHASE EXPLOSION; ABLATION; VAPORIZATION; PARTICLES; VISCOSITY; BREAKDOWN; SURFACE; PULSES AB Intense laser pulses can cause superheating of the near-surface volume of materials. This mechanism is widely used in applications such as laser micromachining, laser ablation, or laser assisted thin film deposition. The relaxation of the near solid density superheated material is not well understood, however. In this work, we investigate the relaxation dynamics of the superheated material formed in several dielectrics with widely differing physical properties. The results suggest that the relaxation process involves a number of distinct phases, which include the delayed explosive ejection of microscale particles starting after the pressure of the superheated material is reduced to about 4 GPa and for a time duration on the order of 1 mu s. The appearance of a subset of collected ejected particles in fused silica is similar to that of micro-tektites and provides information about the state of the superheated material at the time of ejection. These results advance our understanding of a key aspect of the laser-material interaction pathway and can lead to optimization of associated applications ranging from material processing to laser surgery. C1 [Demos, Stavros G.; Negres, Raluca A.; Raman, Rajesh N.; Feit, Michael D.; Manes, Kenneth R.; Rubenchik, Alexander M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Demos, SG (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM demos1@llnl.gov FU U.S. Department of Energy (DOE) [DE-AC52-07NA27344] FX U.S. Department of Energy (DOE) (DE-AC52-07NA27344). NR 37 TC 6 Z9 6 U1 2 U2 5 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2334-2536 J9 OPTICA JI Optica PD AUG 20 PY 2015 VL 2 IS 8 BP 765 EP 772 DI 10.1364/OPTICA.2.000765 PG 8 WC Optics SC Optics GA CV7VV UT WOS:000364484600019 ER PT J AU Carvajal, CDR Dias, AG Nishi, CC Sanchez-Vega, BL AF Carvajal, C. D. R. Dias, A. G. Nishi, C. C. Sanchez-Vega, B. L. TI Axion like particles and the inverse seesaw mechanism (vol 05, 069, 2015) SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Correction C1 [Carvajal, C. D. R.; Dias, A. G.] Univ Fed ABC, Ctr Ciencias Nat & Humanas, BR-09210580 Santo Andre, SP, Brazil. [Nishi, C. C.] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Nishi, C. C.] Univ Fed ABC, Ctr Matemat Comp & Cognicao, BR-09210580 Santo Andre, SP, Brazil. [Sanchez-Vega, B. L.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Carvajal, CDR (reprint author), Univ Fed ABC, Ctr Ciencias Nat & Humanas, Ave Estados 5001, BR-09210580 Santo Andre, SP, Brazil. EM crisdaruiz@gmail.com; alex.dias@ufabc.edu.br; celso.nishi@ufabc.edu.br; brucesanchez@anl.gov RI Nishi, Celso/J-8494-2012 NR 1 TC 2 Z9 2 U1 2 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 20 PY 2015 IS 8 AR 103 DI 10.1007/JHEP08(2015)103 PG 2 WC Physics, Particles & Fields SC Physics GA CU4WN UT WOS:000363531300001 ER PT J AU Chandra, S Zhang, HC Kushwaha, P Singh, KP Bottcher, M Kaur, N Baliyan, KS AF Chandra, Sunil Zhang, Haocheng Kushwaha, Pankaj Singh, K. P. Bottcher, M. Kaur, Navpreet Baliyan, K. S. TI MULTI-WAVELENGTH STUDY OF FLARING ACTIVITY IN BL Lac OBJECT S5 0716+714 DURING THE 2015 OUTBURST SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: individual (S5 0716+714) ID LARGE-AREA TELESCOPE; INVERSE COMPTON VARIABILITY; GAMMA-RAY OUTBURST; ALL-SKY SURVEY; LACERTAE OBJECT; PKS 1510-089; X-RAY; ELECTROMAGNETIC-SPECTRUM; GALACTIC NUCLEI; DATA RELEASE AB We present a detailed investigation of the flaring activity observed from a BL Lac object, S5 0716+714, during its brightest ever optical state in the second half of 2015 January. Observed almost simultaneously in the optical, X-rays, and gamma-rays, a significant change in the degree of optical polarization (PD) and a swing in the position angle (PA) of polarization were recorded. A TeV (VHE) detection was also reported by the MAGIC consortium during this flaring episode. Two prominent sub-flares, peaking about five days apart, were seen in almost all of the energy bands. The multi-wavelength light curves, spectral energy distribution, and polarization are modeled using the time-dependent code developed by Zhang et al. This model assumes a straight jet threaded by large-scale helical magnetic fields taking into account the light travel time effects, incorporating synchrotron flux and polarization in 3D geometry. The rapid variation in PD and rotation in PA are most likely due to reconnections happening in the emission region in the jet, as suggested by the change in the ratio of toroidal to poloidal components of the magnetic field during the quiescent and flaring states. C1 [Chandra, Sunil; Kushwaha, Pankaj; Singh, K. P.] Tata Inst Fundamental Res, Dept Astron & Astrophys, Bombay 400005, Maharashtra, India. [Zhang, Haocheng] Ohio Univ, Dept Phys & Astron, Inst Astrophys, Athens, OH 45701 USA. [Zhang, Haocheng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Bottcher, M.] North West Univ, Ctr Space Res, ZA-2531 Potchefstroom, South Africa. [Kaur, Navpreet; Baliyan, K. S.] Phys Res Lab, Ahmadabad 380009, Gujarat, India. RP Chandra, S (reprint author), Tata Inst Fundamental Res, Dept Astron & Astrophys, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. OI Chandra, Sunil/0000-0002-8776-1835; /0000-0003-0180-8231 FU Fermi Guest Investigator grants [NNX08AW56G, NNX09AU10G, NNX12AO93G]; Tata Institute of Fundamental Research, Mumbai; Physical Research Laboratory, Unit of Dept. of Space, GOI, Ahmedabad; LANL/LDRD program; DoE/Office of Fusion Energy Science through CMSO; South African Research Chairs Initiative (SARChI) of the Department of Science and Technology; National Research Foundation of South Africa FX The authors are grateful to Prof. P. Smith and team, Arizona University, USA, for making the data from the Steward Observatory spectropolarimetric monitoring project accessible. This program is supported by Fermi Guest Investigator grants NNX08AW56G, NNX09AU10G, and NNX12AO93G. The authors also acknowledge the HEASARC and Fermi Science Team for data access from these facilities. S.C. and P.K. acknowledge the help and support of MIRO local staff during the course of campaign. S.C., P.K., K.S.B., and N.K. are thankful to Dr. S. Ganesh for helping in observations at MIRO. S.C., P.K., and K.P.S. are thankful to Tata Institute of Fundamental Research, Mumbai for the funding needed for this project. N.K. and K.S.B. acknowledge support by the Physical Research Laboratory, Unit of Dept. of Space, GOI, Ahmedabad for partial support. H.Z. is supported by the LANL/LDRD program and by DoE/Office of Fusion Energy Science through CMSO. M.B. acknowledges support by the South African Research Chairs Initiative (SARChI) of the Department of Science and Technology and the National Research Foundation of South Africa. The simulations used here were conducted using LANL's Institutional Computing machines. NR 58 TC 4 Z9 4 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 130 DI 10.1088/0004-637X/809/2/130 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100023 ER PT J AU Hovey, L Hughes, JP Eriksen, K AF Hovey, Luke Hughes, John P. Eriksen, Kristoffer TI A DIRECT MEASUREMENT OF THE FORWARD SHOCK SPEED IN SUPERNOVA REMNANT 0509-67.5: CONSTRAINTS ON THE AGE, AMBIENT DENSITY, SHOCK COMPRESSION FACTOR, AND ELECTRON-ION TEMPERATURE EQUILIBRATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic rays; ISM: individual objects (SNR 0509-67.5); ISM: kinematics and dynamics; ISM: supernova remnants; proper motions; shock waves ID LARGE-MAGELLANIC-CLOUD; BALMER-DOMINATED SHOCKS; COSMIC-RAY ACCELERATION; IA SUPERNOVA; PARTICLE-ACCELERATION; NOVA REMNANTS; ASTROPHYSICAL SHOCKS; OPTICAL-EMISSION; LIGHT ECHOES; X-RAY AB Two Hubble Space Telescope narrow-band H alpha images separated in time by 1.03 years are used for a proper motion measurement of the forward shock of the LMC supernova remnant 0509-67.5, the only spectroscopically confirmed LMC remnant of Ia origin. We measure a global shock speed of 6500 +/- 200 km s(-1) and constrain the pre-shock neutral hydrogen density to be 0.084 +/- 0.003 cm(-3), for a typical mean number of H alpha photons produced per neutral hydrogen atom entering the forward shock. Previously published broad H alpha line widths from two locations on the rim and our corresponding shock speed measurements are consistent with Balmer shock models that do not include effects of cosmic-ray acceleration. For the northeastern rim location, we limit the post-shock electron temperature to 10% of the proton temperature by also using the broad-to-narrow flux ratio. Hydrodynamic simulations for different initial ejecta density profiles constrain the age and ambient medium density; for an exponential ejecta profile and initial explosion energy of 1.4 x 10(51) erg, the remnant's age is 310(-30)(+40) years. For all evolutionary models explored, the expansion parameter falls in the range of 0.41-0.73, indicating that the remnant is still firmly in the ejecta-dominated phase of its evolution. Our measured neutral hydrogen density of the ambient medium, combined with the shocked density obtained in Williams et al., disfavors forward shock compression factors greater than similar to 7. C1 [Hovey, Luke; Hughes, John P.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Eriksen, Kristoffer] Los Alamos Natl Lab, Theoret Design Div, Los Alamos, NM 87545 USA. RP Hovey, L (reprint author), Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. EM lhovey@physics.rutgers.edu; jph@physics.rutgers.edu; keriksen@lanl.gov FU NASA from the Space Telescope Science Institute [HST-GO-11015.01-A]; NASA [NAS5-26555] FX L.H. thanks Kevin Heng for providing him with the numerical results of the models found in van Adelsberg et al. (2008); he also thanks Chelsea Sharon, Curtis McCully, and Saurabh Jha for help with various aspects of the analysis. J.P.H. acknowledges Jessica Warren, Carles Badenes, Chris Smith, Jacco Vink, and Parviz Ghavamian for their contributions to the original joint Chandra/HST proposal. Support for Program number HST-GO-11015.01-A was provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. NR 45 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 119 DI 10.1088/0004-637X/809/2/119 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100012 ER PT J AU Krivonos, RA Tsygankov, SS Lutovinov, AA Tomsick, JA Chakrabarty, D Bachetti, M Boggs, SE Chernyakova, M Christensen, FE Craig, WW Furst, F Hailey, CJ Harrison, FA Lansbury, GB Rahoui, F Stern, D Zhang, WW AF Krivonos, Roman A. Tsygankov, Sergey S. Lutovinov, Alexander A. Tomsick, John A. Chakrabarty, Deepto Bachetti, Matteo Boggs, Steven E. Chernyakova, Masha Christensen, Finn E. Craig, William W. Fuerst, Felix Hailey, Charles J. Harrison, Fiona A. Lansbury, George B. Rahoui, Farid Stern, Daniel Zhang, William W. TI NuSTAR DISCOVERY OF AN UNUSUALLY STEADY LONG-TERM SPIN-UP OF THE Be BINARY 2RXP J130159.6-635806 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: individual (2RXP J130159.6-635806); stars: emission-line, Be; X-rays: binaries ID X-RAY BINARIES; NEUTRON-STARS; PULSARS; PERIOD; ACCRETION; EVOLUTION; EMISSION; CATALOG; ENERGY; LINE AB We present spectral and timing analyses of Nuclear Spectroscopic Telescope Array (NuSTAR) observations of the accreting X-ray pulsar 2RXP J130159.6-635806. The source was serendipitously observed during a campaign focused on the gamma-ray binary PSR B1259-63 and was later targeted for a dedicated observation. The spectrum has a typical shape for accreting X-ray pulsars, consisting of a simple power law with an exponential cutoff starting at similar to 7 keV with a folding energy of E-fold similar or equal to 18 keV. There is also an indication of the presence of a 6.4 keV iron line in the spectrum at the similar to 3 sigma significance level. NuSTAR measurements of the pulsation period reveal that the pulsar has undergone a strong and steady spin-up for the last 20 years. The pulsed fraction is estimated to be similar to 80%, and is constant with energy up to 40 keV. The power density spectrum shows a break toward higher frequencies relative to the current spin period. This, together with steady persistent luminosity, points to a long-term mass accretion rate high enough to bring the pulsar out of spin equilibrium. C1 [Krivonos, Roman A.; Tomsick, John A.; Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Krivonos, Roman A.; Tsygankov, Sergey S.; Lutovinov, Alexander A.] Russian Acad Sci, Space Res Inst, Moscow 117997, Russia. [Tsygankov, Sergey S.] Univ Turku, Dept Phys & Astron, Tuorla Observ, FI-21500 Piikkio, Finland. [Chakrabarty, Deepto] MIT Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Bachetti, Matteo] Univ Toulouse 3, Observ Midi Pyrenees, F-31400 Toulouse, France. [Bachetti, Matteo] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse, France. [Chernyakova, Masha] Dublin City Univ, Dublin 9, Ireland. [Chernyakova, Masha] Dublin Inst Adv Studies, Dublin 2, Ireland. [Christensen, Finn E.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fuerst, Felix; Harrison, Fiona A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Lansbury, George B.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Rahoui, Farid] European So Observ, D-85748 Garching, Germany. [Rahoui, Farid] Harvard Univ, Dept Astron, Cambridge, MA 02138 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, William W.] NASA Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Krivonos, RA (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Krivonos, Roman/0000-0003-2737-5673 FU NASA; ESA Member States; Russian Science Foundation [14-12-01287] FX This research has made use of data obtained with NuSTAR, a project led by Caltech, funded by NASA and managed by NASA/JPL, and has utilized the NUSTARDAS software package, jointly developed by the ASDC (Italy) and Caltech (USA). This research has also made use of data obtained with XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States. A.L. and S.T. acknowledge support from Russian Science Foundation (grant 14-12-01287). NR 32 TC 5 Z9 5 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 140 DI 10.1088/0004-637X/809/2/140 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100033 ER PT J AU Lansbury, GB Gandhi, P Alexander, DM Assef, RJ Aird, J Annuar, A Ballantyne, DR Balokovic, M Bauer, FE Boggs, SE Brandt, WN Brightman, M Christensen, FE Civano, F Comastri, A Craig, WW Del Moro, A Grefenstette, BW Hailey, CJ Harrison, FA Hickox, RC Koss, M LaMassa, SM Luo, B Puccetti, S Stern, D Treister, E Vignali, C Zappacosta, L Zhang, WW AF Lansbury, G. B. Gandhi, P. Alexander, D. M. Assef, R. J. Aird, J. Annuar, A. Ballantyne, D. R. Balokovic, M. Bauer, F. E. Boggs, S. E. Brandt, W. N. Brightman, M. Christensen, F. E. Civano, F. Comastri, A. Craig, W. W. Del Moro, A. Grefenstette, B. W. Hailey, C. J. Harrison, F. A. Hickox, R. C. Koss, M. LaMassa, S. M. Luo, B. Puccetti, S. Stern, D. Treister, E. Vignali, C. Zappacosta, L. Zhang, W. W. TI NuSTAR REVEALS EXTREME ABSORPTION IN z < 0.5 TYPE 2 QUASARS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; X-rays: galaxies ID ACTIVE GALACTIC NUCLEI; HARD X-RAY; DIGITAL-SKY-SURVEY; SEYFERT 2 GALAXIES; COMPTON-THICK AGN; XMM-NEWTON OBSERVATIONS; ULTRALUMINOUS INFRARED GALAXIES; RESOLUTION SPECTRAL TEMPLATES; LUMINOUS OBSCURED QUASARS; APPROXIMATE-TO 2 AB The intrinsic column density (N-H) distribution of quasars is poorly known. At the high obscuration end of the quasar population and for redshifts z < 1, the X-ray spectra can only be reliably characterized using broad-band measurements that extend to energies above 10 keV. Using the hard X-ray observatory NuSTAR, along with archival Chandra and XMM-Newton data, we study the broad-band X-ray spectra of nine optically selected (from the SDSS), candidate Compton-thick (N-H > 1.5 x 10(24) cm(-2)) type 2 quasars (CTQSO2s); five new NuSTAR observations are reported herein, and four have been previously published. The candidate CTQSO2s lie at z < 0.5, have observed [O III] luminosities in the range 8.4< log(L-[O III]/L circle dot)< 9.6, and show evidence for extreme, Compton-thick absorption when indirect absorption diagnostics are considered. Among the nine candidate CTQSO2s, five are detected by NuSTAR in the high-energy (8-24 keV) band: two are weakly detected at the approximate to 3 sigma confidence level and three are strongly detected with sufficient counts for spectral modeling (greater than or similar to 90 net source counts at 8-24 keV). For these NuSTAR-detected sources direct (i.e., X-ray spectral) constraints on the intrinsic active galactic nucleus properties are feasible, and we measure column densities approximate to 2.5-1600 times higher and intrinsic (unabsorbed) X-ray luminosities approximate to 10-70 times higher than pre-NuSTAR constraints from Chandra and XMM-Newton. Assuming the NuSTAR-detected type 2 quasars are representative of other Compton-thick candidates, we make a correction to the N-H distribution for optically selected type 2 quasars as measured by Chandra and XMM-Newton for 39 objects. With this approach, we predict a Compton-thick fraction of f(CT) = 36(-12)(+14)%, although higher fractions (up to 76%) are possible if indirect absorption diagnostics are assumed to be reliable. C1 [Lansbury, G. B.; Gandhi, P.; Alexander, D. M.; Annuar, A.; Del Moro, A.] Univ Durham, Ctr Extragalact Astron, Dept Phys, Durham DH1 3LE, England. [Gandhi, P.] Univ Southampton, Sch Phys & Astron, Southampton SO17, Hants, England. [Assef, R. J.] Univ Diego Portales, Nucleo Astron, Fac Ingn, Santiago, Chile. [Aird, J.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Ballantyne, D. R.] Georgia Inst Technol, Sch Phys, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Balokovic, M.; Brightman, M.; Grefenstette, B. W.; Harrison, F. A.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Bauer, F. E.] Pontificia Univ Catolica Chile, Inst Astrofis, Fac Fis, Santiago 22, Chile. [Bauer, F. E.] Millennium Inst Astrophys, Santiago 7820436, Chile. [Bauer, F. E.] Space Sci Inst, Boulder, CO 80301 USA. [Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Brandt, W. N.; Luo, B.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Brandt, W. N.; Luo, B.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Christensen, F. E.; Craig, W. W.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Civano, F.; LaMassa, S. M.] Yale Univ, Dept Phys, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. [Civano, F.] Smithsonian Astrophys Observ, Cambridge, MA 02138 USA. [Civano, F.; Hickox, R. C.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Comastri, A.] INAF Osservatorio Astron Bologna, I-40127 Bologna, Italy. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Koss, M.] Swiss Fed Inst Technol, Inst Astron, Dept Phys, CH-8093 Zurich, Switzerland. [Puccetti, S.] ASDC ASI, I-00133 Rome, Italy. [Puccetti, S.; Zappacosta, L.] INAF Osservatorio Astron Roma, I-00040 Monte Porzio Catone, RM, Italy. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Treister, E.] Univ Concepcion, Dept Astron, Concepcion, Chile. [Vignali, C.] Univ Bologna, Dipartimento Fis & Astron, I-40127 Bologna, Italy. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Lansbury, GB (reprint author), Univ Durham, Ctr Extragalact Astron, Dept Phys, South Rd, Durham DH1 3LE, England. EM g.b.lansbury@durham.ac.uk RI Comastri, Andrea/O-9543-2015; Vignali, Cristian/J-4974-2012; Brandt, William/N-2844-2015; Boggs, Steven/E-4170-2015; OI Comastri, Andrea/0000-0003-3451-9970; Lansbury, George/0000-0002-5328-9827; Puccetti, Simonetta/0000-0002-2734-7835; Vignali, Cristian/0000-0002-8853-9611; Brandt, William/0000-0002-0167-2453; Boggs, Steven/0000-0001-9567-4224; Koss, Michael/0000-0002-7998-9581; Ballantyne, David/0000-0001-8128-6976 FU Science and Technology Facilities Council (STFC) [ST/K501979/1, ST/J003697/1, ST/I001573/1]; Leverhulme Trust; Gemini-CONICYT [32120009]; ERC Advanced Grant FEEDBACK at the University of Cambridge; NSF AST award [1008067]; NASA Earth and Space Science Fellowship Program [NNX14AQ07H]; CONICYT-Chile [PFB-06/2007, FONDECYT 1141218, ACT1101]; Ministry of Economy, Development, and Tourism's Millennium Science Initiative [IC120009]; Caltech NuSTAR subcontract [44A-1092750]; NASA ADP grant [NNX10AC99G]; Caltech Kingsley visitor program; ASI/INAF [I/037/12/0011/13]; NASA ADAP award [NNX12AE38G]; National Science Foundation [1211096]; Swiss National Science Foundation [PP00P2_138979/1]; NASA [NNG08FD60C]; National Aeronautics and Space Administration FX We thank the referee for a careful review, which has improved this work. We acknowledge financial support from: the Science and Technology Facilities Council (STFC) grants ST/K501979/1 (G.B.L.), ST/J003697/1 (P.G.), ST/I001573/1 (D.M.A. and A.D.M.); the Leverhulme Trust (D.M.A.); Gemini-CONICYT grant 32120009 (R.J.A.); the ERC Advanced Grant FEEDBACK at the University of Cambridge (J.A.); NSF AST award 1008067 (D.R.B.); the NASA Earth and Space Science Fellowship Program, grant NNX14AQ07H (M.B.); CONICYT-Chile grants Basal-CATA PFB-06/2007 (F.E.B.), FONDECYT 1141218 (F.E.B.), and "EMBIGGEN" Anillo ACT1101 (F.E.B.); the Ministry of Economy, Development, and Tourism's Millennium Science Initiative grant IC120009, awarded to The Millennium Institute of Astrophysics, MAS (F.E.B.); Caltech NuSTAR subcontract 44A-1092750 (W.N.B. and B.L.); NASA ADP grant NNX10AC99G (W.N.B. and B.L.); the Caltech Kingsley visitor program (A.C.); ASI/INAF grant I/037/12/0011/13 (A.C., S.P., C.V.); NASA ADAP award NNX12AE38G (R.C.H.); National Science Foundation grant 1211096 (R.C.H.); and Swiss National Science Foundation grant PP00P2_138979/1 (M.K.). We thank Andrew Ptak and Jianjun Jia for the useful correspondence. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). NR 112 TC 21 Z9 21 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 115 DI 10.1088/0004-637X/809/2/115 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100008 ER PT J AU Nichols, J Huenemoerder, DP Corcoran, MF Waldron, W Naze, Y Pollock, AMT Moffat, AFJ Lauer, J Shenar, T Russell, CMP Richardson, ND Pablo, H Evans, NR Hamaguchi, K Gull, T Hamann, WR Oskinova, L Ignace, R Hoffman, JL Hole, KT Lomax, JR AF Nichols, J. Huenemoerder, D. P. Corcoran, M. F. Waldron, W. Naze, Y. Pollock, A. M. T. Moffat, A. F. J. Lauer, J. Shenar, T. Russell, C. M. P. Richardson, N. D. Pablo, H. Evans, N. R. Hamaguchi, K. Gull, T. Hamann, W. -R. Oskinova, L. Ignace, R. Hoffman, Jennifer L. Hole, K. T. Lomax, J. R. TI A COORDINATED X-RAY AND OPTICAL CAMPAIGN OF THE NEAREST MASSIVE ECLIPSING BINARY, delta ORIONIS Aa. II. X-RAY VARIABILITY SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: close; binaries: eclipsing; stars: individual ([HD 36486]delta Ori A) ID EARLY-TYPE STARS; SHORT-TERM VARIABILITY; HELIUM-LIKE IONS; O-TYPE STARS; ABSORPTION COMPONENTS; LINE INTENSITIES; COLLIDING WINDS; MAIN-SEQUENCE; ZETA-OPHIUCHI; TIME-SERIES AB We present time-resolved and phase-resolved variability studies of an extensive X-ray high-resolution spectral data set of the delta Ori Aa binary system. The four observations, obtained with Chandra ACIS HETGS, have a total exposure time of approximate to 479 ks and provide nearly complete binary phase coverage. Variability of the total X-ray flux in the range of 5-25 is is confirmed, with a maximum amplitude of about +/- 15% within a single approximate to 125 ks observation. Periods of 4.76 and 2.04 days are found in the total X-ray flux, as well as an apparent overall increase in the flux level throughout the nine-day observational campaign. Using 40 ks contiguous spectra derived from the original observations, we investigate the variability of emission line parameters and ratios. Several emission lines are shown to be variable, including S XV, Si XIII, and Ne IX. For the first time, variations of the X-ray emission line widths as a function of the binary phase are found in a binary system, with the smallest widths at phi = 0.0 when the secondary delta Ori Aa2 is at the inferior conjunction. Using 3D hydrodynamic modeling of the interacting winds, we relate the emission line width variability to the presence of a wind cavity created by a wind-wind collision, which is effectively void of embedded wind shocks and is carved out of the X-ray-producing primary wind, thus producing phase-locked X-ray variability. C1 [Nichols, J.; Lauer, J.; Evans, N. R.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Huenemoerder, D. P.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Corcoran, M. F.; Hamaguchi, K.] NASA GSFC, CRESST, Greenbelt, MD 20771 USA. [Corcoran, M. F.; Hamaguchi, K.] NASA GSFC, XRay Astrophys Lab, Greenbelt, MD 20771 USA. [Waldron, W.] Univ Space Res Assoc, Columbia, MD 21046 USA. [Naze, Y.] Eureka Sci Inc, Oakland, CA 94602 USA. [Pollock, A. M. T.] Univ Liege, FNRS Dept AGO, B-4000 Liege, Belgium. [Moffat, A. F. J.; Richardson, N. D.; Pablo, H.] European Space Agcy, XMM Newton Sci Operat Ctr, European Space Astron Ctr, E-28691 Villanueva De La Canada, Spain. [Shenar, T.; Hamann, W. -R.; Oskinova, L.] Univ Montreal, Dept Phys, Montreal, PQ H3C 3J7, Canada. [Hamaguchi, K.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Gull, T.] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. [Ignace, R.] NASA GSFC, Greenbelt, MD 20771 USA. [Hoffman, Jennifer L.] E Tennessee State Univ, Phys & Astron, Johnson City, TN 37614 USA. [Hole, K. T.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Lomax, J. R.] Weber State Univ, Dept Phys, Ogden, UT 84408 USA. [Russell, C. M. P.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Russell, C. M. P.] NASA Goddard Space Flight Ctr, Xray Astrophys Lab, Greenbelt, MD 20771 USA. Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. RP Nichols, J (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. FU National Aeronautics and Space Administration through Chandra Award [GO3-14015A, G03-14015E, GO3-14015G]; National Aeronautics Space Administration [NAS8-03060]; NASA through the Smithsonian Astrophysical Observatory [SV3-73016]; Fonds National de la Recherche Scientifique (Belgium); Communaute Francaise de Belgique; PRODEX XMM and Integral contracts; Action de Recherche Concertee (CFWB-Academie Wallonie Europe); NSRC (Canada); FRQNT (Quebec); CRAQ (Centre de Recherche en Astrophysique du Quebec) fellowship; DLR [50 OR 1302]; Chandra X-ray Center NASA [NAS8-03060]; NASA [NNX13AF40G]; NSF [AST-0807477] FX The authors acknowledge the constructive comments of the anomymous referee. M.F.C., J.S.N., W.L.W., C.M.P.R., and K.H. are grateful for support provided by the National Aeronautics and Space Administration through Chandra Award Number GO3-14015A, G03-14015E, and GO3-14015G issued by the Chandra X-ray Observatory Center, which is operated by the Smithsonian Astrophysical Observatory for and on behalf of the National Aeronautics Space Administration under contract NAS8-03060. D.P.H. was supported by NASA through the Smithsonian Astrophysical Observatory contract SV3-73016 to MIT for the Chandra X-ray Center and Science Instruments. Y.N. acknowledges support from the Fonds National de la Recherche Scientifique (Belgium), the Communaute Francaise de Belgique, the PRODEX XMM and Integral contracts, and the Action de Recherche Concertee (CFWB-Academie Wallonie Europe). A.F.J.M. is grateful for financial aid from NSRC (Canada) and FRQNT (Quebec). N.D.R. gratefully acknowledges his CRAQ (Centre de Recherche en Astrophysique du Quebec) fellowship. L.M.O. acknowledges support from DLR grant 50 OR 1302. N.R.E. is grateful for support from the Chandra X-ray Center NASA Contract NAS8-03060. J.L.H. acknowledges support from NASA award NNX13AF40G and NSF award AST-0807477. M.F.C., J.S.N., and K.H. also acknowledge helpful discussions with John Houck and Michael Nowak on data analysis with ISIS, and Craig Anderson for technical support. This research has made use of data and/or software provided by the High Energy Astrophysics Science Archive Research Center (HEASARC), which is a service of the Astrophysics Science Division at NASA/GSFC and the High Energy Astrophysics Division of the Smithsonian Astrophysical Observatory. This research made use of the Chandra Transmission Grating Catalog and archive (http://tgcat.mit.edu). This research also has made use of NASA's Astrophysics Data System. NR 80 TC 5 Z9 5 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 133 DI 10.1088/0004-637X/809/2/133 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100026 ER PT J AU Pablo, H Richardson, ND Moffat, AFJ Corcoran, M Shenar, T Benvenuto, O Fuller, J Naze, Y Hoffman, JL Miroshnichenko, A Apellaniz, JM Evans, N Eversberg, T Gayley, K Gull, T Hamaguchi, K Hamann, WR Henrichs, H Hole, T Ignace, R Iping, R Lauer, J Leutenegger, M Lomax, J Nichols, J Oskinova, L Owocki, S Pollock, A Russell, CMP Waldron, W Buil, C Garrel, T Graham, K Heathcote, B Lemoult, T Li, D Mauclaire, B Potter, M Ribeiro, J Matthews, J Cameron, C Guenther, D Kuschnig, R Rowe, J Rucinski, S Sasselov, D Weiss, W AF Pablo, Herbert Richardson, Noel D. Moffat, Anthony F. J. Corcoran, Michael Shenar, Tomer Benvenuto, Omar Fuller, Jim Naze, Yael Hoffman, Jennifer L. Miroshnichenko, Anatoly Apellaniz, Jesus Maiz Evans, Nancy Eversberg, Thomas Gayley, Ken Gull, Ted Hamaguchi, Kenji Hamann, Wolf-Rainer Henrichs, Huib Hole, Tabetha Ignace, Richard Iping, Rosina Lauer, Jennifer Leutenegger, Maurice Lomax, Jamie Nichols, Joy Oskinova, Lida Owocki, Stan Pollock, Andy Russell, Christopher M. P. Waldron, Wayne Buil, Christian Garrel, Thierry Graham, Keith Heathcote, Bernard Lemoult, Thierry Li, Dong Mauclaire, Benjamin Potter, Mike Ribeiro, Jose Matthews, Jaymie Cameron, Chris Guenther, David Kuschnig, Rainer Rowe, Jason Rucinski, Slavek Sasselov, Dimitar Weiss, Werner TI A COORDINATED X-RAY AND OPTICAL CAMPAIGN OF THE NEAREST MASSIVE ECLIPSING BINARY, delta ORIONIS Aa. III. ANALYSIS OF OPTICAL PHOTOMETRIC (MOST) AND SPECTROSCOPIC (GROUND BASED) VARIATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: close; binaries: eclipsing; stars: early-type; stars: individual (delta Ori A); stars: mass-loss; stars: variables: general ID APSIDAL MOTION; STARS; SYSTEM; PULSATIONS; KOI-54; SPECTRA; ORBITS; SPOTS; ORI AB We report on both high-precision photometry from the Microvariability and Oscillations of Stars (MOST) space telescope and ground-based spectroscopy of the triple system delta Ori A, consisting of a binary O9.5II+early-B (Aa1 and Aa2) with P = 5.7 days, and a more distant tertiary (O9 IV P > 400 years). This data was collected in concert with X-ray spectroscopy from the Chandra X-ray Observatory. Thanks to continuous coverage for three weeks, the MOST light curve reveals clear eclipses between Aa1 and Aa2 for the first time in non-phased data. From the spectroscopy, we have a well-constrained radial velocity (RV) curve of Aa1. While we are unable to recover RV variations of the secondary star, we are able to constrain several fundamental parameters of this system and determine an approximate mass of the primary using apsidal motion. We also detected second order modulations at 12 separate frequencies with spacings indicative of tidally influenced oscillations. These spacings have never been seen in a massive binary, making this system one of only a handful of such binaries that show evidence for tidally induced pulsations. C1 [Pablo, Herbert; Richardson, Noel D.; Moffat, Anthony F. J.] Univ Montreal, Dept Phys, Montreal, PQ H3C 3J7, Canada. [Pablo, Herbert; Richardson, Noel D.; Moffat, Anthony F. J.] Univ Montreal, CRAQ, Montreal, PQ H3C 3J7, Canada. [Corcoran, Michael; Hamaguchi, Kenji] NASA GSFC, CRESST, Greenbelt, MD 20771 USA. [Corcoran, Michael; Hamaguchi, Kenji] NASA GSFC, Xray Astrophys Lab, Greenbelt, MD 20771 USA. [Corcoran, Michael; Iping, Rosina] Univ Space Res Assoc, Columbia, MD 21046 USA. [Shenar, Tomer; Hamann, Wolf-Rainer; Oskinova, Lida] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Benvenuto, Omar] Univ Nacl La Plata, Fac Ciencias Astron & Geofis, RA-1900 Buenos Aires, DF, Argentina. [Benvenuto, Omar] UNLP, CONICET, CCT, IALP, La Plata, Buenos Aires, Argentina. [Fuller, Jim] CALTECH, Walter Burke Inst Theoret Phys, TAPIR, Pasadena, CA 91125 USA. [Fuller, Jim; Leutenegger, Maurice] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Naze, Yael] Univ Liege, FNRS Dept AGO, B-4000 Liege, Belgium. [Hoffman, Jennifer L.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Miroshnichenko, Anatoly] Univ N Carolina, Dept Phys & Astron, Greensboro, NC 27402 USA. [Apellaniz, Jesus Maiz] Ctr Astrobiol CSIC INTA, E-28691 Villanueva De La Caada, Spain. [Evans, Nancy; Lauer, Jennifer; Nichols, Joy] Smithsonian Astrophys Observ, Cambridge, MA 02138 USA. [Eversberg, Thomas] Schnorringen Telescope Sci Inst, Waldbrol, Germany. [Gayley, Ken] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Gull, Ted] NASA Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Henrichs, Huib] Univ Amsterdam, Astron Inst Anton Pannekoek, NL-1098 XH Amsterdam, Netherlands. [Hole, Tabetha; Ignace, Richard] E Tennessee State Univ, Dept Phys & Astron, Johnson City, TN 37614 USA. [Lomax, Jamie] Univ Oklahoma, HL Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Owocki, Stan] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Pollock, Andy] European Space Agcy, E-28691 Madrid, Spain. [Russell, Christopher M. P.] NASA Goddard Space Flight Ctr, Xray Astrophys Lab, Greenbelt, MD 20771 USA. [Russell, Christopher M. P.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Waldron, Wayne] Eureka Sci Inc, Oakland, CA 94602 USA. [Buil, Christian] Castanet Tolosan Observ, F-31320 Castanet Tolosan, France. [Garrel, Thierry] Observ Juvignac, F-34990 Juvignac, France. [Heathcote, Bernard] Barfold Observ, Glenhope, Vic 3444, Australia. [Lemoult, Thierry] Chelles Observ, F-77500 Chelles, France. [Li, Dong] Jade Observ, Tianjin 300251, Peoples R China. [Mauclaire, Benjamin] Observ Val Arc, F-13530 Trets, France. [Ribeiro, Jose] Observ Inst Geog Exercito, Lisbon, Portugal. [Matthews, Jaymie; Kuschnig, Rainer] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Cameron, Chris] Cape Breton Univ, Dept Math Phys & Geol, Sydney, NS B1P 6L2, Canada. [Guenther, David] St Marys Univ, Inst Computat Astrophys, Dept Phys & Astron, Halifax, NS B3H 3C3, Canada. [Kuschnig, Rainer] Univ Vienna, Inst Astron, A-1180 Vienna, Austria. [Rowe, Jason] NASA Ames Res Ctr, Moffett Field, CA 94035 USA. [Rucinski, Slavek] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Sasselov, Dimitar] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. RP Pablo, H (reprint author), Univ Montreal, Dept Phys, CP 6128,Succ Ctr Ville, Montreal, PQ H3C 3J7, Canada. EM hpablo@astro.umontreal.ca; richardson@astro.umontreal.ca FU Chandra grant [GO3-14015A, GO3-14015E]; Fonds National de la Recherche Scientifique (Belgium); Communaute Francaise de Belgique; PRODEX XMMAction de Recherche Concertee (CFWB-Academie Wallonie Europe); CRAQ (Centre de Recherche en Astrophysique du Quebec); Spanish Government Ministerio de Economia y Competitividad (MINECO) [AYA2010-15 081, AYA2010-17 631, AYA2013-40 611-P]; Consejeria de Educacion of the Junta de Andalucia [P08-TIC-4075]; Austrian Science Fund (FWF); Chandra X-ray Center NASA [NAS8-03060]; NASA [NNX13AF40G]; NSF [AST-0807477] FX M.F.C., J.S.N., W.L.W., and K.H. are grateful for support via Chandra grant GO3-14015A and GO3-14015E. Y.N. acknowledges support from the Fonds National de la Recherche Scientifique (Belgium), the Communaute Francaise de Belgique, the PRODEX XMM and Integral contracts, and the Action de Recherche Concertee (CFWB-Academie Wallonie Europe). N.D.R. gratefully acknowledges his CRAQ (Centre de Recherche en Astrophysique du Quebec) fellowship. A.F.J.M., D.B.G., J.M.M., and S.M.R. are grateful for financial aid to NSERC (Canada). A.F.J.M. and H.P. also thank FRQNT (Quebec) and the Canadian Space Agency. J.M.A. acknowledges support from (a) the Spanish Government Ministerio de Economia y Competitividad (MINECO) through grants AYA2010-15 081, AYA2010-17 631, and AYA2013-40 611-P and (b) the Consejeria de Educacion of the Junta de Andalucia through grant P08-TIC-4075. R.K. and W.W. acknowledge support by the Austrian Science Fund (FWF). N.R.E. is grateful for support from the Chandra X-ray Center NASA Contract NAS8-03060. J.L.H. acknowledges support from NASA award NNX13AF40G and NSF award AST-0807477. NR 61 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 134 DI 10.1088/0004-637X/809/2/134 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100027 ER PT J AU Webb, T Noble, A DeGroot, A Wilson, G Muzzin, A Bonaventura, N Cooper, M Delahaye, A Foltz, R Lidman, C Surace, J Yee, HKC Chapman, S Dunne, L Geach, J Hayden, B Hildebrandt, H Huang, JS Pope, A Smith, MWL Perlmutter, S Tudorica, A AF Webb, Tracy Noble, Allison DeGroot, Andrew Wilson, Gillian Muzzin, Adam Bonaventura, Nina Cooper, Mike Delahaye, Anna Foltz, Ryan Lidman, Chris Surace, Jason Yee, H. K. C. Chapman, Scott Dunne, Loretta Geach, James Hayden, Brian Hildebrandt, Hendrik Huang, Jiasheng Pope, Alexandra Smith, Matthew W. L. Perlmutter, Saul Tudorica, Alex TI AN EXTREME STARBURST IN THE CORE OF A RICH GALAXY CLUSTER AT z=1.7 SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: clusters: general; galaxies: evolution; galaxies: interactions; galaxies: starburst ID ACTIVE GALACTIC NUCLEI; NEAR-INFRARED PROPERTIES; STAR-FORMATION ACTIVITY; WIDE-FIELD CAMERA; SPECTROSCOPIC CONFIRMATION; COOLING FLOWS; STELLAR MASS; X-RAY; EXTRAGALACTIC SURVEY; PHOTOMETRIC SYSTEM AB We have discovered an optically rich galaxy cluster at z = 1.7089 with star formation occurring in close proximity to the central galaxy. The system, SpARCS104922.6+ 564032.5, was detected within the Spitzer Adaptation of the red-sequence Cluster Survey, and confirmed through Keck-MOSFIRE spectroscopy. The rest-frame optical richness of N-gal (500 kpc) = 30 +/- 8 implies a total halo mass, within 500 kpc, of similar to 3.8 +/- 1.2 x 10(14) M-circle dot, comparable to other clusters at or above this redshift. There is a wealth of ancillary data available, including Canada-France-Hawaii Telescope optical, UKIRT-K, Spitzer-IRAC/MIPS, and Herschel-SPIRE. This work adds submillimeter imaging with the SCUBA2 camera on the James Clerk Maxwell Telescope and near-infrared imaging with the Hubble Space Telescope. The mid/far-infrared (M/FIR) data detect an Ultra-luminous Infrared Galaxy spatially coincident with the central galaxy, with L-IR = 6.2 +/- 0.9 x 10(12) L-circle dot. The detection of polycyclic aromatic hydrocarbons at z = 1.7 in a Spitzer-IRS spectrum of the source implies the FIR luminosity is dominated by star formation (an Active Galactic Nucleus contribution of 20%) with a rate of similar to 860 +/- 130 M-circle dot yr(-1). The optical source corresponding to the IR emission is likely a chain of > 10 individual clumps arranged as " beads on a string" over a linear scale of 66 kpc. Its morphology and proximity to the Brightest Cluster Galaxy (BCG) imply a gas-rich interaction at the center of the cluster triggered the star formation. This system indicates that wet mergers may be an important process in forming the stellar mass of BCGs at early times. C1 [Webb, Tracy; Bonaventura, Nina; Delahaye, Anna] McGill Univ, Dept Phys, Montreal, PQ H3P 1T3, Canada. [Noble, Allison; Yee, H. K. C.] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [DeGroot, Andrew; Wilson, Gillian; Foltz, Ryan] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. [Muzzin, Adam; Chapman, Scott] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Cooper, Mike] Univ Calif Irvine, Ctr Galaxy Evolut, Dept Phys & Astron, Irvine, CA 92697 USA. [Lidman, Chris] Australian Astron Observ, N Ryde, NSW 1670, Australia. [Surace, Jason] CALTECH, Spitzer Space Sci Ctr, Pasadena, CA 91125 USA. [Chapman, Scott] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 2R4, Canada. [Dunne, Loretta] Univ Canterbury, Dept Phys & Astron, Christchurch 8140, New Zealand. [Dunne, Loretta] Univ Edinburgh, Insitute Astron, Royal Observ, Edinburgh EH9 3HJ, Midlothian, Scotland. [Geach, James] Univ Hertfordshire, Sci & Technol Res Inst, Ctr Astrophys Res, Hatfield AL10 9AB, Herts, England. [Hayden, Brian; Perlmutter, Saul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Hildebrandt, Hendrik; Tudorica, Alex] Argelander Inst Astron, D-53121 Bonn, Germany. [Huang, Jiasheng] Chinese Acad Sci, Natl Astron Observ China, Beijing 100012, Peoples R China. [Huang, Jiasheng] Chinese Acad Sci, China Chile Joint Ctr Astron, Santiago 1515, Chile. [Huang, Jiasheng] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Pope, Alexandra] Univ Massachusetts, Dept Astron, Amherst, MA 01100 USA. [Smith, Matthew W. L.] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3AA, S Glam, Wales. [Perlmutter, Saul] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Webb, T (reprint author), McGill Univ, Dept Phys, 3600 Rue Univ, Montreal, PQ H3P 1T3, Canada. FU W. M. Keck Foundation; NASA [NAS 5-26555]; US Department of Energy, Office of Science, Office of High Energy Physics [AC02-05CH11231]; European Research Council; NSERC; NASA from the Space Telescope Science Institute [GO-13306, GO-13677, GO-13747, GO-13845, GO-14327] FX Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W. M. Keck Foundation. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. Financial support for this work was provided by NASA through program GO-13677 from the Space Telescope Science Institute, which is operated by AURA, Inc., under NASA contract NAS 5-26555. This material is based upon work supported in part by the US Department of Energy, Office of Science, Office of High Energy Physics, under contract No. AC02-05CH11231. This work is based in part on observations made with the Spitzer Space Telescope, which is operated by the Jet Propulsion Laboratory, California Institute of Technology under a contract with NASA. L.D. acknowledges support from European Research Council Advanced Grant: cosmicism. T.M.A.W. acknowledges the support of an NSERC Discovery Grant. Financial support for this work was provided by NASA through programs GO-13306, GO-13677, GO-13747, GO-13845, and GO-14327 from the Space Telescope Science Institute, which is operated by AURA, Inc., under NASA contract NAS 5-26555. NR 84 TC 11 Z9 11 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2015 VL 809 IS 2 AR 173 DI 10.1088/0004-637X/809/2/173 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9EC UT WOS:000361655100066 ER PT J AU Barajas, JF Phelan, RM Schaub, AJ Kliewer, JT Kelly, PJ Jackson, DR Luo, R Keasling, JD Tsai, SC AF Barajas, Jesus F. Phelan, Ryan M. Schaub, Andrew J. Kliewer, Jaclyn T. Kelly, Peter J. Jackson, David R. Luo, Ray Keasling, Jay D. Tsai, Shiou-Chuan TI Comprehensive Structural and Biochemical Analysis of the Terminal Myxalamid Reductase Domain for the Engineered Production of Primary Alcohols SO CHEMISTRY & BIOLOGY LA English DT Article ID NONRIBOSOMAL PEPTIDE SYNTHETASES; POLYKETIDE BIOSYNTHESIS; GENE-CLUSTER; FORCE-FIELD; PROTEIN; AMBER; CLASSIFICATION; ANTIBIOTICS; PERFORMANCE; PREDICTION AB The terminal reductase (R) domain from the non-ribosomal peptide synthetase (NRPS) module MxaA in Stigmatella aurantiaca Sga15 catalyzes a non-processive four-electron reduction to produce the myxalamide family of secondary metabolites. Despite widespread use in nature, a lack of structural and mechanistic information concerning reductive release from polyketide synthase (PKS) and NRPS assembly lines principally limits our ability to redesign R domains with altered or improved activity. Here we report crystal structures for MxaA R, both in the absence and, for the first time, in the presence of the NADPH cofactor. Molecular dynamics simulations were employed to provide a deeper understanding of this domain and further identify residues critical for structural integrity, substrate binding, and catalysis. Aggregate computational and structural findings provided a basis for mechanistic investigations and, in the process, delivered a rationally altered variant with improved activity toward highly reduced substrates. C1 [Barajas, Jesus F.; Schaub, Andrew J.; Kliewer, Jaclyn T.; Kelly, Peter J.; Jackson, David R.; Luo, Ray; Tsai, Shiou-Chuan] Univ Calif Irvine, Dept Mol Biol & Biochem Chem & Pharmaceut, Irvine, CA 92697 USA. [Phelan, Ryan M.; Keasling, Jay D.] Joint Bioenergy Inst, Emeryville, CA 94608 USA. [Phelan, Ryan M.; Keasling, Jay D.] Univ Calif Berkeley, Inst QB3, Berkeley, CA 94270 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Joint Bioenergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. EM keasling@berkeley.edu; sctsai@uci.edu RI Luo, Ray/I-6928-2012; OI Luo, Ray/0000-0002-6346-8271; Schaub, Andrew/0000-0001-7770-7045 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; National Science Foundation [CBET-1437775]; Pew Foundation [ES001670] FX We would like to acknowledge Benjamin Adler for assistance with the biochemical assay of the MxaA didomain. We would also like to thank Dr. Gaurav Shakya for his insights in chemistry and Dr. P. Adams, C. Petzold, and L. Chan for assistance with the LC-MS/MS assay. This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. In addition, R.M.P. and J.D.K. would like to acknowledge the National Science Foundation for support through the Catalysis and Biocatalysis Program (CBET-1437775). A portion of this work was supported by grant ES001670 by the Pew Foundation. Crystallographic studies were performed at the Stanford Synchrotron Radiation Laboratory, a national user facility by Stanford University on behalf of the US Department of Energy Office of Basic Energy Sciences and the Advance Light Source at the Lawrence Berkeley National Laboratory. J.D.K. has financial interests in Amyris, LS9, and Lygos. NR 56 TC 9 Z9 9 U1 3 U2 16 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1074-5521 EI 1879-1301 J9 CHEM BIOL JI Chem. Biol. PD AUG 20 PY 2015 VL 22 IS 8 BP 1018 EP 1029 DI 10.1016/j.chembiol.2015.06.022 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CS2DY UT WOS:000361879200008 PM 26235055 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelmanl, J Adomeitl, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzil, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansi, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillaril, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldusm, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemsterl, LJ Beermann, TA Bege, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Bergel, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Berniusll, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbinkl, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosmanu, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bresser, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronnerl, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanesm, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Buttil, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calafiura, P Calandri, A Calderini, G Calfayanl, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Caste, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmorell, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Cher, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chu, ML Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Colel, S Colijnl, AP Collot, J Colombo, T Compostellal, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM 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M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Delucal, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeckl, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W 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Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for production of vector-like quark pairs and of four top quarks in the lepton-plus-jets final state in pp collisions at root 8=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID MODEL HIGGS-BOSON; STANDARD MODEL; ROOT-S=7 TEV; PARTON DISTRIBUTIONS; HADRONIC COLLISIONS; SYMMETRY-BREAKING; MATRIX-ELEMENTS; MONTE-CARLO; LHC; NLO AB A search for pair production of vector-like quarks, both up-type (T) and down-type (B), as well as for four-top-quark production, is presented. The search is based on pp collisions at TeV recorded in 2012 with the ATLAS detector at the CERN Large Hadron Collider and corresponding to an integrated luminosity of 20.3 fb(-1). Data are analysed in the lepton-plus-jets final state, characterised by an isolated electron or muon with high transverse momentum, large missing transverse momentum and multiple jets. Dedicated analyses are performed targeting three cases: a T quark with significant branching ratio to a W boson and a b-quark , and both a T quark and a B quark with significant branching ratio to a Higgs boson and a third-generation quark ( respectively). No significant excess of events above the Standard Model expectation is observed, and 95% CL lower limits are derived on the masses of the vector-like T and B quarks under several branching ratio hypotheses assuming contributions from T -> Wb, Zt, Ht and B -> Wt, Zb, Hb decays. The 95% CL observed lower limits on the T quark mass range between 715 GeV and 950 GeV for all possible values of the branching ratios into the three decay modes, and are the most stringent constraints to date. Additionally, the most restrictive upper bounds on four-top-quark production are set in a number of new physics scenarios. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Bruckman de Renstrom, P. A.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proiss, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Grarnling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nada, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, IN2P3, CNRS, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inarnaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Jinnouchi, O.; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Novgorodova, O.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewel, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewel, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Puesche, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantife, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeitl, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayanl, P.; Chow, B. K. B.; Duckeckl, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Leggerl, F.; Lorenz, J.; Loesel, P. J.; Maierl, T.; Mann, A.; Mehlhase, S.; Meineckl, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemannl, T.; Rauscherl, F.; Ruschkel, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillaril, T.; Bethke, S.; Bronnerl, J.; Compostellal, G.; Cortianal, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Incel, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nage, M.; Nisiusl, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst Phys, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvajl, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvajl, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthautl, F.; Galea, C.; Konig, A. C.; Nektarijevicl, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzil, I.; Beemsterl, L. J.; Bentvelsen, S.; Bergel, D.; Bobbinkl, G. J.; Bos, K.; Brenner, L.; Buttil, P.; Caste, A.; Colijnl, A. P.; de Jong, P.; De Nooijl, L.; Deigaardl, I.; Delucal, C.; Ferraril, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkinal, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedtl, J.; Meyerl, J.; Oussorenl, K. P.; Sabatol, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzil, I.; Beemsterl, L. J.; Bentvelsen, S.; Bergel, D.; Bobbinkl, G. J.; Bos, K.; Brenner, L.; Buttil, P.; Caste, A.; Colijnl, A. P.; de Jong, P.; De Nooijl, L.; Deigaardl, I.; Delucal, C.; Ferraril, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkinal, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedtl, J.; Meyerl, J.; Oussorenl, K. P.; Sabatol, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelmanl, J.; Burghgrave, B.; Chakraborty, D.; Colel, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Berniusll, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethyll, P.; Nevesil, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Haririll, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Chaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Haririll, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Chaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] IN2P3, CNRS, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmorell, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Grarnstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickeringuo, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Bruneliere, R.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dana; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffe, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russe, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Nei, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldusm, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Ner, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hu, C.; March, L.; Mellado Garcia, B. R.; Ruan, X.] Univ Witwatersrand, ZA-2050 Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Pucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Pucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Cher, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Cher, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. 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[Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sack ler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. 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[Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Tries; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Tries; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Tries; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Tries; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. 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L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fac Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riege, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Idea, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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RI Chekulaev, Sergey/O-1145-2015; Ciubancan, Liviu Mihai/L-2412-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Boldyrev, Alexey/M-9684-2015; Tikhomirov, Vladimir/M-6194-2015; Negrini, Matteo/C-8906-2014; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011 OI Ciubancan, Liviu Mihai/0000-0003-1837-2841; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Negrini, Matteo/0000-0003-0101-6963; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; FU Science and Technology Facilities Council [ST/J501074/1, ST/K001388/1, ST/K50208X/1, ST/M000664/1, ST/M503575/1] NR 132 TC 20 Z9 20 U1 9 U2 69 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 20 PY 2015 IS 8 AR 105 DI 10.1007/JHEP08(2015)105 PG 86 WC Physics, Particles & Fields SC Physics GA CQ2CX UT WOS:000360408100001 ER PT J AU Rubenchik, A Wu, S Mitchell, S Golosker, I Leblanc, M Peterson, N AF Rubenchik, A. Wu, S. Mitchell, S. Golosker, I. Leblanc, M. Peterson, N. TI Direct measurements of temperature-dependent laser absorptivity of metal powders SO APPLIED OPTICS LA English DT Article ID IRRADIATION AB A compact system is developed to measure laser absorptivity for a variety of powder materials (metals, ceramics, etc.) with different powder size distributions and thicknesses. The measured results for several metal powders are presented. The results are consistent with those from ray tracing calculations. (C) 2015 Optical Society of America C1 [Rubenchik, A.; Wu, S.; Mitchell, S.; Golosker, I.; Leblanc, M.; Peterson, N.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Wu, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM wu31@llnl.gov FU Laboratory Directed Research and Development [13-SI-002, 15-ERD-037]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Laboratory Directed Research and Development (13-SI-002, 15-ERD-037); Lawrence Livermore National Laboratory (DE-AC52-07NA27344). NR 9 TC 5 Z9 5 U1 1 U2 13 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD AUG 20 PY 2015 VL 54 IS 24 BP 7230 EP 7233 DI 10.1364/AO.54.007230 PG 4 WC Optics SC Optics GA CP9CB UT WOS:000360190200013 PM 26368757 ER PT J AU Li, ZL Bansal, N Azarpira, A Bhalla, A Chen, CH Ralph, J Hegg, EL Hodge, DB AF Li, Zhenglun Bansal, Namita Azarpira, Ali Bhalla, Aditya Chen, Charles H. Ralph, John Hegg, Eric L. Hodge, David B. TI Chemical and structural changes associated with Cu-catalyzed alkaline-oxidative delignification of hybrid poplar SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Plant cell walls; Pretreatment; Catalytic oxidation; Lignin; Alkaline hydrogen peroxide (AHP) pretreatment; NMR spectroscopy; Electron microscopy ID STATE 2D NMR; HYDROGEN-PEROXIDE; CELL-WALL; DILUTE-ACID; ENZYMATIC-HYDROLYSIS; WOOD-PULP; LIGNIN; PRETREATMENT; OXYGEN; COMPLEXES AB Background: Alkaline hydrogen peroxide pretreatment catalyzed by Cu(II) 2,2'-bipyridine complexes has previously been determined to substantially improve the enzymatic hydrolysis of woody plants including hybrid poplar as a consequence of moderate delignification. In the present work, cell wall morphological and lignin structural changes were characterized for this pretreatment approach to gain insights into pretreatment outcomes and, specifically, to identify the extent and nature of lignin modification. Results: Through TEM imaging, this catalytic oxidation process was shown to disrupt cell wall layers in hybrid poplar. Cu-containing nanoparticles, primarily in the Cu(I) oxidation state, co-localized with the disrupted regions, providing indirect evidence of catalytic activity whereby soluble Cu(II) complexes are reduced and precipitated during pretreatment. The concentration of alkali-soluble polymeric and oligomeric lignin was substantially higher for the Cu-catalyzed oxidative pretreatment. This alkali-soluble lignin content increased with time during the catalytic oxidation process, although the molecular weight distributions were unaltered. Yields of aromatic monomers (including phenolic acids and aldehydes) were found to be less than 0.2 % (wt/wt) on lignin. Oxidation of the benzylic alcohol in the lignin side-chain was evident in NMR spectra of the solubilized lignin, whereas minimal changes were observed for the pretreatment-insoluble lignin. Conclusions: These results provide indirect evidence for catalytic activity within the cell wall. The low yields of lignin-derived aromatic monomers, together with the detailed characterization of the pretreatment-soluble and pretreatment-insoluble lignins, indicate that the majority of both lignin pools remained relatively unmodified. As such, the lignins resulting from this process retain features closely resembling native lignins and may, therefore, be amenable to subsequent valorization. C1 [Li, Zhenglun; Chen, Charles H.; Hodge, David B.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Li, Zhenglun; Bansal, Namita; Bhalla, Aditya; Hegg, Eric L.; Hodge, David B.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Bansal, Namita; Bhalla, Aditya; Hegg, Eric L.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Azarpira, Ali; Ralph, John] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Ralph, John] Univ Wisconsin, Dept Biochem, Madison, WI 53705 USA. [Hodge, David B.] Michigan State Univ, Dept Biosyst & Agr Engn, E Lansing, MI 48824 USA. [Hodge, David B.] Lulea Univ Technol, Div Sustainable Proc Engn, S-95187 Lulea, Sweden. RP Hegg, EL (reprint author), Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. EM erichegg@msu.edu; hodgeda@egr.msu.edu RI BHALLA, ADITYA/Q-2792-2015 OI BHALLA, ADITYA/0000-0003-3462-9600 FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; Northeast Sun Grant Initiative FX The authors would like to acknowledge Prof. Daniel Jones (MSU Department of Biochemistry and Molecular Biology) and the MSU Mass Spectrometry core facility for providing assistance in the analysis of aromatic monomers. This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494). Aditya Bhalla was also supported in part by funding from the Northeast Sun Grant Initiative. NR 72 TC 2 Z9 2 U1 6 U2 21 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 20 PY 2015 VL 8 AR 123 DI 10.1186/s13068-015-0300-5 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CP8AR UT WOS:000360113200001 PM 26300970 ER PT J AU Hajer, J Ismail, A Kling, F Li, YY Liu, T Su, SF AF Hajer, Jan Ismail, Ahmed Kling, Felix Li, Ying-Ying Liu, Tao Su, Shufang TI Searches for non-SM heavy Higgses at a 100 TeV pp collider SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Article ID STANDARD MODEL; ATLAS DETECTOR; BOSON; LHC; SUPERSYMMETRY; COLLISIONS; PARTICLE; PHYSICS; MASS AB In this write-up, we summarize the production of non-SM Higgses in the Type II Two Higgs Doublet Model at a 100 TeV pp collider, as well as their decays. We present the reach for pp -> bbH(0)/A -> bbtt, bb tau tau as well as pp -> tbH(+/-) -> tbtb, tb tau nu at the 100 TeV pp collider and outline the possible search channels via Higgs exotic decays. We point out that a combination of these conventional channels potentially yields full coverage for tan beta and pushes the exclusion limits from the O(1)TeV at the LHC to the O(10)TeV at a 100 TeV pp collider, whereas the exotic decays of a heavy Higgs into two light Higgses or one light Higgs plus one SM gauge boson provide alternative discovery channels. C1 [Hajer, Jan; Li, Ying-Ying; Liu, Tao] Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Hajer, Jan] Hong Kong Univ Sci & Technol, Jockey Club Inst Adv Study, Hong Kong, Hong Kong, Peoples R China. [Ismail, Ahmed] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Ismail, Ahmed] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Kling, Felix; Su, Shufang] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. RP Hajer, J (reprint author), Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. EM jan.hajer@ust.hk; aismail@anl.gov; kling@email.arizona.edu; ylict@connect.ust.hk; taoliu@ust.hk; shufang@email.arizona.edu FU Department of Energy [DE-AC02-06CH11357, DE-FG02-12ER41811, DH-FG02-13E1141976]; Hong Kong University of Science and Technology; Hong Kong PhD Fellowship Scheme (HKPFS) FX We would like to thank Tilman Plehn for fruitful discussion. A. I. is supported by the Department of Energy under Grant DE-AC02-06CH11357 and DE-FG02-12ER41811. F. K. and S. S. are supported by the Department of Energy under Grant DH-FG02-13E1141976. T. L. and J. S. are supported by fund at the Hong Kong University of Science and Technology. Y. L. is supported by the the Hong Kong PhD Fellowship Scheme (HKPFS) issued by the Research Grants Council (RGC) of Hong Kong. Y. L., T. L. and S. S. also would like to acknowledge the hospitality of the Jockey Club Institute for Advanced Study, HKUST, where part of this work was completed. NR 52 TC 3 Z9 3 U1 0 U2 4 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD AUG 20 PY 2015 VL 30 IS 23 SI SI AR 1544005 DI 10.1142/S0217751X15440054 PG 12 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CP7NB UT WOS:000360073800006 ER PT J AU Hinchliffe, I Kotwal, A Mangano, ML Quigg, C Wang, LT AF Hinchliffe, Ian Kotwal, Ashutosh Mangano, Michelangelo L. Quigg, Chris Wang, Lian-Tao TI Luminosity goals for a 100-TeV pp collider SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Article ID PHYSICS AB We consider diverse examples of science goals that provide a framework to assess luminosity goals for a future 100-TeV proton-proton collider. C1 [Hinchliffe, Ian] Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Kotwal, Ashutosh] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Kotwal, Ashutosh] Duke Univ, Durham, NC 27708 USA. [Mangano, Michelangelo L.] CERN, TH Unit, PH Dept, CH-1211 Geneva 23, Switzerland. [Quigg, Chris] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Quigg, Chris] Ecole Normale Super, Inst Phys Theor Philippe Meyer, F-75231 Paris 05, France. [Wang, Lian-Tao] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Hinchliffe, I (reprint author), Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. EM i_hinchliffe@lbl.gov; kotwal@phy.duke.edu; michelangelomangano@cern.ch; quigg@fnal.gov; liantaow@uchicago.edu FU ERC [291377]; United States Department of Energy [DE-AC02-07CH11359]; Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This document grew out of discussions held at the Jockey Club Institute for Advanced Study of the Hong Kong University of Science and Technology, during the Programme on The future of high energy physics, January 5-30, 2015. We thank Henry Tye and members of the Institute for the hospitality, the participants for contributing to a stimulating environment, and Prudence Wong for helpful practical assistance. In particular, we acknowledge informative discussions with Stephen Gourlay, Ian Low, Vladimir Shiltsev, Dick Talman, Weiming Yao and Charlie Young, and continuous encouragement from Michael Benedikt and Weiren Chou. The work of MLM was performed in the framework of the ERC grant 291377, "LHCtheory: Theoretical predictions and analyses of LHC physics: advancing the precision frontier". Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. CQ thanks John Iliopoulos and the Fondation Meyer pour le developpement culturel et artistigue for generous hospitality. The work of IH was supported in part by the Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under contract DE-AC02-05CH11231. NR 19 TC 13 Z9 13 U1 0 U2 0 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD AUG 20 PY 2015 VL 30 IS 23 SI SI AR 1544002 DI 10.1142/S0217751X15440029 PG 13 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CP7NB UT WOS:000360073800003 ER PT J AU Shiltsev, VD AF Shiltsev, Vladimir D. TI Accelerator physics and technology challenges of very high energy hadron colliders SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Article DE Colliders; accelerators; Tevatron ID PARTICLE COLLIDERS; SCIENCE AB High energy hadron eel liders have been in the forefront of particle physics for more than three decades. Al present, international particle physics community considers several options for a 100 TeV proton-proton collider as a possible post-LHC energy frontier facility. The method of colliding beams has not fully exhausted its potential but has slowed down considerably in its progress. This paper briefly reviews the accelerator physics and technology challenges of the future very high energy eel liders and outlines the areas of required research and development towards their technical and financial feasibility. C1 US DOE, Fermi Natl Accelerator Lab, Fermi Res Alliance LLC, Batavia, IL 60510 USA. RP Shiltsev, VD (reprint author), US DOE, Fermi Natl Accelerator Lab, Fermi Res Alliance LLC, POB 500, Batavia, IL 60510 USA. EM shiltsev@fnal.gov NR 69 TC 2 Z9 2 U1 0 U2 1 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD AUG 20 PY 2015 VL 30 IS 23 SI SI AR 1544001 DI 10.1142/S0217751X15440017 PG 21 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CP7NB UT WOS:000360073800002 ER PT J AU Zhang, HZ Waychunas, GA Banfield, JF AF Zhang, Hengzhong Waychunas, Glenn A. Banfield, Jillian F. TI Molecular Dynamics Simulation Study of the Early Stages of Nucleation of Iron Oxyhydroxide Nanoparticles in Aqueous Solutions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID RAY ABSORPTION-SPECTROSCOPY; TRANSITION-METAL IONS; HYDROLYSIS PRODUCTS; HYDRATION SHELLS; WATER EXCHANGE; IRON(III); COMPLEXES; CLUSTERS; CRYSTALLIZATION; POTENTIALS AB Nucleation is a fundamental step in crystal growth. Of environmental and materials relevance are reactions that lead to nucleation of iron oxyhydroxides in aqueous solutions. These reactions are difficult to study experimentally due to their rapid kinetics. Here, we used classical molecular dynamics, simulations to investigate nucleation of iron hydroxide/oxyhydroxide nanoparticles in aqueous solutions. Results show that in a solution containing ferric ions and hydroxyl groups, iron-hydroxyl molecular clusters form by merging ferric monomers, dimers, and other oligomers, driven by strong affinity of ferric ions to hydroxyls. When deprotonation reactions are not considered in the simulations, these clusters aggregate to form small iron hydroxide nanocrystals with a six-membered ring-like layered structure allomeric to gibbsite. By comparison, in a solution containing iron chloride and sodium hydroxide, the presence of chlorine drives cluster assembly along a different direction to form long molecular chains (rather than rings) composed of Fe-O octahedra linked by edge sharing. Further, in chlorine-free solutions, when deprotonation reactions are considered, the simulations predict ultimate formation of amorphous iron oxyhydroxide nanoparticles with local atomic structure similar to that of ferrihydrite nanoparticles. our simulation results reveal that nucleation of iron oxyhydroxide nanoparticles proceeds via a cluster aggregation-based nonclassical pathway. C1 [Zhang, Hengzhong; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Waychunas, Glenn A.; Banfield, Jillian F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Zhang, HZ (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. EM heng@eps.berkeley.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-AC02-05CH11231]; National Science Foundation (NSF) [CHE-1213835] FX This research was supported primarily by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under Award no. DE-AC02-05CH11231, and by the National Science Foundation (NSF), under Award no. CHE-1213835. We thank Drs. M. Zhu and B. Legg for helpful discussions. NR 45 TC 8 Z9 9 U1 10 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 20 PY 2015 VL 119 IS 33 BP 10630 EP 10642 DI 10.1021/acs.jpcb.5b03801 PG 13 WC Chemistry, Physical SC Chemistry GA CP6VN UT WOS:000360026400025 PM 26222332 ER PT J AU Zoerb, MC Henderson, JS Glover, SD Lomont, JP Nguyen, SC Hill, AD Kubiak, CP Harris, CB AF Zoerb, Matthew C. Henderson, Jane S. Glover, Starla D. Lomont, Justin P. Nguyen, Son C. Hill, Adam D. Kubiak, Clifford P. Harris, Charles B. TI Electron Dynamics and IR Peak Coalescence in Bridged Mixed Valence Dimers Studied by Ultrafast 2D-IR Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID TO-DELOCALIZED TRANSITION; TRINUCLEAR RUTHENIUM CLUSTERS; DENSITY-FUNCTIONAL THEORY; VIBRATIONAL TIME-SCALE; CHEMICAL-EXCHANGE; LINE-SHAPE; RAMAN-SPECTROSCOPY; BLOCH EQUATIONS; RADICAL-ANIONS; RATE CONSTANTS AB Dynamic IR peak coalescence and simulations based on the optical Bloch equations have been used previously to predict the rates of intramolecular electron transfer in a group of bridged mixed valence dimers of the type [Ru-3(O)(OAc)(6)(CO)L]-BL-[Ru-3(O) (OAc)(6)(CO)L]. However, limitations of the Bloch equations for the analysis of dynamical coalescence in vibrational spectra have been described. We have used ultrafast 2D-IR spectroscopy to investigate the vibrational dynamics of the CO spectator ligands of several dimers in the group. These experiments reveal that no electron site exchange occurs on the time scale required to explain the observed peak coalescence. The high variability in FTIR peak shapes for these mixed valence systems is suggested to be the result of fluctuations in the charge distributions at each metal cluster within a single-well potential energy surface, rather than the previous model of two-site exchange. C1 [Kubiak, Clifford P.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Zoerb, Matthew C.; Lomont, Justin P.; Nguyen, Son C.; Hill, Adam D.; Harris, Charles B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Harris, Charles B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Henderson, Jane S.; Glover, Starla D.; Kubiak, Clifford P.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. RP Kubiak, CP (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. EM ckubiak@ucsd.edu; cbharris@berkeley.edu FU NSF [CHE-0909632, CHE-1213135, CHE-1145893, CHE-1461632, CHE-0840505]; VIED fellowship; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX C.B.H. acknowledges support from NSF awards CHE-0909632 and CHE-1213135. C.P.K. acknowledges support from NSF awards CHE-1145893 and CHE-1461632. S.C.N. acknowledges support through a VIED fellowship. J.P.L. acknowledges support through an NSF graduate research fellowship. This research used resources of the Molecular Graphics and Computation Facility at UC Berkeley (NSF grant CHE-0840505) and the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 71 TC 1 Z9 1 U1 2 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 20 PY 2015 VL 119 IS 33 BP 10738 EP 10749 DI 10.1021/acs.jpcb.5b06734 PG 12 WC Chemistry, Physical SC Chemistry GA CP6VN UT WOS:000360026400036 PM 26204239 ER PT J AU Shard, AG Havelund, R Spencer, SJ Gilmore, IS Alexander, MR Angerer, TB Aoyagi, S Barnes, JP Benayad, A Bernasik, A Ceccone, G Counsell, JDP Deeks, C Fletcher, JS Graham, DJ Heuser, C Lee, TG Marie, C Marzec, MM Mishra, G Rading, D Renault, O Scurr, DJ Shon, HK Spampinato, V Tian, H Wang, FY Winograd, N Wu, K Wucher, A Zhou, YF Zhu, ZH AF Shard, Alexander G. Havelund, Rasmus Spencer, Steve J. Gilmore, Ian S. Alexander, Morgan R. Angerer, Tina B. Aoyagi, Satoka Barnes, Jean-Paul Benayad, Anass Bernasik, Andrzej Ceccone, Giacomo Counsell, Jonathan D. P. Deeks, Christopher Fletcher, John S. Graham, Daniel J. Heuser, Christian Lee, Tae Geol Marie, Camille Marzec, Mateusz M. Mishra, Gautam Rading, Derk Renault, Olivier Scurr, David J. Shon, Hyun Kzong Spampinato, Valentina Tian, Hua Wang, Fuyi Winograd, Nicholas Wu, Kui Wucher, Andreas Zhou, Yufan Zhu, Zihua TI Measuring Compositions in Organic Depth Profiling: Results from a VAMAS Interlaboratory Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ION MASS-SPECTROMETRY; CLUSTER SPUTTERING YIELDS; UNIVERSAL EQUATION; SIZE-DEPENDENCE; TOF-SIMS; BEAMS; FILMS; SUPPRESSION; EFFICIENCY; EMISSION AB We report the results of a VAMAS (Versailles Project on Advanced Materials and Standards) interlaboratory study on the measurement of composition in organic depth profiling. Layered samples with known binary compositions of Irganox 1010 and either Irganox 1098 or Fmoc-pentafluoro-L-phenylalanine in each layer were manufactured in a single batch and distributed to more than 20 participating laboratories. The samples were analyzed using argon cluster ion sputtering and either X-ray photoelectron spectroscopy (XPS) or time-of-flight secondary ion mass spectrometry (ToF-SIMS) to generate depth profiles. Participants were asked to estimate the volume fractions in two of the layers and were provided with the compositions of all other layers. Participants using XPS provided volume fractions within 0.03 of the nominal values. Participants using ToF-SIMS either made no attempt, or used various methods that gave results ranging in error from 0.02 to over 0.10 in volume fraction, the latter representing a 50% relative error for a nominal volume fraction of 0.2. Error was predominantly caused by inadequacy in the ability to compensate for primary ion intensity variations and the matrix effect in SIMS. Matrix effects in these materials appear to be more pronounced as the number of atoms in both the primary analytical ion and the secondary ion increase. Using the participants' data we show that organic SIMS matrix effects can be measured and are remarkably consistent between instruments. We provide recommendations for identifying and compensating for matrix effects. Finally, we demonstrate, using a simple normalization method, that virtually all ToF-SIMS participants could have obtained estimates of volume fraction that were at least as accurate and consistent as XPS. C1 [Shard, Alexander G.; Havelund, Rasmus; Spencer, Steve J.; Gilmore, Ian S.] Natl Phys Lab, Teddington TW11 0LW, Middx, England. [Alexander, Morgan R.; Scurr, David J.] Univ Nottingham, Lab Biophys & Surface Anal, Nottingham NG7 2RD, England. [Angerer, Tina B.; Fletcher, John S.] Univ Gothenburg, Dept Chem & Mol Biol, S-40530 Gothenburg, Sweden. [Aoyagi, Satoka] Seikei Univ, Dept Mat & Life Sci, Tokyo 1808633, Japan. [Barnes, Jean-Paul; Benayad, Anass; Marie, Camille; Renault, Olivier] Univ Grenoble Alpes, F-38000 Grenoble, France. [Barnes, Jean-Paul; Marie, Camille; Renault, Olivier] CEA, LETI, F-38054 Grenoble, France. [Benayad, Anass] CEA, LITEN, DTNM, F-38054 Grenoble, France. [Bernasik, Andrzej; Marzec, Mateusz M.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Ceccone, Giacomo] Inst Hlth & Consumer Protect, I-21027 Ispra, VA, Italy. [Counsell, Jonathan D. P.] Kratos Analyt Ltd, Manchester M17 1GP, Lancs, England. [Deeks, Christopher] Thermo Fisher Sci, E Grinstead RH19 1UB, W Sussex, England. [Mishra, Gautam] Univ Washington, Dept Bioengn, Seattle, WA USA. [Heuser, Christian; Wucher, Andreas] Univ Duisburg Essen, Fac Phys, D-52425 Duisburg, Germany. [Lee, Tae Geol; Shon, Hyun Kzong] Korea Res Inst Stand & Sci, Daejeon 305340, South Korea. [Mishra, Gautam] 3M Deutschland GmbH, CRAL, D-41460 Neuss, Germany. [Rading, Derk] ION TOF GmbH, D-48149 Munster, Germany. [Spampinato, Valentina] CNR, Ist Fis Plasmi, I-20125 Milan, Italy. [Tian, Hua; Winograd, Nicholas] Penn State Univ, University Pk, PA 16802 USA. [Wang, Fuyi] Chinese Acad Sci, CAS Key Lab Analyt Chem Living Biosyst, Beijing 100190, Peoples R China. [Zhou, Yufan; Zhu, Zihua] Pacific NW Natl Lab, EMSL, Richland, WA 99354 USA. RP Shard, AG (reprint author), Natl Phys Lab, Teddington TW11 0LW, Middx, England. EM alex.shard@npl.co.uk RI Scurr, David/E-8441-2012; Alexander, Morgan/C-2506-2009; Zhu, Zihua/K-7652-2012; OI Scurr, David/0000-0003-0859-3886; Alexander, Morgan/0000-0001-5182-493X; Gilmore, Ian/0000-0002-0981-2318; Havelund, Rasmus/0000-0001-7316-9761 FU European Union; EMRP within EURAMET; U.S. National Institutes of Health [EB-002027]; DOE FX We thank Steve A. Smith from NPL for assisting in the production of the samples used in this study and Martin P. Seth from NPL for reviewing the manuscript and providing insightful comments. We thank the following people for providing some of the data used in this study: Dr. Helen Brannon, Kratos Analytical, U.K.; Ms. Tomoko Kawashima, Panasonic Corporation, Japan; Dr. Takuya Miyayama, ULVAC-Phi, Japan; Mr. Kan Shen, Pennsylvania State University; and Mr. Michael Taylor, University of Nottingham, U.K. This work forms part of the Chemical and Biological programme of the National Measurement System of the U.K. Department of Business, Innovation and Skills and with additional funding from the European Union through the European Metrology Research Programme (EMRP) projects SurfChem and TREND. The EMRP is jointly funded by the EMRP participating countries within EURAMET and the European Union. Funding from the U.S. National Institutes of Health Grant EB-002027 is gratefully acknowledged for the experiments done at the National ESCA and Surface Analysis Center for Biomedical Problems, University of Washington. A portion of the data was collected at EMSL, a National Scientific User Facility sponsored by the DOE and located at PNNL. NR 40 TC 12 Z9 12 U1 5 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 20 PY 2015 VL 119 IS 33 BP 10784 EP 10797 DI 10.1021/acs.jpcb.5b05625 PG 14 WC Chemistry, Physical SC Chemistry GA CP6VN UT WOS:000360026400040 PM 26204428 ER PT J AU Swierk, JR Klaus, S Trotochaud, L Bell, AT Tilley, TD AF Swierk, John R. Klaus, Shannon Trotochaud, Lena Bell, Alexis T. Tilley, T. Don TI Electrochemical Study of the Energetics of the Oxygen Evolution Reaction at Nickel Iron (Oxy)Hydroxide Catalysts SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ALKALINE WATER ELECTROLYSIS; OXIDE ELECTRODES; ACIDIC-SOLUTIONS; FILM ELECTRODES; PASSIVE FILM; AC-IMPEDANCE; THIN-FILMS; FE; ELECTROCATALYSTS; NI AB Iron-doped nickel (oxy)hydroxide catalysts (FexNi1-xOOH) exhibit high electrocatalytic behavior for the oxygen evolution reaction in base. Recent findings suggest that the incorporation of Fe3+ into a NiOOH lattice leads to nearly optimal adsorption energies for OER intermediates on active Fe sites. Utilizing electrochemical impedance spectroscopy and activation energy measurements, we find that pure NiOOH and FeOOH catalysts exhibit exceedingly high Faradaic resistances and activation energies 40-50 kJ/mol(-1) higher than those of the most active FexNi1-xOOH catalysts. Furthermore, the most active FexNi1-xOOH catalysts in this study exhibit activation energies that approach those previously reported for IrO2 OER catalysts. C1 [Swierk, John R.; Klaus, Shannon; Trotochaud, Lena; Bell, Alexis T.; Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Div Mat Sci, Berkeley, CA 94720 USA. [Klaus, Shannon; Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Swierk, JR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Div Mat Sci, Berkeley, CA 94720 USA. EM jrswierk@gmail.com; tdtilley@berkeley.edu OI Swierk, John/0000-0001-5811-7285; Bell, Alexis/0000-0002-5738-4645 FU Office of Science of the U.S. Department of Energy [DE-SC0004993] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under award no. DE-SC0004993. We thank Nella Vargas-Barbosa (Pennsylvania State University) for helpful discussions during the preparation of this manuscript. NR 65 TC 29 Z9 30 U1 23 U2 138 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 20 PY 2015 VL 119 IS 33 BP 19022 EP 19029 DI 10.1021/acs.jpcc.5b05861 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP6VL UT WOS:000360026200022 ER PT J AU Wang, J Seifert, S Winans, RE Tolmachoff, E Xin, YX Chen, DP Wang, H Anderson, SL AF Wang, Juan Seifert, Sonke Winans, Randall E. Tolmachoff, Erik Xin, Yuxuan Chen, Dongping Wang, Hai Anderson, Scott L. TI In situ X-ray Scattering and Dynamical Modeling of Pd Catalyst Nanoparticles Formed in Flames SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PARTICLE-SIZE DISTRIBUTION; SOLUBLE NANO-CATALYSTS; SMALL-ANGLE SCATTERING; GAS-PHASE; AEROSOL COAGULATION; MOLECULAR-DYNAMICS; SOOT PARTICLES; GROWTH; FUEL; PERFORMANCE AB It has previously been demonstrated that organopalladium precursors can break down under combustion conditions, forming nanoparticles that catalyze ignition. Here, we use in situ small-angle X-ray scattering (SAXS) to probe the formation and growth of palladium nanoparticles in an ethylene flame doped with 28 ppm (mol) of Pd(acetate)(2). The particles appear to nucleate in the flame front and are observed by SAXS to grow in size and mass in the high-temperature region of the flame (similar to 1200 K) with median diameters that evolve from 1.5 to 3.0 nm. Transmission electron microscopy of particles collected on a grid located outside the flame shows that the particles are metallic palladium with sizes comparable to those determined by SAXS. Molecular dynamics simulation of particles of selected sizes indicates that at the flame temperature the particles are molten and the average mass density of the particle material is notably smaller than that of bulk, liquid Pd at the melting point. Both experimental and computational results point to homogeneous nucleation and particle-particle coalescence as mechanisms for particle formation and growth. Aerosol dynamics simulation reproduces the time evolution of the particle size distribution and suggests that a substantial fraction of the particles must be electrically charged during their growth process. C1 [Wang, Juan] Peac Inst Multiscale Sci, Chengdu 610207, Sichuan, Peoples R China. [Wang, Juan; Anderson, Scott L.] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. [Seifert, Sonke; Winans, Randall E.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Tolmachoff, Erik] Univ So Calif, Aerosp & Mech Engn, Los Angeles, CA 90089 USA. [Xin, Yuxuan] Princeton Univ, Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Chen, Dongping; Wang, Hai] Stanford Univ, Mech Engn, Stanford, CA 94305 USA. [Wang, Juan] Southwest Jiaotong Univ, Key Lab Adv Technol Mat, Minist Educ, Chengdu 610031, Sichuan, Peoples R China. RP Winans, RE (reprint author), Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. EM rewinans@anl.gov RI Wang, Hai/A-1292-2009 OI Wang, Hai/0000-0001-6507-5503 FU U.S. DOE [DE-AC02-06CH11357]; Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; Molecular Dynamics program of the Air Force Office of Scientific Research (AFOSR) through a MURI [FA9550-08-1-0400] FX We thank Dr. Byeongdu Lee and Dr. Xiaobing Zuo for their help with the SAXS data analysis. We also thank Dr. Jan Ilavsky for providing the "IRENA" macro package for Igor Pro for the data fitting. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. The Argonne, Utah, USC, and Stanford groups gratefully acknowledge support for this work from the Molecular Dynamics program of the Air Force Office of Scientific Research (AFOSR) through a MURI grant (FA9550-08-1-0400). NR 50 TC 0 Z9 0 U1 4 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 20 PY 2015 VL 119 IS 33 BP 19073 EP 19082 DI 10.1021/acs.jpcc.5b01226 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP6VL UT WOS:000360026200027 ER PT J AU Shi, W Siefert, NS Morreale, BD AF Shi, Wei Siefert, Nicholas S. Morreale, Bryan D. TI Molecular Simulations of CO2, H-2, H2O, and H2S Gas Absorption into Hydrophobic Poly(dimethylsiloxane) (PDMS) Solvent: Solubility and Surface Tension SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-DIOXIDE; MONTE-CARLO; DYNAMICS; LIQUID; HEXAFLUOROPHOSPHATE; CAPTURE; WATER AB Henry's law constants were calculated for H2S, CO2, H2O, and H-2 gas absorption in the hydrophobic poly(dimethylsiloxane) (PDMS) solvent using an all-atom (AA) PDMS model. Calculations show that the relative gas solubility at 298 K decreases in the following order: H2S (147) > CO2 (19) approximate to H2O (15) > H-2 (1). Both quantum ab initio (AI) and classical force field (FF) gas-phase calculations show that these gases interact with the PDMS molecule in the order of H2S > CO2 > H-2; they decrease in the same order as gas solubility. The AA PDMS model gives CO2 solubility and PDMS surface tension values close to the experimental data, with differences of 14 and 8%, respectively. In addition, by using both the all-atom and united-atom PDMS models, our simulations suggest that it is challenging to develop a solvent which both has a significantly large surface tension and exhibits large CO2 solubility at high CO2 pressure. Finally, gas absorption effects on PDMS surface tension were investigated. CO2 absorption was simulated to decrease the solvent surface tension by 3 X 10(-3)-4 X 10(-3) N/m compared to the simulated neat PDMS solvent surface tension value of 21 x 10(-3) N/m; CO2 molecules exhibit the largest concentration in the gas-liquid interface region. In contrast, H2S absorption does not decrease PDMS surface tension, which is partially due to the strong H2S-PDMS interaction compared to the CO2-PDMS interaction. C1 [Shi, Wei; Siefert, Nicholas S.; Morreale, Bryan D.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Shi, Wei] AECOM, South Pk, PA 15129 USA. [Shi, Wei] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. RP Shi, W (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM shiw@netl.doe.gov FU National Energy Technology Laboratory under RES [DE-FE0004000]; Department of Energy, National Energy Technology Laboratory, an agency of the United States Government; URS Energy & Construction, Inc. FX We thank Bob Enick, Peter Koronaios, David Luebke, Hunaid Nulwala, Fan Ski, Janice Steckel, and David Hopkinson for helpful discussions. This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in computational chemistry under RES contract DE-FE0004000. This project was funded by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with URS Energy & Construction, Inc. Neither the United States Government nor any agency thereof nor any of their employees nor URS Energy & Construction, Inc. nor any of their employees makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed or represents that its use would not infringe on privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of the authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 37 TC 4 Z9 4 U1 6 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 20 PY 2015 VL 119 IS 33 BP 19253 EP 19265 DI 10.1021/acs.jpcc.5b05806 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP6VL UT WOS:000360026200046 ER PT J AU Lopez-Bezanilla, A Littlewood, PB AF Lopez-Bezanilla, Alejandro Littlewood, Peter B. TI sigma-pi-Band Inversion in a Novel Two-Dimensional Material SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GRAPHENE; STRAIN AB We present a theoretical study of a new type of two-dimensional material exhibiting a pentagonal arrangement of C and Si atoms. Pentagonal SiC2 is investigated with density functional theory-based calculations to show that the buckled nanostructure is dynamically stable, and exhibits an indirect energy band gap and an enhanced electronic dispersion with respect to the all-carbon counterpart. Computed Born effective charges exhibit a significant anisotropy for C and Si atoms that deviates substantially from their static effective charges. We establish an accurate tunability of the vertical location of the p-p-sigma and p-p-pi bands and show that under compressive biaxial strain the density of states decreases, and conversely for tensile biaxial strain. This coupling between the tunability of strain-mediated density of states and semiconducting properties in a monolayered structure may allow for the development of applications in semiconducting stretchable electronics. C1 [Lopez-Bezanilla, Alejandro; Littlewood, Peter B.] Argonne Natl Lab, Lemont, IL 60439 USA. [Lopez-Bezanilla, Alejandro; Littlewood, Peter B.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. EM alejandrolb@gmail.com RI Littlewood, Peter/B-7746-2008; Lopez-Bezanilla, Alejandro/B-9125-2015 OI Lopez-Bezanilla, Alejandro/0000-0002-4142-2360 FU DOE-BES [DE-AC02-06CH11357] FX We gratefully acknowledge the computing resources provided on Blues high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. A.L.-B. thanks J. Allred for fruitful discussions. Work at Argonne is supported by DOE-BES under contract no. DE-AC02-06CH11357. NR 18 TC 12 Z9 13 U1 9 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 20 PY 2015 VL 119 IS 33 BP 19469 EP 19474 DI 10.1021/acs.jpcc.5b04726 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP6VL UT WOS:000360026200072 ER PT J AU Wong, CY Folie, BD Cotts, BL Ginsberg, NS AF Wong, Cathy Y. Folie, Brendan D. Cotts, Benjamin L. Ginsberg, Naomi S. TI Discerning Variable Extents of Interdomain Orientational and Structural Heterogeneity in Solution-Cast Polycrystalline Organic Semiconducting Thin Films SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID FIELD-EFFECT TRANSISTORS; SINGLET EXCITON FISSION; CHARGE-TRANSPORT; SOLUBLE ANTHRADITHIOPHENE; FUNCTIONALIZED PENTACENE; GRAIN-ORIENTATION; PROBE MICROSCOPY; DYNAMICS; CRYSTALLIZATION; TEMPERATURE AB By spatially resolving the polarized ultrafast optical transient absorption within several tens of individual domains in solution-processed polycrystalline small-molecule organic semiconducting films, we infer the domains' extents of structural and orientational heterogeneity. As metrics, we observe variations in the time scales of ultrafast excited state dynamics and in the relative strength of competing resonant probe transitions. We find that films of 2,8-difluoro-5,11-bis(triethylsilylethynyl)anthradithiophene (diF-TES-ADT) exhibit a much higher degree of both structural and orientational heterogeneity among their domains than do films of 6,13-bis(triisopropylsilylethynyl)pentacene (TIPS-Pn), despite the apparent structural similarity between these two small molecules. Since both molecules feature prominently in solution-processed organic transistors, correlating the extent of heterogeneity to bulk transport using our approach will be highly valuable toward determining the underlying design principles for creating high-performing devices. Furthermore, our ability to characterize such variation in heterogeneity will enable fundamental studies of the interplay between molecular dynamics and driving forces in controlling emergent unequilibrated structures. C1 [Wong, Cathy Y.; Cotts, Benjamin L.; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Folie, Brendan D.; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Lawrence Berkeley Natl Lab, Phys Biosci, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ginsberg, NS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM nsginsberg@berkeley.edu FU Defense Advanced Research Projects Agency Young Faculty [N66001-12-1-4228]; David and Lucile Packard Foundation Fellowship for Science and Engineering; Natural Sciences and Engineering Research Council, Canada; National Science Foundation Graduate Research Fellowship [DGE 1106400]; Alfred P. Sloan Research Fellowship FX This work has been supported by the Defense Advanced Research Projects Agency Young Faculty Award number N66001-12-1-4228 and by a David and Lucile Packard Foundation Fellowship for Science and Engineering to N.S.G. C.Y.W. thanks the Natural Sciences and Engineering Research Council, Canada for a Postdoctoral Fellowship, B.D.F. and B.L.C. each acknowledge a National Science Foundation Graduate Research Fellowship (DGE 1106400), and N.S.G. acknowledges an Alfred P. Sloan Research Fellowship. NR 48 TC 4 Z9 4 U1 11 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 20 PY 2015 VL 6 IS 16 BP 3155 EP 3162 DI 10.1021/acs.jpclett.5b01416 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP6VT UT WOS:000360027000008 ER PT J AU Watson, BR Yang, B Xiao, K Ma, YZ Doughty, B Calhoun, TR AF Watson, Brianna R. Yang, Bin Xiao, Kai Ma, Ying-Zhong Doughty, Benjamin Calhoun, Tessa R. TI Elucidation of Perovskite Film Micro-Orientations Using Two-Photon Total Internal Reflectance Fluorescence Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; HALIDE PEROVSKITES; EFFICIENCY; CH3NH3PBI3; CHARGE; CRYSTALLIZATION; SEMICONDUCTORS; LUMINESCENCE; DIFFUSION; CRYSTALS AB The emergence of efficient hybrid organic inorganic perovskite photovoltaic materials has brought about the rapid development of a variety of preparation and processing techniques designed to maximize their performance. As processing methods continue to emerge, it is important to understand how the optical properties of these materials are affected on a microscopic scale. Here, polarization-resolved two-photon total internal reflectance microscopy (TIRFM) was used to probe changes in transition dipole moment orientation as a function of thermal annealing time in hybrid organic inorganic lead-iodide-based perovskite (CH3NH3PbI3) thin films on glass. These results show that as thermal annealing time is increased the distribution of transition moments pointing out-of-plane decreases in favor of forming areas with increased in-plane orientations. It was also shown through the axial sensitivity of TIRFM that the surface topography is manifested in the signal intensity and can be used to survey aspects of morphology in coincidence with the optical properties of these films. C1 [Watson, Brianna R.; Calhoun, Tessa R.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Yang, Bin; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ma, Ying-Zhong; Doughty, Benjamin] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Doughty, B (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM doughtybl@ornl.gov; trcalhoun@utk.edu RI Yang, Bin/P-8529-2014; Ma, Yingzhong/L-6261-2016; Doughty, Benjamin /M-5704-2016; OI Yang, Bin/0000-0002-5667-9126; Ma, Yingzhong/0000-0002-8154-1006; Doughty, Benjamin /0000-0001-6429-9329; Watson, Brianna/0000-0001-6540-5330; Xiao, Kai /0000-0002-0402-8276 FU University of Tennessee; UT-ORNL Science Alliance Joint Directed Research and Development program; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX T.RC.'s research is supported by the University of Tennessee and the UT-ORNL Science Alliance Joint Directed Research and Development program. B.D.'s research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. Work by Y.-Z.M. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Work by B.Y. and K.X. was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 42 TC 6 Z9 6 U1 2 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 20 PY 2015 VL 6 IS 16 BP 3283 EP 3288 DI 10.1021/acs.jpclett.5b01474 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP6VT UT WOS:000360027000012 ER PT J AU Kumara, C Zuo, XB Cullen, DA Dass, A AF Kumara, Chanaka Zuo, Xiaobing Cullen, David A. Dass, Amala TI Au329-xAgx(SR)(84) Nanomolecules: Plasmonic Alloy Faradaurate-329 SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID NANOCRYSTAL GOLD MOLECULES; RAY CRYSTAL-STRUCTURE; MASS-SPECTROMETRY; CLUSTER COMPOUNDS; NANOPARTICLES; NANOCLUSTERS; ABSORPTION; RESOLUTION; SCATTERING; RESONANCE AB Though significant progress has been made to improve the monodispersity of larger (>10 nm) alloy metal nanoparticles, there still exists a significant variation in nanoparticle composition, ranging from +/- 1000s of atoms. Here, for the first time, we report the synthesis of atomically precise (+/- 0 metal atom variation) Au329-xAgx(SCH2CH2Ph)(84) alloy nanomolecules. The composition was determined using high resolution electrospray ionization mass spectrometry. In contrast to larger (>10 nm) Au-Ag nanoparticles, the surface plasmon resonance (SPR) peak does not show a major shift, but a minor similar to 10 nm red-shift, upon increasing silver content. The intensity of the SPR peak also varies in an intriguing manner, where a dampening is observed with medium silver incorporation, and a significant sharpening is observed upon higher Ag content. The report outlines (a) an unprecedented advance in nanoparticle mass spectrometry of high mass at atomic precision; and (b) the unexpected optical behavior of Au-Ag alloys in the region where nascent SPR emerges; specifically, in this work, the SPR-like peak does not show a major similar to 100 nm blue-shift with Ag alloying of Au-329 nanomolecules, as shown to be common in larger nanoparticles. C1 [Kumara, Chanaka; Dass, Amala] Univ Mississippi, Dept Chem & Biochem, Oxford, MS 38677 USA. [Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Cullen, David A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Dass, A (reprint author), Univ Mississippi, Dept Chem & Biochem, Oxford, MS 38677 USA. EM amal@olemiss.edu RI Cullen, David/A-2918-2015 OI Cullen, David/0000-0002-2593-7866 FU NSF [CHE-1255519]; ORNL's Center for Nanophase Materials Sciences (CNMS); U.S. DOE [DE-AC02-06CH11357] FX C.K. and A.D. gratefully acknowledge support from NSF CHE-1255519. Electron microscopy research supported through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. Work performed at Argonne and the use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 43 TC 3 Z9 3 U1 3 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 20 PY 2015 VL 6 IS 16 BP 3320 EP 3326 DI 10.1021/acs.jpclett.5b01395 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP6VT UT WOS:000360027000030 ER PT J AU Trabert, E Beiersdorfer, P Hell, N Brown, GV AF Traebert, E. Beiersdorfer, P. Hell, N. Brown, G. V. TI Measurement of the 3s(1/2)-3p(3/2) resonance line of sodiumlike Eu52+ SO PHYSICAL REVIEW A LA English DT Article ID BEAM ION-TRAP; ENERGY-LEVEL SCHEME; X-RAY SPECTROMETER; CU-LIKE IONS; ISOELECTRONIC SEQUENCE; NA-LIKE; TRANSITION-PROBABILITIES; PERTURBATION-THEORY; SPECTROSCOPY; SPECTRA AB We have measured the 3s(1/2)-3p(3/2) transition in sodiumlike Eu52+ situated at 41.232 angstrom with an uncertainty of 73 ppm. Our measurement extends previous high-precision measurements into the 56 < Z < 78 range of atomic numbers. We also present measurements of 3s(1/2)-3p(3/2) and 3p(1/2)-3d(3/2) transitions in the neighboring magnesiumlike, aluminumlike, and siliconlike europium ions. C1 [Traebert, E.; Beiersdorfer, P.; Hell, N.; Brown, G. V.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Trabert, E (reprint author), Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. EM beiersdorfer1@llnl.gov OI Hell, Natalie/0000-0003-3057-1536 FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; German Research Association DFG [Tr171/19]; German Bundesministerium fur Wirtschaft und Technologie under Deutsches Zentrum fur Luft- und Raumfahrt [50OR1113] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. E.T. acknowledges travel support by the German Research Association DFG (Grant No. Tr171/19). N.H. acknowledges support from the German Bundesministerium fur Wirtschaft und Technologie under Deutsches Zentrum fur Luft- und Raumfahrt Grant No. 50OR1113. NR 42 TC 1 Z9 1 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD AUG 20 PY 2015 VL 92 IS 2 AR 022509 DI 10.1103/PhysRevA.92.022509 PG 4 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CP4MY UT WOS:000359857500004 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Brown, AM Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Christy, B Clark, K Classen, L Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M Deyoung, T Diaz-Velez, JC Dumm, JP Dunkman, M Eagan, R Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fadiran, O Fahey, S Fazely, AR Fedynitch, A Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Fuchs, T Glagla, M Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Gluesenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grant, D Gretskov, P Groh, JC Gross, A Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansmann, B Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfe, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jero, K Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohnen, G Kolanoski, H Konietz, R Koob, A Koepke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lesiak-Bzdak, M Leuermann, M Leuner, J Lunemann, J Madsen, J Maggi, G Mahn, KBM Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Middlemas, E Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Olivas, A Omairat, A O'Murchadha, A O'Murchadha, A Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Scheriau, F Schimp, M Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Seckel, D Seunarine, S Shanidze, R Smith, MWE Soldin, D Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S van Eijndhoven, N Vandenbroucke, J van Santen, J Vanheule, S Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Wille, L Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Brown, A. M. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. deYoung, T. Diaz-Velez, J. C. Dumm, J. P. Dunkman, M. Eagan, R. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fadiran, O. Fahey, S. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Fuchs, T. Glagla, M. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansmann, B. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfe, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jero, K. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Kohnen, G. Kolanoski, H. Konietz, R. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Middlemas, E. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Scheriau, F. Schimp, M. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Seckel, D. Seunarine, S. Shanidze, R. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Stroem, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Vandenbroucke, J. van Santen, J. Vanheule, S. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallraff, M. Wandkowsky, N. Weaver, C. Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Zoll, M. CA IceCube Collaboration TI Evidence for Astrophysical Muon Neutrinos from the Northern Sky with IceCube SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-ENERGY NEUTRINOS; GAMMA-RAY BURSTS; ATMOSPHERIC MUON; SPECTRUM; FLUXES; RATIO AB Results from the IceCube Neutrino Observatory have recently provided compelling evidence for the existence of a high energy astrophysical neutrino flux utilizing a dominantly Southern Hemisphere data set consisting primarily of nu(e) and nu(tau) charged-current and neutral-current ( cascade) neutrino interactions. In the analysis presented here, a data sample of approximately 35 000 muon neutrinos from the Northern sky is extracted from data taken during 659.5 days of live time recorded between May 2010 and May 2012. While this sample is composed primarily of neutrinos produced by cosmic ray interactions in Earth's atmosphere, the highest energy events are inconsistent with a hypothesis of solely terrestrial origin at 3.7 sigma significance. These neutrinos can, however, be explained by an astrophysical flux per neutrino flavor at a level of Phi(E-nu) = 9.9(-3.4)(+3.9) x 10(-19) GeV-1 cm(-2) sr(-1) s(-1) (E-nu/100 TeV)(-2), consistent with IceCube's Southern-Hemisphere-dominated result. Additionally, a fit for an astrophysical flux with an arbitrary spectral index is performed. We find a spectral index of 2.2(-0.2)(+0.2), which is also in good agreement with the Southern Hemisphere result. C1 [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Glagla, M.; Gier, D.; Gretskov, P.; Haack, C.; Hansmann, B.; Hellwig, D.; Kemp, J.; Konietz, R.; Koob, A.; Leuermann, M.; Leuner, J.; Paul, L.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schimp, M.; Schoenen, S.; Schukraft, A.; Stahlberg, M.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Phys Inst 3, D-52056 Aachen, Germany. [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Whelan, B. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Tjus, J. Becker; Bos, F.; Eichmann, B.; Fedynitch, A.; Kroll, M.; Saba, S. M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Phys Inst, D-53115 Bonn, Germany. [Aguilar, J. A.; Heereman, D.; Meagher, K.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; de Wasseige, G.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.; Brown, A. M.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Cheung, E.; Christy, B.; Felde, J.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Maunu, R.; Olivas, A.; Redl, P.; Schmidt, T.; Sullivan, G. 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L.; Kheirandish, A.; McNally, F.; Merino, G.; Middlemas, E.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Santen, J.; Wandkowsky, N.; Weaver, C.; Wendt, C.; Westerhoff, S.; Whitehorn, N.; Wille, L.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; Beiser, E.; BenZvi, S.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fadiran, O.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; McNally, F.; Merino, G.; Middlemas, E.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Santen, J.; Wandkowsky, N.; Weaver, C.; Wendt, C.; Westerhoff, S.; Whitehorn, N.; Wille, L.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Archinger, M.; Baum, V.; Boeser, S.; Eberhardt, B.; Ehrhardt, T.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Abraham, K.; Bernhard, A.; Coenders, S.; Gross, A.; Holzapfe, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Veenkamp, J.] Tech Univ Munich, D-85748 Garching, Germany. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Kurahashi, N.; Richman, M.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Bai, X.] South Dakota Sch Mines & Technol, Phys Dept, Rapid City, SD 57701 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Ahrens, M.; Bohm, C.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Ahrens, M.; Bohm, C.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bose, D.; In, S.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Clark, K.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Anderson, T.; Arlen, T. C.; Cowen, D. F.; Dunkman, M.; Eagan, R.; Groh, J. C.; Huang, F.; Keivani, A.; Lanfranchi, J. L.; Quinnan, M.; Smith, M. W. E.; Stanisha, N. A.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Euler, S.; Hallgren, A.; de los Heros, C. Perez; Stroem, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hickford, S.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Kowalski, M.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N. L.; Terliuk, A.; Usner, M.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. RP Aartsen, MG (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. RI Maruyama, Reina/A-1064-2013; Koskinen, David/G-3236-2014; Tjus, Julia/G-8145-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Wiebusch, Christopher/G-6490-2012; OI Maruyama, Reina/0000-0003-2794-512X; Arguelles Delgado, Carlos/0000-0003-4186-4182; Koskinen, David/0000-0002-0514-5917; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Wiebusch, Christopher/0000-0002-6418-3008; Perez de los Heros, Carlos/0000-0002-2084-5866; Strotjohann, Nora Linn/0000-0002-4667-6730 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF); WestGrid and Compute/Calcul Canada FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 46 TC 55 Z9 55 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 20 PY 2015 VL 115 IS 8 AR 081102 DI 10.1103/PhysRevLett.115.081102 PG 7 WC Physics, Multidisciplinary SC Physics GA CP4SL UT WOS:000359872800003 PM 26340177 ER PT J AU Bolintineanu, DS Grest, GS Lechman, JB Silbert, LE AF Bolintineanu, Dan S. Grest, Gary S. Lechman, Jeremy B. Silbert, Leonardo E. TI Diffusion in Jammed Particle Packs SO PHYSICAL REVIEW LETTERS LA English DT Article ID BROWNIAN-MOTION SIMULATION; HETEROGENEOUS MEDIA; ELECTRICAL-CONDUCTIVITY; DISORDERED MEDIA AB Using random walk simulations we explore diffusive transport through monodisperse sphere packings over a range of packing fractions phi in the vicinity of the jamming transition at phi(c). Various diffusion properties are computed over several orders of magnitude in both time and packing pressure. Two well-separated regimes of normal "Fickian" diffusion, where the mean squared displacement is linear in time, are observed. The first corresponds to diffusion inside individual spheres, while the latter is the long-time bulk diffusion. The intermediate anomalous diffusion regime and the long-time value of the diffusion coefficient are both shown to be controlled by particle contacts, which in turn depend on proximity to phi(c). The time required to recover normal diffusion t* scales as (phi - phi(c))(-0.5) and the long-time diffusivity D-infinity similar to (phi - phi(c))(0.5), or D-infinity similar to 1/t*. It is shown that the distribution of mean first passage times associated with the escape of random walkers between neighboring particles controls both t* and D-infinity in the limit phi -> phi(c). C1 [Bolintineanu, Dan S.; Grest, Gary S.; Lechman, Jeremy B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Silbert, Leonardo E.] So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA. RP Bolintineanu, DS (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM dsbolin@sandia.gov FU Sandia Laboratory Directed Research and Development Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Sandia Laboratory Directed Research and Development Program. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a Lockheed-Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. L. E. S. gratefully acknowledges a hospitable stay at SNL. NR 34 TC 0 Z9 0 U1 4 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 20 PY 2015 VL 115 IS 8 AR 088002 DI 10.1103/PhysRevLett.115.088002 PG 5 WC Physics, Multidisciplinary SC Physics GA CP4SL UT WOS:000359872800014 PM 26340211 ER PT J AU Estey, B Yu, CH Muller, H Kuan, PC Lan, SY AF Estey, Brian Yu, Chenghui Mueller, Holger Kuan, Pei-Chen Lan, Shau-Yu TI High-Resolution Atom Interferometers with Suppressed Diffraction Phases SO PHYSICAL REVIEW LETTERS LA English DT Article ID PRECISION-MEASUREMENT; CONSTANT AB We experimentally and theoretically study the diffraction phase of large-momentum transfer beam splitters in atom interferometers based on Bragg diffraction. We null the diffraction phase and increase the sensitivity of the interferometer by combining Bragg diffraction with Bloch oscillations. We demonstrate agreement between experiment and theory, and a 1500-fold reduction of the diffraction phase, limited by measurement noise. In addition to reduced systematic effects, our interferometer has high contrast with up to 4.4 x 10(6) radians of phase difference, and a resolution in the fine structure constant of delta alpha/alpha = 0.25 ppb in 25 h of integration time. C1 [Estey, Brian; Yu, Chenghui; Mueller, Holger] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kuan, Pei-Chen; Lan, Shau-Yu] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. [Mueller, Holger] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Estey, B (reprint author), Univ Calif Berkeley, Dept Phys, 366 Le Conte Hall MS 7300, Berkeley, CA 94720 USA. EM hm@berkeley.edu RI Lan, Shau-Yu/B-5567-2014 OI Lan, Shau-Yu/0000-0003-2608-9472 FU National Science Foundation [PHY-1056620]; David and Lucile Packard Foundation; National Aeronautics and Space Administration [NNH13ZTT002N, NNH10ZDA001N-PIDDP, NNH11ZTT001]; Singapore National Research Foundation [NRFF2013-12] FX We thank Sheng-wey Chiow, Jordan Dudley, Paul Hamilton, Philipp Haslinger, and Erik Urban for discussions and assistance. This material is based upon work supported by the National Science Foundation under CAREER Grant No. PHY-1056620, the David and Lucile Packard Foundation, and National Aeronautics and Space Administration Grants No. NNH13ZTT002N, No. NNH10ZDA001N-PIDDP, and No. NNH11ZTT001. S.-Y. L. and P.-C. K. acknowledge support from the Singapore National Research Foundation under Grant No. NRFF2013-12. NR 34 TC 6 Z9 6 U1 5 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 20 PY 2015 VL 115 IS 8 AR 083002 DI 10.1103/PhysRevLett.115.083002 PG 5 WC Physics, Multidisciplinary SC Physics GA CP4SL UT WOS:000359872800004 PM 26340186 ER PT J AU Wu, DL Potluri, N Lu, JP Kim, YC Rastinejad, F AF Wu, Dalei Potluri, Nalini Lu, Jingping Kim, Youngchang Rastinejad, Fraydoon TI Structural integration in hypoxia-inducible factors SO NATURE LA English DT Article ID RENAL-CELL CARCINOMA; HIF2-ALPHA PAS-B; TRANSCRIPTION FACTOR; LIGAND-BINDING; SUPPRESSOR GENE; SMALL MOLECULES; CANCER BIOLOGY; TUMOR-GROWTH; DOMAIN; HIF-1 AB The hypoxia-inducible factors (HIFs) coordinate cellular adaptations to low oxygen stress by regulating transcriptional programs in erythropoiesis, angiogenesis and metabolism. These programs promote the growth and progression of many tumours, making HIFs attractive anticancer targets. Transcriptionally active HIFs consist of HIF-alpha and ARNT (also called HIF-1 beta) subunits. Here we describe crystal structures for each of mouse HIF-2 alpha-ARNT and HIF-1 alpha-ARNT heterodimers in states that include bound small molecules and their hypoxia response element. A highly integrated quaternary architecture is shared by HIF-2 alpha-ARNT and HIF-1 alpha-ARNT, wherein ARNT spirals around the outside of each HIF-alpha subunit. Five distinct pockets are observed that permit small-molecule binding, including PAS domain encapsulated sites and an interfacial cavity formed through subunit heterodimerization. The DNA-reading head rotates, extends and cooperates with a distal PAS domain to bind hypoxia response elements. HIF-alpha mutations linked to human cancers map to sensitive sites that establish DNA binding and the stability of PAS domains and pockets. C1 [Wu, Dalei; Potluri, Nalini; Lu, Jingping; Rastinejad, Fraydoon] Sanford Burnham Prebys Med Discovery Inst, Metab Dis Program, Orlando, FL 32827 USA. [Kim, Youngchang] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. RP Rastinejad, F (reprint author), Sanford Burnham Prebys Med Discovery Inst, Metab Dis Program, Orlando, FL 32827 USA. EM frastinejad@sbpdiscovery.org NR 64 TC 23 Z9 25 U1 6 U2 32 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 20 PY 2015 VL 524 IS 7565 BP 303 EP + DI 10.1038/nature14883 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2NN UT WOS:000359714000026 PM 26245371 ER PT J AU Liu, Z Guan, DB Wei, W Davis, SJ Ciais, P Bai, J Peng, SS Zhang, Q Hubacek, K Marland, G Andres, RJ Crawford-Brown, D Lin, JT Zhao, HY Hong, CP Boden, TA Feng, KS Peters, GP Xi, FM Liu, JG Li, Y Zhao, Y Zeng, N He, KB AF Liu, Zhu Guan, Dabo Wei, Wei Davis, Steven J. Ciais, Philippe Bai, Jin Peng, Shushi Zhang, Qiang Hubacek, Klaus Marland, Gregg Andres, Robert J. Crawford-Brown, Douglas Lin, Jintai Zhao, Hongyan Hong, Chaopeng Boden, Thomas A. Feng, Kuishuang Peters, Glen P. Xi, Fengming Liu, Junguo Li, Yuan Zhao, Yu Zeng, Ning He, Kebin TI Reduced carbon emission estimates from fossil fuel combustion and cement production in China SO NATURE LA English DT Article ID CO2 EMISSIONS; GDP STATISTICS; DISTRIBUTIONS; UNCERTAINTIES; POLLUTANTS AB Nearly three-quarters of the growth in global carbon emissions from the burning of fossil fuels and cement production between 2010 and 2012 occurred in China(1,2). Yet estimates of Chinese emissions remain subject to large uncertainty; inventories of China's total fossil fuel carbon emissions in 2008 differ by 0.3 gigatonnes of carbon, or 15 per cent(1,3-5). The primary sources of this uncertainty are conflicting estimates of energy consumption and emission factors, the latter being uncertain because of very few actual measurements representative of the mix of Chinese fuels. Here we re-evaluate China's carbon emissions using updated and harmonized energy consumption and clinker production data and two new and comprehensive sets of measured emission factors for Chinese coal. We find that total energy consumption in China was 10 per cent higher in 2000-2012 than the value reported by China's national statistics(6), that emission factors for Chinese coal are on average 40 per cent lower than the default values recommended by the Intergovernmental Panel on Climate Change(7), and that emissions from China's cement production are 45 per cent less than recent estimates(1,4). Altogether, our revised estimate of China's CO2 emissions from fossil fuel combustion and cement production is 2.49 gigatonnes of carbon (2 standard deviations = +/-7.3 per cent) in 2013, which is 14 per cent lower than the emissions reported by other prominent inventories(1,4,8). Over the full period 2000 to 2013, our revised estimates are 2.9 gigatonnes of carbon less than previous estimates of China's cumulative carbon emissions(1,4). Our findings suggest that overestimation of China's emissions in 2000-2013 may be larger than China's estimated total forest sink in 1990-2007 (2.66 gigatonnes of carbon)(9) or China's land carbon sink in 2000-2009 (2.6 gigatonnes of carbon)(10). C1 [Liu, Zhu] Harvard Univ, John F Kennedy Sch Govt, Cambridge, MA 02138 USA. [Guan, Dabo; Davis, Steven J.; Xi, Fengming] Chinese Acad Sci, Inst Appl Ecol, Shenyang 110016, Peoples R China. [Liu, Zhu] CALTECH, Resnick Sustainabil Inst, Pasadena, CA 91125 USA. [Guan, Dabo; Zhang, Qiang; Zhao, Hongyan; Hong, Chaopeng] Tsinghua Univ, Ctr Earth Syst Sci, Key Lab Earth Syst Modeling, Minist Educ, Beijing 100084, Peoples R China. [Guan, Dabo; Li, Yuan] Univ E Anglia, Sch Int Dev, Norwich NR4 7TJ, Norfolk, England. [Wei, Wei] Chinese Acad Sci, Shanghai Adv Res Inst, CAS Key Lab Lowcarbon Convers Sci & Engn, Shanghai 201203, Peoples R China. [Davis, Steven J.] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Ciais, Philippe; Peng, Shushi] CE Orme Merisiers, CEA CNRS UVSQ, Lab Sci Climat & Environm, F-91191 Gif Sur Yvette, France. [Bai, Jin] Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Peoples R China. [Peng, Shushi] CNRS, F-38041 Grenoble, France. [Peng, Shushi] UJF Grenoble 1, LGGE, UMR5183, F-38041 Grenoble, France. [Hubacek, Klaus; Feng, Kuishuang] Univ Maryland, Dept Geog Sci, College Pk, MD 20742 USA. [Marland, Gregg] Appalachian State Univ, Res Inst Environm Energy & Econ, Boone, NC 28608 USA. [Andres, Robert J.; Boden, Thomas A.] Oak Ridge Natl Lab, Carbon Dioxide Informat Anal Ctr, Oak Ridge, TN 37831 USA. [Crawford-Brown, Douglas] Univ Cambridge, Dept Land Econ, Cambridge Ctr Climate Change Mitigat Res, Cambridge CB3 9EP, England. [Lin, Jintai] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China. [Hong, Chaopeng; He, Kebin] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut C, Beijing 100084, Peoples R China. [Peters, Glen P.] CICERO, N-0318 Oslo, Norway. [Xi, Fengming] Chinese Acad Sci, CAS Key Lab Pollut Ecol & Environm Engn, Shenyang 110016, Peoples R China. [Liu, Junguo] Beijing Forestry Univ, Sch Nat Conservat, Beijing 10083, Peoples R China. [Liu, Junguo] Int Inst Appl Syst Anal, Ecosyst Serv & Management Program, A-2361 Laxenburg, Austria. [Liu, Junguo] South Univ Sci & Technol China, Sch Environm Sci & Engn, Shenzhen 518055, Peoples R China. [Zhao, Yu] Nanjing Univ, State Key Lab Pollut Control& Resource Reuse, Nanjing 210023, Jiangsu, Peoples R China. [Zhao, Yu] Nanjing Univ, Sch Environm, Nanjing 210023, Jiangsu, Peoples R China. [Zeng, Ning] Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20742 USA. [Zeng, Ning] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. [Zeng, Ning] Chinese Acad Sci, Inst Atmospher Phys, Beijing 100029, Peoples R China. RP Liu, Z (reprint author), Harvard Univ, John F Kennedy Sch Govt, Cambridge, MA 02138 USA. EM liuzhu@iae.ac.cn; dabo.guan@uea.ac.uk; weiwei@sari.ac.cn; hekb@tsinghua.edu.cn RI Zhang, Qiang/D-9034-2012; Lin, Jintai/A-8872-2012; Liu, Zhu/A-4634-2013; Peng, Shushi/J-4779-2014; Liu, Junguo/B-3021-2012; Zeng, Ning/A-3130-2008; OI Lin, Jintai/0000-0002-2362-2940; Liu, Zhu/0000-0002-8968-7050; Peng, Shushi/0000-0001-5098-726X; Liu, Junguo/0000-0002-5745-6311; Zeng, Ning/0000-0002-7489-7629; Davis, Steven/0000-0002-9338-0844; Bai, Jin/0000-0002-8623-1656; ANDRES, ROBERT/0000-0001-8781-4979; Guan, Dabo/0000-0003-3773-3403 FU Chinese Academy of Sciences; China's National Basic Research Program; National Natural Science Foundation of China (NSFC) [XDA05010109, 2014CB441301, XDA05010110, XDA05010103, XDA05010101, 41328008, 41222036]; Italy's Ministry for Environment, Land and Sea; Economic and Social Research Council [ES/L016028]; Institute of Applied Ecology, Chinese Academy of Sciences; European Research Council [ERC-2013-SyG 610028-IMBALANCE-P]; US Department of Energy, Office of Science, Biological and Environmental Research under US Department of Energy [DE-AC05-00OR22725]; NSFC [41422502, 41175127, 41161140353, 91425303, 41473076]; International Science & Technology Cooperation Program of China [2012DFA91530]; Natural Science Foundation of Beijing, China [8151002]; National Program for Support of Top-notch Young Professionals; Fundamental Research Funds for the Central Universities [TD-JC-2013-2]; China CDM Fund [2013051, 2013124]; Shenyang Science and Technology Planning [F14-232-6-01, F14-134-9-00]; Norwegian Research Council [235523] FX This work was supported by the Strategic Priority Research Program "Climate Change: Carbon Budget and Relevant Issues" of the Chinese Academy of Sciences, and by China's National Basic Research Program and National Natural Science Foundation of China (NSFC) funded projects (grants XDA05010109, 2014CB441301, XDA05010110, XDA05010103, XDA05010101, 41328008 and 41222036). Z.L. acknowledges Harvard University Giorgio Ruffolo fellowship and support from Italy's Ministry for Environment, Land and Sea. D.G. acknowledges the Economic and Social Research Council funded project "Dynamics of Green Growth in European and Chinese Cities" (ES/L016028) and the Philip Leverhulme Prize. S.J.D. acknowledges support from the Institute of Applied Ecology, Chinese Academy of Sciences Fellowships for Young International Distinguished Scientists. P.C. and S.P. acknowledge support of the European Research Council Synergy grant ERC-2013-SyG 610028-IMBALANCE-P. R.J.A. and T.A.B. were sponsored by the US Department of Energy, Office of Science, Biological and Environmental Research under US Department of Energy contract DE-AC05-00OR22725. J. Lin acknowledges the NSFC (41422502 and 41175127). J. Liu acknowledges the International Science & Technology Cooperation Program of China (2012DFA91530), the NSFC (41161140353, 91425303), The Natural Science Foundation of Beijing, China (8151002), the National Program for Support of Top-notch Young Professionals, and Fundamental Research Funds for the Central Universities (TD-JC-2013-2). F.X. acknowledges the NSFC (41473076), China CDM Fund (2013051, 2013124) and Shenyang Science and Technology Planning (F14-232-6-01, F14-134-9-00). G.P.P. acknowledges funding from the Norwegian Research Council (235523). The authors are grateful to S. Piao, L. Cao and J. Yan for insightful comments. NR 43 TC 86 Z9 102 U1 60 U2 283 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 20 PY 2015 VL 524 IS 7565 BP 335 EP + DI 10.1038/nature14677 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2NN UT WOS:000359714000032 PM 26289204 ER PT J AU Kapilevich, GA Riseborough, PS Gray, AX Gulacsi, M Durakiewicz, T Smith, JL AF Kapilevich, G. A. Riseborough, P. S. Gray, A. X. Gulacsi, M. Durakiewicz, Tomasz Smith, J. L. TI Incomplete protection of the surface Weyl cones of the Kondo insulator SmB6: Spin exciton scattering SO PHYSICAL REVIEW B LA English DT Article ID HEAVY-FERMION SEMICONDUCTORS; MAGNETIC EXCITATIONS; NEUTRON-SCATTERING; SINGLE-CRYSTAL; MIXED-VALENCE; GAP; RESONANCE; LATTICE; STATES; YBB12 AB The compound SmB6 is a Kondo insulator, where the lowest-energy bulk electronic excitations are spin-excitons. It also has surface states that are subjected to strong spin-orbit coupling. It has been suggested that SmB6 is also a topological insulator. Here we show that, despite the absence of time-reversal symmetry breaking and the presence of strong spin-orbit coupling, the chiral spin texture of the Weyl cone is not completely protected. In particular, we show that the spin-exciton-mediated scattering produces features in the surface electronic spectrum at energies separated from the surface Fermi energy by the spin-exciton energy. Despite the features being far removed from the surface Fermi energy, they are extremely temperature dependent. The temperature variation occurs over a characteristic scale determined by the dispersion of the spin-exciton. The structures may be observed by electron spectroscopy at low temperatures. C1 [Kapilevich, G. A.; Riseborough, P. S.; Gray, A. X.] Temple Univ, Philadelphia, PA 19122 USA. [Gulacsi, M.] Max Planck Inst Phys Komplexer Syst, Dresden, Germany. [Durakiewicz, Tomasz; Smith, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Kapilevich, GA (reprint author), Temple Univ, Philadelphia, PA 19122 USA. RI Riseborough, Peter/D-4689-2011 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-01ER45872] FX The work at Temple was supported by an award from the U.S. Department of Energy, Office of Basic Energy Sciences, via Grant No. DE-FG02-01ER45872. P.S.R. acknowledges stimulating conversations with Pedro Schlottman, Collin Broholm, Wes Fuhrman, Laura Greene, and Wan-Kyu Park. T.D. acknowledges the NSF IR/D program. NR 58 TC 5 Z9 5 U1 12 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 20 PY 2015 VL 92 IS 8 AR 085133 DI 10.1103/PhysRevB.92.085133 PG 8 WC Physics, Condensed Matter SC Physics GA CP4OG UT WOS:000359861100001 ER PT J AU Mun, E Bud'ko, SL Lee, Y Martin, C Tanatar, MA Prozorov, R Canfield, PC AF Mun, E. Bud'ko, S. L. Lee, Y. Martin, C. Tanatar, M. A. Prozorov, R. Canfield, P. C. TI Quantum oscillations in the heavy-fermion compound YbPtBi SO PHYSICAL REVIEW B LA English DT Article ID MASSIVE ELECTRON STATE; PHASE-TRANSITIONS; TEMPERATURE; YBBIPT; SURFACE; MAGNETISM; BEHAVIOR; SYSTEMS; METALS; CEBIPT AB We present quantum oscillations observed in the heavy-fermion compound YbPtBi in magnetic fields far beyond its field-tuned, quantum critical point. Quantum oscillations are observed in magnetic fields as low as 60 kOe at 60 mK and up to temperatures as high as 3 K, which confirms the very high quality of the samples as well as the small effective mass of the conduction carriers far from the quantum critical point. Although the electronic specific heat coefficient of YbPtBi reaches similar to 7.4 J/mol K-2 in zero field, which is one of the highest effective mass values among heavy-fermion systems, it is suppressed quickly by an applied magnetic field. The quantum oscillations were used to extract the quasiparticle effective masses of the order of the bare electron mass, which is consistent with the behavior observed in specific heat measurements. Such small effective masses at high fields can be understood by considering the suppression of Kondo screening. C1 [Mun, E.; Bud'ko, S. L.; Lee, Y.; Martin, C.; Tanatar, M. A.; Prozorov, R.; Canfield, P. C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Mun, E.; Bud'ko, S. L.; Lee, Y.; Martin, C.; Tanatar, M. A.; Prozorov, R.; Canfield, P. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Mun, E.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. RP Mun, E (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. FU US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; US Department of Energy by Iowa State University [DE-AC02-07CH11358]; Natural Sciences and Engineering Research Council of Canada FX This work was supported by the US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The research was performed at the Ames Laboratory. Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. The work at Simon Fraser University was supported by the Natural Sciences and Engineering Research Council of Canada. NR 30 TC 1 Z9 1 U1 3 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 20 PY 2015 VL 92 IS 8 AR 085135 DI 10.1103/PhysRevB.92.085135 PG 5 WC Physics, Condensed Matter SC Physics GA CP4OG UT WOS:000359861100003 ER PT J AU Neupane, M Xu, SY Sankar, R Gibson, Q Wang, YJ Belopolski, I Alidoust, N Bian, G Shibayev, PP Sanchez, DS Ohtsubo, Y Taleb-Ibrahimi, A Basak, S Tsai, WF Lin, H Durakiewicz, T Cava, RJ Bansil, A Chou, FC Hasan, MZ AF Neupane, Madhab Xu, Su-Yang Sankar, R. Gibson, Q. Wang, Y. J. Belopolski, I. Alidoust, N. Bian, G. Shibayev, P. P. Sanchez, D. S. Ohtsubo, Y. Taleb-Ibrahimi, A. Basak, S. Tsai, W. -F. Lin, H. Durakiewicz, Tomasz Cava, R. J. Bansil, A. Chou, F. C. Hasan, M. Z. TI Topological phase diagram and saddle point singularity in a tunable topological crystalline insulator SO PHYSICAL REVIEW B LA English DT Article ID SPIN TEXTURE; PB1-XSNXSE; TRANSITION; GRAPHENE; SURFACE; SUPERCONDUCTIVITY; SUPERLATTICES; STATES; SNTE AB We report the evolution of the surface electronic structure and surface material properties of a topological crystalline insulator (TCI), Pb1-xSnxSe, as a function of various material parameters including composition x, temperature T, and crystal structure. Our spectroscopic data demonstrate the electronic ground-state condition for the saddle point singularity, the tunability of surface chemical potential, and the surface states' response to circularly polarized light. Our results show that each material parameter can tune the system between the trivial and topological phase in a distinct way, unlike that seen in Bi2Se3 and related compounds, leading to a rich topological phase diagram. Our systematic studies of the TCI Pb1-xSnxSe are a valuable materials guide to realize new topological phenomena. C1 [Neupane, Madhab; Xu, Su-Yang; Belopolski, I.; Alidoust, N.; Bian, G.; Shibayev, P. P.; Sanchez, D. S.; Hasan, M. Z.] Princeton Univ, Dept Phys, Joseph Henry Lab, Princeton, NJ 08544 USA. [Neupane, Madhab; Durakiewicz, Tomasz] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. [Sankar, R.; Chou, F. C.] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Gibson, Q.; Cava, R. J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Wang, Y. J.; Basak, S.; Bansil, A.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Wang, Y. J.] Lawrence Berkeley Natl Lab, Adv Light Source, Stanford, CA 94305 USA. [Ohtsubo, Y.; Taleb-Ibrahimi, A.] Synchrotron SOLEIL, F-91192 Gif Sur Yvette, France. [Taleb-Ibrahimi, A.] UR1 CNRS Synchrotron SOLEIL, F-91192 Gif Sur Yvette, France. [Tsai, W. -F.] Natl Sun Yat Sen Univ, Dept Phys, Kaohsiung 80424, Taiwan. [Lin, H.] Natl Univ Singapore, Ctr Adv Mat 2D, Singapore 117546, Singapore. [Lin, H.] Natl Univ Singapore, Graphene Res Ctr, Singapore 117546, Singapore. [Lin, H.] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore. [Hasan, M. Z.] Princeton Univ, Princeton Ctr Complex Mat, Princeton, NJ 08544 USA. RP Neupane, M (reprint author), Princeton Univ, Dept Phys, Joseph Henry Lab, Princeton, NJ 08544 USA. EM mneupane@lanl.gov; mzhasan@princeton.edu RI Bian, Guang/C-5182-2016; Lin, Hsin/F-9568-2012; Ohtsubo, Yoshiyuki/O-2052-2016 OI Bian, Guang/0000-0001-7055-2319; Lin, Hsin/0000-0002-4688-2315; Ohtsubo, Yoshiyuki/0000-0003-4388-825X FU Office of Basic Energy Sciences, US Department of Energy (DOE) [DE-FG-02-40105ER46200]; Gordon and Betty Moore Foundations EPiQS Initiative [GBMF4547]; DOE, Office of Science, Basic Energy Sciences [DE-FG02-07ER46352]; NERSC supercomputing center through DOE [DE-AC02-05CH11231]; NSF [DMR-0537588]; Singapore National Research Foundation under NRF Award [NRF-NRFF2013-03]; NSF IR/D program; LANL LDRD program; DOE/BES; A.P. Sloan Foundation FX The work at Princeton and synchrotron x-ray-based measurements are supported by the Office of Basic Energy Sciences, US Department of Energy (DOE) Grant No. DE-FG-02-40105ER46200 and partial instrumentation support provided by the Gordon and Betty Moore Foundations EPiQS Initiative through Grant GBMF4547 (M.Z.H.). The work at Northeastern University is supported by the DOE, Office of Science, Basic Energy Sciences Grant Number DE-FG02-07ER46352, and benefited from Northeastern University's Advanced Scientific Computation Center (ASCC) and the NERSC supercomputing center through DOE Grant Number DE-AC02-05CH11231. Use of the Synchrotron Radiation Center (SRC) was supported by the NSF (Grant No. DMR-0537588) under an external user agreement. H.L. acknowledges the Singapore National Research Foundation for the support under NRF Award No. NRF-NRFF2013-03. T.D. acknowledges support from the NSF IR/D program. M.N. at LANL acknowledges support from the LANL LDRD program. We thank Sung-Kwan Mo, Alexi Fedorov, and Makoto Hashimoto for beamline assistance at the LBNL and the SSRL. M.Z.H. acknowledges Visiting Scientist support from LBNL and additional support from DOE/BES and the A.P. Sloan Foundation. NR 47 TC 1 Z9 1 U1 4 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 20 PY 2015 VL 92 IS 7 AR 075131 DI 10.1103/PhysRevB.92.075131 PG 10 WC Physics, Condensed Matter SC Physics GA CP4NV UT WOS:000359859900003 ER PT J AU Henry, TW Bentley, MA Clark, RM Davies, PJ Bader, VM Baugher, T Bazin, D Beausang, CW Berryman, JS Bruce, AM Campbell, CM Crawford, HL Cromaz, M Fallon, P Gade, A Henderson, J Iwasaki, H Jenkins, DG Lee, IY Lemasson, A Lenzi, SM Macchiavelli, AO Napoli, DR Nichols, AJ Paschalis, S Petri, M Recchia, F Rissanen, J Simpson, EC Stroberg, SR Wadsworth, R Weisshaar, D Wiens, A Walz, C AF Henry, T. W. Bentley, M. A. Clark, R. M. Davies, P. J. Bader, V. M. Baugher, T. Bazin, D. Beausang, C. W. Berryman, J. S. Bruce, A. M. Campbell, C. M. Crawford, H. L. Cromaz, M. Fallon, P. Gade, A. Henderson, J. Iwasaki, H. Jenkins, D. G. Lee, I. Y. Lemasson, A. Lenzi, S. M. Macchiavelli, A. O. Napoli, D. R. Nichols, A. J. Paschalis, S. Petri, M. Recchia, F. Rissanen, J. Simpson, E. C. Stroberg, S. R. Wadsworth, R. Weisshaar, D. Wiens, A. Walz, C. TI Triplet energy differences and the low lying structure of Ga-62 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN STATES; SHELL-MODEL; IN-BEAM; NUCLEI; SYMMETRY; T=0; SPECTROSCOPY; MN-50 AB Background: Triplet energy differences (TED) can be studied to yield information on isospin-non-conserving interactions in nuclei. Purpose: The systematic behavior of triplet energy differences (TED) of T = 1, J(pi) = 2(+) states is examined. The A = 62 isobar is identified as having a TED value that deviates significantly from an otherwise very consistent trend. This deviation can be attributed to the tentative assignments of the pertinent states in Ga-62 and Ge-62. Methods: An in-beam gamma-ray spectroscopy experiment was performed to identify excited states in Ga-62 using Gamma-Ray Energy Tracking In-Beam Nuclear Array with the S800 spectrometer at NSCL using a two-nucleon knockout approach. Cross-section calculations for the knockout process and shell-model calculations have been performed to interpret the population and decay properties observed. Results: Using the systematics as a guide, a candidate for the transition from the T = 1, 2(+) state is identified. However, previous work has identified similar states with different J(pi) assignments. Cross-section calculations indicate that the relevant T = 1, 2(+) state should be one of the states directly populated in this reaction. Conclusions: As spins and parities were not measurable, it is concluded that an unambiguous identification of the first T = 1, 2(+) state is required to reconcile our understanding of TED systematics. C1 [Henry, T. W.; Bentley, M. A.; Davies, P. J.; Henderson, J.; Jenkins, D. G.; Nichols, A. J.; Simpson, E. C.; Wadsworth, R.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Clark, R. M.; Campbell, C. M.; Crawford, H. L.; Cromaz, M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Rissanen, J.; Wiens, A.] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bader, V. M.; Baugher, T.; Bazin, D.; Berryman, J. S.; Gade, A.; Iwasaki, H.; Lemasson, A.; Recchia, F.; Stroberg, S. R.; Weisshaar, D.; Walz, C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Bader, V. M.; Baugher, T.; Gade, A.; Iwasaki, H.; Lemasson, A.; Stroberg, S. R.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Beausang, C. W.] Univ Richmond, Richmond, VA 23173 USA. [Bruce, A. M.] Univ Brighton, Sch Comp Engn & Math, Brighton BN2 4GJ, E Sussex, England. [Lemasson, A.] GANIL, CNRS, CEA, DSM,IN2P3, F-14076 Caen 5, France. [Lenzi, S. M.] Dipartimento Fis & Astron, I-35131 Padua, Italy. [Lenzi, S. M.] INFN, Sez Padova, I-35131 Padua, Italy. [Napoli, D. R.] Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Paschalis, S.; Petri, M.; Walz, C.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. RP Henry, TW (reprint author), Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. RI Gade, Alexandra/A-6850-2008; Petri, Marina/H-4630-2016; Paschalis, Stefanos/H-8758-2016; Bruce, Alison/K-7663-2016; Napoli, Daniel R./D-9863-2012; OI Gade, Alexandra/0000-0001-8825-0976; Petri, Marina/0000-0002-3740-6106; Paschalis, Stefanos/0000-0002-9113-3778; Bruce, Alison/0000-0003-2871-0517; Napoli, Daniel R./0000-0002-8154-6958; Stroberg, Ragnar/0000-0002-0635-776X; Recchia, Francesco/0000-0002-8428-0112 FU UK Science and Technology Facilities Council (STFC) [ST/J000124/1, ST/L005727/1]; DOE, Office of Science; NSF (NSCL) [PHY-1102511]; DOE (LBNL) [DE-AC02-05CH11231]; Helmholtz International Center for FAIR within the framework of the LOEWE program FX The authors thank T. Ginter and J. Pereira for their effort during the experiment, and D. Rudolph and H. David for helpful discussions. This work was supported by the UK Science and Technology Facilities Council (STFC) through Grants No. ST/J000124/1 and No. ST/L005727/1. GRETINA was funded by the DOE, Office of Science. Operation of the array at NSCL was supported by NSF under Cooperative Agreement No. PHY-1102511 (NSCL) and DOE under Grant No. DE-AC02-05CH11231 (LBNL). M.P. acknowledges support from the Helmholtz International Center for FAIR within the framework of the LOEWE program (Landesoffensive zur Entwicklung Wissenschaftlich-Okonomischer Exzellenz) launched by the State of Hesse. NR 49 TC 0 Z9 0 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 20 PY 2015 VL 92 IS 2 AR 024315 DI 10.1103/PhysRevC.92.024315 PG 6 WC Physics, Nuclear SC Physics GA CP4PD UT WOS:000359863600002 ER PT J AU Jia, JY Radhakrishnan, S AF Jia, Jiangyong Radhakrishnan, Sooraj TI Limitation of multiparticle correlations for studying the event-by-event distribution of harmonic flow in heavy-ion collisions SO PHYSICAL REVIEW C LA English DT Article ID RELATIVISTIC NUCLEAR COLLISIONS; PLUS PB COLLISIONS; ANGULAR-CORRELATIONS; COLLECTIVE FLOW; ATLAS DETECTOR; LONG-RANGE; PPB; TEV; ANISOTROPY; PARTICLES AB The sensitivity of flow harmonics from cumulants to the event-by-event flow distribution p(nu(n)) is investigated using a simple central moment expansion approach. For a narrow distribution whose width is much smaller than the mean sigma(n) << , the differences between the first three higher-order cumulant estimates nu(n){4}, nu(n){6}, and nu(n){8} are not very sensitive to the shape of p(nu(n)). For a broad distribution sigma(n) greater than or similar to , the higher-order cumulant estimates differ from each other but may change sign and become ill defined. This sign change arises from the choice of p(nu(n)), without the need to invoke nonflow effects. Direct extraction of p(nu(n)) via a data-driven unfolding method used by the ATLAS experiment is a more preferred approach for flow distribution measurement. C1 [Jia, Jiangyong; Radhakrishnan, Sooraj] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Jia, Jiangyong] Brookhaven Natl Lab, Dept Phys, Upton, NY 11796 USA. RP Jia, JY (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM jjia@bnl.gov; sooraj9286@gmail.com FU NSF [PHY-1305037] FX We appreciate valuable comments and fruitful discussions with D. Teaney and A. Bilandzic. This research is supported by the NSF under Grant No. PHY-1305037. NR 37 TC 4 Z9 4 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 20 PY 2015 VL 92 IS 2 AR 024911 DI 10.1103/PhysRevC.92.024911 PG 7 WC Physics, Nuclear SC Physics GA CP4PD UT WOS:000359863600005 ER PT J AU Altunkaynak, B Baer, H Barger, V Huang, P AF Altunkaynak, Baris Baer, Howard Barger, Vernon Huang, Peisi TI Distinguishing LSP archetypes via gluino pair production at LHC13 SO PHYSICAL REVIEW D LA English DT Article ID SUPERSYMMETRIC STANDARD MODEL; PURE GRAVITY MEDIATION; GRAND UNIFIED THEORIES; NONUNIVERSAL HIGGS MASSES; LOCAL SUPERSYMMETRY; DARK-MATTER; BREAKING; SUPERGRAVITY; PARTICLE; BOSON AB The search for supersymmetry at run 1 of the LHC has resulted in gluino mass limits m((g) over tilde) greater than or similar to 1.3 TeV for the case where m((q) over tilde) >> m((g) over tilde) and in models with gaugino mass unification. The increased energy and, ultimately, luminosity of LHC13 will explore the range m((g) over tilde) similar to 1.3-2 TeV. We examine how the discovery of SUSY via gluino pair production would unfold via a comparative analysis of three LSP archetype scenarios: (1) mSUGRA/CMSSM model with a binolike LSP, (2) charged SUSY breaking (CSB) with a winolike LSP, and (3) SUSY with radiatively driven naturalness (RNS) and a Higgsino-like LSP. In all three cases we expect heavy-to-very-heavy squarks as suggested by a decoupling solution to the SUSY flavor and CP problems and by the gravitino problem. For all cases, initial SUSY discovery would likely occur in the multi-b-jet + (E) over bar (T) channel. The CSB scenario would be revealed by the presence of highly ionizing, terminating tracks from quasistable charginos. As further data accrue, the RNS scenario with 100-200 GeV Higgsino-like LSPs would be revealed by the buildup of a mass edge/bump in the opposite sign/same flavor dilepton invariant mass which is bounded by the neutralino mass difference. The mSUGRA/CMSSM archetype would contain neither of these features but would be revealed by a buildup of the usual multilepton cascade decay signatures. C1 [Altunkaynak, Baris; Baer, Howard] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Barger, Vernon] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Huang, Peisi] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Huang, Peisi] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. RP Altunkaynak, B (reprint author), Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. EM baris@nhn.ou.edu; baer@nhn.ou.edu; barger@pheno.wisc.edu; peisi@uchicago.edu OI Huang, Peisi/0000-0003-3360-2641 FU Center for Theoretical Underground Physics and Related Areas (CETUP); U.S. Department of Energy, Office of High Energy Physics FX The authors would like to thank the Center for Theoretical Underground Physics and Related Areas (CETUP) for its hospitality and partial support during the 2015 Summer Program. This work was supported in part by the U.S. Department of Energy, Office of High Energy Physics. NR 85 TC 6 Z9 6 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 20 PY 2015 VL 92 IS 3 AR 035015 DI 10.1103/PhysRevD.92.035015 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CP4PP UT WOS:000359864900006 ER PT J AU Rellan-Alvarez, R Lobet, G Lindner, H Pradier, PL Sebastian, J Yee, MC Geng, Y Trontin, C LaRue, T Schrager-Lavelle, A Haney, CH Nieu, R Maloof, J Vogel, JP Dinneny, JR AF Rellan-Alvarez, Ruben Lobet, Guillaume Lindner, Heike Pradier, Pierre-Luc Sebastian, Jose Yee, Muh-Ching Geng, Yu Trontin, Charlotte LaRue, Therese Schrager-Lavelle, Amanda Haney, Cara H. Nieu, Rita Maloof, Julin Vogel, John P. Dinneny, Jose R. TI GLO-Roots: an imaging platform enabling multidimensional characterization of soil-grown root systems SO ELIFE LA English DT Article ID BOX PROTEIN TIR1; ARABIDOPSIS SEEDLINGS; AUXIN RECEPTOR; ARCHITECTURE; BRACHYPODIUM; REPORTER; SHAPE; PHOTOMORPHOGENESIS; EXPRESSION; MECHANISM AB Root systems develop different root types that individually sense cues from their local environment and integrate this information with systemic signals. This complex multi-dimensional amalgam of inputs enables continuous adjustment of root growth rates, direction, and metabolic activity that define a dynamic physical network. Current methods for analyzing root biology balance physiological relevance with imaging capability. To bridge this divide, we developed an integrated-imaging system called Growth and Luminescence Observatory for Roots (GLO-Roots) that uses luminescence-based reporters to enable studies of root architecture and gene expression patterns in soil-grown, light-shielded roots. We have developed image analysis algorithms that allow the spatial integration of soil properties, gene expression, and root system architecture traits. We propose GLO-Roots as a system that has great utility in presenting environmental stimuli to roots in ways that evoke natural adaptive responses and in providing tools for studying the multi-dimensional nature of such processes. C1 [Rellan-Alvarez, Ruben; Lindner, Heike; Pradier, Pierre-Luc; Sebastian, Jose; Yee, Muh-Ching; Geng, Yu; Trontin, Charlotte; Dinneny, Jose R.] Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA. [Lobet, Guillaume] Univ Liege, PhytoSyst, Liege, Belgium. [Geng, Yu; Vogel, John P.] US DOE, Joint Genome Inst, Walnut Creek, PA USA. [LaRue, Therese] Stanford Univ, Dept Biol, Stanford, CA 94305 USA. [Schrager-Lavelle, Amanda; Maloof, Julin] Univ Calif Davis, Dept Plant Biol, Davis, CA 95616 USA. [Haney, Cara H.] Harvard Univ, Massachusetts Gen Hosp, Sch Med, Dept Genet,Dept Mol Biol, Boston, MA USA. [Nieu, Rita] USDA, Western Reg Res Ctr, Albany, CA USA. RP Dinneny, JR (reprint author), Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA. EM jdinneny@carnegiescience.edu OI Yee, Muh-ching/0000-0002-0445-7927; Sebastian, Jose/0000-0002-1826-0308; Vogel, John/0000-0003-1786-2689; Rellan-Alvarez, Ruben/0000-0001-6843-3716 FU National Science Foundation [MCB-115795, MCB-0519898, IOS-0820854]; U.S. Department of Energy [DE-SC0008769, DE-AI02-07ER64452]; National Institutes of Health [GM48707]; Fonds De La Recherche Scientifique - FNRS (Belgian National Fund for Scientific Research); Consejo Nacional de Ciencia y Tecnologia (National Council of Science and Technology, Mexico) [CB-2014-01-238101] FX National Science Foundation MCB-115795 Jose R Dinneny; U.S. Department of Energy DE-SC0008769 Jose R Dinneny; National Science Foundation MCB-0519898 Cara H Haney; National Science Foundation IOS-0820854 Amanda Schrager-Lavelle, Julin Maloof; National Institutes of Health GM48707 Cara H Haney; Fonds De La Recherche Scientifique - FNRS (Belgian National Fund for Scientific Research) Guillaume Lobet; Consejo Nacional de Ciencia y Tecnologia (National Council of Science and Technology, Mexico) CB-2014-01-238101 Ruben Rellan-Alvarez; U.S. Department of Energy DE-AI02-07ER64452 John P Vogel; The funders had no role in study design, data collection and interpretation, or the decision to submit the work for publication. NR 58 TC 15 Z9 15 U1 7 U2 18 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 19 PY 2015 VL 4 AR e07597 DI 10.7554/eLife.07597 PG 26 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DI9HU UT WOS:000373814300001 ER PT J AU Picon, A Mompart, J Southworth, SH AF Picon, Antonio Mompart, Jordi Southworth, Stephen H. TI Stimulated Raman adiabatic passage with two-color x-ray pulses SO NEW JOURNAL OF PHYSICS LA English DT Article DE XFEL; STIRAP; quantum control ID FREE-ELECTRON LASER; COHERENT POPULATION TRANSFER; EXTREME-ULTRAVIOLET; DELAYED PULSES; LIGHT; SCATTERING; MOLECULES; SPECTRA; CO; SELECTIVITY AB Recent techniques in x-ray free electron lasers allow the generation of highly coherent, intense x-ray pulses with time lengths on the order of femtoseconds. Here we explore the possibilities of using such x-ray pulses to control matter based on coherence. In particular we propose a theoretical scheme to perform stimulated Raman adiabatic passage in the x-ray regime by using inner-hole excited states. Numerical results in two well-known systems, the neon atom and the carbon monoxide molecule, show a robust control of population transfer. In the molecule, vibrational selectivity is achieved with femtosecond x-ray pulses. This work supports the possibility of using two-color x-ray pulses for coherent control. C1 [Picon, Antonio; Southworth, Stephen H.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mompart, Jordi] Univ Autonoma Barcelona, Dept Fis, E-08193 Bellaterra, Spain. RP Picon, A (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM apicon@anl.gov RI Mompart, Jordi/F-9698-2011 OI Mompart, Jordi/0000-0002-9634-9455 FU US Department of Energy, Basic Energy Sciences, Office of Science [DE-AC02-06CH11357] FX We acknowledge discussions with L Cheng about calculating dipole transitions with CFOUR and RW Dunford about metastable states in neon. We also acknowledge fruitful discussions with P Bucksbaum, W Jakubetz, D Moonshiram, P Ho, G Doumy, CS Lehmann, A Zholents, A Marinelli, A Lutman, and C Bostedt, and the financial support of the US Department of Energy, Basic Energy Sciences, Office of Science, under contract # DE-AC02-06CH11357. NR 54 TC 2 Z9 2 U1 4 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD AUG 19 PY 2015 VL 17 AR 083038 DI 10.1088/1367-2630/17/8/083038 PG 7 WC Physics, Multidisciplinary SC Physics GA CQ9TB UT WOS:000360956900001 ER PT J AU Cao, RG Xu, W Lv, DP Xiao, J Zhang, JG AF Cao, Ruiguo Xu, Wu Lv, Dongping Xiao, Jie Zhang, Ji-Guang TI Anodes for Rechargeable Lithium-Sulfur Batteries SO ADVANCED ENERGY MATERIALS LA English DT Review ID LI-S BATTERIES; SOLID-ELECTROLYTE INTERPHASE; GEL POLYMER ELECTROLYTE; IONIC LIQUID ELECTROLYTES; ELECTROSTATIC SHIELD MECHANISM; ETHER-BASED ELECTROLYTES; HIGH SPECIFIC ENERGY; ELECTROCHEMICAL PERFORMANCE; SECONDARY BATTERIES; COMPOSITE ELECTRODE AB With the significant progress that has been made toward the development of cathode materials and electrolytes in lithium-sulfur (Li-S) batteries in recent years, the stability of the anode in Li-S batteries has become one of the more urgent challenges in order to reach long-term stability of Li-S batteries. In Li-S batteries, a passivation layer is easily formed on the metallic Li anode surface because of the presence of polysulfides and electrolyte additives. Although the passivation layer on the Li metal anode can significantly suppress Li dendrite growth and improve the safety of Li-S batteries, continuous corrosion of the Li metal anode eventually leads to battery failure due to the increased cell impedance and the depletion of electrolyte. Here, the recent developments on the protection of the Li metal anode in Li-S batteries are reviewed. Various strategies used to minimize the corrosion of Li anodes and to reduce its impedance increase are analyzed. Other alternative anodes used in sulfur-based rechargeable batteries are also discussed. C1 [Cao, Ruiguo; Xu, Wu; Lv, Dongping; Xiao, Jie; Zhang, Ji-Guang] Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Energy & Environm Directorate, Richland, WA 99354 USA. RP Zhang, JG (reprint author), Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Energy & Environm Directorate, Richland, WA 99354 USA. EM Jiguang.Zhang@pnnl.gov RI Cao, Ruiguo/O-7354-2016; OI Xu, Wu/0000-0002-2685-8684 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences. NR 161 TC 50 Z9 50 U1 150 U2 634 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1402273 DI 10.1002/aenm.201402273 PG 23 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100005 ER PT J AU Cuisinier, M Hart, C Balasubramanian, M Garsuch, A Nazar, LF AF Cuisinier, Marine Hart, Connor Balasubramanian, Mahalingam Garsuch, Arnd Nazar, Linda F. TI Radical or Not Radical: Revisiting Lithium-Sulfur Electrochemistry in Nonaqueous Electrolytes SO ADVANCED ENERGY MATERIALS LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; LI-S BATTERIES; ENERGY DENSITY; PERFORMANCE; REDUCTION; POLYSULFIDES; REACTIVITY; STABILITY; OXYGEN; CELL C1 [Cuisinier, Marine; Hart, Connor; Nazar, Linda F.] Univ Waterloo, Dept Chem, Waterloo Inst Nanotechnol, 200 Univ Ave W, Waterloo, ON N2L 3G1, Canada. [Balasubramanian, Mahalingam] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Garsuch, Arnd] BASF SE, D-67056 Ludwigshafen, Germany. RP Nazar, LF (reprint author), Univ Waterloo, Dept Chem, Waterloo Inst Nanotechnol, 200 Univ Ave W, Waterloo, ON N2L 3G1, Canada. EM lfnazar@uwaterloo.ca OI Cuisinier, Marine/0000-0002-0690-9755; Nazar, Linda/0000-0002-3314-8197 FU BASF International Scientific Network for Electrochemistry and Batteries; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-GeoSciences [DE-FG02-94ER14466]; DOE Office of Science by the Argonne National Laboratory [DE-AC02-06CH11357] FX The research was supported by the BASF International Scientific Network for Electrochemistry and Batteries. XANES experiments were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and the Department of Energy-GeoSciences (DE-FG02-94ER14466). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by the Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors thank Dr. M. Newville and Dr. A. Lanzirotti for helping with the acquisition of the XANES data at the APS. NR 39 TC 31 Z9 31 U1 14 U2 146 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR UNSP 1401801 DI 10.1002/aenm.201401801 PG 6 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100002 ER PT J AU Lv, DP Zheng, JM Li, QY Xie, X Ferrara, S Nie, ZM Mehdi, LB Browning, ND Zhang, JG Graff, GL Liu, J Xiao, J AF Lv, Dongping Zheng, Jianming Li, Qiuyan Xie, Xi Ferrara, Seth Nie, Zimin Mehdi, Layla B. Browning, Nigel D. Zhang, Ji-Guang Graff, Gordon L. Liu, Jun Xiao, Jie TI High Energy Density Lithium-Sulfur Batteries: Challenges of Thick Sulfur Cathodes SO ADVANCED ENERGY MATERIALS LA English DT Article ID LI-S BATTERIES; ELECTROCHEMICAL PERFORMANCE; RECHARGEABLE BATTERIES; LIQUID ELECTROLYTE; POROUS CARBON; CYCLE LIFE; BINDER; COMPOSITE; CELLS; CAPACITY AB High energy and cost-effective lithium sulfur (Li-S) battery technology has been vigorously revisited in recent years due to the urgent need of advanced energy storage technologies for green transportation and large-scale energy storage applications. However, the market penetration of Li-S batteries has been plagued due to the gap in scientific knowledge between the fundamental research and the real application need. Here, a facile and effective approach to integrate commercial carbon nanoparticles into microsized secondary ones for application in high loading sulfur electrodes is proposed The slurry with the integrated particles is easily cast into electrode laminates with practically usable mass loadings. Uniform and crack-free coating with high loading of 2-8 mg cm(-2) sulfur are successfully achieved. Based on the obtained thick electrodes, the dependence of areal specific capacity on mass loading, factors influencing electrode performance, and measures used to address the existing issues are studied and discussed. C1 [Lv, Dongping; Zheng, Jianming; Li, Qiuyan; Xie, Xi; Ferrara, Seth; Nie, Zimin; Zhang, Ji-Guang; Graff, Gordon L.; Liu, Jun; Xiao, Jie] Pacific NW Natl Lab, Energy & Environm Directorate, Electrochem Mat & Syst Grp, Richland, WA 99352 USA. [Mehdi, Layla B.; Browning, Nigel D.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Xiao, J (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Electrochem Mat & Syst Grp, Richland, WA 99352 USA. EM Jie.Xiao@pnnl.gov RI Zheng, Jianming/F-2517-2014; OI Zheng, Jianming/0000-0002-4928-8194; Browning, Nigel/0000-0003-0491-251X FU Office of Vehicle Technologies of the U.S. Department of Energy (DOE) [DEAC02-05CH11231]; Office of Vehicle Technologies of the U.S. Department of Energy (DOE) under Batteries for Advanced Transportation Technologies (BATT) program [DEAC02-98CH10886]; DOE's Office of Biological and Environmental Research (BER); DOE [DE-AC05-76RLO1830] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) under Contract No. DEAC02-05CH11231 for PNNL and under DEAC02-98CH10886 under the Batteries for Advanced Transportation Technologies (BATT) program. The SEM characterization was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL)-a national scientific user facility located at PNNL, which is sponsored, by the DOE's Office of Biological and Environmental Research (BER). PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RLO1830. NR 64 TC 48 Z9 48 U1 39 U2 181 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1402290 DI 10.1002/aenm.201402290 PG 8 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100006 ER PT J AU Pan, HL Wei, XL Henderson, WA Shao, YY Chen, JZ Bhattacharya, P Xiao, J Liu, J AF Pan, Huilin Wei, Xiaoliang Henderson, Wesley A. Shao, Yuyan Chen, Junzheng Bhattacharya, Priyanka Xiao, Jie Liu, Jun TI On the Way Toward Understanding Solution Chemistry of Lithium Polysulfides for High Energy Li-S Redox Flow Batteries SO ADVANCED ENERGY MATERIALS LA English DT Article ID IONIC LIQUID ELECTROLYTES; X-RAY-DIFFRACTION; SULFUR BATTERIES; IN-SITU; POLYMER ELECTROLYTES; SOLVATE STRUCTURES; PHASE-BEHAVIOR; STORAGE; DENSITY; CATHODE AB Lithium-sulfur (Li-S) redox flow battery (RFB) is a promising candidate for high energy large-scale energy storage application due to good solubility of long-chain polysulfide species and low cost of sulfur. Here, the fundamental understanding and control of lithium polysulfide chemistry are studied to enable the development of liquid phase Li-S redox flow prototype cells. These differ significantly from conventional static Li-S batteries targeting for vehicle electrification. A high solubility of the different lithium polysulfides generated at different depths of discharge and states of charge is required for a flow battery in order to take full advantage of the multiple electron transitions. A new dimethyl sulfoxide based electrolyte is proposed for Li-S RFBs, which not only enables the high solubility of lithium polysulfide species, especially for the short-chain species, but also results in excellent cycling with a high Coulombic efficiency. The challenges and opportunities for the Li-S redox flow concept have also been discussed in depth. C1 [Pan, Huilin; Wei, Xiaoliang; Shao, Yuyan; Chen, Junzheng; Xiao, Jie; Liu, Jun] Joint Ctr Energy Storage Res, Washington, DC 20005 USA. [Pan, Huilin; Wei, Xiaoliang; Henderson, Wesley A.; Shao, Yuyan; Chen, Junzheng; Bhattacharya, Priyanka; Xiao, Jie; Liu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Xiao, J (reprint author), Joint Ctr Energy Storage Res, Washington, DC 20005 USA. EM jie.xiao@pnnl.gov; jun.liu@pnnl.gov RI Shao, Yuyan/A-9911-2008; Pan, Huilin/J-9298-2016 OI Shao, Yuyan/0000-0001-5735-2670; FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; U.S. Department of Energy's Office of Biological and Environmental Research FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The Raman and SEM analyses were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). NR 50 TC 14 Z9 14 U1 19 U2 139 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR UNSP 1500113 DI 10.1002/aenm.201500113 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100010 ER PT J AU Wujcik, KH Pascal, TA Pemmaraju, CD Devaux, D Stolte, WC Balsara, NP Prendergast, D AF Wujcik, Kevin H. Pascal, Tod A. Pemmaraju, C. D. Devaux, Didier Stolte, Wayne C. Balsara, Nitash P. Prendergast, David TI Characterization of Polysulfide Radicals Present in an Ether-Based Electrolyte of a Lithium-Sulfur Battery During Initial Discharge Using In Situ X-Ray Absorption Spectroscopy Experiments and First-Principles Calculations SO ADVANCED ENERGY MATERIALS LA English DT Article ID BLOCK-COPOLYMER ELECTROLYTES; ELECTROCHEMICAL REDUCTION; PSEUDOPOTENTIALS; MEDIA; SPECIATION; PRODUCTS; SOLVENTS; SPECTRA AB The presence and role of polysulfide radicals in the electrochemical processes of lithium sulfur (Li-S) batteries is currently being debated. Here, first-principles interpretations of measured X-ray absorption spectra (XAS) of Li-S cells are leveraged with an ether-based electrolyte. Unambiguous evidence is found for significant quantities of polysulfide radical species (LiS3, LiS4, and LiS5), including the trisulfur radical anion S-3(-), present after initial discharge to the first discharge plateau, as evidenced by a low energy shoulder in the S K-edge XAS below 2469 eV. This feature is not present in the XAS of cells at increased depth of discharge, which, by our analysis, exhibit increasing concentrations of progressively shorter polysulfide dianions. Through a combination of first-principles molecular dynamics and associated interpretation of in situ XAS of Li-S cells, atomic level insights into the chemistries are provided that underlie the operation and stability of these batteries. C1 [Wujcik, Kevin H.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Pascal, Tod A.; Pemmaraju, C. D.; Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Devaux, Didier] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Stolte, Wayne C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu; dgprendergast@lbl.gov RI Foundry, Molecular/G-9968-2014 FU Office of Vehicle Technologies of the US Department of Energy under the Batteries for Advanced Transportation Technologies program [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231] FX K.H.W. and T.A.P. contributed equally to this work. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the US Department of Energy under Contract DE-AC02-05CH11231 under the Batteries for Advanced Transportation Technologies program. Theoretical work was supported by a User Project at The Molecular Foundry and calculations were performed at NERSC, while XAS measurements were made at The Advanced Light Source. The Berkeley Lab User Facilities are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 49 TC 9 Z9 9 U1 20 U2 83 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1500285 DI 10.1002/aenm.201500285 PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100017 ER PT J AU Xu, R Lu, J Amine, K AF Xu, Rui Lu, Jun Amine, Khalil TI Progress in Mechanistic Understanding and Characterization Techniques of Li-S Batteries SO ADVANCED ENERGY MATERIALS LA English DT Review ID LITHIUM-SULFUR BATTERIES; X-RAY-DIFFRACTION; IONIC-LIQUID ELECTROLYTE; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; DISCHARGE REACTION-MECHANISM; METAL-ORGANIC FRAMEWORK; GLYCOL) DIMETHYL ETHER; NITROGEN-DOPED CARBON; HIGH SPECIFIC ENERGY; IN-SITU AB Rechargeable lithium-sulfur batteries that operate at room temperature have attracted much research interest as next-generation energy storage systems. Although tremendous advances have been made with Li-S batteries, great challenges still exist in achieving high capacity, high loading, high coulombic efficiency, and long cycle life. These challenges arise from the system complexity, lack of mechanistic understanding of the redox reaction, and operational limitations of Li-S cells. The focus here is on the recent gains in fundamental understanding of the Li-S redox reaction mechanism based on the application of advanced characterization techniques. Research results that help with the understanding of the close relationship between cell design (including development of new and advanced electrode materials, electrolytes, separators, binders, and cell configurations), the Li-S reaction mechanism, characterization methods, and Li-S battery performance are discussed. C1 [Xu, Rui; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Lu, J (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. EM junlu@anl.gov; amine@anl.gov FU U.S. Department of Energy [DE-AC0206CH11357]; Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) FX This work was supported by the U.S. Department of Energy under Contract DE-AC0206CH11357 with the main support provided by the Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE). The authors are also thankful for useful discussions with Dr. David Howell and Mr. Tien Duong of the EERE Vehicle Technologies Office. NR 203 TC 46 Z9 46 U1 88 U2 315 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1500408 DI 10.1002/aenm.201500408 PG 22 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100018 ER PT J AU Yu, XQ Pan, HL Zhou, YN Northrup, P Xiao, J Bak, S Liu, MZ Nam, KW Qu, DY Liu, J Wu, TP Yang, XQ AF Yu, Xiqian Pan, Huilin Zhou, Yongning Northrup, Paul Xiao, Jie Bak, Seongmin Liu, Mingzhao Nam, Kyung-Wan Qu, Deyang Liu, Jun Wu, Tianpin Yang, Xiao-Qing TI Direct Observation of the Redistribution of Sulfur and Polysufides in Li-S Batteries During the First Cycle by In Situ X-Ray Fluorescence Microscopy SO ADVANCED ENERGY MATERIALS LA English DT Article ID ABSORPTION-SPECTROSCOPY; ENERGY-STORAGE; POLYSULFIDE DISSOLUTION; HIGH-CAPACITY; LITHIUM; DIFFRACTION; CATHODE; ELECTROLYTE; CHEMISTRY C1 [Yu, Xiqian; Zhou, Yongning; Northrup, Paul; Bak, Seongmin; Liu, Mingzhao; Yang, Xiao-Qing] Brookhaven Natl Lab, Upton, NY 11973 USA. [Pan, Huilin; Xiao, Jie; Liu, Jun] Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Richland, WA 99352 USA. [Nam, Kyung-Wan] Dongguk Univ Seoul, Dept Energy & Mat Engn, Seoul 100715, South Korea. [Qu, Deyang] Univ Massachusetts, Dept Chem, Boston, MA 02125 USA. Argonne Natl Lab, Xray Sci Div, Lemont, IL 60439 USA. RP Yang, XQ (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM xyang@bnl.gov RI Liu, Mingzhao/A-9764-2011; Yu, Xiqian/B-5574-2014; Pan, Huilin/J-9298-2016; Nam, Kyung-Wan/E-9063-2015; Bak, Seong Min/J-4597-2013; OI Liu, Mingzhao/0000-0002-0999-5214; Yu, Xiqian/0000-0001-8513-518X; Nam, Kyung-Wan/0000-0001-6278-6369; Bak, Seong-Min/0000-0002-1626-5949 FU U.S. Department of Energy (DOE), Office of Vehicle Technologies [DE-SC0012704]; U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES); Energy Efficiency & Resources of the Korea Institute of Energy Technology Evaluation and Planning - Korea government Ministry of Trade, Industry Energy [20142020103090]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704]; U.S. DOE [DE-AC02-06CH11357] FX X.Y. and H.P. contributed equally to this paper. This work at BNL was supported by the U.S. Department of Energy (DOE), the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies under Contract No. DE-SC0012704. The research performed by the scientists at the Pacific Northwest National Laboratory (PNNL) was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES). Dr. Kyung-Wan Nam is supported by the Energy Efficiency & Resources of the Korea Institute of Energy Technology Evaluation and Planning grant funded by the Korea government Ministry of Trade, Industry & Energy (Project No. 20142020103090). SEM characterization was performed at the Center for Functional Nanomaterials (BNL), which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. The authors acknowledge technical supports by the scientists at beamline X15B, X14A of NSLS (BNL) and 9-BM-B of APS (ANL), supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 39 TC 7 Z9 7 U1 23 U2 79 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1500072 DI 10.1002/aenm.201500072 PG 6 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100008 ER PT J AU Zheng, D Qu, DY Yang, XQ Yu, XQ Lee, HS Qu, DY AF Zheng, Dong Qu, Deyu Yang, Xiao-Qing Yu, Xiqian Lee, Hung-Sui Qu, Deyang TI Quantitative and Qualitative Determination of Polysulfide Species in the Electrolyte of a Lithium-Sulfur Battery using HPLC ESI/MS with One-Step Derivatization SO ADVANCED ENERGY MATERIALS LA English DT Article ID LI-S BATTERY; CHROMATOGRAPHIC-SEPARATION; ELECTROCHEMICAL REDUCTION; MEDIA C1 [Zheng, Dong; Qu, Deyang] Univ Massachusetts, Dept Chem, Boston, MA 02125 USA. [Qu, Deyu] Wuhan Univ Technol, Dept Chem, Sch Sci, Wuhan 430070, Hubei, Peoples R China. [Yang, Xiao-Qing; Yu, Xiqian; Lee, Hung-Sui] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Qu, DY (reprint author), Univ Massachusetts, Dept Chem, Boston, MA 02125 USA. EM Deyang.qu@umb.edu RI Zheng, Dong/J-9975-2015; Yu, Xiqian/B-5574-2014 OI Zheng, Dong/0000-0002-5824-3270; Yu, Xiqian/0000-0001-8513-518X FU Office of Vehicle Technologies of the U.S. Department of Energy [DEAC02-98CH10886]; Fundamental Research Funds for the Central Universities China FX The authors from UMB and BNL are indebted to the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy for financial support under Contract No. DEAC02-98CH10886. The author from WUT is grateful for the partially supported by the Fundamental Research Funds for the Central Universities China. NR 23 TC 8 Z9 8 U1 13 U2 50 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1401888 DI 10.1002/aenm.201401888 PG 5 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100003 ER PT J AU Zhou, WD Wang, CM Zhang, QL Abruna, HD He, Y Wang, JW Mao, SX Xiao, XC AF Zhou, Weidong Wang, Chongmin Zhang, Qinglin Abruna, Hector D. He, Yang Wang, Jiangwei Mao, Scott X. Xiao, Xingcheng TI Tailoring Pore Size of Nitrogen-Doped Hollow Carbon Nanospheres for Confining Sulfur in Lithium-Sulfur Batteries SO ADVANCED ENERGY MATERIALS LA English DT Article ID CATHODE; PERFORMANCE; POLYSULFIDES; NANOFIBERS; STABILITY; POROSITY C1 [Zhou, Weidong; Zhang, Qinglin; Xiao, Xingcheng] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA. [Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Abruna, Hector D.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. [He, Yang; Wang, Jiangwei; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. RP Xiao, XC (reprint author), Gen Motors Global Res & Dev Ctr, 30500 Mound Rd, Warren, MI 48090 USA. EM xingcheng.xiao@gm.com RI Wang, Jiangwei/F-8249-2011; Zhang, Qinglin/D-9258-2013 OI Wang, Jiangwei/0000-0003-1191-0782; Zhang, Qinglin/0000-0001-5933-4361 FU Vehicle Technologies Office of the U.S. Department of Energy under Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231, 7056410] FX The authors acknowledge the support by the Assistant Secretary for Energy Efficiency and Renewable Energy, Vehicle Technologies Office of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 7056410 under the Batteries for Advanced Transportation Technologies (BATT) Program. They also would like to thank Yang He and Jiangwei Wang for helping conduct in situ TEM at PNNL. NR 33 TC 44 Z9 45 U1 30 U2 122 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 19 PY 2015 VL 5 IS 16 SI SI AR 1401752 DI 10.1002/aenm.201401752 PG 8 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CQ1OV UT WOS:000360368100001 ER PT J AU Cheng, L Wu, CH Jarry, A Chen, W Ye, YF Zhu, JF Kostecki, R Persson, K Guo, JH Salmeron, M Chen, GY Doeff, M AF Cheng, Lei Wu, Cheng Hao Jarry, Angelique Chen, Wei Ye, Yifan Zhu, Junfa Kostecki, Robert Persson, Kristin Guo, Jinghua Salmeron, Miguel Chen, Guoying Doeff, Marca TI Interrelationships among Grain Size, Surface Composition, Air Stability, and Interfacial Resistance of Al-Substituted Li7La3Zr2O12 Solid Electrolytes SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE interface; interfacial resistance; solid electrolyte; solid state battery; surface stability ID IONIC-CONDUCTIVITY; ELECTROCHEMICAL PROPERTIES; CONDUCTORS LI7LA3ZR2O12; LITHIUM; MICROSTRUCTURE; RAMAN; PHOSPHATE; ENERGY; METAL; GE AB The interfacial resistances of symmetrical lithium cells containing Al-substituted Li7La3Zr2O12 (LLZO) solid electrolytes are sensitive to their microstructures and histories of exposure to air. Air exposure of LLZO samples with large grain sizes (similar to 150 mu m) results in dramatically increased interfacial impedances in cells containing them, compared to those with pristine large-grained samples. In contrast, a much smaller difference is seen between cells with small-grained (similar to 20 mu m) pristine and air-exposed LLZO samples. A combination of soft X-ray absorption (sXAS) and Raman spectroscopy, with probing depths ranging from nanometer to micrometer scales, revealed that the small-grained LLZO pellets are more air-stable than large-grained ones, forming far less surface Li2CO3 under both short- and long-term exposure conditions. Surface sensitive X-ray photoelectron spectroscopy (XPS) indicates that the better chemical stability of the small-grained LLZO is related to differences in the distribution of Al and Li at sample surfaces. Density functional theory calculations show that LLZO can react via two different pathways to form Li2CO3. The first, more rapid, pathway involves a reaction with moisture in air to form LiOH, which subsequently absorbs CO2 to form Li2CO3. The second, slower, pathway involves direct reaction with CO2 and is favored when surface lithium contents are lower, as with the small-grained samples. These observations have important implications for the operation of solid-state lithium batteries containing LLZO because the results suggest that the interfacial impedances of these devices is critically dependent upon specific characteristics of the solid electrolyte and how it is prepared. C1 [Cheng, Lei; Jarry, Angelique; Chen, Wei; Kostecki, Robert; Persson, Kristin; Chen, Guoying; Doeff, Marca] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Cheng, Lei; Salmeron, Miguel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wu, Cheng Hao] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Wu, Cheng Hao; Salmeron, Miguel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Ye, Yifan; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Peoples R China. RP Cheng, L (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. EM leicheng@lbl.gov; mmdoeff@lbl.gov RI Wu, Cheng Hao/C-9565-2014; Zhu, Junfa/E-4020-2010; Chen, Wei/B-3045-2012 OI Zhu, Junfa/0000-0003-0888-4261; Chen, Wei/0000-0002-1135-7721 FU Assistant Secretary for Energy Efficiency and Renewable Energy; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-ACO2-05CH11231]; Director Office of Science; Materials Project Center (BES DOE) [EDCBEE]; Advanced Light Source Doctoral Fellowship; Office of Vehicle Technologies; Chemical Sciences, Geosciences, and Biosciences Division FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies and the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences of the U.S. Department of Energy under contract no. DE-ACO2-05CH11231. The Advanced Light Source is supported by the Director Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. L.C., G.C, and M.D acknowledge illuminating discussions with Dr. Thomas Richardson. Prof. Lutgard De Jonghe is cordially acknowledged for the discussion on solid electrolytes. L.C. would like to acknowledge Mr. James Wu and Mr. Yuyi Li for assistance with instruments and Dr. Wanli Yang and Dr. Ruimin Qiao for helpful discussion on soft X-ray spectroscopy. W.C. gratefully acknowledges the Materials Project Center (BES DOE Grant No. EDCBEE) for funding support. C.H.W. acknowledges the Advanced Light Source Doctoral Fellowship in Residence. NR 42 TC 9 Z9 10 U1 37 U2 145 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 19 PY 2015 VL 7 IS 32 BP 17649 EP 17655 DI 10.1021/acsami.5b02528 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CP6VU UT WOS:000360027100016 PM 26192634 ER PT J AU Tian, CX Zhu, LP Lin, F Boyes, SG AF Tian, Chixia Zhu, Liping Lin, Feng Boyes, Stephen G. TI Poly(acrylic acid) Bridged Gadolinium Metal-Organic Framework-Gold Nanoparticle Composites as Contrast Agents for Computed Tomography and Magnetic Resonance Bimodal Imaging SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE multimodal imaging contrast agent; MRI/CT; gold nanoparticles; gadolinium metal organic framework nanoparticles ID SEMICONDUCTOR QUANTUM DOTS; BIOMEDICAL APPLICATIONS; MULTIFUNCTIONAL NANOPARTICLES; RAFT POLYMERIZATION; PARTICLE-SIZE; CANCER; THERAPY; CT; POLYMERS; NANORODS AB Imaging contrast agents for magnetic resonance imaging (MRI) and computed tomography (CT) have received significant attention in the development of techniques for early stage cancer diagnosis. Gadolinium (Gd)(III), which has seven unpaired electrons and a large magnetic moment, can dramatically influence the water proton relaxation and hence exhibits excellent MRI contrast. On the other hand, gold (Au), which has a high atomic number and high X-ray attenuation coefficient, is an ideal contrast agent candidate for X-ray-based CT imaging. Gd metal organic framework (MOF) nanopartides with tunable size, high Gd(III) loading and multivalency can potentially overcome the limitations of clinically utilized Gd chelate contrast agents. In this work, we report for the first time the integration of GdMOF nanopartides with gold nanopartides (AuNPs) for the preparation of a MRI/CT bimodal imaging agent. Highly stable hybrid GdMOF/AuNPs composites have been prepared by using poly(acrylic acid) as a bridge between the GdMOF nanopartides and AuNPs. The hybrid nanocomposites were then evaluated in MM and CT imaging. The results revealed high longitudinal relaxivity in MM and excellent CT imaging performance. Therefore, these GdMOF/AuNPs hybrid nanocomposites potentially provide a new platform for the development of multimodal imaging probes. C1 [Tian, Chixia; Zhu, Liping; Boyes, Stephen G.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Lin, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Boyes, SG (reprint author), Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. EM sboyes@mines.edu FU State of Colorado; Colorado School of Mines FX The authors thank the State of Colorado for providing a Bioscience Discovery Evaluation Proof of Concept Grant and the Colorado School of Mines for providing a Proof of Concept grant to support this work. NR 63 TC 5 Z9 5 U1 35 U2 148 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 19 PY 2015 VL 7 IS 32 BP 17765 EP 17775 DI 10.1021/acsami.5b03998 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CP6VU UT WOS:000360027100029 PM 26147906 ER PT J AU Page, KA Shin, JW Eastman, SA Rowe, BW Kim, S Kusoglu, A Yager, KG Stafford, GR AF Page, Kirt A. Shin, Jae Wook Eastman, Scott A. Rowe, Brandon W. Kim, Sangcheol Kusoglu, Ahmet Yager, Kevin G. Stafford, Gery R. TI In Situ Method for Measuring the Mechanical Properties of Nafion Thin Films during Hydration Cycles SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE stress; thin films; Nafion; curvature; modulus; humidity ID FUEL-CELL MEMBRANES; POLYMER ELECTROLYTE MEMBRANE; PROTON-EXCHANGE MEMBRANES; (111)-TEXTURED AU; RECAST NAFION(R); WATER-UPTAKE; TEMPERATURE; TRANSPORT; CONFINEMENT; HUMIDITY AB Perfluorinated ionomers, in particular Nafion, are an essential component in hydrogen fuel cells, as both the proton exchange membrane and the binder within the catalyst layer. During normal operation of a hydrogen fuel cell, the ionomer will progressively swell and deswell in response to the changes in hydration, resulting in mechanical fatigue and ultimately failure over time. In this study, we have developed and implemented a cantilever bending technique in order to investigate the swelling-induced stresses in biaxially constrained Nafion thin films. When the deflection of a cantilever beam coated with a polymer film is monitored as it is exposed to varying humidity environments, the swelling induced stressthickness product of the polymer film is measured. By combining the stress-thickness results with a measurement of the swelling strain as a function of humidity, as measured by quartz crystal microbalance (QCM) and X-ray reflectivity (XR), the swelling stress can be determined. An estimate of the Young's modulus of thin Nafion films as a function of relative humidity is obtained. The Young's modulus values indicate orientation of the ionic domains within the polymer films, which were confirmed by grazing incidence small-angle X-ray scattering (GISAXS). This study represents a measurement platform that can be expanded to incorporate novel ionomer systems and fuel cell components to mimic the stress state of a working hydrogen fuel cell. C1 [Page, Kirt A.; Shin, Jae Wook; Rowe, Brandon W.; Kim, Sangcheol; Stafford, Gery R.] NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. [Eastman, Scott A.] United Technol Res Ctr, East Hartford, CT 06108 USA. [Kusoglu, Ahmet] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Stafford, GR (reprint author), NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. EM gery.stafford@nist.gov RI Yager, Kevin/F-9804-2011; OI Yager, Kevin/0000-0001-7745-2513; Kusoglu, Ahmet/0000-0002-2761-1050 FU NIST NRC Fellowship program; U.S. DOE Office of Science Facilities [DE-SC0012704] FX The authors gratefully acknowledge Carlos Beauchamp, Bradley Frieberg, Christopher Stafford, and Christopher L. Soles of NIST for technical contributions, programmatic support, and several lively scientific discussions. S.A.E. and B.W.R. acknowledge support from the NIST NRC Fellowship program. Certain commercial equipment, instruments, or materials are identified in this paper in order to specify the experimental procedure adequately. Such identification is not intended to imply recommendation or endorsement by the National Institute of Standards and Technology, nor is it intended to imply that the materials or equipment identified are necessarily the best available for the purpose. Research used resources of the Center for Functional Nanomaterials, and the National Synchrotron Light Source, which are U.S. DOE Office of Science Facilities, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 46 TC 7 Z9 7 U1 10 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 19 PY 2015 VL 7 IS 32 BP 17874 EP 17883 DI 10.1021/acsami.5b04080 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CP6VU UT WOS:000360027100042 PM 26258630 ER PT J AU Wang, T Li, RP Quan, ZW Loc, WS Bassett, WA Xu, HW Cao, YC Fang, JY Wang, ZW AF Wang, Tie Li, Ruipeng Quan, Zewei Loc, Welley Siu Bassett, William A. Xu, Hongwu Cao, Y. Charles Fang, Jiye Wang, Zhongwu TI Pressure Processing of Nanocube Assemblies Toward Harvesting of a Metastable PbS Phase SO ADVANCED MATERIALS LA English DT Article DE metastable phases; nanocrystal assemblies; porous architectures; pressure processing ID SHAPE-CONTROLLED SYNTHESIS; NANOPARTICLE SUPERLATTICES; STRUCTURAL STABILITY; SIZE DEPENDENCE; NANOCRYSTALS; TRANSFORMATION; SALT; SUPERCONDUCTIVITY; TRANSITION C1 [Wang, Tie] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Analyt Chem Living Biosyst, Beijing 100190, Peoples R China. [Wang, Tie; Cao, Y. Charles] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Li, Ruipeng; Wang, Zhongwu] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. [Quan, Zewei; Loc, Welley Siu; Fang, Jiye] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. [Bassett, William A.] Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY 14853 USA. [Xu, Hongwu] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP Quan, ZW (reprint author), Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. EM zw42@cornell.edu RI Wang, Tie/L-5060-2015; Li, Ruipeng/A-3691-2014; OI Wang, Tie/0000-0001-5965-6520; Li, Ruipeng/0000-0001-8176-3138; Xu, Hongwu/0000-0002-0793-6923 FU National Science Foundation; National Institutes of Health/National Institute of General Medical Sciences under NSF [DMR-1332208]; National Natural Science Foundation of China [21422507, 21321003] FX T.W. and R.L. contributed equally to this work. This work is based upon research conducted at the Cornell High Energy Synchrotron Source (CHESS) which is supported by the National Science Foundation and the National Institutes of Health/National Institute of General Medical Sciences under NSF Award DMR-1332208. T.W. appreciates the financial support by the National Natural Science Foundation of China (Grant Nos. 21422507 and 21321003). NR 37 TC 7 Z9 7 U1 15 U2 97 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 19 PY 2015 VL 27 IS 31 BP 4544 EP 4549 DI 10.1002/adma.201502070 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP5HI UT WOS:000359911500005 PM 26179895 ER PT J AU Hu, L Chen, J Fan, LL Ren, Y Huang, QZ Sanson, A Jiang, Z Zhou, M Rong, YC Wang, Y Deng, JX Xing, XR AF Hu, Lei Chen, Jun Fan, Longlong Ren, Yang Huang, Qingzhen Sanson, Andrea Jiang, Zheng Zhou, Mei Rong, Yangchun Wang, Yong Deng, Jinxia Xing, Xianran TI High-Curie-Temperature Ferromagnetism in (Sc,Fe)F-3 Fluorides and its Dependence on Chemical Valence SO ADVANCED MATERIALS LA English DT Article DE magnetic materials; fluorides; spintronics; multifunctional materials; structure-property relationships ID THERMAL-EXPANSION; ROOM-TEMPERATURE; THIN-FILMS; DOPED ZNO; OXIDES; SEMICONDUCTORS; NANOCRYSTALS; NANOWIRES; EXCHANGE; FE C1 [Hu, Lei; Chen, Jun; Fan, Longlong; Rong, Yangchun; Deng, Jinxia; Xing, Xianran] Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. [Chen, Jun] Univ Sci & Technol Beijing, Beijing Key Lab Special Melting & Preparat High E, Beijing 100083, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Huang, Qingzhen] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Sanson, Andrea] Univ Padua, Dept Phys & Astron, I-35131 Padua, Italy. [Jiang, Zheng; Wang, Yong] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201800, Peoples R China. [Zhou, Mei] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. RP Chen, J (reprint author), Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. EM junchen@ustb.edu.cn; xing@ustb.edu.cn RI Chen, Jun/M-1669-2015; OI Zhou, Mei/0000-0003-1738-2116 FU National Natural Science Foundation of China [21322102, 91422301, 21231001]; Program for Changjiang Scholars and Innovative Research Team in University [IRT1207]; Fundamental Research Funds for the Central Universities, China [FRF-TP-14-012C1]; Program of Introducing Talents of Discipline to Universities [B14003]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; [20140214] FX This work was supported by the National Natural Science Foundation of China (Grant Nos. 21322102, 91422301, 21231001), the Program for Changjiang Scholars and Innovative Research Team in University (IRT1207), the Fundamental Research Funds for the Central Universities, China (FRF-TP-14-012C1), and the Program of Introducing Talents of Discipline to Universities (B14003). The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DE-AC02-06CH11357). We thank the staff at beamlines BL14W and BL08U of the Shanghai Synchrotron Radiation Facility (SSRF) for providing beam time to collect the Fe L- and K-edge EXAFS spectra and for assisting with the XAFS measurements. We are also grateful to the ELETTRA synchrotron radiation facility and the staff of the XAFS beamline for the Sc K-edge EXAFS spectrum of pure ScF3, which was collected during the project N. 20140214. NR 28 TC 7 Z9 7 U1 17 U2 65 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 19 PY 2015 VL 27 IS 31 BP 4592 EP 4596 DI 10.1002/adma.201500868 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP5HI UT WOS:000359911500013 PM 26149472 ER PT J AU Ugur, A Katmis, F Li, MD Wu, LJ Zhu, YM Varanasi, KK Gleason, KK AF Ugur, Asli Katmis, Ferhat Li, Mingda Wu, Lijun Zhu, Yimei Varanasi, Kripa K. Gleason, Karen K. TI Low-Dimensional Conduction Mechanisms in Highly Conductive and Transparent Conjugated Polymers SO ADVANCED MATERIALS LA English DT Article DE chemical vapor deposition; conducting polymers; poly(3, 4-ethylenedioxythiophene) (PEDOT) ID CHEMICAL-VAPOR-DEPOSITION; LIGHT-EMITTING-DIODES; FIELD-EFFECT MOBILITY; THERMOELECTRIC PERFORMANCE; ELECTRICAL-CONDUCTIVITY; FILMS; POLY(3,4-ETHYLENEDIOXYTHIOPHENE); SEMICONDUCTORS; POLYACETYLENE; POLYTHIOPHENE C1 [Ugur, Asli; Gleason, Karen K.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. [Varanasi, Kripa K.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Katmis, Ferhat] MIT, Dept Phys, Cambridge, MA 02139 USA. [Li, Mingda] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Varanasi, KK (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM varanasi@mit.edu; kkg@mit.edu RI Gleason, Karen/G-1471-2013 OI Gleason, Karen/0000-0001-6127-1056 FU MIT Institute for Soldier Nanotechnologies (ISN) [DAAD-19-02D-0002]; U.S. Army Research Office; U.S. Department of Energy, Office of Basic Energy Science, Material Science and Engineering Division [DE-AC02-98CH10886] FX The authors acknowledge financial support from the MIT Institute for Soldier Nanotechnologies (ISN) under Contract DAAD-19-02D-0002 with the U.S. Army Research Office. Part of this work was carried out at the CMSE shared experimental facilities, and the authors would like to thank S. Speakman for assistance and J. Moodera for fruitful discussions. The Work at BNL was supported by the U.S. Department of Energy, Office of Basic Energy Science, Material Science and Engineering Division, under Contract No. DE-AC02-98CH10886. NR 43 TC 15 Z9 15 U1 20 U2 148 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 19 PY 2015 VL 27 IS 31 BP 4604 EP 4610 DI 10.1002/adma.201502340 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP5HI UT WOS:000359911500015 PM 26224113 ER PT J AU Keyshar, K Gong, YJ Ye, GL Brunetto, G Zhou, W Cole, DP Hackenberg, K He, YM Machado, L Kabbani, M Hart, AHC Li, B Galvao, DS George, A Vajtai, R Tiwary, CS Ajayan, PM AF Keyshar, Kunttal Gong, Yongji Ye, Gonglan Brunetto, Gustavo Zhou, Wu Cole, Daniel P. Hackenberg, Ken He, Yongmin Machado, Leonardo Kabbani, Mohamad Hart, Amelia H. C. Li, Bo Galvao, Douglas S. George, Antony Vajtai, Robert Tiwary, Chandra Sekhar Ajayan, Pulickel M. TI Chemical Vapor Deposition of Monolayer Rhenium Disulfide (ReS2) SO ADVANCED MATERIALS LA English DT Article DE 2D materials; chemical vapor deposition; renium disulfide; transition metal dichalcogenides ID HYDROGEN EVOLUTION REACTION; HEXAGONAL BORON-NITRIDE; HIGH-QUALITY MONOLAYER; MOS2 ATOMIC LAYERS; HIGH-PERFORMANCE; GRAIN-BOUNDARY; NANOSHEETS; TRANSISTORS; GROWTH; DICHALCOGENIDES C1 [Keyshar, Kunttal; Ye, Gonglan; Hackenberg, Ken; He, Yongmin; Kabbani, Mohamad; Hart, Amelia H. C.; Li, Bo; George, Antony; Vajtai, Robert; Tiwary, Chandra Sekhar; Ajayan, Pulickel M.] Rice Univ, Dept Mat Sci & Nanoengn, Houston, TX 77005 USA. [Gong, Yongji] Rice Univ, Dept Chem, Houston, TX 77005 USA. [Brunetto, Gustavo; Machado, Leonardo; Galvao, Douglas S.] State Univ Campinas UNICAMP, IFGW DFA, Dept Appl Phys, BR-13083859 Campinas, SP, Brazil. [Zhou, Wu] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Cole, Daniel P.] US Army Res Lab, Vehicle Technol Directorate, Aberdeen Proving Ground, MD 21005 USA. RP Tiwary, CS (reprint author), Rice Univ, Dept Mat Sci & Nanoengn, Houston, TX 77005 USA. EM cst311@gmail.com; ajayan@rice.edu RI Zhou, Wu/D-8526-2011; UNICAMP, CCES - /J-7787-2015; Gong, Yongji/L-7628-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Machado, Leonardo/E-2081-2017 OI Zhou, Wu/0000-0002-6803-1095; FU Army Research Laboratory [W911NF-1O-l-0052]; AFOSR (Air Force Office of Scientific Research) [FA9550-14-1-0268]; CNPq; CAPES; FAPESP; Center for Computational Engineering and Sciences at Unicamp through the FAPESP/CEPID [2013/08293-7] FX Research was sponsored by the Army Research Laboratory and was accomplished under Cooperative Agreement No. W911NF-1O-l-0052. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of the Army Research Laboratory or the U.S. Government. The U.S. Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. The Research was also sponsored by AFOSR (Air Force Office of Scientific Research) under Award No. FA9550-14-1-0268. The authors would also like to acknowlege Sidong Lei from Rice University for aid in device measurements. Gustavo Brunetto, Leonardo Machado and Douglas S. Galvao acknowledge financial support from the Brazilian Agencies CNPq, CAPES and FAPESP and also thank the Center for Computational Engineering and Sciences at Unicamp for financial support through the FAPESP/CEPID Grant 2013/08293-7. NR 45 TC 26 Z9 26 U1 36 U2 178 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 19 PY 2015 VL 27 IS 31 BP 4640 EP 4648 DI 10.1002/adma.201501795 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP5HI UT WOS:000359911500021 PM 26140355 ER PT J AU Yang, XF Kattel, S Senanayake, SD Boscoboinik, JA Nie, XW Graciani, J Rodriguez, JA Liu, P Stacchiola, DJ Chen, JGG AF Yang, Xiaofang Kattel, Shyam Senanayake, Sanjaya D. Boscoboinik, J. Anibal Nie, Xiaowa Graciani, Jesus Rodriguez, Jose A. Liu, Ping Stacchiola, Dario J. Chen, Jingguang G. TI Low Pressure CO2 Hydrogenation to Methanol over Gold Nanoparticles Activated on a CeOx/TiO2 Interface SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LOW-TEMPERATURE OXIDATION; MIXED-METAL OXIDE; CARBON-DIOXIDE; NANOMETER LEVEL; SYNTHESIS GAS; CATALYSTS; CERIA; SPECTROSCOPY; SURFACES; SUPPORT AB Capture and recycling of CO2 into valuable chemicals such as alcohols could help mitigate its emissions into the atmosphere. Due to its inert nature, the activation of CO2 is a critical step in improving the overall reaction kinetics during its chemical conversion. Although pure gold is an inert noble metal and cannot catalyze hydrogenation reactions, it can be activated when deposited as nanoparticles on the appropriate oxide support. In this combined experimental and theoretical study, it is shown that an electronic polarization at the metal-oxide interface of Au nanoparticles anchored and stabilized on a CeOx/TiO2 substrate generates active centers for CO2 adsorption and its low pressure hydrogenation, leading to a higher selectivity toward methanol. This study illustrates the importance of localized electronic properties and structure in catalysis for achieving higher alcohol selectivity from CO2 hydrogenation. C1 [Yang, Xiaofang; Kattel, Shyam; Senanayake, Sanjaya D.; Rodriguez, Jose A.; Liu, Ping; Stacchiola, Dario J.; Chen, Jingguang G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Boscoboinik, J. Anibal] Brookhaven Natl Lab, CFN, Upton, NY 11973 USA. [Nie, Xiaowa] Dalian Univ Technol, Dalian 116024, Liaoning, Peoples R China. [Graciani, Jesus] Univ Seville, Dept Phys Chem, E-41012 Seville, Spain. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. RP Stacchiola, DJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov; jgchen@columbia.edu RI Stacchiola, Dario/B-1918-2009; Senanayake, Sanjaya/D-4769-2009 OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232 FU U.S. Department of Energy, Office of Science [DE-AC02-98CH10886]; U.S. DOE Office of Science User Facilities at Brookhaven National Laboratory [DE-SC0012704]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The work was sponsored under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy, Office of Science. This research used resources of the Center for Functional Nanomaterials and National Synchrotron Light Source, which are U.S. DOE Office of Science User Facilities at Brookhaven National Laboratory under Contract No. DE-SC0012704 and the National Energy Research Scientific Computing Center (NERSC) supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 24 TC 21 Z9 21 U1 41 U2 265 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10104 EP 10107 DI 10.1021/jacs.5b06150 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000020 PM 26218072 ER PT J AU Dalton, DM Ellis, SR Nichols, EM Mathies, RA Toste, FD Bergman, RG Raymond, KN AF Dalton, Derek M. Ellis, Scott R. Nichols, Eva M. Mathies, Richard A. Toste, F. Dean Bergman, Robert G. Raymond, Kenneth N. TI Supramolecular Ga4L612- Cage Photosensitizes 1,3-Rearrangement of Encapsulated Guest via Photoinduced Electron Transfer SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AZA-COPE REARRANGEMENT; ENERGY-TRANSFER; HOST; CYCLODEXTRIN; DERIVATIVES; EXCITATION; PORPHYRIN; CATALYSIS; DYNAMICS; ACCEPTOR AB The K12Ga4L6 supramolecular cage is photoactive and enables an unprecedented photoreaction not observed in bulk solution. Ga4L612- cages photosensitize the 1,3-rearrangement of encapsulated cinnamylammonium cation guests from the linear isomer to the higher energy branched isomer when irradiated with UVA light. The rearrangement requires light and guest encapsulation to occur. The Ga4L612- cage-mediated reaction mechanism was investigated by UV/vis absorption, fluorescence, ultrafast transient absorption, and electrochemical experiments. The results support a photoinduced electron transfer mechanism for the 1,3-rearrangement, in which the Ga4L612- cage absorbs photons and transfers an electron to the encapsulated cinnamylammonium ion, which undergoes C-N bond cleavage, followed by back electron transfer to the cage and recombination of the guest fragments to form the higher energy isomer. C1 [Toste, F. Dean; Bergman, Robert G.; Raymond, Kenneth N.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Toste, FD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu; rbergman@berkeley.edu; raymond@socrates.berkeley.edu FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; National Science Foundation Graduate Research Fellowship Program (NSF GRFP) FX This research was supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL (DE-AC02-05CH11231). E.M.N. gratefully acknowledges support from the National Science Foundation Graduate Research Fellowship Program (NSF GRFP). We thank Dr. Heinz Frei, Dr. Daniel Dietze, and Rebecca Schafer for helpful discussions. NR 35 TC 6 Z9 6 U1 9 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10128 EP 10131 DI 10.1021/jacs.5b06317 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000026 PM 26256754 ER PT J AU Zhu, HY Wu, ZL Su, D Veith, GM Lu, HF Zhang, PF Chai, SH Dai, S AF Zhu, Huiyuan Wu, Zili Su, Dong Veith, Gabriel M. Lu, Hanfeng Zhang, Pengfei Chai, Song-Hai Dai, Sheng TI Constructing Hierarchical Interfaces: TiO2-Supported PtFe-FeOx Nanowires for Room Temperature CO Oxidation SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OXYGEN REDUCTION REACTION; CATALYTIC-OXIDATION; FERROUS CENTERS; NANOPARTICLES; MECHANISM; FEPT; ELECTROCATALYSIS; ELECTROOXIDATION; STABILITY; ULTRATHIN AB In this communication, we report a facile approach to constructing catalytic active hierarchical interfaces in one-dimensional (1D) nanostructure, exemplified by the synthesis of TiO2-supported PtFe-FeOx nanowires (NWs). The hierarchical interface, constituting atomic level interactions between PtFe and FeOx within each NW and the interactions between NWs and support (TiO2), enables CO oxidation with 100% conversion at room temperature. We Identify the role of the two interfaces by probing the CO oxidation reaction with isotopic labeling experiments. Both the oxygen atoms (Os) in FeOx and TiO2 participate in the initial CO oxidation, facilitating the reaction through a redox pathway. Moreover, the intact 1D structure leads to the high stability of the catalyst. After 30 h in the reaction stream, the PtFe-FeOx/TiO2 catalyst exhibits no activity decay. Our results provide a general approach and new insights into the construction of hierarchical interfaces for advanced catalysis. C1 [Zhu, Huiyuan; Wu, Zili; Zhang, Pengfei; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Wu, Zili] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Veith, Gabriel M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Chai, Song-Hai; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Lu, Hanfeng] Zhejiang Univ Technol, Coll Chem Engn, Inst Catalyt React Engn, Hangzhou 310014, Zhejiang, Peoples R China. RP Zhu, HY (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM zhuh@ornl.gov; dais@ornl.gov RI Dai, Sheng/K-8411-2015; Zhang, Pengfei/I-5484-2013; Wu, Zili/F-5905-2012; Chai, Song-Hai/A-9299-2012; Su, Dong/A-8233-2013 OI Dai, Sheng/0000-0002-8046-3931; Wu, Zili/0000-0002-4468-3240; Chai, Song-Hai/0000-0002-4152-2513; Su, Dong/0000-0002-1921-6683 FU Laboratory Directed Research and Development Program at the Oak Ridge National Laboratory; U.S. Department of Energy, Office of Science, Chemical Sciences, Geosciences and Biosciences Division; U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704]; US Department of Energy's Office of Basic Energy Sciences, Division of Materials Science and Engineering FX H.Z. was supported by Liane B. Russell Fellowship sponsored by the Laboratory Directed Research and Development Program at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the US Department of Energy. Z.W. and S.D. were supported by the U.S. Department of Energy, Office of Science, Chemical Sciences, Geosciences and Biosciences Division. Part of the work, including the DRIFTS study, was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Electron Microscopy work used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. Part of the work (XPS-GMV), was supported by the US Department of Energy's Office of Basic Energy Sciences, Division of Materials Science and Engineering. NR 29 TC 15 Z9 15 U1 26 U2 111 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10156 EP 10159 DI 10.1021/jacs.5b07011 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000033 PM 26244820 ER PT J AU Musselwhite, N Na, K Sabyrov, K Aayogu, S Somorjai, GA AF Musselwhite, Nathan Na, Kyungsu Sabyrov, Kairat Aayogu, Selim Somorjai, Gabor A. TI Mesoporous Aluminosilicate Catalysts for the Selective Isomerization of n-Hexane: The Roles of Surface Acidity and Platinum Metal SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SINGLE-CRYSTAL SURFACES; TEMPERATURE-DEPENDENCE; STRUCTURE SENSITIVITY; BETA ZEOLITES; CRACKING; NANOPARTICLES; MECHANISMS; SIZE; AROMATIZATION; SPECTROSCOPY AB Several types of mesoporous aluminosilicates were synthesized and evaluated in the catalytic isomerization of n-hexane, both with and without Pt nanopartides loaded into the mesopores. The materials investigated included mesoporous MFI and BEA type zeolites, MCF-17 mesoporous silica, and an aluminum modified MCF-17. The acidity of the materials was investigated through pyridine adsorption and Fourier Transform-Infrared Spectroscopy (FT-IR). It was found that the strong Bronsted acid sites in the micropores of the zeolite catalysts facilitated the cracking of hexane. However, the medium strength acid sites on the Al modified MCF-17 mesoporous silica greatly enhanced the isomerization reaction. Through the loading of different amounts of Pt into the mesopores of the Al modified MCF-17, the relationship between the metal nanopartides and acidic sites on the support was revealed. C1 [Musselwhite, Nathan; Na, Kyungsu; Sabyrov, Kairat; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Musselwhite, Nathan; Na, Kyungsu; Sabyrov, Kairat; Aayogu, Selim; Somorjai, Gabor A.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Na, Kyungsu] Chonnam Natl Univ, Dept Chem, Gwangju 500757, South Korea. RP Aayogu, S (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu; salayoglu@lbl.gov FU Chevron Energy Technology Company; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the U.S. DOE [DE-AC02-05CH11231]; Korea government (Ministry of Science, ICT & Future Planning) [NRF-2014M1A8A1049254]; Office of Science, Office of Basic Energy Sciences, Division of Material Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work is funded by The Chevron Energy Technology Company. We acknowledge support from the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the U.S. DOE under Contract DE-AC02-05CH11231. K.N. thanks the Korea CCS R&D Center (KCRC) grant funded by the Korea government (Ministry of Science, ICT & Future Planning, NRF-2014M1A8A1049254). Work at the Molecular Foundry was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Material Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 40 TC 5 Z9 5 U1 16 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10231 EP 10237 DI 10.1021/jacs.5b04808 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000043 PM 26168190 ER PT J AU Altman, AB Pemmaraju, CD Camp, C Arnold, J Minasian, SG Prendergast, D Shuh, DK Tyliszczak, T AF Altman, Alison B. Pemmaraju, C. D. Camp, Clement Arnold, John Minasian, Stefan G. Prendergast, David Shuh, David K. Tyliszczak, Tolek TI Theory and X-ray Absorption Spectroscopy for Aluminum Coordination Complexes - Al K-Edge Studies of Charge and Bonding in (BDI)Al, (BDI)AlR2, and (BDI)AlX2 Complexes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AB-INITIO CALCULATIONS; ADVANCED LIGHT-SOURCE; NON-INNOCENT LIGANDS; LOW-VALENT ALUMINUM; MAIN-GROUP; ELECTRONIC-STRUCTURE; HYDROGEN STORAGE; GROUP-13 METALS; LEWIS-ACID; CHEMISTRY AB Polarized aluminum K-edge X-ray absorption near edge structure (XANES) spectroscopy and first-principles calculations were used to probe electronic structure in a series of (BDI)Al, (BDI)AlX2, and (BDI)AlR2 coordination compounds (X = F, Cl, I; R = H, Me; BDI = 2,6-diisopropylphenyl-beta-diketiminate). Spectral interpretations were guided by examination of the calculated transition energies and polarization-dependent oscillator strengths, which agreed well with the XANES spectroscopy measurements. Pre-edge features were assigned to transitions associated with the Al 3p orbitals involved in metalligand bonding. Qualitative trends in Al 1s core energy and valence orbital occupation were established through a systematic comparison of excited states derived from Al 3p orbitals with similar symmetries in a molecular orbital framework. These trends suggested that the higher transition energies observed for (BDI)AlX2 systems with more electronegative X-1 ligands could be ascribed to a decrease in electron density around the aluminum atom, which causes an increase in the attractive potential of the Al nucleus and concomitant increase in the binding energy of the Al 1s core orbitals. For (BDI)Al and (BDI)AlH2 the experimental Al K-edge XANES spectra and spectra calculated using the eXcited electron and CoreHole (XCH) approach had nearly identical energies for transitions to final state orbitals of similar composition and symmetry. These results implied that the charge distributions about the aluminum atoms in (BDI)Al and (BDI)AlH2 are similar relative to the (BDI)AlX2 and (BDI)AlMe2 compounds, despite having different formal oxidation states of +1 and +3, respectively. However, (BDI)Al was unique in that it exhibited a low-energy feature that was attributed to transitions into a low-lying p-orbital of b(1) symmetry that is localized on Al and orthogonal to the (BDI)Al plane. The presence of this low-energy unoccupied molecular orbital on electron-rich (BDI)Al distinguishes its valence electronic structure from that of the formally trivalent compounds (BDI)AlX2 and (BDI)AlR2. The work shows that Al K-edge XANES spectroscopy can be used to provide valuable insight into electronic structure and reactivity relationships for main-group coordination compounds. C1 [Altman, Alison B.; Camp, Clement; Arnold, John] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Altman, Alison B.; Pemmaraju, C. D.; Arnold, John; Minasian, Stefan G.; Shuh, David K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Arnold, J (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM arnold@berkeley.edu; sgminasian@lbl.gov; dgprendergast@lbl.gov; dkshuh@lbl.gov RI Foundry, Molecular/G-9968-2014; Arnold, John/F-3963-2012; CAMP, Clement/I-5072-2015 OI Arnold, John/0000-0001-9671-227X; CAMP, Clement/0000-0001-8528-0731 FU Department of Energy (DOE) Integrated University Program Fellowship at the University of California, Berkeley; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program of the U.S. DOE at LBNL [DE-AC02-05CH11231]; User Project at the Molecular Foundry, LBNL; Office of Science, Office of Basic Energy Sciences, of the U.S. DOE at LBNL [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Condensed Phase and Interfacial Molecular Sciences Program of the U.S. DOE at LBNL [DE-AC02-05CH11231] FX A.B.A. acknowledges support by a Department of Energy (DOE) Integrated University Program Fellowship at the University of California, Berkeley. J.A., S.G.M. and D.K.S. were supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program of the U.S. DOE at LBNL under contract no. DE-AC02-05CH11231. The theory work of C.D.P. and D.P. was supported through a User Project at the Molecular Foundry, LBNL. Calculations were performed on the Cray XE6 Hopper computer at the National Energy Research Scientific Computing Center (NERSC-LBNL) and Molecular Foundry computing resources, Nano and Vulcan, managed by the High Performance Computing Services Group of LBNL. The ALS and T.T. were supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. DOE under contract no. DE-AC02-05CH11231 at LBNL. Research at Beam line 11.0.2 at the ALS was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Condensed Phase and Interfacial Molecular Sciences Program of the U.S. DOE at LBNL under contract no. DE-AC02-05CH11231. NR 128 TC 4 Z9 4 U1 8 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10304 EP 10316 DI 10.1021/jacs.5b05854 PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000052 PM 26258886 ER PT J AU Carrasquillo-Flores, R Ro, I Kumbhalkar, MD Burt, S Carrero, CA Alba-Rubio, AC Miller, JT Hermans, I Huber, GW Dumesic, JA AF Carrasquillo-Flores, Ronald Ro, Insoo Kumbhalkar, Mrunmayi D. Burt, Samuel Carrero, Carlos A. Alba-Rubio, Ana C. Miller, Jeffrey T. Hermans, Ive Huber, George W. Dumesic, James A. TI Reverse Water-Gas Shift on Interfacial Sites Formed by Deposition of Oxidized Molybdenum Moieties onto Gold Nanoparticles SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CO OXIDATION; CARBON-MONOXIDE; ACTIVE-SITES; IN-SITU; HYDROGEN DISSOCIATION; AU NANOPARTICLES; LOW-TEMPERATURE; METAL-OXIDE; QUANTITATIVE-DETERMINATION; AU/CEO2 CATALYST AB We show that MoOx-promoted Au/SiO2 catalysts are active for reverse water gas shift (RWGS) at 573 K. Results from reactivity measurements, CO FTIR studies, Raman spectroscopy, and X-ray absorption spectroscopy (XAS) indicate that the deposition of Mo onto Au nanoparticles occurs preferentially on under-coordinated Au sites, forming Au/MoOx interfacial sites active for reverse water gas shift (RWGS). Au and AuMo sites are quantified from FTIR spectra of adsorbed CO collected at subambient temperatures (e.g., 150-270 K). Bands at 2111 and 2122 cm(-1) are attributed to CO adsorbed on under-coordinated Au and Au-0 and Au delta+ species, respectively. Clausius-Clapeyron analysis of FTIR data yields a heat of CO adsorption (Delta H-ads) of -31 kJ mol(-1) for Au-0 and -64 kJ mol(-1) for Au delta+ at 33% surface coverage. Correlations of RWGS reactivity with changes in FTIR spectra for samples containing different amounts of Mo indicate that interfacial sites are an order of magnitude more active than Au sites for RWGS. Raman spectra of Mo/SiO2 show a feature at 975 cm(-1), attributed to a dioxo (O=)(2)Mo(-O-Si)(2) species not observed in spectra of AuMo/SiO2 catalysts, indicating preferential deposition of Mo on Au. XAS results indicate that Mo is in a +6 oxidation state, and therefore Au and Mo exist as a metal metal oxide combination. Catalyst calcination increases the quantity of under-coordinated Au sites, increasing RWGS activity. This strategy for catalyst synthesis and characterization enables quantification of Au active sites and interfacial sites, and this approach may be extended to describe reactivity changes observed in other reactions on supported gold catalysts. C1 [Carrasquillo-Flores, Ronald; Ro, Insoo; Kumbhalkar, Mrunmayi D.; Burt, Samuel; Alba-Rubio, Ana C.; Hermans, Ive; Huber, George W.; Dumesic, James A.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Burt, Samuel; Carrero, Carlos A.; Hermans, Ive] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn, Argonne, IL 60439 USA. RP Dumesic, JA (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA. EM dumesic@engr.wisc.edu RI BM, MRCAT/G-7576-2011 FU U.S. Department of Energy, Office of Basic Energy Sciences; U.S. DOE [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Basic Energy Sciences. We are thankful for the use of the Advanced Photon Source, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, supported by the U.S. DOE under contract DE-AC02-06CH11357. We wish to thank Canan Sener for valuable discussions and help in catalyst synthesis NR 66 TC 11 Z9 12 U1 20 U2 105 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10317 EP 10325 DI 10.1021/jacs.5b05945 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000053 PM 26225538 ER PT J AU Vjunov, A Derewinski, MA Fulton, JL Camaioni, DM Lercher, JA AF Vjunov, Aleksei Derewinski, Miroslaw A. Fulton, John L. Camaioni, Donald M. Lercher, Johannes A. TI Impact of Zeolite Aging in Hot Liquid Water on Activity for Acid-Catalyzed Dehydration of Alcohols SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HIGH-RESOLUTION SI-29; SOLID-STATE; NMR-SPECTROSCOPY; AL DISTRIBUTION; BETA-ZEOLITE; Y-ZEOLITES; MAS NMR; FRAMEWORK; ALUMINUM; SPECTRA AB The location and stability of Bronsted acid sites catalytically active in zeolites during aqueous phase dehydration of alcohols were studied on the example of cydohexanol. The catalytically active hydronium ions originate from Bronsted acid sites (BAS) of the zeolite that are formed by framework tetrahedral Si atom substitution by Al. Al K-edge extended X-ray absorption fine structure (EXAFS) and Al-27 magic angle spinning (MAS) nuclear magnetic resonance (NMR) spectroscopies in combination with density functional theory (DFT) calculations are used to determine the distribution of tetrahedral Al sites (Al T-sites) both qualitatively and quantitatively for both parent and HBEA catalysts aged in water prior to catalytic testing. The aging procedure leads to partial degradation of the zeolite framework evidenced from the decrease of material crystallinity (XRD) as well as sorption capacity (BET). With the exception of one commercial zeolite sample, which had the highest concentration of framework silanol-defects, there is no evidence of Al coordination modification after aging in water. The catalyst weight-normalized dehydration rate correlated best with the sum of strong and weak Bronsted acidic protons both able to generate the hydrated hydronium ions. All hydronium ions were equally active for the acid-catalyzed reactions in water. Zeolite aging in hot water prior to catalysis decreased the weight normalized dehydration reaction rate compared to that of the parent HBEA, which is attributed to the reduced concentration of accessible Bronsted acid sites. Sites are hypothesized to be blocked due to reprecipitation of silica dissolved during framework hydrolysis in the aging procedure. C1 [Vjunov, Aleksei; Derewinski, Miroslaw A.; Fulton, John L.; Camaioni, Donald M.; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85748 Garching, Germany. [Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Inst, D-85748 Garching, Germany. RP Lercher, JA (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM Johannes.Lercher@pnnl.gov FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Materials Synthesis and Simulation Across Scales (MS3 Initiative); DOE Office of Science, Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL); Physical Science Laboratory located at Pacific Northwest National Laboratory (PNNL) FX Authors thank B. W. Arey (PNNL) for HIM measurements, T. Huthwelker for support during Al XAFS measurements at the Swiss Light Source (PSI, Switzerland), J. Z. Hu and S. D. Burton (PNNL) for support during NMR experiments. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. M.D. acknowledges support by the Materials Synthesis and Simulation Across Scales (MS3 Initiative) conducted under Laboratory Directed Research & Development Program at PNNL. NMR experiments were performed at the Environmental Molecular Science Laboratory, a national scientific user facility sponsored by the DOE Office of Science, Office of Biological and Environmental Research, and Physical Science Laboratory both located at Pacific Northwest National Laboratory (PNNL). NR 42 TC 8 Z9 8 U1 20 U2 125 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 19 PY 2015 VL 137 IS 32 BP 10374 EP 10382 DI 10.1021/jacs.5b06169 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CP5YR UT WOS:000359962000060 PM 26237038 ER PT J AU Kenanakis, G Soukoulis, CM Economou, EN AF Kenanakis, George Soukoulis, Costas M. Economou, Eleftherios N. TI Casimir forces of metallic microstructures into cavities SO PHYSICAL REVIEW B LA English DT Article ID MICROELECTROMECHANICAL SYSTEMS; VACUUM; RANGE AB A theoretical estimate of the Casimir force of a metallic structure embedded into a cubic cavity is proposed. We demonstrate that by calculating the eigenmodes of the system we can determine the Casimir force, which can be either attractive or repulsive, by simply changing the geometry of the structures relative to the walls of the cavity. In this analysis, several cases of structures are taken into account, from rectangular slabs to chiral "omega" particles, and the predicted data are consistent with recent literature. We demonstrate that the sidewalls of the studied cavity contribute decisively to the repulsive Casimir force between the system and the nearby top surface of the cavity. Finally, we provide evidence that the medium embedded into the studied cavity (and especially its permittivity) can change the intensity of the Casimir force, while its repulsive nature, once established (owing to favorable geometrical features), remains quite robust. C1 [Kenanakis, George; Soukoulis, Costas M.; Economou, Eleftherios N.] Fdn Res & Technol Hellas, Inst Elect Struct & Laser, Iraklion 70013, Crete, Greece. [Soukoulis, Costas M.] US DOE, Ames Lab, Ames, IA 50011 USA. [Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Kenanakis, G (reprint author), Fdn Res & Technol Hellas, Inst Elect Struct & Laser, N Plastira 100, Iraklion 70013, Crete, Greece. EM gkenanak@iesl.forth.gr RI Economou, Eleftherios /E-6374-2010; Soukoulis, Costas/A-5295-2008 FU Greek GSRT project [ERC02-EXEL]; European Research Council under ERC Advanced Grant [32081]; Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) [DE-AC02-07CH11358] FX This work was supported by Greek GSRT project ERC02-EXEL, and by the European Research Council under ERC Advanced Grant No. 32081 (PHOTOMETA). Work at Ames Laboratory was partially supported by the Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) under Contract No. DE-AC02-07CH11358 (computational studies). NR 27 TC 1 Z9 1 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 19 PY 2015 VL 92 IS 7 AR 075430 DI 10.1103/PhysRevB.92.075430 PG 6 WC Physics, Condensed Matter SC Physics GA CP4NS UT WOS:000359859600007 ER PT J AU Adolph, C Akhunzyanov, R Alexeev, MG Alexeev, GD Amoroso, A Andrieux, V Anosov, V Austregesilo, A Azevedo, C Badelek, B Balestra, F Barth, J Beck, R Bedfer, Y Bernhard, J Bicker, K Bielert, ER Birsa, R Bisplinghoff, J Bodlak, M Boer, M Bordalo, P Bradamante, F Braun, C Bressan, A Buchele, M Burtin, E Chang, WC Chiosso, M Choi, I Chung, SU Cicuttin, A Crespo, ML Curiel, Q Dalla Torre, S Dasgupta, SS Dasgupta, S Denisov, OY Dhara, L Donskov, SV Doshita, N Dunnweber, W Duic, V Dziewiecki, M Efremov, A Eversheim, PD Eyrich, W Faessler, M Ferrero, A Finger, M Finger, M Fischer, H Franco, C von Hohenesche, ND Friedrich, JM Frolov, V Gautheron, F Gavrichtchouk, OP Gerassimov, S Gnesi, I Gorzellik, M Grabmuller, S Grasso, A Grosse-Perdekamp, M Grube, B Grussenmeyer, T Guskov, A Haas, F Hahne, D von Harrach, D Hashimoto, R Heinsius, FH Herrmann, F Hinterberger, F Horikawa, N d'Hose, N Hsieh, CY Huber, S Ishimoto, S Ivanov, A Ivanshin, Y Iwata, T Jahn, R Jary, V Jorg, P Joosten, R Kabuss, E Ketzer, B Khaustov, GV Khokhlov, YA Kisselev, Y Klein, F Klimaszewski, K Koivuniemi, JH Kolosov, VN Kondo, K Konigsmann, K Konorov, I Konstantinov, VF Kotzinian, AM Kouznetsov, O Kramer, M Kremser, P Krinner, F Kroumchtein, ZV Kuchinski, N Kunne, F Kurek, K Kurjata, RP Lednev, AA Lehmann, A Levillain, M Levorato, S Lichtenstadt, J Maggiora, A Magnon, A Makins, N Makke, N Mallot, GK Marchand, C Martin, A Marzec, J Matousek, J Matsuda, H Matsuda, T Meshcheryakov, G Meyer, W Michigami, T Mikhailov, YV Miyachi, Y Nagaytsev, A Nagel, T Nerling, F Neyret, D Nikolaenko, VI Novy, J Nowak, WD Nunes, AS Olshevsky, AG Orlov, I Ostrick, M Panzieri, D Parsamyan, B Paul, S Peng, JC Pereira, F Pesek, M Peshekhonov, DV Platchkov, S Pochodzalla, J Polyakov, VA Pretz, J Quaresma, M Quintans, C Ramos, S Regali, C Reicherz, G Riedl, C Rocco, E Rossiyskaya, NS Ryabchikov, DI Rychter, A Samoylenko, VD Sandacz, A Santos, C Sarkar, S Savin, IA Sbrizzai, G Schiavon, P Schmeing, S Schmidt, K Schmieden, H Schonning, K Schopferer, S Schluter, T Selyunin, A Shevchenko, OY Silva, L Sinha, L Sirtl, S Slunecka, M Sozzi, F Srnka, A Stolarski, M Sulc, M Suzuki, H Szabelski, A Szameitat, T Sznajder, P Takekawa, S ter Wolbeek, J Tessaro, S Tessarotto, F Thibaud, F Tskhay, V Uhl, S Veloso, J Virius, M Wallner, S Weisrock, T Wilfert, M Zaremba, K Zavertyaev, M Zemlyanichkina, E Ziembicki, M Zink, A AF Adolph, C. Akhunzyanov, R. Alexeev, M. G. Alexeev, G. D. Amoroso, A. Andrieux, V. Anosov, V. Austregesilo, A. Azevedo, C. Badelek, B. Balestra, F. Barth, J. Beck, R. Bedfer, Y. Bernhard, J. Bicker, K. Bielert, E. R. Birsa, R. Bisplinghoff, J. Bodlak, M. Boer, M. Bordalo, P. Bradamante, F. Braun, C. Bressan, A. Buechele, M. Burtin, E. Chang, W. -C. Chiosso, M. Choi, I. Chung, S. U. Cicuttin, A. Crespo, M. L. Curiel, Q. Dalla Torre, S. Dasgupta, S. S. Dasgupta, S. Denisov, O. Yu. Dhara, L. Donskov, S. V. Doshita, N. Duennweber, W. Duic, V. Dziewiecki, M. Efremov, A. Eversheim, P. D. Eyrich, W. Faessler, M. Ferrero, A. Finger, M. Finger, M., Jr. Fischer, H. Franco, C. von Hohenesche, N. du Fresne Friedrich, J. M. Frolov, V. Gautheron, F. Gavrichtchouk, O. P. Gerassimov, S. Gnesi, I. Gorzellik, M. Grabmueller, S. Grasso, A. Grosse-Perdekamp, M. Grube, B. Grussenmeyer, T. Guskov, A. Haas, F. Hahne, D. von Harrach, D. Hashimoto, R. Heinsius, F. H. Herrmann, F. Hinterberger, F. Horikawa, N. d'Hose, N. Hsieh, C. -Yu Huber, S. Ishimoto, S. Ivanov, A. Ivanshin, Yu. Iwata, T. Jahn, R. Jary, V. Joerg, P. Joosten, R. Kabuss, E. Ketzer, B. Khaustov, G. V. Khokhlov, Yu. A. Kisselev, Yu. Klein, F. Klimaszewski, K. Koivuniemi, J. H. Kolosov, V. N. Kondo, K. Koenigsmann, K. Konorov, I. Konstantinov, V. F. Kotzinian, A. M. Kouznetsov, O. Kraemer, M. Kremser, P. Krinner, F. Kroumchtein, Z. V. Kuchinski, N. Kunne, F. Kurek, K. Kurjata, R. P. Lednev, A. A. Lehmann, A. Levillain, M. Levorato, S. Lichtenstadt, J. Maggiora, A. Magnon, A. Makins, N. Makke, N. Mallot, G. K. Marchand, C. Martin, A. Marzec, J. Matousek, J. Matsuda, H. Matsuda, T. Meshcheryakov, G. Meyer, W. Michigami, T. Mikhailov, Yu. V. Miyachi, Y. Nagaytsev, A. Nagel, T. Nerling, F. Neyret, D. Nikolaenko, V. I. Novy, J. Nowak, W. -D. Nunes, A. S. Olshevsky, A. G. Orlov, I. Ostrick, M. Panzieri, D. Parsamyan, B. Paul, S. Peng, J. -C. Pereira, F. Pesek, M. Peshekhonov, D. V. Platchkov, S. Pochodzalla, J. Polyakov, V. A. Pretz, J. Quaresma, M. Quintans, C. Ramos, S. Regali, C. Reicherz, G. Riedl, C. Rocco, E. Rossiyskaya, N. S. Ryabchikov, D. I. Rychter, A. Samoylenko, V. D. Sandacz, A. Santos, C. Sarkar, S. Savin, I. A. Sbrizzai, G. Schiavon, P. Schmeing, S. Schmidt, K. Schmieden, H. Schoenning, K. Schopferer, S. Schlueter, T. Selyunin, A. Shevchenko, O. Yu. Silva, L. Sinha, L. Sirtl, S. Slunecka, M. Sozzi, F. Srnka, A. Stolarski, M. Sulc, M. Suzuki, H. Szabelski, A. Szameitat, T. Sznajder, P. Takekawa, S. ter Wolbeek, J. Tessaro, S. Tessarotto, F. Thibaud, F. Tskhay, V. Uhl, S. Veloso, J. Virius, M. Wallner, S. Weisrock, T. Wilfert, M. Zaremba, K. Zavertyaev, M. Zemlyanichkina, E. Ziembicki, M. Zink, A. CA COMPASS Collaboration TI Observation of a New Narrow Axial-Vector Meson alpha(1)(1420) SO PHYSICAL REVIEW LETTERS LA English DT Article ID RESONANCE AB The COMPASS Collaboration at CERN has measured diffractive dissociation of 190 GeV/c pions into the pi(-) pi(-) pi(+) final state using a stationary hydrogen target. A partial- wave analysis (PWA) was performed in bins of 3 pi mass and four-momentum transfer using the isobar model and the so far largest PWA model consisting of 88 waves. A narrow peak is observed in the f(0)(980)pi channel with spin, parity and C-parity quantum numbers J(PC) = 1(++). We present a resonance- model study of a subset of the spin-density matrix selecting 3 pi states with J(PC) = 2(++) and 4(++) decaying into rho(770)pi and with J(PC) = 1(++) decaying into f(0)(980)pi. We identify a new a 1 meson with mass (1414(-13)(+15)) MeV/c(2) and width (153(-23)(+8)) MeV/c(2). Within the final states investigated in our analysis, we observe the new a(1)(1420) decaying only into f(0)(980)pi, suggesting its exotic nature. C1 [Panzieri, D.] Univ Piemonte Orientale, I-15100 Alessandria, Italy. [Azevedo, C.; Pereira, F.; Veloso, J.] Univ Aveiro, Dept Phys, P-3810193 Aveiro, Portugal. [Gautheron, F.; Koivuniemi, J. H.; Meyer, W.; Reicherz, G.] Ruhr Univ Bochum, Inst Expt Phys, D-44780 Bochum, Germany. [Beck, R.; Bisplinghoff, J.; Eversheim, P. D.; Hinterberger, F.; Jahn, R.; Joosten, R.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Barth, J.; Hahne, D.; Klein, F.; Pretz, J.; Schmieden, H.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Srnka, A.] Acad Sci Czech Republic, Inst Sci Instruments, CS-61264 Brno, Czech Republic. [Dasgupta, S. S.; Dhara, L.; Sarkar, S.; Sinha, L.] Matrivani Inst Expt Res & Educ, Kolkata 700030, W Bengal, India. [Akhunzyanov, R.; Alexeev, G. D.; Anosov, V.; Efremov, A.; Gavrichtchouk, O. P.; Guskov, A.; Ivanov, A.; Ivanshin, Yu.; Kisselev, Yu.; Kouznetsov, O.; Kroumchtein, Z. V.; Kuchinski, N.; Meshcheryakov, G.; Nagaytsev, A.; Olshevsky, A. G.; Orlov, I.; Peshekhonov, D. V.; Rossiyskaya, N. S.; Savin, I. A.; Selyunin, A.; Shevchenko, O. Yu.; Slunecka, M.; Zemlyanichkina, E.] Joint Inst Nucl Res, Dubna 141980, Moscow Region, Russia. [Adolph, C.; Braun, C.; Eyrich, W.; Lehmann, A.; Zink, A.] Univ Erlangen Nurnberg, Inst Phys, D-91054 Erlangen, Germany. [Buechele, M.; Fischer, H.; Gorzellik, M.; Grussenmeyer, T.; Heinsius, F. H.; Herrmann, F.; Joerg, P.; Koenigsmann, K.; Kremser, P.; Nowak, W. -D.; Regali, C.; Schmidt, K.; Schopferer, S.; Sirtl, S.; Szameitat, T.; ter Wolbeek, J.] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Austregesilo, A.; Bedfer, Y.; Bernhard, J.; Bicker, K.; Bielert, E. R.; von Hohenesche, N. du Fresne; Frolov, V.; Mallot, G. K.; Novy, J.; Rocco, E.; Schoenning, K.] CERN, CH-1211 Geneva 23, Switzerland. [Sulc, M.] Tech Univ Liberec, Liberec 46117, Czech Republic. [Bordalo, P.; Franco, C.; Nunes, A. S.; Quaresma, M.; Quintans, C.; Ramos, S.; Silva, L.; Stolarski, M.] LIP, P-1000149 Lisbon, Portugal. [Bernhard, J.; von Hohenesche, N. du Fresne; von Harrach, D.; Kabuss, E.; Nerling, F.; Ostrick, M.; Pochodzalla, J.; Weisrock, T.; Wilfert, M.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Matsuda, T.] Miyazaki Univ, Miyazaki 8892192, Japan. [Gerassimov, S.; Konorov, I.; Tskhay, V.; Zavertyaev, M.] PN Lebedev Phys Inst, Moscow 119991, Russia. [Austregesilo, A.; Bicker, K.; Chung, S. U.; Friedrich, J. M.; Gerassimov, S.; Grabmueller, S.; Grube, B.; Haas, F.; Huber, S.; Ketzer, B.; Konorov, I.; Kraemer, M.; Krinner, F.; Nagel, T.; Paul, S.; Schmeing, S.; Uhl, S.; Wallner, S.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Horikawa, N.] Nagoya Univ, Nagoya, Aichi 464, Japan. [Bodlak, M.; Finger, M.; Finger, M., Jr.; Matousek, J.] Charles Univ Prague, Fac Math & Phys, CR-18000 Prague, Czech Republic. [Jary, V.; Novy, J.; Pesek, M.; Virius, M.] Czech Tech Univ, Prague 16636, Czech Republic. [Donskov, S. V.; Khaustov, G. V.; Khokhlov, Yu. A.; Kolosov, V. N.; Konstantinov, V. F.; Lednev, A. A.; Mikhailov, Yu. V.; Nikolaenko, V. I.; Polyakov, V. A.; Ryabchikov, D. I.; Samoylenko, V. D.] Natl Res Ctr Kurchatov Inst, State Sci Ctr Inst High Energy Phys, Protvino 142281, Russia. [Andrieux, V.; Bedfer, Y.; Boer, M.; Burtin, E.; Curiel, Q.; Ferrero, A.; d'Hose, N.; Kunne, F.; Levillain, M.; Magnon, A.; Marchand, C.; Neyret, D.; Platchkov, S.; Thibaud, F.] CEA IRFU SPhN Saclay, F-91191 Gif Sur Yvette, France. [Chang, W. -C.; Hsieh, C. -Yu] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Lichtenstadt, J.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bradamante, F.; Bressan, A.; Duic, V.; Makke, N.; Martin, A.; Sbrizzai, G.; Schiavon, P.] Univ Trieste, Dept Phys, I-34127 Trieste, Italy. [Birsa, R.; Bradamante, F.; Bressan, A.; Cicuttin, A.; Crespo, M. L.; Dalla Torre, S.; Dasgupta, S.; Levorato, S.; Makke, N.; Martin, A.; Santos, C.; Sbrizzai, G.; Schiavon, P.; Sozzi, F.; Tessaro, S.; Tessarotto, F.] Ist Nazl Fis Nucl, Trieste Sect, I-34127 Trieste, Italy. [Cicuttin, A.; Crespo, M. L.] Abdus Salam Int Ctr Theoret Phys, I-34151 Trieste, Italy. [Alexeev, M. G.; Amoroso, A.; Balestra, F.; Chiosso, M.; Gnesi, I.; Grasso, A.; Kotzinian, A. M.; Parsamyan, B.; Takekawa, S.] Univ Turin, Dept Phys, I-10125 Turin, Italy. [Amoroso, A.; Balestra, F.; Chiosso, M.; Denisov, O. Yu.; Gnesi, I.; Grasso, A.; Kotzinian, A. M.; Maggiora, A.; Panzieri, D.; Parsamyan, B.; Takekawa, S.] INFN, Torino Sect, I-10125 Turin, Italy. [Choi, I.; Grosse-Perdekamp, M.; Makins, N.; Peng, J. -C.; Riedl, C.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Klimaszewski, K.; Kurek, K.; Sandacz, A.; Szabelski, A.; Sznajder, P.] Natl Ctr Nucl Res, PL-00681 Warsaw, Poland. [Badelek, B.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Dziewiecki, M.; Kurjata, R. P.; Marzec, J.; Rychter, A.; Zaremba, K.; Ziembicki, M.] Warsaw Univ Technol, Inst Radioelect, PL-00665 Warsaw, Poland. [Doshita, N.; Hashimoto, R.; Ishimoto, S.; Iwata, T.; Kondo, K.; Matsuda, H.; Michigami, T.; Miyachi, Y.; Suzuki, H.] Yamagata Univ, Yamagata 9928510, Japan. [Bordalo, P.; Ramos, S.] Univ Lisbon, Inst Super Tecn, P-1699 Lisbon, Portugal. [Chung, S. U.] Pusan Natl Univ, Dept Phys, Pusan 609735, South Korea. [Chung, S. U.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Horikawa, N.; Suzuki, H.] Chubu Univ, Kasugai, Aichi 4878501, Japan. [Ishimoto, S.] KEK, Tsukuba, Ibaraki 3050801, Japan. [Khokhlov, Yu. A.] Moscow Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. RP Bressan, A (reprint author), Univ Trieste, Dept Phys, I-34127 Trieste, Italy. EM andrea.bressan@cern.ch; bgrube@tum.de; fabienne.kunne@cea.fr RI Paul, Stephan/K-9237-2016; Silva, Luis/M-4435-2016; Dasgupta, Shuddha Shankar/O-6118-2016; Srnka, A/E-2441-2012; Martin, Anna/I-9381-2012; Koivuniemi, Jaakko/L-2959-2015; Zavertyaev, Mikhail/M-6844-2015; Gerassimov, Sergei/M-8779-2015; Tskhay, Vladimir/N-1711-2015; Azevedo, Carlos/J-5733-2013; Kurjata, Robert/I-5112-2016; Paul, Stephan/F-7596-2015; veloso, joao/J-4478-2013; Friedrich, Jan/B-9024-2013; Olshevskiy, Alexander/I-1580-2016 OI Paul, Stephan/0000-0002-8813-0437; Silva, Luis/0000-0003-0044-3736; Amoroso, Antonio/0000-0002-3095-8610; Martin, Anna/0000-0002-1333-0143; Koivuniemi, Jaakko/0000-0002-6817-5267; Azevedo, Carlos/0000-0002-0012-9918; Kurjata, Robert/0000-0001-8547-910X; Paul, Stephan/0000-0002-8813-0437; Friedrich, Jan/0000-0001-9298-7882; Olshevskiy, Alexander/0000-0002-8902-1793 FU CERN management; MEYS (Czech Republic); European Union; CEA (France); P2I (France); ANR (France); BMBF; DFG cluster of excellence "Origin and Structure of the Universe"; computing facilities of the Computational Center for Particle and Astrophysics (C2PAP); IAS-TUM; Humboldt foundation (Germany); SAIL (CSR) (India); ISF (Israel); INFN (Italy); MEXT (Japan); JSPS (Japan); Daiko (Japan); Yamada Foundations (Japan); NRF (Rep. of Korea); NCN (Poland); FCT (Portugal); CERN-RFBR (Russia); Presidential Grant (Russia) [NSh-999.2014.2] FX We gratefully acknowledge the support of the CERN management and staff as well as the skills and efforts of the technicians of the collaborating institutions. This work is supported by MEYS (Czech Republic); "HadronPhysics2" Integrating Activity in FP7 (European Union); CEA, P2I, and ANR (France); BMBF, DFG cluster of excellence "Origin and Structure of the Universe", the computing facilities of the Computational Center for Particle and Astrophysics (C2PAP), IAS-TUM, and the Humboldt foundation (Germany); SAIL (CSR) (India); ISF (Israel); INFN (Italy); MEXT, JSPS, Daiko, and Yamada Foundations (Japan); NRF (Rep. of Korea); NCN (Poland); FCT (Portugal); CERN-RFBR and Presidential Grant NSh-999.2014.2 (Russia). NR 28 TC 16 Z9 16 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 19 PY 2015 VL 115 IS 8 AR 082001 DI 10.1103/PhysRevLett.115.082001 PG 6 WC Physics, Multidisciplinary SC Physics GA CP4SJ UT WOS:000359872600002 PM 26340182 ER PT J AU Cherkashyna, N DiJulio, DD Panzner, T Rantsiou, E Filges, U Ehlers, G Bentley, PM AF Cherkashyna, Nataliia DiJulio, Douglas D. Panzner, Tobias Rantsiou, Emmanouela Filges, Uwe Ehlers, Georg Bentley, Phillip M. TI Benchmarking shielding simulations for an accelerator-driven spallation neutron source SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB The shielding at an accelerator-driven spallation neutron facility plays a critical role in the performance of the neutron scattering instruments, the overall safety, and the total cost of the facility. Accurate simulation of shielding components is thus key for the design of upcoming facilities, such as the European Spallation Source (ESS), currently in construction in Lund, Sweden. In this paper, we present a comparative study between the measured and the simulated neutron background at the Swiss Spallation Neutron Source (SINQ), at the Paul Scherrer Institute (PSI), Villigen, Switzerland. The measurements were carried out at several positions along the SINQ monolith wall with the neutron dosimeter WENDI-2, which has a well-characterized response up to 5 GeV. The simulations were performed using the Monte-Carlo radiation transport code Geant4, and include a complete transport from the proton beam to the measurement locations in a single calculation. An agreement between measurements and simulations is about a factor of 2 for the points where the measured radiation dose is above the background level, which is a satisfactory result for such simulations spanning many energy regimes, different physics processes and transport through several meters of shielding materials. The neutrons contributing to the radiation field emanating from the monolith were confirmed to originate from neutrons with energies above 1 MeV in the target region. The current work validates Geant4 as being well suited for deep-shielding calculations at accelerator-based spallation sources. We also extrapolate what the simulated flux levels might imply for short (several tens of meters) instruments at ESS. C1 [Cherkashyna, Nataliia; DiJulio, Douglas D.; Bentley, Phillip M.] European Spallat Source ESS AB, SE-22100 Lund, Sweden. [Panzner, Tobias; Rantsiou, Emmanouela; Filges, Uwe] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Ehlers, Georg] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Bentley, Phillip M.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. RP Cherkashyna, N (reprint author), European Spallat Source ESS AB, POB 176, SE-22100 Lund, Sweden. EM nataliia.cherkashyna@esss.se RI Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008 OI Ehlers, Georg/0000-0003-3513-508X FU Scientific User Facilities Division; Office of Basic Energy Sciences; U.S. Department of Energy FX One of the authors (G. E.) acknowledges funding by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 21 TC 1 Z9 1 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD AUG 19 PY 2015 VL 18 IS 8 AR 083501 DI 10.1103/PhysRevSTAB.18.083501 PG 7 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CP5EI UT WOS:000359903700003 ER PT J AU Yoon, J Kim, S Kim, D Kim, ID Hong, S No, K AF Yoon, Jaesung Kim, Sangjoon Kim, Dongjin Kim, Il-Doo Hong, Seungbum No, Kwangsoo TI Fabrication of Highly Ordered and Well-Aligned PbTiO3/TiN Core-Shell Nanotube Arrays SO SMALL LA English DT Article DE core-shell nanostructures; nanotube arrays; PbTiO3; piezoresponse force microscopy ID ATOMIC LAYER DEPOSITION; TITANIUM NITRIDE; MICROSCOPY; PRECURSOR C1 [Yoon, Jaesung; Kim, Sangjoon; Kim, Dongjin; Kim, Il-Doo; Hong, Seungbum; No, Kwangsoo] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Hong, S (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, 291 Daehak Ro, Taejon 305701, South Korea. EM hong@anl.gov; ksno@kaist.ac.kr RI Hong, Seungbum/B-7708-2009; No, Kwangsoo/C-1983-2011; Kim, Il-Doo/C-1850-2011 OI Hong, Seungbum/0000-0002-2667-1983; FU Mid-career Researcher Program through the National Research Foundation of Korea - Ministry of Education, Science and Technology [2010-0015063]; KIMM; National Research Council of Science & Technology (NST), Republic of Korea; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX J.Y. and S.K. contributed equally to this work. This research was supported by the Mid-career Researcher Program (2010-0015063) through the National Research Foundation of Korea funded by Ministry of Education, Science and Technology and the KIMM and the National Research Council of Science & Technology (NST), Republic of Korea. Work at Argonne National Laboratory (S.H., data analysis and writing of manuscript) was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 28 TC 1 Z9 1 U1 5 U2 26 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD AUG 19 PY 2015 VL 11 IS 31 BP 3750 EP 3754 DI 10.1002/smll.201500087 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CP5GI UT WOS:000359908900003 PM 25929761 ER PT J AU Witzel, WM Montano, I Muller, RP Carroll, MS AF Witzel, Wayne M. Montano, Ines Muller, Richard P. Carroll, Malcolm S. TI Multiqubit gates protected by adiabaticity and dynamical decoupling applicable to donor qubits in silicon SO PHYSICAL REVIEW B LA English DT Article ID OPEN QUANTUM-SYSTEMS; PYTHON FRAMEWORK; ELECTRON-SPIN; READOUT; PULSES; QUTIP; DOT AB We present a strategy for producing multiqubit gates that promise high fidelity with minimal tuning requirements. Our strategy combines gap protection from the adiabatic theorem with dynamical decoupling in a complementary manner. Energy-level transition errors are protected by adiabaticity and remaining phase errors are mitigated via dynamical decoupling. This is a powerful way to divide and conquer the various error channels. In order to accomplish this without violating a no-go theorem regarding black-box dynamically corrected gates [Phys. Rev. A 80, 032314 (2009)], we require a robust operating point (sweet spot) in control space where the qubits interact with little sensitivity to noise. There are also energy gap requirements for effective adiabaticity. We apply our strategy to an architecture in Si with P donors where we assume we can shuttle electrons between different donors. Electron spins act as mobile ancillary qubits and P nuclear spins act as long-lived data qubits. This system can have a very robust operating point where the electron spin is bound to a donor in the quadratic Stark shift regime. High fidelity single qubit gates may be performed using well-established global magnetic resonance pulse sequences. Single electron-spin preparation and measurement has also been demonstrated. Putting this all together, we present a robust universal gate set for quantum computation. C1 [Witzel, Wayne M.; Muller, Richard P.] Sandia Natl Labs, Ctr Comp Res, Albuquerque, NM 87185 USA. [Montano, Ines; Carroll, Malcolm S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Witzel, WM (reprint author), Sandia Natl Labs, Ctr Comp Res, POB 5800, Albuquerque, NM 87185 USA. EM wwitzel@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We acknowledge numerous discussions with intellectual contributions to this work from our diverse, multidisciplinary team of quantum device and architecture experts at Sandia National Laboratories including N. Bishop, R. Blume-Kohout, J. Gamble, A. Ganti, M. Grace, N. T. Jacobson, A. Landahl, E. Nielsen, and K. Young. We also acknowledge R. Rahman and G. Klimeck for assistance and support with the NEMO-3D simulations. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 39 TC 0 Z9 0 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 19 PY 2015 VL 92 IS 8 AR 081407 DI 10.1103/PhysRevB.92.081407 PG 5 WC Physics, Condensed Matter SC Physics GA CP4OC UT WOS:000359860700004 ER PT J AU LaHaye, NL Kurian, J Diwakar, PK Alff, L Harilal, SS AF LaHaye, Nicole L. Kurian, Jose Diwakar, Prasoon K. Alff, Lambert Harilal, Sivanandan S. TI Femtosecond laser ablation-based mass spectrometry: An ideal tool for stoichiometric analysis of thin films SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULAR-BEAM EPITAXY; MS SIGNAL INTENSITY; LA-ICP-MS; ELEMENTAL FRACTIONATION; MATERIALS SCIENCE; REPETITION RATE; PULSE DURATION; DEPOSITION; LAYERS; OXIDES AB An accurate and routinely available method for stoichiometric analysis of thin films is a desideratum of modern materials science where a material's properties depend sensitively on elemental composition. We thoroughly investigated femtosecond laser ablation-inductively coupled plasma-mass spectrometry (fs-LA-ICP-MS) as an analytical technique for determination of the stoichiometry of thin films down to the nanometer scale. The use of femtosecond laser ablation allows for precise removal of material with high spatial and depth resolution that can be coupled to an ICP-MS to obtain elemental and isotopic information. We used molecular beam epitaxy-grown thin films of LaPd(x)Sb-2 and T'-La2CuO4 to demonstrate the capacity of fs-LA-ICP-MS for stoichiometric analysis and the spatial and depth resolution of the technique. Here we demonstrate that the stoichiometric information of thin films with a thickness of similar to 10 nm or lower can be determined. Furthermore, our results indicate that fs-LA-ICP-MS provides precise information on the thin film-substrate interface and is able to detect the interdiffusion of cations. C1 [LaHaye, Nicole L.; Harilal, Sivanandan S.] Pacific NW Natl Lab, Richland, WA 99352 USA. [LaHaye, Nicole L.; Diwakar, Prasoon K.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47906 USA. [Kurian, Jose; Alff, Lambert] Tech Univ Darmstadt, Inst Mat Sci, D-64287 Darmstadt, Germany. RP Harilal, SS (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM hari@pnnl.gov RI Harilal, Sivanandan/B-5438-2014; OI Harilal, Sivanandan/0000-0003-2266-7976; LaHaye, Nicole/0000-0001-5047-8078 FU DOE/NNSA Office of Nonproliferation and Verification Research and Development [NA-22]; Laboratory Directed Research and Development (LDRD) Program of PNNL; U.S. National Science Foundation; U.S. Department of Energy [DE-AC05-76RLO1830] FX This work was supported in part by DOE/NNSA Office of Nonproliferation and Verification Research and Development (NA-22), the Laboratory Directed Research and Development (LDRD) Program of PNNL and the U.S. National Science Foundation. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC05-76RLO1830. NR 58 TC 5 Z9 5 U1 7 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 19 PY 2015 VL 5 AR 13121 DI 10.1038/srep13121 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2FL UT WOS:000359692800001 PM 26285795 ER PT J AU Kim, JB Weichman, ML Neumark, DM AF Kim, Jongjin B. Weichman, Marissa L. Neumark, Daniel M. TI Low-lying states of FeO and FeO- by slow photoelectron spectroscopy SO MOLECULAR PHYSICS LA English DT Article DE photoelectron; iron; metal oxide; spectroscopy ID MILLIMETER-WAVE SPECTRUM; 5-DELTA-I GROUND-STATE; ELECTRONIC-STRUCTURE; EXCITED-STATES; IRON MONOXIDE; NEGATIVE-IONS; PHOTODETACHMENT SPECTROSCOPY; ANGULAR-DISTRIBUTIONS; DIATOMIC-MOLECULES; DIPOLE-MOMENTS AB High-resolution anion photoelectron spectra of FeO- were acquired by slow electron velocity-map imaging of trapped and cooled ions. Ions were cooled to different temperatures by controlling the conditions in the trap, allowing us to disentangle contributions in the spectra from two different anion states. The spectra show that photodetachment of the two anion states accesses three low-lying neutral FeO states with one state in common, allowing us to derive term energies of all five states. The ground anion state is confirmed to be the X (4)Delta state, and FeO is found to have an electron affinity of 1.4950 eV. We assign the anion a (6)sigma(+) state, and obtain a term energy of 0.117 eV. The A (5)sigma(+) and a (7)sigma(+) neutral states are reassigned, and have term energies of 0.258 and 0.616 eV, respectively, relative to the neutral X (5)Delta(4) ground state. C1 [Kim, Jongjin B.; Weichman, Marissa L.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009; OI Neumark, Daniel/0000-0002-3762-9473; Weichman, Marissa/0000-0002-2551-9146 FU Air Force Office of Scientific Research [FA9550-12-1-0160]; Defense University Research Instrumentation Program [FA9550-11-1-0330]; National Science Foundation FX This work is funded by the Air Force Office of Scientific Research [grant number FA9550-12-1-0160] and the Defense University Research Instrumentation Program [grant number FA9550-11-1-0330]. Marissa L. Weichman thanks the National Science Foundation for a graduate research fellowship. NR 55 TC 1 Z9 1 U1 4 U2 24 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD AUG 18 PY 2015 VL 113 IS 15-16 SI SI BP 2105 EP 2114 DI 10.1080/00268976.2015.1005706 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ9BN UT WOS:000360906000008 ER PT J AU Savee, JD Zador, J Hemberger, P Sztaray, B Bodi, A Osborn, DL AF Savee, John D. Zador, Judit Hemberger, Patrick Sztaray, Balint Bodi, Andras Osborn, David L. TI Threshold photoelectron spectrum of the benzyl radical SO MOLECULAR PHYSICS LA English DT Article DE PEPICO; benzylium; photoelectron; benzyl ID DIFFUSE INTERSTELLAR BANDS; SPECTROSCOPY; PHOTOIONIZATION; HYDROCARBONS; IONIZATION; RESOLUTION; KINETICS; CARRIERS; CATIONS; STATES AB We measure threshold photoelectron spectra of the benzyl radical, which show transitions to at least three electronic states of the benzylium cation: [GRAPHICS] (1)A(1), [GRAPHICS] B-3(2), and [GRAPHICS] B-1(2), with possible contributions from transitions to [GRAPHICS] (3)A(1). The main features in the vibrationally resolved threshold photoelectron spectrum between 7.1 and 10.5 eV are assigned with the aid of Franck-Condon simulations to these four electronic states of benzylium. We measure the adiabatic ionisation energy of the benzyl radical to be 7.252(5) eV and observe a well-resolved vibrational progression in the lowest triplet state, [GRAPHICS] B-3(2), from which we obtain a measured singlet-triplet splitting of 1.928(7) eV in benzylium. C1 [Savee, John D.; Zador, Judit; Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. [Hemberger, Patrick; Bodi, Andras] Paul Scherrer Inst, Mol Dynam Grp, CH-5232 Villigen, Switzerland. [Sztaray, Balint] Univ Pacific, Dept Chem, Stockton, CA 95211 USA. RP Osborn, DL (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. EM dlosbor@sandia.gov RI Zador, Judit/A-7613-2008; Hemberger, Patrick/E-7909-2017; OI Zador, Judit/0000-0002-9123-8238; Hemberger, Patrick/0000-0002-1251-4549; Bodi, Andras/0000-0003-2742-1051 FU National Nuclear Security Administration [DE-AC04-94-AL85000]; Swiss Federal Office for Energy [BFE] [101969/152433]; National Science Foundation [CHE-1266407] FX Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration [contract DE-AC04-94-AL85000]; Andras Bodi and Patrick Hemberger gratefully acknowledge support by the Swiss Federal Office for Energy [BFE contract number 101969/152433]; Balint Sztaray is supported by the National Science Foundation [CHE-1266407]. NR 37 TC 4 Z9 4 U1 5 U2 18 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD AUG 18 PY 2015 VL 113 IS 15-16 SI SI BP 2217 EP 2227 DI 10.1080/00268976.2015.1021398 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ9BN UT WOS:000360906000019 ER PT J AU Ormond, TK Hemberger, P Troy, TP Ahmed, M Stanton, JF Ellison, GB AF Ormond, Thomas K. Hemberger, Patrick Troy, Tyler P. Ahmed, Musahid Stanton, John F. Ellison, G. Barney TI The ionisation energy of cyclopentadienone: a photoelectron-photoion coincidence study SO MOLECULAR PHYSICS LA English DT Article DE iPEPICO; pyrolysis; microtubular reactor ID THERMAL-DECOMPOSITION; BASIS-SETS; SPECTROSCOPY; PYROLYSIS; STATES; MASS; INTERMEDIATE; DERIVATIVES; COMBUSTION; MOLECULES AB Imaging photoelectron photoion coincidence (iPEPICO) spectra of cyclopentadienone (C5H4=O and C5D4=O) have been measured at the Swiss Light Source Synchrotron (Paul Scherrer Institute, Villigen, Switzerland) at the Vacuum Ultraviolet (VUV) Beamline. Complementary to the photoelectron spectra, photoionisation efficiency curves were measured with tunable VUV radiation at the Chemical Dynamics Beamline at the Advanced Light Source Synchrotron (Lawrence Berkeley National Laboratory, Berkeley, CA, USA). For both experiments, molecular beams diluted in argon and helium were generated from the vacuum flash pyrolysis of o-phenylene sulphite in a resistively heated microtubular SiC flow reactor. The Franck-Condon profiles and ionisation energies were calculated at the CCSD(T) level of theory, and are in excellent agreement with the observed iPEPICO spectra. The ionisation energies of both cyclopentadienone-d(0), IE(C5H4=O), and cyclopentadienone-d(4), IE(C5D4=O), were observed to be the same: 9.41 +/- 0.01 eV. The mass-selected threshold photoelectron spectrum (ms-TPES) of cyclopentadienone reveals that the C=C stretch in the ground state of the cation is excited upon ionisation, supporting computational evidence that the ground state of the cation is [GRAPHICS] (2)A(2), and is in agreement with previous studies. However, the previously reported ionisation potential has been improved considerably in this work. In addition, since o-benzoquinone (o-O=C6H4=O and o-O=C6D4=O) is also produced in this process, its ms-TPES has been recorded. From the iPEPICO and photoionisation efficiency spectra, we infer an adiabatic ionisation energy of IE(o-O=C6H4=O) = 9.3 +/- 0.1 eV, but the rather structureless spectrum indicates a strong change in geometry upon ionisation making this value less reliable. C1 [Ormond, Thomas K.; Ellison, G. Barney] Univ Colorado, Dept Chem, Boulder, CO 80309 USA. [Hemberger, Patrick] Paul Scherrer Inst, Mol Dynam Grp, Villigen, Switzerland. [Troy, Tyler P.; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Dynam Beamline, Berkeley, CA 94720 USA. [Stanton, John F.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. RP Ellison, GB (reprint author), Univ Colorado, Dept Chem, Boulder, CO 80309 USA. EM barney@jila.colorado.edu RI Ahmed, Musahid/A-8733-2009; Hemberger, Patrick/E-7909-2017 OI Hemberger, Patrick/0000-0002-1251-4549 FU US National Science Foundation [CHE-1112466]; US Department of Energy, Office of Science, Basic Energy Sciences [DE-FG02-07ER1588]; Robert A. Welch Foundation of Houston, TX [F-1283]; Chemical Sciences Division of the US Department of Energy [DE-AC02-05CH11231]; Swiss Federal Office for Energy [BFE] [101969/152433] FX T.K. Ormond, G.B. Ellison and J.F. Stanton: US National Science Foundation [grant number CHE-1112466]; J.F. Stanton: US Department of Energy, Office of Science, Basic Energy Sciences [award number DE-FG02-07ER1588]; Robert A. Welch Foundation of Houston, TX [grant number F-1283]; T.P. Troy and M. Ahmed: Director of the Office of Energy Research; Office of Basic Energy Sciences; Chemical Sciences Division of the US Department of Energy [contract number DE-AC02-05CH11231]. Swiss Federal Office for Energy [BFE contract number 101969/152433]. NR 39 TC 2 Z9 2 U1 1 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD AUG 18 PY 2015 VL 113 IS 15-16 SI SI BP 2350 EP 2358 DI 10.1080/00268976.2015.1042936 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ9BN UT WOS:000360906000030 ER PT J AU Varghese, NJ Mukherjee, S Ivanova, N Konstantinidis, KT Mavrommatis, K Kyrpides, NC Pati, A AF Varghese, Neha J. Mukherjee, Supratim Ivanova, Natalia Konstantinidis, Konstantinos T. Mavrommatis, Kostas Kyrpides, Nikos C. Pati, Amrita TI Microbial species delineation using whole genome sequences SO NUCLEIC ACIDS RESEARCH LA English DT Article ID BACILLUS-CEREUS GROUP; REAL-TIME PCR; BURKHOLDERIA-PSEUDOMALLEI; SP NOV.; MALLEI; IDENTIFICATION; THAILANDENSIS; DEFINITION; PHYLOGENY; BOTULINUM AB Increased sequencing of microbial genomes has revealed that prevailing prokaryotic species assignments can be inconsistent with whole genome information for a significant number of species. The long-standing need for a systematic and scalable species assignment technique can be met by the genome-wide Average Nucleotide Identity (gANI) metric, which is widely acknowledged as a robust measure of genomic relatedness. In this work, we demonstrate that the combination of gANI and the alignment fraction (AF) between two genomes accurately reflects their genomic relatedness. We introduce an efficient implementation of AF, gANI and discuss its successful application to 86.5M genome pairs between 13,151 prokaryotic genomes assigned to 3032 species. Subsequently, by comparing the genome clusters obtained from complete linkage clustering of these pairs to existing taxonomy, we observed that nearly 18% of all prokaryotic species suffer from anomalies in species definition. Our results can be used to explore central questions such as whether microorganisms form a continuum of genetic diversity or distinct species represented by distinct genetic signatures. We propose that this precise and objective AF, gANI-based species definition: the MiSI (Microbial Species Identifier) method, be used to address previous inconsistencies in species classification and as the primary guide for new taxonomic species assignment, supplemented by the traditional polyphasic approach, as required. C1 [Varghese, Neha J.; Mukherjee, Supratim; Ivanova, Natalia; Kyrpides, Nikos C.; Pati, Amrita] DOE Joint Genom Inst, Microbial & Metagenome Superprogram, Walnut Creek, CA 94598 USA. [Konstantinidis, Konstantinos T.] Georgia Inst Technol, Dept Civil & Environm Engn, Atlanta, GA 30332 USA. [Mavrommatis, Kostas] Celgene Corp, San Francisco, CA 94158 USA. RP Varghese, NJ (reprint author), DOE Joint Genom Inst, Microbial & Metagenome Superprogram, Walnut Creek, CA 94598 USA. EM njvarghese@lbl.gov; nckyrpides@lbl.gov; apati@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU LDRD grant [YLD012]; US Department of Energy Joint Genome Institute, Office of Science of the US Department of Energy [DE-AC02-05CH11231, DE-AC02-5CH11231] FX LDRD grant YLD012: Computational, Data Management and Analysis Methods for the Study of a Rapidly Expanding Genome and Metagenome Sequence Data Space (YLD012); US Department of Energy Joint Genome Institute, Office of Science of the US Department of Energy [DE-AC02-05CH11231]. Funding for open access charge: US Department of Energy Joint Genome Institute, Office of Science of the US Department of Energy [DE-AC02-5CH11231]. NR 30 TC 40 Z9 40 U1 6 U2 28 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 18 PY 2015 VL 43 IS 14 BP 6761 EP 6771 DI 10.1093/nar/gkv657 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CQ4PX UT WOS:000360588200017 PM 26150420 ER PT J AU Kukshal, V Kim, IK Hura, GL Tomkinson, AE Tainer, JA Ellenberger, T AF Kukshal, Vandna Kim, In-Kwon Hura, Gregory L. Tomkinson, Alan E. Tainer, John A. Ellenberger, Tom TI Human DNA ligase III bridges two DNA ends to promote specific intermolecular DNA end joining SO NUCLEIC ACIDS RESEARCH LA English DT Article ID STRAND BREAK REPAIR; X-RAY-SCATTERING; ZINC-FINGER; POLY(ADP-RIBOSE) POLYMERASE; NICK RECOGNITION; BINDING; XRCC1; CELLS; MITOCHONDRIA; LIGATION AB Mammalian DNA ligase III (LigIII) functions in both nuclear and mitochondrial DNA metabolism. In the nucleus, LigIII has functional redundancy with DNA ligase I whereas LigIII is the only mitochondrial DNA ligase and is essential for the survival of cells dependent upon oxidative respiration. The unique LigIII zinc finger (ZnF) domain is not required for catalytic activity but senses DNA strand breaks and stimulates intermolecular ligation of two DNAs by an unknown mechanism. Consistent with this activity, LigIII acts in an alternative pathway of DNA double strand break repair that buttresses canonical non-homologous end joining (NHEJ) and is manifest in NHEJ-defective cancer cells, but how LigIII acts in joining intermolecular DNA ends versus nick ligation is unclear. To investigate how LigIII efficiently joins two DNAs, we developed a real-time, fluorescence-based assay of DNA bridging suitable for high-throughput screening. On a nicked duplex DNA substrate, the results reveal binding competition between the ZnF and the oligonucleotide/oligosaccharide-binding domain, one of three domains constituting the LigIII catalytic core. In contrast, these domains collaborate and are essential for formation of a DNA-bridging intermediate by adenylated LigIII that positions a pair of blunt-ended duplex DNAs for efficient and specific intermolecular ligation. C1 [Kukshal, Vandna; Kim, In-Kwon; Ellenberger, Tom] Washington Univ, Sch Med, Dept Biochem & Mol Biophys, St Louis, MO 63110 USA. [Hura, Gregory L.; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Tomkinson, Alan E.] Univ New Mexico, Dept Internal Med, Albuquerque, NM 87131 USA. [Tomkinson, Alan E.] Univ New Mexico, Ctr Canc, Albuquerque, NM 87131 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, Houston, TX 77030 USA. RP Ellenberger, T (reprint author), Washington Univ, Sch Med, Dept Biochem & Mol Biophys, St Louis, MO 63110 USA. EM tome@biochem.wustl.edu OI kukshal, vandna/0000-0002-6207-2638 FU National Institutes of Health [GM052504, P01 CA92584, ES0112512] FX National Institutes of Health [GM052504 to T.E., P01 CA92584 to J.A.T., A.T., T.E., ES0112512 to A.T.]. Funding for the open access charge: Institutional startup funds. NR 48 TC 3 Z9 3 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 18 PY 2015 VL 43 IS 14 BP 7021 EP 7031 DI 10.1093/nar/gkv652 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CQ4PX UT WOS:000360588200036 PM 26130724 ER PT J AU Gonzalez, TL Liang, Y Nguyen, BN Staskawicz, BJ Loque, D Hammond, MC AF Gonzalez, Tania L. Liang, Yan Nguyen, Bao N. Staskawicz, Brian J. Loque, Dominique Hammond, Ming C. TI Tight regulation of plant immune responses by combining promoter and suicide exon elements SO NUCLEIC ACIDS RESEARCH LA English DT Article ID BACTERIAL SPOT DISEASE; III EFFECTOR PROTEINS; CELL-DEATH; RESISTANCE PROTEIN; GENE-EXPRESSION; AVIRULENCE GENE; CLIMATE-CHANGE; ARABIDOPSIS; PEPPER; EDS1 AB Effector-triggered immunity (ETI) is activated when plant disease resistance (R) proteins recognize the presence of pathogen effector proteins delivered into host cells. The ETI response generally encompasses a defensive 'hypersensitive response' (HR) that involves programmed cell death at the site of pathogen recognition. While many R protein and effector protein pairs are known to trigger HR, other components of the ETI signaling pathway remain elusive. Effector genes regulated by inducible promoters cause background HR due to leaky protein expression, preventing the generation of relevant transgenic plant lines. By employing the HyP5SM suicide exon, we have developed a strategy to tightly regulate effector proteins such that HR is chemically inducible and non-leaky. This alternative splicing-based gene regulation system was shown to successfully control Bs2/AvrBs2-dependent and RPP1/ATR1 Delta 51-dependent HR in Nicotiana benthamiana and Nicotiana tabacum, respectively. It was also used to generate viable and healthy transgenic Arabidopsis thaliana plants that inducibly initiate HR. Beyond enabling studies on the ETI pathway, our regulatory strategy is generally applicable to reduce or eliminate undesired background expression of transgenes. C1 [Gonzalez, Tania L.; Hammond, Ming C.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Liang, Yan; Loque, Dominique] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Liang, Yan; Loque, Dominique; Hammond, Ming C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Nguyen, Bao N.] Univ Calif Berkeley, Dept Integrat Biol, Berkeley, CA 94720 USA. [Staskawicz, Brian J.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Hammond, Ming C.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Hammond, MC (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM mingch@berkeley.edu RI Gonzalez, Tania/E-4812-2011; Loque, Dominique/A-8153-2008; Liang, Yan/K-8199-2016 OI Gonzalez, Tania/0000-0003-3825-8544; Liang, Yan/0000-0002-2144-1388 FU National Institutes of Health New Innovator Award [1DP2-OD008677]; Burroughs Wellcome Fund [CASI 1007224]; UC Berkeley Chancellor's Opportunity Fellowship; NIGMS Center for RNA Systems Biology at UC Berkeley [P50-GM102706]; DOE Early Career Award; DOE Joint BioEnergy Institute - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX National Institutes of Health New Innovator Award (1DP2-OD008677 to M.C.H.); Career Award at the Scientific Interface from the Burroughs Wellcome Fund (CASI 1007224 to M.C.H.); UC Berkeley Chancellor's Opportunity Fellowship (to T.L.G); NIGMS Center for RNA Systems Biology at UC Berkeley (P50-GM102706, in part to M.C.H.); DOE Early Career Award and DOE Joint BioEnergy Institute supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research through contract (DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy to Y.L. and D.L.). Funding for open access charge: Burroughs Wellcome Fund. NR 46 TC 1 Z9 1 U1 1 U2 10 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 18 PY 2015 VL 43 IS 14 BP 7152 EP 7161 DI 10.1093/nar/gkv655 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CQ4PX UT WOS:000360588200046 PM 26138488 ER PT J AU Nutaro, J Fugate, D Kuruganti, T Sanyal, J Starke, M AF Nutaro, James Fugate, David Kuruganti, Teja Sanyal, Jibonananda Starke, Michael TI Cost-effective retrofit technology for reducing peak power demand in small and medium commercial buildings SO SCIENCE AND TECHNOLOGY FOR THE BUILT ENVIRONMENT LA English DT Article AB This article describes a cost-effective retrofit technology that uses collective control of multiple rooftop air-conditioning units to reduce the peak power consumption of small and medium commercial buildings. The proposed control uses a model of the building and air-conditioning units to select an operating schedule for the air-conditioning units that maintains a temperature set-point subject to a constraint on the number of units that may operate simultaneously. A prototype of this new control system was built and deployed in a large gymnasium to coordinate four rooftop air-conditioning units. Based on data collected while operating this prototype, it is estimated that the cost savings achieved by reducing peak power consumption is sufficient to repay the cost of the prototype within a year. C1 [Nutaro, James; Kuruganti, Teja] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. [Fugate, David; Starke, Michael] Oak Ridge Natl Lab, Elect & Elect Syst Res Div, Oak Ridge, TN 37831 USA. [Sanyal, Jibonananda] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Kuruganti, T (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM kurugantipv@ornl.gov OI Nutaro, James/0000-0001-7360-2836 FU U.S. Department of Energy [DE-AC05-00OR22725] FX This manuscript has been authored by UT-Battelle, LLC under contract DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. Government retains, and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. The U.S. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 7 TC 0 Z9 0 U1 0 U2 5 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 2374-4731 EI 2374-474X J9 SCI TECHNOL BUILT EN JI Sci. Technol. Built Environ. PD AUG 18 PY 2015 VL 21 IS 6 SI SI BP 761 EP 772 DI 10.1080/23744731.2015.1047719 PG 12 WC Thermodynamics; Construction & Building Technology; Engineering, Mechanical SC Thermodynamics; Construction & Building Technology; Engineering GA CQ3FQ UT WOS:000360487700003 ER PT J AU Hess, M Peterson, K Harvey-Thompson, A AF Hess, M. Peterson, K. Harvey-Thompson, A. TI An efficient method for unfolding kinetic pressure driven VISAR data SO HIGH POWER LASER SCIENCE AND ENGINEERING LA English DT Article DE laser driven blast wave; pulsed-power; VISAR AB Velocity Interferometer System for Any Reflector (VISAR) [Barker and Hollenbach, J. Appl. Phys. 43, 4669 (1972)] is a well-known diagnostic that is employed on many shock physics and pulsed-power experiments. With the VISAR diagnostic, the velocity on the surface of any metal flyer can be found. For most experiments employing VISAR, either a kinetic pressure [Grady, Mech. Mater. 29, 181 (1998)] or a magnetic pressure [Lemke et al., Intl J. Impact Eng. 38, 480 (2011)] drives the motion of the flyer. Moreover, reliable prediction of the time-dependent pressure is often a critical component to understanding the physics of these experiments. Although VISAR can provide a precise measurement of a flyer's surface velocity, the real challenge of this diagnostic implementation is using this velocity to unfold the time-dependent pressure. The purpose of this paper is to elucidate a new method for quickly and reliably unfolding VISAR data. C1 [Hess, M.; Peterson, K.; Harvey-Thompson, A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Hess, M (reprint author), POB 5800,MS 1186, Albuquerque, NM 87185 USA. EM mhess@sandia.gov NR 19 TC 1 Z9 1 U1 0 U2 3 PU CAMBRIDGE UNIV PRESS PI CAMBRIDGE PA EDINBURGH BLDG, SHAFTESBURY RD, CB2 8RU CAMBRIDGE, ENGLAND SN 2095-4719 EI 2052-3289 J9 HIGH POWER LASER SCI JI High Power Laser Sci. Eng. PD AUG 18 PY 2015 VL 3 DI 10.1017/hpl.2015.23 PG 9 WC Optics SC Optics GA CQ0HO UT WOS:000360276300001 ER PT J AU Deng, LL Chen, XF Li, W Wang, Z Wong, YE Chat, TWD AF Deng, Liulin Chen, Xiangfeng Li, Wan Wang, Ze Wong, Yiling Elaine Chan, T. -W. Dominic TI Sensitivity and Robustness Enhancements by Using a V-Shape Ion Funnel in FTICR-MS SO ANALYTICAL CHEMISTRY LA English DT Article ID IONIZATION MASS-SPECTROMETRY; ELECTROSPRAY-IONIZATION; ATMOSPHERIC-PRESSURE; MOLECULAR-BEAMS; TRANSMISSION; INTERFACE; PROTEINS; IMPLEMENTATION; EVAPORATION; PRINCIPLES AB In this paper, a new configuration of the ion funnel interface (i.e., V-shape ion funnel (V-IF)) for high ion transmission efficiency and robustness enhancement was developed and implemented on FTICR-MS. The performance of the V-IF was compared with that of a home-built orthogonal ion funnel. An order of magnitude of improvement in sensitivity was achieved for various peptides and proteins. The performance of the instrument was maintained for a long period by neutral molecule removal. Other ion transmission patterns, such as gentle ion transmission, adduct ion removal, and radio frequency (RF)-driven collision induced dissociation (OD), was also realized in V-IF by varying the RF potentials. V-IF is believed to be a novel ion guide that has promising applications in mass spectrometry. C1 [Deng, Liulin; Chen, Xiangfeng; Li, Wan; Wang, Ze; Wong, Yiling Elaine; Chan, T. -W. Dominic] Chinese Univ Hong Kong, Dept Chem, Hong Kong, Hong Kong, Peoples R China. [Chen, Xiangfeng] Shandong Acad Sci, Jinan 250014, Shandong, Peoples R China. [Deng, Liulin] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Deng, Liulin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Chen, XF (reprint author), Chinese Univ Hong Kong, Dept Chem, Hong Kong, Hong Kong, Peoples R China. EM xiangfchensdas@163.com; twdchan@cuhk.edu.hk OI Chen, Xiangfeng/0000-0001-9266-7707 FU National Natural Science Foundation of China [NSFC 21205071]; Research Grant Council of the Hong Kong Special Administrative Region [2060351]; Natural Science Foundation of Shandong Province [ZR2012BQ009]; Funds for Fostering Distinguished Young Scholar of Shandong Academy of Sciences FX The authors would like to acknowledge the financial support from National Natural Science Foundation of China (NSFC 21205071), Research Grant Council of the Hong Kong Special Administrative Region (Research Grant Direct Allocation, ref. 2060351), Natural Science Foundation of Shandong Province (ZR2012BQ009), and Funds for Fostering Distinguished Young Scholar of Shandong Academy of Sciences. The authors thank the staff in the mechanical and electronic workshops of The Chinese University of Hong Kong. NR 32 TC 0 Z9 0 U1 2 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD AUG 18 PY 2015 VL 87 IS 16 BP 8073 EP 8077 DI 10.1021/acs.analchem.5b01828 PG 5 WC Chemistry, Analytical SC Chemistry GA CP4ZW UT WOS:000359892100008 PM 26218276 ER PT J AU Qiu, YH Yang, C Hinkle, P Vlassiouk, IV Siwy, ZS AF Qiu, Yinghua Yang, Crystal Hinkle, Preston Vlassiouk, Ivan V. Siwy, Zuzanna S. TI Anomalous Mobility of Highly Charged Particles in Pores SO ANALYTICAL CHEMISTRY LA English DT Article ID RESISTIVE-PULSE TECHNIQUE; ELECTROPHORETIC MOBILITY; SURFACE-CHARGE; COUNTERION CONDENSATION; COLLOIDAL PARTICLES; CYLINDRICAL PORE; ELECTROKINETIC PROPERTIES; INDIVIDUAL NANOPARTICLES; SUBMICRON PARTICLES; ION CONDENSATION AB Single micropores in resistive-pulse technique were used to understand a complex dependence of particle mobility on its surface charge density. We show that the mobility of highly charged carboxylated particles decreases with the increase of the solution pH due to an interplay of three effects: (i) ion condensation, (ii) formation of an asymmetric electrical double layer around the particle, and (iii) electroosmotic flow induced by the charges on the pore walls and the particle surfaces. The results are important for applying resistive-pulse technique to determine surface charge density and zeta potential of the particles. The experiments also indicate the presence of condensed ions, which contribute to the measured current if a sufficiently high electric field is applied across the pore. C1 [Qiu, Yinghua; Hinkle, Preston; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Yang, Crystal; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA. [Siwy, Zuzanna S.] Univ Calif Irvine, Dept Biomed Engn, Irvine, CA 92717 USA. [Qiu, Yinghua] Southeast Univ, Sch Mech Engn, Nanjing 211189, Jiangsu, Peoples R China. [Qiu, Yinghua] Southeast Univ, Jiangsu Key Lab Design & Mfg Micronano Biomed Ins, Nanjing 211189, Jiangsu, Peoples R China. [Vlassiouk, Ivan V.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Siwy, ZS (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. EM zsiwy@uci.edu RI Qiu, Yinghua/N-6497-2014; Vlassiouk, Ivan/F-9587-2010 OI Qiu, Yinghua/0000-0003-2489-0784; Vlassiouk, Ivan/0000-0002-5494-0386 FU National Science Foundation [CHE 1306058]; China Scholarship Council [CSC 201406090034] FX Irradiation with swift heavy ions was performed at the GSI Helmholtzzentrum fur Schwerionenforschung GmbH, Darmstadt, Germany. We very much appreciate helpful discussions with Prof. Salvador Mafe from the University of Valencia in Spain. This research was supported by the National Science Foundation (CHE 1306058). Y.Q, acknowledges financial support from the China Scholarship Council (CSC 201406090034). NR 48 TC 10 Z9 10 U1 3 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD AUG 18 PY 2015 VL 87 IS 16 BP 8517 EP 8523 DI 10.1021/acs.analchem.5b02060 PG 7 WC Chemistry, Analytical SC Chemistry GA CP4ZW UT WOS:000359892100069 PM 26177843 ER PT J AU Diallo, MS Baier, G Moyer, BA Hamelers, B AF Diallo, Mamadou S. Baier, Gretchen Moyer, Bruce A. Hamelers, Bert TI Critical Materials Recovery from Solutions and Wastes: Retrospective and Outlook SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Editorial Material C1 [Diallo, Mamadou S.] Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea. [Diallo, Mamadou S.] CALTECH, Environm Sci & Engn, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Baier, Gretchen] Dow Chem Co USA, Midland, MI 48674 USA. [Moyer, Bruce A.] Oak Ridge Natl Lab, Chem Separat Grp, Oak Ridge, TN 37831 USA. [Moyer, Bruce A.] Oak Ridge Natl Lab, Crit Mat Inst, Oak Ridge, TN 37831 USA. [Hamelers, Bert] European Ctr Excellence Sustainable Water Technol, Wetsus, NL-8900 CC Leeuwarden, Netherlands. RP Diallo, MS (reprint author), Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea. EM mdiallo@kaist.ac.kr RI Moyer, Bruce/L-2744-2016; Diallo, Mamadou/C-2075-2011 OI Moyer, Bruce/0000-0001-7484-6277; NR 0 TC 2 Z9 2 U1 2 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9387 EP 9389 DI 10.1021/acs.est.5b03694 PG 3 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700001 PM 26281889 ER PT J AU Kim, D Powell, LE Delmau, LH Peterson, ES Herchenroeder, J Bhave, RR AF Kim, Daejin Powell, Lawrence E. Delmau, Laetitia H. Peterson, Eric S. Herchenroeder, Jim Bhave, Ramesh R. TI Selective Extraction of Rare Earth Elements from Permanent Magnet Scraps with Membrane Solvent Extraction SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CHLORIDE MEDIA; CYANEX 923; RECOVERY; REMOVAL; WASTE; LANTHANIDES; ACID; ND AB The rare earth elements (REEs) such as neodymium, praseodymium, and dysprosium were successfully recovered from commercial NdFeB magnets and industrial scrap magnets via membrane assisted solvent extraction (MSX). A hollow fiber membrane system was evaluated to extract REEs in a single step with the feed and strip solutions circulating continuously through the MSX system. The effects of several experimental variables on REE extraction such as flow rate, concentration of REEs in the feed solution, membrane configuration, and composition of acids were investigated with the MSX system. A multimembrane module configuration with REEs dissolved in aqueous nitric acid solutions showed high selectivity for REE extraction with no coextraction of non-REEs, whereas the use of aqueous hydrochloric acid solution resulted in coextraction of non-REEs due to the formation of chloroanions of non-REEs. The REE oxides were recovered from the strip solution through precipitation, drying, and annealing steps. The resulting REE oxides were characterized with XRD, SEM-EDX, and ICP-OES, demonstrating that the membrane assisted solvent extraction is capable of selectively recovering pure REEs from the industrial scrap magnets. C1 [Kim, Daejin; Powell, Lawrence E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Delmau, Laetitia H.] Oak Ridge Natl Lab, Nucl Mat Proc Grp, Oak Ridge, TN 37831 USA. [Peterson, Eric S.] Idaho Natl Lab, Ctr Adv Energy Studies, Idaho Falls, ID 83415 USA. [Herchenroeder, Jim] Molycorp Magnequench, Greenwood Village, CO 80111 USA. EM bhaverr@ornl.gov RI Peterson, Eric/B-9127-2017 OI Peterson, Eric/0000-0002-2292-4939 FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office FX This research/work is supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. We thank Dr. Huseyin Ucar at ORNL for his assistance in XRD analysis. NR 30 TC 5 Z9 5 U1 7 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9452 EP 9459 DI 10.1021/acs.est.5b01306 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700008 PM 26107531 ER PT J AU Fujita, Y Barnes, J Eslamimanesh, A Lencka, MM Anderko, A Riman, RE Navrotsky, A AF Fujita, Yoshiko Barnes, Joni Eslamimanesh, Ali Lencka, Malgorzata M. Anderko, Andrzej Riman, Richard E. Navrotsky, Alexandra TI Effects of Simulated Rare Earth Recycling Wastewaters on Biological Nitrification SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NORMAL-BUTYL PHOSPHATE; SOLVENT ELECTROLYTE SYSTEMS; TRIBUTYL-PHOSPHATE; NITROSOMONAS-EUROPAEA; NITRIFYING BACTERIA; WASTE-WATER; PSEUDOMONAS-AERUGINOSA; LANTHANIDE ADSORPTION; MEMBRANE-PERMEABILITY; AQUEOUS-SOLUTIONS AB Increasing rare earth element (REE) supplies by recycling and expanded ore processing will result in generation of new wastewaters. In some cases, disposal to a sewage treatment plant may be favored, but plant performance must be maintained. To assess the potential effects of such wastewaters on biological treatment, model nitrifying organisms Nitrosomonas europaea and Nitrobacter winogradskyi were exposed to simulated wastewaters containing varying levels of yttrium or europium (10, 50, and 100 ppm), and the extractant tributyl phosphate (TBP, at 0.1 g/L). Y and Eu additions at 50 and 100 ppm inhibited N. europaea, even when virtually all of the REE was insoluble. Provision of TBP with Eu increased N. europaea inhibition, although TBP alone did not substantially alter activity. For N. winogradskyi cultures, Eu or Y additions at all tested levels induced significant inhibition, and nitrification shut down completely with TBP addition. REE solubility was calculated using the previously developed MSE (Mixed-Solvent Electrolyte) thermodynamic model. The model calculations reveal a strong pH dependence of solubility, typically controlled by the precipitation of REE hydroxides but also likely affected by the formation of unknown phosphate phases, which determined aqueous concentrations experienced by the microorganisms. C1 [Fujita, Yoshiko; Barnes, Joni] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Eslamimanesh, Ali; Lencka, Malgorzata M.; Anderko, Andrzej] OLI Syst Inc, Cedar Knolls, NJ 07927 USA. [Riman, Richard E.] Rutgers State Univ, Dept Mat Sci & Engn, Piscataway, NJ 08855 USA. [Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Navrotsky, Alexandra] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. RP Fujita, Y (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM yoshikolujita@inl.gov RI Fujita, Yoshiko/S-2007-2016; OI Fujita, Yoshiko/0000-0002-4472-4102; Anderko, Andrzej/0000-0002-1522-4889; Eslamimanesh, Ali/0000-0003-2555-4838 FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; DOE Idaho Operations Office [DE-AC07-05ID14517] FX We express our appreciation to D. LaCroix and J. Taylor at the University of Idaho/Center for Advanced Energy Studies for ICP-MS measurements. We also thank M. Greenhalgh of INL for advice regarding wastewater composition and for provision of the TBP and Isopar L. We also thank anonymous reviewers for their helpful comments. This research is supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. Funding was provided via the DOE Idaho Operations Office Contract DE-AC07-05ID14517. NR 64 TC 2 Z9 2 U1 10 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9460 EP 9468 DI 10.1021/acs.est.5b01753 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700009 PM 26132866 ER PT J AU Qu, YT Baumann, TF Santiago, JG Stadermann, M AF Qu, Yatian Baumann, Theodore F. Santiago, Juan G. Stadermann, Michael TI Characterization of Resistances of a Capacitive Deionization System SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID DOUBLE-LAYER CAPACITOR; CONSTANT PHASE ELEMENT; AL CURRENT-COLLECTOR; IMPEDANCE SPECTROSCOPY; ENERGY-CONSUMPTION; CARBON ELECTRODES; MEMBRANE; DESALINATION; ADSORPTION; SUPERCAPACITORS AB Capacitive deionization (CDI) is a promising desalination technology, which operates at low pressure, low temperature, requires little infrastructure, and has the potential to consume less energy for brackish water desalination. However, CDI devices consume significantly more energy than the theoretical thermodynamic minimum, and this is at least partly due to resistive power dissipation. We here report our efforts to characterize electric resistances in a CDI system, with a focus on the resistance associated with the contact between current collectors and porous electrodes. We present an equivalent circuit model to describe resistive components in a CDI cell. We propose measurable figures of merit to characterize cell resistance. We also show that contact pressure between porous electrodes and current collectors can significantly reduce contact resistance. Lastly, we propose and test an alternative electrical contact configuration which uses a pore-filling conductive adhesive (silver epoxy) and achieves significant reductions in contact resistance. C1 [Qu, Yatian; Santiago, Juan G.] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. [Qu, Yatian; Baumann, Theodore F.; Stadermann, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Santiago, JG (reprint author), Stanford Univ, Dept Mech Engn, 440 Escondido Mall, Stanford, CA 94305 USA. EM juan.santiago@stanford.edu; stadermann2@llnl.gov FU US DOE by LLNL [DE-AC52-07NA27344] FX Y.Q. would like to thank the Lawrence Scholar program. Work at LLNL was performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344. NR 44 TC 7 Z9 7 U1 22 U2 87 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9699 EP 9706 DI 10.1021/acs.est.5b02542 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700037 PM 26214554 ER PT J AU Zhang, HF Worton, DR Shen, S Nah, T Isaacman-VanWertz, G Wilson, KR Goldstein, AH AF Zhang, Haofei Worton, David R. Shen, Steve Nah, Theodora Isaacman-VanWertz, Gabriel Wilson, Kevin R. Goldstein, Allen H. TI Fundamental Time Scales Governing Organic Aerosol Multiphase Partitioning and Oxidative Aging SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID AIR-POLLUTION SOURCES; KINETIC MULTILAYER MODEL; HETEROGENEOUS OXIDATION; MOTOR-VEHICLES; MEXICO-CITY; GAS; EMISSIONS; PHASE; OH; SEMIVOLATILE AB Traditional descriptions of gas particle partitioning of organic aerosols (OA) rely solely on thermodynamic properties (e.g., volatility). Under realistic conditions where phase partitioning is dynamic rather than static, the transformation of OA involves the interplay of multiphase partitioning with oxidative aging. A key challenge remains in quantifying the fundamental time scales for evaporation and oxidation of semivolatile OA. In this paper, we use isomer-resolved product measurements of a series of normal-alkanes (C-18, C-20, C-22, and C-24) to distinguish between gas-phase and heterogeneous oxidation products formed by reaction with hydroxyl radicals (OH). The product isomer distributions when combined with kinetics measurements of evaporation and oxidation enable a quantitative description of the multiphase time scales to be simulated using a single-particle kinetic model. Multiphase partitioning and oxidative transformation of semivolatile normal-alkanes under laboratory conditions is largely controlled by the particle phase state, since the time scales of heterogeneous oxidation and evaporation are found to occur on competing time scales (on the order of 10(-1) h). This is in contrast to atmospheric conditions where heterogeneous oxidation time scales are expected to be much longer (on the order of 10(2) h), with gas-phase oxidation being the dominant process regardless of the evaporation kinetics. Our results demonstrate the dynamic nature of OA multiphase partitioning and oxidative aging and reveal that the fundamental time scales of these processes are crucial for reliably extending laboratory measurements of OA phase partitioning and aging to the atmosphere. C1 [Zhang, Haofei; Worton, David R.; Isaacman-VanWertz, Gabriel; Goldstein, Allen H.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Shen, Steve] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Nah, Theodora] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Goldstein, Allen H.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Zhang, Haofei; Nah, Theodora; Wilson, Kevin R.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Worton, David R.] Aerosol Dynam Inc, Berkeley, CA 94710 USA. RP Wilson, KR (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM krwilson@lbl.gov; ahg@berkeley.edu RI Worton, David/A-8374-2012 OI Worton, David/0000-0002-6558-5586 FU Camille & Henry Dreyfus Foundation; Laboratory-Directed Research and Development (LDRD) Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy, Office of Science FX This work was supported by the Camille & Henry Dreyfus Foundation and the Laboratory-Directed Research and Development (LDRD) Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract DE-AC02-05CH11231. K.R.W. is additionally supported by the Department of Energy, Office of Science Early Career Research Program. NR 44 TC 1 Z9 1 U1 8 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9768 EP 9777 DI 10.1021/acs.est.5b02115 PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700045 PM 26200667 ER PT J AU Waples, JT Bordewyk, JK Knesting, KM Orlandini, KA AF Waples, James T. Bordewyk, Jason K. Knesting, Kristina M. Orlandini, Kent A. TI Using Naturally Occurring Radionuclides To Determine Drinking Water Age in a Community Water System SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID TRACE INORGANIC CONTAMINANTS; U-234/U-238 ACTIVITY RATIOS; PIPE-SCALE DEPOSITS; RADIOACTIVITY; MODELS; TH-234; SR-90; TIME AB Drinking water quality in a community water system is closely linked to the age of water from initial treatment to time of delivery. However, water age is difficult to measure with conventional chemical tracers; particularly in stagnant water, where the relationship between disinfectant decay, microbial growth, and water age is poorly understood. Using radionuclides that were naturally present in source water, we found that measured activity ratios of Y-90/Sr-90 and Th-234/U-238 in discrete drinking water samples of known age accurately estimated water age up to 9 days old (sigma(est): +/- 3.8 h, P < 0.0001, r(2) = 0.998, n = 11) and 25 days old (sigma(est): +/- 13.3 h, P < 0.0001, r(2) = 0.996, n = 12), respectively. Moreover, 90Y-derived water ages in a community water system (6.8 x 10(4) m(3) d(-1) capacity) were generally consistent with water ages derived from an extended period simulation model. Radionuclides differ from conventional chemical tracers in that they are ubiquitous in distribution mains and connected premise plumbing. The ability to measure both water age and an analyte (e.g., chemical or microbe) in any water sample at any time allows for new insight into factors that control drinking water quality. C1 [Waples, James T.; Knesting, Kristina M.] Univ Wisconsin, Sch Freshwater Sci, 600 East Greenfield Ave, Milwaukee, WI 53204 USA. [Bordewyk, Jason K.] Stantec, St Paul, MN 55113 USA. [Orlandini, Kent A.] Argonne Natl Lab, Div Environm Res, Argonne, IL 60439 USA. RP Waples, JT (reprint author), Univ Wisconsin, Sch Freshwater Sci, 600 East Greenfield Ave, Milwaukee, WI 53204 USA. EM jwaples@uwm.edu FU National Science Foundation [OCE 0351824, BES 0630847]; NSF [OCE 0354031]; University of Wisconsin-Milwaukee School of Freshwater Sciences FX We thank D. Szmania, and K. Weckerly for sampling assistance, and V. Klump for assistance with gamma analysis. We are particularly grateful to R. Johnson and E. Kiefer for information and access to the NSWC treatment plant and distribution system. This research was supported by the National Science Foundation (OCE 0351824, BES 0630847), the NSF Research Experience for Undergraduates Program (OCE 0354031) and the University of Wisconsin-Milwaukee School of Freshwater Sciences. NR 43 TC 1 Z9 1 U1 3 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9850 EP 9857 DI 10.1021/acs.est.5b03227 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700054 PM 26200208 ER PT J AU Delaire, C van Genuchten, CM Nelson, KL Amrose, SE Gadgil, AJ AF Delaire, Caroline van Genuchten, Case M. Nelson, Kara L. Amrose, Susan E. Gadgil, Ashok J. TI Escherichia coli Attenuation by Fe Electrocoagulation in Synthetic Bengal Groundwater: Effect of pH and Natural Organic Matter SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID TUBEWELL WATER-QUALITY; IRON ELECTROCOAGULATION; ARSENIC REMOVAL; DRINKING-WATER; ENHANCED COAGULATION; BACTERIAL ADHESION; ZEROVALENT IRON; SURFACE-WATER; VIRUS REMOVAL; FERROUS ION AB Technologies addressing both arsenic and microbial contamination of Bengal groundwater are needed. Fe electrocoagulation (Fe-EC), a simple process relying on the dissolution of an Fe(0) anode to produce Fe(III) precipitates, has been shown to efficiently remove arsenic from groundwater at low cost. We investigated Escherichia con (E. coli) attenuation by Fe-EC in synthetic Bengal groundwater as a function of Fe dosage rate, total Fe dosed, pH, and presence of natural organic matter (NOM). A 2.5 mil4 Fe dosage simultaneously achieved over 4-log E. coli attenuation and arsenic removal from 450 to below 10 mu g/L. E. coli reduction was significantly enhanced at pH 6.6 compared to pH 7.5, which we linked to the decreased rate of Fe(II) oxidation at lower pH. 3 mg/L-C of NOM (Suwanee River fulvic acid) did not significantly affect E. coli attenuation. Live dead staining and comparisons of Fe-EC with chemical coagulation controls showed that the primary mechani sm of E. coli attenuation is physical removal with Fe(III) precipitates, with inactivation likely contributing as well at lower pH. Transmission electron microscopy showed that EC precipitates adhere to and bridge individual E. coli cells, resulting in large bacteria Fe aggregates that can be removed by gravitational settling. Our results point to the promising ability of Fe-EC to treat arsenic and bacterial contamination simultaneously at low cost. C1 [Delaire, Caroline; van Genuchten, Case M.; Nelson, Kara L.; Amrose, Susan E.; Gadgil, Ashok J.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Gadgil, Ashok J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. RP Delaire, C (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. EM caroline.delaire@orange.fr RI Foundry, Molecular/G-9968-2014 FU Development Impact Lab (USAID) part of the USAID Higher Education Solutions Network [AID-OAA-A-13-00002]; Andrew and Virginia Rudd Family Foundation; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Development Impact Lab (USAID Cooperative Agreement AID-OAA-A-13-00002), part of the USAID Higher Education Solutions Network, and by the Andrew and Virginia Rudd Family Foundation. This work would not have been possible without the generous assistance from David Sedlak, Andrew Torkelson, Andrea Silverman, Samantha Beardsley, Jannis Wenk, Denise Schichnes and Reena Zalpouri. We are grateful to James Britt Abrahamson for conducting zeta-potential measurements. We thank the CNR Biological Imaging Facility and the Electron Microscope Lab at UC Berkeley. Work at the Molecular Foundry (zeta-potential measurements) was supported by the Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 63 TC 3 Z9 3 U1 14 U2 63 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 9945 EP 9953 DI 10.1021/acs.est.5b01696 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700065 PM 26172118 ER PT J AU Deng, H Fitts, JP Crandall, D McIntyre, D Peters, CA AF Deng, Hang Fitts, Jeffrey P. Crandall, Dustin McIntyre, Dustin Peters, Catherine A. TI Alterations of Fractures in Carbonate Rocks by CO2-Acidified Brines SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CALCITE DISSOLUTION RATES; PORE-SCALE; LIMESTONE DISSOLUTION; REACTIVE TRANSPORT; CO2 SEQUESTRATION; SINGLE FRACTURE; ATM PCO(2); PERMEABILITY; FLOW; CAPROCK AB Fractures in geological formations may enable migration of environmentally relevant fluids, as in leakage of CO2 through caprocks in geologic carbon sequestration. We investigated geochemically induced alterations of fracture geometry in Indiana Limestone specimens. Experiments were the first of their kind, with periodic high-resolution imaging using X-ray computed tomography (xCT) scanning while maintaining high pore pressure (100 bar). We studied two CO2-acidified brines having the same pH (3.3) and comparable thermodynamic disequilibrium but different equilibrated pressures of CO2 (P-CO2 values of 12 and 77 bar). High-P-CO2 brine has a faster calcite dissolution kinetic rate because of the accelerating effect of carbonic acid. Contrary to expectations, dissolution extents were comparable in the two experiments. However, progressive xCT images revealed extensive channelization for high P-CO2, explained by strong positive feedback between ongoing flow and reaction. The pronounced channel increasingly directed flow to a small region of the fracture, which explains why the overall dissolution was lower than expected. Despite this, flow simulations revealed large increases in permeability in the high-P-CO2 experiment. This study shows that the permeability evolution of dissolving fractures will be larger for faster-reacting fluids. The overall mechanism is not because more rock dissolves, as would be commonly assumed, but because of accelerated fracture channelization. C1 [Deng, Hang; Fitts, Jeffrey P.; Peters, Catherine A.] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [Crandall, Dustin; McIntyre, Dustin] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Peters, CA (reprint author), Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. EM cap@princeton.edu RI Deng, Hang/E-5302-2015; OI Deng, Hang/0000-0001-5784-996X; Peters, Catherine/0000-0003-2418-795X FU National Science Foundation (NSF) [CBET-1133849] FX This research was funded by the National Science Foundation (NSF) grant CBET-1133849. H.D. acknowledges additional support by an appointment to the U.S. Department of Energy (DOE) Postgraduate Research Program at NETL administered by ORISE. We also acknowledge the use of the ICP-OES facility in Dr. Higgins' lab in the Department of Geosciences at Princeton University. Finally, we acknowledge the reviewers for their detailed and thorough assessments, which were extremely helpful in improving this manuscript. NR 68 TC 8 Z9 9 U1 5 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 18 PY 2015 VL 49 IS 16 BP 10226 EP 10234 DI 10.1021/acs.est.5b01980 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CP4ZS UT WOS:000359891700096 PM 26205851 ER PT J AU Piao, HL Hawley, E Kopf, S DeScenzo, R Sealock, S Henick-Kling, T Hess, M AF Piao, Hailan Hawley, Erik Kopf, Scott DeScenzo, Richard Sealock, Steven Henick-Kling, Thomas Hess, Matthias TI Insights into the bacterial community and its temporal succession during the fermentation of wine grapes SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE wine bacteria; wine fermentation; temporal succession; organic grape products; 16S rRNA gene profile; next-generation sequencing ID ACETIC-ACID BACTERIA; MICROBIAL COMMUNITIES; STARTER CULTURES; RED WINE; POPULATIONS; DIVERSITY; SPOILAGE; YEAST; BRUXELLENSIS; SEQUENCES AB Grapes harbor complex microbial communities. It is well known that yeasts, typically Saccharomyces cerevisiae, and bacteria, commonly the lactic acid fermenting Oenococcus oeni, work sequentially during primary and secondary wine fermentation. In addition to these main players, several microbes, often with undesirable effects on wine quality, have been found in grapes and during wine fermentation. However, still little is known about the dynamics of the microbial community during the fermentation process. In previous studies culture dependent methods were applied to detect and identify microbial organisms associated with grapes and grape products, which resulted in a picture that neglected the non-culturable fraction of the microbes. To obtain a more complete picture of how microbial communities change during grape fermentation and how different fermentation techniques might affect the microbial community composition, we employed next-generation sequencing (NGS) a culture-independent method. A better understanding of the microbial dynamics and their effect on the final product is of great importance to help winemakers produce wine styles of consistent and high quality. In this study, we focused on the bacterial community dynamics during wine vinification by amplifying and sequencing the hypervariable V1-V3 region of the 16S rRNA gene a phylogenetic marker gene that is ubiquitous within prokaryotes. Bacterial communities and their temporal succession was observed for communities associated with organically and conventionally produced wines. In addition, we analyzed the chemical characteristics of the grape musts during the organic and conventional fermentation process. These analyses revealed distinct bacterial population with specific temporal changes as well as different chemical profiles for the organically and conventionally produced wines. In summary these results suggest a possible correlation between the temporal succession of the bacterial population and the chemical wine profiles. C1 [Piao, Hailan; Henick-Kling, Thomas] Washington State Univ, Dept Viticulture & Enol, Richland, WA USA. [Hawley, Erik] ZeaChem Inc, Boardman, OR USA. [Kopf, Scott; Sealock, Steven] Pacific Rim Winemakers, West Richland, WA USA. [DeScenzo, Richard] ETS Labs, St Helena, CA USA. [Hess, Matthias] Univ Calif Davis, Dept Anim Sci, Funct Syst Microbiol Lab, Davis, CA 95616 USA. [Hess, Matthias] US DOE, Joint Genome Inst, Walnut Creek, CA USA. RP Hess, M (reprint author), Univ Calif Davis, Dept Anim Sci, Funct Syst Microbiol Lab, 2251 Meyer Hall,One Shields Ave, Davis, CA 95616 USA. EM mhess@ucdavis.edu NR 44 TC 6 Z9 6 U1 8 U2 58 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 18 PY 2015 VL 6 AR 809 DI 10.3389/fmicb.2015.00809 PG 12 WC Microbiology SC Microbiology GA CP6UM UT WOS:000360023700001 PM 26347718 ER PT J AU Smith-Moritz, AM Hao, Z Fernandez-Nino, SG Fangel, JU Verhertbruggen, Y Holman, HYN Willats, WGT Ronald, PC Scheller, HV Heazlewood, JL Vega-Sanchez, ME AF Smith-Moritz, Andreia M. Hao, Zhao Fernandez-Nino, Susana G. Fangel, Jonatan U. Verhertbruggen, Yves Holman, Hoi-Ying N. Willats, William G. T. Ronald, Pamela C. Scheller, Henrik V. Heazlewood, Joshua L. Vega-Sanchez, Miguel E. TI Structural characterization of a mixed-linkage glucan deficient mutant reveals alteration in cellulose microfibril orientation in rice coleoptile mesophyll cell walls SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE type II cell walls; cellulose; FT-MIR spectroscopy; mixed-linkage glucan; primary cell wall; rice ID PLANT-CELL; POLYSACCHARIDES; XYLOGLUCAN; SYNTHASE; ARABIDOPSIS; GRASSES; GROWTH; GENE; MICROSPECTROSCOPY; MICROTUBULES AB The CELLULOSE SYNTHASE-LIKE F6 (CslF6) gene was previously shown to mediate the biosynthesis of mixed-linkage glucan (MLG), a cell wall polysaccharide that is hypothesized to be tightly associated with cellulose and also have a role in cell expansion in the primary cell wall of young seedlings in grass species. We have recently shown that loss-of-function cslf6 rice mutants do not accumulate MLG in most vegetative tissues. Despite the absence of a structurally important polymer, MLG, these mutants are unexpectedly viable and only show a moderate growth compromise compared to wild type. Therefore these mutants are ideal biological systems to test the current grass cell wall model. In order to gain a better understanding of the role of MLG in the primary wall, we performed in-depth compositional and structural analyses of the cell walls of 3 day-old rice seedlings using various biochemical and novel microspectroscopic approaches. We found that cellulose content as well as matrix polysaccharide composition was not significantly altered in the MLG deficient mutant. However, we observed a significant change in cellulose microfibril bundle organization in mesophyll cell walls of the cslf6 mutant. Using synchrotron source Fourier Transform Mid-Infrared (FTM-IR) Spectromicroscopy for high-resolution imaging, we determined that the bonds associated with cellulose and arabinoxylan, another major component of the primary cell walls of grasses, were in a lower energy configuration compared to wild type, suggesting a slightly weaker primary wall in MLG deficient mesophyll cells. Taken together, these results suggest that MLG may influence cellulose deposition in mesophyll cell walls without significantly affecting anisotropic growth thus challenging MLG importance in cell wall expansion. C1 [Smith-Moritz, Andreia M.; Fernandez-Nino, Susana G.; Verhertbruggen, Yves; Ronald, Pamela C.; Scheller, Henrik V.; Heazlewood, Joshua L.; Vega-Sanchez, Miguel E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Hao, Zhao; Holman, Hoi-Ying N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Synchrotron Infrared Struct Biol Program, Berkeley, CA 94720 USA. [Fangel, Jonatan U.; Willats, William G. T.] Univ Copenhagen, Dept Plant & Environm Sci, Copenhagen, Denmark. [Ronald, Pamela C.] Univ Calif Davis, UC Davis Genome Ctr, Dept Plant Pathol, Davis, CA 95616 USA. RP Ronald, PC (reprint author), Univ Calif Davis, UC Davis Genome Ctr, Dept Plant Pathol, One Shield Ave, Davis, CA 95616 USA. EM pcronald@ucdavis.edu; mevega-sanchez@lbl.gov RI Heazlewood, Joshua/A-2554-2008; Hao, Zhao/G-2391-2015; Holman, Hoi-Ying/N-8451-2014; Scheller, Henrik/A-8106-2008; OI Heazlewood, Joshua/0000-0002-2080-3826; Hao, Zhao/0000-0003-0677-8529; Holman, Hoi-Ying/0000-0002-7534-2625; Scheller, Henrik/0000-0002-6702-3560; Verhertbruggen, Yves/0000-0003-4114-5428 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science and Office of Biological and Environmental Research [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Jeemeng Lao for technical assistance with the HPAEC analysis. This work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The synchrotron mid-infrared spectromicroscopy and associated imaging work were performed at Infrared Beamline 1.4 and 5.4 under the Berkeley Synchrotron Infrared Structural Biology (BSISB) Program funded by the U.S. Department of Energy, Office of Science and Office of Biological and Environmental Research through contracts DE-AC02-05CH11231. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 2 Z9 2 U1 4 U2 25 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD AUG 18 PY 2015 VL 6 AR 628 DI 10.3389/fpls.2015.00628 PG 13 WC Plant Sciences SC Plant Sciences GA CP5JK UT WOS:000359917200001 PM 26347754 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Henry, S Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. Datta, M. de Barbaro, P. Demortier, L. Deninno, M. D'Errico, M. Devoto, F. Di Canto, A. Di Ruzza, B. Dittmann, J. R. Donati, S. D'Onofrio, M. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Elagin, A. Erbacher, R. Errede, S. Esham, B. Farrington, S. Fernandez Ramos, J. P. Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Galloni, C. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Gonzalez Lopez, O. Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Henry, S. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, W. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. H. Kim, S. B. Kim, Y. J. Kim, Y. K. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, H. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Lucchesi, D. Luca, A. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. 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Simonenko, A. Sliwa, K. Smith, J. R. Snider, F. D. Song, H. Sorin, V. Denis, R. St. Stancari, M. Stentz, D. Strologas, J. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thomson, E. Thukral, V. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Ukegawa, F. Uozumi, S. Vazquez, F. Velev, G. Vellidis, C. Vernieri, C. Vidal, M. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Wagner, P. Wallny, R. Wang, S. M. Waters, D. Wester, W. C., III Whiteson, D. Wicklund, A. B. Wilbur, S. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamato, D. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Zanetti, A. M. Zeng, Y. Zhou, C. Zucchelli, S. CA CDf Collaboration TI First measurement of the forward-backward asymmetry in bottom-quark pair production at high mass SO PHYSICAL REVIEW D LA English DT Article AB We measure the particle-level forward-backward production asymmetry in b (b) over bar pairs with masses (m(b (b) over bar)) larger than 150 GeV/c(2), using events with hadronic jets and employing jet charge to distinguish b from (b) over bar. The measurement uses 9.5 fb(-1) of p (p) over bar collisions at a center-of-mass energy of 1.96 TeV recorded by the CDF II detector. The asymmetry as a function of m(b (b) over bar) is consistent with zero, as well as with the predictions of the standard model. The measurement disfavors a simple model including an axigluon with a mass of 200 GeV/c(2), whereas a model containing a heavier 345 GeV/c(2) axigluon is not excluded. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. 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RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Paulini, Manfred/N-7794-2014; OI Marino, Pietro/0000-0003-0554-3066; Simonenko, Alexander/0000-0001-6580-3638; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; Casarsa, Massimo/0000-0002-1353-8964; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Paulini, Manfred/0000-0002-6714-5787; iori, maurizio/0000-0002-6349-0380; Devoto, Francesco/0000-0002-3415-7677; Margaroli, Fabrizio/0000-0002-3869-0153; Latino, Giuseppe/0000-0002-4098-3502; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756 FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Korean World Class University Program, the National Research Foundation of Korea; Science and Technology Facilities Council and the Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Australian Research Council; Bundesministerium fur Bildung und Forschung, Germany; Academy of Finland; EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, United Kingdom; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council; and the EU community Marie Curie Fellowship Contract No. 302103. NR 26 TC 3 Z9 3 U1 2 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 18 PY 2015 VL 92 IS 3 AR 032006 DI 10.1103/PhysRevD.92.032006 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CP4PX UT WOS:000359865700002 ER PT J AU Agrawal, A Perahia, D Grest, GS AF Agrawal, Anupriya Perahia, Dvora Grest, Gary S. TI Clustering effects in ionic polymers: Molecular dynamics simulations SO PHYSICAL REVIEW E LA English DT Article ID SULFONATED POLYSTYRENE IONOMERS; RAY-SCATTERING DATA; VISCOELASTIC BEHAVIOR; MODEL; MORPHOLOGY; MULTIPLETS; ENERGY; WATER AB Ionic clusters control the structure, dynamics, and transport in soft matter. Incorporating a small fraction of ionizable groups in polymers substantially reduces the mobility of the macromolecules in melts. These ionic groups often associate into random clusters in melts, where the distribution and morphology of the clusters impact the transport in these materials. Here, using molecular dynamic simulations we demonstrate a clear correlation between cluster size and morphology with the polymer mobility in melts of sulfonated polystyrene. We show that in low dielectric media ladderlike clusters that are lower in energy compared with spherical assemblies are formed. Reducing the electrostatic interactions by enhancing the dielectric constant leads to morphological transformation from ladderlike clusters to globular assemblies. Decrease in electrostatic interaction significantly enhances the mobility of the polymer. C1 [Agrawal, Anupriya; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Agrawal, A (reprint author), Washington Univ, Dept Mech Engn & Mat Sci, St Louis, MO 63130 USA. FU Office of Science of the United States Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; [DE-SC007908] FX We gratefully acknowledge financial support from Grant No. DE-SC007908. We acknowledge computational resources at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the United States Department of Energy, under Contract No. DE-AC02-05CH11231 and Clemson Computing and Information Technology. This work was performed, in part, at the Center for Integrated Nanotechnology, a U.S. Department of Energy and Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 40 TC 4 Z9 4 U1 13 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD AUG 18 PY 2015 VL 92 IS 2 AR 022601 DI 10.1103/PhysRevE.92.022601 PG 6 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CP4QV UT WOS:000359868300002 PM 26382420 ER PT J AU Bousso, R Engelhardt, N AF Bousso, Raphael Engelhardt, Netta TI New Area Law in General Relativity SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTICLE CREATION; BLACK-HOLES; HORIZONS AB We report a new area law in general relativity. A future holographic screen is a hypersurface foliated by marginally trapped surfaces. We show that their area increases monotonically along the foliation. Future holographic screens can easily be found in collapsing stars and near a big crunch. Past holographic screens exist in any expanding universe and obey a similar theorem, yielding the first rigorous area law in big bang cosmology. Unlike event horizons, these objects can be identified at finite time and without reference to an asymptotic boundary. The Bousso bound is not used, but it naturally suggests a thermodynamic interpretation of our result. C1 [Bousso, Raphael] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Engelhardt, Netta] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP Bousso, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM bousso@lbl.gov; engeln@physics.ucsb.edu FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644, 1316783]; fqxi Grant [RFP3-1323]; U.S. Department of Energy [DE-AC02-05CH11231]; U.S. NSF [DGE-1144085]; NSF [PHY12-05500] FX It is a pleasure to thank M. Aganagic, D. Engelhardt, S. Fischetti, D. Harlow, G. Horowitz, W. Kelly, S. Leichenauer, T. Jacobson, D. Marolf, M. Moosa, R. Wald, and A. Wall for discussions and correspondence. The work of R. B. is supported in part by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Grants No. 1214644 and No. 1316783), by fqxi Grant No. RFP3-1323, and by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work of N. E. is supported in part by the U.S. NSF Graduate Research Fellowship under Grant No. DGE-1144085 and by NSF Grant No. PHY12-05500. NR 21 TC 14 Z9 14 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 18 PY 2015 VL 115 IS 8 AR 081301 DI 10.1103/PhysRevLett.115.081301 PG 5 WC Physics, Multidisciplinary SC Physics GA CP4SG UT WOS:000359872300003 PM 26340179 ER PT J AU Wang, X Chai, YS Zhou, L Cao, HB Cruz, CD Yang, JY Dai, JH Yin, YY Yuan, Z Zhang, SJ Yu, RZ Azuma, M Shimakawa, Y Zhang, HM Dong, S Sun, Y Jin, CQ Long, YW AF Wang, Xiao Chai, Yisheng Zhou, Long Cao, Huibo Cruz, Clarina-dela Yang, Junye Dai, Jianhong Yin, Yunyu Yuan, Zhen Zhang, Sijia Yu, Runze Azuma, Masaki Shimakawa, Yuichi Zhang, Huimin Dong, Shuai Sun, Young Jin, Changqing Long, Youwen TI Observation of Magnetoelectric Multiferroicity in a Cubic Perovskite System: LaMn3Cr4O12 SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHARGE; FERROELECTRICITY; POLARIZATION; PROGRESS AB Magnetoelectric multiferroicity is not expected to occur in a cubic perovskite system because of the high structural symmetry. By versatile measurements in magnetization, dielectric constant, electric polarization, neutron and x-ray diffraction, Raman scattering, as well as theoretical calculations, we reveal that the A-site ordered perovskite LaMn3Cr4O12 with cubic symmetry is a novel spin-driven multiferroic system with strong magnetoelectric coupling effects. When a magnetic field is applied in parallel (perpendicular) to an electric field, the ferroelectric polarization can be enhanced (suppressed) significantly. The unique multiferroic phenomenon observed in this cubic perovskite cannot be understood by conventional spin-driven microscopic mechanisms. Instead, a nontrivial effect involving the interactions between two magnetic sublattices is likely to play a crucial role. C1 [Wang, Xiao; Chai, Yisheng; Zhou, Long; Yang, Junye; Dai, Jianhong; Yin, Yunyu; Yuan, Zhen; Zhang, Sijia; Sun, Young; Jin, Changqing; Long, Youwen] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. [Wang, Xiao; Jin, Changqing; Long, Youwen] Collaborat Innovat Ctr Quantum Matter, Beijing 100190, Peoples R China. [Cao, Huibo; Cruz, Clarina-dela] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Neutron Scattering Sci Directorate, Oak Ridge, TN 37831 USA. [Yu, Runze; Azuma, Masaki] Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, Yokohama, Kanagawa 2268503, Japan. [Shimakawa, Yuichi] Kyoto Univ, Inst Chem Res, Uji, Kyoto 6110011, Japan. [Zhang, Huimin; Dong, Shuai] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. RP Long, YW (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. EM youngsun@iphy.ac.cn; ywlong@iphy.ac.cn RI chai, Yisheng/A-8402-2011; Dong (董), Shuai (帅)/A-5513-2008; Cao, Huibo/A-6835-2016; Long, Youwen/B-2930-2011; Sun, Young/A-7772-2013 OI chai, Yisheng/0000-0003-0034-7488; Dong (董), Shuai (帅)/0000-0002-6910-6319; Cao, Huibo/0000-0002-5970-4980; Sun, Young/0000-0001-8879-3508 FU 973 Project of the Ministry of Science and Technology of China [2014CB92 1500]; Strategic Priority Research Program of the Chinese Academy of Sciences [XDB070 30300, XDB07030200]; NSFC [11374 347, 11227405, 51322206]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX We thank H. J. Xiang for useful discussion. This work was partially supported by the 973 Project of the Ministry of Science and Technology of China (Grant No. 2014CB92 1500), the Strategic Priority Research Program of the Chinese Academy of Sciences (Grants No. XDB070 30300 and No. XDB07030200). Y. C., Y. Sun, H. Z., and S. D. were supported by the NSFC (Grants No. 11374 347, No. 11227405, and No. 51322206). Research conducted at the ORNL High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. X. W., Y. C., and L. Z. contributed equally to this work. NR 48 TC 17 Z9 17 U1 20 U2 106 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 18 PY 2015 VL 115 IS 8 AR 087601 DI 10.1103/PhysRevLett.115.087601 PG 5 WC Physics, Multidisciplinary SC Physics GA CP4SG UT WOS:000359872300004 PM 26340207 ER PT J AU Donatelli, JJ Zwart, PH Sethian, JA AF Donatelli, Jeffrey J. Zwart, Peter H. Sethian, James A. TI Iterative phasing for fluctuation X-ray scattering SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE fluctuation scattering; iterative phasing; polar Fourier transform ID FOURIER-TRANSFORM; RECONSTRUCTION; PARTICLES; SAXS AB Fluctuation X-ray scattering (FXS) is an extension of small-and wide-angle X-ray scattering in which the X-ray snapshots are taken below rotational diffusion times. This technique, performed using a free electron laser or ultrabright synchrotron source, provides significantly more experimental information compared with traditional solution scattering methods. We develop a multitiered iterative phasing algorithm to determine the underlying structure of the scattering object from FXS data. C1 [Donatelli, Jeffrey J.; Sethian, James A.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Donatelli, Jeffrey J.; Sethian, James A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. [Zwart, Peter H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Sethian, JA (reprint author), Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. EM sethian@math.berkeley.edu FU Applied Mathematical Sciences subprogram of the Office of Energy Research, US Department of Energy [DE-AC02-05CH11231]; Division of Mathematical Sciences of the National Science Foundation; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; National Institute of General Medical Sciences of the National Institutes of Health [R01GM109019] FX This research was supported in part by the Applied Mathematical Sciences subprogram of the Office of Energy Research, US Department of Energy, under Contract DE-AC02-05CH11231 and by the Division of Mathematical Sciences of the National Science Foundation and used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract DE-AC02-05CH11231. J.A.S. was also supported by an Einstein Visiting Fellowship of the Einstein Foundation, Berlin. Further support originates from the National Institute of General Medical Sciences of the National Institutes of Health under Award R01GM109019. The content of this article is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. NR 27 TC 9 Z9 10 U1 1 U2 17 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10286 EP 10291 DI 10.1073/pnas.1513738112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300054 PM 26240348 ER PT J AU You, L Lee, O Bhowmik, D Labanowski, D Hong, J Bokor, J Salahuddin, S AF You, Long Lee, OukJae Bhowmik, Debanjan Labanowski, Dominic Hong, Jeongmin Bokor, Jeffrey Salahuddin, Sayeef TI Switching of perpendicularly polarized nanomagnets with spin orbit torque without an external magnetic field by engineering a tilted anisotropy SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE spin orbit torque; perpendicular anisotropy; nanomagnets ID DOMAIN-WALLS; MGO AB Spin orbit torque (SOT) provides an efficient way to significantly reduce the current required for switching nanomagnets. However, SOT generated by an in-plane current cannot deterministically switch a perpendicularly polarized magnet due to symmetry reasons. On the other hand, perpendicularly polarized magnets are preferred over in-plane magnets for high-density data storage applications due to their significantly larger thermal stability in ultrascaled dimensions. Here, we show that it is possible to switch a perpendicularly polarized magnet by SOT without needing an external magnetic field. This is accomplished by engineering an anisotropy in the magnets such that the magnetic easy axis slightly tilts away from the direction, normal to the film plane. Such a tilted anisotropy breaks the symmetry of the problem and makes it possible to switch the magnet deterministically. Using a simple Ta/CoFeB/MgO/Ta heterostructure, we demonstrate reversible switching of the magnetization by reversing the polarity of the applied current. This demonstration presents a previously unidentified approach for controlling nanomagnets with SOT. C1 [You, Long; Lee, OukJae; Bhowmik, Debanjan; Labanowski, Dominic; Hong, Jeongmin; Bokor, Jeffrey; Salahuddin, Sayeef] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Salahuddin, Sayeef] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Salahuddin, S (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM sayeef@berkeley.edu FU Intel Fellowship; US Department of Energy Office of Basic Energy Sciences; National Science Foundation E3S Center; Semiconductor Technology Advanced Research Network Function Accelerated Nanomaterial Engineering Center FX This work was supported in part by the US Department of Energy Office of Basic Energy Sciences, National Science Foundation E3S Center, Semiconductor Technology Advanced Research Network Function Accelerated Nanomaterial Engineering Center. D.B. acknowledges support from an Intel Fellowship. NR 21 TC 10 Z9 11 U1 8 U2 49 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10310 EP 10315 DI 10.1073/pnas.1507474112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300058 PM 26240358 ER PT J AU Zaliznyak, I Savici, AT Lumsden, M Tsvelik, A Hu, RW Petrovic, C AF Zaliznyak, Igor Savici, Andrei T. Lumsden, Mark Tsvelik, Alexei Hu, Rongwei Petrovic, Cedomir TI Spin-liquid polymorphism in a correlated electron system on the threshold of superconductivity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE spin liquid; magnetism; superconductivity; neutron scattering; polymorphism ID RESOLUTION FUNCTION; WATER; EXCITATIONS; STATE; SCATTERING AB We report neutron scattering measurements which reveal spin-liquid polymorphism in an "11" iron chalcogenide superconductor. It occurs when a poorly metallic magnetic state of FeTe is tuned toward superconductivity by substitution of a small amount of tellurium with iso-electronic sulfur. We observe a liquid-like magnetic response, which is described by the coexistence of two disordered magnetic phases with different local structures whose relative abundance depends on temperature. One is the ferromagnetic (FM) plaquette phase observed in undoped, nonsuperconducting FeTe, which preserves the C-4 symmetry of the underlying square lattice and is favored at high temperatures, whereas the other is the antiferromagnetic plaquette phase with broken C-4 symmetry, which emerges with doping and is predominant at low temperatures. These findings suggest the coexistence of and competition between two distinct liquid states, and a liquid-liquid phase transformation between these states, in the electronic spin system of FeTe1-x(S,Se)(x). We have thus discovered the remarkable physics of competing spin-liquid polymorphs in a correlated electron system approaching superconductivity. Our results facilitate an understanding of large swaths of recent experimental data in unconventional superconductors. In particular, the phase with lower C-2 local symmetry, whose emergence precedes superconductivity, naturally accounts for a propensity for forming electronic nematic states which have been observed experimentally, in cuprate and iron-based superconductors alike. C1 [Zaliznyak, Igor; Tsvelik, Alexei; Hu, Rongwei; Petrovic, Cedomir] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Savici, Andrei T.; Lumsden, Mark] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Zaliznyak, I (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM zaliznyak@bnl.gov RI Savici, Andrei/F-2790-2013; Lumsden, Mark/F-5366-2012 OI Savici, Andrei/0000-0001-5127-8967; Lumsden, Mark/0000-0002-5472-9660 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy (DOE) [DE-SC00112704]; Center for Emergent Superconductivity, an Energy Frontier Research Center - US DOE, Office for Basic Energy Science; Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE FX We acknowledge discussions with J. Tranquada, W. Ku, G. Xu, and B. Ocko. Work at Brookhaven National Laboratory was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy (DOE) under Contract DE-SC00112704 and in part by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office for Basic Energy Science (R.H. and C.P.). Research conducted at Oak Ridge National Laboratory's High Flux Isotope Reactor and Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE. NR 44 TC 4 Z9 4 U1 2 U2 31 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10316 EP 10320 DI 10.1073/pnas.1503559112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300059 PM 26240327 ER PT J AU Allred, BE Rupert, PB Gauny, SS An, DD Ralston, CY Sturzbecher-Hoehne, M Strong, RK Abergel, RJ AF Allred, Benjamin E. Rupert, Peter B. Gauny, Stacey S. An, Dahlia D. Ralston, Corie Y. Sturzbecher-Hoehne, Manuel Strong, Roland K. Abergel, Rebecca J. TI Siderocalin-mediated recognition, sensitization, and cellular uptake of actinides SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE actinide transport; siderocalin; protein crystallography; luminescence spectroscopy; antenna effect ID DECORPORATION AGENTS; IRON ACQUISITION; IMMUNE-SYSTEM; PROTEIN; PLUTONIUM; BINDING; CARBOXYMYCOBACTINS; SIDEROPHORE; TRANSFERRIN; COMPLEX AB Synthetic radionuclides, such as the transuranic actinides plutonium, americium, and curium, present severe health threats as contaminants, and understanding the scope of the biochemical interactions involved in actinide transport is instrumental in managing human contamination. Here we show that siderocalin, a mammalian siderophore-binding protein from the lipocalin family, specifically binds lanthanide and actinide complexes through molecular recognition of the ligands chelating the metal ions. Using crystallography, we structurally characterized the resulting siderocalin-transuranic actinide complexes, providing unprecedented insights into the biological coordination of heavy radioelements. In controlled in vitro assays, we found that intracellular plutonium uptake can occur through siderocalin-mediated endocytosis. We also demonstrated that siderocalin can act as a synergistic antenna to sensitize the luminescence of trivalent lanthanide and actinide ions in ternary protein-ligand complexes, dramatically increasing the brightness and efficiency of intramolecular energy transfer processes that give rise to metal luminescence. Our results identify siderocalin as a potential player in the biological trafficking of f elements, but through a secondary ligand-based metal sequestration mechanism. Beyond elucidating contamination pathways, this work is a starting point for the design of two-stage biomimetic platforms for photoluminescence, separation, and transport applications. C1 [Allred, Benjamin E.; Gauny, Stacey S.; An, Dahlia D.; Sturzbecher-Hoehne, Manuel; Abergel, Rebecca J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Rupert, Peter B.; Strong, Roland K.] Fred Hutchinson Canc Res Ctr, Div Basic Sci, Seattle, WA 98109 USA. [Ralston, Corie Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. RP Abergel, RJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM rjabergel@lbl.gov FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231]; National Institutes of Health [R01DK073462]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Marc Allaire, Simon Morton, Jeffrey Bramble, and Israel Tadesse for assistance in planning and implementing diffraction data collection on radioactive crystals at the ALS 5.0.2 beamline. We thank Anthony D'Aleo for luminescence spectroscopy discussions and Kenneth Raymond for providing us with purified Ent. This work was funded by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy under Contract DE-AC02-05CH11231 (to R.J.A.), and by the National Institutes of Health under Award R01DK073462 (subcontract to R.K.S.). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 41 TC 8 Z9 8 U1 5 U2 31 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10342 EP 10347 DI 10.1073/pnas.1508902112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300064 PM 26240330 ER PT J AU Velarde, MC Demaria, M Melov, S Campisi, J AF Velarde, Michael C. Demaria, Marco Melov, Simon Campisi, Judith TI Pleiotropic age-dependent effects of mitochondrial dysfunction on epidermal stem cells SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE cellular senescence; oxidative stress; skin aging; stem cell proliferation; superoxide dismutase 2 ID MANGANESE SUPEROXIDE-DISMUTASE; OXIDATIVE STRESS; LIFE-SPAN; CELLULAR SENESCENCE; HAIR FOLLICLE; KERATINOCYTE DIFFERENTIATION; MOUSE EPIDERMIS; MUTANT MICE; IN-VIVO; SKIN AB Tissue homeostasis declines with age partly because stem/progenitor cells fail to self-renew or differentiate. Because mitochondrial damage can accelerate aging, we tested the hypothesis that mitochondrial dysfunction impairs stem cell renewal or function. We developed a mouse model, Tg(KRT14-cre/Esr1)(20Efu/J) x Sod2(tm1Smel), that generates mitochondrial oxidative stress in keratin 14-expressing epidermal stem/progenitor cells in a temporally controlled manner owing to deletion of Sod2, a nuclear gene that encodes the mitochondrial antioxidant enzyme superoxide dismutase 2 (Sod2). Epidermal Sod2 loss induced cellular senescence, which irreversibly arrested proliferation in a fraction of keratinocytes. Surprisingly, in young mice, Sod2 deficiency accelerated wound closure, increasing epidermal differentiation and reepithelialization, despite the reduced proliferation. In contrast, at older ages, Sod2 deficiency delayed wound closure and reduced epidermal thickness, accompanied by epidermal stem cell exhaustion. In young mice, Sod2 deficiency accelerated epidermal thinning in response to the tumor promoter 12-O-tetradecanoylphorbol-13-acetate, phenocopying the reduced regeneration of older Sod2-deficient skin. Our results show a surprising beneficial effect of mitochondrial dysfunction at young ages, provide a potential mechanism for the decline in epidermal regeneration at older ages, and identify a previously unidentified age-dependent role for mitochondria in skin quality and wound closure. C1 [Velarde, Michael C.; Demaria, Marco; Melov, Simon; Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Campisi, J (reprint author), Buck Inst Res Aging, Novato, CA 94945 USA. EM jcampisi@buckinstitute.org OI Demaria, Marco/0000-0002-8429-4813 FU National Institutes of Health [AG009909, AG18679, AG025901, AG041221] FX We thank the Buck Morphology Core for processing tissues, San Francisco VA Medical Center's Flow Cytomtery Core for flow cytometry, Ethan Sarnoski and Isaac Daviet for help with immunostaining, Nuno Luis for instruction on processing whole mounts, Kevin Perrott and Elvira Rafikova for blind ranking of activity staining, Sally D. Pennypacker for instruction on separating epidermis from dermis, and Leila Mashouf for measuring epidermal thickness. We especially thank Pierre-Yves Desprez for critically reading the manuscript. This work was funded by National Institutes of Health Grants AG009909 (to J.C.), AG18679 (to S.M.), AG025901 (to S.M. and J.C.), and AG041221 (to M.C.V.). NR 53 TC 9 Z9 9 U1 1 U2 3 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10407 EP 10412 DI 10.1073/pnas.1505675112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300075 PM 26240345 ER PT J AU Schumann, K Lin, S Boyer, E Simeonov, DR Subramaniam, M Gate, RE Haliburton, GE Yee, CJ Bluestone, JA Doudna, JA Marson, A AF Schumann, Kathrin Lin, Steven Boyer, Eric Simeonov, Dimitre R. Subramaniam, Meena Gate, Rachel E. Haliburton, Genevieve E. Yee, Chun J. Bluestone, Jeffrey A. Doudna, Jennifer A. Marson, Alexander TI Generation of knock-in primary human T cells using Cas9 ribonucleoproteins SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE CRISPR/Cas9; genome engineering; Cas9 ribonucleoprotein; RNP; primary human T cells ID ADOPTIVE IMMUNOTHERAPY; HEMATOPOIETIC STEM; RECEPTOR; CANCER; CCR5; HIV; 7-TRANSMEMBRANE; THERAPY; TUMORS; CXCR4 AB T-cell genome engineering holds great promise for cell-based therapies for cancer, HIV, primary immune deficiencies, and autoimmune diseases, but genetic manipulation of human T cells has been challenging. Improved tools are needed to efficiently "knock out" genes and "knock in" targeted genome modifications to modulate T-cell function and correct disease-associated mutations. CRISPR/Cas9 technology is facilitating genome engineering in many cell types, but in human T cells its efficiency has been limited and it has not yet proven useful for targeted nucleotide replacements. Here we report efficient genome engineering in human CD4(+) T cells using Cas9:single-guide RNA ribonucleoproteins (Cas9 RNPs). Cas9 RNPs allowed ablation of CXCR4, a coreceptor for HIV entry. Cas9 RNP electroporation caused up to similar to 40% of cells to lose high-level cell-surface expression of CXCR4, and edited cells could be enriched by sorting based on low CXCR4 expression. Importantly, Cas9 RNPs paired with homology-directed repair template oligonucleotides generated a high frequency of targeted genome modifications in primary T cells. Targeted nucleotide replacement was achieved in CXCR4 and PD-1 (PDCD1), a regulator of T-cell exhaustion that is a validated target for tumor immunotherapy. Deep sequencing of a target site confirmed that Cas9 RNPs generated knock-in genome modifications with up to similar to 20% efficiency, which accounted for up to approximately one-third of total editing events. These results establish Cas9 RNP technology for diverse experimental and therapeutic genome engineering applications in primary human T cells. C1 [Schumann, Kathrin; Boyer, Eric; Simeonov, Dimitre R.; Haliburton, Genevieve E.; Bluestone, Jeffrey A.; Marson, Alexander] Univ Calif San Francisco, Ctr Diabet, San Francisco, CA 94143 USA. [Schumann, Kathrin; Boyer, Eric; Simeonov, Dimitre R.; Haliburton, Genevieve E.; Marson, Alexander] Univ Calif San Francisco, Dept Med, Div Infect Dis, San Francisco, CA 94143 USA. [Lin, Steven; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Simeonov, Dimitre R.] Univ Calif San Francisco, Biomed Sci Grad Program, San Francisco, CA 94143 USA. [Subramaniam, Meena; Gate, Rachel E.; Yee, Chun J.] Univ Calif San Francisco, Inst Human Genet, Dept Epidemiol & Biostat, Dept Bioengn & Therapeut Sci, San Francisco, CA 94143 USA. [Subramaniam, Meena; Gate, Rachel E.] Univ Calif San Francisco, Biol & Med Informat Grad Program, San Francisco, CA 94158 USA. [Doudna, Jennifer A.; Marson, Alexander] Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM doudna@berkeley.edu; alexander.marson@ucsf.edu FU UCSF Sandler Fellowship; NIH funding for the HIV Accessory & Regulatory Complexes Center [P50GM082250]; National MS Society Collaborative MS Research Center Award; Howard Hughes Medical Institute (HHMI); NIH [T32 DK741834] FX We thank Mary Rieck, Jacqueline Howells, Amy Putnam, and Caroline Raffin in the J.A.B. laboratory; Richard Lao and the University of California at San Francisco (UCSF) Institute for Human Genetics Genomics Core; Michael Lee, Vinh Nguyen, and the UCSF Flow Cytometry Core; Amy Lee in the Cate laboratory; all members of the A.M., J.A.B., and J.A.D. laboratories for suggestions and technical assistance; and K.M. Ansel for critical reading of the manuscript. This research was supported by the UCSF Sandler Fellowship (to A.M.); a gift from Jake Aronov (to A.M.); NIH funding for the HIV Accessory & Regulatory Complexes Center (P50GM082250) (to A.M. and J.A.D.); a National MS Society Collaborative MS Research Center Award (to A.M. and J.A.D.); and the Howard Hughes Medical Institute (HHMI) (J.A.D.). S.L. is an HHMI Fellow of the Damon Runyon Cancer Research Foundation [DRG-(2176-13)], and G.E.H. is supported by an NIH training grant to UCSF Diabetes, Endocrinology and Metabolism (T32 DK741834). NR 25 TC 72 Z9 76 U1 24 U2 83 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP 10437 EP 10442 DI 10.1073/pnas.1512503112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300080 PM 26216948 ER PT J AU Vilarrasa, V Carrera, J AF Vilarrasa, Victor Carrera, Jesus TI Reply to Zoback and Gorelick: Geologic carbon storage remains a safe strategy to significantly reduce CO2 emissions SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Letter C1 [Vilarrasa, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Vilarrasa, Victor] Ecole Polytech Fed Lausanne, Sch Architecture Civil & Environm Engn, Soil Mech Lab, CH-1015 Lausanne, Switzerland. [Carrera, Jesus] Spanish Natl Res Council, Groundwater Hydrol Grp GHS UPC CSIC, Inst Environm Assessment & Water Res, Barcelona 08034, Spain. RP Vilarrasa, V (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM victor.vilarrasa@upc.edu RI Vilarrasa, Victor/A-1700-2016 OI Vilarrasa, Victor/0000-0003-1169-4469 NR 5 TC 4 Z9 5 U1 2 U2 8 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 18 PY 2015 VL 112 IS 33 BP E4511 EP E4511 DI 10.1073/pnas.1511302112 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CP2WL UT WOS:000359738300002 PM 26240341 ER PT J AU Tringe, JW Ileri, N Levie, HW Stroeve, P Ustach, V Faller, R Renaud, P AF Tringe, J. W. Ileri, N. Levie, H. W. Stroeve, P. Ustach, V. Faller, R. Renaud, P. TI Molecular Dynamics and Monte Carlo simulations resolve apparent diffusion rate differences for proteins confined in nanochannels SO CHEMICAL PHYSICS LA English DT Article DE Molecular Dynamics; Monte Carlo; Nanochannel; Protein; Nanopore; Membrane ID NANOFLUIDIC CHANNELS; LYSOZYME ADSORPTION; TRANSPORT; MEMBRANES; SURFACES; CHIP AB We use Molecular Dynamics and Monte Carlo simulations to examine molecular transport phenomena in nanochannels, explaining four orders of magnitude difference in wheat germ agglutinin (WGA) protein diffusion rates observed by fluorescence correlation spectroscopy (FCS) and by direct imaging of fluorescently-labeled proteins. We first use the ESPResSo Molecular Dynamics code to estimate the surface transport distance for neutral and charged proteins. We then employ a Monte Carlo model to calculate the paths of protein molecules on surfaces and in the bulk liquid transport medium. Our results show that the transport characteristics depend strongly on the degree of molecular surface coverage. Atomic force microscope characterization of surfaces exposed to WGA proteins for 1000 s show large protein aggregates consistent with the predicted coverage. These calculations and experiments provide useful insight into the details of molecular motion in confined geometries. (C) 2015 The Authors. Published by Elsevier B.V. C1 [Tringe, J. W.; Ileri, N.; Levie, H. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Ileri, N.; Stroeve, P.; Ustach, V.; Faller, R.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Renaud, P.] Ecole Polytech Fed Lausanne, Swiss Fed Inst Technol, CH-1015 Lausanne, Switzerland. RP Tringe, JW (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM tringe2@llnl.gov FU University of California Office of the President UCOP Lab Fee Program [12-LR-237353]; U.S. National Science Foundation I2CAM International Materials Institute Award [DMR-0844115]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by a Grant from the University of California Office of the President UCOP Lab Fee Program (Grant Number 12-LR-237353). One of us, Nazar Ileri, acknowledges the support of the U.S. National Science Foundation I2CAM International Materials Institute Award, Grant DMR-0844115. We are grateful for helpful discussions with Dr. Christine Orme at LLNL and Dr. Paul Ashby at Lawrence Berkeley National Lab regarding protein imaging with AFM. This work was partially performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 29 TC 1 Z9 1 U1 7 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD AUG 18 PY 2015 VL 457 BP 19 EP 27 DI 10.1016/j.chemphys.2015.04.021 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO7FU UT WOS:000359325800004 ER PT J AU Bousso, R Engelhardt, N AF Bousso, Raphael Engelhardt, Netta TI Proof of a new area law in general relativity SO PHYSICAL REVIEW D LA English DT Article ID BLACK-HOLE DYNAMICS; THERMODYNAMICS; HORIZONS; ENTROPY AB A future holographic screen is a hypersurface of indefinite signature, foliated by marginally trapped surfaces with area A(r). We prove that A(r) grows strictly monotonically. Future holographic screens arise in gravitational collapse. Past holographic screens exist in our own Universe; they obey an analogous area law. Both exist more broadly than event horizons or dynamical horizons. Working within classical general relativity, we assume the null curvature condition and certain generiticity conditions. We establish several nontrivial intermediate results. If a surface sigma divides a Cauchy surface into two disjoint regions, then a null hypersurface N that contains sigma splits the entire spacetime into two disjoint portions: the future-and-interior, K+; and the past-and-exterior, K-. If a family of surfaces sigma(r) foliate a hypersurface, while flowing everywhere to the past or exterior, then the future-and-interior K+(r) grows monotonically under inclusion. If the surfaces sigma(r) are marginally trapped, we prove that the evolution must be everywhere to the past or exterior, and the area theorem follows. A thermodynamic interpretation as a second law is suggested by the Bousso bound, which relates A(r) to the entropy on the null slices N(r) foliating the spacetime. In a companion letter, we summarize the proof and discuss further implications. C1 [Bousso, Raphael] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Engelhardt, Netta] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP Bousso, R (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. EM bousso@lbl.gov; engeln@physics.ucsb.edu FU Berkeley Center for Theoretical Physics; fqxi grant [RFP3-1323]; US Department of Energy [DE-AC02-05CH11231]; US NSF Graduate Research Fellowship [DGE-1144085]; NSF Grant [PHY12-05500]; National Science Foundation [1214644, 1316783] FX It is a pleasure to thank S. Fischetti, D. Harlow, G. Horowitz, W. Kelly, S. Leichenauer, D. Marolf, R. Wald, and A. Wall for discussions and correspondence. N. E. thanks the Berkeley Center for Theoretical Physics and the UC Berkeley Physics Department for their hospitality. The work of R. B. is supported in part by the Berkeley Center for Theoretical Physics, by the National Science Foundation (award numbers 1214644 and 1316783), by fqxi grant RFP3-1323, and by the US Department of Energy under Contract No. DE-AC02-05CH11231. The work of N. E. is supported in part by the US NSF Graduate Research Fellowship under Grant No. DGE-1144085 and by NSF Grant No. PHY12-05500. NR 44 TC 9 Z9 9 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 18 PY 2015 VL 92 IS 4 AR 044031 DI 10.1103/PhysRevD.92.044031 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CP4QH UT WOS:000359866900006 ER PT J AU Burms, J Caluwaerts, K Dambre, J AF Burms, Jeroen Caluwaerts, Ken Dambre, Joni TI Reward-modulated Hebbian plasticity as leverage for partially embodied control in compliant robotics SO FRONTIERS IN NEUROROBOTICS LA English DT Article DE compliant robotics; Hebbian plasticity; morphological computation; recurrent neural networks; tensegrity ID LEARNING RULE; TENSEGRITY; NETWORKS; NOISE; MODEL AB In embodied computation (or morphological computation), part of the complexity of motor control is offloaded to the body dynamics. We demonstrate that a simple Hebbian-like learning rule can be used to train systems with (partial) embodiment, and can be extended outside of the scope of traditional neural networks. To this end, we apply the learning rule to optimize the connection weights of recurrent neural networks with different topologies and for various tasks. We then apply this learning rule to a simulated compliant tensegrity robot by optimizing static feedback controllers that directly exploit the dynamics of the robot body. This leads to partially embodied controllers, i.e., hybrid controllers that naturally integrate the computations that are performed by the robot body into a neural network architecture. Our results demonstrate the universal applicability of reward-modulated Hebbian learning. Furthermore, they demonstrate the robustness of systems trained with the learning rule. This study strengthens our belief that compliant robots should or can be seen as computational units, instead of dumb hardware that needs a complex controller. This link between compliant robotics and neural networks is also the main reason for our search for simple universal learning rules for both neural networks and robotics. C1 [Burms, Jeroen; Caluwaerts, Ken; Dambre, Joni] Univ Ghent, Elect & Informat Syst Dept ELIS, Comp Syst Lab Reservoir Team, B-9000 Ghent, Belgium. [Caluwaerts, Ken] Oak Ridge Associated Univ, NASA Ames Res Ctr, Intelligent Robot Grp, Moffett Field, CA USA. RP Dambre, J (reprint author), Sint Pietersnieuwstr 41, Ghent, Belgium. EM joni.dambre@ugent.be RI Dambre, Joni/C-2926-2013 OI Dambre, Joni/0000-0002-9373-1210 FU Ph.D. fellowship of Research Foundation - Flanders (FWO); European Union Seventh Framework Programme (FP7) (Human Brain Project) [248311, 604102] FX We would like to thank Andrea Soltoggio for useful discussions in the preparation of this letter. Funding: This research was funded by a Ph.D. fellowship of the Research Foundation - Flanders (FWO) and the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreements No. 248311 (AMARSi), and No. 604102 (Human Brain Project). NR 30 TC 3 Z9 3 U1 4 U2 8 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1662-5218 J9 FRONT NEUROROBOTICS JI Front. Neurorobotics PD AUG 17 PY 2015 VL 9 AR 9 DI 10.3389/fnbot.2015.00009 PG 15 WC Computer Science, Artificial Intelligence; Robotics; Neurosciences SC Computer Science; Robotics; Neurosciences & Neurology GA DE1RB UT WOS:000370403000001 PM 26347645 ER PT J AU Qi, YR Mu, LQ Zhao, JM Hu, YS Liu, HZ Dai, S AF Qi, Yuruo Mu, Linqin Zhao, Junmei Hu, Yong-Sheng Liu, Huizhou Dai, Sheng TI Superior Na-Storage Performance of Low-Temperature-Synthesized Na-3(VO1-xPO4)(2)F1+2x (0 <= x <= 1) Nanoparticles for Na-Ion Batteries SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE cathode; Na-3(VOPO4)(2)F; Na-ion batteries; nanoparticles; solvothermal synthesis ID SODIUM VANADIUM FLUOROPHOSPHATE; CATHODE MATERIALS; LITHIUM-ION; ELECTROCHEMICAL PROPERTIES; NA3V2(PO4)(2)F-3 CATHODE; ELECTRODE MATERIALS; CRYSTAL-STRUCTURE; INSERTION; OXIDE; NA3V2O2X(PO4)(2)F3-2X AB Na-ion batteries are becoming comparable to Li-ion batteries because of their similar chemical characteristics and abundant sources of sodium. However, the materials production should be cost-effective in order to meet the demand for large-scale application. Here, a series of nanosized high-performance cathode materials, Na-3(VO1-xPO4)(2)F1+2x (0 <= x <= 1), has been synthesized by a solvothermal low-temperature (60-120 degrees C) strategy without the use of organic ligands or surfactants. The as-synthesized Na-3(VOPO4)(2)F nanoparticles show the best Na-storage performance reported so far in terms of both high rate capability (up to 10C rate) and long cycle stability over 1200 cycles. To the best of our knowledge, the current developed synthetic strategy for Na-3(VO1-xPO4)(2)F1+2x is by far one of the least expensive and energy-consuming methods, much superior to the conventional high-temperature solid-state method. C1 [Qi, Yuruo; Zhao, Junmei; Liu, Huizhou] Chinese Acad Sci, Inst Proc Engn, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China. [Qi, Yuruo] Univ Chinese Acad Sci, Beijing 100190, Peoples R China. [Mu, Linqin; Hu, Yong-Sheng] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Zhao, Junmei; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Zhao, JM (reprint author), Chinese Acad Sci, Inst Proc Engn, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China. EM jmzhao@ipe.ac.cn; yshu@aphy.iphy.ac.cn; hzliu@ipe.ac.cn RI Hu, Yong-Sheng/H-1177-2011; Dai, Sheng/K-8411-2015 OI Hu, Yong-Sheng/0000-0002-8430-6474; Dai, Sheng/0000-0002-8046-3931 FU Beijing Natural Science Foundation [2142030, 51222210]; State Scholarship Fund from China Scholarship Council; U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering FX The authors thank Yuesheng Wang for performing the XRD Rietveld refinement. This work was supported by Beijing Natural Science Foundation (2142030, 51222210) and the State Scholarship Fund from China Scholarship Council. S.D. was supported by the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering. NR 39 TC 20 Z9 20 U1 25 U2 180 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 17 PY 2015 VL 54 IS 34 BP 9911 EP 9916 DI 10.1002/anie.201503188 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA CP9LF UT WOS:000360215100027 PM 26179243 ER PT J AU Mogesa, B Perera, E Rhoda, HM Gibson, JK Oomens, J Berden, G van Stipdonk, MJ Nemykin, VN Basu, P AF Mogesa, Benjamin Perera, Eranda Rhoda, Hannah M. Gibson, John K. Oomens, Jos Berden, Giel van Stipdonk, Michael J. Nemykin, Victor N. Basu, Partha TI Solution, Solid, and Gas Phase Studies on a Nickel Dithiolene System: Spectator Metal and Reactor Ligand SO INORGANIC CHEMISTRY LA English DT Article ID PHOTON DISSOCIATION SPECTROSCOPY; RAY-ABSORPTION SPECTROSCOPY; DENSITY-FUNCTIONAL CALCULATIONS; ELECTRON-TRANSFER PROCESSES; CROWN THIOETHER CHEMISTRY; MIXED-VALENCE; BIS(DITHIOLENE) COMPLEX; COORDINATION-COMPLEXES; INFRARED-SPECTROSCOPY; SPECTRAL PROPERTIES AB The syntheses of cationic nickel complexes using N,N'-dimethyl piperazine 2,3-dithione (Me(2)Dt(0)) and N,N'-diisopropyl piperazine 2,3-dithione ((i)Pr(2)Dt(0)) ligands are reported. These ligands were used in synthesizing bis and tris(dithione)Ni(II) complexes as tetrafluoroborate or hexafluorophosphate salts, i.e., [Ni((i)Pr(2)Dt)(2)][BBO2 ([1a] [BF4](2)), [Ni(1Pr(2)Dt)(2)][PF6](2) Oa] [PF6](2)), [Ni(Me(2)Dt)] I-BF 4, 1 2 [ib] [BF4](2)), [Ni(iPr(2)Dt)3] [BF4](2) ([2a] [BF4](2)), and (Pr(2)Dt)(3)][PF6](2) ([2a] [PF6](2)), respectively. Complex [2a][PF6](2) was isolated from a methanolic solution of [la] [PF6](2). Compound [la] [BF4](2) crystallizes in a trigonal crystal system (space group, P31/c) and exhibits unique packing features, whereas [2a] [BF4](2) crystallizes in a monoclinic (P21/n) space group. Cyclic voltammograms of [1a][BF4], and [1b][BF4], are indicative of four reduction processes associated with stepwise single-electron reduction of the ligands. Spectroelectrochemical experiments on [la] [BF4](2) exhibit an intervalence charge transfer (IVCT) transition as a spectroscopic signature of the mixed-valence [Ni(Pr(2)Dt)((i)Pr(2)Dt(0))]- species. Analysis of this IVCT band suggests that this ligand based mixed valence complex, [Ni(iPr(2)Dt)((i)Pr(2)Dti(0))]-, behaves more like a traditional class metal based mixed-valence complex. The density functional theory (DFT) and time dependent DFT calculations provide a theoretical framework for understanding the electronic structures and the nature of excited states of the target compounds that are consistent with their spectroscopic and redox properties. Vibrational spectra of [1a](2+) and [2a](2+) were investigated as discrete species in the gas phase using infrared multiple photon dissociation (IRMPD) spectroscopy. C1 [Mogesa, Benjamin; Perera, Eranda; van Stipdonk, Michael J.; Basu, Partha] Duquesne Univ, Dept Chem & Biochem, Pittsburgh, PA 15282 USA. [Rhoda, Hannah M.; Nemykin, Victor N.] Univ Minnesota, Dept Chem & Biochem, Duluth, MN 55812 USA. [Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Oomens, Jos; Berden, Giel] Radboud Univ Nijmegen, Inst Mol & Mat, FELIX Lab, NL-6525 ED Nijmegen, Netherlands. RP van Stipdonk, MJ (reprint author), Duquesne Univ, Dept Chem & Biochem, Pittsburgh, PA 15282 USA. EM Vanstipdonkm@duq.edu; vnemykin@d.umn.edu; Basu@duq.edu RI Nemykin, Victor/J-3747-2013; Berden, Giel/F-9690-2015; Oomens, Jos/F-9691-2015 OI Nemykin, Victor/0000-0003-4345-0848; FU National Institutes of Health [GM 061555]; U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; Netherlands Organisation for Scientific Research (NWO) [724.011.002]; National High Field FT-ICR Facility at the National High Magnetic Field Laboratory, Tallahassee, FL [CHE-9909502] FX We thank the National Institutes of Health (GM 061555 to P.B.) for partial financial support of this work. V.N.N. wishes to acknowledge Minnesota Supercomputing Institute grant and assistance of A. Purchell with spectroelectrochemical data. Stephen Ratvasky is acknowledged for his assistance with crystallography during the preparation of this manuscript. The work of J.K.G. was fully supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract No. DE-AC02-05CH11231. J.O. acknowledges The Netherlands Organisation for Scientific Research (NWO) for Vici Grant No. 724.011.002 and the Stichting Physica. Construction and shipping of the FT-ICR-MS was made possible through funding from the National High Field FT-ICR Facility (Grant CHE-9909502) at the National High Magnetic Field Laboratory, Tallahassee, FL. The excellent support by Dr. B. Redlich and others of the FELIX staff is gratefully acknowledged. NR 110 TC 6 Z9 6 U1 1 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 17 PY 2015 VL 54 IS 16 BP 7703 EP 7716 DI 10.1021/acs.inorgchem.5b00531 PG 14 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CP4AM UT WOS:000359824400006 PM 26244772 ER PT J AU Tong, LP Kopecky, A Zong, RF Gagnon, KJ Ahlquist, MSG Thummel, RP AF Tong, Lianpeng Kopecky, Andrew Zong, Ruifa Gagnon, Kevin J. Ahlquist, Marten S. G. Thummel, Randolph P. TI Light-Driven Proton Reduction in Aqueous Medium Catalyzed by a Family of Cobalt Complexes with Tetradentate Polypyridine-Type Ligands SO INORGANIC CHEMISTRY LA English DT Article ID ELECTROCATALYTIC HYDROGEN EVOLUTION; VISIBLE-LIGHT; HOMOGENEOUS CATALYSIS; WATER OXIDATION; MOLECULAR ELECTROCATALYSTS; PHOTO-REDUCTION; ENERGY; H-2; PHOTOGENERATION; POTENTIALS AB A series of tetradentate 2,2':6',2":6",2"-quaterpyridine-type ligands related to ppq (ppq = 8-(1",10"phenanthrol-2"-y1)-2-(pyrid-2'-yOquinoline) have been synthesized. One ligand replaces the 1,10-phenanthroline (phen) moiety of ppq with 2,2'-bipyridine and the other two ligands have a 3,3'-polymethylene subunit bridging the quinoline and pyridine. The structural result is that both the planarity and flexibility of the ligand are modified. Co (II) complexes are prepared and characterized by ultraviolet-visible light (UVvis) and mass spectroscopy, cyclic voltammetry, and X-ray analysis. The light-driven H-2-evolving activity of these Co complexes was evaluated under homogeneous aqueous conditions using [Ru(bpy)(3)](2) as the photosensitizer, ascorbic acid as a sacrificial electron donor, and a blue light-emitting diode (LED) as the light source. At pH 4.5, all three complexes plus [Co(ppq)Cl-2] showed the fastest rate, with the dimethylene-bridged system giving the highest turnover frequency (2125 h(-1)). Cyclic voltammograms showed a significant catalytic current for H2 production in both aqueous buffer and H2O/DMF medium. Combined experimental and theoretical study suggest a formal Co(L)-hydride species as a key intermediate that triggers H-2 generation. Spin density analysis shows involvement of the tetradentate ligand in the redox sequence from the initial Co(II) state to the Co(II)-hydride intermediate. How the ligand scaffold influences the catalytic activity and stability of catalysts is discussed, in terms of the rigidity and differences in conjugation for this series of ligands. C1 [Tong, Lianpeng; Kopecky, Andrew; Zong, Ruifa; Thummel, Randolph P.] Univ Houston, Dept Chem, Houston, TX 77204 USA. [Ahlquist, Marten S. G.] KTH Royal Inst Technol, Sch Biotechnol, Div Theoret Chem & Biol, S-10691 Stockholm, Sweden. [Gagnon, Kevin J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Ahlquist, MSG (reprint author), KTH Royal Inst Technol, Sch Biotechnol, Div Theoret Chem & Biol, S-10691 Stockholm, Sweden. EM ahlqui@kth.se; thummel@uh.edu RI Ahlquist, Marten/D-2601-2010 OI Ahlquist, Marten/0000-0002-1553-4027 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-FG02-07ER15888]; Robert A. Welch Foundation [E-621]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (Grant No. DE-FG02-07ER15888) and the Robert A. Welch Foundation (Grant No. E-621) for financial support of this work. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 54 TC 8 Z9 9 U1 4 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 17 PY 2015 VL 54 IS 16 BP 7873 EP 7884 DI 10.1021/acs.inorgchem.5b00915 PG 12 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CP4AM UT WOS:000359824400022 PM 26213196 ER PT J AU Bugaris, DE Han, F Im, J Chung, DY Freeman, AJ Kanatzidis, MG AF Bugaris, Daniel E. Han, Fei Im, Jino Chung, Duck Young Freeman, Arthur J. Kanatzidis, Mercouri G. TI Crystal Growth, Structures, and Properties of the Complex Borides, LaOs2Al2B and La2Os2AlB2 SO INORGANIC CHEMISTRY LA English DT Article ID PHYSICAL-PROPERTIES; TERNARY BORIDES; SINGLE-CRYSTALS; STRUCTURE REFINEMENT; MAGNETIC-PROPERTIES; CHANNEL STRUCTURE; IRIDIUM BORIDE; SUPERCONDUCTIVITY; EARTH; BORON AB Single crystals of two novel quaternary metal borides, LaOs2Al2B and La2Os2AlB2, have been grown from La/Ni eutectic fluxes. LaOs2Al2B crystallizes in tetragonal space group P4/mmm with the CeCr2Si2C-type structure, and lattice parameters a = 4.2075(6) angstrom and c = 5.634(1) angstrom. La2Os2AlB2 exhibits a new crystal structure in monoclinic space group C2/c with lattice parameters a = 16.629(3) angstrom, b = 6.048(1) angstrom, c = 10.393(2) angstrom, and beta = 113.96(3)degrees. Both structures are three-dimensional frameworks with unusual coordination (for solid-state compounds) of the boron atoms by transition metal atoms. The boron atom is square planar in LaOs2Al2B, whereas it exhibits linear and T-shaped geometries in La2Os2AlB2. Electrical resistivity measurements reveal poor metal behavior (rho(30)0 (K) similar to 900 mu Omega cm) for La2Os2AlB2, consistent with the electronic band structure calculations, which also predict a metallic character for LaOs2Al2B. C1 [Bugaris, Daniel E.; Han, Fei; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Im, Jino; Freeman, Arthur J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Im, Jino] Korea Res Inst Chem Technol, Adv Mat Div, Taejon 305600, South Korea. [Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013 OI Han, Fei/0000-0001-7782-2713 FU Center for Emergent Superconductivity, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This work was supported as part of the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 77 TC 4 Z9 4 U1 2 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 17 PY 2015 VL 54 IS 16 BP 8049 EP 8057 DI 10.1021/acs.inorgchem.5b01275 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CP4AM UT WOS:000359824400042 PM 26241801 ER PT J AU Myers, TW Chavez, DE Hanson, SK Scharff, RJ Scott, BL Veauthier, JM Wu, RL AF Myers, Thomas W. Chavez, David E. Hanson, Susan K. Scharff, R. Jason Scott, Brian L. Veauthier, Jacqueline M. Wu, Ruilian TI Independent Control of Optical and Explosive Properties: Pyrazole-Tetrazine Complexes of First Row Transition Metals SO INORGANIC CHEMISTRY LA English DT Article ID IGNITABLE PRIMARY EXPLOSIVES; NITROGEN-RICH; LIGAND; COMBUSTION; COPPER; STATES; DECOMPOSITION; PERCHLORATE; ABSORPTION; INITIATION AB Complexes of 3-amino-6-(3,5-dimethylpyrazole)-tetrazine) (NH(2)TzDMP, 1) and 3-(3,3'-dinitroazetidine)-6-(3,5-dimethylpyrazole)tetrazine) (DNAZTzDMP, 2) with first row transition metal centers were synthesized. Reactions of Fe-II(H2O)(6)(BF4)(2) and Fe(NO3)(3)center dot 9H(2)O with 1 and 2 both led to complexes of the form [(RTzDMP)(3)Fe]X-2 (X = BF4, R = NH2 (3), DNAZ (4); X = NO3, R = NH2 (5), DNAZ (6)), which showed intense MLCT bands in the visible region of the spectrum. Ligands 1 and 2 also reacted with Cu-II(NO3)(2)center dot 5/2H(2)O to form [(RTzDMP)(2)Cu(NO3)][NO3] (R = NH2 (7), DNAZ (8)) in addition to reacting with Cu-I(CH3CN)(4)(PF6) to form [(RTzDMP)(2)Cu][PF6] (R = NH2 (9), DNAZ (10)). Lastly reactions of 1 and 2 with Co(NO3)(2)center dot 6H(2)O and Ni(NO3)(2)center dot 6H(2)O led to [(NH(2)TzDMP)(2)Co(H2O) (NO3)] [NO3] (11), [(DNAZTzDMP)(2)Co(H2O)(2)] [NO3](2) (12), [(NH(2)TzDMP)(3)Ni][NO3](2) (13), and [(DNAZTzDMP)(2)Ni(H2O)(2)[NO3](2) (14). The complexes display rich electrochemical and photophysical properties that are unaffected by derivation with explosive groups. C1 [Myers, Thomas W.; Chavez, David E.; Scharff, R. Jason] Los Alamos Natl Lab, M Div, Los Alamos, NM 87545 USA. [Hanson, Susan K.; Veauthier, Jacqueline M.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat, Los Alamos, NM 87545 USA. [Wu, Ruilian] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Myers, TW (reprint author), Los Alamos Natl Lab, M Div, POB 1663, Los Alamos, NM 87545 USA. EM twmyers@lanl.gov; dechavez@lanl.gov; veauthier@lanl.gov RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Scharff, Robert/0000-0002-1708-8964; Veauthier, Jacqueline/0000-0003-2206-7786 FU Los Alamos National Laboratory LDRD [20150005DR] FX This work was supported by Los Alamos National Laboratory LDRD (20150005DR) and by a Director's Postdoctoral Fellowship for T.W.M. NR 55 TC 8 Z9 8 U1 2 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 17 PY 2015 VL 54 IS 16 BP 8077 EP 8086 DI 10.1021/acs.inorgchem.5b01313 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CP4AM UT WOS:000359824400045 PM 26237120 ER PT J AU Manbeck, GF Canterbury, T Zhou, RW King, S Nam, G Brewer, KJ AF Manbeck, Gerald F. Canterbury, Theodore Zhou, Rongwei King, Skye Nam, Geewoo Brewer, Karen J. TI Electrocatalytic H-2 Evolution by Supramolecular Ru-II-Rh-III-Ru-II Complexes: Importance of Ligands as Electron Reservoirs and Speciation upon Reduction SO INORGANIC CHEMISTRY LA English DT Article ID PHOTOCATALYTIC HYDROGEN-PRODUCTION; ARTIFICIAL PHOTOSYNTHESIS; WATER REDUCTION; HETEROGENEOUS CATALYSIS; MOLECULAR CATALYSTS; PHOTOELECTROCHEMICAL CELLS; ELECTROCHEMICAL PROPERTIES; CYCLIC VOLTAMMETRY; LOW OVERPOTENTIALS; IRIDIUM COMPLEXES AB The supramolecular water reduction photocatalysts (Ph(2)phen)(2)Ru(dpp)}(2)RhX2] (PF6)(5) (Ph(2)phen = 4,7-diphenyl-1,10-phenanthroline, dpp =2,3-bis(2-pyridyl)pyrazine X = Cl, Br) are efficient electrocatalysts for the reduction of CF3SO3H, CF3CO2H, and CH3CO2H to H-2 in DMF or DMF/H2O mixtures. The onset of catalytic current occurs at 0.82 V versus Ag/AgCl for CF3SO3H, -0.90 V for CF3CO2H, and -1.1 V for CH3CO2H with overpotentials of 0.61, 0.45, and 0.10 V, respectively. In each case, catalysis is triggered by the first dpp ligand reduction implicating the dpp as an electron reservoir in catalysis. A new species with E-pc similar to -0.75 V was observed in the presence of stoichiometric amounts of strong acid, and its identity is proposed as the Rh(H)(III/II) redox couple. H-2 was produced in 72-85% Faradaic yields and 95-116 turnovers after 2 h and 435 turnovers after 10 h of bulk electrolysis. The identities of Rh(I) species upon reduction have been studied. In contrast to the expected dissociation of halides in the Rh(I) state, the halide loss depends on solvent and water content. In dry CH3CN, in which Cl is poorly solvated, a [Ru] complex dissociates and [(Ph(2)phen)(2)Ru(dpp)(RhCl2)-Cl-I](+) and [(Ph(2)phen)(2)Ru(dpp)](2+) are formed. In contrast, for X = Br-, the major product of reduction is the intact trimetallic Rh(I) complex [{(Ph(2)phen)(2)Ru(dpp)}(2)Rh-I](5+). Chloride loss in CH3CN is facilitated by addition of 3 M H2O. In DMF, the reduced species is [{(Ph(2)phen)(2)Ru(dpp)}(2)Rh-I](5+) regardless of X = Cl- or Br-. C1 [Manbeck, Gerald F.; Canterbury, Theodore; Zhou, Rongwei; King, Skye; Nam, Geewoo; Brewer, Karen J.] Virginia Tech, Dept Chem, Blacksburg, VA 24061 USA. RP Manbeck, GF (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM gmanbeck@bnl.gov FU Department of Energy [DE-FG02-05ER15751] FX This material is based upon work supported by the Department of Energy under award number DE-FG02-05ER15751. The authors would like to thank Dr. Etsuko Fujita for helpful comments during the preparation of this manuscript. NR 115 TC 3 Z9 3 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 17 PY 2015 VL 54 IS 16 BP 8148 EP 8157 DI 10.1021/acs.inorgchem.5b01536 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CP4AM UT WOS:000359824400053 PM 26247428 ER PT J AU Agrawal, P Chacko, Z Kilic, C Verhaaren, CB AF Agrawal, Prateek Chacko, Zackaria Kilic, Can Verhaaren, Christopher B. TI A couplet from flavored dark matter SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Global Symmetries ID X-RAY-LINE; GALAXY CLUSTERS; SIGNAL; SCALE; MODELS; HIGGS AB We show that a couplet, a pair of closely spaced photon lines, in the X-ray spectrum is a distinctive feature of lepton flavored dark matter models for which the mass spectrum is dictated by Minimal Flavor Violation. In such a scenario, mass splittings between different dark matter flavors are determined by Standard Model Yukawa couplings and can naturally be small, allowing all three flavors to be long-lived and contribute to the observed abundance. Then, in the presence of a tiny source of flavor violation, heavier dark matter flavors can decay via a dipole transition on cosmological timescales, giving rise to three photon lines. Two of these lines are closely spaced, and constitute the couplet. Provided the flavor violation is sufficiently small, the ratios of the line energies are determined in terms of the charged lepton masses, and constitute a prediction of this framework. For dark matter masses of order the weak scale, the couplet lies in the keV-MeV region, with a much weaker line in the eV-keV region. This scenario constitutes a potential explanation for the recent claim of the observation of a 3.5 keV line. The next generation of X-ray telescopes may have the necessary resolution to resolve the double line structure of such a couplet. C1 [Agrawal, Prateek] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Chacko, Zackaria; Verhaaren, Christopher B.] Univ Maryland, Dept Phys, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Kilic, Can] Univ Texas Austin, Dept Phys, Theory Grp, Austin, TX 78712 USA. [Kilic, Can] Univ Texas Austin, Texas Cosmol Ctr, Austin, TX 78712 USA. RP Agrawal, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM prateek@fnal.gov; zchacko@umd.edu; kilic@physics.utexas.edu; cver@umd.edu OI Verhaaren, Christopher/0000-0001-6798-804X FU National Science Foundation [PHYS-1066293]; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation; NSF [PHY-1315155, PHY-1315983, PHY-1316033]; United States Department of Energy [De-AC02-07CH11359] FX We thank Ilias Cholis and Dan Hooper for useful discussions. CK would also like to thank the Aspen Center for Physics (supported by the National Science Foundation under Grant No. PHYS-1066293) as well as the Perimeter Institute for Theoretical Physics (supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation), where part of this work was completed, for their hospitality. ZC and CV are supported by NSF under grant PHY-1315155. CK is supported by NSF grant numbers PHY-1315983 and PHY-1316033. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 123 TC 5 Z9 5 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 17 PY 2015 IS 8 AR 072 DI 10.1007/JHEP08(2015)072 PG 21 WC Physics, Particles & Fields SC Physics GA CP6YZ UT WOS:000360035700002 ER PT J AU Li, MD Chang, CZ Kirby, BJ Jamer, ME Cui, WP Wu, LJ Wei, P Zhu, YM Heiman, D Li, J Moodera, JS AF Li, Mingda Chang, Cui-Zu Kirby, Brian. J. Jamer, Michelle E. Cui, Wenping Wu, Lijun Wei, Peng Zhu, Yimei Heiman, Don Li, Ju Moodera, Jagadeesh S. TI Proximity-Driven Enhanced Magnetic Order at Ferromagnetic-Insulator-Magnetic-Topological-Insulator Interface SO PHYSICAL REVIEW LETTERS LA English DT Article ID EXCHANGE BIAS; SURFACE; STATE AB Magnetic exchange driven proximity effect at a magnetic-insulator-topological-insulator (MI-TI) interface provides a rich playground for novel phenomena as well as a way to realize low energy dissipation quantum devices. Here we report a dramatic enhancement of proximity exchange coupling in the MI/magnetic- TI EuS/Sb2-xVxTe3 hybrid heterostructure, where V doping is used to drive the TI (Sb2Te3) magnetic. We observe an artificial antiferromagneticlike structure near the MI-TI interface, which may account for the enhanced proximity coupling. The interplay between the proximity effect and doping in a hybrid heterostructure provides insights into the engineering of magnetic ordering. C1 [Li, Mingda; Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Li, Mingda; Chang, Cui-Zu; Wei, Peng; Moodera, Jagadeesh S.] MIT, Fracsis Bitter Magnet Lab, Cambridge, MA 02139 USA. [Li, Mingda; Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Kirby, Brian. J.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Jamer, Michelle E.; Heiman, Don] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Cui, Wenping] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Moodera, Jagadeesh S.] MIT, Dept Phys, Cambridge, MA 02139 USA. RP Li, MD (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM mingda@mit.edu; czchang@mit.edu; moodera@mit.edu RI Li, Ju/A-2993-2008; Wei, Peng/L-5738-2013; Chang, Cui-Zu/P-3049-2014; OI Li, Ju/0000-0002-7841-8058; Wei, Peng/0000-0003-2289-6007; Jamer, Michelle/0000-0001-5316-8817 FU STC CIQM under NSF [DMR-1231319]; NSF DMR [1207469]; ONR [N00014-13-1-0301]; MRSEC Program of the NSF [DMR-0819762]; NSF [DMR-907007, ECCS-1402738, DMR-1410636]; DOE-BES [DE-SC0012704] FX M. L. and C. Z. C. would thank the helpful discussion with Prof. Albert Fert. J. S. M. and C. Z. C. are thankful for support from the STC CIQM under NSF Grant No. DMR-1231319, NSF DMR Grant No. 1207469 and ONR Grant No. N00014-13-1-0301, and MRSEC Program of the NSF under Award No. DMR-0819762. M. J. and D. H. acknowledge support from NSF DMR-907007 and NSF ECCS-1402738. L. W. and Y. Z. were supported by DOE-BES under Contract No. DE-SC0012704. M. L. and J. L. acknowledge support from NSF DMR-1410636. NR 41 TC 9 Z9 9 U1 14 U2 59 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 17 PY 2015 VL 115 IS 8 AR 087201 DI 10.1103/PhysRevLett.115.087201 PG 5 WC Physics, Multidisciplinary SC Physics GA CP4SD UT WOS:000359872000006 PM 26340203 ER PT J AU Chen, X Hogan, T Walkup, D Zhou, WW Pokharel, M Yao, ML Tian, W Ward, TZ Zhao, Y Parshall, D Opeil, C Lynn, JW Madhavan, V Wilson, SD AF Chen, Xiang Hogan, Tom Walkup, D. Zhou, Wenwen Pokharel, M. Yao, Mengliang Tian, Wei Ward, Thomas Z. Zhao, Y. Parshall, D. Opeil, C. Lynn, J. W. Madhavan, Vidya Wilson, Stephen D. TI Influence of electron doping on the ground state of (Sr1-xLax)(2)IrO4 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-GLASS; SR2IRO4; MAGNETORESISTANCE; CONDUCTIVITY; SYSTEMS; LOCALIZATION; TRANSPORT; PHASE AB The evolution of the electronic properties of electron-doped (Sr1-x La-x)(2)IrO4 is experimentally explored as the doping limit of La is approached. As electrons are introduced, the electronic ground-state transitions from a spin-orbit Mott phase into an electronically phase separated state, where long-range magnetic order vanishes beyond x = 0.02 and charge transport remains percolative up to the limit of La substitution (x approximate to 0.06). In particular, the electronic ground state remains inhomogeneous even beyond the collapse of the parent state's longrange antiferromagnetic order, while persistent short-range magnetism survives up to the highest La-substitution levels. Furthermore, as electrons are doped into Sr2IrO4, we observe the appearance of a low-temperature magnetic glasslike state intermediate to the complete suppression of antiferromagnetic order. Universalities and differences in the electron-doped phase diagrams of single-layer and bilayer Ruddlesden-Popper strontium iridates are discussed. C1 [Chen, Xiang; Hogan, Tom; Walkup, D.; Zhou, Wenwen; Pokharel, M.; Yao, Mengliang; Opeil, C.] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Chen, Xiang; Hogan, Tom; Wilson, Stephen D.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Tian, Wei] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Ward, Thomas Z.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Zhao, Y.; Parshall, D.; Lynn, J. W.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Zhao, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Madhavan, Vidya] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Madhavan, Vidya] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. RP Chen, X (reprint author), Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. EM stephendwilson@engineering.ucsb.edu RI Ward, Thomas/I-6636-2016; Zhou, Wenwen/K-9854-2016; Tian, Wei/C-8604-2013 OI Ward, Thomas/0000-0002-1027-9186; Tian, Wei/0000-0001-7735-3187 FU NSF CAREER award [DMR-1056625]; NSF [DMR-0944772, DMR-1305647]; US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; [DMR-1337567] FX X.C. gratefully acknowledges Brandon Isaac and the 11-BM beam line staff for assistance with experiments. This work was supported in part by NSF CAREER award DMR-1056625 (S.D.W. and X.C.). This work utilized facilities supported in part under NSF award DMR-0944772 and SQUID measurements were supported in part by grant DMR-1337567. Part of this effort was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division, (TZW). STM work was supported by NSF DMR-1305647 (V.M.). Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Research conducted at ORNLs High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The identification of any commercial product or trade name does not imply endorsement or recommendation by the National Institute of Standards and Technology. NR 49 TC 10 Z9 10 U1 3 U2 50 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 17 PY 2015 VL 92 IS 7 AR 075125 DI 10.1103/PhysRevB.92.075125 PG 11 WC Physics, Condensed Matter SC Physics GA CP1ZD UT WOS:000359675600002 ER PT J AU Jeong, J Yang, I Yang, J Ayala-Valenzuela, OE Wulferding, D Zhou, JS Goodenough, JB de Lozanne, A Mitchell, JF Leon, N Movshovich, R Jeong, YH Yeom, HW Kim, J AF Jeong, Juyoung Yang, Ilkyu Yang, Jinho Ayala-Valenzuela, Oscar E. Wulferding, Dirk Zhou, J. -S. Goodenough, John B. de Lozanne, Alex Mitchell, J. F. Leon, Neliza Movshovich, Roman Jeong, Yoon Hee Yeom, Han Woong Kim, Jeehoon TI Magnetic domain tuning and the emergence of bubble domains in the bilayer manganite La2-2xSr1+2xMn2O7 (x=0.32) SO PHYSICAL REVIEW B LA English DT Article ID LAYERED MANGANITE; ANISOTROPY; CRYSTAL; PHYSICS; SPIN AB We report a magnetic force microscopy study of the magnetic domain evolution in the layered manganite La2-2x Sr1+2x Mn2O7 (with x = 0.32). This strongly correlated electron compound is known to exhibit a wide range of magnetic phases, including a recently uncovered biskyrmion phase. We observe a continuous transition from dendritic to stripelike domains, followed by the formation of magnetic bubbles due to a field-and temperaturedependent competition between in-plane and out-of-plane spin alignments. The magnetic bubble phase appears at comparable field and temperature ranges as the biskyrmion phase, suggesting a close relation between both phases. Based on our real-space images we construct a temperature-field phase diagram for this composition. C1 [Jeong, Juyoung; Yang, Ilkyu; Yang, Jinho; Ayala-Valenzuela, Oscar E.; Wulferding, Dirk; Yeom, Han Woong; Kim, Jeehoon] Inst for Basic Sci Korea, Ctr Artificial Low Dimens Elect Syst, Pohang 790784, South Korea. [Jeong, Juyoung; Yang, Ilkyu; Yang, Jinho; Ayala-Valenzuela, Oscar E.; Wulferding, Dirk; Jeong, Yoon Hee; Yeom, Han Woong; Kim, Jeehoon] Pohang Univ Sci & Technol, Dept Phys, Pohang 790784, South Korea. [Zhou, J. -S.; Goodenough, John B.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [de Lozanne, Alex] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Mitchell, J. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Leon, Neliza; Movshovich, Roman] Los Alamos Natl Lab, MPA CMMS, Los Alamos, NM 87545 USA. RP Kim, J (reprint author), Inst for Basic Sci Korea, Ctr Artificial Low Dimens Elect Syst, 77 Cheongam Ro, Pohang 790784, South Korea. EM jeehoon@postech.ac.kr OI Wulferding, Dirk/0000-0003-4279-2109; Goodenough, John Bannister/0000-0001-9350-3034 FU Institute for Basic Science (IBS) in Korea [IBS-R014-D1]; NSF DMR in the USA [1122603]; U.S. DOE, Office of Science, Basic Energy Science, Materials Science and Engineering Division; Center for Topological Matter at POSTECH [2011-0030786] FX We gratefully acknowledge important discussions with N. Haberkorn. This work was supported by the Institute for Basic Science (IBS), Grant No. IBS-R014-D1, in Korea and NSF DMR 1122603 in the USA. Work at Argonne National Laboratory (crystal growth and sample characterization) was sponsored by the U.S. DOE, Office of Science, Basic Energy Science, Materials Science and Engineering Division. Y.H.J. was supported by the Center for Topological Matter at POSTECH (Grant No. 2011-0030786). NR 26 TC 2 Z9 2 U1 7 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 17 PY 2015 VL 92 IS 5 AR 054426 DI 10.1103/PhysRevB.92.054426 PG 5 WC Physics, Condensed Matter SC Physics GA CP1YD UT WOS:000359672900001 ER PT J AU Ahmad, I Chasman, RR Greene, JP Kondev, FG Zhu, S AF Ahmad, I. Chasman, R. R. Greene, J. P. Kondev, F. G. Zhu, S. TI Electron capture decay of 58-min U-229(92) and levels in Pa-229(91) SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; OCTUPOLE DEFORMATION; PARITY DOUBLETS; AC-225; ODD AB Electron capture decay of U-229 is investigated by measuring the gamma-ray and conversion electron spectra of mass-separated and unseparated U-229 sources with high-resolution germanium and silicon detectors, respectively. Gamma-gamma coincidence measurements are also performed using germanium detectors. These studies provide level energies and level ordering in Pa-229. Single-particle assignments are given to these levels which are in agreement with the systematics in this region and also with theory. In a previous study, we report the observation of a 5/2(+/-) parity doublet in the Pa-229 ground state, which is a signature of octupole deformation. The present analysis of the data still shows a splitting of 60 +/- 50 eV, but with this large uncertainty the existence of the doublet is not certain. C1 [Ahmad, I.; Chasman, R. R.; Greene, J. P.; Kondev, F. G.; Zhu, S.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Ahmad, I (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM kondev@anl.gov FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 23 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 17 PY 2015 VL 92 IS 2 AR 024313 DI 10.1103/PhysRevC.92.024313 PG 10 WC Physics, Nuclear SC Physics GA CP2AI UT WOS:000359678800004 ER PT J AU Bedaque, PF Steiner, AW AF Bedaque, Paulo F. Steiner, Andrew W. TI Hypernuclei and the hyperon problem in neutron stars SO PHYSICAL REVIEW C LA English DT Article ID EQUATION-OF-STATE; MASS-RADIUS RELATION; LAMBDA-HYPERNUCLEI; SYMMETRY ENERGY; LATTICE QCD; MATTER; SCATTERING AB The likely presence of Lambda baryons in dense hadronic matter tends to soften the equation of state to an extent that the observed heaviest neutron stars are difficult to explain. We analyze this "hyperon problem" with a phenomenological approach. First, we review what can be learned about the interaction of Lambda particle with dense matter from the observed hypernuclei and extend this phenomenological analysis to asymmetric matter. We add to this the current knowledge on nonstrange dense matter, including its uncertainties, to conclude that the interaction between Lambda's and dense matter has to become repulsive at densities below three times the nuclear saturation density. C1 [Bedaque, Paulo F.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Steiner, Andrew W.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Steiner, Andrew W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Steiner, Andrew W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Bedaque, PF (reprint author), Univ Maryland, Dept Phys, College Pk, MD 20742 USA. FU U.S. Department of Energy Office of Science, Office of Nuclear Physics [DE-FG02-93ER-40762] FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Nuclear Physics under Grant No. DE-FG02-93ER-40762. The solver for the stellar structure equations was obtained from O2scl [38] and the Monte Carlo was based on the Bayesian analysis routines in [39]. NR 39 TC 4 Z9 4 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 17 PY 2015 VL 92 IS 2 AR 025803 DI 10.1103/PhysRevC.92.025803 PG 7 WC Physics, Nuclear SC Physics GA CP2AI UT WOS:000359678800007 ER PT J AU Noji, S Zegers, RGT Austin, SM Baugher, T Bazin, D Brown, BA Campbell, CM Cole, AL Doster, HJ Gade, A Guess, CJ Gupta, S Hitt, GW Langer, C Lipschutz, S Lunderberg, E Meharchand, R Meisel, Z Perdikakis, G Pereira, J Recchia, F Schatz, H Scott, M Stroberg, SR Sullivan, C Valdez, L Walz, C Weisshaar, D Williams, SJ Wimmer, K AF Noji, S. Zegers, R. G. T. Austin, Sam M. Baugher, T. Bazin, D. Brown, B. A. Campbell, C. M. Cole, A. L. Doster, H. J. Gade, A. Guess, C. J. Gupta, S. Hitt, G. W. Langer, C. Lipschutz, S. Lunderberg, E. Meharchand, R. Meisel, Z. Perdikakis, G. Pereira, J. Recchia, F. Schatz, H. Scott, M. Stroberg, S. R. Sullivan, C. Valdez, L. Walz, C. Weisshaar, D. Williams, S. J. Wimmer, K. TI Gamow-Teller transitions to Ca-45 via the Sc-45(t,He-3 + gamma) reaction at 115 MeV/u and its application to stellar electron-capture rates SO PHYSICAL REVIEW C LA English DT Article ID WEAK-INTERACTION RATES; INTERMEDIATE-MASS NUCLEI; SHELL-MODEL CALCULATIONS; SECONDARY TRITON BEAM; RANGE A=45-65; IA SUPERNOVAE; RATE TABLES; DATA SHEETS; STRENGTH; ENVIRONMENTS AB Background: Stellar electron-capture reactions on medium-heavy nuclei are important for many astrophysical phenomena, including core-collapse and thermonuclear supernovae and neutron stars. Estimates of electron-capture rates rely on accurate estimates of Gamow-Teller strength distributions, which can be extracted from charge-exchange reactions at intermediate beam energies. Measured Gamow-Teller transition strength distributions for stable pf-shell nuclei are reasonably well reproduced by theoretical calculations in the shell model, except for lower mass nuclei where admixtures from the sd shell can become important. Purpose: This paper presents a beta(+) charge-exchange experiment on Sc-45, one of the lightest pf-shell nuclei. The focus was on Gamow-Teller transitions to final states at low excitation energies, which are particularly important for accurate estimations of electron-capture rates at relatively low stellar densities. The experimental results are compared with various theoretical models. Method: The double-differential cross section for the Sc-45(t, He-3 + gamma) reaction was measured using the NSCL Coupled-Cyclotron Facility at 115 MeV/u. Gamow-Teller contributions to the excitation-energy spectra were extracted by means of a multipole-decomposition analysis. gamma rays emitted due to the deexcitation of Ca-45 were measured using GRETINA to allow for the extraction of Gamow-Teller strengths from very weak transitions at low excitation energies. Results: Gamow-Teller transition strengths to Ca-45 were extracted up to an excitation energy of 20 MeV, and that to the first excited state in Ca-45 at 174 keV was extracted from the gamma-ray measurement, which, even though weak, is important for the astrophysical applications and dominates under certain stellar conditions. Shell-model calculations performed in the pf shell-model space with the GXPF1A, KB3G, and FPD6 interactions did not reproduce the experimental Gamow-Teller strength distribution, and a calculation using the quasiparticle random phase approximation that is often used in astrophysical simulations also could not reproduce the experimental strength distribution. Conclusions: Theoretical models aimed at describing Gamow-Teller transition strengths from nuclei in the lower pf shell for the purpose of estimating electron-capture rates for astrophysical simulations require further development. The likely cause for the relatively poor performance of the shell-model theory is the influence of intruder configurations from the sd shell. The combination of charge-exchange experiments at intermediate beam energy and high-resolution gamma-ray detection provides a powerful technique to identify weak transitions to low-lying final states that are nearly impossible to identify without the coincidences. Identification of these weak low-lying transitions is important for providing accurate electron-capture rates for astrophysical simulations. C1 [Noji, S.; Zegers, R. G. T.; Austin, Sam M.; Baugher, T.; Bazin, D.; Brown, B. A.; Doster, H. J.; Gade, A.; Langer, C.; Lipschutz, S.; Lunderberg, E.; Meisel, Z.; Perdikakis, G.; Pereira, J.; Recchia, F.; Schatz, H.; Scott, M.; Stroberg, S. R.; Sullivan, C.; Walz, C.; Weisshaar, D.; Williams, S. J.; Wimmer, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Noji, S.; Zegers, R. G. T.; Austin, Sam M.; Brown, B. A.; Cole, A. L.; Langer, C.; Lipschutz, S.; Meisel, Z.; Perdikakis, G.; Pereira, J.; Schatz, H.; Sullivan, C.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Zegers, R. G. T.; Baugher, T.; Brown, B. A.; Doster, H. J.; Gade, A.; Lipschutz, S.; Lunderberg, E.; Meisel, Z.; Schatz, H.; Scott, M.; Stroberg, S. R.; Sullivan, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Campbell, C. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Cole, A. L.] Kalamazoo Coll, Dept Phys, Kalamazoo, MI 49006 USA. [Guess, C. J.] Univ Massachusetts, Dept Phys & Appl Phys, Lowell, MA 01854 USA. [Gupta, S.] Indian Inst Technol Ropar, Rupnagar 140001, Punjab, India. [Hitt, G. W.] Khalifa Univ Sci Technol & Res, Dept Appl Math & Sci, Abu Dhabi, U Arab Emirates. [Meharchand, R.] Los Alamos Natl Lab, Neutron & Nucl Sci Grp, Los Alamos, NM 87545 USA. [Perdikakis, G.; Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Valdez, L.] Orange High Sch, Orange, NJ 07050 USA. RP Noji, S (reprint author), Osaka Univ, Nucl Phys Res Ctr, Ibaraki, Osaka 5670047, Japan. EM noji@rcnp.osaka-u.ac.jp RI Perdikakis, Georgios/K-4525-2014; Gade, Alexandra/A-6850-2008; Zegers, Remco/A-6847-2008; Langer, Christoph/L-3422-2016 OI Perdikakis, Georgios/0000-0002-8539-8737; Gade, Alexandra/0000-0001-8825-0976; FU U.S. NSF Grant [PHY-08-22648, PHY-14-04442]; U.S. DOE Office of Science; NSF [PHY-11-02511]; DOE [DE-AC02-05CH11231] FX We thank all the staff at NSCL for their outstanding efforts and support. This work was supported by the U.S. NSF Grant No. PHY-08-22648 (Joint Institute for Nuclear Astrophysics) and PHY-14-04442. GRETINA was funded by the U.S. DOE Office of Science. Operation of the array at NSCL is supported by NSF under Cooperative Agreement No. PHY-11-02511 (NSCL) and by DOE under Grant No. DE-AC02-05CH11231 (LBNL). NR 62 TC 2 Z9 2 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 17 PY 2015 VL 92 IS 2 AR 024312 DI 10.1103/PhysRevC.92.024312 PG 9 WC Physics, Nuclear SC Physics GA CP2AI UT WOS:000359678800003 ER PT J AU Thersleff, T Rusz, J Rubino, S Hjorvarsson, B Ito, Y Zaluzec, NJ Leifer, K AF Thersleff, Thomas Rusz, Jan Rubino, Stefano Hjorvarsson, Bjorgvin Ito, Yasuo Zaluzec, Nestor J. Leifer, Klaus TI Quantitative analysis of magnetic spin and orbital moments from an oxidized iron (110) surface using electron magnetic circular dichroism SO SCIENTIFIC REPORTS LA English DT Article ID VERWEY TRANSITION; CHIRAL DICHROISM; EMCD EXPERIMENTS; MICROSCOPE; DIFFRACTION; BILAYER AB Understanding the ramifications of reduced crystalline symmetry on magnetic behavior is a critical step in improving our understanding of nanoscale and interfacial magnetism. However, investigations of such effects are often controversial largely due to the challenges inherent in directly correlating nanoscale stoichiometry and structure to magnetic behavior. Here, we describe how to use Transmission Electron Microscope (TEM) to obtain Electron Magnetic Circular Dichroism (EMCD) signals as a function of scattering angle to locally probe the magnetic behavior of thin oxide layers grown on an Fe (1 1 0) surface. Experiments and simulations both reveal a strong dependence of the magnetic orbital to spin ratio on its scattering vector in reciprocal space. We exploit this variation to extract the magnetic properties of the oxide cladding layer, showing that it locally may exhibit an enhanced orbital to spin moment ratio. This finding is supported here by both spatially and angularly resolved EMCD measurements, opening up the way for compelling investigations into how magnetic properties are affected by nanoscale features. C1 [Thersleff, Thomas; Rubino, Stefano] Uppsala Univ, Dept Engn Sci, Div Appl Mat, Uppsala, Sweden. [Rusz, Jan; Hjorvarsson, Bjorgvin; Leifer, Klaus] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Rubino, Stefano] Univ Oslo, Dept Phys, Oslo, Norway. [Ito, Yasuo] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Zaluzec, Nestor J.] Argonne Natl Lab, NanoSci & Technol Div, Electron Microscopy Ctr, Argonne, IL 60439 USA. RP Thersleff, T (reprint author), Uppsala Univ, Dept Engn Sci, Div Appl Mat, Uppsala, Sweden. EM thomas.thersleff@angstrom.uu.se; klaus.leifer@angstrom.uu.se RI Rubino, Stefano/I-4063-2012; Rusz, Jan/A-3324-2008; OI Rubino, Stefano/0000-0001-5738-0591; Rusz, Jan/0000-0002-0074-1349; Thersleff, Thomas/0000-0002-0999-3569; Leifer, Klaus/0000-0002-8360-1877; Hjorvarsson, Bjorgvin/0000-0003-1803-9467 FU STINT research grant [1G2009-2017]; Argonne National Laboratory, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX The authors acknowledge the STINT research grant (1G2009-2017). In addition, part of this study was accomplished in the Electron Microscopy Center at the Center for Nanoscale Materials of Argonne National Laboratory, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. J. R. and K. L. acknowledge the Swedish Research Council. K. L. also acknowledges the Knut and Alice Wallenberg Foundation while J. R. also acknowledges the Goran Gustafsson's Foundation and Swedish National Infrastructure for Computing (NSC center). Special thanks are also due to Paul Thomas at Gatan Inc. for providing the authors with an automated procedure to execute the high quality dark reference correction. NR 59 TC 8 Z9 8 U1 11 U2 43 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 17 PY 2015 VL 5 AR 13012 DI 10.1038/srep13012 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO9UQ UT WOS:000359521900001 PM 26278134 ER PT J AU Johnson, T Bozinoski, R Ye, JJ Sartor, G Zheng, JY Yang, J AF Johnson, Terry Bozinoski, Radoslav Ye, Jianjun Sartor, George Zheng, Jinyang Yang, Jian TI Thermal model development and validation for rapid filling of high pressure hydrogen tanks SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE High pressure hydrogen storage; Fast filling; Real gas equation; One-dimensional and 3D models ID CYLINDER; VESSELS; MASS AB This paper describes the development of thermal models for the filling of high pressure hydrogen tanks with experimental validation. Two models are presented; the first uses a one-dimensional, transient, network flow analysis code developed at Sandia National Labs, and the second uses the commercially available CFD analysis tool Fluent. These models were developed to help assess the safety of Type IV high pressure hydrogen tanks during the filling process. The primary concern for these tanks is due to the increased susceptibility to fatigue failure of the liner caused by the fill process. Therefore, a thorough understanding of temperature changes of the hydrogen gas and the heat transfer to the tank walls is essential. The effects of initial pressure, filling time, and fill procedure were investigated to quantify the ternperature change and verify the accuracy of the models. In this paper we show that the predictions of mass averaged gas temperature for the one and three-dimensional models compare well with the experiment and both can be used to make predictions for final mass delivery. Due to buoyancy and other three-dimensional effects, however, the maximum wall temperature cannot be predicted using one-dimensional tools alone which means that a three-dimensional analysis is required for a safety assessment of the system. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Johnson, Terry; Sartor, George] Sandia Natl Labs, Transportat Energy Ctr, Livermore, CA USA. [Bozinoski, Radoslav] Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. [Ye, Jianjun; Zheng, Jinyang; Yang, Jian] Zhejiang Univ, Inst Proc Equipment, Hangzhou 310003, Zhejiang, Peoples R China. RP Bozinoski, R (reprint author), Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. EM rbozino@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to acknowledge Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 23 TC 2 Z9 2 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD AUG 17 PY 2015 VL 40 IS 31 BP 9803 EP 9814 DI 10.1016/j.ijhydene.2015.05.157 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CN7PI UT WOS:000358626100019 ER PT J AU Pusateri, EN Morris, HE Nelson, EM Ji, W AF Pusateri, Elise N. Morris, Heidi E. Nelson, Eric M. Ji, Wei TI Determination of equilibrium electron temperature and times using an electron swarm model with BOLSIG plus calculated collision frequencies and rate coefficients SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE swarm model; electron collision frequency; electron energy distribution; electron temperature; electron cross sections; equilibrium ID CROSS-SECTIONS; TRANSPORT-COEFFICIENTS; ELECTROMAGNETIC PULSE; MOMENTUM-TRANSFER; IMPACT EXCITATION; ENERGY; AIR; PARAMETERS; IONIZATION; ATTACHMENT AB Electromagnetic pulse (EMP) events produce low-energy conduction electrons from Compton electron or photoelectron ionizations with air. It is important to understand how conduction electrons interact with air in order to accurately predict EMP evolution and propagation. An electron swarm model can be used to monitor the time evolution of conduction electrons in an environment characterized by electric field and pressure. Here a swarm model is developed that is based on the coupled ordinary differential equations (ODEs) described by Higgins et al. (1973), hereinafter HLO. The ODEs characterize the swarm electric field, electron temperature, electron number density, and drift velocity. Important swarm parameters, the momentum transfer collision frequency, energy transfer collision frequency, and ionization rate, are calculated and compared to the previously reported fitted functions given in HLO. These swarm parameters are found using BOLSIG+, a two term Boltzmann solver developed by Hagelaar and Pitchford (2005), which utilizes updated cross sections from the LXcat website created by Pancheshnyi et al. (2012). We validate the swarm model by comparing to experimental effective ionization coefficient data in Dutton (1975) and drift velocity data in Ruiz-Vargas et al. (2010). In addition, we report on electron equilibrium temperatures and times for a uniform electric field of 1StatV/cm for atmospheric heights from 0 to 40km. It is shown that the equilibrium temperature and time are sensitive to the modifications in the collision frequencies and ionization rate based on the updated electron interaction cross sections. C1 [Pusateri, Elise N.; Ji, Wei] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA. [Pusateri, Elise N.; Morris, Heidi E.; Nelson, Eric M.] Los Alamos Natl Lab, X Div, Los Alamos, NM USA. RP Pusateri, EN (reprint author), Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA. EM elisep@lanl.gov; jiw2@rpi.edu OI Pusateri, Elise/0000-0002-8345-2429; Ji, Wei/0000-0001-9832-254X FU Los Alamos National Laboratory; Rensselaer Polytechnic Institute FX The electron scattering cross-section data used in this research are from the Phelps database contributed by the LXcat workgroup (www.lxcat.net). The first author would like to acknowledge the Graduate Research Assistantship support from Los Alamos National Laboratory and Rensselaer Polytechnic Institute. NR 48 TC 1 Z9 1 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2015 VL 120 IS 15 BP 7300 EP 7315 DI 10.1002/2015JD023100 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CQ3KV UT WOS:000360501900002 ER PT J AU Kulkarni, G Zhang, K Zhao, C Nandasiri, M Shutthanandan, V Liu, XH Fast, J Berg, L AF Kulkarni, Gourihar Zhang, Kai Zhao, Chun Nandasiri, Manjula Shutthanandan, Vaithiyalingam Liu, Xiaohong Fast, Jerome Berg, Larry TI Ice formation on nitric acid-coated dust particles: Laboratory and modeling studies SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE ice nucleation; mineral dust; ice clouds; XPS; single-column model ID MINERAL DUST; NUCLEATION PROPERTIES; MASS-BALANCE; DESERT DUST; AEROSOL; IMPACT; CLIMATE; SULFATE; NUCLEI; SIZE AB Changes in the ice nucleation characteristics of atmospherically relevant mineral dust particles caused by a coating of nitric acid are not well understood. Further, the atmospheric implications of dust coatings on ice-cloud properties under different assumptions of primary ice nucleation mechanisms are unknown. We investigated the ice nucleation ability of Arizona Test Dust, illite, K-feldspar, and quartz as a function of temperature (-25 degrees C to -30 degrees C) and relative humidity with respect to water (75% to 110%). The particles (bare or nitric acid coated) were size selected at 250 nm, and the fraction of particles nucleating ice at various temperature and saturation conditions was determined. All of the dust species nucleated ice at subsaturated conditions, although the coated particles (except quartz) showed a reduction in their ice nucleation ability relative to bare particles. However, at supersaturated conditions, bare and coated particles had nearly equivalent ice nucleation characteristics. The results of a single-column model showed that simulated ice crystal number concentrations are mostly dependent upon the coated particle fraction, primary ice nucleation mechanisms, and competition among ice nucleation mechanisms to nucleate ice. In general, coatings were observed to modify ice-cloud properties, and the complexity of ice-cloud and mixed-phase-cloud evolution when different primary ice nucleation mechanisms compete for fixed water vapor budgets was supported. C1 [Kulkarni, Gourihar; Zhang, Kai; Zhao, Chun; Fast, Jerome; Berg, Larry] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Nandasiri, Manjula; Shutthanandan, Vaithiyalingam] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Liu, Xiaohong] Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA. RP Kulkarni, G (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM Gourihar.Kulkarni@pnnl.gov RI Liu, Xiaohong/E-9304-2011; Zhao, Chun/A-2581-2012; Zhang, Kai/F-8415-2010 OI Liu, Xiaohong/0000-0002-3994-5955; Zhao, Chun/0000-0003-4693-7213; Zhang, Kai/0000-0003-0457-6368 FU Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program; U.S. DOE by Battelle Memorial Institute [DE-AC05-76RL0 1830] FX The work was supported by the Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program. We are grateful for the technical support provided by Danny Nelson. We thank three anonymous reviewers for their assistance in evaluating this paper. This research was performed at the Atmospheric Measurement Laboratory, an atmospheric sciences laboratory at Pacific Northwest National Laboratory (PNNL). XPS analysis was performed in Environmental Molecular Sciences Laboratory (EMSL), which is a national scientific user facility located at PNNL, and was supported by the Laboratory Directed Research and Development program of PNNL as a part of Chemical Imaging Initiative. Data used to produce the results of this paper are available upon request. Please request any data or additional information using Gourihar.Kulkarni@pnnl.gov address. PNNL is operated by the U.S. DOE by Battelle Memorial Institute under contract DE-AC05-76RL0 1830. NR 64 TC 3 Z9 3 U1 8 U2 33 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2015 VL 120 IS 15 BP 7682 EP 7698 DI 10.1002/2014JD022637 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CQ3KV UT WOS:000360501900024 ER PT J AU Titova, EE Kozelov, BV Demekhov, AG Manninen, J Santolik, O Kletzing, CA Reeves, G AF Titova, E. E. Kozelov, B. V. Demekhov, A. G. Manninen, J. Santolik, O. Kletzing, C. A. Reeves, G. TI Identification of the source of quasiperiodic VLF emissions using ground-based and Van Allen Probes satellite observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE VLF waves; quasiperiodic emissions; Van Allen Probes; energetic electrons ID ELF/VLF WAVE EMISSIONS; ELECTRON-PRECIPITATION; MAGNETIC PULSATIONS; AURORAL PULSATIONS; CYCLOTRON MASER; MAGNETOSPHERE; MODULATION; MECHANISM; FREQUENCY AB We report on simultaneous spacecraft and ground-based observations of quasiperiodic VLF emissions and related energetic-electron dynamics. Quasiperiodic emissions in the frequency range 2-6kHz were observed during a substorm on 25 January 2013 by Van Allen Probe-A and a ground-based station in the Northern Finland. The spacecraft detected the VLF signals near the geomagnetic equator in the night sector at L=3.0-4.2 when it was inside the plasmasphere. During the satellite motion toward higher latitudes, the time interval between quasiperiodic elements decreased from 6min to 3min. We find one-to-one correspondence between the quasiperiodic elements detected by Van Allen Probe-A and on the ground, which indicates the temporal nature of the observed variation in the time interval between quasiperiodic elements. Multi?omponent measurements of the wave electric and magnetic fields by the Van Allen Probe-A show that the quasiperiodic emissions were almost circularly right-hand polarized whistler mode waves and had predominantly small (below 30 degrees) wave vector angles with respect to the magnetic field. In the probable source region of these signals (L about 4), we observed synchronous variations of electron distribution function at energies of 10-20keV and the quasiperiodic elements. In the pause between the quasiperiodic elements pitch angle distribution of these electrons had a maximum near 90 degrees, while they become more isotropic during the development of quasiperiodic elements. The parallel energies of the electrons for which the data suggest direct evidence of the wave-particle interactions is in a reasonable agreement with the estimated cyclotron resonance energy for the observed waves. C1 [Titova, E. E.; Kozelov, B. V.; Demekhov, A. G.] RAS, Polar Geophys Inst, Kola Sci Ctr, Apatity, Russia. [Titova, E. E.] RAS, Space Res Inst, Moscow 117901, Russia. [Demekhov, A. G.] RAS, Inst Appl Phys, Nizhnii Novgorod, Russia. [Manninen, J.] Sodankyla Geophys Observ, Sodankyla, Finland. [Santolik, O.] ASCR, Inst Atmospher Phys, Prague, Czech Republic. [Santolik, O.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Reeves, G.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Demekhov, AG (reprint author), RAS, Polar Geophys Inst, Kola Sci Ctr, Apatity, Russia. EM andrei@appl.sci-nnov.ru RI Santolik, Ondrej/F-7766-2014; Reeves, Geoffrey/E-8101-2011; Demekhov, Andrei/F-1444-2016; Kozelov, Boris/N-2731-2013; Titova, Elena/R-2613-2016; OI Reeves, Geoffrey/0000-0002-7985-8098; Demekhov, Andrei/0000-0002-8062-8492; Kozelov, Boris/0000-0003-2738-2443; Titova, Elena/0000-0001-7622-3452; Kletzing, Craig/0000-0002-4136-3348 FU Russian Science Foundation [15-12-20005]; Premium Academiae; JHU/APL contract under NASA Prime contract [921647, NAS5-01072]; [P209-11-2280]; [LH14010] FX Van Allen Probe data used in this paper can be found in the EMFISIS (http://emfisis.physics.uiowa.edu/data/index) and ECT (http://www.rbsp-ect.lanl.gov/rbsp_ect.php) archives. The ground-based data for this paper are available on request from Sodankyla Geophysical Observatory (contact J. Manninen). E.T., B.K., and A.D. thank the Russian Science Foundation for funding the work on this paper under grant 15-12-20005 and the Sodankyla Geophysical Observatory for hosting their visits during which the data for this study were selected. O.S. acknowledges funding from grants P209-11-2280, LH14010, and Premium Academiae. The work of C.K. was partially supported by JHU/APL contract 921647 under NASA Prime contract NAS5-01072. Processing and analysis of data from the RBSP-ECT (Energetic Particle, Composition, and Thermal Plasma) instruments was supported by funding under NASA Prime contract NAS5-01072. NR 37 TC 8 Z9 8 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2015 VL 42 IS 15 BP 6137 EP 6145 DI 10.1002/2015GL064911 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CQ2FM UT WOS:000360414900002 ER PT J AU Dai, L Wang, C Duan, SP He, ZH Wygant, JR Cattell, CA Tao, X Su, ZP Kletzing, C Baker, DN Li, XL Malaspina, D Blake, JB Fennell, J Claudepierre, S Turner, DL Reeves, GD Funsten, HO Spence, HE Angelopoulos, V Fruehauff, D Chen, LJ Thaller, S Breneman, A Tang, XW AF Dai, Lei Wang, Chi Duan, Suping He, Zhaohai Wygant, John R. Cattell, Cynthia A. Tao, Xin Su, Zhenpeng Kletzing, Craig Baker, Daniel N. Li, Xinlin Malaspina, David Blake, J. Bernard Fennell, Joseph Claudepierre, Seth Turner, Drew L. Reeves, Geoffrey D. Funsten, Herbert O. Spence, Harlan E. Angelopoulos, Vassilis Fruehauff, Dennis Chen, Lunjin Thaller, Scott Breneman, Aaron Tang, Xiangwei TI Near-Earth injection of MeV electrons associated with intense dipolarization electric fields: Van Allen Probes observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE substorm injection; substorm dipolarization; radiation belt electrons; electric fields ID ENERGETIC PARTICLE INJECTIONS; RADIATION BELT; SUBSTORM INJECTION; RELATIVISTIC ELECTRONS; GEOSYNCHRONOUS ORBIT; INNER MAGNETOSPHERE; PLASMA SHEET; DRIFT ECHOES; MARCH 24; SIMULATION AB Substorms generally inject tens to hundreds of keV electrons, but intense substorm electric fields have been shown to inject MeV electrons as well. An intriguing question is whether such MeVelectron injections can populate the outer radiation belt. Here we present observations of a substorm injection of MeV electrons into the inner magnetosphere. In the premidnight sector at L approximate to 5.5, Van Allen Probes (Radiation Belt Storm Probes)-A observed a large dipolarization electric field (50mV/m) over approximate to 40s and a dispersionless injection of electrons up to approximate to 3MeV. Pitch angle observations indicated betatron acceleration of MeV electrons at the dipolarization front. Corresponding signals of MeV electron injection were observed at LANL-GEO, THEMIS-D, and GOES at geosynchronous altitude. Through a series of dipolarizations, the injections increased the MeV electron phase space density by 1 order of magnitude in less than 3h in the outer radiation belt (L > 4.8). Our observations provide evidence that deep injections can supply significant MeV electrons. C1 [Dai, Lei; Wang, Chi; Duan, Suping; He, Zhaohai] Chinese Acad Sci, Natl Space Sci Ctr, State Key Lab Space Weather, Beijing, Peoples R China. [Dai, Lei; Wygant, John R.; Cattell, Cynthia A.; Thaller, Scott; Breneman, Aaron; Tang, Xiangwei] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Tao, Xin; Su, Zhenpeng] Univ Sci & Technol China, Dept Geophys & Planetary Sci, Hefei 230026, Peoples R China. [Kletzing, Craig] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Baker, Daniel N.; Li, Xinlin; Malaspina, David] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. [Blake, J. Bernard; Fennell, Joseph; Claudepierre, Seth; Turner, Drew L.] Aerosp Corp, Dept Space Sci, Los Angeles, CA 90009 USA. [Reeves, Geoffrey D.; Funsten, Herbert O.] Los Alamos Natl Lab, Los Alamos, NM USA. [Spence, Harlan E.] Univ New Hampshire, Inst Earth Oceans & Space, Dept Phys, Durham, NH 03824 USA. [Angelopoulos, Vassilis] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA USA. [Angelopoulos, Vassilis] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90024 USA. [Fruehauff, Dennis] Braunschweig Univ Technol, Inst Geophys & Extraterr Phys, Braunschweig, Germany. [Chen, Lunjin] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. RP Dai, L (reprint author), Chinese Acad Sci, Natl Space Sci Ctr, State Key Lab Space Weather, Beijing, Peoples R China. EM ldai@spaceweather.ac.cn RI Reeves, Geoffrey/E-8101-2011; Su, Zhenpeng/E-1641-2011; OI Reeves, Geoffrey/0000-0002-7985-8098; Cattell, Cynthia/0000-0002-3805-320X; Su, Zhenpeng/0000-0001-5577-4538; Kletzing, Craig/0000-0002-4136-3348; Funsten, Herbert/0000-0002-6817-1039; Duan, Suping/0000-0002-4835-6888 FU NNSFC [41231067]; State Key Laboratories of China; APL for the development of RBSP/EFW; JHU/APL [921647]; NASA grant [NNX15AF55G]; International Space Science Institute's (ISSI) International Teams program FX This work was supported by NNSFC grant 41231067 and in part by the Specialized Research Fund for State Key Laboratories of China. Work at UMN was supported by a contract from APL for the development of RBSP/EFW. EMFISIS is supported by a JHU/APL contract 921647. L.C. would like to acknowledge the support of the NASA grant NNX15AF55G. D.L.T., G.D.R., and X.L. are thankful for the support from the International Space Science Institute's (ISSI) International Teams program. L.D. greatly appreciates Judy Hohl from UCLA for editorial help. The RBSP EMFISIS data are available at . The RBSP EFW data are available at . The RBSP ECT data are available at . THEMIS data are available at . LANL-GEO data are provided by Geoffrey D. Reeves. GOES data are available at . The OMNI data are available at CDAWeb. The SYM-H data are provided by the World Data Center for Geomagnetism, Kyoto. NR 56 TC 5 Z9 6 U1 6 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2015 VL 42 IS 15 BP 6170 EP 6179 DI 10.1002/2015GL064955 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CQ2FM UT WOS:000360414900006 ER PT J AU Dai, S Cha, JH Rosenbaum, EJ Zhang, W Seol, Y AF Dai, Sheng Cha, Jong-Ho Rosenbaum, Eilis J. Zhang, Wu Seol, Yongkoo TI Thermal conductivity measurements in unsaturated hydrate-bearing sediments SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE methane hydrate; hydrate-bearing sediments; thermal conductivity; single-sided TPS; gas production; analytical model ID METHANE-HYDRATE; DIFFUSIVITY MEASUREMENTS; TETRAHYDROFURAN HYDRATE; VARIATIONAL APPROACH; MULTIPHASE MATERIALS; CLATHRATE; SIMULATION; MIXTURES; MEDIA; HEAT AB Current database on the thermal properties of hydrate-bearing sediments remains limited and has not been able to capture their consequential changes during gas production where vigorous phase changes occur in this unsaturated system. This study uses the transient plane source (TPS) technique to measure the thermal conductivity of methane hydrate-bearing sediments with various hydrate/water/gas saturations. We propose a simplified method to obtain thermal properties from single-sided TPS signatures. Results reveal that both volume fraction and distribution of the pore constituents govern the thermal conductivity of unsaturated specimens. Thermal conductivity hysteresis is observed due to water redistribution and fabric change caused by hydrate formation and dissociation. Measured thermal conductivity increases evidently when hydrate saturation S-h>30-40%, shifting upward from the geometric mean model prediction to a Pythagorean mixing model. These observations envisage a significant drop in sediment thermal conductivity when residual hydrate/water saturation falls below similar to 40%, hindering further gas production. C1 [Dai, Sheng; Cha, Jong-Ho; Rosenbaum, Eilis J.; Zhang, Wu; Seol, Yongkoo] USDA, Natl Energy Technol Lab, Morgantown, WV 26505 USA. RP Seol, Y (reprint author), USDA, Natl Energy Technol Lab, Morgantown, WV 26505 USA. EM Yongkoo.Seol@netl.doe.gov OI Dai, Sheng/0000-0003-0221-3993 FU ORISE fellowship - NETL/DOE FX TThis study benefitted from the technical support of Karl Jarvis (AECOM). S.D. and J.H.C. are supported by the ORISE fellowship granted by NETL/DOE. NR 34 TC 1 Z9 1 U1 6 U2 24 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2015 VL 42 IS 15 BP 6295 EP 6305 DI 10.1002/2015GL064492 PG 11 WC Geosciences, Multidisciplinary SC Geology GA CQ2FM UT WOS:000360414900021 ER PT J AU Li, X Chomvong, K Yu, VY Liang, JM Lin, YP Cate, JHD AF Li, Xin Chomvong, Kulika Yu, Vivian Yaci Liang, Julie M. Lin, Yuping Cate, Jamie H. D. TI Cellobionic acid utilization: from Neurospora crassa to Saccharomyces cerevisiae SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Aldonic acid; LPMO; AA9; beta-glucosidase; Phosphorylase; Transporter; Metabolic engineering; Biofuels; Cellobionic acid ID CELLODEXTRIN TRANSPORTERS; CELLULOSE DEGRADATION; CRYSTAL-STRUCTURE; PHOSPHORYLASE; FERMENTATION; YEAST; SEARCH; XYLOSE AB Background: Economical production of fuels and chemicals from plant biomass requires the efficient use of sugars derived from the plant cell wall. Neurospora crassa, a model lignocellulosic degrading fungus, is capable of breaking down the complex structure of the plant cell wall. In addition to cellulases and hemicellulases, N. crassa secretes lytic polysaccharide monooxygenases (LPMOs), which cleave cellulose by generating oxidized sugars-particularly aldonic acids. However, the strategies N. crassa employs to utilize these sugars are unknown. Results: We identified an aldonic acid utilization pathway in N. crassa, comprised of an extracellular hydrolase (NCU08755), cellobionic acid transporter (CBT-1, NCU05853) and cellobionic acid phosphorylase (CAP, NCU09425). Extracellular cellobionic acid could be imported directly by CBT-1 or cleaved to gluconic acid and glucose by a beta-glucosidase (NCU08755) outside the cells. Intracellular cellobionic acid was further cleaved to glucose 1-phosphate and gluconic acid by CAP. However, it remains unclear how N. crassa utilizes extracellular gluconic acid. The aldonic acid pathway was successfully implemented in Saccharomyces cerevisiae when N. crassa gluconokinase was coexpressed, resulting in cellobionic acid consumption in both aerobic and anaerobic conditions. Conclusions: We successfully identified a branched aldonic acid utilization pathway in N. crassa and transferred its essential components into S. cerevisiae, a robust industrial microorganism. C1 [Li, Xin; Yu, Vivian Yaci; Lin, Yuping; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Chomvong, Kulika] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Liang, Julie M.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM jcate@lbl.gov FU Energy Biosciences Institute FX This work was supported by funding from the Energy Biosciences Institute to JHDC. The authors thank Dr. Soo Rin Kim for generously providing S. cerevisiae SR8. NR 34 TC 4 Z9 4 U1 12 U2 43 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 16 PY 2015 VL 8 AR 120 DI 10.1186/s13068-015-0303-2 PG 9 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CP7FT UT WOS:000360053300001 PM 26279678 ER PT J AU Kilaru, A Cao, X Dabbs, PB Sung, HJ Rahman, MM Thrower, N Zynda, G Podicheti, R Ibarra-Laclette, E Herrera-Estrella, L Mockaitis, K Ohlrogge, JB AF Kilaru, Aruna Cao, Xia Dabbs, Parker B. Sung, Ha-Jung Rahman, Md Mahbubur Thrower, Nicholas Zynda, Greg Podicheti, Ram Ibarra-Laclette, Enrique Herrera-Estrella, Luis Mockaitis, Keithanne Ohlrogge, John B. TI Oil biosynthesis in a basal angiosperm: transcriptome analysis of Persea Americana mesocarp SO BMC PLANT BIOLOGY LA English DT Article ID ACYL-CARRIER PROTEIN; FATTY-ACID BIOSYNTHESIS; BRASSICA-NAPUS EMBRYOS; COENZYME-A SYNTHETASE; ARABIDOPSIS-THALIANA; AVOCADO FRUIT; DIACYLGLYCEROL ACYLTRANSFERASE; TRIACYLGLYCEROL SYNTHESIS; DEVELOPING OILSEEDS; (+)-ABSCISIC ACID AB Background: The mechanism by which plants synthesize and store high amounts of triacylglycerols (TAG) in tissues other than seeds is not well understood. The comprehension of controls for carbon partitioning and oil accumulation in nonseed tissues is essential to generate oil-rich biomass in perennial bioenergy crops. Persea americana (avocado), a basal angiosperm with unique features that are ancestral to most flowering plants, stores similar to 70 % TAG per dry weight in its mesocarp, a nonseed tissue. Transcriptome analyses of select pathways, from generation of pyruvate and leading up to TAG accumulation, in mesocarp tissues of avocado was conducted and compared with that of oil-rich monocot (oil palm) and dicot (rapeseed and castor) tissues to identify tissue-and species-specific regulation and biosynthesis of TAG in plants. Results: RNA-Seq analyses of select lipid metabolic pathways of avocado mesocarp revealed patterns similar to that of other oil-rich species. However, only some predominant orthologs of the fatty acid biosynthetic pathway genes in this basal angiosperm were similar to those of monocots and dicots. The accumulation of TAG, rich in oleic acid, was associated with higher transcript levels for a putative stearoyl-ACP desaturase and endoplasmic reticulum (ER)-associated acyl-CoA synthetases, during fruit development. Gene expression levels for enzymes involved in terminal steps to TAG biosynthesis in the ER further indicated that both acyl-CoA-dependent and -independent mechanisms might play a role in TAG assembly, depending on the developmental stage of the fruit. Furthermore, in addition to the expression of an ortholog of WRINKLED1 (WRI1), a regulator of fatty acid biosynthesis, high transcript levels for WRI2-like and WRI3-like suggest a role for additional transcription factors in nonseed oil accumulation. Plastid pyruvate necessary for fatty acid synthesis is likely driven by the upregulation of genes involved in glycolysis and transport of its intermediates. Together, a comparative transcriptome analyses for storage oil biosynthesis in diverse plants and tissues suggested that several distinct and conserved features in this basal angiosperm species might contribute towards its rich TAG content. Conclusions: Our work represents a comprehensive transcriptome resource for a basal angiosperm species and provides insight into their lipid metabolism in mesocarp tissues. Furthermore, comparison of the transcriptome of oil-rich mesocarp of avocado, with oil-rich seed and nonseed tissues of monocot and dicot species, revealed lipid gene orthologs that are highly conserved during evolution. The orthologs that are distinctively expressed in oil-rich mesocarp tissues of this basal angiosperm, such as WRI2, ER-associated acyl-CoA synthetases, and lipid-droplet associated proteins were also identified. This study provides a foundation for future investigations to increase oil-content and has implications for metabolic engineering to enhance storage oil content in nonseed tissues of diverse species. C1 [Kilaru, Aruna; Dabbs, Parker B.; Sung, Ha-Jung; Rahman, Md Mahbubur] E Tennessee State Univ, Dept Biol Sci, Johnson City, TN 37614 USA. [Kilaru, Aruna; Rahman, Md Mahbubur] E Tennessee State Univ, Dept Biomed Sci, Johnson City, TN 37614 USA. [Kilaru, Aruna; Cao, Xia; Thrower, Nicholas; Ohlrogge, John B.] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Cao, Xia] Bayer CropSci, Morrisville, NC 27560 USA. [Zynda, Greg; Podicheti, Ram] Indiana Univ, Sch Informat & Comp, Bloomington, IN 47408 USA. [Ibarra-Laclette, Enrique; Herrera-Estrella, Luis] IPN, Ctr Invest & Estudios Avanzados, Unidad Genom Avanzada UGA, Lab Nacl Genom Biodiversidad Langebio, Guanajuato 36500, Mexico. [Ibarra-Laclette, Enrique] Inst Ecol AC, Red Estudios Mol Avanzados, Xalapa 91070, Veracruz, Mexico. [Mockaitis, Keithanne] Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. [Ohlrogge, John B.] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. RP Kilaru, A (reprint author), E Tennessee State Univ, Dept Biol Sci, Johnson City, TN 37614 USA. EM kilaru@etsu.edu OI Kilaru, Aruna/0000-0003-1270-2299 FU DOE Great Lakes Bioenergy Research Center, Bayer CropScience [DE-FC02-07ER64494]; Research and Development Committee, East Tennessee State University; Sigma Xi GIAR Award; METACyt Initiative of Indiana University from the Lilly Endowment, Inc. FX We thank Mary Lu Arpaia, University of California at Riverside, for providing avocado fruits, and the staff of Research Technology Support Facility at Michigan State University, and Peter Denholf at Bayer Cropscience, for advice on sequence analysis. This work was supported by the DOE Great Lakes Bioenergy Research Center Cooperative Agreement (DE-FC02-07ER64494), Bayer CropScience. AK was supported in part by major and minor grants from Research and Development Committee, East Tennessee State University. HS and PD received Sigma Xi GIAR Award. RP, GZ and KM were supported in part by the METACyt Initiative of Indiana University, funded in part through a major grant from the Lilly Endowment, Inc. NR 92 TC 13 Z9 13 U1 5 U2 35 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2229 J9 BMC PLANT BIOL JI BMC Plant Biol. PD AUG 16 PY 2015 VL 15 AR 203 DI 10.1186/s12870-015-0586-2 PG 18 WC Plant Sciences SC Plant Sciences GA CO9TH UT WOS:000359518400002 PM 26276496 ER PT J AU Shetty, AR de Gannes, V Obi, CC Lucas, S Lapidus, A Cheng, JF Goodwin, LA Pitluck, S Peters, L Mikhailova, N Teshima, H Han, C Tapia, R Land, M Hauser, LJ Kyrpides, N Ivanova, N Pagani, I Chain, PSG Denef, VJ Woyke, T Hickey, WJ AF Shetty, Ameesha R. de Gannes, Vidya Obi, Chioma C. Lucas, Susan Lapidus, Alla Cheng, Jan-Fang Goodwin, Lynne A. Pitluck, Samuel Peters, Linda Mikhailova, Natalia Teshima, Hazuki Han, Cliff Tapia, Roxanne Land, Miriam Hauser, Loren J. Kyrpides, Nikos Ivanova, Natalia Pagani, Ioanna Chain, Patrick S. G. Denef, Vincent J. Woyke, Tanya Hickey, William J. TI Complete genome sequence of the phenanthrene-degrading soil bacterium Delftia acidovorans Cs 1-4 SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Delftio acidovorans Cs1-4; Genome; phn island; Phenanthrene; polycyclic aromatic hydrocarbons; Nanopods ID METABOLISM; PATHWAY; SYSTEM; FAMILY AB Polycyclic aromatic hydrocarbons (PAH) are ubiquitous environmental pollutants and microbial biodegradation is an important means of remediation of PAH-contaminated soil. Delltio acidovorons Cs1-4 (formerly Delftia sp. Cs1-4) was isolated by using phenanthrene as the sole carbon source from PAH contaminated soil in Wisconsin. Its full genome sequence was determined to gain insights into a mechanisms underlying biodegradation of PAH. Three genomic libraries were constructed and sequenced: an Illumina GAii shotgun library (916,416,493 reads), a 454 Titanium standard library (770,171 reads) and one paired end 454 library (average insert size of 8 kb, 508,092 reads). The initial assembly contained 40 contigs in two scaffolds. The 454 Titanium standard data and the 454 paired end data were assembled together and the consensus sequences were computationally shredded into 2 kb overlapping shreds. Illumina sequencing data was assembled, and the consensus sequence was computationally shredded into 1.5 kb overlapping shreds. Gaps between contigs were closed by editing in Consed, by PCR and by Bubble PCR primer walks. A total of 182 additional reactions were needed to close gaps and to raise the quality of the finished sequence. The final assembly is based on 253.3 Mb of 454 draft data (averaging 38.4 X coverage) and 5902 Mb of Illumina draft data (averaging 89.4 X coverage). The genome of strain Cs1-4 consists of a single circular chromosome of 6,685,842 bp (66.7 %G+C) containing 6,028 predicted genes; 5,931 of these genes were protein encoding and 4,425 gene products were assigned to a putative function. Genes encoding phenanthrene degradation were localized to a 232 kb genomic island (ternned the phn island), which contained near its 3' end a bacteriophage P4 like integrase, an enzyme often associated with chromosomal integration of mobile genetic elements. Other biodegradation pathways reconstructed from the genome sequence included: benzoate (by the acetyl-CoA pathway), styrene, nicotinic acid (by the maleamate pathway) and the pesticides Dicamba and Fenitrothion. Determination of the complete genome sequence of D. acidovorons Cs1-4 has provided new insights the microbial mechanisms of PAH biodegradation that may shape the process in the environment. C1 [Shetty, Ameesha R.; Hickey, William J.] Univ Wisconsin, Dept Soil Sci, ON Allen Lab Soil Microbiol, Madison, WI 53706 USA. [de Gannes, Vidya] Univ W Indies, Dept Food Prod, St Augustine, Trinid & Tobago. [Obi, Chioma C.] Univ Lagos, Dept Microbiol, Lagos, Nigeria. [Lucas, Susan; Cheng, Jan-Fang; Pitluck, Samuel; Peters, Linda; Mikhailova, Natalia; Kyrpides, Nikos; Ivanova, Natalia; Pagani, Ioanna; Woyke, Tanya] DOE Joint Genome Inst, Walnut Creek, CA USA. [Lapidus, Alla] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg, Russia. [Goodwin, Lynne A.; Teshima, Hazuki; Han, Cliff; Tapia, Roxanne; Chain, Patrick S. G.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Land, Miriam; Hauser, Loren J.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Denef, Vincent J.] Univ Michigan, Dept Ecol & Evolutionary Biol, Ann Arbor, MI 48109 USA. RP Hickey, WJ (reprint author), Univ Wisconsin, Dept Soil Sci, ON Allen Lab Soil Microbiol, Madison, WI 53706 USA. EM wjhickey@wisc.edu RI Land, Miriam/A-6200-2011; Kyrpides, Nikos/A-6305-2014; OI Land, Miriam/0000-0001-7102-0031; Ivanova, Natalia/0000-0002-5802-9485; Kyrpides, Nikos/0000-0002-6131-0462; Chain, Patrick/0000-0003-3949-3634 FU U.S. Department of Energy, Office of Science [DE-AC02-05CH11231]; O.N. Allen Professorship in Soil Microbiology FX Sequencing, assembly and computational annotation of the D. acidovorans Cs1-4 genome was done by U.S Department of Energy, Joint Genome Institute through the Community Sequendng Project (CSP795673 to Wliiam J. Hickey). lhe Wolk conducted by the U.S. Department of Energy, Joint Genome Institute was supported by U.S. Department of Energy, Office of Science under contract No. DE-AC02-05CH11231. Research in the cor-espondng author's laboratory genomic and phenotypic cllaracteristics of D. acidovorons Cs1-4 was supported by the O.N. Allen Professorship in Soil Microbiology (to William J. Hickey). NR 32 TC 2 Z9 2 U1 2 U2 17 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 15 PY 2015 VL 10 AR 55 DI 10.1186/s40793-015-0041-x PG 10 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NY UT WOS:000367992200001 PM 26380642 ER PT J AU Ortiz-Bernardin, A Puso, MA Sukumar, N AF Ortiz-Bernardin, A. Puso, M. A. Sukumar, N. TI Improved robustness for nearly-incompressible large deformation meshfree simulations on Delaunay tessellations SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING LA English DT Article DE Hyperelasticity; Large deformations; Meshfree methods; Maximum-entropy approximation; F-bar method; Delaunay meshes ID FINITE-ELEMENT FORMULATION; CONFORMING NODAL INTEGRATION; FREE GALERKIN METHOD; NUMERICAL-INTEGRATION; LAGRANGIAN-MULTIPLIERS; TETRAHEDRAL ELEMENT; LINEAR TRIANGLES; ELASTICITY; SOLIDS; APPROXIMATION AB A displacement-based Galerkin meshfree method for large deformation analysis of nearly-incompressible elastic solids is presented. Nodal discretization of the domain is defined by a Delaunay tessellation (three-node triangles and four-node tetrahedra), which is used to form the meshfree basis functions and to numerically integrate the weak form integrals. In the proposed approach for nearly-incompressible solids, a volume-averaged nodal projection operator is constructed to average the dilatational constraint at a node from the displacement field of surrounding nodes. The nodal dilatational constraint is then projected onto the linear approximation space. The displacement field is constructed on the linear space and enriched with bubble-like meshfree basis functions for stability. The new procedure leads to a displacement-based formulation that is similar to F-bar methodologies in finite elements and isogeometric analysis. We adopt maximum-entropy meshfree basis functions, and the performance of the meshfree method is demonstrated on benchmark problems using structured and unstructured background meshes in two and three dimensions. The nonlinear simulations reveal that the proposed methodology provides improved robustness for nearlyincompressible large deformation analysis on Delaunay meshes. (C) 2015 Elsevier BV. All rights reserved. C1 [Ortiz-Bernardin, A.] Univ Chile, Dept Mech Engn, Santiago 8370456, Chile. [Puso, M. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Sukumar, N.] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA. RP Ortiz-Bernardin, A (reprint author), Univ Chile, Dept Mech Engn, Av Beauchef 851, Santiago 8370456, Chile. EM aortizb@ing.uchile.cl RI Sukumar, N/B-1660-2008; Ortiz-Bernardin, Alejandro/B-2660-2009 OI Ortiz-Bernardin, Alejandro/0000-0001-9221-2470 FU Chilean National Fund for Scientific and Technological Development (Fondecyt) [11110389]; U.S. National Science Foundation [CMMI-1334783] FX AOB acknowledges the research support of the Chilean National Fund for Scientific and Technological Development (Fondecyt) through Grant No. 11110389. NS gratefully acknowledges the research support of the U.S. National Science Foundation through contract grant CMMI-1334783 to the University of California at Davis. NR 53 TC 3 Z9 3 U1 2 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0045-7825 EI 1879-2138 J9 COMPUT METHOD APPL M JI Comput. Meth. Appl. Mech. Eng. PD AUG 15 PY 2015 VL 293 BP 348 EP 374 DI 10.1016/j.cma.2015.05.009 PG 27 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA CR6RV UT WOS:000361475900017 ER PT J AU Wang, Y Du, ZD Park, YS Chen, C Zhang, X Pan, L AF Wang, Yuan Du, Zhidong Park, Yongshik Chen, Chen Zhang, Xiang Pan, Liang TI Y Quasi-3D plasmonic coupling scheme for near-field optical lithography and imaging SO OPTICS LETTERS LA English DT Article ID SUBWAVELENGTH APERTURE; MICROSCOPY; RESOLUTION; PROBES; LIGHT; TRANSMISSION; OPTIMIZATION; DIFFRACTION AB Near-field optical imaging and lithography rely on achieving both high resolution and efficient coupling. Particularly conventional near-field scanning optical microscopy (NSOM) suffers from the trade-off between resolution and efficiency. Planar plasmonic lens schemes can partially solve this issue utilizing plasmonic resonances, but the performance is not robust over a large range of sample materials. In this work we show a novel quasi-3D plasmonic scheme to focus light into the extreme subwavelength region in the near field with an efficiency orders higher than NSOM. The superb performance comes from the strong coupling between the localized mode with an off-plane E-field component and the sample being processed. Our scheme can efficiently focus light to a spot with a diameter down to 1/20 of its wavelength, and the coupling efficiency can be as high as 10%. Theoretically, we demonstrate that the FWHM of the focus spot can be 7 nm with an enhancement of about 800 at the UV region. The focusing performance is constantly good over a large variety of materials and the illumination and collection imaging scheme has been demonstrated by simulation. An example design of this quasi-3D coupling scheme is fabricated and its imaging performance is characterized by the apertureless optical near-field measurement. The high coupling efficiency at extreme subwavelength resolution of this quasi-3D coupling scheme opens the door to many applications, such as optical lithography, nanoscale imaging, heat-assisted magnetic recording, plasmon-enhanced Raman spectroscopy, etc. (C) 2015 Optical Society of America C1 [Wang, Yuan; Park, Yongshik; Zhang, Xiang; Pan, Liang] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Du, Zhidong; Chen, Chen; Pan, Liang] Purdue Univ, Birck Nanotechnol Ctr, Sch Mech Engn, W Lafayette, IN 47906 USA. [Zhang, Xiang] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Zhang, Xiang] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. RP Pan, L (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM liangpan@purdue.edu RI Wang, Yuan/F-7211-2011; Zhang, Xiang/F-6905-2011 FU National Science Foundation (NSF) [CMMI-0751621, CMMI-1405078] FX National Science Foundation (NSF) (CMMI-0751621, CMMI-1405078). NR 24 TC 4 Z9 4 U1 5 U2 24 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD AUG 15 PY 2015 VL 40 IS 16 BP 3918 EP 3921 DI 10.1364/OL.40.003918 PG 4 WC Optics SC Optics GA CP2SQ UT WOS:000359727800061 PM 26274694 ER PT J AU Sun, C Uberuaga, BP Yin, L Li, J Chen, Y Kirk, MA Li, M Maloy, SA Wang, H Yu, C Zhang, X AF Sun, C. Uberuaga, B. P. Yin, L. Li, J. Chen, Y. Kirk, M. A. Li, M. Maloy, S. A. Wang, H. Yu, C. Zhang, X. TI Resilient ZnO nanowires in an irradiation environment: An in situ study SO ACTA MATERIALIA LA English DT Article DE ZnO nanowires; Radiation damage; Extreme environments; Defect denuded zone ID RADIATION-DAMAGE; CERAMICS; DEFECTS; NANOSTRUCTURES; AMORPHIZATION; BOUNDARIES; METALS; GROWTH AB ZnO nanowires (NWs) have been extensively studied for various device applications. Although these nanowires are often suspected to be impractical and highly unstable under hostile radiation environments, to date little is known on their radiation tolerance. Here, we show outstanding resilience of ZnO NWs by using in situ Kr ion irradiation at room temperature inside a transmission electron microscope. Our studies show that ZnO nanowires with certain diameters become nearly immune to radiation damage due to the existence of dislocation loop denuded zones. A remarkable size effect also holds: the smaller the nanowire diameter, the lower the defect density. Rate theory modeling suggests that the size effect arises from fast interstitial migration and a limit in size to which interstitial loops can grow. In situ studies also revealed a surprising phenomenon: the pristine prismatic loops can prevail over the strongest known defect sinks, free surfaces, to trap radiation-induced defect clusters. This study comprises the first critical step toward in-depth understanding of radiation response of functional oxide nanowires for electronic device applications in extreme environments. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Sun, C.; Li, J.; Chen, Y.; Zhang, X.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sun, C.; Uberuaga, B. P.; Maloy, S. A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Yin, L.; Yu, C.; Zhang, X.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Kirk, M. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, M.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Wang, H.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. RP Zhang, X (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. EM zhangx@tamu.edu RI Maloy, Stuart/A-8672-2009; Chen, Youxing/P-5006-2016 OI Maloy, Stuart/0000-0001-8037-1319; Chen, Youxing/0000-0003-1111-4495 FU NSF-DMR-Metallic Materials and Nanostructures Program [1304101]; DOE-NEUP [DE-AC07-051D14517-00088120]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE-Office of Nuclear Energy; Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396] FX We acknowledge financial support by NSF-DMR-Metallic Materials and Nanostructures Program under Grant no. 1304101. C.S. was supported by DOE-NEUP under contract no. DE-AC07-051D14517-00088120. B.P.U. acknowledges support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. The IVEM facility at Argonne National Laboratory is supported by DOE-Office of Nuclear Energy. NR 41 TC 3 Z9 3 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2015 VL 95 BP 156 EP 163 DI 10.1016/j.actamat.2015.05.003 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CN7PJ UT WOS:000358626200017 ER PT J AU Zhang, XM Hu, T Rufner, JF LaGrange, TB Campbell, GH Lavernia, EJ Schoenung, JM van Benthem, K AF Zhang, Xinming Hu, Tao Rufner, Jorgen F. LaGrange, Thomas B. Campbell, Geoffrey H. Lavernia, Enrique J. Schoenung, Julie M. van Benthem, Klaus TI Metal/ceramic interface structures and segregation behavior in aluminum-based composites SO ACTA MATERIALIA LA English DT Article DE Aluminum alloy; Transmission electron microscopy; Segregation; Interface ID NANOSTRUCTURED MATERIALS; ELECTRON-DIFFRACTION; MECHANICAL-BEHAVIOR; THERMAL-OXIDATION; BORON-CARBIDE; PRECESSION TECHNIQUE; MATRIX-COMPOSITES; AL; NANOCRYSTALLINE; STRENGTH AB Trimodal Al alloy (AA) matrix composites consisting of ultrafine-grained (UFG) and coarse-grained (CG) Al phases and micron-sized B4C ceramic reinforcement particles exhibit combinations of strength and ductility that render them useful for potential applications in the aerospace, defense and automotive Industries. Tailoring of microstructures with specific mechanical properties requires a detailed understanding of interfacial structures to enable strong interface bonding between ceramic reinforcement and metal matrix, and thereby allow for effective load transfer. Trimodal AA metal matrix composites typically show three characteristics that are noteworthy: nanocrystalline grains in the vicinity of the B4C reinforcement particles; Mg segregation at AA/B4C interfaces; and the presence of amorphous interfacial layers separating nanocrystalline grains from B4C particles. Interestingly, however, fundamental information related to the mechanisms responsible for these characteristics as well as information on local compositions and phases are absent in the current literature. In this study, we use high-resolution transmission electron microscopy, energy-dispersive X-ray spectroscopy, electron energy-loss spectroscopy, and precession assisted electron diffraction to gain fundamental insight into the mechanisms that affect the characteristics of AA/B4C interfaces. Specifically, we determined interfacial structures, local composition and spatial distribution of the interfacial constituents. Near atomic resolution characterization revealed amorphous multilayers and a nanocrystalline region between Al phase and B4C reinforcement particles. The amorphous layers consist of nonstoichiometric AlxOy, while the nanocrystalline region is comprised of MgO nanograins. The experimental results are discussed in terms of the possible underlying mechanisms at AA/B4C interfaces. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Zhang, Xinming; Hu, Tao; Rufner, Jorgen F.; Lavernia, Enrique J.; Schoenung, Julie M.; van Benthem, Klaus] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [LaGrange, Thomas B.; Campbell, Geoffrey H.] Lawrence Livermore Natl Lab, Phys & Life Sci Directory, Livermore, CA 94550 USA. RP van Benthem, K (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. EM benthem@ucdavis.edu RI Foundry, Molecular/G-9968-2014; Hu, Tao /H-5137-2011 OI Hu, Tao /0000-0001-6937-4017 FU University of California Laboratory Fee Grant [12-LR-238313]; Office of Naval Research [N00014-12-1-0237, N00014-13-1-0668]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering at Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Center for Electron Microscopy, Lawrence Berkeley National Lab; US Department of Energy [DE-AC02-05CH11231]; [FWP SCW0974] FX X.Z., J.F.R. and K.v.B. were financially supported by a University of California Laboratory Fee Grant (#12-LR-238313). J.M.S., T.H. and E.J.L received funding from the Office of Naval Research (Program Manager: Dr. Lawrence Kabacoff) under Grant Number N00014-12-1-0237. The FIB instrument at UC Davis was acquired with Grant number N00014-13-1-0668 from Office of Naval Research (program manager: Dr. Lawrence Kabacoff). The precession electron diffraction experiments were performed under the auspices of the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering at Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and supported by FWP SCW0974 with equipment capabilities established under FWP SCW0939. We acknowledge support from the National Center for Electron Microscopy, Lawrence Berkeley National Lab, which is supported by the US Department of Energy under contract no. DE-AC02-05CH11231. X.Z. acknowledges Dr. Huikai Cheng and Dr. Jessica Riesterer (FEI Company) for their invaluable help during data acquisition at the FEI Nanoport. NR 50 TC 6 Z9 6 U1 4 U2 52 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2015 VL 95 BP 254 EP 263 DI 10.1016/j.actamat.2015.05.021 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CN7PJ UT WOS:000358626200028 ER PT J AU Sun, C Kirk, M Li, M Hattar, K Wang, Y Anderoglu, O Valdez, J Uberuaga, BP Dickerson, R Maloy, SA AF Sun, C. Kirk, M. Li, M. Hattar, K. Wang, Y. Anderoglu, O. Valdez, J. Uberuaga, B. P. Dickerson, R. Maloy, S. A. TI Microstructure, chemistry and mechanical properties of Ni-based superalloy Rene N4 under irradiation at room temperature SO ACTA MATERIALIA LA English DT Article DE Ni-based superalloy; Ion irradiation; Order-disorder transition; Dissolution; Mechanical properties ID ION IRRADIATION; STRUCTURAL-MATERIALS; STAINLESS-STEELS; PHASE-STABILITY; NI3AL; DISSOLUTION; ALLOYS; KINETICS; SIMULATION; STRESS AB Nickel superalloys with cubic L1(2) structured gamma' (Ni-3(Al, Ti)) precipitates exhibit high strength at high temperatures and excellent corrosion resistance when exposed to water. Unlike prior studies on irradiation damage of other Ni-based superalloys, our study on Rene N4 involves much larger gamma' precipitates, similar to 450 nm in size, a size regime where the irradiation-induced disordering and dissolution kinetics and the corresponding mechanical property evolution are unknown. We report that under heavy ion irradiation at room temperature, the submicron-sized gamma' precipitates were fully disordered at similar to 0.3 dpa and only later partially dissolved after 75 dpa irradiation. Nanoindentation experiments indicate that the mechanical properties of the alloy change significantly, with a dramatic decrease in hardness, with irradiation dose. Three contributions to the change in hardness were examined: defect clusters, disordering and dissolution. The generation of defect clusters in the matrix and precipitates slightly increased the indentation hardness, while disordering of the submicron-sized gamma' precipitates resulted in a dramatic decrease in the total hardness, which decreased further during the early stages of the intermixing between gamma' precipitates and matrix (<18 dpa). Controlling the long-range-ordering and chemical intermixing can be used to tailor the mechanical properties of Ni-based superalloys under irradiation. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Sun, C.; Wang, Y.; Anderoglu, O.; Valdez, J.; Uberuaga, B. P.; Dickerson, R.; Maloy, S. A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Kirk, M.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, M.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Hattar, K.] Sandia Natl Labs, Dept Radiat Solid Interact, Albuquerque, NM 87123 USA. RP Sun, C (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM csun@lanl.gov RI Maloy, Stuart/A-8672-2009 OI Maloy, Stuart/0000-0001-8037-1319 FU U.S. Department of Energy (DOE) through the LANL/LDRD Program; U.S. Department of Energy [DE-AC52-06NA25396]; DOE Office of Nuclear Energy; University of Chicago, Argonne, LLC [DE-AC02-06CH1 1357]; U.S. DOE's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. DOE, Office of Science, Basic Energy Sciences (BES) FX We acknowledge financial support of the U.S. Department of Energy (DOE) through the LANL/LDRD Program. We thank Prof. T. Pollock for providing the materials. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. The electron microscopy with in situ ion irradiation was accomplished at Argonne National Laboratory at the IVEM-Tandem, a Facility funded by the DOE Office of Nuclear Energy, operated under Contract No. DE-AC02-06CH1 1357 by University of Chicago, Argonne, LLC. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's National Nuclear Security Administration under contract DE-AC04-94AL85000. K.H. was supported by the U.S. DOE, Office of Science, Basic Energy Sciences (BES). NR 51 TC 2 Z9 2 U1 9 U2 35 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2015 VL 95 BP 357 EP 365 DI 10.1016/j.actamat.2015.04.061 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CN7PJ UT WOS:000358626200038 ER PT J AU Juan, PA Pradalier, C Berbenni, S McCabe, RJ Tome, CN Capolungo, L AF Juan, P. -A. Pradalier, C. Berbenni, S. McCabe, R. J. Tome, C. N. Capolungo, L. TI A statistical analysis of the influence of microstructure and twin-twin junctions on twin nucleation and twin growth in Zr SO ACTA MATERIALIA LA English DT Article DE Zirconium; Twinning; Twin-twin junction; Twin nucleation; Twin growth ID CLOSE-PACKED METALS; HCP METALS; DEFORMATION MODES; CONSTITUTIVE LAW; SLIP SYSTEMS; ZIRCONIUM; TEMPERATURE; DISLOCATION; MAGNESIUM; ALLOYS AB The purpose of the present work is (1) to study the statistical relevance of twin-twin junctions and (2) to study statistically the influence of twin-twin junctions and microstructure on nucleation and growth of twins in h.c.p. materials. A new automated twin recognition technique has been developed and is used to extract statistics from EBSD scans of high purity clock-rolled zirconium specimens loaded along the through-thickness and one of the in-plane directions. The technique allows for recognition of tensile and compressive twin systems within each individual grain. The ten possible twin-twin junction types that may occur in Zr between first generation twins are introduced as well as their associated frequencies in cases of through-thickness and in-plane compression. The present study shows that twin-twin junctions between twins belonging to the most active twinning modes are statistically relevant. It is also shown that twin-twin junctions hinder twin growth. In agreement with previous studies, it is found that irrespective of the loading direction and twin mode, both grain size and crystallographic orientation largely influence the propensity of grains for twin activation. However, the study suggests large differences in nucleation and growth mechanisms for each twinning mode. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Juan, P. -A.; Capolungo, L.] Georgia Inst Technol, GW Woodruff Sch Mech Engn, UMI GT CNRS 2958, Metz, France. [Pradalier, C.] Georgia Tech Lorraine, UMI GT CNRS 2958, Metz, France. [Juan, P. -A.; Berbenni, S.] Univ Lorraine, UMR CNRS 7239, LEM3, Metz, France. [McCabe, R. J.; Tome, C. N.] Los Alamos Natl Lab, MST, Los Alamos, NM 87545 USA. RP Capolungo, L (reprint author), Georgia Inst Technol, GW Woodruff Sch Mech Engn, UMI GT CNRS 2958, Metz, France. OI McCabe, Rodney /0000-0002-6684-7410 FU French State through the National Research Agency (ANR) under the program "Investment in the future" (Labex DAMAS) [ANR-11-LABX-0008-01]; project MAGTWIN [ANR-12-BS09-0010-02]; Office of Basic Energy Science [FWP 06SCPE401] FX P.-A. Juan and S. Berbenni would like to thank the support of the French State through the National Research Agency (ANR) under the program "Investment in the future" (Labex DAMAS referenced as ANR-11-LABX-0008-01) and the project MAGTWIN (referenced as ANR-12-BS09-0010-02) for its support. C.N. Tome, R.J. McCabe, L. Capolungo were fully supported by Office of Basic Energy Science, Project FWP 06SCPE401. NR 34 TC 3 Z9 3 U1 8 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2015 VL 95 BP 399 EP 410 DI 10.1016/j.actamat.2015.05.022 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CN7PJ UT WOS:000358626200042 ER PT J AU Allen, KA Sikes, EL Honisch, B Elmore, AC Guilderson, TP Rosenthal, Y Anderson, RF AF Allen, Katherine A. Sikes, Elisabeth L. Hoenisch, Baerbel Elmore, Aurora C. Guilderson, Thomas P. Rosenthal, Yair Anderson, Robert F. TI Southwest Pacific deep water carbonate chemistry linked to high southern latitude climate and atmospheric CO2 during the Last Glacial Termination SO QUATERNARY SCIENCE REVIEWS LA English DT Article DE Ice age cycles; Marine carbon cycle; Benthic foraminifera; B/Ca; Carbon isotopes; Glacial termination ID ANTARCTIC INTERMEDIATE WATER; NORTHERN NEW-ZEALAND; OCEAN CIRCULATION; INTERGLACIAL CHANGES; ICE-AGE; OVERTURNING CIRCULATION; ISOTOPIC COMPOSITION; YOUNGER DRYAS; COLD REVERSAL; BOTTOM WATER AB A greater amount of CO2 was stored in the deep sea during glacial periods, likely via greater efficiency of the biologic pump and increased uptake by a more alkaline ocean. Reconstructing past variations in seawater carbonate ion concentration (a major component of alkalinity) enables quantification of the relative roles of different oceanic CO2 storage mechanisms and also places constraints on the timing, magnitude, and location of subsequent deep ocean ventilation. Here, we present a record of deep-water inorganic carbon chemistry since the Last Glacial Maximum (LGM; similar to 19-23 ka BP), derived from sediment core RR0503-83 raised from 1627 m in New Zealand's Bay of Plenty. The core site lies within the upper limit of southern-sourced Circumpolar Deep Water (CDW), just below the lower boundary of Antarctic Intermediate Water (AAIW). We reconstruct past changes in bottom water inorganic carbon chemistry from the trace element and stable isotopic composition of calcite shells of the epibenthic foraminifer Cibicidoides wuellerstorfi. A record of Delta CO32- (Delta CO32- = [CO32-](in situ) - [CO32-](saturation)) derived from the foraminiferal boron to calcium ratio (B/Ca) provides evidence for greater ice-age storage of respired CO2 and reveals abrupt deglacial shifts in [CO32-](in situ) of up to 30 mu mol/kg (5 times larger than the difference between average LGM and Holocene values). The rapidity of these changes suggests the influence of changing water mass structure and atmospheric circulation in addition to a decrease in CO2 content of interior waters. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Allen, Katherine A.; Sikes, Elisabeth L.; Rosenthal, Yair] Rutgers State Univ, Dept Marine & Coastal Sci, New Brunswick, NJ 08903 USA. [Allen, Katherine A.; Hoenisch, Baerbel; Anderson, Robert F.] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY USA. [Elmore, Aurora C.] Univ Durham, Dept Earth Sci, Durham, England. [Guilderson, Thomas P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Guilderson, Thomas P.] Univ Calif Santa Cruz, Dept Ocean Sci, Santa Cruz, CA 95064 USA. RP Allen, KA (reprint author), Dept Marine & Coastal Sci, 71 Dudley Rd, New Brunswick, NJ 08901 USA. EM kat.allen@rutgers.edu RI Hoenisch, Baerbel/C-7530-2013 OI Hoenisch, Baerbel/0000-0001-5844-3398 FU NSF [430044, OCE-0823549, OCE 07-51764]; U.S. Department of Energy [DE-AC52-07NA27344]; NOAA Climate and Global Change Program (KAA) FX Many thanks to Maziet Choseby and Mysti Weber at Oregon State University core repository, to Jim Wright for stable isotopic analytical assistance, to Mea Cook for laboratory support and insightful discussions, to Phil Shane for identification of cryptic tephra layers, and to Julie Kalansky for support with trace metal analysis. Funding was provided by NSF Grants 430044 and OCE-0823549 (ELS and TG) and NSF Grant OCE 07-51764 (BH), and a portion of this work was performed under the auspices of the U.S. Department of Energy (DE-AC52-07NA27344). Funding was also provided by the NOAA Climate and Global Change Program (KAA), administered by the University Corporation for Atmospheric Research. NR 104 TC 5 Z9 5 U1 4 U2 38 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-3791 J9 QUATERNARY SCI REV JI Quat. Sci. Rev. PD AUG 15 PY 2015 VL 122 BP 180 EP 191 DI 10.1016/j.quascirev.2015.05.007 PG 12 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA CN0IM UT WOS:000358097300012 ER PT J AU Fan, R Gao, Y Pan, YQ Zhang, YQ AF Fan, Rui Gao, Yan Pan, Yiqun Zhang, Yingqi TI Research on cool injection and extraction performance of borehole cool energy storage for ground coupled heat pump system SO ENERGY AND BUILDINGS LA English DT Article DE Borehole cool energy storage; Ground coupled heat pump; Thermal performance analysis; Diurnal cool energy injection and extraction AB To solve the low performance of Ground Coupled Heat Pump (GCHP) system in summer in cooling-load-dominated area, Borehole Cool Energy Storage (BCES), which uses soil for the storage and exchange of energy, was combined with hybrid GCHP systems (cooling tower as auxiliary equipment) to achieve efficient heating and cooling of buildings. Compared with GHE, BCES can provide more cool energy for buildings during periods of peak demand as a result of injection of cooling energy. Based on the coupled heat conduction and heat advection model for BCES, a diurnal cool-injection and extraction strategy for BCES in summer was adopted to determine the optimized thermal performance of the hybrid GCHP systems. With diurnal injection and extraction of cooling energy, the BCES system with 1 m pipe spacing supplied three times the cooling energy (88.9% from cool injection) of GHE without injection. After 90 days, the average increase in soil temperature was 0.96 degrees C for BCES compared with 4.29 degrees C for GHE. Furthermore, the effect of borehole depth and spacing showed that a hybrid BCES and GCHP system is useful in significantly decreasing the required borehole area, and in mitigating peak power load and improve ng operational efficiency. (C) 2015 Elsevier B.V. All rights reserved. C1 [Fan, Rui] Tongji Univ, Sino German Coll Appl Sci, Shanghai 200092, Peoples R China. [Gao, Yan] Beijing Univ Civil Engn & Architecture, Beijing Key Lab Heating Gas Supply Ventilating &, Beijing, Peoples R China. [Pan, Yiqun] Tongji Univ, Sch Mech Engn, Shanghai 200092, Peoples R China. [Zhang, Yingqi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Fan, R (reprint author), Tongji Univ, Sino German Coll Appl Sci, Shanghai 200092, Peoples R China. EM fan_rui@tongji.edu.cn RI Zhang, Yingqi/D-1203-2015 FU National Natural Science Fund of China [50806052]; Shanghai Municipal Science and Technology Commission [13dz1203103] FX The project was financially supported by the National Natural Science Fund of China (Grant no. 50806052) and the Shanghai Municipal Science and Technology Commission (13dz1203103). The funding source had no role in study design/concept, data collection/analysis/interpretation, or in manuscript writing/submission. NR 22 TC 2 Z9 2 U1 2 U2 14 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 EI 1872-6178 J9 ENERG BUILDINGS JI Energy Build. PD AUG 15 PY 2015 VL 101 BP 35 EP 44 DI 10.1016/j.enbuild.2015.05.006 PG 10 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA CL8QB UT WOS:000357238100004 ER PT J AU von Lilienfeld, OA Ramakrishnan, R Rupp, M Knoll, A AF von Lilienfeld, O. Anatole Ramakrishnan, Raghunathan Rupp, Matthias Knoll, Aaron TI Fourier series of atomic radial distribution functions: A molecular fingerprint for machine learning models of quantum chemical properties SO INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY LA English DT Article DE machine learning; representation; descriptor; quantum chemistry; molecules ID POTENTIAL-ENERGY SURFACES; VIRTUAL EXPLORATION; NEURAL-NETWORKS; DRUG DISCOVERY; UNIVERSE; DESCRIPTORS; SIMILARITY; CHEMISTRY; SYSTEMS; DESIGN AB We introduce a fingerprint representation of molecules based on a Fourier series of atomic radial distribution functions. This fingerprint is unique (except for chirality), continuous, and differentiable with respect to atomic coordinates and nuclear charges. It is invariant with respect to translation, rotation, and nuclear permutation, and requires no preconceived knowledge about chemical bonding, topology, or electronic orbitals. As such, it meets many important criteria for a good molecular representation, suggesting its usefulness for machine learning models of molecular properties trained across chemical compound space. To assess the performance of this new descriptor, we have trained machine learning models of molecular enthalpies of atomization for training sets with up to 10 k organic molecules, drawn at random from a published set of 134 k organic molecules with an average atomization enthalpy of over 1770 kcal/mol. We validate the descriptor on all remaining molecules of the 134 k set. For a training set of 10 k molecules, the fingerprint descriptor achieves a mean absolute error of 8.0 kcal/mol. This is slightly worse than the performance attained using the Coulomb matrix, another popular alternative, reaching 6.2 kcal/mol for the same training and test sets. (c) 2015 Wiley Periodicals, Inc. C1 [von Lilienfeld, O. Anatole; Ramakrishnan, Raghunathan; Rupp, Matthias] Univ Basel, Inst Phys Chem, Dept Chem, CH-4056 Basel, Switzerland. [von Lilienfeld, O. Anatole; Ramakrishnan, Raghunathan; Rupp, Matthias] Univ Basel, Natl Ctr Computat Design & Discovery Novel Mat, Basel, Switzerland. [von Lilienfeld, O. Anatole] Argonne Natl Lab, Argonne Leadership Comp Facil, Lemont, IL 60439 USA. [Knoll, Aaron] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Knoll, Aaron] Univ Texas Austin, Texas Adv Comp Ctr, Austin, TX 78712 USA. RP von Lilienfeld, OA (reprint author), Univ Basel, Inst Phys Chem, Dept Chem, Klingelbergstr 80, CH-4056 Basel, Switzerland. EM anatole.vonlilienfeld@unibas.ch RI Ramakrishnan, Raghunathan/C-7250-2015; von Lilienfeld, O. Anatole/D-8529-2011; Rupp, Matthias/P-8680-2016 OI Ramakrishnan, Raghunathan/0000-0003-0866-3645; Rupp, Matthias/0000-0002-2934-2958 FU Office of Science of the U.S. DOE [DE-AC02-06CH11357]; LDRD; Swiss National Science foundation [PP00P2_138932] FX Contract grant sponsor: Office of Science of the U.S. DOE; contract grant number: DE-AC02-06CH11357.; Contract grant sponsor: LDRD funding (to OAvL).; Contract grant sponsor: Swiss National Science foundation; contract grant number: PP00P2_138932 (to OAvL). NR 73 TC 17 Z9 17 U1 6 U2 30 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0020-7608 EI 1097-461X J9 INT J QUANTUM CHEM JI Int. J. Quantum Chem. PD AUG 15 PY 2015 VL 115 IS 16 SI SI BP 1084 EP 1093 DI 10.1002/qua.24912 PG 10 WC Chemistry, Physical; Mathematics, Interdisciplinary Applications; Physics, Atomic, Molecular & Chemical SC Chemistry; Mathematics; Physics GA CM3TB UT WOS:000357606000009 ER PT J AU Faber, F Lindmaa, A von Lilienfeld, OA Armiento, R AF Faber, Felix Lindmaa, Alexander von Lilienfeld, O. Anatole Armiento, Rickard TI Crystal structure representations for machine learning models of formation energies SO INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY LA English DT Article DE machine learning; formation energies; representations; crystal structure; periodic systems ID CHEMICAL UNIVERSE; VIRTUAL EXPLORATION AB We introduce and evaluate a set of feature vector representations of crystal structures for machine learning (ML) models of formation energies of solids. ML models of atomization energies of organic molecules have been successful using a Coulomb matrix representation of the molecule. We consider three ways to generalize such representations to periodic systems: (i) a matrix where each element is related to the Ewald sum of the electrostatic interaction between two different atoms in the unit cell repeated over the lattice; (ii) an extended Coulomb-like matrix that takes into account a number of neighboring unit cells; and (iii) an ansatz that mimics the periodicity and the basic features of the elements in the Ewald sum matrix using a sine function of the crystal coordinates of the atoms. The representations are compared for a Laplacian kernel with Manhattan norm, trained to reproduce formation energies using a dataset of 3938 crystal structures obtained from the Materials Project. For training sets consisting of 3000 crystals, the generalization error in predicting formation energies of new structures corresponds to (i) 0.49, (ii) 0.64, and (iii) 0.37eV/atom for the respective representations. (c) 2015 Wiley Periodicals, Inc. C1 [Faber, Felix; von Lilienfeld, O. Anatole] Univ Basel, Dept Chem, CH-4003 Basel, Switzerland. [Faber, Felix; von Lilienfeld, O. Anatole] Univ Basel, Inst Phys Chem, CH-4003 Basel, Switzerland. [Faber, Felix; von Lilienfeld, O. Anatole] Univ Basel, Natl Ctr Computat Design & Discovery Novel Mat, CH-4003 Basel, Switzerland. [Lindmaa, Alexander; Armiento, Rickard] Linkoping Univ, Dept Phys Chem & Biol, SE-58183 Linkoping, Sweden. [von Lilienfeld, O. Anatole] Argonne Leadership Comp Facil, Lemont, IL 60439 USA. [von Lilienfeld, O. Anatole] Argonne Natl Lab, Lemont, IL 60439 USA. RP Faber, F (reprint author), Univ Basel, Dept Chem, CH-4003 Basel, Switzerland. EM rickard.armiento@liu.se; rickard.armiento@liu.se RI von Lilienfeld, O. Anatole/D-8529-2011; Armiento, Rickard/E-1413-2011 OI Armiento, Rickard/0000-0002-5571-0814 FU Swedish Research Council (VR) [621-2011-4249]; Linnaeus Environment at Linkoping on Nanoscale Functional Materials - VR; Swiss National Science foundation [PP00P2_138932]; Office of Science of the U.S. DOE [DE-AC02-06CH11357]; Air Force Office of Scientific Research, Air Force Material Command, USAF [FA9550-15-1-0026] FX Contract grant sponsor: Swedish Research Council (VR); contract grant number: 621-2011-4249 (R.A.).; Contract grant sponsor: Linnaeus Environment at Linkoping on Nanoscale Functional Materials (Funded by VR).; Contract grant sponsor: Swiss National Science foundation; contract grant number: PP00P2_138932 (O.A.v.L.).; Contract grant sponsor: Office of Science of the U.S. DOE; contract grant number: DE-AC02-06CH11357.; Contract grant sponsor: Air Force Office of Scientific Research, Air Force Material Command, USAF; contract grant number: FA9550-15-1-0026. NR 41 TC 15 Z9 15 U1 3 U2 24 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0020-7608 EI 1097-461X J9 INT J QUANTUM CHEM JI Int. J. Quantum Chem. PD AUG 15 PY 2015 VL 115 IS 16 SI SI BP 1094 EP 1101 DI 10.1002/qua.24917 PG 8 WC Chemistry, Physical; Mathematics, Interdisciplinary Applications; Physics, Atomic, Molecular & Chemical SC Chemistry; Mathematics; Physics GA CM3TB UT WOS:000357606000010 ER PT J AU Josell, D Bonevich, JE Nguyen, TM Johnson, RN AF Josell, D. Bonevich, J. E. Nguyen, T. M. Johnson, R. N. TI Heat transfer through nanoscale multilayered thermal barrier coatings at elevated temperatures SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Thermal barrier coating; Heat transfer; Interfacial thermal resistance; Interfacial thermal conductance; Multilayer; Alumina; Zirconia; 7YSZ ID EB-PVD; TAILORED MICROSTRUCTURE; PULSE EXPERIMENTS; FLASH METHOD; CONDUCTIVITY; DIFFUSIVITY; FILMS; ALUMINUM/TITANIUM; REFLECTANCE; DEPOSITION AB Heat transfer through thermal barrier coatings (TBCs) composed of alternating nanometer thick layers of aluminum oxide and 7% yttria stabilized zirconia (7YSZ) was studied by pulsed heating at temperatures in the range 1275 K to 1375 K. The thermal diffusivity of the TBCs, deposited on thin metal foils by electron beam evaporation and coated with an opaque, submicrometer metal capping layer, was studied by applying a sub-mu s duration heating pulse from a Q-switched laser to the substrate and then monitoring the temperature rise on the opposing, metal-capped surface of the TBC. The recorded temperature transients were modeled using properties of the constituent materials in order to obtain an upper bound of the thermal resistance associated with the interfaces between layers. The results thus provide insight into the feasibility of using interfacial thermal resistance in this material system to improve TBC performance by decreasing thermal conductivity. Published by Elsevier B.V. C1 [Josell, D.; Bonevich, J. E.; Nguyen, T. M.] Natl Inst Stand & Technol, Mat Measurement Lab, Gaithersburg, MD 20899 USA. [Johnson, R. N.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Josell, D (reprint author), NIST, 100 Bur Dr, Gaithersburg, MD 20899 USA. EM daniel.josell@nist.gov NR 38 TC 0 Z9 0 U1 4 U2 23 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD AUG 15 PY 2015 VL 275 BP 75 EP 83 DI 10.1016/j.surfcoat2015.05.036 PG 9 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA CM5UG UT WOS:000357753900012 ER PT J AU Trugman, DT Wu, CQ Guyer, RA Johnson, PA AF Trugman, Daniel T. Wu, Chunquan Guyer, Robert A. Johnson, Paul A. TI Synchronous low frequency earthquakes and implications for deep San Andreas Fault slip SO EARTH AND PLANETARY SCIENCE LETTERS LA English DT Article DE low frequency earthquakes; lower crustal deformation; acoustic emission; Parkfield seismicity; earthquake clustering ID CASCADIA SUBDUCTION ZONE; EPISODIC TREMOR; CENTRAL CALIFORNIA; RECURRENCE; BENEATH; JAPAN AB Low Frequency Earthquakes (LFEs) are slip events that occur repeatedly at source locations within the lower crust. LFEs, and the associated seismic broadcast known as tremor, have been observed In a diverse array of tectonic environments. Here we develop a suite of statistical tools to conduct a systematic study of the spatial and temporal correlations of the event occurrence patterns of the 88 LFE sources beneath the greater Parkfield section of the San Andreas Fault. We first examine correlations in the occurrence patterns on long time scales to show that the regions to the north and south of Parkfield behave independently. We next use the cumulative event signatures of each source to characterize the individual occurrence patterns on shorter time scales. Through application of a statistical clustering algorithm, we demonstrate that individual LFE sources form spatially coherent clusters that may represent localized elastic structures or asperities on the deep fault interface. We conclude by examining the fine-scale features of the event rates within the LFE occurrence patterns. Through quantitative comparison to analogous laboratory shear experiments on granular, fault gouge-like materials, we infer that the distinctive features of LFE occurrence patterns reflect variations in the in-situ stress and frictional conditions at the individual LFE source locations. These observations provide a framework to understand the spatial and temporal diversity of fault slip that occurs within the lower crust beneath Parkfield and that may influence seismic hazard in the region. (C) 2015 Elsevier B.V. All rights reserved. C1 [Trugman, Daniel T.; Wu, Chunquan; Guyer, Robert A.; Johnson, Paul A.] Los Alamos Natl Lab, Geophys Grp EES 17, Los Alamos, NM 87545 USA. [Trugman, Daniel T.] Scripps Inst Oceanog, Inst Geophys & Planetary Phys, San Diego, CA USA. [Wu, Chunquan] Univ Memphis, Ctr Earthquake Res & Informat, Memphis, TN 38152 USA. [Guyer, Robert A.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. RP Trugman, DT (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, Inst Geophys & Planetary Phys, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM dtrugman@ucsd.edu OI Trugman, Daniel/0000-0002-9296-4223 FU Institutional Support at Los Alamos National Laboratory; National Science Foundation Graduate Research Fellowship Program (NSFGRFP) [DGE-1144086] FX This research was supported by Institutional Support at Los Alamos National Laboratory, and is based upon work supported by the National Science Foundation Graduate Research Fellowship Program (NSFGRFP) under grant number DGE-1144086. Discussions with W. Frank, A. Delorey, J. Gomberg, and D. Shelly helped to guide this study. We are also grateful for the thoughtful reviews provided by A. Thomas, an anonymous reviewer, and the Editor, all of which greatly improved the manuscript. NR 37 TC 3 Z9 3 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-821X EI 1385-013X J9 EARTH PLANET SC LETT JI Earth Planet. Sci. Lett. PD AUG 15 PY 2015 VL 424 BP 132 EP 139 DI 10.1016/j.epsl.2015.05.029 PG 8 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CL8KJ UT WOS:000357223300012 ER PT J AU Perillo, AC Kucharik, CJ Meehan, TD Serbin, SP Singh, A Townsend, PA Whitney, KS Gratton, C AF Perillo, Amelia C. Kucharik, Christopher J. Meehan, Timothy D. Serbin, Shawn P. Singh, Aditya Townsend, Philip A. Whitney, Kaitlin Stack Gratton, Claudio TI Use of insect exclusion cages in soybean creates an altered microclimate and differential crop response SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Plant-insect interactions; Soybean; Aphids; Microclimate; Insect exclusion cages; Plant ecology ID APHIS-GLYCINES MATSUMURA; RADIATION USE EFFICIENCY; FIELD CAGE; GENERALIST PREDATORS; AGRICULTURAL SCREENS; POPULATION-DYNAMICS; STOMATAL-RESISTANCE; BIOLOGICAL-CONTROL; WATER-STRESS; PHOTOSYNTHESIS AB Insect exclusion cages are commonly used in agricultural and ecological studies to examine plant-insect interactions in a field setting while maintaining control over insect populations. However, these insect cages can unintentionally alter the climate inside of the cage and impact plant physiology, growth and yield as well as insect populations. This can subsequently affect interpretations of experimental results obtained from caged experiments. To address this concern, we measured meteorological variables in conjunction with soybean physiology, growth, and yield over a two-year period. In a 2011 field study in southern Wisconsin, we compared photosynthetic rates, leaf area index (LA!), soil environmental-conditions, and various components of yield for plants grown inside and outside of an industry standard insect cage (Lumite 32 x 32 mesh). Inside of cages, several variables were higher (P < 0.05) including surface (0-6 cm) soil moisture (38%), stomatal conductance (42%), and total plant biomass (30%), while LAI was 20% lower (P < 0.001) inside of the cages. During the 2012 growing season, we measured wind speed, wind gusts, solar radiation, air temperature and relative humidity inside of cages compared to open field conditions. We found that wind speed and solar radiation were 89% and 42% lower, respectively, and air temperature, relative humidity and vapor pressure deficit were not significantly affected. There was also a significant (P < 0.0001) effect of the time of day on differences in wind speed and radiation between cages and open field plots. Our findings suggest that commonly used insect cages significantly alter the microclimate inside of the cage, and create a radiation regime in which the amount of direct and diffuse radiation received by plants is altered compared to the open field. Plant physiological processes and growth are affected by these environmental changes, adding a confounding factor when comparing caged to open field plants. Because the effects are likely a function of the type of cage, and mesh size and color, we recommend that future studies more thoroughly measure the microclimate for a variety of common cage types used in experiments. (C) 2015 Elsevier B.V. All rights reserved. C1 [Perillo, Amelia C.; Kucharik, Christopher J.] Univ Wisconsin, Dept Agron, Madison, WI 53706 USA. [Kucharik, Christopher J.] Univ Wisconsin, Nelson Inst Ctr Sustainabil & Global Environm SAG, Madison, WI 53726 USA. [Meehan, Timothy D.; Whitney, Kaitlin Stack; Gratton, Claudio] Univ Wisconsin, Dept Entomol, Madison, WI 53706 USA. [Serbin, Shawn P.] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Singh, Aditya; Townsend, Philip A.] Univ Wisconsin, Dept Forest & Wildlife Ecol, Madison, WI 53706 USA. RP Kucharik, CJ (reprint author), Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. EM kucharik@wisc.edu RI Serbin, Shawn/B-6392-2009; Townsend, Philip/B-5741-2008; OI Serbin, Shawn/0000-0003-4136-8971; Townsend, Philip/0000-0001-7003-8774; Kucharik, Christopher/0000-0002-0400-758X FU USDA Agriculture and Food Research Initiative Competitive Grant [2011-67009-3002] FX The authors thank Trip Hook, Clayton Kingdon, Skye Greenler, Mike Cruse, Joey Lechelt, and Tyler Davis for assisting with fieldwork. We appreciate the helpful discussions and input from Daniel Kleinman. The research was funded through USDA Agriculture and Food Research Initiative Competitive Grant #2011-67009-3002. NR 50 TC 1 Z9 1 U1 4 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD AUG 15 PY 2015 VL 208 BP 50 EP 61 DI 10.1016/j.agrformet.2015.04.014 PG 12 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA CK3KF UT WOS:000356114300005 ER PT J AU Liu, YY Liu, CX Zhang, CY Yang, XF Zachara, JM AF Liu, Yuanyuan Liu, Chongxuan Zhang, Changyong Yang, Xiaofan Zachara, John M. TI Pore and continuum scale study of the effect of subgrid transport heterogeneity on redox reaction rates SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID POROUS-MEDIA; REDUCTIVE DISSOLUTION; WEATHERING RATES; IRON(III) REDUCTION; SILICATE MINERALS; FIELD-SCALE; SEDIMENTS; KINETICS; ANTHRAQUINONE-2,6-DISULFONATE; DESORPTION AB A micromodel system, which corresponds to one or part of a numerical grid in the continuum model, was used to investigate the effect of subgrid transport heterogeneity on redox reaction rates. Hematite reductive dissolution by injecting a reduced form of flavin mononucleotide (FMNH2) at variable flow rates was used as an example to probe the variations of redox reaction rates in different subgrid transport domains. Experiments, pore-scale simulations, and macroscopic continuum modeling were performed to measure and simulate in-situ hematite reduction and to evaluate the scaling behavior of the redox reaction rates from the pore to continuum scales. The results indicated that the measured pore-scale rates of hematite reduction were consistent with the predictions from a pore-scale reactive transport model. A general trend is that hematite reduction followed reductant transport pathways, starting from the advection-dominated pores toward the interior of diffusion-dominated domains. Two types of diffusion domains were considered in the micromodel: a micropore diffusion domain, which locates inside solid grains or aggregates where reactant transport is limited by diffusion; and a macropore diffusion domain, which locates at wedged, dead-end pore spaces created by the grain-grain contacts. The rate of hematite reduction in the advection-dominated domain was faster than those in the diffusion-controlled domains, and the rate in the macropore diffusion domain was faster than that in the micropore domain. The reduction rates in the advection and macropore diffusion domains increased with increasing flow rate, but were affected by different mechanisms. The rate increase in the advection domain was controlled by the mass action effect as a faster flow supplied more reactants, and the rate increase in the macropore domain was more affected by the rate of mass exchange with the advection domain, which increased with increasing flow rate. The hematite reduction rate in the micropore domain was, however, not affected by the flow rate because molecular diffusion limits reductant supply to the micropore domain interior. Domain-based macroscopic models were evaluated to scale redox reaction rates from the pore to continuum scales. Simulation results from the single domain model, which ignores subgrid transport heterogeneity, deviated significantly from the pore-scale results. Further analysis revealed that the rate expression for hematite reduction was not scalable from the pore to porous media using the single domain model. A three-domain model, which effectively considers subgrid reactive diffusion in the micropore and macropore domains, significantly improved model description. Overall this study revealed the importance of subgrid transport heterogeneity in the manifestation of redox reaction rates in porous media and in scaling reactions from the pore to porous media. The research also supported that the domain-based scaling approach can be used to directly scale redox reactions in porous media with subgrid transport heterogeneity. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Liu, Yuanyuan; Liu, Chongxuan; Zhang, Changyong; Yang, Xiaofan; Zachara, John M.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Liu, CX (reprint author), Pacific NW Natl Lab, K8-96, Richland, WA 99354 USA. EM Chongxuan.liu@pnnl.gov RI Liu, Chongxuan/C-5580-2009; Zhang, Changyong/A-8012-2013; Yang, Xiaofan/L-6472-2015; Liu, Yuanyuan/L-1369-2016 OI Yang, Xiaofan/0000-0003-4514-0229; Liu, Yuanyuan/0000-0001-6076-9733 FU U.S. DOE, Office of Science, Biological and Environmental Research (BER), Subsurface Biogeochemical Research (SBR) Program through Pacific Northwest National Laboratory (PNNL) SBR Science Focus Area (SFA) Research Project; DOE [DE-AC05-76RL01830] FX This research is supported by the U.S. DOE, Office of Science, Biological and Environmental Research (BER) as part of the Subsurface Biogeochemical Research (SBR) Program through Pacific Northwest National Laboratory (PNNL) SBR Science Focus Area (SFA) Research Project. This research was performed using Environmental Molecular Science Laboratory (EMSL), a DOE Office of Science user facility sponsored by the DOE DOE's Office of BER and located at PNNL. PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. NR 46 TC 3 Z9 3 U1 5 U2 31 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2015 VL 163 BP 140 EP 155 DI 10.1016/j.gca.2015.04.039 PG 16 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CK0WT UT WOS:000355926900009 ER PT J AU Wang, ZM Shi, Z Shi, L White, GF Richardson, DJ Clarke, TA Fredrickson, JK Zachara, JM AF Wang, Zheming Shi, Zhi Shi, Liang White, Gaye F. Richardson, David J. Clarke, Thomas A. Fredrickson, Jim K. Zachara, John M. TI Effects of soluble flavin on heterogeneous electron transfer between surface-exposed bacterial cytochromes and iron oxides SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SHEWANELLA-ONEIDENSIS MR-1; OUTER-MEMBRANE; DISSIMILATORY FE(III); REDUCTIVE DISSOLUTION; REDOX REACTIONS; FERRIHYDRITE; GOETHITE; TRANSFORMATION; (HYDR)OXIDES; RESPIRATION AB Dissimilatory iron-reducing bacteria can utilize insoluble Fe(Mn)-oxides as a terminal electron acceptor under anaerobic conditions. For Shewanella species specifically, evidence suggests that iron reduction is associated with the secretion of flavin mononucleotide (FMN) and riboflavin. However, the exact mechanism of flavin involvement is unclear; while some indicate that flavins mediate electron transfer (Marsili et al., 2008), others point to flavin serving as co-factors to outer membrane proteins (Okamoto et al., 2013). In this work, we used methyl viologen (MV center dot+)-encapsulated, porin-cytochrome complex (MtrCAB) embedded liposomes (MELs) as a synthetic model of the Shewanella outer membrane to investigate the proposed mediating behavior of microbially produced flavins. The reduction kinetics of goethite, hematite and lepidocrocite (200 mu M) by MELs ([ MV center dot+] similar to 40 mu M and MtrABC <= 1 nM) were determined in the presence FMN at pH 7.0 in N-2 atmosphere by monitoring the concentrations of MV center dot+ and FMN through their characteristic UV-visible absorption spectra. Experiments were performed where (i) FMN and Fe(III)-oxide were mixed and then reacted with the reduced MELs and (ii) FMN was reacted with the reduced MELs followed by addition of Fe(III)-oxide. The redox reactions proceeded in two steps: a fast step that was completed in a few seconds, and a slower one lasting over 400 s. For all three Fe(III)-oxides, the initial reaction rate in the presence of a low concentration of FMN (<= 1 mu M) was at least a factor of five faster than those with MELs alone, and orders of magnitude faster than those by FMNH2, suggesting that FMN may serve as a co-factor that enhances electron transfer from outer-membrane c-cytochromes to Fe(III)-oxides. The rate and extent of the initial reaction followed the order of lepidocrocite > hematite > goethite, the same as their reduction potentials, implying thermodynamic control on reaction rate. For LEP, with the highest reduction potential among the three Fe(III)-oxides, its reduction by FMNH2 was completed in less than 10 min, suggesting that FMN was capable of mediating electron transfer to LEP. At higher FMN concentrations (>1 mu M), the reaction rates for both steps decreased and varied inversely with FMN concentration, indicating that FMN inhibited the MEL to Fe(III)-oxide electron transfer reaction under these conditions. The implications of the observed kinetic behaviors to flavin-mediated Fe(III)-oxide reduction in natural environments are discussed. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Wang, Zheming; Shi, Zhi; Shi, Liang; Fredrickson, Jim K.; Zachara, John M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [White, Gaye F.; Richardson, David J.; Clarke, Thomas A.] Univ E Anglia, Sch Biol Sci, Ctr Mol & Struct Biochem, Norwich NR4 7TJ, Norfolk, England. [White, Gaye F.; Richardson, David J.; Clarke, Thomas A.] Univ E Anglia, Sch Chem, Norwich NR4 7TJ, Norfolk, England. RP Wang, ZM (reprint author), Pacific NW Natl Lab, POB 999,MS K8-96, Richland, WA 99352 USA. EM zheming.wang@pnnl.gov; john.zachara@pnnl.gov RI clarke, tom/D-1837-2009; Wang, Zheming/E-8244-2010; Richardson, David/N-5129-2014 OI clarke, tom/0000-0002-6234-1914; Wang, Zheming/0000-0002-1986-4357; Richardson, David/0000-0002-7751-1058 FU Geoscience Research Program of the Office of Basic Energy Science (BES); U.S. Department of Energy (DOE); Pacific Northwest National Laboratory Scientific Focus Area (PNNL SFA); Pacific Northwest National Laboratory is operated for the U.S. Department of Energy [DE-AC06-76RLO 1830] FX This research was supported by the Geoscience Research Program of the Office of Basic Energy Science (BES), U.S. Department of Energy (DOE). The contributions of Jim Fredrickson and Liang Shi were supported by Pacific Northwest National Laboratory Scientific Focus Area (PNNL SFA). Part of this research was performed at EMSL, a national scientific user facility at PNNL managed by the Department of Energy's Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle under Contract DE-AC06-76RLO 1830. NR 43 TC 6 Z9 6 U1 8 U2 73 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2015 VL 163 BP 299 EP 310 DI 10.1016/j.gca.2015.03.039 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CK0WT UT WOS:000355926900017 ER PT J AU Zheng, D Zhang, XR Qu, DY Yang, XQ Lee, HS Qu, DY AF Zheng, Dong Zhang, Xuran Qu, Deyu Yang, Xiao-Qing Lee, Hung-Sui Qu, Deyang TI Investigation of the electrocatalytic oxygen reduction and evolution reactions in lithium-oxygen batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Carbon edge and basal orientations; Li-air battery; Electro-catalytic redox reaction of O-2; Lewis acid; Li2O2 solubility ID LI-AIR BATTERIES; CATALYTIC DISPROPORTIONATION; ANION RECEPTORS; ELECTROLYTES; CATHODE AB Oxygen reduction and oxygen evolution reactions were studied on graphite electrodes with different crystal orientations. The kinetics for the redox couple O-2/O-2(center dot-) are very fast, therefore no catalyst seems necessary to assist the charge transfer process. Apparently, the main source of the overpotential for the O-2 reduction reaction is from mass diffusion. Li2O2 becomes soluble in non-aqueous electrolytes in the presence of the tetraethylammonium tetrafluoroborate additive. The soluble B - O-2(2-) ions can be oxidized electro-catalytically. The edge orientation of graphite demonstrates superior catalytic activity for the oxidation over basal orientation. The findings reveal an opportunity for recharging Li-air batteries efficiently and a new strategy of developing the catalyst for oxygen evolution reaction. (c) 2015 Elsevier B.V. All rights reserved. C1 [Zheng, Dong; Qu, Deyang] Univ Wisconsin, Dept Mech Engn, Coll Engn & Appl Sci, Milwaukee, WI 53211 USA. [Zhang, Xuran; Qu, Deyu] Wuhan Univ Technol, Sch Sci, Dept Chem, Wuhan 430070, Hubei, Peoples R China. [Yang, Xiao-Qing; Lee, Hung-Sui] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Qu, DY (reprint author), Univ Wisconsin, Dept Mech Engn, Coll Engn & Appl Sci, Milwaukee, WI 53211 USA. EM qud@uwm.edu RI Zheng, Dong/J-9975-2015 OI Zheng, Dong/0000-0002-5824-3270 FU Office of Vehicle Technologies, under the program of Vehicle Technology Program [DEAC02-98CH10886] FX The authors from University of Wisconsin and Brookhaven National Laboratory are indebted to the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under the program of Vehicle Technology Program, under Contract Number DEAC02-98CH10886. NR 19 TC 0 Z9 0 U1 5 U2 156 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2015 VL 288 BP 9 EP 12 DI 10.1016/j.jpowsour.2015.04.108 PG 4 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CJ7UX UT WOS:000355706900002 ER PT J AU Sathre, R Scown, CD Kavvada, O Hendrickson, TP AF Sathre, Roger Scown, Corinne D. Kavvada, Olga Hendrickson, Thomas P. TI Energy and climate effects of second-life use of electric vehicle batteries in California through 2050 SO JOURNAL OF POWER SOURCES LA English DT Article DE Battery; Lithium ion; Degradation; Energy balance; Climate change mitigation; Grid storage ID GREENHOUSE-GAS EMISSIONS; LIFE; STORAGE; GENERATION AB As the use of plug-in electric vehicles (PEVs) further increases in the coming decades, a growing stream of batteries will reach the end of their service lives. Here we study the potential of those batteries to be used in second-life applications to enable the expansion of intermittent renewable electricity Supply in California through the year 2050. We develop and apply a parametric life-cycle system model integrating battery supply, degradation, logistics, and second-life use. We calculate and compare several metrics of second-life system performance, including cumulative electricity delivered, energy balance, greenhouse gas (GHG) balance, and energy stored on invested. We find that second-life use of retired PEV batteries may play a modest, though not insignificant, role in California's future energy system. The electricity delivered by second-life batteries in 2050 under base-case modeling conditions is 15 TWh per year, about 5% of total current and projected electricity use in California. If used instead of natural gas-fired electricity generation, this electricity would reduce GHG emissions by about 7 million metric tons of CO(2)e per year in 2050. Published by Elsevier B.V. C1 [Sathre, Roger; Scown, Corinne D.; Kavvada, Olga; Hendrickson, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. [Kavvada, Olga; Hendrickson, Thomas P.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. RP Sathre, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. EM rsathre@lbl.gov RI Scown, Corinne/D-1253-2013 FU DOE [DE-AC-02-05CH11231]; California Energy Commission (CEC); DOE FX We would like to thank Jeffery Greenblatt, Venkat Srinivasan, Samveg Saxena, Mark Caffarey, Brad Smith, and Dirk Spiers for their advice and guidance. The Lawrence Berkeley National Laboratory (LBNL) is a national laboratory of the US Department of Energy (DOE) managed by the University of California for the DOE under Contract Number DE-AC-02-05CH11231. This report was prepared as an account of work sponsored by the California Energy Commission (CEC) and pursuant to an M&O Contract with the DOE. Neither LBNL, DOE, CEC, nor any of their employees, contractors, or subcontractors, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe on privately owned rights. The views and opinions of authors expressed herein do not necessarily state or reflect those of LBNL, DOE, CEC, or any of their employees, or the Government, or any agency thereof, or the State of California. This report has not been approved or disapproved by LBNL, the DOE, or the CEC, nor has LBNL, the DOE, or the Sponsor passed upon the accuracy or adequacy of the information in this report. NR 39 TC 2 Z9 3 U1 9 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2015 VL 288 BP 82 EP 91 DI 10.1016/j.jpowsour.2015.04.097 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CJ7UX UT WOS:000355706900012 ER PT J AU Beland, LK Osetsky, YN Stoller, RE Xu, HX AF Beland, Laurent Karim Osetsky, Yuri N. Stoller, Roger E. Xu, Haixuan TI Interstitial loop transformations in FeCr SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Off-lattice kinetic Monte Carlo; Iron; Radiation damage; Chrome; Interstitial-loop ID MONTE-CARLO SIMULATIONS; CR ALLOYS; DISLOCATION LOOPS; IRON; CLUSTERS; IRRADIATION; RELAXATION; SURFACES; DAMAGE AB We improve the Self-Evolving Atomistic Kinetic Monte Carlo (SEAKMC) algorithm by integrating the Activation Relaxation Technique nouveau (ARTn), a powerful open-ended saddle-point search method, into the algorithm. We use it to investigate the reaction of 37-interstitial 1/2[111] and 1/2[(11) over bar1] loops in FeCr at 10 at.% Cr. They transform into 1/2[111], 1/2[(11) over bar1], [100] and [010] 74-interstitial clusters with an overall barrier of 0.85 eV. We find that Cr decoration locally inhibits the rotation of crowdions, which dictates the final loop orientation. The final loop orientation depends on the details of the Cr decoration. Generally, a region of a given orientation is favored if Cr near its interface with a region of another orientation is able to inhibit reorientation at this interface more than the Cr present at the other interfaces. We also find that substitutional Cr atoms can diffuse from energetically unfavorable to energetically favorable sites within the interlocked 37-interstitial loops conformation with barriers of less than 0.35 eV. (C) 2015 Elsevier B.V. All rights reserved. C1 [Beland, Laurent Karim; Osetsky, Yuri N.; Stoller, Roger E.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Xu, Haixuan] Univ Tennessee, Dept Mat Sci, Knoxville, TN 37996 USA. RP Xu, HX (reprint author), Univ Tennessee, Dept Mat Sci, Knoxville, TN 37996 USA. EM xhx@utk.edu RI Xu, Haixuan/C-9841-2009; OI Osetskiy, Yury/0000-0002-8109-0030 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, ''Center for Defect Physics,'' an Energy Frontier Research Center; Fonds Quebecois de recherche Nature et Technologies FX We thank Normand Mousseau for making ARTn available online. Research at the Oak Ridge National Laboratory sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, ''Center for Defect Physics,'' an Energy Frontier Research Center. LKB acknowledges a fellowship awarded by the Fonds Quebecois de recherche Nature et Technologies. NR 45 TC 4 Z9 4 U1 0 U2 17 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD AUG 15 PY 2015 VL 640 BP 219 EP 225 DI 10.1016/j.jallcom.2015.03.173 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CH7DK UT WOS:000354195600034 ER PT J AU Sondak, D Shadid, JN Oberai, AA Pawlowski, RP Cyr, EC Smith, TM AF Sondak, D. Shadid, J. N. Oberai, A. A. Pawlowski, R. P. Cyr, E. C. Smith, T. M. TI A new class of finite element variational multiscale turbulence models for incompressible magnetohydrodynamics SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Turbulence models; Magnetohydrodynamics; Finite elements; Variational multiscale formulation ID LARGE-EDDY SIMULATION; COMPUTATIONAL FLUID-DYNAMICS; NUMERICAL-SIMULATION; STABILIZED METHODS; RESISTIVE MHD; FLOWS; FORMULATION; EQUATIONS; APPROXIMATION; VISCOSITY AB New large eddy simulation (LES) turbulence models for incompressible magnetohydrodynamics (MHD) derived from the variational multiscale (VMS) formulation for finite element simulations are introduced. The new models include the variational multiscale formulation, a residual-based eddy viscosity model, and a mixed model that combines both of these component models. Each model contains terms that are proportional to the residual of the incompressible MHD equations and is therefore numerically consistent. Moreover, each model is also dynamic, in that its effect vanishes when this residual is small. The new models are tested on the decaying MHD Taylor Green vortex at low and high Reynolds numbers. The evaluation of the models is based on comparisons with available data from direct numerical simulations (DNS) of the time evolution of energies as well as energy spectra at various discrete times. A numerical study, on a sequence of meshes, is presented that demonstrates that the large eddy simulation approaches the DNS solution for these quantities with spatial mesh refinement. (C) 2015 Elsevier Inc. All rights reserved. C1 [Sondak, D.] Univ Wisconsin, Dept Math, Madison, WI 53706 USA. [Shadid, J. N.; Pawlowski, R. P.; Cyr, E. C.; Smith, T. M.] Sandia Natl Labs, Computat Math Dept, Livermore, CA 94550 USA. [Oberai, A. A.] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12181 USA. RP Sondak, D (reprint author), Univ Wisconsin, Dept Math, Madison, WI 53706 USA. EM sondak@math.wisc.edu OI Sondak, David/0000-0002-2730-9097 FU Department of Energy (DOE) Office of Science Graduate Fellowship (SCGF) [DE-AC05-06OR23100]; NSF-DMS grant [1147523]; DOE Office of Science Applied Mathematics Program at Sandia National Laboratories [DE-AC04-94AL85000] FX This work was initiated with support from the Department of Energy (DOE) Office of Science Graduate Fellowship (SCGF) under Contract No. DE-AC05-06OR23100. Support from NSF-DMS grant 1147523 is gratefully acknowledged during preparation of this paper. Additionally the work of Shadid, Pawlowski, Cyr and Smith was partially supported by the DOE Office of Science Applied Mathematics Program at Sandia National Laboratories under contract DE-AC04-94AL85000. The authors would like to acknowledge helpful discussions with Luis Chacon (Los Alamos Laboratory) with reference to the underlying resistive MHD model. NR 72 TC 4 Z9 4 U1 1 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD AUG 15 PY 2015 VL 295 BP 596 EP 616 DI 10.1016/j.jcp.2015.04.035 PG 21 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CI0BD UT WOS:000354399700028 ER PT J AU Guo, XQ Wang, H Qiao, H Mao, XB AF Guo, X. Q. Wang, H. Qiao, H. Mao, X. B. TI Numerical study of the large strain behavior of extruded magnesium alloy AM30 tube by elastic viscoplastic self-consistent model SO MATERIALS & DESIGN LA English DT Article DE Magnesium alloy; Twinning; Crystal plasticity; Ring hoop tension test (RHTT) ID SITU NEUTRON-DIFFRACTION; MECHANICAL-PROPERTIES; DETWINNING BEHAVIOR; TEXTURE DEVELOPMENT; CYCLIC DEFORMATION; STRESS-RELAXATION; MG ALLOYS; AZ31B; EVOLUTION; CREEP AB The anisotropic mechanical behaviors of the newly developed magnesium alloy AM30 are modeled by the elastic viscoplastic self-consistent (EVPSC) model. This is the first time to numerically study the mechanical behavior of AM30 based on EVPSC model. Three tests of uniaxial tension and compression along extrusion direction (ED) and ring hoop tension at temperature of 200 degrees C and strain rate of 0.1 s(-1) are studied. It is found that extension twinning is an important deformation mechanism under both uniaxial compression along extrusion direction and ring hoop tension test. However the initial texture of the extruded AM30 tubes results in significantly different activities for these two tests. The twin volume fraction of extension twinning under ring hoop tension is less than that under uniaxial compression along extrusion direction. Numerical results are in good agreement with corresponding experimental results. Published by Elsevier Ltd. C1 [Guo, X. Q.; Mao, X. B.] China Univ Min & Technol, State Key Lab Geomech & Deep Underground Engn, Xuzhou 221116, Jiangsu, Peoples R China. [Guo, X. Q.; Wang, H.; Qiao, H.] McMaster Univ, Dept Mech Engn, Hamilton, ON L8S 4L7, Canada. [Wang, H.] Los Alamos Natl Lab, Mat Sci & Technol, Los Alamos, NM 87544 USA. RP Wang, H (reprint author), Los Alamos Natl Lab, Mat Sci & Technol, POB 1663, Los Alamos, NM 87544 USA. EM wanghm@lanl.gov RI Wang, Huamiao/F-7693-2010 OI Wang, Huamiao/0000-0002-7167-2483 FU Ontario Ministry of Research and Innovation; State Key Laboratory Fund of China [SKLGDUEK1102]; State Key Development Program for Basic Research of China [2013CB227900]; Joint Funds of the National Natural Science Foundation of China [U1261201]; China Council Scholarship [201206420031] FX This research was supported by the Ontario Ministry of Research and Innovation and the State Key Laboratory Fund of China (No. SKLGDUEK1102). X.Q. GUO acknowledges the support of the State Key Development Program for Basic Research of China (Grant No. 2013CB227900), the Joint Funds of the National Natural Science Foundation of China (Grant No. U1261201) and China Council Scholarship (No. 201206420031). NR 46 TC 8 Z9 8 U1 4 U2 28 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0264-1275 EI 1873-4197 J9 MATER DESIGN JI Mater. Des. PD AUG 15 PY 2015 VL 79 BP 99 EP 105 DI 10.1016/j.matdes.2015.04.044 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA CH8LQ UT WOS:000354288300013 ER PT J AU Reeve, W Sullivan, J Ronson, C Tian, R Munk, C Han, C Reddy, TBK Seshadri, R Woyke, T Pati, A Markowitz, V Ivanova, N Kyrpides, N AF Reeve, Wayne Sullivan, John Ronson, Clive Tian, Rui Munk, Christine Han, Cliff Reddy, T. B. K. Seshadri, Rekha Woyke, Tanja Pati, Amrita Markowitz, Victor Ivanova, Natalia Kyrpides, Nikos TI High-Quality draft genome sequence of the Lotus spp. microsymbiont Mesorhizobium loti strain CJ3Sym SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Symbiosis; Alphaproteobacteria; GEBA-RNB ID SYMBIOSIS ISLAND; RHIZOBIUM-LOTI; METAGENOMIC PROJECTS; DATABASE GOLD; GENE; SYSTEM; IDENTIFICATION; METADATA; BACTERIA; MELILOTI AB Mesorhizobium loti strain CJ3Sym was isolated in 1998 following transfer of the integrative and conjugative element ICEMlSym(R7A), also known as the R7A symbiosis island, in a laboratory mating from the donor M. loti strain R7A to a nonsymbiotic recipient Mesorhizobium strain CJ3. Strain CJ3 was originally isolated from a field site in the Rocklands range in New Zealand in 1994. CJ3Sym is an aerobic, Gram-negative, non-spore-forming rod. This report reveals the genome of M. loti strain CJ3Sym currently comprises 70 scaffolds totaling 7,563,725 bp. The high-quality draft genome is arranged in 70 scaffolds of 71 contigs, contains 7,331 protein-coding genes and 70 RNA-only encoding genes, and is part of the GEBA-RNB project proposal. C1 [Reeve, Wayne; Tian, Rui] Murdoch Univ, Ctr Rhizobium Studies, Perth, WA, Australia. [Sullivan, John; Ronson, Clive] Univ Otago, Dept Microbiol & Immunol, Dunedin, New Zealand. [Munk, Christine; Han, Cliff] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Reddy, T. B. K.; Seshadri, Rekha; Woyke, Tanja; Pati, Amrita; Ivanova, Natalia; Kyrpides, Nikos] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos] King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Perth, WA, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 37 TC 0 Z9 0 U1 0 U2 3 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 14 PY 2015 VL 10 AR 54 DI 10.1186/s40793-015-0049-2 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NX UT WOS:000367992100001 PM 26380641 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalosa, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Dimitrievska, A Dingfelder, J Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Doherty, T Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dwuznik, M Dyndal, M Ecker, KM Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G 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Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for production of WW/WZ resonances decaying to a lepton, neutrino and jets in pp collisions at root s = 8 TeV with the ATLAS detector (vol 75, pg 209, 2015) SO EUROPEAN PHYSICAL JOURNAL C LA English DT Correction C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Auerbach, B.; Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Paramonov, A.; Price, L. E.; Proudfoot, J.; van Gemmeren, P.; Vaniachine, A.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, GR-15773 Zografos, Greece. [Abdinov, O.; Acharya, B. S.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. 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[Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Latour, B. Martin dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; Nedden, M. zur] Humboldt Univ, Dept Phys, D-10099 Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. 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Yau; Zimmermann, R.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixasa, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarrod, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero y; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Messina, A.; Milic, A.; Mornacchi, G.; Nairz, A. 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J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shana, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. 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[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Coll Cosenza, Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Picazio, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Klugea, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Glonti, G. L.; Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, ON, Canada. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] Univ Coll London, Dept Phys & Astron, London, ON, Canada. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. 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[Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meyer, J.; Oussoren, K. 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C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. 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[Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Mi Guens, J.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Mi Guens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrania, F. 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[Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. 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F-W.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalosa, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Orama, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Majarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Investigac, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, G.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kwan, T.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, IN2P3, Villeurbanne, France. Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Victoria, BC, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Warburton, Andreas/N-8028-2013; Gladilin, Leonid/B-5226-2011; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017; Tikhomirov, Vladimir/M-6194-2015; Garcia, Jose /H-6339-2015; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Jones, Roger/H-5578-2011; Boyko, Igor/J-3659-2013; Vranjes Milosavljevic, Marija/F-9847-2016; Chekulaev, Sergey/O-1145-2015; SULIN, VLADIMIR/N-2793-2015; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Snesarev, Andrey/H-5090-2013; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Guo, Jun/O-5202-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016 OI Warburton, Andreas/0000-0002-2298-7315; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Tikhomirov, Vladimir/0000-0002-9634-0581; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Jones, Roger/0000-0002-6427-3513; Boyko, Igor/0000-0002-3355-4662; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Guo, Jun/0000-0001-8125-9433; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620 NR 1 TC 6 Z9 6 U1 9 U2 40 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 14 PY 2015 VL 75 IS 8 AR 370 DI 10.1140/epjc/s10052-015-3593-4 PG 14 WC Physics, Particles & Fields SC Physics GA CY3IH UT WOS:000366302100001 ER PT J AU Moortgat-Pick, G Baer, H Battaglia, M Belanger, G Fujii, K Kalinowski, J Heinemeyer, S Kiyo, Y Olive, K Simon, F Uwer, P Wackeroth, D Zerwas, PM Arbey, A Asano, M Bagger, J Bechtle, P Bharucha, A Brau, J Brummer, F Choi, SY Denner, A Desch, K Dittmaier, S Ellwanger, U Englert, C Freitas, A Ginzburg, I Godfrey, S Greiner, N Grojean, C Grunewald, M Heisig, J Hocker, A Kanemura, S Kawagoe, K Kogler, R Krawczyk, M Kronfeld, AS Kroseberg, J Liebler, S List, J Mahmoudi, F Mambrini, Y Matsumoto, S Mnich, J Monig, K Muhlleitner, MM Poschl, R Porod, W Rolbiecki, SPK Rolbiecki, K Schmitt, M Serpico, P Stanitzki, M Stal, O Stoefaniak, T Stockinger, D Weiglein, G Wilson, GW Zeune, L Moortgat, F Xella, S Bagger, J Brau, J Ellis, J Kawagoe, K Komamiya, S Kronfeld, AS Mnich, J Peskin, M Schlatter, D Wagner, A Yamamoto, H AF Moortgat-Pick, G. Baer, H. Battaglia, M. Belanger, G. Fujii, K. Kalinowski, J. Heinemeyer, S. Kiyo, Y. Olive, K. Simon, F. Uwer, P. Wackeroth, D. Zerwas, P. M. Arbey, A. Asano, M. Bagger, J. Bechtle, P. Bharucha, A. Brau, J. Bruemmer, F. Choi, S. Y. Denner, A. Desch, K. Dittmaier, S. Ellwanger, U. Englert, C. Freitas, A. Ginzburg, I. Godfrey, S. Greiner, N. Grojean, C. Gruenewald, M. Heisig, J. Hoecker, A. Kanemura, S. Kawagoe, K. Kogler, R. Krawczyk, M. Kronfeld, A. S. Kroseberg, J. Liebler, S. List, J. Mahmoudi, F. Mambrini, Y. Matsumoto, S. Mnich, J. Moenig, K. Muehlleitner, M. M. Poschl, R. Porod, W. Porto, S. Rolbiecki, K. Schmitt, M. Serpico, P. Stanitzki, M. Stal, O. Stoecfaniak, T. Stockinger, D. Weiglein, G. Wilson, G. W. Zeune, L. Moortgat, F. Xella, S. Bagger, J. Brau, J. Ellis, J. d Kawagoe, K. Komamiya, S. Kronfeld, A. S. Mnich, J. Peskin, M. Schlatter, D. Wagner, A. Yamamoto, H. TI Physics at the e(+) e(-) linear collider SO EUROPEAN PHYSICAL JOURNAL C LA English DT Review ID LITTLEST HIGGS-MODEL; SUPERSYMMETRIC STANDARD MODEL; QUARK PAIR PRODUCTION; TO-LEADING-ORDER; PRODUCTION NEAR-THRESHOLD; ELECTROWEAK SYMMETRY-BREAKING; LEPTON FLAVOR VIOLATION; GAUGE-BOSON COUPLINGS; 2-LOOP QCD CORRECTIONS; PHOTON-PHOTON COLLISIONS AB A comprehensive review of physics at an e(+) e(-) linear collider in the energy range of root s = 92 GeV-3 TeV is presented in view of recent and expected LHC results, experiments from low-energy as well as astroparticle physics. The report focusses in particular on Higgs-boson, top-quark and electroweak precision physics, but also discusses several models of beyond the standard model physics such as super-symmetry, little Higgs models and extra gauge bosons. The connection to cosmology has been analysed as well. C1 [Moortgat-Pick, G.; Liebler, S.; Porto, S.] Univ Hamburg, Inst Theoret Phys 2, D-22761 Hamburg, Germany. [Moortgat-Pick, G.; Zerwas, P. M.; Greiner, N.; Grojean, C.; Liebler, S.; List, J.; Moenig, K.; Stanitzki, M.; Weiglein, G.; Wagner, A.] Deutsch Elektronen Synchrotron DESY Hamburg & Zeu, D-22603 Hamburg, Germany. [Baer, H.] Univ Oklahoma, Dept Phys & Astron, Norman, OK 73019 USA. [Battaglia, M.; Stoecfaniak, T.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Belanger, G.; Serpico, P.] Univ Savoie Mont Blanc, CNRS, Lab Phys Theor LAPTh, F-74941 Annecy Le Vieux, France. [Fujii, K.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki, Japan. [Kalinowski, J.; Krawczyk, M.; Rolbiecki, K.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Heinemeyer, S.] CSIC UC, Inst Fis Cantabria, Santander 39005, Spain. [Kiyo, Y.] Juntendo Univ, Dept Phys, Inzai, Chiba 2701695, Japan. [Olive, K.] Univ Minnesota, William I Fine Theoret Phys Inst, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Simon, F.; Greiner, N.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Uwer, P.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Wackeroth, D.] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. [Asano, M.; Bechtle, P.; Desch, K.; Kroseberg, J.] Univ Bonn, Phys Inst, D-53115 Bonn, Germany. [Asano, M.] Univ Bonn, Bethe Ctr Theoret Phys, D-53115 Bonn, Germany. [Bharucha, A.] Tech Univ Munich, Phys Dept T31, D-85748 Garching, Germany. [Bruemmer, F.] Univ Montpellier 2, UMR 5299, LUPM, F-34095 Montpellier, France. [Bruemmer, F.] CNRS, F-34095 Montpellier, France. [Choi, S. Y.] Chonbuk Natl Univ, Dept Phys, Jeonju 561756, South Korea. [Denner, A.; Porod, W.] Univ Wurzburg, Inst Theoret Phys & Astrophys, D-97074 Wurzburg, Germany. [Dittmaier, S.] Univ Freiburg, Phys Inst, D-79104 Freiburg, Germany. [Ellwanger, U.; Mambrini, Y.] Univ Paris 11, CNRS, UMR 8627, Lab Phys, F-91405 Orsay, France. [Englert, C.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Freitas, A.] Univ Pittsburgh, PITT PACC, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Ginzburg, I.] Sobolev Inst Math, Novosibirsk 630090, Russia. [Ginzburg, I.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Godfrey, S.] Carleton Univ, Dept Phys, Ottawa Carleton Inst Phys, Ottawa K1S 5B6, ON, Canada. [Grojean, C.] Univ Autonoma Barcelona, ICREA IFAE, Bellaterra 08193, Spain. [Gruenewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Heisig, J.] Rhein Westfal TH Aachen, Inst Theoret Particle Phys & Cosmol, D-52056 Aachen, Germany. [Hoecker, A.; Moortgat, F.; Ellis, J. d; Schlatter, D.] CERN, Geneva, Switzerland. [Kanemura, S.] Toyama Univ, Dept Phys, Toyama 9308555, Japan. [Kogler, R.; Wagner, A.] Univ Hamburg, Hamburg, Germany. [Matsumoto, S.] Univ Tokyo, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. [Muehlleitner, M. M.] Karlsruhe Inst Technol, Inst Theoret Phys, D-76128 Karlsruhe, Germany. [Rolbiecki, K.] Univ Autonoma Madrid, Inst Fis Teor, IFT UAM CSIC, E-28049 Madrid, Spain. [Schmitt, M.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60091 USA. [Stal, O.] Stockholm Univ, Dept Phys, Oskar Klein Ctr, S-10691 Stockholm, Sweden. [Stockinger, D.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01069 Dresden, Germany. [Arbey, A.; Mahmoudi, F.] Univ Lyon 1, F-69622 Villeurbanne, France. [Arbey, A.; Mahmoudi, F.] CNRS, UMR 5574, Ctr Rech Astrophys Lyon, F-69561 St Genis Laval, France. [Arbey, A.; Mahmoudi, F.] Ecole Normale Super Lyon, F-69364 Lyon, France. [Wilson, G. W.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Zeune, L.] Univ Amsterdam, ITFA, NL-1018 XE Amsterdam, Netherlands. [Poschl, R.] CNRS, IN2P3, LAL, F-91405 Orsay, France. [Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Bagger, J.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Brau, J.] Univ Oregon, Dept Phys, Eugene, OR 97403 USA. [Ellis, J. d] Kings Coll London, Dept Phys, Theoret Particle Phys & Cosmol Grp, London WC2R 2LS, England. [Kawagoe, K.] Kyushu Univ, Dept Phys, Higashi Ku, Fukuoka 8128581, Japan. [Komamiya, S.] Univ Tokyo, Dept Phys, Grad Sch Sci, Tokyo 1130033, Japan. [Komamiya, S.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo 1130033, Japan. [Kronfeld, A. S.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Peskin, M.] Stanford Univ, SLAC, Menlo Pk, CA 94025 USA. [Yamamoto, H.] Tohoku Univ, Dept Phys, Sendai, Miyagi 980, Japan. [Bharucha, A.] Aix Marseille U, CNRS, CPT, U Toulon, F-13288 Marseille, France. Tech Univ Munich, Inst Adv Study, D-85748 Garching, Germany. [Bagger, J.] TRIUMF, Vancouver, BC V6T 2A3, Canada. RP Moortgat-Pick, G (reprint author), Univ Hamburg, Inst Theoret Phys 2, D-22761 Hamburg, Germany. EM gudrid.moortgat-pick@desy.de RI Krawczyk, Maria/B-3184-2012; U-ID, Kyushu/C-5291-2016; Rolbiecki, Krzysztof/A-5402-2017; OI Rolbiecki, Krzysztof/0000-0002-9645-9670; Denner, Ansgar/0000-0002-7179-1132; grojean, christophe/0000-0002-7196-7361 FU DFG [SFB676]; European Commission [PITN-GA-2012-316704]; Japan Society for Promotions of Science (JSPS) [18GS0202]; JSPS [22244031, 23000002]; Dutch Ministry of Education, Culture and Science (OCW); Spanish Ministry MICNN [FPA2010-17747]; European Commission under ERC [226371]; German Research Foundation (DFG) [BR 3954/1-1, DFG TRR33]; MEXT, Japan [22244031, 26287039]; WPI Initiative, MEXT, Japan; MICINN, Spain [FPA2013-44773-P, CPAN CSD2007-00042]; Spanish MINECO Centro de excelencia Severo Ochoa Program [SEV-2012-0249]; Natural Sciences and Engineering Research Council of Canada [121209-2009 SAPIN]; Basic Science Research Program through National Research Foundation (NRF) - Ministry of Education, Science and Technology [2012-0002746]; Polish National Center for Science [NCN OPUS 2012/05/B/ST2/03306, NCN DEC-2012/05/B/ST2/02597]; BMBF; DAAD PPP Poland [56269947]; German Excellence Initiative; European Union [291763]; Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy; DOE at the University of Minnesota [DE-SC0011842]; [DFG/SFB-TR9]; [RFBR 11-02-00242]; [NSh-3802.2012.2] FX Several authors acknowledge the support of the DFG through the Grant SFB676 'Particles, Strings and the early universe'. This work was supported by European Commission through the contract PITN-GA-2012-316704 (HIGGSTOOLS). This work is supported in part by the Creative Scientific Research Grant No. 18GS0202 of the Japan Society for Promotions of Science (JSPS), the JSPS Grant-in-Aid for Science Research No. 22244031, and the JSPS Specially Promoted Research No. 23000002. This work is part of the D-ITP consortium, a programme of the Netherlands Organisation for Scientific Research (NWO) that is funded by the Dutch Ministry of Education, Culture and Science (OCW). G. Moortgat-Pick would like to thank A.A. Mikhailichenko for useful discussions and valuable comments on collider aspects. C. Grojean is supported by the Spanish Ministry MICNN under contract FPA2010-17747 and by the European Commission under the ERC Advanced Grant 226371 MassTeV and M.M. Muhlleitner is supported by the DFG/SFB-TR9 Computational Particle Physics. M. Asano acknowledges support from the German Research Foundation (DFG) through Grant BR 3954/1-1 and DFG TRR33 "The Dark Universe". S. Matsumoto acknowledges supports from the MEXT, Japan through Grants Nos. 22244031 and 26287039, and also from the WPI Initiative, MEXT, Japan. K. Rolbiecki has been supported by the MICINN, Spain, under contract FPA2013-44773-P, Consolider-Ingenio CPAN CSD2007-00042 and the Spanish MINECO Centro de excelencia Severo Ochoa Program under Grant SEV-2012-0249. S. Godfrey was supported in part by the Natural Sciences and Engineering Research Council of Canada under Grant Number 121209-2009 SAPIN. The work of S.Y. Choi was supported by Basic Science Research Program through the National Research Foundation (NRF) funded by the Ministry of Education, Science and Technology (2012-0002746). The work was partly supported by Polish National Center for Science, Grant NCN OPUS 2012/05/B/ST2/03306 (2012-2016) and the Grant NCN DEC-2012/05/B/ST2/02597, and by BMBF, DAAD PPP Poland Project 56269947, "Dark Matter at Colliders" (M. Krawczyk), Grants RFBR 11-02-00242, NSh-3802.2012.2 (I. Ginzburg). A. S. Kronfeld is supported in part by the German Excellence Initiative and the European Union Seventh Framework Programme under Grant Agreement No. 291763 as well as the European Union's Marie Curie COFUND programme. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. The work of K.A. Olive was supported in part by DOE Grant DE-SC0011842 at the University of Minnesota. NR 1426 TC 26 Z9 26 U1 6 U2 19 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 14 PY 2015 VL 75 IS 8 AR 371 DI 10.1140/epjc/s10052-015-3511-9 PG 178 WC Physics, Particles & Fields SC Physics GA CP3LK UT WOS:000359780200001 ER PT J AU Sinsabaugh, RL Belnap, J Rudgers, J Kuske, CR Martinez, N Sandquist, D AF Sinsabaugh, Robert L. Belnap, Jayne Rudgers, Jennifer Kuske, Cheryl R. Martinez, Noelle Sandquist, Darren TI Soil microbial responses to nitrogen addition in arid ecosystems SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE arid ecosystems; nitrogen deposition; microbial biomass; ecoenzyme activity; meta-analysis ID SEMIARID MEDITERRANEAN ECOSYSTEMS; GURBANTUNGGUT DESERT; NORTHWESTERN CHINA; FUNGAL COMMUNITIES; ENZYME-ACTIVITY; UNITED-STATES; DEPOSITION; GRASSLAND; CARBON; STOICHIOMETRY AB The N cycle of arid ecosystems is influenced by low soil organic matter, high soil pH, and extremes in water potential and temperature that lead to open canopies and development of biological soil crusts (biocrusts). We investigated the effects of N amendment on soil microbial dynamics in a Larrea tridentata-Ambrosia dumosa shrubland site in southern Nevada USA. Sites were fertilized with a NO3-NH4 mix at 0, 7, and 15 kg N ha(-1) y(-1) from March 2012 to March 2013. In March 2013, biocrust (0-0.5 cm) and bulk soils (0-10 cm) were collected beneath Ambrosia canopies and in the interspaces between plants. Biomass responses were assessed as bacterial and fungal SSU rRNA gene copy number and chlorophyll a concentration. Metabolic responses were measured by five ecoenzyme activities and rates of N transformation. By most measures, nutrient availability, microbial biomass, and process rates were greater in soils beneath the shrub canopy compared to the interspace between plants, and greater in the surface biocrust horizon compared to the deeper 10 cm soil profile. Most measures responded positively to experimental N addition. Effect sizes were generally greater for bulk soil than biocrust. Results were incorporated into a meta-analysis of arid ecosystem responses to N amendment that included data from 14 other studies. Effect sizes were calculated for biomass and metabolic responses. Regressions of effect sizes, calculated for biomass, and metabolic responses, showed similar trends in relation to N application rate and N load (rate x duration). The critical points separating positive from negative treatment effects were 88 kg ha(-1) y(-1) and 159 kg ha(-1), respectively, for biomass, and 70 kg ha(-1) y(-1) and 114 kg ha(-1), respectively, for metabolism. These critical values are comparable to those for microbial biomass, decomposition rates and respiration reported in broader meta-analyses of N amendment effects in mesic ecosystems. However, large effect sizes at low N addition rates indicate that arid ecosystems are sensitive to modest increments in anthropogenic N deposition. C1 [Sinsabaugh, Robert L.; Rudgers, Jennifer; Martinez, Noelle] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. [Belnap, Jayne] US Geol Survey, Southwest Biol Sci Ctr, Moab, UT USA. [Kuske, Cheryl R.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Sandquist, Darren] Calif State Univ Fullerton, Fullerton, CA 92634 USA. RP Sandquist, D (reprint author), Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. EM dsandquist@fullerton.edu FU Lake Mead National Recreation Area; USGS Ecosystems and Climate Change and Land Use programs; Science Focus Area grant by the U.S. Department of Energy, Office of Science, Biological and Environmental Research Division FX This research was generously supported by Lake Mead National Recreation Area. JB also acknowledges the support of USGS Ecosystems and Climate Change and Land Use programs. CK, RS, JR were supported by a Science Focus Area grant to Los Alamos National Laboratory by the U.S. Department of Energy, Office of Science, Biological and Environmental Research Division. The authors thank La Verne Gallegos-Graves, Aaron Cohodas, and Travis Reilly for excellent technical support. Many thanks to Erika Geiger, Hilda Smith, and other USGS technicians involved in data collection and analysis. Any use of trade names is for descriptive purposes only and does not imply endorsement by the U.S. Government. NR 57 TC 3 Z9 4 U1 46 U2 145 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 14 PY 2015 VL 6 AR 819 DI 10.3389/fmicb.2015.00819 PG 12 WC Microbiology SC Microbiology GA CP6TP UT WOS:000360021400001 PM 26322030 ER PT J AU Monahan, DM Whaley-Mayda, L Ishizaki, A Fleming, GR AF Monahan, Daniele M. Whaley-Mayda, Lukas Ishizaki, Akihito Fleming, Graham R. TI Influence of weak vibrational-electronic couplings on 2D electronic spectra and inter-site coherence in weakly coupled photosynthetic complexes SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID LIGHT-HARVESTING COMPLEXES; QUANTUM COHERENCE; ENERGY-TRANSFER; 2-DIMENSIONAL SPECTROSCOPY; PHYSIOLOGICAL TEMPERATURE; VIBRONIC COHERENCE; ANTENNA COMPLEX; SUDDEN-DEATH; FMO COMPLEX; ENTANGLEMENT AB Coherence oscillations measured in two-dimensional (2D) electronic spectra of pigment-protein complexes may have electronic, vibrational, or mixed-character vibronic origins, which depend on the degree of electronic-vibrational mixing. Oscillations from intrapigment vibrations can obscure the inter-site coherence lifetime of interest in elucidating the mechanisms of energy transfer in photosynthetic light-harvesting. Huang-Rhys factors (S) for low-frequency vibrations in Chlorophyll and Bacteriochlorophyll are quite small (S <= 0.05), so it is often assumed that these vibrations influence neither 2D spectra nor inter-site coherence dynamics. In this work, we explore the influence of S within this range on the oscillatory signatures in simulated 2D spectra of a pigment heterodimer. To visualize the inter-site coherence dynamics underlying the 2D spectra, we introduce a formalism which we call the "site-probe response." By comparing the calculated 2D spectra with the site-probe response, we show that an on-resonance vibration with Huang-Rhys factor as small as S = 0.005 and the most strongly coupled off-resonance vibrations (S = 0.05) give rise to long-lived, purely vibrational coherences at 77 K. We moreover calculate the correlation between optical pump interactions and subsequent entanglement between sites, as measured by the concurrence. At 77 K, greater long-lived inter-site coherence and entanglement appear with increasing S. This dependence all but vanishes at physiological temperature, as environmentally induced fluctuations destroy the vibronic mixing. (C) 2015 AIP Publishing LLC. C1 [Monahan, Daniele M.; Whaley-Mayda, Lukas; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Monahan, Daniele M.; Whaley-Mayda, Lukas; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Monahan, Daniele M.; Whaley-Mayda, Lukas; Fleming, Graham R.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Ishizaki, Akihito] Natl Inst Nat Sci, Inst Mol Sci, Okazaki, Aichi 4448585, Japan. RP Monahan, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM grfleming@lbl.gov OI Fleming, Graham/0000-0003-0847-1838 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geo-sciences, and Biosciences Division, Office of Basic Energy Sciences [DE-AC03-76SF000098]; Japan Society for the Promotion of Science [25708003]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation Graduate Research Fellowship [DGE-1106400] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231; the Division of Chemical Sciences, Geo-sciences, and Biosciences Division, Office of Basic Energy Sciences, through Grant No. DE-AC03-76SF000098 (at Lawrence Berkeley National Laboratory and University of California, Berkeley); and Grants-in-Aid for Scientific Research (Grant No. 25708003) from the Japan Society for the Promotion of Science. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. D.M.M. received a National Science Foundation Graduate Research Fellowship under Grant No. DGE-1106400. NR 79 TC 11 Z9 11 U1 3 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2015 VL 143 IS 6 AR 065101 DI 10.1063/1.4928068 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CP3RT UT WOS:000359799600049 PM 26277167 ER PT J AU Zarkevich, NA Johnson, DD AF Zarkevich, N. A. Johnson, D. D. TI Magneto-structural transformations via a solid-state nudged elastic band method: Application to iron under pressure SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID BCC-HCP TRANSITION; EARTHS INNER-CORE; AB-INITIO; SIMULATION; MAGNETISM; DYNAMICS; POINTS; ENERGY AB We extend the solid-state nudged elastic band method to handle a non-conserved order parameter, in particular, magnetization, that couples to volume and leads to many observed effects in magnetic systems. We apply this formalism to the well-studied magneto-volume collapse during the pressure-induced transformation in iron-from ferromagnetic body-centered cubic (bcc) austenite to hexagonal close-packed (hcp) martensite. We find a bcc-hcp equilibrium coexistence pressure of 8.4 GPa, with the transition-state enthalpy of 156 meV/Fe at this pressure. A discontinuity in magnetization and coherent stress occurs at the transition state, which has a form of a cusp on the potential-energy surface (yet all the atomic and cell degrees of freedom are continuous); the calculated pressure jump of 25 GPa is related to the observed 25 GPa spread in measured coexistence pressures arising from martensitic and coherency stresses in samples. Our results agree with experiments, but necessarily differ from those arising from drag and restricted parametrization methods having improperly constrained or uncontrolled degrees of freedom. (C) 2015 AIP Publishing LLC. C1 [Zarkevich, N. A.; Johnson, D. D.] US DOE, Ames Lab, Ames, IA 50011 USA. [Johnson, D. D.] Iowa State Univ, Mat Sci & Engn, Ames, IA 50011 USA. RP Zarkevich, NA (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM zarkev@ameslab.gov; ddj@ameslab.gov OI Zarkevich, Nikolai/0000-0003-1919-0177; Johnson, Duane/0000-0003-0794-7283 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX We thank Anatoly Belonoshko, Igor Abrikosov, and Iver Anderson for useful discussions. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 39 TC 0 Z9 0 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 14 PY 2015 VL 143 IS 6 AR 064707 DI 10.1063/1.4927778 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CP3RT UT WOS:000359799600038 PM 26277156 ER PT J AU McGonegle, D Milathianaki, D Remington, BA Wark, JS Higginbotham, A AF McGonegle, David Milathianaki, Despina Remington, Bruce A. Wark, Justin S. Higginbotham, Andrew TI Simulations of in situ x-ray diffraction from uniaxially compressed highly textured polycrystalline targets SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SHOCK-WAVE COMPRESSION; HIGH-PRESSURE; PHASE-TRANSITION; LOADED ZIRCONIUM; OMEGA-PHASE; FCC METALS; DEFORMATION; CRYSTALS; ORIENTATION; TRANSFORMATION AB A growing number of shock compression experiments, especially those involving laser compression, are taking advantage of in situ x-ray diffraction as a tool to interrogate structure and microstructure evolution. Although these experiments are becoming increasingly sophisticated, there has been little work on exploiting the textured nature of polycrystalline targets to gain information on sample response. Here, we describe how to generate simulated x-ray diffraction patterns from materials with an arbitrary texture function subject to a general deformation gradient. We will present simulations of Debye-Scherrer x-ray diffraction from highly textured polycrystalline targets that have been subjected to uniaxial compression, as may occur under planar shock conditions. In particular, we study samples with a fibre texture, and find that the azimuthal dependence of the diffraction patterns contains information that, in principle, affords discrimination between a number of similar shock-deformation mechanisms. For certain cases, we compare our method with results obtained by taking the Fourier transform of the atomic positions calculated by classical molecular dynamics simulations. Illustrative results are presented for the shock-induced alpha-epsilon phase transition in iron, the alpha-omega transition in titanium and deformation due to twinning in tantalum that is initially preferentially textured along [001] and [011]. The simulations are relevant to experiments that can now be performed using 4th generation light sources, where single-shot x-ray diffraction patterns from crystals compressed via laser-ablation can be obtained on timescales shorter than a phonon period. (C) 2015 AIP Publishing LLC. C1 [McGonegle, David; Wark, Justin S.; Higginbotham, Andrew] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Milathianaki, Despina] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Remington, Bruce A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP McGonegle, D (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. EM d.mcgonegle1@physics.ox.ac.uk FU LLNL [B595954]; AWE; EPSRC [EP/J017256/1] FX D.M. acknowledges support from LLNL under Subcontract No. B595954. A.H. acknowledges financial support from AWE. J.S.W. is grateful for the support from EPSRC under Grant No. EP/J017256/1 NR 70 TC 2 Z9 2 U1 6 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 14 PY 2015 VL 118 IS 6 AR 065902 DI 10.1063/1.4927275 PG 10 WC Physics, Applied SC Physics GA CP3RK UT WOS:000359798600044 ER PT J AU Jamison, RD Shen, YL AF Jamison, Ryan D. Shen, Yu-Lin TI Indentation-derived elastic modulus of multilayer thin films: Effect of unloading-induced plasticity SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID SINGLE-CRYSTAL MULTILAYERS; METAL-CERAMIC COMPOSITES; X-RAY MICRODIFFRACTION; MECHANICAL-BEHAVIOR; NANOINDENTATION; HARDNESS; MICROSTRUCTURE; COATINGS; DEPTH; WEAR AB Nanoindentation is useful for evaluating the mechanical properties, such as elastic modulus, of multilayer thin film materials. A fundamental assumption in the derivation of the elastic modulus from nanoindentation is that the unloading process is purely elastic. In this work, the validity of elastic assumption as it applies to multilayer thin films is studied using the finite element method. The elastic modulus and hardness from the model system are compared to experimental results to show validity of the model. Plastic strain is shown to increase in the multilayer system during the unloading process. The indentation-derived modulus of a monolayer material shows no dependence on unloading plasticity while the modulus of the multilayer system is dependent on unloading-induced plasticity. Lastly, the cyclic behavior of the multilayer thin film is studied in relation to the influence of unloading-induced plasticity. It is found that several cycles are required to minimize unloading-induced plasticity. C1 [Jamison, Ryan D.] Sandia Natl Labs, Component Sci & Mech, Albuquerque, NM 87185 USA. [Shen, Yu-Lin] Univ New Mexico, Dept Mech Engn, Albuquerque, NM 87131 USA. RP Jamison, RD (reprint author), Sandia Natl Labs, Component Sci & Mech, POB 5800, Albuquerque, NM 87185 USA. EM rdjamis@sandia.gov RI Shen, Yu-Lin/C-1942-2008 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 43 TC 1 Z9 1 U1 0 U2 8 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD AUG 14 PY 2015 VL 30 IS 15 BP 2279 EP 2290 DI 10.1557/jmr.2015.200 PG 12 WC Materials Science, Multidisciplinary SC Materials Science GA CP2PG UT WOS:000359718800002 ER PT J AU He, LY Lu, HF Cao, GQ Hu, H Liu, XJ AF He, Lianyi Lu, Haifeng Cao, Gaoqing Hu, Hui Liu, Xia-Ji TI Quantum fluctuations in the BCS-BEC crossover of two-dimensional Fermi gases SO PHYSICAL REVIEW A LA English DT Article ID EQUATION-OF-STATE; BOSE-CONDENSATION; UNIVERSAL THERMODYNAMICS; 2 DIMENSIONS; SUPERCONDUCTIVITY; TEMPERATURE; SUPERFLUIDITY; TRANSITION; PSEUDOGAP AB We present a theoretical study of the ground state of the BCS-BEC crossover in dilute two-dimensional Fermi gases. While the mean-field theory provides a simple and analytical equation of state, the pressure is equal to that of a noninteracting Fermi gas in the entire BCS-BEC crossover, which is not consistent with the features of a weakly interacting Bose condensate in the BEC limit and a weakly interacting Fermi liquid in the BCS limit. The inadequacy of the two-dimensional mean-field theory indicates that the quantum fluctuations are much more pronounced than those in three dimensions. In this work, we show that the inclusion of the Gaussian quantum fluctuations naturally recovers the above features in both the BEC and the BCS limits. In the BEC limit, the missing logarithmic dependence on the boson chemical potential is recovered by the quantum fluctuations. Near the quantum phase transition from the vacuum to the BEC phase, we compare our equation of state with the known grand canonical equation of state of two-dimensional Bose gases and determine the ratio of the composite boson scattering length a(B) to the fermion scattering length a(2D). We find a(B) similar or equal to 0.56a(2D), in good agreement with the exact four-body calculation. We compare our equation of state in the BCS-BEC crossover with recent results from the quantum Monte Carlo simulations and the experimental measurements and find good agreements. C1 [He, Lianyi] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Lu, Haifeng] Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. [Cao, Gaoqing] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Cao, Gaoqing] Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, Beijing 100084, Peoples R China. [Hu, Hui; Liu, Xia-Ji] Swinburne Univ Technol, Ctr Quantum & Opt Sci, Hawthorn, Vic 3122, Australia. RP He, LY (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM lianyi@lanl.gov RI He, Lianyi/G-5110-2010; HU, Hui/C-6878-2009; Liu, Xia-Ji/C-6888-2009 OI He, Lianyi/0000-0002-9965-0446; HU, Hui/0000-0002-1541-1756; Liu, Xia-Ji/0000-0003-4158-5474 FU U.S. Department of Energy Nuclear Physics Office [DE-AC02-05CH11231]; NSFC [61474018, 11335005]; MOST [2013CB922000, 2014CB845400]; ARC [FT130100815, FT140100003, DP140103231, DP140100637] FX We thank Shiwei Zhang and Hao Shi for helpful discussions and Andrey Turlapov for useful communications. The work of Lianyi He was supported by the U.S. Department of Energy Nuclear Physics Office (Contract No. DE-AC02-05CH11231). Haifeng Lu was supported by NSFC (Grant No. 61474018). Gaoqing Cao acknowledges the support from NSFC (Grant No. 11335005) and MOST (Grants No. 2013CB922000 and No. 2014CB845400). Hui Hu and Xia-Ji Liu were supported by the ARC Discovery Projects (Grants No. FT130100815, No. FT140100003, No. DP140103231, and No. DP140100637). NR 97 TC 17 Z9 17 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD AUG 14 PY 2015 VL 92 IS 2 AR 023620 DI 10.1103/PhysRevA.92.023620 PG 15 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CO9HQ UT WOS:000359486000007 ER PT J AU Cao, SS Qin, GY Bass, SA AF Cao, Shanshan Qin, Guang-You Bass, Steffen A. TI Energy loss, hadronization, and hadronic interactions of heavy flavors in relativistic heavy-ion collisions SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; PB-PB COLLISIONS; ELLIPTIC FLOW; QCD MATTER; MODEL; TEV; COALESCENCE; SCATTERING; MESONS AB We construct a theoretical framework to describe the evolution of heavy flavors produced in relativistic heavy-ion collisions. The in-medium energy loss of heavy quarks is described using our modified Langevin equation that incorporates both quasielastic scatterings and the medium-induced gluon radiation. The space-time profiles of the fireball are described by a (2+1)-dimensional hydrodynamics simulation. A hybrid model of fragmentation and coalescence is utilized for heavy quark hadronization, after which the produced heavy mesons together with the soft hadrons produced from the bulk quark-gluon plasma (QGP) are fed into the hadron cascade ultrarelativistic quantum molecular dynamics (UrQMD) model to simulate the subsequent hadronic interactions. We find that the medium-induced gluon radiation contributes significantly to heavy quark energy loss at high p(T); heavy-light quark coalescence enhances heavy meson production at intermediate pT; and scatterings inside the hadron gas further suppress the D meson R-AA at large p(T) and enhance its v(2). Our calculations provide good descriptions of heavy meson suppression and elliptic flow observed at both the Large Hadron Collider and the Relativistic Heavy-Ion Collider. C1 [Cao, Shanshan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Cao, Shanshan; Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Qin, Guang-You] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Qin, Guang-You] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. RP Cao, SS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367]; Natural Science Foundation of China (NSFC) [11375072] FX We are grateful to the Ohio State University group (Z. Qiu, C. Shen, H. Song, and U. Heinz) for providing the numerical codes of the hydrodynamical evolution and its initialization, and the Texas A&M University group (K. C. Han, R. Fries, and C. M. Ko) for discussions on constructing the coalescence model. We also acknowledge the helpful advice from X.-N. Wang, and the computational resources provided by the Open Science Grid (OSG). This work is funded by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contracts No. DE-AC02-05CH11231 and No. DE-FG02-05ER41367, and within the framework of the JET Collaboration, and by the Natural Science Foundation of China (NSFC) under Grant No. 11375072. NR 77 TC 22 Z9 22 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 14 PY 2015 VL 92 IS 2 AR 024907 DI 10.1103/PhysRevC.92.024907 PG 12 WC Physics, Nuclear SC Physics GA CO9IG UT WOS:000359487800001 ER PT J AU Kumar, V Shukla, P Vogt, R AF Kumar, Vineet Shukla, Prashant Vogt, Ramona TI Quarkonia suppression in PbPb collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; J/PSI SUPPRESSION; LHC; RAPIDITY; PLASMA AB We estimate the modification of quarkonia yields due to different processes in the medium produced in PbPb collisions at LHC energy. The quarkonia and heavy flavor cross sections calculated up to next-to-leading order (NLO) are used in the study. Shadowing corrections are obtained with the NLO EPS09 parametrization. A kinetic model is employed which incorporates quarkonia suppression inside a QGP, suppression due to hadronic comovers, and regeneration from charm pairs. The quarkonia dissociation cross section due to gluon collisions has been considered and the regeneration rate has been obtained using the principle of detailed balance. The modification in quarkonia yields due to collisions with hadronic comovers has been estimated assuming that the comovers are pions. The manifestations of these effects on the nuclear modification factors for both J/psi and Upsilon in different kinematic regions has been demonstrated for PbPb collisions at root s(NN) = 2.76 TeV in comparison with the measurements. Both the suppression and regeneration due to a deconfined medium strongly affect the low and intermediate p(T) range. The large observed suppression of J/psi at p(T) > 10 GeV/c exceeds the estimates of suppression by gluon dissociation. C1 [Kumar, Vineet; Shukla, Prashant] Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. [Kumar, Vineet; Shukla, Prashant] Homi Bhabha Natl Inst, Bombay, Maharashtra, India. [Vogt, Ramona] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94551 USA. [Vogt, Ramona] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. RP Shukla, P (reprint author), Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. EM pshukla@barc.gov.in FU US Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors thank their CMS colleagues for the fruitful discussions, help, and comments. Many of these results were presented at WHEPP and we acknowledge discussions with the participants of the meeting, in particular with D. Das, S. Datta, R. Gavai, S. Gupta, and R. Sharma. The work of R. V. was performed under the auspices of the US Department of Energy, Lawrence Livermore National Laboratory, Contract DE-AC52-07NA27344. NR 43 TC 0 Z9 0 U1 8 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 14 PY 2015 VL 92 IS 2 AR 024908 DI 10.1103/PhysRevC.92.024908 PG 9 WC Physics, Nuclear SC Physics GA CO9IG UT WOS:000359487800002 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJD Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dwuznik, M Dyndal, M Ecker, KM Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M 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Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Francis, D Franconi, L Franklin, M Fraternali, M Freeborn, D French, ST Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fulsom, BG Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gadatsch, S Gadomski, S Gagliardi, G Gagnon, P Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, YS Walls, FMG Garberson, F Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Gatti, C Gaudio, G Gaur, B Gauthier, L Gauzzi, P Gavrilenko, IL Gay, C Gaycken, G Gazis, EN Ge, P Gecse, Z Gee, CNP Geerts, DAA Geich-Gimbel, C Gemme, C Genest, MH Gentile, S George, M George, S Gerbaudo, D Gershon, A Ghazlane, H Ghodbane, N Giacobbe, B Giagu, S Giangiobbe, V Giannetti, P Gianotti, F Gibbard, B Gibson, SM Gilchriese, M Gillam, TPS Gillberg, D Gilles, G Gingrich, DM Giokaris, N Giordani, MP Giorgi, FM Giorgi, FM 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CA ATLAS Collaboration TI Search for high-mass diphoton resonances in pp collisions at pffisffi root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID PHOTON PAIR PRODUCTION; LHC; HIERARCHY; MODEL AB This article describes a search for high-mass resonances decaying to a pair of photons using a sample of 20.3 fb(-1) of pp collisions at root s = 8 TeV recorded with the ATLAS detector at the Large Hadron Collider. The data are found to be in agreement with the Standard Model prediction, and limits are reported in the framework of the Randall-Sundrum model. This theory leads to the prediction of graviton states, the lightest of which could be observed at the Large Hadron Collider. A lower limit of 2.66 (1.41) TeV at 95% confidence level is set on the mass of the lightest graviton for couplings of k/(M) over bar (Pl) = 0.1 (0.01). C1 [Jackson, P.; Lee, L.; McPherson, R. A.; Robertson, S. H.; Soni, N.; White, M. 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[Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Auerbach, B.; Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Paramonov, A.; Price, L. E.; Proudfoot, J.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Carrillo-Montoya, G. D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Phys Dept, Zografos, Greece. [Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; Zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys Engn, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Piccinini, M.; Sbrizzi, A.; Semprini-Cesari, N.; Tupputi, S. A.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hagebck, S.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Isotop & Mol Technol, Natl Inst Res & Dev, Dept Phys, Cluj Napoca, Romania. Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, L.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Guo, J.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Mnig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Mnig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Physik, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Durglishvili, A.; Jejelava, J.; Tskhadadze, E. G.] Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys 4, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Sato, K.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IN USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Phys Dept, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Oda, S.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, School Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Iengo, P.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrument Fis Expt Particula, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.; Wolters, H.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Jakubek, J.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commiss Energie Atom & Energies Alternat, Inst Rech Lois Fondamentales Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. 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RI Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Chekulaev, Sergey/O-1145-2015; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Negrini, Matteo/C-8906-2014; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Tassi, Enrico/K-3958-2015; Livan, Michele/D-7531-2012; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Tikhomirov, Vladimir/M-6194-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Boldyrev, Alexey/M-9684-2015 OI Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Negrini, Matteo/0000-0003-0101-6963; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Livan, Michele/0000-0002-5877-0062; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Tikhomirov, Vladimir/0000-0002-9634-0581; Mitsou, Vasiliki/0000-0002-1533-8886; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; NRC, Canada; I-CORE, Israel FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 39 TC 55 Z9 55 U1 20 U2 100 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 14 PY 2015 VL 92 IS 3 AR 032004 DI 10.1103/PhysRevD.92.032004 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO9IL UT WOS:000359488300001 ER PT J AU Politano, A de Juan, F Chiarello, G Fertig, HA AF Politano, Antonio de Juan, Fernando Chiarello, Gennaro Fertig, Herbert A. TI Emergence of an Out-of-Plane Optical Phonon (ZO) Kohn Anomaly in Quasifreestanding Epitaxial Graphene SO PHYSICAL REVIEW LETTERS LA English DT Article ID GRAPHITE MONOLAYER; NI(111); INTERCALATION; DISPERSION; SURFACE; SPECTROSCOPY; SPECTRUM; PT(111); METAL; YB AB In neutral graphene, two prominent cusps known as Kohn anomalies are found in the phonon dispersion of the highest optical phonon at q = Gamma (LO branch) and q = K (TO branch), reflecting a significant electron-phonon coupling (EPC) to undoped Dirac electrons. In this work, high-resolution electron energy loss spectroscopy is used to measure the phonon dispersion around the Gamma point in quasifreestanding graphene epitaxially grown on Pt(111). The Kohn anomaly for the LO phonon is observed at finite momentum q similar to 2k(F) from Gamma, with a shape in excellent agreement with the theory and consistent with known values of the EPC and the Fermi level. More strikingly, we also observe a Kohn anomaly at the same momentum for the out-of-plane optical phonon (ZO) branch. This observation is the first direct evidence of the coupling of the ZO mode with Dirac electrons, which is forbidden for freestanding graphene but becomes allowed in the presence of a substrate. Moreover, we estimate the EPC to be even greater than that of the LO mode, making graphene on Pt(111) an optimal system to explore the effects of this new coupling in the electronic properties. C1 [Politano, Antonio; Chiarello, Gennaro] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Cs, Italy. [de Juan, Fernando] Lawrence Berkeley Natl Labs, Mat Sci Div, Berkeley, CA 94720 USA. [de Juan, Fernando] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Chiarello, Gennaro] Consorzio Nazl Interuniv Sci Fis Mat, I-00146 Rome, Italy. [Fertig, Herbert A.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. RP Politano, A (reprint author), Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Cs, Italy. RI de Juan, Fernando/B-9392-2008; OI de Juan, Fernando/0000-0001-6852-1484; CHIARELLO, Gennaro/0000-0002-3888-2980 FU "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD); US-Israel Binational Science Foundation FX We thank Davide Campi and Sinisa Coh for helpful discussions. A. P. and G. C. thank Fabio Vito for technical support. F. de J. acknowledges support from the "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD). This work was supported in part by the US-Israel Binational Science Foundation. NR 47 TC 5 Z9 5 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 14 PY 2015 VL 115 IS 7 AR 075504 DI 10.1103/PhysRevLett.115.075504 PG 5 WC Physics, Multidisciplinary SC Physics GA CO9HF UT WOS:000359484800012 PM 26317732 ER PT J AU Kim, J Baik, SS Ryu, SH Sohn, Y Park, S Park, BG Denlinger, J Yi, Y Choi, HJ Kim, KS AF Kim, Jimin Baik, Seung Su Ryu, Sae Hee Sohn, Yeongsup Park, Soohyung Park, Byeong-Gyu Denlinger, Jonathan Yi, Yeonjin Choi, Hyoung Joon Kim, Keun Su TI Observation of tunable band gap and anisotropic Dirac semimetal state in black phosphorus SO SCIENCE LA English DT Article ID ELECTRONIC-STRUCTURE; BILAYER GRAPHENE; FIELD; HETEROSTRUCTURES; MOBILITY; FERMIONS AB Black phosphorus consists of stacked layers of phosphorene, a two-dimensional semiconductor with promising device characteristics. We report the realization of a widely tunable band gap in few-layer black phosphorus doped with potassium using an in situ surface doping technique. Through band structure measurements and calculations, we demonstrate that a vertical electric field from dopants modulates the band gap, owing to the giant Stark effect, and tunes the material from a moderate-gap semiconductor to a band-inverted semimetal. At the critical field of this band inversion, the material becomes a Dirac semimetal with anisotropic dispersion, linear in armchair and quadratic in zigzag directions. The tunable band structure of black phosphorus may allow great flexibility in design and optimization of electronic and optoelectronic devices. C1 [Kim, Jimin; Ryu, Sae Hee; Sohn, Yeongsup; Kim, Keun Su] Pohang Univ Sci & Technol, Dept Phys, Pohang 790784, South Korea. [Baik, Seung Su; Park, Byeong-Gyu; Yi, Yeonjin; Choi, Hyoung Joon] Yonsei Univ, Dept Phys, Seoul 120749, South Korea. [Baik, Seung Su; Choi, Hyoung Joon] Yonsei Univ, Ctr Computat Studies Adv Elect Mat Properties, Seoul 120749, South Korea. [Ryu, Sae Hee; Sohn, Yeongsup; Kim, Keun Su] Inst for Basic Sci Korea, Ctr Artificial Low Dimens Elect Syst, Pohang 790784, South Korea. [Park, Byeong-Gyu] Pohang Univ Sci & Technol, Pohang Accelerator Lab, Pohang 790784, South Korea. [Denlinger, Jonathan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kim, KS (reprint author), Pohang Univ Sci & Technol, Dept Phys, Pohang 790784, South Korea. EM keunsukim@postech.edu RI Choi, Hyoung Joon/N-8933-2015; OI Choi, Hyoung Joon/0000-0001-8565-8597; Kim, Jimin/0000-0002-1690-9396 FU National Research Foundation of Korea [2011-0018306, 2013R1A1A1004778]; Korea Institute of Science and Technology Information Supercomputing Center [KSC-2013-C3-062]; Yonsei University Future-Leading Research Initiative [2014-22-0123]; Ministry of Science, ICT and Future Planning; Pohang University of Science and Technology; U.S. Department of Energy, Office of Sciences [DE-AC02-05CH11231]; [IBS-R014-D1] FX This work was supported by IBS-R014-D1. S.S.B. and H.J.C. acknowledge support from the National Research Foundation of Korea (grant 2011-0018306). Computational resources have been provided by Korea Institute of Science and Technology Information Supercomputing Center (project KSC-2013-C3-062). S.P. and Y.Y. acknowledge support from the National Research Foundation of Korea (grant 2013R1A1A1004778) and Yonsei University Future-Leading Research Initiative of 2014 (2014-22-0123). PLS-II was supported in part by the Ministry of Science, ICT and Future Planning and Pohang University of Science and Technology. The Advanced Light Source was supported by the U.S. Department of Energy, Office of Sciences, under contract DE-AC02-05CH11231. We thank S. W. Jung, W. J. Shin, Y. K. Kim, and B. Kim for help with ARPES experiments. NR 31 TC 93 Z9 95 U1 66 U2 330 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 14 PY 2015 VL 349 IS 6249 BP 723 EP 726 DI 10.1126/science.aaa6486 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO8JO UT WOS:000359415100033 PM 26273052 ER PT J AU Vasseur, R Moore, JE AF Vasseur, Romain Moore, Joel E. TI Multifractal orthogonality catastrophe in one-dimensional random quantum critical points SO PHYSICAL REVIEW B LA English DT Article ID MATRIX RENORMALIZATION-GROUP; ANTI-FERROMAGNETIC CHAIN; ISING SPIN CHAINS; ABSORPTION; METALS AB We study the response of random-singlet quantum critical points to local perturbations. Despite being insulating, these systems are dramatically affected by a local cut in the system, so that the overlap G = vertical bar vertical bar of the ground-state wave functions with and without a cut vanishes algebraically in the thermodynamic limit. We analyze this Anderson orthogonality catastrophe in detail using a real-space renormalization group approach. We show that both the typical value of the overlap G and the disorder average of G(alpha) with alpha > 0 decay as power laws of the system size. In particular, the disorder average of G(alpha) shows a "multifractal" behavior, with a nontrivial limit alpha -> infinity that is dominated by rare events. We also discuss the case of more generic local perturbations and generalize these results to local quantum quenches. C1 [Vasseur, Romain] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Vasseur, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Moore, Joel/O-4959-2016 OI Moore, Joel/0000-0002-4294-5761 FU Quantum Materials program of LBNL; Simons Foundation; NSF [DMR-1206515] FX This work was supported by the Quantum Materials program of LBNL (R.V.), NSF Grant No. DMR-1206515, and the Simons Foundation (J.E.M.). We thank N. Laflorencie, A. Lazarescu, A. C. Potter, Z. Ringel, H. Saleur, and M. Serbyn for insightful discussions. NR 53 TC 4 Z9 4 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 14 PY 2015 VL 92 IS 5 AR 054203 DI 10.1103/PhysRevB.92.054203 PG 11 WC Physics, Condensed Matter SC Physics GA CO9HX UT WOS:000359486700001 ER PT J AU He, W Scharadin, TM Saldana, M Gellner, C Hoang-Phou, S Takanishi, C Hura, GL Tainer, JA Carraway, KL Henderson, PT Coleman, MA AF He, Wei Scharadin, Tiffany M. Saldana, Matthew Gellner, Candice Hoang-Phou, Steven Takanishi, Christina Hura, Gregory L. Tainer, John A. Carraway, Kermit L., III Henderson, Paul T. Coleman, Matthew A. TI Cell-free expression of functional receptor tyrosine kinases SO SCIENTIFIC REPORTS LA English DT Article ID GROWTH-FACTOR RECEPTOR; X-RAY-SCATTERING; NANOLIPOPROTEIN PARTICLES; MEMBRANE-PROTEINS; SAXS; ACTIVATION; ERBB2 AB Receptor tyrosine kinases (RTKs) play critical roles in physiological and pathological processes, and are important anticancer drug targets. In vitro mechanistic and drug discovery studies of full-length RTKs require protein that is both fully functional and free from contaminating proteins. Here we describe a rapid cell-free and detergent-free co-translation method for producing full-length and functional ERBB2 and EGFR receptor tyrosine kinases supported by water-soluble apolipoprotein A-I based nanolipoprotein particles. C1 [He, Wei; Hoang-Phou, Steven; Coleman, Matthew A.] Univ Calif Davis, Sch Med, Radiat Oncol, Sacramento, CA 95817 USA. [Scharadin, Tiffany M.; Gellner, Candice; Takanishi, Christina; Henderson, Paul T.] Univ Calif Davis, Sch Med, Internal Med, Div Hematol Oncol, Sacramento, CA 95817 USA. [Saldana, Matthew; Carraway, Kermit L., III] Univ Calif Davis, Sch Med Biochem & Mol, Sacramento, CA 95817 USA. [Hura, Gregory L.; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Hura, Gregory L.] Univ Calif Santa Cruz, Chem & Biochem, Santa Cruz, CA 95064 USA. [Tainer, John A.] Scripps Res Inst, La Jolla, CA 92037 USA. [Carraway, Kermit L., III; Henderson, Paul T.; Coleman, Matthew A.] Univ Calif Davis, Ctr Comprehens Canc, Sacramento, CA 95817 USA. [Coleman, Matthew A.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Henderson, PT (reprint author), Univ Calif Davis, Sch Med, Internal Med, Div Hematol Oncol, Sacramento, CA 95817 USA. EM paul.henderson@ucdmc.ucdavis.edu; mcoleman@ucdavis.edu OI Coleman, Matthew/0000-0003-1389-4018 FU NIH/NCI [RO1-CA155642-01A]; National Science Foundation grant through the Center for Biophotonics Science and Technology Center [PHY 0120999]; U.S. Department of Energy [DE-AC52-07NA27344]; IDAT through the US Department of Energy, Biological and Environmental Research FX This work was supported by funding from the NIH/NCI (RO1-CA155642-01A) and National Science Foundation grant through the Center for Biophotonics Science and Technology Center, managed by the University of California, Davis under Cooperative Agreement No. PHY 0120999. Work was also performed under the auspices of the U.S. Department of Energy under contract number DE-AC52-07NA27344, which includes IDAT funding through the US Department of Energy, Biological and Environmental Research. NR 24 TC 5 Z9 5 U1 3 U2 13 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 14 PY 2015 VL 5 AR 012896 DI 10.1038/srep12896 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO9EB UT WOS:000359474500001 PM 26274523 ER PT J AU Chaluvadi, H Ozer, ZN Dogan, M Ning, CG Colgan, J Madison, D AF Chaluvadi, Hari Ozer, Zehra Nur Dogan, Mevlut Ning, Chuangang Colgan, James Madison, Don TI Observation of two-center interference effects for electron impact ionization of N-2 SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE electron impact ionization; two-center interference; N-2 ID INTERMEDIATE ENERGIES; MOLECULES AB In 1966, Cohen and Fano (1966 Phys. Rev. 150 30) suggested that one should be able to observe the equivalent of Young's double slit interference if the double slits were replaced by a diatomic molecule. This suggestion inspired many experimental and theoretical studies searching for double slit interference effects both for photon and particle ionization of diatomic molecules. These effects turned out to be so small for particle ionization that this work proceeded slowly and evidence for interference effects were only found by looking at cross section ratios. Most of the early particle work concentrated on double differential cross sections for heavy particle scattering and the first evidence for two-center interference for electron-impact triple differential cross section (TDCS) did not appear until 2006 for ionization of H-2. Subsequent work has now firmly established that two-center interference effects can be seen in the TDCS for electron-impact ionization of H-2. However, in spite of several experimental and theoretical studies, similar effects have not been found for electron-impact ionization of N-2. Here we report the first evidence for two-center interference for electron-impact ionization of N-2. C1 [Chaluvadi, Hari; Madison, Don] Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA. [Ozer, Zehra Nur; Dogan, Mevlut] Afyon Kocatepe Univ, Dept Phys, E COL Lab, TR-03200 Afyon, Turkey. [Ning, Chuangang] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Ning, Chuangang] Tsinghua Univ, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China. [Colgan, James] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Chaluvadi, H (reprint author), Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA. EM zehraerengil@aku.edu.tr RI Ning, chuangang/C-3506-2012 OI Ning, chuangang/0000-0002-3158-1253 FU US National Science Foundation [PHY-1068237]; Texas Advanced Computing Center [TG-MCA07S029]; National Natural Science Foundation of China [11174175]; Scientific and Technological Research Council of Turkey (TUBITAK) [109T738]; BAPK [12.FENED.05] FX H C and D M acknowledge the support of the US National Science Foundation under Grant No. PHY-1068237, XSEDE resources provided [27] by the Texas Advanced Computing Center (Grant No. TG-MCA07S029) and partial computational work was performed with Institutional Computing resources made available through Los Alamos National Laboratory. C G N would like to acknowledge the support of the National Natural Science Foundation of China under Contract No. 11174175. The experimental part of this work was supported by the Scientific and Technological Research Council of Turkey (TUBITAK) through Grant No. 109T738 and by BAPK through Grant No. 12.FENED.05. NR 27 TC 2 Z9 2 U1 3 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD AUG 14 PY 2015 VL 48 IS 15 SI SI AR 155203 DI 10.1088/0953-4075/48/15/155203 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CN6ZV UT WOS:000358584200006 ER PT J AU Jang, GG Jacobs, CB Ivanov, IN Joshi, PC Iii, HMM Kidder, M Armstrong, BL Datskos, PG Graham, DE Moon, JW AF Jang, Gyoung Gug Jacobs, Christopher B. Ivanov, Ilia N. Joshi, Pooran C. Iii, Harry M. Meyer Kidder, Michelle Armstrong, Beth L. Datskos, Panos G. Graham, David E. Moon, Ji-Won TI In situ capping for size control of monochalcogenide (ZnS, CdS and SnS) nanocrystals produced by anaerobic metal-reducing bacteria SO NANOTECHNOLOGY LA English DT Article DE biosynthesis; nanocrystal; quantum dot; monochalcogenide ID QUANTUM DOTS; EXTRACELLULAR SYNTHESIS; NANOPARTICLES AB Metal monochalcogenide quantum dot nanocrystals of ZnS, CdS and SnS were prepared by anaerobic, metal-reducing bacteria using in situ capping by oleic acid or oleylamine. The capping agent preferentially adsorbs on the surface of the nanocrystal, suppressing the growth process in the early stages, thus leading to production of nanocrystals with a diameter of less than 5 nm. C1 [Jang, Gyoung Gug; Datskos, Panos G.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Jacobs, Christopher B.; Ivanov, Ilia N.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Joshi, Pooran C.; Iii, Harry M. Meyer; Armstrong, Beth L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Kidder, Michelle] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Graham, David E.; Moon, Ji-Won] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Jang, GG (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. EM moonj@ornl.gov RI Moon, Ji-Won/A-9186-2011; Graham, David/F-8578-2010; Armstrong, Beth/E-6752-2017; OI Moon, Ji-Won/0000-0001-7776-6889; Graham, David/0000-0001-8968-7344; Armstrong, Beth/0000-0001-7149-3576; Jacobs, Christopher/0000-0001-7906-6368; ivanov, ilia/0000-0002-6726-2502 FU US Department of Energy (DOE), Office of Energy Efficiency & Renewable Energy's Advanced Manufacturing Office, Low Temperature Material Synthesis Program of the Manufacturing Demonstration Facility [CPS 24762]; DOE [DE-AC05-00OR22725]; ORNL Scientific User Facilities Division; DOE Office of Basic Research Sciences; US DOE, Office of Science, Basic Energy Sciences [ERKCC96] FX The authors gratefully acknowledge support from the US Department of Energy (DOE), Office of Energy Efficiency & Renewable Energy's Advanced Manufacturing Office, Low Temperature Material Synthesis Program (CPS 24762) of the Manufacturing Demonstration Facility. Part of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored by the ORNL Scientific User Facilities Division and DOE Office of Basic Research Sciences. FTIR work by M K was supported by the US DOE, Office of Science, Basic Energy Sciences under Award ERKCC96. ORNL is managed by UT-Battelle, LLC, for DOE under contract DE-AC05-00OR22725. The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. NR 20 TC 2 Z9 2 U1 2 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 14 PY 2015 VL 26 IS 32 AR 325602 DI 10.1088/0957-4484/26/32/325602 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CN8IS UT WOS:000358684400011 PM 26207018 ER PT J AU Lavini, F Yang, N Vasudevan, RK Strelcov, E Jesse, S Okatan, MB Kravchenko, I Di Castro, D Kalinin, SV Balestrino, G Aruta, C Foglietti, V AF Lavini, Francesco Yang, Nan Vasudevan, Rama K. Strelcov, E. Jesse, S. Okatan, M. B. Kravchenko, I. Di Castro, Daniele Kalinin, Sergei V. Balestrino, Giuseppe Aruta, Carmela Foglietti, Vittorio TI Bias assisted scanning probe microscopy direct write lithography enables local oxygen enrichment of lanthanum cuprates thin films SO NANOTECHNOLOGY LA English DT Article DE AFM lithography; surface electrochemical processes; tip-induced local oxidation ID DYNAMIC FORCE MICROSCOPY; ELECTROCHEMICAL OXIDATION; NANOSCALE; INTERFACE; SURFACE AB Scanning probe bias techniques have been used as a method to locally dope thin epitaxial films of La2CuO4 (LCO) fabricated by pulsed laser deposition. The local electrochemical oxidation of LCO very efficiently introduces interstitial oxygen defects in the thin film. Details on the influence of the tip voltage bias and environmental conditions on the surface morphology have been investigated. The results show that a local uptake of oxygen occurs in the oxidized films. C1 [Lavini, Francesco; Yang, Nan; Di Castro, Daniele; Balestrino, Giuseppe; Aruta, Carmela; Foglietti, Vittorio] Univ Roma Tor Vergata, Natl Res Council, CNR SPIN, I-00133 Rome, Italy. [Lavini, Francesco; Yang, Nan] Univ Roma Tor Vergata, NAST Ctr, I-00133 Rome, Italy. [Yang, Nan] Univ Niccolo Cusano, Fac Engn, I-00166 Rome, Italy. [Vasudevan, Rama K.; Strelcov, E.; Jesse, S.; Okatan, M. B.; Kravchenko, I.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Di Castro, Daniele; Balestrino, Giuseppe; Aruta, Carmela; Foglietti, Vittorio] Univ Roma Tor Vergata, Dept DICII, I-00133 Rome, Italy. RP Lavini, F (reprint author), Univ Roma Tor Vergata, Natl Res Council, CNR SPIN, I-00133 Rome, Italy. EM vittorio.foglietti@cnr.it RI Kalinin, Sergei/I-9096-2012; Kravchenko, Ivan/K-3022-2015; Aruta, Carmela/L-2957-2015; Jesse, Stephen/D-3975-2016; Okatan, M. Baris/E-1913-2016; Foglietti, Vittorio/J-7052-2012; Vasudevan, Rama/Q-2530-2015 OI Kalinin, Sergei/0000-0001-5354-6152; Kravchenko, Ivan/0000-0003-4999-5822; Aruta, Carmela/0000-0002-6917-6667; Jesse, Stephen/0000-0002-1168-8483; Okatan, M. Baris/0000-0002-9421-7846; Foglietti, Vittorio/0000-0002-9588-5379; DI CASTRO, DANIELE/0000-0002-0878-6904; Vasudevan, Rama/0000-0003-4692-8579 FU Oak Ridge National Laboratory [CNMS2014-053]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; META-Materials Enhancement for Technological Applications Project (FP7-PEOPLE-IRSES-Marie Curie Actions) [PIRSES-GA-2010-269182]; Italian MIUR through the FIRB Project 'Oxides at the nanoscale: multifunctionality and applications' [RBAP115AYN]; PRIN Project OXIDE, 'Oxide Interfaces: Emerging New Properties, Multi-functionality, and Devices for Electronics and Energy' FX The AFM portion of this research was conducted at the Center for Nanophase Materials Sciences (ID: CNMS2014-053), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The authors acknowledge META-Materials Enhancement for Technological Applications Project (FP7-PEOPLE-2010-IRSES-Marie Curie Actions, PIRSES-GA-2010-269182. Italian MIUR is acknowledged for support through the FIRB Project RBAP115AYN 'Oxides at the nanoscale: multifunctionality and applications' and PRIN Project 2010-2011 OXIDE, 'Oxide Interfaces: Emerging New Properties, Multi-functionality, and Devices for Electronics and Energy'. NR 33 TC 0 Z9 0 U1 4 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 14 PY 2015 VL 26 IS 32 AR 325302 DI 10.1088/0957-4484/26/32/325302 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CN8IS UT WOS:000358684400007 PM 26207015 ER PT J AU Ntougias, S Lapidus, A Copeland, A Reddy, TBK Pati, A Ivanova, NN Markowitz, VM Klenk, HP Woyke, T Fasseas, C Kyrpides, NC Zervakis, GI AF Ntougias, Spyridon Lapidus, Alla Copeland, Alex Reddy, T. B. K. Pati, Amrita Ivanova, Natalia N. Markowitz, Victor M. Klenk, Hans-Peter Woyke, Tanja Fasseas, Constantinos Kyrpides, Nikos C. Zervakis, Georgios I. TI High-quality permanent draft genome sequence of the extremely osmotolerant diphenol degrading bacterium Halotalea alkalilenta AW-7(T), and emended description of the genus Halotalea SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Alkaline two-phase olive mill waste; Halomonadaceae; Protocatechuate ortho-cleavage; Catechol to beta-ketoadipate degradation pathway; Cyanate and acrylonitrile detoxification; GEBA-KMG ID MODERATELY HALOPHILIC BACTERIUM; ET-AL. 1989; FAMILY HALOMONADACEAE; SP NOV.; MICROBIAL GENOMES; FRANZMANN 1996; COMB.-NOV.; PROPOSAL; SYSTEM; CLASSIFICATION AB Members of the genus Halotalea (family Halomonadaceae) are of high significance since they can tolerate the greatest glucose and maltose concentrations ever reported for known bacteria and are involved in the degradation of industrial effluents. Here, the characteristics and the permanent-draft genome sequence and annotation of Halotalea alkalilenta AW-7(T) are described. The microorganism was sequenced as a part of the Genomic Encyclopedia of Type Strains, Phase I: the one thousand microbial genomes (KMG) project at the DOE Joint Genome Institute, and it is the only strain within the genus Halotalea having its genome sequenced. The genome is 4,467,826 bp long and consists of 40 scaffolds with 64.62 % average GC content. A total of 4,104 genes were predicted, comprising of 4,028 protein-coding and 76 RNA genes. Most protein-coding genes (87.79 %) were assigned to a putative function. Halotalea alkalilenta AW-7T encodes the catechol and protocatechuate degradation to beta-ketoadipate via the beta-ketoadipate and protocatechuate ortho-cleavage degradation pathway, and it possesses the genetic ability to detoxify fluoroacetate, cyanate and acrylonitrile. An emended description of the genus Halotalea Ntougias et al. 2007 is also provided in order to describe the delayed fermentation ability of the type strain. C1 [Ntougias, Spyridon] Democritus Univ Thrace, Dept Environm Engn, Lab Wastewater Management & Treatment Technol, GR-67100 Xanthi, Greece. [Lapidus, Alla] St Petersburg State Univ, Theodosius Dobzhansky Ctr Genome Bioinformat, St Petersburg 199034, Russia. [Lapidus, Alla] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg, Russia. [Copeland, Alex; Reddy, T. B. K.; Pati, Amrita; Ivanova, Natalia N.; Woyke, Tanja; Kyrpides, Nikos C.] Joint Genome Inst, Genome Biol Program, Dept Energy, Walnut Creek, CA USA. [Markowitz, Victor M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Klenk, Hans-Peter] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Fasseas, Constantinos] Agr Univ Athens, Electron Microscopy Lab, GR-11855 Athens, Greece. [Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Zervakis, Georgios I.] Agr Univ Athens, Lab Gen & Agr Microbiol, GR-11855 Athens, Greece. RP Zervakis, GI (reprint author), Agr Univ Athens, Lab Gen & Agr Microbiol, GR-11855 Athens, Greece. EM zervakis@aua.gr RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017; Lapidus, Alla/I-4348-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Lapidus, Alla/0000-0003-0427-8731; Ntougias, Spyridon/0000-0002-6389-692X; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Russian Ministry of Science Mega-grant [11.G34.31.0068] FX This work was performed under the auspices of the US Department of Energy Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, A.L. was supported in part by Russian Ministry of Science Mega-grant no. 11.G34.31.0068 (PI. Dr Stephen J O'Brien). NR 50 TC 0 Z9 0 U1 0 U2 0 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 13 PY 2015 VL 10 AR 52 DI 10.1186/s40793-015-0052-7 PG 8 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NW UT WOS:000367992000001 PM 26380640 ER PT J AU Aurisano, J Reda, K Johnson, A Marai, EG Leigh, J AF Aurisano, Jillian Reda, Khairi Johnson, Andrew Marai, Elisabeta G. Leigh, Jason TI BactoGeNIE: a large-scale comparative genome visualization for big displays SO BMC BIOINFORMATICS LA English DT Article; Proceedings Paper CT 5th Symposium on Biological Data Visualization CY JUL 10-11, 2015 CL Dublin, IRELAND ID SYNTENY BROWSER; SEQUENCE; CHALLENGES; ALIGNMENT AB Background: The volume of complete bacterial genome sequence data available to comparative genomics researchers is rapidly increasing. However, visualizations in comparative genomics-which aim to enable analysis tasks across collections of genomes-suffer from visual scalability issues. While large, multi-tiled and high-resolution displays have the potential to address scalability issues, new approaches are needed to take advantage of such environments, in order to enable the effective visual analysis of large genomics datasets. Results: In this paper, we present Bacterial Gene Neighborhood Investigation Environment, or BactoGeNIE, a novel and visually scalable design for comparative gene neighborhood analysis on large display environments. We evaluate BactoGeNIE through a case study on close to 700 draft Escherichia coli genomes, and present lessons learned from our design process. Conclusions: BactoGeNIE accommodates comparative tasks over substantially larger collections of neighborhoods than existing tools and explicitly addresses visual scalability. Given current trends in data generation, scalable designs of this type may inform visualization design for large-scale comparative research problems in genomics. C1 [Aurisano, Jillian; Johnson, Andrew; Marai, Elisabeta G.] Univ Illinois, Elect Visualizat Lab, Chicago, IL 60607 USA. [Reda, Khairi] Argonne Natl Lab, Lemont, IL 60439 USA. [Reda, Khairi; Leigh, Jason] Univ Hawaii Manoa, Honolulu, HI 96822 USA. RP Aurisano, J (reprint author), Univ Illinois, Elect Visualizat Lab, Chicago, IL 60607 USA. EM jauris2@uic.edu FU NSF CAREER [IIS1541277, CNS-0959053, OCI-0943559] FX This work and publication has been supported by grants NSF CAREER IIS1541277, CNS-0959053 (CAVE2) and OCI-0943559 (SAGE). Special thanks to the Computational Biology team at Monsanto for providing the motivation and drive for this project, as well as for their help in evaluating BactoGeNIE. Any opinions, findings, and conclusions or recommendations expressed in this publication are those of the authors and do not necessarily reflect the views of the funding agencies and companies. NR 21 TC 1 Z9 1 U1 0 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2105 J9 BMC BIOINFORMATICS JI BMC Bioinformatics PD AUG 13 PY 2015 VL 16 SU 11 AR S6 DI 10.1186/1471-2105-16-S11-S6 PG 14 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Mathematical & Computational Biology SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Mathematical & Computational Biology GA DA5YP UT WOS:000367878900006 PM 26329021 ER PT J AU Chung, D Young, J Cha, M Brunecky, R Bomble, YJ Himmel, ME Westpheling, J AF Chung, Daehwan Young, Jenna Cha, Minseok Brunecky, Roman Bomble, Yannick J. Himmel, Michael E. Westpheling, Janet TI Expression of the Acidothermus cellulolyticus E1 endoglucanase in Caldicellulosiruptor bescii enhances its ability to deconstruct crystalline cellulose SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article ID THERMOPHILUM DSM 6725; PLANT BIOMASS; ANAEROCELLUM-THERMOPHILUM; CLOSTRIDIUM-THERMOCELLUM; DEGRADATION; CONVERSION; CELA; BIOTECHNOLOGY; TEMPERATURE; CELLULASES AB Background: The Caldicellulosiruptor bescii genome encodes a potent set of carbohydrate-active enzymes (CAZymes), found primarily as multi-domain enzymes that exhibit high cellulolytic and hemicellulolytic activity on and allow utilization of a broad range of substrates, including plant biomass without conventional pretreatment. CelA, the most abundant cellulase in the C. bescii secretome, uniquely combines a GH9 endoglucanase and a GH48 exoglucanase in one protein. The most effective commercial enzyme cocktails used in vitro to pretreat biomass are derived from fungal cellulases (cellobiohydrolases, endoglucanases and a beta-D-glucosidases) that act synergistically to release sugars for microbial conversion. The C. bescii genome contains six GH5 domains in five different open reading frames. Four exist in multi-domain proteins and two as single catalytic domains. E1 is a GH5 endoglucanase reported to have high specific activity and simple architecture and is active at the growth temperature of C. bescii. E1 is an endo-1,4-beta-glucanase linked to a family 2 carbohydrate-binding module shown to bind primarily to cellulosic substrates. We tested if the addition of this protein to the C. bescii secretome would improve its cellulolytic activity. Results: In vitro analysis of E1 and CelA shows synergistic interaction. The E1 gene from Acidothermus cellulolyticus was cloned and expressed in C. bescii under the transcriptional control of the C. bescii S-layer promoter, and secretion was directed by the addition of the C. bescii CelA signal peptide sequence. The vector was integrated into the C. bescii chromosome at a site previously showing no detectable detrimental consequence. Increased activity of the secretome of the strain containing E1 was observed on both carboxymethylcellulose (CMC) and Avicel. Activity against CMC increased on average 10.8 % at 65 degrees C and 12.6 % at 75 degrees C. Activity against Avicel increased on average 17.5 % at 65 degrees C and 16.4 % at 75 degrees C. Conclusions: Expression and secretion of E1 in C. bescii enhanced the cellulolytic ability of its secretome. These data agree with in vitro evidence that E1 acts synergistically with CelA to digest cellulose and offer the possibility of engineering additional enzymes for improved biomass deconstruction with the knowledge that C. bescii can express a gene from Acidothermus, and perhaps other heterologous genes, effectively. C1 [Chung, Daehwan; Young, Jenna; Cha, Minseok; Westpheling, Janet] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Brunecky, Roman; Bomble, Yannick J.; Himmel, Michael E.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO USA. [Chung, Daehwan; Young, Jenna; Cha, Minseok; Brunecky, Roman; Bomble, Yannick J.; Himmel, Michael E.; Westpheling, Janet] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA. RP Westpheling, J (reprint author), Univ Georgia, Dept Genet, Athens, GA 30602 USA. EM janwest@uga.edu FU Office of Biological and Environmental Research in the DOE Office of Science FX We thank Elise Snyder for outstanding technical assistance, Sidney Kushner for expert technical advice, Joe Groom for critical review of the manuscript, Charles Wyman and Rajeev Kumar for information about commercial enzyme cocktails. The BioEnergy Science Center is a US Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 37 TC 6 Z9 6 U1 4 U2 21 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 13 PY 2015 VL 8 AR 113 DI 10.1186/s13068-015-0296-x PG 9 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CP8AT UT WOS:000360113600001 PM 26269712 ER PT J AU Tsai, CL Williams, GJ Perry, JJP Tainer, JA AF Tsai, Chi-Lin Williams, Gareth J. Perry, J. Jefferson P. Tainer, John A. TI An AAA plus ATPase Clamshell Targets Transposition SO CELL LA English DT Editorial Material ID ELEMENTS; PROTEINS; MU AB DNA transposition plays key roles in genome diversity, pathogenesis, and evolution. Yet, structural and mechanistic information on transposition targeting and regulation is limited. Arias-Palomo and Berger now define the decameric organization of the AAA+ ATPase IstB, unveiling key insights into its targeting and regulation of IstA transposase activity. C1 [Tsai, Chi-Lin; Williams, Gareth J.; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Perry, J. Jefferson P.] Univ Calif Riverside, Dept Biochem, Riverside, CA 92521 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, Houston, TX 77030 USA. RP Tainer, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. EM jatainer@lbl.gov OI Tsai, Chi-Lin/0000-0002-0365-2405 FU NCI NIH HHS [P01 CA092584]; NIEHS NIH HHS [R21 ES025895, R21ES025895] NR 10 TC 0 Z9 0 U1 0 U2 13 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD AUG 13 PY 2015 VL 162 IS 4 BP 700 EP 702 DI 10.1016/j.cell.2015.07.050 PG 3 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CP2XP UT WOS:000359741400003 PM 26276624 ER PT J AU Zhang, R Alushin, GM Brown, A Nogales, E AF Zhang, Rui Alushin, Gregory M. Brown, Alan Nogales, Eva TI Mechanistic Origin of Microtubule Dynamic Instability and Its Modulation by EB Proteins SO CELL LA English DT Article ID ALPHA-BETA-TUBULIN; GTP HYDROLYSIS; PLUS-END; CRYO-EM; RESOLUTION; LATTICE; TRANSITIONS; TRACKING; COMPLEX; GROWTH AB Microtubule (MT) dynamic instability is driven by GTP hydrolysis and regulated by microtubule-associated proteins, including the plus-end tracking end-binding protein (EB) family. We report six cryo-electron microscopy (cryo-EM) structures of MTs, at 3.5 angstrom or better resolution, bound to GMPCPP, GTP gamma S, or GDP, either decorated with kinesin motor domain after polymerization or copolymerized with EB3. Subtle changes around the E-site nucleotide during hydrolysis trigger conformational changes in alpha-tubulin around an "anchor point,'' leading to global lattice rearrangements and strain generation. Unlike the extended lattice of the GMPCPP-MT, the EB3-bound GTP gamma S-MT has a compacted lattice that differs in lattice twist from that of the also compacted GDP-MT. These results and the observation that EB3 promotes rapid hydrolysis of GMPCPP suggest that EB proteins modulate structural transitions at growing MT ends by recognizing and promoting an intermediate state generated during GTP hydrolysis. Our findings explain both EBs end-tracking behavior and their effect on microtubule dynamics. C1 [Zhang, Rui; Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Alushin, Gregory M.] Univ Calif Berkeley, Biophys Grad Program, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Brown, Alan] MRC, Mol Biol Lab, Cambridge CB2 0QH, England. RP Nogales, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. EM enogales@lbl.gov OI Brown, Alan/0000-0002-0021-0476 FU NIGMS [GM051487] FX We are grateful to Robert Glaeser for the use of the Titan microscope and for stimulating discussions. We thank Anchi Cheng and Tom Houwelling for assistance with Leginon installation and APPION data processing. We thank Alexis Rohou and Nikolaus Grigorieff for guidance in the use of FREALIGN. We also thank Stuart Howes for the purification of kinesin. The kinesin expression construct was a gift from Erik Jonsson and Ron Vale, and the EB3 cDNA was a gift from Clare Waterman. This work was funded by a grant from the NIGMS (GM051487 to E.N.). E.N. is a Howard Hughes Medical Institute investigator. NR 39 TC 48 Z9 48 U1 3 U2 34 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD AUG 13 PY 2015 VL 162 IS 4 BP 849 EP 859 DI 10.1016/j.cell.2015.07.012 PG 11 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CP2XP UT WOS:000359741400017 PM 26234155 ER PT J AU De Silva, N Zahariev, F Hay, BP Gordon, MS Windus, TL AF De Silva, Nuwan Zahariev, Federico Hay, Benjamin P. Gordon, Mark S. Windus, Theresa L. TI Conformations of Organophosphine Oxides SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MOLECULAR-FORCE FIELD; ELECTRON LOCALIZATION FUNCTION; SUPPORTED LIQUID-MEMBRANE; STRUCTURE-BASED DESIGN; PHOSPHINE OXIDE; SOLVENT-EXTRACTION; AQUEOUS-SOLUTIONS; N-DODECANE; MMFF94; ACTINIDES AB The conformations of a series of organophosphine oxides, OP(CH3)(2)R, where R = methyl, ethyl, isopropyl, tert-butyl, vinyl, and phenyl, are predicted using the MP2/cc-pVTZ level of theory. Comparison of potential energy surfaces for rotation about P-C bonds with crystal structure data reveals a strong correlation between predicted location and energetics of minima and histograms of dihedral angle distributions observed in the solid state. In addition, the most stable conformers are those that minimize the extent of steric repulsion between adjacent rotor substituents, and the torsional barriers tend to increase with the steric bulk of the rotating alkyl group. MM3 force field parameters were adjusted to fit the MP2 results, providing a fast and accurate model for predicting organophosphine oxides shapes-an essential part of understanding the chemistry of these compounds. The predictive power of the modified MM3 model was tested against MP2/cc-pVTZ conformations for triethylphosphine oxide, OP(CH2CH3)(3), and triphenylphosphine oxide, OP(Ph)(3). C1 [De Silva, Nuwan; Zahariev, Federico; Gordon, Mark S.; Windus, Theresa L.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [De Silva, Nuwan; Zahariev, Federico; Gordon, Mark S.; Windus, Theresa L.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Hay, Benjamin P.] Supramol Design Inst, Oak Ridge, TN 37830 USA. RP Windus, TL (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM twindus@iastate.edu FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This work is supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 54 TC 1 Z9 1 U1 4 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD AUG 13 PY 2015 VL 119 IS 32 BP 8765 EP 8773 DI 10.1021/acs.jpca.5b04687 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CP2BV UT WOS:000359683400021 PM 26186383 ER PT J AU Ruther, RE Dixit, H Pezeshki, AM Sacci, RL Cooper, VR Nanda, J Veith, GM AF Ruther, Rose E. Dixit, Hemant Pezeshki, Alan M. Sacci, Robert L. Cooper, Valentino R. Nanda, Jagjit Veith, Gabriel M. TI Correlating Local Structure with Electrochemical Activity in Li2MnO3 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LITHIUM-ION BATTERIES; TOTAL-ENERGY CALCULATIONS; SITU RAMAN-SPECTROSCOPY; AUGMENTED-WAVE METHOD; X-RAY-DIFFRACTION; LATTICE-VIBRATIONS; MANGANESE OXIDES; CATHODE MATERIAL; SOLID-SOLUTION; ELECTRODE MATERIALS AB Li2MnO3 is believed to be a critical component of the high capacity Li-rich-manganese-rich oxide materials; however, the mechanism of its electrochemical activity remains controversial. Here, Raman spectroscopy and mapping are used to follow the chemical and structural changes that occur in Li2MnO3 during electrochemical cycling. Conventional composite electrodes cast from a slurry and thin films are studied as a function of the state of charge (voltage) and cycle number. Thin films have similar electrochemical properties as electrodes prepared from slurries but enable spectroscopy of uniform samples without carbon additives and binder. First-principles density functional theory is used to calculate the phonon spectra and identify the Raman-active modes. On the basis of the calculations of phonon spectra for pristine Li2MnO3 and structures with Li vacancies, we discuss the origin of Raman-active peaks observed during the electrochemical cycling. The spectral changes correlate well with the electrochemical behavior and support a mechanism whereby capacity is lost upon extended cycling due to the formation of new manganese oxide phases. C1 [Ruther, Rose E.; Dixit, Hemant; Pezeshki, Alan M.; Sacci, Robert L.; Cooper, Valentino R.; Nanda, Jagjit; Veith, Gabriel M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Pezeshki, Alan M.; Nanda, Jagjit] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. RP Ruther, RE (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM rutherre@ornl.gov; nandaj@ornl.gov RI Cooper, Valentino /A-2070-2012; Ruther, Rose/I-9207-2016 OI Cooper, Valentino /0000-0001-6714-4410; Ruther, Rose/0000-0002-1391-902X FU Assistant Secretary for Energy Efficiency and Renewable Energy; Office of Vehicle Technologies of the U.S. Department of Energy; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science Early Career Research Program; Office of Science of the U.S. Department of Energy [DE-ACO2-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy. H.D. and V.R.C. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, and the Office of Science Early Career Research Program (V.R.C.). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-ACO2-05CH11231. We thank Michael Naguib for assistance with SEM. NR 63 TC 5 Z9 5 U1 10 U2 103 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18022 EP 18029 DI 10.1021/acs.jpcc.5b03900 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800003 ER PT J AU Luo, WF Cowgill, DF AF Luo, Weifang Cowgill, Donald F. TI Kinetics of Hydrogen Isotope Exchange in beta-Phase Pd-H-D SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PALLADIUM; DEUTERIUM; GAS AB Hydrogen isotope gas exchange within palladium powders is examined using a batch-type reactor coupled to a residual gas analyzer (RGA). Exchange rates in both directions (H-2 + PdD and D-2 + PdH) are measured in the temperature range 178-323 K for the samples with different particle sizes. The results show this batch-type exchange is closely approximated as a first-order kinetic process with a rate directly proportional to the surface area of the powder particles. An exchange rate constant of 1.40 +/- 0.24 mu mol H-2/atm cm(2) s is found for H-2 + PdD at 298 K, 1.4 times higher than that for D-2 + PdH, with an activation energy of 25.0 +/- 3.2 kJ/mol H for both exchange directions. A comparison of exchange measurement techniques shows these coefficients, and the fundamental exchange probabilities are in good agreement with those obtained by NMR and flow techniques. C1 [Luo, Weifang; Cowgill, Donald F.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Luo, WF (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM wluo@sandia.gov FU US Department of Energy; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Prof. Ted Flanagan, University of Vermont, for his insight regarding the first-order kinetic behavior, Mr. Kenneth Stewart for design and construction of the experimental apparatus, Dr. Thomas Felter for suggestions regarding the experimental measurements, and Dr. Dave Robinson and Dr. Robert Kolasinski of Sandia National Laboratories for valuable technical review. This work was supported in part by the US Department of Energy. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 14 TC 3 Z9 3 U1 1 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18099 EP 18109 DI 10.1021/acs.jpcc.5b06848 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800012 ER PT J AU Aich, P Wei, HJ Basan, B Kropf, AJ Schweitzer, NM Marshall, CL Miller, JT Meyer, R AF Aich, Payoli Wei, Haojuan Basan, Bridget Kropf, A. Jeremy Schweitzer, Neil M. Marshall, Christopher L. Miller, Jeffrey T. Meyer, Randall TI Single-Atom Alloy Pd-Ag Catalyst for Selective Hydrogenation of Acrolein SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; HETEROGENEOUS CATALYSIS; ALPHA,BETA-UNSATURATED ALDEHYDES; CROTONALDEHYDE HYDROGENATION; SILVER; SENSITIVITY; ADSORPTION; REACTIVITY; MECHANISM AB Pd-Ag alloy catalysts with very dilute amounts of Pd were synthesized. EXAFS results demonstrated that when the concentration of Pd was as low as 0.01 wt %, Pd was completely dispersed as isolated single atoms in Ag nanoparticles. The activity for the hydrogenation of acrolein was improved by the presence of these isolated Pd atoms due to the creation of sites with lower activation energy for H-2 dissociation. In addition, for the same particle size, the 0.01% Pd/8% Ag alloy nanoparticles exhibited higher selectivity than their monometallic counterparts, suggesting that the Pd atom may act as a site for the favorable bonding of the acrolein molecule for facile hydrogenation of the aldehyde functionality. C1 [Aich, Payoli; Wei, Haojuan; Basan, Bridget; Meyer, Randall] Univ Illinois, Dept Chem Engn, Chicago, IL 60607 USA. [Kropf, A. Jeremy; Schweitzer, Neil M.; Marshall, Christopher L.; Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Miller, Jeffrey T.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. RP Meyer, R (reprint author), Univ Illinois, Dept Chem Engn, 810 South Clinton St, Chicago, IL 60607 USA. EM rjm@uic.edu RI ID, MRCAT/G-7586-2011 FU National Science Foundation (CBET) [0747646]; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences; U.S. DOE [DE-ACO2-06CH11357, GU-20770, GU-25167] FX R.J.M., PA., and H.W. gratefully acknowledge funding for this work from the National Science Foundation (CBET Grant Number 0747646). This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. Use of the 10-BM and 10-ID beamlines at the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-ACO2-06CH11357 and general user proposals GU-20770 and GU-25167. We also acknowledge Dr. Hongbo Zhang, Dr. Michael Schwartz, Dr. Richard Pauls, and Dr. Robert McCoy at Argonne National Lab for their discussion, help, and advice while constructing and running the reactor. We also thank Dr. James Gallagher and Guanghui Zhang for helping with the EXAFS experiments done at APS, Argonne National Lab. NR 52 TC 7 Z9 7 U1 28 U2 109 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18140 EP 18148 DI 10.1021/acs.jpcc.5b01357 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800015 ER PT J AU Zeng, ZH Chan, MKY Zhao, ZJ Kubal, J Fan, DX Greeley, J AF Zeng, Zhenhua Chan, Maria K. Y. Zhao, Zhi-Jian Kubal, Joseph Fan, Dingxin Greeley, Jeffrey TI Towards First Principles-Based Prediction of Highly Accurate Electrochemical Pourbaix Diagrams SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID AUGMENTED-WAVE METHOD; MAGNETIC-PROPERTIES; OXYGEN REDUCTION; TRANSITION-METALS; GAMMA-MNOOH; TEMPERATURE; OXIDES; WATER; NICKEL; ADSORPTION AB Electrochemical potential/pH (Pourbaix) diagrams underpin many aqueous electrochemical processes and are central to the identification of stable phases of metals for processes ranging from electrocatalysis to corrosion. Even though standard DFT calculations are potentially powerful tools for the prediction of such diagrams, inherent errors in the description of transition metal (hydroxy)oxides, together with neglect of van der Waals interactions, have limited the reliability of such predictions for even the simplest pure metal bulk compounds, and corresponding predictions for more complex alloy or surface structures are even more challenging. In the present work, through synergistic use of a Hubbard U correction, a state-of-the-art dispersion correction, and a water-based bulk reference state for the calculations, these errors are systematically corrected. The approach describes the weak binding that occurs between hydroxyl-containing functional groups in certain compounds in Pourbaix diagrams, corrects for self-interaction errors in transition metal compounds, and reduces residual errors on oxygen atoms by preserving a consistent oxidation state between the reference state, water, and the relevant bulk phases. The strong performance is illustrated on a series of bulk transition metal (Mn, Fe, Co, and Ni) hydroxides, oxyhydroxides, binary, and ternary oxides, where the corresponding thermodynamics of redox and (de)hydration are described with standard errors of 0.04 eV per reaction formula unit. The approach further preserves accurate descriptions of the overall thermodynamics of electrochemically relevant bulk reactions, such as water formation, which is an essential condition for facilitating accurate analysis of reaction energies for electrochemical processes on surfaces. The overall generality and transferability of the scheme suggests that it may find useful application in the construction of a broad array of electrochemical phase diagrams, including both bulk Pourbaix diagrams and surface phase diagrams of interest for corrosion and electrocatalysis. C1 [Zeng, Zhenhua; Zhao, Zhi-Jian; Kubal, Joseph; Fan, Dingxin; Greeley, Jeffrey] Purdue Univ, Sch Chem Engn, Indiana, PA 47907 USA. [Chan, Maria K. Y.] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. RP Greeley, J (reprint author), Purdue Univ, Sch Chem Engn, Indiana, PA 47907 USA. EM jgreeley@purdue.edu RI Zeng, Zhenhua/E-1795-2012; Zhao, Zhi-Jian/C-8965-2009 OI Zeng, Zhenhua/0000-0002-3087-8581; Zhao, Zhi-Jian/0000-0002-8856-5078 FU DOE Early Career Award of the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported through a DOE Early Career Award of the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. Use of computational resources through the National Energy Research Scientific Computing Center (NERSC) is gratefully acknowledged. NR 80 TC 14 Z9 14 U1 17 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18177 EP 18187 DI 10.1021/acs.jpcc.5b03169 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800019 ER PT J AU Gautam, S Liu, TT Rother, G Jalaivo, N Marmontov, E Welch, S Sheets, J Droege, M Cole, DR AF Gautam, Siddharth Liu, Tingting Rother, Gernot Jalaivo, Niina Marmontov, Eugene Welch, Susan Sheets, Julie Droege, Michael Cole, David R. TI Dynamics of Propane in Nanoporous Silica Aerogel: A Quasielastic Neutron Scattering Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID 2-DIMENSIONAL LATTICE-GAS; POROUS CARBON AEROGEL; MOLECULAR-DYNAMICS; SORBATE CONCENTRATION; SUPERCOOLED WATER; SELF-DIFFUSION; NA-Y; METHANE; FLUID; ADSORPTION AB Molecular motion of hydrocarbons under confinement exhibits several peculiarities and has important implications in industries like gas recovery. A quasielastic neutron scattering (QENS) study of the dynamics of propane in nanoporous silica aerogel was carried out to quantify its molecular mobility. The dynamical properties of propane were studied as a function of temperature, pressure and presence of CO,. The effects of pressure, i.e., fluid density and composition, are found to be more pronounced than the effects of temperature. At low pressures of propane, many propane molecules are adsorbed onto the pore surfaces and are thus immobile. As the pressure of propane loading is increased, more molecules become available to take part in the diffusional dynamics and thus enhance the diffusivity. At low pressure the propane molecules take part in a continuous diffusion, while at higher pressures, the diffusion of propane molecules within the aerogel occurs via the mechanism of jumps. Presence of CO, enhances the jump rate of propane molecules, thereby increasing the diffusion coefficient. This study aims to aid in understanding the complex processes involved in hydrocarbon migration in porous quartz-rich rocks and enhanced hydrocarbon recovery. C1 [Gautam, Siddharth; Liu, Tingting; Welch, Susan; Sheets, Julie; Cole, David R.] Ohio State Univ, Sch Earth Sci, Mendenhall Lab 275, Columbus, OH 43210 USA. [Rother, Gernot] Oak Ridge Natl Lab, Geochem & Interfacial Sci Grp, Div Chem Sci, Oak Ridge, TN 37831 USA. [Jalaivo, Niina] Oak Ridge Natl Lab, Julich Ctr Neutron Sci JCNS 1, Outstat Spallat Neutron Source SNS, Oak Ridge, TN 37831 USA. [Jalaivo, Niina; Marmontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Droege, Michael] Ocellus Inc, Livermore, CA 94551 USA. RP Gautam, S (reprint author), Ohio State Univ, Sch Earth Sci, Mendenhall Lab 275, 125 S Oval Mall, Columbus, OH 43210 USA. EM gautam.25@osu.edu RI Gautam, Siddharth/F-5835-2014; Rother, Gernot/B-7281-2008; OI Gautam, Siddharth/0000-0003-1443-5382; Rother, Gernot/0000-0003-4921-6294; Jalarvo, Niina/0000-0003-0644-6866 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division [DE-SC0006878]; Sloan Foundation; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX This research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research at OSU was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division for S. G. (Contract No. DE-SC0006878) and the Sloan Foundation-funded Deep Carbon Observatory for D.R.C. and J.S. G.R. was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. NR 41 TC 2 Z9 2 U1 5 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18188 EP 18195 DI 10.1021/acs.jpcc.5b03444 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800020 ER PT J AU Liu, ZY Duchon, T Wang, HR Peterson, EW Zhou, YH Luo, S Zhou, J Matolin, V Stacchiola, DJ Rodriguez, JA Senanayake, SD AF Liu, Zongyuan Duchon, Tomas Wang, Huanru Peterson, Erik W. Zhou, Yinghui Luo, Si Zhou, Jing Matolin, Vladimir Stacchiola, Dario J. Rodriguez, Jose A. Senanayake, Sanjaya D. TI Mechanistic Insights of Ethanol Steam Reforming over Ni-CeOx(111): The Importance of Hydroxyl Groups for Suppressing Coke Formation SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TEMPERATURE-PROGRAMMED DESORPTION; RAY PHOTOELECTRON-SPECTROSCOPY; FILM CERIUM OXIDE; H-2 PRODUCTION; THIN-FILMS; THERMAL-REACTIONS; SINGLE-CRYSTAL; PARTICLE-SIZE; CU CATALYSTS; FUEL-CELL AB We have studied the reaction of ethanol and water over Ni-CeO2-x(111) model surfaces to elucidate the mechanistic steps associated with the ethanol steam reforming (ESR) reaction. Our results provide insights about the importance of hydroxyl groups to the ESR reaction over Ni-based catalysts. Systematically, we have investigated the reaction of ethanol on Ni-CeO2-x(111) at varying Ce3+ concentrations (CeO1.8-2.0) with absence/presence of water using a combination of soft X-ray photoelectron spectroscopy (sXPS) and temperature-programmed desorption (TPD). Consistent with previous reports, upon annealing, metallic Ni formed on reduced ceria while NiO was the main component on fully oxidized ceria. Ni is the active phase leading to both the C-C and C-H cleavage of ethanol but is also responsible for carbon accumulation or coking. We have identified a Ni3C phase that formed prior to the formation of coke. At temperatures above 600 K, the lattice oxygen from ceria and the hydroxyl groups from water interact cooperatively in the removal of coke, likely through a strong metal support interaction between nickel and ceria that facilitates oxygen transfer. C1 [Senanayake, Sanjaya D.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Liu, Zongyuan; Luo, Si; Rodriguez, Jose A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Liu, Zongyuan; Luo, Si; Stacchiola, Dario J.; Rodriguez, Jose A.; Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Duchon, Tomas; Matolin, Vladimir] Charles Univ Prague, Fac Math & Phys, Prague 8, Czech Republic. [Wang, Huanru] Beijing Res Inst Chem Ind, Analyt Res Div, Beijing, Peoples R China. [Peterson, Erik W.; Zhou, Yinghui; Zhou, Jing] Univ Wyoming, Dept Chem, Laramie, WY 82071 USA. RP Senanayake, SD (reprint author), Brookhaven Natl Lab, Bldg 555A,POB 5000, Upton, NY 11973 USA. EM ssenanay@bnl.gov RI Stacchiola, Dario/B-1918-2009; Peterson, Erik/L-4236-2013; Senanayake, Sanjaya/D-4769-2009; OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232; Liu, Zongyuan/0000-0001-8526-5590 FU U.S. Department of Energy, Office of Science [DE-SC0012704]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704]; Department of Chemistry, University of Wyoming [CHE1151846] FX The research carried out at National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences under Contract No. DE-SC0012704. The STM data were obtained at Department of Chemistry, University of Wyoming under Contract No. CHE1151846). This work used resources of the National Synchrotron Light Source (NSLS) which are DOE Office of Science User Facilities. NR 55 TC 8 Z9 8 U1 13 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18248 EP 18256 DI 10.1021/acs.jpcc.5b04310 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800028 ER PT J AU Klaus, S Louie, MW Trotochaud, L Bell, AT AF Klaus, Shannon Louie, Mary W. Trotochaud, Lena Bell, Alexis T. TI Role of Catalyst Preparation on the Electrocatalytic Activity of Ni1-xFexOOH for the Oxygen Evolution Reaction SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ALKALINE WATER ELECTROLYSIS; SITU RAMAN-SPECTROSCOPY; ELECTROCHEMICAL EVOLUTION; FILM ELECTRODES; HYDROXIDE FILM; NICKEL-OXIDE; THIN-FILMS; IRON; METAL; PHOTOANODES AB Ni1-xFexOOH thin films prepared via cathodic electrodeposition have been demonstrated to be highly active catalysts for the oxygen evolution reaction (OER) in basic media: Integration of these catalysts with light-absorbing semiconductors is required for photoelectrochemical fuel generation. However, the application of cathodic potentials required for typical electrochemical catalyst deposition limits the library of compatible photoanode materials. Sputter deposition of catalysts circumvents this limitation by enabling facile catalyst layering without cathodic potentials. In this work, we compare the structure and OER activity of sputter-deposited and electrodeposited Ni1-xFexOOH thin films. Electrochemical cycling converts sputtered Ni1-xFex metallic films to the desired mddes/(oxy)hydroxides. Both film preparation methods give catalysts with similar electrochemical behavior across all compositions. Additionally, OER activity is comparable between the deposition methods, with maximum activity for films with similar to 20% Fe content (320 mV overpotential at j = 10 mA cm(-2) geometric). Electrochemical cycling to convert sputtered metallic Ni1-xFex films to metal oxides/(oxy)hydroxides is found to lower the Fe/Ni ratio, while the electrodeposited films exhibit comparable Fe/Ni ratios before and after electrochemical cycling and characterization. Structurally, Fe is found to incorporate within the Ni(OH)(2)/NiOOH lattice for films formed through both sputter-deposition and electrodeposition. Layered films were also compared to codeposited 1:1 Fe/Ni films. It is found that, for layered films, an Fe top layer inhibits the electrochemical conversion of metallic Ni to Ni(OH)(2)/NiOOH, thus reducing the amount of Ni1-xFexOOH OER-active phase formed. In contrast, migration of metals within Ni-on-top films occurs readily during electrochemical cycling, resulting in films that are structurally and electrochemically indistinguishable from codeposited Ni1-xFexOOH. These findings enable direct application of Ni1-xFexOOH sputtered films to a wider library of photoanodes for light-driven water-splitting applications. C1 [Bell, Alexis T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Bell, AT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM bell@cchem.berkeley.edu FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; University of California President's Postdoctoral Fellowship Program FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. M.W.L. was partially supported by the University of California President's Postdoctoral Fellowship Program. The authors gratefully acknowledge Le Chen and Alan Lyon (Joint Center for Artificial Photosynthesis) for helpful discussions and assistance with sputter deposition, Jason Cooper and Jinhui Yang for assistance with XPS measurements, and Eric Granlund (University of California, Berkeley, College of Chemistry) for the fabrication of our electrode and sputtering components. NR 46 TC 20 Z9 20 U1 17 U2 128 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18303 EP 18316 DI 10.1021/acs.jpcc.5b04776 PG 14 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800034 ER PT J AU Kestell, J Boscoboinik, JA Cheng, LX Garvey, M Bennett, DW Tysoe, WT AF Kestell, John Boscoboinik, J. Anibal Cheng, Lanxia Garvey, Michael Bennett, Dennis W. Tysoe, Wilfred T. TI Structural Changes in Self-Catalyzed Adsorption of Carbon Monoxide on 1,4-Phenylene Diisocyanide Modified Au(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; COORDINATION POLYMERS; CO CHEMISORPTION; CHEMICAL-STABILITY; ARYL ISOCYANIDES; METAL-SURFACES; POWDERED GOLD; BASIS-SET; PALLADIUM AB The self-accelerated adsorption of CO on 1,4-phenylene diisoc-yanide (PDI)-derived oligomers on Au(111) is explored by reflection absorption infrared spectroscopy and scanning tunneling microscopy. PDI incorporates gold adatoms from the Au(111) surface to form one-dimensional -(Au-PDI)(n)- chains that can also connect between gold nanoparticles on mica to form a conductive pathway between them. CO adsorption occurs in two stages; it first adsorbs adjacent to the oligomers that move to optimize CO adsorption. Further CO exposure induces PDI decoordination to form Au PDI adatom complexes thereby causing the conductivity of a PDI-linked gold nanoparticle array on mica to decrease to act as a chemically drive molecular switch. This simple system enables the adsorption process to be explored in detail. DFT calculations reveal that both the (Au-PDI)(n)- oligomer chain and the Au PDI adatom complex are stabilized by coadsorbed CO. A kinetic "foot-in-the-door" model is proposed in which fluctuations in PDI coordination allow CO to diffuse into the gap between gold adatoms to prevent the PDI from reattaching, thereby allowing additional CO to adsorb, to provide kinetic model for allosteric CO adsorption on PDI-covered gold. C1 [Kestell, John; Cheng, Lanxia; Garvey, Michael; Bennett, Dennis W.; Tysoe, Wilfred T.] Univ Wisconsin, Dept Chem, Milwaukee, WI 53211 USA. [Kestell, John; Cheng, Lanxia; Garvey, Michael; Bennett, Dennis W.; Tysoe, Wilfred T.] Univ Wisconsin, Surface Studies Lab, Milwaukee, WI 53211 USA. [Boscoboinik, J. Anibal] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Tysoe, WT (reprint author), Univ Wisconsin, Dept Chem, POB 413, Milwaukee, WI 53211 USA. EM wtt@uwm.edu OI Cheng, Lanxia/0000-0002-3712-0693 NR 51 TC 5 Z9 5 U1 4 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18317 EP 18325 DI 10.1021/acs.jpcc.5b04783 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800035 ER PT J AU Zhu, K Xia, YB Tang, MR Wang, ZT Lyubinetsky, I Ge, QF Dohnalek, Z Park, KT Zhang, ZR AF Zhu, Ke Xia, Yaobiao Tang, Miru Wang, Zhi-Tao Lyubinetsky, Igor Ge, Qingfeng Dohnalek, Zdenek Park, Kenneth T. Zhang, Zhenrong TI Low-Temperature Reductive Coupling of Formaldehyde on Rutile TiO2(110) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENERGY-LOSS SPECTROSCOPY; REDUCED TIO2(110); TITANIUM-DIOXIDE; SURFACE; ADSORPTION; MODEL; OXIDE; 1ST-PRINCIPLES; DECOMPOSITION; ACETALDEHYDE AB The formation and coupling of methylene upon dissociation of formaldehyde on reduced TiO2(110) are studied using variable temperature scanning tunneling microscopy (STM). In agreement with prior studies, formaldehyde preferably adsorbs on the bridging-bonded oxygen vacancy (V-O) defect site. V-O-bound formaldehyde couples with Ti-bound formaldehyde forming a diolate species, which appears as the majority species on the surface at 300 K. Here, STM images directly visualize a low-temperature coupling reaction channel. Two V-O-bound formaldehyde molecules can couple and form Ti-bound species, which desorbs above similar to 215 K. This coupling reaction heals both V-O sites indicating the formation and the desorption of ethylene. We also directly observed the diffusion of methylene groups to nearby empty V-O sites upon dissociation of the C-O bond in V-O-bound formaldehyde, which suggests that the ethylene formation occurs via coupling of the methylene groups. Statistical analysis shows that the sum of visible reaction products on the surface can only account for a half of the consumption of the initial V-O coverage, which further supports the desorption of the coupling reaction product, ethylene, after formaldehyde exposure between 215 and 300 K. C1 [Zhu, Ke; Xia, Yaobiao; Park, Kenneth T.; Zhang, Zhenrong] Baylor Univ, Dept Phys, Waco, TX 76798 USA. [Tang, Miru; Ge, Qingfeng] So Illinois Univ, Dept Chem & Biochem, Carbondale, IL 62901 USA. [Wang, Zhi-Tao; Lyubinetsky, Igor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Dohnalek, Zdenek] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Inst Interfacial Catalysis, Richland, WA 99354 USA. RP Zhang, ZR (reprint author), Baylor Univ, Dept Phys, Waco, TX 76798 USA. EM Kenneth_Park@baylor.edu; Zhenrong_Zhang@baylor.edu RI Ge, Qingfeng/A-8498-2009 OI Ge, Qingfeng/0000-0001-6026-6693 FU American Chemical Society Petroleum Research Fund; U.S. Department of Energy (DOE) Basic Energy Science (BES) [DE-FG-05ER46231]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL); U.S. DOE [DE-AC06-76RLO 1830] FX Acknowledgment is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research. M.T. and Q.G. acknowledge support by U.S. Department of Energy (DOE) Basic Energy Science (BES) Grant DE-FG-05ER46231. Z.T.W., I.L, and Z.D. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. A part of the experimental work was performed using EMSL, a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the U.S. DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. NR 34 TC 8 Z9 8 U1 4 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18452 EP 18457 DI 10.1021/acs.jpcc.5b05639 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800048 ER PT J AU Stoerzinger, KA Hong, WT Azimi, G Giordano, L Lee, YL Crumlin, EJ Biegalski, MD Bluhm, H Varanasi, KK Shao-Horn, Y AF Stoerzinger, Kelsey A. Hong, Wesley T. Azimi, Gisele Giordano, Livia Lee, Yueh-Lin Crumlin, Ethan J. Biegalski, Michael D. Bluhm, Hendrik Varanasi, Kripa K. Shao-Horn, Yang TI Reactivity of Perovskites with Water: Role of Hydroxylation in Wetting and Implications for Oxygen Electrocatalysis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; NEAR-AMBIENT CONDITIONS; METAL-OXIDE SURFACES; CONTACT-ANGLE; ELECTRONIC-STRUCTURE; NEUTRON-DIFFRACTION; FUNDAMENTAL-ASPECTS; SOLID-SURFACES; PRESSURE; FILMS AB Oxides are instrumental to applications such as catalysis, sensing, and wetting, where the reactivity with water can greatly influence their functionalities. We find that the coverage of hydroxyls (*OH) measured at fixed relative humidity trends with the electron-donor (basic) character of wetted perovskite oxide surfaces. Using ambient pressure X-ray photoelectron spectroscopy, we report that the affinity toward hydroxylation, coincident with strong adsorption energies calculated for dissociated water and hydroxyl groups, leads to strong H bonding that is favorable for wetting while detrimental to catalysis of the oxygen reduction reaction (ORR). Our findings provide novel insights into the coupling between wetting and catalytic activity and suggest that catalyst hydrophobicity should be considered in aqueous oxygen electrocatalysis. C1 [Stoerzinger, Kelsey A.; Hong, Wesley T.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Azimi, Gisele; Giordano, Livia; Lee, Yueh-Lin; Varanasi, Kripa K.; Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Giordano, Livia] Univ Milano Biocca, Dipartimento Sci Mat, I-20125 Milan, Italy. [Crumlin, Ethan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Varanasi, KK (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM varanasi@mit.edu; shaohorn@mit.edu RI LEE, YUEH-LIN/F-6274-2011; OI LEE, YUEH-LIN/0000-0003-2477-6412; Stoerzinger, Kelsey/0000-0002-3431-8290 FU MRSEC Program of the NSF [DMR-0819762]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US DOE at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; NSF Graduate Research Fellowship [DGE-1122374]; NSF Career Award [0952564] FX This work was supported in part by the MRSEC Program of the NSF under Award DMR-0819762. The ALS and the MES beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US DOE at the Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. The PLD film growth was conducted at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility. Computations benefited from use of the National Energy Research Scientific Computing Center allocation at Oak Ridge National Laboratory. K.A.S. was supported in part by the NSF Graduate Research Fellowship under Grant DGE-1122374. K.K.V. acknowledges the support from NSF Career Award (0952564). We thank Srinivas P. B. Subramanyam and Andrey Shavorskiy for experimental assistance and Milind Gadre and Dane Morgan for helpful discussions. NR 68 TC 11 Z9 11 U1 6 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 13 PY 2015 VL 119 IS 32 BP 18504 EP 18512 DI 10.1021/acs.jpcc.5b06621 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CP2BZ UT WOS:000359683800054 ER PT J AU Albertin, CB Simakov, O Mitros, T Wang, ZY Pungor, JR Edsinger-Gonzales, E Brenner, S Ragsdale, CW Rokhsar, DS AF Albertin, Caroline B. Simakov, Oleg Mitros, Therese Wang, Z. Yan Pungor, Judit R. Edsinger-Gonzales, Eric Brenner, Sydney Ragsdale, Clifton W. Rokhsar, Daniel S. TI The octopus genome and the evolution of cephalopod neural and morphological novelties SO NATURE LA English DT Article ID RNA-SEQ; SACCHAROMYCES-CEREVISIAE; PHYLOGENETIC TREES; BINDING DOMAIN; GENE-CLUSTER; GENERATION; ALIGNMENT; COMPLEXITY; ELEMENTS; DATABASE AB Coleoid cephalopods (octopus, squid and cuttlefish) are active, resourceful predators with a rich behavioural repertoire(1). They have the largest nervous systems among the invertebrates(2) and present other striking morphological innovations including camera-like eyes, prehensile arms, a highly derived early embryogenesis and a remarkably sophisticated adaptive colouration system(1,3). To investigate the molecular bases of cephalopod brain and body innovations, we sequenced the genome and multiple transcriptomes of the California two-spot octopus, Octopus bimaculoides. We found no evidence for hypothesized whole-genome duplications in the octopus lineage(4-6). The core developmental and neuronal gene repertoire of the octopus is broadly similar to that found across invertebrate bilaterians, except for massive expansions in two gene families previously thought to be uniquely enlarged in vertebrates: the protocadherins, which regulate neuronal development, and the C2H2 superfamily of zinc-finger transcription factors. Extensive messenger RNA editing generates transcript and protein diversity in genes involved in neural excitability, as previously described(7), as well as in genes participating in a broad range of other cellular functions. We identified hundreds of cephalopod-specific genes, many of which showed elevated expression levels in such specialized structures as the skin, the suckers and the nervous system. Finally, we found evidence for large-scale genomic rearrangements that are closely associated with transposable element expansions. Our analysis suggests that substantial expansion of a handful of gene families, along with extensive remodelling of genome linkage and repetitive content, played a critical role in the evolution of cephalopod morphological innovations, including their large and complex nervous systems. C1 [Albertin, Caroline B.; Ragsdale, Clifton W.] Univ Chicago, Dept Organismal Biol & Anat, Chicago, IL 60637 USA. [Simakov, Oleg; Edsinger-Gonzales, Eric; Brenner, Sydney; Rokhsar, Daniel S.] Grad Univ, Okinawa Inst Sci & Technol, Onna, Okinawa 9040495, Japan. [Simakov, Oleg] Heidelberg Univ, Ctr Organismal Studies, D-69117 Heidelberg, Germany. [Mitros, Therese; Edsinger-Gonzales, Eric; Rokhsar, Daniel S.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Wang, Z. Yan; Pungor, Judit R.; Ragsdale, Clifton W.] Univ Chicago, Dept Neurobiol, Chicago, IL 60637 USA. [Rokhsar, Daniel S.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Ragsdale, CW (reprint author), Univ Chicago, Dept Organismal Biol & Anat, 1025 E 57Th St, Chicago, IL 60637 USA. EM cragsdale@uchicago.edu; dsrokhsar@gmail.com RI Simakov, Oleg/G-4572-2015; OI Simakov, Oleg/0000-0002-3585-4511; Wang, Z Yan/0000-0002-7094-1696 FU Molecular Genetics Unit of the Okinawa Institute of Science and Technology Graduate University; NSF [IOS-1354898, DGE-0903637]; NIH [R03 HD064887, S10RR029668, S10RR027303]; University of Chicago Functional Genomics Facility by NIH [UL1 TR000430] FX We thank C. T. Brown and J. Rosenthal for making Doryteuthis RNA-seq data available before publication; C. Ha, J. Orenstein, J. Brandenburger, M. Glotzer and H. Gui for bioinformatic assistance; S. Shigeno for help with tissue dissection; C. Huffard and R. Caldwell for providing the O. bimaculoides specimen used for genomic DNA isolation; and E. Begovic for genomic DNA preparation. This work was supported by the Molecular Genetics Unit of the Okinawa Institute of Science and Technology Graduate University (S.B. and D.S.R.) and by funding from the NSF (IOS-1354898) and NIH (R03 HD064887) to C.W.R. and from the NSF (DGE-0903637) to Z.Y.W. This work used the Vincent J. Coates Genomics Sequencing Laboratory at UC Berkeley, supported by NIH S10 instrumentation grants S10RR029668 and S10RR027303, and the University of Chicago Functional Genomics Facility, supported by NIH grant UL1 TR000430. NR 58 TC 59 Z9 59 U1 26 U2 171 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 13 PY 2015 VL 524 IS 7564 BP 220 EP + DI 10.1038/nature14668 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO8AM UT WOS:000359386900032 PM 26268193 ER PT J AU Bai, YH McCoy, JG Levin, EJ Sobrado, P Rajashankar, KR Fox, BG Zhou, M AF Bai, Yonghong McCoy, Jason G. Levin, Elena J. Sobrado, Pablo Rajashankar, Kanagalaghatta R. Fox, Brian G. Zhou, Ming TI X-ray structure of a mammalian stearoyl-CoA desaturase SO NATURE LA English DT Article ID FATTY-ACID DESATURATION; COENZYME-A DESATURASE; SUBSTRATE-SPECIFICITY; CRYSTAL-STRUCTURE; DIIRON PROTEINS; RIBONUCLEOTIDE REDUCTASE; SACCHAROMYCES-CEREVISIAE; MECHANISM; ENZYME; IDENTIFICATION AB Stearoyl-CoA desaturase (SCD) is conserved in all eukaryotes and introduces the first double bond into saturated fatty acyl-CoAs1-4. Because the monounsaturated products of SCD are key precursors of membrane phospholipids, cholesterol esters and triglycerides, SCD is pivotal in fatty acid metabolism. Humans have two SCD homologues (SCD1 and SCD5), while mice have four (SCD1-SCD4). SCD1-deficient mice do not become obese or diabetic when fed a high-fat diet because of improved lipid metabolic profiles and insulin sensitivity(5,6). Thus, SCD1 is a pharmacological target in the treatment of obesity, diabetes and other metabolic diseases(7). SCD1 is an integral membrane protein located in the endoplasmic reticulum, and catalyses the formation of a cis-double bond between the ninth and tenth carbons of stearoyl-or palmitoyl-CoA(8,9). The reaction requires molecular oxygen, which is activated by a di-iron centre, and cytochrome b(5), which regenerates the di-iron centre(10). To understand better the structural basis of these characteristics of SCD function, here we crystallize and solve the structure of mouse SCD1 bound to stearoyl-CoA at 2.6 angstrom resolution. The structure shows a novel fold comprising four transmembrane helices capped by a cytosolic domain, and a plausible pathway for lateral substrate access and product egress. The acyl chain of the bound stearoyl-CoA is enclosed in a tunnel buried in the cytosolic domain, and the geometry of the tunnel and the conformation of the bound acyl chain provide a structural basis for the regioselectivity and stereospecificity of the desaturation reaction. The dimetal centre is coordinated by a unique spacial arrangement of nine conserved histidine residues that implies a potentially novel mechanism for oxygen activation. The structure also illustrates a possible route for electron transfer from cytochrome b5 to the di-iron centre. C1 [Bai, Yonghong; McCoy, Jason G.; Levin, Elena J.; Zhou, Ming] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Sobrado, Pablo; Fox, Brian G.] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, NE CAT, Argonne, IL 60439 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, Dept Chem & Chem Biol, Argonne, IL 60439 USA. RP Zhou, M (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. EM bgfox@biochem.wisc.edu; mzhou@bcm.edu FU US National Institutes of Health [R01DK088057, R01GM098878, R01HL086392, U54GM095315, U54GM094584, R01GM050853]; American Heart Association [12EIA8850017]; Cancer Prevention and Research Institute of Texas [R12MZ]; National Institute of General Medical Sciences [P41GM103403] FX This work was supported by the US National Institutes of Health (R01DK088057, R01GM098878, R01HL086392, U54GM095315, U54GM094584 and R01GM050853), the American Heart Association (12EIA8850017), and the Cancer Prevention and Research Institute of Texas (R12MZ). Final data were collected at Northeastern Collaborative Access Team (NE-CAT) beamlines, which are supported by a grant from the National Institute of General Medical Sciences (P41GM103403). Crystals were screened at beamline 17-ID at the Advanced Photon Source, beamlines 8.2.2 and 5.0.2 at Berkeley Center for Structural Biology at the Lawrence Berkeley Laboratory. NR 49 TC 16 Z9 19 U1 12 U2 42 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 13 PY 2015 VL 524 IS 7564 BP 252 EP + DI 10.1038/nature14549 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO8AM UT WOS:000359386900039 PM 26098370 ER PT J AU Aguilar-Arevalo, A Aoki, M Blecher, M Britton, DI Bryman, DA vom Bruch, D Chen, S Comfort, J Ding, M Doria, L Cuen-Rochin, S Gumplinger, P Hussein, A Igarashi, Y Ito, S Kettell, SH Kurchaninov, L Littenberg, LS Malbrunot, C Mischke, RE Numao, T Protopopescu, D Sher, A Sullivan, T Vavilov, D Yamada, K AF Aguilar-Arevalo, A. Aoki, M. Blecher, M. Britton, D. I. Bryman, D. A. vom Bruch, D. Chen, S. Comfort, J. Ding, M. Doria, L. Cuen-Rochin, S. Gumplinger, P. Hussein, A. Igarashi, Y. Ito, S. Kettell, S. H. Kurchaninov, L. Littenberg, L. S. Malbrunot, C. Mischke, R. E. Numao, T. Protopopescu, D. Sher, A. Sullivan, T. Vavilov, D. Yamada, K. TI Improved Measurement of the pi -> e nu Branching Ratio SO PHYSICAL REVIEW LETTERS LA English DT Article ID DECAYS; NEUTRINOS; DETECTOR; MODEL AB A new measurement of the branching ratio R-e/mu= Gamma(pi(+) -> e(+)nu + pi(+) -> e(+)nu gamma)/Gamma(pi(+) -> mu(+)nu+pi(+) -> mu(+)nu gamma) resulted in R-e/mu(exp) = [1.2344 +/- 0.0023(stat) +/- 0.0019(syst)] x 10(-4). This is in agreement with the standard model prediction and improves the test of electron-muon universality to the level of 0.1%. C1 [Aguilar-Arevalo, A.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Aoki, M.; Ito, S.; Sullivan, T.] Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan. [Blecher, M.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Britton, D. I.; Protopopescu, D.] Univ Glasgow, Dept Phys, Glasgow G12 8QQ, Lanark, Scotland. [Bryman, D. A.; vom Bruch, D.; Cuen-Rochin, S.; Malbrunot, C.; Sullivan, T.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Chen, S.; Ding, M.] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Comfort, J.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Doria, L.; Gumplinger, P.; Kurchaninov, L.; Mischke, R. E.; Numao, T.; Sher, A.; Vavilov, D.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Hussein, A.] Univ No British Columbia, Prince George, BC V2N 4Z9, Canada. [Igarashi, Y.] KEK, Tsukuba, Ibaraki 3050801, Japan. [Kettell, S. H.; Littenberg, L. S.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Aguilar-Arevalo, A (reprint author), Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. OI Aguilar-Arevalo, Alexis A./0000-0001-9279-3375 FU Natural Sciences and Engineering Research Council; TRIUMF from the National Research Council of Canada; Research Fund for the Doctoral Program of Higher Education of China; CONACYT doctoral fellowship from Mexico; JSPS KAKENHI in Japan [18540274, 21340059, 24224006] FX This work was supported by the Natural Sciences and Engineering Research Council and TRIUMF through a contribution from the National Research Council of Canada, and by the Research Fund for the Doctoral Program of Higher Education of China, by CONACYT doctoral fellowship from Mexico, and by JSPS KAKENHI Grants No. 18540274, No. 21340059, and No. 24224006 in Japan. We are grateful to Brookhaven National Laboratory for the loan of the crystals and to the TRIUMF operations, detector, electronics, and DAQ groups for their engineering and technical support. NR 21 TC 3 Z9 3 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 13 PY 2015 VL 115 IS 7 AR 071801 DI 10.1103/PhysRevLett.115.071801 PG 5 WC Physics, Multidisciplinary SC Physics GA CO8RC UT WOS:000359437000007 PM 26317713 ER PT J AU Li, XF Bond, PL Van Nostrand, JD Zhou, JZ Huang, LB AF Li, Xiaofang Bond, Philip L. Van Nostrand, Joy D. Zhou, Jizhong Huang, Longbin TI From lithotroph- to organotroph-dominant: directional shift of microbial community in sulphidic tailings during phytostabilization SO SCIENTIFIC REPORTS LA English DT Article ID COMPLETE GENOME SEQUENCE; SOLUBLE ORGANIC-CARBON; PORPHYRY COPPER TAILINGS; RIBOSOMAL-RNA GENES; MINE TAILINGS; SP-NOV.; BACTERIAL COMMUNITY; PRIMARY SUCCESSION; OXIDATIVE STRESS; SOIL AB Engineering microbial diversity to enhance soil functions may improve the success of direct revegetation in sulphidic mine tailings. Therefore, it is essential to explore how remediation and initial plant establishment can alter microbial communities, and, which edaphic factors control these changes under field conditions. A long-term revegetation trial was established at a Pb-Zn-Cu tailings impoundment in northwest Queensland. The control and amended and/or revegetated treatments were sampled from the 3-year-old trial. In total, 24 samples were examined using pyrosequencing of 16S rRNA genes and various chemical properties. The results showed that the microbial diversity was positively controlled by soil soluble Si and negatively controlled by soluble S, total Fe and total As, implying that pyrite weathering posed a substantial stress on microbial development in the tailings. All treatments were dominated by typical extremophiles and lithotrophs, typically Truepera, Thiobacillus, Rubrobacter; significant increases in microbial diversity, biomass and frequency of organotrophic genera (typically Nocardioides and Altererythrobacter) were detected in the revegetated and amended treatment. We concluded that appropriate phytostabilization options have the potential to drive the microbial diversity and community structure in the tailings toward those of natural soils, however, inherent environmental stressors may limit such changes. C1 [Li, Xiaofang; Huang, Longbin] Univ Queensland, Sustainable Minerals Inst, Ctr Mined Land Rehabil, Brisbane, Qld 4072, Australia. [Bond, Philip L.] Univ Queensland, Adv Water Management Ctr, Brisbane, Qld 4072, Australia. [Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Huang, LB (reprint author), Univ Queensland, Sustainable Minerals Inst, Ctr Mined Land Rehabil, Brisbane, Qld 4072, Australia. EM l.huang@uq.edu.au RI Van Nostrand, Joy/F-1740-2016; OI Van Nostrand, Joy/0000-0001-9548-6450; Bond, Philip/0000-0002-9025-4797 FU UQ Postdoctoral Fund; Mount Isa Mines, Glencore Ltd FX We thank Dr Fiona May of the Australian Centre for Ecogenomics, The University of Queensland for her work on pyrosequencing of the samples and Mr Yang Lu of the Advanced Water Management Centre, The University of Queensland for his help in processing the data. This project is financially supported by UQ Postdoctoral Fund and Mount Isa Mines, Glencore Ltd (formerly Xstrata Copper Ltd.). NR 97 TC 1 Z9 1 U1 6 U2 30 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 13 PY 2015 VL 5 AR 12978 DI 10.1038/srep12978 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO8HU UT WOS:000359409300001 PM 26268667 ER PT J AU Mishra, V Koshelev, AE AF Mishra, Vivek Koshelev, Alexei E. TI Local spin-density-wave order inside vortex cores in multiband superconductors SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTOR; QUASI-PARTICLE STATES; ANTIFERROMAGNETIC ORDER; II SUPERCONDUCTORS; MAGNETIC-FIELD; VORTICES AB Coexistence of antiferromagnetic order with superconductivity in many families of newly discovered iron-based superconductors has renewed interest to this old problem. Due to competition between the two types of order, one can expect appearance of the antiferromagnetism inside the cores of the vortices generated by the external magnetic field. The structure of a vortex in type II superconductors holds significant importance from the theoretical and the application points of view. Here we consider the internal vortex structure in a two-band s(+/-) superconductor near a spin-density-wave instability. We treat the problem in a completely self-consistent manner within the quasiclassical Eilenberger formalism. We study the structure of the s(+/-) superconducting order and magnetic field-induced spin-density-wave order near an isolated vortex. We examine the effect of this spin-density-wave state inside the vortex cores on the local density of states. C1 [Mishra, Vivek; Koshelev, Alexei E.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Mishra, V (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RI Koshelev, Alexei/K-3971-2013 OI Koshelev, Alexei/0000-0002-1167-5906 FU Center for Emergent Superconductivity, an Energy Frontier Research Center - US DOE, Office of Science [DE-AC0298CH1088] FX This work was supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office of Science, under Award No. DE-AC0298CH1088. NR 54 TC 1 Z9 1 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 13 PY 2015 VL 92 IS 6 AR 064511 DI 10.1103/PhysRevB.92.064511 PG 9 WC Physics, Condensed Matter SC Physics GA CO8SE UT WOS:000359440400003 ER PT J AU Sherwin, BD Schmittfull, M AF Sherwin, Blake D. Schmittfull, Marcel TI Delensing the CMB with the cosmic infrared background SO PHYSICAL REVIEW D LA English DT Article ID POWER SPECTRUM; GRAVITY-WAVES; POLARIZATION; ANISOTROPY; GALAXIES; HERMES; MASS AB As confusion with lensing B modes begins to limit experiments that search for primordial B-mode polarization, robust methods for delensing the cosmic microwave background (CMB) polarization sky are becoming increasingly important. We investigate in detail the possibility of delensing the CMB with the cosmic infrared background (CIB), emission from dusty star-forming galaxies that is an excellent tracer of the CMB lensing signal, in order to improve constraints on the tensor-to-scalar ratio r. We find that the maps of the CIB, such as current Planck satellite maps at 545 GHz, can be used to remove more than half of the lensing B-mode power. Calculating optimal combinations of different large-scale-structure tracers for delensing, we find that coadding CIB data and external arcminute-resolution CMB lensing reconstruction can lead to significant additional improvements in delensing performance. We investigate whether measurement uncertainty in the CIB power spectra will degrade the delensing performance if no model of the CIB spectra is assumed, and instead the CIB power spectra are marginalized over, when constraining r. We find that such uncertainty does not significantly affect B-mode surveys smaller than a few thousand degrees. Even for larger surveys it causes only a moderate reduction in CIB delensing performance, especially if the surveys have high (arcminute) resolution, which allows self calibration of the delensing procedure. Though further work on the impact of foreground residuals is required, our overall conclusions for delensing with current CIB data are optimistic: this delensing method can tighten constraints on r by a factor up to approximate to 2.2, and by a factor up to approximate to 4 when combined with external lensing reconstruction for approximate to 3 mu K-arcmin noise, without requiring the modeling of CIB properties. CIB delensing is thus a promising method for the upcoming generation of CMB polarization surveys. C1 [Sherwin, Blake D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sherwin, Blake D.] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Sherwin, Blake D.; Schmittfull, Marcel] LBNL, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Sherwin, Blake D.; Schmittfull, Marcel] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Sherwin, BD (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sherwin@berkeley.edu FU Miller Institute for Basic Research in Science at the University of California, Berkeley FX We thank R. Keisler, U. Seljak, A. van Engelen, O. Dore, J. C. Hill, E. Linder, S. Ferraro, J. Errard and J. Dunkley for helpful discussions and/or feedback on the paper draft. We are particularly grateful to G. Lagache for making the CIB halo model from [46] available. B. D. S. was supported by a fellowship from the Miller Institute for Basic Research in Science at the University of California, Berkeley. B. D. S also acknowledges the hospitality of the Beecroft Institute of Particle Astrophysics and Cosmology at Oxford University, where part of this work was completed. NR 57 TC 10 Z9 10 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 13 PY 2015 VL 92 IS 4 AR 043005 DI 10.1103/PhysRevD.92.043005 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO8TG UT WOS:000359444000001 ER PT J AU Kang, HY Peng, CY Wang, HP Lin, WK Sun, IW Chang, SG AF Kang, H. Y. Peng, C. Y. Wang, H. Paul Lin, W. -K. Sun, I. -W. Chang, S. -G. TI Preparation of Ag nanospheres filled with Cu SO JOURNAL OF EXPERIMENTAL NANOSCIENCE LA English DT Article DE Cu; Ag; growth of nanoparticles; core-shell nanoparticles; SAXS ID CORE-SHELL NANOPARTICLES; SMALL-ANGLE SCATTERING; BIMETALLIC NANOPARTICLES; HYBRID NANOPARTICLES; FREE-ENERGY; COPPER; NANOSCALE AB Surface properties of Ag nanoparticles may not be perturbed when they are filled with the relatively cheap Cu. To better understand how Ag can be coated on Cu, growth of the Cu and Ag bimetal during the temperature-programmed carbonisation (TPC) of Ag+- and Cu2+-beta-cyclodextrin (CD) complexes having the Cu/Ag ratios of 0.5, 1 and 2 was studied by in situ synchrotron small angle X-ray scattering (SAXS) spectroscopy. The SAXS spectra provide the detailed structural changes corresponding to the growth of Ag and Cu nanoparticles as the Ag+- and Cu2+-CD complexes are carbonised at the temperature range of 363-513K. It seems that Cu having a relatively high surface free energy is enriched in the core of the cherry-like Cu@Ag bimetal nanoparticles. The Cu@Ag bimetals are encapsulated in the carbon-shell formed from carbon unconsumed in the oxidation of CD during TPC. A rapid growth of the bimetal nanoparticles occurs at 393-423K. As Ag+ and Cu2+ are reduced during the CD oxidation, the Ag nanospheres are filled with Cu, and eventually encapsulated in the carbon-shell. Note that the carbon-shell coated on Cu@Ag can be removed by steam reforming at 573K. C1 [Kang, H. Y.; Peng, C. Y.; Wang, H. Paul] Natl Cheng Kung Univ, Dept Environm Engn, Tainan 70101, Taiwan. [Lin, W. -K.] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan. [Sun, I. -W.] Natl Cheng Kung Univ, Dept Chem, Tainan 70101, Taiwan. [Chang, S. -G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Wang, HP (reprint author), Natl Cheng Kung Univ, Dept Environm Engn, Tainan 70101, Taiwan. EM wanghp@mail.ncku.edu.tw FU Taiwan Ministry of Science and Technology [NSC 100-2221-E-006-031-MY3]; Taiwan Bureau of Energy [NSC 102-2623-E-006-014-IT] FX We gratefully thank Dr. Yaw-Wen Yang and Dr. Jyh-Fu Lee at the NSRRC for the SAXS experiments and analysis. This work was supported by the Taiwan Ministry of Science and Technology [NSC 100-2221-E-006-031-MY3] and Taiwan Bureau of Energy [NSC 102-2623-E-006-014-IT]. NR 46 TC 3 Z9 3 U1 4 U2 61 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1745-8080 EI 1745-8099 J9 J EXP NANOSCI JI J. Exp. Nanosci. PD AUG 13 PY 2015 VL 10 IS 12 BP 937 EP 946 DI 10.1080/17458080.2014.938316 PG 10 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CI1TK UT WOS:000354527300004 ER PT J AU Anastasiou, C Duhr, C Dulat, F Furlan, E Herzog, F Mistlberger, B AF Anastasiou, Charalampos Duhr, Claude Dulat, Falko Furlan, Elisabetta Herzog, Franz Mistlberger, Bernhard TI Soft expansion of double-real-virtual corrections to Higgs production at (NLO)-L-3 SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE QCD Phenomenology; NLO Computations ID 3-LOOP SPLITTING FUNCTIONS; MELLIN-BARNES INTEGRALS; QCD BETA-FUNCTION; BOSON PRODUCTION; FEYNMAN-INTEGRALS; DIMENSIONAL REGULARIZATION; ANOMALOUS DIMENSIONS; ASYMPTOTIC-EXPANSION; PROTON COLLIDERS; HADRON COLLIDERS AB We present methods to compute higher orders in the threshold expansion for the one-loop production of a Higgs boson in association with two partons at hadron colliders. This process contributes to the (NLO)-L-3 Higgs production cross section beyond the soft-virtual approximation. We use reverse unitarity to expand the phase-space integrals in the small kinematic parameters and to reduce the coefficients of the expansion to a small set of master integrals. We describe two methods for the calculation of the master integrals. The first was introduced for the calculation of the soft triple-real radiation relevant to (NLO)-L-3 Higgs production. The second uses a particular factorization of the three body phase-space measure and the knowledge of the scaling properties of the integral itself. Our result is presented as a Laurent expansion in the dimensional regulator, although some of the master integrals are computed to all orders in this parameter. C1 [Anastasiou, Charalampos; Dulat, Falko; Mistlberger, Bernhard] ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. [Duhr, Claude] CERN, Div Theory, CH-1211 Geneva, Switzerland. [Duhr, Claude] Catholic Univ Louvain, Ctr Cosmol Particle Phys & Phenomenol CP3, B-1348 Louvain La Neuve, Belgium. [Furlan, Elisabetta] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Herzog, Franz] Nikhef, Theory Grp, NL-1098 XG Amsterdam, Netherlands. RP Anastasiou, C (reprint author), ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. EM babis@phys.ethz.ch; claude.duhr@cern.ch; falko.dulat@gmail.com; efurlan@fnal.gov; fherzog@nikhef.nl; bmistlbe@phys.ethz.ch FU Swiss National Science Foundation (SNF) [200021-143781, 200020-149517]; European Commission through the ERC [320651]; FP7 Marie Curie Initial Training Network "LHCPhenoNet" [PITN-GA-2010-264564]; U.S. Department of Energy [DE-AC02-07CH11359]; "Fonds National de la Recherche Scientifique" (FNRS), Belgium FX Some of the algebraic manipulations needed for this work were performed using FORM [61] and diagrams were generated using QGRAF [60]. This research was supported by the Swiss National Science Foundation (SNF) under contracts 200021-143781 and 200020-149517, the European Commission through the ERC grants "MathAm", "IterQCD", "HEPGAME" (320651) and the FP7 Marie Curie Initial Training Network "LHCPhenoNet" (PITN-GA-2010-264564), by the U.S. Department of Energy under contract no. DE-AC02-07CH11359 and the "Fonds National de la Recherche Scientifique" (FNRS), Belgium. NR 61 TC 5 Z9 5 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 12 PY 2015 IS 8 AR 051 DI 10.1007/JHEP08(2015)051 PG 32 WC Physics, Particles & Fields SC Physics GA CU4SB UT WOS:000363519200005 ER PT J AU Wang, CM Schreiber, DK Olszta, MJ Baer, DR Bruemmer, SM AF Wang, Chong-Min Schreiber, Daniel K. Olszta, Matthew J. Baer, Donald R. Bruemmer, Stephen M. TI Direct in Situ TEM Observation of Modification of Oxidation by the Injected Vacancies for Ni-4Al Alloy Using a Microfabricated Nanopost SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE in situ TEM; oxidation; Ni-Al alloy; vacancy injection; cavity formation ID TRANSMISSION ELECTRON-MICROSCOPY; ATOM-PROBE TOMOGRAPHY; NI NANOPARTICLES; HIGH-TEMPERATURE; KIRKENDALL; DIFFUSION; NICKEL; FILMS; IRON AB Vacancy injection and selective oxidation of one species in bimetallic alloy at high temperature is a well-known phenomenon. However, detailed understanding of the behavior of the injected vacancies and consequently their effect on oxidation remains elusive. The current research examines the oxidation of high-purity Ni doped with 4.1 at. % Al using in situ transmission electron microscopy (TEM). Experiments are performed on nanoposts fabricated from solution-annealed bulk material that are essentially single crystal samples. Initial oxidation is observed to occur by multisite oxide nucleation, formation of an oxide shell followed by cavity nucleation and growth at the metal/oxide interface. One of the most interesting in situ TEM observations is the formation of a cavity that leads to the faceting of the metal and subsequent oxidation occurring by an atomic ledge migration mechanism on the faceted metal surface. Further, it is directly observed that metal atoms diffuse through the oxide layer to combine with oxygen at the outer surface of the oxide. The present work indicates that injection of vacancies and formation of cavity will lead to a situation where the oxidation rate is essentially controlled by the low surface energy plane of the metal, rather than by the initial terminating plane at the metal surface exposed to the oxidizing environment. C1 [Wang, Chong-Min; Baer, Donald R.] Environm Mol Sci Lab, Richland, WA 99352 USA. [Schreiber, Daniel K.; Olszta, Matthew J.; Bruemmer, Stephen M.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Wang, CM (reprint author), Environm Mol Sci Lab, Richland, WA 99352 USA. EM Chongmin.wang@pnnl.gov FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences; DOE [DE-AC06-76RLO 1830] FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences. The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a DOE User Facility operated by Battelle for the DOE Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the DOE under Contract DE-AC06-76RLO 1830. NR 28 TC 3 Z9 3 U1 4 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 12 PY 2015 VL 7 IS 31 BP 17272 EP 17277 DI 10.1021/acsami.5b04341 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CP2BX UT WOS:000359683600045 PM 26186484 ER PT J AU Verdaguer-Casadevall, A Li, CW Johansson, TP Scott, SB McKeown, JT Kumar, M Stephens, IEL Kanan, MW Chorkendorff, I AF Verdaguer-Casadevall, Arnau Li, Christina W. Johansson, Tobias P. Scott, Soren B. McKeown, Joseph T. Kumar, Mukul Stephens, Ifan E. L. Kanan, Matthew W. Chorkendorff, Ib TI Probing the Active Surface Sites for CO Reduction on Oxide-Derived Copper Electrocatalysts SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TEMPERATURE-PROGRAMMED DESORPTION; OXYGEN ELECTROREDUCTION ACTIVITY; AU NANOPARTICLES; CARBON-MONOXIDE; ADSORPTION; ELECTRODES; CU(100); SIZE AB CO electroreduction activity on oxide-derived Cu (OD-Cu) was found to correlate with metastable surface features that bind CO strongly. OD-Cu electrodes prepared by H-2 reduction of Cu2O precursors reduce CO to acetate and ethanol with nearly 50% Faradaic efficiency at moderate overpotential. Temperature-programmed desorption of CO on OD-Cu revealed the presence of surface sites with strong CO binding that are distinct from the terraces and stepped sites found on polycrystalline Cu foil. After annealing at 350 degrees C, the surface-area corrected current density for CO reduction is 44-fold lower and the Faradaic efficiency is less than 5%. These changes are accompanied by a reduction in the proportion of strong CO binding sites. We propose that the active sites for CO reduction on OD-Cu surfaces are strong CO binding sites that are supported by grain boundaries. Uncovering these sites is a first step toward understanding the surface chemistry necessary for efficient CO electroreduction. C1 [Verdaguer-Casadevall, Arnau; Johansson, Tobias P.; Scott, Soren B.; Stephens, Ifan E. L.; Chorkendorff, Ib] Tech Univ Denmark DTU, Dept Phys, Ctr Individual Nanoparticle Funct, Lyngby, Denmark. [Li, Christina W.; Kanan, Matthew W.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [McKeown, Joseph T.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Kumar, Mukul] Lawrence Livermore Natl Lab, Mat Engn Div, Livermore, CA 94550 USA. RP Kanan, MW (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA. EM mkanan@stanford.edu; ibchork@fysik.dtu.dk RI Stephens, Ifan/B-7191-2013; Chorkendorff, Ib/C-7282-2008 OI Stephens, Ifan/0000-0003-2157-492X; Chorkendorff, Ib/0000-0003-2738-0325 FU Danish National Research Foundation [DNRF54]; Global Climate and Energy Project [106765]; U.S. Department of Energy [DE-ACS2-07NA27344]; Office of Basic Energy Sciences, Division of Materials Science and Engineering under FWP [SCW0939] FX The Danish National Research Foundation's Center for Individual Nanoparticle Functionality is supported by the Danish National Research Foundation (DNRF54). We thank the Global Climate and Energy Project (106765) and the AFOSR (FA9550-14-1-0132). C.W.L. gratefully acknowledges a Stanford Graduate Fellowship. Sample characterization was performed at the Stanford Nano Shared Facilities. Lawrence Livermore National Laboratory is under the auspices of the U.S. Department of Energy, Contract No. DE-ACS2-07NA27344. J.T.M. and M.K. were supported by the Office of Basic Energy Sciences, Division of Materials Science and Engineering under FWP #SCW0939. NR 27 TC 38 Z9 38 U1 31 U2 142 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 12 PY 2015 VL 137 IS 31 BP 9808 EP 9811 DI 10.1021/jacs.5b06227 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CP1CK UT WOS:000359613300013 PM 26196863 ER PT J AU Meihaus, KR Fieser, ME Corbey, JF Evans, WJ Long, JR AF Meihaus, Katie R. Fieser, Megan E. Corbey, Jordan F. Evans, William J. Long, Jeffrey R. TI Record High Single-Ion Magnetic Moments Through 4f(n)5d(1) Electron Configurations in the Divalent Lanthanide Complexes [(C5H4SiMe3)(3)Ln](-) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ORGANOMETALLIC COMPLEXES; F-ELEMENTS; MOLECULE MAGNETS; ANISOTROPY; NANOMAGNETS; EXCHANGE; BLOCKING; ADDUCT; WELL AB The recently reported series of divalent lanthanide complex salts, namely [K(2.2.2-cryptand)][Cp'(3)Ln] (Ln = Y, La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm; Cp' = C5H4SiMe3) and the analogous trivalent complexes, Cp'(3)Ln, have been characterized via dc and ac magnetic susceptibility measurements. The salts of the complexes [Cp'Dy-3](-) and [Cp'Ho-3](-) exhibit magnetic moments of 11.3 and 11.4 respectively, which are the highest moments reported to date for any monometallic molecular species. The magnetic moments measured at room temperature support the assignments of a 4f(n+1) configuration for Ln = Sm, Eu, Tm and a 4f(n)5d(1) configuration for Ln = Y, La, Gd, Tb, Dy, Ho, Er. In the cases of Ln = Ce, Pr, Nd, simple models do not accurately predict the experimental room temperature magnetic moments. Although an LS coupling scheme is a useful starting point, it is not sufficient to describe the complex magnetic behavior and electronic structure of these intriguing molecules. While no slow magnetic relaxation was observed for any member of the series under zero applied dc field, the large moments accessible with such mixed configurations present important case studies in the pursuit of magnetic materials with inherently larger magnetic moments. This is essential for the design of new bulk magnetic materials and for diminishing processes such as quantum tunneling of the magnetization in single-molecule magnets. C1 [Meihaus, Katie R.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fieser, Megan E.; Corbey, Jordan F.; Evans, William J.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Evans, WJ (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. EM wevans@uci.edu; jrlong@berkeley.edu FU NSF [CHE-1464841, CHE-1265396] FX We are grateful to Wayne W. Lukens for helpful discussions and to Matthew R. MacDonald for preliminary sample preparation. This research was supported by NSF Grants CHE-1464841 (J.R.L.) and CHE-1265396 (WJ.E.). NR 34 TC 15 Z9 15 U1 16 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 12 PY 2015 VL 137 IS 31 BP 9855 EP 9860 DI 10.1021/jacs.5b03710 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA CP1CK UT WOS:000359613300020 PM 26168303 ER PT J AU Winter, JM Cascio, D Dietrich, D Sato, M Watanabe, K Sawaya, MR Vederas, JC Tang, Y AF Winter, Jaclyn M. Cascio, Duilio Dietrich, David Sato, Michio Watanabe, Kenji Sawaya, Michael R. Vederas, John C. Tang, Yi TI Biochemical and Structural Basis for Controlling Chemical Modularity in Fungal Polyketide Biosynthesis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ACYL-CARRIER PROTEIN; COA-ACP TRANSACYLASE; ASPERGILLUS-NIDULANS; CRYSTAL-STRUCTURE; MALONYL-COA; IKARUGAMYCIN BIOSYNTHESIS; ACYLTRANSFERASE DOMAIN; ENZYMATIC-SYNTHESIS; GENE-CLUSTER; I-TASSER AB Modular collaboration between iterative fungal polyketide synthases (IPKSs) is an important mechanism for generating structural diversity of polyketide natural products. Inter-PKS communication and substrate channeling are controlled in large by the starter unit acyl carrier protein transacylase (SAT) domain found in the accepting IPKS module. Here, we reconstituted the modular biosynthesis of the benzaldehyde core of the chaetoviridin and chaetomugilin azaphilone natural products using the IPKSs CazF and CazM. Our studies revealed a critical role of CazM's SAT domain in selectively transferring a highly reduced triketide product from CazF. In contrast, a more oxidized triketide that is also produced by CazF and required in later stages of biosynthesis of the final product is not recognized by the SAT domain. The structural basis for the acyl unit selectivity was uncovered by the first X-ray structure of a fungal SAT domain, highlighted by a covalent hexanoyl thioester intermediate in the SAT active site. The crystal structure of SAT domain will enable protein engineering efforts aimed at mixing and matching different IPKS modules for the biosynthesis of new compounds. C1 [Winter, Jaclyn M.; Tang, Yi] Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA 90095 USA. [Tang, Yi] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Cascio, Duilio; Sawaya, Michael R.] Univ Calif Los Angeles, Inst Genom & Prote, Dept Energy DOE, Los Angeles, CA 90095 USA. [Dietrich, David; Vederas, John C.] Univ Alberta, Dept Chem, Edmonton, AB T6G 2G2, Canada. [Sato, Michio; Watanabe, Kenji] Univ Shizuoka, Dept Pharmaceut Sci, Shizuoka 4228526, Japan. RP Tang, Y (reprint author), Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA 90095 USA. EM yitang@ucla.edu RI Watanabe, Kenji/N-2012-2015; OI Winter, Jaclyn/0000-0001-6273-5377; Sawaya, Michael/0000-0003-0874-9043; Vederas, John/0000-0002-2996-0326 FU US NIH [1R01GM085128, 1DP1GM106413]; NSERC; JSPS [LS103]; DOE [DE-FC02-02ER63421, DE-AC02-06CH11357]; NIH [5P41RR015301-10, 8 P41 GM103403-10]; L'Oreal USA for Women in Science FX This work was supported by the US NIH (1R01GM085128 and 1DP1GM106413) to Y.T; NSERC to J.C.V.; and JSPS (No. LS103) to K.W. We thank Mike Collazo at the UCLA-DOE X-ray Crystallization and Crystallography Core Facilities, which are supported by DOE Grant DE-FC02-02ER63421, and M. Cappel, K. Rajashankar, N. Sukumar, J. Schuermann, I. Kourinov and F. Murphy at NECAT beamlines 24-ID at APS, which are supported by grants from the NIH (5P41RR015301-10 and 8 P41 GM103403-10). Use of the APS is supported by the DOE under Contract DE-AC02-06CH11357. J.M.W. thanks L'Oreal USA for Women in Science for a postdoctoral fellowship. NMR instrumentation was supported by the NSF Equipment Grant CHE-1048804. NR 55 TC 7 Z9 8 U1 14 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 12 PY 2015 VL 137 IS 31 BP 9885 EP 9893 DI 10.1021/jacs.5b04520 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CP1CK UT WOS:000359613300024 PM 26172141 ER PT J AU Wu, JK Fan, CC Xue, GB Ye, T Liu, S Lin, RQ Chen, HZ Xin, HLL Xiong, RG Li, HY AF Wu, Jiake Fan, Congcheng Xue, Guobiao Ye, Tao Liu, Shuang Lin, Ruoqian Chen, Hongzheng Xin, Huolin L. Xiong, Ren-Gen Li, Hanying TI Interfacing Solution-Grown C-60 and (3-Pyrrolinium)(CdCl3) Single Crystals for High-Mobility Transistor-Based Memory Devices SO ADVANCED MATERIALS LA English DT Article DE field-effect transistors; memory; organic electronics; single crystals; solution processing ID FIELD-EFFECT TRANSISTORS; AMBIPOLAR CHARGE-TRANSPORT; THIN-FILM TRANSISTORS; NONVOLATILE MEMORY; ORGANIC TRANSISTORS; GATE INSULATOR; ELECTRONICS; STORAGE; ARRAYS AB Aligned ferroelectric single crystals of (3-pyrrolinium)(CdCl3) can be prepared from solution on top of aligned semiconducting C-60 single crystals using an orthogonal solvent. Memory devices based on these ferroelectric/semiconductor bilayered heterojunctions exhibit much larger hysteresis compared with that of only C-60 single crystals. More importantly, the introduction of the ferroelectric layer induces the memory window without dramatically reducing the charge mobility. C1 [Wu, Jiake; Fan, Congcheng; Xue, Guobiao; Ye, Tao; Liu, Shuang; Chen, Hongzheng; Li, Hanying] Zhejiang Univ, Dept Polymer Sci & Engn, MOE Key Lab Macromol Synth & Functionalizat, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. [Lin, Ruoqian; Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Xiong, Ren-Gen] Southeast Univ, Ordered Matter Sci Res Ctr, Nanjing 211189, Jiangsu, Peoples R China. RP Xiong, RG (reprint author), Southeast Univ, Ordered Matter Sci Res Ctr, Nanjing 211189, Jiangsu, Peoples R China. EM xiongrg@seu.edu.cn; hanying_li@zju.edu.cn RI Xin, Huolin/E-2747-2010 OI Xin, Huolin/0000-0002-6521-868X FU 973 Program [2014CB643503]; National Natural Science Foundation of China [51461165301, 51222302, 51373150, 21290172]; Zhejiang Province Natural Science Foundation [LZ13E030002]; Fundamental Research Funds for the Central Universities; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX This work was supported by 973 Program (2014CB643503), National Natural Science Foundation of China (51461165301, 51222302, 51373150, and 21290172), Zhejiang Province Natural Science Foundation (LZ13E030002), and Fundamental Research Funds for the Central Universities. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 48 TC 8 Z9 8 U1 38 U2 164 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 12 PY 2015 VL 27 IS 30 BP 4476 EP 4480 DI 10.1002/adma.201501577 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7NV UT WOS:000359347300012 ER PT J AU Lu, X Utama, MIB Lin, JH Luo, X Zhao, YY Zhang, J Pantelides, ST Zhou, W Quek, SY Xiong, QH AF Lu, Xin Utama, M. Iqbal Bakti Lin, Junhao Luo, Xin Zhao, Yanyuan Zhang, Jun Pantelides, Sokrates T. Zhou, Wu Quek, Su Ying Xiong, Qihua TI Rapid and Nondestructive Identification of Polytypism and Stacking Sequences in Few-Layer Molybdenum Diselenide by Raman Spectroscopy SO ADVANCED MATERIALS LA English DT Article DE few layer MoSe2; interlayer shear mode; molybdenum diselenide; polytypism; stacking ID ELECTRONIC-STRUCTURE; VALLEY POLARIZATION; MONOLAYER MOS2; BILAYER MOS2; WSE2; TRANSISTORS; DISULFIDE; FILMS AB Various combinations of interlayer shear modes emerge in few-layer molybdenum diselenide grown by chemical vapor deposition depending on the stacking configuration of the sample. Raman measurements may also reveal polytypism and stacking faults, as supported by first principles calculations and high-resolution transmission electron microscopy. Thus, Raman spectroscopy is an important tool in probing stacking-dependent properties in few-layer 2D materials. C1 [Lu, Xin; Utama, M. Iqbal Bakti; Zhao, Yanyuan; Zhang, Jun; Xiong, Qihua] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. [Lin, Junhao; Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Lin, Junhao; Pantelides, Sokrates T.; Zhou, Wu] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Luo, Xin; Quek, Su Ying] Natl Univ Singapore, Dept Phys, Ctr Adv Mat 2D, Singapore 117546, Singapore. [Luo, Xin; Quek, Su Ying] Natl Univ Singapore, Graphene Res Ctr, Singapore 117546, Singapore. [Luo, Xin; Quek, Su Ying] Inst High Performance Comp, Singapore 138632, Singapore. [Xiong, Qihua] Nanyang Technol Univ, Sch Elect & Elect Engn, Nanoelect Ctr Excellence, NOVITAS, Singapore 639798, Singapore. RP Xiong, QH (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. EM qihua@ntu.edu.sg RI Zhou, Wu/D-8526-2011; Xiong, Qihua/A-4979-2011; Lin, Junhao/D-7980-2015; Zhang, Jun/K-7978-2012; Quek, Su Ying/I-2934-2014; OI Zhou, Wu/0000-0002-6803-1095; Xiong, Qihua/0000-0002-2555-4363; Lin, Junhao/0000-0002-2195-2823; Zhang, Jun/0000-0002-9831-6796; Utama, Iqbal/0000-0002-4454-8348 FU Singapore National Research Foundation [NRF-RF2009-06, NRF-NRFI2015-03]; Ministry of Education [MOE2012-T2-2-086, 2013-T1-002-232]; Singapore National Research Foundation (NRF) under NRF [NRF-NRFF2013-07]; National Research Foundation; Prime Minister Office, Singapore under Medium Sized Centre Programme; U.S. DOE [DE-FG02-09ER46554]; U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division; ORNL's Center for Nanophase Materials Sciences (CNMS), DOE Office of Science User Facility FX Q.X. gratefully thanks Singapore National Research Foundation via a Fellowship grant (NRF-RF2009-06) and an Investigatorship grant (NRF-NRFI2015-03), Ministry of Education via a tier2 grant (MOE2012-T2-2-086) and a tier1 grant (2013-T1-002-232). S.Y.Q. and X.L. gratefully acknowledge the Singapore National Research Foundation (NRF) for funding under the NRF Fellowship (NRF-NRFF2013-07), and the National Research Foundation, Prime Minister Office, Singapore, under its Medium Sized Centre Programme. The computations were performed on the cluster of NUS Graphene Research Centre. This research was supported in part by U.S. DOE grant DE-FG02-09ER46554 (J.L. and S.T.P.), by the U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division (W.Z.), and through a user project at ORNL's Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 29 TC 16 Z9 16 U1 15 U2 93 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 12 PY 2015 VL 27 IS 30 BP 4502 EP 4508 DI 10.1002/adma.201501086 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7NV UT WOS:000359347300016 ER PT J AU Jarvis, KG White, JR Grim, CJ Ewing, L Ottesen, AR Beaubrun, JJG Pettengill, JB Brown, E Hanes, DE AF Jarvis, Karen G. White, James R. Grim, Christopher J. Ewing, Laura Ottesen, Andrea R. Beaubrun, Junia Jean-Gilles Pettengill, James B. Brown, Eric Hanes, Darcy E. TI Cilantro microbiome before and after nonselective pre-enrichment for Salmonella using 16S rRNA and metagenomic sequencing SO BMC MICROBIOLOGY LA English DT Article ID BACTERIAL DIVERSITY; SOFT-ROT; ALIGNMENT; IDENTIFICATION; PHYLLOSPHERE; COMMUNITIES; CLOSTRIDIA; TAXONOMY; ENTERICA; ECOLOGY AB Background: Salmonella enterica is a common cause of foodborne gastroenteritis in the United States and is associated with outbreaks in fresh produce such as cilantro. Salmonella culture-based detection methods are complex and time consuming, and improvments to increase detection sensitivity will benefit consumers. In this study, we used 16S rRNA sequencing to determine the microbiome of cilantro. We also investigated changes to the microbial community prior to and after a 24-hour nonselective pre-enrichment culture step commonly used by laboratory analysts to resuscitate microorganisms in foods suspected of contamination with pathogens. Cilantro samples were processed for Salmonella detection according to the method in the United States Food and Drug Administration Bacteriological Analytical Manual. Genomic DNA was extracted from culture supernatants prior to and after a 24-hour nonselective pre-enrichment step and 454 pyrosequencing was performed on 16S rRNA amplicon libraries. A database of Enterobacteriaceae 16S rRNA sequences was created, and used to screen the libraries for Salmonella, as some samples were known to be culture positive. Additionally, culture positive cilantro samples were examined for the presence of Salmonella using shotgun metagenomics on the Illumina MiSeq. Results: Time zero uncultured samples had an abundance of Proteobacteria while the 24-hour enriched samples were composed mostly of Gram-positive Firmicutes. Shotgun metagenomic sequencing of Salmonella culture positive cilantro samples revealed variable degrees of Salmonella contamination among the sequenced samples. Conclusions: Our cilantro study demonstrates the use of high-throughput sequencing to reveal the microbiome of cilantro, and how the microbiome changes during the culture-based protocols employed by food safety laboratories to detect foodborne pathogens. Finding that culturing the cilantro shifts the microbiome to a predominance of Firmicutes suggests that changing our culture-based methods will improve detection sensitivity for foodborne enteric pathogens. C1 [Jarvis, Karen G.; Grim, Christopher J.; Ewing, Laura; Beaubrun, Junia Jean-Gilles; Hanes, Darcy E.] US FDA, Ctr Food Safety & Appl Nutr, OARSA, Laurel, MD 20708 USA. [White, James R.; Grim, Christopher J.] Oak Ridge Inst Sci & Technol, Oak Ridge, TN USA. [Ottesen, Andrea R.; Pettengill, James B.; Brown, Eric] US FDA, Ctr Food Safety & Appl Nutr, ORS, College Pk, MD USA. RP Jarvis, KG (reprint author), US FDA, Ctr Food Safety & Appl Nutr, OARSA, Laurel, MD 20708 USA. EM karen.jarvis@fda.hhs.gov FU Department of Energy FX C. J. Grim and J. R. White are Oak Ridge Institute for Science and Education fellows, and we thank the Department of Energy for their support. We also thank Charles Wang for his guidance and support with the 454 pyrosequencing. NR 42 TC 5 Z9 5 U1 4 U2 27 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2180 J9 BMC MICROBIOL JI BMC Microbiol. PD AUG 12 PY 2015 VL 15 AR 160 DI 10.1186/s12866-015-0497-2 PG 13 WC Microbiology SC Microbiology GA CO7NQ UT WOS:000359346600002 PM 26264042 ER PT J AU Doona, CJ Feeherry, FE Kustin, K Olinger, GG Setlow, P Malkin, AJ Leighton, T AF Doona, Christopher J. Feeherry, Florence E. Kustin, Kenneth Olinger, Gene G. Setlow, Peter Malkin, Alexander J. Leighton, Terrance TI Fighting Ebola with novel spore decontamination technologies for the military SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Ebola; decontamination technologies; spores; chrloine dioxide; military medicine ID BACILLUS-SUBTILIS SPORES; DRINKING-WATER TREATMENT; CHLORINE DIOXIDE GAS; BACTERIAL-SPORES; HIGH-PRESSURE; DIPICOLINIC ACID; CLOSTRIDIUM-PERFRINGENS; ENDOSPORE INACTIVATION; STRUCTURAL DYNAMICS; CORTEX HYDROLYSIS AB Recently, global public health organizations such as Doctors without Borders (MSF), the World Health Organization (WHO), Public Health Canada, National Institutes of Health (NIH), and the U.S. government developed and deployed Field Decontamination Kits (FDKs), a novel, lightweight, compact, reusable decontamination technology to sterilize Ebola-contaminated medical devices at remote clinical sites lacking infrastructure in crisis-stricken regions of West Africa (medical waste materials are placed in bags and burned). The basis for effectuating sterilization with FDKs is chlorine dioxide (CIO2) produced from a patented invention developed by researchers at the US Army Natick Soldier RD&E Center (NSRDEC) and commercialized as a dry mixed-chemical for bacterial spore decontamination. In fact, the NSRDEC research scientists developed an ensemble of ClO2 technologies designed for different applications in decontaminating fresh produce; food contact and handling surfaces; personal protective equipment; textiles used in clothing, uniforms, tents, and shelters; graywater recycling; airplanes; surgical instruments; and hard surfaces in latrines, laundries, and deployable medical facilities. These examples demonstrate the far-reaching impact, adaptability, and versatility of these innovative technologies. We present herein the unique attributes of NSRDEC's novel decontamination technologies and a Case Study of the development of FDKs that were deployed in West Africa by international public health organizations to sterilize Ebola-contaminated medical equipment. FDKs use bacterial spores as indicators of sterility. We review the properties and structures of spores and the mechanisms of bacterial spore inactivation by ClO2. We also review mechanisms of bacterial spore inactivation by novel, emerging, and established non-thermal technologies for food preservation, such as high pressure processing, irradiation, cold plasma, and chemical sanitizers, using an array of Bacillus subtilis mutants to probe mechanisms of spore germination and inactivation. We employ techniques of high-resolution atomic force microscopy and phase contrast microscopy to examine the effects of 'y-irradiation on bacterial spores of Bacillus anthracis, Bacillus thuringiensis, and Bacillus atrophaeus spp. and of ClO2 on B. subtilis spores, and present in detail assays using spore bio-indicators to ensure sterility when decontaminating with ClO2. C1 [Doona, Christopher J.; Feeherry, Florence E.] US Army Natick, Soldier RD&E Ctr, Warfighter Directorate, Natick, MA 01760 USA. [Kustin, Kenneth] Brandeis Univ, Dept Chem, Waltham, MA 02254 USA. [Olinger, Gene G.] NIAID, Integrated Res Facil, Div Clin Res, Ft Detrick, MD USA. [Setlow, Peter] Univ Connecticut, Ctr Hlth, Dept Mol Biol & Biophys, Farmington, CT USA. [Malkin, Alexander J.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, Livermore, CA USA. [Leighton, Terrance] Univ Calif San Francisco Benioff, Childrens Hosp, Oakland Res Inst, Oakland, CA USA. RP Doona, CJ (reprint author), US Army Natick, Soldier RD&E Ctr, Warfighter Directorate, Kansas St, Natick, MA 01760 USA. EM christopher.j.doona.civ@mail.mil FU Army Research Office; Defense Threat Reduction Agency; NIH; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Federal Bureau of Investigation; Lawrence Livermore National Laboratory through Laboratory Directed Research and Development [04-ERD-002]; Defense Advanced Research Projects Agency (DARPA) FX Work carried out in the Set low laboratory on spore resistance and killing has received generous support over many years from the Army Research Office, the Defense Threat Reduction Agency, and the NIH.; The AFM work in the Malkin laboratory was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and supported by a grant from the Federal Bureau of Investigation and by Lawrence Livermore National Laboratory through Laboratory Directed Research and Development Grant 04-ERD-002. The authors are grateful to Marco Plomp for his critical contributions in the AFM characterization and data analysis.; Work in the Leighton laboratory was funded by The Defense Advanced Research Projects Agency (DARPA). We acknowledge with pleasure and gratitude the contributions of Katie Wheeler and Gordon Eggum to the study of ClO2 bioindicators. NR 92 TC 1 Z9 1 U1 1 U2 22 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 12 PY 2015 VL 6 AR 663 DI 10.3389/fmicb.2015.00663 PG 25 WC Microbiology SC Microbiology GA CP3XF UT WOS:000359815400001 PM 26322021 ER PT J AU Davoudiasl, H Marciano, WJ AF Davoudiasl, Hooman Marciano, William J. TI Running of the U(1) coupling in the dark sector SO PHYSICAL REVIEW D LA English DT Article ID BETA-FUNCTION AB The "dark photon" gamma(d) of a gauged U(1)(d) can become practically invisible if it primarily decays into light states from a dark sector. We point out that, in such scenarios, the running of the U(1)(d) "fine structure constant" alpha(d), with momentum transfer q(2), can be significant and potentially measurable. The gamma(d) kinetic mixing parameter epsilon(2) is also expected to run with q(2), through its dependence on alpha(d). We show how the combined running of epsilon(2)alpha(d) may provide a probe of the spectrum of dark particles and, for alpha(d) greater than or similar to few x 0.1, substantially modify predictions for "beam dump" or other intense source experiments. These features are demonstrated in simple models that contain light dark matter and a scalar that breaks U(1)(d). We also discuss theoretic considerations, regarding the U(1)(d) model in the ultraviolet regime, that may suggest the infrared upper bound alpha(d) less than or similar to 0.1. C1 [Davoudiasl, Hooman; Marciano, William J.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hooman@bnl.gov; marciano@bnl.gov FU US Department of Energy [DE-SC0012704] FX Work supported by the US Department of Energy under Grant Contract No. DE-SC0012704. NR 29 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 12 PY 2015 VL 92 IS 3 AR 035008 DI 10.1103/PhysRevD.92.035008 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO8SV UT WOS:000359442400003 ER PT J AU Keys, AS Chandler, D Garrahan, JP AF Keys, Aaron S. Chandler, David Garrahan, Juan P. TI Using the s ensemble to probe glasses formed by cooling and aging SO PHYSICAL REVIEW E LA English DT Article ID CORRESPONDING STATES; SUPERCOOLED LIQUIDS; CRYSTAL-NUCLEATION; ISING-MODEL; FREE-ENERGY; SPACE-TIME; TRANSITION; DYNAMICS; HETEROGENEITIES; SYSTEMS AB From length scale distributions characterizing frozen amorphous domains, we relate the s ensemble method with standard cooling and aging protocols for forming glass. We show that in a class of models where space-time scaling is in harmony with that of experiment, the spatial distributions of excitations obtained with the s ensemble are identical to those obtained through cooling or aging, but the computational effort for applying the s ensemble is generally many orders of magnitude smaller than that of straightforward numerical simulation of cooling or aging. We find that in contrast to the equilibrium ergodic state, a nonequilibrium length scale characterizes the anticorrelation between excitations and encodes the preparation history of glass states. C1 [Keys, Aaron S.; Chandler, David] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Keys, Aaron S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Garrahan, Juan P.] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. RP Garrahan, JP (reprint author), Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. EM Juan.Garrahan@nottingham.ac.uk OI Garrahan, Juan/0000-0002-0185-3924 FU Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL; Laboratory Directed Research and Development Program at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Leverhulme Trust Grant [F/00114/BG]; NSF [CHE-1048789] FX We thank D. T. Limmer, R. L. Jack, P. Sollich, T. Speck, and Y. S. Elmatad for helpful discussions. Support was provided by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL, by the Laboratory Directed Research and Development Program at Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, and by Leverhulme Trust Grant No. F/00114/BG. NSF Award No. CHE-1048789 provided computational resources. NR 40 TC 3 Z9 3 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD AUG 12 PY 2015 VL 92 IS 2 AR 022304 DI 10.1103/PhysRevE.92.022304 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CO8TK UT WOS:000359444500002 PM 26382403 ER PT J AU Lazicki, A Rygg, JR Coppari, F Smith, R Fratanduono, D Kraus, RG Collins, GW Briggs, R Braun, DG Swift, DC Eggert, JH AF Lazicki, A. Rygg, J. R. Coppari, F. Smith, R. Fratanduono, D. Kraus, R. G. Collins, G. W. Briggs, R. Braun, D. G. Swift, D. C. Eggert, J. H. TI X-Ray Diffraction of Solid Tin to 1.2 TPa SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-PRESSURE; TRANSITION-METALS; BCC; HCP; CRYSTALS; SPECTRA; PHASE AB We report direct in situ measurements of the crystal structure of tin between 0.12 and 1.2 TPa, the highest stress at which a crystal structure has ever been observed. Using angle-dispersive powder x-ray diffraction, we find that dynamically compressed Sn transforms to the body-centered-cubic (bcc) structure previously identified by ambient-temperature quasistatic-compression studies and by zero-kelvin density-functional theory predictions between 0.06 and 0.16 TPa. However, we observe no evidence for the hexagonal close-packed (hcp) phase found by those studies to be stable above 0.16 TPa. Instead, our results are consistent with bcc up to 1.2 TPa. We conjecture that at high temperature bcc is stabilized relative to hcp due to differences in vibrational free energy. C1 [Lazicki, A.; Rygg, J. R.; Coppari, F.; Smith, R.; Fratanduono, D.; Kraus, R. G.; Collins, G. W.; Braun, D. G.; Swift, D. C.; Eggert, J. H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Briggs, R.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. RP Lazicki, A (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge helpful discussions with P.F. McMillan, D. Klug, Y. Yao, L. Burakovsky, A. Salamat, and C. Pickard, target fabrication by S. Uhlich, W. Unites, and T. Uphaus, and support at the Laboratory for Laser Energetics by C. Sorce, N. Whiting, and J. Tellinghuisen. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 34 TC 8 Z9 8 U1 9 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 12 PY 2015 VL 115 IS 7 AR 075502 DI 10.1103/PhysRevLett.115.075502 PG 5 WC Physics, Multidisciplinary SC Physics GA CO8QU UT WOS:000359436100002 PM 26317730 ER PT J AU Ledee, D Smith, L Bruce, M Kajimoto, M Isern, N Portman, MA Olson, AK AF Ledee, Dolena Smith, Lincoln Bruce, Margaret Kajimoto, Masaki Isern, Nancy Portman, Michael A. Olson, Aaron K. TI c-Myc Alters Substrate Utilization and O-GlcNAc Protein Posttranslational Modifications without Altering Cardiac Function during Early Aortic Constriction SO PLOS ONE LA English DT Article ID PRESSURE-OVERLOAD HYPERTROPHY; C-13 ISOTOPOMER ANALYSIS; CITRIC-ACID CYCLE; HEART-FAILURE; FAILING HEART; MYOCYTE HYPERTROPHY; N-ACETYLGLUCOSAMINE; GENE-EXPRESSION; METABOLISM; GROWTH AB Hypertrophic stimuli cause transcription of the proto-oncogene c-Myc (Myc). Prior work showed that myocardial knockout of c-Myc (Myc) attenuated hypertrophy and decreased expression of metabolic genes after aortic constriction. Accordingly, we assessed the interplay between Myc, substrate oxidation and cardiac function during early pressure overload hypertrophy. Mice with cardiac specific, inducible Myc knockout (MycKO-TAC) and non-transgenic littermates (Cont-TAC) were subjected to transverse aortic constriction (TAC; n = 7/group). Additional groups underwent sham surgery (Cont-Sham and MycKO-Sham, n = 5 per group). After two weeks, function was measured in isolated working hearts along with substrate fractional contributions to the citric acid cycle by using perfusate with C-13 labeled mixed fatty acids, lactate, ketone bodies and unlabeled glucose and insulin. Cardiac function was similar between groups after TAC although + dP/dT and -dP/dT trended towards improvement in MycKO-TAC versus Cont-TAC. In sham hearts, Myc knockout did not affect cardiac function or substrate preferences for the citric acid cycle. However, Myc knockout altered fractional contributions during TAC. The unlabeled fractional contribution increased in MycKO-TAC versus Cont-TAC, whereas ketone and free fatty acid fractional contributions decreased. Additionally, protein posttranslational modifications by O-GlcNAc were significantly greater in Cont-TAC versus both Cont-Sham and MycKO-TAC. In conclusion, Myc alters substrate preferences for the citric acid cycle during early pressure overload hypertrophy without negatively affecting cardiac function. Myc also affects protein posttranslational modifications by O-GlcNAc during hypertrophy, which may regulate Myc-induced metabolic changes. C1 [Ledee, Dolena; Bruce, Margaret; Kajimoto, Masaki; Portman, Michael A.; Olson, Aaron K.] Seattle Childrens Res Inst, Seattle, WA 98105 USA. [Smith, Lincoln] Univ Washington, Dept Pediat, Div Crit Care Med, Seattle, WA 98195 USA. [Isern, Nancy] Pacific NW Natl Lab, EMSL, Richland, WA 99352 USA. [Portman, Michael A.; Olson, Aaron K.] Univ Washington, Dept Pediat, Div Cardiol, Seattle, WA 98195 USA. RP Olson, AK (reprint author), Seattle Childrens Res Inst, Seattle, WA 98105 USA. EM Aaron.olson@seattlechildrens.org FU National Heart, Lung, and Blood Institute [K08-HL-092333] FX This work was supported by the National Heart, Lung, and Blood Institute, Grant K08-HL-092333 to A. K. Olson. NR 38 TC 2 Z9 2 U1 1 U2 5 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 12 PY 2015 VL 10 IS 8 AR e0135262 DI 10.1371/journal.pone.0135262 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO9JT UT WOS:000359492300088 PM 26266538 ER PT J AU Kutepov, AL AF Kutepov, A. L. TI Full self-consistency versus quasiparticle self-consistency in diagrammatic approaches: exactly solvable two-site Hubbard model SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE GW plus DMFT; Hubbard model; strongly correlated systems ID ELECTRON-GAS; GW AB Self-consistent solutions of Hedin's equations (HE) for the two-site Hubbard model (HM) have been studied. They have been found for three-point vertices of increasing complexity (Gamma = 1 (GW approximation), Gamma(1) from the first-order perturbation theory, and the exact vertex Gamma(E)). Comparison is made between the cases when an additional quasiparticle (QP) approximation for Green's functions is applied during the self-consistent iterative solving of HE and when QP approximation is not applied. The results obtained with the exact vertex are directly related to the present open question-which approximation is more advantageous for future implementations, GW + DMFT or QPGW + DMFT. It is shown that in a regime of strong correlations only the originally proposed GW + DMFT scheme is able to provide reliable results. Vertex corrections based on perturbation theory (PT) systematically improve the GW results when full self-consistency is applied. The application of QP self-consistency combined with PT vertex corrections shows similar problems to the case when the exact vertex is applied combined with QP sc. An analysis of Ward Identity violation is performed for all studied in this work's approximations and its relation to the general accuracy of the schemes used is provided. C1 US DOE, Ames Lab, Ames, IA 50011 USA. RP Kutepov, AL (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM kutepov@physics.rutgers.edu NR 31 TC 1 Z9 1 U1 4 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 12 PY 2015 VL 27 IS 31 AR 315603 DI 10.1088/0953-8984/27/31/315603 PG 13 WC Physics, Condensed Matter SC Physics GA CN7DZ UT WOS:000358595500010 PM 26199232 ER PT J AU Modin, A Suzuki, MT Vegelius, J Yun, Y Shuh, DK Werme, L Nordgren, J Oppeneer, PM Butorin, SM AF Modin, A. Suzuki, M-T Vegelius, J. Yun, Y. Shuh, D. K. Werme, L. Nordgren, J. Oppeneer, P. M. Butorin, S. M. TI 5 f-Shell correlation effects in dioxides of light actinides studied by O 1s x-ray absorption and emission spectroscopies and first-principles calculations SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE actinide dioxides; x-ray spectroscopy; DFT plus U ID DENSITY-FUNCTIONAL THEORY; ELECTRONIC-STRUCTURE; URANIUM-DIOXIDE; NUCLEAR-FUELS; PHOTOEMISSION SPECTRA; LDA+U METHOD; OXIDES; UO2; PERFORMANCE; RADIATION AB Soft x-ray emission and absorption spectroscopic data are reported for the O 1s region of a single crystal of UO2, a polycrystalline NpO2 sample, and a single crystal of PuO2. The experimental data are interpreted using first-principles correlated-electron calculations within the framework of the density functional theory with added Coulomb U interaction (DFT+U). A detailed analysis regarding the origin of different structures in the x-ray emission and x-ray absorption spectra is given and the effect of varying the intra-atomic Coulomb interaction-U for the 5f electrons is investigated. Our data indicate that O 1s x-ray absorption and emission spectroscopies can, in combination with DFT+U calculations, successfully be used to study 5f-shell Coulomb correlation effects in dioxides of light actinides. The values for the Coulomb U parameter in these dioxides are derived to be in the range of 4-5 eV. C1 [Modin, A.; Suzuki, M-T; Vegelius, J.; Yun, Y.; Werme, L.; Nordgren, J.; Oppeneer, P. M.; Butorin, S. M.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Suzuki, M-T] Japan Atom Energy Agcy, CCSE, Kashiwa, Chiba 2778587, Japan. [Yun, Y.] Paul Scherrer Inst, Lab Reactor Phys & Syst Behav, CH-5232 Villigen, Switzerland. [Shuh, D. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Modin, A (reprint author), Uppsala Univ, Dept Phys & Astron, POB 516, SE-75120 Uppsala, Sweden. EM sergei.butorin@physics.uu.se RI Suzuki, Michi-To/G-6298-2013 FU Vetenskapsradet (VR); Svensk Karnbranslehantering AB (SKB); U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX Financial support for this work was provided by Vetenskapsradet (VR) and by Svensk Karnbranslehantering AB (SKB). Computer time received through the Swedish National Infrastructure for Computing (SNIC) is acknowledged. The personnel at beamline 7.0.1 at the Advanced Light Source and beamline I511-3 at MAX-lab are greatly acknowledged for their assistance during the measurements. The work at the Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences and this research (DKS) was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program, both of the U.S. Department of Energy at Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. NR 63 TC 5 Z9 5 U1 9 U2 27 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 12 PY 2015 VL 27 IS 31 AR 315503 DI 10.1088/0953-8984/27/31/315503 PG 8 WC Physics, Condensed Matter SC Physics GA CN7DZ UT WOS:000358595500007 PM 26202182 ER PT J AU Lau, SCK Riedel, T Fiebig, A Han, J Huntemann, M Petersen, J Ivanova, NN Markowitz, V Woyke, T Goker, M Kyrpides, NC Klenk, HP Qian, PY AF Lau, Stanley C. K. Riedel, Thomas Fiebig, Anne Han, James Huntemann, Marcel Petersen, Joern Ivanova, Natalia N. Markowitz, Victor Woyke, Tanja Goeker, Markus Kyrpides, Nikos C. Klenk, Hans-Peter Qian, Pei-Yuan TI Genome sequence of the pink-pigmented marine bacterium Loktanella hongkongensis type strain (UST950701-009P(T)), a representative of the Roseobacter group SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Biofilms; Marine; Roseobacter group; Rhodobacteraceae; Alphaproteobacteria; Plasmids ID POLYCHAETE HYDROIDS-ELEGANS; SP-NOV.; LARVAL SETTLEMENT; EMENDED DESCRIPTION; GENUS LOKTANELLA; SEAWATER; ARCHAEA; SYSTEM; TOOL; CLASSIFICATION AB Loktanella hongkongensis UST950701-009P(T) is a Gram-negative, non-motile and rod-shaped bacterium isolated from a marine biofilm in the subtropical seawater of Hong Kong. When growing as a monospecies biofilm on polystyrene surfaces, this bacterium is able to induce larval settlement and metamorphosis of a ubiquitous polychaete tubeworm Hydroides elegans. The inductive cues are low-molecular weight compounds bound to the exopolymeric matrix of the bacterial cells. In the present study we describe the features of L. hongkongensis strain DSM 17492(T) together with its genome sequence and annotation and novel aspects of its phenotype. The 3,198,444 bp long genome sequence encodes 3104 protein-coding genes and 57 RNA genes. The two unambiguously identified extrachromosomal replicons contain replication modules of the RepB and the Rhodobacteraceae-specific DnaA-like type, respectively. C1 [Lau, Stanley C. K.; Qian, Pei-Yuan] Hong Kong Univ Sci & Technol, Div Life Sci, Hong Kong, Hong Kong, Peoples R China. [Riedel, Thomas; Petersen, Joern; Goeker, Markus; Klenk, Hans-Peter] Leibniz Inst DSMZ German Collect Microorganisms C, Braunschweig, Germany. [Fiebig, Anne] Helmholtz Ctr Infect Res, Braunschweig, Germany. [Han, James; Huntemann, Marcel; Ivanova, Natalia N.; Woyke, Tanja; Kyrpides, Nikos C.] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. RP Goker, M (reprint author), Leibniz Inst DSMZ German Collect Microorganisms C, Braunschweig, Germany. EM markus.goeker@dsmz.de RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU German Research Foundation (DFG) Transregio-Roseobacter [SFB 51]; U.S. Department of Energy FX The authors gratefully acknowledge the help of Iljana Schroder, DSMZ, for growing cells of DSM 17492T and of Evelyne Brambilla, DSMZ, for DNA extraction and quality control. The work was performed under the auspices of the German Research Foundation (DFG) Transregio-SFB 51 Roseobacter grant and as part of the KMG-2 project funded by the U.S. Department of Energy. NR 49 TC 0 Z9 0 U1 1 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 11 PY 2015 VL 10 AR 51 DI 10.1186/s40793-015-0050-9 PG 8 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NV UT WOS:000367991900001 PM 26380639 ER PT J AU Rontsch, R Schulze, M AF Roentsch, Raoul Schulze, Markus TI Probing top-Z dipole moments at the LHC and ILC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE QCD Phenomenology; NLO Computations ID E(+)E(-) ANNIHILATION; HADRON COLLIDERS; QCD CORRECTIONS; LEADING ORDER; ELECTROWEAK; PHYSICS AB We investigate the weak electric and magnetic dipole moments of top quarkZ boson interactions at the Large Hadron Collider (LHC) and the International Linear Collider (ILC). Their vanishingly small magnitude in the Standard Model makes these couplings ideal for probing New Physics interactions and for exploring the role of top quarks in electroweak symmetry breaking. In our analysis, we consider the production of two top quarks in association with a Z boson at the LHC, and top quark pairs mediated by neutral gauge bosons at the ILC. These processes yield direct sensitivity to top quark-Z boson interactions and complement indirect constraints from electroweak precision data. Our computation is accurate to next-to-leading order in QCD, we include the full decay chain of top quarks and the Z boson, and account for theoretical uncertainties in our constraints. We find that LHC experiments will soon be able to probe weak dipole moments for the first time. C1 [Roentsch, Raoul] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Schulze, Markus] CERN, TH Unit, PH Dept, CH-1211 Geneva 23, Switzerland. RP Rontsch, R (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM rontsch@fnal.gov; markus.schulze@cern.ch FU United States Department of Energy [De-AC02-07CH11359]; National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX R.R. is grateful to the CERN Theory Group for their hospitality and support during the preparation of this paper. We are thankful to Andrei Gritsan, Uli Haisch, Roman Poschl, and Francois Richard for helpful discussions. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. This research used resources of the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 56 TC 6 Z9 6 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 11 PY 2015 IS 8 AR 044 DI 10.1007/JHEP08(2015)044 PG 19 WC Physics, Particles & Fields SC Physics GA CU4RZ UT WOS:000363519000005 ER PT J AU Kole, C Muthamilarasan, M Henry, R Edwards, D Sharma, R Abberton, M Batley, J Bentley, A Blakeney, M Bryant, J Cai, HW Cakir, M Cseke, LJ Cockram, J de Oliveira, AC De Pace, C Dempewolf, H Ellison, S Gepts, P Greenland, A Hall, A Hori, K Hughes, S Humphreys, MW Iorizzo, M Ismail, AM Marshall, A Mayes, S Nguyen, HT Ogbonnaya, FC Ortiz, R Paterson, AH Simon, PW Tohme, J Tuberosa, R Valliyodan, B Varshney, RK Wullschleger, SD Yano, M Prasad, M AF Kole, Chittaranjan Muthamilarasan, Mehanathan Henry, Robert Edwards, David Sharma, Rishu Abberton, Michael Batley, Jacqueline Bentley, Alison Blakeney, Michael Bryant, John Cai, Hongwei Cakir, Mehmet Cseke, Leland J. Cockram, James de Oliveira, Antonio Costa De Pace, Ciro Dempewolf, Hannes Ellison, Shelby Gepts, Paul Greenland, Andy Hall, Anthony Hori, Kiyosumi Hughes, Stephen Humphreys, Mike W. Iorizzo, Massimo Ismail, Abdelbagi M. Marshall, Athole Mayes, Sean Nguyen, Henry T. Ogbonnaya, Francis C. Ortiz, Rodomiro Paterson, Andrew H. Simon, Philipp W. Tohme, Joe Tuberosa, Roberto Valliyodan, Babu Varshney, Rajeev K. Wullschleger, Stan D. Yano, Masahiro Prasad, Manoj TI Application of genomics-assisted breeding for generation of climate resilient crops: progress and prospects SO FRONTIERS IN PLANT SCIENCE LA English DT Review DE climate change; crop improvement; stress tolerance; breeding; genomics ID QUANTITATIVE TRAIT LOCI; RICE ORYZA-SATIVA; SETARIA-ITALICA (L.); SCALE GENOTYPING APPLICATIONS; ADVENTITIOUS ROOT-FORMATION; ABSCISIC-ACID ACCUMULATION; ARACHIS-HYPOGAEA L.; CRISPR-CAS SYSTEM; CAJANUS-CAJAN L.; DROUGHT-RESISTANCE AB Climate change affects agricultural productivity worldwide. Increased prices of food commodities are the initial indication of drastic edible yield loss, which is expected to increase further due to global warming. This situation has compelled plant scientists to develop climate change-resilient crops, which can withstand broad-spectrum stresses such as drought, heat, cold, salinity, flood, submergence and pests, thus helping to deliver increased productivity. Genomics appears to be a promising tool for deciphering the stress responsiveness of crop species with adaptation traits or in wild relatives toward identifying underlying genes, alleles or quantitative trait loci. Molecular breeding approaches have proven helpful in enhancing the stress adaptation of crop plants, and recent advances in high-throughput sequencing and phenotyping platforms have transformed molecular breeding to genomics-assisted breeding (GAB). In view of this, the present review elaborates the progress and prospects of GAB for improving climate change resilience in crops, which is likely to play an ever increasing role in the effort to ensure global food security. C1 [Kole, Chittaranjan] Bidhan Chandra Krishi Viswavidyalaya, Mohanpur, India. [Muthamilarasan, Mehanathan; Prasad, Manoj] Natl Inst Plant Genome Res, Dept Plant Mol Genet & Genom, New Delhi 110067, India. [Henry, Robert] Univ Queensland, Queensland Alliance Agr & Food Innovat, St Lucia, Qld, Australia. [Edwards, David] Univ Queensland, Sch Agr & Food Sci, Brisbane, Qld, Australia. [Sharma, Rishu] Bidhan Chandra Krishi Viswavidyalaya, Fac Agr, Dept Plant Pathol, Mohanpur, India. [Abberton, Michael] Int Inst Trop Agr, Genet Resources Ctr, Ibadan, Nigeria. [Batley, Jacqueline] Univ Queensland, Ctr Integrated Legume Res, Brisbane, Qld, Australia. [Bentley, Alison; Cockram, James; Greenland, Andy] Natl Inst Agr Bot, John Bingham Lab, Cambridge, England. [Blakeney, Michael] Univ Western Australia, Sch Law, Perth, WA 6009, Australia. [Bryant, John] Univ Exeter, Hatherly Labs, CLES, Exeter, Devon, England. [Cai, Hongwei] Japan Grassland Agr & Forage Seed Assoc, Forage Crop Res Inst, Nasushiobara, Japan. [Cai, Hongwei] China Agr Univ, Coll Agron & Biotechnol, Dept Plant Genet & Breeding, Beijing 100094, Peoples R China. [Cakir, Mehmet] Murdoch Univ, Sch Biol Sci & Biotechnol, Fac Sci & Engn, Murdoch, WA 6150, Australia. [Cseke, Leland J.] Univ Alabama, Dept Biol Sci, Huntsville, AL 35899 USA. [de Oliveira, Antonio Costa] Univ Fed Pelotas, Plant Genom & Breeding Ctr, Pelotas, Brazil. [De Pace, Ciro] Univ Tuscia, Dept Agr Forests Nat & Energy, Viterbo, Italy. [Dempewolf, Hannes] Global Crop Divers Trust, Bonn, Germany. [Ellison, Shelby; Iorizzo, Massimo] Univ Wisconsin, Dept Hort, Madison, WI 53706 USA. [Gepts, Paul] Univ Calif Davis, Dept Plant Sci, Sect Crop & Ecosyst Sci, Davis, CA 95616 USA. [Hall, Anthony] Univ Calif Riverside, Dept Bot & Plant Sci, Riverside, CA 92521 USA. [Hori, Kiyosumi] Natl Inst Agrobiol Sci, Agrogen Res Ctr, Tsukuba, Ibaraki, Japan. [Hughes, Stephen] Univ Exeter, Exeter, Devon, England. [Humphreys, Mike W.; Marshall, Athole] Aberystwyth Univ, Inst Biol Environm & Rural Sci, Aberystwyth, Ceredigion, Wales. [Ismail, Abdelbagi M.] Int Rice Res Inst, Manila 1099, Philippines. [Mayes, Sean] Crops Future, Biotechnol & Crop Genet, Semenyih, Malaysia. [Nguyen, Henry T.; Valliyodan, Babu] Univ Missouri, Natl Ctr Soybean Biotechnol, Columbia, MO USA. [Nguyen, Henry T.; Valliyodan, Babu] Univ Missouri, Div Plant Sci, Columbia, MO USA. [Ogbonnaya, Francis C.] Grains Res & Dev Corp, Kingston, ACT, Australia. [Ortiz, Rodomiro] Swedish Univ Agr Sci, Dept Plant Breeding, Sundvagen, Sweden. [Paterson, Andrew H.] Univ Georgia, Plant Genome Mapping Lab, Athens, GA 30602 USA. [Simon, Philipp W.] Univ Wisconsin, Dept Hort, USDA, ARS, Madison, WI 53706 USA. [Tohme, Joe] Ctr Int Agr Trop, Agrobiodivers & Biotechnol Project, Cali, Colombia. [Tuberosa, Roberto] Dept Agr Sci, Bologna, Italy. [Varshney, Rajeev K.] Int Crops Res Inst Semi Arid Trop, Ctr Excellence Genom, Patancheru 502324, Andhra Pradesh, India. [Wullschleger, Stan D.] Oak Ridge Natl Lab, Div Environm Sci, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Yano, Masahiro] Natl Agr & Food Res Org, Inst Crop Sci, Tsukuba, Ibaraki, Japan. RP Kole, C (reprint author), Bidhan Chandra Krishi Viswavidyalaya, Nadia 741252, W Bengal, India. EM ckole2012@gmail.com; manoj_prasad@nipgr.ac.in RI Varshney, Rajeev/C-5295-2014; Tuberosa, Roberto/A-2781-2016; Henry, Robert/B-5824-2008; Wullschleger, Stan/B-8297-2012; Oliveira, Antonio/F-7508-2012; Ogbonnaya, Francis/C-5237-2014; OI Varshney, Rajeev/0000-0002-4562-9131; Valliyodan, Babu/0000-0001-9457-9508; Tuberosa, Roberto/0000-0001-9143-9569; Henry, Robert/0000-0002-4060-0292; Wullschleger, Stan/0000-0002-9869-0446; Oliveira, Antonio/0000-0001-8835-8071; Ogbonnaya, Francis/0000-0002-8596-7362; Prasad, Manoj/0000-0003-0691-0163 FU Biotechnology and Biological Sciences Research Council [BB/E006868/1, BBS/E/G/00003002] NR 204 TC 5 Z9 5 U1 9 U2 102 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD AUG 11 PY 2015 VL 6 AR 563 DI 10.3389/fpls.2015.00563 PG 16 WC Plant Sciences SC Plant Sciences GA CP5HJ UT WOS:000359911600001 PM 26322050 ER PT J AU Lyu, YC Zhao, NJ Hu, EY Xiao, RJ Yu, XQ Gu, L Yang, XQ Li, H AF Lyu, Yingchun Zhao, Nijie Hu, Enyuan Xiao, Ruijuan Yu, Xiqian Gu, Lin Yang, Xiao-Qing Li, Hong TI Probing Reversible Multielectron Transfer and Structure Evolution of Li1.2Cr0.4Mn0.4O2 Cathode Material for Li-Ion Batteries in a Voltage Range of 1.0-4.8 V SO CHEMISTRY OF MATERIALS LA English DT Article ID X-RAY-ABSORPTION; RECHARGEABLE LITHIUM BATTERIES; LAYERED COMPOSITE CATHODE; NICKEL MANGANESE OXIDES; IN-SITU; HIGH-CAPACITY; LOCAL-STRUCTURE; ELECTROCHEMICAL-BEHAVIOR; ELECTRON-MICROSCOPY; ATOMIC-STRUCTURE AB Li1.2Cr0.4Mn0.4O2 (0.4LiCrO(2)center dot 0.4Li(2)MnO(3)) is an interesting intercalation-type cathode material with high theoretical capacity of 387 mAh g(-1) based on multiple-electron transfer of Cr3+/Cr6+. In this work, it has been demonstrated that the reversible Cr3+/Cr6+ redox reaction can only be realized in a wide voltage range between 1.0 and 4.8 V. This is mainly due to large polarization during the discharge. The reversible migration of the Cr ions between octahedral and tetrahedral sites leads to large extent of cation mixing between lithium and transition metal layers, which does not affect the lithium storage capacity and stabilize the structure. In addition, a distorted spinel phase (Li3M2O4) is identified in the deeply discharged sample (1.0 V, Li1.5Cr0.4Mn0.4O2) The above results can explain the high reversible capacity and high structural stability achieved on Li1.2Cr0.4Mn0.4O2. These new findings will provide further in depth understanding on multielectron transfer and local structure stabilization mechanisms in intercalation chemistry, which are essential for understanding and developing a high capacity intercalation-type cathode for next generation high energy density Li-ion batteries. C1 [Lyu, Yingchun; Zhao, Nijie; Xiao, Ruijuan; Gu, Lin; Li, Hong] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. [Zhao, Nijie; Gu, Lin] Collaborat Innovat Ctr Quantum Matter, Beijing 100190, Peoples R China. [Hu, Enyuan; Yu, Xiqian; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Yu, XQ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM xyu@bnl.gov; l.gu@iphy.ac.cn; hli@iphy.ac.cn RI Gu, Lin/D-9631-2011; Li, Hong/C-4643-2008; Hu, Enyuan/D-7492-2016; Yu, Xiqian/B-5574-2014; Lyu, Yingchun/F-9893-2015 OI Gu, Lin/0000-0002-7504-031X; Li, Hong/0000-0002-8659-086X; Hu, Enyuan/0000-0002-1881-4534; Yu, Xiqian/0000-0001-8513-518X; Lyu, Yingchun/0000-0003-3229-1175 FU National Science Foundation of China [51325206]; Chinese Academy of Sciences [XDA09010102]; National project 973 [2012CB932900]; U.S. Department of Energy, Office of Vehicle Technologies [DE-SC0012704] FX This work was supported by National Science Foundation of China (51325206), "Strategic Priority Research Program" of the Chinese Academy of Sciences, Grant No. XDA09010102 and National project 973 (2012CB932900). The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies under Contract Number DE-SC0012704. The authors acknowledge Dr. Steven N. Ehrlich at beamline X18A (NSLS, U.S.A.), Dr. Tianpin Wu at beamline 9BM-B(APS, U.S.A.), Dr. Sunksik Lee at beamline 12BM-B (APS, U.S.A.) and Dr. Jingyuan Ma at beamline BL14W1 (SSRF, China). NR 79 TC 11 Z9 12 U1 11 U2 75 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 11 PY 2015 VL 27 IS 15 BP 5238 EP 5252 DI 10.1021/acs.chemmater.5b01362 PG 15 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO9ME UT WOS:000359499100012 ER PT J AU Yan, PF Zheng, JM Lv, DP Wei, Y Zheng, JX Wang, ZG Kuppan, S Yu, JG Luo, LL Edwards, D Olszta, M Amine, K Liu, J Xiao, J Pan, F Chen, GY Zhang, JG Wang, CM AF Yan, Pengfei Zheng, Jianming Lv, Dongping Wei, Yi Zheng, Jiaxin Wang, Zhiguo Kuppan, Saravanan Yu, Jianguo Luo, Langli Edwards, Danny Olszta, Matthew Amine, Khalil Liu, Jun Xiao, Jie Pan, Feng Chen, Guoying Zhang, Ji-Guang Wang, Chong-Min TI Atomic-Resolution Visualization of Distinctive Chemical Mixing Behavior of Ni, Co, and Mn with Li in Layered Lithium Transition-Metal Oxide Cathode Materials SO CHEMISTRY OF MATERIALS LA English DT Article ID AUGMENTED-WAVE METHOD; ION BATTERIES; ELECTROCHEMICAL PROPERTIES; ELECTRODE MATERIALS; LOCAL-STRUCTURE; SOLID-SOLUTION; HIGH-CAPACITY; VOLTAGE FADE; RICH; PHASE AB Capacity and voltage fading of layered structured cathode based on lithium transition-metal oxide is closely related to the lattice position and migration behavior of the transition-metal ions. However, it is scarcely clear about the behavior of each of these transition-metal ions in this category of cathode material. We report direct atomic resolution visualization of interatomic layer mixing of transition metals (Ni, Co, Mn) and lithium ions in layered structured oxide cathodes for lithium-ion batteries. Using chemical imaging with an aberration-corrected scanning transmission electron microscope (STEM) and density function theory calculations, we discovered that, in the layered cathodes, Mn and Co tend to reside almost exclusively at the lattice site of transition-metal (TM) layer in the structure or little interlayer mixing with Li. In contrast, Ni shows a high degree of interlayer mixing with Li. The fraction of Ni ions resides in the Li layer followed by a near linear dependence on total Ni concentration before reaching saturation. The observed distinctively different behavior of Ni with respect to Co and Mn provides new insights on both capacity and voltage fade in this class of cathode materials based on lithium and TM oxides, therefore providing scientific basis for selective tailoring of oxide cathode materials for enhanced performance. C1 [Yan, Pengfei; Luo, Langli; Wang, Chong-Min] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Zheng, Jianming; Lv, Dongping; Edwards, Danny; Olszta, Matthew; Liu, Jun; Xiao, Jie; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Wei, Yi; Zheng, Jiaxin; Pan, Feng] Peking Univ, Shenzhen Grad Sch, Sch Adv Mat, Shenzhen 518055, Peoples R China. [Wang, Zhiguo] Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. [Kuppan, Saravanan; Chen, Guoying] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Yu, Jianguo] Idaho Natl Lab, Ctr Adv Modeling & Simulat, Idaho Falls, ID 83415 USA. [Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Zhang, JG (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99352 USA. EM jiguang.zhang@pnnl.gov; Chongmin.wang@pnnl.gov RI Yu, Jianguo/C-3424-2013; yan, pengfei/E-4784-2016; Wang, Zhiguo/B-7132-2009; Zheng, Jianming/F-2517-2014; Luo, Langli/B-5239-2013; OI Yu, Jianguo/0000-0001-5604-8132; yan, pengfei/0000-0001-6387-7502; Zheng, Jianming/0000-0002-4928-8194; kuppan, saravanan/0000-0003-4976-4514; Luo, Langli/0000-0002-6311-051X FU Office of Vehicle Technologies of the U.S. Department of Energy under the Batteries for Advanced Battery Materials Research (BMR) [DE-AC02-05CH11231, 6951379]; DOE's Office of Biological and Environmental Research; Department of Energy [DE-AC05-76RLO1830]; National Natural Science Foundation of China [11474047]; Guangdong Innovation Team Project [2013N080]; Shenzhen Science and Technology Research Grant [ZDSY20130331145131323, CXZZ20120829172325895] FX We appreciate the beneficial discussion of Dr. Ping Lu of Sandia National Laboratory and Dr. Anmin Nie from Michigan Technological University during the course of this work. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy, under contract no. DE-AC02-05CH11231 and subcontract no. 6951379 under the Batteries for Advanced Battery Materials Research (BMR). Part of the STEM-EDS mapping was supported by the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the Department of Energy under contract no. DE-AC05-76RLO1830. Z.W. was supported by the National Natural Science Foundation of China (11474047). Y.W., J.Z., and F.P. were financially supported by Guangdong Innovation Team Project (no. 2013N080) and Shenzhen Science and Technology Research Grant (nos. ZDSY20130331145131323 and CXZZ20120829172325895). NR 55 TC 18 Z9 18 U1 9 U2 94 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 11 PY 2015 VL 27 IS 15 BP 5393 EP 5401 DI 10.1021/acs.chemmater.5b02016 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO9ME UT WOS:000359499100029 ER PT J AU Unemoto, A Ikeshoji, T Yasaku, S Matsuo, M Stavila, V Udovic, TJ Orimo, S AF Unemoto, Atsushi Ikeshoji, Tamio Yasaku, Syun Matsuo, Motoaki Stavila, Vitalie Udovic, Terrence J. Orimo, Shin-ichi TI Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; LI-ION BATTERIES; HYDROGEN-STORAGE; INTERCALATION COMPOUNDS; SUPERIONIC CONDUCTOR; COMPLEX HYDRIDES; ENERGY-STORAGE; CONVERSION; DECOMPOSITION; BOROHYDRIDE AB In this study, we assembled a bulk-type all-solid-state battery comprised of a TiS2 positive electrode, LiBH4 electrolyte, and Li negative electrode. Our battery retained high capacity over 300 discharge charge cycles when operated at 393 K and 0.2 C. The second discharge capacity was as high as 205 mAh g(-1), corresponding to a TiS2 utilization ratio of 85%. The 300th discharge capacity remained as high as 180 mAh g(-1) with nearly 100% Coulombic efficiency from the second cycle. Negligible impact of the exposure of LiBH4 to atmospheric-pressure oxygen on battery cycle life was also confirmed. To investigate the origin of the cycle durability for this bulk-type all-solid-state TiS2/Li battery, electrochemical measurements, thermogravimetry coupled with gas composition analysis, powder X-ray diffraction measurements, and first-principles molecular dynamics simulations were carried out. Chemical and/or electrochemical oxidation of LiBH4 occurred at the TiS2 surface at the battery operating temperature of 393 K and/or during the initial charge. During this oxidation reaction of LiBH4 with hydrogen (H-2) release just beneath the TiS2 surface, a third phase, likely including Li2B12H12, precipitated at the interface between LiBH4 and TiS2. Li2B12H12 has a lithium ionic conductivity of log(sigma / S cm(-1)) = -4.4, charge transfer reactivity with Li electrodes, and superior oxidative stability to LiBH4, and thereby can act as a stable interface that enables numerous discharge-charge cycles. Our results strongly suggest that the creation of such a stable interfacial layer is due to the propensity of forming highly stable, hydrogen-deficient polyhydro-closo-polyborates such as Li2B12H12, which are thermodynamically available in the ternary Li-B-H system. C1 [Unemoto, Atsushi; Ikeshoji, Tamio; Orimo, Shin-ichi] Tohoku Univ, WPI Adv Inst Mat Res WPI AIMR, Aoba Ku, Sendai, Miyagi 9808577, Japan. [Ikeshoji, Tamio; Yasaku, Syun; Matsuo, Motoaki; Orimo, Shin-ichi] Tohoku Univ, Inst Mat Res, Aoba Ku, Sendai, Miyagi 9808577, Japan. [Stavila, Vitalie] Sandia Natl Labs, Energy Nanomat, Livermore, CA 94551 USA. [Udovic, Terrence J.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. RP Unemoto, A (reprint author), Tohoku Univ, WPI Adv Inst Mat Res WPI AIMR, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan. EM unemoto@imr.tohoku.ac.jp RI ORIMO, Shin-ichi/A-4971-2011; Unemoto, Atsushi/D-3051-2013 OI ORIMO, Shin-ichi/0000-0002-4216-0446; FU WPI-AIMR, Tohoku University; Integrated Materials Research Center for the Low-Carbon Society (LC-IMR), Tohoku University; JSPS KAKENHI [25220911]; Advanced Low Carbon Technology Research and Development Program (ALCA) from the Japan Science and Technology Agency; U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy [DE-EE0002978] FX The crystal structures in Figure 7 were drawn using the VESTA program.57 The authors would like to thank Mr. K. Sato, Ms. H. Ohmiya, and Ms. N. Warifune for technical assistances. Fruitful discussion with Mr. G. Nogami, Mr. M. Tazawa, and Dr. M. Taniguchi of Mitsubishi Gas Chemicals Co., Ltd., is also acknowledged. This work was partially supported by the Target Project 4 of WPI-AIMR, Tohoku University, the Integrated Materials Research Center for the Low-Carbon Society (LC-IMR), Tohoku University, JSPS KAKENHI Grant No. 25220911, the Advanced Low Carbon Technology Research and Development Program (ALCA) from the Japan Science and Technology Agency, and the U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy under Grant No. DE-EE0002978. The FPMD calculations have been performed under the interuniversity cooperative research program of the Center for Computational Materials Science, Institute for Materials Research, Tohoku University. The battery assembly in a dry room was carried out at NIMS Battery Research Platform, Tsukuba, Japan. NR 56 TC 15 Z9 15 U1 42 U2 207 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 11 PY 2015 VL 27 IS 15 BP 5407 EP 5416 DI 10.1021/acs.chemmater.5b02110 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO9ME UT WOS:000359499100031 ER PT J AU Li, H Malliakas, CD Han, F Chung, DY Kanatzidis, MG AF Li, Hao Malliakas, Christos D. Han, Fei Chung, Duck Young Kanatzidis, Mercouri G. TI TlNgInS(3): An Indirect-Band-Gap Semiconductor With X-ray Photoconductivity Response SO CHEMISTRY OF MATERIALS LA English DT Article ID TEMPERATURE RADIATION DETECTORS; GAMMA-RAY; CRYSTAL-STRUCTURE; DIMENSIONAL REDUCTION; SPECTROSCOPIC PERFORMANCE; SOLID-STATE; SE; TE; CHARGE; SN AB The quaternary compound TlHgInS3 crystallizes in a new structure type of space group, C2/c, with cell parameters a = 13.916(3) angstrom, b = 3.9132(8) angstrom, c = 21.403(4) angstrom, beta = 104.16(3)degrees, V = 1130.1(8) angstrom(3), and rho = 7.241 g/cm(3). The structure is a unique three-dimensional framework with parallel tunnels, which is formed by (1)(infinity)[InS33-] infinite chains bridged by linearly coordinated Hg2+ ions. TlHgInS3 is a semiconductor with a band gap of 1.74 eV and a resistivity of similar to 4.32 G Omega cm. TlHgInS3 single crystals exhibit photocurrent response when exposed to Ag X-rays. The mobility-lifetime product (mu tau) of the electrons and holes estimated from the photocurrent measurements are (mu tau)(e) approximate to 3.6 x 10(-4) cm(2)/V and (mu tau)(h) approximate to 2.0 x 10(-4) cm(2)/V. Electronic structure calculations at the density functional theory level indicate an indirect band gap and a relatively small effective mass for both electrons and holes. Based on the photoconductivity data, TlHgInS3 is a potential material for radiation detection applications. C1 [Li, Hao; Han, Fei; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013 OI Han, Fei/0000-0001-7782-2713 FU Office of Nonproliferation and Verification Research and Development under the National Nuclear Security Administration, U.S. Department of Energy [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work is supported by the Office of Nonproliferation and Verification Research and Development under the National Nuclear Security Administration, U.S. Department of Energy (under Contract No. DE-AC02-06CH11357). Use of the Center for Nanoscale Materials, including resources in the Electron Microscopy Center, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (under Contract No. DE-AC02-06CH11357). NR 80 TC 2 Z9 2 U1 3 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 11 PY 2015 VL 27 IS 15 BP 5417 EP 5424 DI 10.1021/acs.chemmater.5b02242 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO9ME UT WOS:000359499100032 ER PT J AU Le, TP Shang, ZR Wang, LZ Li, NW Kesava, SV O'Connor, JW Chang, Y Bae, C Zhu, CH Hexemer, A Gomez, EW Salleo, A Hickner, MA Gomez, ED AF Le, Thinh P. Shang, Zhengrong Wang, Lizhu Li, Nanwen Kesava, Sameer Vajjala O'Connor, Joseph W. Chang, Ying Bae, Chulsung Zhu, Chenhui Hexemer, Alexander Gomez, Esther W. Salleo, Alberto Hickner, Michael A. Gomez, Enrique D. TI Miscibility and Acid Strength Govern Contact Doping of Organic Photovoltaics with Strong Polyelectrolytes SO MACROMOLECULES LA English DT Article ID POLYMER SOLAR-CELLS; FIELD-EFFECT TRANSISTORS; LIGHT-EMITTING-DIODES; OPEN-CIRCUIT VOLTAGE; THIN-FILMS; PHOTOELECTRON-SPECTROSCOPY; DEVICE CHARACTERISTICS; CROSS-LINKING; WORK-FUNCTION; ELECTRON AB Interfacial barriers at electrode-semiconductor contacts can greatly limit charge collection efficiency and hamper device performance. Doping of the semiconductor near the interface can mitigate charge extraction or injection problems by allowing charge tunneling through barriers with reduced width. Here we demonstrate that polymer acids can act as p-type dopants near electrode interfaces for active layers containing poly(3-hexylthiophene-2,5-diyl) (P3HT). By varying the pendant acidic groups between aromatic sulfonic acid, trifluoromethane sulfonimide, and perfluorosulfonic acid, we find the effectiveness of doping the conjugated polymer at the interface depends on the strength of the pendant acid group with stronger acid moieties being capable of creating more carriers in the doped system. Deposition of acidic polymeric dopants at the anode allows high carrier densities, of order 10(20) cm(-3), to be obtained in polymer semiconductors near the electrode interface. The charge carrier density also depends on the miscibility between polymeric dopants and conjugated polymers. The overall doping efficacy near electrodes therefore depends on the interplay between the strength of pendant acid groups and miscibility between polymeric dopants and conjugated polymers. C1 [Le, Thinh P.; Kesava, Sameer Vajjala; O'Connor, Joseph W.; Gomez, Esther W.; Gomez, Enrique D.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Wang, Lizhu; Li, Nanwen; Hickner, Michael A.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Gomez, Enrique D.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Shang, Zhengrong; Salleo, Alberto] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Chang, Ying; Bae, Chulsung] Rensselaer Polytech Inst, Dept Chem & Chem Biol, Troy, NY 12180 USA. [Zhu, Chenhui; Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Gomez, ED (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM edg12@psu.edu FU NSF [CBET-1067470]; U.S. Department of Energy [DE-AC02-05CH11231] FX Funding support from NSF under Award CBET-1067470 is acknowledged. The Advanced Light Source is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Lawrence Berkeley National Laboratory and supported by the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 62 TC 4 Z9 4 U1 1 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 11 PY 2015 VL 48 IS 15 BP 5162 EP 5171 DI 10.1021/acs.macromol.5b00724 PG 10 WC Polymer Science SC Polymer Science GA CO9MO UT WOS:000359500100012 ER PT J AU Shi, WC Hamilton, AL Delaney, KT Fredrickson, GH Kramer, EJ Ntaras, C Avgeropoulos, A Lynd, NA Demassieux, Q Creton, C AF Shi, Weichao Hamilton, Andrew L. Delaney, Kris T. Fredrickson, Glenn H. Kramer, Edward J. Ntaras, Christos Avgeropoulos, Apostolos Lynd, Nathaniel A. Demassieux, Quentin Creton, Costantino TI Aperiodic "Bricks and Mortar" Mesophase: a New Equilibrium State of Soft Matter and Application as a Stiff Thermoplastic Elastomer SO MACROMOLECULES LA English DT Article ID ORDER-DISORDER TRANSITION; BLOCK-COPOLYMER ARCHITECTURES; GRAFTED POLYMER BRUSH; X-RAY-SCATTERING; DIBLOCK COPOLYMER; BICONTINUOUS MICROEMULSIONS; MICROPHASE SEPARATION; HOMOPOLYMER BLENDS; MOLECULAR-WEIGHT; PHASE-BEHAVIOR AB A new thermodynamically stable, aperiodic "bricks-and-mortar" (B&M) cellular mesophase structure is reported in PS1-b-(PI-b-PS2)(3) miktoarm copolymer and PS homopolymer blends [PSI, long polystyrene; PI, poly(isoprene); PS2, short polystyrene], where PS comprises discrete hard "bricks" and PI the continuous soft "mortar". The mesophase is unique in its extreme domain volume fractions, its lack of positional order, and quasi-long-range orientational order. On the basis of this unusual mesophase structure, a series of PS-based thermoplastic elastomers are realized, combining rigidity from an exceptionally high content of discrete glassy PS domains (up to 82 wt %) and high extensibility with recoverable elasticity from a low content of continuous rubbery PI (down to 18 wt %). The new elastomers show sharp yielding behavior while maintaining good elasticity at large strains. Tensile-SAXS experiments reveal that voiding plays an important role for the mechanical behavior and voids can open/dose reversibly with/without loading. Plastic deformation only results in a slight loss of recoverable elasticity. C1 [Shi, Weichao; Hamilton, Andrew L.; Delaney, Kris T.; Fredrickson, Glenn H.; Kramer, Edward J.] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [Fredrickson, Glenn H.; Kramer, Edward J.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Fredrickson, Glenn H.; Kramer, Edward J.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Ntaras, Christos; Avgeropoulos, Apostolos] Univ Ioannina, Dept Mat Sci & Engn, GR-45110 Ioannina, Greece. [Lynd, Nathaniel A.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. [Lynd, Nathaniel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Demassieux, Quentin; Creton, Costantino] ESPCI Paristech CNRS UPMC, Lab Soft Matter Sci & Engn, F-75005 Paris, France. RP Fredrickson, GH (reprint author), Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. EM ghf@mrl.ucsb.edu; aavger@cc.uoi.gr RI CRETON, COSTANTINO/B-4077-2008; Avgeropoulos, Apostolos/I-5772-2012; Delaney, Kris/D-4324-2011 OI CRETON, COSTANTINO/0000-0002-0177-9680; Delaney, Kris/0000-0003-0356-1391 FU Institute for Collaborative Biotechnologies from U.S. Army Research Office [W911NF-09-0001]; MRSEC Program of the NSF [DMR 1121053]; NSF; E.I. DuPont de Nemours Co.; Dow Chemical Company; Northwestern University; U.S. DOE [DE-AC02-06CH11357] FX This research was supported by the Institute for Collaborative Biotechnologies through Grant W911NF-09-0001 from the U.S. Army Research Office. The content of the information does not necessarily reflect the position or the policy of the Government, and no official endorsement should be inferred. Extensive use was made of the MRL Shared Experimental Facilities supported by the MRSEC Program of the NSF under Award No. DMR 1121053; a member of the NSF-funded Materials Research Facilities Network. This work was performed at the DuPont-Northwestern-Dow Collaborative Access Team (DND-CAT) located at Sector 5 of the Advanced Photon Source (APS). DND-CAT is supported by E.I. DuPont de Nemours & Co., The Dow Chemical Company and Northwestern University. Use of the APS, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 59 TC 7 Z9 8 U1 6 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 11 PY 2015 VL 48 IS 15 BP 5378 EP 5384 DI 10.1021/acs.macromol.5b01210 PG 7 WC Polymer Science SC Polymer Science GA CO9MO UT WOS:000359500100034 ER PT J AU Kamano, H Nakamura, SX Lee, TSH Sato, T AF Kamano, H. Nakamura, S. X. Lee, T-S. H. Sato, T. TI Dynamical coupled-channels model of K- p reactions. II. Extraction of Lambda* and Sigma* hyperon resonances SO PHYSICAL REVIEW C LA English DT Article ID CHIRAL DYNAMICS; SCATTERING; STATES; MASS AB Resonance parameters (pole masses and residues) associated with the excited states of hyperons, Lambda* and Sigma*, are extracted within a dynamical coupled-channels model developed recently by us [Phys. Rev. C 90, 065204 (2014)] through a comprehensive partial-wave analysis of the K- p --> (K) over bar N, pi Sigma, pi Lambda, eta Lambda, K Xi data up to invariant mass W = 2.1 GeV. We confirm the existence of resonances corresponding to most, if not all, of the four-star resonances rated by the Particle Data Group. We also find several new resonances, and in particular propose a possible existence of a new narrow J(P) = 3/2(+) Lambda resonance that couples strongly to the eta Lambda channel. The J(P) = 1/2(-) Lambda resonances located below the (K) over bar N threshold are also discussed. Comparing our extracted pole masses with the ones from a recent analysis by the Kent State University group, some significant differences in the extracted resonance parameters are found, suggesting the need of more extensive and accurate data of K- p reactions including polarization observables to eliminate such an analysis dependence of the resonance parameters. In addition, the determined large branching ratios of the decays of high-mass resonances to the pi Sigma* and (K) over bar *N channels also suggest the importance of the data of 2 --> 3 reactions such as K- p --> pi pi Lambda and K- p --> pi(K) over bar N. Experiments on measuring cross sections and polarization observables of these fundamental reactions are highly desirable at hadron beam facilities such as J-PARC for establishing the Lambda* and Sigma* spectrum. C1 [Kamano, H.] Osaka Univ, Res Ctr Nucl Phys, Ibaraki, Osaka 5670047, Japan. [Nakamura, S. X.; Sato, T.] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan. [Lee, T-S. H.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Kamano, H (reprint author), Osaka Univ, Res Ctr Nucl Phys, Ibaraki, Osaka 5670047, Japan. EM kamano@rcnp.osaka-u.ac.jp RI Nakamura, Satoshi/M-9097-2016 OI Nakamura, Satoshi/0000-0002-7542-8859 FU Japan Society for the Promotion of Science (JSPS) KAKENHI [25800149, 24540273, 25105010]; US Department of Energy, Office of Nuclear Physics Division [DE-AC02-06CH11357]; HPCI Strategic Program (Field 5 "The Origin of Matter and the Universe") of Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Japan Society for the Promotion of Science (JSPS) KAKENHI Grant No. 25800149 (H.K.) and No. 24540273 and No. 25105010 (T.S.), and by the US Department of Energy, Office of Nuclear Physics Division, under Contract No. DE-AC02-06CH11357. H.K. acknowledges the support of the HPCI Strategic Program (Field 5 "The Origin of Matter and the Universe") of Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231, and resources provided on Blues and/or Fusion, high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 34 TC 6 Z9 6 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 11 PY 2015 VL 92 IS 2 AR 025205 DI 10.1103/PhysRevC.92.025205 PG 16 WC Physics, Nuclear SC Physics GA CO7QL UT WOS:000359355800002 ER PT J AU Barth, I Dodin, IY Fisch, NJ AF Barth, I. Dodin, I. Y. Fisch, N. J. TI Ladder Climbing and Autoresonant Acceleration of Plasma Waves SO PHYSICAL REVIEW LETTERS LA English DT Article AB When the background density in a bounded plasma is modulated in time, discrete modes become coupled. Interestingly, for appropriately chosen modulations, the average plasmon energy might be made to grow in a ladderlike manner, achieving upconversion or downconversion of the plasmon energy. This reversible process is identified as a classical analog of the effect known as quantum ladder climbing, so that the efficiency and the rate of this process can be written immediately by analogy to a quantum particle in a box. In the limit of a densely spaced spectrum, ladder climbing transforms into continuous autoresonance; plasmons may then be manipulated by chirped background modulations much like electrons are autoresonantly manipulated by chirped fields. By formulating the wave dynamics within a universal Lagrangian framework, similar ladder climbing and autoresonance effects are predicted to be achievable with general linear waves in both plasma and other media. C1 [Barth, I.; Dodin, I. Y.; Fisch, N. J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Dodin, I. Y.; Fisch, N. J.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08540 USA. RP Barth, I (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. OI Barth, Ido/0000-0001-8198-896X FU NNSA [DE274-FG52-08NA28553]; DOE [DE-AC02-09CH11466]; DTRA [HDTRA1-11-1-0037] FX The work was supported by NNSA Grant No. DE274-FG52-08NA28553, DOE Contract No. DE-AC02-09CH11466, and DTRA Grant No. HDTRA1-11-1-0037. NR 41 TC 0 Z9 0 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 11 PY 2015 VL 115 IS 7 AR 075001 DI 10.1103/PhysRevLett.115.075001 PG 5 WC Physics, Multidisciplinary SC Physics GA CO7QY UT WOS:000359357100003 PM 26317725 ER PT J AU Moura, MCP Smith, SJ Belzer, DB AF Moura, Maria Cecilia P. Smith, Steven J. Belzer, David B. TI 120 Years of US Residential Housing Stock and Floor Space SO PLOS ONE LA English DT Article ID ENERGY-CONSUMPTION; BUILDING CHARACTERISTICS; SECTOR; HOUSEHOLD AB Residential buildings are a key driver of energy consumption and also impact transportation and land-use. Energy consumption in the residential sector accounts for one-fifth of total U.S. energy consumption and energy-related CO2 emissions, with floor space a major driver of building energy demands. In this work a consistent, vintage-disaggregated, annual long-term series of U.S. housing stock and residential floor space for 1891-2010 is presented. An attempt was made to minimize the effects of the incompleteness and inconsistencies present in the national housing survey data. Over the 1891-2010 period, floor space increased almost tenfold, from approximately 24,700 to 235,150 million square feet, corresponding to a doubling of floor space per capita from approximately 400 to 800 square feet. While population increased five times over the period, a 50% decrease in household size contributed towards a tenfold increase in the number of housing units and floor space, while average floor space per unit remains surprisingly constant, as a result of housing retirement dynamics. In the last 30 years, however, these trends appear to be changing, as household size shows signs of leveling off, or even increasing again, while average floor space per unit has been increasing. GDP and total floor space show a remarkably constant growth trend over the period and total residential sector primary energy consumption and floor space show a similar growth trend over the last 60 years, decoupling only within the last decade. C1 [Moura, Maria Cecilia P.; Smith, Steven J.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Smith, Steven J.] Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20742 USA. [Belzer, David B.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Moura, MCP (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM cecilia.moura@pnnl.gov FU Office of Science of the U.S. Department of Energy, Integrated Assessment Research Program; DOE [DE-AC05-76RL01830] FX This research was supported by the Office of Science of the U.S. Department of Energy as part of the Integrated Assessment Research Program http://science.energy.gov/. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 25 TC 2 Z9 2 U1 2 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 11 PY 2015 VL 10 IS 8 AR e0134135 DI 10.1371/journal.pone.0134135 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO7PP UT WOS:000359353300020 PM 26263391 ER PT J AU Chorin, AJ Lu, F AF Chorin, Alexandre J. Lu, Fei TI Discrete approach to stochastic parametrization and dimension reduction in nonlinear dynamics SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE discrete approximation; stochastic parametrization; dimension reduction; chaotic systems; NARMAX ID PARAMETER-ESTIMATION; MODELS; IDENTIFICATION; SYSTEMS; ARMAX; DIFFUSIONS AB Many physical systems are described by nonlinear differential equations that are too complicated to solve in full. A natural way to proceed is to divide the variables into those that are of direct interest and those that are not, formulate solvable approximate equations for the variables of greater interest, and use data and statistical methods to account for the impact of the other variables. In the present paper we consider time-dependent problems and introduce a fully discrete solution method, which simplifies both the analysis of the data and the numerical algorithms. The resulting time series are identified by a NARMAX (nonlinear auto-regression moving average with exogenous input) representation familiar from engineering practice. The connections with the Mori-Zwanzig formalism of statistical physics are discussed, as well as an application to the Lorenz 96 system. C1 [Chorin, Alexandre J.; Lu, Fei] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Chorin, Alexandre J.; Lu, Fei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Math Grp, Berkeley, CA 94720 USA. RP Chorin, AJ (reprint author), Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. EM chorin@math.berkeley.edu FU Office of Science, Computational and Technology Research, US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMS-1217065, DMS-1419044] FX The authors thank the referees, as well as Prof. Jonathan Goodman, for reading the manuscript carefully and for their helpful suggestions, and Dr. Matthias Morzfeld, Prof. Kevin Lin, Prof. Xuemin Tu, and Prof. Robert Miller for helpful comments and good advice. This work was supported in part by the Director, Office of Science, Computational and Technology Research, US Department of Energy, under Contract DE-AC02-05CH11231, and by the National Science Foundation under Grants DMS-1217065 and DMS-1419044. NR 38 TC 4 Z9 4 U1 2 U2 12 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 11 PY 2015 VL 112 IS 32 BP 9804 EP 9809 DI 10.1073/pnas.1512080112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO6RY UT WOS:000359285100033 PM 26216975 ER PT J AU Kennett, JP Kennett, DJ Culleton, BJ Tortosa, JEA Bischoff, JL Bunch, TE Daniel, IR Erlandson, JM Ferraro, D Firestone, RB Goodyear, AC Israde-Alcantara, I Johnson, JR Pardo, JFJ Kimbel, DR LeCompte, MA Lopinot, NH Mahaney, WC Moore, AMT Moore, CR Ray, JH Stafford, TW Tankersley, KB Wittke, JH Wolbach, WS West, A AF Kennett, James P. Kennett, Douglas J. Culleton, Brendan J. Aura Tortosa, J. Emili Bischoff, James L. Bunch, Ted E. Daniel, I. Randolph, Jr. Erlandson, Jon M. Ferraro, David Firestone, Richard B. Goodyear, Albert C. Israde-Alcantara, Isabel Johnson, John R. Jorda Pardo, Jesus F. Kimbel, David R. LeCompte, Malcolm A. Lopinot, Neal H. Mahaney, William C. Moore, Andrew M. T. Moore, Christopher R. Ray, Jack H. Stafford, Thomas W., Jr. Tankersley, Kenneth Barnett Wittke, James H. Wolbach, Wendy S. West, Allen TI Bayesian chronological analyses consistent with synchronous age of 12,835-12,735 Cal BP for Younger Dryas boundary on four continents SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE Younger Dryas; comet; Bayesian; radiocarbon; synchroneity ID IMPACT HYPOTHESIS; EXTRATERRESTRIAL IMPACT; COSMIC IMPACT; DEPTH MODELS; BLACK MAT; NANODIAMONDS; TERMINATION; CALIFORNIA; SPHERULES; WILDFIRE AB The Younger Dryas impact hypothesis posits that a cosmic impact across much of the Northern Hemisphere deposited the Younger Dryas boundary (YDB) layer, containing peak abundances in a variable assemblage of proxies, including magnetic and glassy impact-related spherules, high-temperature minerals and melt glass, nanodiamonds, carbon spherules, aciniform carbon, platinum, and osmium. Bayesian chronological modeling was applied to 354 dates from 23 stratigraphic sections in 12 countries on four continents to establish a modeled YDB age range for this event of 12,835-12,735 Cal B.P. at 95% probability. This range overlaps that of a peak in extraterrestrial platinum in the Greenland Ice Sheet and of the earliest age of the Younger Dryas climate episode in six proxy records, suggesting a causal connection between the YDB impact event and the Younger Dryas. Two statistical tests indicate that both modeled and unmodeled ages in the 30 records are consistent with synchronous deposition of the YDB layer within the limits of dating uncertainty (similar to 100 y). The widespread distribution of the YDB layer suggests that it may serve as a datum layer. C1 [Kennett, James P.] Univ Calif Santa Barbara, Dept Earth Sci, Santa Barbara, CA 93106 USA. [Kennett, James P.] Univ Calif Santa Barbara, Inst Marine Sci, Santa Barbara, CA 93106 USA. [Kennett, Douglas J.; Culleton, Brendan J.] Penn State Univ, Dept Anthropol, University Pk, PA 16802 USA. [Aura Tortosa, J. Emili] Univ Valencia, Dept Prehist & Arqueol, E-46010 Valencia, Spain. [Bischoff, James L.] Berkeley Geochronol Lab, Berkeley, CA 94709 USA. [Bunch, Ted E.; Wittke, James H.] No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Geol Program, Flagstaff, AZ 86011 USA. [Daniel, I. Randolph, Jr.] E Carolina Univ, Dept Anthropol, Greenville, NC 27858 USA. [Erlandson, Jon M.] Univ Oregon, Museum Nat & Cultural Hist, Eugene, OR 97403 USA. [Ferraro, David] Viejo Calif Associates, Joshua Tree, CA 92252 USA. [Firestone, Richard B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Goodyear, Albert C.; Moore, Christopher R.] Univ S Carolina, South Carolina Inst Archaeol & Anthropol, Columbia, SC 29208 USA. [Israde-Alcantara, Isabel] Univ Michoacana, Inst Invest Met, Dept Geol & Mineral, Morelia 58060, Michoacan, Mexico. [Johnson, John R.] Santa Barbara Museum Nat Hist, Santa Barbara, CA 93105 USA. [Jorda Pardo, Jesus F.] Univ Nacl Educ Distancia, Fac Geog & Hist, Dept Prehist & Arqueol, E-28040 Madrid, Spain. [Kimbel, David R.] Kimstar Res, Fayetteville, NC 28312 USA. [LeCompte, Malcolm A.] Elizabeth City State Univ, Ctr Excellence Remote Sensing Educ & Res, Elizabeth City, NC 27909 USA. [Lopinot, Neal H.; Ray, Jack H.] SW Missouri State Univ, Ctr Archaeol Res, Springfield, MO 65897 USA. [Mahaney, William C.] Quaternary Surveys, Thornhill, ON L4J 1J4, Canada. [Moore, Andrew M. T.] Rochester Inst Technol, Coll Liberal Arts, Rochester, NY 14623 USA. [Stafford, Thomas W., Jr.] Univ Aarhus, Dept Phys & Astron, AMS Dating Ctr 14C, DK-8000 Aarhus C, Denmark. [Stafford, Thomas W., Jr.] Geol Museum, Nat Hist Museum Denmark, Ctr GeoGenet, DK-1350 Copenhagen, Denmark. [Tankersley, Kenneth Barnett] Univ Cincinnati, Dept Anthropol, Cincinnati, OH 45221 USA. [Tankersley, Kenneth Barnett] Univ Cincinnati, Dept Geol, Cincinnati, OH 45221 USA. [Wolbach, Wendy S.] Depaul Univ, Dept Chem, Chicago, IL 60614 USA. [West, Allen] GeoSci Consulting, Dewey, AZ 86327 USA. RP Kennett, JP (reprint author), Univ Calif Santa Barbara, Dept Earth Sci, Santa Barbara, CA 93106 USA. EM kennett@geol.ucsb.edu RI Jorda, Jesus F./M-9193-2014; OI Jorda, Jesus F./0000-0002-3937-9199; Erlandson, Jon/0000-0002-4705-4319 NR 49 TC 14 Z9 14 U1 7 U2 24 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 11 PY 2015 VL 112 IS 32 BP E4344 EP E4353 DI 10.1073/pnas.1507146112 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO6RY UT WOS:000359285100005 PM 26216981 ER PT J AU Mandadapu, KK Nirody, JA Berry, RM Oster, G AF Mandadapu, Kranthi K. Nirody, Jasmine A. Berry, Richard M. Oster, George TI Mechanics of torque generation in the bacterial flagellar motor SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE bacterial flagellar motor; torque generation; mechanochemistry; molecular motors; steric forces ID ESCHERICHIA-COLI; CONFORMATIONAL-CHANGE; OPTICAL TWEEZERS; ROTARY MOTOR; DYNAMICS; STATOR; ROTATION; COMPLEX; ROTOR; ARRANGEMENT AB The bacterial flagellar motor (BFM) is responsible for driving bacterial locomotion and chemotaxis, fundamental processes in pathogenesis and biofilm formation. In the BFM, torque is generated at the interface between transmembrane proteins (stators) and a rotor. It is well established that the passage of ions down a transmembrane gradient through the stator complex provides the energy for torque generation. However, the physics involved in this energy conversion remain poorly understood. Here we propose a mechanically specific model for torque generation in the BFM. In particular, we identify roles for two fundamental forces involved in torque generation: electrostatic and steric. We propose that electrostatic forces serve to position the stator, whereas steric forces comprise the actual "power stroke." Specifically, we propose that ion-induced conformational changes about a proline "hinge" residue in a stator a-helix are directly responsible for generating the power stroke. Our model predictions fit well with recent experiments on a single-stator motor. The proposed model provides a mechanical explanation for several fundamental properties of the flagellar motor, including torque-speed and speed-ion motive force relationships, backstepping, variation in step sizes, and the effects of key mutations in the stator. C1 [Mandadapu, Kranthi K.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mandadapu, Kranthi K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Nirody, Jasmine A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Berry, Richard M.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Oster, George] Univ Calif Berkeley, Dept Mol & Cellular Biol, Berkeley, CA 94720 USA. RP Oster, G (reprint author), Univ Calif Berkeley, Dept Mol & Cellular Biol, Berkeley, CA 94720 USA. EM goster@berkeley.edu FU Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US Department of Energy; National Institutes of Health [R01-GM110066]; National Science Foundation; Biotechnology and Biological Sciences Research Council; Engineering and Physical Sciences Research Council FX This manuscript includes an author (K.K.M.) at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231 with the US Department of Energy. The authors acknowledge funding from National Institutes of Health Grant R01-GM110066 (to G.O. and J.A.N.) and a National Science Foundation Integrative Graduate Education and Research Traineeship administered by the Center for Integrative Biomechanics in Education and Research (to J.A.N.). R.M.B. was supported by the Biotechnology and Biological Sciences Research Council and the Engineering and Physical Sciences Research Council. NR 36 TC 5 Z9 5 U1 4 U2 28 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 11 PY 2015 VL 112 IS 32 BP E4381 EP E4389 DI 10.1073/pnas.1501734112 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO6RY UT WOS:000359285100009 PM 26216959 ER PT J AU Lan, T Li, CW Hellman, O Kim, DS Munoz, JA Smith, H Abernathy, DL Fultz, B AF Lan, Tian Li, C. W. Hellman, O. Kim, D. S. Munoz, J. A. Smith, H. Abernathy, D. L. Fultz, B. TI Phonon quarticity induced by changes in phonon-tracked hybridization during lattice expansion and its stabilization of rutile TiO2 SO PHYSICAL REVIEW B LA English DT Article ID TITANIUM-DIOXIDE; PHASE-STABILITY; PLANE-WAVE; AB-INITIO; SOLIDS; SCATTERING; PRESSURE; DYNAMICS; CRYSTAL; SPECTRA AB Although the rutile structure of TiO2 is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly predicting a structural collapse at temperatures well below 1000 K. Inelastic neutron scattering was used to measure the temperature dependence of the phonon density of states (DOS) of rutile TiO2 from 300 to 1373 K. Surprisingly, these anomalous acoustic phonons were found to increase in frequency with temperature. First-principles calculations showed that with lattice expansion, the potentials for the anomalous acoustic phonons transform from quadratic to quartic, stabilizing the rutile phase at high temperatures. In these modes, the vibrational displacements of adjacent Ti and O atoms cause variations in hybridization of 3d electrons of Ti and 2p electrons of O atoms. With thermal expansion, the energy variation in this "phonon-tracked hybridization" flattens the bottom of the interatomic potential well between Ti and O atoms, and induces a quarticity in the phonon potential. C1 [Lan, Tian; Hellman, O.; Kim, D. S.; Munoz, J. A.; Smith, H.; Fultz, B.] CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. [Li, C. W.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Lan, T (reprint author), CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. EM tianlan@caltech.edu RI Abernathy, Douglas/A-3038-2012; BL18, ARCS/A-3000-2012; OI Abernathy, Douglas/0000-0002-3533-003X; Hellman, Olle/0000-0002-3453-2975; Kim, Dennis S/0000-0002-5707-2609 FU DOE Office of Science, Basic Energy Sciences [DE-FG02-03ER46055]; Scientific User Facilities Division, BES, DOE FX Research at the SNS at the Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, BES, DOE. This work was supported by the DOE Office of Science, Basic Energy Sciences, under Contract No. DE-FG02-03ER46055. NR 44 TC 5 Z9 5 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 11 PY 2015 VL 92 IS 5 AR 054304 DI 10.1103/PhysRevB.92.054304 PG 7 WC Physics, Condensed Matter SC Physics GA CO7QA UT WOS:000359354600003 ER PT J AU Xu, B Mao, ZL Ji, XL Yao, MM Chen, MJ Zhang, XM Hang, B Liu, Y Tang, W Tang, QS Xia, YK AF Xu, Bo Mao, Zhilei Ji, Xiaoli Yao, Mengmeng Chen, Minjian Zhang, Xuemei Hang, Bo Liu, Yi Tang, Wei Tang, Qiusha Xia, Yankai TI miR-98 and its host gene Huwe1 target Caspase-3 in Silica nanoparticles-treated male germ cells SO SCIENTIFIC REPORTS LA English DT Article ID INDUCED CYTOTOXICITY; APOPTOTIC PATHWAY; OXIDATIVE STRESS; EPITHELIAL-CELLS; CANCER CELLS; MITOCHONDRIA; TOXICITY; ACTIVATION; INHIBITORS; EXPOSURE AB Silica nanoparticles (NP) is one of the most commonly used nanomaterials with potential health hazards. However, the effects of Silica NP on germ cells and the underlying mechanisms are still unclear. In this study, GC-2 and TM-4, which are two different types of male germ cells were exposed to Silica NP for 24h, and then general cytotoxicity and multi-parameter cytotoxicity were evaluated. Our results showed that Silica NP could induce apoptosis in GC-2 cells. Transmission electron microscopy (TEM) results showed that Silica NP was localized in the lysosomes of GC-2 cells. High content screening (HCS) showed that Silica NP exposure could increased cell permeabilization and decreased mitochondrial membrane potential in GC-2 cells. The mRNA and protein levels of apoptosis markers (Bax, Caspase-3, Caspase-9) in GC-2 cells were significantly increased, while Bcl-2 was decreased. Accordingly, the expression level of miR-98, which can regulate Caspase-3, was significantly decreased. Huwe1, the host gene of miR-98, was positively associated with miR-98 expression after Silica NP exposure. Dual luciferase reporter assay suggested that miR-98 directly targets Caspase-3. These results suggest that Silica NP induces apoptosis via loss of mitochondrial membrane potential and Caspase-3 activation, while miR-98 plays key role in modulating this effect. C1 [Xu, Bo; Mao, Zhilei; Ji, Xiaoli; Yao, Mengmeng; Chen, Minjian; Zhang, Xuemei; Xia, Yankai] Nanjing Med Univ, Inst Toxicol, State Key Lab Reprod Med, Nanjing 211166, Jiangsu, Peoples R China. [Xu, Bo; Mao, Zhilei; Ji, Xiaoli; Yao, Mengmeng; Chen, Minjian; Zhang, Xuemei; Xia, Yankai] Nanjing Med Univ, Sch Publ Hlth, Key Lab Modern Toxicol, Minist Educ, Nanjing 211166, Jiangsu, Peoples R China. [Xu, Bo; Tang, Wei] Nanjing Med Univ, Affiliated Jiangyin Hosp, Dept Endocrinol, Wuxi Clin Sch Med, Jiangyin 214400, Peoples R China. [Hang, Bo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Canc & DNA Damage Responses, Div Life Sci, Berkeley, CA 94720 USA. [Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Tang, Qiusha] Southeast Univ, Sch Med, Nanjing 210009, Jiangsu, Peoples R China. RP Xia, YK (reprint author), Nanjing Med Univ, Inst Toxicol, State Key Lab Reprod Med, Nanjing 211166, Jiangsu, Peoples R China. EM yankaixia@njmu.edu.cn RI Liu, yi/A-3384-2008; Foundry, Molecular/G-9968-2014 OI Liu, yi/0000-0002-3954-6102; FU National 973 Program [2012CBA01306]; National Science Fund for Outstanding Young Scholars [81322039]; National Natural Science Foundation [31371524]; Distinguished Young Scholars of Jiangsu Province [BK20130041]; Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD); New Century Excellent Talents in University [NCET-13-0870] FX This study was supported by National 973 Program (2012CBA01306); National Science Fund for Outstanding Young Scholars (81322039); National Natural Science Foundation (31371524); Distinguished Young Scholars of Jiangsu Province (BK20130041); Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD); New Century Excellent Talents in University (NCET-13-0870). NR 47 TC 1 Z9 1 U1 1 U2 7 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 11 PY 2015 VL 5 AR 12938 DI 10.1038/srep12938 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO6TZ UT WOS:000359290500001 PM 26263183 ER PT J AU Aguilar-Arevalo, AA Aoki, M Blecher, M vom Bruch, D Bryman, D Comfort, J Cuen-Rochin, S Doria, L Gumplinger, P Hussein, A Igarashi, Y Ito, N Ito, S Kettell, SH Kurchaninov, L Littenberg, L Malbrunot, C Mischke, RE Muroi, A Numao, T Sheffer, G Sher, A Sullivan, T Tauchi, K Vavilov, D Yamada, K Yoshida, M AF Aguilar-Arevalo, A. A. Aoki, M. Blecher, M. vom Bruch, D. Bryman, D. Comfort, J. Cuen-Rochin, S. Doria, L. Gumplinger, P. Hussein, A. Igarashi, Y. Ito, N. Ito, S. Kettell, S. H. Kurchaninov, L. Littenberg, L. Malbrunot, C. Mischke, R. E. Muroi, A. Numao, T. Sheffer, G. Sher, A. Sullivan, T. Tauchi, K. Vavilov, D. Yamada, K. Yoshida, M. TI Detector for measuring the pi(+) -> e(+)nu(e) branching fraction SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Nal(Tl); CsI; Scintillation detectors; Pion decay ID ENDCAP PHOTON DETECTOR; PION DECAY; RATIO; PERFORMANCE; CRYSTAL AB The PIENU experiment at TRIUMF is aimed at a measurement of the branching ratio R-e/u = Gamma((pi(+) -> e(+)nu(e)) + [pi(+) -> e(+)nu(e)gamma))Gamma((pi(+)->mu(+)nu(mu))+(pi(+)->mu(+)nu(mu)gamma) with precision <0.1%. Incident pions, delivered at the rate of 60 kHz with momentum 75 MeVic, were degraded and stopped in a plastic scintillator target. Pions and their decay product positrons were detected with plastic scintillators and tracked with multiwire proportional chambers and silicon strip detectors. The energies of the positrons were measured in a spectrometer consisting of a large NaI(Tl) crystal surrounded by an array of pure Cs! crystals. This paper provides a description of the PIENU experimental apparatus and its performance in pursuit of R-e/mu . (C) 2015 Elsevier B.V. All rights reserved, C1 [Aguilar-Arevalo, A. A.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Aoki, M.; Ito, N.; Ito, S.; Muroi, A.; Yamada, K.; Yoshida, M.] Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan. [Blecher, M.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Doria, L.; Gumplinger, P.; Kurchaninov, L.; Mischke, R. E.; Numao, T.; Sheffer, G.; Sher, A.; Vavilov, D.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [vom Bruch, D.; Bryman, D.; Cuen-Rochin, S.; Malbrunot, C.; Sullivan, T.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Hussein, A.] Univ No British Columbia, Prince George, BC V2N 4Z9, Canada. [Igarashi, Y.; Tauchi, K.] KEK, Tsukuba, Ibaraki, Japan. [Kettell, S. H.; Littenberg, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Comfort, J.] Arizona State Univ, Tempe, AZ 85287 USA. RP Doria, L (reprint author), TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. EM luca@triumf.ca; chloe.m@cern.cb; sher@triumf.ca OI Aguilar-Arevalo, Alexis A./0000-0001-9279-3375 FU Natural Science and Engineering Council (NSERC); National Research Council of Canada; JSPS KAKENHI [18540274, 21340059, 24224006] FX We wish to thank P. Amaudruz, R. Bula, S. Chan, M. Constable, C. Lim, N. Khan, R. Kokke, P. Lu, K. Olchanski, R. Openshaw, C. Pearson and R. Poutissou for their contributions to the engineering, installation and commissioning of the detector and DAQ-related work, We are also grateful to Brookhaven National Laboratory for providing the NaI(Tl) and CsI crystals. This work was supported by the Natural Science and Engineering Council (NSERC) and the National Research Council of Canada through its contribution to TRIUMF and supported by JSPS KAKENHI Grant numbers 18540274, 21340059, 24224006. NR 23 TC 1 Z9 1 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 11 PY 2015 VL 791 BP 38 EP 46 DI 10.1016/j.nima.2015.04.004 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI9ZB UT WOS:000355128900007 ER PT J AU Neudecker, D Talou, P Kawano, T Smith, DL Capote, R Rising, ME Kahler, AC AF Neudecker, D. Talou, P. Kawano, T. Smith, D. L. Capote, R. Rising, M. E. Kahler, A. C. TI Evaluation of the (PU)-P-239 prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Nuclear data evaluation; Pu-239 prompt fission neutron spectrum; Uncertainty quantification ID UNCERTAINTY QUANTIFICATION; NUCLEAR-DATA; PLUTONIUM ISOTOPES; CROSS-SECTIONS; PU-239; MODEL; U-235; PARAMETERS; URANIUM AB We present evaluations of the prompt fission neutron spectrum (PFNS) of (PU)-P-239 induced by 500 keV neutrons, and associated covariances. In a previous evaluation by Talon et al. (2010), surprisingly low evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough uncertainty quantification of experimental data and of the Los Alamos model predicted values entering the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was employed that takes into account the qualitative differences between normalized model predicted values and experimental shape data These improvements lead to changes in the evaluated PENS and overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties are still smaller than those obtained in a statistical analysis using experimental information only, due to strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented. which lead to more reasonable evaluated uncertainties. The calculated k(eff) of selected criticality benchmarks obtained with these new evaluations agree with each other within their uncertainties despite the different approaches to estimate model defect uncertainties. The k(eff) one standard deviations overlap with some of those obtained using ENDF/B-VILl, albeit their mean values are further away from unity. Spectral indexes for the Jezebel critical assembly calculated with the newly evaluated PFNS agree with the experimental data for selected (n,) and (n,f) reactions, and show improvements for highenergy threshold (n,2n) reactions compared to ENDF/B-VII.l. (C) 2015 Elsevier B.V. All rights reserved. C1 [Neudecker, D.; Talou, P.; Kawano, T.; Kahler, A. C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Smith, D. L.] Argonne Natl Lab, Nucl Engn Div, Coronado, CA 92118 USA. [Capote, R.] Vienna Int Ctr, Nucl Data Sect, Int Atom Energy Agcy Vienna, A-1400 Vienna, Austria. [Rising, M. E.] Los Alamos Natl Lab, X Div, Los Alamos, NM 87545 USA. RP Neudecker, D (reprint author), Los Alamos Natl Lab, Div Theoret, POB 1663 MS-B283, Los Alamos, NM 87545 USA. EM dneudecker@lan1.gov; talou@lan1.gov; kawano@lan1.gov; donaldlarnedsmith@lan1.gov; r.capotenoy@iaea.org; mrising@lan1.gov; akahler@lan1.gov RI Capote Noy, Roberto/M-1245-2014 OI Capote Noy, Roberto/0000-0002-1799-3438 FU NNSA of the U.S. Department of Energy at LANL [DE-AC52-06NA25396] FX One of the authors (D.N.) wants to thank W. Mannhart, V. Pronyaev, J. Lestone, N. Kornilov, N. Otsuka, P. Schillebeeckx, J.J. Egan and P. Staples for helpful and insightful discussions as well as providing information needed to estimate experimental uncertainties. Special thanks also go to R.C. Haight, T.N. Taddeucci, M.C. White and H.Y. Lee for providing important insight into the experimental data. Three authors (D.N., R.C., D.L.S.) also want to thank A. Trkov for extensive discussion on the evaluation methodology as part of a closely related evaluation. We also thank M.B. Chadwick for stimulating discussions as well as his continuing and inquisitive interest in this subject. This work was partly carried out under the auspices of the NNSA of the U.S. Department of Energy at LANL under Contract No, DE-AC52-06NA25396. NR 56 TC 3 Z9 3 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 11 PY 2015 VL 791 BP 80 EP 92 DI 10.1016/j.nima.2015.04.044 PG 13 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI9ZB UT WOS:000355128900013 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Brown, AM Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Christy, B Clark, K Classen, L Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC Dumm, JP Dunkman, M Eagan, R Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fadiran, O Fahey, S Fazely, AR Fedynitch, A Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Glagla, M Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grant, D Gretskov, P Groh, JC Gross, A Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansmann, B Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jero, K Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohnen, G Kolanoski, H Konietz, R Koob, A Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lesiak-Bzdak, M Leuermann, M Leuner, J Lunemann, J Madsen, J Maggi, G Mahn, KBM Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Middlemas, E Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Olivas, A Omairat, A O'Murchadha, A Palczewski, T Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Scheriau, F Schimp, M Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Seckel, D Seunarine, S Shanidze, R Smith, MWE Soldin, D Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S Vandenbroucke, J van Eijndhoven, N Vanheule, S van Santen, J Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallace, A Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Wille, L Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Brown, A. M. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. Dumm, J. P. Dunkman, M. Eagan, R. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fadiran, O. Fahey, S. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Glagla, M. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansmann, B. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jero, K. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Kohnen, G. Kolanoski, H. Konietz, R. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Middlemas, E. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Scheriau, F. Schimp, M. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Seckel, D. Seunarine, S. Shanidze, R. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. Vandenbroucke, J. van Eijndhoven, N. Vanheule, S. van Santen, J. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallace, A. Wallraff, M. Wandkowsky, N. Weaver, Ch Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Zoll, M. CA IceCube Collaboration TI A COMBINED MAXIMUM-LIKELIHOOD ANALYSIS OF THE HIGH-ENERGY ASTROPHYSICAL NEUTRINO FLUX MEASURED WITH ICECUBE SO ASTROPHYSICAL JOURNAL LA English DT Article DE astroparticle physics; methods: data analysis; neutrinos ID GAMMA-RAY SOURCES; COSMIC-RAYS; POINT-LIKE; PERFORMANCE; TELESCOPE; EMISSION; GALAXIES; SPECTRUM; SEARCHES; SIGNALS AB Evidence for an extraterrestrial flux of high-energy neutrinos has now been found in multiple searches with the IceCube detector. The first solid evidence was provided by a search for neutrino events with deposited energies greater than or similar to 30 TeV and interaction vertices inside the instrumented volume. Recent analyses suggest that the extraterrestrial flux extends to lower energies and is also visible with throughgoing, nu(mu)-induced tracks from the Northern Hemisphere. Here, we combine the results from six different IceCube searches for astrophysical neutrinos in a maximum-likelihood analysis. The combined event sample features high-statistics samples of shower-like and track-like events. The data are fit in up to three observables: energy, zenith angle, and event topology. Assuming the astrophysical neutrino flux to be isotropic and to consist of equal flavors at Earth, the all-flavor spectrum with neutrino energies between 25 TeV and 2.8 PeV is well described by an unbroken power law with best-fit spectral index -2.50 +/- 0.09 and a flux at 100 TeV of (6.7(-1.2)(+1.1)) x 10(-18) GeV-1 s(-1) sr(-1) cm(-2). Under the same assumptions, an unbroken power law with index -2 is disfavored with a significance of 3.8 sigma (p = 0.0066%) with respect to the best fit. This significance is reduced to 2.1 sigma (p = 1.7%) if instead we compare the best fit to a spectrum with index -2 that has an exponential cut-off at high energies. Allowing the electron-neutrino flux to deviate from the other two flavors, we find a nu(e) fraction of 0.18 +/- 0.11 at Earth. 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G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Koskinen, D. J.; Larson, M. J.; Medici, M.; Sandroos, J.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Kurahashi, N.; Richman, M.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Mohrmann, L (reprint author), DESY, D-15735 Zeuthen, Germany. EM lars.mohrmann@desy.de RI Tjus, Julia/G-8145-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Maruyama, Reina/A-1064-2013; Wiebusch, Christopher/G-6490-2012; Koskinen, David/G-3236-2014; OI Strotjohann, Nora Linn/0000-0002-4667-6730; Arguelles Delgado, Carlos/0000-0003-4186-4182; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Maruyama, Reina/0000-0003-2794-512X; Wiebusch, Christopher/0000-0002-6418-3008; Koskinen, David/0000-0002-0514-5917; Maunu, Ryan/0000-0002-5755-3437; Perez de los Heros, Carlos/0000-0002-2084-5866 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) at the University of Wisconsin-Madison; Open Science Grid (OSG); U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI); Natural Sciences and Engineering Research Council of Canada; WestGrid; Compute/Calcul Canada; Swedish Research Council, Sweden; Swedish Polar Research Secretariat, Sweden; Swedish National Infrastructure for Computing (SNIC), Sweden; Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Germany; Deutsche Forschungsgemeinschaft (DFG), Germany; Helmholtz Alliance for Astroparticle Physics (HAP), Germany; Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 68 TC 78 Z9 78 U1 1 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 98 DI 10.1088/0004-637X/809/1/98 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500098 ER PT J AU Arnett, WD Meakin, C Viallet, M Campbell, SW Lattanzio, JC Mocak, M AF Arnett, W. David Meakin, Casey Viallet, Maxime Campbell, Simon W. Lattanzio, John C. Mocak, Miroslav TI BEYOND MIXING-LENGTH THEORY: A STEP TOWARD 321D SO ASTROPHYSICAL JOURNAL LA English DT Article DE convection; stars: evolution; stars: oscillations; supernovae: general; turbulence ID SUBDWARF B STARS; TURBULENT COMPRESSIBLE CONVECTION; HORIZONTAL-BRANCH EVOLUTION; STELLAR ASTROPHYSICS MESA; PRE-SUPERNOVA EVOLUTION; MASSIVE STARS; ATOMIC DIFFUSION; SOLAR CONVECTION; RED GIANTS; NUMERICAL TREATMENT AB We examine the physical basis for algorithms to replace mixing-length theory (MLT) in stellar evolutionary computations. Our 321D procedure is based on numerical solutions of the Navier-Stokes equations. These implicit large eddy simulations (ILES) are three-dimensional (3D), time-dependent, and turbulent, including the Kolmogorov cascade. We use the Reynolds-averaged Navier-Stokes (RANS) formulation to make concise the 3D simulation data, and use the 3D simulations to give closure for the RANS equations. We further analyze this data set with a simple analytical model, which is non-local and time-dependent, and which contains both MLT and the Lorenz convective roll as particular subsets of solutions. A characteristic length (the damping length) again emerges in the simulations; it is determined by an observed balance between (1) the large-scale driving, and (2) small-scale damping. The nature of mixing and convective boundaries is analyzed, including dynamic, thermal and compositional effects, and compared to a simple model. We find that (1) braking regions (boundary layers in which mixing occurs) automatically appear beyond the edges of convection as defined by the Schwarzschild criterion, (2) dynamic (non-local) terms imply a non-zero turbulent kinetic energy flux (unlike MLT), (3) the effects of composition gradients on flow can be comparable to thermal effects, and (4) convective boundaries in neutrino-cooled stages differ in nature from those in photon-cooled stages (different Peclet numbers). The algorithms are based upon ILES solutions to the Navier-Stokes equations, so that, unlike MLT, they do not require any calibration to astronomical systems in order to predict stellar properties. Implications for solar abundances, helioseismology, asteroseismology, nucleosynthesis yields, supernova progenitors and core collapse are indicated. C1 [Arnett, W. David; Meakin, Casey] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [Arnett, W. David] Aspen Ctr Phys, Aspen, CO 81611 USA. [Viallet, Maxime; Campbell, Simon W.] Max Planck Inst Astrophys, D-85748 Garching, Germany. [Campbell, Simon W.; Lattanzio, John C.] Monash Univ, Clayton, Vic, Australia. [Meakin, Casey; Mocak, Miroslav] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Arnett, WD (reprint author), Univ Arizona, Steward Observ, 933 N Cherry Ave, Tucson, AZ 85721 USA. OI Lattanzio, John/0000-0003-2952-859X; Arnett, David/0000-0002-6114-6973 FU NSF [0708871, 1107445]; NASA at the University of Arizona [NNX08AH19G]; Australian Research Council [DP1095368, DP120101815]; European Research Council [341157-COCO2CASA]; National Science Foundation [OCI-1053575, PHYS-1066293]; Australian Government; Government of Western Australia; National Computational Infrastructure under the National Computational Merit Allocation Scheme FX This work was supported in part by NSF 0708871, 1107445, NASA NNX08AH19G at the University of Arizona, and by Australian Research Council grants DP1095368 and DP120101815 (J. Lattanzio, P. I.) at Monash University, Clayton, Australia, and by the European Research Council through grant ERC-AdG No. 341157-COCO2CASA. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant No. OCI-1053575, and made use of ORNL/Kraken and TACC/Stampede. This work was supported in part by resources provided by the Pawsey Supercomputing Centre with funding from the Australian Government and the Government of Western Australia, and through the National Computational Infrastructure under the National Computational Merit Allocation Scheme. This work was supported in part by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. We wish to thank Alvio Renzini for asking W. D. A. (repeatedly) "why does MLT work?," Vitorio Canuto for helpful hints, and Marco Limongi, Alessando Chieffi, Norman Murray, Bill Paxton, and Stan Owocki for helpful and encouraging discussions. One of us (W. D. A.) wishes to thank Prof. Remo Ruffini of ICRAnet, and Prof. Lars Bildsten of the Kavli Institute of Theoretical Physics, for their hospitality and support. We wish to thank an anonymous referee for extensive comments which helped improve the paper. NR 169 TC 21 Z9 21 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 30 DI 10.1088/0004-637X/809/1/30 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500030 ER PT J AU Bennert, VN Treu, T Auger, MW Cosens, M Park, D Rosen, R Harris, CE Malkan, MA Woo, JH AF Bennert, Vardha N. Treu, Tommaso Auger, Matthew W. Cosens, Maren Park, Daeseong Rosen, Rebecca Harris, Chelsea E. Malkan, Matthew A. Woo, Jong-Hak TI A LOCAL BASELINE OF THE BLACK HOLE MASS SCALING RELATIONS FOR ACTIVE GALAXIES. III. THE M-BH-sigma RELATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion; accretion disks; black hole physics; galaxies: active; galaxies: evolution; quasars: general ID AGN MONITORING PROJECT; RADIUS-LUMINOSITY RELATIONSHIP; REVERBERATION MAPPING DATA; QUASAR HOST GALAXY; VELOCITY DISPERSION CORRELATION; NEAR-INFRARED LUMINOSITY; SPACE-TELESCOPE IMAGES; DIGITAL SKY SURVEY; GALACTIC NUCLEI; COSMIC EVOLUTION AB We create a baseline of the black hole (BH) mass (M-BH)-stellar-velocity dispersion (sigma) relation for active galaxies, using a sample of 66 local (0.02 < z < 0.09) Seyfert-1 galaxies, selected from the Sloan Digital Sky Survey (SDSS). Analysis of SDSS images yields AGN luminosities free of host-galaxy contamination, and morphological classification. 51/66 galaxies have spiral morphology. Out of these, 28 bulges have Sersic index n < 2 and are considered candidate pseudo-bulges, with eight being definite pseudo-bulges based on multiple classification criteria met. Only 4/66 galaxies show signs of interaction/merging. High signal-to-noise ratio Keck spectra provide the width of the broad H beta emission line free of Fe II emission and stellar absorption. AGN luminosity and H beta line widths are used to estimate M-BH. The Keck-based spatially resolved kinematics is used to determine stellar-velocity dispersion within the spheroid effective radius (sigma(spat,reff)). We find that sigma can vary on average by up to 40% across definitions commonly used in the literature, emphasizing the importance of using self-consistent definitions in comparisons and evolutionary studies. The M-BH-sigma relation for our Seyfert-1 galaxy sample has the same intercept and scatter as that of reverberation-mapped AGNs as well as that of quiescent galaxies, consistent with the hypothesis that our single epoch M-BH estimator and sample selection function do not introduce significant biases. Barred galaxies, merging galaxies, and those hosting pseudo-bulges do not represent outliers in the M-BH-sigma relation. This is in contrast with previous work, although no firm conclusion can be drawn on this matter due to the small sample size and limited resolution of the SDSS images. C1 [Bennert, Vardha N.; Cosens, Maren; Rosen, Rebecca] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Treu, Tommaso] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Treu, Tommaso; Malkan, Matthew A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Auger, Matthew W.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Park, Daeseong] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. [Harris, Chelsea E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Woo, Jong-Hak] Seoul Natl Univ, Dept Astron, Seoul 151, South Korea. RP Bennert, VN (reprint author), Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. EM vbennert@calpoly.edu; tt@astro.ucla.edu; mauger@ast.cam.ac.uk; mcosens@calpoly.edu; daeseong.park@nao.cas.cn; rosenrr@prodigy.net; ChelseaHarris@lbl.gov; malkan@astro.ucla.edu; woo@astro.snu.ac.kr FU NASA through a grant from the Space Telescope Science Institute [HST-AR-12625.11-A]; Association of Universities for Research in Astronomy, Incorporated, under NASA [NAS5-26555]; Packard Foundations; NSF [NSF-AST-1412315]; EACOA Fellowship from The East Asian Core Observatories Association; National Research Foundation of Korea to the Center for Galaxy Evolution Research [2010-0027919]; W. M. Keck Foundation; National Aeronautics and Space Administration; National Astronomical Observatories, Chinese Academy of Science (NAOC); National Astronomical Observatory of Japan (NAOJ); Korean Astronomy and Space Science Institute (KASI); Academia Sinica Institute of Astronomy and Astrophysics (ASIAA) FX We thank the anonymous referee for valuable comments helping to improve the paper. V.N.B. thanks Aaron Barth, Stephane Courteau, Eric Emsellem, and Stefanie Komossa for discussions. V.N.B. acknowledges assistance from a National Science Foundation (NSF) Research at Undergraduate Institutions (RUI) grant AST-1312296. Note that findings and conclusions do not necessarily represent views of the NSF. V.N.B. and T.T. acknowledge support for program number HST-AR-12625.11-A, provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. T.T. acknowledges support from the Packard Foundations in the form of a Packard Fellowship. T.T. gratefully acknowledges support from NSF through grant NSF-AST-1412315. D.P. acknowledges support through the EACOA Fellowship from The East Asian Core Observatories Association, which consists of the National Astronomical Observatories, Chinese Academy of Science (NAOC), the National Astronomical Observatory of Japan (NAOJ), Korean Astronomy and Space Science Institute (KASI), and Academia Sinica Institute of Astronomy and Astrophysics (ASIAA). J.H.W. acknowledges support by the National Research Foundation of Korea to the Center for Galaxy Evolution Research (2010-0027919). Data presented in this paper were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among Caltech, the University of California, and NASA. The Observatory was made possible by the generous financial support of the W. M. Keck Foundation. The authors recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. This research has made use of the public archive of the Sloan Digital Sky Survey and the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. NR 117 TC 6 Z9 6 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 20 DI 10.1088/0004-637X/809/1/20 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500020 ER PT J AU Broderick, AE Tchekhovskoy, A AF Broderick, Avery E. Tchekhovskoy, Alexander TI HORIZON-SCALE LEPTON ACCELERATION IN JETS: EXPLAINING THE COMPACT RADIO EMISSION IN M87 SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; black hole physics; galaxies: individual (M87); galaxies: jets; gamma rays: galaxies; radio continuum: galaxies ID ACTIVE GALACTIC NUCLEI; SUPERMASSIVE BLACK-HOLE; RELATIVISTIC MAGNETOHYDRODYNAMIC SIMULATIONS; ADVECTION-DOMINATED ACCRETION; SAGITTARIUS-A-ASTERISK; FAST TEV VARIABILITY; GRMHD SIMULATIONS; PAIR PRODUCTION; STELLAR ORBITS; FLOW AB It has now become clear that the radio jet in the giant elliptical galaxy M87 must turn on very close to the black hole. This implies the efficient acceleration of leptons within the jet at scales much smaller than feasible by the typical dissipative events usually invoked to explain jet synchrotron emission. Here we show that the stagnation surface, the separatrix between material that falls back into the black hole and material that is accelerated outward forming the jet, is a natural site of pair formation and particle acceleration. This occurs via an inverse Compton pair catastrophe driven by unscreened electric fields within the charge-starved region about the stagnation surface and substantially amplified by a post-gap cascade. For typical estimates of the jet properties in M87, we find excellent quantitive agreement between the predicted relativistic lepton densities and those required by recent high-frequency radio observations of M87. This mechanism fails to adequately fill a putative jet from Sagittarius A* with relativistic leptons, which may explain the lack of an obvious radio jet in the Galactic center. Finally, this process implies a relationship between the kinetic jet power and the gamma-ray luminosity of blazars, produced during the post-gap cascade. C1 [Broderick, Avery E.] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Broderick, Avery E.] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Broderick, AE (reprint author), Perimeter Inst Theoret Phys, 31 Caroline St North, Waterloo, ON N2L 2Y5, Canada. FU Perimeter Institute for Theoretical Physics; Natural Sciences and Engineering Research Council of Canada; Princeton Center for Theoretical Science Fellowship; NASA through the Einstein Fellowship Program [PF3-140131]; Perimeter Institute FX The authors thank Jon Arens, Dimitrios Giannios, Ramesh Narayan, and Alexander Philippov for helpful discussions. The authors would also like to thank the anonymous referee for many helpful suggestions that have resulted in a much improved presentation. A.E.B. receives financial support from Perimeter Institute for Theoretical Physics and the Natural Sciences and Engineering Research Council of Canada through a Discovery Grant. A.T. was supported by a Princeton Center for Theoretical Science Fellowship and by NASA through the Einstein Fellowship Program, grant PF3-140131. The simulations presented in this article used computational resources supported by XSEDE allocation TG-AST100040 on NICS Kraken and Nautilus and TACC Lonestar, Longhorn, Ranch, and Stampede. A.T. thanks Perimeter Institute for hospitality and financial support of three visits to Perimeter Institute during which most of the work on this project was carried out. NR 70 TC 10 Z9 10 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 97 DI 10.1088/0004-637X/809/1/97 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500097 ER PT J AU Dong, RB Zhu, ZH Whitney, B AF Dong, Ruobing Zhu, Zhaohuan Whitney, Barbara TI OBSERVATIONAL SIGNATURES OF PLANETS IN PROTOPLANETARY DISKS. I. GAPS OPENED BY SINGLE AND MULTIPLE YOUNG PLANETS IN DISKS SO ASTROPHYSICAL JOURNAL LA English DT Article DE circumstellar matter; planet-disk interactions; planets and satellites: formation; protoplanetary disks; stars: pre-main sequence; stars: variables: T Tauri, Herbig Ae/Be ID 2-DIMENSIONAL RADIATIVE-TRANSFER; INFRARED IMAGING POLARIMETRY; POLARIZED SCATTERED-LIGHT; LOW-MASS PLANETS; T TAURI STARS; CIRCUMSTELLAR DISKS; TRANSITIONAL DISKS; GIANT PLANETS; PRETRANSITIONAL DISKS; EMBEDDED PLANETS AB It has been suggested that the gaps and cavities recently discovered in transitional disks are opened by planets. To explore this scenario, we combine two-dimensional two fluid (gas + particle) hydrodynamical calculations with three-dimensional Monte Carlo Radiative Transfer simulations and study the observational signatures of gaps opened by one or several planets, making qualitative comparisons with observations. We find that a single planet as small as 0.2 M-J can produce a deep gap at millimeter wavelengths and almost no features at near-infrared (NIR) wavelengths, while multiple planets can open up a few x10 AU wide common gap at both wavelengths. Both the contrast ratio of the gaps and the wavelength dependence of the gap sizes are broadly consistent with data. We also confirm previous results that NIR gap sizes may be smaller than millimeter gap sizes due to dust-gas coupling and radiative transfer effects. When viewed at a moderate inclination angle, a physically circular on-centered gap could appear to be off-centered from the star due to shadowing. Planet-induced spiral arms are more apparent at NIR than at millimeter wavelengths. Overall, our results suggest that the planet-opening-gap scenario is a promising way to explain the origin of the transitional disks. Finally, inspired by the recent Atacama Large Millimeter Array release of the image of the HL Tau disk, we show that multiple narrow gaps, well separated by bright rings, can be opened by 0.2M(J) planets soon after their formation in a relatively massive disk. C1 [Dong, Ruobing] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Dong, Ruobing] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Zhu, Zhaohuan] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Whitney, Barbara] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. RP Dong, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM rdong2013@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; NASA through Hubble Fellowship - Space Telescope Science Institute [HST-HF-51333.01-A, HST-HF-51320.01-A]; NASA [NAS 5-26555] FX We thank Anthony Boccaletti, Nuria Calvet, Eugene Chiang, Gaspard Duchene, Paul Duffell, Jeffery Fung, Lee Hartmann, Jun Hashimoto, Andrea Isella, Stefan Kraus, John Monnier, Paola Pinilla, Dick Plambeck, Roman Rafikov, Tom Robitaille, Jiming Shi, Jonathan Williams, Mike Wolff, and Ke Zhang for useful discussions and help. This research used the SAVIO computational cluster at UC Berkeley, and the Lawrencium computational cluster resource provided by the IT Division at the Lawrence Berkeley National Laboratory (Supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231). R.D. particularly acknowledges the help from Yong Qin and Kai Song. R.D. would like to thank Zhao Zhu for her support and encouragement in the period of this work. This project is partially supported by NASA through Hubble Fellowship grants HST-HF-51333.01-A (Z.Z.) and HST-HF-51320.01-A (R.D.) awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. We also thank the anonymous referee for constructive suggestions that largely improved the quality of the paper. This paper makes use of the following ALMA data: ADS/JAO.ALMA#2011.0.00015.SV. ALMA is a partnership of ESO (representing its member states), NSF (USA), and NINS (Japan), together with NRC (Canada), NSC and ASIAA (Taiwan), and KASI (Republic of Korea), in cooperation with the Republic of Chile. The Joint ALMA Observatory is operated by ESO, AUI/NRAO, and NAOJ. The National Radio Astronomy Observatory is a facility of the National Science Foundation operated under cooperative agreement by Associated Universities, Inc. NR 123 TC 37 Z9 37 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 93 DI 10.1088/0004-637X/809/1/93 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500093 ER PT J AU Errard, J Ade, PAR Akiba, Y Arnold, K Atlas, M Baccigalupi, C Barron, D Boettger, D Borrill, J Chapman, S Chinone, Y Cukierman, A Delabrouille, J Dobbs, M Ducout, A Elleflot, T Fabbian, G Feng, C Feeney, S Gilbert, A Goeckner-Wald, N Halverson, NW Hasegawa, M Hattori, K Hazumi, M Hill, C Holzapfel, WL Hori, Y Inoue, Y Jaehnig, GC Jaffe, AH Jeong, O Katayama, N Kaufman, J Keating, B Kermish, Z Keskitalo, R Kisner, T Le Jeune, M Lee, AT Leitch, EM Leon, D Linder, E Matsuda, F Matsumura, T Miller, NJ Myers, MJ Navaroli, M Nishino, H Okamura, T Paar, H Peloton, J Poletti, D Puglisi, G Rebeiz, G Reichardt, CL Richards, PL Ross, C Rotermund, KM Schenck, DE Sherwin, BD Siritanasak, P Smecher, G Stebor, N Steinbach, B Stompor, R Suzuki, A Tajima, O Takakura, S Tikhomirov, A Tomaru, T Whitehorn, N Wilson, B Yadav, A Zahn, O AF Errard, J. Ade, P. A. R. Akiba, Y. Arnold, K. Atlas, M. Baccigalupi, C. Barron, D. Boettger, D. Borrill, J. Chapman, S. Chinone, Y. Cukierman, A. Delabrouille, J. Dobbs, M. Ducout, A. Elleflot, T. Fabbian, G. Feng, C. Feeney, S. Gilbert, A. Goeckner-Wald, N. Halverson, N. W. Hasegawa, M. Hattori, K. Hazumi, M. Hill, C. Holzapfel, W. L. Hori, Y. Inoue, Y. Jaehnig, G. C. Jaffe, A. H. Jeong, O. Katayama, N. Kaufman, J. Keating, B. Kermish, Z. Keskitalo, R. Kisner, T. Le Jeune, M. Lee, A. T. Leitch, E. M. Leon, D. Linder, E. Matsuda, F. Matsumura, T. Miller, N. J. Myers, M. J. Navaroli, M. Nishino, H. Okamura, T. Paar, H. Peloton, J. Poletti, D. Puglisi, G. Rebeiz, G. Reichardt, C. L. Richards, P. L. Ross, C. Rotermund, K. M. Schenck, D. E. Sherwin, B. D. Siritanasak, P. Smecher, G. Stebor, N. Steinbach, B. Stompor, R. Suzuki, A. Tajima, O. Takakura, S. Tikhomirov, A. Tomaru, T. Whitehorn, N. Wilson, B. Yadav, A. Zahn, O. TI MODELING ATMOSPHERIC EMISSION FOR CMB GROUND-BASED OBSERVATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE atmospheric effects; methods: data analysis; methods: observational ID MICROWAVE BACKGROUND EXPERIMENTS; COMPONENT SEPARATION; FLUCTUATIONS; POLARIZATION; TURBULENCE; SITES; NOISE AB Atmosphere is one of the most important noise sources for ground-based cosmic microwave background (CMB) experiments. By increasing optical loading on the detectors, it amplifies their effective noise, while its fluctuations introduce spatial and temporal correlations between detected signals. We present a physically motivated 3D-model of the atmosphere total intensity emission in the millimeter and sub-millimeter wavelengths. We derive a new analytical estimate for the correlation between detectors time-ordered data as a function of the instrument and survey design, as well as several atmospheric parameters such as wind, relative humidity, temperature and turbulence characteristics. Using an original numerical computation, we examine the effect of each physical parameter on the correlations in the time series of a given experiment. We then use a parametric-likelihood approach to validate the modeling and estimate atmosphere parameters from the POLARBEAR-I project first season data set. We derive a new 1.0% upper limit on the linear polarization fraction of atmospheric emission. We also compare our results to previous studies and weather station measurements. The proposed model can be used for realistic simulations of future ground-based CMB observations. C1 [Errard, J.; Borrill, J.; Kisner, T.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Errard, J.; Borrill, J.; Keskitalo, R.; Kisner, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Ade, P. A. R.] Cardiff Univ, Sch Phys & Astron, Cardiff CF10 3XQ, S Glam, Wales. [Akiba, Y.; Chinone, Y.; Hasegawa, M.; Hattori, K.; Hazumi, M.; Inoue, Y.; Okamura, T.; Tajima, O.; Takakura, S.; Tomaru, T.] High Energy Accelerator Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Arnold, K.; Atlas, M.; Barron, D.; Elleflot, T.; Kaufman, J.; Keating, B.; Leon, D.; Matsuda, F.; Navaroli, M.; Paar, H.; Siritanasak, P.; Stebor, N.; Wilson, B.; Yadav, A.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Baccigalupi, C.; Fabbian, G.; Puglisi, G.] Int Sch Adv Studies SISSA, I-34014 Trieste, Italy. [Boettger, D.] Pontificia Univ Catolica Chile, Dept Astron, Santiago, Chile. [Chapman, S.; Ross, C.; Rotermund, K. M.; Tikhomirov, A.] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 4R2, Canada. [Chinone, Y.; Cukierman, A.; Goeckner-Wald, N.; Hill, C.; Holzapfel, W. L.; Hori, Y.; Jeong, O.; Lee, A. T.; Myers, M. J.; Richards, P. L.; Sherwin, B. D.; Steinbach, B.; Suzuki, A.; Whitehorn, N.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Delabrouille, J.; Le Jeune, M.; Peloton, J.; Poletti, D.; Stompor, R.] Univ Paris Diderot, Sorbonne Paris Cite, AstroParticule & Cosmol, CNRS,IN2P3,CEA,Irfu,Obs Paris, Paris, France. [Dobbs, M.; Gilbert, A.; Smecher, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 0G4, Canada. [Ducout, A.; Feeney, S.; Jaffe, A. H.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England. [Feng, C.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Halverson, N. W.; Jaehnig, G. C.; Schenck, D. E.] Univ Colorado, Ctr Astrophys & Space Astron, Boulder, CO 80309 USA. [Halverson, N. W.; Schenck, D. E.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Halverson, N. W.; Jaehnig, G. C.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Hasegawa, M.; Hazumi, M.] Grad Univ Adv Studies, Miura Dist, Kanagawa 2400115, Japan. [Hazumi, M.; Katayama, N.; Nishino, H.] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Kermish, Z.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Lee, A. T.; Linder, E.; Zahn, O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Leitch, E. M.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Leitch, E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Matsumura, T.] JAXA, Chofu, Tokyo, Japan. [Miller, N. J.] NASA, Goddard Space Flight Ctr, Observat Cosmol Lab, Greenbelt, MD 20771 USA. [Rebeiz, G.] Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92093 USA. [Reichardt, C. L.] Univ Melbourne, Sch Phys, Parkville, Vic 3010, Australia. [Sherwin, B. D.] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Takakura, S.] Osaka Univ, Toyonaka, Osaka 5600043, Japan. RP Errard, J (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. OI Fabbian, Giulio/0000-0002-3255-4695; Reichardt, Christian/0000-0003-2226-9169; Chinone, Yuji/0000-0002-3266-857X FU Department of Energy [DE-AC02-05CH11231]; National Science Foundation [AST-0618398, AST-1212230]; Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT) FX Calculations were performed on the National Energy Research Scientific Computing (NERSC), supported by the Department of Energy under Contract No. DE-AC02-05CH11231. The POLARBEAR project is funded by the National Science Foundation under grants AST-0618398 and AST-1212230. The James Ax Observatory operates in the Parque Astronomico Atacama in Northern Chile under the auspices of the Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT). Finally, we would like to acknowledge the tremendous contributions by Huan Tran to the POLARBEAR instrument and who has been at the initiation of this particular project on atmosphere characterization. NR 39 TC 3 Z9 3 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 10 PY 2015 VL 809 IS 1 AR 63 DI 10.1088/0004-637X/809/1/63 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CR9DN UT WOS:000361653500063 ER PT J AU Mendoza-Garcia, A Zhu, HY Yu, YS Li, Q Zhou, L Su, D Kramer, MJ Sun, SH AF Mendoza-Garcia, Adriana Zhu, Huiyuan Yu, Yongsheng Li, Qing Zhou, Lin Su, Dong Kramer, Matthew J. Sun, Shouheng TI Controlled Anisotropic Growth of Co-Fe-P from Co-Fe-O Nanoparticles SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE cobalt-iron phosphides; metal oxide phosphidation; nanorods; oxygen evolution reaction ID COBALT PHOSPHIDE NANOPARTICLES; HYDROGEN EVOLUTION REACTION; MAGNETIC-PROPERTIES; OXYGEN EVOLUTION; IRON; REACTIVITY; OXIDATION; CATALYSTS; OXIDES; WATER AB A facile approach to bimetallic phosphides, Co-Fe-P, by a high-temperature (300 degrees C) reaction between Co-Fe-O nanoparticles and trioctylphosphine is presented. The growth of Co-Fe-P from the Co-Fe-O is anisotropic. As a result, Co-Fe-P nanorods (from the polyhedral Co-Fe-O nanoparticles) and sea-urchin-like Co-Fe-P (from the cubic Co-Fe-O nanoparticles) are synthesized with both the nanorod and the sea-urchin-arm dimensions controlled by Co/Fe ratios. The Co-Fe-P structure, especially the sea-urchin-like (Co0.54Fe0.46)(2)P, shows enhanced catalysis for the oxygen evolution reaction in KOH with its catalytic efficiency surpassing the commercial Ir catalyst. Our synthesis is simple and may be readily extended to the preparation of other multimetallic phosphides for important catalysis and energy storage applications. C1 [Mendoza-Garcia, Adriana; Zhu, Huiyuan; Yu, Yongsheng; Li, Qing; Sun, Shouheng] Brown Univ, Dept Chem, Providence, RI 02912 USA. [Zhou, Lin; Kramer, Matthew J.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Sun, SH (reprint author), Brown Univ, Dept Chem, Providence, RI 02912 USA. EM ssun@brown.edu RI Li, Qing/G-4502-2011 OI Li, Qing/0000-0003-4807-030X FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE) under Vehicle Technologies Program through Ames Laboratory; Iowa State University [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE), under its Vehicle Technologies Program, through the Ames Laboratory. The Ames Laboratory is operated by Iowa State University under contract DE-AC02-07CH11358. Electron microscopy work carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886. NR 21 TC 17 Z9 17 U1 35 U2 206 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 10 PY 2015 VL 54 IS 33 BP 9642 EP 9645 DI 10.1002/anie.201503386 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CO2LI UT WOS:000358987300036 PM 26118355 ER PT J AU Procter, RA Magnus, F Andersson, G Sanchez-Hanke, C Hjorvarsson, B Hase, TPA AF Procter, R. A. Magnus, F. Andersson, G. Sanchez-Hanke, C. Hjorvarsson, B. Hase, T. P. A. TI Magnetic leverage effects in amorphous SmCo/CoAlZr heterostructures SO APPLIED PHYSICS LETTERS LA English DT Article ID MEDIUM-RANGE ORDER; PERCOLATION THRESHOLDS; THERMAL-STABILITY; METALLIC GLASSES; CAPPING LAYERS; LATTICES; FILMS; FCC AB Although magnetic heterostructures are the basis of many magnetic technologies, the mechanisms involved in magnetization reversals in such structures are not fully understood, especially in amorphous multilayers. Here, we report on the SmCo/CoAlZr system and exploit resonant magnetic x-ray scattering to probe the element specific magnetization reversals. When combined into a tri-layer structure, two different switching fields and reversal mechanisms are observed for the Sm and Co sub-lattices. We argue that the decoupling of the sub-lattices arises from the local distribution of atomic species within the amorphous matrix leading to a strong magnetic leverage effect and exchange pinning. The decoupling arises due to strong interactions between regions of high Co density which span the interface. The relatively sparse interactions between Sm and Co induce a localized pinning of the Co-rich areas, resulting in an exchange bias in minor loops and an enhanced coercivity. (C) 2015 AIP Publishing LLC. C1 [Procter, R. A.; Hase, T. P. A.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Magnus, F.; Andersson, G.; Hjorvarsson, B.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Sanchez-Hanke, C.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Procter, RA (reprint author), Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. EM r.a.procter@warwick.ac.uk RI Magnus, Fridrik/A-5659-2016; OI Magnus, Fridrik/0000-0003-2606-8559; Hjorvarsson, Bjorgvin/0000-0003-1803-9467; Hase, Thomas/0000-0001-5274-5942; Andersson, Gabriella/0000-0002-9479-1952 FU UK-EPSRC; Swedish Research Council (VR); Knut and Alice Wallenberg Foundation (KAW); Swedish Foundation for International Cooperation in Research and Higher Education (STINT); Carl Trygger Foundation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-AC02-06CH11357] FX The authors acknowledge the financial support of the UK-EPSRC and the Swedish Research Council (VR) as well as the Knut and Alice Wallenberg Foundation (KAW), the Swedish Foundation for International Cooperation in Research and Higher Education (STINT) and the Carl Trygger Foundation. Work undertaken at the NSLS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract Nos. DE-AC02-98CH10886 and DE-AC02-06CH11357. B.H. thanks V. Kapaklis for useful discussions. NR 28 TC 1 Z9 1 U1 4 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 10 PY 2015 VL 107 IS 6 AR 062403 DI 10.1063/1.4928632 PG 4 WC Physics, Applied SC Physics GA CP3QB UT WOS:000359794200017 ER PT J AU Dong, RB Zhu, ZH Rafikov, RR Stone, JM AF Dong, Ruobing Zhu, Zhaohuan Rafikov, Roman R. Stone, James M. TI OBSERVATIONAL SIGNATURES OF PLANETS IN PROTOPLANETARY DISKS II: SPIRAL ARMS OBSERVED IN SCATTERED LIGHT IMAGING CAN BE INDUCED BY PLANETS SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE circumstellar matter; planet-disk interactions; planets and satellites: formation; protoplanetary disks; radiative transfer; stars: variables: T Tauri, Herbig Ae/Be ID LOW-MASS PLANETS; UNSPLIT GODUNOV METHOD; TRANSITIONAL DISKS; CONSTRAINED TRANSPORT; SAO 206462; IDEAL MHD; CAVITY; SIMULATIONS; EVOLUTION; RADIATION AB Using 3D global hydro simulations coupled with radiative transfer calculations, we study the appearance of density waves induced by giant planets in direct imaging observations at near-infrared wavelengths. We find that a 6M(J) planet in a typical disk around a 1M(circle dot) star can produce prominent and detectable spiral arms both interior and exterior to its orbit. The inner arms have (1) two well separated arms in roughly m = 2 symmetry, (2) exhibit similar to 10 degrees-15 degrees pitch angles, (3) similar to 180 degrees-270 degrees extension in the azimuthal direction, and (4) similar to 150% surface brightness enhancement, all broadly consistent with observed spiral arms in the SAO 206462 and MWC 758 systems. The outer arms cannot explain observations as they are too tightly wound given typical disk scale height. We confirm previous results that the outer density waves excited by a 1M(J) planet exhibit low contrast in the IR and are practically not detectable. We also find that 3D effects of the waves are important. Compared to isothermal models, density waves in adiabatic disks exhibit weaker contrast in surface density but stronger contrast in scattered light images, due to a more pronounced vertical structure in the former caused by shock heating and maybe hydraulic jump effect. To drive observed pairs of arms with an external companion on a circular orbit, a massive planet, possibly a brown dwarf, is needed at around [r similar to 0."7, PA similar to 10 degrees] (position angle PA from north to east) in SAO 206462 and [ r similar to 0."6, PA similar to 10 degrees] in MWC 758. Their existence may be confirmed by direct imaging planet searches. C1 [Dong, Ruobing] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Dong, Ruobing] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Zhu, Zhaohuan; Rafikov, Roman R.; Stone, James M.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. RP Dong, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM rdong2013@berkeley.edu FU NASA by the Space Telescope Science Institute [HST-HF-51333.01-A, HST-HF-51320.01-A]; NASA [NAS 5-26555]; XSEDE grant [TG-AST130002] FX We thank Eugene Chiang, Barbara Whitney, Eric Pantin, Eduard Vorobyov, and Jun Hashimoto for insightful discussions and help in this work. We also thank the anonymous referee for constructive suggestions that largely improved the quality of the paper. We thank Myriam Benisty for kindly sharing with us the VLT/SPHERE image of MWC 758. This project is partially motivated by the Subaru based SEEDS program (PI: M. Tamura). This project is supported by NASA through Hubble Fellowship grants HST-HF-51333.01-A (Z.Z.) and HST-HF-51320.01-A (R.D.) awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. All hydrodynamic simulations are carried out at the Texas Advanced Computing Center (TACC) at The University of Texas at Austin using Stampede through XSEDE grant TG-AST130002. NR 39 TC 29 Z9 29 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD AUG 10 PY 2015 VL 809 IS 1 AR L5 DI 10.1088/2041-8205/809/1/L5 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO7EJ UT WOS:000359321900005 ER PT J AU Drlica-Wagner, A Albert, A Bechtol, K Wood, M Strigari, L Sanchez-Conde, M Baldini, L Essig, R Cohen-Tanugi, J Anderson, B Bellazzini, R Bloom, ED Caputo, R Cecchi, C Charles, E Chiang, J de Angelis, A Funk, S Fusco, P Gargano, F Giglietto, N Giordano, F Guiriec, S Gustafsson, M Kuss, M Loparco, F Lubrano, P Mirabal, N Mizuno, T Morselli, A Ohsugi, T Orlando, E Persic, M Raino, S Sehgal, N Spada, F Suson, DJ Zaharijas, G Zimmer, S Abbott, T Allam, S Balbinot, E Bauer, AH Benoit-Levy, A Bernstein, RA Bernstein, GM Bertin, E Brooks, D Buckley-Geer, E Burke, DL Rosell, AC Castander, FJ Covarrubias, R D'Andrea, CB da Costa, LN DePoy, DL Desai, S Diehl, HT Cunha, CE Eifler, TF Estrada, J Evrard, AE Neto, AF Fernandez, E Finley, DA Flaugher, B Frieman, J Gaztanaga, E Gerdes, D Gruen, D Gruendl, RA Gutierrez, G Honscheid, K Jain, B James, D Jeltema, T Kent, S Kron, R Kuehn, K Kuropatkin, N Lahav, O Li, TS Luque, E Maia, MAG Makler, M March, M Marshall, J Martini, P Merritt, KW Miller, C Miquel, R Mohr, J Neilsen, E Nord, B Ogando, R Peoples, J Petravick, D Pieres, A Plazas, AA Queiroz, A Romer, AK Roodman, A Rykoff, ES Sako, M Sanchez, E Santiago, B Scarpine, V Schubnell, M Sevilla, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Tucker, D Walker, AR Wechsler, RH Wester, W Williams, P Yanny, B Zuntz, J AF Drlica-Wagner, A. Albert, A. Bechtol, K. Wood, M. Strigari, L. Sanchez-Conde, M. Baldini, L. Essig, R. Cohen-Tanugi, J. Anderson, B. Bellazzini, R. Bloom, E. D. Caputo, R. Cecchi, C. Charles, E. Chiang, J. de Angelis, A. Funk, S. Fusco, P. Gargano, F. Giglietto, N. Giordano, F. Guiriec, S. Gustafsson, M. Kuss, M. Loparco, F. Lubrano, P. Mirabal, N. Mizuno, T. Morselli, A. Ohsugi, T. Orlando, E. Persic, M. Raino, S. Sehgal, N. Spada, F. Suson, D. J. Zaharijas, G. Zimmer, S. Abbott, T. Allam, S. Balbinot, E. Bauer, A. H. Benoit-Levy, A. Bernstein, R. A. Bernstein, G. M. Bertin, E. Brooks, D. Buckley-Geer, E. Burke, D. L. Carnero Rosell, A. Castander, F. J. Covarrubias, R. D'Andrea, C. B. da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Cunha, C. E. Eifler, T. F. Estrada, J. Evrard, A. E. Fausti Neto, A. Fernandez, E. Finley, D. A. Flaugher, B. Frieman, J. Gaztanaga, E. Gerdes, D. Gruen, D. Gruendl, R. A. Gutierrez, G. Honscheid, K. Jain, B. James, D. Jeltema, T. Kent, S. Kron, R. Kuehn, K. Kuropatkin, N. Lahav, O. Li, T. S. Luque, E. Maia, M. A. G. Makler, M. March, M. Marshall, J. Martini, P. Merritt, K. W. Miller, C. Miquel, R. Mohr, J. Neilsen, E. Nord, B. Ogando, R. Peoples, J. Petravick, D. Pieres, A. Plazas, A. A. Queiroz, A. Romer, A. K. Roodman, A. Rykoff, E. S. Sako, M. Sanchez, E. Santiago, B. Scarpine, V. Schubnell, M. Sevilla, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Tucker, D. Walker, A. R. Wechsler, R. H. Wester, W. Williams, P. Yanny, B. Zuntz, J. CA Fermi-LAT Collaboration DES Collaboration TI SEARCH FOR GAMMA-RAY EMISSION FROM DES DWARF SPHEROIDAL GALAXY CANDIDATES WITH FERMI-LAT DATA SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE dark matter; galaxies: dwarf; gamma rays: galaxies; Local Group ID LARGE-AREA TELESCOPE; UNIVERSAL MASS PROFILE; DARK-MATTER; LOCAL GROUP; CONSTRAINTS AB Due to their proximity, high dark-matter (DM) content, and apparent absence of non-thermal processes, Milky Way dwarf spheroidal satellite galaxies (dSphs) are excellent targets for the indirect detection of DM. Recently, eight new dSph candidates were discovered using the first year of data from the Dark Energy Survey (DES). We searched for gamma-ray emission coincident with the positions of these new objects in six years of Fermi Large Area Telescope data. We found no significant excesses of gamma-ray emission. Under the assumption that the DES candidates are dSphs with DM halo properties similar to the known dSphs, we computed individual and combined limits on the velocity-averaged DM annihilation cross section for these new targets. If the estimated DM content of these dSph candidates is confirmed, they will constrain the annihilation cross section to lie below the thermal relic cross section for DM particles with masses less than or similar to 20 GeV annihilating via the b (b) over bar or pi(+)pi(-) channels. C1 [Drlica-Wagner, A.; Allam, S.; Buckley-Geer, E.; Diehl, H. T.; Estrada, J.; Finley, D. A.; Flaugher, B.; Frieman, J.; Gutierrez, G.; Kent, S.; Kuropatkin, N.; Merritt, K. W.; Neilsen, E.; Nord, B.; Peoples, J.; Scarpine, V.; Soares-Santos, M.; Sobreira, F.; Tucker, D.; Wester, W.; Yanny, B.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Albert, A.; Wood, M.; Bloom, E. D.; Charles, E.; Chiang, J.; Funk, S.; Orlando, E.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Albert, A.; Wood, M.; Bloom, E. D.; Charles, E.; Chiang, J.; Funk, S.; Orlando, E.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Bechtol, K.; Frieman, J.; Kron, R.; Williams, P.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Strigari, L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Sanchez-Conde, M.; Zimmer, S.] AlbaNova, Oskar Klein Ctr Cosmoparticle Phys, SE-10691 Stockholm, Sweden. [Sanchez-Conde, M.; Zimmer, S.] Stockholm Univ, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Baldini, L.] Univ Pisa, I-56127 Pisa, Italy. [Baldini, L.; Bellazzini, R.; Kuss, M.; Spada, F.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Essig, R.] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. [Cohen-Tanugi, J.] Univ Montpellier 2, CNRS, IN2P3, Lab Univers & Particules Montpellier, Montpellier, France. [Caputo, R.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Dept Phys, Santa Cruz, CA 95064 USA. [Caputo, R.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Cecchi, C.; Lubrano, P.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Cecchi, C.; Lubrano, P.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [de Angelis, A.] Univ Udine, Dipartimento Fis, I-33100 Udine, Italy. [de Angelis, A.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, I-33100 Udine, Italy. [Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.] Univ Bari, Dipartimento Fis M Merlin, I-70126 Bari, Italy. [Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.] Politecn Bari, I-70126 Bari, Italy. [Fusco, P.; Gargano, F.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Guiriec, S.; Mirabal, N.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Gustafsson, M.] Univ Gottingen, Inst Theoret Phys, Fac Phys, D-37077 Gottingen, Germany. [Mizuno, T.; Ohsugi, T.] Hiroshima Univ, Hiroshima Astrophys Sci Ctr, Hiroshima 7398526, Japan. [Morselli, A.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Persic, M.; Zaharijas, G.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Persic, M.] Osserv Astron Trieste, Ist Nazl Astrofis, I-34143 Trieste, Italy. [Sehgal, N.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Suson, D. J.] Purdue Univ Calumet, Dept Chem & Phys, Hammond, IN 46323 USA. [Zaharijas, G.] Univ Trieste, I-34127 Trieste, Italy. [Zaharijas, G.] Univ Nova Gorica, Lab Astroparticle Phys, SI-5000 Nova Gorica, Slovenia. [Abbott, T.; James, D.; Smith, R. C.; Walker, A. R.] Cerro Tololo Interamer Observ, Natl Opt Astron Observ, La Serena, Chile. [Allam, S.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Balbinot, E.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Balbinot, E.; Carnero Rosell, A.; da Costa, L. N.; Fausti Neto, A.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Bauer, A. H.; Castander, F. J.; Gaztanaga, E.] Fac Ciencies, IEEC CSIC, Inst Ciencies Espai, E-08193 Barcelona, Spain. [Benoit-Levy, A.; Brooks, D.; Lahav, O.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Bernstein, R. A.] Carnegie Observat, Pasadena, CA 91101 USA. [Bernstein, G. M.; Eifler, T. F.; Jain, B.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bertin, E.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.] CNRS, UMR7095, F-75014 Paris, France. [Burke, D. L.; Roodman, A.; Rykoff, E. S.; Wechsler, R. H.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Covarrubias, R.; Gruendl, R. A.; Petravick, D.; Swanson, M. E. C.] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [D'Andrea, C. B.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [DePoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Mohr, J.] Excellence Cluster Universe, D-85748 Garching, Germany. [Desai, S.; Mohr, J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Cunha, C. E.; Roodman, A.; Wechsler, R. H.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Eifler, T. F.; Plazas, A. A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Evrard, A. E.; Gerdes, D.; Miller, C.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Fernandez, E.; Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Fernandez, E.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Gruen, D.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Gruendl, R. A.; Sevilla, I.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Honscheid, K.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Honscheid, K.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Jeltema, T.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Jeltema, T.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Kuehn, K.] Argonne Natl Lab, Lemont, IL 60639 USA. [Luque, E.; Pieres, A.; Queiroz, A.; Santiago, B.] Univ Fed Rio Grande do Sul, Inst Fis, BR-91501970 Porto Alegre, RS, Brazil. [Makler, M.] Ctr Brasileiro Pesquisas Fis, ICRA, BR-22290180 Rio De Janeiro, RJ, Brazil. [Martini, P.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Miller, C.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Plazas, A. A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Romer, A. K.] Univ Sussex, Ctr Astron, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla, I.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Thaler, J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Wechsler, R. H.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. RP Drlica-Wagner, A (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. EM kadrlica@fnal.gov; aalbert@slac.stanford.edu; bechtol@kicp.uchicago.edu; mdwood@slac.stanford.edu; strigari@physics.tamu.edu RI Balbinot, Eduardo/E-8019-2015; Gaztanaga, Enrique/L-4894-2014; Morselli, Aldo/G-6769-2011; Funk, Stefan/B-7629-2015; Ogando, Ricardo/A-1747-2010; Loparco, Francesco/O-8847-2015; Gargano, Fabio/O-8934-2015; Makler, Martin/G-2639-2012; giglietto, nicola/I-8951-2012; Sanchez, Eusebio/H-5228-2015; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Orlando, E/R-5594-2016 OI Giordano, Francesco/0000-0002-8651-2394; Balbinot, Eduardo/0000-0002-1322-3153; Zaharijas, Gabrijela/0000-0001-8484-7791; Persic, Massimo/0000-0003-1853-4900; Strigari, Louis/0000-0001-5672-6079; Baldini, Luca/0000-0002-9785-7726; Tucker, Douglas/0000-0001-7211-5729; Gaztanaga, Enrique/0000-0001-9632-0815; Morselli, Aldo/0000-0002-7704-9553; Funk, Stefan/0000-0002-2012-0080; Suchyta, Eric/0000-0002-7047-9358; Ogando, Ricardo/0000-0003-2120-1154; Loparco, Francesco/0000-0002-1173-5673; Gargano, Fabio/0000-0002-5055-6395; Makler, Martin/0000-0003-2206-2651; giglietto, nicola/0000-0002-9021-2888; Sanchez, Eusebio/0000-0002-9646-8198; Sobreira, Flavia/0000-0002-7822-0658; Fernandez, Enrique/0000-0002-6405-9488; FU U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Union; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; University of Edinburgh; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat Munchen; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory; Stanford University; University of Sussex; Texas AM University; PAPDRJ CAPES/FAPERJ; DOE [DE-AC02-98CH10886]; JPL; National Aeronautics and Space Administration FX The Fermi-LAT Collaboration acknowledges support for LAT development, operation and data analysis from NASA and DOE (United States), CEA/Irfu and IN2P3/CNRS (France), ASI and INFN (Italy), MEXT, KEK, and JAXA (Japan), and the K. A. Wallenberg Foundation, the Swedish Research Council and the National Space Board (Sweden). Science analysis support in the operations phase from INAF (Italy) and CNES (France) is also gratefully acknowledged. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, the Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. A.C.R. acknowledges financial support provided by the PAPDRJ CAPES/FAPERJ Fellowship. A.A.P. was supported by DOE grant DE-AC02-98CH10886 and by JPL, run by Caltech under a contract for NASA. This research has made use of the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. We would like to thank the anonomous referee for many helpful comments. NR 43 TC 43 Z9 43 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD AUG 10 PY 2015 VL 809 IS 1 AR L4 DI 10.1088/2041-8205/809/1/L4 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO7EJ UT WOS:000359321900004 ER PT J AU Berkelbach, TC Hybertsen, MS Reichman, DR AF Berkelbach, Timothy C. Hybertsen, Mark S. Reichman, David R. TI Bright and dark singlet excitons via linear and two-photon spectroscopy in monolayer transition-metal dichalcogenides SO PHYSICAL REVIEW B LA English DT Article ID VALLEY POLARIZATION; MOS2; STATES; PHOTOLUMINESCENCE; SEMICONDUCTOR; ABSORPTION; GRAPHENE; WSE2; GAP AB We discuss the linear and two-photon spectroscopic selection rules for spin-singlet excitons in monolayer transition-metal dichalcogenides. Our microscopic formalism combines a fully k-dependent few-orbital band structure with a many-body Bethe-Salpeter equation treatment of the electron-hole interaction, using a model dielectric function. We show analytically a nd numerically that the single-particle, valley-dependent selection rules are preserved in the presence of excitonic effects. Furthermore, we definitively demonstrate that the bright (one-photon allowed) excitons have s-type azimuthal symmetry and that dark p-type excitons can be probed via two-photon spectroscopy. The screened Coulomb interaction in these materials substantially deviates from the 1/epsilon(0)r form; this breaks the "accidental" angular momentum degeneracy in the exciton spectrum, such that the 2p exciton has a lower energy than the 2s exciton by at least 50 meV. We compare our calculated two-photon absorption spectra to recent experimental measurements. C1 [Berkelbach, Timothy C.] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA. [Hybertsen, Mark S.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Reichman, David R.] Columbia Univ, Dept Chem, New York, NY 10027 USA. RP Berkelbach, TC (reprint author), Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA. FU Princeton Center for Theoretical Science (TCB); U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory [DE-SC0012704] FX The authors would like to thank Alexey Chernikov and Tony F. Heinz for invaluable discussions. T.C.B. thanks Ajit Srivastava for informative correspondence regarding Ref. [30]. Part of this work was supported by the Princeton Center for Theoretical Science (TCB), and part of this work was done using resources of the Center for Functional Nanomaterials which is a U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704 (MSH). NR 37 TC 11 Z9 11 U1 13 U2 61 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 10 PY 2015 VL 92 IS 8 AR 085413 DI 10.1103/PhysRevB.92.085413 PG 9 WC Physics, Condensed Matter SC Physics GA CO7MY UT WOS:000359344700017 ER PT J AU Feygenson, M Bauer, JC Gai, Z Marques, C Aronson, MC Teng, XW Su, D Stanic, V Urban, VS Beyer, KA Dai, S AF Feygenson, Mikhail Bauer, John C. Gai, Zheng Marques, Carlos Aronson, Meigan C. Teng, Xiaowei Su, Dong Stanic, Vesna Urban, Volker S. Beyer, Kevin A. Dai, Sheng TI Exchange bias effect in Au-Fe3O4 dumbbell nanoparticles induced by the charge transfer from gold SO PHYSICAL REVIEW B LA English DT Article ID DYNAMIC MAGNETIC-PROPERTIES; FE3O4 NANOPARTICLES; HYBRID NANOPARTICLES; NEUTRON-SCATTERING; FEO NANOPARTICLES; DRUG-DELIVERY; SPIN DISORDER; THIN-FILMS; SIZE; NANOCRYSTALS AB We have studied the origin of the exchange bias effect in the Au-Fe3O4 dumbbell nanoparticles in two samples with different sizes of the Au seed nanoparticles (4.1 and 2.7 nm) and same size of Fe3O4 nanoparticles (9.8 nm). The magnetization, small-angle neutron-scattering, synchrotron x-ray diffraction, and scanning transmission electron microscope measurements determined the antiferromagnetic FeO wustite phase within Fe3O4 nanoparticles, originating at the interface with the Au nanoparticles. The interface between antiferromagnetic FeO and ferrimagnetic Fe3O4 is giving rise to the exchange bias effect. The strength of the exchange bias fields depends on the interfacial area and lattice mismatch between both phases. We propose that the charge transfer from the Au nanoparticles is responsible for a partial reduction of the Fe3O4 into the FeO phase at the interface with Au nanoparticles. The Au-O bonds are formed, presumably across the interface to accommodate an excess of oxygen released during the reduction of magnetite. C1 [Feygenson, Mikhail] Oak Ridge Natl Lab, Spallat Neutron Source, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Bauer, John C.; Dai, Sheng] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Gai, Zheng] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Marques, Carlos; Aronson, Meigan C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Aronson, Meigan C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Teng, Xiaowei] Univ New Hampshire, Dept Chem Engn, Durham, NH 03824 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Stanic, Vesna] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Urban, Volker S.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Beyer, Kevin A.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Feygenson, M (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM feygensonm@ornl.gov RI Dai, Sheng/K-8411-2015; Urban, Volker/N-5361-2015; Gai, Zheng/B-5327-2012; Feygenson, Mikhail /H-9972-2014; OI Dai, Sheng/0000-0002-8046-3931; Urban, Volker/0000-0002-7962-3408; Gai, Zheng/0000-0002-6099-4559; Feygenson, Mikhail /0000-0002-0316-3265; Stanic, Vesna/0000-0003-0318-9454 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. DOE Office of Science [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geo-sciences, and Biosciences Division; Office of Biological and Environmental Research of the U.S. Department of Energy FX We are grateful to W. Dmowski and Y. Tong for helping with the x-ray measurements. We thank J. Simonson for his help with magnetization measurements at Brookhaven National Laboratory. We also acknowledge P. Konarev, S. Disch, J. C. Neuefeind, and K. Page for the stimulating discussions. V.S.U. acknowledges support by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. Portions of this research at the Oak Ridge National Laboratory's High Flux Isotope Reactor and Brookhaven National Laboratory's National Synchrotron Light Source were sponsored by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The Office of Biological and Environmental Research of the U.S. Department of Energy sponsored neutron-data collection on the CG-3 Bio-SANS instrument. Part of this research was conducted at the Center for Nanophase Materials Sciences (ORNL) and Center for Functional Nanomaterials (BNL), which are sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Work at Brookhaven National Laboratory (C.M. and M.C.A.) was carried out under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Contract No. DE-AC02-98CH1886. J.C.B. and S.D. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geo-sciences, and Biosciences Division. NR 92 TC 4 Z9 4 U1 9 U2 52 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 10 PY 2015 VL 92 IS 5 AR 054416 DI 10.1103/PhysRevB.92.054416 PG 13 WC Physics, Condensed Matter SC Physics GA CO7MN UT WOS:000359343600004 ER PT J AU Heinonen, O AF Heinonen, Olle TI Magnetization dynamics of coupled ferromagnetic disks SO PHYSICAL REVIEW B LA English DT Article ID ARTIFICIAL SPIN-ICE; DRIVEN AB The magnetization configuration in two stacked micron-size ferromagnetic disks can assume different equilibrium states depending on the interfacial coupling between the disks. Here I examine the magnetization dynamics in response to an out-of-plane field pulse for different equilibrium states. For antiferromagnetic coupling, the response spectrum generally consists of a lower-frequency part and a higher-frequency part. The former is related to the response of the core region, which has a significant in-plane response coupled to the out-of-plane one; the latter is related to spin waves generated at the edges of the disk. For a meron structure the response in the two disks to an out-of-plane pulse is also asymmetric. C1 [Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Heinonen, Olle] Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. RP Heinonen, O (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Heinonen, Olle/0000-0002-3618-6092 FU Department of Energy, Office of Science, Materials Science and Engineering Division FX This work was supported by the Department of Energy, Office of Science, Materials Science and Engineering Division. I gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 39 TC 0 Z9 0 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 10 PY 2015 VL 92 IS 5 AR 054420 DI 10.1103/PhysRevB.92.054420 PG 7 WC Physics, Condensed Matter SC Physics GA CO7MN UT WOS:000359343600008 ER PT J AU Sadigh, B Erhart, P Aberg, D AF Sadigh, Babak Erhart, Paul Aberg, Daniel TI Variational polaron self-interaction-corrected total-energy functional for charge excitations in insulators SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; ALKALI-HALIDES; BAND-GAPS; ELECTRON; SEMICONDUCTORS; SIMULATION; RESONANCE; EXCHANGE; SPECTRA AB We conduct a detailed investigation of the polaron self-interaction (pSI) error in standard approximations to the exchange-correlation (XC) functional within density-functional theory (DFT). The pSI leads to delocalization error in the polaron wave function and energy, as calculated from the Kohn-Sham (KS) potential in the native charge state of the polaron. This constitutes the origin of the systematic failure of DFT to describe the polaron formation in band insulators. It is shown that the delocalization error in these systems is, however, largely absent in the KS potential of the closed-shell neutral charge state. This leads to a modification of the DFT total-energy functional that corrects the pSI in the XC functional. The resulting pSIC-DFT method constitutes an accurate parameter-free ab initio methodology for calculating polaron properties in insulators at a computational cost that is orders of magnitude smaller than hybrid XC functionals. Unlike approaches that rely on parametrized localized potentials such as DFT+U, the pSIC-DFT method properly captures both site and bond-centered polaron configurations. This is demonstrated by studying formation and migration of self-trapped holes in alkali halides (bond-centered) as well as self-trapped electrons in an elpasolite compound (site-centered). The pSIC-DFT approach consistently reproduces the results obtained by hybrid XC functionals parametrized by DFT+G(0)W(0) calculations. Finally, we generalize the pSIC approach to hybrid functionals, and show that in stark contrast to conventional hybrid calculations of polaron energies, the pSIC-hybrid method is insensitive to the parametrization of the hybrid XC functional. On this basis, we further rationalize the success of the pSIC-DFT approach. C1 [Sadigh, Babak; Aberg, Daniel] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Erhart, Paul] Chalmers, Dept Appl Phys, S-41296 Gothenburg, Sweden. RP Sadigh, B (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM sadigh1@llnl.gov RI Erhart, Paul/G-6260-2011 OI Erhart, Paul/0000-0002-2516-6061 FU US DOE-NNSA [DE-AC52-07NA27344]; NA-22 agency; Knut and Alice Wallenberg Foundation; Area of Advance-Materials Science at Chalmers FX We thank Michael Surh at LLNL for very helpful discussions. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the US DOE-NNSA under Contract DE-AC52-07NA27344. Funding for this work was received from the NA-22 agency. P.E. acknowledges funding from the Knut and Alice Wallenberg Foundation and the Area of Advance-Materials Science at Chalmers. Computer time allocations by the Swedish National Infrastructure for Computing at NSC (Linkoping) and C3SE (Gothenburg) are gratefully acknowledged. NR 51 TC 5 Z9 5 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 10 PY 2015 VL 92 IS 7 AR 075202 DI 10.1103/PhysRevB.92.075202 PG 10 WC Physics, Condensed Matter SC Physics GA CO7MS UT WOS:000359344100009 ER PT J AU Wang, Y Wohlfeld, K Moritz, B Jia, CJ van Veenendaal, M Wu, K Chen, CC Devereaux, TP AF Wang, Y. Wohlfeld, K. Moritz, B. Jia, C. J. van Veenendaal, M. Wu, K. Chen, C. -C. Devereaux, T. P. TI Origin of strong dispersion in Hubbard insulators SO PHYSICAL REVIEW B LA English DT Article ID T-J MODEL; SINGLE-PARTICLE; QUANTUM ANTIFERROMAGNET; COPPER OXIDES; CUPRATE SUPERCONDUCTORS; CHARGE EXCITATIONS; SPECTRAL-FUNCTION; SPIN POLARONS; CUO2 PLANES; HOLE AB Using cluster perturbation theory, we explain the origin of the strongly dispersive feature found at high binding energy in the spectral function of the Hubbard model. By comparing the Hubbard and t-J-3s model spectra, we show that this dispersion does not originate from either coupling to spin fluctuations (proportional to J) or the free hopping (proportional to t). Instead, it should be attributed to a long-range, correlated hopping proportional to t(2)/U, which allows an effectively free motion of the hole within the same antiferromagnetic sublattice. This origin explains both the formation of the high-energy anomaly in the single-particle spectrum and the sensitivity of the high-binding-energy dispersion to the next-nearest-neighbor hopping t'. C1 [Wang, Y.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Wang, Y.; Wohlfeld, K.; Moritz, B.; Jia, C. J.; Wu, K.; Devereaux, T. P.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Wang, Y.; Wohlfeld, K.; Moritz, B.; Jia, C. J.; Wu, K.; Devereaux, T. P.] Stanford Univ, Menlo Pk, CA 94025 USA. [Wohlfeld, K.] Univ Warsaw, Fac Phys, Inst Theoret Phys, PL-02093 Warsaw, Poland. [Moritz, B.] Univ N Dakota, Dept Phys & Astrophys, Grand Forks, ND 58202 USA. [van Veenendaal, M.; Chen, C. -C.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [van Veenendaal, M.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Wang, Y (reprint author), Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. EM yaowang@stanford.edu; krzysztof.wohlfeld@fuw.edu.pl RI Moritz, Brian/D-7505-2015; OI Moritz, Brian/0000-0002-3747-8484; Jia, Chunjing/0000-0001-7999-1932 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515]; Computational Materials and Chemical Sciences Network (CMCSN) [DE-SC0007091]; Stanford Graduate Fellows in Science and Engineering; Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory (ANL); U.S. Department of Energy (DOE) [DE-AC02-06CH11357]; DOE Office of Basic Energy Sciences (BES) Award [DE-FG02-03ER46097]; NIU Institute for Nanoscience, Engineering and Technology; Polish National Science Center (NCN) [2012/04/A/ST3/00331]; U.S. Department of Energy, Office of Science [DE-AC02-05CH11231] FX We thank J. van den Brink, Y. He, A. M. Oles, Z.-X. Shen, and J. Spalek for insightful discussions. This work was supported at SLAC and Stanford University by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-76SF00515 and by the Computational Materials and Chemical Sciences Network (CMCSN) under Contract No. DE-SC0007091 for the collaboration. Y.W. was supported by the Stanford Graduate Fellows in Science and Engineering. C.C.C. is supported by the Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory (ANL), operated by U.S. Department of Energy (DOE) Contract No. DE-AC02-06CH11357. M.v.V. is supported by DOE Office of Basic Energy Sciences (BES) Award No. DE-FG02-03ER46097 and the NIU Institute for Nanoscience, Engineering and Technology. K. Wohlfeld acknowledges support from the Polish National Science Center (NCN) under Project No. 2012/04/A/ST3/00331. A portion of the computational work was performed using the resources of the National Energy Research Scientific Computing Center supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-05CH11231. NR 76 TC 6 Z9 6 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 10 PY 2015 VL 92 IS 7 AR 075119 DI 10.1103/PhysRevB.92.075119 PG 7 WC Physics, Condensed Matter SC Physics GA CO7MS UT WOS:000359344100006 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R Dascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M DErrico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S DOnofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, N Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Redondo Fernandez, I Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester , WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. Dascenzo, N. Datta, M. de Barbaro, P. Demortier, L. Deninno, M. DErrico, M. Devoto, F. Di Canto, A. Di Ruzza, B. Dittmann, J. R. Donati, S. DOnofrio, M. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Elagin, A. Erbacher, R. Errede, S. Esham, B. Farrington, S. Ramos, J. P. Fernandez Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Galloni, C. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Lopez, O. Gonzalez Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, N. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. H. Kim, S. B. Kim, Y. J. Kim, Y. K. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, H. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Lucchesi, D. Luca, A. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. Moore, R. Morello, M. J. Mukherjee, A. Muller, Th. Murat, P. Mussini, M. Nachtman, J. Nagai, Y. Naganoma, J. Nakano, I. Napier, A. Nett, J. Neu, C. Nigmanov, T. Nodulman, L. Noh, S. Y. Norniella, O. Oakes, L. Oh, S. H. Oh, Y. D. Oksuzian, I. Okusawa, T. Orava, R. Ortolan, L. Pagliarone, C. Palencia, E. Palni, P. Papadimitriou, V. Parker, W. Pauletta, G. Paulini, M. Paus, C. Phillips, T. J. Piacentino, G. Pianori, E. Pilot, J. Pitts, K. Plager, C. Pondrom, L. Poprocki, S. Potamianos, K. Pranko, A. Prokoshin, F. Ptohos, F. Punzi, G. Redondo Fernandez, I. Renton, P. Rescigno, M. Rimondi, F. Ristori, L. Robson, A. Rodriguez, T. Rolli, S. Ronzani, M. Roser, R. Rosner, J. L. Ruffini, F. Ruiz, A. Russ, J. Rusu, V. Sakumoto, W. K. Sakurai, Y. Santi, L. Sato, K. Saveliev, V. Savoy-Navarro, A. Schlabach, P. Schmidt, E. E. Schwarz, T. Scodellaro, L. Scuri, F. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shochet, M. Shreyber-Tecker, I. Simonenko, A. 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RI Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Paulini, Manfred/N-7794-2014 OI Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Paulini, Manfred/0000-0002-6714-5787 NR 1 TC 1 Z9 1 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 10 PY 2015 VL 92 IS 3 AR 039901 DI 10.1103/PhysRevD.92.039901 PG 4 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO7OI UT WOS:000359348800007 ER PT J AU Bailey, JA Bazavov, A Bernard, C Bouchard, CM Detar, C Du, D El-Khadra, AX Foley, J Freeland, ED Gamiz, E Gottlieb, S Heller, UM Komijani, J Kronfeld, AS Laiho, J Levkova, L Mackenzie, PB Neil, ET Qiu, SW Simone, J Sugar, R Toussaint, D van de Water, RS Zhou, R AF Bailey, Jon A. Bazavov, A. Bernard, C. Bouchard, C. M. DeTar, C. Du, Daping El-Khadra, A. X. Foley, J. Freeland, E. D. Gamiz, E. Gottlieb, Steven Heller, U. M. Komijani, J. Kronfeld, A. S. Laiho, J. Levkova, L. Mackenzie, P. B. Neil, E. T. Qiu, Si-Wei Simone, J. Sugar, R. Toussaint, D. van de Water, R. S. Zhou, Ran TI B -> Dl nu form factors at nonzero recoil and vertical bar V-cb vertical bar from 2+1-flavor lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID DECAY-RATE; D-ASTERISK; HEAVY; MESONS; QUARKS AB We present the first unquenched lattice-QCD calculation of the hadronic form factors for the exclusive decay (B) over bar -> Dl (nu) over bar at nonzero recoil. We carry out numerical simulations on 14 ensembles of gauge-field configurations generated with 2 + 1 flavors of asqtad-improved staggered sea quarks. The ensembles encompass a wide range of lattice spacings (approximately 0.045 to 0.12 fm) and ratios of light (up and down) to strange sea-quark masses ranging from 0.05 to 0.4. For the b and c valence quarks we use improved Wilson fermions with the Fermilab interpretation, while for the light valence quarks we use asqtad-improved staggered fermions. We extrapolate our results to the physical point using rooted staggered heavy-light meson chiral perturbation theory. We then parametrize the form factors and extend them to the full kinematic range using model-independent functions based on analyticity and unitarity. We present our final results for f + (q(2)) and f (0)(q(2)), including statistical and systematic errors, as coefficients of a series in the variable z and the covariance matrix between these coefficients. We then fit the lattice formfactor data jointly with the experimentally measured differential decay rate from BABAR to determine the CKM matrix element, vertical bar V-cb vertical bar = (39.6 +/- 1.7(QCD+exp) +/- 0.2(QED)) x 10(-3). As a byproduct of the joint fit we obtain the form factors with improved precision at large recoil. Finally, we use them to update our calculation of the ratio R(D) in the Standard Model, which yields R(D) = 0.299(11). C1 [Bailey, Jon A.] Seoul Natl Univ, Dept Phys & Astron, Seoul 151742, South Korea. [Bazavov, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Bernard, C.; Komijani, J.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Bouchard, C. M.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Bouchard, C. M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [DeTar, C.; Foley, J.; Levkova, L.; Qiu, Si-Wei] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Du, Daping; El-Khadra, A. X.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Freeland, E. D.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL 60603 USA. [Gamiz, E.] Univ Granada, CAFPE, Granada 18002, Spain. [Gamiz, E.] Univ Granada, Dept Fis Teor & Cosmos, Granada 18002, Spain. [Gottlieb, Steven; Zhou, Ran] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Kronfeld, A. S.; Mackenzie, P. B.; Simone, J.; van de Water, R. S.; Zhou, Ran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Kronfeld, A. S.] Tech Univ Munich, Inst Adv Study, D-85748 Garching, Germany. [Neil, E. T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Neil, E. T.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Sugar, R.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Toussaint, D.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. RP Bailey, JA (reprint author), Seoul Natl Univ, Dept Phys & Astron, Seoul 151742, South Korea. EM detar@physics.utah.edu; qiu@physics.utah.edu RI Gamiz, Elvira/E-8009-2016; Bouchard, Christopher/N-3723-2016 OI Gamiz, Elvira/0000-0001-5125-2687; Bouchard, Christopher/0000-0003-1639-7164 FU Office of Science of the U.S. Department of Energy; National Science Foundation's Teragrid/XSEDE Program; U.S. Department of Energy [DE-FG02-91ER40628, DE-FC02-06ER41446, DE-SC0010120, DE-FG02-91ER40661, DE-FG02-13ER42001, DE-FG02-ER41976]; U.S. National Science Foundation [PHY10-67881, PHY10-034278, PHY14-17805, PHY09-03571, PHY13-16748]; URA Visiting Scholars' program; MICINN (Spain) [FPA2010-16696]; Ramon y Cajal program; Junta de Andalucia (Spain) [FQM-101, FQM-6552]; European Commission [PCIG10-GA-2011-303781]; German Excellence Initiative; European Union Seventh Framework Programme [291763]; European Union's Marie Curie COFUND program; National Research Foundation of Korea (NRF) - Ministry of Education [2014027937]; NRF grant - Korean government (MEST) [2014001852]; Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; Fermi Research Alliance, LLC [DE-AC02-07CH11359] FX Computations for this work were carried out with resources provided by the USQCD Collaboration, the National Energy Research Scientific Computing Center, and the Argonne Leadership Computing Facility, which is funded by the Office of Science of the U.S. Department of Energy; and with resources provided by the National Institute for Computational Science and the Texas Advanced Computing Center, which are funded through the National Science Foundation's Teragrid/XSEDE Program. This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG02-91ER40628 (C. B., J. K.), No. DE-FC02-06ER41446 (C. D., J. F., L. L.), No. DE-SC0010120 (S. G.), No. DE-FG02-91ER40661 (S. G., R. Z.), No. DE-FG02-13ER42001 (D. D., A. X. K.), No. DE-FG02-ER41976 (D. T.); by the U.S. National Science Foundation under Grants No. PHY10-67881 and No. PHY10-034278 (C. D.), No. PHY14-17805 (J. L., D. D.), No. PHY09-03571 (S.-W.Q.), and No. PHY13-16748 (R. S.); by the URA Visiting Scholars' program (C. M. B., D. D., A. X. K.); by the MICINN (Spain) under Grant No. FPA2010-16696 and Ramon y Cajal program (E. G.); by the Junta de Andalucia (Spain) under Grants No. FQM-101 and No. FQM-6552 (E. G.); by the European Commission (E. C.) under Grant No. PCIG10-GA-2011-303781 (E. G.); by the German Excellence Initiative and the European Union Seventh Framework Programme under Grant Agreement No. 291763 as well as the European Union's Marie Curie COFUND program (A. S. K.); and by the Basic Science Research Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Education (No. 2014027937) and the Creative Research Initiatives Program (No. 2014001852) of the NRF grant funded by the Korean government (MEST) (J. A. B.). This manuscript has been co-authored by an employee of Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 62 TC 28 Z9 28 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 10 PY 2015 VL 92 IS 3 AR 034506 DI 10.1103/PhysRevD.92.034506 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO7OI UT WOS:000359348800004 ER PT J AU Berkowitz, E Buchoff, MI Rinaldi, E AF Berkowitz, Evan Buchoff, Michael I. Rinaldi, Enrico TI Lattice QCD input for axion cosmology SO PHYSICAL REVIEW D LA English DT Article ID STRONG-CP PROBLEM; INVISIBLE AXION; EARLY UNIVERSE; GAUGE-THEORIES; STRONG P; COMPUTER-SIMULATIONS; FINITE-TEMPERATURE; PARTICLE PHYSICS; GLOBAL STRINGS; HARMLESS AXION AB One intriguing beyond-the-Standard-Model particle is the QCD axion, which could simultaneously provide a solution to the Strong CP Problemand account for some, if not all, of the dark matter density in the Universe. This particle is a pseudo-Nambu-Goldstone boson of the conjectured Peccei-Quinn symmetry of the Standard Model. Its mass and interactions are suppressed by a heavy symmetry-breaking scale, f(a), the value of which is roughly greater than 10(9) GeV (or, conversely, the axion mass, m(a), is roughly less than 10(4) mu eV). The density of axions in the Universe, which cannot exceed the relic dark matter density and is aquantity of great interest in axion experiments like ADMX, is a result of the early Universe interplay between cosmological evolution and the axion mass as a function of temperature. The latter quantity is proportional to the second derivative of the temperature-dependent QCD free energy with respect to the CP-violating phase, theta. However, this quantity is generically nonperturbative, and previous calculations have only employed instanton models at the high temperatures of interest (roughly 1 GeV). In this and future works, we aim to calculate the temperature-dependent axion mass at small theta from first-principle lattice calculations, with controlled statistical and systematic errors. Once calculated, this temperature-dependent axion mass is input for the classical evolution equations of the axion density of the Universe, which is required to be less than or equal to the dark matter density. Due to a variety of lattice systematic effects at the very high temperatures required, we perform a calculation of the leading small-theta cumulant of the theta vacua on large volume lattices for SU(3) Yang-Mills with high statistics as a first proof of concept, before attempting a full QCD calculation in the future. From these pure glue results, the misalignment mechanism yields the axion mass bound m(a) >= (14.6 +/- 0.1) mu eV when Peccei-Quinn breaking occurs after inflation. C1 [Berkowitz, Evan; Rinaldi, Enrico] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Buchoff, Michael I.] Inst Nucl Theory, Seattle, WA 98195 USA. RP Berkowitz, E (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. OI Berkowitz, Evan/0000-0003-1082-1374; Rinaldi, Enrico/0000-0003-4134-809X FU U.S. Department of Energy by LLNL [DE-AC52-07NA27344]; DOE [DE-FG02-00ER41132]; LLNL Multiprogrammatic and Institutional Computing program through a Tier 1 Grand Challenge award FX We are indebted to David Kaplan for many useful discussions and pointing us toward these questions in axion cosmology. We would also like to thank Gianpaolo Carosi, Guido Cossu, Graham Kribs, Thorsten Kurth, Biagio Lucini, Pierre Sikivie, and Pavlos Vranas for useful discussions. We generated gauge configurations using CHROMA [98] on the GPU clusters (Edge and Surface) at LLNL. CHROMA was configured to use the QDP-JIT GPU library [99] to accelerate the production. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract No. DE-AC52-07NA27344. M. I. B. is supported by DOE Grant No. DE-FG02-00ER41132. This research was partially supported by the LLNL Multiprogrammatic and Institutional Computing program through a Tier 1 Grand Challenge award. NR 101 TC 20 Z9 20 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 10 PY 2015 VL 92 IS 3 AR 034507 DI 10.1103/PhysRevD.92.034507 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO7OI UT WOS:000359348800005 ER PT J AU Martinez-Macias, C Chen, MY Dixon, DA Gates, BC AF Martinez-Macias, Claudia Chen, Mingyang Dixon, David A. Gates, Bruce C. TI Single-Site Zeolite-Anchored Organoiridium Carbonyl Complexes: Characterization of Structure and Reactivity by Spectroscopy and Computational Chemistry SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE CO probe molecule; DFT calculations; iridium carbonyls; iridium hydride; zeolites ID RELATIVISTIC EFFECTIVE POTENTIALS; DEALUMINATED Y-ZEOLITE; SPIN-ORBIT OPERATORS; IRIDIUM COMPLEXES; CO; CATALYSTS; CLUSTERS; SUPPORTS; DENSITY; HYDROGENATION AB A family of HY zeolite-supported cationic organoiridium carbonyl complexes was formed by reaction of Ir(CO)(2)(acac) (acac=acetylacetonate) to form supported Ir(CO)(2) complexes, which were treated at 298K and 1atm with flowing gas-phase reactants, including C2H4, H-2, (CO)-C-12, (CO)-C-13, and D2O. Mass spectrometry was used to identify effluent gases, and infrared and X-ray absorption spectroscopies were used to characterize the supported species, with the results bolstered by DFT calculations. Because the support is crystalline and presents a nearly uniform array of bonding sites for the iridium species, these were characterized by a high degree of uniformity, which allowed a precise determination of the species involved in the replacement, for example, of one CO ligand of each Ir(CO)(2) complex with ethylene. The supported species include the following: Ir(CO)(2), Ir(CO)(C2H4)(2), Ir(CO)(C2H4), Ir(CO)(C2H5), and (tentatively) Ir(CO)(H). The data determine a reaction network involving all of these species. C1 [Martinez-Macias, Claudia; Gates, Bruce C.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Chen, Mingyang; Dixon, David A.] Univ Alabama, Dept Chem, Tuscaloosa, AL 35487 USA. [Chen, Mingyang] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. RP Gates, BC (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, One Shields Ave, Davis, CA 95616 USA. EM bcgates@ucdavis.edu RI ID, MRCAT/G-7586-2011 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-FG02-04ER15513, DE-SC0005822]; UC-MEXUS-CONACYT; DOE Office of Advanced Scientific Computing Research; Robert Ramsay Chair Fund of The University of Alabama; DOE Office of Science by Argonne National Laboratory (ANL) [DE-AC02-06CH11357]; DOE-NNSA [DE-NA0001974]; DOE-BES [DE-AC02-06CH11357, DE-FG02-99ER45775]; NSF; [De-AC05-00OR22725] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Grants DE-FG02-04ER15513 (C.M.M.) at the University of California, Davis, and DE-SC0005822 (M.C.) at The University of Alabama. C.M.M. was supported in part by the UC-MEXUS-CONACYT doctoral fellowship program. M.C. was also sponsored by the DOE Office of Advanced Scientific Computing Research and performed calculations at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, under Contract No. De-AC05-00OR22725. D.A.D. thanks the Robert Ramsay Chair Fund of The University of Alabama for support. This research was aided by resources of the Advanced Photon Source, a DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory (ANL) under Contract No. DE-AC02-06CH11357. Experiments were performed at beamline 10-ID-B (the MRCAT) at ANL; MRCAT operations are supported by the DOE and the MRCAT member institutions. We thank HPCAT (Sector 16) of APS for access to a glovebox for sample preparation and storage during our beam time. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. A.P.S. is supported by DOE-BES under Contract No. DE-AC02-06CH11357. NR 37 TC 7 Z9 7 U1 4 U2 23 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD AUG 10 PY 2015 VL 21 IS 33 BP 11825 EP 11835 DI 10.1002/chem.201501277 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA CO3UE UT WOS:000359084700028 PM 26140330 ER PT J AU Gilbert, JA Kariuki, NN Wang, XP Kropf, AJ Yu, K Groom, DJ Ferreira, PJ Morgan, D Myers, DJ AF Gilbert, James A. Kariuki, Nancy N. Wang, Xiaoping Kropf, A. Jeremy Yu, Kang Groom, Daniel J. Ferreira, Paulo J. Morgan, Dane Myers, Deborah J. TI Pt Catalyst Degradation in Aqueous and Fuel Cell Environments studied via In-Operando Anomalous Small-Angle X-ray Scattering SO ELECTROCHIMICA ACTA LA English DT Article DE Anomalous small-angle X-ray scattering; Catalyst durability; Membrane electrode assembly; Particle size distribution; Platinum Dissolution ID RING-DISK ELECTRODE; CARBON-SUPPORTED ELECTROCATALYSTS; QUARTZ-CRYSTAL MICROBALANCE; HIGH HUMIDITY CONDITIONS; PLATINUM DISSOLUTION; OXYGEN REDUCTION; SULFURIC-ACID; PARTICLE-SIZE; DURABILITY; MEMBRANE AB The evolution of Pt nanoparticle cathode electrocatalyst size distribution in a polymer electrolyte membrane fuel cell (PEMFC) was followed during accelerated stress tests using in-operando anomalous small-angle X-ray scattering (ASAXS). This evolution was compared to that observed in an aqueous electrolyte environment using stagnant electrolyte, flowing electrolyte, and flowing electrolyte at elevated temperature to reveal the different degradation trends in the PEMFC and aqueous environments and to determine the relevance of aqueous measurements to the stability of Pt nanoparticle catalyst in the fuel cell environment. The observed changes in the particle size distributions (PSDs) were analyzed to elucidate the extent and mechanisms of particle growth and corresponding mass and active surface area losses in the different environments. These losses indicate a Pt nanoparticle surface area loss mechanism controlled by Pt dissolution, the particle size dependence of Pt dissolution, the loss of dissolved Pt into the membrane and electrolyte, and, to a lesser extent, the re-deposition of dissolved Pt onto larger particles. Based on the geometric surface area loss, mass loss, and mean particle size increase trends, the aqueous environment best reflecting the fuel cell environment was found to be one in which the electrolyte is flowing rather than stagnant. Pt nanoparticle surface area loss resulting from potential cycling can be inhibited by reducing the number of particles smaller than a critical particle diameter (CPD), which was found to be similar to 3.5 to similar to 4 nm, with the CPD dependent on both the cycling protocol (square wave vs triangle wave) and the catalyst environment (fuel cell, aqueous stagnant, aqueous flowing electrolyte, or elevated temperature flowing electrolyte) (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gilbert, James A.; Morgan, Dane] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Kariuki, Nancy N.; Wang, Xiaoping; Kropf, A. Jeremy; Myers, Deborah J.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Yu, Kang; Groom, Daniel J.; Ferreira, Paulo J.] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. RP Gilbert, JA (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. FU Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX The authors would like to thank Sarah Ball, Jonathan Sharman, Brian Theobald, and Graham Hards from Johnson Matthey Technology Centre for the catalyst and catalyst-coated membrane fabrication and for their supportive discussions. We would also like to thank the staff of Sector 12 at Advanced Photon Source, especially Soenke Seifert and Sungsik Lee for their knowledge and assistance during the ASAXS experiments. We would also like to thank Jan Ilavsky for his expertise and many helpful discussions regarding the ASAXS data analysis. Electron microscopy was performed at University of Texas-Austin. We would like to thank Andres Godoy for his help with the TEM sample preparation. Finally, we thank the Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program (Nancy Garland, DOE Program Manager), for funding this work, and the U.S. Department of Energy, Office of Basic Energy Sciences for support of the Advanced Photon Source. Argonne is a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 56 TC 8 Z9 8 U1 12 U2 55 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD AUG 10 PY 2015 VL 173 BP 223 EP 234 DI 10.1016/j.electacta.2015.05.032 PG 12 WC Electrochemistry SC Electrochemistry GA CL1AP UT WOS:000356674900029 ER PT J AU Keravec, M Mounier, J Prestat, E Vallet, S Jansson, JK Burgaud, G Rosec, S Gouriou, S Rault, G Coton, E Barbier, G Hery-Arnaud, G AF Keravec, Marlene Mounier, Jerome Prestat, Emmanuel Vallet, Sophie Jansson, Janet K. Burgaud, Gaetan Rosec, Sylvain Gouriou, Stephanie Rault, Gilles Coton, Emmanuel Barbier, Georges Hery-Arnaud, Genevieve TI Insights into the respiratory tract microbiota of patients with cystic fibrosis during early Pseudomonas aeruginosa colonization SO SPRINGERPLUS LA English DT Article DE Cystic fibrosis; Respiratory tract microbiota; Pseudomonas aeruginosa; Early colonization; Anaerobes; Respiratory viruses ID AIRWAY MICROBIOTA; COMMUNITIES; INFECTION; CHILDREN; VIRUSES; DISEASE; LUNG AB Pseudomonas aeruginosa plays a major role in cystic fibrosis (CF) progression. Therefore, it is important to understand the initial steps of P. aeruginosa infection. The structure and dynamics of CF respiratory tract microbial communities during the early stages of P. aeruginosa colonization were characterized by pyrosequencing and cloning-sequencing. The respiratory microbiota showed high diversity, related to the young age of the CF cohort (mean age 10 years). Wide inter- and intra-individual variations were revealed. A common core microbiota of 5 phyla and 13 predominant genera was found, the majority of which were obligate anaerobes. A few genera were significantly more prevalent in patients never infected by P. aeruginosa. Persistence of an anaerobic core microbiota regardless of P. aeruginosa status suggests a major role of certain anaerobes in the pathophysiology of lung infections in CF. Some genera may be potential biomarkers of pulmonary infection state. C1 [Keravec, Marlene; Mounier, Jerome; Vallet, Sophie; Burgaud, Gaetan; Gouriou, Stephanie; Coton, Emmanuel; Barbier, Georges; Hery-Arnaud, Genevieve] Univ Brest, Fac Med & Sci Sante Brest, Grp Bacteriol Virol, EA 3882,LUBEM, F-29238 Brest 3, France. [Prestat, Emmanuel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Vallet, Sophie; Hery-Arnaud, Genevieve] Univ Hosp Brest, Dept Bacteriol Virol Hyg & Parasitol Mycol, Brest, France. [Jansson, Janet K.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Rosec, Sylvain] Univ Hosp Brest, INSERM, CIC 0502, Brest, France. [Rault, Gilles] CF Ctr, Roscoff, France. RP Hery-Arnaud, G (reprint author), Univ Brest, Fac Med & Sci Sante Brest, Grp Bacteriol Virol, EA 3882,LUBEM, 22 Ave Camille Desmoulins,CS 93837, F-29238 Brest 3, France. EM hery@univ-brest.fr FU French Cystic Fibrosis Association: 'Vaincre la Mucoviscidose' [RC20120600696]; French Ministry of Higher Education and Research (Ministere de l'Enseignement Superieur et de la Recherche: MESR, France) FX This work was supported by a Grant to GHA from the French Cystic Fibrosis Association: 'Vaincre la Mucoviscidose' (contract no. RC20120600696) and the French Ministry of Higher Education and Research (Ministere de l'Enseignement Superieur et de la Recherche: MESR, France). The Association had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. Written informed consent was obtained from the CF patients or their relatives for publication of this manuscript and accompanying images. The authors are very grateful to the patients involved in this study. NR 36 TC 5 Z9 6 U1 1 U2 10 PU SPRINGER INTERNATIONAL PUBLISHING AG PI CHAM PA GEWERBESTRASSE 11, CHAM, CH-6330, SWITZERLAND SN 2193-1801 J9 SPRINGERPLUS JI SpringerPlus PD AUG 9 PY 2015 VL 4 AR 405 DI 10.1186/s40064-015-1207-0 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO8QX UT WOS:000359436400001 PM 26266076 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bigliettia, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R 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Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for heavy long-lived multi-charged particles in pp collisions at root s=8 TeV using the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID MATTER; MODEL AB Asearch for heavy long-lived multi-charged particles is performed using the ATLAS detector at the LHC. Data collected in 2012 at root s = 8TeV from pp collisions corresponding to an integrated luminosity of 20.3 fb(-1) are examined. Particles producing anomalously high ionisation, consistent with long-livedmassive particleswith electric charges from vertical bar q vertical bar = 2e to vertical bar q vertical bar = 6e are searched for. No signal candidate events are observed, and 95% confidence level crosssection upper limits are interpreted as lower mass limits for a Drell-Yan production model. The mass limits range between 660 and 785 GeV. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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[Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiua, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Gonzalez, B. Alvarez; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. 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Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Richter-Was, E.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; GSsling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Jin, S.; Kiss, F.; Kueneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Genoa, Sect Phys, Genoa, Italy. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Clear Water Bay, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Glonti, G. L.; Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Sansoni, A.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, A.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, A.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Cheng, H. C.; Diehl, E. B.; Feng, H.; Ferretti, C.; Levin, D.; McCarn, A.; Neal, H. A.; Qian, J.; Searcy, J.; Wilson, A.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Doria, A.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Cervelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Mincer, A. I.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Bassalat, A.; Becot, C.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. F.; Hariri, F.; Hrivnac, J.; Iconomidou-Fayard, L.; Ideal, E.; Li, Y.; Lounis, A.; Nellist, C.; Poggioli, L.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Zerwas, D.] Univ Paris 11, LAL, Orsay, France. [Bassalat, A.; Becot, C.; Bourdarios, C.; Delgove, D.; Fournier, D.; Gkougkousis, E. L.; Hariri, F.; Ideal, E.; Li, Y.; Lounis, A.; Nellist, C.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Zerwas, D.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Shimojima, M.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, Kurchatov Inst BP Konstantinov, Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Aloisio, A.; Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedisa, D.; De Salvoa, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzanoa, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Bigliettia, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimic, M.; Goujdamic, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Mourslie, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Recherches Lois Fondamentles Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamiltona, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamityc, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul, Inst Natl Phys Nucl & Phys Particules IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Bawa, H. S.; Bobrovnikov, V. S.; Bortolotto, V.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Prokofiev, K.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Victoria, BC, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Univ Adelaide, Dept Phys, Adelaide, SA, Australia. RI Boldyrev, Alexey/M-9684-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Negrini, Matteo/C-8906-2014; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Gorelov, Igor/J-9010-2015; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Garcia, Jose /H-6339-2015; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014 OI Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Negrini, Matteo/0000-0003-0101-6963; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Gorelov, Igor/0000-0001-5570-0133; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; MOST; NSFC, China; COLCIEN-CIAS, Colombia; MSMT CR; MPO CR; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; NSRF; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT; NSRF, Greece; RGC, Hong Kong SAR, China; ISF; MINERVA; GIF; I-CORE; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, Netherlands; BRF; RCN, Norway; MNiSW; NCN, Poland; GRICES; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC; NSC, Taiwan; SER; TAEK, Turkey; STFC; Royal Society and Leverhulme Trust, United Kingdom; DOE; NSF, United States of America; ERC; European Union; Benoziyo Center, Israel; Wallenberg Foundation, Sweden; SNSF; Canton of Bern, Switzerland; Canton of Geneva, Switzerland FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIEN-CIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFNCNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 29 TC 2 Z9 2 U1 11 U2 58 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 8 PY 2015 VL 75 IS 8 AR 362 DI 10.1140/epjc/s10052-015-3534-2 PG 23 WC Physics, Particles & Fields SC Physics GA CS2OA UT WOS:000361909400004 ER PT J AU Airapetian, A Akopov, N Akopov, Z Aschenauer, EC Augustyniak, W Avakian, R Avetissian, A Avetisyan, E Belostotski, S Bianchi, N Blok, HP Borissov, A Bryzgalov, V Burns, J Capiluppi, M Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Sanctis, E Diefenthaler, M Di Nezza, P Duren, M Elbakian, G Ellinghaus, F Etzelmuller, E Fabbri, R Fantoni, A Felawka, L Frullani, S Gapienko, G Gapienko, V Garcia, JG Garibaldi, F Gavrilov, G Gharibyan, V Giordano, F Gliske, S Hartig, M Hasch, D Holler, Y Hristova, I Imazu, Y Ivanilov, A Jackson, HE Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Korotkov, V Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lapikas, L Lehmann, I Lenisa, P Ruiz, AL Lorenzon, W Lu, XG Ma, BQ Mahon, D Makins, NCR Mao, Y Marianski, B de la Ossa, AM Marukyan, H Miyachi, Y Movsisyan, A Murray, M Mussgiller, A Nappi, E Naryshkin, Y Nass, A Negodaev, M Nowak, WD Pappalardo, LL Perez-Benito, R Petrosyan, A Reimer, PE Reolon, AR Riedl, C Rith, K Rosner, G Rostomyan, A Rubin, J Ryckbosch, D Salomatin, Y Schafer, A Schnell, G Seitz, B Shibata, TA Shutov, V Stahl, M Stancari, M Statera, M Steijger, JJM Taroian, S Terkulov, A Truty, R Trzcinski, A Tytgat, M Van Haarlem, Y Van Hulse, C Veretennikov, D Vikhrov, V Vilardi, I Wang, S Yaschenko, S Ye, Z Yen, S Zihlmann, B Zupranski, P AF Airapetian, A. Akopov, N. Akopov, Z. Aschenauer, E. C. Augustyniak, W. Avakian, R. Avetissian, A. Avetisyan, E. Belostotski, S. Bianchi, N. Blok, H. P. Borissov, A. Bryzgalov, V. Burns, J. Capiluppi, M. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Sanctis, E. Diefenthaler, M. Di Nezza, P. Dueren, M. Elbakian, G. Ellinghaus, F. Etzelmueller, E. Fabbri, R. Fantoni, A. Felawka, L. Frullani, S. Gapienko, G. Gapienko, V. Garay Garcia, J. Garibaldi, F. Gavrilov, G. Gharibyan, V. Giordano, F. Gliske, S. Hartig, M. Hasch, D. Holler, Y. Hristova, I. Imazu, Y. Ivanilov, A. Jackson, H. E. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Korotkov, V. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lapikas, L. Lehmann, I. Lenisa, P. Ruiz, A. Lopez Lorenzon, W. Lu, X. -G. Ma, B. -Q. Mahon, D. Makins, N. C. R. Mao, Y. Marianski, B. de la Ossa, A. Martinez Marukyan, H. Miyachi, Y. Movsisyan, A. Murray, M. Mussgiller, A. Nappi, E. Naryshkin, Y. Nass, A. Negodaev, M. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Petrosyan, A. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rosner, G. Rostomyan, A. Rubin, J. Ryckbosch, D. Salomatin, Y. Schaefer, A. Schnell, G. Seitz, B. Shibata, T. -A. Shutov, V. Stahl, M. Stancari, M. Statera, M. Steijger, J. J. M. Taroian, S. Terkulov, A. Truty, R. Trzcinski, A. Tytgat, M. Van Haarlem, Y. Van Hulse, C. Veretennikov, D. Vikhrov, V. Vilardi, I. Wang, S. Yaschenko, S. Ye, Z. Yen, S. Zihlmann, B. Zupranski, P. TI Bose-Einstein correlations in hadron-pairs from lepto-production on nuclei ranging from hydrogen to xenon SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DEEP-INELASTIC SCATTERING; IDENTICAL PARTICLES; MULTIPLE PRODUCTION; INTERFERENCE; ANNIHILATION; NEUTRINO; INTERFEROMETRY; FRAGMENTATION; HADRONIZATION; ENVIRONMENT AB Bose-Einstein correlations of like-sign charged hadrons produced in deep-inelastic electron and positron scattering are studied in the HERMES experiment using nuclear targets of H-1, H-2, He-3, He-4, N, Ne, Kr, and Xe. A Gaussian approach is used to parametrize a two-particle correlation function determined from events with at least two charged hadrons of the same sign charge. This correlation function is compared to two different empirical distributions that do not include the Bose-Einstein correlations. One distribution is derived from unlike-sign hadron pairs, and the second is derived from mixing like-sign pairs from different events. The extraction procedure used simulations incorporating the experimental setup in order to correct the results for spectrometer acceptance effects, and was tested using the distribution of unlike-sign hadron pairs. Clear signals of Bose-Einstein correlations for all target nuclei without a significant variation with the nuclear target mass are found. Also, no evidence for a dependence on the invariant mass W of the photon-nucleon system is found when the results are compared to those of previous experiments. C1 [Jackson, H. E.; Reimer, P. E.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Nappi, E.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Garay Garcia, J.; Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. [Schnell, G.] Ikerbasque, Basque Fdn Sci, Bilbao 48013, Spain. [Ellinghaus, F.; Kinney, E.] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Akopov, Z.; Avetisyan, E.; Borissov, A.; Deconinck, W.; Garay Garcia, J.; Gavrilov, G.; Hartig, M.; Holler, Y.; Lu, X. -G.; de la Ossa, A. Martinez; Mussgiller, A.; Rostomyan, A.; Yaschenko, S.; Ye, Z.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Aschenauer, E. C.; Fabbri, R.; Hristova, I.; Negodaev, M.; Nowak, W. -D.; Riedl, C.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.; Shutov, V.] Joint Inst Nucl Res, Dubna 141980, Russia. [Diefenthaler, M.; Kravchenko, P.; Mussgiller, A.; Nass, A.; Rith, K.; Yaschenko, S.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Ist Nazl Fis Nucl, Sez Ferrara, I-44122 Ferrara, Italy. [Capiluppi, M.; Ciullo, G.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Dipartimento Fis Sci & Terra, I-44122 Ferrara, Italy. [Bianchi, N.; Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Fantoni, A.; Hasch, D.; Reolon, A. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Joosten, S.; Ruiz, A. Lopez; Ryckbosch, D.; Schnell, G.; Tytgat, M.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Airapetian, A.; Dueren, M.; Etzelmueller, E.; Keri, T.; Perez-Benito, R.; Stahl, M.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Burns, J.; Kaiser, R.; Lehmann, I.; Mahon, D.; Murray, M.; Rosner, G.; Seitz, B.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Diefenthaler, M.; Giordano, F.; Makins, N. C. R.; Riedl, C.; Rubin, J.; Truty, R.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Airapetian, A.; Gliske, S.; Lorenzon, W.; Rubin, J.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.; Terkulov, A.] Lebedev Phys Inst, Moscow 117924, Russia. [Blok, H. P.; Lapikas, L.; Steijger, J. J. M.] Natl Inst Subat Phys Nikhef, NL-1009 DB Amsterdam, Netherlands. [Belostotski, S.; Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Naryshkin, Y.; Veretennikov, D.; Vikhrov, V.] BP Konstantinov Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Bryzgalov, V.; Gapienko, G.; Gapienko, V.; Ivanilov, A.; Korotkov, V.; Salomatin, Y.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Nazl Fis Nucl, Grp Collegato Sanita, Sez Roma, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Super Sanita, I-00161 Rome, Italy. [Felawka, L.; Gavrilov, G.; Yen, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Imazu, Y.; Miyachi, Y.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Natl Ctr Nucl Res, PL-00689 Warsaw, Poland. [Akopov, N.; Avakian, R.; Avetissian, A.; Elbakian, G.; Gharibyan, V.; Karyan, G.; Marukyan, H.; Petrosyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Airapetian, A (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM gunar.schnell@desy.de RI Terkulov, Adel/M-8581-2015; Cisbani, Evaristo/C-9249-2011; Kozlov, Valentin/M-8000-2015; Negodaev, Mikhail/A-7026-2014 OI Cisbani, Evaristo/0000-0002-6774-8473; FU Ministry of Education and Science of Armenia; FWO-Flanders; IWT, Belgium; Natural Sciences and Engineering Research Council of Canada; National Natural Science Foundation of China; Alexander von Humboldt Stiftung; German Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Italian Istituto Nazionale di Fisica Nucleare (INFN); MEXT; JSPS; G-COE of Japan; Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); Russian Academy of Science; Russian Federal Agency for Science and Innovations; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; U.K. Engineering and Physical Sciences Research Council; Science and Technology Facilities Council; Scottish Universities Physics Alliance; U.S. Department of Energy (DOE); National Science Foundation (NSF); DESY management FX We gratefully acknowledge the DESY management for its support and the staff at DESY and the collaborating institutions for their significant effort. This work was supported by the Ministry of Education and Science of Armenia; the FWO-Flanders and IWT, Belgium; the Natural Sciences and Engineering Research Council of Canada; the National Natural Science Foundation of China; the Alexander von Humboldt Stiftung, the German Bundesministerium fur Bildung und Forschung (BMBF), and the Deutsche Forschungsgemeinschaft (DFG); the Italian Istituto Nazionale di Fisica Nucleare (INFN); the MEXT, JSPS, and G-COE of Japan; the Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); the Russian Academy of Science and the Russian Federal Agency for Science and Innovations; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the U.K. Engineering and Physical Sciences Research Council, the Science and Technology Facilities Council, and the Scottish Universities Physics Alliance; as well as the U.S. Department of Energy (DOE) and the National Science Foundation (NSF). NR 38 TC 0 Z9 0 U1 1 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 8 PY 2015 VL 75 IS 8 AR 361 DI 10.1140/epjc/s10052-015-3566-7 PG 9 WC Physics, Particles & Fields SC Physics GA CS2OA UT WOS:000361909400003 ER PT J AU Bjorgaard, JA Velizhanin, KA Tretiak, S AF Bjorgaard, J. A. Velizhanin, K. A. Tretiak, S. TI Solvent effects in time-dependent self-consistent field methods. II. Variational formulations and analytical gradients SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; POLARIZABLE CONTINUUM MODEL; STATE MOLECULAR-DYNAMICS; RANDOM-PHASE-APPROXIMATION; RESTRICTED HARTREE-FOCK; COUPLED-CLUSTER THEORY; CHARGE-TRANSFER STATES; EXCITED-STATES; EXCITATION-ENERGIES; ELECTRONIC EXCITATIONS AB This study describes variational energy expressions and analytical excited state energy gradients for time-dependent self-consistent field methods with polarizable solvent effects. Linear response, vertical excitation, and state-specific solvent models are examined. Enforcing a variational ground state energy expression in the state-specific model is found to reduce it to the vertical excitation model. Variational excited state energy expressions are then provided for the linear response and vertical excitation models and analytical gradients are formulated. Using semiempirical model chemistry, the variational expressions are verified by numerical and analytical differentiation with respect to a static external electric field. Analytical gradients are further tested by performing microcanonical excited state molecular dynamics with p-nitroaniline. (C) 2015 AIP Publishing LLC. C1 [Bjorgaard, J. A.] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Velizhanin, K. A.; Tretiak, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Tretiak, S.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Bjorgaard, JA (reprint author), Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. EM jbjorgaard@lanl.gov; serg@lanl.gov RI Velizhanin, Kirill/C-4835-2008; Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Bjorgaard, Josiah/0000-0003-3679-2487 FU U.S. Department of Energy through Los Alamos National Laboratory (LANL) LDRD Program; U.S. Department of Energy [DE-AC52-06NA25396]; Center for Nonlinear Studies (CNLS); Center for Integrated Nanotechnology (CINT) at LANL FX We thank Giovanni Scalmani, Ivan Cristov, and Anders Niklasson for insightful conversations. We acknowledge support of the U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We also acknowledge support of the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnology (CINT) at LANL. NR 87 TC 2 Z9 2 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 7 PY 2015 VL 143 IS 5 AR 054305 DI 10.1063/1.4927167 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO7XP UT WOS:000359377200020 PM 26254651 ER PT J AU Xu, SY Belopolski, I Alidoust, N Neupane, M Bian, G Zhang, CL Sankar, R Chang, GQ Yuan, ZJ Lee, CC Huang, SM Zheng, H Ma, J Sanchez, DS Wang, BK Bansil, A Chou, FC Shibayev, PP Lin, H Jia, S Hasan, MZ AF Xu, Su-Yang Belopolski, Ilya Alidoust, Nasser Neupane, Madhab Bian, Guang Zhang, Chenglong Sankar, Raman Chang, Guoqing Yuan, Zhujun Lee, Chi-Cheng Huang, Shin-Ming Zheng, Hao Ma, Jie Sanchez, Daniel S. Wang, BaoKai Bansil, Arun Chou, Fangcheng Shibayev, Pavel P. Lin, Hsin Jia, Shuang Hasan, M. Zahid TI Discovery of a Weyl fermion semimetal and topological Fermi arcs SO SCIENCE LA English DT Article ID DIRAC SEMIMETALS; PHASE-TRANSITION; METAL; INSULATORS; ARSENIDES; TANTALUM AB A Weyl semimetal is a new state of matter that hosts Weyl fermions as emergent quasiparticles and admits a topological classification that protects Fermi arc surface states on the boundary of a bulk sample. This unusual electronic structure has deep analogies with particle physics and leads to unique topological properties. We report the experimental discovery of a Weyl semimetal, tantalum arsenide (TaAs). Using photoemission spectroscopy, we directly observe Fermi arcs on the surface, as well as the Weyl fermion cones and Weyl nodes in the bulk of TaAs single crystals. We find that Fermi arcs terminate on the Weyl fermion nodes, consistent with their topological character. Our work opens the field for the experimental study of Weyl fermions in physics and materials science. C1 [Xu, Su-Yang; Belopolski, Ilya; Alidoust, Nasser; Neupane, Madhab; Bian, Guang; Zheng, Hao; Sanchez, Daniel S.; Shibayev, Pavel P.; Hasan, M. Zahid] Princeton Univ, Dept Phys, Lab Topol Quantum Matter & Spect B7, Princeton, NJ 08544 USA. [Xu, Su-Yang; Alidoust, Nasser; Hasan, M. Zahid] Princeton Univ, Princeton Inst Sci & Technol Mat, Princeton Ctr Complex Mat, Princeton, NJ 08544 USA. [Neupane, Madhab] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. [Zhang, Chenglong; Yuan, Zhujun; Jia, Shuang] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing, Peoples R China. [Sankar, Raman; Chou, Fangcheng] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Chang, Guoqing; Lee, Chi-Cheng; Huang, Shin-Ming; Wang, BaoKai; Lin, Hsin] Natl Univ Singapore, Ctr Adv Mat 2D, Singapore 117546, Singapore. [Chang, Guoqing; Lee, Chi-Cheng; Huang, Shin-Ming; Wang, BaoKai; Lin, Hsin] Natl Univ Singapore, Graphene Res Ctr, Singapore 117546, Singapore. [Chang, Guoqing; Lee, Chi-Cheng; Huang, Shin-Ming; Wang, BaoKai; Lin, Hsin] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore. [Ma, Jie] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Wang, BaoKai; Bansil, Arun] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Shibayev, Pavel P.] Princeton Univ, Princeton Inst Sci & Technol Mat, Princeton, NJ 08544 USA. [Jia, Shuang] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. RP Hasan, MZ (reprint author), Princeton Univ, Dept Phys, Lab Topol Quantum Matter & Spect B7, Princeton, NJ 08544 USA. EM mzhasan@princeton.edu RI Ma, Jie/C-1637-2013; zheng, hao/H-8636-2015; Bian, Guang/C-5182-2016; Lin, Hsin/F-9568-2012; OI zheng, hao/0000-0002-6495-874X; Bian, Guang/0000-0001-7055-2319; Lin, Hsin/0000-0002-4688-2315; chang, guoqing/0000-0003-1180-3127 FU Gordon and Betty Moore Foundations EPiQS Initiative [GBMF4547]; National Research Foundation, Prime Minister's Office, Singapore [NRF-NRFF2013-03]; National Basic Research Program of China [2013CB921901, 2014CB239302]; U.S. Department of Energy [DE-FG-02-05ER46200]; MOST-Taiwan [102-2119-M-002-004] FX Work at Princeton University and Princeton-led synchrotron-based ARPES measurements were supported by the Gordon and Betty Moore Foundations EPiQS Initiative through grant GBMF4547 (Hasan). First-principles band structure calculations at National University of Singapore were supported by the National Research Foundation, Prime Minister's Office, Singapore, under its NRF fellowship (NRF Award no. NRF-NRFF2013-03). Single-crystal growth was supported by National Basic Research Program of China (grant nos. 2013CB921901 and 2014CB239302) and characterization by U.S. Department of Energy DE-FG-02-05ER46200. F.C. acknowledges the support provided by MOST-Taiwan under project no. 102-2119-M-002-004. We gratefully acknowledge J. D. Denlinger, S. K. Mo, A. V. Fedorov, M. Hashimoto, M. Hoesch, T. Kim, and V. N. Strocov for their beamline assistance at the Advanced Light Source, the Stanford Synchrotron Radiation Lightsource, the Diamond Light Source, and the Swiss Light Source under their external user programs. Part of the work was carried out at the Swiss Light Source through the external/international facility user program. We thank T.-R. Chang for help on theoretical band structure calculations. We also thank L. Balents, D. Huse, I. Klebanov, T. Neupert, A. Polyakov, P. Steinhardt, H. Verlinde, and A. Vishwanath for discussions. R. S. and H. L. acknowledge visiting scientist support from Princeton University. M. Z. H. acknowledges hospitality of the Lawrence Berkeley National Laboratory and Aspen Center for Physics as a visiting scientist. A patent application is being prepared on behalf of the authors on the discovery of a Weyl semimetal. NR 29 TC 414 Z9 416 U1 97 U2 334 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 7 PY 2015 VL 349 IS 6248 BP 613 EP 617 DI 10.1126/science.aaa9297 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO3WW UT WOS:000359092900034 PM 26184916 ER PT J AU Gumbs, G Iurov, A Huang, DH Pan, W AF Gumbs, Godfrey Iurov, Andrii Huang, Danhong Pan, Wei TI Tunable surface plasmon instability leading to emission of radiation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INFRARED TRANSMISSION SPECTRA; LATERALLY CONFINED 2D-PLASMA; SILICON INVERSION LAYERS; QUANTUM-CASCADE LASERS; 2-DIMENSIONAL PLASMA; INTERCALATED GRAPHITE; DIELECTRIC FUNCTION; GRAPHENE; SYSTEMS; WIRES AB We propose a new approach for energy conversion from a dc electric field to tunable terahertz emission based on hybrid semiconductors by combining two-dimensional (2D) crystalline layers and a thick conducting material with possible applications for chemical analysis, security scanning, medical (single-molecule) imaging, and telecommunications. The hybrid nano-structure may consist of a single or pair of sheets of graphene, sificene, or a 2D electron gas. When an electric current is passed through a 2D layer, we discover that two low-energy plasmon branches exhibit a characteristic loop in their dispersion before they merge into an unstable region beyond a critical wave vector q(c). This finite q(c) gives rise to a wavenumber cutoff in the emission dispersion of the surface plasmon induced instability and emission of radiation (spiler). However, there is no instability for a single driven layer far from the conductor, and the instability of an isolated pair of 2D layers occurs without a wavenumber cutoff. The wavenumber cutoff is found to depend on the conductor electron density, layer separation, distances of layers from the conductor surface, and the driving-current strength. (C) 2015 AIP Publishing LLC, C1 [Gumbs, Godfrey; Iurov, Andrii] CUNY Hunter Coll, Dept Phys & Astron, 695 Pk Ave, New York, NY 10065 USA. [Gumbs, Godfrey] Donostia Int Phys Ctr, San Sebastian 20018, Basque Country, Spain. [Iurov, Andrii] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87106 USA. [Huang, Danhong] US Air Force, Res Lab, Space Vehicles Directorate, Kirtland AFB, NM 87117 USA. [Pan, Wei] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Iurov, A (reprint author), CUNY Hunter Coll, Dept Phys & Astron, 695 Pk Ave, New York, NY 10065 USA. EM aiurov@chtm.unm.edu RI DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014 FU AFRL [FA 9453-13-1-0291]; Air Force Office of Scientific Research (AFOSR); U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This research was supported by Contract No. FA 9453-13-1-0291 of AFRL. D.H. thank the Air Force Office of Scientific Research (AFOSR) for its support. W.P. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. We thank Oleksiy Roslyak and Antonios Balassis for helpful discussions. NR 53 TC 7 Z9 7 U1 4 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 7 PY 2015 VL 118 IS 5 AR 054303 DI 10.1063/1.4927101 PG 10 WC Physics, Applied SC Physics GA CO7XK UT WOS:000359376700027 ER PT J AU Ishchuk, V Olynick, DL Liu, ZW Rangelow, IW AF Ishchuk, Valentyn Olynick, Deirdre L. Liu, Zuwei Rangelow, Ivo W. TI Profile simulation model for sub-50nm cryogenic etching of silicon using SF6/O-2 inductively coupled plasma SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FEATURE-SCALE-MODEL; HIGH-DENSITY PLASMA; ASPECT-RATIO FEATURES; ANGULAR-DEPENDENCE; PASSIVATION LAYER; SURFACE KINETICS; ION ENERGY; SI; TRENCHES; MIXTURES AB Cryogenic etching of silicon is a route to high aspect ratio silicon features with high mask selectivity and smooth sidewalls. These benefits have been realized even down to 10 nm half-pitch features. In this work, we develop a semi-empirical simulation model to understand mechanisms responsible for nanoscale profile evolution during plasma etching of silicon in SF6/O-2 chemistry at cryogenic temperatures. The model parameters are first calibrated to the etching equipment using features from 500 nm to 2 mu m. Using the calibrated model, we show the experimental finding that smaller features need more oxygen to achieve vertical anisotropic profiles. This is a consequence of two related effects: (1) the SiOxFy passivation layer sputtering yield is strongly dependent on the oxygen content at the feature sidewalls and (2) Knudsen transport within small features or higher aspect ratios depletes oxygen faster than fluorine due to the higher sticking coefficient of oxygen. The simulation was applied to 25 nm half-pitch features with excellent results. (C) 2015 AIP Publishing LLC. C1 [Ishchuk, Valentyn; Rangelow, Ivo W.] Tech Univ Ilmenau, Fac Elect Engn & Informat Technol, Inst Micro & Nanoelect, Dept Micro & Nanoelect Syst, D-98693 Ilmenau, Germany. [Ishchuk, Valentyn; Olynick, Deirdre L.; Liu, Zuwei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Liu, Zuwei] Oxford Instruments, Concord, MA 01742 USA. RP Ishchuk, V (reprint author), Tech Univ Ilmenau, Fac Elect Engn & Informat Technol, Inst Micro & Nanoelect, Dept Micro & Nanoelect Syst, Gustav Kirchhoff Str 1, D-98693 Ilmenau, Germany. EM dlolynick@lbl.gov; ivo.rangelow@tu-ilmenau.de OI Ishchuk, Valentyn/0000-0002-8834-7089 FU European Unions [318804]; Oxford Instruments; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work has received funding from the European Unions Seventh Framework Programme for research, technological development; and demonstration under Grant Agreement No. 318804 ("Single Nanometer Manufacturing for beyond CMOS devices"-acronym SNM). Experimental work was conducted at the Molecular Foundry at Lawrence Berkeley National Laboratory and supported by Oxford Instruments (Z.L.) and the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (D.O. and experimental work by V.I.). V.I. wishes to thank B. E. Volland and M. Hauguth for fruitful discussions and contribution to the software development. NR 55 TC 2 Z9 2 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 7 PY 2015 VL 118 IS 5 AR 053302 DI 10.1063/1.4927731 PG 13 WC Physics, Applied SC Physics GA CO7XK UT WOS:000359376700004 ER PT J AU Willey, TM Lauderbach, L Gagliardi, F van Buuren, T Glascoe, EA Tringe, JW Lee, JRI Springer, HK Ilavsky, J AF Willey, Trevor M. Lauderbach, Lisa Gagliardi, Franco van Buuren, Tony Glascoe, Elizabeth A. Tringe, Joseph W. Lee, Jonathan R. I. Springer, H. Keo Ilavsky, Jan TI Mesoscale evolution of voids and microstructural changes in HMX-based explosives during heating through the beta-delta phase transition SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PLASTIC BONDED EXPLOSIVES; ELEVATED-TEMPERATURES; DAMAGED PBX-9501; DECOMPOSITION; SIMULATIONS; SCATTERING; SURFACES AB HMX-based explosives LX-10 and PBX-9501 were heated through the beta-delta phase transition. Ultra-small angle x-ray scattering (USAXS) and molecular diffraction were simultaneously recorded as the HMX was heated. Mesoscale voids and structure dramatically change promptly with the beta-delta phase transition, rather than with other thermal effects. Also, x-ray induced damage, observed in the USAXS, occurs more readily at elevated temperatures; as such, the dose was reduced to mitigate this effect. Optical microscopy performed during a similar heating cycle gives an indication of changes on longer length scales, while x-ray microtomography, performed before and after heating, shows the character of extensive microstructural damage resulting from the temperature cycle and solid-state phase transition. (C) 2015 AIP Publishing LLC. C1 [Willey, Trevor M.; Lauderbach, Lisa; Gagliardi, Franco; van Buuren, Tony; Glascoe, Elizabeth A.; Tringe, Joseph W.; Lee, Jonathan R. I.; Springer, H. Keo] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Ilavsky, Jan] Argonne Natl Lab, Argonne, IL 60439 USA. RP Willey, TM (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM willey1@llnl.gov RI Ilavsky, Jan/D-4521-2013; Willey, Trevor/A-8778-2011 OI Ilavsky, Jan/0000-0003-1982-8900; Willey, Trevor/0000-0002-9667-8830 FU Joint DoD-DOE Munitions Technology Development Program; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Science Foundation/Department of Energy [NSF/CHE-1346572]; U.S. DOE [DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank I. Tran, C. Divin, and C. Tarver of LLNL, and D. Parkinson, ALS, LBNL. This research was partially supported by the Joint DoD-DOE Munitions Technology Development Program. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No, DE-AC52-07NA27344, ChemMatCARS Sector 15 is supported by the National Science Foundation/Department of Energy under grant number NSF/CHE-1346572. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No, DE-AC02-06CH11357. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. A condensed subset of the data presented herein and a preliminary analysis of this data appeared in the Proceedings of the International Detonation Symposium.31 NR 30 TC 4 Z9 4 U1 3 U2 38 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 7 PY 2015 VL 118 IS 5 AR 055901 DI 10.1063/1.4927614 PG 6 WC Physics, Applied SC Physics GA CO7XK UT WOS:000359376700047 ER PT J AU Norman, MR AF Norman, M. R. TI Dichroism as a probe for parity-breaking phases of spin-orbit coupled metals SO PHYSICAL REVIEW B LA English DT Article ID CD2RE2O7; CRYSTALS; ORDER AB Recently, a general formalism was presented for gyrotropic, ferroelectric, and multipolar order in spin-orbit coupled metals induced by spin-spin interactions. Here, I point out that the resulting order parameters are equivalent to expectation values of operators that determine natural circular dichroic signals in optical and x-ray absorption. Some general properties of these operator equivalents and the resulting dichroisms are mentioned, and I list several material examples in this connection, including Weyl semimetals. The particular case of the tensor order in the pyrochlore superconductor Cd2Re2O7 is treated in more detail, including calculations of the x-ray absorption and circular dichroism at the O K edge. C1 Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Norman, MR (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Norman, Michael/C-3644-2013 FU Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, U.S. DOE FX The author thanks L. Fu and S. Di Matteo for several helpful discussions. This work was supported by the Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, U.S. DOE. NR 43 TC 1 Z9 1 U1 1 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 7 PY 2015 VL 92 IS 7 AR 075113 DI 10.1103/PhysRevB.92.075113 PG 4 WC Physics, Condensed Matter SC Physics GA CO4FN UT WOS:000359116500003 ER PT J AU Perren, G Moller, JS Huvonen, D Podlesnyak, AA Zheludev, A AF Perren, G. Moeller, J. S. Huevonen, D. Podlesnyak, A. A. Zheludev, A. TI Spin dynamics in pressure-induced magnetically ordered phases in (C4H12N2)Cu2Cl6 SO PHYSICAL REVIEW B LA English DT Article ID SYSTEM TLCUCL3; QUANTUM; CRITICALITY AB We present inelastic neutron-scattering experiments on the S = 1/2 frustrated gapped quantum magnet piperazinium hexachlorodicuprate (PHCC) under applied hydrostatic pressure. These results show that at 9 kbar the magnetic triplet excitations in the system are gapless, contrary to what was previously reported. Our results are in agreement with recent muon-spin relaxation experiments which found magnetic order above a quantum-critical point at 4.3 kbar. We show that the changes in the excitation spectrum can be primarily attributed to the change in a single exchange pathway. C1 [Perren, G.; Moeller, J. S.; Huevonen, D.; Zheludev, A.] Swiss Fed Inst Technol, Solid State Phys Lab, Neutron Scattering & Magnetism, CH-8093 Zurich, Switzerland. [Huevonen, D.] NICPB, EE-12618 Tallinn, Estonia. [Podlesnyak, A. A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Perren, G (reprint author), Swiss Fed Inst Technol, Solid State Phys Lab, Neutron Scattering & Magnetism, CH-8093 Zurich, Switzerland. EM gperren@phys.ethz.ch; jmoeller@phys.ethz.ch RI Huvonen, Dan/A-6664-2008; Instrument, CNCS/B-4599-2012; Podlesnyak, Andrey/A-5593-2013 OI Huvonen, Dan/0000-0002-8906-6588; Podlesnyak, Andrey/0000-0001-9366-6319 FU Swiss National Fund; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; ETH Fellowship; European Union [246543, 608881]; Estonian Ministry of Education and Research [IUT23-03]; Estonian Research Council [PUT451] FX We thank Georg Ehlers for technical assistance and David Schmidiger for useful discussions. This work is partially supported by the Swiss National Fund. Research at Oak Ridge National Laboratory's Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. J.S.M. gratefully acknowledges support through an ETH Fellowship. This project has received funding from the European Union's Seventh Framework Programme for research, technological development, and demonstration under Grant No. 246543 (2011-2016) and under Grant No. 608881 (2015-2019). D.H. acknowledges support by the Estonian Ministry of Education and Research under Grant No. IUT23-03 and Estonian Research Council Grant No. PUT451. NR 18 TC 4 Z9 4 U1 7 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 7 PY 2015 VL 92 IS 5 AR 054413 DI 10.1103/PhysRevB.92.054413 PG 5 WC Physics, Condensed Matter SC Physics GA CO4FD UT WOS:000359115400001 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Bouchet, J Brandin, AV Bunzarov, I Burton, TP Butterworth, J Caines, H S'anchez, MCD Campbell, JM Cebra, D Cervantes, MC Chakaberia, I Chaloupka, P Chang, Z Chattopadhyay, S Chen, X Chen, JH Cheng, J Cherney, M Christie, W Codrington, MJM Contin, G Crawford, HJ Das, S De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA di Ruzza, B Didenko, L Dilks, C Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Eppley, G Esha, R Evdokimov, O Eyser, O Fatemi, R Fazio, S Federic, P Fedorisin, J Feng Filip, P Fisyak, Y Flores, CE Fulek, L Gagliardi, CA Garand, D Geurts, F Gibson, A Girard, M Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Hamad, A Hamed, A Haque, R Harris, JW He, L Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, HZ Huang, B Huang, X Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Klein, SR Koetke, DD Kollegger, T Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Li, W Li, ZM Li, C Li, Y Li, X Li, X Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, L Ma, R Ma, GL Ma, YG Magdy, N Majka, R Manion, A Margetis, S Markert, C Masui, H Matis, HS McDonald, D Meehan, K Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Okorokov, V Olvitt, DL Page, BS Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peterson, A Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, S Raniwala, R Ray, RL Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, MK Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Sikora, R Simko, M Skoby, MJ Smirnov, D Smirnov, N Solanki, D Song, L Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stock, R Strikhanov, M Stringfellow, B Sumbera, M Summa, BJ Sun, Z Sun, Y Sun, XM Sun, X Surrow, B Svirida, DN Szelezniak, MA Takahashi, J Tang, AH Tang, Z Tarnowsky, T Tawfik, AN Thomas, JH Tian, J Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Tripathy, SK Trzeciak, BA Tsai, OD Ullrich, T Underwood, DG Upsal, I Van Buren, G van Nieuwenhuizen, G Vandenbroucke, M Varma, R Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Voloshin, SA Vossen, A Wang, Y Wang, F Wang, JS Wang, H Wang, G Wang, Y Webb, JC Webb, G Wen, L Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, N Xu, H Xu, YF Xu, QH Xu, Z Yang, Y Yang, S Yang, C Yang, Y Yang, Q Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zbroszczyk, H Zha, W Zhang, J Zhang, Y Zhang, S Zhang, XP Zhang, JB Zhang, JL Zhang, Z Zhao, F Zhao, J Zhong, C Zhu, X Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Bouchet, J. Brandin, A. V. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. S'anchez, M. Calder'on de la Barca Campbell, J. M. Cebra, D. Cervantes, M. C. Chakaberia, I. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, X. Chen, J. H. Cheng, J. Cherney, M. Christie, W. Codrington, M. J. M. Contin, G. Crawford, H. J. Das, S. De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. di Ruzza, B. Didenko, L. Dilks, C. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Eppley, G. Esha, R. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Federic, P. Fedorisin, J. Feng Filip, P. Fisyak, Y. Flores, C. E. Fulek, L. Gagliardi, C. A. Garand, D. Geurts, F. Gibson, A. Girard, M. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Hamad, A. Hamed, A. Haque, R. Harris, J. W. He, L. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, H. Z. Huang, B. Huang, X. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Klein, S. R. Koetke, D. D. Kollegger, T. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Li, W. Li, Z. M. Li, C. Li, Y. Li, X. Li, X. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, L. Ma, R. Ma, G. L. Ma, Y. G. Magdy, N. Majka, R. Manion, A. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. Meehan, K. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Okorokov, V. Olvitt, D. L., Jr. Page, B. S. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peterson, A. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, S. Raniwala, R. Ray, R. L. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, M. K. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Sikora, R. Simko, M. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Song, L. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Summa, B. J. Sun, Z. Sun, Y. Sun, X. M. Sun, X. Surrow, B. Svirida, D. N. Szelezniak, M. A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Tawfik, A. N. Thomas, J. H. Tian, J. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Tripathy, S. K. Trzeciak, B. A. Tsai, O. D. Ullrich, T. Underwood, D. G. Upsal, I. Van Buren, G. van Nieuwenhuizen, G. Vandenbroucke, M. Varma, R. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Vossen, A. Wang, Y. Wang, F. Wang, J. S. Wang, H. Wang, G. Wang, Y. Webb, J. C. Webb, G. Wen, L. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, N. Xu, H. Xu, Y. F. Xu, Q. H. Xu, Z. Yang, Y. Yang, S. Yang, C. Yang, Y. Yang, Q. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I. -K. Yu, N. Zbroszczyk, H. Zha, W. Zhang, J. Zhang, Y. Zhang, S. Zhang, X. P. Zhang, J. B. Zhang, J. L. Zhang, Z. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Energy dependence of K pi, p pi, and Kp fluctuations in Au plus Au collisions from root s(NN)=7.7 to 200 GeV SO PHYSICAL REVIEW C LA English DT Article ID DECONFINEMENT PHASE-TRANSITION; NUCLEUS-NUCLEUS COLLISIONS; BY-EVENT FLUCTUATIONS; STAR EXPERIMENT AB A search for the quantum chromodynamics (QCD) critical point was performed by the STAR experiment at the BNL Relativistic Heavy Ion Collider, using dynamical fluctuations of unlike particle pairs. Heavy ion collisions were studied over a large range of collision energies with homogeneous acceptance and excellent particle identification, covering a significant range in the QCD phase diagram where a critical point may be located. Dynamical K pi, p pi, and Kp fluctuations as measured by the STAR experiment in central 0-5% Au + Au collisions from center-of-mass collision energies root s(NN) = 7.7 to 200 GeV are presented. The observable nu(dyn) was used to quantify the magnitude of the dynamical fluctuations in event-by-event measurements of the Kp, pp, and Kp pairs. The energy dependences of these fluctuations from central 0-5% Au + Au collisions all demonstrate a smooth evolution with collision energy. C1 [Adamczyk, L.; Fulek, L.; Sikora, R.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Arkhipkin, D.; Aschenauer, E. C.; Bland, L. C.; Burton, T. P.; Chakaberia, I.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; Li, X.; Ljubicic, T.; Longacre, R. S.; Ma, R.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Webb, G.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [S'anchez, M. Calder'on de la Barca; Cebra, D.; Draper, J. E.; Flores, C. E.; Meehan, K.; Romero, J. L.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Esha, R.; Huang, H. Z.; Igo, G.; Landry, K. D.; Nasim, Md.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Wen, L.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Takahashi, J.] Univ Estadual Campinas, BR-13131 Sao Paulo, Brazil. [Aparin, A.; Banerjee, A.; Feng; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Sun, X. M.; Wang, Y.; Wu, Y. F.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Huang, B.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Cherney, M.; De Silva, L. C.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Rusnakova, O.; Trzeciak, B. A.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Bielcikova, J.; Federic, P.; Rusnak, J.; Simko, M.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] Frankfurt Inst Adv Studies, D-60438 Frankfurt, Germany. [Das, S.; Sahu, P. K.; Tripathy, S. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.; Sharma, M. K.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Hamad, A.; Kabana, S.; Keane, D.; Lomnitz, M.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Ramachandran, S.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Adv Inst Sci & Technol, Taejon 305701, South Korea. [Chen, X.; Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.; Zhang, J.] Inst Modern Phys, Lanzhou 730000, Peoples R China. [Contin, G.; Dong, X.; Greiner, L.; Klein, S. R.; Manion, A.; Masui, H.; Matis, H. S.; Mustafa, M. K.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Szelezniak, M. A.; Thomas, J. H.; Wieman, H.; Xu, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [van Nieuwenhuizen, G.] MIT, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Nigmatkulov, G.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Mohanty, B.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Campbell, J. M.; Humanic, T. J.; Lisa, M. A.; Peterson, A.; Upsal, I.] Ohio State Univ, Columbus, OH 43210 USA. [Kycia, R. A.; Pawlik, B.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Dilks, C.; Heppelmann, S.; Summa, B. J.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Garand, D.; He, L.; Hirsch, A.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, S.; Raniwala, R.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Yang, S.; Yang, C.; Yang, Q.; Zha, W.; Zhang, Y.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.; Zhang, J. L.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Li, W.; Ma, L.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Tian, J.; Xu, Y. F.; Zhang, S.; Zhang, Z.; Zhong, C.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D. L., Jr.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Hoffmann, G. W.; Markert, C.; Ray, R. L.; Schambach, J.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Song, L.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Roy, A.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pawlak, T.; Pluta, J.; Poniatowska, K.; Sandacz, A.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Llope, W. J.; Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Magdy, N.; Tawfik, A. N.] WLCAPP, Cairo 11571, Egypt. [Caines, H.; Harris, J. W.; Horvat, S.; Majka, R.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Alekseev, Igor/J-8070-2014; Kycia, Radoslaw/J-4397-2015; Svirida, Dmitry/R-4909-2016; Tawfik, Abdel Nasser/M-6220-2013; Fazio, Salvatore /G-5156-2010; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Chaloupka, Petr/E-5965-2012; Takahashi, Jun/B-2946-2012; Huang, Bingchu/H-6343-2015; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017 OI Alekseev, Igor/0000-0003-3358-9635; Kycia, Radoslaw/0000-0002-6390-4627; Tawfik, Abdel Nasser/0000-0002-1679-0225; Sumbera, Michal/0000-0002-0639-7323; Takahashi, Jun/0000-0002-4091-1779; Huang, Bingchu/0000-0002-3253-3210; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418 FU Office of Nuclear Physics within the US DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; MoST of China (973 Program) [2014CB845400]; CAS; MoE of China; Korean Research Foundation; GA of the Czech Republic; FIAS of Germany; DAE of India; DST of India; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia; MSMT of the Czech Republic FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Office of Nuclear Physics within the US DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, the NNSFC, the MoST of China (973 Program No. 2014CB845400), CAS, the MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, the National Science Centre of Poland, National Research Foundation (NRF-2012004024), the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 36 TC 2 Z9 2 U1 1 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 7 PY 2015 VL 92 IS 2 AR 021901 DI 10.1103/PhysRevC.92.021901 PG 7 WC Physics, Nuclear SC Physics GA CO4FZ UT WOS:000359117700001 ER PT J AU Boughezal, R Focke, C Liu, XH Petriello, F AF Boughezal, Radja Focke, Christfried Liu, Xiaohui Petriello, Frank TI W-Boson Production in Association with a Jet at Next-to-Next-to-Leading Order in Perturbative QCD SO PHYSICAL REVIEW LETTERS LA English DT Article ID NNLO QCD; MCFM; LHC AB We present the complete calculation of W-boson production in association with a jet in hadronic collisions through next-to-next-to-leading order (NNLO) in perturbative QCD. To cancel infrared divergences, we discuss a new subtraction method that exploits the fact that the N-jettiness event-shape variable fully captures the singularity structure of QCD amplitudes with final-state partons. This method holds for processes with an arbitrary number of jets and is easily implemented into existing frameworks for higher-order calculations. We present initial phenomenological results for W + jet production at the LHC. The NNLO corrections are small and lead to a significantly reduced theoretical error, opening the door to precision measurements in the W + jet channel at the LHC. C1 [Boughezal, Radja; Petriello, Frank] Argonne Natl Lab, High Energy Phys Div, Argonne, IL 60439 USA. [Focke, Christfried; Petriello, Frank] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Liu, Xiaohui] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Liu, Xiaohui] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. RP Boughezal, R (reprint author), Argonne Natl Lab, High Energy Phys Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rboughezal@anl.gov; christfried.focke@northwestern.edu; xhliu@umd.edu; f-petriello@northwestern.edu OI liu, xiaohui/0000-0002-7701-1205 FU DOE [DE-AC02-06CH11357, DE-FG02-91ER40684]; U.S. DOE; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX R. B. is supported by the DOE Contract No. DE-AC02-06CH11357. C. F. is supported by the DOE Grant No. DE-FG02-91ER40684. X. L. is supported by the U.S. DOE. F. P. is supported by the DOE Grants No. DE-FG02-91ER40684 and No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 42 TC 47 Z9 47 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 7 PY 2015 VL 115 IS 6 AR 062002 DI 10.1103/PhysRevLett.115.062002 PG 5 WC Physics, Multidisciplinary SC Physics GA CO4GU UT WOS:000359119900002 PM 26296111 ER PT J AU Poelking, VGD Giordano, A Ricci-Silva, ME Williams, TCR Pecanha, DA Ventrella, MC Rencoret, J Ralph, J Barbosa, MHP Loureiro, M AF de Carli Poelking, Viviane Guzzo Giordano, Andrea Ricci-Silva, Maria Esther Rhys Williams, Thomas Christopher Pecanha, Diego Alves Ventrella, Marilia Contin Rencoret, Jorge Ralph, John Pereira Barbosa, Marcio Henrique Loureiro, Marcelo TI Analysis of a Modern Hybrid and an Ancient Sugarcane Implicates a Complex Interplay of Factors in Affecting Recalcitrance to Cellulosic Ethanol Production SO PLOS ONE LA English DT Article ID CINNAMYL ALCOHOL-DEHYDROGENASE; CELL-WALL DEGRADABILITY; LIGNIN BIOSYNTHESIS PERTURBATIONS; HYDROXYCINNAMIC ACID CONTENT; ION MASS-SPECTROMETRY; LIGNOCELLULOSIC BIOMASS; ARABIDOPSIS-THALIANA; BIOFUEL PRODUCTION; COA REDUCTASE; STRUCTURAL-CHARACTERIZATION AB Abundant evidence exists to support a role for lignin as an important element in biomass recalcitrance. However, several independent studies have also shown that factors apart from lignin are also relevant and overall, the relative importance of different recalcitrance traits remains in dispute. In this study we used two genetically distant sugarcane genotypes, and performed a correlational study with the variation in anatomical parameters, cell wall composition, and recalcitrance factors between these genotypes. In addition we also tracked alterations in these characteristics in internodes at different stages of development. Significant differences in the development of the culm between the genotypes were associated with clear differential distributions of lignin content and composition that were not correlated with saccharification and fermentation yield. Given the strong influence of the environment on lignin content and composition, we hypothesized that sampling within a single plant could allow us to more easily interpret recalcitrance and changes in lignin biosynthesis than analysing variations between different genotypes with extensive changes in plant morphology and culm anatomy. The syringyl/guaiacyl (S/G) ratio was higher in the oldest internode of the modern genotype, but S/G ratio was not correlated with enzymatic hydrolysis yield nor fermentation efficiency. Curiously we observed a strong positive correlation between ferulate ester level and cellulose conversion efficiency. Together, these data support the hypothesis that biomass enzymatic hydrolysis recalcitrance is governed by a quantitative heritage rather than a single trait. C1 [de Carli Poelking, Viviane Guzzo; Giordano, Andrea; Ricci-Silva, Maria Esther; Rhys Williams, Thomas Christopher; Pecanha, Diego Alves; Ventrella, Marilia Contin; Loureiro, Marcelo] Univ Fed Vicosa, Dept Biol Vegetal, Vicosa, MG, Brazil. [Rencoret, Jorge; Ralph, John] Univ Wisconsin, Dept Biochem, Madison, WI 53705 USA. [Rencoret, Jorge; Ralph, John] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Pereira Barbosa, Marcio Henrique] Univ Fed Vicosa, Dept Fitotecnia, Vicosa, MG, Brazil. RP Loureiro, M (reprint author), Univ Fed Vicosa, Dept Biol Vegetal, Vicosa, MG, Brazil. EM mehlersloureiro@gmail.com RI RENCORET, JORGE/E-1747-2013 OI RENCORET, JORGE/0000-0003-2728-7331 FU Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao Coordenacao de Projetos, Pesquisas e Estudos Tecnologicos; DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; Fondo Social Europeo (FSE) FX VCGP was funded by Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (http:// www.cnpq.br/) and AG by Fundacao Coordenacao de Projetos, Pesquisas e Estudos Tecnologicos (http:// www.coppetec.coppe.ufrj.br/site/). JR and JR were funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494); Jorge Rencoret also thanks the CSIC for a JAE-DOC contract of the program "Junta para la Ampliacion de Estudios" cofinanced by Fondo Social Europeo (FSE). NR 98 TC 2 Z9 2 U1 1 U2 21 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD AUG 7 PY 2015 VL 10 IS 8 AR e0134964 DI 10.1371/journal.pone.0134964 PG 25 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO4HF UT WOS:000359121100091 ER PT J AU Shioda, K Kambhampati, A Hall, AJ Lopman, BA AF Shioda, Kayoko Kambhampati, Anita Hall, Aron J. Lopman, Ben A. TI Global age distribution of pediatric norovirus cases SO VACCINE LA English DT Article DE Norovirus; Gastroenteritis; Age distribution; Vaccines; Vaccine; Socioeconomic factors ID VACCINE; GASTROENTERITIS; CHILDREN; DISEASE AB Norovirus is increasingly recognized as a major cause of acute gastroenteritis among children <5 years of age. We searched for publications that reported detailed age distributions of pediatric norovirus cases, and assessed associations between age distribution and socio-demographic factors to identify the most critical age periods to prevent norovirus cases among young children. Approximately 70% of pediatric norovirus cases occurred between 6 and 23 months of age. A younger age distribution was found in lower income countries and inpatient settings. These findings suggest that a norovirus immunization schedule completed by 6 months could have the potential to prevent about 85% of pediatric cases, while a vaccine delivered at 12 months of age would only have the potential to prevent about 50% of pediatric cases. With a younger age distribution in lower income settings, early prevention would be even more critical. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Shioda, Kayoko; Kambhampati, Anita; Hall, Aron J.; Lopman, Ben A.] Ctr Dis Control & Prevent, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA. [Shioda, Kayoko; Kambhampati, Anita] Oak Ridge Inst Sci & Technol, Oak Ridge, TN 37831 USA. RP Shioda, K (reprint author), Ctr Dis Control & Prevent, Natl Ctr Immunizat & Resp Dis, 1600 Clifton Rd NE, Atlanta, GA 30333 USA. EM yji4@cdc.gov; wyc4@cdc.gov; esg3@cdc.gov; iow4@cdc.gov FU Food-borne Disease Burden Epidemiology Reference Group (FERG) of the World Health Organization (WHO) FX This research was supported by (a) an appointment to the Research Participation Program at the Centers for Disease Control and Prevention administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and CDC (to K.S. and A.K.) and (b) the Food-borne Disease Burden Epidemiology Reference Group (FERG) of the World Health Organization (WHO). We thank Marion Koopmans and Linda Verhoef at the National Institute for Public Health and the Environment in the Netherlands for their previous contribution to developing the database. NR 14 TC 7 Z9 7 U1 1 U2 3 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0264-410X EI 1873-2518 J9 VACCINE JI Vaccine PD AUG 7 PY 2015 VL 33 IS 33 BP 4065 EP 4068 DI 10.1016/j.vaccine.2015.05.051 PG 4 WC Immunology; Medicine, Research & Experimental SC Immunology; Research & Experimental Medicine GA CO2FD UT WOS:000358970600005 PM 26051514 ER PT J AU Zhang, M Shao, JH Xiao, J Deng, WB Yu, HJ AF Zhang, Min Shao, Jinhui Xiao, Juan Deng, Wenbing Yu, Hongjun TI A novel approach to make homogeneous protease-stable monovalent streptavidin SO BIOCHEMICAL AND BIOPHYSICAL RESEARCH COMMUNICATIONS LA English DT Article DE Streptavidin; Homogeneity; Protease stability ID BIOTIN TECHNOLOGY; AVIDIN; PROTEINS AB The interaction between the tetramer streptavidin and biotin is recognized as one of the strongest non-covalent associations. Owing to the tight and specific binding, the streptavidin-biotin system has been used widely for bimolecular labeling, purification, immobilization, and even for targeted delivery of therapeutics drugs. Here, we report a novel approach to make homogeneous monovalent tetramer streptavidin. The purified monovalent protein showed both thermal stability and protease stability. Unexpectedly, we found that two proteases, Proteinase K (PK) and Subtilisin (SU), can efficiently remove the His(8)-tag from the wild-type subunit without affecting the tetramer architecture of monovalent streptavidin, thus making it more homogeneous. In addition, crystallization was performed to assure the homogeneity of the monovalent protein prepared. Overall, monovalent streptavidin shows increased homogeneity and will likely be valuable for many future applications in a wide range of research areas. (C) 2015 Elsevier Inc. All rights reserved. C1 [Zhang, Min; Shao, Jinhui; Xiao, Juan] Hubei Univ Arts & Sci, Coll Med, Xiangyang, Hubei, Peoples R China. [Zhang, Min; Deng, Wenbing] Univ Calif Davis, Sch Med, Dept Biochem & Mol Med, Davis, CA 95616 USA. [Yu, Hongjun] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Deng, WB (reprint author), Univ Calif Davis, Sch Med, Dept Biochem & Mol Med, Davis, CA 95616 USA. EM wbdeng@ucdavis.edu; yuhongjun05@gmail.com FU Natural Science Foundation of Hubei Province, China [2015CFC801]; Foundation of Health and Family planning Commission of Hubei Province, China [WJ2015MB189]; Doctoral Research Fund of Hubei University of Arts and Science; National Institutes of Health [R01NS061983]; National Multiple Sclerosis Society; Shriners Hospitals for Children FX This research was supported by the grants from the Natural Science Foundation of Hubei Province, China (2015CFC801), the Foundation of Health and Family planning Commission of Hubei Province, China (WJ2015MB189) and the Doctoral Research Fund of Hubei University of Arts and Science. W.D. was supported by grants from National Institutes of Health (R01NS061983), the National Multiple Sclerosis Society, and Shriners Hospitals for Children. NR 14 TC 2 Z9 2 U1 1 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0006-291X EI 1090-2104 J9 BIOCHEM BIOPH RES CO JI Biochem. Biophys. Res. Commun. PD AUG 7 PY 2015 VL 463 IS 4 BP 1059 EP 1063 DI 10.1016/j.bbrc.2015.06.058 PG 5 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CN5FN UT WOS:000358455300094 PM 26074145 ER PT J AU Haddad, J Steinruck, HG Hlaing, H Kewalramani, S Pontoni, D Reichert, H Murphy, BM Festersen, S Runge, B Magnussen, OM Magerl, A Deutsch, M Ocko, BM AF Haddad, Julia Steinrueck, Hans-Georg Hlaing, Htay Kewalramani, Sumit Pontoni, Diego Reichert, Harald Murphy, Bridget M. Festersen, Sven Runge, Benjamin Magnussen, Olaf M. Magerl, Andreas Deutsch, Moshe Ocko, Benjamin M. TI Order and Melting in Self-Assembled Alkanol Monolayers on Amorphous SiO2 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY REFLECTIVITY; AIR-WATER-INTERFACE; GRAZING-INCIDENCE; OCTADECANOL MONOLAYERS; 1-ALCOHOL MONOLAYERS; CATALYTIC-ACTIVITY; MOLECULAR-MOTION; CHAIN MOLECULES; ALCOHOLS; DIFFRACTION AB Molecular self-assembly is a key to wide-ranging nano- and microscale applications in numerous fields. Understanding its underlying molecular level science is therefore of prime importance. This study resolves the angstrom-scale structure of the earliest and simplest self-assembled monolayer (SAM), octadecanol on amorphous-SiO2-terminated Si(001) substrate, and determines the structures temperature evolution. At low temperatures lateral hexagonal order exists, with close-packed, surface-normal molecules. At similar to 12 degrees C above the alkanols bulk melting, a fully reversible disordering transition occurs to a novel stretched liquid phase, laterally disordered, but only similar to 15% thinner SAM than in the crystalline phase. The SAM persists to >= 100 degrees C. A thermodynamic model yields here a headgroup-substrate bond energy similar to 40% lower than on crystalline sapphire, highlighting the importance of the substrates order, and near-epitaxy, for the SAMs ordering and stability. C1 [Haddad, Julia; Deutsch, Moshe] Bar Ilan Univ, Dept Phys, IL-52900 Ramat Gan, Israel. [Haddad, Julia; Deutsch, Moshe] Bar Ilan Univ, Inst Nanotechnol, IL-52900 Ramat Gan, Israel. [Steinrueck, Hans-Georg] Univ Erlangen Nurnberg, Crystallog & Struct Phys, D-91058 Erlangen, Germany. [Hlaing, Htay; Kewalramani, Sumit; Ocko, Benjamin M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Pontoni, Diego; Reichert, Harald] ESRF, F-38000 Grenoble, France. [Murphy, Bridget M.; Festersen, Sven; Runge, Benjamin; Magnussen, Olaf M.] Univ Kiel, Ruprecht Haensel Lab, D-24098 Kiel, Germany. [Magerl, Andreas] Univ Erlangen Nurnberg, Dept Phys, D-91058 Erlangen, Germany. RP Ocko, BM (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM ocko@bnl.gov RI Steinruck, Hans-Georg/A-6382-2015 FU U.S. Department of Energy, Basic Energy Sciences, by the Materials Sciences and Engineering Division [DE-AC02-98CH10886]; U.S.-Israel Binational Foundation, Jerusalem; DFG [1878]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; PSCM (ESRF) FX This work was supported by the U.S. Department of Energy, Basic Energy Sciences, by the Materials Sciences and Engineering Division (B.O., H.H., & S.K.) under contract No. DE-AC02-98CH10886, the U.S.-Israel Binational Foundation, Jerusalem (M.D.), and DFG research unit 1878, "Functional Molecular Structures on Complex Oxide Surfaces" (H.-G.S., A.M.). Use of the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. We thank the NSLS, PETRA III, and ESRF for beam time, the PSCM (ESRF) for support, and V. Honkimaki (ESRF) and O. Seeck (PETRA III) for advice. NR 60 TC 5 Z9 5 U1 9 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 6 PY 2015 VL 119 IS 31 BP 17648 EP 17654 DI 10.1021/acs.jpcc.5b03554 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO7IG UT WOS:000359332200017 ER PT J AU Song, J Rodenbough, PP Xu, WQ Senanayake, SD Chana, SW AF Song, Junhua Rodenbough, Philip P. Xu, Wenqian Senanayake, Sanjaya D. Chana, Siu-Wai TI Reduction of Nano-Cu2O: Crystallite Size Dependent and the Effect of Nano-Ceria Support SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-MONOXIDE; X-RAY; CU2O; NANOPARTICLES; OXIDATION; SELECTIVITY; CATALYSTS; CUO; XPS AB Copper(I) oxide (Cu2O) is an effective catalyst in the CO oxidation reaction. While high surface to volume ratio in nanoparticles will increase their catalytic efficiency, it posts a stability problem. Here we study the stability of nano-cuprite against reduction as a function of its crystallite size and upon interaction with a nano-ceria support. A systematic analysis of isothermal reduction of a series size of monodispersed Cu2O nanocrystals (+/- 7%) with time-resolved X-ray diffraction (TR-XRD) provides the time-resolved phase fraction of Cu2O and the time when reduction product of Cu (fcc) first appears. The initial phase fraction of nano-Cu2O is less than one with the balance attributed to an amorphous CuO shell. Since no peaks of crystalline CuO (monoclinic) were observed, a coreshell structure with an amorphous CuO shell is proposed. From the analysis, Cu2+ content in corresponding to shell increases from 0 to 33% as Cu2O decreases to 8 nm from the bulk. Based on the reduction profiles, a time size reduction (TSR) diagram is constructed for the observed Cu2O phase behavior during reduction. The incorporation onto a nano-CeO2 support (7 nm) significantly stabilizes our nano-Cu2O in a reducing atmosphere. The oxygen supply propensity in terms of oxygen nonstoichiometry of CeO2-y is shown to be lower when a larger crystallite size CeO2 (20 nm) support is used. The larger oxygen capacity in smaller nano-CeO2 support is analyzed and explained by the Madelung model with size-dependent bulk modulus of nano-ceria. C1 [Song, Junhua; Rodenbough, Philip P.; Chana, Siu-Wai] Columbia Univ, Dept Appl Phys & Appl Math, Mat Sci & Engn Program, New York, NY 10027 USA. [Rodenbough, Philip P.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Xu, Wenqian; Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Chana, SW (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, Mat Sci & Engn Program, New York, NY 10027 USA. EM sc174@columbia.edu RI Senanayake, Sanjaya/D-4769-2009 OI Senanayake, Sanjaya/0000-0003-3991-4232 FU National Science Foundation [DMR 1206764]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704] FX This work was primarily supported by National Science Foundation-DMR 1206764. Research at Brookhaven National Laboratory, in the Chemistry Department and at the National Synchrotron Light Source, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-SC0012704. The authors thank Professor James Im for his constructive discussion. We also acknowledge SWC's former student Jenna Pike for her investigation in cuprite nanoparticle synthesis and Yousun Hardware Manufactory, Shenzhen, China for machining parts for the heating stage, which makes in situ XRD possible. NR 24 TC 6 Z9 6 U1 7 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 6 PY 2015 VL 119 IS 31 BP 17667 EP 17672 DI 10.1021/acs.jpcc.5b04121 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO7IG UT WOS:000359332200020 ER PT J AU Kronawitter, CX Lessio, M Zhao, P Riplinger, C Boscoboinik, A Starr, DE Sutter, P Carter, EA Koel, BE AF Kronawitter, Coleman X. Lessio, Martina Zhao, Peng Riplinger, Christoph Boscoboinik, Anibal Starr, David E. Sutter, Peter Carter, Emily A. Koel, Bruce E. TI Observation of Surface-Bound Negatively Charged Hydride and Hydroxide on GaP(110) in H2O Environments SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; TOTAL-ENERGY CALCULATIONS; CO2 REDUCTION-MECHANISMS; NEAR-AMBIENT CONDITIONS; AQUEOUS CARBON-DIOXIDE; WAVE BASIS-SET; ELECTROCHEMICAL REDUCTION; WATER-ADSORPTION; DISSOCIATIVE ADSORPTION; THEORETICAL INSIGHTS AB Surface-bound species on GaP(110) formed upon interaction with water were investigated through experiment and theory. These studies are motivated by and discussed in the context of electrocatalytic and photoelectrocatalytic schemes for solar fuel production, including especially observations of selective CO2 reduction to methanol in acidified aqueous solutions of CO2 and nitrogen-containing heteroaromatics. Experimentally, surface-bound species over 10 orders of magnitude of pressure were spectroscopically identified in situ using synchrotron-based ambient pressure photoelectron spectroscopy. Ga 3d and O 1s core-level spectra indicate that the interaction of GaP(110) with H2O induces formation of a partially dissociated adlayer, characterized by the presence of both Ga-OH and molecular H2O species. Measurements of the P 2p core level indicate formation of a negatively charged hydride that irreversibly bonds to surface P in vacuum. The surface densities of the hydroxide and hydride species increase with increasing pressure (surface coverage) of water. Periodic slab calculations using density functional theory were used to study several relevant water configurations at 298 K on this surface. Consistent with earlier theoretical predictions at 0 K, the calculations confirm that Ga-OH, molecular H2O, and P-H species are thermodynamically stable on the GaP(110) surface under experimental conditions. Isobaric measurements at elevated pressures were used to probe the thermal stabilities of adsorbed species as well as the oxidation of surface Ga and P. The observation of stable surface hydride formation induced by interaction with water is especially notable given the critical role of hydride transfer to catalysts and CO2 during chemical fuel synthesis reactions in aqueous environments. It is hypothesized that the observed high stability of the hydride on GaP may contribute to its associated remarkable near-100% faradaic efficiency for methanol generation by solar-driven CO2 reduction in acidified aqueous pyridine solutions [J. Am. Chem. Soc.2008, 130, 6342] because such stability is known to yield high overpotentials for the competing hydrogen evolution reaction. C1 [Kronawitter, Coleman X.; Zhao, Peng; Koel, Bruce E.] Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08544 USA. [Lessio, Martina] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Riplinger, Christoph; Carter, Emily A.] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Boscoboinik, Anibal; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Starr, David E.] Helmholtz Zentrum Berlin Mat & Energie GmbH, Inst Solar Fuels, D-14109 Berlin, Germany. [Carter, Emily A.] Princeton Univ, Program Appl & Computat Math, Princeton, NJ 08544 USA. [Carter, Emily A.] Princeton Univ, Andlinger Ctr Energy & Environm, Princeton, NJ 08544 USA. RP Koel, BE (reprint author), A311 EQuad, Princeton, NJ 08544 USA. EM bkoel@princeton.edu RI Carter, Emily/P-4075-2014 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [DE-SC0012455]; Air Force Office of Scientific Research under AFOSR Award [FA9550-10-1-0572]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences under Award DE-SC0012455. M.L. and E.A.C. acknowledge financial support from the Air Force Office of Scientific Research under AFOSR Award FA9550-10-1-0572. Research was carried out in part at the Center for Functional Nanomaterials and National Synchrotron Light Source, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. We thank Professor John Keith, Andrew Ritzmann, and Nima Alidoust for helpful discussions. NR 65 TC 9 Z9 9 U1 7 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 6 PY 2015 VL 119 IS 31 BP 17762 EP 17772 DI 10.1021/acs.jpcc.5b05361 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO7IG UT WOS:000359332200031 ER PT J AU Bowers, GM Argersinger, HE Reddy, UV Johnson, TA Arey, B Bowden, M Kirkpatrick, RJ AF Bowers, Geoffrey M. Argersinger, Haley E. Reddy, U. Venkataswara Johnson, Timothy A. Arey, Bruce Bowden, Mark Kirkpatrick, R. James TI Integrated Molecular and Microscopic Scale Insight into Morphology and Ion Dynamics in Ca2+-Mediated Natural Organic Matter Floccs SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY REFLECTIVITY; ATOMIC-FORCE MICROSCOPY; SORBED HUMIC SUBSTANCES; FULVIC-ACID; CA-43 NMR; CLAY-MINERALS; SUPRAMOLECULAR STRUCTURE; AQUEOUS-SOLUTIONS; COMPLEX-FORMATION; POLYACRYLIC-ACID AB Combined X-ray diffraction (XRD), helium ion microscopy (HeIM), and Ca-43 nuclear magnetic resonance (NMR) results provide novel insight into the nano- and microstructure of flocculated NOM; the molecular-scale interaction among natural organic matter (NOM), dissolved Ca2+ ions, and water in NOM floccs; and the effects of pH and ionic strength on these characteristics. Suwannee River humic acid (HA), fulvic acid (FA), and NOM flocculated from Ca2+ bearing solutions share similar morphological characteristics on the 100 nm to micron scales, including micron-sized equant fragments and rounded, rough areas with features on the 100 nm scale. HeIM suggests that the NOM floccs are built from a fundamental spheroidal structure that is similar to 10 nm in diameter, in agreement with published AFM and small-angle X-ray scattering results. Calcium is incorporated into these floccs at 100% relative humidity in a wide range of disordered structural environments, with basic pH leading to shorter mean Ca-O distances and lower mean coordination numbers with respect to floccs formed under acidic conditions. The NMR results show that dynamical processes involving water and Ca2+ occurring at frequencies >10(4) Hz are important for hydrated OM floccs, in agreement with published molecular dynamics simulations of OM in solution. From the NMR results, we find evidence for two Ca2+ dynamic averaging mechanisms: one related to rapid exchange (>100 kHz) between surface proximity-restricted (those within 5 angstrom of a surface) and bulk solution environments when excess Ca2+ is present in the pore solution when pore water is unfrozen and a second consisting of intermediate scale (tens of kHz) site exchange among strongly sorbed inner-sphere sites when excess Ca2+ is absent and the carboxylic and phenolic functional groups of the NOM are deprotonated. C1 [Bowers, Geoffrey M.; Argersinger, Haley E.; Johnson, Timothy A.] Alfred Univ, Div Chem, Alfred, NY 14802 USA. [Reddy, U. Venkataswara] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Kirkpatrick, R. James] Michigan State Univ, Coll Nat Sci, E Lansing, MI 48824 USA. [Arey, Bruce; Bowden, Mark] Pacific NW Natl Lab, William R Wiley Environm & Mol Sci Lab, Richland, WA 99354 USA. RP Bowers, GM (reprint author), Alfred Univ, Div Chem, 1 Saxon Dr, Alfred, NY 14802 USA. EM bowers@alfred.edu OI Bowers, Geoffrey/0000-0003-4876-9305 FU United States Department of Energy, Office of Science, Office of Basic Energy Science [DE-FG02-10ER16128, DE-FG02-08ER15929]; United States Department of Energy Office of Science, Office of Biological and Environmental Research FX This material is based on work supported by the United States Department of Energy, Office of Science, Office of Basic Energy Science, under Awards DE-FG02-10ER16128 (G.M.B., P.I.) and DE-FG02-08ER15929 (R.J.K., P.I.). The 43Ca NMR spectra were obtained using the High Field Magnetic Resonance User Facility housed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the United States Department of Energy Office of Science, Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We thank Sarah Burton for assistance with setting up and accessing the NMR spectrometers. Helium ion microscopy images and the XRD patterns of the flocculated NOM were also obtained using instrumentation at EMSL. Thanks also to Ms. Arielle Polakos and Dr. Andrew Eklund for assistance in devising the 43Ca-enriched solution preparation procedure. NR 78 TC 1 Z9 1 U1 7 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 6 PY 2015 VL 119 IS 31 BP 17773 EP 17783 DI 10.1021/acs.jpcc.5b05509 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO7IG UT WOS:000359332200032 ER PT J AU Marshall, AR Young, MR Nozik, AJ Beard, MC Luther, JM AF Marshall, Ashley R. Young, Matthew R. Nozik, Arthur J. Beard, Matthew C. Luther, Joseph M. TI Exploration of Metal Chloride Uptake for Improved Performance Characteristics of PbSe Quantum Dot Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MULTIPLE EXCITON GENERATION; FIELD-EFFECT TRANSISTORS; OPEN-CIRCUIT VOLTAGE; CARRIER MULTIPLICATION; COLLOIDAL NANOCRYSTALS; CORE/SHELL NANOCRYSTALS; ELECTRICAL-PROPERTIES; PHOTOVOLTAIC DEVICES; CDSE NANOCRYSTALS; EFFICIENCY AB We explored the uptake of metal chloride salts with +1 to +3 metals of Na+, K+, Zn2+, Cd2+, Sn2+, Cu2+, and In3+ by PbSe QD solar cells. We also compared CdCl2 to Cd acetate and Cd nitrate treatments. PbSe QD solar cells fabricated with a CdCl2 treatment are stable for more than 270 days stored in air. We studied how temperature and immersion times affect optoelectronic properties and photovoltaic cell performance. Uptake of Cd2+ and Zn2+ increase open circuit voltage, whereas In3+ and K+ increase the photocurrent without influencing the spectral response or first exciton peak position. Using the most beneficial treatments we varied the bandgap of PbSe QD solar cells from 0.78 to 1.3 eV and find the improved V-OC is more prevalent for lower bandgap QD solar cells. C1 [Marshall, Ashley R.; Young, Matthew R.; Nozik, Arthur J.; Beard, Matthew C.; Luther, Joseph M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Marshall, Ashley R.; Nozik, Arthur J.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Luther, JM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM joey.luther@nrel.gov RI Nozik, Arthur/A-1481-2012; Nozik, Arthur/P-2641-2016; OI BEARD, MATTHEW/0000-0002-2711-1355 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers program within the Center for Advanced Solar Photophysics (CASP); DOE [DE-AC36-08G028308] FX The authors would like to thank Bobby To for SEM images, Fredrick Luiszer for ICP measurements, and Nathan Neale for supplying TiO2 nanoparticles. This work was supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers program within the Center for Advanced Solar Photophysics (CASP). DOE funding was provided to NREL through contract DE-AC36-08G028308. NR 74 TC 11 Z9 11 U1 7 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 2892 EP 2899 DI 10.1021/acs.jpclett.5b01214 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100008 PM 26267176 ER PT J AU Hoffman, DP Leblebici, SY Schwartzberg, AM Mathies, RA AF Hoffman, David P. Leblebici, Sibel Y. Schwartzberg, Adam M. Mathies, Richard A. TI Exciton Mobility in Organic Photovoltaic Heterojunctions from Femtosecond Stimulated Raman SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID RANGE CHARGE SEPARATION; SOLAR-CELLS; SPECTROSCOPY; DYNAMICS; DISSOCIATION; TIME AB Exciton mobility is crucial to organic photovoltaic (OPV) efficiency, but accurate, quantitative measures and therefore precise understanding of this process are currently lacking. Here, we exploit the unique capabilities of femtosecond stimulated Raman spectroscopy (FSRS) to disentangle the signatures of the bulk and interfacial donor response in a bulk heterojunction composed of poly[2-methoxy-5-(3',7'-dimethyloctyloxy)-1,4-phenylenevinylene] (MDMO-PPV) and phenyl-C-61-butyric acid methyl ester (PCBM). Surprisingly, we find that donor excitons are very mobile for the first similar to 300 fs following excitation (before thermalization) even though their overall lifetime is significantly longer (170 ps). A sharp decrease in mobility occurs after the system relaxes out of the Franck-Condon (FC) region. From this observation we predict that any polymer lacking a significant resonance Raman effect and fluorescence Stokes shift, indicating slow FC relaxation and small reorganization energy, will make an efficient OPV material. C1 [Hoffman, David P.; Mathies, Richard A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Leblebici, Sibel Y.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Leblebici, Sibel Y.; Schwartzberg, Adam M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Schwartzberg, AM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM amschwartzberg@lbl.gov; ramathies@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU Mathies Royalty fund; NSF 262 grant [NSF DGE 1106400]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Mathies Royalty fund, NSF 262 grant NSF DGE 1106400 and work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 28 TC 3 Z9 3 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 2919 EP 2923 DI 10.1021/acs.jpclett.5b01436 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100013 PM 26267181 ER PT J AU Wagle, DV Baker, GA Mamontov, E AF Wagle, Durgesh V. Baker, Gary A. Mamontov, Eugene TI Differential Microscopic Mobility of Components within a Deep Eutectic Solvent SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID TEMPERATURE IONIC LIQUID; 1-BUTYL-3-METHYL IMIDAZOLIUM HEXAFLUOROPHOSPHATE; ELASTIC NEUTRON-SCATTERING; RELAXATION PROCESSES; MOLECULAR LIQUIDS; MESOPOROUS CARBON; CHOLINE CHLORIDE; FAST DIFFUSION; HOLE THEORY; MIXTURES AB From macroscopic measurements of deep eutectic solvents such as glyceline (1:2 molar ratio of choline chloride to glycerol), the long-range translational diffusion of the larger cation (choline) is known to be slower compared to that of the smaller hydrogen bond donor (glycerol). However, when the diffusion dynamics are analyzed on the subnanometer length scale, we find that the displacements associated with the localized diffusive motions are actually larger for choline. This counterintuitive diffusive behavior can be understood as follows. The localized diffusive motions confined in the transient cage of neighbor particles, which precede the cage-breaking long-range diffusion jumps, are more spatially constrained for glycerol than for choline because of the stronger hydrogen bonds the former makes with chloride anions. The implications of such differential localized mobility of the constituents should be especially important for applications where deep eutectic solvents are confined on the nanometer length scale and their long-range translational diffusion is strongly inhibited (e.g., within microporous media). C1 [Wagle, Durgesh V.; Baker, Gary A.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Mamontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Mamontov, E (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM bakergar@missouri.edu; mamontove@ornl.gov RI Mamontov, Eugene/Q-1003-2015; Baker, Gary/H-9444-2016 OI Mamontov, Eugene/0000-0002-5684-2675; Baker, Gary/0000-0002-3052-7730 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy (DOE) [DE-AC05- 00OR22725]; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX The neutron scattering experiment at Oak Ridge National Laboratory's (ORNL) Spoliation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) under Contract No. DE-AC05- 00OR22725. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 25 TC 3 Z9 3 U1 5 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 2924 EP 2928 DI 10.1021/acs.jpclett.5b01192 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100014 PM 26267182 ER PT J AU Brookes, DH Head-Gordon, T AF Brookes, David H. Head-Gordon, Teresa TI Family of Oxygen-Oxygen Radial Distribution Functions for Water SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID LIQUID WATER; MOLECULAR-DYNAMICS; DIFFRACTION; AMBIENT; COMPRESSIBILITY AB In a typical X-ray diffraction experiment, the elastically scattered intensity, I(Q), is the experimental observable. I(Q) contains contributions from both intramolecular as well as intermolecular correlations embodied in the scattering factors, H-OO(Q) and H-OH(Q), with negligible contributions from H-HH(Q). Thus, to accurately define the oxygen-oxygen radial distribution function, g(OO)(r), a model of the electron density is required to accurately weigh the H-OO(Q) component relative to the intramolecular and oxygen-hydrogen correlations from the total intensity observable. In this work, we carefully define the electron density model and its underlying assumptions and more explicitly utilize two restraints on the allowable g(OO)(r) functions, which must conform to both very low experimental errors at high Q and the need to satisfy the isothermal compressibility at low Q Although highly restrained by these conditions, the underdetermined nature of the problem is such that we present a family of g(OO)(r) values that provide equally good agreement with the high-Q intensity and compressibility restraints and with physically correct behavior at small r. C1 [Head-Gordon, Teresa] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Brookes, David H.; Head-Gordon, Teresa] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Univ Calif Berkeley, Div Chem Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Head-Gordon, T (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM thg@berkeley.edu FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-1265731] FX This work was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy contract no. DE-AC02-05CH11231. We also thank the National Science Foundation grant CHE-1265731 for undergraduate training support for D.H.B. NR 28 TC 2 Z9 2 U1 2 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 2938 EP 2943 DI 10.1021/acs.jpclett.5b01066 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100017 PM 26267185 ER PT J AU Zheng, KB Zhu, QS Abdellah, M Messing, ME Zhang, W Generalov, A Niu, YR Ribaud, L Canton, SE Pullerits, T AF Zheng, Kaibo Zhu, Qiushi Abdellah, Mohamed Messing, Maria E. Zhang, Wei Generalov, Alexander Niu, Yuran Ribaud, Lynn Canton, Sophie E. Pullerits, Tonu TI Exciton Binding Energy and the Nature of Emissive States in Organometal Halide Perovskites SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CDSE QUANTUM DOTS; SOLAR-CELLS; ELECTRONIC-STRUCTURE; RECOMBINATION; DYNAMICS; DEPOSITION; LENGTHS; NANOPARTICLES; LUMINESCENT; EFFICIENCY AB Characteristics of nanoscale materials are often different from the corresponding bulk properties providing new, sometimes unexpected, opportunities for applications. Here we investigate the properties of 8 nm colloidal nanoparticles of MAPbBr(3) perovskites and contrast them to the ones of large microcrystallites representing a bulk. X-ray spectroscopies provide an exciton binding energy of 0.32 +/- 0.10 eV in the nanoparticles. This is 5 times higher than the value of bulk crystals (0.084 +/- 0.010 eV), and readily explains the high fluorescence quantum yield in nanoparticles. In the bulk, at high excitation concentrations, the fluorescence intensity has quadratic behavior following the Saha-Langmuir model due to the nongeminate recombination of charges forming the emissive exciton states. In the nanoparticles, a linear dependence is observed since the excitation concentration per particle is significantly less than one. Even the bulk shows linear emission intensity dependence at lower excitation concentrations. In this case, the average excitation spacing becomes larger than the carrier diffusion length suppressing the nongeminate recombination. From these considerations we obtain the charge carrier diffusion length in MAPbBr(3) of 100 nm. C1 [Zheng, Kaibo; Abdellah, Mohamed; Zhang, Wei; Pullerits, Tonu] Lund Univ, Dept Chem Phys, S-22100 Lund, Sweden. [Abdellah, Mohamed] South Valley Univ, Qena Fac Sci, Dept Chem, Qena 83523, Egypt. [Zhu, Qiushi] Lund Univ, Dept Synchrotron Radiat Instrumentat, S-22100 Lund, Sweden. [Messing, Maria E.] Lund Univ, Deptartment Solid State Phys, S-22100 Lund, Sweden. [Generalov, Alexander; Niu, Yuran] Lund Univ, MAX Lab 4, S-22100 Lund, Sweden. [Ribaud, Lynn] Argonne Natl Lab, Xray Sci Div, Adv Photon Source & Mat Sci Div, Argonne, IL 60439 USA. [Canton, Sophie E.] Max Planck Inst Biophys Chem, IFG Struct Dynam Bio Chem Syst, D-37077 Gottingen, Germany. [Canton, Sophie E.] DESY, FS SCS, Struct Dynam Ultrashort Pulsed Xrays, D-22607 Hamburg, Germany. RP Pullerits, T (reprint author), Max Planck Inst Biophys Chem, IFG Struct Dynam Bio Chem Syst, Fassberg 11, D-37077 Gottingen, Germany. EM sophie.canton@desy.de; Tonu.Pullerits@chemphys.lu.se RI Messing, Maria/D-5546-2009; Pullerits, Tonu/A-5603-2010; Canton, Sophie/A-8432-2016 OI Messing, Maria/0000-0003-1834-236X; Pullerits, Tonu/0000-0003-1428-5564; FU Knut and Alice Wallenberg Foundation; Swedish Research Council; DOE Office of Science [DE-AC02-06CH11357] FX We thank Dr. Arkady Yartsev and Prof. Ivan Scheblykin for critical reading of the manuscript. We thank Dr. Alexei Preobrajenski, MAX IV Laboratory, at Beamline D1011 for the helpful discussion and support. The study was financially supported by the Knut and Alice Wallenberg Foundation and the Swedish Research Council. Collaboration within nmC@LU is acknowledged. The mail-in program of Beamline 11-BM at Advanced Photon Source (APS) are greatly acknowledged. Use of APS at Argonne National Laboratory was supported by the U.S. Department of Energy, operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 45 TC 32 Z9 32 U1 15 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 2969 EP 2975 DI 10.1021/acs.jpclett.5b01252 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100022 PM 26267190 ER PT J AU Simpson, MJ Doughty, B Yang, B Xiao, K Ma, YZ AF Simpson, Mary Jane Doughty, Benjamin Yang, Bin Xiao, Kai Ma, Ying-Zhong TI Spatial Localization of Excitons and Charge Carriers in Hybrid Perovskite Thin Films SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITE; SOLAR-CELLS; HIGH-EFFICIENCY; RECOMBINATION; DYNAMICS; PHOTOLUMINESCENCE; CH3NH3PBI3; MOBILITIES; MICROSCOPY; MECHANISM AB The fundamental photophysics underlying the remarkably high-power conversion efficiency of organic-inorganic hybrid perovskite-based solar cells has been increasingly studied using complementary spectroscopic techniques. However, the spatially heterogeneous polycrystalline morphology of the photoactive layers owing to the presence of distinct crystalline grains has been generally neglected in optical measurements; therefore, the reported results are typically averaged over hundreds or even thousands of such grains. Here we apply femtosecond transient absorption microscopy to spatially and temporally probe ultrafast electronic excited-state dynamics in pristine methylammonium lead tri-iodide (CH3NH3PbI3) thin films and composite structures. We found that the electronic excited-state relaxation kinetics are extremely sensitive to the sample location probed, which was manifested by position-dependent decay time scales and transient signals. Analysis of transient absorption kinetics acquired at distinct spatial positions enabled us to identify contributions of excitons and free charge carriers. C1 [Simpson, Mary Jane; Doughty, Benjamin; Ma, Ying-Zhong] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Yang, Bin; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Ma, YZ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM may1@ornl.gov RI Yang, Bin/P-8529-2014; Ma, Yingzhong/L-6261-2016; Doughty, Benjamin /M-5704-2016; OI Yang, Bin/0000-0002-5667-9126; Ma, Yingzhong/0000-0002-8154-1006; Doughty, Benjamin /0000-0001-6429-9329; Simpson, Mary Jane/0000-0002-3511-8370 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX Work by M.J.S., B.D., and Y.-Z.M. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Perovskite sample preparation by B.Y. and K.X. was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 38 TC 15 Z9 15 U1 10 U2 111 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 3041 EP 3047 DI 10.1021/acs.jpclett.5b01050 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100032 PM 26267200 ER PT J AU Bolmatov, D Zhernenkov, M Zav'yalov, D Stoupin, S Cai, YQ Cunsolo, A AF Bolmatov, Dima Zhernenkov, Mikhail Zav'yalov, Dmitry Stoupin, Stanislav Cai, Yong Q. Cunsolo, Alessandro TI Revealing the Mechanism of the Viscous-to-Elastic Crossover in Liquids SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SOUND-WAVES; BEHAVIOR; FLUIDS; ARGON; DYNAMICS; MATTER; WATER; NEON; LINE AB In this work, we report on inelastic X-ray scattering experiments combined with the molecular dynamics simulations on deeply supercritical Ar. The presented results unveil the mechanism and regimes of sound propagation in the liquid matter and provide compelling evidence for the adiabatic-to-isothermal longitudinal sound propagation transition. We introduce a Hamiltonian predicting low-frequency transverse sound propagation gaps, which is confirmed by experimental findings and molecular dynamics calculations. As a result, a universal link is established between the positive sound dispersion (PSD) phenomenon and the origin of transverse sound propagation revealing the viscous-to-elastic crossover in liquids. The PSD and transverse phononic excitations evolve consistently with theoretical predictions. Both can be considered as a universal fingerprint of the dynamic response of a liquid, which is also observable in a subdomain of supercritical phase. The simultaneous disappearance of both these effects at elevated temperatures is a manifestation of the Frenkel line. We expect that these findings will advance the current understanding of fluids under extreme thermodynamic conditions. C1 [Bolmatov, Dima; Zhernenkov, Mikhail; Cai, Yong Q.; Cunsolo, Alessandro] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Zav'yalov, Dmitry] Volgograd State Tech Univ, Volgograd 400005, Russia. [Stoupin, Stanislav] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Bolmatov, D (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM d.bolmatov@gmail.com; acunsolo@bnl.gov RI Cai, Yong/C-5036-2008; Zavyalov, Dmitriy/N-7609-2015; OI Cai, Yong/0000-0002-9957-6426; Zhernenkov, Mikhail/0000-0003-3604-0672 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC00112704, DE-AC02-06CH11357] FX We thank Bogdan M. Leu and Ayman H. Said for their support during the experiment at Sector 30 at APS and Sergey N. Tkachev for his help with the GSECARS gas loading system. The work at the National Synchrotron Light Source-II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC00112704. The synchrotron experiment was performed at 30-ID beamline, Advanced Photon Source (APS), Argonne National Laboratory. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 31 TC 9 Z9 9 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 6 PY 2015 VL 6 IS 15 BP 3048 EP 3053 DI 10.1021/acs.jpclett.5b01338 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO7IP UT WOS:000359333100033 PM 26267201 ER PT J AU Al Ma'Mari, F Moorsom, T Teobaldi, G Deacon, W Prokscha, T Luetkens, H Lee, S Sterbinsky, GE Arena, DA MacLaren, DA Flokstra, M Ali, M Wheeler, MC Burnell, G Hickey, BJ Cespedes, O AF Al Ma'Mari, Fatma Moorsom, Timothy Teobaldi, Gilberto Deacon, William Prokscha, Thomas Luetkens, Hubertus Lee, Steve Sterbinsky, George E. Arena, Dario A. MacLaren, Donald A. Flokstra, Machiel Ali, Mannan Wheeler, May C. Burnell, Gavin Hickey, Bryan J. Cespedes, Oscar TI Beating the Stoner criterion using molecular interfaces SO NATURE LA English DT Article ID COLLECTIVE ELECTRON FERROMAGNETISM; POSITIVE MUONS; GENERATION; ENERGY; SPINTRONICS; LENGTH AB Only three elements are ferromagnetic at room temperature: the transition metals iron, cobalt and nickel. The Stoner criterion explains why iron is ferromagnetic but manganese, for example, is not, even though both elements have an unfilled 3d shell and are adjacent in the periodic table: according to this criterion, the product of the density of states and the exchange integral must be greater than unity for spontaneous spin ordering to emerge(1,2). Here we demonstrate that it is possible to alter the electronic states of non-ferromagnetic materials, such as diamagnetic copper and paramagnetic manganese, to overcome the Stoner criterion and make them ferromagnetic at room temperature. This effect is achieved via interfaces between metallic thin films and C-60 molecular layers. The emergent ferromagnetic state exists over several layers of the metal before being quenched at large sample thicknesses by the material's bulk properties. Although the induced magnetization is easily measurable by magnetometry, low-energy muon spin spectroscopy(3) provides insight into its distribution by studying the depolarization process of low-energy muons implanted in the sample. This technique indicates localized spin-ordered states at, and close to, the metal-molecule interface. Density functional theory simulations suggest a mechanism based on magnetic hardening of the metal atoms, owing to electron transfer(4,5). This mechanism might allow for the exploitation of molecular coupling to design magnetic metamaterials using abundant, non-toxic components such as organic semiconductors. Charge transfer at molecular interfaces may thus be used to control spin polarization or magnetization, with consequences for the design of devices for electronic, power or computing applications (see, for example, refs 6 and 7). C1 [Al Ma'Mari, Fatma; Moorsom, Timothy; Deacon, William; Ali, Mannan; Wheeler, May C.; Burnell, Gavin; Hickey, Bryan J.; Cespedes, Oscar] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [Teobaldi, Gilberto] Univ Liverpool, Stephenson Inst Renewable Energy, Dept Chem, Liverpool L69 3BX, Merseyside, England. [Prokscha, Thomas; Luetkens, Hubertus] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland. [Lee, Steve; Flokstra, Machiel] Univ St Andrews, Sch Phys & Astron, SUPA, St Andrews KY16 9SS, Fife, Scotland. [Sterbinsky, George E.; Arena, Dario A.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [MacLaren, Donald A.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. RP Cespedes, O (reprint author), Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. EM o.cespedes@leeds.ac.uk RI Hickey, B J/B-3333-2016; MacLaren, D/A-5568-2010; Lee, Stephen/G-9791-2016; Luetkens, Hubertus/G-1831-2011; OI Hickey, B J/0000-0001-8289-5618; TEOBALDI, Gilberto/0000-0001-6068-6786; MacLaren, D/0000-0003-0641-686X; Lee, Stephen/0000-0002-2020-3310; Burnell, Gavin/0000-0002-9486-0639 FU Engineering and Physical Sciences Research Council [EP/K00512X/1, EP/K036408/1, EP/J01060X/1, EP/I004483/1]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the Engineering and Physical Sciences Research Council through grants EP/K00512X/1, EP/K036408/1, EP/J01060X/1 and EP/I004483/1. Use of the N8 POLARIS (EPSRC EP/K000225/1), ARCHER (via the UKCP Consortium, EP/K013610/1), and the High Performance Computing (HPC) Wales facilities is acknowledged. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract number DE-AC02-98CH10886. NR 37 TC 16 Z9 16 U1 168 U2 266 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 6 PY 2015 VL 524 IS 7563 BP 69 EP U128 DI 10.1038/nature14621 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO2QS UT WOS:000359002300033 ER PT J AU El-Khatib, S Phelan, D Barker, JG Zheng, H Mitchell, JF Leighton, C AF El-Khatib, S. Phelan, D. Barker, J. G. Zheng, H. Mitchell, J. F. Leighton, C. TI Neutron-scattering-based evidence for interacting magnetic excitons in LaCoO3 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-STATE TRANSITION; PHASE-SEPARATION; CONDUCTIVITY AB Recent progress with the thermally driven spin-state crossover in LaCoO3 has made it increasingly apparent that the nominally nonmagnetic low-spin ground state of this material actually hosts defect-based magnetism. This is investigated here via a small-angle neutron scattering (SANS) study of LaCoO3-d crystals. The results provide (i) the surprising finding that the spin-state crossover is clearly reflected in SANS via quasieleastic and inelastic scattering from paramagnetic spin fluctuations and excitations, and (ii) evidence for the formation, likely around oxygen defects, of local entities known as magnetic excitons. The latter generate distinct magnetic scattering below 60 K, providing valuable quantitative information on exciton densities and interactions. Potential relevance to the unexpected ferromagnetism recently discovered in epitaxial LaCoO3 films is discussed. C1 [El-Khatib, S.] Amer Univ Sharjah, Dept Phys, Sharjah, U Arab Emirates. [El-Khatib, S.; Phelan, D.; Leighton, C.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [El-Khatib, S.; Barker, J. G.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Phelan, D.; Zheng, H.; Mitchell, J. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Leighton, C (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. EM leighton@umn.edu FU US DOE [DE-FG02-06ER46275]; DOE Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; NSF through UMN MRSEC [DMR-1420013]; AUS [FRG-2012, FRG2013] FX Work supported primarily by the US DOE under DE-FG02-06ER46275. Work at ANL (crystal growth and characterization) supported by DOE Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Part of this work was carried out in the UMN Characterization Facility, which receives capital equipment funding from the NSF through the UMN MRSEC under Grant No. DMR-1420013. S.E-K. acknowledges travel support from AUS (Grants No. FRG-2012 and No. FRG2013). We thank F.S. Bates for useful discussions, and J. A. Borchers for experimental assistance. NR 34 TC 5 Z9 5 U1 5 U2 43 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 6 PY 2015 VL 92 IS 6 AR 060404 DI 10.1103/PhysRevB.92.060404 PG 5 WC Physics, Condensed Matter SC Physics GA CO3HD UT WOS:000359046500001 ER PT J AU Wang, ZT Garcia, JC Deskins, NA Lyubinetsky, I AF Wang, Zhi-Tao Garcia, Juan C. Deskins, N. Aaron Lyubinetsky, Igor TI Ability of TiO2(110) surface to be fully hydroxylated and fully reduced SO PHYSICAL REVIEW B LA English DT Article ID BAND-GAP; ADSORPTION; TIO2; DESORPTION; HYDROGEN; STATES; WATER; OXIDE; MICROSCOPY; DIFFUSION AB Many TiO2 applications (e.g., in heterogeneous catalysis) involve contact with ambient atmosphere and/or water. The resulting hydroxylation can significantly alter its surface properties. While the behavior of a single, isolated OH species on the model metal oxide surface of rutile TiO2(110) is relatively well understood, much less is known regarding highly hydroxylated surfaces and/or whether TiO2(110) could be fully hydroxylated under ultrahigh vacuum conditions. Here we report the in situ formation of a well-ordered, fully hydroxylated TiO2(110)-(1 x 1) surface using an enhanced photochemical approach, the key parts of which are predosing of water and multistep dissociative adsorption and subsequent photolysis of the carboxylic (trimethyl acetic) acid. Combining scanning tunneling microscopy, ultraviolet photoelectron spectroscopy, and density functional theory results, we show that the attained "super OH" surface is also fully reduced, as a result of the photochemical charging of electron traps associated with the OH groups. C1 [Wang, Zhi-Tao; Lyubinetsky, Igor] EMSL, Inst Integrated Catalysis, Richland, WA 99352 USA. [Wang, Zhi-Tao; Lyubinetsky, Igor] Pacific NW Natl Lab, Richland, WA 99352 USA. [Garcia, Juan C.; Deskins, N. Aaron] Worcester Polytech Inst, Dept Chem Engn, Worcester, MA 01609 USA. RP Lyubinetsky, I (reprint author), EMSL, Inst Integrated Catalysis, Richland, WA 99352 USA. EM igor.lyubinetsky@pnnl.gov OI Garcia, Juan/0000-0002-5911-8850 FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences; DOE's Office of Biological and Environmental Research FX We thank M. A. Henderson, G. A. Kimmel, N. G. Petrik, Z. Dohnalek, and Y. Du for stimulating discussions, and also acknowledge computational support from S. Najafi at WPI. This work was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, and performed at EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. NR 38 TC 6 Z9 6 U1 5 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 6 PY 2015 VL 92 IS 8 AR 081402 DI 10.1103/PhysRevB.92.081402 PG 5 WC Physics, Condensed Matter SC Physics GA CO3HY UT WOS:000359048700003 ER PT J AU Agakishiev, G Arnold, O Belver, D Belyaev, A Berger-Chen, JC Blanco, A Bohmer, M Boyard, JL Cabanelas, P Chernenko, S Dybczak, A Epple, E Fabbietti, L Fateev, O Finocchiaro, P Fonte, P Friese, J Frolich, I Galatyuk, T Garzon, JA Gernhauser, R Gobel, K Golubeva, M Gonzalez-Diaz, D Guber, F Gumberidze, M Heinz, T Hennino, T Holzmann, R Ierusalimov, A Iori, I Ivashkin, A Jurkovic, M Kampfer, B Karavicheva, T Koenig, I Koenig, W Kolb, BW Korcyl, G Kornakov, G Kotte, R Krasa, A Krizek, F Krucken, R Kuc, H Kuhn, W Kugler, A Kunz, T Kurepin, A Ladygin, V Lalik, R Lapidus, K Lebedev, A Lopes, L Lorenz, M Maier, L Mangiarotti, A Markert, J Metag, V Michel, J Mihaylov, D Muntz, C Munzer, R Naumann, L Pachmayer, YC Palka, M Parpottas, Y Pechenov, V Pechenova, O Pietraszko, J Przygoda, W Ramstein, B Reshetin, A Rustamov, A Sadovsky, A Salabura, P Schmah, A Schwab, E Siebenson, J Sobolev, YG Spataro, S Spruck, B Strobele, H Stroth, J Sturm, C Svoboda, O Tarantola, A Teilab, K Tlusty, P Traxler, M Tsertos, H Vasiliev, T Wagner, V Weber, M Wendisch, C Wustenfeld, J Yurevich, S Zanevsky, Y AF Agakishiev, G. Arnold, O. Belver, D. Belyaev, A. Berger-Chen, J. C. Blanco, A. Boehmer, M. Boyard, J. L. Cabanelas, P. Chernenko, S. Dybczak, A. Epple, E. Fabbietti, L. Fateev, O. Finocchiaro, P. Fonte, P. Friese, J. Froehlich, I. Galatyuk, T. Garzon, J. A. Gernhaeuser, R. Goebel, K. Golubeva, M. Gonzalez-Diaz, D. Guber, F. Gumberidze, M. Heinz, T. Hennino, T. Holzmann, R. Ierusalimov, A. Iori, I. Ivashkin, A. Jurkovic, M. Kaempfer, B. Karavicheva, T. Koenig, I. Koenig, W. Kolb, B. W. Korcyl, G. Kornakov, G. Kotte, R. Krasa, A. Krizek, F. Kruecken, R. Kuc, H. Kuehn, W. Kugler, A. Kunz, T. Kurepin, A. Ladygin, V. Lalik, R. Lapidus, K. Lebedev, A. Lopes, L. Lorenz, M. Maier, L. Mangiarotti, A. Markert, J. Metag, V. Michel, J. Mihaylov, D. Muentz, C. Muenzer, R. Naumann, L. Pachmayer, Y. C. Palka, M. Parpottas, Y. Pechenov, V. Pechenova, O. Pietraszko, J. Przygoda, W. Ramstein, B. Reshetin, A. Rustamov, A. Sadovsky, A. Salabura, P. Schmah, A. Schwab, E. Siebenson, J. Sobolev, Yu. G. Spataro, S. Spruck, B. Stroebele, H. Stroth, J. Sturm, C. Svoboda, O. Tarantola, A. Teilab, K. Tlusty, P. Traxler, M. Tsertos, H. Vasiliev, T. Wagner, V. Weber, M. Wendisch, C. Wuestenfeld, J. Yurevich, S. Zanevsky, Y. CA HADES Collaboration TI K*(892)(+) production in proton-proton collisions at E-beam=3.5 GeV SO PHYSICAL REVIEW C LA English DT Article ID PP-INTERACTIONS; BEAM ENERGY; MESONS AB We present results on the K*(892)(+) production in proton-proton collisions at a beam energy of E = 3.5 GeV, which is hitherto the lowest energy at which this mesonic resonance has been observed in nucleon-nucleon reactions. The data are interpreted within a two-channel model that includes the three-body production of K*(892)(+) associated with the Lambda or Sigma hyperon. The relative contributions of both channels are estimated. Besides the total cross section sigma(p + p -> K*(892)(+) + X) = 9.5 +/- 0.9(-0.9)(+1.1) +/- 0.7 mu b, which adds a new data point to the excitation function of the K*(892)+ production in the region of low excess energy, transverse momenta and angular spectra are extracted and compared with the predictions of the two-channel model. The spin characteristics of K*(892)(+) are discussed as well in terms of the spin-alignment. C1 [Finocchiaro, P.] Ist Nazl Fis Nucl, Lab Nazl Sud, I-95125 Catania, Italy. [Blanco, A.; Fonte, P.; Lopes, L.; Mangiarotti, A.] LIP Lab Instrumentacao & Fis Expt Particulas, P-3004516 Coimbra, Portugal. [Dybczak, A.; Korcyl, G.; Kuc, H.; Palka, M.; Przygoda, W.; Salabura, P.] Jagiellonian Univ, Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Heinz, T.; Holzmann, R.; Koenig, I.; Koenig, W.; Kolb, B. W.; Pechenov, V.; Pietraszko, J.; Schwab, E.; Stroth, J.; Sturm, C.; Traxler, M.; Wendisch, C.; Yurevich, S.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Galatyuk, T.; Gonzalez-Diaz, D.; Gumberidze, M.; Kornakov, G.] Tech Univ Darmstadt, D-64289 Darmstadt, Germany. [Kaempfer, B.; Kotte, R.; Naumann, L.; Wuestenfeld, J.] Helmholtz Zentrum Dresden Rossendorf, Inst Strahlenphys, D-01314 Dresden, Germany. [Agakishiev, G.; Belyaev, A.; Chernenko, S.; Fateev, O.; Ierusalimov, A.; Ladygin, V.; Vasiliev, T.; Zanevsky, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Froehlich, I.; Goebel, K.; Lorenz, M.; Markert, J.; Muentz, C.; Pachmayer, Y. C.; Pechenova, O.; Rustamov, A.; Stroebele, H.; Stroth, J.; Tarantola, A.; Teilab, K.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Arnold, O.; Berger-Chen, J. C.; Epple, E.; Fabbietti, L.; Lalik, R.; Lapidus, K.; Mihaylov, D.; Muenzer, R.; Siebenson, J.] Excellence Cluster Origin & Struct Universe, D-85748 Garching, Germany. [Arnold, O.; Berger-Chen, J. C.; Boehmer, M.; Epple, E.; Fabbietti, L.; Friese, J.; Gernhaeuser, R.; Jurkovic, M.; Kruecken, R.; Kunz, T.; Lalik, R.; Lapidus, K.; Maier, L.; Mihaylov, D.; Muenzer, R.; Siebenson, J.; Weber, M.] Tech Univ Munich, Phys Dept E12, D-85748 Garching, Germany. [Kuehn, W.; Metag, V.; Spruck, B.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Iori, I.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Golubeva, M.; Guber, F.; Ivashkin, A.; Karavicheva, T.; Kurepin, A.; Reshetin, A.; Sadovsky, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Lebedev, A.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Parpottas, Y.; Tsertos, H.] Univ Cyprus, Dept Phys, CY-1678 Nicosia, Cyprus. [Boyard, J. L.; Hennino, T.; Kuc, H.; Ramstein, B.] Univ Paris 11, CNRS IN2P3, UMR 8608, Inst Phys Nucl, F-91406 Orsay, France. [Krasa, A.; Krizek, F.; Kugler, A.; Sobolev, Yu. G.; Svoboda, O.; Tlusty, P.; Wagner, V.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Belver, D.; Cabanelas, P.; Garzon, J. A.] Univ Santiago de Compostela, LabCAF F Fis, Santiago De Compostela 15706, Spain. [Schmah, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Fonte, P.] ISEC Coimbra, Coimbra, Portugal. [Galatyuk, T.; Gumberidze, M.] ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Kaempfer, B.] Tech Univ Dresden, D-01062 Dresden, Germany. [Iori, I.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Parpottas, Y.] Frederick Univ, CY-1036 Nicosia, Cyprus. [Spataro, S.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Spataro, S.] Univ Turin, Ist Nazl Fis Nucl, I-10125 Turin, Italy. [Lorenz, M.] Univ Utrecht, NL-3584 CC Utrecht, Netherlands. RP Agakishiev, G (reprint author), Joint Inst Nucl Res, Dubna 141980, Russia. EM kirill.lapidus@ph.tum.de; dimitar.mihaylov@mytum.de RI Guber, Fedor/I-4271-2013; Gonzalez Diaz, Diego/K-7265-2014; Cabanelas, Pablo/B-2034-2016; Svoboda, Ondrej/G-7982-2014; Wagner, Vladimir/G-5650-2014; Gobel, Kathrin/B-8531-2016; Kurepin, Alexey/H-4852-2013; Mangiarotti, Alessio/I-1072-2012; Kruecken, Reiner/A-1640-2013; Fonte, Paulo/B-1842-2008; OI Guber, Fedor/0000-0001-8790-3218; Gonzalez Diaz, Diego/0000-0002-6809-5996; Cabanelas, Pablo/0000-0002-5416-4647; Gobel, Kathrin/0000-0003-2832-8465; Kurepin, Alexey/0000-0002-1851-4136; Mangiarotti, Alessio/0000-0001-7837-6057; Kruecken, Reiner/0000-0002-2755-8042; Fonte, Paulo/0000-0002-2275-9099; Tsertos, Charalambos/0000-0001-5966-343X FU LIP Coimbra, Coimbra (Portugal) [PTDC/FIS/113339/2009]; SIP JUC Cracow, Cracow (Poland), NCN Poland [2013/10/M/ST2/00042]; Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Dresden (Germany), BMBF [05P12CRGHE]; TU Munchen, Garching (Germany) MLL Munchen, DFG EClust [153, VH-NG-330 BMBF, 06MT9156]; TP5GSI TMKrue [1012]; NPI AS CR, Rez, Rez (Czech Republic) [M100481202]; GACR [13-06759S]; USC-S; de Compostela, Santiago de Compostela (Spain) CPAN [CSD2007-00042]; Goethe University, Frankfurt (Germany) [HA216/EMMI HIC for FAIR (LOEWE) BMBF, 06FY9100I]; GSI FE EU [HP3-283286] FX The HADES collaboration gratefully acknowledges support by the following grants: LIP Coimbra, Coimbra (Portugal), Grant No. PTDC/FIS/113339/2009; SIP JUC Cracow, Cracow (Poland), NCN Poland, Grant No. 2013/10/M/ST2/00042; Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Dresden (Germany), BMBF, Grant No. 05P12CRGHE; TU Munchen, Garching (Germany) MLL Munchen, DFG EClust, Grant No. 153, VH-NG-330 BMBF, Grant No. 06MT9156; TP5GSI TMKrue, Grant No. 1012; NPI AS CR, Rez, Rez (Czech Republic), Grant No. M100481202 and GACR, Grant No. 13-06759S; USC-S. de Compostela, Santiago de Compostela (Spain) CPAN, Grant No. CSD2007-00042; Goethe University, Frankfurt (Germany), Grant No. HA216/EMMI HIC for FAIR (LOEWE) BMBF, Grant No. 06FY9100I; GSI F&E EU Contract No. HP3-283286. NR 22 TC 1 Z9 1 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 6 PY 2015 VL 92 IS 2 AR 024903 DI 10.1103/PhysRevC.92.024903 PG 7 WC Physics, Nuclear SC Physics GA CO3IF UT WOS:000359049500005 ER PT J AU Benhar, O Lovato, A Rocco, N AF Benhar, Omar Lovato, Alessandro Rocco, Noemi TI Contribution of two-particle-two-hole final states to the nuclear response SO PHYSICAL REVIEW C LA English DT Article ID SPECTRAL-FUNCTION; FORM-FACTORS; SCATTERING; MATTER AB The excitation of two-particle-two-hole final states in neutrino-nucleus scattering has been advocated by many authors as the source of the excess cross section observed by the MiniBooNE Collaboration in the quasielastic sector. We analyze the mechanisms leading to the appearance of these final states and illustrate their significance through the results of accurate calculations of the nuclear electromagnetic response in the transverse channel. A novel approach, allowing for a consistent treatment of the amplitudes involving one-and two-nucleon currents in the kinematical region in which the nonrelativistic approximation breaks down, is outlined, and its preliminary results are reported. C1 [Benhar, Omar; Rocco, Noemi] Univ Roma La Sapienza, Ist Nazl Fis Nucl, I-00185 Rome, Italy. [Benhar, Omar; Rocco, Noemi] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Benhar, Omar] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. [Lovato, Alessandro] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Lovato, Alessandro] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Benhar, O (reprint author), Univ Roma La Sapienza, Ist Nazl Fis Nucl, I-00185 Rome, Italy. OI Lovato, Alessandro/0000-0002-2194-4954 FU INFN under Grant MANYBODY; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357] FX We are deeply indebted to A. M. Ankowski, J. Carlson, S. Gandolfi, C. Mariani, S. Pieper, and R. Schiavilla for many illuminating discussions. The work of O.B. and N.R. was supported by INFN under Grant MANYBODY. The work of AL was supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357. Under an award of computer time provided by the INCITE program, this research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 32 TC 8 Z9 8 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 6 PY 2015 VL 92 IS 2 AR 024602 DI 10.1103/PhysRevC.92.024602 PG 8 WC Physics, Nuclear SC Physics GA CO3IF UT WOS:000359049500002 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. 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CA CDF Collaboration TI Measurement of the top-quark mass in the t(t)over-bar dilepton channel using the full CDF Run II data set SO PHYSICAL REVIEW D LA English DT Article AB We present a measurement of the top-quark mass in events containing two leptons (electrons or muons) with a large transverse momentum, two or more energetic jets, and a transverse-momentum imbalance. We use the full proton-antiproton collision data set collected by the CDF experiment during the Fermilab Tevatron Run II at center-of-mass energy root s = 1.96 TeV, corresponding to an integrated luminosity of 9.1 fb(-1). A special observable is exploited for an optimal reduction of the dominant systematic uncertainty, associated with the knowledge of the absolute energy of the hadronic jets. The distribution of this observable in the selected events is compared to simulated distributions of t (t) over bar dilepton signal and background. 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D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Ewha Womans Univ, Seoul 120750, South Korea. [Barbaro-Galtieri, A.; Cerri, A.; Lujan, P.; Lys, J.; Potamianos, K.; Pranko, A.; Yao, W. -M.] Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [D'Onofrio, M.; Manca, G.; McNulty, R.; Mehta, A.; Shears, T.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Campanelli, M.; Cerrito, L.; Lancaster, M.; Waters, D.] UCL, London WC1E 6BT, England. [Fernandez Ramos, J. P.; Gonzalez Lopez, O.; Redondo Fernandez, I.] Ctr Invest Energet Medioambient & Tecnol, E-28040 Madrid, Spain. [Gomez-Ceballos, G.; Goncharov, M.; Paus, C.] MIT, Cambridge, MA 02139 USA. [Amidei, D.; Edgar, R.; Mietlicki, D.; Schwarz, T.; Tecchio, M.; Wilson, J. S.; Wright, T.] Univ Michigan, Ann Arbor, MI 48109 USA. [Bromberg, C.; Hussein, M.; Huston, J.; Tollefson, K.] Michigan State Univ, E Lansing, MI 48824 USA. [Shreyber-Tecker, I.] ITEP, Moscow 117259, Russia. [Gold, M.; Gorelov, I.; Palni, P.; Seidel, S.; Strologas, J.; Vogel, M.] Univ New Mexico, Albuquerque, NM 87131 USA. [Hughes, R. E.; Lannon, K.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Okayama 7008530, Japan. [Kato, Y.; Okusawa, T.; Seiya, Y.; Yamamoto, K.; Yamato, D.; Yoshida, T.] Osaka City Univ, Osaka 5588585, Japan. [Azfar, F.; Farrington, S.; Hays, C.; Oakes, L.; Renton, P.] Univ Oxford, Oxford OX1 3RH, England. [Amerio, S.; Bauce, M.; Busetto, G.; D'Errico, M.; Lucchesi, D.; Totaro, P.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Amerio, S.; Bauce, M.; Busetto, G.; D'Errico, M.; Lucchesi, D.] Univ Padua, I-35131 Padua, Italy. [Heinrich, J.; Keung, J.; Kroll, J.; Lipeles, E.; Pianori, E.; Rodriguez, T.; Thomson, E.; Wagner, P.; Whiteson, D.; Williams, H. H.] Univ Penn, Philadelphia, PA 19104 USA. [Barria, P.; Bedeschi, F.; Bellettini, G.; Butti, P.; Carosi, R.; Chiarelli, G.; Cremonesi, M.; Di Canto, A.; Donati, S.; Galloni, C.; Garosi, P.; Introzzi, G.; Latino, G.; Leone, S.; Maestro, P.; Marino, P.; Morello, M. J.; Punzi, G.; Ristori, L.; Ronzani, M.; Ruffini, F.; Scuri, F.; Sforza, F.; Trovato, M.; Vernieri, C.] Ist Nazl Fis Nucl, I-56127 Pisa, Italy. [Bellettini, G.; Butti, P.; Di Canto, A.; Donati, S.; Galloni, C.; Punzi, G.; Ronzani, M.; Sforza, F.] Univ Pisa, I-56127 Pisa, Italy. [Barria, P.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-56127 Pisa, Italy. [Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Introzzi, G.] Ist Nazl Fis Nucl, I-27100 Pavia, Italy. [Introzzi, G.] Univ Pavia, I-27100 Pavia, Italy. [Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; de Barbaro, P.; Han, J. Y.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [Giagu, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Iori, M.] Sapienza Univ Roma, I-00185 Rome, Italy. [Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA. [Casarsa, M.; Cauz, D.; Dorigo, M.; Driutti, A.; Pagliarone, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Grp Collegato Udine, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy. [Dorigo, M.] Univ Trieste, I-34127 Trieste, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Introzzi, Gianluca/K-2497-2015; Paulini, Manfred/N-7794-2014; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011 OI Brucken, Jens Erik/0000-0001-6066-8756; Introzzi, Gianluca/0000-0002-1314-2580; Paulini, Manfred/0000-0002-6714-5787; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368 FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, United Kingdom; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 29 TC 3 Z9 3 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 6 PY 2015 VL 92 IS 3 AR 032003 DI 10.1103/PhysRevD.92.032003 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO3IR UT WOS:000359050900001 ER PT J AU Tain, JL Valencia, E Algora, A Agramunt, J Rubio, B Rice, S Gelletly, W Regan, P Zakari-Issoufou, AA Fallot, M Porta, A Rissanen, J Eronen, T Aysto, J Batist, L Bowry, M Bui, VM Caballero-Folch, R Cano-Ott, D Elomaa, VV Estevez, E Farrelly, GF Garcia, AR Gomez-Hornillos, B Gorlychev, V Hakala, J Jordan, MD Jokinen, A Kolhinen, VS Kondev, FG Martinez, T Mendoza, E Moore, I Penttila, H Podolyak, Z Reponen, M Sonnenschein, V Sonzogni, AA AF Tain, J. L. Valencia, E. Algora, A. Agramunt, J. Rubio, B. Rice, S. Gelletly, W. Regan, P. Zakari-Issoufou, A. -A. Fallot, M. Porta, A. Rissanen, J. Eronen, T. Aysto, J. Batist, L. Bowry, M. Bui, V. M. Caballero-Folch, R. Cano-Ott, D. Elomaa, V. -V. Estevez, E. Farrelly, G. F. Garcia, A. R. Gomez-Hornillos, B. Gorlychev, V. Hakala, J. Jordan, M. D. Jokinen, A. Kolhinen, V. S. Kondev, F. G. Martinez, T. Mendoza, E. Moore, I. Penttila, H. Podolyak, Zs. Reponen, M. Sonnenschein, V. Sonzogni, A. A. TI Enhanced gamma-Ray Emission from Neutron Unbound States Populated in beta Decay SO PHYSICAL REVIEW LETTERS LA English DT Article ID TOTAL ABSORPTION-SPECTRA; NUCLEAR-DATA SHEETS; PENNING TRAP; SPECTROSCOPY; BR-87; PURIFICATION; COMPETITION; SIMULATION; JYFLTRAP; SCHEMES AB Total absorption spectroscopy is used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in Br-87,Br-88 and Rb-94. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large. intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For Br-87 and Br-88 the gamma branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich Rb-94 the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled by introducing an enhancement of 1 order of magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proves to be correct, leads to a similar increase in the (n, gamma) cross section that would have an impact on r process abundance calculations. C1 [Tain, J. L.; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M. D.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain. [Rice, S.; Gelletly, W.; Regan, P.; Bowry, M.; Farrelly, G. F.; Podolyak, Zs.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Zakari-Issoufou, A. -A.; Fallot, M.; Porta, A.; Bui, V. M.] Univ Nantes, Ecole Mines, CNRS IN2P3, SUBATECH, F-44307 Nantes, France. [Rissanen, J.; Eronen, T.; Elomaa, V. -V.; Hakala, J.; Jokinen, A.; Kolhinen, V. S.; Moore, I.; Penttila, H.; Reponen, M.; Sonnenschein, V.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. [Aysto, J.] Univ Helsinki, Helsinki Inst Phys, FI-00014 Helsinki, Finland. [Batist, L.] Petersburg Nucl Phys Inst, RU-188300 Gatchina, Russia. [Caballero-Folch, R.; Gomez-Hornillos, B.; Gorlychev, V.] Univ Politecn Cataluna, E-08028 Barcelona, Spain. [Cano-Ott, D.; Garcia, A. R.; Martinez, T.; Mendoza, E.] Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Sonzogni, A. A.] Brookhaven Natl Lab, NNDC, Upton, NY 11973 USA. RP Tain, JL (reprint author), Univ Valencia, CSIC, Inst Fis Corpuscular, Apdo Correos 22085, E-46071 Valencia, Spain. EM tain@ific.uv.es RI Moore, Iain/D-7255-2014; Algora, Alejandro/E-2960-2015; Mendoza Cembranos, Emilio/K-5789-2014; Martinez, Trinitario/K-6785-2014; Jokinen, Ari/C-2477-2017 OI Moore, Iain/0000-0003-0934-8727; Algora, Alejandro/0000-0002-5199-1794; Mendoza Cembranos, Emilio/0000-0002-2843-1801; Martinez, Trinitario/0000-0002-0683-5506; Jokinen, Ari/0000-0002-0451-125X FU Spanish Ministerio de Economia y Competitividad [FPA2008-06419, FPA2010-17142, FPA2011-24553]; CPAN [CSD-2007-00042]; EPSRC; STFC (UK); U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by Spanish Ministerio de Economia y Competitividad under Grants No. FPA2008-06419, No. FPA2010-17142, and No. FPA2011-24553, CPAN CSD-2007-00042 (Ingenio2010), and by EPSRC and STFC (UK). Work at ANL was supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 43 TC 10 Z9 10 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 6 PY 2015 VL 115 IS 6 AR 062502 DI 10.1103/PhysRevLett.115.062502 PG 5 WC Physics, Multidisciplinary SC Physics GA CO3LN UT WOS:000359059100002 PM 26296113 ER PT J AU Wu, Y Wang, H Cheng, YQ Liu, XJ Hui, XD Nieh, TG Wang, YD Lu, ZP AF Wu, Yuan Wang, Hui Cheng, Yongqiang Liu, Xiongjun Hui, Xidong Nieh, Taigang Wang, Yandong Lu, Zhaoping TI Inherent structure length in metallic glasses: simplicity behind complexity SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY-DIFFRACTION; SOFT-MAGNETIC PROPERTIES; ZR AMORPHOUS-ALLOYS; MEDIUM-RANGE ORDER; FORMING ABILITY; ELASTIC PROPERTIES; THERMAL-STABILITY; MECHANICAL-PROPERTIES; ELECTRONIC-STRUCTURE; ULTRAHIGH-STRENGTH AB One of the central themes in materials science is the structure-property relationship. In conventional crystalline metals, their mechanical behaviour is often dictated by well-defined structural defects such as dislocations, impurities, and twins. However, the structure-property relationship in amorphous alloys is far from being understood, due to great difficulties in characterizing and describing the disordered atomic-level structure. Herein, we report a universal, yet simple, correlation between the macroscopic mechanical properties (i.e., yield strength and shear modulus) and a unique characteristic structural length in metallic glasses (MGs). Our analysis indicates that this characteristic length can incorporate effects of both the inter-atomic distance and valence electron density in MGs, and result in the observed universal correlation. The current findings shed lights on the basic understanding of mechanical properties of MGs from their disordered atomic structures. C1 [Wu, Yuan; Wang, Hui; Liu, Xiongjun; Hui, Xidong; Wang, Yandong; Lu, Zhaoping] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Cheng, Yongqiang] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Nieh, Taigang] Univ Tennessee, Mat Sci & Engn Dept, Knoxville, TN 37919 USA. RP Lu, ZP (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. EM luzp@ustb.edu.cn RI wang, yandong/G-9404-2013; Lu, Zhao-Ping/A-2718-2009; Hui, Xidong/A-1741-2010; Wang, Hui/A-5775-2017; Liu, Xiong-Jun/C-7119-2009 OI Wang, Hui/0000-0002-4915-3396; FU National Natural Science Foundation of China [51371003, 51422101, 51271212]; International Science & Technology Cooperation Program of China, 111 Project [B07003]; Program for Changjiang Scholars and Innovative Research Team in University; Fundamental Research Funds for the Central Universities; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX This research was supported in part by National Natural Science Foundation of China ( Nos. 51371003, 51422101, 51271212), International Science & Technology Cooperation Program of China, 111 Project (B07003) and Program for Changjiang Scholars and Innovative Research Team in University. Y.W. and X.J.L. acknowledge the financial support from "the Fundamental Research Funds for the Central Universities". Y.Q.C was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Fruitful discussion with Profs. E. Ma at Johns Hopkins University, U. Ramamurty at Indian Institute of Science and Y.M. Wang at Dalian University of Technology are gratefully acknowledged. NR 105 TC 4 Z9 4 U1 11 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 6 PY 2015 VL 5 AR 12137 DI 10.1038/srep12137 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO4HS UT WOS:000359122400001 PM 26245801 ER PT J AU Dixit, H Lee, JH Krogel, JT Okamoto, S Cooper, VR AF Dixit, Hemant Lee, Jun Hee Krogel, Jaron T. Okamoto, Satoshi Cooper, Valentino R. TI Stabilization of weak ferromagnetism by strong magnetic response to epitaxial strain in multiferroic BiFeO3 SO SCIENTIFIC REPORTS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; NEUTRON-DIFFRACTION; THIN-FILMS; TEMPERATURE; SEMICONDUCTORS AB Multiferroic BiFeO3 exhibits excellent magnetoelectric coupling critical for magnetic information processing with minimal power consumption. However, the degenerate nature of the easy spin axis in the (111) plane presents roadblocks for real world applications. Here, we explore the stabilization and switchability of the weak ferromagnetic moments under applied epitaxial strain using a combination of first-principles calculations and group-theoretic analyses. We demonstrate that the antiferromagnetic moment vector can be stabilized along unique crystallographic directions ([110] and [-110]) under compressive and tensile strains. A direct coupling between the anisotropic antiferrodistortive rotations and the Dzyaloshinskii-Moria interactions drives the stabilization of the weak ferromagnetism. Furthermore, energetically competing C- and G-type magnetic orderings are observed at high compressive strains, suggesting that it may be possible to switch the weak ferromagnetism "on" and "off" under the application of strain. These findings emphasize the importance of strain and antiferrodistortive rotations as routes to enhancing induced weak ferromagnetism in multiferroic oxides. C1 [Dixit, Hemant; Lee, Jun Hee; Krogel, Jaron T.; Okamoto, Satoshi; Cooper, Valentino R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. [Krogel, Jaron T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Dixit, H (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. EM dixithm@ornl.gov; leej@ornl.gov; coopervr@ornl.gov RI Cooper, Valentino /A-2070-2012; OI Cooper, Valentino /0000-0001-6714-4410; Krogel, Jaron/0000-0002-1859-181X FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division; Office of Science Early Career Research Program; Office of Science of US Department of Energy [DE-AC02-05CH11231] FX Research supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division (J.H.L., S.O., H.D. and V.R.C.), and the Office of Science Early Career Research Program (V.R.C.). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. Research by J.T.K. (Nexus workflows) was conducted at the Center for Nanophase Materials Sciences, which is a DOE office of Science User Facility. NR 33 TC 1 Z9 1 U1 6 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 6 PY 2015 VL 5 AR 12969 DI 10.1038/srep12969 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO4JY UT WOS:000359128200001 PM 26246030 ER PT J AU Sandoval, L Urbassek, HM AF Sandoval, Luis Urbassek, Herbert M. TI Collision-spike Sputtering of Au Nanoparticles SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Molecular dynamics; Sputtering; Nanoparticles; Clusters AB Ion irradiation of nanoparticles leads to enhanced sputter yields if the nanoparticle size is of the order of the ion penetration depth. While this feature is reasonably well understood for collision-cascade sputtering, we explore it in the regime of collision-spike sputtering using molecular-dynamics simulation. For the particular case of 200-keV Xe bombardment of Au particles, we show that collision spikes lead to abundant sputtering with an average yield of 397 +/- 121 atoms compared to only 116 +/- 48 atoms for a bulk Au target. Only around 31% of the impact energy remains in the nanoparticles after impact; the remainder is transported away by the transmitted projectile and the ejecta. The sputter yield of supported nanoparticles is estimated to be around 80% of that of free nanoparticles due to the suppression of forward sputtering. C1 [Sandoval, Luis] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Urbassek, Herbert M.] Univ Kaiserslautern, Dept Phys, Erwin Schrodinger Str, D-67663 Kaiserslautern, Germany. [Urbassek, Herbert M.] Univ Kaiserslautern, Res Ctr OPTIMAS, Erwin Schrodinger Str, D-67663 Kaiserslautern, Germany. RP Urbassek, HM (reprint author), Univ Kaiserslautern, Dept Phys, Erwin Schrodinger Str, D-67663 Kaiserslautern, Germany.; Urbassek, HM (reprint author), Univ Kaiserslautern, Res Ctr OPTIMAS, Erwin Schrodinger Str, D-67663 Kaiserslautern, Germany. EM urbassek@rhrk.uni-kl.de FU US Department of Energy by Lawrence Livermore National Laboratory; U.S. DOE [DE-AC52-07NA27344, DE-AC52-O6NA25396]; US Department of Energy by Los Alamos National Laboratory FX Discussions with P. Ziemann are gratefully acknowledged. Part of the simulations were performed at the High Performance Cluster Elwetritsch (RHRK, TU Kaiserslautern, Germany). This work was partially performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory and Los Alamos National Laboratory. LLNL is operated by Lawrence Livermore National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE, under contract DE-AC52-07NA27344. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE, under contract DE-AC52-O6NA25396. NR 40 TC 5 Z9 5 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD AUG 6 PY 2015 VL 10 AR 314 DI 10.1186/s11671-015-1009-x PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA V46ED UT WOS:000209866600001 ER PT J AU Yassin, AF Lapidus, A Han, J Reddy, TBK Huntemann, M Pati, A Ivanova, N Markowitz, V Woyke, T Klenk, HP Kyrpides, NC AF Yassin, Atteyet F. Lapidus, Alla Han, James Reddy, T. B. K. Huntemann, Marcel Pati, Amrita Ivanova, Natalia Markowitz, Victor Woyke, Tanja Klenk, Hans-Peter Kyrpides, Nikos C. TI High quality draft genome sequence of Corynebacterium ulceribovis type strain IMMIB-L1395(T) (DSM 45146(T)) SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Gram-positive; Bovine skin; Corynebacteriaceae; Actinobacteria; GEBA ID MYCOBACTERIUM-TUBERCULOSIS H37RV; MYCOLIC ACID BIOSYNTHESIS; ESCHERICHIA-COLI; FATTY-ACID; ACTINOBACILLUS-ACTINOMYCETEMCOMITANS; PHOSPHATIDYLINOSITOL MANNOSIDES; TAXONOMIC IMPLICATIONS; CLASSIFICATION-SYSTEM; SOLUTE TRANSPORTERS; TREHALOSE SYNTHASE AB Corynebacterium ulceribovis strain IMMIB L-1395(T) (= DSM 45146(T)) is an aerobic to facultative anaerobic, Gram-positive, non-spore-forming, non-motile rod-shaped bacterium that was isolated from the skin of the udder of a cow, in Schleswig Holstein, Germany. The cell wall of C. ulceribovis contains corynemycolic acids. The cellular fatty acids are those described for the genus Corynebacterium, but tuberculostearic acid is not present. Here we describe the features of C. ulceribovis strain IMMIB L-1395(T), together with genome sequence information and its annotation. The 2,300,451 bp long genome containing 2,104 protein-coding genes and 54 RNA-encoding genes and is part of the Genomic Encyclopedia of Type Strains, Phase I: the one thousand microbial genomes (KMG) project. C1 [Yassin, Atteyet F.] Univ Bonn, Inst Med Mikrobiol & Immunol, Bonn, Germany. [Lapidus, Alla] St Petersburg State Univ, Theodosius Dobzhansky Ctr Genome Bioinformat, St Petersburg 199034, Russia. [Lapidus, Alla] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg, Russia. [Han, James; Reddy, T. B. K.; Huntemann, Marcel; Pati, Amrita; Ivanova, Natalia; Woyke, Tanja; Kyrpides, Nikos C.] US DOE, Joint Genome Inst, Genome Biol Program, Washington, DC 20585 USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Klenk, Hans-Peter] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah, Saudi Arabia. RP Yassin, AF (reprint author), Univ Bonn, Inst Med Mikrobiol & Immunol, Bonn, Germany. EM yassin@mibi03.meb.uni-bonn.de RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Lapidus, Alla/I-4348-2013; Faculty of, Sciences, KAU/E-7305-2017 OI Kyrpides, Nikos/0000-0002-6131-0462; Lapidus, Alla/0000-0003-0427-8731; Ivanova, Natalia/0000-0002-5802-9485; FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Russian Ministry of Science [11.G34.31.0068] FX The authors gratefully acknowledge the help of Gabriele Potter for growing cells of DSM 30083T and of Evelyne-Marie Brambilla for DNA extraction and quality control (both at DSMZ). This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231. A.L. was supported in part by Russian Ministry of Science Mega-grant no. 11.G34.31.0068 (PI. Dr Stephen J O'Brien). NR 128 TC 0 Z9 0 U1 1 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 5 PY 2015 VL 10 AR 50 DI 10.1186/s40793-015-0036-7 PG 20 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NU UT WOS:000367991800002 PM 26380638 ER PT J AU Smith, MW Shekhawat, D Berry, DA Haynes, DJ Floyd, DL Spivey, JJ Ranasingha, O AF Smith, Mark W. Shekhawat, Dushyant Berry, David A. Haynes, Daniel J. Floyd, Donald L. Spivey, James J. Ranasingha, Oshadha TI Carbon formation on Rh-substituted pyrochlore catalysts during partial oxidation of liquid hydrocarbons SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Catalytic partial oxidation; Liquid hydrocarbon fuel; Pyrochlore catalyst; Carbon deposition; Temperature programmed oxidation ID N-TETRADECANE; SYNTHESIS GAS; REFORMING CATALYSTS; METHANE; DEACTIVATION; PEROVSKITE; SULFUR; METAL; DEPOSITION; PERFORMANCE AB Rh-substituted pyrochlore catalysts were prepared and tested for the partial oxidation (PDX) of n-tetradecane (TD), a diesel fuel surrogate. The catalysts were substituted lanthanum zirconates with the chemical formula La1.89Ca0.11Zr1.75-xRhxY0.25O7-y (with either 0, 1, 2, or 3 wt% of Rh loading). The catalysts underwent a variety of pre- and post-reaction characterization with a focus on deposited carbon, the primary cause of catalyst deactivation. To assess the nature of potential catalytic sites (typically attributed to Rh), each substituted catalyst produced three temperature programmed reduction peaks, with an increase in the most reducible sites at higher Rh loadings. In additions, the catalysts with 2 and 3 wt% Rh substitution displayed a secondary crystal phase in their XRD spectra; however, this phase disappeared when the sample was reduced up to 900 degrees C, representative of reaction conditions. To assess carbbn deposition after reaction testing, a temperature programmed oxidation (TPO) was conducted on each sample from 250 to 750 degrees C. Each sample produced three CO2 peaks between 250 and 550 degrees C, referred to as low temperature carbon (LTC) peaks, and two peaks at higher temperatures (>600 degrees C). The 2 wt% catalyst was run for different times under PDX of TD, and the TPO results showed that the amount of LTC reached a steady state within 2 h and did not increase even up to 18 h under reaction conditions. This indicates that the LTC is not likely responsible for catalyst deactivation. In contrast, the quantity of carbon associated with the higher temperature peaks under TPO increased with reaction time. The carbon associated with the high temperature peaks was highly graphitic, and is typically attributed to deposits on the catalyst inert surfaces and/or inert bed material. After a partial burn-off of the LTC, Raman analysis showed no significant change in the surface carbon. These results suggest that improvement in catalyst performance may be accomplished by modification of the catalyst formulation to increase the resistance to carbon formation on the oxide surface. Such modifications include surface promoters, B-site dopant level, and addition of an oxygen-conducting support. Future work will explore these approaches. (C) 2015 Elsevier B.V. All rights reserved. C1 [Smith, Mark W.; Shekhawat, Dushyant; Berry, David A.; Haynes, Daniel J.; Floyd, Donald L.; Ranasingha, Oshadha] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Smith, Mark W.; Floyd, Donald L.] AECOM, Morgantown, WV 26507 USA. [Smith, Mark W.; Ranasingha, Oshadha] W Virginia Univ, Morgantown, WV 26506 USA. [Spivey, James J.] Louisiana State Univ, Baton Rouge, LA 70803 USA. RP Smith, MW (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM mark.smith@contr.netl.doe.gov FU National Energy Technology Laboratory's [DE-FE0004000]; Pyrochem Catalyst Co.; NETL FX This work was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. This work was also supported by Pyrochem Catalyst Co. through a Cooperative Research and Development Agreement with NETL. The authors would also like to thank Dr. Devendra Pakhare for his help with data deconvolution. NR 42 TC 2 Z9 2 U1 3 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD AUG 5 PY 2015 VL 502 BP 96 EP 104 DI 10.1016/j.apcata.2015.05.019 PG 9 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA CR2LU UT WOS:000361162200012 ER PT J AU Campbell, J Van Landingham, C Crowell, S Gentry, R Kaden, D Fiebelkorn, S Loccisano, A Clewell, H AF Campbell, Jerry Van Landingham, Cynthia Crowell, Susan Gentry, Robinan Kaden, Debra Fiebelkorn, Stacy Loccisano, Anne Clewell, Harvey TI A preliminary regional PBPK model of lung metabolism for improving species dependent descriptions of 1,3-butadiene and its metabolites SO CHEMICO-BIOLOGICAL INTERACTIONS LA English DT Article DE 1,3-Butadiene; Physiologically - based pharmacokinetic model; PBPK; Lung metabolism ID HUMAN LIVER-MICROSOMES; TOXICOKINETIC MODEL; IN-VITRO; PHARMACOKINETIC MODEL; BUTADIENE MONOXIDE; RESPIRATORY-TRACT; CLARA CELL; INHALATION PHARMACOKINETICS; BLOOD-CONCENTRATIONS; VINYL-ACETATE AB 1,3-Butadiene (BD), a volatile organic chemical (VOC), is used in synthetic rubber production and other industrial processes. It is detectable at low levels in ambient air as well as in tobacco smoke and gasoline vapors. Inhalation exposures to high concentrations of BD have been associated with lung cancer in both humans and experimental animals, although differences in species sensitivity have been observed. Metabolically active lung cells such as Pulmonary Type I and Type II epithelial cells and club cells (Clara cells)1 are potential targets of BD metabolite-induced toxicity. Metabolic capacities of these cells, their regional densities, and distributions vary throughout the respiratory tract as well as between species and cell types. Here we present a physiologically based pharmacoldnetic (PBPK) model for BD that includes a regional model of lung metabolism, based on a previous model for styrene, to provide species-dependent descriptions of BD metabolism in the mouse, rat, and human. Since there are no in vivo data on BD pharmacokinetics in the human, the rat and mouse models were parameterized to the extent possible on the basis of in vitro metabolic data. Where it was necessary to use in vivo data, extrapolation from rat to mouse was performed to evaluate the level of uncertainty in the human model. A kidney compartment and description of downstream metabolism were also included in the model to allow for eventual use of available urinary and blood biomarker data in animals and humans to calibrate the model for estimation of BD exposures and internal metabolite levels. Results from simulated inhalation exposures to BD indicate that incorporation of differential lung region metabolism is important in describing species differences in pulmonary response and that these differences may have implications for risk assessments of human exposures to BD. (C) 2015 The Authors. Published by Elsevier Ireland Ltd. C1 [Campbell, Jerry; Clewell, Harvey] Hamner Inst Hlth Res, Res Triangle Pk, NC USA. [Van Landingham, Cynthia; Gentry, Robinan; Clewell, Harvey] Ramboll Environ, Monroe, LA 71201 USA. [Crowell, Susan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kaden, Debra] Ramboll Environ, Boston, MA 02110 USA. [Fiebelkorn, Stacy] British Amer Tobacco Investments Ltd, Res & Dev, Southampton SO15 8TL, Hants, England. [Loccisano, Anne] RJ Reynolds Tobacco Co, Winston Salem, NC 27102 USA. RP Van Landingham, C (reprint author), Ramboll Environ, 1900 N 18th St,Suite 804, Monroe, LA 71201 USA. EM jcampbell@thehamner.org; cvanlandingham@environcorp.com; susan.r.crowell@gmail.com; rgentry@environcorp.com; dkaden@environcorp.com; Stacy_Fiebelkorn@bat.com; loccisa@rjrt.com; hclewell@environcorp.com FU British American Tobacco (Investments) Ltd; RJ Reynolds Tobacco Company FX The authors with the exception of Dr. Crowell are either employees of British American Tobacco or RJ Reynolds Tobacco Company, or are contractors to the aforementioned companies. All work was funded by British American Tobacco (Investments) Ltd and RJ Reynolds Tobacco Company. The Authors declare that no financial or personal conflicts of interest exist with regard to the submission of this manuscript. NR 66 TC 1 Z9 1 U1 2 U2 6 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0009-2797 EI 1872-7786 J9 CHEM-BIOL INTERACT JI Chem.-Biol. Interact. PD AUG 5 PY 2015 VL 238 BP 102 EP 110 DI 10.1016/j.cbi.2015.05.025 PG 9 WC Biochemistry & Molecular Biology; Pharmacology & Pharmacy; Toxicology SC Biochemistry & Molecular Biology; Pharmacology & Pharmacy; Toxicology GA CP5WZ UT WOS:000359957400014 PM 26079054 ER PT J AU Guo, ZP Takeuchi, E AF Guo, Zaiping Takeuchi, Esther TI Best Practices for Reporting on Energy Storage SO ACS APPLIED MATERIALS & INTERFACES LA English DT Editorial Material ID LITHIUM ION BATTERIES C1 [Takeuchi, Esther] SUNY Stony Brook, Stony Brook, NY USA. [Takeuchi, Esther] Brookhaven Natl Lab, Upton, NY 11973 USA. NR 12 TC 1 Z9 1 U1 3 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 5 PY 2015 VL 7 IS 30 BP 16131 EP 16132 DI 10.1021/acsami.5b06029 PG 2 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CO6PY UT WOS:000359279800001 PM 26242201 ER PT J AU Avila, JR Kim, DW Rimoldi, M Farha, OK Hupp, JT AF Avila, Jason R. Kim, Dong Wook Rimoldi, Martino Farha, Omar K. Hupp, Joseph T. TI Fabrication of Thin Films of alpha-Fe2O3 via Atomic Layer Deposition Using Iron Bisamidinate and Water under Mild Growth Conditions SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE atomic layer deposition; quartz crystal microbalance; in situ; iron oxide; hematite; iron bisamidinate ID OXIDE; HEMATITE; OXIDATION; TEMPERATURE; NANOPARTICLES; FERROCENE; OXYGEN; TIME AB Atomic layer deposition (ALD) has been shown to be an excellent Method for depositing thin films, of iron oxide. With limited iron precursors available; the methods widely used require harsh Conditions such as high temperatures and/or the use of oxidants such as ozone Or peroxide. This letter aims to show that bis(N,N'-di-t-butylacetamidinato) iron(II) (iron bisamidinate or FeAMD) is an ideal ALD precursor because of it'S reactivity with water and relative,volatility. Using, in situ QCM,analysis, we show outstanding conformal self-limiting growth of FeOx using FeAMD and water at temperatures lower than 200 degrees C. By annealing thin films of FeOx at 500 degrees C, we observe the formation of alpha-Fe2O3, confirming that we can Use FeAMD to fabricate thin films of catalytically promising iron oxide materials using moderate growth conditions. C1 [Avila, Jason R.; Kim, Dong Wook; Rimoldi, Martino; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah, Saudi Arabia. [Avila, Jason R.; Kim, Dong Wook; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, Evanston, IL 60208 USA. [Hupp, Joseph T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Farha, OK (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM o-farha@northwestern.edu; j-hupp@northwestern.edu RI Faculty of, Sciences, KAU/E-7305-2017 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; MRSEC program of the National Science Foundation at the Materials Research Center of Northwestern University [DMR-1121262]; Swiss National Science Foundation; Early Postdoc Mobility Fellowship; NSF-NSEC; NSF-MRSEC; KECK Foundation; State of Illinois; Northwestern University FX This work was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001059. Ellipsometry, XPS, and Raman spectroscopy was performed in KECK II facilities of the NUANCE Center at Northwestern University. The NUANCE center is supported by NSF-NSEC, NSF-MRSEC, the KECK Foundation, the State of Illinois, and Northwestern University. This work made use of the J.B.Cohen X-ray Diffraction Facility supported by the MRSEC program of the National Science Foundation (DMR-1121262) at the Materials Research Center of Northwestern University. M.R. was supported by the Swiss National Science Foundation with an Early Postdoc Mobility Fellowship. NR 28 TC 5 Z9 5 U1 8 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 5 PY 2015 VL 7 IS 30 BP 16138 EP 16142 DI 10.1021/acsami.5b04043 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CO6PY UT WOS:000359279800003 PM 26192606 ER PT J AU Duncan, DA Kephart, JM Horsley, K Blum, M Mezher, M Weinhardt, L Haming, M Wilks, RG Hofmann, T Yang, WL Bar, M Sampath, WS Heske, C AF Duncan, Douglas A. Kephart, Jason M. Horsley, Kimberly Blum, Monika Mezher, Michelle Weinhardt, Lothar Haeming, Marc Wilks, Regan G. Hofmann, Timo Yang, Wanli Baer, Marcus Sampath, Walajabad S. Heske, Clemens TI Characterization of Sulfur Bonding in CdS:O Buffer Layers for CdTe-based Thin-Film Solar Cells SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE solar cells; CdS; CdTe; alternative buffer layers; XPS AB On the basis of a combination of X-ray photoelectron spectroscopy and synchrotron-based X-ray emission spectroscopy, we present a detailed characterization of the chemical structure of CdS:O thin films that can be employed as a substitute for CdS layers in thin-film solar cells. It is possible to analyze the local chemical environment of the probed elements, in particular sulfur, hence allowing insights into the species-specific composition of the films and their surfaces. A detailed quantification of the observed sulfur environments (i.e., sulfide, sulfate, and an intermediate oxide) as a function of oxygen content is presented, allowing a deliberate optimization of CdS:O thin films for their use as alternative buffer layers in thin-film photovoltaic devices. C1 [Duncan, Douglas A.; Horsley, Kimberly; Blum, Monika; Mezher, Michelle; Weinhardt, Lothar; Haeming, Marc; Hofmann, Timo; Baer, Marcus; Heske, Clemens] Univ Nevada, Dept Chem & Biochem, Las Vegas, NV 89154 USA. [Duncan, Douglas A.; Wilks, Regan G.; Baer, Marcus] Helmholtz Zentrum Berlin Mat & Energie GmbH, Renewable Energy, D-14109 Berlin, Germany. [Kephart, Jason M.; Sampath, Walajabad S.] Colorado State Univ, Dept Mech Engn, Ft Collins, CO 80523 USA. [Blum, Monika; Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Weinhardt, Lothar; Heske, Clemens] Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, D-76344 Eggenstein Leopoldshafen, Germany. [Weinhardt, Lothar; Haeming, Marc; Heske, Clemens] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat, D-76344 Eggenstein Leopoldshafen, Germany. [Weinhardt, Lothar; Heske, Clemens] Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem, D-76128 Karlsruhe, Germany. [Baer, Marcus] Brandenburg Tech Univ Cottbus Senftenberg, Inst Chem & Phys, D-03046 Cottbus, Germany. RP Duncan, DA (reprint author), Univ Nevada, Dept Chem & Biochem, Las Vegas, NV 89154 USA. EM Hanksd5@unlv.nevada.edu; Heske@unlv.nevada.edu RI Yang, Wanli/D-7183-2011 OI Yang, Wanli/0000-0003-0666-8063 FU NSF Accelerated Innovation Research program at Colorado State University [11P-1127362]; DAAD RISE Professional program; Department of Energy, Basic Energy Sciences [DE-ACo2-05CD11231]; Helmholtz-Association [VH-NG-423] FX This work was supported by the NSF Accelerated Innovation Research program at Colorado State University, award number 11P-1127362. D. A. Duncan (ne Hanks) gratefully acknowledges financial support through the DAAD RISE Professional program. The ALS is supported by the Department of Energy, Basic Energy Sciences, Contract No. DE-ACo2-05CD11231. R. G. Wilks and M. Bar are grateful to the Helmholtz-Association for financial support (VH-NG-423). NR 28 TC 7 Z9 7 U1 4 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 5 PY 2015 VL 7 IS 30 BP 16382 EP 16386 DI 10.1021/acsami.5b03503 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CO6PY UT WOS:000359279800032 PM 26200260 ER PT J AU McCree-Grey, J Cole, JM Evans, PJ AF McCree-Grey, Jonathan Cole, Jacqueline M. Evans, Peter J. TI Preferred Molecular Orientation of Coumarin 343 on TiO2 Surfaces: Application to Dye-Sensitized Solar Cells SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE reflectometry; dye-sensitized solar cells; Coumarin 343; molecular orientation ID OPTOELECTRONIC PROPERTIES; PHOTOVOLTAIC PERFORMANCE; ORGANIC-DYES; DESIGN RULES; ORIGINS; FILMS; RAMAN; SPECTROSCOPY; AGGREGATION; ADSORPTION AB The dye...TiO2 interfacial structure in working electrodes of dye-sensitized solar cells (DSCs) is known to influence its photovoltaic device performance. Despite this, direct and quantitative reports of such structure remain sparse. This case study presents the application of X-ray reflectometry to determine the preferred structural orientation and molecular packing of the organic dye, Coumarin 343, adsorbed onto amorphous TiO2. Results show that the dye molecules are, on average, tilted by 61.1 degrees relative to the TiO2 surface, and are separated from each other by 8.2 angstrom. These findings emulate the molecular packing arrangement of a monolayer of Coumarin 343 within its crystal structure. This suggests that the dye adsorbs onto TiO2 in one of its lowest energy configurations; that is, dye...TiO2 self-assembly is driven more by thermodynamic rather than kinetic means. Complementary DSC device tests illustrate that this interfacial structure compromises photovoltaic performance, unless a suitably sized coadsorbant is interdispersed between the Coumarin 343 chromophores on the TiO2 surface. C1 [McCree-Grey, Jonathan; Cole, Jacqueline M.] Univ Cambridge, Dept Phys, Cavendish Lab, Cambridge CB3 0HE, England. [McCree-Grey, Jonathan; Evans, Peter J.] Australian Nucl Sci & Technol Org, Lucas Heights, NSW 2234, Australia. [Cole, Jacqueline M.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cole, JM (reprint author), Univ Cambridge, Dept Phys, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England. EM jmc61@cam.ac.uk RI Cole, Jacqueline/C-5991-2008 FU ANSTO; 1851 Royal Commission; DOE Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We wish to thank Stephen Holt from ANSTO for induction on X-ray reflectometry instrumentation at OPAL, and also Andrew Nelson and Gerry Triani for their guidance on data analysis and TiO2 deposition, respectively. J.M-G. acknowledges ANSTO for a part-funded Ph.D. studentship. J.M.C. is grateful to the 1851 Royal Commission for the 2014 Design Fellowship, and Argonne National Laboratory where work done was supported by DOE Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 37 TC 3 Z9 3 U1 7 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 5 PY 2015 VL 7 IS 30 BP 16404 EP 16409 DI 10.1021/acsami.5b03572 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CO6PY UT WOS:000359279800035 PM 26159229 ER PT J AU Lukatskaya, MR Bak, SM Yu, XQ Yang, XQ Barsoum, MW Gogotsi, Y AF Lukatskaya, Maria R. Bak, Seong-Min Yu, Xiqian Yang, Xiao-Qing Barsoum, Michel W. Gogotsi, Yury TI Probing the Mechanism of High Capacitance in 2D Titanium Carbide Using In Situ X-Ray Absorption Spectroscopy SO ADVANCED ENERGY MATERIALS LA English DT Article DE capacitance; carbide; MXene; pseudocapacitance; X-ray absorption spectroscopy (XAS) ID HIGH VOLUMETRIC CAPACITANCE; ELECTROCHEMICAL CAPACITORS; SUPERCAPACITOR APPLICATIONS; MANGANESE OXIDE; THIN-FILMS; STORAGE; BATTERIES; RELEVANCE; MXENE C1 [Lukatskaya, Maria R.; Barsoum, Michel W.; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Lukatskaya, Maria R.; Barsoum, Michel W.; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Bak, Seong-Min; Yu, Xiqian; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Gogotsi, Y (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. EM xyang@bnl.gov; gogotsi@drexel.edu RI Lukatskaya, Maria/A-8118-2012; Yu, Xiqian/B-5574-2014; Bak, Seong Min/J-4597-2013; OI Yu, Xiqian/0000-0001-8513-518X; Bak, Seong-Min/0000-0002-1626-5949 FU Office of Electricity Delivery and Energy Reliability, Energy Storage Systems Program, through Sandia National Laboratories; Assistant Secretary for the Energy Efficiency and Renewable Energy Office, Vehicle Technologies, of the U.S. Department of Energy (DOE) [DE-SC0012704] FX M.R.L. and S.-M.B. contributed equally to this work. The authors thank Michael Ghidiu for help with material synthesis and Sankalp Kota for suggestions on the paper improvement. The work performed at Drexel University was supported by the Office of Electricity Delivery and Energy Reliability, Energy Storage Systems Program, through Sandia National Laboratories. The XANES work performed at Brookhaven National Laboratory was supported by the Assistant Secretary for the Energy Efficiency and Renewable Energy Office, Vehicle Technologies, of the U.S. Department of Energy (DOE), under Contract No. DE-SC0012704. The authors acknowledge technical supports by the scientists at beamline X18A and X19A at NSLS (BNL) and beamline 9-BM-B at APS (ANL). NR 26 TC 30 Z9 30 U1 36 U2 185 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 5 PY 2015 VL 5 IS 15 AR 1500589 DI 10.1002/aenm.201500589 PG 4 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CO7WT UT WOS:000359374900012 ER PT J AU Brown, JL Batista, ER Boncella, JM Gaunt, AJ Reilly, SD Scott, BL Tomson, NC AF Brown, Jessie L. Batista, Enrique R. Boncella, James M. Gaunt, Andrew J. Reilly, Sean D. Scott, Brian L. Tomson, Neil C. TI A Linear trans-Bis(imido) Neptunium(V) Actinyl Analog: Np-V(NDipp)(2)((t)Bu(2)bipy)(2)Cl (Dipp=2,6-(Pr2C6H3)-Pr-i) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID STARTING MATERIALS; URANYL-ION; COMPLEXES; CHEMISTRY; REACTIVITY; LIGAND AB The discovery that imido analogs Of actinyl dioxo cations can be extended beyond uranium into the transuranic elements is presented. Synthesis of the Np(V) Complex, Np(NDipp)(2)(tBu(2)bipy)(2)Cl (1), is achieved through treatment of a Np (IV) precursor with a bipyridine coligand and lithium-amide reagent. Complex 1 has been structurally characterized, analyzed by H-1 NMR and UV-vis-NIR spectroscopies, and the electronic structure evaluated by DFT calculations. C1 [Brown, Jessie L.; Boncella, James M.; Gaunt, Andrew J.; Reilly, Sean D.; Tomson, Neil C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Batista, Enrique R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Batista, ER (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM erb@lanl.gov; gaunt@lanl.gov RI Tomson, Neil/R-6686-2016; Scott, Brian/D-8995-2017 OI Tomson, Neil/0000-0001-9131-1039; Scott, Brian/0000-0003-0468-5396 FU Heavy Element Chemistry Program of the Office of Basic Energy Sciences of the U.S. Department of Energy; National Nuclear Security Administration of the Department of Energy [DE-AC52-06NA25396] FX The neptunium chemistry and characterization was performed under a U.S. Department of Energy, Office of Science, Basic Energy Sciences, Early Career Research Program award. The Heavy Element Chemistry Program of the Office of Basic Energy Sciences of the U.S. Department of Energy funded J.M.B and E.R.B. Los Alamos National Security, LLC, operates Los Alamos National Laboratory for the National Nuclear Security Administration of the Department of Energy under contract DE-AC52-06NA25396. NR 27 TC 3 Z9 3 U1 4 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 5 PY 2015 VL 137 IS 30 BP 9583 EP 9586 DI 10.1021/jacs.5b06667 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CO6PV UT WOS:000359279500021 PM 26200434 ER PT J AU Chen, L Yang, JH Klaus, S Lee, LJ Woods-Robinson, R Ma, J Lum, Y Cooper, JK Toma, FM Wang, LW Sharp, ID Bell, AT Ager, JW AF Chen, Le Yang, Jinhui Klaus, Shannon Lee, Lyman J. Woods-Robinson, Rachel Ma, Jie Lum, Yanwei Cooper, Jason K. Toma, Francesca M. Wang, Lin-Wang Sharp, Ian D. Bell, Alexis T. Ager, Joel W. TI p-Type Transparent Conducting Oxide/n-Type Semiconductor Heterojunctions for Efficient and Stable Solar Water Oxidation SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SILICON PHOTOANODES; ELECTROCHEMICAL EVOLUTION; HYDROGEN-PRODUCTION; RAMAN-SPECTROSCOPY; ION BATTERIES; THIN-FILMS; ELECTRODES; LAYER; PERFORMANCE; OXYGEN AB Achieving stable operation of photoanodes used as components of solar water splitting devices is critical to realizing the promise of this renewable energy technology. It is shown that p-type transparent conducting oxides (p-TCOs) can function both as a selective hole contact and corrosion protection layer for photoanodes used in light-driven water oxidation. Using NiCo2O4 as the p-TCO and n-type Si as a prototypical light absorber, a rectifying heterojunction capable of light driven water oxidation was created. By placing the charge separating junction in the Si using a np(+) structure and by incorporating a highly active heterogeneous Ni-Fe oxygen evolution catalyst, efficient light-driven water oxidation can be achieved. In this structure, oxygen evolution under AM1.5G illumination occurs at 0.95 V vs RHE, and the current density at the reversible potential for water oxidation (1.23 V vs RHE) is >25 mA cm(-2). Stable operation was confirmed by observing a constant current density over 72 h and by sensitive measurements of corrosion products in the electrolyte. In situ Raman spectroscopy was employed to investigate structural transformation of NiCo2O4 during electrochemical oxidation. The interface between the light absorber and p-TCO is crucial to produce selective hole conduction to the surface under illumination. For example, annealing to produce more crystalline NiCo2O4 produces only small changes in its hole conductivity, while a thicker SiOx layer is formed at the n-Si/p-NiCo2O4 interface, greatly reducing the PEC performance. The generality of the p-TCO protection approach is demonstrated by multihour, stable, water oxidation with n-InP/p-NiCo2O4 heterojunction photoanodes. C1 [Chen, Le; Yang, Jinhui; Klaus, Shannon; Lee, Lyman J.; Ma, Jie; Lum, Yanwei; Cooper, Jason K.; Toma, Francesca M.; Wang, Lin-Wang; Sharp, Ian D.; Bell, Alexis T.; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Chen, Le; Yang, Jinhui; Lee, Lyman J.; Woods-Robinson, Rachel; Ma, Jie; Wang, Lin-Wang; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Toma, Francesca M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Klaus, Shannon; Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Lum, Yanwei; Cooper, Jason K.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Ager, JW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM JWAger@lbl.gov RI Foundry, Molecular/G-9968-2014; OI Woods-Robinson, Rachel/0000-0001-5009-9510; Bell, Alexis/0000-0002-5738-4645 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Bay Area Photovoltaic Consortium; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH1123] FX We thank Raffaella Buonsanti for assistance with SEM imaging, Karl Walczak and Jeffery Beeman for Faradaic efficiency measurements and for processing np-Si wafers, and Prof. All Javey's group for providing n-InP wafers. We thank NCEM staff Marissa Libbee and Chengyu Song for generous help on TEM sample preparation and imaging. This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under award no. DE-SC0004993. Characterization work by R.W.R. was supported by the Bay Area Photovoltaic Consortium. Work at the National Center for Electron Microscopy and Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH1123. NR 60 TC 22 Z9 22 U1 29 U2 193 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 5 PY 2015 VL 137 IS 30 BP 9595 EP 9603 DI 10.1021/jacs.5b03536 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CO6PV UT WOS:000359279500023 PM 26161845 ER PT J AU Bauers, SR Wood, SR Jensen, KMO Blichfeld, AB Iversen, BB Billinge, SJL Johnson, DC AF Bauers, Sage R. Wood, Suzannah R. Jensen, Kirsten M. O. Blichfeld, Anders B. Iversen, Bo B. Billinge, Simon J. L. Johnson, David C. TI Structural Evolution of Iron Antimonides from Amorphous Precursors to Crystalline Products Studied by Total Scattering Techniques SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MODULATED ELEMENTAL REACTANTS; IN-SITU; REACTION-MECHANISM; MARCASITE; PYRITE; ARSENOPYRITE; COMPOUND; DESIGN; GROWTH; ENERGY AB Homogeneous reaction precursors may be used to form several solid-state compounds inaccessible by traditional synthetic routes, but there has been little development of techniques that allow for a priori prediction of what may crystallize in a given material system. Here, the local structures Of FeSbx designed precursors are determined and compared with the Structural Motifs of their crystalline products. X-ray total scattering and atomic pair distribution function (PDF) analysis are used to show that precursors that first nucleate a metastable FeSb3 compound share similar local structure to the product. Interestingly, precursors that directly crystallize to thermodynamically stable FeSb2 products also contain local structural motifs of the metastable phase, despite their compositional disagreement. While both crystalline phases consist of distorted FeSb6 octahedra with Sb shared between either two or three octahedra as required for stoichiometry; a corner-sharing arrangement: indicative of AX(3)-type structures is the only motif apparent in the PDF Of either precursor. Prior Speculation was that local: composition controlled which compounds nucleate from amorphous intermediates, with different compositions favoring different local arrangements and hence different products. This data suggests that local environments in these amorphous intermediates May not be very sensitive to overall composition. This can provide insight into potential metastable phases which may form in a material system, even with a precursor that does not crystallize to the kinetically stabilized product: Determination of local structure in homogeneous amorphous reaction intermediates from techniques such as PDF can be a valuable asset in the development of systematic methods to prepare targeted solid-state compounds from designed precursors. C1 [Bauers, Sage R.; Wood, Suzannah R.; Johnson, David C.] Univ Oregon, Dept Chem, Eugene, OR 97403 USA. [Bauers, Sage R.; Wood, Suzannah R.; Johnson, David C.] Univ Oregon, Inst Mat Sci, Eugene, OR 97403 USA. [Jensen, Kirsten M. O.; Billinge, Simon J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Blichfeld, Anders B.; Iversen, Bo B.] Aarhus Univ, Dept Chem, Ctr Mat Crystallog, DK-8000 Aarhus C, Denmark. [Blichfeld, Anders B.; Iversen, Bo B.] Aarhus Univ, iNANO, DK-8000 Aarhus C, Denmark. [Billinge, Simon J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Johnson, DC (reprint author), Univ Oregon, Dept Chem, Eugene, OR 97403 USA. EM davej@uoregon.edu RI Jensen, Kirsten Marie Ornsbj/I-9367-2012; Blichfeld, Anders/G-4418-2016; Wood, Suzannah/H-8917-2016 OI Jensen, Kirsten Marie Ornsbj/0000-0003-0291-217X; Blichfeld, Anders/0000-0001-5631-4197; Wood, Suzannah/0000-0002-7208-7681 FU National Science Foundation [DMR-1266217]; National Science Foundation through CCI grant [CHE-1102637]; Danish National Research Foundation (Center for Materials Crystallography) [DNRF93]; Sino-Danish Center; Villum Foundation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES) [DE-SC00112704]; DOE-BES [DE-AC02-98CH10886] FX The authors acknowledge support from the National Science Foundation under grant DMR-1266217. S.B. and S.W. were supported by the National Science Foundation through CCI grant no. CHE-1102637. B.B.I. was supported in part by the Danish National Research Foundation (Center for Materials Crystallography, DNRF93). A.B. would like to acknowledge the Sino-Danish Center for funding. K.J. is grateful for funding from the Villum Foundation, and work in the Billinge group was supported by U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES) under contract DE-SC00112704. The authors thank Milinda Abeykoon for assistance at Beam line X17A at the National Synchrotron Light Source, Brookhaven National Laboratory. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the DOE-BES, under contract no. DE-AC02-98CH10886. NR 41 TC 7 Z9 7 U1 4 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 5 PY 2015 VL 137 IS 30 BP 9652 EP 9658 DI 10.1021/jacs.5b04838 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CO6PV UT WOS:000359279500029 PM 26161946 ER PT J AU Mara, MW Bowman, DN Buyukcakir, O Shelby, ML Haldrup, K Huang, J Harpham, MR Stickrath, AB Zhang, XY Stoddart, JF Coskun, A Jakubikova, E Chen, LX AF Mara, Michael W. Bowman, David N. Buyukcakir, Onur Shelby, Megan L. Haldrup, Kristoffer Huang, Jier Harpham, Michael R. Stickrath, Andrew B. Zhang, Xiaoyi Stoddart, J. Fraser Coskun, Ali Jakubikova, Elena Chen, Lin X. TI Electron Injection from Copper Diimine Sensitizers into TiO2: Structural Effects and Their Implications for Solar Energy Conversion Devices SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; TRANSIENT MOLECULAR-STRUCTURES; DENSITY-FUNCTIONAL THEORY; TRANSFER EXCITED-STATES; WAVE BASIS-SET; X-RAY; ANATASE 101; MN(II)-TERPYRIDINE COMPLEXES; PHOTOPHYSICAL PROPERTIES; COORDINATION-COMPOUNDS AB Copper(I) diimine complexes have emerged as low cost replacements for ruthenium complexes as light sensitizers and electron donors, but their shorter metal-to-ligand-charge-transfer (MLCT) states lifetimes and lability of transient Cu(II) species impede their intended functions. Two carboxylated Cu(I) bis-2,9-diphenylphenanthroline (dpp) complexes [Cu(I)(dpp-O(CH2CH2O)(5))(dpp-(COOH)(2))](+) and [Cu(I)(dpp-O(CH2CH2O)(5))(dpp-(F-COOH)(2))](+) (F = tolyl) with different linker lengths were synthesized in which the MLCT-state solvent quenching pathways are effectively blocked, the lifetime of the singlet MLCT state is prolonged, and the transient Cu(II) ligands are stabilized. Aiming at understanding the mechanisms of structural influence to the interfacial charge transfer in the dye-sensitized solar cell mimics, electronic and geometric structures as well as dynamics for the MLCT state of these complexes and their hybrid with TiO2 nanoparticles were investigated using optical transient spectroscopy, X-ray transient absorption spectroscopy, time-dependent density functional theory, and quantum dynamics simulations. The combined results show that these complexes exhibit strong absorption throughout the visible spectrum due to the severely flattened ground state, and a long-lived charge-separated Cu(II) has been achieved via ultrafast electron injection (<300 fs) from the 1MLCT state into TiO2 nanoparticles. The results also indicate that the TiO2-phen distance in these systems does not have significant effect on the efficiency of the interfacial electron-transfer process. The mechanisms for electron transfer in these systems are discussed and used to develop new strategies in optimizing copper(I) diimine complexes in solar energy conversion devices. C1 [Mara, Michael W.; Shelby, Megan L.; Stoddart, J. Fraser; Chen, Lin X.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Mara, Michael W.; Shelby, Megan L.; Huang, Jier; Harpham, Michael R.; Stickrath, Andrew B.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Zhang, Xiaoyi] Argonne Natl Lab, Xray Sci Div Adv Photon Source, Argonne, IL 60439 USA. [Bowman, David N.; Jakubikova, Elena] N Carolina State Univ, Dept Chem, Raleigh, NC 27695 USA. [Buyukcakir, Onur; Coskun, Ali] Korea Adv Inst Sci & Technol, Grad Sch Energy Environm Water & Sustainabil EEWS, Taejon 305701, South Korea. [Haldrup, Kristoffer] Tech Univ Denmark, NEXMAP Sect, Dept Phys, Ctr Mol Movies, DK-2800 Lyngby, Denmark. RP Coskun, A (reprint author), Korea Adv Inst Sci & Technol, Grad Sch Energy Environm Water & Sustainabil EEWS, Taejon 305701, South Korea. EM coskun@kaist.ac.kr; ejakubi@ncsu.edu; lchen@anl.gov RI Huang, Jiaxing/B-7521-2009; COSKUN, Ali/C-1045-2008; Haldrup, Kristoffer/J-6875-2013 OI COSKUN, Ali/0000-0002-4760-1546; Haldrup, Kristoffer/0000-0002-0565-6397 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Joint Center of Excellence in Integrated Nanosystems at King Abdul-Aziz City for Science and Technology (KACST) [34-946]; Northwestern University (NU); National Research Foundation of Korea (NRF) - Korea government (MEST) [NRF-2014R1A4A1003712]; Carlsberg Foundation; Villum Foundation; U. S. Army Research Office [W911NF-15-1-0124]; U.S. Department of Education Graduate Assistantship In Areas Of National Need (GAANN) Fellowship Program at North Carolina State University FX The work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. The synthetic work is also part (Project 34-946) of the Joint Center of Excellence in Integrated Nanosystems at King Abdul-Aziz City for Science and Technology (KACST) and Northwestern University (NU). We thank both KACST and NU for the continued support of this research. The synthetic work was also partially supported by the National Research Foundation of Korea (NRF) Grant funded by the Korea government (MEST), NRF-2014R1A4A1003712. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. K.H. gratefully acknowledges support from the Carlsberg and Villum Foundations. E.J. and D.N.B. gratefully acknowledge support from the U. S. Army Research Office under contract number W911NF-15-1-0124. D.N.B. also acknowledges the support from the U.S. Department of Education Graduate Assistantship In Areas Of National Need (GAANN) Fellowship Program at North Carolina State University. We gratefully acknowledge Prof. Jean-Pierre Sauvage for his advice in synthesis and Prof. Victor S. Batista (Yale University) for providing us with a copy of the code for the JET simulations (IETsim). NR 116 TC 15 Z9 15 U1 6 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 5 PY 2015 VL 137 IS 30 BP 9670 EP 9684 DI 10.1021/jacs.5b04612 PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA CO6PV UT WOS:000359279500031 PM 26154849 ER PT J AU Pramanick, A Jorgensen, MRV Diallo, SO Christianson, AD Fernandez-Baca, JA Hoffmann, C Wang, XP Lan, S Wang, XL AF Pramanick, Abhijit Jorgensen, Mads R. V. Diallo, Souleymane O. Christianson, Andrew D. Fernandez-Baca, Jaime A. Hoffmann, Christina Wang, Xiaoping Lan, Si Wang, Xun-Li TI Nanoscale Atomic Displacements Ordering for Enhanced Piezoelectric Properties in Lead-Free ABO(3) Ferroelectrics SO ADVANCED MATERIALS LA English DT Article DE ceramics; ferroelectrics; materials science; nanotechnology; piezoelectric properties ID STRUCTURAL PHASE-TRANSITIONS; INELASTIC NEUTRON-SCATTERING; ORTHORHOMBIC KNBO3; SINGLE-CRYSTALS; ELECTROMECHANICAL RESPONSE; FREE PIEZOCERAMICS; CHAIN-STRUCTURE; BATIO3; INSTABILITY; DYNAMICS C1 [Pramanick, Abhijit; Lan, Si; Wang, Xun-Li] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. [Jorgensen, Mads R. V.] Aarhus Univ, Ctr Mat Crystallog, iNano & Dept Chem, Aarhus, Denmark. [Diallo, Souleymane O.; Hoffmann, Christina; Wang, Xiaoping; Lan, Si] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Christianson, Andrew D.; Fernandez-Baca, Jaime A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Pramanick, A (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. EM abhijit.pramanick@gmail.com RI Wang, Xiaoping/E-8050-2012; Pramanick, Abhijit/D-9578-2011; Jorgensen, Mads Ry Vogel/C-6109-2017; christianson, andrew/A-3277-2016; Fernandez-Baca, Jaime/C-3984-2014; Diallo, Souleymane/B-3111-2016; Wang, Xun-Li/C-9636-2010; hoffmann, christina/D-2292-2016 OI Wang, Xiaoping/0000-0001-7143-8112; Pramanick, Abhijit/0000-0003-0687-4967; Jorgensen, Mads Ry Vogel/0000-0001-5507-9615; christianson, andrew/0000-0003-3369-5884; Fernandez-Baca, Jaime/0000-0001-9080-5096; Diallo, Souleymane/0000-0002-3369-8391; Wang, Xun-Li/0000-0003-4060-8777; hoffmann, christina/0000-0002-7222-5845 FU DOE Office of Science [DE-AC02-06CH11357]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; City University of Hong Kong; Danish National Research Foundation [DNRF93]; Danish Research Council for Nature and Universe (Danscatt) FX This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Technical assistance for X-ray scattering measurement from Y. Ren and his students at Sector 11-IDB is gratefully acknowledged. Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. A.P. acknowledges funding support from the City University of Hong Kong. M.R.V.J. is grateful for the support by the Danish National Research Foundation (DNRF93), and the Danish Research Council for Nature and Universe (Danscatt). A.P. gratefully acknowledges helpful discussions with Prof. Sunil K. Sinha NR 38 TC 1 Z9 1 U1 11 U2 88 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 5 PY 2015 VL 27 IS 29 BP 4330 EP 4335 DI 10.1002/adma.201501274 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO2WY UT WOS:000359018900011 PM 26076654 ER PT J AU Chen, RY Zhang, SJ Schneeloch, JA Zhang, C Li, Q Gu, GD Wang, NL AF Chen, R. Y. Zhang, S. J. Schneeloch, J. A. Zhang, C. Li, Q. Gu, G. D. Wang, N. L. TI Optical spectroscopy study of the three-dimensional Dirac semimetal ZrTe5 SO PHYSICAL REVIEW B LA English DT Article ID CD3AS2; PHASE AB Three-dimensional (3D) topological Dirac materials have been under intensive study recently. The layered compound ZrTe5 has been suggested to be one such material as a result of transport and angle-resolved photoemission spectroscopy experiments. Here, we perform infrared reflectivity measurements to investigate the underlying physics of this material. The derived optical conductivity increases linearly with frequency below normal interband transitions, which provides optical spectroscopic proof of a 3D Dirac semimetal. In addition, the plasma edge shifts dramatically to lower energy upon temperature cooling, which might be due to the shrinking of the lattice parameters. In addition, an extremely sharp peak shows up in the frequency-dependent optical conductivity, indicating the presence of a Van Hove singularity in the joint density of state. C1 [Chen, R. Y.; Zhang, S. J.; Wang, N. L.] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Schneeloch, J. A.; Zhang, C.; Li, Q.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Wang, N. L.] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. RP Chen, RY (reprint author), Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. RI Zhang, Cheng/R-6593-2016 OI Zhang, Cheng/0000-0001-6531-4703 FU National Science Foundation of China [11120101003, 11327806]; 973 project of Ministry of Science and Technology of China [2011CB921701, 2012CB821403]; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-SC00112704] FX We acknowledge very helpful discussions with H. M. Weng, F. Wang, X. C. Xie, Z. Fang, X. Dai, and H. W. Liu. This work was supported by the National Science Foundation of China (Grants No. 11120101003 and No. 11327806), and the 973 project of the Ministry of Science and Technology of China (Grants No. 2011CB921701 and No. 2012CB821403). Work at Brookhaven was supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy under Contract No. DE-SC00112704 NR 36 TC 34 Z9 34 U1 14 U2 73 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD AUG 5 PY 2015 VL 92 IS 7 AR 075107 DI 10.1103/PhysRevB.92.075107 PG 5 WC Physics, Condensed Matter SC Physics GA CO3HI UT WOS:000359047000003 ER PT J AU Martin, SP AF Martin, Stephen P. TI Nonstandard supersymmetry breaking and Dirac gaugino masses without supersoftness SO PHYSICAL REVIEW D LA English DT Article ID SCALE SUPERSYMMETRY; MEDIATION; GLUINOS AB I consider models in which nonstandard supersymmetry-breaking terms, including Dirac gaugino masses, arise from F-term breaking mediated by operators with a 1/M-3 suppression. In these models, the supersoft properties found in the case of D-term breaking are absent in general, but can be obtained as a special case that is a fixed point of the renormalization group equations. The mu-term is replaced by three distinct supersymmetry-breaking parameters, decoupling the Higgs scalar potential from the Higgsino masses. Both holomorphic and nonholomorphic scalar cubic interactions with minimal flavor violation are induced in the supersymmetric Standard Model Lagrangian. C1 [Martin, Stephen P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Martin, Stephen P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Martin, SP (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. FU National Science Foundation [PHY-1417028] FX I thank Paddy Fox and Ann Nelson for useful conversations. This work was supported in part by the National Science Foundation Grant No. PHY-1417028. NR 75 TC 13 Z9 13 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 5 PY 2015 VL 92 IS 3 AR 035004 DI 10.1103/PhysRevD.92.035004 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO3IL UT WOS:000359050300004 ER PT J AU Reichhardt, CJO Lopatina, LM Jia, X Johnson, PA AF Reichhardt, C. J. Olson Lopatina, L. M. Jia, X. Johnson, P. A. TI Softening of stressed granular packings with resonant sound waves SO PHYSICAL REVIEW E LA English DT Article ID NONLINEAR ELASTICITY; 1994 NORTHRIDGE; ACOUSTIC-WAVES; CYCLIC SHEAR; MEDIA; EARTHQUAKES; PRESSURE; SIMULATIONS; DYNAMICS; FAULT AB We perform numerical simulations of a two-dimensional bidisperse granular packing subjected to both a static confining pressure and a sinusoidal dynamic forcing applied by a wall on one edge of the packing. We measure the response experienced by a wall on the opposite edge of the packing and obtain the resonant frequency of the packing as the static or dynamic pressures are varied. Under increasing static pressure, the resonant frequency increases, indicating a velocity increase of elastic waves propagating through the packing. In contrast, when the dynamic amplitude is increased for fixed static pressure, the resonant frequency decreases, indicating a decrease in the wave velocity. This occurs both for compressional and for shear dynamic forcing and is in agreement with experimental results. We find that the average contact number Z(c) at the resonant frequency decreases with increasing dynamic amplitude, indicating that the elastic softening of the packing is associated with a reduced number of grain-grain contacts through which the elastic waves can travel. We image the excitations created in the packing and show that there are localized disturbances or soft spots that become more prevalent with increasing dynamic amplitude. Our results are in agreement with experiments on glass bead packings and earth materials such as sandstone and granite and may be relevant to the decrease in elastic wave velocities that has been observed to occur near fault zones after strong earthquakes, in surficial sediments during strong ground motion, and in structures during earthquake excitation. C1 [Reichhardt, C. J. Olson; Lopatina, L. M.; Johnson, P. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Jia, X.] ESPCI ParisTech, Inst Langevin, CNRS, UMR 7587, F-75005 Paris, France. RP Reichhardt, CJO (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU Institutional Support (LDRD) at Los Alamos National Laboratory; NNSA of the U.S. Department of Energy at LANL [DE-AC52-06NA25396] FX This work was supported by Institutional Support (LDRD) at Los Alamos National Laboratory. This work was carried out under the auspices of the NNSA of the U.S. Department of Energy at LANL under Contract No. DE-AC52-06NA25396. NR 86 TC 3 Z9 3 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 5 PY 2015 VL 92 IS 2 AR 022203 DI 10.1103/PhysRevE.92.022203 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CO3JR UT WOS:000359053800005 PM 26382390 ER PT J AU Zhu, HY Zhang, S Su, D Jiang, GM Sun, SH AF Zhu, Huiyuan Zhang, Sen Su, Dong Jiang, Guangming Sun, Shouheng TI Surface Profile Control of FeNiPt/Pt Core/Shell Nanowires for Oxygen Reduction Reaction SO SMALL LA English DT Article DE core; shell; metal nanowires; nanowires; oxygen reduction reaction; Pt-skin surfaces ID SHAPE-CONTROLLED SYNTHESIS; PT-SKIN SURFACES; NANOPARTICLES; CATALYSTS; ELECTROCATALYSIS; NANOCRYSTALS; PD; DESIGN; CO; CU C1 [Zhu, Huiyuan; Zhang, Sen; Jiang, Guangming; Sun, Shouheng] Brown Univ, Dept Chem, Providence, RI USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Sun, SH (reprint author), Brown Univ, Dept Chem, Providence, RI 02912 USA. EM ssun@brown.edu FU U.S. Army Research Laboratory; U.S. Army Research Office under the Multi University Research Initiative (MURI) [W911NF-11-1-0353]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC-0011270] FX This work was supported by the U.S. Army Research Laboratory and the U.S. Army Research Office under the Multi University Research Initiative (MURI, Grant No. W911NF-11-1-0353) on "Stress-Controlled Catalysis via Engineered Nanostructures," and by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program. Electron microscopy research was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-SC-0011270. NR 28 TC 13 Z9 13 U1 17 U2 98 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD AUG 5 PY 2015 VL 11 IS 29 BP 3545 EP 3549 DI 10.1002/smll.201500330 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CO2ZI UT WOS:000359025300005 PM 25786658 ER PT J AU Zhou, CLE AF Zhou, Carol L. Ecale TI CombAlign: a code for generating a one-to-many sequence alignment from a set of pairwise structure-based sequence alignments SO SOURCE CODE FOR BIOLOGY AND MEDICINE LA English DT Article DE Multiple sequence alignment; Multiple structure alignment; Matrix protein; Msa; Mssa; VP40; Secreted glycoprotein; sGP; Ebola ID PROTEIN-STRUCTURE ALIGNMENT; EBOLA-VIRUS; MATRIX PROTEIN; VP40; TARGET; ENTRY AB Background: In order to better define regions of similarity among related protein structures, it is useful to identify the residue-residue correspondences among proteins. Few codes exist for constructing a one-to-many multiple sequence alignment derived from a set of structure or sequence alignments, and a need was evident for creating such a tool for combining pairwise structure alignments that would allow for insertion of gaps in the reference structure. Results: This report describes a new Python code, CombAlign, which takes as input a set of pairwise sequence alignments (which may be structure based) and generates a one-to-many, gapped, multiple structure-or sequence-based sequence alignment (MSSA). The use and utility of CombAlign was demonstrated by generating gapped MSSAs using sets of pairwise structure-based sequence alignments between structure models of the matrix protein (VP40) and pre-small/secreted glycoprotein (sGP) of Reston Ebolavirus and the corresponding proteins of several other filoviruses. The gapped MSSAs revealed structure-based residue-residue correspondences, which enabled identification of structurally similar versus differing regions in the Reston proteins compared to each of the other corresponding proteins. Conclusions: CombAlign is a new Python code that generates a one-to-many, gapped, multiple structure-or sequence-based sequence alignment (MSSA) given a set of pairwise sequence alignments (which may be structure based). CombAlign has utility in assisting the user in distinguishing structurally conserved versus divergent regions on a reference protein structure relative to other closely related proteins. CombAlign was developed in Python 2.6, and the source code is available for download from the GitHub code repository. C1 Lawrence Livermore Natl Lab, Global Secur Comp Applicat Div, Computat Biol Grp, Livermore, CA 94550 USA. RP Zhou, CLE (reprint author), Lawrence Livermore Natl Lab, Global Secur Comp Applicat Div, Computat Biol Grp, 7000 East Ave, Livermore, CA 94550 USA. EM zhou4@llnl.gov NR 19 TC 0 Z9 0 U1 2 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1751-0473 J9 SOURCE CODE BIOL MED JI Source Code Biol. Med. PD AUG 5 PY 2015 VL 10 AR 9 DI 10.1186/s13029-015-0039-1 PG 8 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA CO2JY UT WOS:000358983500001 PM 26246852 ER PT J AU Samolyuk, GD Osetsky, YN AF Samolyuk, G. D. Osetsky, Y. N. TI Thermodynamic approach to the stability of multi-phase systems: application to the Y2O3-Fe system SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE multi-phase; multi-scale simulations; yttria; iron; computational thermodynamics ID NANOSTRUCTURED FERRITIC ALLOYS; AB-INITIO; 1ST-PRINCIPLES CALCULATIONS; MOLECULAR-DYNAMICS; NANOCLUSTERS; DISPERSION; OXIDE; PSEUDOPOTENTIALS; MECHANISMS; DEFECTS AB Oxide-metal systems are important in many practical applications, and they are undergoing extensive study using a wide range of techniques. The most accurate theoretical approaches are based on density functional theory (DFT), which is limited to similar to 10(2) atoms. Multi-scale approaches, e.g. DFT + Monte Carlo, are often used to model oxide metal systems at the atomic level. These approaches can qualitatively describe the kinetics of some processes but not the overall stability of individual phases. In this article, we propose a thermodynamic approach to study equilibrium in multi-phase systems, which can be sequentially enhanced by considering different defects and microstructures. We estimate the thermodynamic equilibrium by minimization of the free energy of the whole multi-phase system using a limited set of defects and microstructural objects for which the properties are calculated by DFT. As an example, we consider Y2O3 + bcc Fe with vacancies in both the Y2O3 and bcc Fe phases, Y substitutions and O interstitials in Fe, Fe impurities, and antisite defects in Y2O3. The output of these calculations is the thermal equilibrium concentration of all the defects for a particular temperature and composition. The results obtained confirmed the high temperature stability of yttria in iron. Model development toward more accurate calculations is discussed. C1 [Samolyuk, G. D.; Osetsky, Y. N.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Samolyuk, GD (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM osetskiyyn@ornl.gov FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC05-000R22725] FX This research was sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy (DE-AC05-000R22725). NR 33 TC 2 Z9 2 U1 3 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 5 PY 2015 VL 27 IS 30 AR 305001 DI 10.1088/0953-8984/27/30/305001 PG 9 WC Physics, Condensed Matter SC Physics GA CN7AM UT WOS:000358585900003 PM 26151413 ER PT J AU Li, YL Xu, K Hu, SY Suter, J Schreiber, DK Ramuhalli, P Johnson, BR McCloy, J AF Li, Yulan Xu, Ke Hu, Shenyang Suter, Jon Schreiber, Daniel K. Ramuhalli, Pradeep Johnson, Bradley R. McCloy, John TI Computational and experimental investigations of magnetic domain structures in patterned magnetic thin films SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article DE nondestructive magnetic signatures; LLG equation; magnetic force microscopy; phase field approach; iron thin films ID IRON FILMS; WALLS; SIMULATIONS; STEELS; FORCE; MICROMAGNETICS; PRECIPITATION; MICROSCOPY; SIGNATURES; PLATELET AB The use of nondestructive magnetic signatures for continuous monitoring of the degradation of structural materials in nuclear reactors is a promising yet challenging application for advanced functional materials behavior modeling and measurement. In this work, a numerical model, which is based on the Landau-Lifshitz-Gilbert equation of magnetization dynamics and the phase field approach, was developed to study the impact of defects such as nonmagnetic precipitates and/or voids, free surfaces and crystal orientation on magnetic domain structures and magnetic responses in magnetic materials, with the goal of exploring the correlation between microstructures and magnetic signatures. To validate the model, single crystal iron thin films (similar to 240 nm thickness) were grown on MgO substrates and a focused ion beam was used to pattern micrometer-scale specimens with different geometries. Magnetic force microscopy (MFM) was used to measure magnetic domain structure and its field-dependence. Numerical simulations were constructed with the same geometry as the patterned specimens and under similar applied magnetic field conditions as tested by MFM. The results from simulations and experiments show that 1) magnetic domain structures strongly depend on the film geometry and the external applied field and 2) the predicted magnetic domain structures from the simulations agree quantitatively with those measured by MFM. The results demonstrate the capability of the developed model, used together with key experiments, for improving the understanding of the signal physics in magnetic sensing, thereby providing guidance to the development of advanced nondestructive magnetic techniques. C1 [Li, Yulan; Hu, Shenyang; Suter, Jon; Schreiber, Daniel K.; Ramuhalli, Pradeep; Johnson, Bradley R.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Xu, Ke; McCloy, John] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Xu, Ke; McCloy, John] Washington State Univ, Mat Sci & Engn Program, Pullman, WA 99164 USA. RP Li, YL (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM yulan.li@pnnl.gov OI Suter, Jonathan/0000-0001-5709-6988; Ramuhalli, Pradeep/0000-0001-6372-1743; HU, Shenyang/0000-0002-7187-3082 FU Department of Energy, Office of Nuclear Energy; U.S. DOE [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research at PNNL FX The authors would like acknowledge funding from the Department of Energy, Office of Nuclear Energy. A portion of the research was performed at Pacific Northwest National Laboratory (PNNL), operated by Battelle Memorial Institute for the U.S. DOE under contract DE-AC05-76RL01830. A portion of this research was performed using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. NR 33 TC 3 Z9 3 U1 5 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD AUG 5 PY 2015 VL 48 IS 30 AR 305001 DI 10.1088/0022-3727/48/30/305001 PG 15 WC Physics, Applied SC Physics GA CM5PD UT WOS:000357739500001 ER PT J AU Ren, AM Rajashankar, KR Patel, DJ AF Ren, Aiming Rajashankar, Kanagalaghatta R. Patel, Dinshaw J. TI Global RNA Fold and Molecular Recognition for a pfl Riboswitch Bound to ZMP, a Master Regulator of One-Carbon Metabolism SO STRUCTURE LA English DT Article ID C-DI-AMP; BACTERIAL GENE-EXPRESSION; SENSING RIBOSWITCH; STRUCTURAL BASIS; EUBACTERIA SENSE; YDAO RIBOSWITCH; LIGAND; 2'-DEOXYGUANOSINE; PRINCIPLES; GMP AB ZTP, the pyrophosphorylated analog of ZMP (5amino-4-imidazole carboxamide ribose-50-monophosphate), was identified as an alarmone that senses 10-formyl-tetrahydroflate deficiency in bacteria. Recently, a pfl riboswitch was identified that selectively binds ZMP and regulates genes associated with purine biosynthesis and one-carbon metabolism. We report on the structure of the ZMP-bound Thermosinus carboxydivorans pfl riboswitch sensing domain, thereby defining the pseudoknot-based tertiary RNA fold, the binding-pocket architecture, and principles underlying ligand recognition specificity. Molecular recognition involves shape complementarity, with the ZMP 5-amino and carboxamide groups paired with the Watson-Crick edge of an invariant uracil, and the imidazole ring sandwiched between guanines, while the sugar hydroxyls form intermolecular hydrogen bond contacts. The burial of the ZMP base and ribose moieties, together with unanticipated coordination of the carboxamide by Mg2+, contrasts with exposure of the 50-phosphate to solvent. Our studies highlight the principles underlying RNA-based recognition of ZMP, a master regulator of one-carbon metabolism. C1 [Ren, Aiming; Patel, Dinshaw J.] Mem Sloan Kettering Canc Ctr, Struct Biol Program, New York, NY 10065 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, Dept Chem & Chem Biol, NE CAT,Adv Photon Source, Argonne, IL 60439 USA. RP Patel, DJ (reprint author), Mem Sloan Kettering Canc Ctr, Struct Biol Program, New York, NY 10065 USA. EM pateld@mskcc.org FU NIH [U19 CA179564]; National Institute of General Medical Sciences from the NIH [P41 GM103403]; NIH-ORIP HEI grant [S10 RR029205]; DOE Office of Science [DE-AC02-06CH11357] FX D.J.P. was supported by NIH U19 CA179564. This work is based upon research conducted at the Northeastern Collaborative Access Team beamlines, which are funded by the National Institute of General Medical Sciences from the NIH (P41 GM103403). The Pilatus 6M detector on 24-ID-C beamline is funded by a NIH-ORIP HEI grant (S10 RR029205). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 33 TC 3 Z9 3 U1 3 U2 12 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD AUG 4 PY 2015 VL 23 IS 8 BP 1375 EP 1381 DI 10.1016/j.str.2015.05.016 PG 7 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA CR1VD UT WOS:000361112300003 PM 26118534 ER PT J AU Quaile, AT Urbanus, ML Stogios, PJ Nocek, B Skarina, T Ensminger, AW Savchenko, A AF Quaile, Andrew T. Urbanus, Malene L. Stogios, Peter J. Nocek, Boguslaw Skarina, Tatiana Ensminger, Alexander W. Savchenko, Alexei TI Molecular Characterization of LubX: Functional Divergence of the U-Box Fold by Legionella pneumophila SO STRUCTURE LA English DT Article ID E3 UBIQUITIN LIGASE; CONJUGATING ENZYMES; SYSTEM; REVEALS; COMPLEX; GENOME; DOMAIN; CHIP; SET AB LubX is part of the large arsenal of effectors in Legionella pneumophila that are translocated into the host cytosol during infection. Despite such unique features as the presence of two U-box motifs and its targeting of another effector SidH, the molecular basis of LubX activity remains poorly understood. Here we show that the N terminus of LubX is able to activate an extended number of ubiquitin-conjugating (E2) enzymes including UBE2W, UBEL6, and all tested members of UBE2D and UBE2E families. Crystal structures of LubX alone and in complex with UBE2D2 revealed drastic molecular diversification between the two U-box domains, with only the N-terminal U-box retaining E2 recognition features typical for its eukaryotic counterparts. Extensive mutagenesis followed by functional screening in a yeast model system captured functionally important LubX residues including Arg121, critical for interactions with SidH. Combined, these data provide a new molecular insight into the function of this unique pathogenic factor. C1 [Quaile, Andrew T.; Stogios, Peter J.; Skarina, Tatiana; Savchenko, Alexei] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON M5S 3E5, Canada. [Urbanus, Malene L.; Ensminger, Alexander W.] Univ Toronto, Dept Mol Genet, Toronto, ON M5S 1A8, Canada. [Nocek, Boguslaw] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. [Nocek, Boguslaw; Skarina, Tatiana; Savchenko, Alexei] Argonne Natl Lab, Biosci Div, Midwest Ctr Struct Genom, Lemont, IL 60439 USA. RP Savchenko, A (reprint author), Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON M5S 3E5, Canada. EM alexei.savchenko@utoronto.ca OI Stogios, Peter/0000-0001-8663-1425 FU NIH through the Midwest Center for Structural Genomics [GM094585]; US Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; CIHR Operating Grant [MOP-13340]; University of Toronto Department of Molecular Genetics; Canada Foundation for Innovation; Ontario Research Fund FX Genomic DNA for Legionella pneumophila str. Paris was a generously provided by Carmen Buchrieser. Human E2 expression constructs were received as a generous gift from the S. Dhe-Paganon laboratory at the Structural Genomics Consortium. We also thank Adam Stein and Marianne Cuff at the Structural Biology Center, Advanced Photon Source, for X-ray diffraction data collection and processing, and Veronica Yim and Rosa Di Leo for cloning. This work was supported by the NIH grant GM094585 (to A.S. through the Midwest Center for Structural Genomics) and by the US Department of Energy, Office of Biological and Environmental Research, under contract DE-AC02-06CH11357. A.W.E. is supported by a CIHR Operating Grant (MOP-13340), the University of Toronto Department of Molecular Genetics, and infrastructure grants from the Canada Foundation for Innovation and the Ontario Research Fund. NR 44 TC 3 Z9 3 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD AUG 4 PY 2015 VL 23 IS 8 BP 1459 EP 1469 DI 10.1016/j.str.2015.05.020 PG 11 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA CR1VD UT WOS:000361112300011 PM 26146184 ER PT J AU Giannone, RJ Wurch, LL Podar, M Hettich, RL AF Giannone, Richard J. Wurch, Louie L. Podar, Mircea Hettich, Robert L. TI Rescuing Those Left Behind: Recovering and Characterizing Underdigested Membrane and Hydrophobic Proteins To Enhance Proteome Measurement Depth SO ANALYTICAL CHEMISTRY LA English DT Article ID ESCHERICHIA-COLI PROTEOME; TANDEM MASS-SPECTROMETRY; QUALITY ASSESSMENT; PEPTIDE IDENTIFICATION; SODIUM DEOXYCHOLATE; LABEL-FREE; QUANTIFICATION; COVERAGE; EXTRACTION; CHALLENGES AB The marine archaeon Nanoarchaeum equitans is dependent on direct physical contact with its host, the hyperthermophile Ignicoccus hospitalis. As this interaction is thought to be membrane-associated, involving a myriad of membrane-anchored proteins, proteomic efforts to better characterize this difficult to analyze interface are paramount to uncovering the mechanism of their association. By extending multienzyme digestion strategies that use sample filtration to recover underdigested proteins for reprocessing/consecutive proteolytic digestion, we applied chymotrypsin to redigest the proteinaceous material left over after initial proteolysis with trypsin of sodium dodecyl sulfate (SDS)-extracted I. hospitalis-N. equitans proteins. Using this method, we show that proteins with increased hydrophobic character, including membrane proteins with multiple transmembrane helices, are enriched and recovered in the underdigested fraction. Chymotryptic reprocessing provided significant sequence coverage gains in both soluble and hydrophobic proteins alike, with the latter benefiting more so in terms of membrane protein representation. These gains were despite a large proportion of high-quality peptide spectra remaining unassigned in the underdigested fraction suggesting high levels of protein modification on these often surface-exposed proteins. Importantly, these gains were achieved without applying extensive fractionation strategies usually required for thorough characterization of membrane-associated proteins and were facilitated by the generation of a distinct, complementary set of peptides that aid in both the identification and quantitation of this important, under-represented class of proteins. C1 [Giannone, Richard J.; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Wurch, Louie L.; Podar, Mircea] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Wurch, Louie L.] James Madison Univ, Dept Biol, Harrisonburg, VA 22807 USA. [Podar, Mircea] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. RP Giannone, RJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM giannonerj@ornl.gov RI Hettich, Robert/N-1458-2016; OI Hettich, Robert/0000-0001-7708-786X; Podar, Mircea/0000-0003-2776-0205 FU U.S. Department of Energy, Office of Biological and Environmental Research [DE-SC0006654]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); UT-Battelle, LLC [DE-AC05-00OR22725]; Department of Energy FX This research was supported by a grant from the U.S. Department of Energy, Office of Biological and Environmental Research (DE-SC0006654) and by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL). ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy. The authors would like to thank Harald Huber, Thomas Heimerl, and Reinhard Rachel for providing samples and Paul Abraham for his valuable suggestions and critical reading of this manuscript. Raw LC-MS/MS data evaluated in this study is available upon request. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 38 TC 5 Z9 5 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD AUG 4 PY 2015 VL 87 IS 15 BP 7720 EP 7728 DI 10.1021/acs.analchem.5b01187 PG 9 WC Chemistry, Analytical SC Chemistry GA CO6PF UT WOS:000359277900034 PM 26110888 ER PT J AU Cark, EL Singh, MR Kwon, Y Bell, AT AF Cark, Ezra L. Singh, Meenesh R. Kwon, Youngkook Bell, Alexis T. TI Differential Electrochemical Mass Spectrometer Cell Design for Online Quantification of Products Produced during Electrochemical Reduction of CO2 SO ANALYTICAL CHEMISTRY LA English DT Article ID AQUEOUS HYDROGENCARBONATE SOLUTION; CARBON-DIOXIDE; COPPER ELECTRODE; METAL-ELECTRODES; ELECTROREDUCTION; HYDROCARBONS; SELECTIVITY; ETHYLENE; METHANE; ELECTROOXIDATION AB The discovery of electrocatalysts that can efficiently reduce CO2 to fuels with high selectivity is a subject of contemporary interest. Currently, the available analytical methods for characterizing the products of CO2 reduction require tens of hours to obtain the dependence of product distribution on applied potential. As a consequence, there is a need to develop novel analytical approaches that can reduce this analysis time down to about an hour. We report here the design, construction, and operation of a novel differential electrochemical mass spectrometer (DEMS) cell geometry that enables the partial current densities of volatile electrochemical reaction products to be quantified in real time. The capabilities of the novel DEMS cell design are demonstrated by carrying out the electrochemical reduction of CO2 over polycrystalline copper. The reaction products are quantified in real time as a function of the applied potential during linear sweep voltammetry, enabling the product spectrum produced by a given electrocatalyst to be determined as a function of applied potential on a time scale of roughly 1 h. C1 [Cark, Ezra L.; Singh, Meenesh R.; Kwon, Youngkook; Bell, Alexis T.] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Cark, Ezra L.; Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Bell, AT (reprint author), Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM alexbell@berkeley.edu OI Singh, Meenesh/0000-0002-3638-8866 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation (NSF) FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award DE-SC0004993. E.L.C. is supported by the National Science Foundation (NSF). We also acknowledge Professor Tom Jaramillo, Dr. Mary Louie, Eric Granlund, Etosha Cave, and Gerry Duffy for contributions made through helpful discussions. NR 37 TC 1 Z9 1 U1 5 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD AUG 4 PY 2015 VL 87 IS 15 BP 8013 EP 8020 DI 10.1021/acs.analchem.5b02080 PG 8 WC Chemistry, Analytical SC Chemistry GA CO6PF UT WOS:000359277900072 ER PT J AU Snyder, RA Betzu, J Butch, SE Reig, AJ DeGrado, WF Solomon, EI AF Snyder, Rae Ana Betzu, Justine Butch, Susan E. Reig, Amanda J. DeGrado, William F. Solomon, Edward I. TI Systematic Perturbations of Binuclear Non-heme Iron Sites: Structure and Dioxygen Reactivity of de Novo Due Ferri Proteins SO BIOCHEMISTRY LA English DT Article ID METHANE MONOOXYGENASE HYDROXYLASE; METHYLOCOCCUS-CAPSULATUS BATH; MAGNETIC CIRCULAR-DICHROISM; COLI RIBONUCLEOTIDE REDUCTASE; BIFERROUS ACTIVE-SITE; CRYSTAL-STRUCTURE; DIIRON PROTEINS; O-2 REACTIVITY; XYLENE MONOOXYGENASE; ELECTRONIC-STRUCTURE AB DFsc (single-chain due ferri) proteins allow for modeling binuclear non-heme iron enzymes with a similar fold. Three 4A -> 4G variants of DFsc were studied to investigate the effects of (1) increasing the size of the substrate/solvent access channel (G4DFsc), (2) including an additional His residue in the first coordination sphere along with three additional helix-stabilizing mutations [3His-G4DFsc(Mut3)], and (3) the three helix-stabilizing mutations alone [G4DFsc(Mut3)] on the biferrous structures and their O-2 reactivities. Near-infrared circular dichroism and magnetic circular dichroism (MCD) spectroscopy show that the 4A -> 4G mutations increase coordination of the diiron site from 4-coordinate/5-coordinate to 5-coordinate/5-coordinate, likely reflecting increased solvent accessibility. While the three helix-stabilizing mutations [G4DFsc(Mut3)] do not affect the coordination number, addition of the third active site His residue [3His-G4DFsc(Mut3)] results in a 5-coordinate/6-coordinate site. Although all 4A? 4G variants have significantly slower pseudo-first-order rates when reacting with excess O2 than DFsc (similar to 2 s(-1)), G4DFsc and 3His-G4DFsc(Mut3) have rates (similar to 0.02 and similar to 0.04 s(-1)) faster than that of G4DFsc(Mut3) (similar to 0.002 s(-1)). These trends in the rate of O-2 reactivity correlate with exchange coupling between the Fe(II) sites and suggest that the two-electron reduction of O-2 occurs through end-on binding at one Fe(II) rather than through a peroxy-bridged intermediate. UV-vis absorption and MCD spectroscopies indicate that an Fe(III)Fe(III)-OH species first forms in all three variants but converts into an Fe(III)-mu-OH-Fe(III) species only in the 2-His forms, a process inhibited by the additional active site His ligand that coordinatively saturates one of the iron centers in 3His-G4DFsc(Mut3). C1 [Snyder, Rae Ana; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Betzu, Justine; Butch, Susan E.; Reig, Amanda J.] Ursinus Coll, Dept Chem, Collegeville, PA 19426 USA. [DeGrado, William F.] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94143 USA. [Solomon, Edward I.] Stanford Univ, SLAC, Stanford Synchrotron Radiat Lab, Menlo Pk, CA 94025 USA. RP Reig, AJ (reprint author), Ursinus Coll, Dept Chem, Collegeville, PA 19426 USA. EM areig@ursinus.edu; Bill.DeGrado@ucsf.edu; edward.solomon@stanford.edu FU National Science Foundation [MCB-1404866, CHE-1413295]; National Institutes of Health [F32-GM808852, R15-GM110657, GM54616, GM71628] FX This work was supported by the National Science Foundation (MCB-1404866 to E.I.S. and CHE-1413295 to W.F.D.) and the National Institutes of Health (F32-GM808852 and R15-GM110657 to AJ.R and GM54616 and GM71628 to W.F.D.). NR 54 TC 2 Z9 2 U1 2 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD AUG 4 PY 2015 VL 54 IS 30 BP 4637 EP 4651 DI 10.1021/acs.biochem.5b00324 PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CO6PE UT WOS:000359277800007 PM 26154739 ER PT J AU Henry, H Naujokas, MF Attanayake, C Basta, NT Cheng, ZQ Hettiarachchi, GM Maddaloni, M Schadt, C Scheckel, KG AF Henry, Heather Naujokas, Marisa F. Attanayake, Chammi Basta, Nicholas T. Cheng, Zhongqi Hettiarachchi, Ganga M. Maddaloni, Mark Schadt, Christopher Scheckel, Kirk G. TI Bioavailability-Based In Situ Remediation To Meet Future Lead (Pb) Standards in Urban Soils and Gardens SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Review ID FIRING RANGE SOILS; SMELTER-CONTAMINATED SOIL; ZERO-VALENT IRON; BLOOD LEAD; RELATIVE BIOAVAILABILITY; MANGANESE OXIDE; CHEMICAL IMMOBILIZATION; ORAL BIOACCESSIBILITY; PHOSPHORUS AMENDMENTS; METAL IMMOBILIZATION AB Recently the Centers for Disease Control and Prevention lowered the blood Pb reference value to 5 mu g/dL. The lower reference value combined with increased repurposing of postindustrial lands are heightening concerns and driving interest in reducing soil Pb exposures. As a result, regulatory decision makers may lower residential soil screening levels (SSLs), used in setting Pb cleanup levels, to levels that may be difficult to achieve, especially in urban areas. This paper discusses challenges in remediation and bioavailability assessments of Pb in urban soils in the context of lower SSLs and identifies research needs to better address those challenges. Although in situ remediation with phosphate amendments is a viable option, the scope of the problem and conditions in urban settings may necessitate that SSLs be based on bioavailable rather than total Pb concentrations. However, variability in soil composition can influence bioavailability testing and soil amendment effectiveness. More urgently needed to better understand this variability and increase confidence in using these approaches in risk-based making, particularly in urban areas. data are decision C1 [Naujokas, Marisa F.] MDB Inc, Durham, NC 27713 USA. [Basta, Nicholas T.] Ohio State Univ, Sch Environm & Nat Resources, Columbus, OH 43210 USA. [Cheng, Zhongqi] CUNY Brooklyn Coll, Brooklyn, NY 11210 USA. [Hettiarachchi, Ganga M.] Kansas State Univ, Dept Agron, Manhattan, KS 66506 USA. [Maddaloni, Mark] US EPA Reg 2, New York, NY 10007 USA. [Schadt, Christopher] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Scheckel, Kirk G.] US EPA, Natl Risk Management Res Lab, Cincinnati, OH 45224 USA. [Attanayake, Chammi] Univ Peradeniya, Dept Soil Sci, Peradeniya 20400, Sri Lanka. [Henry, Heather] NIEHS, Hazardous Subst Res Branch, Res Triangle Pk, NC 27709 USA. RP Naujokas, MF (reprint author), MDB Inc, 2525 Meridian Pkwy,Suite 50, Durham, NC 27713 USA. EM mnaujokas@michaeldbaker.com RI Schadt, Christopher/B-7143-2008; OI Schadt, Christopher/0000-0001-8759-2448; Scheckel, Kirk/0000-0001-9326-9241 FU National Institutes of Health's National Institute of Environmental Health Sciences (NIEHS); U.S. Department of Defense/Department of Energy/EPA Strategic Environmental Research and Development Program (SERDP); Kansas Agricultural Experimental Station [14-296-J]; Ohio Agricultural Research and Development Center of The Ohio State University FX This work was supported in part by the National Institutes of Health's National Institute of Environmental Health Sciences (NIEHS); and the joint U.S. Department of Defense/Department of Energy/EPA Strategic Environmental Research and Development Program (SERDP). This work was also supported in part through Contribution Number 14-296-J from the Kansas Agricultural Experimental Station. Partial salary support for N. Basta was provided by the Ohio Agricultural Research and Development Center of The Ohio State University. Although researchers from the EPA contributed to this article, the research presented was not subject to EPA's quality system requirements. Consequently, the views, interpretations, and conclusions expressed in this article are solely those of the authors and do not necessarily reflect or represent views or policies of EPA, NIH, NIEHS, or the United States Government, nor does mention of trade names, commercial products, or organizations imply endorsement by the U.S. Government. NR 146 TC 13 Z9 14 U1 28 U2 110 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 4 PY 2015 VL 49 IS 15 BP 8948 EP 8958 DI 10.1021/acs.est.5b01693 PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CO6PK UT WOS:000359278400004 PM 26140328 ER PT J AU Zhang, Y Tian, Z Liu, MM Shi, ZJ Hale, L Zhou, JZ Yang, M AF Zhang, Yu Tian, Zhe Liu, Miaomiao Shi, Zhou Jason Hale, Lauren Zhou, Jizhong Yang, Min TI High Concentrations of the Antibiotic Spiramycin in Wastewater Lead to High Abundance of Ammonia-Oxidizing Archaea in Nitrifying Populations SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID TETRACYCLINE RESISTANCE GENES; MICROBIAL COMMUNITY; TREATMENT-PLANT; NITROSOSPHAERA-VIENNENSIS; ACTIVATED-SLUDGE; RECEIVING RIVER; NITROGEN; AMOA; SOIL; DIVERSITY AB To evaluate the potential effects of antibiotics on ammonia-oxidizing microbes, multiple tools including quantitative PCR (qPCR), 454-pyrosequencing, and a high-throughput functional gene array (GeoChip) were used to reveal the distribution of ammonia-oxidizing archaea (AOA) and archaeal amoA (Arch-amoA) genes in three wastewater treatment systems receiving spiramycin or oxytetracycline production wastewaters. The qPCR results revealed that the copy number ratios of Arch-amoA to ammonia-oxidizing bacteria (AOB) amoA genes were the highest in the spiramycin full-scale (5.30) and pilot-scale systems (1.49 X 10(-1)), followed by the oxytetracycline system (4.90 X 10(-4)), with no Arch-amoA genes detected in the control systems treating sewage or inosine production wastewater. The pyrosequencing result showed that the relative abundance of AOA affiliated with Thaumarchaeota accounted for 78.5-99.6% of total archaea in the two spiramycin systems, which was in accordance with the qPCR results. Mantel test based on GeoChip data showed that Arch-amoA gene signal intensity correlated with the presence of spiramycin (P < 0.05). Antibiotics explained 25.8% of variations in amoA functional gene structures by variance partitioning analysis. This study revealed the selection of AOA in the presence of high concentrations of spiramycin in activated sludge systems. C1 [Zhang, Yu; Tian, Zhe; Liu, Miaomiao; Yang, Min] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, State Key Lab Environm Aquat Chem, Beijing 100085, Peoples R China. [Shi, Zhou Jason; Hale, Lauren; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Shi, Zhou Jason; Hale, Lauren; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Zhang, Y (reprint author), Chinese Acad Sci, Ecoenvironm Sci Res Ctr, State Key Lab Environm Aquat Chem, POB 2871, Beijing 100085, Peoples R China. EM zhangyu@rcees.ac.cn; yangmin@rcees.ac.cn FU National Natural Scientific Foundation of China (NSFC) [21437005, 51178449]; Ministry of Science and Technology, Peoples Republic of China [2012AA063401]; State Key Joint Laboratory of Environmental Simulation and Pollution Control [14l03ESPC]; Office of the Vice President for Research at the University of Oklahoma FX This study was supported by National Natural Scientific Foundation of China (NSFC: 21437005; 51178449), State Hi-tech Research and Development Project of the Ministry of Science and Technology, Peoples Republic of China (Grand) (2012AA063401), special fund of State Key Joint Laboratory of Environmental Simulation and Pollution Control (14l03ESPC), and the Office of the Vice President for Research at the University of Oklahoma. We thank Dr. Huaqun Yin, Dr. Tong Zhang, Dr. Limei Zhang, and Dr. Ye Deng for their help in experiments, statistical analysis, and paper revising. NR 64 TC 7 Z9 7 U1 38 U2 153 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 4 PY 2015 VL 49 IS 15 BP 9124 EP 9132 DI 10.1021/acs.est.5b01293 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CO6PK UT WOS:000359278400024 PM 26125322 ER PT J AU Zhang, T Hammack, RW Vidic, RD AF Zhang, Tieyuan Hammack, Richard W. Vidic, Radisav D. TI Fate of Radium in Marcellus Shale Flowback Water Impoundments and Assessment of Associated Health Risks SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID GAS EXTRACTION; WASTE-WATER; MANAGEMENT; DISPOSAL; QUALITY; PENNSYLVANIA; PARAMETERS; RADIATION; SULFATE; BARIUM AB Natural gas extraction from Marcellus Shale generates large quantities of flowback water that contain high levels of salinity, heavy metals, and naturally occurring radioactive material (NORM). This water is typically stored in centralized storage impoundments or tanks prior to reuse, treatment or disposal. The fate of Ra-226, which is the dominant NORM component in flowback water, in three centralized storage impoundments in southwestern Pennsylvania was investigated during a 2.5-year period. Field sampling revealed that Ra-226 concentration in these storage facilities depends on the management strategy but is generally increasing during the reuse of flowback water for hydraulic fracturing. In addition, Ra-226 is enriched in the bottom solids (e.g., impoundment sludge), where it increased from less than 10 pCi/g for fresh sludge to several hundred pCi/g for aged sludge. A combination of sequential extraction procedure (SEP) and chemical composition analysis of impoundment sludge revealed that Barite is the main carrier of Ra-226 in the sludge. Toxicity characteristic leaching procedure (TCLP) (EPA Method 1311) was used to assess the leaching behavior of Ra-226 in the impoundment sludge and its implications for waste management strategies for this low-level radioactive solid waste. Radiation exposure for on-site workers calculated using the RESRAD model showed that the radiation dose equivalent for the baseline conditions was well below the NRC limit for the general public. C1 [Zhang, Tieyuan; Vidic, Radisav D.] Univ Pittsburgh, Dept Civil & Environm Engn, Pittsburgh, PA 15261 USA. [Zhang, Tieyuan; Hammack, Richard W.; Vidic, Radisav D.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Vidic, RD (reprint author), Univ Pittsburgh, Dept Civil & Environm Engn, Pittsburgh, PA 15261 USA. EM vidic@pitt.edu OI Vidic, Radisav/0000-0001-7969-6845 FU National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL [4.605.920.009.812] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this study was performed under Task Release No. TR 131, Project Activity No. 4.605.920.009.812. We thank Dr. Kelvin Gregory and Dr. Arvind Murali Mohan for the assistance with sampling and Dr. Daniel Bain and David Pompeani for radionuclide measurement. NR 37 TC 8 Z9 8 U1 9 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD AUG 4 PY 2015 VL 49 IS 15 BP 9347 EP 9354 DI 10.1021/acs.est.5b01393 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CO6PK UT WOS:000359278400050 PM 26154523 ER PT J AU Jahed, Z Shams, H Mofrad, MRK AF Jahed, Zeinab Shams, Hengameh Mofrad, Mohammad R. K. TI A Disulfide Bond Is Required for the Transmission of Forces through SUN-KASH Complexes SO BIOPHYSICAL JOURNAL LA English DT Article ID NUCLEAR-ENVELOPE; LINC COMPLEXES; STRUCTURAL INSIGHTS; COILED-COIL; MECHANOTRANSDUCTION; DISEASE; PROTEINS; HEALTH; NESPRINS; BINDING AB Numerous biological functions of a cell, including polarization, differentiation, division, and migration, rely on its ability to endure mechanical forces generated by the cytoskeleton on the nucleus. Coupling of the cytoskeleton and nucleoskeleton is ultimately mediated by LINC complexes that are formed via a strong interaction between SUN- and KASH-domain-containing proteins in the nuclear envelope. These complexes are mechanosensitive and essential for the transmission of forces between the cytoskeleton and nucleoskeleton, and the progression of cellular mechanotransduction. Herein, using molecular dynamics, we examine the effect of tension on the human SUN2-KASH2 complex and show that it is remarkably stable under physiologically relevant tensile forces and large strains. However, a covalent disulfide bond between two highly conserved cysteine residues of SUN2 and KASH2 is crucial for the stability of this interaction and the transmission of forces through the complex. C1 [Jahed, Zeinab; Shams, Hengameh; Mofrad, Mohammad R. K.] Univ Calif Berkeley, Dept Bioengn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA. [Jahed, Zeinab; Shams, Hengameh; Mofrad, Mohammad R. K.] Univ Calif Berkeley, Dept Mech Engn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA. [Mofrad, Mohammad R. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Mofrad, MRK (reprint author), Univ Calif Berkeley, Dept Bioengn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA. EM mofrad@berkeley.edu FU National Science Foundation (CAREER award) [CBET-0955291]; Natural Sciences and Engineering Research Council of Canada; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by grants from the National Science Foundation (CAREER award CBET-0955291 to M.R.K.M.) and the Natural Sciences and Engineering Research Council of Canada (to Z.J.). This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 41 TC 2 Z9 2 U1 0 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD AUG 4 PY 2015 VL 109 IS 3 BP 501 EP 509 DI 10.1016/j.bpj.2015.06.057 PG 9 WC Biophysics SC Biophysics GA CO5DS UT WOS:000359180400007 PM 26244732 ER PT J AU Bhatt, S Gupta, MK Khamaisi, M Martinez, R Gritsenko, MA Wagner, BK Guye, P Busskamp, V Shirakawa, J Wu, GX Liew, CW Clauss, TR Valdez, I El Ouaamari, A Dirice, E Takatani, T Keenan, HA Smith, RD Church, G Weiss, R Wagers, AJ Qian, WJ King, GL Kulkarni, RN AF Bhatt, Shweta Gupta, Manoj K. Khamaisi, Mogher Martinez, Rachael Gritsenko, Marina A. Wagner, Bridget K. Guye, Patrick Busskamp, Volker Shirakawa, Jun Wu, Gongxiong Liew, Chong Wee Clauss, Therese R. Valdez, Ivan El Ouaamari, Abdelfattah Dirice, Ercument Takatani, Tomozumi Keenan, Hillary A. Smith, Richard D. Church, George Weiss, Ron Wagers, Amy J. Qian, Wei-Jun King, George L. Kulkarni, Rohit N. TI Preserved DNA Damage Checkpoint Pathway Protects against Complications in Long-Standing Type 1 Diabetes SO CELL METABOLISM LA English DT Article ID DOUBLE-STRAND BREAKS; PLURIPOTENT STEM-CELLS; VASCULAR COMPLICATIONS; PHOSPHORYLATION DYNAMICS; MRE11-RAD50-NBS1 COMPLEX; HISTONE H2AX; MECHANISMS; CHROMATIN; REPAIR; MDC1 AB The mechanisms underlying the development of complications in type 1 diabetes (T1D) are poorly understood. Disease modeling of induced pluripotent stem cells (iPSCs) from patients with longstanding T1D(disease duration >= 50 years) with severe (Medalist +C) or absent to mild complications (Medalist -C) revealed impaired growth, reprogramming, and differentiation in Medalist +C. Genomics and proteomics analyses suggested differential regulation of DNA damage checkpoint proteins favoring protection from cellular apoptosis in Medalist -C. In silico analyses showed altered expression patterns of DNA damage checkpoint factors among the Medalist groups to be targets of miR200, whose expression was significantly elevated in Medalist +C serum. Notably, neurons differentiated from Medalist +C iPSCs exhibited enhanced susceptibility to genotoxic stress that wors-ened upon miR200 overexpression. Furthermore, knockdown of miR200 in Medalist +C fibroblasts and iPSCs rescued checkpoint protein expression and reduced DNA damage. We propose miR200-regulated DNA damage checkpoint pathway as a potential therapeutic target for treating complications of diabetes. C1 [Bhatt, Shweta; Gupta, Manoj K.; Martinez, Rachael; Shirakawa, Jun; Liew, Chong Wee; Valdez, Ivan; El Ouaamari, Abdelfattah; Dirice, Ercument; Takatani, Tomozumi; Wagers, Amy J.; Kulkarni, Rohit N.] Harvard Univ, Sch Med, Joslin Diabet Ctr, Sect Islet Cell & Regenerat Biol, Boston, MA 02215 USA. [Bhatt, Shweta; Gupta, Manoj K.; Khamaisi, Mogher; Shirakawa, Jun; Liew, Chong Wee; Valdez, Ivan; El Ouaamari, Abdelfattah; Dirice, Ercument; Takatani, Tomozumi; Keenan, Hillary A.; King, George L.; Kulkarni, Rohit N.] Harvard Univ, Sch Med, Brigham & Womens Hosp, Dept Med, Boston, MA 02215 USA. [Khamaisi, Mogher; Wu, Gongxiong; King, George L.] Harvard Univ, Sch Med, Joslin Diabet Ctr, Sect Vasc Cell Biol, Boston, MA 02215 USA. [Gritsenko, Marina A.; Clauss, Therese R.; Smith, Richard D.; Qian, Wei-Jun] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Wagner, Bridget K.] Broad Inst Harvard & Massachusetts Inst Technol, Cambridge, MA 02142 USA. [Guye, Patrick; Weiss, Ron] MIT, Dept Biol Engn, Cambridge, MA 02139 USA. [Busskamp, Volker; Church, George] Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. [Wagers, Amy J.] Harvard Univ, Dept Stem Cell & Regenerat Biol, Howard Hughes Med Inst, Harvard Stem Cell Inst, Cambridge, MA 02138 USA. RP Kulkarni, RN (reprint author), Harvard Univ, Sch Med, Joslin Diabet Ctr, Sect Islet Cell & Regenerat Biol, Boston, MA 02215 USA. EM rohit.kulkarni@joslin.harvard.edu RI Smith, Richard/J-3664-2012; Busskamp, Volker/E-6339-2015; Dirice, Ercument/B-2825-2017; OI Smith, Richard/0000-0002-2381-2349; Busskamp, Volker/0000-0001-7517-8944; Shirakawa, Jun/0000-0002-0822-8750 FU NIH [RO1 DK67536, RO1 103215, UC4 DK104167-01, DP2OD006668, DP3 DK094333-01, JDRF 17-2013-310, K99DK090210, R00DK090210, 3-APF-2014-182-A-N, JDRF 10-2012-240, P41 GM103493]; Mary K. Iacocca Foundation; DOE/BER and located at Pacific Northwest National Laboratory; DOE [DE-AC05-76RL0 1830] FX The authors acknowledge the microarray facility, Children's Hospital, Boston; C. Cahill, Advanced Microscopy Facility; iPS Core Facility, DRC, Joslin Diabetes Center (NIH DK036836); and Therese Rw Clauss, Pacific Northwest National Laboratory. The authors thank G. Daley (Children's Hospital, Boston) for discussions. This research was supported in part by NIH RO1 DK67536 and NIH RO1 103215 (R.N.K.), UC4 DK104167-01 (W.J.Q., R.N.K.), DP2OD006668 (W.J.Q.), NIH DP3 DK094333-01 (G.L.K.), JDRF 17-2013-310 (H.K.), K99DK090210 and R00DK090210 (C.W.L.), 3-APF-2014-182-A-N (A.E.), JDRF 10-2012-240 (G.W.), and P41 GM103493 (R.D.S.). S.B. is the recipient of postdoctoral research fellowship from Mary K. Iacocca Foundation. Proteomics experiments were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by DOE/BER and located at Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the DOE under Contract DE-AC05-76RL0 1830. A.J.W. is an Early Career Scientist of the Howard Hughes Medical Institute. Content is solely the responsibility of the authors and does not necessarily represent the official views of the NIH or other funding agencies. NR 51 TC 6 Z9 6 U1 4 U2 11 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1550-4131 EI 1932-7420 J9 CELL METAB JI Cell Metab. PD AUG 4 PY 2015 VL 22 IS 2 BP 239 EP 252 DI 10.1016/j.cmet.2015.07.015 PG 14 WC Cell Biology; Endocrinology & Metabolism SC Cell Biology; Endocrinology & Metabolism GA CO2QA UT WOS:000359000500010 PM 26244933 ER PT J AU Tremblay, J Singh, K Fern, A Kirton, ES He, SM Woyke, T Lee, J Chen, F Dangl, JL Tringe, SG AF Tremblay, Julien Singh, Kanwar Fern, Alison Kirton, Edward S. He, Shaomei Woyke, Tanja Lee, Janey Chen, Feng Dangl, Jeffery L. Tringe, Susannah G. TI Primer and platform effects on 16S rRNA tag sequencing SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE 16S rRNA gene sequencing; microbial population and community ecology; high throughput sequencing; microbial diversity; community assembly; amplification; sequencing error ID HIGH-THROUGHPUT; RHIZOSPHERE MICROBIOME; RARE BIOSPHERE; GENE DATABASE; PCR; DIVERSITY; BIAS; ILLUMINA; HETERODUPLEXES; AMPLIFICATION AB Sequencing of 16S rRNA gene tags is a popular method for profiling and comparing microbial communities. The protocols and methods used, however, vary considerably with regard to amplification primers, sequencing primers, sequencing technologies; as well as quality filtering and clustering. How results are affected by these choices, and whether data produced with different protocols can be meaningfully compared, is often unknown. Here we compare results obtained using three different amplification primer sets (targeting V4, V6-V8, and V7-V8) and two sequencing technologies (454 pyrosequencing and Illumina MiSeq) using DNA from a mock community containing a known number of species as well as complex environmental samples whose PCR-independent profiles were estimated using shotgun sequencing. We find that paired-end MiSeq reads produce higher quality data and enabled the use of more aggressive quality control parameters over 454, resulting in a higher retention rate of high quality reads for downstream data analysis. While primer choice considerably influences quantitative abundance estimations, sequencing platform has relatively minor effects when matched primers are used. Beta diversity metrics are surprisingly robust to both primer and sequencing platform biases. C1 [Tremblay, Julien; Singh, Kanwar; Fern, Alison; Kirton, Edward S.; He, Shaomei; Woyke, Tanja; Lee, Janey; Tringe, Susannah G.] Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Tremblay, Julien] Natl Res Council Canada, Montreal, PQ, Canada. [Chen, Feng] Illumina Inc, San Francisco, CA USA. [Dangl, Jeffery L.] Univ N Carolina, Dept Biol, Chapel Hill, NC USA. [Dangl, Jeffery L.] Univ N Carolina, Dept Microbiol & Immunol, Howard Hughes Med Inst, Curriculum Genet & Mol Biol,Carolina Ctr Genome S, Chapel Hill, NC USA. RP Tringe, SG (reprint author), Dept Energy Joint Genome Inst, 2800 Mitchell Dr Bldg 400, Walnut Creek, CA 94598 USA. EM sgtringe@lbl.gov OI Tringe, Susannah/0000-0001-6479-8427 FU DOE Office of Science User Facility [DE-ACO2-05CH11231]; US NSF grant [IOS-0958245]; DOE Early Career Research Program [KP/CH57/1] FX We thank Mingkun Li, Alex Copeland, and James Han for the DUK kmer matching tool. We also thank Chris Daum for technical insight on the MiSeq system. The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-ACO2-05CH11231. JT was supported by a subcontract to US NSF grant IOS-0958245 (JD) and SH and SGT were supported by the DOE Early Career Research Program, grant number KP/CH57/1. We also thank the two reviewers for their time, constructive comments and suggestions. JT planned experimental design, wrote software, analyzed data and wrote manuscript. EK wrote software. KS, AF, and FC did 16S library preparation and DNA sequence generation. ST participated in experimental design and manuscript writing/editing and analyzed data. SH prepared wetlands metagenome samples. TW and JL prepared isolate genomic DNA for P. suwonensis and synthetic community experiments. JD edited manuscript. NR 65 TC 33 Z9 33 U1 11 U2 77 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 4 PY 2015 VL 6 AR 771 DI 10.3389/fmicb.2015.00771 PG 15 WC Microbiology SC Microbiology GA CO9HA UT WOS:000359484200001 PM 26300854 ER PT J AU Lougovski, P Uskov, DB AF Lougovski, P. Uskov, D. B. TI Channel-capacity gain in entanglement-assisted communication protocols based exclusively on linear optics, single-photon inputs, and coincidence photon counting SO PHYSICAL REVIEW A LA English DT Article ID TELEPORTATION AB Entanglement can effectively increase communication channel capacity as evidenced by dense coding that predicts a capacity gain of 1 bit when compared to entanglement-free protocols. However, dense coding relies on Bell states and when implemented using photons the capacity gain is bounded by 0.585 bits due to one's inability to discriminate between the four optically encoded Bell states. In this paper we study the following question: Are there alternative entanglement-assisted protocols that rely only on linear optics, coincidence photon counting, and separable single-photon input states and at the same time provide a greater capacity gain than 0.585 bits? We show that besides the Bell states there is a class of bipartite four-mode two-photon entangled states that facilitate an increase in channel capacity. We also discuss how the proposed scheme can be generalized to the case of two-photon N-mode entangled states for N = 6,8. C1 [Lougovski, P.] Oak Ridge Natl Lab, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. [Uskov, D. B.] Univ Brescia, Dept Math & Nat Sci, Owensboro, KY 42301 USA. [Uskov, D. B.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. RP Lougovski, P (reprint author), Oak Ridge Natl Lab, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. EM lougovskip@ornl.gov; dmitry.uskov@brescia.edu FU US Department of Energy [DE-AC05-00OR22725]; NSF [PHY-1005709] FX This work was performed at Oak Ridge National Laboratory, operated by UT-Battelle for the US Department of Energy under Contract No. DE-AC05-00OR22725. P.L. would like to thank W.P. Grice for useful discussion. D.B.U. acknowledges support from the NSF under Grant No. PHY-1005709. NR 12 TC 2 Z9 2 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD AUG 4 PY 2015 VL 92 IS 2 AR 022303 DI 10.1103/PhysRevA.92.022303 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CO1MT UT WOS:000358920100002 ER PT J AU Bahran, R Barry, D Block, R Leinweber, G Rapp, M Daskalakis, A Blain, E Williams, D McDermott, B Leal, L Danon, Y AF Bahran, R. Barry, D. Block, R. Leinweber, G. Rapp, M. Daskalakis, A. Blain, E. Williams, D. McDermott, B. Leal, L. Danon, Y. TI Isotopic molybdenum total neutron cross section in the unresolved resonance region SO PHYSICAL REVIEW C LA English DT Article ID ENERGY-RANGE; NUCLEAR-DATA; FLUCTUATIONS; ENDF/B-VII.1; COVARIANCES; PARAMETERS; JENDL-4.0 AB Accurate isotopic molybdenum nuclear data are important because molybdenum can exist in nuclear reactor components including fuel, cladding, or as a high yield fission product. High-resolution time-of-flight neutron transmission measurements on highly enriched isotopic metallic samples of Mo-95, Mo-96, Mo-98, and Mo-100 were performed in the resonance energy range from 1 to 620 keV. The measurements were taken with the newly developed modular Li-6-glass transmission detector positioned at the 100-m experimental flight station. In the unresolved energy region (URR), new comprehensive methods of analysis were developed and validated in order to obtain accurate neutron total cross-section data from the measurement by correcting for background and transmission enhancement effects. Average parameters and fits to the total cross section for 95Mo were obtained using the Hauser-Feshbach statistical model code FITACS, which is currently incorporated into the SAMMY code. The fits to the experimental data deviate from the current evaluated nuclear data file/B-VII.1 isotopic Mo evaluations by several percent in the URR. C1 [Bahran, R.; Daskalakis, A.; Blain, E.; Williams, D.; McDermott, B.; Danon, Y.] Rensselaer Polytech Inst, Gaerttner LINAC Ctr, Troy, NY 12180 USA. [Barry, D.; Block, R.; Leinweber, G.; Rapp, M.] Bechtel Marine Prop Corp, Knolls Atom Power Lab, Schenectady, NY 12301 USA. [Leal, L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Bahran, R (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM bahran@lanl.gov FU Knolls Atomic Power Laboratory (KAPL) FX The authors would like to thank P. Brand, M. Gray, M. Strock, and A. Kerdoun for their efforts in operating the LINAC and their help in setting up experiments. They would also like to thank T. Sutton, P. Romano, C. Lubitz, B. Becker, P. Schillebeeckx, and T. Trumbull for helpful discussions regarding theory and analysis methods in the unresolved resonance region. This research endeavor was made possible with funding generously provided by Knolls Atomic Power Laboratory (KAPL). NR 52 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 4 PY 2015 VL 92 IS 2 AR 024601 DI 10.1103/PhysRevC.92.024601 PG 10 WC Physics, Nuclear SC Physics GA CO1RU UT WOS:000358933700003 ER PT J AU Detmold, W Lehner, C Meinel, S AF Detmold, William Lehner, Christoph Meinel, Stefan TI Lambda(b) -> pl(-)(nu)over-bar(l) and Lambda(b) -> Lambda(c)l(-)(nu)over-bar(l) form factors from lattice QCD with relativistic heavy quarks SO PHYSICAL REVIEW D LA English DT Article ID SEMILEPTONIC DECAY; CHIRAL FERMIONS; GAUGE-THEORY; SUM-RULES; BARYONS; RENORMALIZATION AB Measurements of the Lambda(b) -> pl(-)(nu) over bar (l) and Lambda(b) ->Lambda(c)l(-)(nu) over bar (l) decay rates can be used to determine the magnitudes of the Cabibbo-Kobayashi-Maskawa matrix elements V-ub and V-cb, provided that the relevant hadronic form factors are known. Here we present a precise calculation of these form factors using lattice QCD with 2 + 1 flavors of dynamical domain-wall fermions. The b and c quarks are implemented with relativistic heavy-quark actions, allowing us to work directly at the physical heavy-quark masses. The lattice computation is performed for six different pion masses and two different lattice spacings, using gauge-field configurations generated by the RBC and UKQCD Collaborations. The b -> u and b -> c currents are renormalized with a mostly nonperturbative method. We extrapolate the form factor results to the physical pion mass and the continuum limit, parametrizing the q(2) dependence using z expansions. The form factors are presented in such a way as to enable the correlated propagation of both statistical and systematic uncertainties into derived quantities such as differential decay rates and asymmetries. Using these form factors, we present predictions for the Lambda(b) -> pl(-)(nu) over bar (l) and Lambda(b) ->Lambda(c)l(-)(nu) over bar (l) differential and integrated decay rates. Combined with experimental data, our results enable determinations of vertical bar V-ub vertical bar, vertical bar V-cb vertical bar, and vertical bar V-ub/V-cb vertical bar with theory uncertainties of 4.4%, 2.2%, and 4.9%, respectively. C1 [Detmold, William] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. [Lehner, Christoph] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Meinel, Stefan] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Meinel, Stefan] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Meinel, S (reprint author), Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. EM smeinel@email.arizona.edu FU National Science Foundation [OCI-1053575]; U.S. Department of Energy [DE-AC02-05CH11231, DE-AC02-98CH10886]; RHIC Physics Fellow Program of the RIKEN BNL Research Center; U.S. Department of Energy Early Career Research Award [DE-SC0010495]; Solomon Buchsbaum Fund at MIT FX We thank William Sutcliffe, Ulrik Egede, and Patrick Owen for numerous discussions about the analysis of the decays Lambdab -> p mu(nu) over bar mu and Lambdab -> Lambdacmu(nu) over bar mu using LHCb data, and Gil Paz for comments regarding the z expansion. We are grateful to the RBC and UKQCD collaborations for making their gauge-field configurations available. The lattice calculations were carried out using the CHROMA software [72] on high-performance computing resources provided by XSEDE (supported by National Science Foundation Grant No. OCI-1053575) and NERSC (supported by U.S. Department of Energy Grant No. DE-AC02-05CH11231). S. M. is supported by the RHIC Physics Fellow Program of the RIKEN BNL Research Center. W. D. is supported by the U.S. Department of Energy Early Career Research Award No. DE-SC0010495 and the Solomon Buchsbaum Fund at MIT. C. L. is supported by the U.S. Department of Energy Contract No. DE-AC02-98CH10886(BNL). NR 72 TC 21 Z9 21 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 4 PY 2015 VL 92 IS 3 AR 034503 DI 10.1103/PhysRevD.92.034503 PG 34 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO1SP UT WOS:000358935800002 ER PT J AU Ticknor, C Collins, LA Kress, JD AF Ticknor, Christopher Collins, Lee A. Kress, Joel D. TI Transport properties and equation of state for HCNO mixtures in and beyond the warm dense matter regime SO PHYSICAL REVIEW E LA English DT Article ID UNIVERSAL SCALING LAW; AVERAGE ATOM MODELS; STATISTICAL-MECHANICS; MOLECULAR-DYNAMICS; COEFFICIENTS; DIFFUSION; SYSTEMS; SPHERE AB We present simulations of a four-component mixture of HCNO with orbital free molecular dynamics (OFMD). These simulations were conducted for 5-200 eV with densities ranging between 0.184 and 36.8 g/cm(3). We extract the equation of state from the simulations and compare to average atom models. We found that we only need to add a cold curve model to find excellent agreement. Additionally, we studied mass transport properties. We present fits to the self-diffusion and shear viscosity that are able to reproduce the transport properties over the parameter range studied. We compare these OFMD results to models based on the Coulomb coupling parameter and one-component plasmas. C1 [Ticknor, Christopher; Collins, Lee A.; Kress, Joel D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ticknor, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Ticknor, Christopher/B-8651-2014; OI Ticknor, Christopher/0000-0001-9972-4524 FU Advanced Simulation and Computing (ASC) Program; NNSA of the U.S. Department of Energy [DE-AC52-06NA25396] FX The authors acknowledge illuminating discussions with E. Meyer and J. Coe. The authors gratefully acknowledge support from Advanced Simulation and Computing (ASC) Program, computing resources from CCC, and LANL, which is operated by LANS, LLC for the NNSA of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 54 TC 1 Z9 1 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 4 PY 2015 VL 92 IS 2 AR 023101 DI 10.1103/PhysRevE.92.023101 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CO1SZ UT WOS:000358936800010 PM 26382529 ER PT J AU Travesset, A AF Travesset, Alex TI Binary nanoparticle superlattices of soft-particle systems SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE phase separation; superlattices; crystalline phases; stoichiometry ID DNA; CRYSTALLIZATION; PACKING; MIXTURES; PHASES AB The solid-phase diagram of binary systems consisting of particles of diameter sigma(A) = sigma and sigma(B) = gamma sigma (gamma <= 1) interacting with an inverse p = 12 power law is investigated as a paradigm of a soft potential. In addition to the diameter ratio. that characterizes hard-sphere models, the phase diagram is a function of an additional parameter that controls the relative interaction strength between the different particle types. Phase diagrams are determined from extremes of thermodynamic functions by considering 15 candidate lattices. In general, it is shown that the phase diagram of a soft repulsive potential leads to the morphological diversity observed in experiments with binary nanoparticles, thus providing a general framework to understand their phase diagrams. Particular emphasis is given to the two most successful crystallization strategies so far: evaporation of solvent from nanoparticles with grafted hydrocarbon ligands and DNA programmable self-assembly. C1 Iowa State Univ, Dept Phys & Astron, Ames Lab, Ames, IA 50011 USA. RP Travesset, A (reprint author), Iowa State Univ, Dept Phys & Astron, Ames Lab, Ames, IA 50011 USA. EM trvsst@ameslab.gov FU US Department of Energy (DOE), Basic Energy Sciences, Materials Science and Engineering Division; US DOE [DE-AC02-07CH11358] FX A.T. acknowledges interesting discussions with M. Boles, C. Calero, N. Horst, C. Knorowski, O. Gang, G. Miller, D. Talapin, and D. Vaknin. I thank T. Kennedy for many important discussions and encouragement during the course of this work. Warm thanks for the use of computer cluster Cystorm at Iowa State, which has been purchased from multiple National Science Foundation (NSF) grants. This work is supported by the US Department of Energy (DOE), Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the US DOE by Iowa State University under Contract DE-AC02-07CH11358. NR 39 TC 11 Z9 11 U1 5 U2 27 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 4 PY 2015 VL 112 IS 31 BP 9563 EP 9567 DI 10.1073/pnas.1504677112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO1QQ UT WOS:000358930600045 PM 26195799 ER PT J AU Tan, BS Harrison, N Zhu, Z Balakirev, F Ramshaw, BJ Srivastava, A Sabok, SA Dabrowski, B Lonzarich, GG Sebastian, SE AF Tan, B. S. Harrison, N. Zhu, Z. Balakirev, F. Ramshaw, B. J. Srivastava, A. Sabok, S. A. Dabrowski, B. Lonzarich, G. G. Sebastian, Suchitra E. TI Fragile charge order in the nonsuperconducting ground state of the underdoped high-temperature superconductors SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE superconductivity; strongly correlated electron systems; high-Tc cuprate superconductors; Fermi surface; charge order ID T-C SUPERCONDUCTORS; FERMI-SURFACE; QUANTUM OSCILLATIONS; DENSITY-WAVE; PSEUDOGAP; YBA2CU3OY; DISORDER; CUPRATE AB The normal state in the hole underdoped copper oxide superconductors has proven to be a source of mystery for decades. The measurement of a small Fermi surface by quantum oscillations on suppression of superconductivity by high applied magnetic fields, together with complementary spectroscopic measurements in the hole underdoped copper oxide superconductors, point to a nodal electron pocket from charge order in YBa2Cu3O6+delta. Here, we report quantum oscillation measurements in the closely related stoichiometric material YBa2Cu4O8, which reveals similar Fermi surface properties to YBa2Cu3O6+delta, despite the nonobservation of charge order signatures in the same spectroscopic techniques, such as X-ray diffraction, that revealed signatures of charge order in YBa2Cu3O6+delta. Fermi surface reconstruction in YBa2Cu4O8 is suggested to occur from magnetic field enhancement of charge order that is rendered fragile in zero magnetic fields because of its potential unconventional nature and/or its occurrence as a subsidiary to more robust underlying electronic correlations. C1 [Tan, B. S.; Srivastava, A.; Lonzarich, G. G.; Sebastian, Suchitra E.] Univ Cambridge, Cavendish Lab, Cambridge CB3 OHE, England. [Harrison, N.; Zhu, Z.; Balakirev, F.; Ramshaw, B. J.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Sabok, S. A.; Dabrowski, B.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Sebastian, SE (reprint author), Univ Cambridge, Cavendish Lab, Cambridge CB3 OHE, England. EM suchitra@phy.cam.ac.uk FU Royal Society; Winton Programme for the Physics of Sustainability; European Research Council (ERC) under European Union Seventh Framework Programme Grant FP/ERC [337425]; US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES)-Materials Sciences and Engineering (MSE) Science of 100 Tesla Programme; Engineering and Physical Sciences Research Council (EPSRC) [EP/K012894/1]; Institute for Nanoscience, Engineering, and Technology; National Science Foundation [DMR-0654118]; State of Florida; DOE FX We thank B. Keimer, S. A. Kivelson, M. le Tacon, P. A. Lee, C. Pepin, S. Sachdev, and T. Senthil for useful discussions. We also thank the National High Magnetic Field Laboratory personnel, including J. B. Betts, Y. Coulter, M. J. Gordon, C. H. Mielke, M. D. Pacheco, A. Parish, R. D. McDonald, D. Rickel, and D. Roybal, for experimental assistance. B.S.T., A.S., and S.E.S. acknowledge support from the Royal Society, the Winton Programme for the Physics of Sustainability, and the European Research Council (ERC) under European Union Seventh Framework Programme Grant FP/2007-2013/ERC Grant Agreement 337425. N.H., Z.Z., F.B., and B.J.R. acknowledge support for high-magnetic field experiments from US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES)-Materials Sciences and Engineering (MSE) Science of 100 Tesla Programme. G.G.L. acknowledges support from Engineering and Physical Sciences Research Council (EPSRC) Grant EP/K012894/1. Work at Northern Illinois University was supported by the Institute for Nanoscience, Engineering, and Technology. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement DMR-0654118, the State of Florida, and the DOE. NR 42 TC 5 Z9 5 U1 4 U2 23 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 4 PY 2015 VL 112 IS 31 BP 9568 EP 9572 DI 10.1073/pnas.1504164112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO1QQ UT WOS:000358930600046 PM 26199413 ER PT J AU Chen, JG AF Chen, Jin-Gui TI Phosphorylation of RACK1 in plants SO PLANT SIGNALING & BEHAVIOR LA English DT Review DE Arabidopsis; kinase; phosphorylation; protein degradation; RACK1; scaffold protein; WNK8 ID ARABIDOPSIS-THALIANA; PROTEIN; TRANSLATION; REGULATOR; RIBOSOME; KINASE AB Receptor for Activated C Kinase 1 (RACK1) is a versatile scaffold protein that interacts with a large, diverse group of proteins to regulate various signaling cascades. RACK1 has been shown to regulate hormonal signaling, stress responses and multiple processes of growth and development in plants. However, little is known about the molecular mechanism underlying these regulations. Recently, it has been demonstrated that Arabidopsis RACK1 is phosphorylated by an atypical serine/threonine protein kinase, WITH NO LYSINE 8 (WNK8). Furthermore, RACK1 phosphorylation by WNK8 negatively regulates RACK1 function by influencing its protein stability. These findings promote a new regulatory system in which the action of RACK1 is controlled by phosphorylation and subsequent protein degradation. C1 Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Chen, JG (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM chenj@ornl.gov RI Chen, Jin-Gui/A-4773-2011 OI Chen, Jin-Gui/0000-0002-1752-4201 NR 23 TC 1 Z9 1 U1 0 U2 3 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1559-2316 EI 1559-2324 J9 PLANT SIGNAL BEHAV JI Plant Signal. Behav. PD AUG 3 PY 2015 VL 10 IS 8 AR e1022013 DI 10.1080/15592324.2015.1022013 PG 2 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA CQ0WG UT WOS:000360317900004 PM 26322575 ER PT J AU Forlani, G Makarova, KS Ruszkowski, M Bertazzini, M Nocek, B AF Forlani, Giuseppe Makarova, Kira S. Ruszkowski, Milosz Bertazzini, Michele Nocek, Boguslaw TI Evolution of plant delta(1)-pyrroline-5-carboxylate reductases from phylogenetic and structural perspectives SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE P5C reductase; phylogenetic analysis; 3-D structures of P5CRs; oligomer structure prediction; cofactor preference ID PROTEIN-PROTEIN INTERACTIONS; PYRROLINE-5-CARBOXYLATE REDUCTASE; PROLINE BIOSYNTHESIS; STREPTOCOCCUS-PYOGENES; ESCHERICHIA-COLI; COFACTOR BINDING; P5C REDUCTASE; AMINO-ACID; PURIFICATION; SEQUENCE AB Proline plays a crucial role in cell growth and stress responses, and its accumulation is essential for the tolerance of adverse environmental conditions in plants. Two routes are used to biosynthesize proline in plants. The main route uses glutamate as a precursor, while in the other route proline is derived from ornithine. The terminal step of both pathways, the conversion of delta(1)-pyrroline-5-carboxylate (P5C) to L-proline, is catalyzed by P5C reductase (P5CR) using NADH or NADPH as a cofactor. Since P5CRs are important housekeeping enzymes, they are conserved across all domains of life and appear to be relatively unaffected throughout evolution. However, global analysis of these enzymes unveiled significant functional diversity in the preference for cofactors (NADPH vs. NADH), variation in metal dependence and the differences in the oligomeric state. In our study we investigated evolutionary patterns through phylogenetic and structural analysis of P5CR representatives from all kingdoms of life, with emphasis on the plant species. We also attempted to correlate local sequence/structure variation among the functionally and structurally characterized members of the family. C1 [Forlani, Giuseppe; Bertazzini, Michele] Univ Ferrara, Dept Life Sci & Biotechnol, I-44100 Ferrara, Italy. [Makarova, Kira S.] NIH, Natl Ctr Biotechnol Informat, Natl Lib Med, Bethesda, MD 20892 USA. [Ruszkowski, Milosz] NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne Natl Lab, Argonne, IL USA. [Nocek, Boguslaw] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Nocek, B (reprint author), Argonne Natl Lab, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM bnocek@anl.gov RI Forlani, Giuseppe/B-7869-2009 OI Forlani, Giuseppe/0000-0003-2598-5718 FU Intramural Research Program of the NCI, Center for Cancer Research FX We are grateful to Rory Mulligan, Cathy Hatzos-Skintges, Magdalena Makowska-Grzyska, Jurek Osipiuk, and Zbyszek Dauter for their comments and critical reading of the manuscript. Project was partially supported by the Intramural Research Program of the NCI, Center for Cancer Research. NR 70 TC 4 Z9 4 U1 4 U2 11 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD AUG 3 PY 2015 VL 6 AR 567 DI 10.3389/fpls.2015.00567 PG 15 WC Plant Sciences SC Plant Sciences GA CP5DJ UT WOS:000359901200001 PM 26284089 ER PT J AU Dau, PD Wilson, RE Gibson, JK AF Dau, Phuong D. Wilson, Richard E. Gibson, John K. TI Elucidating Protactinium Hydrolysis: The Relative Stabilities of PaO2(H2O)(+) and PaO(OH)(2)(+) SO INORGANIC CHEMISTRY LA English DT Article ID GAS-PHASE URANYL; AQUEOUS-SOLUTION; SOLVENT-EXTRACTION; ACTINIDE CHEMISTRY; PERCHLORIC-ACID; OXO-EXCHANGE; PROTACTINIUM(V); COMPLEXES; DISSOCIATION; HYDRATION AB It is demonstrated that the gas-phase oxo-exchange of PaO2+ with water is substantially faster than that of UO2+, indicating that the Pa-O bonds are more susceptible to activation and formation of the bis-hydroxide intermediate, PaO(OH)(2)(+). To elucidate the nature of the water adduct of PaO2+, hydration of PaO2+ and UO2+, as well as collision induced dissociation (CID) and ligand-exchange of the water adducts of PaO2+ and UO2+, was studied. The results indicate that, in contrast to UO2(H2O)(+), the protactinium oxo bis-hydroxide isomer, PaO(OH)(2)(+), is produced as a gas-phase species close in energy to the hydrate isomer, PaO2(H2O)(+). CID behavior similar to that of Th(OH)(3) supports the assignment as PaO(OH)(2)(+). The gas-phase results are consistent with the spontaneous hydrolysis of PaO2 in aqueous solution, this in contrast to later AnO(2)(+) (An = U, Np, Pu), which forms stable hydrates in both solution and gas phase. In view of the known propensity for Th(IV) to hydrolyze, and previous gas-phase studies of other AnO(2)(+), it is concluded that the stabilities of oxo-hydroxides relative to oxide hydrates decreases in the order: Th(IV) > Pa(V) > U(V) > Np(V) > Pu(V). This trend suggests increasing covalency and decreasing ionicity of An-O bonds upon proceeding across the actinide series. C1 [Dau, Phuong D.; Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Wilson, Richard E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Gibson, JK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jkgibson@lbl.gov RI Wilson, Richard/H-1763-2011 OI Wilson, Richard/0000-0001-8618-5680 FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; U.S. Department of Energy Basic Energy Sciences, Early Career Research Award Program [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract No. DE-AC02-05CH11231 (to P.D.D. and J.K.G), and by the U.S. Department of Energy Basic Energy Sciences, Early Career Research Award Program, under Contract DE-AC02-06CH11357 (to R.E.W.). NR 66 TC 5 Z9 5 U1 11 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 3 PY 2015 VL 54 IS 15 BP 7474 EP 7480 DI 10.1021/acs.inorgchem.5b01078 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CO3YE UT WOS:000359096400039 PM 26203499 ER PT J AU Landon, CD Wilke, RHT Brumbach, MT Brennecka, GL Blea-Kirby, M Ihlefeld, JF Marinella, MJ Beechem, TE AF Landon, Colin D. Wilke, Rudeger H. T. Brumbach, Michael T. Brennecka, Geoff L. Blea-Kirby, Mia Ihlefeld, Jon F. Marinella, Matthew J. Beechem, Thomas E. TI Thermal transport in tantalum oxide films for memristive applications (vol 107, 023108, 2015) SO APPLIED PHYSICS LETTERS LA English DT Correction C1 [Landon, Colin D.; Wilke, Rudeger H. T.; Brumbach, Michael T.; Blea-Kirby, Mia; Ihlefeld, Jon F.; Marinella, Matthew J.; Beechem, Thomas E.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Brennecka, Geoff L.] Colorado Sch Mines, Golden, CO 80401 USA. RP Landon, CD (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. RI Brennecka, Geoff/J-9367-2012 OI Brennecka, Geoff/0000-0002-4476-7655 NR 3 TC 0 Z9 0 U1 3 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 3 PY 2015 VL 107 IS 5 AR 059902 DI 10.1063/1.4928532 PG 1 WC Physics, Applied SC Physics GA CO7XB UT WOS:000359375700056 ER PT J AU Shi, XY Yu, WL Hawkins, SD Klem, JF Pan, W AF Shi, Xiaoyan Yu, Wenlong Hawkins, S. D. Klem, J. F. Pan, W. TI McMillan-Rowell like oscillations in a superconductor-InAs/GaSb-superconductor junction SO APPLIED PHYSICS LETTERS LA English DT Article ID TOPOLOGICAL INSULATORS; ANDREEV REFLECTIONS; MAJORANA FERMIONS; NANOWIRE; TRANSITION; EDGE; SIGNATURE; SYMMETRY AB We have fabricated a superconductor (Ta)-InAs/GaSb bilayer-superconductor (Ta) junction device that has a long mean free path and can preserve the wavelike properties of particles (electrons and holes) inside the junction. Differential conductance measurements were carried out at low temperatures in this device, and McMillan-Rowell like oscillations (MROs) were observed. Surprisingly, a much larger Fermi velocity, compared to that from Shubnikov-de Haas oscillations, was obtained from the frequency of MROs. Possible mechanisms are discussed for this discrepancy. (C) 2015 AIP Publishing LLC. C1 [Shi, Xiaoyan; Yu, Wenlong; Hawkins, S. D.; Klem, J. F.; Pan, W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Shi, XY (reprint author), Sandia Natl Labs, Albuquerque, NM 87185 USA. EM xshi@sandia.gov RI Shi, Xiaoyan/L-4893-2015 OI Shi, Xiaoyan/0000-0002-9974-4637 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory [DEAC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX X.S. thanks Meenakshi Singh for helpful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Device fabrication was performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory (Contract No. DEAC52-06NA25396), and Sandia National Laboratories (Contract No. DE-AC04-94AL85000). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 31 TC 2 Z9 2 U1 5 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 3 PY 2015 VL 107 IS 5 AR 052601 DI 10.1063/1.4928186 PG 3 WC Physics, Applied SC Physics GA CO7XB UT WOS:000359375700021 ER PT J AU Winchester, B Balke, N Cheng, XX Morozovska, AN Kalinin, S Chen, LQ AF Winchester, B. Balke, N. Cheng, X. X. Morozovska, A. N. Kalinin, S. Chen, L. Q. TI Electroelastic fields in artificially created vortex cores in epitaxial BiFeO3 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROELECTRIC DOMAIN-STRUCTURES AB We employ phase-field modeling to explore the elastic properties of artificially created 1-D domain walls in (001)(p)-oriented BiFeO3 thin films, composed of a junction of the four polarization variants, all with the same out-of-plane polarization. It was found that these junctions exhibit peculiarly high electroelastic fields induced by the neighboring ferroelastic/ferroelectric domains. The vortex core exhibits a volume expansion, while the anti-vortex core is more compressive. Possible ways to control the electroelastic field, such as varying material constant and applying transverse electric field, are also discussed. (C) 2015 AIP Publishing LLC. C1 [Winchester, B.; Cheng, X. X.; Chen, L. Q.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Balke, N.; Kalinin, S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Ridge, TN 37831 USA. [Morozovska, A. N.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, Kiev, Ukraine. RP Winchester, B (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. EM benjaminwinchester@gmail.com RI Balke, Nina/Q-2505-2015 OI Balke, Nina/0000-0001-5865-5892 FU Department of Energy Basic Sciences [DOE DE-FG02-07ER46417]; Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility FX The authors appreciate the financial support of the Department of Energy Basic Sciences under Grant No. DOE DE-FG02-07ER46417. N.B. and S.K. were supported by the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 19 TC 2 Z9 2 U1 4 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 3 PY 2015 VL 107 IS 5 AR 052903 DI 10.1063/1.4927750 PG 5 WC Physics, Applied SC Physics GA CO7XB UT WOS:000359375700024 ER PT J AU Moses-DeBusk, M Allard, LF Blom, DA Narula, CK AF Moses-DeBusk, Melanie Allard, Lawrence F. Blom, Douglas A. Narula, Chaitanya K. TI Oxidation-Induced Structural Changes in Sub-Nanometer Platinum Supported on Alumina SO CHEMCATCHEM LA English DT Article DE aluminum; oxidation; platinum; scanning probe microscopy; supported catalysts ID CARBON-MONOXIDE; CO OXIDATION; THETA-AL2O3(010) SURFACE; CATALYTIC-OXIDATION; GOLD NANOPARTICLES; ELEMENTARY STEPS; SINGLE; ATOMS; GAMMA-AL2O3 AB Pt supported on alumina is an essential component of emission treatment catalysts used in transportation. Theoretical, experimental, and mechanistic aspects of Pt particles supported on a variety of supports have been studied extensively; however, available experimental information on the behavior of single versus sub-nanometer Pt is extremely limited. To bridge the knowledge gap between single supported Pt and well-formed supported Pt nanoparticles, we have performed the synthesis, characterization, and CO and NO oxidation studies of sub-nanometer Pt supported on -, -, and -Al2O3 and monitored the changes in structure upon exposure to CO and NO oxidation conditions. We find that sub-nanometer Pt is highly effective for CO oxidation because of the high Pt dispersion, but it is not very efficient as a NO oxidation catalyst. Furthermore, sub-nanometer Pt agglomerates rapidly under CO or NO oxidation conditions to form nanoparticles. C1 [Allard, Lawrence F.; Blom, Douglas A.; Narula, Chaitanya K.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Moses-DeBusk, Melanie] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Narula, CK (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM narulack@ornl.gov OI Moses-DeBusk, Melanie/0000-0003-0382-0824 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program [DE-AC05-ooOR22725]; UT-Battelle, LLC FX The research was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program under contract DE-AC05-ooOR22725 with UT-Battelle, LLC. The Hitachi HD-2000 work was performed at the Oak Ridge National Laboratory's Center for Nanophase Materials Sciences (user proposal #CNMS2008-042). NR 34 TC 0 Z9 0 U1 8 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1867-3880 EI 1867-3899 J9 CHEMCATCHEM JI ChemCatChem PD AUG 3 PY 2015 VL 7 IS 15 BP 2391 EP 2396 DI 10.1002/cctc.201500267 PG 6 WC Chemistry, Physical SC Chemistry GA CO3OA UT WOS:000359066500017 ER PT J AU Mirmelstein, A Podlesnyak, A dos Santos, AM Ehlers, G Kerbel, O Matvienko, V Sefat, AS Saparov, B Halder, GJ Tobin, JG AF Mirmelstein, A. Podlesnyak, A. dos Santos, Antonio M. Ehlers, G. Kerbel, O. Matvienko, V. Sefat, A. S. Saparov, B. Halder, G. J. Tobin, J. G. TI Pressure-induced structural phase transition in CeNi: X-ray and neutron scattering studies and first-principles calculations SO PHYSICAL REVIEW B LA English DT Article ID CRYSTAL; COMPETITION; STATE; TBNI AB The pressure-induced structural phase transition in the intermediate-valence compound CeNi has been investigated by x-ray and neutron powder diffraction techniques. It is shown that the structure of the pressure-induced CeNi phase (phases) can be described in terms of the Pnma space group. Equations of state for CeNi on both sides of the phase transition are derived and an approximate P-T phase diagram is suggested for P < 8 GPa andT < 300 K. The observed Cmcm -> Pnma structural transition is analyzed using density functional theory calculations, which successfully reproduce the ground state volume, the phase transition pressure, and the volume collapse associated with the phase transition. C1 [Mirmelstein, A.; Kerbel, O.; Matvienko, V.] RFNC, EI Zababakhin Res Inst Tech Phys, Dept Expt Phys, VNIITF, Snezhinsk 456770, Russia. [Podlesnyak, A.; dos Santos, Antonio M.; Ehlers, G.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Sefat, A. S.; Saparov, B.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Halder, G. J.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Tobin, J. G.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. RP Podlesnyak, A (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM podlesnyakaa@ornl.gov RI Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; Tobin, James/O-6953-2015; Podlesnyak, Andrey/A-5593-2013; dos Santos, Antonio/A-5602-2016; Sefat, Athena/R-5457-2016 OI Ehlers, Georg/0000-0003-3513-508X; Podlesnyak, Andrey/0000-0001-9366-6319; dos Santos, Antonio/0000-0001-6900-0816; Sefat, Athena/0000-0002-5596-3504 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; US Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; LLNL [B601122]; RFNC-VNIITF [B601122]; DOE Office of Science [DE-AC02-06CH11357] FX We are grateful to M. V. Ryzhkov for enlightening discussions on the DFT calculations. Research at Oak Ridge National Laboratory's Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Part of this work was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the US Department of Energy, National Nuclear Security Administration, under Contract No. DE-AC52-07NA27344. J.G.T. wishes to thank the Office of Advanced Simulation and Computing for support of his travel to Oak Ridge National Laboratory for experiments at the Spallation Neutron Source. Work at RFNC-VNIITF was supported in part by Contract No. B601122 between LLNL and RFNC-VNIITF. This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 32 TC 0 Z9 0 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 3 PY 2015 VL 92 IS 5 AR 054102 DI 10.1103/PhysRevB.92.054102 PG 8 WC Physics, Condensed Matter SC Physics GA CO1OP UT WOS:000358925200002 ER PT J AU Somoza, AM Ortuno, M Baturina, TI Vinokur, VM AF Somoza, Andres M. Ortuno, Miguel Baturina, Tatyana I. Vinokur, Valerii M. TI Density of states of two-dimensional systems with long-range logarithmic interactions SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR-TRANSITION; CONTINUOUS SYMMETRY GROUP; DIELECTRIC-CONSTANT; CRITICAL-BEHAVIOR; LOCALIZED-ELECTRONS; DISORDERED SYSTEMS; GRANULAR ALUMINUM; PHASE-TRANSITIONS; COULOMB GAP; FILMS AB permittivity systems with logarithmic Coulomb interaction between particles. We derive self-consistent DOS at zero temperature and show that it is appreciably suppressed as compared to the DOS expected from the Efros-Shklovskii approach. We carry out zero-and finite-temperature Monte Carlo numerical studies of the DOS and find the perfect agreement between the numerical and analytical results at zero temperature, observing, in particular, a hardening of the Coulomb gap with the increasing electrostatic screening length. At finite temperatures, we reveal a striking scaling of the DOS as a function of energy normalized to the temperature of the system. C1 [Somoza, Andres M.; Ortuno, Miguel] Univ Murcia, Dept Fis, CIOyN, E-30071 Murcia, Spain. [Baturina, Tatyana I.] Univ Regensburg, D-93053 Regensburg, Germany. [Baturina, Tatyana I.] RAS, AV Rzhanov Inst Semicond Phys, SB, Novosibirsk 630090, Russia. [Baturina, Tatyana I.] Novosibirsk State Univ, Dept Phys, Novosibirsk 630090, Russia. [Vinokur, Valerii M.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60637 USA. RP Somoza, AM (reprint author), Univ Murcia, Dept Fis, CIOyN, E-30071 Murcia, Spain. RI Ortuno, Miguel/A-2107-2008 FU MINECO (Spain); FEDER (EU) [FIS2012-38206]; Ministry of Education and Science of the Russian Federation; Alexander von Humboldt Foundation; US Department of Energy, Office of Science, Materials Sciences and Engineering Division (via the Materials Theory Institute) FX The work was supported by the MINECO (Spain) and FEDER (EU) Grant No. FIS2012-38206; by the Ministry of Education and Science of the Russian Federation and by the Alexander von Humboldt Foundation (T.B.); and by the US Department of Energy, Office of Science, Materials Sciences and Engineering Division (V.V. and partly M.O. and T.B. via the Materials Theory Institute). M.O. thanks Kavli Institute of Theoretical Physics (KITP), University of California, Santa Barbara for hospitality. NR 46 TC 1 Z9 1 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 3 PY 2015 VL 92 IS 6 AR 064201 DI 10.1103/PhysRevB.92.064201 PG 5 WC Physics, Condensed Matter SC Physics GA CO1QH UT WOS:000358929600002 ER PT J AU Gates, JM Gregorich, KE Gothe, OR Uribe, EC Pang, GK Bleuel, DL Block, M Clark, RM Campbell, CM Crawford, HL Cromaz, M Di Nitto, A Dullmann, CE Esker, NE Fahlander, C Fallon, P Farjadi, RM Forsberg, U Khuyagbaatar, J Loveland, W Macchiavelli, AO May, EM Mudder, PR Olive, DT Rice, AC Rissanen, J Rudolph, D Sarmiento, LG Shusterman, JA Stoyer, MA Wiens, A Yakushev, A Nitsche, H AF Gates, J. M. Gregorich, K. E. Gothe, O. R. Uribe, E. C. Pang, G. K. Bleuel, D. L. Block, M. Clark, R. M. Campbell, C. M. Crawford, H. L. Cromaz, M. Di Nitto, A. Duellmann, Ch. E. Esker, N. E. Fahlander, C. Fallon, P. Farjadi, R. M. Forsberg, U. Khuyagbaatar, J. Loveland, W. Macchiavelli, A. O. May, E. M. Mudder, P. R. Olive, D. T. Rice, A. C. Rissanen, J. Rudolph, D. Sarmiento, L. G. Shusterman, J. A. Stoyer, M. A. Wiens, A. Yakushev, A. Nitsche, H. TI Decay spectroscopy of element 115 daughters:(280)Rg -> (276)Mt and (276)Mt -> (272)Bh SO PHYSICAL REVIEW C LA English DT Article ID SIMULATION; NUCLEI AB Forty-six decay chains, assigned to the decay of (288)115, were produced using the Am-243(Ca-48, 3n) (288)115 reaction at the Lawrence Berkeley National Laboratory 88-in. cyclotron. The resulting series of a decays were studied using alpha-photon and alpha-x-ray spectroscopies. Multiple alpha-photon coincidences were observed in the element 115 decay chain members, particularly in the third-and fourth-generation decays (presumed to be (280)Rg and (276)Mt, respectively). Upon combining these data with those from 22 (288)115 decay chains observed in a similar experiment, updated level schemes in (276)Mt and (272)Bh (populated by the alpha decay of (280)Rg and (276)Mt, respectively) are proposed. Photons were observed in the energy range expected for K x rays coincident with the a decay of both (280)Rg and (276)Mt. However, Compton scattering of higher-energy gamma rays and discrete transitions are present in the K x-ray region preventing a definitive Z identification to be made based on observation of characteristic K x-ray energies. C1 [Gates, J. M.; Gregorich, K. E.; Gothe, O. R.; Uribe, E. C.; Pang, G. K.; Clark, R. M.; Campbell, C. M.; Crawford, H. L.; Cromaz, M.; Esker, N. E.; Fallon, P.; Farjadi, R. M.; Macchiavelli, A. O.; May, E. M.; Mudder, P. R.; Olive, D. T.; Rice, A. C.; Rissanen, J.; Shusterman, J. A.; Wiens, A.; Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gothe, O. R.; Uribe, E. C.; Esker, N. E.; May, E. M.; Mudder, P. R.; Olive, D. T.; Rice, A. C.; Shusterman, J. A.; Nitsche, H.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Bleuel, D. L.; Stoyer, M. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Block, M.; Duellmann, Ch. E.; Khuyagbaatar, J.; Yakushev, A.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Di Nitto, A.; Duellmann, Ch. E.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Duellmann, Ch. E.; Khuyagbaatar, J.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Fahlander, C.; Forsberg, U.; Rudolph, D.; Sarmiento, L. G.] Lund Univ, S-22100 Lund, Sweden. [Loveland, W.] Oregon State Univ, Corvallis, OR 97331 USA. RP Gates, JM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM jmgates@lbl.gov RI Rudolph, Dirk/D-4259-2009; Block, Michael/I-2782-2015; Di Nitto, Antonio/C-5069-2011; OI Rudolph, Dirk/0000-0003-1199-3055; Block, Michael/0000-0001-9282-8347; Di Nitto, Antonio/0000-0002-9319-366X; Uribe, Eva/0000-0001-7755-2653 FU US Department of Energy, Office of Science, Office of High Energy and Nuclear Physics [DE-AC02-05CH11231, DE-FG06-97ER41026]; Royal Physiographic Society in Lund; Swedish Research Council; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Helmholtz-Institute Mainz FX We gratefully acknowledge the operations staff of the 88-in. cyclotron for proving the intense beams of 48Ca. The authors are indebted (for the use of 243Am) to the Division of Chemical Sciences, Office of Basic Energy Services, US Department of Energy, through the transplutonium element production facilities at Oak Ridge National Laboratory. This material is based upon work supported by the US Department of Energy, Office of Science, Office of High Energy and Nuclear Physics under Contracts No. DE-AC02-05CH11231 and No. DE-FG06-97ER41026, the Swedish Research Council, and the Royal Physiographic Society in Lund. The LLNL contribution was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. A.DiN. is financially supported by the Helmholtz-Institute Mainz. NR 27 TC 15 Z9 15 U1 3 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD AUG 3 PY 2015 VL 92 IS 2 AR 021301 DI 10.1103/PhysRevC.92.021301 PG 6 WC Physics, Nuclear SC Physics GA CO1RS UT WOS:000358933500001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D 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Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for type-III seesaw heavy leptons in pp collisions at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID NEUTRINO MASSES; LHC AB A search for the pair production of heavy leptons (N-0, L-+/-) predicted by the type-III seesaw theory formulated to explain the origin of small neutrino masses is presented. The decay channels N-0 -> W(+/-)l(+/-) (l = e, mu, tau) and L-+/- -> W(+/-)v (v = v(e), v(mu), v(tau)) are considered. The analysis is performed using the final state that contains two leptons (electrons or muons), two jets from a hadronically decaying W boson and large missing transverse momentum. The data used in the measurement correspond to an integrated luminosity of 20.3 fb(-1) of pp collisions at root s = 8 TeV collected by the ATLAS detector at the LHC. No evidence of heavy lepton pair production is observed. 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J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ma, L. L.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.] Univ Sci & Technol China, Dept Modern Phys, Hebei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Zhang, X.; Zhao, Y.; Zhu, C. G.; Zhu, H.; Zhu, Y.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Pozdnyakov, V.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Genoa, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Plotnikova, E.; Poley, A.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Plotnikova, E.; Poley, A.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Kuday, S.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Lambourne, L.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Djobava, T.; Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St. Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Potrap, I. N.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Becker, M.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Ponce, J. M. Iturbe; Keyes, R. A.; Mantifel, R.; Masik, J.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Aad, G.; Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Beddall, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fac Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Graduate Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, SB, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hakobyan, H.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hakobyan, H.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Giannetti, P.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Rome, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Dell'Orso, M.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Departamento Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Fac Ciencias & Tecnol, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Solodkov, A. A.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Giordani, M. P.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Barisonzi, M.; Ceradini, F.; Di Micco, B.; Giordani, M. P.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.; Tayalati, Y.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondament Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Horton, A. J.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Yao, W-M.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Orr, R. S.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Mc Goldrick, G.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.; Valero, A.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Maxfield, S. J.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fac Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Mattig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. RI Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Korol, Aleksandr/A-6244-2014; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Veneziano, Stefano/J-1610-2012; Boldyrev, Alexey/M-9684-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015 OI Price, Darren/0000-0003-2750-9977; Belanger-Champagne, Camille/0000-0003-2368-2617; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Coccaro, Andrea/0000-0003-2368-4559; Della Volpe, Domenico/0000-0001-8530-7447; Sotiropoulou, Calliope-Louisa/0000-0001-9851-1658; Lacasta, Carlos/0000-0002-2623-6252; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Sannino, Mario/0000-0001-7700-8383; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS and CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society, and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, and Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (U.K.) and BNL (USA) and in the Tier-2 facilities worldwide. NR 53 TC 4 Z9 4 U1 9 U2 70 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD AUG 3 PY 2015 VL 92 IS 3 AR 032001 DI 10.1103/PhysRevD.92.032001 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO1SL UT WOS:000358935400001 ER PT J AU Padmanath, M Lang, CB Prelovsek, S AF Padmanath, M. Lang, C. B. Prelovsek, S. TI X(3872) and Y(4140) using diquark-antidiquark operators with lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID QUANTUM-FIELD THEORIES; SCATTERING MATRIX; VOLUME DEPENDENCE; ENERGY-SPECTRUM; FINITE-VOLUME; GAUGE-THEORY; STATES; J/PSI; PARTICLES; RESONANCE AB We perform a lattice study of charmonium-like mesons with JPC(+) = 1(++) and three quark contents (c) over barc (d) over baru, (c) over barc((u) over baru + (d) over bard) and (c) over barc (s) over bars, where the later two can mix with (c) over barc. This simulation with N-f = 2 and m(pi) similar or equal to 266 MeV aims at the possible signatures of four-quark exotic states. We utilize a large basis of (c) over barc, two-meson and diquark-antidiquark interpolating fields, with diquarks in both antitriplet and sextet color representations. A lattice candidate for X(3872) with I = 0 is observed very close to the experimental state only if both (c) over barc and D (D) over bar* interpolators are included; the candidate is not found if diquark-antidiquark and D (D) over bar* are used in the absence of (c) over barc. No candidate for neutral or charged X(3872), or any other exotic candidates are found in the I = 1 channel. We also do not find signatures of exotic (c) over barc (s) over bars ss candidates below 4.2 GeV, such as Y(4140). Possible physics and methodology related reasons for that are discussed. Along the way, we present the diquark-antidiquark operators as linear combinations of the two-meson operators via the Fierz transformations. C1 [Padmanath, M.; Lang, C. B.] Graz Univ, Inst Phys, A-8010 Graz, Austria. [Prelovsek, S.] Univ Ljubljana, Dept Phys, Ljubljana 1000, Slovenia. [Prelovsek, S.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Prelovsek, S.] Ctr Theory, Jefferson Lab, Newport News, VA 23606 USA. RP Padmanath, M (reprint author), Graz Univ, Inst Phys, A-8010 Graz, Austria. EM padmanath.madanagopalan@uni-graz.at; christian.lang@uni-graz.at; sasa.prelovsek@ijs.si FU Austrian Science Fund [FWF:I1313-N27]; Slovenian Research Agency ARRS Project [N1-0020]; U.S. Department of Energy [DE-AC05-06OR23177] FX We thank Anna Hasenfratz and the PACS-CS for providing the gauge configurations. We acknowledge the discussions with R. Briceno, L. Leskovec, D. Mohler, S. Ozaki, S. Sasaki and C. DeTar. The calculations were performed on computing clusters at the University of Graz (NAWI Graz), at the Vienna Scientific Cluster (VSC) and at Jozef Stefan Institute. This work is supported in part by the Austrian Science Fund FWF:I1313-N27 and by the Slovenian Research Agency ARRS Project No. N1-0020. S. P. acknowledges support from U.S. Department of Energy Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates Jefferson Laboratory. NR 91 TC 17 Z9 17 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 3 PY 2015 VL 92 IS 3 AR 034501 DI 10.1103/PhysRevD.92.034501 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO1SL UT WOS:000358935400008 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Anza, F Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bianchi, L Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V St Denis, R Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vzquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Anza, F. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bianchi, L. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. 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CA CDF Collaboration TI Search for Resonances Decaying to Top and Bottom Quarks with the CDF Experiment SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLLISIONS; DETECTOR; ENERGY; MODEL; QCD; W' AB We report on a search for charged massive resonances decaying to top (t) and bottom (b) quarks in the full data set of proton-antiproton collisions at a center-of-mass energy of root s = 1.96 TeV collected by the CDF II detector at the Tevatron, corresponding to an integrated luminosity of 9.5 fb(-1). No significant excess above the standard model background prediction is observed. We set 95% Bayesian credibility mass-dependent upper limits on the heavy charged-particle production cross section times branching ratio to tb. Using a standard model extension with a W' -> tb and left-right-symmetric couplings as a benchmark model, we constrain the W' mass and couplings in the 300-900 GeV/c(2) range. The limits presented here are the most stringent for a charged resonance with mass in the range 300-600 GeV/c(2) decaying to top and bottom quarks. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, Athens 15771, Greece. [Camarda, S.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, ICREA, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Bland, K. R.; Dittmann, J. R.; Hatakeyama, K.; Kasmi, A.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Brigliadori, L.; Castro, A.; Deninno, M.; Gramellini, E.; Marchese, L.; Mazzanti, P.; Moggi, N.; Mussini, M.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl, I-40127 Bologna, Italy. [Brigliadori, L.; Castro, A.; Mussini, M.; Zucchelli, S.] Univ Bologna, I-40127 Bologna, Italy. [Chertok, M.; Conway, J.; Cox, C. A.; Cox, D. J.; Erbacher, R.; Forrest, R.; Ivanov, A.; Pilot, J.; Shalhout, S. Z.; Smith, J. R.; Wilbur, S.] Univ Calif Davis, Davis, CA 95616 USA. [Plager, C.] Univ Calif Los Angeles, Los Angeles, CA 90024 USA. [Casal, B.; Cuevas, J.; Gomez, G.; Palencia, E.; Ruiz, A.; Scodellaro, L.; Vilar, R.; Vizan, J.] Univ Cantabria, CSIC, Inst Fis Cantabria, Santander 39005, Spain. [Calamba, A.; Jang, D.; Jun, S. Y.; Paulini, M.; Russ, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Boveia, A.; Canelli, F.; Frisch, H.; Grosso-Pilcher, C.; Ketchum, W.; Kim, Y. K.; Rosner, J. L.; Shochet, M.; Tang, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Comenius Univ, Bratislava 84248, Slovakia. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Slovak Acad Sci, Inst Expt Phys, Kosice 04001, Slovakia. Joint Inst Nucl Res, RU-141980 Dubna, Russia. [Benjamin, D.; Bocci, A.; Goshaw, A. T.; Kotwal, A. V.; Kruse, M.; Limosani, A.; Oh, S. H.; Phillips, T. 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C.; Yu, I.] Seoul Natl Univ, Seoul 151742, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Chonnam Natl Univ, Gwangju 500757, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. 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[Heinrich, J.; Keung, J.; Kroll, J.; Lipeles, E.; Pianori, E.; Rodriguez, T.; Thomson, E.; Wagner, P.; Whiteson, D.; Williams, H. H.] Univ Penn, Philadelphia, PA 19104 USA. [Barria, P.; Bedeschi, F.; Bellettini, G.; Butti, P.; Carosi, R.; Chiarelli, G.; Cremonesi, M.; Di Canto, A.; Donati, S.; Galloni, C.; Garosi, P.; Introzzi, G.; Latino, G.; Leone, S.; Maestro, P.; Marino, P.; Morello, M. J.; Punzi, G.; Ristori, L.; Ronzani, M.; Ruffini, F.; Scuri, F.; Sforza, F.; Trovato, M.; Vernieri, C.] Ist Nazl Fis Nucl, I-56127 Pisa, Italy. [Bellettini, G.; Butti, P.; Di Canto, A.; Donati, S.; Galloni, C.; Punzi, G.; Ronzani, M.; Sforza, F.] Univ Pisa, I-56127 Pisa, Italy. [Barria, P.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-53100 Siena, Italy. [Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Introzzi, G.] INFN Pavia, I-27100 Pavia, Italy. [Introzzi, G.] Univ Pavia, I-27100 Pavia, Italy. [Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; de Barbaro, P.; Han, J. Y.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [Giagu, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma 1, I-00185 Rome, Italy. [Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy. [Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA. [Casarsa, M.; Cauz, D.; Dorigo, M.; Driutti, A.; Pagliarone, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl, I-34127 Trieste, Italy. 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RP Aaltonen, T (reprint author), Acad Sinica, Inst Phys, Taipei 11529, Taiwan. RI Paulini, Manfred/N-7794-2014; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; OI Paulini, Manfred/0000-0002-6714-5787; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Simonenko, Alexander/0000-0001-6580-3638; Casarsa, Massimo/0000-0002-1353-8964; Devoto, Francesco/0000-0002-3415-7677; Margaroli, Fabrizio/0000-0002-3869-0153; Latino, Giuseppe/0000-0002-4098-3502; iori, maurizio/0000-0002-6349-0380; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756 FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science, and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, U.K.; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science, and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, U.K.; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 34 TC 2 Z9 2 U1 1 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 3 PY 2015 VL 115 IS 6 AR 061801 DI 10.1103/PhysRevLett.115.061801 PG 8 WC Physics, Multidisciplinary SC Physics GA CO1TG UT WOS:000358937600003 PM 26296108 ER PT J AU de Jong, M Kacher, J Sluiter, MHF Qi, L Olmsted, DL van de Walle, A Morris, JW Minor, AM Asta, M AF de Jong, Maarten Kacher, J. Sluiter, M. H. F. Qi, L. Olmsted, D. L. van de Walle, A. Morris, J. W., Jr. Minor, A. M. Asta, M. TI Electronic Origins of Anomalous Twin Boundary Energies in Hexagonal Close Packed Transition Metals SO PHYSICAL REVIEW LETTERS LA English DT Article ID RHENIUM SINGLE-CRYSTALS; QUASI-RANDOM STRUCTURES; WAVE BASIS-SET; AB-INITIO; MOMENTS DEVELOPMENTS; HCP METALS; DEFORMATION; ALLOYS; SYSTEMS; PSEUDOPOTENTIALS AB Density-functional-theory calculations of twin-boundary energies in hexagonal close packed metals reveal anomalously low values for elemental Tc and Re, which can be lowered further by alloying with solutes that reduce the electron per atom ratio. The anomalous behavior is linked to atomic geometries in the interface similar to those observed in bulk tetrahedrally close packed phases. The results establish a link between twin-boundary energetics and the theory of bulk structural stability in transition metals that may prove useful in controlling mechanical behavior in alloy design. C1 [de Jong, Maarten; Kacher, J.; Qi, L.; Olmsted, D. L.; Morris, J. W., Jr.; Minor, A. M.; Asta, M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Kacher, J.; Minor, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Sluiter, M. H. F.] Delft Univ Technol, Dept Mat Sci & Engn, 3mE, NL-2628 CD Delft, Netherlands. [van de Walle, A.] Brown Univ, Sch Engn, Providence, RI 02912 USA. RP de Jong, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM maartendft@gmail.com RI van de Walle, Axel/L-5676-2013; Qi, Liang/A-3851-2010; Sluiter, Marcel/E-6086-2010 OI van de Walle, Axel/0000-0002-3415-1494; Qi, Liang/0000-0002-0201-9333; Sluiter, Marcel/0000-0002-6514-4318 FU Office of Naval Research [N00014-11-1-0886]; National Science Foundation [OCI-1053575]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The research was supported by the Office of Naval Research under Grant No. N00014-11-1-0886, and made use of computational resources through the Extreme Science and Engineering Discovery Environment (XSEDE) program supported by National Science Foundation Grant No. OCI-1053575. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 59 TC 4 Z9 4 U1 9 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 3 PY 2015 VL 115 IS 6 AR 065501 DI 10.1103/PhysRevLett.115.065501 PG 5 WC Physics, Multidisciplinary SC Physics GA CO1TG UT WOS:000358937600007 PM 26296121 ER PT J AU Lemery, F Piot, P AF Lemery, F. Piot, P. TI Tailored electron bunches with smooth current profiles for enhanced transformer ratios in beam-driven acceleration SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID WAKE-FIELD; DIELECTRIC STRUCTURES AB Collinear high-gradient O(GV/m) beam-driven wakefield methods for charged-particle acceleration could be critical to the realization of compact, cost-efficient, accelerators, e.g., in support of TeV-scale lepton colliders or multiple-user free-electron laser facilities. To make these options viable, the high accelerating fields need to be complemented with large transformer ratios >2, a parameter characterizing the efficiency of the energy transfer between a wakefield-exciting "drive" bunch to an accelerated "witness" bunch. While several potential current distributions have been discussed, their practical realization appears challenging due to their often discontinuous nature. In this paper we propose several alternative continuously differentiable (smooth) current profiles which support enhanced transformer ratios. We especially demonstrate that one of the devised shapes can be implemented in a photo-emission electron source by properly shaping the photocathode-laser pulse. We finally discuss a possible superconducting linear-accelerator concept that could produce shaped drive bunches at high-repetition rates to drive a dielectric-wakefield accelerator with accelerating fields on the order of similar to 60 MV/m and a transformer ratio similar to 5 consistent with a recently proposed multiuser free-electron laser facility. C1 [Lemery, F.; Piot, P.] No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. [Lemery, F.; Piot, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Piot, P.] Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, Batavia, IL 60510 USA. RP Lemery, F (reprint author), No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. FU U.S. Department of Energy [DE-SC0011831, DE-AC02-07CH11359]; Defense Threat Reduction Agency, Basic Research Award [HDTRA1-10-1-0051]; Fermi Research Alliance, LLC; dissertation-completion award - Graduate School of Northern Illinois University FX We would like to acknowledge members of the ANL-LANL-NIU working group on DWFA-based short wavelength FEL led by J. G. Power and A. Zholents for useful discussions that motivated the study presented in this paper. P. P. thanks R. Legg (Jefferson Lab) and J. Bisognano (U. Wisconsin) for providing the 200-MHz quarter-wave field map used in Sec. IV. This work was supported by the U.S. Department of Energy Contract No. DE-SC0011831 to Northern Illinois University, and the Defense Threat Reduction Agency, Basic Research Award # HDTRA1-10-1-0051, to Northern Illinois University. P. P. work is also supported by the U.S. Department of Energy under Contract No. DE-AC02-07CH11359 with the Fermi Research Alliance, LLC, and F. L. was partially supported by a dissertation-completion award granted by the Graduate School of Northern Illinois University. NR 42 TC 3 Z9 3 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD AUG 3 PY 2015 VL 18 IS 8 AR 081301 DI 10.1103/PhysRevSTAB.18.081301 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CO1TR UT WOS:000358938700001 ER PT J AU Calta, NP Im, J Rodriguez, AP Fang, L Bugaris, DE Chasapis, TC Freeman, AJ Kanatzidis, MG AF Calta, Nicholas P. Im, Jino Rodriguez, Alexandra P. Fang, Lei Bugaris, Daniel E. Chasapis, Thomas C. Freeman, Arthur J. Kanatzidis, Mercouri G. TI Hybridization Gap and Dresselhaus Spin Splitting in EuIr4In2Ge4 SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE crystal growth; electronic structure; hybridization; intermetallic phases; X-ray diffraction ID HALL COEFFICIENT; INSULATORS; PLANE AB EuIr4In2Ge4 is a new intermetallic semiconductor that adopts a non-centrosymmetric structure in the tetragonal I (4) over bar 2m space group with unit cell parameters a=6.9016(5)angstrom and c=8.7153(9)angstrom. The compound features an indirect optical band gap E-g=0.26(2)eV, and electronic-structure calculations show that the energy gap originates primarily from hybridization of the Ir 5d orbitals, with small contributions from the Ge 4p and In 5p orbitals. The strong spin-orbit coupling arising from the Ir atoms, and the lack of inversion symmetry leads to significant spin splitting, which is described by the Dresselhaus term, at both the conduction- and valence-band edges. The magnetic Eu2+ ions present in the structure, which do not play a role in gap formation, order antiferromagnetically at 2.5K. C1 [Calta, Nicholas P.; Rodriguez, Alexandra P.; Fang, Lei; Chasapis, Thomas C.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Im, Jino; Freeman, Arthur J.] Northwestern Univ, Dept Phys, Evanston, IL 60208 USA. [Fang, Lei; Bugaris, Daniel E.; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu FU Northwestern University's International Institute for Nanotechnology and the State of Illinois Department of Commerce and Economic Opportunity (DCEO) Award [10-203031]; MRSEC program at the Materials Research Center [NSF DMR-1121262]; International Institute for Nanotechnology (IIN); State of Illinois, through the IIN; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering; Undergraduate Research Grant FX We acknowledge the assistance of Prof. Danna Freedman and her research group, as well as support from the Northwestern University's International Institute for Nanotechnology and the State of Illinois Department of Commerce and Economic Opportunity (DCEO) Award (10-203031), which facilitated the magnetic measurements. This work made use of the EPIC facility (NUANCE Center-Northwestern University), which has received support through the MRSEC program (NSF DMR-1121262) at the Materials Research Center, the International Institute for Nanotechnology (IIN), and the State of Illinois, through the IIN. The work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering. A.P.R. acknowledges support through an Undergraduate Research Grant administered by the Northwestern University Office of Undergraduate Research. NR 36 TC 2 Z9 2 U1 3 U2 16 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 3 PY 2015 VL 54 IS 32 BP 9186 EP + DI 10.1002/anie.201504315 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA CN7NO UT WOS:000358621500001 PM 26111038 ER PT J AU Barnhart, EP McClure, MA Johnson, K Cleveland, S Hunt, KA Fields, MW AF Barnhart, Elliott P. McClure, Marcella A. Johnson, Kiki Cleveland, Sean Hunt, Kristopher A. Fields, Matthew W. TI Potential Role of Acetyl-CoA Synthetase (acs) and Malate Dehydrogenase (mae) in the Evolution of the Acetate Switch in Bacteria and Archaea SO SCIENTIFIC REPORTS LA English DT Article ID PROTEIN HOMOLOGY DETECTION; PERMIAN MASS EXTINCTION; ESCHERICHIA-COLI; METHANOSARCINA-THERMOPHILA; COENZYME-A; STRUCTURE PREDICTION; PYROCOCCUS-FURIOSUS; METHANE; SEQUENCE; KINASE AB Although many Archaea have AMP-Acs (acetyl-coenzyme A synthetase) and ADP-Acs, the extant methanogenic genus Methanosarcina is the only identified Archaeal genus that can utilize acetate via acetate kinase (Ack) and phosphotransacetylase (Pta). Despite the importance of ack as the potential urkinase in the ASKHA phosphotransferase superfamily, an origin hypothesis does not exist for the acetate kinase in Bacteria, Archaea, or Eukarya. Here we demonstrate that Archaeal AMP-Acs and ADP-Acs contain paralogous ATPase motifs previously identified in Ack, which demonstrate a novel relation between these proteins in Archaea. The identification of ATPase motif conservation and resulting structural features in AMP- and ADP-acetyl-CoA synthetase proteins in this study expand the ASKHA superfamily to include acetyl-CoA synthetase. Additional phylogenetic analysis showed that Pta and MaeB sequences had a common ancestor, and that the Pta lineage within the halophilc archaea was an ancestral lineage. These results suggested that divergence of a duplicated maeB within an ancient halophilic, archaeal lineage formed a putative pta ancestor. These results provide a potential scenario for the establishment of the Ack/Pta pathway and provide novel insight into the evolution of acetate metabolism for all three domains of life. C1 [Barnhart, Elliott P.; McClure, Marcella A.; Johnson, Kiki; Cleveland, Sean; Fields, Matthew W.] Montana State Univ, Dept Microbiol & Immunol, Bozeman, MT 59717 USA. [Barnhart, Elliott P.; Hunt, Kristopher A.; Fields, Matthew W.] Montana State Univ, Ctr Biofilm Engn, Bozeman, MT 59717 USA. [Barnhart, Elliott P.] US Geol Survey, Helena, MT USA. [Hunt, Kristopher A.] Montana State Univ, Dept Chem & Biol Engn, Bozeman, MT 59717 USA. [Fields, Matthew W.] Montana State Univ, Energy Res Inst, Bozeman, MT 59717 USA. [Fields, Matthew W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, ENIGMA, Berkeley, CA 94720 USA. [Fields, Matthew W.] Natl Ctr Genome Resources, Santa Fe, NM USA. RP Fields, MW (reprint author), Montana State Univ, Dept Microbiol & Immunol, Bozeman, MT 59717 USA. EM matthew.fields@biofilm.montana.edu FU U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231]; U.S. Geological Survey Energy Program; DOE-ZERT Program [DE-FC26-04NT42262] FX This material by ENIGMA- Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research under contract number DE-AC02-05CH11231. We thank many students from Dr. Marcie McClure's Molecular Evolution and Genomic Analysis Lab for their insightful comments and guidance as well as Hannah Schweitzer for helpful discussions. E.P.B. was also supported by the U.S. Geological Survey Energy Program and the DOE-ZERT Program under grant No. DE-FC26-04NT42262. Any use of trade, product, or firm names is for descriptive purposes only and does not imply endorsement by the US Government. NR 62 TC 0 Z9 0 U1 3 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 3 PY 2015 VL 5 AR 12498 DI 10.1038/srep12498 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0PA UT WOS:000358853100001 PM 26235787 ER PT J AU Chen, D Li, YX Liao, SJ Su, D Song, HY Li, YW Yang, LJ Li, C AF Chen, Dan Li, Yuexia Liao, Shijun Su, Dong Song, Huiyu Li, Yingwei Yang, Lijun Li, Can TI Ultra-high-performance core-shell structured Ru@Pt/C catalyst prepared by a facile pulse electrochemical deposition method SO SCIENTIFIC REPORTS LA English DT Article ID OXYGEN REDUCTION REACTION; PLATINUM-MONOLAYER ELECTROCATALYSTS; FUEL-CELLS; O-2 REDUCTION; NANOPARTICLES; STABILITY; ELECTRODE; METAL AB Core-shell structured catalysts, made by placing either a monolayer or a thin layer of a noble metal on relatively cheap core-metal nanoparticles, are fascinating and promising fuel cell catalysts due to their high utilization of noble metals. Here, we report our development of a core-shell structured catalyst, Ru@Pt/C, generated by a novel and facile pulse electrochemical deposition (PED) approach. We demonstrate that compared with a commercial Pt/C catalyst, this novel catalyst achieves over four times higher mass activity towards the anodic oxidation of methanol, and 3.6 times higher mass activity towards the cathodic reduction of oxygen. Importantly, we find that the intrinsic activity of Pt in this Ru@Pt/C catalyst is doubled due to the formation of the core-shell structure. The catalyst also shows superior stability: even after 2000 scans, it still retains up to 90% of the peak current. Our findings demonstrate that this novel PED approach is a promising method for preparing high-performance core-shell catalysts for fuel cell applications. C1 [Chen, Dan; Li, Yuexia; Liao, Shijun; Song, Huiyu; Li, Yingwei; Yang, Lijun] S China Univ Technol, Sch Chem & Chem Engn, Key Lab Fuel Cell Technol Guangdong Prov, Guangzhou 510641, Guangdong, Peoples R China. [Li, Yuexia] Datong Univ, Dept Chem, Datong 037009, Peoples R China. [Su, Dong] Brookhaven Natl Lab, Funct Nanomat Ctr, Upton, NY 11973 USA. [Li, Can] Acad China, Dalian Inst Phys & Chem, Dalian 116023, Peoples R China. RP Liao, SJ (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Key Lab Fuel Cell Technol Guangdong Prov, Guangzhou 510641, Guangdong, Peoples R China. EM chsjliao@scut.edu.cn RI Liao, Shijun/C-1745-2012; Li, Yingwei/M-6479-2014 OI Li, Yingwei/0000-0003-1527-551X FU National Natural Scientific Foundation of China [21276098, 21076089]; Ministry of Science and Technology of China [2012AA053402]; Natural Scientific Foundation of Guangdong Province [S2012020011061] FX We thank Brookhaven National Laboratory for allowing us to use its STEM. This work was supported by the National Natural Scientific Foundation of China (grant numbers 21276098 and 21076089), the Ministry of Science and Technology of China (grant number 2012AA053402), and the Natural Scientific Foundation of Guangdong Province (grant number S2012020011061). NR 20 TC 4 Z9 4 U1 12 U2 102 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 3 PY 2015 VL 5 AR 11604 DI 10.1038/srep11604 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0NT UT WOS:000358849400001 PM 26235385 ER PT J AU Crook, CB Constantin, C Ahmed, T Zhu, JX Balatsky, AV Haraldsen, JT AF Crook, Charles B. Constantin, Costel Ahmed, Towfiq Zhu, Jian-Xin Balatsky, Alexander V. Haraldsen, Jason T. TI Proximity-induced magnetism in transition-metal substituted graphene SO SCIENTIFIC REPORTS LA English DT Article ID SEMICONDUCTOR SPINTRONICS; MOLECULAR SPINTRONICS; DIRAC FERMIONS; FUNDAMENTALS; ATOM AB We investigate the interactions between two identical magnetic impurities substituted into a graphene superlattice. Using a first-principles approach, we calculate the electronic and magnetic properties for transition-metal substituted graphene systems with varying spatial separation. These calculations are compared for three different magnetic impurities, manganese, chromium, and vanadium. We determine the electronic band structure, density of states, and Millikan populations (magnetic moment) for each atom, as well as calculate the exchange parameter between the two magnetic atoms as a function of spatial separation. We find that the presence of magnetic impurities establishes a distinct magnetic moment in the graphene lattice, where the interactions are highly dependent on the spatial and magnetic characteristic between the magnetic and carbon atoms, which leads to either ferromagnetic or antiferromagnetic behavior. Furthermore, through an analysis of the calculated exchange energies and partial density of states, it is determined that interactions between the magnetic atoms can be classified as an RKKY interaction. C1 [Crook, Charles B.; Constantin, Costel; Haraldsen, Jason T.] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22802 USA. [Ahmed, Towfiq; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] NORDITA, S-10691 Stockholm, Sweden. RP Haraldsen, JT (reprint author), James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22802 USA. EM j.t.haraldsen@unf.edu FU Tickle Summer Fellowship Program; U.S. DOE; NNSA [DEAC52-06NA25396]; U.S. DOE Basic Energy Sciences Office; European Research Council (ERC) [DM 321031]; Center for Integrated Nanotechnologies; U.S. DOE Office of Basic Energy Sciences FX C.B.C., C.C. and J.T.H thank the support of the Tickle Summer Fellowship Program. The work at Los Alamos National Laboratory was carried out under the auspice of the U.S. DOE and NNSA under Contract No. DEAC52-06NA25396 and supported by U.S. DOE Basic Energy Sciences Office (T.A. and A.V.B.). Work of A.V.B. was also supported by European Research Council (ERC) DM 321031. This work was also, in part, supported by the Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences user facility (J.-X.Z). NR 50 TC 5 Z9 5 U1 3 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 3 PY 2015 VL 5 AR 12322 DI 10.1038/srep12322 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0NX UT WOS:000358849800001 PM 26235646 ER PT J AU Trahan, TJ Larsen, EW AF Trahan, Travis J. Larsen, Edward W. TI Asymptotic, multigroup flux reconstruction and consistent discontinuity factors SO JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY LA English DT Article; Proceedings Paper CT International Conference on the Physics of Reactors (PHYSOR 2014) CY SEP 28-OCT 03, 2014 CL Kyoto, JAPAN DE flux reconstruction; discontinuity factors; asymptotic analysis; neutron diffusion equation; reactor physics; numerical simulation ID ASSEMBLY HOMOGENIZATION TECHNIQUES AB Recent theoretical work has led to an asymptotically derived expression for reconstructing the neutron flux from lattice functions and multigroup diffusion solutions. The leading-order asymptotic term is the standard expression for flux reconstruction, i.e., it is the product of a shape function, obtained through a lattice calculation, and the multigroup diffusion solution. The first-order asymptotic correction term is significant only where the gradient of the diffusion solution is not small. Inclusion of this first-order correction term can significantly improve the accuracy of the reconstructed flux. One may define discontinuity factors (DFs) to make certain angular moments of the reconstructed flux continuous across interfaces between assemblies in 1-D. Indeed, the standard assembly discontinuity factors make the zeroth moment (scalar flux) of the reconstructed flux continuous. The inclusion of the correction term in the flux reconstruction provides an additional degree of freedom that can be used to make two angular moments of the reconstructed flux continuous across interfaces by using current DFs in addition to flux DFs. Numerical results demonstrate that using flux and current DFs together can be more accurate than using only flux DFs, and that making the second angular moment continuous can be more accurate than making the zeroth moment continuous. C1 [Trahan, Travis J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Larsen, Edward W.] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Trahan, Travis J.] Univ Michigan, Ann Arbor, MI 48109 USA. RP Trahan, TJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM tjtrahan@lanl.gov FU DOE Computational Science Graduate Fellowship [DE-FG02-97ER25308] FX The authors would like to thank Thomas Saller for his extensive assistance in the implementation of the asymptotic diffusion method into the MPACT code. This work was supported by the DOE Computational Science Graduate Fellowship [grant number DE-FG02-97ER25308]. NR 8 TC 1 Z9 1 U1 0 U2 6 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0022-3131 EI 1881-1248 J9 J NUCL SCI TECHNOL JI J. Nucl. Sci. Technol. PD AUG 3 PY 2015 VL 52 IS 7-8 SI SI BP 917 EP 931 DI 10.1080/00223131.2015.1041568 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CL5PN UT WOS:000357012200002 ER PT J AU Sanchez, R Bounds, J Bredeweg, T Goda, J Grove, T Hayes, D Jackman, K Mckenzie, G Myers, W AF Sanchez, Rene Bounds, John Bredeweg, Todd Goda, Joetta Grove, Travis Hayes, David Jackman, Kevin Mckenzie, George Myers, William TI Reaction rate, fission product yield, and Rossi-alpha measurements using a HEU metal, copper reflected critical assembly SO JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY LA English DT Article; Proceedings Paper CT International Conference on the Physics of Reactors (PHYSOR 2014) CY SEP 28-OCT 03, 2014 CL Kyoto, JAPAN DE uranium; critical experiments; spectral indices; Rossi- AB A critical experiment was performed on the Comet assembly to provide nuclear data in a non-thermal neutron spectrum and to re-establish experimental measurement capabilities relevant to the United States Department of Energy's general purpose nuclear criticality experiments capability and to the Technical Nuclear Forensic program. Activation and fission foils were placed at specific locations in the Zeus all-oralloy core, copper reflected critical experiment to infer spectral indices data and obtain reaction rates data. After the irradiation, passive gamma-ray measurements were performed on all the foils and several of them were packaged and shipped to Los Alamos National Laboratory for further radiochemical analysis. The results from the non-destructive and radiochemical analyses are presented in this paper. Finally, Rossi- measurements were performed on a slightly modified configuration from the configuration used for the activation measurements. The Rossi- results are presented and compared to past measurements performed using other critical assemblies. C1 [Sanchez, Rene; Bounds, John; Goda, Joetta; Grove, Travis; Hayes, David; Mckenzie, George; Myers, William] Los Alamos Natl Lab, Adv Nucl Technol NEN 2, Los Alamos, NM 87545 USA. [Bredeweg, Todd; Jackman, Kevin] Los Alamos Natl Lab, C NR Nucl & Radiochem, Los Alamos, NM 87545 USA. RP Sanchez, R (reprint author), Los Alamos Natl Lab, Adv Nucl Technol NEN 2, POB 1663, Los Alamos, NM 87545 USA. EM rsanchez@lanl.gov FU DOE Nuclear Criticality Safety Program - National Nuclear Security Administration for the Department of Energy FX This work was supported by the DOE Nuclear Criticality Safety Program, funded and managed by the National Nuclear Security Administration for the Department of Energy. NR 11 TC 0 Z9 0 U1 2 U2 4 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0022-3131 EI 1881-1248 J9 J NUCL SCI TECHNOL JI J. Nucl. Sci. Technol. PD AUG 3 PY 2015 VL 52 IS 7-8 SI SI BP 1018 EP 1025 DI 10.1080/00223131.2015.1027157 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CL5PN UT WOS:000357012200013 ER PT J AU Stauff, NE Kim, TK Taiwo, TA AF Stauff, Nicolas E. Kim, Taek K. Taiwo, Temitope A. TI Variations in nuclear waste management performance of various fuel-cycle options SO JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY LA English DT Article; Proceedings Paper CT International Conference on the Physics of Reactors (PHYSOR 2014) CY SEP 28-OCT 03, 2014 CL Kyoto, JAPAN DE fuel cycle; radioactive waste management; spent nuclear fuel; high-level waste; activity; toxicity; decay heat; transmutation AB The variations in the nuclear waste management performance have been assessed for 40 fuel-cycle examples with the calculation of the mass, activity, toxicity and decay heat of spent nuclear fuel and high-level waste at 10, 100 and 100,000 years after reactor discharge. The variation in the 10 years activity is primarily due to the variation in the specific activity of the fission products, which is higher for thorium fuel cycles, and is reduced when the fuel residence time is long. The variation in the 100,000 years activity is primarily explained by the quantity of U-233 and Pu-239 sent to nuclear waste, which is linked to the type of fuel and of reprocessing scheme employed. The difference between the inhalation toxicity and the activity is explained by the variations in the effective dose coefficients since heavy actinides such as Pu, Am and Cm have a predominant effect on the inhalation toxicity. Materials for disposal such as fission products and transuranics are responsible for most of the mass, and radiotoxicity of high-level waste, but the reprocessing/separation losses also have a potentially significant impact on the results. C1 [Stauff, Nicolas E.; Kim, Taek K.; Taiwo, Temitope A.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Stauff, NE (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM nstauff@anl.gov FU UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a US Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; US DOE Office of Nuclear Energy FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a US Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The US Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. The direction and support of the US DOE Office of Nuclear Energy is greatly appreciated. NR 4 TC 2 Z9 2 U1 4 U2 29 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0022-3131 EI 1881-1248 J9 J NUCL SCI TECHNOL JI J. Nucl. Sci. Technol. PD AUG 3 PY 2015 VL 52 IS 7-8 SI SI BP 1058 EP 1073 DI 10.1080/00223131.2015.1032380 PG 16 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CL5PN UT WOS:000357012200018 ER PT J AU Sakamoto, M Lapidus, AL Han, J Trong, S Haynes, M Reddy, TBK Mikhailova, N Huntemann, M Pati, A Ivanova, NN Pukall, R Markowitz, VM Woyke, T Klenk, HP Kyrpides, NC Ohkuma, M AF Sakamoto, Mitsuo Lapidus, Alla L. Han, James Trong, Stephan Haynes, Matthew Reddy, T. B. K. Mikhailova, Natalia Huntemann, Marcel Pati, Amrita Ivanova, Natalia N. Pukall, Rudiger Markowitz, Victor M. Woyke, Tanja Klenk, Hans-Peter Kyrpides, Nikos C. Ohkuma, Moriya TI High quality draft genome sequence of Bacteroides barnesiae type strain BL2(T) (DSM 18169(T)) from chicken caecum SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Strictly anaerobic; Non-motile; Rod-shaped; Gram-negative; Cecum; Poultry; Bacteroidaceae ID MICROBIAL GENOMES; BACTERIA; IDENTIFICATION; ARCHAEA; ENCYCLOPEDIA; ANNOTATION; PROJECTS; DATABASE; SYSTEM; STARCH AB Bacteroides barnesiae Lan et al. 2006 is a species of the genus Bacteroides, which belongs to the family Bacteroidaceae. Strain BL2(T) is of interest because it was isolated from the gut of a chicken and the growing awareness that the anaerobic microbiota of the caecum is of benefit for the host and may impact poultry farming. The 3,621,509 bp long genome with its 3,059 protein-coding and 97 RNA genes is a part of the Genomic Encyclopedia of Type Strains, Phase I: the one thousand microbial genomes (KMG) project. C1 [Sakamoto, Mitsuo; Ohkuma, Moriya] RIKEN BioResource Ctr, Microbe Div Japan Collect Microorganisms, Tsukuba, Ibaraki, Japan. [Lapidus, Alla L.] St Petersburg State Univ, Theodosius Dobzhansky Ctr Genome Bionformat, St Petersburg 199034, Russia. [Lapidus, Alla L.] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg, Russia. [Han, James; Trong, Stephan; Haynes, Matthew; Reddy, T. B. K.; Mikhailova, Natalia; Huntemann, Marcel; Pati, Amrita; Ivanova, Natalia N.; Woyke, Tanja; Kyrpides, Nikos C.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Pukall, Rudiger; Klenk, Hans-Peter] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Markowitz, Victor M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah, Saudi Arabia. RP Sakamoto, M (reprint author), RIKEN BioResource Ctr, Microbe Div Japan Collect Microorganisms, Tsukuba, Ibaraki, Japan. EM sakamoto@jcm.riken.jp RI Ohkuma, Moriya/A-8100-2011; Sakamoto, Mitsuo/C-3612-2017; Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017; Lapidus, Alla/I-4348-2013; OI Sakamoto, Mitsuo/0000-0002-3622-4642; Kyrpides, Nikos/0000-0002-6131-0462; Lapidus, Alla/0000-0003-0427-8731; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Russian Ministry of Science Mega-grant [11.G34.31.0068] FX We would like to gratefully acknowledge the help of Iljana Schroder for growing B. barnesiae cultures, and Evelyne-Marie Brambilla for DNA extraction and quality control (both at DSMZ). This work was performed under the auspices of the US Department of Energy Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under contract No. DE-AC52-07NA27344. A.L. was supported in part by Russian Ministry of Science Mega-grant no. 11.G34.31.0068 (PI. Dr Stephen J O'Brien). NR 39 TC 1 Z9 1 U1 0 U2 6 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 2 PY 2015 VL 10 AR 48 DI 10.1186/s40793-015-0045-6 PG 6 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NR UT WOS:000367991500001 PM 26380636 ER PT J AU Balhorn, MC Hok, S Balhorn, R AF Balhorn, Monique Cosman Hok, Saphon Balhorn, Rod TI Multiple mechanisms of action may contribute to the lymphoma cell-killing activity of SH7139 SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Balhorn, Monique Cosman; Balhorn, Rod] SHAL Technol Inc, Livermore, CA USA. [Hok, Saphon] Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA 5498 DI 10.1158/1538-7445.AM2015-5498 PG 1 WC Oncology SC Oncology GA DF8HA UT WOS:000371597106156 ER PT J AU Balhorn, R Hok, S Balhorn, MC AF Balhorn, Rod Hok, Saphon Balhorn, Monique Cosman TI Physical and metabolic stability of SH7139, a new drug candidate for non-Hodgkin's lymphoma targeting HLA-DR10 SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Balhorn, Rod; Balhorn, Monique Cosman] SHAL Technol Inc, Livermore, CA USA. [Hok, Saphon] Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA 4494 DI 10.1158/1538-7445.AM2015-4494 PG 1 WC Oncology SC Oncology GA DF8HA UT WOS:000371597104122 ER PT J AU Lambert, MW Sridharan, D Zhang, P AF Lambert, Muriel W. Sridharan, Deepa Zhang, Pan TI FANCF, a Fanconi anemia core protein, functions outside of monoubiquitinating FANCD2 in DNA interstrand crosslink repair SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Lambert, Muriel W.] Rutgers New Jersey Med Sch, Newark, NJ USA. [Sridharan, Deepa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zhang, Pan] Cornell Univ, Weill Cornell Med Coll, New York, NY 10021 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA 3018 DI 10.1158/1538-7445.AM2015-3018 PG 1 WC Oncology SC Oncology GA DF8HA UT WOS:000371597101068 ER PT J AU Rodland, KD AF Rodland, Karin D. TI Proteogenomic and phosphoproteomic analysis of ovarian cancer SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Rodland, Karin D.] Pacific NW Natl Lab, Richland, WA 99352 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA SY44-03 DI 10.1158/1538-7445.AM2015-SY44-03 PG 1 WC Oncology SC Oncology GA DF8HA UT WOS:000371597101037 ER PT J AU Staquicini, F Dobroff, A Ferrara, F D'Angelo, S Bradbury, ARM Arap, W Pasqualini, R AF Staquicini, Fernanda Dobroff, Andrey Ferrara, Fortunato D'Angelo, Sara Bradbury, Andrew R. M. Arap, Wadih Pasqualini, Renata TI Receptor tyrosine kinase EphA5 is a functional molecular target in human lung cancer SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Staquicini, Fernanda; Dobroff, Andrey; Ferrara, Fortunato; D'Angelo, Sara; Arap, Wadih; Pasqualini, Renata] Univ New Mexico, Ctr Canc, Albuquerque, NM 87131 USA. [Bradbury, Andrew R. M.] Los Alamos Natl Lab, Los Alamos, NM USA. OI Bradbury, Andrew/0000-0002-5567-8172 NR 0 TC 0 Z9 0 U1 1 U2 2 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA LB-006 DI 10.1158/1538-7445.AM2015-LB-006 PG 3 WC Oncology SC Oncology GA DF8HA UT WOS:000371597100114 ER PT J AU He, JT Schepmoes, A Rastogi, A Tan, SH Yan, WS Huang, W Banerjee, S Shi, TJ Wu, CC Fillmore, T Gao, YQ Kagan, J Srivastava, S Smith, R Qian, WJ McLeod, D Petrovics, G Dobi, A Srinivasan, A Srivastava, S Rodland, K Liu, T Camp, D AF He, Jintang Schepmoes, Athena Rastogi, Anshu Tan, Shyh-Han Yan, Wusheng Huang, Wei Banerjee, Sreedatta Shi, Tujin Wu, Chaochao Fillmore, Thomas Gao, Yuqian Kagan, Jacob Srivastava, Sudhir Smith, Richard Qian, Wei-Jun McLeod, David Petrovics, Gyorgy Dobi, Albert Srinivasan, Alagarsamy Srivastava, Shiv Rodland, Karin Liu, Tao Camp, David TI Analytical platform evaluation for quantification of ERG oncoprotein in prostate cancer using protein and mRNA detection methods SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [He, Jintang; Schepmoes, Athena; Shi, Tujin; Wu, Chaochao; Fillmore, Thomas; Gao, Yuqian; Smith, Richard; Qian, Wei-Jun; Rodland, Karin; Liu, Tao; Camp, David] Pacific NW Natl Lab, Richland, WA 99352 USA. [Rastogi, Anshu; Tan, Shyh-Han; Yan, Wusheng; Huang, Wei; Banerjee, Sreedatta; Petrovics, Gyorgy; Dobi, Albert; Srinivasan, Alagarsamy; Srivastava, Shiv] Ctr Prostate Dis Res, Bethesda, MD USA. [Kagan, Jacob; Srivastava, Sudhir] NCI, Bethesda, MD 20892 USA. [McLeod, David] Walter Reed Natl Mil Med Ctr, Ctr Prostate Dis Res, Bethesda, MD USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA 1818 DI 10.1158/1538-7445.AM2015-1818 PG 2 WC Oncology SC Oncology GA DF8AH UT WOS:000371578503303 ER PT J AU Skates, SJ Anderson, KS Liu, T Kulasingam, V Rabideau, D Wu, CC Gillette, M Godwin, AK Urban, N Lokshin, A Marks, J Diamandis, E Zhang, Z Srivastava, S Kagan, J Patriotis, C Rodland, K AF Skates, Steven J. Anderson, Karen S. Liu, Tao Kulasingam, Vathany Rabideau, Dustin Wu, Chaochao Gillette, Michael Godwin, Andrew K. Urban, Nicole Lokshin, Anna Marks, Jeffrey Diamandis, Eleftherios Zhang, Zhen Srivastava, Sudhir Kagan, Jacob Patriotis, Christos Rodland, Karin TI Early Detection Research Network (EDRN) validation of circulating ovarian cancer biomarkers SO CANCER RESEARCH LA English DT Meeting Abstract CT 106th Annual Meeting of the American-Association-for-Cancer-Research (AACR) CY APR 18-22, 2015 CL Philadelphia, PA SP Amer Assoc Canc Res C1 [Skates, Steven J.; Rabideau, Dustin; Gillette, Michael] Massachusetts Gen Hosp, Boston, MA 02114 USA. [Anderson, Karen S.] Arizona State Univ, Phoenix, AZ USA. [Liu, Tao; Wu, Chaochao; Rodland, Karin] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kulasingam, Vathany; Diamandis, Eleftherios] Univ Toronto, Toronto, ON, Canada. [Gillette, Michael] Broad Inst, Cambridge, MA USA. [Godwin, Andrew K.] Univ Kansas, Med Ctr, Kansas City, KS 66103 USA. [Urban, Nicole] Fred Hutchinson Canc Res Ctr, Seattle, WA 98104 USA. [Lokshin, Anna] Univ Pittsburgh, Pittsburgh, PA USA. [Marks, Jeffrey] Duke Univ, Durham, NC USA. [Zhang, Zhen] Johns Hopkins Univ, Baltimore, MD USA. [Srivastava, Sudhir; Kagan, Jacob; Patriotis, Christos] NCI, Rockville, MD USA. NR 0 TC 0 Z9 0 U1 1 U2 4 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD AUG 1 PY 2015 VL 75 SU 15 MA 1570 DI 10.1158/1538-7445.AM2015-1570 PG 2 WC Oncology SC Oncology GA DF8AH UT WOS:000371578503064 ER PT J AU Archambault, S Archer, A Beilicke, M Benbow, W Bird, R Biteau, J Bouvier, A Bugaev, V Cardenzana, JV Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dickinson, HJ Dumm, J Eisch, JD Errando, M Falcone, A Feng, Q Finley, JP Fleischhack, H Fortin, P Fortson, L Furniss, A Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hakansson, N Hanna, D Holder, J Humensky, TB Johnson, CA Kaaret, P Kar, P Kertzman, M Khassen, Y Kieda, D Krause, M Krennrich, F Kumar, S Lang, MJ Maier, G McArthur, S McCann, A Meagher, K Millis, J Moriarty, P Mukherjee, R Nieto, D de Bhroithe, AO Ong, RA Otte, AN Park, N Pohl, M Popkow, A Prokoph, H Pueschel, E Quinn, J Ragan, K Reyes, LC Reynolds, PT Richards, GT Roache, E Santander, M Sembroski, GH Shahinyan, K Smith, AW Staszak, D Telezhinsky, I Tucci, JV Tyler, J Varlotta, A Vincent, S Wakely, SP Weinstein, A Welsing, R Wilhelm, A Williams, DA Zitzer, B Hughes, ZD AF Archambault, S. Archer, A. Beilicke, M. Benbow, W. Bird, R. Biteau, J. Bouvier, A. Bugaev, V. Cardenzana, J. V. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dickinson, H. J. Dumm, J. Eisch, J. D. Errando, M. Falcone, A. Feng, Q. Finley, J. P. Fleischhack, H. Fortin, P. Fortson, L. Furniss, A. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hakansson, N. Hanna, D. Holder, J. Humensky, T. B. Johnson, C. A. Kaaret, P. Kar, P. Kertzman, M. Khassen, Y. Kieda, D. Krause, M. Krennrich, F. Kumar, S. Lang, M. J. Maier, G. McArthur, S. McCann, A. Meagher, K. Millis, J. Moriarty, P. Mukherjee, R. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Park, N. Pohl, M. Popkow, A. Prokoph, H. Pueschel, E. Quinn, J. Ragan, K. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Santander, M. Sembroski, G. H. Shahinyan, K. Smith, A. W. Staszak, D. Telezhinsky, I. Tucci, J. V. Tyler, J. Varlotta, A. Vincent, S. Wakely, S. P. Weinstein, A. Welsing, R. Wilhelm, A. Williams, D. A. Zitzer, B. Hughes, Z. D. CA Veritas Collaboration TI VERITAS DETECTION OF gamma-RAY FLARING ACTIVITY FROM THE BL LAC OBJECT 1ES 1727+502 DURING BRIGHT MOONLIGHT OBSERVATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: individual (1ES 1727+502); galaxies: active; gamma rays: galaxies; radiation mechanisms: non-thermal ID LARGE-AREA TELESCOPE; SELF-COMPTON MODEL; SPECTRAL ENERGY-DISTRIBUTION; LACERTAE OBJECTS; GALACTIC NUCLEI; HOST GALAXIES; SOURCE CATALOG; CRAB-NEBULA; TEV BLAZARS; FERMI ERA AB During moonlit nights, observations with ground-based Cherenkov telescopes at very high energies (VHEs, E > 100 GeV) are constrained since the photomultiplier tubes (PMTs) in the telescope camera are extremely sensitive to the background moonlight. Observations with the VERITAS telescopes in the standard configuration are performed only with a moon illumination less than 35% of full moon. Since 2012, the VERITAS collaboration has implemented a new observing mode under bright moonlight, by either reducing the voltage applied to the PMTs (reduced-high-voltage; RHV configuration), or by utilizing UV-transparent filters. While these operating modes result in lower sensitivity and increased energy thresholds, the extension of the available observing time is useful for monitoring variable sources such as blazars and sources requiring spectral measurements at the highest energies. In this paper we report the detection of gamma-ray flaring activity from the BL Lac object 1ES 1727+502 during RHV observations. This detection represents the first evidence of VHE variability from this blazar. The integral flux is (1.1 +/- 0.2) x 10(-11) cm(-2) s(-1) above 250 GeV, which is about five times higher than the low-flux state. The detection triggered additional VERITAS observations during standard dark-time. Multiwavelength observations with the FLWO 48 '' telescope, and the Swift and Fermi satellites are presented and used to produce the first spectral energy distribution (SED) of this object during gamma-ray flaring activity. The SED is then fitted with a standard synchrotron-self-Compton model, placing constraints on the properties of the emitting region and of the acceleration mechanism at the origin of the relativistic particle population in the jet. C1 [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. [Archer, A.; Beilicke, M.; Bugaev, V.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Fortin, P.; Roache, E.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Khassen, Y.; Pueschel, E.; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Biteau, J.; Bouvier, A.; Furniss, A.; Johnson, C. A.; Williams, D. A.; Hughes, Z. D.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Biteau, J.; Bouvier, A.; Furniss, A.; Johnson, C. A.; Williams, D. A.; Hughes, Z. D.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Cardenzana, J. V.; Dickinson, H. J.; Eisch, J. D.; Krennrich, F.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chen, X.; Hakansson, N.; Pohl, M.; Telezhinsky, I.; Wilhelm, A.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, X.; Fleischhack, H.; Krause, M.; Maier, G.; de Bhroithe, A. O'Faolain; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Vincent, S.; Welsing, R.; Wilhelm, A.] DESY, D-15738 Zeuthen, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.; Moriarty, P.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Tucci, J. V.; Varlotta, A.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.; Shahinyan, K.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Errando, M.; Mukherjee, R.; Santander, M.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Holder, J.; Kumar, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Holder, J.; Kumar, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kar, P.; Kieda, D.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Millis, J.] Anderson Univ, Dept Phys Sci & Engn, Anderson, IN 46012 USA. [Ong, R. A.; Popkow, A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Sci, Cork, Ireland. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Archambault, S (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. EM matteo.cerruti@cfa.harvard.edu; griffins@physics.mcgill.ca RI Nieto, Daniel/J-7250-2015; OI Nieto, Daniel/0000-0003-3343-0755; Pueschel, Elisa/0000-0002-0529-1973 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland (SFI) [10/RFP/AST2748]; STFC in the U.K. FX The authors wish to thank Kari Nilsson for useful discussions about the host-galaxy contribution, as well as the anonymous referee for his/her comments which improved the present work. This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. The VERITAS Collaboration is grateful to Trevor Weekes for his seminal contributions and leadership in the field of VHE gamma-ray astrophysics, which made this study possible. NR 88 TC 6 Z9 6 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 1 PY 2015 VL 808 IS 2 AR 110 DI 10.1088/0004-637X/808/2/110 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF0BA UT WOS:000371002400005 ER PT J AU Civano, F Hickox, RC Puccetti, S Comastri, A Mullaney, JR Zappacosta, L LaMassa, SM Aird, J Alexander, DM Ballantyne, DR Bauer, FE Brandt, WN Boggs, SE Christensen, FE Craig, WW Del-Moro, A Elvis, M Forster, K Gandhi, P Grefenstette, BW Hailey, CJ Harrison, FA Lansbury, GB Luo, B Madsen, K Saez, C Stern, D Treister, E Urry, MC Wik, DR Zhang, W AF Civano, F. Hickox, R. C. Puccetti, S. Comastri, A. Mullaney, J. R. Zappacosta, L. LaMassa, S. M. Aird, J. Alexander, D. M. Ballantyne, D. R. Bauer, F. E. Brandt, W. N. Boggs, S. E. Christensen, F. E. Craig, W. W. Del-Moro, A. Elvis, M. Forster, K. Gandhi, P. Grefenstette, B. W. Hailey, C. J. Harrison, F. A. Lansbury, G. B. Luo, B. Madsen, K. Saez, C. Stern, D. Treister, E. Urry, M. C. Wik, D. R. Zhang, W. TI THE NuSTAR EXTRAGALACTIC SURVEYS: OVERVIEW AND CATALOG FROM THE COSMOS FIELD SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: nuclei; X-rays: general ID ACTIVE GALACTIC NUCLEI; X-RAY LUMINOSITY; MEDIUM-SENSITIVITY SURVEY; POINT-SOURCE CATALOG; CHANDRA DEEP SURVEY; COMPTON-THICK AGN; SWIFT-BAT SURVEY; ALL-SKY SURVEY; XMM-NEWTON; HELLAS2XMM SURVEY AB To provide the census of the sources contributing to the X-ray background peak above 10 keV, Nuclear Spectroscopic Telescope Array (NuSTAR) is performing extragalactic surveys using a three-tier "wedding cake" approach. We present the NuSTAR survey of the COSMOS field, the medium sensitivity, and medium area tier, covering 1.7 deg(2) and overlapping with both Chandra and XMM-Newton data. This survey consists of 121 observations for a total exposure of similar to 3 Ms. To fully exploit these data, we developed a new detection strategy, carefully tested through extensive simulations. The survey sensitivity at 20% completeness is 5.9, 2.9, and 6.4 x 10(-14) erg cm(-2) s(-1) in the 3-24, 3-8, and 8-24 keV bands, respectively. By combining detections in 3 bands, we have a sample of 91 NuSTAR sources with 10(42)-10(45.5) erg s(-1) luminosities and redshift z = 0.04-2.5. Thirty-two sources are detected in the 8-24 keV band with fluxes similar to 100 times fainter than sources detected by Swift-BAT. Of the 91 detections, all but 4 are associated with a Chandra and/or XMM-Newton point-like counterpart. One source is associated with an extended lower energy X-ray source. We present the X-ray (hardness ratio and luminosity) and optical-to-X-ray properties. The observed fraction of candidate Compton-thick active galactic nuclei measured from the hardness ratio is between 13%-20%. We discuss the spectral properties of NuSTAR J100259+0220.6 (ID 330) at z = 0.044, with the highest hardness ratio in the entire sample. The measured column density exceeds 10(24) cm(-2), implying the source is Compton-thick. This source was not previously recognized as such without the >10 keV data. C1 [Civano, F.; LaMassa, S. M.; Urry, M. C.] Yale Ctr Astron & Astrophys, 260 Whitney Ave, New Haven, CT 06520 USA. [Civano, F.; Hickox, R. C.] Dartmouth Coll, Dept Phys & Astron, Wilder Lab 6127, Hanover, NH 03755 USA. [Civano, F.; Elvis, M.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Puccetti, S.] ASDC ASI, I-00133 Rome, Italy. [Comastri, A.] INAF Osservatorio Astron Bologna, I-40127 Bologna, Italy. [Mullaney, J. R.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England. [Zappacosta, L.] INAF Osservatorio Astron Roma, I-00040 Monte Porzio Catone, RM, Italy. [Aird, J.; Alexander, D. M.; Del-Moro, A.; Gandhi, P.; Lansbury, G. B.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Aird, J.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Ballantyne, D. R.] Georgia Inst Technol, Sch Phys, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Bauer, F. E.; Luo, B.; Saez, C.] Pontificia Univ Catolica Chile, Inst Astrofis, Fac Fis, Santiago 22, Chile. [Bauer, F. E.; Luo, B.] Millennium Inst Astrophys, Santiago, Chile. [Bauer, F. E.] Space Sci Inst, Boulder, CO 80301 USA. [Brandt, W. N.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Brandt, W. N.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Brandt, W. N.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Forster, K.; Grefenstette, B. W.; Harrison, F. A.; Madsen, K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Gandhi, P.] Univ Southampton, Sch Phys Astron, Southampton SO17 1BJ, Hants, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Treister, E.] Univ Concepcion, Dept Astron, Concepcion, Chile. [Wik, D. R.; Zhang, W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Civano, F (reprint author), Yale Ctr Astron & Astrophys, 260 Whitney Ave, New Haven, CT 06520 USA. RI Boggs, Steven/E-4170-2015; OI Puccetti, Simonetta/0000-0002-2734-7835; Boggs, Steven/0000-0001-9567-4224; Comastri, Andrea/0000-0003-3451-9970; Ballantyne, David/0000-0001-8128-6976; Urry, Meg/0000-0002-0745-9792 FU National Aeronautics and Space Administration; NASA [11-ADAP110218, GO3-14150C]; Science and Technology Facilities Council [ST/I001573/1]; NSF [AST 1008067]; NuSTAR grant [44A-1092750]; NASA ADP grant [NNX10AC99G]; V. M. Willaman Endowment; CONICYT-Chile [Basal-CATA PFB-06/2007]; FONDECYT [1141218, 1120061]; "EMBIGGEN" Anillo [ACT1101]; Ministry of Economy, Development, and Tourism's Millennium Science Initiative [IC120009]; Center of Excellence in Astrophysics and Associated Technologies; ASI/INAF [I/037/12/0] FX We thank the anonymous referee for interesting comments and A. Goulding and M. Rose for useful discussions. This work made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NUSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). We acknowledge support from the NASA grants 11-ADAP110218 and GO3-14150C (FC); from the Science and Technology Facilities Council ST/I001573/1 (ADM, DMA); NSF award AST 1008067 (DRB); NuSTAR grant 44A-1092750, NASA ADP grant NNX10AC99G, and the V. M. Willaman Endowment (WNB, BL); CONICYT-Chile grants Basal-CATA PFB-06/2007 (FEB), FONDECYT 1141218 (FEB), and "EMBIGGEN" Anillo ACT1101 (FEB, ET); the Ministry of Economy, Development, and Tourism's Millennium Science Initiative through grant IC120009, awarded to The Millennium Institute of Astrophysics, MAS (FEB); the Center of Excellence in Astrophysics and Associated Technologies (PFB 06) and by the FONDECYT regular grant 1120061 (ET); financial support under ASI/INAF contract I/037/12/0 (LZ). NR 96 TC 10 Z9 10 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 1 PY 2015 VL 808 IS 2 AR 185 DI 10.1088/0004-637X/808/2/185 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF0BA UT WOS:000371002400081 ER PT J AU Furst, F Nowak, MA Tomsick, JA Miller, JM Corbel, S Bachetti, M Boggs, SE Christensen, FE Craig, WW Fabian, AC Gandhi, P Grinberg, V Hailey, CJ Harrison, FA Kara, E Kennea, JA Madsen, KK Pottschmidt, K Stern, D Walton, DJ Wilms, J Zhang, WW AF Fuerst, F. Nowak, M. A. Tomsick, J. A. Miller, J. M. Corbel, S. Bachetti, M. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Gandhi, P. Grinberg, V. Hailey, C. J. Harrison, F. A. Kara, E. Kennea, J. A. Madsen, K. K. Pottschmidt, K. Stern, D. Walton, D. J. Wilms, J. Zhang, W. W. TI THE COMPLEX ACCRETION GEOMETRY OF GX 339-4 AS SEEN BY NuSTAR AND SWIFT SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; stars: black holes; X-rays: binaries; X-rays: individual (GX 339-4) ID BLACK-HOLE SPIN; X-RAY REFLECTION; ADVECTION-DOMINATED ACCRETION; HARD STATE; LOW/HARD STATE; CANDIDATE GX-339-4; EMISSION; BINARIES; SPECTROSCOPY; DISC AB We present spectral analyses of five Nuclear Spectroscopic Telescope Array and Swift observations of GX 339-4 taken during a failed outburst during the summer of 2013. These observations cover Eddington luminosity fractions in the range approximate to 0.9%-6%. Throughout this outburst GX 339-4 stayed in the hard state and all five observations show similar X-ray spectra, with a hard power law with a photon index near 1.6, and significant contribution from reflection. Using simple reflection models we find unrealistically high iron abundances. Allowing for different photon indices for the continuum incident on the reflector relative to the underlying observed continuum results in a statistically better fit and reduced iron abundances. With a photon index around 1.3, the input power law on the reflector is significantly harder than that which is directly observed. We study the influence of different emissivity profiles and geometries and consistently find an improvement when using separate photon indices. The inferred inner accretion disk radius is strongly model dependent, but we do not find evidence for a truncation radius larger than 100 r(g) in any model. The data do not allow independent spin constraints, but the results are consistent with the literature (i.e., a > 0). Our best-fit models indicate an inclination angle in the range 40 degrees-60 degrees, consistent with limits on the orbital inclination but higher than reported in the literature using standard reflection models. The iron line around 6.4 keV is clearly broadened, and we detect a superimposed narrow core as well. This core originates from a fluorescent region outside the influence of the strong gravity of the black hole. Additionally, we discuss possible geometries. C1 [Fuerst, F.; Harrison, F. A.; Madsen, K. K.; Walton, D. J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Nowak, M. A.; Grinberg, V.] MIT, Kavli Inst Astrophys, Cambridge, MA 02139 USA. [Tomsick, J. A.; Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Miller, J. M.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Corbel, S.] Univ Paris Diderot, Lab AIM, CEA IRFU CNRS INSU, CEA DSM IRFU SAp, F-91191 Gif Sur Yvette, France. [Corbel, S.] Univ Orleans, OSUC, Stn Radioastron Nancay, Observ Paris,CNRS INSU,USR 704, F-18330 Nancay, France. [Bachetti, M.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Bachetti, M.] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Bachetti, M.] Osservatorio Astron Cagliari, INAF, I-09047 Selargius, CA, Italy. [Christensen, F. E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fabian, A. C.; Kara, E.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Gandhi, P.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Gandhi, P.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Kennea, J. A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Pottschmidt, K.; Zhang, W. W.] UMBC, CRESST, Greenbelt, MD 20771 USA. [Pottschmidt, K.; Zhang, W. W.] NASA GSFC, Greenbelt, MD 20771 USA. [Pottschmidt, K.] NASA Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wilms, J.] Univ Erlangen Nurnberg, Dr Karl Remeis Sternwarte, D-96049 Bamberg, Germany. [Wilms, J.] Univ Erlangen Nurnberg, ECAP, D-96049 Bamberg, Germany. RP Furst, F (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. RI Wilms, Joern/C-8116-2013; Boggs, Steven/E-4170-2015; OI Wilms, Joern/0000-0003-2065-5410; Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337 FU NASA [NNG08FD60C, NNX13AJ81G, NNX14AC56G]; National Aeronautics and Space Administration; ANR "CHAOS" [ANR-12-BS05-0009] FX We thank the anonymous referee for very constructive and helpful comments. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS), jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). J.A.T. acknowledges partial support from NASA Swift Guest Investigator grants NNX13AJ81G and NNX14AC56G. S.C. acknowledges funding support from the ANR "CHAOS" (ANR-12-BS05-0009). We would like to thank John E. Davis for the slxfig module, which was used to produce all figures in this work. NR 66 TC 12 Z9 12 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 1 PY 2015 VL 808 IS 2 AR 122 DI 10.1088/0004-637X/808/2/122 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF0BA UT WOS:000371002400017 ER PT J AU Ochsendorf, BB Brown, AGA Bally, J Tielens, AGGM AF Ochsendorf, Bram B. Brown, Anthony G. A. Bally, John Tielens, Alexander G. G. M. TI NESTED SHELLS REVEAL THE REJUVENATION OF THE ORION-ERIDANUS SUPERBUBBLE SO ASTROPHYSICAL JOURNAL LA English DT Article DE H II regions; ISM: bubbles; ISM: clouds; ISM: kinematics and dynamics; stars: formation ID H-II REGIONS; X-RAY ENHANCEMENT; INTERSTELLAR-MEDIUM; MOLECULAR CLOUDS; LAMBDA-ORIONIS; STAR-FORMATION; OB ASSOCIATIONS; NEBULA CLUSTER; BARNARDS LOOP; YOUNG STARS AB The Orion-Eridanus superbubble is the prototypical superbubble owing to its proximity and evolutionary state. Here. we provide a synthesis of recent observational data from WISE and Planck with archival data, allowing us to draw a new and more complete picture on the history and evolution of the Orion-Eridanus region. We discuss the general morphological structures and observational characteristics of the superbubble. and derive quantitative properties of the gas. and dust inside Barnard's Loop. We reveal that Barnard's Loop is a complete bubble structure that, together with the lambda Ori region and other smaller-scale bubbles, expands within the Orion-Eridanus superbubble. We argue that the Orion-Eridanus superbubble is larger and more complex than previously thought, and that it can be viewed as a series of nested shells, superimposed along the line of sight. During the lifetime of the superbubble, H II region champagne flows and thermal evaporation of embedded clouds continuously mass-load the superbubble interior, while winds or supernovae from the Orion OB association rejuvenate the superbubble by sweeping up the material from the interior cavities in an episodic fashion, possibly triggering the formation of new stars that form shells of their own. The steady supply of material into the superbubble cavity implies that dust processing from interior supernova remnants is more efficient than previously thought. The cycle of mass. loading, interior cleansing, and star formation repeats until the molecular reservoir is depleted or the clouds have been disrupted. While the nested shells come and go, the superbubble remains for tens of millions of years. C1 [Ochsendorf, Bram B.; Brown, Anthony G. A.; Tielens, Alexander G. G. M.] Leiden Univ, Leiden Observ, POB 9513, NL-2300 RA Leiden, Netherlands. [Bally, John] Univ Colorado, CASA, APS, Boulder, CO 80389 USA. RP Ochsendorf, BB (reprint author), Leiden Univ, Leiden Observ, POB 9513, NL-2300 RA Leiden, Netherlands. EM ochsendorf@strw.leidenuniv.nl FU ERC from European Research Council [246976]; Dutch Science Agency, NWO as part of the Dutch Astrochemistry Network; Spinoza premie from the Dutch Science Agency, NWO; National Science Foundatoin (NSF) [AST-1009847] FX The authors thank the anonymous referee for detailed comments that significantly increased the quality of this paper. Studies of interstellar dust and chemistry at Leiden Observatory are supported through advanced ERC grant 246976 from the European Research Council; through a grant by the Dutch Science Agency, NWO, as part of the Dutch Astrochemistry Network; and through the Spinoza premie from the Dutch Science Agency, NWO. J.B. was supported in part by National Science Foundatoin (NSF) grant AST-1009847. NR 117 TC 7 Z9 7 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 1 PY 2015 VL 808 IS 2 AR 111 DI 10.1088/0004-637X/808/2/111 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF0BA UT WOS:000371002400006 ER PT J AU Reynolds, CS Lohfink, AM Ogle, PM Harrison, FA Madsen, KK Fabian, AC Wik, DR Madejski, G Ballantyne, DR Boggs, SE Christensen, FE Craig, WW Fuerst, F Hailey, CJ Lanz, L Miller, JM Saez, C Stern, D Walton, DJ Zhang, W AF Reynolds, Christopher S. Lohfink, Anne M. Ogle, Patrick M. Harrison, Fiona A. Madsen, Kristin K. Fabian, Andrew C. Wik, Daniel R. Madejski, Grzegorz Ballantyne, David R. Boggs, Steven E. Christensen, Finn E. Craig, William W. Fuerst, Felix Hailey, Charles J. Lanz, Lauranne Miller, Jon M. Saez, Cristian Stern, Daniel Walton, Dominic J. Zhang, William TI NuSTAR OBSERVATIONS OF THE POWERFUL RADIO-GALAXY CYGNUS A SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; galaxies: clusters: intracluster medium; galaxies: jets; X-rays: individual (Cygnus A) ID ACTIVE GALACTIC NUCLEI; HOLE ACCRETION DISKS; X-RAY OBSERVATIONS; BLACK-HOLE; WINDS; REFLECTION; EMISSION; FEEDBACK; SPECTRA; ENERGY AB We present NuSTAR observations of the powerful radio galaxy Cygnus A, focusing on the central absorbed active galactic nucleus (AGN). Cygnus A is embedded in a cool-core galaxy cluster, and hence we also examine archival XMM-Newton data to facilitate the decomposition of the spectrum into the AGN and intracluster medium components. NuSTAR gives a source-dominated spectrum of the AGN out to >70 keV. In gross terms, the NuSTAR spectrum of the AGN has the form of a power law (Gamma similar to 1.6-1.7) absorbed by a neutral column density of N-H similar to 1.6 10(23) cm(-2). However, we also detect curvature in the hard (>10 keV) spectrum resulting from reflection by Compton-thick matter out of our line of sight to the X-ray source. Compton reflection, possibly from the outer accretion disk or obscuring torus, is required even permitting a high-energy cut off in the continuum source; the limit on the cut-off energy is E-cut > 111 keV(90% confidence). Interestingly, the absorbed power law plus reflection model leaves residuals suggesting the absorption/emission from a fast (15,000-26,000 km s(-1)), high column-density (N-W > 3 x 10(23) cm(-2)), highly ionized (xi similar to 2500 erg cm s(-1)) wind. A second, even faster ionized wind component is also suggested by these data. We show that the ionized wind likely carries a significant mass and momentum flux, and may carry sufficient kinetic energy to exercise feedback on the host galaxy. If confirmed, the simultaneous presence of a strong wind and powerful jets in Cygnus A demonstrates that feedback from radio-jets and sub-relativistic winds are not mutually exclusive phases of AGN activity but can occur simultaneously. C1 [Reynolds, Christopher S.; Saez, Cristian] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Reynolds, Christopher S.] Joint Space Sci Inst JSI, College Pk, MD 20742 USA. [Lohfink, Anne M.; Fabian, Andrew C.] Inst Astron, Cambridge CB3 OHA, England. [Ogle, Patrick M.; Lanz, Lauranne] CALTECH, Ctr Infrared Proc & Anal, Pasadena, CA 91125 USA. [Harrison, Fiona A.; Madsen, Kristin K.; Fuerst, Felix; Walton, Dominic J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Wik, Daniel R.; Zhang, William] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Madejski, Grzegorz] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Ballantyne, David R.] Georgia Inst Technol, Sch Phys, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Miller, Jon M.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Reynolds, CS (reprint author), Univ Maryland, Dept Astron, College Pk, MD 20742 USA. EM chris@astro.umd.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Lanz, Lauranne/0000-0002-3249-8224; Reynolds, Christopher/0000-0002-1510-4860; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNX14AF86G, NNG08FD60C]; National Aeronautics and Space Administration FX We thank the anonymous referee for their thorough and constructive comments that improved the quality of the manuscript. The authors also thank Francesco Tombesi for stimulating conversations throughout the course of this work. C.S.R. thanks NASA for support under grant NNX14AF86G. Our analysis makes use of the XSPEC_EMCEE package developed and distributed by Jeremy Sanders. This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). NR 49 TC 8 Z9 8 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 1 PY 2015 VL 808 IS 2 AR 154 DI 10.1088/0004-637X/808/2/154 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF0BA UT WOS:000371002400049 ER PT J AU Cai, WZ Liu, P Jin, YC Xue, QF Liu, F Russell, TP Huang, F Yip, HL Cao, Y AF Cai, Wanzhu Liu, Peng Jin, Yaocheng Xue, Qifan Liu, Feng Russell, Thomas P. Huang, Fei Yip, Hin-Lap Cao, Yong TI Morphology Evolution in High-Performance Polymer Solar Cells Processed from Nonhalogenated Solvent SO ADVANCED SCIENCE LA English DT Article ID NON-CHLORINATED SOLVENTS; BULK HETEROJUNCTION PHOTOCELLS; PHASE-SEPARATION; CONVERSION EFFICIENCY; BLENDS; SOLUBILITY; ADDITIVES; COMPOSITES; DESIGN C1 [Cai, Wanzhu; Liu, Peng; Jin, Yaocheng; Xue, Qifan; Huang, Fei; Yip, Hin-Lap; Cao, Yong] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. [Liu, Feng; Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. RP Liu, F (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM iamfengliu@gmail.com; tom.p.russell@gmail.com; msfhuang@scut.edu.cn; msangusyip@scut.edu.cn RI Liu, Feng/J-4361-2014 OI Liu, Feng/0000-0002-5572-8512 FU Ministry of Science and Technology of the People's Republic of China [2014CB643500]; Natural Science Foundation of China [51323003, 21125419]; Guangdong Natural Science Foundation [S2012030006232]; Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center - US Department of Energy, Office of Basic Energy Sciences [DE-SC0001087]; DOE, Office of Science; China Postdoctoral Science Foundation [2012M521595, 2013T60799]; Fundamental Research Funds for the Central Universities [2013ZB0014]; DOE, Office of Basic Energy Sciences FX This work was financially supported by the Ministry of Science and Technology of the People's Republic of China (No. 2014CB643500), the Natural Science Foundation of China (Nos. 51323003 and 21125419), and the Guangdong Natural Science Foundation (No. S2012030006232). F.L. and T.P.R. were supported by Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center funded by the US Department of Energy, Office of Basic Energy Sciences under award number DE-SC0001087. Portions of this research were carried out at beamline 7.3.3 and 11.0.1.2 at the Advanced Light Source, Lawrence Berkeley National Laboratory, which was supported by the DOE, Office of Science, and Office of Basic Energy Sciences. W.C. thanks the support of China Postdoctoral Science Foundation (2012M521595 and 2013T60799) and Fundamental Research Funds for the Central Universities (2013ZB0014). NR 43 TC 11 Z9 11 U1 14 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA EI 2198-3844 J9 ADV SCI JI Adv. Sci. PD AUG PY 2015 VL 2 IS 8 AR 1500095 DI 10.1002/advs.201500095 PG 7 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DC1SO UT WOS:000368997300008 PM 27980968 ER PT J AU Dixit, H Beekman, C Schleputz, CM Siemons, W Yang, Y Senabulya, N Clarke, R Chi, MF Christen, HM Cooper, VR AF Dixit, Hemant Beekman, Christianne Schlepuetz, Christian M. Siemons, Wolter Yang, Yongsoo Senabulya, Nancy Clarke, Roy Chi, Miaofang Christen, Hans M. Cooper, Valentino R. TI Understanding Strain-Induced Phase Transformations in BiFeO3 Thin Films SO ADVANCED SCIENCE LA English DT Article ID POLARIZATION; CRYSTAL; VISUALIZATION; PROPER AB Experiments demonstrate that under large epitaxial strain a coexisting striped phase emerges in BiFeO3 thin films, which comprises a tetragonal-like (T') and an intermediate S' polymorph. It exhibits a relatively large piezoelectric response when switching between the coexisting phase and a uniform T' phase. This strain-induced phase transformation is investigated through a synergistic combination of first-principles theory and experiments. The results show that the S' phase is energetically very close to the T' phase, but is structurally similar to the bulk rhombohedral (R) phase. By fully characterizing the intermediate S' polymorph, it is demonstrated that the flat energy landscape resulting in the absence of an energy barrier between the T' and S' phases fosters the above-mentioned reversible phase transformation. This ability to readily transform between the S' and T' polymorphs, which have very different octahedral rotation patterns and c/a ratios, is crucial to the enhanced piezoelectricity in strained BiFeO3 films. Additionally, a blueshift in the band gap when moving from R to S' to T' is observed. These results emphasize the importance of strain engineering for tuning electromechanical responses or, creating unique energy harvesting photonic structures, in oxide thin film architectures. C1 [Dixit, Hemant; Beekman, Christianne; Siemons, Wolter; Cooper, Valentino R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Schlepuetz, Christian M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Yang, Yongsoo; Senabulya, Nancy; Clarke, Roy] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Chi, Miaofang; Christen, Hans M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Dixit, H (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM dixithm@ornl.gov; christenhm@ornl.gov; coopervr@ornl.gov RI Cooper, Valentino /A-2070-2012; Chi, Miaofang/Q-2489-2015; Yang, Yongsoo/P-7716-2014; Christen, Hans/H-6551-2013; OI Cooper, Valentino /0000-0001-6714-4410; Chi, Miaofang/0000-0003-0764-1567; Yang, Yongsoo/0000-0001-8654-302X; Christen, Hans/0000-0001-8187-7469; Schleputz, Christian/0000-0002-0485-2708; Senabulya, Nancy/0000-0002-3394-5452 FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division; Office of Science Early Career Research Program; Scientific User Facilities Division; ORNL's Center for Nanophase Materials Sciences; ANL's Advanced Photon Source; DOE Office of Science [DE-AC02-05CH11231]; US Department of Energy [DE-FG02-06ER46273] FX This research was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division (authors H.D. V.R.C.: first-principles modeling; C.B., W.S., and H.M.C.: film growth, XRD, AFM, PFM), the Office of Science Early Career Research Program (V.R.C) and the Scientific User Facilities Division (author M.C.: STEM). User projects were supported at ORNL's Center for Nanophase Materials Sciences and ANL's Advanced Photon Source, which are DOE Office of Science user facilities. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the DOE Office of Science under Contract No. DE-AC02-05CH11231. Work in Michigan was supported by US Department of Energy (Contract No. DE-FG02-06ER46273, PI: R.C.). NR 36 TC 4 Z9 4 U1 7 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA EI 2198-3844 J9 ADV SCI JI Adv. Sci. PD AUG PY 2015 VL 2 IS 8 AR 1500041 DI 10.1002/advs.201500041 PG 7 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DC1SO UT WOS:000368997300002 PM 27980962 ER PT J AU Elliott, DC AF Elliott, Douglas C. TI Biofuel from fast pyrolysis and catalytic hydrodeoxygenation SO CURRENT OPINION IN CHEMICAL ENGINEERING LA English DT Article ID NI-CU CATALYSTS; BIO-OIL; PD/C CATALYST; LIQUID FUEL; HYDROTREATMENT; BIOMASS; HYDROGENATION; PRODUCTS; REACTOR; IMPACT AB This review addresses recent developments in biomass fast pyrolysis bio-oil upgrading by catalytic hydrotreating. The research in the field has expanded dramatically in the past few years with numerous new research groups entering the field while existing efforts from others grow. The issues revolve around the catalyst formulation and operating conditions. Much work in batch reactor tests with precious metal catalysts needs further validation to verify long-term operability in continuous flow systems. The effect of the low level of sulfur in bio-oil needs more study to be better understood. Utilization of the upgraded bio-oil for feedstock to finished fuels is still in an early stage of understanding. C1 [Elliott, Douglas C.] Pacific NW Natl Lab, POB 999,MSIN P8-60, Richland, WA 99352 USA. RP Elliott, DC (reprint author), Pacific NW Natl Lab, POB 999,MSIN P8-60, Richland, WA 99352 USA. EM dougc.elliott@pnnl.gov OI Elliott, Douglas/0000-0002-2807-4648 FU U.S. Department of Energy (DOE) [DE-AC05-76RL01830]; DOE Bioenergy Technologies Office FX This review was supported by the U.S. Department of Energy (DOE) under Contract DE-AC05-76RL01830 at the Pacific Northwest National Laboratory. Funding was provided by the DOE Bioenergy Technologies Office. NR 47 TC 3 Z9 3 U1 4 U2 23 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 2211-3398 J9 CURR OPIN CHEM ENG JI Curr. Opin. Chem. Eng. PD AUG PY 2015 VL 9 BP 59 EP 65 DI 10.1016/j.coche.2015.08.008 PG 7 WC Biotechnology & Applied Microbiology; Engineering, Chemical SC Biotechnology & Applied Microbiology; Engineering GA DB7AY UT WOS:000368668000010 ER PT J AU Benson, AR Ballard, G AF Benson, Austin R. Ballard, Grey TI A Framework for Practical Parallel Fast Matrix Multiplication SO ACM SIGPLAN NOTICES LA English DT Article DE fast matrix multiplication; dense linear algebra; parallel linear algebra; shared memory ID ALGORITHMS; COMPLEXITY AB Matrix multiplication is a fundamental computation in many scientific disciplines. In this paper, we show that novel fast matrix multiplication algorithms can significantly outperform vendor implementations of the classical algorithm and Strassen's fast algorithm on modest problem sizes and shapes. Furthermore, we show that the best choice of fast algorithm depends not only on the size of the matrices but also the shape. We develop a code generation tool to automatically implement multiple sequential and shared-memory parallel variants of each fast algorithm, including our novel parallelization scheme. This allows us to rapidly benchmark over 20 fast algorithms on several problem sizes. Furthermore, we discuss a number of practical implementation issues for these algorithms on shared-memory machines that can direct further research on making fast algorithms practical. C1 [Benson, Austin R.] Stanford Univ, Inst Computat & Math Engn, Stanford, CA 94305 USA. [Ballard, Grey] Sandia Natl Labs, Livermore, CA USA. RP Benson, AR (reprint author), Stanford Univ, Inst Computat & Math Engn, Stanford, CA 94305 USA. EM arbenson@stanford.edu; gmballa@sandia.gov FU Sandia Corporation under U.S. Department of Energy [DE-AC04-94AL85000]; Office of Technology Licensing Stanford Graduate Fellowship; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported in part by an appointment to the Sandia National Laboratories Truman Fellowship in National Security Science and Engineering, sponsored by Sandia Corporation (a wholly owned subsidiary of Lockheed Martin Corporation) as Operator of Sandia National Laboratories under its U.S. Department of Energy Contract No. DE-AC04-94AL85000. Austin R. Benson is also supported by an Office of Technology Licensing Stanford Graduate Fellowship.; This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 37 TC 1 Z9 1 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 42 EP 53 DI 10.1145/2688500.2688513 PG 12 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800005 ER PT J AU Chabbi, M Lavrijsen, W de Jong, W Sen, K Mellor-Crummey, J Iancu, C AF Chabbi, Milind Lavrijsen, Wim de Jong, Wibe Sen, Koushik Mellor-Crummey, John Iancu, Costin TI Barrier Elision for Production Parallel Programs SO ACM SIGPLAN NOTICES LA English DT Article DE Algorithms; Design; Performance; Barrier Elision; Synchronization; PGAS; NWChem; HPC; Dynamic Analysis; Dynamic Optimization AB Large scientific code bases are often composed of several layers of runtime libraries, implemented in multiple programming languages. In such situation, programmers often choose conservative synchronization patterns leading to suboptimal performance. In this paper, we present context-sensitive dynamic optimizations that elide barriers redundant during the program execution. In our technique, we perform data race detection alongside the program to identify redundant barriers in their calling contexts; after an initial learning, we start eliding all future instances of barriers occurring in the same calling context. We present an automatic on-the-fly optimization and a multi-pass guided optimization. We apply our techniques to NWChem-a 6 million line computational chemistry code written in C/C++/Fortran that uses several runtime libraries such as Global Arrays, ComEx, DMAPP, and MPI. Our technique elides a surprisingly high fraction of barriers (as many as 63%) in production runs. This redundancy elimination translates to application speedups as high as 14% on 2048 cores. Our techniques also provided valuable insight about the application behavior, later used by NWChem developers. Overall, we demonstrate the value of holistic context-sensitive analyses that consider the domain science in conjunction with the associated runtime software stack. C1 [Chabbi, Milind; Mellor-Crummey, John] Rice Univ, Houston, TX 77251 USA. [Lavrijsen, Wim; de Jong, Wibe; Iancu, Costin] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Sen, Koushik] Univ Calif Berkeley, Berkeley, CA USA. RP Chabbi, M (reprint author), Rice Univ, Houston, TX 77251 USA. EM milind.chabbi@rice.edu; wlavrijsen@lbl.gov; wadejong@lbl.gov; ksen@cs.berkeley.edu; johnmc@rice.edu; cciancu@lbl.gov RI DE JONG, WIBE/A-5443-2008 OI DE JONG, WIBE/0000-0002-7114-8315 FU U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research [DE-SC0008699, DE-SC0010473] FX Support for this work was provided in part through the X-Stack program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research under collaborative agreement numbers DE-SC0008699 and DE-SC0010473. NR 34 TC 0 Z9 0 U1 2 U2 4 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 109 EP 119 DI 10.1145/2688500.2688502 PG 11 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800011 ER PT J AU Tallent, NR Vishnu, A Van Dam, H Daily, J Kerbyson, DJ Hoisie, A AF Tallent, Nathan R. Vishnu, Abhinav Van Dam, Hubertus Daily, Jeff Kerbyson, Darren J. Hoisie, Adolfy TI Diagnosing the Causes and Severity of One-Sided Message Contention SO ACM SIGPLAN NOTICES LA English DT Article DE Network contention/congestion; one-sided messages; performance analysis; performance modeling ID PERFORMANCE; ALGORITHMS; PROGRAMS AB Two trends suggest network contention for one-sided messages is poised to become a performance problem that concerns application developers: an increased interest in one-sided programming models and a rising ratio of hardware threads to network injection bandwidth. Often it is difficult to reason about when one-sided tasks decrease or increase network contention. We present effective and portable techniques for diagnosing the causes and severity of one-sided message contention. To detect that a message is affected by contention, we maintain statistics representing instantaneous network resource demand. Using lightweight measurement and modeling, we identify the portion of a message's latency that is due to contention and whether contention occurs at the initiator or target. We attribute these metrics to program statements in their full static and dynamic context. We characterize contention for an important computational chemistry benchmark on InfiniBand, Cray Aries, and IBM Blue Gene/Q interconnects. We pinpoint the sources of contention, estimate their severity, and show that when message delivery time deviates from an ideal model, there are other messages contending for the same network links. With a small change to the benchmark, we reduce contention by 50% and improve total runtime by 20%. C1 [Tallent, Nathan R.; Vishnu, Abhinav; Van Dam, Hubertus; Daily, Jeff; Kerbyson, Darren J.; Hoisie, Adolfy] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Tallent, NR (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM tallent@pnnl.gov; vishnu@pnnl.gov; HubertusJJ.vanDam@pnnl.gov; Jeff.Daily@pnnl.gov; Darren.Kerbyson@pnnl.gov; Adolfy.Hoisie@pnnl.gov OI Daily, Jeff/0000-0001-6212-5173; van Dam, Hubertus Johannes Jacobus/0000-0002-0876-3294 FU U.S. Department of Energy (DOE), Office of Science, Advanced Scientific Computing Research [62426, 62855, 59542]; DOE [DE-AC05-76RL01830] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Advanced Scientific Computing Research, under award numbers 62426 (Performance Insight for Programmers and Exascale), 62855 (Beyond the Standard Model), and 59542 (Performance Health Monitoring for Large-Scale Systems). We used resources of the Oak Ridge and Argonne Leadership Computing Facilities under INCITE (Innovative and Novel Computational Impact on Theory and Experiment) award Performance Evaluation and Analysis Consortium (PEAC) End Station.; Pacific Northwest National Laboratory is operated by Battelle for the DOE under contract DE-AC05-76RL01830. NR 44 TC 0 Z9 0 U1 1 U2 4 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 130 EP 139 DI 10.1145/2688500.2688516 PG 10 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800013 ER PT J AU Amer, A Lu, HW Wei, YJ Balaji, P Matsuoka, S AF Amer, Abdelhalim Lu, Huiwei Wei, Yanjie Balaji, Pavan Matsuoka, Satoshi TI MPI plus Threads: Runtime Contention and Remedies SO ACM SIGPLAN NOTICES LA English DT Article DE MPI; threads; runtime contention; critical section ID PERFORMANCE AB Hybrid MPI+Threads programming has emerged as an alternative model to the "MPI everywhere" model to better handle the increasing core density in cluster nodes. While the MPI standard allows multithreaded concurrent communication, such flexibility comes with the cost of maintaining thread safety within the MPI implementation, typically implemented using critical sections. In contrast to previous works that studied the importance of critical-section granularity in MPI implementations, in this paper we investigate the implication of critical-section arbitration on communication performance. We first analyze the MPI runtime when multithreaded concurrent communication takes place on hierarchical memory systems. Our results indicate that the mutex-based approach that most MPI implementations use today can incur performance penalties due to unfair arbitration. We then present methods to mitigate these penalties with a first-come, first-served arbitration and a priority locking scheme that favors threads doing useful work. Through evaluations using several benchmarks and applications, we demonstrate up to 5-fold improvement in performance. C1 [Amer, Abdelhalim; Matsuoka, Satoshi] Tokyo Inst Technol, Tokyo, Japan. [Lu, Huiwei; Balaji, Pavan] Argonne Natl Lab, Argonne, IL 60439 USA. [Wei, Yanjie] Chinese Acad Sci, Shenzhen Inst Adv Technol, Beijing 100864, Peoples R China. RP Amer, A (reprint author), Tokyo Inst Technol, Tokyo, Japan. EM amer@matsulab.is.titech.ac.jp; huiweilu@anl.gov; yj.wei@siat.ac.cn; balaji@anl.gov; matsu@is.titech.ac.jp FU JSPS [23220003]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX This work was supported by JSPS KAKENHI Grant Number 23220003 and by the U.S. Department of Energy, Office of Science, under Contract DE-AC02-06CH11357. NR 24 TC 1 Z9 1 U1 1 U2 1 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 239 EP 248 DI 10.1145/2688500.2688522 PG 10 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800023 ER PT J AU Kim, J Lee, S Vetter, JS AF Kim, Jungwon Lee, Seyong Vetter, Jeffrey S. TI An OpenACC-Based Unified Programming Model for Multi-accelerator Systems SO ACM SIGPLAN NOTICES LA English DT Article DE OpenACC; Programming models; Heterogeneous computing; Accelerators AB This paper proposes a novel SPMD programming model of OpenACC. Our model integrates the different granularities of parallelism from vector-level parallelism to node-level parallelism into a single, unified model based on OpenACC. It allows programmers to write programs for multiple accelerators using a uniform programming model whether they are in shared or distributed memory systems. We implement a prototype of our model and evaluate its performance with a GPU-based supercomputer using three benchmark applications. C1 [Kim, Jungwon; Lee, Seyong; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Vetter, Jeffrey S.] Georgia Inst Technol, Atlanta, GA 30332 USA. RP Kim, J (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM kimj@ornl.gov; lees2@ornl.gov; vetter@computer.org FU U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research; U.S. Department of Energy [DE-AC0500OR22725] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research.; This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC0500OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. NR 1 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 257 EP 258 DI 10.1145/2688500.2688531 PG 2 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800028 ER PT J AU Haidar, A Dong, TX Luszczek, P Tomov, S Dongarra, J AF Haidar, Azzam Dong, Tingxing Luszczek, Piotr Tomov, Stanimire Dongarra, Jack TI Towards Batched Linear Solvers on Accelerated Hardware Platforms SO ACM SIGPLAN NOTICES LA English DT Article DE batched factorization; numerical linear algebra; hardware accelerators; numerical software libraries; one-sided factorization algorithms AB As hardware evolves, an increasingly effective approach to develop energy efficient, high-performance solvers, is to design them to work on many small and independent problems. Indeed, many applications already need this functionality, especially for GPUs, which are known to be currently about four to five times more energy efficient than multicore CPUs for every floating-point operation. In this paper, we describe the development of the main one-sided factorizations: LU, QR, and Cholesky; that are needed for a set of small dense matrices to work in parallel. We refer to such algorithms as batched factorizations. Our approach is based on representing the algorithms as a sequence of batched BLAS routines for GPU-contained execution. Note that this is similar in functionality to the LAPACK and the hybrid MAGMA algorithms for large-matrix factorizations. But it is different from a straightforward approach, whereby each of GPU's symmetric multiprocessors factorizes a single problem at a time. We illustrate how our performance analysis together with the profiling and tracing tools guided the development of batched factorizations to achieve up to 2-fold speedup and 3-fold better energy efficiency compared to our highly optimized batched CPU implementations based on the MKL library on a two-sockets, Intel Sandy Bridge server. Compared to a batched LU factorization featured in the NVIDIA's CUBLAS library for GPUs, we achieves up to 2.5-fold speedup on the K40 GPU. C1 [Haidar, Azzam; Dong, Tingxing; Luszczek, Piotr; Tomov, Stanimire; Dongarra, Jack] Univ Tennessee, Knoxville, TN 37916 USA. [Dongarra, Jack] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Dongarra, Jack] Univ Manchester, Manchester M13 9PL, Lancs, England. RP Haidar, A (reprint author), Univ Tennessee, Knoxville, TN 37916 USA. EM haidar@eecs.utk.edu; tdong@eecs.utk.edu; luszczek@eecs.utk.edu; tomov@eecs.utk.edu; dongarra@eecs.utk.edu NR 0 TC 0 Z9 0 U1 1 U2 1 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 261 EP 262 DI 10.1145/2688500.2688534 PG 2 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800030 ER PT J AU Pearce, O Gamblin, T de Supinski, BR Schulz, M Amato, NM AF Pearce, Olga Gamblin, Todd de Supinski, Bronis R. Schulz, Martin Amato, Nancy M. TI Decoupled Load Balancing SO ACM SIGPLAN NOTICES LA English DT Article DE load balance; parallel algorithm; performance AB Modern scientific simulations divide work between parallel processors by decomposing a spatial domain of mesh cells, particles, or other elements. A balanced assignment of the computational load is critical for parallel performance. If the computation per element changes over the simulation time, simulations can use dynamic load balance algorithms to evenly redistribute work to processes. Graph partitioners are widely used and balance very effectively, but they do not strong scale well. Typical SPMD simulations wait while a load balance algorithm runs on all processors, so a poorly scaling algorithm can itself become a bottleneck. We observe that the load balance algorithm is separate from the main application computation and has its own scaling properties. We propose to decouple the load balance algorithm from the application, and to offload the load balance computation so that it runs concurrently with the application on a smaller number of processors. We demonstrate the costs of decoupling and offloading the load balancing algorithm from a Barnes-Hut application. C1 [Pearce, Olga; Amato, Nancy M.] Texas A&M Univ, Dept Comp Sci & Engn, College Stn, TX 77834 USA. [Pearce, Olga; Gamblin, Todd; de Supinski, Bronis R.; Schulz, Martin] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA USA. RP Pearce, O (reprint author), Texas A&M Univ, Dept Comp Sci & Engn, College Stn, TX 77834 USA. EM olga@cse.tamu.edu; tgamblin@llnl.gov; bronis@llnl.gov; schulzm@llnl.gov; amato@cse.tamu.edu NR 4 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 267 EP 268 DI 10.1145/2688500.2688539 PG 2 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800033 ER PT J AU Jin, Y Liu, ML Ma, XS Liu, Q Logan, J Podhorszki, N Choi, JY Klasky, S AF Jin, Ye Liu, Mingliang Ma, Xiaosong Liu, Qing Logan, Jeremy Podhorszki, Norbert Choi, Jong Youl Klasky, Scott TI Combining Phase Identification and Statistic Modeling for Automated Parallel Benchmark Generation SO ACM SIGPLAN NOTICES LA English DT Article DE HPC applications; trace; phase identification; statistical profiling; automatic benchmark generation AB Parallel application benchmarks are indispensable for evaluating/optimizing HPC software and hardware. However, it is very challenging and costly to obtain high-fidelity benchmarks reflecting the scale and complexity of state-of-the-art parallel applications. Hand-extracted synthetic benchmarks are time-and labor-intensive to create. Real applications themselves, while offering most accurate performance evaluation, are expensive to compile, port, reconfigure, and often plainly inaccessible due to security or ownership concerns. This work contributes APPRIME, a novel tool for trace-based automatic parallel benchmark generation. Taking as input standard communication-I/O traces of an application's execution, it couples accurate automatic phase identification with statistical regeneration of event parameters to create compact, portable, and to some degree reconfigurable parallel application benchmarks. Experiments with four NAS Parallel Benchmarks (NPB) and three real scientific simulation codes confirm the fidelity of APPRIME benchmarks. They retain the original applications' performance characteristics, in particular the relative performance across platforms. C1 [Jin, Ye; Liu, Mingliang; Ma, Xiaosong] NCSU, Raleigh, NC 27695 USA. [Jin, Ye; Liu, Mingliang; Ma, Xiaosong] QCRI, Doha, Qatar. [Liu, Qing; Logan, Jeremy; Podhorszki, Norbert; Choi, Jong Youl; Klasky, Scott] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Jin, Y (reprint author), NCSU, Raleigh, NC 27695 USA. EM yjin@qf.org.qa; mliu@qf.org.qa; xma@qf.org.qa; liuq@ornl.gov; loganjs@ornl.gov; pnorbert@ornl.gov; choij@ornl.gov; klasky@ornl.gov NR 11 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 269 EP 270 DI 10.1145/2688500.2688541 PG 2 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800034 ER PT J AU Shi, XH Liang, JL Di, S He, BS Jin, H Lu, L Wang, ZX Luo, X Zhong, JL AF Shi, Xuanhua Liang, Junling Di, Sheng He, Bingsheng Jin, Hai Lu, Lu Wang, Zhixiang Luo, Xuan Zhong, Jianlong TI Optimization of Asynchronous Graph Processing on GPU with Hybrid Coloring Model SO ACM SIGPLAN NOTICES LA English DT Article DE Graph Processing; Asynchronous Computing; GPGPU AB Modern GPUs have been widely used to accelerate the graph processing for complicated computational problems regarding graph theory. Many parallel graph algorithms adopt the asynchronous computing model to accelerate the iterative convergence. Unfortunately, the consistent asynchronous computing requires locking or the atomic operations, leading to significant penalties/overheads when implemented on GPUs. To this end, coloring algorithm is adopted to separate the vertices with potential updating conflicts, guaranteeing the consistency/correctness of the parallel processing. We propose a light-weight asynchronous processing framework called Frog with a hybrid coloring model. We find that majority of vertices (about 80%) are colored with only a few colors, such that they can be read and updated in a very high degree of parallelism without violating the sequential consistency. Accordingly, our solution will separate the processing of the vertices based on the distribution of colors. C1 [Shi, Xuanhua; Liang, Junling; Jin, Hai; Lu, Lu; Wang, Zhixiang; Luo, Xuan] Huazhong Univ Sci & Technol, Sch Comp Sci & Technol, Serv Comp Technol & Syst Lab, Cluster & Grid Comp Lab, Wuhan, Peoples R China. [Di, Sheng] Argonne Natl Lab, Argonne, IL 60439 USA. [He, Bingsheng; Zhong, Jianlong] Nanyang Technol Univ, Sch Comp Engn, Singapore 639798, Singapore. RP Shi, XH (reprint author), Huazhong Univ Sci & Technol, Sch Comp Sci & Technol, Serv Comp Technol & Syst Lab, Cluster & Grid Comp Lab, Wuhan, Peoples R China. EM xhshi@hust.edu.cn; junlingliang@hust.edu.cn; disheng222@gmail.com; bshe@ntu.edu.sg; hjin@hust.edu.cn; llu@hust.edu.cn; wangzhx123@hust.edu.cn; luoxuan@hust.edu.cn; jlzhong@ntu.edu.sg FU NSFC [61133008, 61370104]; Chinese Universities Scientific Fund [2014TS008]; U.S. Department of Energy, Office of Science, and Tencent [DE-ACO2-06CH11357]; MoE AcRF Tier 2 grant in Singapore [MOE2012-T2-2-067] FX This work is supported by the NSFC under grants No.61133008 and No. 61370104, Chinese Universities Scientific Fund under grant No. 2014TS008, the U.S. Department of Energy, Office of Science, under Contract DE-ACO2-06CH11357, and Tencent. Bingsheng He and Jianlong Zhong are partly supported by a MoE AcRF Tier 2 grant (MOE2012-T2-2-067) in Singapore. NR 5 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD AUG PY 2015 VL 50 IS 8 BP 271 EP 272 DI 10.1145/2688500.2688542 PG 2 WC Computer Science, Software Engineering SC Computer Science GA CZ7BL UT WOS:000367254800035 ER PT J AU Joubert, W Archibald, R Berrill, M Brown, WM Eisenbach, M Grout, R Larkin, J Levesque, J Messer, B Norman, M Philip, B Sankaran, R Tharrington, A Turner, J AF Joubert, Wayne Archibald, Rick Berrill, Mark Brown, W. Michael Eisenbach, Markus Grout, Ray Larkin, Jeff Levesque, John Messer, Bronson Norman, Matt Philip, Bobby Sankaran, Ramanan Tharrington, Arnold Turner, John TI Accelerated application development: The ORNL Titan experience SO COMPUTERS & ELECTRICAL ENGINEERING LA English DT Article DE High performance computing; Accelerated computing; GPU graphics processing units; Science applications; Code refactoring; Software optimization AB The use of computational accelerators such as NVIDIA GPUs and Intel Xeon Phi processors is now widespread in the high performance computing community, with many applications delivering impressive performance gains. However, programming these systems for high performance, performance portability and software maintainability has been a challenge. In this paper we discuss experiences porting applications to the Titan system. Titan, which began planning in 2009 and was deployed for general use in 2013, was the first multi-petaflop system based on accelerator hardware. To ready applications for accelerated computing, a preparedness effort was undertaken prior to delivery of Titan. In this paper we report experiences and lessons learned from this process and describe how users are currently making use of computational accelerators on Titan. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Joubert, Wayne; Archibald, Rick; Berrill, Mark; Brown, W. Michael; Eisenbach, Markus; Messer, Bronson; Norman, Matt; Philip, Bobby; Sankaran, Ramanan; Tharrington, Arnold; Turner, John] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Levesque, John] Cray Inc, Knoxville, TN USA. [Grout, Ray] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Larkin, Jeff] NVIDIA Corp, Oak Ridge, TN 37831 USA. RP Joubert, W (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM joubert@ornl.gov RI Archibald, Rick/I-6238-2016; Sankaran, Ramanan/D-9254-2015; Messer, Bronson/G-1848-2012; OI Archibald, Rick/0000-0002-4538-9780; Sankaran, Ramanan/0000-0002-5352-9915; Messer, Bronson/0000-0002-5358-5415; Philip, Bobby/0000-0001-6716-3515; Eisenbach, Markus/0000-0001-8805-8327; Berrill, Mark/0000-0002-4525-3939; Turner, John/0000-0003-2521-4091 FU Office of Science of the U.S. Department of Energy [DE-ACO5-000R22725] FX This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-ACO5-000R22725. NR 30 TC 1 Z9 1 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7906 EI 1879-0755 J9 COMPUT ELECTR ENG JI Comput. Electr. Eng. PD AUG PY 2015 VL 46 BP 123 EP 138 DI 10.1016/j.compeleceng.2015.04.008 PG 16 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Engineering, Electrical & Electronic SC Computer Science; Engineering GA CZ5DN UT WOS:000367122800011 ER PT J AU Frumhoff, PC Burkett, V Jackson, RB Newmark, R Overpeck, J Webber, M AF Frumhoff, Peter C. Burkett, Virginia Jackson, Robert B. Newmark, Robin Overpeck, Jonathan Webber, Michael TI Vulnerabilities and opportunities at the nexus of electricity, water and climate SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Editorial Material DE electricty; water; climate; vulnerability; adaptation; resilience ID DROUGHT; CALIFORNIA; RISK AB The articles in this special issue examine the critical nexus of electricity, water, and climate, emphasizing connections among resources; the prospect of increasing vulnerabilities of water resources and electricity generation in a changing climate; and the opportunities for research to inform integrated energy and water policy and management measures aimed at reducing vulnerability and increasing resilience. Here, we characterize several major themes emerging from this research and highlight some of the uptake of this work in both scientific and public spheres. Underpinning much of this research is the recognition that water resources are expected to undergo substantial changes based on the global warming that results primarily from fossil energy-based carbon emissions. At the same time, the production of electricity from fossil fuels, nuclear power, and some renewable technologies (biomass, geothermal and concentrating solar power) can be highly water-intensive. Energy choices now and in the near future will have a major impact not just on the global climate, but also on water supplies and the resilience of energy systems that currently depend heavily on them. C1 [Frumhoff, Peter C.] Union Concerned Scientists, Cambridge, MA 02138 USA. [Burkett, Virginia] US Geol Survey, Reston, VA 22092 USA. [Jackson, Robert B.] Stanford Univ, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA. [Newmark, Robin] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Overpeck, Jonathan] Univ Arizona, Inst Environm, Tucson, AZ 85721 USA. [Webber, Michael] Univ Texas Austin, Austin, TX 78712 USA. RP Frumhoff, PC (reprint author), Union Concerned Scientists, Cambridge, MA 02138 USA. EM pfrumhoff@ucsusa.org NR 38 TC 3 Z9 3 U1 9 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD AUG PY 2015 VL 10 IS 8 AR 080201 DI 10.1088/1748-9326/10/8/080201 PG 5 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA CZ3JD UT WOS:000366999400001 ER PT J AU Sigrin, B Pless, J Drury, E AF Sigrin, Ben Pless, Jacquelyn Drury, Easan TI Diffusion into new markets: evolving customer segments in the solar photovoltaics market SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE renewable energy; data analysis; technology diffusion; solar photovoltaics; distributed generation; customer acquisition ID ENERGY TECHNOLOGY ADOPTION; POWER-SYSTEMS AB The US residential solar market is growing quickly, and as solar adoption diffuses into new populations, later adopters may differ significantly from earlier ones. Using a unique household-level survey dataset including 1234 adopters and 790 non-adopters from San Diego County, California, we explore differences in attitudinal and socio-economic factors for three groups: (i) adopters and nonadopters; (ii) early and more recent adopters; (iii) consumers adopting via buying or leasing. Our results suggest that adopters overall have higher incomes, are more educated, live in larger homes, and expect to stay in their homes for longer than their non-adopting peers. They also differ in their expectations of electricity retail rate changes and the impact solar could have on their home resale value. When examining differences between early and more recent adopters, we find that recent adopters are more representative of general homeowners and more politically moderate. They are also increasingly installing solar to protect against future electricity price increases and to lower electricity costs as opposed to adopting strictly for environmental reasons. Furthermore, more recent adopters differ significantly from earlier adopters in the situations that prompted them to adopt. The findings demonstrate how solar markets are evolving, reflecting changes in the underlying drivers of consumer adoption as well as innovative solar marketing strategies. C1 [Sigrin, Ben; Pless, Jacquelyn; Drury, Easan] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Pless, Jacquelyn] Colorado Sch Mines, Golden, CO 80401 USA. [Drury, Easan] SunEdison, Denver, CO 80202 USA. RP Sigrin, B (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM benjamin.sigrin@nrel.gov; jacquelyn.pless@nrel.gov; edrury@sunedison.com FU US Department of Energy [DE-AC36-08GO28308, SM13SB01] FX This work was funded by the US Department of Energy under contract number DE-AC36-08GO28308, prepared under task number SM13SB01. The authors thank Tim Treadwell and Georgina Arreola of the California Center for Sustainable Energy, who contributed to fielding the consumer surveys. Any errors are those of the authors alone. NR 27 TC 3 Z9 3 U1 4 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD AUG PY 2015 VL 10 IS 8 AR 084001 DI 10.1088/1748-9326/10/8/084001 PG 8 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA CZ3JD UT WOS:000366999400002 ER PT J AU Cuesta, C Abgrall, N Arnquist, IJ Avignone, FT Barabash, AS Bertrand, FE Brudanin, V Busch, M Buuck, M Byram, D Caldwell, AS Chan, YD Christofferson, CD Detwiler, JA Efremenko, Y Ejiri, H Elliott, SR Galindo-Uribarri, A Giovanetti, GK Goett, J Green, MP Gruszko, J Guinn, IS Guiseppe, VE Henning, R Hoppe, EW Howard, S Howe, MA Jasinski, BR Keeter, KJ Kidd, MF Konovalov, SI Kouzes, RT LaFerriere, BD Leon, J MacMullin, J Martin, RD Meijer, SJ Mertens, S Orrell, JL O'Shaughnessy, C Overman, NR Poon, AWP Radford, DC Rager, J Rielage, K Robertson, RGH Romero-Romero, E Schmitt, C Shanks, B Shirchenko, M Snyder, N Suriano, AM Tedeschi, D Timkin, V Trimble, JE Varner, RL Vasilyev, S Vetter, K Vorren, K White, BR Wilkerson, JF Wiseman, C Xu, W Yakushev, E Yu, CH Yumatov, V AF Cuesta, C. Abgrall, N. Arnquist, I. J. Avignone, F. T., III Barabash, A. S. Bertrand, F. E. Brudanin, V. Busch, M. Buuck, M. Byram, D. Caldwell, A. S. Chan, Y-D. Christofferson, C. D. Detwiler, J. A. Efremenko, Yu Ejiri, H. Elliott, S. R. Galindo-Uribarri, A. Giovanetti, G. K. Goett, J. Green, M. P. Gruszko, J. Guinn, I. S. Guiseppe, V. E. Henning, R. Hoppe, E. W. Howard, S. Howe, M. A. Jasinski, B. R. Keeter, K. J. Kidd, M. F. Konovalov, S. I. Kouzes, R. T. LaFerriere, B. D. Leon, J. MacMullin, J. Martin, R. D. Meijer, S. J. Mertens, S. Orrell, J. L. O'Shaughnessy, C. Overman, N. R. Poon, A. W. P. Radford, D. C. Rager, J. Rielage, K. Robertson, R. G. H. Romero-Romero, E. Schmitt, C. Shanks, B. Shirchenko, M. Snyder, N. Suriano, A. M. Tedeschi, D. Timkin, V. Trimble, J. E. Varner, R. L. Vasilyev, S. Vetter, K. Vorren, K. White, B. R. Wilkerson, J. F. Wiseman, C. Xu, W. Yakushev, E. Yu, C. -H. Yumatov, V. TI Status of the MAJORANA DEMONSTRATOR SO NUCLEAR AND PARTICLE PHYSICS PROCEEDINGS LA English DT Proceedings Paper CT 8th Neutrino Oscillation Workshop (NOW) CY SEP 07-13, 2014 CL Conca Specchiulla, ITALY SP Ist Nazl Fisica Nucleare, Dipartimento Interateneo Fisica Michelangelo Merlin, Ist Nazl Fisica Nucleare, Dipartimento Matematica & Fisica Ennio Giorgi, Univ Bari, Univ Salento, Ist Nazl Fisica Nucleare, Italian Ministero Istruzione, Univ Ric DE neutrinoless double-beta decay; germanium detector; majorana AB The MAJORANA Collaboration is constructing the MAJORANA DEMONSTRATOR, an ultra-low background, 40-kg modular high purity Ge detector array to search for neutrinoless double-beta decay in Ge-76. In view of the next generation of tonne-scale Ge-based neutrinoless double-beta decay searches that will probe the neutrino mass scale in the inverted-hierarchy region, a major goal of the DEMONSTRATOR IS to demonstrate a path forward to achieving a background rate at or below 1 count/tonne/year in the 4 keV region of interest around the Q-value at 2039 keV. The current status of the DEMONSTRATOR is discussed, as are plans for its completion. C1 [Cuesta, C.; Buuck, M.; Detwiler, J. A.; Gruszko, J.; Guinn, I. S.; Leon, J.; Robertson, R. G. H.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA. [Cuesta, C.; Buuck, M.; Detwiler, J. A.; Gruszko, J.; Guinn, I. S.; Leon, J.; Robertson, R. G. H.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Abgrall, N.; Chan, Y-D.; Mertens, S.; Poon, A. W. P.; Schmitt, C.; Vetter, K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Arnquist, I. J.; Hoppe, E. W.; Kouzes, R. T.; LaFerriere, B. D.; Orrell, J. L.; Overman, N. R.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Avignone, F. T., III; Guiseppe, V. E.; Tedeschi, D.; Wiseman, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Avignone, F. T., III; Bertrand, F. E.; Galindo-Uribarri, A.; Green, M. P.; Radford, D. C.; Romero-Romero, E.; Varner, R. L.; White, B. R.; Wilkerson, J. F.; Yu, C. -H.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Barabash, A. S.; Konovalov, S. I.; Yumatov, V.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Elliott, S. R.; Goett, J.; Rielage, K.; Xu, W.] Los Alamos Natl Lab, Los Alamos, NM USA. [Brudanin, V.; Shirchenko, M.; Timkin, V.; Vasilyev, S.; Yakushev, E.] Joint Inst Nucl Res, Dubna, Russia. [Busch, M.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Busch, M.; Giovanetti, G. K.; Henning, R.; Howe, M. A.; MacMullin, J.; Meijer, S. J.; O'Shaughnessy, C.; Rager, J.; Shanks, B.; Trimble, J. E.; Vorren, K.; Wilkerson, J. F.] Triangle Univ Nucl Lab, Durham, NC 27706 USA. [Byram, D.; Jasinski, B. R.; Martin, R. D.; Snyder, N.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. [Caldwell, A. S.; Christofferson, C. D.; Howard, S.; Suriano, A. M.] South Dakota Sch Mines & Technol, Rapid City, SD USA. [Efremenko, Yu; Romero-Romero, E.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Ejiri, H.] Osaka Univ, Nucl Phys Res Ctr, Osaka, Japan. [Ejiri, H.] Osaka Univ, Dept Phys, Osaka, Japan. [Giovanetti, G. K.; Henning, R.; Howe, M. A.; MacMullin, J.; Meijer, S. J.; O'Shaughnessy, C.; Rager, J.; Shanks, B.; Trimble, J. E.; Vorren, K.; Wilkerson, J. F.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC USA. [Keeter, K. J.] Black Hills State Univ, Dept Phys, Spearfish, SD 57799 USA. [Kidd, M. F.] Tennessee Technol Univ, Cookeville, TN USA. [Vetter, K.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Cuesta, C (reprint author), Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA. RI Barabash, Alexander/S-8851-2016; Cuesta, Clara/L-5466-2014; OI Cuesta, Clara/0000-0003-1190-7233; Rielage, Keith/0000-0002-7392-7152 NR 2 TC 0 Z9 0 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2405-6014 EI 1873-3832 J9 NUCL PART PHYS P JI Nucl. Part. Phys. Proc. PD AUG-SEP PY 2015 VL 265 BP 70 EP 72 DI 10.1016/j.nuclphysbps.2015.06.019 PG 3 GA CQ9QT UT WOS:000360950700019 ER PT J AU Canonica, L Artusa, DR Avignone, FT Azzolini, O Balata, M Banks, TI Bari, G Beeman, J Bellini, F Bersani, A Biassoni, M Brofferio, C Bucci, C Cai, XZ Camacho, A Caminata, A Cao, XG Capelli, S Cappelli, L Carbone, L Cardani, L Casali, N Cassina, L Chiesa, D Chott, N Clemenza, M Copello, S Cosmelli, C Cremonesi, O Creswick, RJ Cushman, JS Dafinei, I Dally, A Datskov, V Dell'Oro, S Deninno, MM Di Domizio, S Di Vacri, ML Drobizhev, A Ejzak, L Fang, DQ Farach, HA Faverzani, M Fernandes, G Ferri, E Ferroni, F Fiorini, E Franceschi, MA Freedman, SJ Fujikawa, BK Giachero, A Gironi, L Giuliani, A Gorla, P Gotti, C Gutierrez, TD Haller, EE Han, K Hansen, E Heeger, KM Hennings-Yeomans, R Hickerson, KP Huang, HZ Kadel, R Keppel, G Kolomensky, YG Li, YL Ligi, C Lim, KE Liu, X Ma, YG Maiano, C Maino, M Martinez, M Maruyama, RH Mei, Y Moggi, N Morganti, S Napolitano, T Nisi, S Nones, C Norman, EB Nucciotti, A O'Donnell, T Orio, F Orlandi, D Ouellet, JL Pagliarone, CE Pallavicini, M Palmieri, V Pattavina, L Pavan, M Pessina, G Pettinacci, V Piperno, G Pira, C Pirro, S Pozzi, S Previtali, E Rosenfeld, C Rusconi, C Sala, E Sangiorgio, S Santone, D Scielzo, ND Sisti, M Smith, AR Taffarello, L Tenconi, M Terranova, F Tian, WD Tomei, C Trentalange, S Ventura, G Vignati, M Wang, BS Wang, HW Wielgus, L Wilson, J Winslow, LA Wise, T Woodcraft, A Zanotti, L Zarra, C Zhang, GQ Zhu, BX Zucchelli, S AF Canonica, L. Artusa, D. R. Avignone, F. T., III Azzolini, O. Balata, M. Banks, T. I. Bari, G. Beeman, J. Bellini, F. Bersani, A. Biassoni, M. Brofferio, C. Bucci, C. Cai, X. Z. Camacho, A. Caminata, A. Cao, X. G. Capelli, S. Cappelli, L. Carbone, L. Cardani, L. Casali, N. Cassina, L. Chiesa, D. Chott, N. Clemenza, M. Copello, S. Cosmelli, C. Cremonesi, O. Creswick, R. J. Cushman, J. S. Dafinei, I. Dally, A. Datskov, V. Dell'Oro, S. Deninno, M. M. Di Domizio, S. Di Vacri, M. L. Drobizhev, A. Ejzak, L. Fang, D. Q. Farach, H. A. Faverzani, M. Fernandes, G. Ferri, E. Ferroni, F. Fiorini, E. Franceschi, M. A. Freedman, S. J. Fujikawa, B. K. Giachero, A. Gironi, L. Giuliani, A. Gorla, P. Gotti, C. Gutierrez, T. D. Haller, E. E. Han, K. Hansen, E. Heeger, K. M. Hennings-Yeomans, R. Hickerson, K. P. Huang, H. Z. Kadel, R. Keppel, G. Kolomensky, Yu G. Li, Y. L. Ligi, C. Lim, K. E. Liu, X. Ma, Y. G. Maiano, C. Maino, M. Martinez, M. Maruyama, R. H. Mei, Y. Moggi, N. Morganti, S. Napolitano, T. Nisi, S. Nones, C. Norman, E. B. Nucciotti, A. O'Donnell, T. Orio, F. Orlandi, D. Ouellet, J. L. Pagliarone, C. E. Pallavicini, M. Palmieri, V. Pattavina, L. Pavan, M. Pessina, G. Pettinacci, V. Piperno, G. Pira, C. Pirro, S. Pozzi, S. Previtali, E. Rosenfeld, C. Rusconi, C. Sala, E. Sangiorgio, S. Santone, D. Scielzo, N. D. Sisti, M. Smith, A. R. Taffarello, L. Tenconi, M. Terranova, F. Tian, W. D. Tomei, C. Trentalange, S. Ventura, G. Vignati, M. Wang, B. S. Wang, H. W. Wielgus, L. Wilson, J. Winslow, L. A. Wise, T. Woodcraft, A. Zanotti, L. Zarra, C. Zhang, G. Q. Zhu, B. X. Zucchelli, S. TI Results of CUORE-0 and prospects for the CUORE experiment SO NUCLEAR AND PARTICLE PHYSICS PROCEEDINGS LA English DT Proceedings Paper CT 8th Neutrino Oscillation Workshop (NOW) CY SEP 07-13, 2014 CL Conca Specchiulla, ITALY SP Ist Nazl Fisica Nucleare, Dipartimento Interateneo Fisica Michelangelo Merlin, Ist Nazl Fisica Nucleare, Dipartimento Matematica & Fisica Ennio Giorgi, Univ Bari, Univ Salento, Ist Nazl Fisica Nucleare, Italian Ministero Istruzione, Univ Ric DE Double Beta Decay; Bolometers; Neutrino Mass ID RADIOACTIVE CONTAMINATION; VALIDATION AB The CUORE (Cryogenic Underground Observatory for Rare Events) experiment is an array of 741 kg of TeO2 bolometers to search for neutrinoless double beta decay (beta beta 0 nu) of Te-130. The detector is being constructed at the Laboratori Nazionali del Gran Sasso (Italy) where it will start operation in 2015. To test and demonstrate the possibility of realising such a large scale bolometric detector, a prototype (CUORE-0) has been realised. The CUORE-0 detector is a single tower of 52 CUORE-like bolometers. CUORE-0 data taking started in Spring 2013. The status of CUORE and the first CUORE-0 data are here reported. C1 [Canonica, L.; Artusa, D. R.; Balata, M.; Bucci, C.; Cappelli, L.; Casali, N.; Dell'Oro, S.; Di Vacri, M. L.; Gorla, P.; Nisi, S.; Orlandi, D.; Pagliarone, C. E.; Pattavina, L.; Pirro, S.; Santone, D.; Zarra, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. [Artusa, D. R.; Avignone, F. T., III; Chott, N.; Creswick, R. J.; Farach, H. A.; Rosenfeld, C.; Wilson, J.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Azzolini, O.; Camacho, A.; Keppel, G.; Palmieri, V.; Pira, C.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. [Banks, T. I.; Drobizhev, A.; Freedman, S. J.; Hennings-Yeomans, R.; Kolomensky, Yu G.; O'Donnell, T.; Ouellet, J. L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Banks, T. I.; Freedman, S. J.; Fujikawa, B. K.; Hennings-Yeomans, R.; Mei, Y.; O'Donnell, T.; Ouellet, J. L.; Smith, A. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bari, G.; Deninno, M. M.; Moggi, N.; Zucchelli, S.] Ist Nazl Fis Nucl, Sez Bologna, I-40127 Bologna, Italy. [Beeman, J.; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Cosmelli, C.; Ferroni, F.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Bellini, F.; Cardani, L.; Cosmelli, C.; Dafinei, I.; Ferroni, F.; Morganti, S.; Orio, F.; Pettinacci, V.; Piperno, G.; Tomei, C.; Vignati, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bersani, A.; Di Domizio, S.; Fernandes, G.; Pallavicini, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Cassina, L.; Chiesa, D.; Clemenza, M.; Faverzani, M.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Pozzi, S.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carbone, L.; Cassina, L.; Chiesa, D.; Clemenza, M.; Cremonesi, O.; Datskov, V.; Faverzani, M.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Pessina, G.; Pozzi, S.; Previtali, E.; Rusconi, C.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Cai, X. Z.; Cao, X. G.; Fang, D. Q.; Li, Y. L.; Ma, Y. G.; Tian, W. D.; Wang, H. W.; Zhang, G. Q.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Caminata, A.; Copello, S.; Di Domizio, S.; Fernandes, G.; Pallavicini, M.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Cappelli, L.; Pagliarone, C. E.] Univ Cassino & Lazio Meridionale, Dipartimento Ingn Civile & Meccan, I-03043 Cassino, Italy. [Casali, N.; Di Vacri, M. L.; Santone, D.] Univ Aquila, Dipartimento Sci Fis & Chim, I-67100 Laquila, Italy. [Cushman, J. S.; Han, K.; Heeger, K. M.; Lim, K. E.; Maruyama, R. H.; Wise, T.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Dally, A.; Ejzak, L.; Wielgus, L.; Wise, T.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Dell'Oro, S.] Ist Nazl Fis Nucl, Gran Sasso Sci Inst, I-67100 Laquila, Italy. [Franceschi, M. A.; Ligi, C.; Napolitano, T.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Rome, Italy. [Giuliani, A.; Tenconi, M.] Ctr Spectrometrie Nucl & Spectrometrie Masse, F-91405 Orsay, France. [Gutierrez, T. D.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Hansen, E.] MIT, Cambridge, MA 02139 USA. [Hickerson, K. P.; Huang, H. Z.; Liu, X.; Trentalange, S.; Winslow, L. A.; Zhu, B. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Kadel, R.; Kolomensky, Yu G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Martinez, M.] Univ Zaragoza, Lab Fis Nucl & Astroparticulas, E-50009 Zaragoza, Spain. [Moggi, N.] Univ Bologna, Alma Mater Studiorum, Dipartimento Sci Qualita Vita, I-47921 Bologna, Italy. [Nones, C.] CEA Saclay, Serv Phys Particules, F-91191 Gif Sur Yvette, France. [Norman, E. B.; Sangiorgio, S.; Scielzo, N. D.; Wang, B. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Norman, E. B.; Wang, B. S.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Taffarello, L.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Ventura, G.] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy. [Ventura, G.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Woodcraft, A.] Univ Edinburgh, Inst Astron, SUPA, Edinburgh EH9 3HJ, Midlothian, Scotland. [Zucchelli, S.] Univ Bologna, Alma Mater Studiorum, Dipartimento Fis & Astron, I-40127 Bologna, Italy. RP Canonica, L (reprint author), Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. RI Bellini, Fabio/D-1055-2009; capelli, silvia/G-5168-2012; Casali, Nicola/C-9475-2017; Chiesa, Davide/H-7240-2014; Vignati, Marco/H-1684-2013; Giachero, Andrea/I-1081-2013; Ferri, Elena/L-8531-2014; Ligi, Carlo/M-4007-2016; Martinez, Maria/K-4827-2012; Gironi, Luca/P-2860-2016; Pattavina, Luca/I-7498-2015 OI Clemenza, Massimiliano/0000-0002-8064-8936; pavan, maura/0000-0002-9723-7834; Gotti, Claudio/0000-0003-2501-9608; Pessina, Gianluigi Ezio/0000-0003-3700-9757; Pozzi, Stefano/0000-0003-2986-1990; Bellini, Fabio/0000-0002-2936-660X; capelli, silvia/0000-0002-0300-2752; Casali, Nicola/0000-0003-3669-8247; Canonica, Lucia/0000-0001-8734-206X; Chiesa, Davide/0000-0003-1978-1727; Vignati, Marco/0000-0002-8945-1128; Giachero, Andrea/0000-0003-0493-695X; Ferri, Elena/0000-0003-1425-3669; Ligi, Carlo/0000-0001-7943-7704; Martinez, Maria/0000-0002-9043-4691; Gironi, Luca/0000-0003-2019-0967; Pattavina, Luca/0000-0003-4192-849X NR 12 TC 0 Z9 0 U1 2 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2405-6014 EI 1873-3832 J9 NUCL PART PHYS P JI Nucl. Part. Phys. Proc. PD AUG-SEP PY 2015 VL 265 BP 73 EP 76 DI 10.1016/j.nuclphysbps.2015.06.020 PG 4 GA CQ9QT UT WOS:000360950700020 ER PT J AU Descamps, F AF Descamps, F. CA SNO Collaboration TI Neutrino Physics with SNO SO NUCLEAR AND PARTICLE PHYSICS PROCEEDINGS LA English DT Proceedings Paper CT 8th Neutrino Oscillation Workshop (NOW) CY SEP 07-13, 2014 CL Conca Specchiulla, ITALY SP Ist Nazl Fisica Nucleare, Dipartimento Interateneo Fisica Michelangelo Merlin, Ist Nazl Fisica Nucleare, Dipartimento Matematica & Fisica Ennio Giorgi, Univ Bari, Univ Salento, Ist Nazl Fisica Nucleare, Italian Ministero Istruzione, Univ Ric DE SNO; neutrinoless double beta decay; neutrino ID GEO-NEUTRINOS AB SNO+ is the successor to the Sudbury Neutrino Observatory (SNO) for which SNO's heavy water target is replaced by approximately 780 T of liquid scintillator (LAB). The combination of the 2 km underground location, the use of ultra-clean materials and the high light-yield of the liquid scintillator means that a low background level and a low energy threshold can be achieved. This creates a new multipurpose neutrino detector with the potential to address a diverse set of physics goals, including the detection of reactor, solar, geo- and supernova neutrinos. The main physics goal of SNO+ is the search for neutrinoless double beta decay. By loading the liquid scintillator with 0.3% of natural Tellurium, resulting in about 800 kg of Te-130 (isotopic abundance is slightly over 34%), a competitive sensitivity to the effective neutrino mass can be reached. C1 [Descamps, F.; SNO Collaboration] Lawrence Berkeley Natl Lab, Berkeley, CA 94730 USA. RP Descamps, F (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94730 USA. EM fbdescamps@lbl.gov NR 9 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2405-6014 EI 1873-3832 J9 NUCL PART PHYS P JI Nucl. Part. Phys. Proc. PD AUG-SEP PY 2015 VL 265 BP 143 EP 145 DI 10.1016/j.nuclphysbps.2015.06.037 PG 3 GA CQ9QT UT WOS:000360950700037 ER PT J AU Worcester, E AF Worcester, Elizabeth TI Precision Measurements of Long-Baseline Neutrino Oscillation at LBNF SO NUCLEAR AND PARTICLE PHYSICS PROCEEDINGS LA English DT Proceedings Paper CT 8th Neutrino Oscillation Workshop (NOW) CY SEP 07-13, 2014 CL Conca Specchiulla, ITALY SP Ist Nazl Fisica Nucleare, Dipartimento Interateneo Fisica Michelangelo Merlin, Ist Nazl Fisica Nucleare, Dipartimento Matematica & Fisica Ennio Giorgi, Univ Bari, Univ Salento, Ist Nazl Fisica Nucleare, Italian Ministero Istruzione, Univ Ric DE neutrino oscillation AB In a long-baseline neutrino oscillation experiment, the primary physics objectives are to determine the neutrino mass hierarchy, to determine the octant of the neutrino mixing angle 023, to search for CP violation in neutrino oscillation, and to precisely measure the size of any CP-violating effect that is discovered. This presentation provides a brief introduction to these measurements and reports on efforts to optimize the design of a long-baseline neutrino oscillation experiment, the status of LBNE, and the transition to an international collaboration at LBNF. C1 Brookhaven Natl Lab, Upton, NY 11973 USA. RP Worcester, E (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM etw@bnl.gov NR 11 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2405-6014 EI 1873-3832 J9 NUCL PART PHYS P JI Nucl. Part. Phys. Proc. PD AUG-SEP PY 2015 VL 265 BP 189 EP 191 DI 10.1016/j.nuclphysbps.2015.06.048 PG 3 GA CQ9QT UT WOS:000360950700048 ER PT J AU Dwyer, DA Ludhova, L AF Dwyer, D. A. Ludhova, L. TI Oscillations at low energies SO NUCLEAR AND PARTICLE PHYSICS PROCEEDINGS LA English DT Proceedings Paper CT 8th Neutrino Oscillation Workshop (NOW) CY SEP 07-13, 2014 CL Conca Specchiulla, ITALY SP Ist Nazl Fisica Nucleare, Dipartimento Interateneo Fisica Michelangelo Merlin, Ist Nazl Fisica Nucleare, Dipartimento Matematica & Fisica Ennio Giorgi, Univ Bari, Univ Salento, Ist Nazl Fisica Nucleare, Italian Ministero Istruzione, Univ Ric DE neutrino oscillation; neutrino mass hierarchy; sterile neutrinos; reactor antineutrinos; solar neutrinos; supernova neutrinos; geoneutrinos ID NEUTRON FISSION-PRODUCTS; GEO-NEUTRINOS; BOREXINO; SPECTRA; PU-239 AB A concise summary of the "Oscillation at low energies" parallel session at the 2014 Neutrino Oscillation Workshop is provided. Plans to use man-made neutrinos and antineutrinos to determine the neutrino mass hierarchy, search for sterile neutrinos, and to observe coherent neutrino-nucleus scattering were discussed. Potential measurements of solar neutrinos, supernova neutrinos, and geoneutrinos are also summarized. C1 [Dwyer, D. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ludhova, L.] Ist Nazl Fis Nucl, I-20133 Milan, Italy. RP Dwyer, DA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM dadwyer@lbl.gov; ludhova@gmail.com NR 56 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2405-6014 EI 1873-3832 J9 NUCL PART PHYS P JI Nucl. Part. Phys. Proc. PD AUG-SEP PY 2015 VL 265 BP 339 EP 345 DI 10.1016/j.nuclphysbps.2015.06.086 PG 7 GA CQ9QT UT WOS:000360950700086 ER PT J AU Lu, Y Ozcan, S AF Lu, Yuan Ozcan, Soydan TI Green nanomaterials: On track for a sustainable future SO NANO TODAY LA English DT Article DE Green nanotechnology; Natural sources; Environmentally friendly green synthesis ID METAL NANOPARTICLES; GOLD NANOPARTICLES; CHEMISTRY; GRAPHENE; AGENTS; SILVER; SIZE AB Nanotechnology is one of the most significant scientific and industrial breakthroughs of the twenty-first century. With applications that cross scientific boundaries from electronics to medicine, to advanced manufacturing, to cosmetics nanotechnology has the potential to dramatically change lifestyles, jobs, and whole economies [1]. However, many of the materials and processes currently used not only are dependent on nonrenewable resources but also create hazardous wastes. The combination of green chemistry techniques with nanotechnology applications has thus become a key component of the nanotechnology future. The use of natural ingredients to synthesize nanomaterials and design environmentally benign synthetic processes has been extensively explored. While many of these so-called "green nanotechnologies" are now finding their way from the laboratory to commercial application, green nanotechnology still faces significant challenges. This article presents the recent advances and challenges in green nanotechnology, and suggests ways to improve the commercial readiness of these technologies. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lu, Yuan; Ozcan, Soydan] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Ozcan, S (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM ozcans@ornl.gov OI Ozcan, Soydan/0000-0002-3825-4589 FU U.S. Department of Energy [DE-AC05-00OR22725] FX This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 30 TC 4 Z9 4 U1 2 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1748-0132 EI 1878-044X J9 NANO TODAY JI Nano Today PD AUG PY 2015 VL 10 IS 4 BP 417 EP 420 DI 10.1016/j.nantod.2015.04.010 PG 4 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CY9ZX UT WOS:000366766000005 ER PT J AU Leheny, RL Rogers, MC Chen, K Narayanan, S Harden, JL AF Leheny, Robert L. Rogers, Michael C. Chen, Kui Narayanan, Suresh Harden, James L. TI Rheo-XPCS SO CURRENT OPINION IN COLLOID & INTERFACE SCIENCE LA English DT Review DE X-ray photon correlation spectroscopy; Rheology; Large amplitude oscillatory shear; Heterodyne methods; Yielding ID PHOTON-CORRELATION SPECTROSCOPY; X-RAY; LIGHT-SCATTERING; DYNAMICS; FLOW; HOMODYNE; SHEAR; REARRANGEMENTS; MICRORHEOLOGY; NANOPARTICLES AB We review recent efforts and discuss future prospects in research employing X-ray photon correlation spectroscopy (XPCS) to interrogate the nanometer-scale structural dynamics of soft materials undergoing in situ mechanical deformation and flow. Examples of such rheo-XPCS experiments include those incorporating conventional homogeneous shear deformation, including notably large amplitude oscillatory shear (LAOS), as well as other modes of flow and deformation, such as tensile strain and flow within microfluidic environments. Particular attention is given to opportunities in such studies to reveal the structural dynamics associated with nonlinear rheological behavior such as yielding. We also review recent related work employing XPCS as a microrheological tool by tracking nanoparticle mobility within complex fluids. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Leheny, Robert L.; Chen, Kui] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Rogers, Michael C.; Harden, James L.] Univ Ottawa, Dept Phys, Ottawa, ON K1N 6N5, Canada. [Narayanan, Suresh] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Leheny, RL (reprint author), Johns Hopkins Univ, Dept Phys & Astron, 3400 N Charles St, Baltimore, MD 21218 USA. EM leheny@jhu.edu; jharden@uottawa.ca FU NSF [CBET-1336166]; NSERC discovery [RGPIN-327200-2012, RGPIN-04478-2014]; RTI [EQPEQ/ 390318-2010]; DOE BES [DE-AC02-06CH11357] FX We thank W. Burghardt, L. Lurio, S. Ramakrishnan, A. Sandy, and M. Sutton for helpful discussions. We also acknowledge support from the NSF (CBET-1336166), and the NSERC discovery (RGPIN-327200-2012 and RGPIN-04478-2014) and RTI (EQPEQ/ 390318-2010) programs. RL also thanks the X-ray Sciences Division Visitor Program at Argonne National Laboratory. Use of the APS was supported by DOE BES under contract no. DE-AC02-06CH11357. NR 58 TC 3 Z9 3 U1 3 U2 23 PU ELSEVIER SCIENCE LONDON PI LONDON PA 84 THEOBALDS RD, LONDON WC1X 8RR, ENGLAND SN 1359-0294 EI 1879-0399 J9 CURR OPIN COLLOID IN JI Curr. Opin. Colloid Interface Sci. PD AUG PY 2015 VL 20 IS 4 BP 261 EP 271 DI 10.1016/j.cocis.2015.10.001 PG 11 WC Chemistry, Physical SC Chemistry GA CY0FB UT WOS:000366080700007 ER PT J AU Glanville, J D'Angelo, S Khan, TA Reddy, ST Naranjo, L Ferrara, F Bradbury, ARM AF Glanville, J. D'Angelo, S. Khan, T. A. Reddy, S. T. Naranjo, L. Ferrara, F. Bradbury, A. R. M. TI Deep sequencing in library selection projects: what insight does it bring? SO CURRENT OPINION IN STRUCTURAL BIOLOGY LA English DT Article ID ANTIBODY VARIABLE DOMAINS; ANKYRIN REPEAT PROTEIN; PHAGE DISPLAY; CRYSTAL-STRUCTURE; V-H; MONOCLONAL-ANTIBODIES; SYNTHETIC ANTIBODIES; THERMAL-STABILITY; CLONAL SELECTION; SURFACE DISPLAY AB High throughput sequencing is poised to change all aspects of the way antibodies and other binders are discovered and engineered. Millions of available sequence reads provide an unprecedented sampling depth able to guide the design and construction of effective, high quality naive libraries containing tens of billions of unique molecules. Furthermore, during selections, high throughput sequencing enables quantitative tracing of enriched clones and position-specific guidance to amino acid variation under positive selection during antibody engineering. Successful application of the technologies relies on specific PCR reagent design, correct sequencing platform selection, and effective use of computational tools and statistical measures to remove error, identify antibodies, estimate diversity, and extract signatures of selection from the clone down to individual structural positions. Here we review these considerations and discuss some of the remaining challenges to the widespread adoption of the technology. C1 [Glanville, J.] Stanford Univ, Program Computat & Syst Immunol, Inst Immun Transplantat & Infect, Sch Med, Stanford, CA 94305 USA. [D'Angelo, S.; Ferrara, F.] Univ New Mexico, Sch Med, Ctr Comprehens Canc, Albuquerque, NM 87131 USA. [D'Angelo, S.; Ferrara, F.] Univ New Mexico, Sch Med, Div Mol Med, Albuquerque, NM 87131 USA. [Khan, T. A.; Reddy, S. T.] Swiss Fed Inst Technol, Dept Biosyst Sci & Engn, Basel, Switzerland. [Naranjo, L.; Bradbury, A. R. M.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Bradbury, ARM (reprint author), Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. EM amb@lanl.gov RI Reddy, Sai/B-4190-2012; OI Reddy, Sai/0000-0002-9177-0857; Bradbury, Andrew/0000-0002-5567-8172 FU NIH U54 Grant 'Technology Development for New Affinity Reagents Against the Human Proteome (U54) [RFA-RM-10-018, 1-U54-DK093500-01]; Swiss National Science Foundation SystemsX.ch - AntibodyX RTD project grant; Whitaker International Program Scholarship FX This work was supported by: NIH U54 Grant 'Technology Development for New Affinity Reagents Against the Human Proteome (U54) RFA-RM-10-018,' grant number 1-U54-DK093500-01 (to AB); the Swiss National Science Foundation SystemsX.ch - AntibodyX RTD project grant (to STR), and a Whitaker International Program Scholarship (to TAK). NR 92 TC 7 Z9 7 U1 2 U2 10 PU CURRENT BIOLOGY LTD PI LONDON PA 84 THEOBALDS RD, LONDON WC1X 8RR, ENGLAND SN 0959-440X EI 1879-033X J9 CURR OPIN STRUC BIOL JI Curr. Opin. Struct. Biol. PD AUG PY 2015 VL 33 BP 146 EP 160 DI 10.1016/j.sbi.2015.09.001 PG 15 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CX0BR UT WOS:000365362400017 PM 26451649 ER PT J AU Cao, GH Jian, GY Liu, N Zhang, WH Russell, AM Gerthsen, D AF Cao, G. H. Jian, G. Y. Liu, N. Zhang, W. H. Russell, A. M. Gerthsen, D. TI Microstructure and mechanical properties of an ultrafine Ti-Si-Nb alloy SO MATERIALS CHEMISTRY AND PHYSICS LA English DT Article DE Alloys; Electron microscopy; Mechanical testing; Ductility; Microstructure ID TENSILE DUCTILITY; HIGH-STRENGTH; ENHANCED PLASTICITY; METALS; INTERMETALLICS; NANOCRYSTALLINE; BEHAVIOR; IMPROVE; COPPER; TI5SI3 AB Nb-modified ultrafine Ti-Si eutectic alloy was made by cold crucible levitation melting, tested in compression at room temperature, and characterized by electron microscopy. Compression tests of (Ti86.5Si3.5)(97)Nb-3 specimens measured an ultimate compressive strength of 1180 MPa and a compressive plastic strain of 12%, both of which are higher than in eutectic Ti86.5Si13.5 alloy. Electron microscopy showed that the Ti Si Nb alloy had a bimodal microstructure with micrometer-scale primary alpha-Ti dendrites distributed in an ultrafine eutectic (alpha-Ti Ti5Si3) matrix. The enhanced ductility is attributed to the morphology of the phase constituents and to the larger lattice mismatches between alpha-Ti and Ti5Si3 phases caused by the NU addition. The crystallographic orientation relationship of Ti5Si3 with alpha-Ti is (1 (1) over bar 00)[(1) over bar(1) over bar 26] Ti5Si3(1) over bar1 (01T1)[5143] alpha-Ti. (C) 2015 Elsevier B.V. All rights reserved. C1 [Cao, G. H.; Jian, G. Y.; Liu, N.] Shanghai Univ, Dept Mat Engn, Shanghai 200072, Peoples R China. [Cao, G. H.; Jian, G. Y.; Liu, N.] Shanghai Univ, State Key Lab Adv Special Steels, Shanghai 200072, Peoples R China. [Zhang, W. H.] Changzhou Technician Coll Jiangsu Prov, Dept Mech Engn, Changzhou 213032, Peoples R China. [Russell, A. M.] Iowa State Univ, Dept Mat Sci & Engn, US DOE, Div Mat Sci & Engn,Ames Lab, Ames, IA 50011 USA. [Gerthsen, D.] Karlsruher Inst Technol, Lab Elektronenmikroskopie, D-76128 Karlsruhe, Germany. RP Cao, GH (reprint author), Shanghai Univ, Dept Mat Engn, 149 Yanchang Rd, Shanghai 200072, Peoples R China. EM ghcao@shu.edu.cn RI Gerthsen, Dagmar/I-4448-2012; OI Russell, Alan/0000-0001-5264-0104 FU National Natural Science Foundation of China (NSFC) [51271107]; Shanghai Municipal Education Commission [13ZZ077]; Network for Functional Nanostructures - Baden-Wurttemberg Foundation; US Department of Energy [DE-AC02-07CH11358] FX This work was supported by the National Natural Science Foundation of China (NSFC) under Grant no. 51271107, the Innovation Program of Shanghai Municipal Education Commission under Grant no. 13ZZ077, and the Network for Functional Nanostructures funded by the Baden-Wurttemberg Foundation. The Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 29 TC 0 Z9 0 U1 6 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0254-0584 EI 1879-3312 J9 MATER CHEM PHYS JI Mater. Chem. Phys. PD AUG 1 PY 2015 VL 163 BP 512 EP 517 DI 10.1016/j.matchemphys.2015.08.007 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA CX0BI UT WOS:000365361500061 ER PT J AU Harris, BB Norton, TM Nibbelink, NP Tuberville, TD AF Harris, Bess B. Norton, Terry M. Nibbelink, Nathan P. Tuberville, Tracey D. TI OVERWINTERING ECOLOGY OF JUVENILE GOPHER TORTOISES (GOPHERUS POLYPHEMUS) SO HERPETOLOGICAL CONSERVATION AND BIOLOGY LA English DT Article DE activity; dormancy; Georgia; reptile; temperature ID DELAYED EMERGENCE; HATCHLING TURTLES; DESERT TORTOISES; HOME RANGE; HIBERNATION; AGASSIZII; TEMPERATURES; POPULATION; PHYSIOLOGY; MOVEMENT AB The Gopher Tortoise (Gopherus polyphemus) is a large terrestrial turtle that excavates and occupies extensive burrows, which protect individuals from predators and temperature extremes. Individuals can thermoregulate behaviorally by adjusting their position inside the burrow and through surface activity, even in winter when they are thought to be relatively inactive. Much of what is known about the overwintering behavior of Gopher Tortoises is based on adults; however, the ecology of juveniles may differ due to their smaller body size and higher surface area to volume ratio. We investigated the overwintering ecology of 11 juvenile Gopher Tortoises on St. Catherines Island, Georgia using externally attached temperature loggers. Temperatures experienced by tortoises were compared to burrow and surface air temperatures collected at the same site, allowing us to infer surface activity of individuals. We examined the onset, termination, and duration of overwintering and occurrences of juvenile surface activity during the overwinter period. Tortoises initiated overwintering over a 48-d period (median date of 14 November) and terminated overwintering over a 32-d period (median date of 8 April). Mean overwintering duration was 130 +/- 7 d (1 SE). Individuals emerged on 2-22 d during the 2012-2013 winter. Mean temperature experienced by overwintering tortoises was 17.9 +/- 0.02 degrees C (range 11.5-38.5 degrees C) and the minimum surface air temperature when a juvenile tortoise emerged from its burrow to bask was 15.8 degrees C. Timing of overwintering in juvenile Gopher Tortoises is similar to that reported for adult tortoises from similar latitudes. However, juveniles are active more frequently on the surface during the winter and emerge from burrows at lower air temperatures than has been reported for adults. C1 [Harris, Bess B.; Tuberville, Tracey D.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Harris, Bess B.; Nibbelink, Nathan P.] Univ Georgia, Daniel B Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. [Norton, Terry M.] Jekyll Isl Author, Georgia Sea Turtle Ctr, Jekyll Isl, GA 31527 USA. [Norton, Terry M.] St Catherines Isl Fdn, Midway, GA 31320 USA. RP Harris, BB (reprint author), Florida Fish & Wildlife Conservat Commiss, Lovett E Williams Jr Wildlife Res Lab, 1105 SW Williston Rd, Gainesville, FL 32641 USA. EM bess.harris@myfwc.com FU St. Catherines Island Foundation; TERN: Friends of Georgia's Nongame Wildlife; Riverbanks Zoo and Garden Conservation Support Fund; Department of Energy [DE-FC09-07SR22506] FX We extend our gratitude to Veronica Greco and the St. Catherines Island interns that assisted in deploying and collecting temperature loggers and in processing turtles. We thank Jack Tuberville for constructing environmental stations. We are grateful for the assistance Elizabeth Hunter provided in capturing tortoises prior to winter. We are especially appreciative of the logistical support provided by Royce Hayes and the St. Catherines Island Foundation staff throughout the study. Jessica McGuire, Brett DeGregorio, Brian Crawford, and Elizabeth Schlimm provided valuable feedback during the preparation of this manuscript. Funding was provided by grants from the St. Catherines Island Foundation, TERN: Friends of Georgia's Nongame Wildlife, and Riverbanks Zoo and Garden Conservation Support Fund. Data analysis and manuscript preparation was supported by the Department of Energy under Award Number DE-FC09-07SR22506 from Department of Energy to the University of Georgia Research Foundation. All research was conducted in accordance with Georgia scientific collecting permits 29-WBH-12-166 and 29-WJH-13-83 and using procedures approved by University of Georgia's Institutional Animal Care and Use Committee under Animal Use Proposal #A2011 05-20-Y1. NR 36 TC 1 Z9 1 U1 10 U2 22 PU HERPETOLOGICAL CONSERVATION & BIOLOGY PI CORVALLIS PA C/O R BRUCE BURY, USGS FOREST & RANGELAND, CORVALLIS, OR 00000 USA SN 2151-0733 EI 1931-7603 J9 HERPETOL CONSERV BIO JI Herpetol. Conserv. Biol. PD AUG PY 2015 VL 10 IS 2 BP 645 EP 653 PG 9 WC Zoology SC Zoology GA CW6CU UT WOS:000365085900009 ER PT J AU Anovitz, LM Cole, DR Sheets, JM Swift, A Elston, HW Welch, S Chipera, SJ Littrell, KC Mildner, DFR Wasbrough, MJ AF Anovitz, Lawrence Michael Cole, David Robert Sheets, Julia Meyer Swift, Alexander Elston, Harold William Welch, Susan Chipera, Steve James Littrell, Kenneth Charles Mildner, David Francis Raymond Wasbrough, Matthew John TI Effects of maturation on multiscale (nanometer to millimeter) porosity in the Eagle Ford Shale SO Interpretation-A Journal of Subsurface Characterization LA English DT Article ID ANGLE NEUTRON-SCATTERING; MICROSTRUCTURE; SANDSTONE; CRYSTALS; FLUIDS; PORES; ROCKS; EARTH AB Porosity and permeability are key variables that link the thermal-hydrologic, geomechanical, and geochemical behavior in rock systems and are thus important input parameters for transport models. Neutron scattering studies indicate that the scales of pore sizes in rocks extend over many orders of magnitude from nanometer-sized pores with huge amounts of total surface area to large open fracture systems (multiscale porosity). However, despite considerable efforts combining conventional petrophysics, neutron scattering, and electron microscopy, the quantitative nature of this porosity in tight gas shales, especially at smaller scales and over larger rock volumes, remains largely unknown. Nor is it well understood how pore networks are affected by regional variation in rock composition and properties, thermal changes across the oil window (maturity), and, most critically, hydraulic fracturing. To improve this understanding, we have used a combination of small-and ultrasmall-angle neutron scattering (U)SANS with scanning electron microscope (SEM)/backscattered electron imaging to analyze the pore structure of clay-and carbonate-rich samples of the Eagle Ford Shale. This formation is hydrocarbon rich, straddles the oil window, and is one of the most actively drilled oil and gas targets in the United States. Several important trends in the Eagle Ford rock pore structure have been identified using our approach. The (U) SANS results reflected the connected (effective) and unconnected porosity, as well as the volume occupied by organic material. The latter could be separated using total organic carbon data and, at all maturities, constituted a significant fraction of the apparent porosity. At lower maturities, the pore structure was strongly anisotropic. However, this decreased with increasing maturity, eventually disappearing entirely for carbonate-rich samples. In clay-and carbonate-rich samples, a significant reduction in total porosity occurred at (U) SANS scales, much of it during initial increases in maturity. This apparently contradicted SEM observations that showed increases in intraorganic porosity with increasing maturity. Organic-rich shales are, however, a very complex material from the point of view of scattering studies, and a more detailed analysis is needed to better understand these observations. C1 [Anovitz, Lawrence Michael] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Cole, David Robert; Sheets, Julia Meyer; Swift, Alexander; Elston, Harold William; Welch, Susan] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. [Chipera, Steve James] Chesapeake Energy Corp, Oklahoma City, OK USA. [Littrell, Kenneth Charles] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN USA. [Mildner, David Francis Raymond; Wasbrough, Matthew John] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. RP Anovitz, LM (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM anovitzlm@ornl.gov; sheets.2@osu.edu; swift.63@osu.edu; elston.22@osu.edu; welch.318@osu.edu; steve.chipera@chk.com; littrellkc@ornl.gov; david.mildner@nist.gov; matthew.wasbrough@nist.gov RI Wasbrough, Matthew/H-2252-2013; Anovitz, Lawrence/P-3144-2016; Littrell, Kenneth/D-2106-2013 OI Wasbrough, Matthew/0000-0002-3225-7447; Anovitz, Lawrence/0000-0002-2609-8750; Littrell, Kenneth/0000-0003-2308-8618 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences through the Energy Frontier Research Center - Nanoscale Control of Geologic CO2 (neutron scattering); National Science Foundation (NSF) Dimensions Environmental Biology program [DEB-1342701]; NSF [DMR-0944772] FX The work of L. M. Anovitz was supported by research sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. D. R. Cole and A. Swift were funded by the Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences through the Energy Frontier Research Center - Nanoscale Control of Geologic CO2 (neutron scattering). The microscopy assessment (J. Sheets, S. Welch, H. Elston) was supported from the National Science Foundation (NSF) Dimensions Environmental Biology program through grant no. DEB-1342701. The samples analyzed were kindly provided by Chesapeake Energy. We acknowledge the support of the National Institute of Standards and Technology, Center for Neutron Research, the U.S. Department of Commerce, and the HFIR at ORNL in providing the research neutron facilities used in this work. This work used facilities supported in part by the NSF under agreement no. DMR-0944772. Certain commercial equipment, instruments, materials, and software are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the National Institute of Standards and Technology, the Department of Energy, or ORNL, nor does it imply that the materials or equipment identified are necessarily the best available for the purpose. NR 46 TC 1 Z9 1 U1 6 U2 27 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 2324-8858 EI 2324-8866 J9 INTERPRETATION-J SUB JI Interpretation PD AUG PY 2015 VL 3 IS 3 BP SU59 EP SU70 DI 10.1190/INT-2014-0280.1 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CV6EG UT WOS:000364362900023 ER PT J AU Schuster, G Shemeta, J Paulsson, B Xiao, X Hornby, B Karrenbach, M Fehler, M Hardage, B Huang, LJ Yu, G Yu, JH AF Schuster, Gerard Shemeta, Julie Paulsson, Bjorn Xiao, Xiang Hornby, Brian Karrenbach, Martin Fehler, Mike Hardage, Bob Huang, Lianjie Yu, Grace Yu, Jianhua TI Introduction to special section: Recent advances with well whisperers SO Interpretation-A Journal of Subsurface Characterization LA English DT Editorial Material C1 [Schuster, Gerard] KAUST, Thuwal, Saudi Arabia. [Shemeta, Julie] MEQ GEO Inc, Denver, CO USA. [Paulsson, Bjorn] Paulsson Geo, Van Nuys, CA USA. [Xiao, Xiang] TGS, Houston, TX USA. [Hornby, Brian; Yu, Jianhua] BP, Houston, TX USA. [Karrenbach, Martin] Optasense, Houston, TX USA. [Fehler, Mike] MIT, Cambridge, MA 02139 USA. [Hardage, Bob] UT Austin, Austin, TX USA. [Huang, Lianjie] LANL, Los Alamos, NM USA. [Yu, Grace] Anadarko, Houston, TX USA. RP Schuster, G (reprint author), KAUST, Thuwal, Saudi Arabia. EM gerard.schuster@kaust.edu.sa; julie@meqgeo.com; bjorn.paulsson@paulsson.com; xiang.xiao.utah@gmail.com; brian_hornby@yahoo.com; martin.karrenbach@optasense.com; fehler@mit.edu; bob.hardage@beg.utexas.edu; ljh@lanl.gov; grace.yu@anadarko.com; jianhua.yu@bp.com NR 0 TC 0 Z9 0 U1 0 U2 2 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 2324-8858 EI 2324-8866 J9 INTERPRETATION-J SUB JI Interpretation PD AUG PY 2015 VL 3 IS 3 BP SWI EP SWI DI 10.1190/INT2015-0701-SPSEINTRO.1 PG 1 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CV6EG UT WOS:000364362900032 ER PT J AU Zhang, R Daley, TM Vasco, D AF Zhang, Rui Daley, Thomas M. Vasco, Donald TI Improving thin-bed resolution: Application of a sparse-layer inversion on 3D seismic observations from the In Salah carbon dioxide storage project SO Interpretation-A Journal of Subsurface Characterization LA English DT Article ID REFLECTIVITY INVERSION; ALGERIA AB The In Salah carbon dioxide storage project in Algeria has injected more than 3 million tons of carbon dioxide into a thin water-filled tight-sand formation. Interferometric synthetic aperture radar range change data revealed a double-lobe pattern of surface uplift, which has been interpreted as the existence of a subvertical fracture, or damage, zone. The reflection seismic data found a subtle linear push-down feature located along the depression between the two lobes thought to be due to the injection of carbon dioxide. Understanding of the CO2 distribution within the injection interval and migration within the fracture zone requires a precise subsurface layer model from the injection interval to above the top of the fracture zone. To improve the resolution of the existing seismic model, we applied a sparse-layer seismic inversion, with basis pursuit decomposition on the 3D seismic data between 1.0 and 1.5 s. The inversion results, including reflection coefficients and band-limited impedance cubes, provided improved subsurface imaging for two key layers (seismic horizons) above the injection interval. These horizons could be used as part of a more detailed earth model to study the CO2 storage at In Salah. C1 [Zhang, Rui; Daley, Thomas M.; Vasco, Donald] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zhang, R (reprint author), Univ SW Louisiana, Lafayette, LA 70504 USA. EM rxz1961@louisiana.edu; tmdaley@lbl.gov; dwvasco@lbl.gov RI Daley, Thomas/G-3274-2015; Vasco, Donald/I-3167-2016; Vasco, Donald/G-3696-2015 OI Daley, Thomas/0000-0001-9445-0843; Vasco, Donald/0000-0003-1210-8628; Vasco, Donald/0000-0003-1210-8628 FU BP; GEOSEQ project for the Assistant Secretary for Fossil Energy, Office of Coal and Power Systems through the National Energy Technology Laboratory of the U.S. Department of Energy [DE-AC02-05CH11231]; Statoil; Sonatrach FX This work was supported by the InSalah Joint Industry Project, a partnership of BP, Statoil, and Sonatrach. This work was partially supported by the GEOSEQ project for the Assistant Secretary for Fossil Energy, Office of Coal and Power Systems through the National Energy Technology Laboratory of the U.S. Department of Energy, under contract no. DE-AC02-05CH11231. Some of the seismic data processing in this report was performed using the VISTA software package provided by GEDCO, now a Schlumberger company. NR 11 TC 0 Z9 0 U1 0 U2 3 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 2324-8858 EI 2324-8866 J9 INTERPRETATION-J SUB JI Interpretation PD AUG PY 2015 VL 3 IS 3 BP SS65 EP SS71 DI 10.1190/INT-2014-0204.1 PG 7 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CV6EG UT WOS:000364362900009 ER PT J AU Aab, A Abreu, P Aglietta, M Ahn, EJ Al Samarai, I Albuquerque, IFM Allekotte, I Allison, P Almela, A Castillo, JA Alvarez-Muniz, J Batista, RA Ambrosio, M Aminaei, A Anchordoqui, L Andringa, S Aramo, C Aranda, VM Arqueros, F Arsene, N Asorey, H Assis, P Aublin, J Ave, M Avenier, M Avila, G Awal, N Badescu, AM Barber, KB Bauml, J Baus, C Beatty, JJ Becker, KH Bellido, JA Berat, C Bertaina, ME Bertou, X Biermann, PL Billoir, P Blaess, SG Blanco, A Blanco, M Bleve, C Bluemer, H Bohacova, M Boncioli, D Bonifazi, C Borodai, N Brack, J Brancus, I Bridgeman, A Brogueira, P Brown, WC Buchholz, P Bueno, A Buitink, S Buscemi, M Caballero-Mora, KS Caccianiga, B Caccianiga, L Candusso, M Caramete, L Caruso, R Castellina, A Cataldi, G Cazon, L Cester, R Chavez, AG Chiavassa, A Chinellato, JA Chudoba, J Cilmo, M Clay, RW Cocciolo, G Colalillo, R Coleman, A Collica, L Coluccia, MR Conceicao, R Contreras, F Cooper, MJ Cordier, A Coutu, S Covault, CE Cronin, J Dallier, R Daniel, B Dasso, S Daumiller, K Dawson, BR de Almeida, RM de Jong, SJ De Mauro, G Neto, JRTD De Mitri, I de Oliveira, J de Souza, V del Pera, L Deligny, O Dembinski, H Dhital, N Di Giulio, C Di Matteo, A Diaz, JC Castro, MLD Diogo, F Dobrigkeit, C Docters, W D'Olivo, JC Dorofeev, A Hasankiadeh, QD Dova, MT Ebr, J Engel, R Erdmann, M Erfani, M Escobar, CO Espadanal, J Etchegoyen, A Falcke, H Fang, K Farrar, G Fauth, AC Fazzini, N Ferguson, AP Fernandes, M Fick, B Figueira, JM Filevich, A Filipcic, A Fox, BD Fratu, O Freire, MM Fuchs, B Fujii, T Garcia, B Garcia-Pinto, D Gate, F Gemmeke, H Gherghel-Lascu, A Ghia, PL Giaccari, U Giammarchi, M Giller, M Glas, D Glaser, C Glass, H Golup, G Berisso, MG Vitale, PFG Gonzalez, N Gookin, B Gordon, J Gorgi, A Gorham, P Gouffon, P Griffith, N Grillo, AF Grubb, TD Guarino, F Guedes, GP Hampel, MR Hansen, P Harari, D Harrison, TA Hartmann, S Harton, JL Haungs, A Hebbeker, T Heck, D Heimann, P Herve, AE Hill, GC Hojvat, C Hollon, N Holt, E Homola, P Horandel, JR Horvath, P Hrabovsky, M Huber, D Huege, T Insolia, A Isar, PG Jandt, I Jansen, S Jarne, C Johnsen, JA Josebachuili, M Kaapaa, A Kambeitz, O Kampert, KH Kasper, P Katkov, I Kegl, B Keilhauer, B Keivani, A Kemp, E Kieckhafer, RM Klages, HO Kleifges, M Kleinfeller, J Krause, R Krohm, N Kromer, O Kuempe, D Kunka, N LaHurd, D Latronico, L Lauer, R Lauscher, M Lautridou, P Le Coz, S Lebrun, D Lebrun, P de Oliveira, MAL Letessier-Selvon, A Lhenry-Yvon, I Link, K Lopes, L Lopez, R Casado, AL Louedec, K Lu, L Lucero, A Malacari, M Maldera, S Mallamaci, M Maller, J Mandat, D Mantsch, P Mariazzi, AG Marin, V Maris, IC Marsella, G Martello, D Martin, L Martinez, H Bravo, OM Martraire, D Meza, JJM Mathes, HJ Mathys, S Matthews, J Matthews, JAJ Matthiae, G Maure, D Maurizio, D Mayotte, E Mazur, PO Medina, C Medina-Tanco, G Meissner, R Mello, VBB Melo, D Menshikov, A Messina, S Meyhandan, R Micheletti, MI Middendorf, L Minaya, IA Miramonti, L Mitrica, B Molina-Bueno, L Mollerach, S Montanet, F Morello, C Mostafa, M Moura, CA Muller, MA Muller, G Muller, S Mussa, R Navarra, G Navas, S Necesa, P Nellen, L Nelles, A Neuser, J Newton, D Nguyen, PH Niculescu-Oglinzanu, M Niechcio, M Niemietz, L Niggemann, T Nitz, D Nosek, D Novotny, V Nozka, L Ochilo, L Oikonomou, F Olinto, A Olmos-Gilbaja, VM Pacheco, N Selmi-Dei, DP Palatka, M Pallotta, J Papenbreer, P Parente, G Parra, A Paul, T Pech, M Pekala, J Pelayo, R Pepe, IM Perrone, L Petermann, E Peters, C Petrera, S Petrov, Y Phuntsok, J Piegaia, R Pierog, T Pieroni, P Pimenta, M Pirronello, V Platino, M Plum, M Porcelli, A Porowski, C Prado, RR Privitera, P Prouza, M Purrello, V Quel, EJ Querchfeld, S Quinn, S Rautenberg, J Ravel, O Ravignani, D Revenu, B Ridky, J Riggi, S Risse, M Ristori, P Rizi, V de Carvalho, WR Fernandez, GR Rojo, JR Rodriguez-Frias, MD Rogozin, D Rosado, J Roth, M Rouletl, E Rovero, AC Saffi, SJ Saftoiu, A Salamida, F Salazar, H Saleh, A Greus, FS Salina, G Sanchez, F Sanchez-Lucas, P Santos, E Santos, EM Sarazin, F Sarkar, B Sarmento, R Sato, R Scarso, C Schauer, M Scherini, V Schieler, H Schiffer, P Schmidt, D Scholten, O Schoorlemmer, H Schovanek, P Schroder, FG Schulz, A Schulz, J Schumacher, J Sciutto, SJ Segreto, A Settimo, M Shadkam, A Shellard, RC Sidelnik, I Sigl, G Sima, O Smialkowski, A Smida, R Snow, GR Sommers, P Sorokin, J Squartini, R Srivastava, YN Stanca, D Stanic, S Stapleton, J Stasielak, J Stephan, M Stutz, A Suarez, F Suomijarvi, T Supanitsky, AD Sutherland, MS Swain, J Szadkowski, Z Taborda, OA Tapia, A Tepe, A Theodoro, VM Timmermans, C Peixoto, CJT Toma, G Tomankova, L Tome, B Tonachini, A Elipe, GT Machado, DT Travnicek, P Ulrich, R Unger, M Urban, M Galicia, JFV Valino, I Valore, L van Aar, G van Bodegom, P van den Berg, AM van Velzen, S van Vliet, A Varela, E Cardenas, BV Varner, G Vasquez, R Vazquez, JR Vazquez, RA Veberic, D Verzi, V Vicha, J Videla, M Villasenor, L Vlcek, B Vorobiov, S Wahlberg, H Wainberg, O Walz, D Watson, AA Weber, M Weidenhaupt, K Weindl, A Werner, F Widom, A Wiencke, L Wilczynski, H Winchen, T Wittkowski, D Wundheiler, B Wykes, S Yang, L Yapici, T Yushkov, A Zas, E Zavrtanik, D Zavrtanik, M Zepeda, A Zhu, Y Zimmermann, B Ziolkowski, M Zuccarello, F AF Aab, A. Abreu, P. Aglietta, M. Ahn, E. J. Al Samarai, I. Albuquerque, I. F. M. Allekotte, I. Allison, P. Almela, A. Alvarez Castillo, J. Alvarez-Muniz, J. Batista, R. Alves Ambrosio, M. Aminaei, A. Anchordoqui, L. Andringa, S. Aramo, C. Aranda, V. M. Arqueros, F. Arsene, N. Asorey, H. Assis, P. Aublin, J. Ave, M. Avenier, M. Avila, G. Awal, N. Badescu, A. M. Barber, K. B. Baeuml, J. Baus, C. Beatty, J. J. Becker, K. H. Bellido, J. A. Berat, C. Bertaina, M. E. Bertou, X. Biermann, P. L. Billoir, P. Blaess, S. G. Blanco, A. Blanco, M. Bleve, C. Bluemer, H. Bohacova, M. Boncioli, D. Bonifazi, C. Borodai, N. Brack, J. Brancus, I. Bridgeman, A. Brogueira, P. Brown, W. C. Buchholz, P. Bueno, A. Buitink, S. Buscemi, M. Caballero-Mora, K. S. Caccianiga, B. Caccianiga, L. Candusso, M. Caramete, L. Caruso, R. Castellina, A. Cataldi, G. Cazon, L. Cester, R. Chavez, A. G. Chiavassa, A. Chinellato, J. A. Chudoba, J. Cilmo, M. Clay, R. W. Cocciolo, G. Colalillo, R. Coleman, A. Collica, L. Coluccia, M. R. Conceicao, R. Contreras, F. Cooper, M. J. Cordier, A. Coutu, S. Covault, C. E. Cronin, J. Dallier, R. Daniel, B. Dasso, S. Daumiller, K. Dawson, B. R. de Almeida, R. M. de Jong, S. J. De Mauro, G. de Mello Neto, J. R. T. De Mitri, I. de Oliveira, J. de Souza, V. del Pera, L. Deligny, O. Dembinski, H. Dhital, N. Di Giulio, C. Di Matteo, A. Diaz, J. C. Diaz Castro, M. L. Diogo, F. Dobrigkeit, C. Docters, W. D'Olivo, J. C. Dorofeev, A. Dorosti Hasankiadeh, Q. Dova, M. T. Ebr, J. Engel, R. Erdmann, M. Erfani, M. Escobar, C. O. Espadanal, J. Etchegoyen, A. Falcke, H. Fang, K. Farrar, G. Fauth, A. C. Fazzini, N. Ferguson, A. P. Fernandes, M. Fick, B. Figueira, J. M. Filevich, A. Filipcic, A. Fox, B. D. Fratu, O. Freire, M. M. Fuchs, B. Fujii, T. Garcia, B. Garcia-Pinto, D. Gate, F. Gemmeke, H. Gherghel-Lascu, A. Ghia, P. L. Giaccari, U. Giammarchi, M. Giller, M. Glas, D. Glaser, C. Glass, H. Golup, G. Gomez Berisso, M. Gomez Vitale, P. F. Gonzalez, N. Gookin, B. Gordon, J. Gorgi, A. Gorham, P. Gouffon, P. Griffith, N. Grillo, A. F. Grubb, T. D. Guarino, F. Guedes, G. P. Hampel, M. R. Hansen, P. Harari, D. Harrison, T. A. Hartmann, S. Harton, J. L. Haungs, A. Hebbeker, T. Heck, D. Heimann, P. Herve, A. E. Hill, G. C. Hojvat, C. Hollon, N. Holt, E. Homola, P. Hoerandel, J. R. Horvath, P. Hrabovsky, M. Huber, D. Huege, T. Insolia, A. Isar, P. G. Jandt, I. Jansen, S. Jarne, C. Johnsen, J. A. Josebachuili, M. Kaapa, A. Kambeitz, O. Kampert, K. H. Kasper, P. Katkov, I. Kegl, B. Keilhauer, B. Keivani, A. Kemp, E. Kieckhafer, R. M. Klages, H. O. Kleifges, M. Kleinfeller, J. Krause, R. Krohm, N. Kroemer, O. Kuempe, D. Kunka, N. LaHurd, D. Latronico, L. Lauer, R. Lauscher, M. Lautridou, P. Le Coz, S. Lebrun, D. Lebrun, P. Leigui de Oliveira, M. A. Letessier-Selvon, A. Lhenry-Yvon, I. Link, K. Lopes, L. Lopez, R. Lopez Casado, A. Louedec, K. Lu, L. Lucero, A. Malacari, M. Maldera, S. Mallamaci, M. Maller, J. Mandat, D. Mantsch, P. Mariazzi, A. G. Marin, V. Maris, I. C. Marsella, G. Martello, D. Martin, L. Martinez, H. Martinez Bravo, O. Martraire, D. Masias Meza, J. J. Mathes, H. J. Mathys, S. Matthews, J. Matthews, J. A. J. Matthiae, G. Maure, D. Maurizio, D. Mayotte, E. Mazur, P. O. Medina, C. Medina-Tanco, G. Meissner, R. Mello, V. B. B. Melo, D. Menshikov, A. Messina, S. Meyhandan, R. Micheletti, M. I. Middendorf, L. Minaya, I. A. Miramonti, L. Mitrica, B. Molina-Bueno, L. Mollerach, S. Montanet, F. Morello, C. Mostafa, M. Moura, C. A. Muller, M. A. Mueller, G. Mueller, S. Mussa, R. Navarra, G. Navas, S. Necesa, P. Nellen, L. Nelles, A. Neuser, J. Newton, D. Nguyen, P. H. Niculescu-Oglinzanu, M. Niechcio, M. Niemietz, L. Niggemann, T. Nitz, D. Nosek, D. Novotny, V. Nozka, L. Ochilo, L. Oikonomou, F. Olinto, A. Olmos-Gilbaja, V. M. Pacheco, N. Selmi-Dei, D. Pakk Palatka, M. Pallotta, J. Papenbreer, P. Parente, G. Parra, A. Paul, T. Pech, M. Pekala, J. Pelayo, R. Pepe, I. M. Perrone, L. Petermann, E. Peters, C. Petrera, S. Petrov, Y. Phuntsok, J. Piegaia, R. Pierog, T. Pieroni, P. Pimenta, M. Pirronello, V. Platino, M. Plum, M. Porcelli, A. Porowski, C. Prado, R. R. Privitera, P. Prouza, M. Purrello, V. Quel, E. J. Querchfeld, S. Quinn, S. Rautenberg, J. Ravel, O. Ravignani, D. Revenu, B. Ridky, J. Riggi, S. Risse, M. Ristori, P. Rizi, V. Rodrigues de Carvalho, W. Fernandez, G. Rodriguez Rodriguez Rojo, J. Rodriguez-Frias, M. D. Rogozin, D. Rosado, J. Roth, M. Rouletl, E. Rovero, A. C. Saffi, S. J. Saftoiu, A. Salamida, F. Salazar, H. Saleh, A. Salesa Greus, F. Salina, G. Sanchez, F. Sanchez-Lucas, P. Santos, E. Santos, E. M. Sarazin, F. Sarkar, B. Sarmento, R. Sato, R. Scarso, C. Schauer, M. Scherini, V. Schieler, H. Schiffer, P. Schmidt, D. Scholten, O. Schoorlemmer, H. Schovanek, P. Schroeder, F. G. Schulz, A. Schulz, J. Schumacher, J. Sciutto, S. J. Segreto, A. Settimo, M. Shadkam, A. Shellard, R. C. Sidelnik, I. Sigl, G. Sima, O. Smialkowski, A. Smida, R. Snow, G. R. Sommers, P. Sorokin, J. Squartini, R. Srivastava, Y. N. Stanca, D. Stanic, S. Stapleton, J. Stasielak, J. Stephan, M. Stutz, A. Suarez, F. Suomijarvi, T. Supanitsky, A. D. Sutherland, M. S. Swain, J. Szadkowski, Z. Taborda, O. A. Tapia, A. Tepe, A. Theodoro, V. M. Timmermans, C. Todero Peixoto, C. J. Toma, G. Tomankova, L. Tome, B. Tonachini, A. Elipe, G. Torralba Torres Machado, D. Travnicek, P. Ulrich, R. Unger, M. Urban, M. Valdes Galicia, J. F. Valino, I. Valore, L. van Aar, G. van Bodegom, P. van den Berg, A. M. van Velzen, S. van Vliet, A. Varela, E. Vargas Cardenas, B. Varner, G. Vasquez, R. Vazquez, J. R. Vazquez, R. A. Veberic, D. Verzi, V. Vicha, J. Videla, M. Villasenor, L. Vlcek, B. Vorobiov, S. Wahlberg, H. Wainberg, O. Walz, D. Watson, A. A. Weber, M. Weidenhaupt, K. Weindl, A. Werner, F. Widom, A. Wiencke, L. Wilczynski, H. Winchen, T. Wittkowski, D. Wundheiler, B. Wykes, S. Yang, L. Yapici, T. Yushkov, A. Zas, E. Zavrtanik, D. Zavrtanik, M. Zepeda, A. Zhu, Y. Zimmermann, B. Ziolkowski, M. Zuccarello, F. CA Pierre Auger Collaboration TI Measurement of the cosmic ray spectrum above 4 x 10(18) eV using inclined events detected with the Pierre Auger Observatory SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE ultra high energy cosmic rays; cosmic ray experiments ID TELESCOPE ARRAY EXPERIMENT; HIGH ENERGY NEUTRINOS; SURFACE DETECTOR; ZENITH ANGLES; AIR-SHOWERS; FLUORESCENCE AB A measurement of the cosmic-ray spectrum for energies exceeding 4x10(18) eV is presented, which is based on the analysis of showers with zenith angles greater than 60 degrees detected with the Pierre Auger Observatory between 1 January 2004 and 31 December 2013. The measured spectrum confirms a flux suppression at the highest energies. Above 5.3x10(18) eV, the "ankle", the flux can be described by a power law E-gamma with index gamma = 2.70 +/- 0.02 (stat) +/- 0.1 (sys) followed by a smooth suppression region. 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RP Aab, A (reprint author), Univ Siegen, D-57068 Siegen, Germany. EM auger_spokespersons@fnal.gov RI Arqueros, Fernando/K-9460-2014; Cazon, Lorenzo/G-6921-2014; Conceicao, Ruben/L-2971-2014; Bueno, Antonio/F-3875-2015; Beatty, James/D-9310-2011; de Mello Neto, Joao/C-5822-2013; de souza, Vitor/D-1381-2012; Guarino, Fausto/I-3166-2012; Colalillo, Roberta/R-5088-2016; Buscemi, Mario/R-5071-2016; Horvath, Pavel/G-6334-2014; Zuccarello, Francesca/R-1834-2016; Moura Santos, Edivaldo/K-5313-2016; Tome, Bernardo/J-4410-2013; Alvarez-Muniz, Jaime/H-1857-2015; Gouffon, Philippe/I-4549-2012; de Almeida, Rogerio/L-4584-2016; Fauth, Anderson/F-9570-2012; Todero Peixoto, Carlos Jose/G-3873-2012; Sao Carlos Institute of Physics, IFSC/USP/M-2664-2016; Abreu, Pedro/L-2220-2014; Assis, Pedro/D-9062-2013; Navas, Sergio/N-4649-2014; van den Berg, Adriaan/P-6792-2015; Chinellato, Carola Dobrigkeit /F-2540-2011; Valino, Ines/J-8324-2012; Vazquez, Jose Ramon/K-2272-2015; Pech, Miroslav/G-5760-2014; Brogueira, Pedro/K-3868-2012; Badescu, Alina/B-6087-2012; Garcia Pinto, Diego/J-6724-2014; Caramete, Laurentiu/C-2328-2011; Rosado, Jaime/K-9109-2014; zas, enrique/I-5556-2015; Chinellato, Jose Augusto/I-7972-2012; Rodriguez Frias, Maria /A-7608-2015; Inst. of Physics, Gleb Wataghin/A-9780-2017; De Mitri, Ivan/C-1728-2017; Mitrica, Bogdan/D-5201-2009; Alves Batista, Rafael/K-6642-2012; Rodriguez Fernandez, Gonzalo/C-1432-2014; Nosek, Dalibor/F-1129-2017 OI Arqueros, Fernando/0000-0002-4930-9282; Cazon, Lorenzo/0000-0001-6748-8395; Conceicao, Ruben/0000-0003-4945-5340; Bueno, Antonio/0000-0002-7439-4247; Beatty, James/0000-0003-0481-4952; de Mello Neto, Joao/0000-0002-3234-6634; Guarino, Fausto/0000-0003-1427-9885; Colalillo, Roberta/0000-0002-4179-9352; Buscemi, Mario/0000-0003-2123-5434; Horvath, Pavel/0000-0002-6710-5339; Zuccarello, Francesca/0000-0003-1853-2550; Moura Santos, Edivaldo/0000-0002-2818-8813; Tome, Bernardo/0000-0002-7564-8392; Alvarez-Muniz, Jaime/0000-0002-2367-0803; Gouffon, Philippe/0000-0001-7511-4115; de Almeida, Rogerio/0000-0003-3104-2724; Fauth, Anderson/0000-0001-7239-0288; Todero Peixoto, Carlos Jose/0000-0003-3669-8212; Abreu, Pedro/0000-0002-9973-7314; Assis, Pedro/0000-0001-7765-3606; Navas, Sergio/0000-0003-1688-5758; Chinellato, Carola Dobrigkeit /0000-0002-1236-0789; Valino, Ines/0000-0001-7823-0154; Vazquez, Jose Ramon/0000-0001-9217-5219; Brogueira, Pedro/0000-0001-6069-4073; Garcia Pinto, Diego/0000-0003-1348-6735; Rosado, Jaime/0000-0001-8208-9480; zas, enrique/0000-0002-4430-8117; Chinellato, Jose Augusto/0000-0002-3240-6270; Rodriguez Frias, Maria /0000-0002-2550-4462; De Mitri, Ivan/0000-0002-8665-1730; Alves Batista, Rafael/0000-0003-2656-064X; Rodriguez Fernandez, Gonzalo/0000-0002-4683-230X; Nosek, Dalibor/0000-0001-6219-200X FU Comision Nacional de Energia Atomica, Argentina; Fundacion Antorchas, Argentina; Gobierno de la Provincia de Mendoza, Argentina; Municipalidad de Malargue, Argentina; NDM Holdings, Argentina; Valle Las Lenas, Argentina; Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Brazil; Financiadora de Estudos e Projetos (FINEP), Brazil; Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Brazil; Sao Paulo Research Foundation (FAPESP), Brazil [2010/07359-6, 1999/05404-3]; Ministerio de Ciencia e Tecnologia (MCT), Brazil [MSMT-CR LG13007, 7AMB14AR005]; Czech Science Foundation, Czech Republic [14-17501S]; Centre de Calcul IN2P3/CNRS, France; Centre National de la Recherche Scientifique (CNRS), France; Conseil Regional Ile-de-France, France; Departement Physique Nucleaire et Corpusculaire, France [PNC-IN2P3/CNRS]; Departement Sciences de l'Univers (SDU-INSU/CNRS), Institut Lagrange de Paris (ILP), France [ANR-11-IDEX-0004-02]; Bundesministerium fur Bildung und Forschung (BMBF), Germany; Deutsche Forschungsgemeinschaft (DFG), Germany; Finanzministerium Baden-Wurttemberg, Germany; Helmholtz Alliance for Astroparticle Physics (HAP), Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Germany; Ministerium fur Wissenschaft und Forschung, Germany; Nordrhein Westfalen, Germany; Ministerium fur Wissenschaft, Germany; Forschung und Kunst, Germany; Baden-Wurttemberg, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Italy; Gran Sasso Center for Astroparticle Physics (CFA), Italy; CETEMPS Center of Excellence, Ministero degli Affari Esteri (MAE), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development, Poland [ERA-NET-ASPERA/01/11, ERA-NET-ASPERA/02/11]; National Science Centre, Poland [2013/08/M/5T9/00322, 2013/08/M/5T9/00728, HARMONIA 5 - 2013/10/M/ST9/00062]; Portuguese national funds, Portugal; FEDER funds within Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia (COMPETE), Portugal; Romanian Authority for Scientific Research ANCS, Romania; CNDI-UEFISCDI partnership projects, Romania [20/2012, 194/2012, 1/AS-PERA2/2012 ERA-NET, PN-II-RU-PD-2011-3-0145-17, PN-II-RU-PD-2011-3-0062]; Minister of National Education, Programme Space Technology and Advanced Research (STAR), Romania [83/2013]; Slovenian Research Agency, Slovenia; Comunidad de Madrid, Spain; FEDER funds, Spain; Ministerio de Educacion y Ciencia, Spain; Xunta de Galicia, Spain; European Community 7th Framework Program, Spain [FP7-PEOPLE-2012-IEF-328826]; Science and Technology Facilities Council, United Kingdom; Department of Energy [DE-AC02-07CH11359, DE-FR02-04ER41300, DE-FG02-99ER41107, DE-SC0011689]; National Science Foundation [0450696]; Grainger Foundation, U.S.A.; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET, European Particle Physics Latin American Network, European Union 7th Framework Program [PIRSES-2009-GA-246806]; UNESCO FX The successful installation, commissioning, and operation of the Pierre Auger Observatory would not have been possible without the strong commitment and effort from the technical and administrative staff in Malargue. We are very grateful to the following agencies and organizations for financial support: Comision Nacional de Energia Atomica, Fundacion Antorchas, Gobierno de la Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas, in gratitude for their continuing cooperation over land access, Argentina; the Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Sao Paulo Research Foundation (FAPESP) Grants No. 2010/07359-6 and No. 1999/05404-3, Ministerio de Ciencia e Tecnologia (MCT), Brazil; Grant No. MSMT-CR LG13007, No. 7AMB14AR005, and the Czech Science Foundation Grant No. 14-17501S, Czech Republic; Centre de Calcul IN2P3/CNRS, Centre National de la Recherche Scientifique (CNRS), Conseil Regional Ile-de-France, Departement Physique Nucleaire et Corpusculaire (PNC-IN2P3/CNRS), Departement Sciences de l'Univers (SDU-INSU/CNRS), Institut Lagrange de Paris (ILP) Grant No. LABEX ANR-10-LABX-63, within the Investissements d'Avenir Programme Grant No. ANR-11-IDEX-0004-02, France; Bundesministerium fur Bildung und Forschung (BMBF), Deutsche Forschungsgemeinschaft (DFG), Finanzministerium Baden-Wurttemberg, Helmholtz Alliance for Astroparticle Physics (HAP), Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Ministerium fur Wissenschaft und Forschung, Nordrhein Westfalen, Ministerium fur Wissenschaft, Forschung und Kunst, Baden-Wurttemberg, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Gran Sasso Center for Astroparticle Physics (CFA), CETEMPS Center of Excellence, Ministero degli Affari Esteri (MAE), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development, Grants No. ERA-NET-ASPERA/01/11 and No. ERA-NET-ASPERA/02/11, National Science Centre, Grants No. 2013/08/M/5T9/00322, No. 2013/08/M/5T9/00728 and No. HARMONIA 5 - 2013/10/M/ST9/00062, Poland; Portuguese national funds and FEDER funds within Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia (COMPETE), Portugal; Romanian Authority for Scientific Research ANCS, CNDI-UEFISCDI partnership projects Grants No. 20/2012 and No. 194/2012, Grants No. 1/AS-PERA2/2012 ERA-NET, No. PN-II-RU-PD-2011-3-0145-17 and No. PN-II-RU-PD-2011-3-0062, the Minister of National Education, Programme Space Technology and Advanced Research (STAR), Grant No. 83/2013, Romania; Slovenian Research Agency, Slovenia; Comunidad de Madrid, FEDER funds, Ministerio de Educacion y Ciencia, Xunta de Galicia, European Community 7th Framework Program, Grant No. FP7-PEOPLE-2012-IEF-328826, Spain; Science and Technology Facilities Council, United Kingdom; Department of Energy, Contracts No. DE-AC02-07CH11359, No. DE-FR02-04ER41300, No. DE-FG02-99ER41107 and No. DE-SC0011689, National Science Foundation, Grant No. 0450696, The Grainger Foundation, U.S.A.; ; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET, European Particle Physics Latin American Network, European Union 7th Framework Program, Grant No. PIRSES-2009-GA-246806; and UNESCO. NR 47 TC 4 Z9 4 U1 7 U2 47 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD AUG PY 2015 IS 8 AR 049 DI 10.1088/1475-7516/2015/08/049 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CW5OT UT WOS:000365046600049 ER PT J AU Blazek, J Vlah, Z Seljak, U AF Blazek, Jonathan Vlah, Zvonimir Seljak, Uros TI Tidal alignment of galaxies SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE weak gravitational lensing; galaxy morphology; galaxy clustering; cosmic web ID LARGE-SCALE STRUCTURE; INTRINSIC ELLIPTICITY CORRELATION; MASSIVEBLACK-II SIMULATION; WEAK-LENSING MEASUREMENTS; LUMINOUS RED GALAXIES; DARK-MATTER HALOS; COSMIC SHEAR; POWER SPECTRA; MODEL; CONSTRAINTS AB We develop an analytic model for galaxy intrinsic alignments (IA) based on the theory of tidal alignment. We calculate all relevant nonlinear corrections at one-loop order, including effects from nonlinear density evolution, galaxy biasing, and source density weighting. Contributions from density weighting are found to be particularly important and lead to bias dependence of the IA amplitude, even on large scales. This effect may be responsible for much of the luminosity dependence in IA observations. The increase in IA amplitude for more highly biased galaxies reflects their locations in regions with large tidal fields. We also consider the impact of smoothing the tidal field on halo scales. We compare the performance of this consistent nonlinear model in describing the observed alignment of luminous red galaxies with the linear model as well as the frequently used "nonlinear alignment model," finding a significant improvement on small and intermediate scales. We also show that the cross-correlation between density and IA (the "GI" term) can be effectively separated into source alignment and source clustering, and we accurately model the observed alignment down to the one-halo regime using the tidal field from the fully nonlinear halo-matter cross correlation. Inside the one-halo regime, the average alignment of galaxies with density tracers no longer follows the tidal alignment prediction, likely reflecting nonlinear processes that must be considered when modeling IA on these scales. Finally, we discuss tidal alignment in the context of cosmic shear measurements. C1 [Blazek, Jonathan] Ohio State Univ, Ctr Cosmol & AstroParticle Phys, Columbus, OH 43210 USA. [Blazek, Jonathan] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Vlah, Zvonimir] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94305 USA. [Vlah, Zvonimir] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Vlah, Zvonimir] SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA USA. [Vlah, Zvonimir] Stanford Univ, Menlo Pk, CA USA. [Seljak, Uros] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Seljak, Uros] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Seljak, Uros] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Blazek, J (reprint author), Ohio State Univ, Ctr Cosmol & AstroParticle Phys, Columbus, OH 43210 USA. EM blazek@berkeley.edu; zvlah@stanford.edu; useljak@berkeley.edu FU CCAPP fellowship; U.S. Department of Energy [DE-AC02-76SF00515]; NASA ATP grant [NNX12AG71G] FX We thank Chris Hirata, Rachel Mandelbaum, David Weinberg, and Benjamin Joachimi for helpful discussions. We also thank Sukhdeep Singh and Teppei Okumura for sharing and discussing their measurements and an anonymous referee for useful suggestions. J.B. acknowledges the support of a CCAPP fellowship. Z.V. is supported in part by the U.S. Department of Energy contract to SLAC no. DE-AC02-76SF00515. U.S. is supported in part by the NASA ATP grant NNX12AG71G. NR 56 TC 15 Z9 15 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD AUG PY 2015 IS 8 AR 015 DI 10.1088/1475-7516/2015/08/015 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CW5OT UT WOS:000365046600015 ER PT J AU Wu, JB Pan, YT Su, D Yang, H AF Wu, Jianbo Pan, Yung-Tin Su, Dong Yang, Hong TI Ultrathin and stable AgAu alloy nanowires SO SCIENCE CHINA-MATERIALS LA English DT Article ID GOLD NANORODS; AU NANOWIRES; CO OXIDATION; SOLAR-CELLS; TEMPERATURE; CATALYSTS; SURFACES; SIZE; NANOPARTICLES; NANOCRYSTALS AB Stable sub-two nanometer AgAu nanowires were synthesized using a CO-mediated gas reducing agent in liquid solution (GRAILS) method. These AgAu nanowires are stable, and do not readily break into short nanorods upon heating or electron beam irradiation. The surfaces along the longitudinal direction of the AgAu nanowires were largely bounded by the stable {111} facets. This structure differs from those ultrathin Au nanowires made without the use of CO gas, which were bounded by the {100} facets and unstable under e-beam irradiation. These differences in structure and composition lead to enhanced stability. C1 [Wu, Jianbo; Pan, Yung-Tin; Yang, Hong] Univ Illinois, Dept Chem & Biomol Engn, Urbana, IL 61801 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Yang, H (reprint author), Univ Illinois, Dept Chem & Biomol Engn, Urbana, IL 61801 USA. EM hy66@illinois.edu RI Yang, Hong/G-1583-2012 OI Yang, Hong/0000-0003-3459-4516 NR 59 TC 2 Z9 2 U1 5 U2 15 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 2095-8226 EI 2199-4501 J9 SCI CHINA MATER JI Sci. China-Mater. PD AUG PY 2015 VL 58 IS 8 BP 595 EP 602 DI 10.1007/s40843-015-0072-z PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA CV7UF UT WOS:000364480200001 ER PT J AU Tanaka, K Han, L Zhou, X Anders, A AF Tanaka, Koichi Han, Liang Zhou, Xue Anders, Andre TI Adding high time resolution to charge-state-specific ion energy measurements for pulsed copper vacuum arc plasmas SO PLASMA SOURCES SCIENCE & TECHNOLOGY LA English DT Article DE arc discharges; plasma diagnostics; ion energy distributions; time-resolved measurements ID CATHODE SPOT; DISTRIBUTIONS; FLUX AB Charge-state-resolved ion energy-time distributions of pulsed Cu arc plasma were obtained by using direct (time-dependent) acquisition of the ion detection signal from a commercial ion mass-per-charge and energy-per-charge analyzer. We find a shift of energies of Cu2+, Cu3+ and Cu4+ ions to lower values during the first few hundred microseconds after arc ignition, which is evidence for particle collisions in the plasma. The generation of Cu+ ions in the later part of the pulse, measured by the increase of Cu+ signal intensity and an associated slight reduction of the mean charge state, points to charge exchange reactions between ions and neutrals. At the very beginning of the pulse, when the plasma expands into vacuum and the plasma potential strongly fluctuates, ions with much higher energy (over 200 eV) are observed. Early in the pulse, the ion energies observed are approximately proportional to the ion charge state, and we conclude that the acceleration mechanism is primarily based on acceleration in an electric field. This field is directed away from the cathode, indicative of a potential hump. Measurements by a floating probe suggest that potential structures travel, and ions moving in the traveling field can gain high energies up to a few hundred electron-volts. Later in the pulse, the approximate proportionality is lost, which is related to increased smearing out of different energies due to collisions with neutrals, and/or to a change of the acceleration character from electrostatic to 'gas-dynamic', i.e. dominated by pressure gradient. C1 [Tanaka, Koichi] Mitsubishi Mat Corp, Cent Res Inst, Naka, Ibaraki 3110102, Japan. [Tanaka, Koichi; Han, Liang; Zhou, Xue; Anders, Andre] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Han, Liang] Xidian Univ, Sch Phys & Optoelect Engn, Xian 710071, Shaanxi, Peoples R China. [Zhou, Xue] Harbin Inst Technol, Sch Elect Engn & Automat, Harbin 150001, Heilongjiang, Peoples R China. RP Tanaka, K (reprint author), Mitsubishi Mat Corp, Cent Res Inst, 1002-14 Mukohyama, Naka, Ibaraki 3110102, Japan. EM tanak@mmc.co.jp RI Anders, Andre/B-8580-2009; OI Anders, Andre/0000-0002-5313-6505; Tanaka, Koichi/0000-0002-3180-7881 FU Mitsubishi Materials Corporation [WF010678]; US Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge the Mitsubishi Materials Corporation for supporting this study under Contract No WF010678. Work at Berkeley Lab is supported by the US Department of Energy under Contract No DE-AC02-05CH11231. NR 31 TC 1 Z9 1 U1 2 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0963-0252 EI 1361-6595 J9 PLASMA SOURCES SCI T JI Plasma Sources Sci. Technol. PD AUG PY 2015 VL 24 IS 4 AR 045010 DI 10.1088/0963-0252/24/4/045010 PG 10 WC Physics, Fluids & Plasmas SC Physics GA CV2PO UT WOS:000364098900022 ER PT J AU Pickard, BR Daniel, J Mehaffey, M Jackson, LE Neale, A AF Pickard, Brian R. Daniel, Jessica Mehaffey, Megan Jackson, Laura E. Neale, Anne TI EnviroAtlas: A new geospatial tool to foster ecosystem services science and resource management SO ECOSYSTEM SERVICES LA English DT Article DE Ecosystem services; Geospatial; Mapping; Web-services ID HEALTH; TREES; URBAN AB In this article we present EnviroAtlas, a web-based, open access tool that seeks to meet a range of needs by bringing together environmental, economic and demographic data in an ecosystem services framework. Within EnviroAtlas, there are three primary types of geospatial data: research-derived ecosystem services indicator data in their native resolution, indicator data that have been summarized to standard reporting units, and reference data. Reporting units include watershed basins across the contiguous U.S. and Census block groups throughout featured urban areas. EnviroAtlas includes both current and future drivers of change, such as land use and climate, for addressing issues of adaptation, conservation, equity, and resiliency. In addition to geospatial data, EnviroAtlas includes geospatial and statistical tools, and resources that support research, education, and decision-making. With the development of EnviroAtlas, we facilitate the practice of ecosystem services science by providing a framework to track conditions across political boundaries and assess policies and regulations. EnviroAtlas is a robust research and educational resource, with consistent, systems-oriented information to support nationally, regionally, and locally focused decisions. Published by Elsevier B.V. This is an open access article under the CC BY-NC-ND license (littp://creativecommons.org/licenses/by-nc-nd/4.0/). C1 [Pickard, Brian R.] US EPA, Off Res & Dev, Oak Ridge Inst Sci & Educ, Durham, NC 27711 USA. [Daniel, Jessica; Jackson, Laura E.] US EPA, Off Res & Dev, Natl Hlth & Environm Effects Res Lab, Durham, NC 27711 USA. [Mehaffey, Megan; Neale, Anne] US EPA, Off Res & Dev, Natl Exposure Res Lab, Durham, NC 27711 USA. RP Mehaffey, M (reprint author), US EPA, Off Res & Dev, 109 TW Alexander Dr, Durham, NC 27711 USA. EM mehaffey.megan@epa.gov FU US Environmental Protection Agency, through its Office of Research and Development FX EnviroAtlas is a collaborative project developed by US EPA, in cooperation with the US Geological Survey, the US Department of Agriculture's Natural Resources Conservation Service and Forest Service, and Landscope America. We would like to acknowledge the many federal employees, contractors, research fellows, and non-governmental organizations that have contributed to this work. The US Environmental Protection Agency, through its Office of Research and Development, partially funded and collaborated on the research described here. It has been subject to Agency review and approved for publication. Approval does not signify that the contents reflect the views of the Agency. NR 50 TC 8 Z9 8 U1 2 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2212-0416 J9 ECOSYST SERV JI Ecosyst. Serv. PD AUG PY 2015 VL 14 BP 45 EP 55 DI 10.1016/j.ecoser.2015.04.005 PG 11 WC Ecology; Environmental Sciences; Environmental Studies SC Environmental Sciences & Ecology GA CU6TQ UT WOS:000363666900006 ER PT J AU Han, GX Chu, XJ Xing, QH Li, DJ Yu, JB Luo, YQ Wang, GM Mao, PL Rafique, R AF Han, Guangxuan Chu, Xiaojing Xing, Qinghui Li, Dejun Yu, Junbao Luo, Yiqi Wang, Guangmei Mao, Peili Rafique, Rashad TI Effects of episodic flooding on the net ecosystem CO2 exchange of a supratidal wetland in the Yellow River Delta SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article ID CARBON-DIOXIDE EXCHANGE; CLIMATE-CHANGE; INTERANNUAL VARIABILITY; FLUX MEASUREMENTS; OMBROTROPHIC BOG; COASTAL WETLAND; PEATLAND; CHINA; RESPIRATION; TOLERANCE AB Episodic flooding due to intense rainfall events is characteristic in many wetlands, which may modify wetland-atmosphere exchange of CO2. However, the degree to which episodic flooding affects net ecosystem CO2 exchange (NEE) is poorly documented in supratidal wetlands of coastal zone, where rainfall-driven episodic flooding often occurs. To address this issue, the ecosystem CO2 fluxes were continuously measured using the eddy covariance technique for 4 years (2010-2013) in a supratidal wetland in the Yellow River Delta. Our results showed that over the growing season, the daily average uptake in the supratidal wetland was -1.4, -1.3, -1.0, and -1.3 g Cm-2 d(-1) for 2010, 2011, 2012, and 2013, respectively. On the annual scale, the supratidal wetland functioned as a strong sink for atmospheric CO2, with the annual NEE of -223, -164, and -247 g Cm-2 yr(-1) for 2011, 2012, and 2013, respectively. The mean diurnal pattern of NEE exhibited a smaller range of variation before episodic flooding than after it. Episodic flooding reduced the average daytime net CO2 uptake and the maximum rates of photosynthesis. In addition, flooding clearly suppressed the nighttime CO2 release from the wetland but increased its temperature sensitivity. Therefore, effects of episodic flooding on the direction and magnitude of NEE should be considered when predicting the ecosystem responses to future climate change in supratidal wetlands. C1 [Han, Guangxuan; Chu, Xiaojing; Xing, Qinghui; Yu, Junbao; Wang, Guangmei; Mao, Peili] Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai, Peoples R China. [Li, Dejun] Chinese Acad Sci, Inst Subtrop Agr, Changsha, Hunan, Peoples R China. [Luo, Yiqi] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Rafique, Rashad] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA. RP Han, GX (reprint author), Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai, Peoples R China. EM gxhan@yic.ac.cn; jbyu@yic.ac.cn FU National Natural Science Foundation of China [41301083, 41301052]; National Science and Technology Support Program of China [2011BAC02B01] FX This research was funded by the National Natural Science Foundation of China (41301083 and 41301052) and the National Science and Technology Support Program of China (2011BAC02B01). We wish to thank Liqiong Yang, Huabing Li, Yuhong Liu, Baohua Xie, and Bo Guan for their helpful work during this study. We also thank two anonymous reviewers for their expert advice and fruitful comments that significantly improved the paper. The data used in this study can be accessed by contacting the corresponding author. NR 66 TC 2 Z9 3 U1 7 U2 21 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD AUG PY 2015 VL 120 IS 8 BP 1506 EP 1520 DI 10.1002/2015JG002923 PG 15 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA CU2DG UT WOS:000363332300004 ER PT J AU Clark, MP Fan, Y Lawrence, DM Adam, JC Bolster, D Gochis, DJ Hooper, RP Kumar, M Leung, LR Mackay, DS Maxwell, RM Shen, CP Swenson, SC Zeng, XB AF Clark, Martyn P. Fan, Ying Lawrence, David M. Adam, Jennifer C. Bolster, Diogo Gochis, David J. Hooper, Richard P. Kumar, Mukesh Leung, L. Ruby Mackay, D. Scott Maxwell, Reed M. Shen, Chaopeng Swenson, Sean C. Zeng, Xubin TI Improving the representation of hydrologic processes in Earth System Models SO WATER RESOURCES RESEARCH LA English DT Review ID LAND-SURFACE SCHEME; SOIL-MOISTURE HETEROGENEITY; GENERAL-CIRCULATION MODELS; STORAGE BOUSSINESQ MODEL; WATER-TABLE DYNAMICS; VARIABLE SOURCE AREAS; RICHARDS EQUATION; SUBSURFACE FLOW; CLIMATE MODELS; PART I AB Many of the scientific and societal challenges in understanding and preparing for global environmental change rest upon our ability to understand and predict the water cycle change at large river basin, continent, and global scales. However, current large-scale land models (as a component of Earth System Models, or ESMs) do not yet reflect the best hydrologic process understanding or utilize the large amount of hydrologic observations for model testing. This paper discusses the opportunities and key challenges to improve hydrologic process representations and benchmarking in ESM land models, suggesting that (1) land model development can benefit from recent advances in hydrology, both through incorporating key processes (e.g., groundwater-surface water interactions) and new approaches to describe multiscale spatial variability and hydrologic connectivity; (2) accelerating model advances requires comprehensive hydrologic benchmarking in order to systematically evaluate competing alternatives, understand model weaknesses, and prioritize model development needs, and (3) stronger collaboration is needed between the hydrology and ESM modeling communities, both through greater engagement of hydrologists in ESM land model development, and through rigorous evaluation of ESM hydrology performance in research watersheds or Critical Zone Observatories. Such coordinated efforts in advancing hydrology in ESMs have the potential to substantially impact energy, carbon, and nutrient cycle prediction capabilities through the fundamental role hydrologic processes play in regulating these cycles. C1 [Clark, Martyn P.; Lawrence, David M.; Gochis, David J.; Swenson, Sean C.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Fan, Ying] Rutgers State Univ, Dept Earth & Planetary Sci, New Brunswick, NJ 08903 USA. [Adam, Jennifer C.] Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USA. [Bolster, Diogo] Univ Notre Dame, Dept Civil & Environm Engn & Earth Sci, South Bend, IN USA. [Hooper, Richard P.] Consortium Univ, Adv Hydrol Sci Inc, Durham, NC USA. [Kumar, Mukesh] Duke Univ, Nicholas Sch Environm, Durham, NC 27708 USA. [Leung, L. Ruby] Pacific NW Natl Lab, Richland, WA 99352 USA. [Mackay, D. Scott] SUNY Buffalo, Dept Geog, Buffalo, NY 14260 USA. [Maxwell, Reed M.] Colorado Sch Mines, Dept Geol & Geol Engn, Golden, CO 80401 USA. [Shen, Chaopeng] Penn State Univ, Dept Civil & Environm Engn, State Coll, PA USA. [Zeng, Xubin] Univ Arizona, Dept Atmospher Sci, Tucson, AZ USA. RP Clark, MP (reprint author), Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. EM mclark@ucar.edu RI Mackay, Scott/J-7569-2012; Lawrence, David/C-4026-2011; Bolster, Diogo/D-9667-2011; Samaniego, Luis/G-8651-2011; OI Mackay, Scott/0000-0003-0477-9755; Lawrence, David/0000-0002-2968-3023; Bolster, Diogo/0000-0003-3960-4090; Samaniego, Luis/0000-0002-8449-4428; Zeng, Xubin/0000-0001-7352-2764 FU National Science Foundation, through CUAHSI cooperative agreement [NSF-EAR-0753521]; INSPIRE grant [NSF-EAR-1528298] FX This paper is produced as part of a new CUAHSI initiative to improve the representation of hydrologic processes in Earth System Models. Support from the National Science Foundation, through CUAHSI cooperative agreement (NSF-EAR-0753521) and an INSPIRE grant (NSF-EAR-1528298), is gratefully acknowledged. NR 282 TC 32 Z9 32 U1 23 U2 73 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD AUG PY 2015 VL 51 IS 8 BP 5929 EP 5956 DI 10.1002/2015WR017096 PG 28 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA CU3CZ UT WOS:000363402800005 ER PT J AU Mackay, DS Roberts, DE Ewers, BE Sperry, JS McDowell, NG Pockman, WT AF Mackay, D. Scott Roberts, David E. Ewers, Brent E. Sperry, John S. McDowell, Nathan G. Pockman, William T. TI Interdependence of chronic hydraulic dysfunction and canopy processes can improve integrated models of tree response to drought SO WATER RESOURCES RESEARCH LA English DT Article ID PINYON-JUNIPER WOODLAND; VAPOR-PRESSURE DEFICIT; PLANT WATER-USE; STOMATAL CONDUCTANCE; VEGETATION MORTALITY; ANISOHYDRIC BEHAVIORS; CARBON ALLOCATION; TRANSPORT MODEL; PONDEROSA PINE; CLIMATE-CHANGE AB Hydraulic systems of plants have evolved in the context of carbon allocation and fitness trade-offs of maximizing carbon gain and water transport in the face of short and long-term fluctuations in environmental conditions. The resulting diversity of traits include a continuum of isohydry-anisohydry or high to low relative stomatal closure during drought, shedding of canopy foliage or disconnecting roots from soil to survive drought, and adjusting root areas to efficiently manage canopy water costs associated with photosynthesis. These traits are examined within TREES, an integrated model that explicitly couples photosynthesis and carbon allocation to soil-plant hydraulics and canopy processes. Key advances of the model are its ability to account for differences in soil and xylem cavitation, transience of hydraulic impairment associated with delayed or no refilling of xylem, and carbon allocation to plant structures based on photosynthetic uptake of carbon and hydraulic limitations to water transport. The model was used to examine hydraulic traits of cooccurring isohydric (pinon pine) and anisohydric (one-seed juniper) trees from a field-based experimental drought. Model predictions of both transpiration and leaf water potential were improved when there was no refilling of xylem over simulations where xylem was able refill in response to soil water recharge. Model experiments with alternative root-to-leaf area ratios (R-R/L) showed the R-R/L that supports maximum cumulative water use is not beneficial for supporting maximum carbon gain during extended drought, illustrating how a process model reveals trade-offs in plant traits. C1 [Mackay, D. Scott; Roberts, David E.] SUNY Buffalo, Dept Geog, Buffalo, NY 14260 USA. [Ewers, Brent E.] Univ Wyoming, Dept Bot, Laramie, WY 82071 USA. [Ewers, Brent E.] Univ Wyoming, Program Ecol, Laramie, WY 82071 USA. [Sperry, John S.] Univ Utah, Dept Biol, Salt Lake City, UT 84112 USA. [McDowell, Nathan G.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Pockman, William T.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. RP Mackay, DS (reprint author), SUNY Buffalo, Dept Geog, Buffalo, NY 14260 USA. EM dsmackay@buffalo.edu RI Mackay, Scott/J-7569-2012; Pockman, William/D-4086-2014 OI Mackay, Scott/0000-0003-0477-9755; Pockman, William/0000-0002-3286-0457 FU National Science Foundation [EAR-0405306, EAR-0405381]; Department of Energy Office of Biological and Environmental Research; National Institute for Climatic Change Research (NICCR) Midwestern region [050516Z20]; College of Arts & Sciences at the University at Buffalo FX Development of TREES was partially supported by grants from the National Science Foundation (EAR-0405306, EAR-0405381), Department of Energy Office of Biological and Environmental Research, National Institute for Climatic Change Research (NICCR) Midwestern region sub-agreement 050516Z20, and the College of Arts & Sciences at the University at Buffalo. The long-term experimental data used in this study were supported by the U.S. Department of Energy Office of Science (BER). The statements made in this manuscript reflect the views of the authors and do not necessarily reflect the views of the funding agencies. We are grateful to Simone Fatichi and two anonymous reviewers whose comments helped improve the manuscript. Data used in this manuscript are available from the LTER network [see Pockman and McDowell, 2014a, 2014b, 2014c]. TREES can be obtained by contacting the first author. NR 97 TC 13 Z9 13 U1 5 U2 26 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD AUG PY 2015 VL 51 IS 8 BP 6156 EP 6176 DI 10.1002/2015WR017244 PG 21 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA CU3CZ UT WOS:000363402800017 ER PT J AU Johnson, T Versteeg, R Thomle, J Hammond, G Chen, XY Zachara, J AF Johnson, Tim Versteeg, Roelof Thomle, Jon Hammond, Glenn Chen, Xingyuan Zachara, John TI Four-dimensional electrical conductivity monitoring of stage-driven river water intrusion: Accounting for water table effects using a transient mesh boundary and conditional inversion constraints SO WATER RESOURCES RESEARCH LA English DT Article ID SURFACE-WATER; HYPORHEIC ZONE; RESISTIVITY TOMOGRAPHY; SEAWATER INTRUSION; OCCAMS INVERSION; CROSSHOLE ERT; GROUND-WATER; TRACER; AQUIFER; STREAM AB This paper describes and demonstrates two methods of providing a priori information to the surface-based time-lapse three-dimensional electrical resistivity tomography (ERT) problem for monitoring stage-driven or tide-driven surface water intrusion into aquifers. First, a mesh boundary is implemented that conforms to the known location of the water table through time, thereby enabling the inversion to place a sharp bulk conductivity contrast at that boundary without penalty. Second, a nonlinear inequality constraint is used to allow only positive or negative transient changes in EC to occur within the saturated zone, dependent on the relative contrast in fluid electrical conductivity between surface water and groundwater. A 3-D field experiment demonstrates that time-lapse imaging results using traditional smoothness constraints are unable to delineate river water intrusion. The water table and inequality constraints provide the inversion with the additional information necessary to resolve the spatial extent of river water intrusion through time. C1 [Johnson, Tim; Thomle, Jon; Chen, Xingyuan] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Versteeg, Roelof] Subsurface Insights LLC, Hanover, NH USA. [Hammond, Glenn] Sandia Natl Labs, Appl Syst Anal & Res, Albuquerque, NM USA. [Zachara, John] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Johnson, T (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM tj@pnnl.gov FU U.S. Department of Energy (DOE), Office of Biological and Environmental Research (BER), BER's Subsurface Biogeochemistry Research Program (SBR) FX We appreciate helpful reviews by Joseph Doetsch and two anonymous referees. Data used to produce this manuscript may be acquired in digital form from the corresponding author (tj@pnnl.gov). This research was supported by the U.S. Department of Energy (DOE), Office of Biological and Environmental Research (BER), as part of BER's Subsurface Biogeochemistry Research Program (SBR). This contribution originates from the SBR Scientific Focus Area (SFA) at the Pacific Northwest National Laboratory (PNNL). NR 66 TC 1 Z9 1 U1 4 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD AUG PY 2015 VL 51 IS 8 BP 6177 EP 6196 DI 10.1002/2014WR016129 PG 20 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA CU3CZ UT WOS:000363402800018 ER PT J AU Morrell-Falvey, JL Elkins, JG Wang, ZW AF Morrell-Falvey, Jennifer L. Elkins, James G. Wang, Zhi-Wu TI Determination of the cellulase activity distribution in Clostridium thermocellum and Caldicellulosiruptor obsidiansis cultures using a fluorescent substrate SO JOURNAL OF ENVIRONMENTAL SCIENCES LA English DT Article DE Thermophilic; Biofilm; Cellulose; Cellulase; Biofuel ID EXTRACELLULAR GLYCOCALYX; CELLULOLYTIC BACTERIA; DEGRADATION; MODEL; MICROORGANISMS; POPULATIONS; HYDROLYSIS; BIOFUELS; ENZYMES; WATER AB This study took advantage of resorufin cellobioside as a fluorescent substrate to determine the distribution of cellulase activity in cellulosic biomass fermentation systems. Cellulolytic biofilms were found to express nearly four orders greater cellulase activity compared to planktonic cultures of Clostridium thermocellum and Caldicellulosiruptor obsidiansis, which can be primarily attributed to the high cell concentration and surface attachment. The formation of biofilms results in cellulases being secreted close to their substrates, which appears to be an energetically favorable stategy for insoluble substrate utilization. For the same reason, cellulases should be closely associated with the surfaces of suspended cell in soluble substrate-fed culture, which has been verified with cellobiose-fed cultures of C. thermocellum and C. obsidiansis. This study addressed the importance of cellulase activity distribution in cellulosic biomass fermentation, and provided theoretical foundation for the leading role of biofilm in cellulose degradation. System optimization and reactor designs that promote biofilm formation in cellulosic biomass hydrolysis may promise an improved cellulosic biofuel process. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V. C1 [Morrell-Falvey, Jennifer L.; Elkins, James G.; Wang, Zhi-Wu] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Biosci Div, Oak Ridge, TN 37831 USA. [Wang, Zhi-Wu] Ohio State Univ ATI, Wooster, OH 44691 USA. RP Wang, ZW (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Biosci Div, Oak Ridge, TN 37831 USA. EM wzw@vt.edu RI Morrell-Falvey, Jennifer/A-6615-2011 OI Morrell-Falvey, Jennifer/0000-0002-9362-7528 FU BioEnergy Science Center (BESC), which is a US Department of Energy Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; US Department of Energy [DE-AC05-00OR22725] FX This work was supported by the BioEnergy Science Center (BESC), which is a US Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the US Department of Energy under contract DE-AC05-00OR22725. NR 33 TC 1 Z9 1 U1 2 U2 21 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 1001-0742 EI 1878-7320 J9 J ENVIRON SCI-CHINA JI J. Environ. Sci. PD AUG 1 PY 2015 VL 34 BP 212 EP 218 DI 10.1016/j.jes.2015.03.009 PG 7 WC Environmental Sciences SC Environmental Sciences & Ecology GA CT7FT UT WOS:000362980400023 PM 26257364 ER PT J AU Brauer, S Cadillo-Quiroz, H Kyrpides, N Woyke, T Goodwin, L Detter, C Podell, S Yavitt, JB Zinder, SH AF Braeuer, Suzanna Cadillo-Quiroz, Hinsby Kyrpides, Nikos Woyke, Tanja Goodwin, Lynne Detter, Chris Podell, Sheila Yavitt, Joseph B. Zinder, Stephen H. TI Genome of Methanoregula boonei 6A8 reveals adaptations to oligotrophic peatland environments SO MICROBIOLOGY-SGM LA English DT Article ID NEW-YORK-STATE; AMINO-ACID SUBSTITUTIONS; ESCHERICHIA-COLI; METHANOGENIC ARCHAEA; KDPFABC COMPLEX; HYDROGENOTROPHIC METHANOGEN; ATP SYNTHESIS; KDP-ATPASE; ACIDIPHILIC METHANOGEN; MINEROTROPHIC FEN AB Analysis of the genome sequence of Methanoregula boonei strain 6A8, an acidophilic methanogen isolated from an ombrotrophic (rain-fed) peat bog, has revealed unique features that likely allow it to survive in acidic, nutrient-poor conditions. First, M. boonei is predicted to generate ATP using protons that are abundant in peat, rather than sodium ions that are scarce, and the sequence of a membrane-bound methyltransferase, believed to pump Na+ in all methanogens, shows differences in key amino acid residues. Further, perhaps reflecting the hypokalennic status of many peat bogs, M. boonei demonstrates redundancy in the predicted potassium uptake genes trk, kdp and kup, some of which may have been horizontally transferred to methanogens from bacteria, possibly Geobacter spp. Overall, the putative functions of the potassium uptake, ATPase and methyltransferase genes may, at least in part, explain the cosmopolitan success of group E1/E2 and related methanogenic archaea in acidic peat bogs. C1 [Braeuer, Suzanna] Appalachian State Univ, Dept Biol, Boone, NC 28608 USA. [Cadillo-Quiroz, Hinsby] Arizona State Univ, Biodesign Inst, Swette Ctr Environm Biotechnol, Tempe, AZ 85287 USA. [Kyrpides, Nikos; Woyke, Tanja] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Goodwin, Lynne; Detter, Chris] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Podell, Sheila] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Yavitt, Joseph B.] Cornell Univ, Dept Nat Resources, Ithaca, NY 14853 USA. [Zinder, Stephen H.] Cornell Univ, Dept Microbiol, Ithaca, NY 14853 USA. RP Brauer, S (reprint author), Appalachian State Univ, Dept Biol, Boone, NC 28608 USA. EM brauersl@appstate.edu RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 FU Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The authors thank the following employees of the US Department of Energy Joint Genome Institute - Marcel Huntemann, Alex Copeland, Amy Chen, Victor Markowitz, Krishnaveni Palaniappan, Natalia Ivanova, Natalia Mikhailova, Galina Ovchinnikova, Evan Andersen, Amrita Pati, Dimitrios Stamatis, T. B. K. Reddy, Chew Yee Ngan, Mansi Chovatia, Chris Daum, Nicole Shapiro and Michael N. Cantor - as well as the following employees of the Los Alamos National Lab - Hazuki Teshima, Olga Chertkov, Hajnalka Daligault, Karen Davenport, Wei Gu, Christine Munk, Xiaojing Zhang, David Bruce, Yan Xu, Beverly Quintana, Krista Reitenga, Yulia Kunde, Lance Green, Tracy Erkkila, Cliff Han and Patrick Chain - for assistance with genome sequencing. The work conducted by the US Department of Energy Joint Genome Institute, a Department of Energy Office of Science User Facility, is supported by the Office of Science of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 65 TC 2 Z9 2 U1 4 U2 13 PU SOC GENERAL MICROBIOLOGY PI READING PA MARLBOROUGH HOUSE, BASINGSTOKE RD, SPENCERS WOODS, READING RG7 1AG, BERKS, ENGLAND SN 1350-0872 EI 1465-2080 J9 MICROBIOL-SGM JI Microbiology-(UK) PD AUG PY 2015 VL 161 BP 1572 EP 1581 DI 10.1099/mic.0.000117 PN 8 PG 10 WC Microbiology SC Microbiology GA CT7OW UT WOS:000363005400004 PM 25998264 ER PT J AU Boyer, MD Schuster, E AF Boyer, Mark D. Schuster, Eugenio TI Nonlinear burn condition control in tokamaks using isotopic fuel tailoring SO NUCLEAR FUSION LA English DT Article DE nonlinear control; burn control; thermal stability ID THERMONUCLEAR EXPERIMENTAL REACTOR; ARTIFICIAL NEURAL-NETWORKS; SAFE IGNITED OPERATION; FUSION-REACTOR; STABILIZATION; DENSITY; PLASMAS; RATIO; ITER; JET AB One of the fundamental problems in tokamak fusion reactors is how to control the plasma density and temperature in order to regulate the amount of fusion power produced by the device. Control of these parameters will be critical to the success of burning plasma experiments like ITER. The most previous burn condition control efforts use either non-model based control designs or techniques based on models linearized around particular operating points. Such strategies limit the potential operational space and must be carefully retuned or redesigned to accommodate changes in operating points or plasma parameters. In this work, a nonlinear dynamic model of the spatial averages of energy and ion species densities is used to synthesize a nonlinear feedback controller for stabilizing the burn condition. The nonlinear model-based control strategy guarantees a much larger operational space than previous linear controllers. Because it is not designed around a particular operating point, the controller can be used to move from one burn condition to another. The proposed scheme first attempts to use regulation of the auxiliary heating power to reject temperature perturbations, then, if necessary, uses isotopic fuel tailoring as a way to reduce fusion heating during positive temperature perturbations. A global model of hydrogen recycling is incorporated into the model used for design and simulation, and the proposed control scheme is tested for a range of recycling model parameters. As we find the possibility of changing the isotopic mix can be limited for certain unfavorable recycling conditions, we also consider impurity injection as a back-up method for controlling the system. A simple supervisory control strategy is proposed to switch between the primary and back-up control schemes based on stability and performance criteria. A zero-dimensional simulation study is used to study the performance of the control scheme for several scenarios and model parameters. Finally, a one-dimensional simulation is done to test the robustness of the control scheme to spatially varying parameters. C1 [Boyer, Mark D.; Schuster, Eugenio] Lehigh Univ, Dept Mech Engn & Mech, Bethlehem, PA 18015 USA. RP Boyer, MD (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. EM mboyer@pppl.gov FU National Science Foundation [ECCS-0645086]; US Department of Energy [DE-SC0001334, DE-SC0010661] FX This work was supported by the National Science Foundation CAREER award program (ECCS-0645086) and by the US Department of Energy under contracts DE-SC0001334 and DE-SC0010661. NR 42 TC 0 Z9 1 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 083021 DI 10.1088/0029-5515/55/8/083021 PG 24 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700021 ER PT J AU Heidbrink, WW Austin, ME Collins, CS Gray, T Grierson, BA Kramer, GJ Lanctot, M Pace, DC Van Zeeland, MA Mclean, AG AF Heidbrink, W. W. Austin, M. E. Collins, C. S. Gray, T. Grierson, B. A. Kramer, G. J. Lanctot, M. Pace, D. C. Van Zeeland, M. A. Mclean, A. G. TI Synergy between fast-ion transport by core MHD and test blanket module fields in DIII-D experiments SO NUCLEAR FUSION LA English DT Article DE fast ions; sawtooth; Alfven eigenmodes; neoclassical tearing modes ID D TOKAMAK; CODE AB Fast-ion transport caused by the combination of MHD and a mock-up test-blanket module (TBM) coil is measured in the DIII-D tokamak. The primary diagnostic is an infrared camera that measures the heat flux on the tiles surrounding the coil. The combined effects of the TBM and four other potential sources of transport are studied: neoclassical tearing modes, Alfen eigenmodes, sawteeth, and applied resonant magnetic perturbation fields for the control of edge localized modes. A definitive synergistic effect is observed at sawtooth crashes where, in the presence of the TBM, the localized heat flux at a burst increases from 0.36 +/- 0.27 to 2.6 +/- 0.5 MW m(-2). C1 [Heidbrink, W. W.; Austin, M. E.] Univ Calif Irvine, Irvine, CA 92697 USA. [Collins, C. S.] Univ Texas Austin, Austin, TX 78712 USA. [Gray, T.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Grierson, B. A.; Kramer, G. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Lanctot, M.; Pace, D. C.; Van Zeeland, M. A.] Gen Atom Co, San Diego, CA USA. [Mclean, A. G.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Heidbrink, WW (reprint author), Univ Calif Irvine, Irvine, CA 92697 USA. EM Bill.Heidbrink@uci.edu RI Lanctot, Matthew J/O-4979-2016 OI Lanctot, Matthew J/0000-0002-7396-3372 FU U.S. Department of Energy [SC-G903402, DE-AC52-07NA27344, DE-FG03-97ER54415, DE-AC05-0000R22725, DE-AC02-09CH11466, DE-FC02-04ER54698] FX This work was supported by the U.S. Department of Energy under SC-G903402, DE-AC52-07NA27344, DE-FG03-97ER54415, DE-AC05-0000R22725, DE-AC02-09CH11466, and DE-FC02-04ER54698. We thank R. Nazikian and C. Petty for helpful suggestions, D. Orlov for the TRIP3D calculation, and the entire DIII-D team for their support. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. NR 25 TC 2 Z9 2 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 083023 DI 10.1088/0029-5515/55/8/083023 PG 12 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700023 ER PT J AU Meier, ET Gerhardt, S Menard, JE Rognlien, TD Soukhanovskii, VA AF Meier, E. T. Gerhardt, S. Menard, J. E. Rognlien, T. D. Soukhanovskii, V. A. TI Modeling divertor concepts for spherical tokamaks NSTX-U and ST-FNSF SO NUCLEAR FUSION LA English DT Article DE spherical tokamak; divertor; UEDGE; snowflake ID PHYSICS AB The compact nature of the spherical tokamak (ST) presents an economically attractive path to fusion commercialization, but concentrates power exhaust, threatening the integrity of plasma-facing components. To address this challenge, experimentally constrained divertor modeling in the National Spherical Torus Experiment (NSTX) is extrapolated to investigate divertor concepts for future ST devices. Analysis of NSTX Upgrade with UEDGE shows that the secondary snowflake X-point position can be adjusted for favorable neutral transport, enabling stable partial detachment at reduced core densities. For a notional ST-based Fusion Nuclear Science Facility, divertor concepts are identified that provide heat flux mitigation (<10 MW m(-2)) and low temperatures (<10 eV) compatible with high-Z targets. This research provides guidance for upcoming experiments and a basis for continued development of predictive capability for divertor performance in STs. C1 [Meier, E. T.; Rognlien, T. D.; Soukhanovskii, V. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Gerhardt, S.; Menard, J. E.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Meier, ET (reprint author), Coll William & Mary, Williamsburg, VA 23187 USA. EM emeier@wm.edu OI Menard, Jonathan/0000-0003-1292-3286 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, DE-AC02-09CH11466]; U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences FX Discussions with LLNL scientists D.D. Ryutov, M.V. Umansky, M.E. Rensink, and G.D. Porter, about divertor and snowflake physics, and about UEDGE, have been much appreciated. Special thanks also to D.A. Gates and F.M. Poli of PPPL, who provided valuable advice for running ISOLVER. Insightful input from the referees is also gratefully acknowledged. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contracts DE-AC52-07NA27344 and DE-AC02-09CH11466. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences. NR 22 TC 2 Z9 2 U1 1 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 086002 DI 10.1088/0029-5515/55/8/086002 PG 8 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700029 ER PT J AU Meneghini, O Smith, SP Lao, LL Izacard, O Ren, Q Park, JM Candy, J Wang, Z Luna, CJ Izzo, VA Grierson, BA Snyder, PB Holland, C Penna, J Lu, G Raum, P McCubbin, A Orlov, DM Belli, EA Ferraro, NM Prater, R Osborne, TH Turnbull, AD Staebler, GM AF Meneghini, O. Smith, S. P. Lao, L. L. Izacard, O. Ren, Q. Park, J. M. Candy, J. Wang, Z. Luna, C. J. Izzo, V. A. Grierson, B. A. Snyder, P. B. Holland, C. Penna, J. Lu, G. Raum, P. McCubbin, A. Orlov, D. M. Belli, E. A. Ferraro, N. M. Prater, R. Osborne, T. H. Turnbull, A. D. Staebler, G. M. CA AToM Team TI Integrated modeling applications for tokamak experiments with OMFIT SO NUCLEAR FUSION LA English DT Article DE OMFIT; integrated; modeling; DIII-D tokamak ID COLLISIONALITY REGIME; CYCLOTRON WAVES; PLASMAS; SIMULATION; TRANSPORT; STABILITY; CODE; PEDESTAL; PHYSICS; MODES AB One modeling framework for integrated tasks (OMFIT) is a comprehensive integrated modeling framework which has been developed to enable physics codes to interact in complicated workflows, and support scientists at all stages of the modeling cycle. The OMFIT development follows a unique bottom-up approach, where the framework design and capabilities organically evolve to support progressive integration of the components that are required to accomplish physics goals of increasing complexity. OMFIT provides a workflow for easily generating full kinetic equilibrium reconstructions that are constrained by magnetic and motional Stark effect measurements, and kinetic profile information that includes fast-ion pressure modeled by a transport code. It was found that magnetic measurements can be used to quantify the amount of anomalous fast-ion diffusion that is present in DIII-D discharges, and provide an estimate that is consistent with what would be needed for transport simulations to match the measured neutron rates. OMFIT was used to streamline edge-stability analyses, and evaluate the effect of resonant magnetic perturbation (RMP) on the pedestal stability, which have been found to be consistent with the experimental observations. The development of a five-dimensional numerical fluid model for estimating the effects of the interaction between magnetohydrodynamic (MHD) and microturbulence, and its systematic verification against analytic models was also supported by the framework. OMFIT was used for optimizing an innovative high-harmonic fast wave system proposed for DIII-D. For a parallel refractive index n(parallel to) > 3, the conditions for strong electron-Landau damping were found to be independent of launched n(parallel to) and poloidal angle. OMFIT has been the platform of choice for developing a neural-network based approach to efficiently perform a non-linear multivariate regression of local transport fluxes as a function of local dimensionless parameters. Transport predictions for thousands of DIII-D discharges showed excellent agreement with the power balance calculations across the whole plasma radius and over a broad range of operating regimes. Concerning predictive transport simulations, the framework made possible the design and automation of a workflow that enables self-consistent predictions of kinetic profiles and the plasma equilibrium. It is found that the feedback between the transport fluxes and plasma equilibrium can significantly affect the kinetic profiles predictions. Such a rich set of results provide tangible evidence of how bottom-up approaches can potentially provide a fast track to integrated modeling solutions that are functional, cost-effective, and in sync with the research effort of the community. C1 [Meneghini, O.; Smith, S. P.; Lao, L. L.; Candy, J.; Snyder, P. B.; Belli, E. A.; Ferraro, N. M.; Prater, R.; Osborne, T. H.; Turnbull, A. D.; Staebler, G. M.] Gen Atom Co, San Diego, CA 92121 USA. [Izacard, O.; Izzo, V. A.; Holland, C.; Orlov, D. M.] Univ Calif San Diego, La Jolla, CA 92186 USA. [Ren, Q.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China. [Park, J. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Wang, Z.] Oak Ridge Inst Sci Educ, Oak Ridge, TN 37830 USA. [Luna, C. J.] Arizona State Univ, Phoenix, AZ 85004 USA. [Grierson, B. A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Penna, J.] MIT, Cambridge, MA 02139 USA. [Lu, G.] Univ Texas Austin, Austin, TX 78712 USA. [Raum, P.] Virginia Tech, Blacksburg, VA 24061 USA. [McCubbin, A.] Hope Coll, Holland, MI 49423 USA. [AToM Team] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Meneghini, O (reprint author), Gen Atom Co, San Diego, CA 92121 USA. EM meneghini@fusion.gat.com RI Orlov, Dmitriy/D-2406-2016; Izacard, Olivier/D-9670-2011 OI Orlov, Dmitriy/0000-0002-2230-457X; Izacard, Olivier/0000-0002-5949-8427 FU US Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FG02-95ER54309, DE-FG02-07ER54917, DE-AC05-00OR22725, DE-AC05-060R23100, DE-AC02-09CH1146, DE-FG02-06ER54871, DE-AC52-07NA27344] FX This material is based upon work supported in part by the US Department of Energy, Office of Science, Office of Fusion Energy Sciences, Theory Program, using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under awards DE-FG02-95ER54309, DE-FG02-07ER54917, DE-AC05-00OR22725, DE-AC05-060R23100, DE-AC02-09CH1146, DE-FG02-06ER54871, and DE-AC52-07NA27344. The authors would like to thank the the DIII-D team and all of the OMFIT users for their valuable feedback. The most up-to-date news, documentation, and publications relating to the OMFIT project can be found online at gafusion.github.io/OMFIT-source. NR 65 TC 6 Z9 6 U1 5 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 083008 DI 10.1088/0029-5515/55/8/083008 PG 13 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700008 ER PT J AU Paz-Soldan, C Logan, NC Lanctot, MJ Hanson, JM King, JD La Haye, RJ Nazikian, R Park, JK Strait, EJ AF Paz-Soldan, C. Logan, N. C. Lanctot, M. J. Hanson, J. M. King, J. D. La Haye, R. J. Nazikian, R. Park, J. -K. Strait, E. J. TI Decoupled recovery of energy and momentum with correction of n=2 error fields SO NUCLEAR FUSION LA English DT Article DE error fields; plasma response; resonant magnetic pertubations; neoclassical toroidal viscosity; density pumpout ID DIII-D; MAGNETIC-FIELDS; TOKAMAK PLASMAS; PERTURBATIONS; STABILITY; MODES AB Experiments applying known n = 2 'proxy' error fields (EFs) find that the rotation braking introduced by the proxy EF cannot be completely alleviated through optimal n = 2 correction with poorly matched poloidal spectra. This imperfect performance recovery demonstrates the importance of correcting multiple components of the n = 2 field spectrum and is in contrast to previous results with n = 1 EFs despite a similar execution. Measured optimal n = 2 proxy EF correction currents are consistent with those required to null dominant mode coupling to the resonant surfaces and minimize the neoclassical toroidal viscosity (NTV) torque, calculated using ideal MHD plasma response computation. Unlike rotation braking, density pumpout can be fully corrected despite poorly matched spectra, indicating density pumpout is driven only by a single component proportional to the resonant coupling. Through precise n = 2 spectral control density pumpout and rotation braking can thus be decoupled. Rotation braking with n = 2 fields is also found to be proportional to the level of co-current toroidal rotation, consistent with NTV theory. Plasmas with modest counter-current rotation are insensitive to the n = 2 field with neither rotation braking nor density pumpout observed. C1 [Paz-Soldan, C.; Lanctot, M. J.; King, J. D.; La Haye, R. J.; Strait, E. J.] Gen Atom Co, San Diego, CA 92186 USA. [Logan, N. C.; Nazikian, R.; Park, J. -K.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Hanson, J. M.] Columbia Univ, New York, NY 10027 USA. RP Paz-Soldan, C (reprint author), Gen Atom Co, POB 85608, San Diego, CA 92186 USA. EM paz-soldan@fusion.gat.com RI Lanctot, Matthew J/O-4979-2016 OI Lanctot, Matthew J/0000-0002-7396-3372 FU US Department of Energy, Office of Science, Office of Fusion Energy Sciences, using the DIII-D National Fusion Facility, a DOE Office of Science [DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-04ER54761, DE-AC05-06OR23100, DE-SC0001961, DE-AC05-00OR22725] FX This material is based upon work supported by the US Department of Energy, Office of Science, Office of Fusion Energy Sciences, using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under Awards DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-04ER54761, DE-AC05-06OR23100, DE-SC0001961, and DE-AC05-00OR22725. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D DMP. The authors wish to thank D.J. Battaglia, N.M. Ferraro, M. Okabayashi and F. Turco for operational support and useful discussions. NR 35 TC 9 Z9 9 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 083012 DI 10.1088/0029-5515/55/8/083012 PG 11 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700012 ER PT J AU Snyder, PB Solomon, WM Burrell, KH Garofalo, AM Grierson, BA Groebner, RJ Leonard, AW Nazikian, R Osborne, TH Belli, EA Candy, J Wilson, HR AF Snyder, P. B. Solomon, W. M. Burrell, K. H. Garofalo, A. M. Grierson, B. A. Groebner, R. J. Leonard, A. W. Nazikian, R. Osborne, T. H. Belli, E. A. Candy, J. Wilson, H. R. TI Super H-mode: theoretical prediction and initial observations of a new high performance regime for tokamak operation SO NUCLEAR FUSION LA English DT Article DE tokamak; pedestal; Super H-Mode; fusion performance; pedestal height; theoretical predictions; EPED AB A new 'Super H-mode' regime is predicted, which enables pedestal height and predicted fusion performance substantially higher than for H-mode operation. This new regime is predicted to exist by the EPED pedestal model, which calculates criticality constraints for peeling-ballooning and kinetic ballooning modes, and combines them to predict the pedestal height and width. EPED usually predicts a single ('H-mode') pedestal solution for each set of input parameters, however, in strongly shaped plasmas above a critical density, multiple pedestal solutions are found, including the standard 'H-mode' solution, and a 'Super H-Mode' solution at substantially larger pedestal height and width. The Super H-mode regime is predicted to be accessible by controlling the trajectory of the density, and to increase fusion performance for ITER, as well as for DEMO designs with strong shaping. A set of experiments on DIII-D has identified the predicted Super H-mode regime, and finds pedestal height and width, and their variation with density, in good agreement with theoretical predictions from the EPED model. The very high pedestal enables operation at high global beta and high confinement, including the highest normalized beta achieved on DIII-D with a quiescent edge. C1 [Snyder, P. B.; Burrell, K. H.; Garofalo, A. M.; Groebner, R. J.; Leonard, A. W.; Osborne, T. H.; Belli, E. A.; Candy, J.] Gen Atom Co, San Diego, CA 92186 USA. [Solomon, W. M.; Grierson, B. A.; Nazikian, R.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Wilson, H. R.] Univ York, York Plasma Inst, York YO10 5DD, N Yorkshire, England. RP Snyder, PB (reprint author), Gen Atom Co, POB 85608, San Diego, CA 92186 USA. EM snyder@fusion.gat.com OI Solomon, Wayne/0000-0002-0902-9876 FU U S Department of Energy, Office of Science, Office of Fusion Energy Sciences, Theory Program, using the DIII-D National Fusion Facility, a DOE Office of Science [DE-FG02-95ER54309, DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FC02-06ER54873] FX This material is based upon work supported in part by the U S Department of Energy, Office of Science, Office of Fusion Energy Sciences, Theory Program, using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under Awards DE-FG02-95ER54309, DE-FC02-04ER54698, DE-AC02-09CH11466, and DE-FC02-06ER54873. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. NR 16 TC 2 Z9 2 U1 1 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD AUG PY 2015 VL 55 IS 8 AR 083026 DI 10.1088/0029-5515/55/8/083026 PG 8 WC Physics, Fluids & Plasmas SC Physics GA CT5ES UT WOS:000362831700026 ER PT J AU Mieler, M Stojadinovic, B Budnitz, R Comerio, M Mahin, S AF Mieler, Michael Stojadinovic, Bozidar Budnitz, Robert Comerio, Mary Mahin, Stephen TI A Framework for Linking Community-Resilience Goals to Specific Performance Targets for the Built Environment SO EARTHQUAKE SPECTRA LA English DT Article ID KOBE EARTHQUAKE; RECOVERY AB An important task in the effort to improve the resilience of communities to both natural and manmade disasters involves rethinking the current approach for designing individual components within the built environment. In the United States, a patchwork of building codes and engineering standards results in a set of performance objectives for individual components that is often inadequate with respect to the broad principles of resilience. This paper outlines a conceptual framework that can be used to explicitly link community-level resilience goals to specific design targets for individual systems and components within the built environment. It then presents a proof-of-concept example that demonstrates how to derive a consistent performance target for individual residential buildings from a community-level resilience goal. Lastly, it discusses potential applications of the proposed framework, including a critical evaluation of current building codes to verify whether their target performance objectives are compatible with community-level resilience goals. C1 [Mieler, Michael; Mahin, Stephen] Johns Hopkins Univ, Dept Civil Engn, Baltimore, MD 21218 USA. [Stojadinovic, Bozidar] Swiss Fed Inst Technol, Dept Civil Environm & Geomat Engn, Zurich, Switzerland. [Budnitz, Robert] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Comerio, Mary] Univ Calif Berkeley, Dept Architecture, Berkeley, CA 94720 USA. RP Mieler, M (reprint author), Johns Hopkins Univ, Dept Civil Engn, Baltimore, MD 21218 USA. FU Department of Civil and Environmental Engineering at the University of California, Berkeley; Earth Sciences Division at the Lawrence Berkeley National Laboratory FX The authors would like to acknowledge the support of the Department of Civil and Environmental Engineering at the University of California, Berkeley, and the Earth Sciences Division at the Lawrence Berkeley National Laboratory in performing this work. The authors would also like to acknowledge the three anonymous reviewers for their valuable comments that helped improve this article. NR 25 TC 1 Z9 1 U1 3 U2 10 PU EARTHQUAKE ENGINEERING RESEARCH INST PI OAKLAND PA 499 14TH ST, STE 320, OAKLAND, CA 94612-1934 USA SN 8755-2930 EI 1944-8201 J9 EARTHQ SPECTRA JI Earthq. Spectra PD AUG PY 2015 VL 31 IS 3 BP 1267 EP 1283 DI 10.1193/082213EQS237M PG 17 WC Engineering, Civil; Engineering, Geological SC Engineering GA CS7YW UT WOS:000362303900003 ER PT J AU Dong, JJ Skinner, B Breecher, N Schmittmann, B Zia, RKP AF Dong, J. J. Skinner, B. Breecher, N. Schmittmann, B. Zia, R. K. P. TI Spatial structures in a simple model of population dynamics for parasite-host interactions SO EPL LA English DT Article ID EVOLUTION; STABILITY; DISCRETE AB Spatial patterning can be crucially important for understanding the behavior of interacting populations. Here we investigate a simple model of parasite and host populations in which parasites are random walkers that must come into contact with a host in order to reproduce. We focus on the spatial arrangement of parasites around a single host, and we derive using analytics and numerical simulations the necessary conditions placed on the parasite fecundity and lifetime for the populations long-term survival. We also show that the parasite population can be pushed to extinction by a large drift velocity, but, counterintuitively, a small drift velocity generally increases the parasite population. Copyright (C) EPLA, 2015 C1 [Dong, J. J.] Bucknell Univ, Dept Phys & Astron, Lewisburg, PA 17837 USA. [Skinner, B.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Breecher, N.] Univ Wisconsin, Dept Math Sci, Milwaukee, WI 53201 USA. [Schmittmann, B.; Zia, R. K. P.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Zia, R. K. P.] Virginia Polytech Inst & State Univ, Dept Phys, Blacksburg, VA 24061 USA. [Zia, R. K. P.] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. RP Dong, JJ (reprint author), Bucknell Univ, Dept Phys & Astron, Lewisburg, PA 17837 USA. EM jiajia.dong@bucknell.edu FU US National Science Foundation [DMR-1005417, DMR-1244666, DMR-1248387, PHY11-25915]; US Department of Energy, Office of Science [DE-AC02-06CH11357] FX 5 This research is supported in part by grants from the US National Science Foundation: DMR-1005417, DMR-1244666, DMR-1248387 and PHY11-25915. Work at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. JJD acknowledges the hospitality of Dr KEVIN BASSLER and Max Planck Institute for the Physics of Complex Systems, and the Kavli Institute for Theoretical Physics, where part of the work was performed. NR 20 TC 0 Z9 0 U1 4 U2 4 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD AUG PY 2015 VL 111 IS 4 AR 48001 DI 10.1209/0295-5075/111/48001 PG 6 WC Physics, Multidisciplinary SC Physics GA CS8SB UT WOS:000362357500029 ER PT J AU Ma, TX Lin, HQ Gubernatis, JE AF Ma, Tianxing Lin, Hai-Qing Gubernatis, J. E. TI Triplet p plus ip pairing correlations in the doped Kane-Mele-Hubbard model: A quantum Monte Carlo study SO EPL LA English DT Article ID FERMION GROUND-STATES; NUCLEON SYSTEMS; GRAPHENE; SUPERCONDUCTORS; COMPUTATION; GAS AB By using the constrained-phase quantum Monte Carlo method, we performed a systematic study of the pairing correlations in the ground state of the doped Kane-Mele-Hubbard model on a honeycomb lattice. We find that pairing correlations with d + id symmetry dominate close to half-filling, but pairing correlations with p + ip symmetry dominate as hole doping moves the system below three-quarters filling. We correlate these behaviors of the pairing correlations with the topology of the Fermi surfaces of the non-interacting problem. We also find that the effective pairing correlation is enhanced greatly as the interaction increases, and these superconducting correlations are robust against varying the spin-orbit coupling strength. Our numerical results suggest a possible way to realize spin triplet superconductivity in doped honeycomb-like materials or ultracold atoms in optical traps. Copyright (C) EPLA, 2015 C1 [Ma, Tianxing] Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China. [Ma, Tianxing; Lin, Hai-Qing] Beijing Computat Sci Res Ctr, Beijing 100094, Peoples R China. [Gubernatis, J. E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ma, TX (reprint author), Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China. RI Ma, Tianxing/D-1846-2012 FU NSCFs [11374034, 11334012, U1530401]; Fundamental Research Funds for the Central Universities [2014KJJCB26]; US Department of Energy FX We thank F. YANG, H. YAO and A. MURAMATSU for stimulating discussions. TM thanks CAEP for partial financial support. This work is supported by NSCFs (Grant Nos. 11374034, 11334012 and U1530401) and the Fundamental Research Funds for the Central Universities (Grant No. 2014KJJCB26). The work of JEG was supported by the US Department of Energy. NR 47 TC 5 Z9 5 U1 4 U2 4 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD AUG PY 2015 VL 111 IS 4 AR 47003 DI 10.1209/0295-5075/111/47003 PG 6 WC Physics, Multidisciplinary SC Physics GA CS8SB UT WOS:000362357500026 ER PT J AU Aguilar-Arevalo, A Amidei, D Bertou, X Bole, D Butner, M Cancelo, G Vazquez, AC Chavarria, AE Neto, JRTD Dixon, S D'Olivo, JC Estrada, J Moroni, GF Torres, KPH Izraelevitch, F Kavner, A Kilminster, B Lawson, I Liao, J Lopez, M Molina, J Moreno-Granados, G Pena, J Privitera, P Sarkis, Y Scarpine, V Schwarz, T Haro, MS Tiffenberg, J Machado, DT Trillaud, F You, X Zhou, J AF Aguilar-Arevalo, A. Amidei, D. Bertou, X. Bole, D. Butner, M. Cancelo, G. Castaneda Vazquez, A. Chavarria, A. E. de Mello Neto, J. R. T. Dixon, S. D'Olivo, J. C. Estrada, J. Moroni, G. Fernandez Hernandez Torres, K. P. Izraelevitch, F. Kavner, A. Kilminster, B. Lawson, I. Liao, J. Lopez, M. Molina, J. Moreno-Granados, G. Pena, J. Privitera, P. Sarkis, Y. Scarpine, V. Schwarz, T. Sofo Haro, M. Tiffenberg, J. Torres Machado, D. Trillaud, F. You, X. Zhou, J. CA DAMIC Collaboration TI Measurement of radioactive contamination in the high-resistivity silicon CCDs of the DAMIC experiment SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Search for radioactive and fissile materials; Solid state detectors; Very low-energy charged particle detectors; Dark Matter detectors (WIMPs, axions, etc.) ID DARK-MATTER AB We present measurements of radioactive contamination in the high-resistivity silicon charge-coupled devices (CCDs) used by the DAMIC experiment to search for dark matter particles. Novel analysis methods, which exploit the unique spatial resolution of CCDs, were developed to identify alpha and beta particles. Uranium and thorium contamination in the CCD bulk was measured through alpha spectroscopy, with an upper limit on the U-238 (Th-232) decay rate of 5 (15) kg(-1) d(-1) at 95% CL. We also searched for pairs of spatially correlated electron tracks separated in time by up to tens of days, as expected from Si-32-P-32 or Pb-210-Bi-210 sequences of beta decays. The decay rate of Si-32 was found to be 80(-65)(+110) kg(-1) d(-1) (95% CI). An upper limit of similar to 35 kg(-1) d(-1) (95% CL) on the Pb-210 decay rate was obtained independently by a spectroscopy and the beta decay sequence search. These levels of radioactive contamination are sufficiently low for the successful operation of CCDs in the forthcoming 100 g DAMIC detector. C1 [Aguilar-Arevalo, A.; Castaneda Vazquez, A.; D'Olivo, J. C.; Hernandez Torres, K. P.; Moreno-Granados, G.; Sarkis, Y.; Trillaud, F.] Univ Nacl Autonoma Mexico, Mexico City 04510, DF, Mexico. [Amidei, D.; Bole, D.; Kavner, A.; Schwarz, T.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Bertou, X.; Sofo Haro, M.] Consejo Nacl Invest Cient & Tecn, CNEA, Ctr Atom Bariloche, Inst Balseiro, RA-1033 Buenos Aires, DF, Argentina. [Butner, M.; Cancelo, G.; Estrada, J.; Moroni, G. Fernandez; Izraelevitch, F.; Scarpine, V.; Tiffenberg, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Chavarria, A. E.; Dixon, S.; Pena, J.; Privitera, P.; Zhou, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Chavarria, A. E.; Dixon, S.; Pena, J.; Privitera, P.; Zhou, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [de Mello Neto, J. R. T.; Torres Machado, D.; You, X.] Univ Fed Rio de Janeiro, Inst Fis, Rio De Janeiro, RJ, Brazil. [Kilminster, B.; Liao, J.] Univ Zurich, Inst Phys, Zurich, Switzerland. [Lawson, I.] SNOLAB, Lively, ON, Canada. [Lopez, M.; Molina, J.] Univ Nacl Asunc, Fac Ingn, Asuncion, Paraguay. [Butner, M.] No Illinois Univ, De Kalb, IL 60115 USA. RP Chavarria, AE (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. EM alvaro@kicp.uchicago.edu RI de Mello Neto, Joao/C-5822-2013; OI de Mello Neto, Joao/0000-0002-3234-6634; Aguilar-Arevalo, Alexis A./0000-0001-9279-3375 FU Kavli Institute for Cosmological Physics at the University of Chicago [NSF PHY-1125897]; endowment from the Kavli Foundation; Natural Sciences and Engineering Research Council of Canada; Ontario Ministry of Research and Innovation; Northern Ontario Heritage Fund; Canada Foundation for Innovation; DGAPA-UNAM [IN112213, IB100413]; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico [240666]; Swiss National Science Foundation [153654]; Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (CAPES); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ) FX The DAMIC Collaboration would like to thank SNOLAB and its staff for providing underground laboratory space and outstanding technical support, and Vale S.A. for hosting SNOLAB. We thank G. E. Derylo and K. R. Kuk for their contributions to the design, construction and installation of the detector. We are grateful to the following agencies and organizations for financial support: Kavli Institute for Cosmological Physics at the University of Chicago through grant NSF PHY-1125897 and an endowment from the Kavli Foundation, the Natural Sciences and Engineering Research Council of Canada, the Ontario Ministry of Research and Innovation, the Northern Ontario Heritage Fund, the Canada Foundation for Innovation, DGAPA-UNAM through grants PAPIIT No. IN112213 and No. IB100413, Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico, through grant No. 240666, the Swiss National Science Foundation through grant 153654, and the Brazilian agencies Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (CAPES), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) and Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ). NR 17 TC 3 Z9 3 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR P08014 DI 10.1088/1748-0221/10/08/P08014 PG 20 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700033 ER PT J AU Bubna, M Bortoletto, D Bolla, G Shipsey, I Manfra, MJ Khan, K Arndt, K Hinton, N Godshalk, A Kumar, A Menasce, D Moroni, L Chramowicz, J Lei, CM Prosser, A Rivera, R Uplegger, L Lo Vetere, M Robutti, E Ferro, F Ravera, F Costa, M AF Bubna, M. Bortoletto, D. Bolla, G. Shipsey, I. Manfra, M. J. Khan, K. Arndt, K. Hinton, N. Godshalk, A. Kumar, A. Menasce, D. Moroni, L. Chramowicz, J. Lei, C. M. Prosser, A. Rivera, R. Uplegger, L. Lo Vetere, M. Robutti, E. Ferro, F. Ravera, F. Costa, Marco CA CMS Tracker Collaboration TI Laboratory and testbeam results for thin and epitaxial planar sensors for HL-LHC SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT International Workshop on Semiconductor Pixel Detectors for Particles and Imaging (PIXEL) CY SEP 01-05, 2014 CL Niagara Falls, CANADA DE Radiation-hard detectors; Particle tracking detectors (Solid-state detectors); Instrumentation for particle accelerators and storage rings - high energy (linear accelerators, synchrotrons) ID CMS PIXEL DETECTOR; SILICON SENSORS; READOUT CHIP; SYSTEM AB The High-Luminosity LHC (HL-LHC) upgrade of the CMS pixel detector will require the development of novel pixel sensors which can withstand the increase in instantaneous luminosity to L = 5 x 1034 cm(-2)s(-1) and collect similar to 3000 fb(-1) of data. The innermost layer of the pixel detector will be exposed to doses of about 10(16) n(eq)/cm(2). Hence, new pixel sensors with improved radiation hardness need to be investigated. A variety of silicon materials (Float-zone, Magnetic Czochralski and Epitaxially grown silicon), with thicknesses from 50 mu m to 320 mu m in p-type and n-type substrates have been fabricated using single-sided processing. The effect of reducing the sensor active thickness to improve radiation hardness by using various techniques (deep diffusion, wafer thinning, or growing epitaxial silicon on a handle wafer) has been studied. The results for electrical characterization, charge collection efficiency, and position resolution of various n-on-p pixel sensors with different substrates and different pixel geometries (different bias dot gaps and pixel implant sizes) will be presented. C1 [Bubna, M.; Bortoletto, D.; Bolla, G.; Shipsey, I.; Manfra, M. J.; Khan, K.; Arndt, K.; Hinton, N.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Godshalk, A.; Kumar, A.] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. [Menasce, D.] INFN Milano Bicocca, I-20133 Milan, Italy. [Moroni, L.] Univ Milano Bicocca, I-20126 Milan, Italy. [Moroni, L.] INFN Milano Bicocca, I-20126 Milan, Italy. [Bolla, G.; Chramowicz, J.; Lei, C. M.; Prosser, A.; Rivera, R.; Uplegger, L.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Lo Vetere, M.; Robutti, E.; Ferro, F.] INFN Genova, I-16146 Genoa, Italy. [Lo Vetere, M.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Ravera, F.; Costa, Marco] Univ Torino, I-10125 Turin, Italy. [Ravera, F.; Costa, Marco] INFN Sez Torino, I-10125 Turin, Italy. [Bubna, M.; Manfra, M. J.] Purdue Univ, Dept Elect & Comp Engn, W Lafayette, IN 47907 USA. [Bubna, M.; Manfra, M. J.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Manfra, M. J.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. RP Bubna, M (reprint author), Purdue Univ, Dept Phys & Astron, 525 Northwestern Ave, W Lafayette, IN 47907 USA. EM mbubna@purdue.edu RI Menasce, Dario/A-2168-2016; OI Menasce, Dario/0000-0002-9918-1686; Arndt, Kirk/0000-0002-6826-8340 NR 13 TC 1 Z9 1 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR C08002 DI 10.1088/1748-0221/10/08/C08002 PG 13 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700002 ER PT J AU Carls, B Horton-Smith, G James, CC Kubinski, RM Pordes, S Schukraft, A Strauss, T AF Carls, B. Horton-Smith, G. James, C. C. Kubinski, R. M. Pordes, S. Schukraft, A. Strauss, T. TI Design and operation of a setup with a camera and adjustable mirror to inspect the sense-wire planes of the Time Projection Chamber inside the MicroBooNE cryostat SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Time projection chambers; Detector design and construction technologies and materials; Cryogenic detectors AB Detectors in particle physics, particularly when including cryogenic components, are often enclosed in vessels that do not provide any physical or visual access to the detectors themselves after installation. However, it can be desirable for experiments to visually investigate the inside of the vessel. The MicroBooNE cryostat hosts a TPC with sense-wire planes, which had to be inspected for damage such as breakage or sagging. This inspection was performed after the transportation of the vessel with the enclosed detector to its final location, but before filling with liquid argon. This paper describes an approach to view the inside of the MicroBooNE cryostat with a setup of a camera and a mirror through one of its cryogenic service nozzles. The paper describes the camera and mirror chosen for the operation, the illumination, and the mechanical structure of the setup. It explains how the system was operated and demonstrates its performance. C1 [Carls, B.; James, C. C.; Kubinski, R. M.; Pordes, S.; Schukraft, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Horton-Smith, G.] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA. [Strauss, T.] Univ Bern, LHEP, CH-3012 Bern, Switzerland. RP Schukraft, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM aschu@fnal.gov FU United States Department of Energy [DE-AC02-07CH11359] FX We would like to acknowledge mechanical support by Patrick Healey and Peter Simon, as well as Keith Anderson for exploring the possibility of using a borescope. We thank Reidar Hahn of Fermilab's Visual Media Services for assistance in selecting and operating the camera. We thank the Fermilab Alignment and Metrology Department for assistance with the calibration of the mirror. We would like to thank the MicroBooNE collaboration for providing test setups and help with the analysis of photographs. Fermilab is operated by the Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 2 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR T08006 DI 10.1088/1748-0221/10/08/T08006 PG 15 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700042 ER PT J AU Chen, K Chen, H Kierstead, J Takai, H Rescia, S Hu, X Xu, H Mead, J Lanni, F Minelli, M AF Chen, K. Chen, H. Kierstead, J. Takai, H. Rescia, S. Hu, X. Xu, H. Mead, J. Lanni, F. Minelli, M. TI Evaluation of commercial ADC radiation tolerance for accelerator experiments SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Radiation damage evaluation methods; Data acquisition circuits; Radiation-hard electronics; Front-end electronics for detector readout ID SINGLE EVENT UPSET; DEVICES; DAMAGE; NIEL; SRAM AB Electronic components used in high energy physics experiments are subjected to a radiation background composed of high energy hadrons, mesons and photons. These particles can induce permanent and transient effects that affect the normal device operation. Ionizing dose and displacement damage can cause chronic damage which disable the device permanently. Transient effects or single event effects are in general recoverable with time intervals that depend on the nature of the failure. The magnitude of these effects is technology dependent with feature size being one of the key parameters. Analog to digital converters are components that are frequently used in detector front end electronics, generally placed as close as possible to the sensing elements to maximize signal fidelity. We report on the development of a technique for testing analog to digital converters for radiation effects, in particular for single event effects. A total of seventeen commercial ADCs were evaluated for ionizing dose tolerance and extensive SEU measurements performed on a twelve and fourteen bit ADCs. Mitigation strategies for single event effects (SEE) are discussed for their use in the large hadron collider environment. C1 [Chen, K.; Chen, H.; Kierstead, J.; Takai, H.; Rescia, S.; Hu, X.; Xu, H.; Mead, J.; Lanni, F.; Minelli, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Takai, H (reprint author), Brookhaven Natl Lab, POB 5000, Upton, NY 11973 USA. EM takai@bnl.gov FU Unites States Department of Energy [DE-AC02-98CH10886] FX We acknowledge the excellent service and help provided by Mr. E. Cascio at the MGH facility, Dr. B. von Przewoski at IUCF and Dr. S. Wender at LANSCE. Their expert guidance was invaluable in the execution of single event upset tests. This work was supported in part by the Unites States Department of Energy Contract No. DE-AC02-98CH10886. NR 20 TC 2 Z9 2 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR P08009 DI 10.1088/1748-0221/10/08/P08009 PG 17 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700028 ER PT J AU Choong, WS Abu-Nimeh, F Moses, WW Peng, Q Vu, CQ Wu, JY AF Choong, W. -S. Abu-Nimeh, F. Moses, W. W. Peng, Q. Vu, C. Q. Wu, J. -Y. TI A front-end readout Detector Board for the OpenPET electronics system SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Front-end electronics for detector readout; Analogue electronic circuits; Gamma camera, SPECT, PET PET/CT, coronary CT angiography (CTA); Digital electronic circuits ID RESOLUTION AB We present a 16-channel front-end readout board for the OpenPET electronics system. A major task in developing a nuclear medical imaging system, such as a positron emission computed tomograph (PET) or a single-photon emission computed tomograph (SPECT), is the electronics system. While there are a wide variety of detector and camera design concepts, the relatively simple nature of the acquired data allows for a common set of electronics requirements that can be met by a flexible, scalable, and high-performance OpenPET electronics system. The analog signals from the different types of detectors used in medical imaging share similar characteristics, which allows for a common analog signal processing. The OpenPET electronics processes the analog signals with Detector Boards. Here we report on the development of a 16-channel Detector Board. Each signal is digitized by a continuously sampled analog-to-digital converter (ADC), which is processed by a field programmable gate array (FPGA) to extract pulse height information. A leading edge discriminator creates a timing edge that is "time stamped" by a time-to-digital converter (TDC) implemented inside the FPGA. This digital information from each channel is sent to an FPGA that services 16 analog channels, and then information from multiple channels is processed by this FPGA to perform logic for crystal lookup, DOI calculation, calibration, etc. C1 [Choong, W. -S.; Abu-Nimeh, F.; Moses, W. W.; Peng, Q.; Vu, C. Q.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Wu, J. -Y.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Choong, WS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM wschoong@lbl.gov FU Office of Science, Office of Biological and Environmental Research, Medical Science Division, U.S. Department of Energy [DE-AC02-05CH11231]; National Institutes of Health, National Institute of Biomedical Imaging and Bioengineering [R01EB016104] FX This work was supported in part by the Director, Office of Science, Office of Biological and Environmental Research, Medical Science Division, U.S. Department of Energy under contract DE-AC02-05CH11231, and in part by the National Institutes of Health, National Institute of Biomedical Imaging and Bioengineering, under Grant Number R01EB016104. NR 10 TC 0 Z9 0 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR T08002 DI 10.1088/1748-0221/10/08/T08002 PG 13 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700038 ER PT J AU Fisher-Levine, M Nomerotski, A AF Fisher-Levine, M. Nomerotski, A. TI Characterising CCDs with cosmic rays SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Photon detectors for UV visible and IR photons (solid-state) (PIN diodes, APDs, Si-PMTs, G-APDs, CCDs, EBCCDs, EMCCDs etc); Instrument optimisation AB The properties of cosmic ray muons make them a useful probe for measuring the properties of thick, fully depleted CCD sensors. The known energy deposition per unit length allows measurement of the gain of the sensor's amplifiers, whilst the straightness of the tracks allows for a crude assessment of the static lateral electric fields at the sensor's edges. Furthermore, the small volume in which the muons deposit their energy allows measurement of the contribution to the PSF from the diffusion of charge as it drifts across the sensor. In this work we present a validation of the cosmic ray gain measurement technique by comparing with radioisotope gain measurments, and calculate the charge diffusion coefficient for prototype LSST sensors. C1 [Fisher-Levine, M.; Nomerotski, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fisher-Levine, M (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM mfisherlevine@bnl.gov RI Nomerotski, Andrei/A-5169-2010 NR 14 TC 0 Z9 0 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR C08006 DI 10.1088/1748-0221/10/08/C08006 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700006 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-conde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Fagot, A Garcia, G Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Molina, J Herrera, CM Pol, ME Teles, PR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zhang, L Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Chapon, E Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Edelhoff, M Feld, L Heister, A Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Sammet, J Schael, S Schulte, JF Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behr, J Behrens, U Bell, AJ Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Krucker, D Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Roland, B Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trevino, ADRV Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Kirschenmann, H Klanner, R Kogler, R Lapsien, T Lenz, T Marchesini, I Marconi, D Ott, J Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Poehlsen, T Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Vanhoefer, A Barth, C Baus, C Berger, J Boser, C Butz, E 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Halkiadakis, E. Hidas, D. Kaplan, S. Lath, A. Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Suarez, I. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Performance of photon reconstruction and identification with the CMS detector in proton-proton collisions at root s=8TeV SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Pattern recognition; cluster finding; calibration and fitting methods; Performance of High Energy Physics Detectors ID CALORIMETER; ELECTRONS; CRYSTALS; ENERGY; TEV AB A description is provided of the performance of the CMS detector for photon reconstruction and identification in proton-proton collisions at a centre-of-mass energy of 8 TeV at the CERN LHC. Details are given on the reconstruction of photons from energy deposits in the electromagnetic calorimeter (ECAL) and the extraction of photon energy estimates. The reconstruction of electron tracks from photons that convert to electrons in the CMS tracker is also described, as is the optimization of the photon energy reconstruction and its accurate modelling in simulation, in the analysis of the Higgs boson decay into two photons. In the barrel section of the ECAL, an energy resolution of about 1% is achieved for unconverted or late-converting photons from H -> gamma gamma decays. Different photon identification methods are discussed and their corresponding selection efficiencies in data are compared with those found in simulated events. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Dobur, D.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Leonard, A.; Mohammadi, A.; Pernie, L.; Randle-conde, A.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.; Zenoni, F.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Fagot, A.; Garcia, G.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Nuttens, C.; Pagano, D.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Dos Reis Martins, T.; Molina, J.; Mora Herrera, C.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dogra, S.; Fernandez Perez Tomei, T. R.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Hadjiiska, R.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Tao, J.; Wang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Sierra, L. F. Chaparro; Florez, C.; Gomez, J. P.; Moreno, B. Gomez; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Kamel, A. Ellithi; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Baffioni, S.; Beaudette, F.; Busson, P.; Chapon, E.; Charlot, C.; Dalchenko, M.; Dobrzynski, L.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Veelken, C.; Yilmaz, Y.; Zabi, A.; Dahmes, B.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, CNRS, IN2P3, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Bernet, C.; Boudoul, G.; Bouvier, E.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS, Inst Phys Nucl Lyon, CNRS,IN2P3, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Edelhoff, M.; Feld, L.; Heister, A.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Sammet, J.; Schael, S.; Schulte, J. F.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behr, J.; Behrens, U.; Bell, A. J.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Ron, E.; Sahin, M. Oe; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Tziaferi, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Banerjee, S.; Aziz, T.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Bisello, D.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Fantinel, S.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kaminskiy, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Naegeli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Xiao, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bierwagen, K.; Busza, W.; Cali, I. A.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.; Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Verzetti, M.; Vishnevskiy, D.] Univ Rochester, Rochester, NY USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. 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[Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Yang, Yong/D-9724-2017; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; VARDARLI, Fuat Ilkehan/B-6360-2013; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012 OI Gerosa, Raffaele/0000-0001-8359-3734; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Gallinaro, Michele/0000-0003-1261-2277; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Silvestris, Lucia/0000-0002-8985-4891; Boccali, Tommaso/0000-0002-9930-9299; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research of Thailand; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science - European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis - EU-ESF; Aristeia - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 40 TC 6 Z9 6 U1 7 U2 34 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR P08010 DI 10.1088/1748-0221/10/08/P08010 PG 60 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700029 ER PT J AU Okura, Y Plazas, AA May, M Tamagawa, T AF Okura, Y. Plazas, A. A. May, M. Tamagawa, T. TI Spurious shear induced by the tree rings of the LSST CCDs SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Image processing; Photon detectors for UV, visible and IR photons (solid-state) (PIN diodes, APDs, Si-PMTs, G-APDs, CCDs, EBCCDs, EMCCDs etc) ID WEAK LENSING SURVEYS; DARK ENERGY SURVEY; CALIBRATION AB We present an analysis of the impact of the tree rings seen in the candidate sensors of the Large Synoptic Survey Telescope (LSST) on galaxy-shape measurements. The tree rings are a consequence of transverse electric fields caused by circularly symmetric impurity gradients in the silicon of the sensors. They effectively modify the pixel area and shift the photogenerated charge around, displacing the observed photon positions. The displacement distribution generates distortions that cause spurious shears correlated with the tree-rings patterns, potentially biasing cosmic shear measurements. In this paper we quantify the amplitude of the spurious shear caused by the tree rings on the LSST candidate sensors, and calculate its 2-point correlation function. We find that 2-point correlation function of the spurious shear on an area equivalent to the LSST field of view is order of about 10 13, providing a negligible contribution to the 2-point correlation of the cosmic shear signal. Additional work is underway, and the final results and analysis will be published elsewhere (Okura et al. (2015), in prep.) C1 [Okura, Y.; Tamagawa, T.] RIKEN, Wako, Saitama 3510198, Japan. [Okura, Y.] Brookhaven Natl Lab, Dept Phys, RIKEN BNL Res Ctr, Upton, NY 11792 USA. [Plazas, A. A.; May, M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11792 USA. [Plazas, A. A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Okura, Y (reprint author), RIKEN, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. EM yuki.okura@riken.jp FU U.S. Department of Energy [DE-AC02-98CH10886, DE-SC0012704]; JPL; NASA FX We thank G. Bernstein and P. O'Connor for useful comments and discussions. This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886 and Contract No. DE-SC0012704. AAP is also supported by JPL, which is run under a contract for NASA by Caltech. NR 14 TC 1 Z9 1 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR C08010 DI 10.1088/1748-0221/10/08/C08010 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700010 ER PT J AU Yoo, J Jaskierny, WF AF Yoo, J. Jaskierny, W. F. TI Electron drift in a large scale solid xenon SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Charge transport and multiplication in solid media; Cryogenic detectors; Time projection chambers ID AR KR; LIQUID; ARGON; XE; SCINTILLATORS; LUMINESCENCE; PARTICLE; KRYPTON AB A study of charge drift in a large scale optically transparent solid xenon is reported. A pulsed high power xenon light source is used to liberate electrons from a photocathode. The drift speeds of the electrons are measured using a 8.7 cm long electrode in both the liquid and solid phase of xenon. In the liquid phase (163 K), the drift speed is 0.193 +/- 0.003 cm/mu s while the drift speed in the solid phase (157 K) is 0.397 +/- 0.006 cm/mu s at 900 V/cm over 8.0 cm of uniform electric fields. Therefore, it is demonstrated that a factor two faster electron drift speed in solid phase xenon compared to that in liquid in a large scale solid xenon. C1 [Yoo, J.; Jaskierny, W. F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Yoo, J (reprint author), Fermilab Natl Accelerator Lab, Kirk & Pine St, Batavia, IL 60510 USA. EM yoo@fnal.gov RI Yoo, Jonghee/K-8394-2016 FU Department Of Energy Advanced Detector RD funding FX We are very grateful to M. Miyajima, J. White, and A. Bolozdnya for the initial discussions of the solid xenon particle detector and sharing their ideas. We would like to thank the Fermilab technical staff who aided in the design and construction of the apparatus. This work supported by the Department Of Energy Advanced Detector R&D funding. NR 28 TC 1 Z9 1 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD AUG PY 2015 VL 10 AR P08011 DI 10.1088/1748-0221/10/08/P08011 PG 12 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS8ZP UT WOS:000362378700030 ER PT J AU Huang, R Su, P Burge, JH Huang, L Idir, M AF Huang, Run Su, Peng Burge, James H. Huang, Lei Idir, Mourad TI High-accuracy aspheric x-ray mirror metrology using Software Configurable Optical Test System/deflectometry SO OPTICAL ENGINEERING LA English DT Article DE optics; metrology; deflectometry; calibration; x-ray optics; interferometry ID ORTHONORMAL VECTOR POLYNOMIALS; MEASURING DEFLECTOMETRY; UNIT-CIRCLE; BASIS-SET AB The Software Configurable Optical Test System (SCOTS) uses deflectometry to measure surface slopes of general optical shapes without the need for additional null optics. Careful alignment of test geometry and calibration of inherent system error improve the accuracy of SCOTS to a level where it competes with interferometry. We report a SCOTS surface measurement of an off-axis superpolished elliptical x-ray mirror that achieves <1 nm root-mean-square accuracy for the surface measurement with low-order term included. (C) 2015 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Huang, Run; Su, Peng; Burge, James H.] Univ Arizona, Coll Opt Sci, Tucson, AZ 85721 USA. [Huang, Lei; Idir, Mourad] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Huang, R (reprint author), Univ Arizona, Coll Opt Sci, 1630 East Univ Blvd, Tucson, AZ 85721 USA. EM rhuang@optics.arizona.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC-02-98CH10886] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC-02-98CH10886. NR 29 TC 8 Z9 8 U1 5 U2 8 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 0091-3286 EI 1560-2303 J9 OPT ENG JI Opt. Eng. PD AUG PY 2015 VL 54 IS 8 AR 084103 DI 10.1117/1.OE.54.8.084103 PG 10 WC Optics SC Optics GA CT0SN UT WOS:000362507000017 ER PT J AU Kontou, E Yin, YF Lin, ZH AF Kontou, Eleftheria Yin, Yafeng Lin, Zhenhong TI Socially optimal electric driving range of plug-in hybrid electric vehicles SO TRANSPORTATION RESEARCH PART D-TRANSPORT AND ENVIRONMENT LA English DT Article DE Plug-in hybrid electric vehicle (PHEV); Optimal all-electric driving range; Minimum social cost; Recharging opportunities ID GREENHOUSE-GAS EMISSIONS; LIFE-CYCLE COST; CHARGING INFRASTRUCTURE; CONSUMPTION; IMPACT AB This study determines the optimal electric driving range of plug-in hybrid electric vehicles (PHEVs) that minimizes the daily cost borne by the society when using this technology. An optimization framework is developed and applied to datasets representing the US market. Results indicate that the optimal range is 16 miles with an average social cost of $3.19 per day when exclusively charging at home, compared to $3.27 per day of driving a conventional vehicle. The optimal range is found to be sensitive to the cost of battery packs and the price of gasoline. When workplace charging is available, the optimal electric driving range surprisingly increases from 16 to 22 miles, as larger batteries would allow drivers to better take advantage of the charging opportunities to achieve longer electrified travel distances, yielding social cost savings. If workplace charging is available, the optimal density is to deploy a workplace charger for every 3.66 vehicles. Moreover, the diversification of the battery size, i.e., introducing a pair and triple of electric driving ranges to the market, could further decrease the average societal cost per PHEV by 7.45% and 11.5% respectively. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Kontou, Eleftheria; Yin, Yafeng] Univ Florida, Dept Civil & Coastal Engn, Gainesville, FL 32611 USA. [Lin, Zhenhong] Oak Ridge Natl Lab, Knoxville, TN 37932 USA. RP Yin, YF (reprint author), Univ Florida, Dept Civil & Coastal Engn, Gainesville, FL 32611 USA. EM yafeng@ufl.edu OI Kontou, Eleftheria/0000-0003-1367-4226 FU U.S. National Science Foundation [CNS-1239364]; National Natural Science Foundation of China [71228101]; Lloyd's Register Foundation (LRF) FX The work described in this paper was partly supported by the U.S. National Science Foundation (CNS-1239364) and National Natural Science Foundation of China (71228101). We would also like to thank the support from Lloyd's Register Foundation (LRF). LRF helps to protect life and property by supporting engineering-related education, public engagement and the application of research. Lin acknowledges U.S. Department of Energy's Vehicle Technologies Office. The authors would like to thank three anonymous reviewers for their comments and suggestions. NR 32 TC 1 Z9 1 U1 4 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1361-9209 J9 TRANSPORT RES D-TR E JI Transport. Res. Part D-Transport. Environ. PD AUG PY 2015 VL 39 BP 114 EP 125 DI 10.1016/j.trd.2015.07.002 PG 12 WC Environmental Studies; Transportation; Transportation Science & Technology SC Environmental Sciences & Ecology; Transportation GA CS9BI UT WOS:000362383700009 ER PT J AU Dambournet, D Chapman, KW Duttine, M Borkiewicz, O Chupas, PJ Groult, H AF Dambournet, Damien Chapman, Karena W. Duttine, Mathieu Borkiewicz, Olaf Chupas, Peter J. Groult, Henri TI Lithium Insertion Mechanism in Iron-Based Oxyfluorides with Anionic Vacancies Probed by PDF Analysis SO CHEMISTRYOPEN LA English DT Article DE anionic partitioning; cathode materials; ferric fluoride; pair distribution function ID ION BATTERIES; ELECTRODE MATERIALS; CONVERSION REACTION; LI BATTERIES; FLUORIDE; NANOCOMPOSITE; LITHIATION; NMR AB The mechanism of lithium insertion that occurs in an iron oxyfluoride sample with a hexagonal-tungsten-bronze (HTB)-type structure was investigated by the pair distribution function. This study reveals that upon lithiation, the HTB framework collapses to yield disordered rutile and rock salt phases followed by a conversion reaction of the fluoride phase toward lithium fluoride and nanometer-sized metallic iron. The occurrence of anionic vacancies in the pristine framework was shown to strongly impact the electrochemical activity, that is, the reversible capacity scales with the content of anionic vacancies. Similar to FeOF-type electrodes, upon de-lithiation, a disordered rutile phase forms, showing that the anionic chemistry dictates the atomic arrangement of the re-oxidized phase. Finally, it was shown that the nanoscaling and structural rearrangement induced by the conversion reaction allow the in situ formation of new electrode materials with enhanced electrochemical properties. C1 [Dambournet, Damien; Duttine, Mathieu; Groult, Henri] Univ Paris 06, Sorbonne Univ, UMR 8234, PHENIX, F-75005 Paris, France. [Dambournet, Damien; Duttine, Mathieu; Groult, Henri] CNRS, UMR 8234, PHENIX, F-75005 Paris, France. [Chapman, Karena W.; Borkiewicz, Olaf; Chupas, Peter J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Duttine, Mathieu] Univ Bordeaux, CNRS, ICMCB, UPR 9048, F-33600 Pessac, France. RP Dambournet, D (reprint author), Univ Paris 06, Sorbonne Univ, UMR 8234, PHENIX, F-75005 Paris, France. EM damien.dambournet@upmc.fr FU U.S. DOE [DE-AC02-06CH11357]; European Union [321879]; Hydro-Quebec Company FX Work performed at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, were supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Research leading to these results received funding from the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme (FP7/2007-2013) under REA grant agreement no. [321879] (FLUOSYNES) and from the Hydro-Quebec Company. NR 24 TC 2 Z9 2 U1 9 U2 40 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2191-1363 J9 CHEMISTRYOPEN JI ChemistryOpen PD AUG PY 2015 VL 4 IS 4 BP 443 EP 447 DI 10.1002/open.201500031 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CS6LY UT WOS:000362191700004 PM 26478837 ER PT J AU Miller, EK AF Miller, Edmund K. TI Adaptive Sparse Sampling to Estimate Radiation and Scattering Patterns to a Specified Uncertainty with Model-Based Parameter Estimation Compute patterns using as few as two to four samples per lobe. SO IEEE ANTENNAS AND PROPAGATION MAGAZINE LA English DT Article ID INTERPOLATION; FIELDS C1 [Miller, Edmund K.] Univ Michigan, Radiat & High Altitude Engn Labs, Ann Arbor, MI 48109 USA. Lawrence Livermore Natl Lab, Livermore, CA USA. Los Alamos Natl Lab, Los Alamos, NM USA. [Miller, Edmund K.] Michigan Technol Univ, Phys, Houghton, MI 49931 USA. RP Miller, EK (reprint author), Univ Michigan, Radiat & High Altitude Engn Labs, Ann Arbor, MI 48109 USA. EM e.miller@ieee.org NR 14 TC 1 Z9 1 U1 1 U2 9 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1045-9243 EI 1558-4143 J9 IEEE ANTENN PROPAG M JI IEEE Antennas Propag. Mag. PD AUG PY 2015 VL 57 IS 4 BP 103 EP 113 DI 10.1109/MAP.2015.2453920 PG 11 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA CS3YJ UT WOS:000362011400009 ER PT J AU Daub, EG Trugman, DT Johnson, PA AF Daub, Eric G. Trugman, Daniel T. Johnson, Paul A. TI Statistical tests on clustered global earthquake synthetic data sets SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE earthquake hazard; statistical seismology; earthquake clustering; earthquake interaction ID GREAT EARTHQUAKES; AFTERSHOCKS; MAGNITUDE; TIME; DEFORMATIONS; CALIFORNIA; SEQUENCE; CATALOGS; RELEASE; STRESS AB We study the ability of statistical tests to identify nonrandom features of earthquake catalogs, with a focus on the global earthquake record since 1900. We construct four types of synthetic data sets containing varying strengths of clustering, with each data set containing on average 10,000 events over 100years with magnitudes above M = 6. We apply a suite of statistical tests to each synthetic realization in order to evaluate the ability of each test to identify the sequences of events as nonrandom. Our results show that detection ability is dependent on the quantity of data, the nature of the type of clustering, and the specific signal used in the statistical test. Data sets that exhibit a stronger variation in the seismicity rate are generally easier to identify as nonrandom for a given background rate. We also show that we can address this problem in a Bayesian framework, with the clustered data sets as prior distributions. Using this new Bayesian approach, we can place quantitative bounds on the range of possible clustering strengths that are consistent with the global earthquake data. At M = 7, we can estimate 99th percentile confidence bounds on the number of triggered events, with an upper bound of 20% of the catalog for global aftershock sequences, with a stronger upper bound on the fraction of triggered events of 10% for long-term event clusters. At M = 8, the bounds are less strict due to the reduced number of events. However, our analysis shows that other types of clustering could be present in the data that we are unable to detect. Our results aid in the interpretation of the results of statistical tests on earthquake catalogs, both worldwide and regionally. C1 [Daub, Eric G.] Univ Memphis, Ctr Earthquake Res & Informat, Memphis, TN 38152 USA. [Trugman, Daniel T.; Johnson, Paul A.] Los Alamos Natl Lab, Geophys Grp, Los Alamos, NM USA. [Trugman, Daniel T.] Univ Calif San Diego, Scripps Inst Oceanog, San Diego, CA 92103 USA. RP Daub, EG (reprint author), Univ Memphis, Ctr Earthquake Res & Informat, Memphis, TN 38152 USA. EM egdaub@memphis.edu OI Trugman, Daniel/0000-0002-9296-4223 FU DOE [DE-AC52-06NA25396]; Los Alamos FX We thank Andrew Michael and an anonymous reviewer for their constructive reviews. This research was supported by DOE grant DE-AC52-06NA25396 and institutional (LDRD) funding at Los Alamos. Figures were generated using the Python plotting library Matplotlib [Hunter, 2007]. NR 44 TC 0 Z9 0 U1 3 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD AUG PY 2015 VL 120 IS 8 BP 5693 EP 5716 DI 10.1002/2014JB011777 PG 24 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CS6WN UT WOS:000362224100017 ER PT J AU Posch, JL Engebretson, MJ Olson, CN Thaller, SA Breneman, AW Wygant, JR Boardsen, SA Kletzing, CA Smith, CW Reeves, GD AF Posch, J. L. Engebretson, M. J. Olson, C. N. Thaller, S. A. Breneman, A. W. Wygant, J. R. Boardsen, S. A. Kletzing, C. A. Smith, C. W. Reeves, G. D. TI Low-harmonic magnetosonic waves observed by the Van Allen Probes SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE magnetosonic waves; equatorial noise; waves in plasmas; inner magnetosphere ID EQUATORIAL NOISE; CLUSTER SPACECRAFT; MAGNETIC EQUATOR; ULF WAVES; MAGNETOSPHERE; DISTRIBUTIONS; EXCITATION; PULSATIONS; FREQUENCY; PROTON AB Purely compressional electromagnetic waves (fast magnetosonic waves), generated at multiple harmonics of the local proton gyrofrequency, have been observed by various types of satellite instruments (fluxgate and search coil magnetometers and electric field sensors), but most recent studies have used data from search coil sensors, and many have been restricted to high harmonics. We report here on a survey of low-harmonic waves, based on electric and magnetic field data from the Electric Fields and Waves double probe and Electric and Magnetic Field Instrument Suite and Integrated Science fluxgate magnetometer instruments, respectively, on the Van Allen Probes spacecraft during its first full precession through all local times, from 1 October 2012 to 13 July 2014. These waves were observed both inside and outside the plasmapause (PP), at L shells from 2.4 to similar to 6 (the spacecraft apogee), and in regions with plasma number densities ranging from 10 to >1000cm(-3). Consistent with earlier studies, wave occurrence was sharply peaked near the magnetic equator. Waves appeared at all local times but were more common from noon to dusk, and often occurred within 3h after substorm injections. Outside the PP occurrence maximized broadly across noon, and inside the PP occurrence maximized in the dusk sector, in an extended plasmasphere. We confirm recent ray-tracing studies showing wave refraction and/or reflection at PP-like boundaries. Comparison with waveform receiver data indicates that in some cases these low-harmonic magnetosonic wave events occurred independently of higher-harmonic waves; this indicates the importance of including this population in future studies of radiation belt dynamics. C1 [Posch, J. L.; Engebretson, M. J.; Olson, C. N.] Augsburg Coll, Dept Phys, Minneapolis, MN 55454 USA. [Thaller, S. A.; Breneman, A. W.; Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Boardsen, S. A.] Univ Maryland, Goddard Planetary Heliophys Inst, Baltimore, MD 21201 USA. [Boardsen, S. A.] NASA, Goddard Space Flight Ctr, Heliophys Sci Div, Greenbelt, MD 20771 USA. [Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Smith, C. W.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. RP Posch, JL (reprint author), Augsburg Coll, Dept Phys, Minneapolis, MN 55454 USA. EM posch@augsburg.edu RI Reeves, Geoffrey/E-8101-2011; OI Reeves, Geoffrey/0000-0002-7985-8098; Kletzing, Craig/0000-0002-4136-3348 FU NSF [AGS-1202267, PLR-1341493]; NASA [NAS5-01072] FX We thank both referees for suggestions that greatly improved this manuscript. We thank Augsburg undergraduates Joseph Perrin and Sadie Tetrick for their help in identifying wave events, and Eun-Hwa Kim and Jay Johnson of Princeton University, Richard Horne of the British Antarctic Survey, and Brian Anderson of JHU/APL for their helpful discussions. We acknowledge the use of NASA/GSFC's Space Physics Data Facility's OMNIWeb and CDAWeb data. The EMFISIS data from the Van Allen Probes is available at http://emfisis.physics.uiowa.edu/. The Van Allen Probes EFW data is available at: http://www.space.umn.edu/missions/rbspefw-home-university-of-minnesota/. Research at Augsburg College was supported by NSF grants AGS-1202267 and PLR-1341493, and research at the University of Minnesota, University of Iowa, University of New Hampshire, and Los Alamos National Laboratory was supported by NASA prime contract NAS5-01072 to the Johns Hopkins University Applied Physics Laboratory NR 35 TC 11 Z9 11 U1 0 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD AUG PY 2015 VL 120 IS 8 BP 6230 EP 6257 DI 10.1002/2015JA021179 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CS5NP UT WOS:000362125300015 ER PT J AU Chen, YG Fujimoto, K Xiao, CJ Ji, HT AF Chen, Yangao Fujimoto, Keizo Xiao, Chijie Ji, Hantao TI Plasma waves around separatrix in collisionless magnetic reconnection with weak guide field SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE magnetic reconnection; separatrix; electron beam; electrostatic wave; electromagnetic wave ID ELECTRON-DIFFUSION REGION; WHISTLER WAVES AB Electrostatic and electromagnetic waves excited by electron beam around the separatrix region are analyzed in detail during the collisionless magnetic reconnection with a weak guide field by using 2-D particle-in-cell simulation with the adaptive mesh refinement. Broadband electrostatic waves are excited both in the inflow and outflow regions around the separatrices due to the electron bump-on-tail, two-stream, and Buneman instabilities. In contrast, the quasi-monochromatic electromagnetic waves are excited only in the inflow side of the separatrices due to a beam-driven whistler instability. The localization of the whistler waves is attributed to the nonuniformity of the out-of-plane magnetic field B-y. The whistler instability is suppressed in the outflow side where B-y is too small for the oblique propagation. The electrostatic waves with distinct speeds can explain the in situ spacecraft observations. From the causality point of view, the waves are generated as the consequence of the electron bulk acceleration to thermalize the particles through wave-particle interactions. These simulation results provide guidance to analyze high-resolution wave observations during reconnection in the ongoing and upcoming satellite missions, as well as in dedicated laboratory experiments. C1 [Chen, Yangao; Xiao, Chijie] Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Chen, Yangao; Xiao, Chijie] Peking Univ, Fus Simulat Ctr, Beijing 100871, Peoples R China. [Chen, Yangao; Ji, Hantao] Princeton Univ, Princeton Plasma Phys Lab, Ctr Magnet Self Org, Princeton, NJ 08543 USA. [Fujimoto, Keizo] Natl Inst Nat Sci, Natl Astron Observ Japan, Div Theoret Astron, Mitaka, Tokyo, Japan. [Ji, Hantao] Harbin Inst Technol, Lab Space Environm & Phys Sci, Harbin 150006, Peoples R China. RP Chen, YG (reprint author), Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. EM chenyg07@pku.edu.cn FU STEL, Nagoya University; China Scholarship Council [201406010040]; NSFC [41421003, 41274168]; 973 project [2011CB811404] FX We thank the NAOJ Visiting Research Fellow Program which gave us a chance to start the current research. The simulations were carried out by Fujitsu CX400 at ITC, Nagoya University, with support from a joint research program at STEL, Nagoya University. This work was also supported by the China Scholarship Council, 201406010040, NSFC (grants 41421003 and 41274168), and 973 project (grant 2011CB811404). The results in this paper are generated from our computer simulation code as described in section 2. The data can be obtained by contacting the authors through e-mail (chenyg07@pku.edu.cn). NR 28 TC 3 Z9 3 U1 2 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD AUG PY 2015 VL 120 IS 8 BP 6309 EP 6319 DI 10.1002/2015JA021267 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CS5NP UT WOS:000362125300020 ER EF