FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Calafiore, G Koshelev, A Dhuey, S Sassolini, S Messerschmidt, M Schleunitz, A Goltsov, A Pina-Hernandez, C Pirri, FC Yankov, V Cabrini, S Peroz, C AF Calafiore, Giuseppe Koshelev, Alexander Dhuey, Scott Sassolini, Simone Messerschmidt, Martin Schleunitz, Ame Goltsov, Alexander Pina-Hernandez, Carlos Pirri, Fabrizio C. Yankov, Vladimir Cabrini, Stefano Peroz, Christophe TI Step-and-repeat nanoimprint on pre-spin coated film for the fabrication of integrated optical devices SO JOURNAL OF MICRO-NANOLITHOGRAPHY MEMS AND MOEMS LA English DT Article DE nanoimprint lithography; integrated optics; digital planar hologram; nanoimprint resist ID LITHOGRAPHY AB A step-and-repeat nanoimprint lithography (SR-NIL) process on a pre-spin-coated film is employed for the fabrication of an integrated optical device for on-chip spectroscopy. The complex device geometry has a footprint of about 3 cm(2) and comprises several integrated optical components with different pattern size and density. Here, a new resist formulation for SR-NIL was tested for the first time and proved effective at dramatically reducing the occurrence of systematic defects due to film dewetting, trapped bubbles, and resist peel-off. A batch of 180 dies were imprinted, and statistics on the imprint success rate is discussed. Devices were optically characterized and benchmarked to an identical chip that was fabricated by electron-beam lithography. The overall performance of the imprinted nanospectrometers is well-aligned with that of the reference chip, which demonstrates the great potential of our SR-NIL for the low-cost manufacturing of integrated optical devices. (C) 2015 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Calafiore, Giuseppe; Koshelev, Alexander; Pina-Hernandez, Carlos; Peroz, Christophe] aBeam Technol Inc, Hayward, CA 94541 USA. [Calafiore, Giuseppe; Pirri, Fabrizio C.] Polytech Univ Turin, I-10129 Turin, Italy. [Calafiore, Giuseppe; Dhuey, Scott; Sassolini, Simone; Cabrini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Koshelev, Alexander] Moscow Inst Phys & Technol, Moscow 141700, Russia. [Messerschmidt, Martin; Schleunitz, Ame] Micro Resist Technol GmbH, D-12555 Berlin, Germany. [Goltsov, Alexander; Yankov, Vladimir] Nanoopt Devices, Santa Clara, CA 95054 USA. RP Calafiore, G (reprint author), aBeam Technol Inc, 22290 Foothill Blvd,St 2 Hayward, Hayward, CA 94541 USA. EM gc@abeamtech.com; scabrini@lbl.gov RI Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DEAC02-05CH11231]; Air Force Office of Scientific Research, Air Force Material Command, USAF [FA9550-12-C-0077] FX The authors would like to thank Dr. D. Olynick for her useful discussion. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under contract DEAC02-05CH11231. This study is supported by the Air Force Office of Scientific Research, Air Force Material Command, USAF, under grant/contract FA9550-12-C-0077. NR 20 TC 2 Z9 2 U1 3 U2 10 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1932-5150 EI 1932-5134 J9 J MICRO-NANOLITH MEM JI J. Micro-Nanolithogr. MEMS MOEMS PD JUL PY 2015 VL 14 IS 3 AR 033506 DI 10.1117/1.JMM.14.3.033506 PG 7 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics SC Engineering; Science & Technology - Other Topics; Materials Science; Optics GA CR4PG UT WOS:000361317500023 ER PT J AU Mojsoska, B Zuckermann, RN Jenssen, H AF Mojsoska, Biljana Zuckermann, Ronald N. Jenssen, Havard TI Structure-Activity Relationship Study of Novel Peptoids That Mimic the Structure of Antimicrobial Peptides SO ANTIMICROBIAL AGENTS AND CHEMOTHERAPY LA English DT Article ID ANTIBACTERIAL PEPTIDES; DESIGN; MECHANISM; MODEL; AMPHIPHILICITY; HYDROPHOBICITY; RICH AB The constant emergence of new bacterial strains that resist the effectiveness of marketed antimicrobials has led to an urgent demand for and intensive research on new classes of compounds to combat bacterial infections. Antimicrobial peptoids comprise one group of potential candidates for antimicrobial drug development. The present study highlights a library of 22 cationic amphipathic peptoids designed to target bacteria. All the peptoids share an overall net charge of +4 and are 8 to 9 residues long; however, the hydrophobicity and charge distribution along the abiotic backbone varied, thus allowing an examination of the structure-activity relationship within the library. In addition, the toxicity profiles of all peptoids were assessed in human red blood cells (hRBCs) and HeLa cells, revealing the low toxicity exerted by the majority of the peptoids. The structural optimization also identified two peptoid candidates, 3 and 4, with high selectivity ratios of 4 to 32 and 8 to 64, respectively, and a concentration- dependent bactericidal mode of action against Gram-negative Escherichia coli. C1 [Mojsoska, Biljana; Jenssen, Havard] Roskilde Univ, Dept Sci Syst & Models, Roskilde, Denmark. [Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Jenssen, H (reprint author), Roskilde Univ, Dept Sci Syst & Models, Roskilde, Denmark. EM jenssen@ruc.dk RI Foundry, Molecular/G-9968-2014 FU Danish Council for Independent Research [10-085287]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by The Danish Council for Independent Research (grant 10-085287).; We also acknowledge the Molecular Foundry, whose work was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract DE-AC02-05CH11231. NR 38 TC 15 Z9 16 U1 8 U2 48 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0066-4804 EI 1098-6596 J9 ANTIMICROB AGENTS CH JI Antimicrob. Agents Chemother. PD JUL PY 2015 VL 59 IS 7 BP 4112 EP 4120 DI 10.1128/AAC.00237-15 PG 9 WC Microbiology; Pharmacology & Pharmacy SC Microbiology; Pharmacology & Pharmacy GA CQ8YF UT WOS:000360896000051 PM 25941221 ER PT J AU Smalley, NE Taipale, S De Marco, P Doronina, NV Kyrpides, N Shapiro, N Woyke, T Kalyuzhnaya, MG AF Smalley, Nicole E. Taipale, Sami De Marco, Paolo Doronina, Nina V. Kyrpides, Nikos Shapiro, Nicole Woyke, Tanja Kalyuzhnaya, Marina G. TI Functional and genomic diversity of methylotrophic Rhodocyclaceae: description of Methyloversatilis discipulorum sp nov. SO INTERNATIONAL JOURNAL OF SYSTEMATIC AND EVOLUTIONARY MICROBIOLOGY LA English DT Article ID PHOSPHORUS REMOVAL; SEQUENCE; BACTERIA; PLANTS AB Three strains of methylotrophic Rhodocyclaceae (FAM1(T), RZ18-153 and RZ94) isolated from Lake Washington sediment samples were characterized. Based on phylogenetic analysis of 16S rRNA gene sequences the strains should be assigned to the genus Methyloversatilis. Similarly to other members of the family, the strains show broad metabolic capabilities and are able to utilize a number of organic acids, alcohols and aromatic compounds in addition to methanol and methylamine. The main fatty acids were 16:1 omega 7c (49-59%) and 16:0 (32-29%). Genomes of all isolates were sequenced, assembled and annotated in collaboration with the DOE Joint Genome Institute (JGI). Genome comparison revealed that the strains FAM1(T), RZ18-153 and RZ94 are closely related to each other and almost equally distant from two previously described species of the genus Methyloversatilis, Methyloversatilis universalis and Methyloversatilis thermotolerans. Like other methylotrophic species of the genus Methyloversatilis, all three strains possess one-subunit PQQ-dependent ethanol/methanol dehydrogenase (Mdh-2), the N-methylglutamate pathway and the serine cycle (isocitrate lyase/malate synthase, lcl/ms(+) variant). Like M. universalis, strains FAM1(T), RZ18-153 and RZ94 have a quinohemoprotein amine dehydrogenase, a tungsten-containing formaldehyde ferredoxin oxidoreductase, phenol hydroxylase, and the complete Calvin cycle. Similarly to M. thermotolerans, the three strains possess two-subunit methanol dehydrogenase (MxaFI), monoamine oxidase (MAO) and nitrogenase. Based on the phenotypic and genomic data, the strains FAM1(T), RZ18-153 and RZ94 represent a novel species of the genus Methyloversatilis, for which the name Methyloversatilis discipulorum sp. nov. is proposed. The type strain is FAM1(T) (=JCM 30542(T)=VKM=B-2888(T)). C1 [Smalley, Nicole E.; Kalyuzhnaya, Marina G.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Taipale, Sami] Univ Jyvaskyla, Dept Biol & Environm Sci, Jyvaskyla 40014, Finland. [De Marco, Paolo] Univ Porto, IBMC, P-4100 Oporto, Portugal. [De Marco, Paolo] IINFACTS, CESPU, Gandra Prd, Portugal. [Doronina, Nina V.] Russian Acad Sci, Skryabin GK Inst Biochem & Physiol Microorganisms, Moscow 142290, Russia. [Kyrpides, Nikos; Shapiro, Nicole; Woyke, Tanja] US DOE Joint Genome Inst, Walnut Creek, CA 94598 USA. [Kalyuzhnaya, Marina G.] San Diego State Univ, Dept Biol, San Diego, CA 92182 USA. RP Kalyuzhnaya, MG (reprint author), Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. EM mkalyuzhnaya@mail.sdsu.edu RI De Marco, Paolo/B-4281-2008; Kyrpides, Nikos/A-6305-2014; OI De Marco, Paolo/0000-0002-9322-6986; Kyrpides, Nikos/0000-0002-6131-0462; Kalyuzhnaya, Marina/0000-0002-9058-7794 FU NSF [MCB-0604269]; [DE-AC02-05CH11231] FX This research was supported by a grant from the NSF (grant no. MCB-0604269). The work conducted by the US Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under contract no. DE-AC02-05CH11231. NR 24 TC 5 Z9 5 U1 3 U2 18 PU SOC GENERAL MICROBIOLOGY PI READING PA MARLBOROUGH HOUSE, BASINGSTOKE RD, SPENCERS WOODS, READING RG7 1AG, BERKS, ENGLAND SN 1466-5026 EI 1466-5034 J9 INT J SYST EVOL MICR JI Int. J. Syst. Evol. Microbiol. PD JUL PY 2015 VL 65 BP 2227 EP 2233 DI 10.1099/ijs.0.000190 PN 7 PG 7 WC Microbiology SC Microbiology GA CQ8QN UT WOS:000360873600033 PM 26231539 ER PT J AU Muwamba, A Amatya, DM Ssegane, H Chescheir, GM Appelboom, T Tollner, EW Nettles, JE Youssef, MA Birgand, F Skaggs, RW Tian, S AF Muwamba, A. Amatya, D. M. Ssegane, H. Chescheir, G. M. Appelboom, T. Tollner, E. W. Nettles, J. E. Youssef, M. A. Birgand, F. Skaggs, R. W. Tian, S. TI Effects of Site Preparation for Pine Forest/Switchgrass Intercropping on Water Quality SO JOURNAL OF ENVIRONMENTAL QUALITY LA English DT Article ID THINNING LOBLOLLY-PINE; NORTH-CAROLINA; MANAGEMENT-PRACTICES; CONTROLLED DRAINAGE; COASTAL-PLAIN; SOUTH-CAROLINA; TAEDA L.; FOREST; SOIL; PLANTATION AB A study was initiated to investigate the sustainability effects of intercropping switchgrass (Panicum virgatum L.) in a loblolly pine (Pinus taeda L.) plantation. This forest-based biofuel system could possibly provide biomass from the perennial energy grass while maintaining the economics and environmental benefits of a forest managed for sawtimber. Operations necessary for successful switchgrass establishment and growth, such as site preparation, planting, fertilizing, mowing and baling, may affect hydrology and nutrient runoff. The objectives of this study were (i) to characterize the temporal effects of management on nutrient concentrations and loadings and (ii) to use pretreatment data to predict those treatment effects. The study watersheds (similar to 25 ha each) in the North Carolina Atlantic Coastal Plain were a pine/switchgrass intercropped site (D1), a midrotation thinned pine site with natural understory (D2), and a switchgrass-only site (D3). Rainfall, drainage, water table elevation, nitrogen (total Kjedahl N, NH4-N, and NO3-N), and phosphate were monitored for the 2007-2008 pretreatment and the 2009-2012 treatment periods. From 2010 to 2011 in site D1, the average NO3-N concentration effects decreased from 0.18 to -0.09 mg L-1, and loads effects decreased from 0.86 to 0.49 kg ha(-1). During the same period in site D3, the average NO3 -N concentration effects increased from 0.03 to 0.09 mg L-1, and loads effects increased from -0.26 to 1.24 kg ha(-1). This study shows the importance of considering water quality effects associated with intensive management operations required for switchgrass establishment or other novel forest-based biofuel systems. C1 [Muwamba, A.; Tollner, E. W.] Univ Georgia, Athens, GA 30602 USA. [Amatya, D. M.] USDA Forest Serv, Ctr Forested Wetlands Res, Cordesville, SC 29434 USA. [Ssegane, H.] Argonne Natl Lab, Argonne, IL 60439 USA. [Chescheir, G. M.; Appelboom, T.; Youssef, M. A.; Birgand, F.; Skaggs, R. W.; Tian, S.] N Carolina State Univ, Raleigh, NC 27695 USA. [Nettles, J. E.] Weyerhaeuser Co, Columbus, MS 39701 USA. RP Amatya, DM (reprint author), USDA Forest Serv, Ctr Forested Wetlands Res, Cordesville, SC 29434 USA. EM damatya@fs.fed.us FU Weyerhauser Company; Catch light Energy LLC (A Chevron/Weyerhaeuser Joint Venture); US Department of Energy FX The authors thank Weyerhauser Company, Catch light Energy LLC (A Chevron/Weyerhaeuser Joint Venture), and the US Department of Energy for logistical and financial support for this work; Tyson Cliff for helping in field data collection; and the peer and anonymous reviewers for their review and suggestions. NR 49 TC 0 Z9 0 U1 0 U2 4 PU AMER SOC AGRONOMY PI MADISON PA 677 S SEGOE RD, MADISON, WI 53711 USA SN 0047-2425 EI 1537-2537 J9 J ENVIRON QUAL JI J. Environ. Qual. PD JUL-AUG PY 2015 VL 44 IS 4 BP 1263 EP 1272 DI 10.2134/jeq2014.11.0505 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA CQ8JC UT WOS:000360852600025 PM 26437108 ER PT J AU Mahajan, D Chai, XL Holuj, B Wu, HL Novelli, CA AF Mahajan, Devinder Chai Xiaoli Holuj, Brian Wu Hongliang Novelli, Catherine A. TI Preface to Special Topic: US-China EcoPartnerships: Approaches to Challenges in Energy and Environment SO JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY LA English DT Editorial Material C1 [Mahajan, Devinder] SUNY Stony Brook, Low Carbon Energy Management L CEM Lab, Chem & Mol Engn, Stony Brook, NY 11790 USA. [Chai Xiaoli] Tongji Univ, Sch Environm Sci & Engn, State Key Lab Pollut Control, Shanghai 200092, Peoples R China. [Holuj, Brian] US DOE, Int Sci & Technol Collaborat, Off Int Affairs, Washington, DC 20585 USA. [Wu Hongliang] Natl Dev Reform Commiss, Beijing, Peoples R China. [Novelli, Catherine A.] US Dept State, Washington, DC 20520 USA. RP Mahajan, D (reprint author), SUNY Stony Brook, Low Carbon Energy Management L CEM Lab, Chem & Mol Engn, Stony Brook, NY 11790 USA. NR 0 TC 1 Z9 1 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1941-7012 J9 J RENEW SUSTAIN ENER JI J. Renew. Sustain. Energy PD JUL PY 2015 VL 7 IS 4 AR 041301 DI 10.1063/1.4929547 PG 3 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CQ5OS UT WOS:000360655500001 ER PT J AU Mirocha, JD Rajewski, DA Marjanovic, N Lundquist, JK Kosovic, B Draxl, C Churchfield, MJ AF Mirocha, Jeffrey D. Rajewski, Daniel A. Marjanovic, Nikola Lundquist, Julie K. Kosovic, Branko Draxl, Caroline Churchfield, Matthew J. TI Investigating wind turbine impacts on near-wake flow using profiling lidar data and large-eddy simulations with an actuator disk model SO JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY LA English DT Article ID COMPUTATIONAL FLUID-DYNAMICS; BOUNDARY-LAYERS; TURBULENCE; FARM; AERODYNAMICS; SODAR; HEAT; IOWA AB Wind turbine impacts on the atmospheric flow are investigated using data from the Crop Wind Energy Experiment (CWEX-11) and large-eddy simulations (LESs) utilizing a generalized actuator disk (GAD) wind turbine model. CWEX-11 employed velocity-azimuth display (VAD) data from two Doppler lidar systems to sample vertical profiles of flow parameters across the rotor depth both upstream and in the wake of an operating 1.5MW wind turbine. Lidar and surface observations obtained during four days of July 2011 are analyzed to characterize the turbine impacts on wind speed and flow variability, and to examine the sensitivity of these changes to atmospheric stability. Significant velocity deficits (VD) are observed at the downstream location during both convective and stable portions of four diurnal cycles, with large, sustained deficits occurring during stable conditions. Variances of the streamwise velocity component, sigma(u), likewise show large increases downstream during both stable and unstable conditions, with stable conditions supporting sustained small increases of sigma(u), while convective conditions featured both larger magnitudes and increased variability, due to the large coherent structures in the background flow. Two representative case studies, one stable and one convective, are simulated using LES with a GAD model at 6m resolution to evaluate the compatibility of the simulation framework with validation using vertically profiling lidar data in the near wake region. Virtual lidars were employed to sample the simulated flow field in a manner consistent with the VAD technique. Simulations reasonably reproduced aggregated wake VD characteristics, albeit with smaller magnitudes than observed, while sigma(u) values in the wake are more significantly underestimated. The results illuminate the limitations of using a GAD in combination with coarse model resolution in the simulation of near wake physics, and validation thereof using VAD data. (C) 2015 Author(s). C1 [Mirocha, Jeffrey D.; Marjanovic, Nikola] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Rajewski, Daniel A.] Iowa State Univ, Dept Agron, Ames, IA 50011 USA. [Marjanovic, Nikola] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94770 USA. [Lundquist, Julie K.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Lundquist, Julie K.; Kosovic, Branko; Churchfield, Matthew J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Kosovic, Branko] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. RP Mirocha, JD (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM jmirocha@llnl.gov RI Draxl, Caroline/O-6206-2016; OI Draxl, Caroline/0000-0001-5532-6268; Rajewski, Daniel/0000-0002-9609-2303 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. DOE Office of Energy Efficiency and Renewable Energy; LLNL Graduate Scholars Program; National Science Foundation under the State of Iowa EPSCoR [1101284] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and was supported by the U.S. DOE Office of Energy Efficiency and Renewable Energy, and the LLNL Graduate Scholars Program. NREL is a national laboratory of the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, operated by the Alliance for Sustainable Energy, LLC. Data analysis was supported in part by the National Science Foundation under the State of Iowa EPSCoR Grant No. 1101284. The authors thank Sven Schmitz of Penn State University for the parameters of the 1.5 MW turbine used in the simulations. We also thank the team who collected the CWEX-11 dataset, including Matthew Aitken, Russell Doorenbos, Thomas Horst, Steven Oncley, Michael Rhodes, Eugene Takle, and Kristopher Spoth. NR 41 TC 5 Z9 5 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1941-7012 J9 J RENEW SUSTAIN ENER JI J. Renew. Sustain. Energy PD JUL PY 2015 VL 7 IS 4 AR 043143 DI 10.1063/1.4928873 PG 21 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CQ5OS UT WOS:000360655500062 ER PT J AU Hadjithomas, M Chen, IMA Chu, K Ratner, A Palaniappan, K Szeto, E Huang, JH Reddy, TBK Cimermancic, P Fischbach, MA Ivanova, NN Markowitz, VM Kyrpides, NC Pati, A AF Hadjithomas, Michalis Chen, I-Min Amy Chu, Ken Ratner, Anna Palaniappan, Krishna Szeto, Ernest Huang, Jinghua Reddy, T. B. K. Cimermancic, Peter Fischbach, Michael A. Ivanova, Natalia N. Markowitz, Victor M. Kyrpides, Nikos C. Pati, Amrita TI IMG-ABC: A Knowledge Base To Fuel Discovery of Biosynthetic Gene Clusters and Novel Secondary Metabolites SO MBIO LA English DT Article ID COMPARATIVE-ANALYSIS SYSTEM; PSEUDOMONAS-FLUORESCENS; INFORMATION-SYSTEM; MICROBIAL GENOMES; NATURAL-PRODUCTS; DRUG DISCOVERY; 4 VERSION; INSIGHTS; DATABASE; POLYKETIDE AB In the discovery of secondary metabolites, analysis of sequence data is a promising exploration path that remains largely underutilized due to the lack of computational platforms that enable such a systematic approach on a large scale. In this work, we present IMG-ABC (https://img.jgi.doe.gov/abc), an atlas of biosynthetic gene clusters within the Integrated Microbial Genomes (IMG) system, which is aimed at harnessing the power of "big" genomic data for discovering small molecules. IMG-ABC relies on IMG's comprehensive integrated structural and functional genomic data for the analysis of biosynthetic gene clusters (BCs) and associated secondary metabolites (SMs). SMs and BCs serve as the two main classes of objects in IMG-ABC, each with a rich collection of attributes. A unique feature of IMG-ABC is the incorporation of both experimentally validated and computationally predicted BCs in genomes as well as metagenomes, thus identifying BCs in uncultured populations and rare taxa. We demonstrate the strength of IMG-ABC's focused integrated analysis tools in enabling the exploration of microbial secondary metabolism on a global scale, through the discovery of phenazine-producing clusters for the first time in Alphaproteobacteria. IMG-ABC strives to fill the long-existent void of resources for computational exploration of the secondary metabolism universe; its underlying scalable framework enables traversal of uncovered phylogenetic and chemical structure space, serving as a doorway to a new era in the discovery of novel molecules. IMPORTANCE IMG-ABC is the largest publicly available database of predicted and experimental biosynthetic gene clusters and the secondary metabolites they produce. The system also includes powerful search and analysis tools that are integrated with IMG's extensive genomic/metagenomic data and analysis tool kits. As new research on biosynthetic gene clusters and secondary metabolites is published and more genomes are sequenced, IMG-ABC will continue to expand, with the goal of becoming an essential component of any bioinformatic exploration of the secondary metabolism world. C1 [Hadjithomas, Michalis; Reddy, T. B. K.; Ivanova, Natalia N.; Kyrpides, Nikos C.; Pati, Amrita] DOE Joint Genome Inst, Prokaryot Super Program, Walnut Creek, CA 94598 USA. [Chen, I-Min Amy; Chu, Ken; Ratner, Anna; Palaniappan, Krishna; Szeto, Ernest; Huang, Jinghua; Markowitz, Victor M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Biosci Comp, Berkeley, CA 94720 USA. [Cimermancic, Peter; Fischbach, Michael A.] Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, San Francisco, CA 94143 USA. RP Pati, A (reprint author), DOE Joint Genome Inst, Prokaryot Super Program, Walnut Creek, CA 94598 USA. EM nckyrpides@lbl.gov; apati@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU Office of Science, Office of Biological and Environmental Research, Life Sciences Division, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; University of California; Howard Hughes Medical Institute Predoctoral Fellowship FX The Director, Office of Science, Office of Biological and Environmental Research, Life Sciences Division, U.S. Department of Energy under contract number DE-AC02-05CH11231; this research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under contract number DE-AC02-05CH11231. Funding for open access charges was provided by the: University of California. P.C. was supported by a Howard Hughes Medical Institute Predoctoral Fellowship. NR 39 TC 17 Z9 18 U1 3 U2 8 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2015 VL 6 IS 4 AR e00932-15 DI 10.1128/mBio.00932-15 PG 10 WC Microbiology SC Microbiology GA CQ8EN UT WOS:000360839400025 PM 26173699 ER PT J AU Kourist, R Bracharz, F Lorenzen, J Kracht, ON Chovatia, M Daum, C Deshpande, S Lipzen, A Nolan, M Ohm, RA Grigoriev, IV Sun, S Heitman, J Bruck, T Nowrousian, M AF Kourist, Robert Bracharz, Felix Lorenzen, Jan Kracht, Octavia N. Chovatia, Mansi Daum, Chris Deshpande, Shweta Lipzen, Anna Nolan, Matt Ohm, Robin A. Grigoriev, Igor V. Sun, Sheng Heitman, Joseph Brueck, Thomas Nowrousian, Minou TI Genomics and Transcriptomics Analyses of the Oil-Accumulating Basidiomycete Yeast Trichosporon oleaginosus: Insights into Substrate Utilization and Alternative Evolutionary Trajectories of Fungal Mating Systems SO MBIO LA English DT Article ID PATHOGEN CRYPTOCOCCUS-NEOFORMANS; FATTY-ACID SYNTHASE; SEXUAL REPRODUCTION; YARROWIA-LIPOLYTICA; LIPID-ACCUMULATION; SEQUENCE; VIRULENCE; PROTEIN; ALIGNMENT; STRAIN AB Microbial fermentation of agro-industrial waste holds great potential for reducing the environmental impact associated with the production of lipids for industrial purposes from plant biomass. However, the chemical complexity of many residues currently prevents efficient conversion into lipids, creating a high demand for strains with the ability to utilize all energy-rich components of agricultural residues. Here, we present results of genome and transcriptome analyses of Trichosporon oleaginosus. This oil-accumulating yeast is able to grow on a wide variety of substrates, including pentoses and N-acetylglucosamine, making it an interesting candidate for biotechnological applications. Transcriptomics shows specific changes in gene expression patterns under lipid-accumulating conditions. Furthermore, gene content and expression analyses indicate that T. oleaginosus is well-adapted for the utilization of chitin-rich biomass. We also focused on the T. oleaginosus mating type, because this species is a member of the Tremellomycetes, a group that has been intensively analyzed as a model for the evolution of sexual development, the best-studied member being Cryptococcus neoformans. The structure of the T. oleaginosus mating-type regions differs significantly from that of other Tremellomycetes and reveals a new evolutionary trajectory paradigm. Comparative analysis shows that recruitment of developmental genes to the ancestral tetrapolar mating-type loci occurred independently in the Trichosporon and Cryptococcus lineages, supporting the hypothesis of a trend toward larger mating-type regions in fungi. IMPORTANCE Finite fossil fuel resources pose sustainability challenges to society and industry. Microbial oils are a sustainable feedstock for biofuel and chemical production that does not compete with food production. We describe genome and transcriptome analyses of the oleaginous yeast Trichosporon oleaginosus, which can accumulate up to 70% of its dry weight as lipids. In contrast to conventional yeasts, this organism not only shows an absence of diauxic effect while fermenting hexoses and pentoses but also effectively utilizes xylose and N-acetylglucosamine, which are building blocks of lignocellulose and chitin, respectively. Transcriptome analysis revealed metabolic networks that govern conversion of xylose or N-acetylglucosamine as well as lipid accumulation. These data form the basis for a targeted strain optimization strategy. Furthermore, analysis of the mating type of T. oleaginosus supports the hypothesis of a trend toward larger mating-type regions in fungi, similar to the evolution of sex chromosomes in animals and plants. C1 [Kourist, Robert; Kracht, Octavia N.] Ruhr Univ Bochum, Jr Res Grp Microbial Biotechnol, Bochum, Germany. [Bracharz, Felix; Lorenzen, Jan; Brueck, Thomas] Tech Univ Munich, Fachgebiet Ind Biokatalyse, Garching, Germany. [Chovatia, Mansi; Daum, Chris; Deshpande, Shweta; Lipzen, Anna; Nolan, Matt; Ohm, Robin A.; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Ohm, Robin A.] Univ Utrecht, Dept Microbiol, Utrecht, Netherlands. [Sun, Sheng; Heitman, Joseph] Duke Univ, Med Ctr, Dept Mol Genet & Microbiol, Durham, NC USA. [Nowrousian, Minou] Ruhr Univ Bochum, Lehrstuhl Allgemeine & Mol Bot, Bochum, Germany. RP Kourist, R (reprint author), Ruhr Univ Bochum, Jr Res Grp Microbial Biotechnol, Univ Str 150, Bochum, Germany. EM robert.kourist@rub.de; brueck@tum.de; minou.nowrousian@rub.de RI Bruck, Prof.Dr. Thomas/B-6018-2016; Ohm, Robin/I-6689-2016; OI Bruck, Prof.Dr. Thomas/0000-0002-2113-6957; Nowrousian, Minou/0000-0003-0075-6695; Kourist, Robert/0000-0002-2853-3525 FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; German Research Foundation (DFG); NIAID/NIH R37 merit award [AI39115-17]; Federal Ministry for Education and Research (BMBF) project "Advance Biomass Value" [03SF0446A]; Ministry for Innovation, Science and Investigation of the State of North Rhine-Westphalia [005-1503-0006] FX The work conducted by the U.S. Department of Energy Joint Genome Institute was supported by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Minou Nowrousian acknowledges funding by the German Research Foundation (DFG) and would like to thank Ulrich Kuck for his support at the Department of General and Molecular Botany. Sheng Sun and Joseph Heitman were supported by NIAID/NIH R37 merit award AI39115-17. Thomas Bruck, Felix Bracharz, and Jan Lorenzen acknowledge funding through the Federal Ministry for Education and Research (BMBF) project "Advance Biomass Value" (award 03SF0446A). Robert Kourist gratefully acknowledges financial support from the Ministry for Innovation, Science and Investigation of the State of North Rhine-Westphalia (grant 005-1503-0006). NR 75 TC 7 Z9 7 U1 6 U2 22 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2015 VL 6 IS 4 AR e00918-15 DI 10.1128/mBio.00918-15 PG 13 WC Microbiology SC Microbiology GA CQ8EN UT WOS:000360839400029 PM 26199329 ER PT J AU Shi, SJ Nuccio, E Herman, DJ Rijkers, R Estera, K Li, JB da Rocha, UN He, ZL Pett-Ridge, J Brodie, EL Zhou, JZ Firestone, M AF Shi, Shengjing Nuccio, Erin Herman, Donald J. Rijkers, Ruud Estera, Katerina Li, Jiabao da Rocha, Ulisses Nunes He, Zhili Pett-Ridge, Jennifer Brodie, Eoin L. Zhou, Jizhong Firestone, Mary TI Successional Trajectories of Rhizosphere Bacterial Communities over Consecutive Seasons SO MBIO LA English DT Article ID SOIL MICROBIAL COMMUNITY; DIVERSITY; ECOLOGY; MICROORGANISMS; CARBON; ROOTS; RNA; PHYLOGENIES; GENERATION; MAGNITUDE AB It is well known that rhizosphere microbiomes differ from those of surrounding soil, and yet we know little about how these root-associated microbial communities change through the growing season and between seasons. We analyzed the response of soil bacteria to roots of the common annual grass Avena fatua over two growing seasons using high-throughput sequencing of 16S rRNA genes. Over the two periods of growth, the rhizosphere bacterial communities followed consistent successional patterns as plants grew, although the starting communities were distinct. Succession in the rhizosphere was characterized by a significant decrease in both taxonomic and phylogenetic diversity relative to background soil communities, driven by reductions in both richness and evenness of the bacterial communities. Plant roots selectively stimulated the relative abundance of Alphaproteobacteria, Betaproteobacteria, and Bacteroidetes but reduced the abundance of Acidobacteria, Actinobacteria, and Firmicutes. Taxa that increased in relative abundance in the rhizosphere soil displayed phylogenetic clustering, suggesting some conservation and an evolutionary basis for the response of complex soil bacterial communities to the presence of plant roots. The reproducibility of rhizosphere succession and the apparent phylogenetic conservation of rhizosphere competence traits suggest adaptation of the indigenous bacterial community to this common grass over the many decades of its presence. IMPORTANCE We document the successional patterns of rhizosphere bacterial communities associated with a "wild" annual grass, Avena fatua, which is commonly a dominant plant in Mediterranean-type annual grasslands around the world; the plant was grown in its grassland soil. Most studies documenting rhizosphere microbiomes address "domesticated" plants growing in soils to which they are introduced. Rhizosphere bacterial communities exhibited a pattern of temporal succession that was consistent and repeatable over two growing seasons. There are few studies assessing the reproducibility over multiple seasons. Through the growing season, the rhizosphere community became progressively less diverse, likely reflecting root homogenization of soil microniches. Phylogenetic clustering of the rhizosphere dynamic taxa suggests evolutionary adaptation to Avena roots. The reproducibility of rhizosphere succession and the apparent phylogenetic conservation of rhizosphere competence traits suggest adaptation of the indigenous bacterial community to this common grass over the many decades of its presence. C1 [Shi, Shengjing; Nuccio, Erin; Herman, Donald J.; Rijkers, Ruud; Estera, Katerina; Brodie, Eoin L.; Firestone, Mary] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Shi, Shengjing; Li, Jiabao; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Nuccio, Erin; Pett-Ridge, Jennifer] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA USA. [Herman, Donald J.; da Rocha, Ulisses Nunes; Brodie, Eoin L.; Zhou, Jizhong; Firestone, Mary] Lawrence Livermore Natl Lab, Div Earth Sci, Livermore, CA USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Firestone, M (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. EM mkfstone@berkeley.edu RI Brodie, Eoin/A-7853-2008 OI Brodie, Eoin/0000-0002-8453-8435 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research Genomic Science Program [DE-SC0004730, DE-SC0010570]; DOE under UC [00008322]; Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy at Lawrence Livermore National Laboratory [SA-DOE-29318] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research Genomic Science Program, under award no. DE-SC0004730 and DE-SC0010570. Part of this work was performed at the University of Oklahoma, funded by the DOE under UC subcontract no. 00008322. Part of this work (E.L.B. and U.N.D.) was performed at Lawrence Berkeley National Laboratory under Department of Energy contract no. DE-AC02-05CH11231; the work of J.P.-R. was conducted under the auspices of the U.S. Department of Energy at Lawrence Livermore National Laboratory under contract SA-DOE-29318. NR 59 TC 6 Z9 6 U1 15 U2 50 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2015 VL 6 IS 4 AR e00746-15 DI 10.1128/mBio.00746-15 PG 8 WC Microbiology SC Microbiology GA CQ8EN UT WOS:000360839400048 PM 26242625 ER PT J AU Maze, I Wenderski, W Noh, KM Bagot, RC Tzavaras, N Purushothaman, I Elsasser, SJ Guo, Y Ionete, C Hurd, YL Tamminga, CA Halene, T Farrelly, L Soshnev, AA Wen, DC Rafii, S Birtwistle, MR Akbarian, S Buchholz, BA Blitzer, RD Nestler, EJ Yuan, ZF Garcia, BA Shen, L Molina, H Allis, CD AF Maze, Ian Wenderski, Wendy Noh, Kyung-Min Bagot, Rosemary C. Tzavaras, Nikos Purushothaman, Immanuel Elsaesser, Simon J. Guo, Yin Ionete, Carolina Hurd, Yasmin L. Tamminga, Carol A. Halene, Tobias Farrelly, Lorna Soshnev, Alexey A. Wen, Duancheng Rafii, Shahin Birtwistle, Marc R. Akbarian, Schahram Buchholz, Bruce A. Blitzer, Robert D. Nestler, Eric J. Yuan, Zuo-Fei Garcia, Benjamin A. Shen, Li Molina, Henrik Allis, C. David TI Critical Role of Histone Turnover in Neuronal Transcription and Plasticity SO NEURON LA English DT Article ID H3 VARIANTS; RAT-BRAIN; CHROMATIN; DYNAMICS; RECRUITMENT; PROTEASOME; PROTEINS; MEMORY; CELLS AB Turnover and exchange of nucleosomal histones and their variants, a process long believed to be static in post-replicative cells, remains largely unexplored in brain. Here, we describe a novel mechanistic role for HIRA (histone cell cycle regulator) and proteasomal degradation-associated histone dynamics in the regulation of activity-dependent transcription, synaptic connectivity, and behavior. We uncover a dramatic developmental profile of nucleosome occupancy across the lifespan of both rodents and humans, with the histone variant H3.3 accumulating to near-saturating levels throughout the neuronal genome by mid-adolescence. Despite such accumulation, H3.3-containing nucleosomes remain highly dynamic-in a modification-independent manner-to control neuronal- and glial-specific gene expression patterns throughout life. Manipulating H3.3 dynamics in both embryonic and adult neurons confirmed its essential role in neuronal plasticity and cognition. Our findings establish histone turnover as a critical and previously undocumented regulator of cell type-specific transcription and plasticity in mammalian brain. C1 [Maze, Ian; Wenderski, Wendy; Noh, Kyung-Min; Elsaesser, Simon J.; Soshnev, Alexey A.; Allis, C. David] Rockefeller Univ, Lab Chromatin Biol & Epigenet, New York, NY 10065 USA. [Maze, Ian; Tzavaras, Nikos; Hurd, Yasmin L.; Farrelly, Lorna; Birtwistle, Marc R.; Blitzer, Robert D.; Nestler, Eric J.] Icahn Sch Med Mt Sinai, Dept Pharmacol & Syst Therapeut, New York, NY 10029 USA. [Maze, Ian; Bagot, Rosemary C.; Purushothaman, Immanuel; Hurd, Yasmin L.; Akbarian, Schahram; Nestler, Eric J.; Shen, Li] Icahn Sch Med Mt Sinai, Dept Neurosci, New York, NY 10029 USA. [Guo, Yin; Ionete, Carolina] UMass Mem Med Ctr, Dept Neurol, Worcester, MA 01605 USA. [Hurd, Yasmin L.; Halene, Tobias; Akbarian, Schahram; Blitzer, Robert D.; Nestler, Eric J.] Icahn Sch Med Mt Sinai, Dept Psychiat, New York, NY 10029 USA. [Tamminga, Carol A.] Univ Texas SW Med Ctr Dallas, Dept Psychiat, Dallas, TX 75235 USA. [Wen, Duancheng] Ronald O Perleman & Claudia Cohen Ctr Reprod Med, New York, NY 10021 USA. [Wen, Duancheng; Rafii, Shahin] Weill Cornell Med Coll, Ansary Stem Cell Inst, New York, NY 10065 USA. [Buchholz, Bruce A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. [Yuan, Zuo-Fei; Garcia, Benjamin A.] Univ Penn, Dept Biochem & Biophys, Philadelphia, PA 19104 USA. [Molina, Henrik] Rockefeller Univ, Rockefeller Univ Prote Resource Ctr, New York, NY 10065 USA. RP Maze, I (reprint author), Rockefeller Univ, Lab Chromatin Biol & Epigenet, New York, NY 10065 USA. EM ian.maze@mssm.edu; c.david.allis@rockefeller.edu RI Elsasser, Simon/B-8911-2014; OI Elsasser, Simon/0000-0001-8724-4849; Maze, Ian/0000-0003-1490-7781 FU National Institute of Mental Health (NIMH) [5R01 MH094698, P50 MH096890]; NIH [R21MH102679, RO1GM110174, 8P41GM103483]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-653296] FX We would like to thank members of the C.D.A. laboratory for critical readings of the manuscript and contribution of reagents (particularly Dr. Ronen Sadeh). We would also like to thank Dr. Kunihiro Uryu (The Rockefeller University Electron Microscopy Resource Center) for assistance with TEM experiments, Ms. Kelly Gleason for help with human postmortem brain dissections, and Mr. Charlie Li for assistance with mESC FACS. This work was supported by grants from the National Institute of Mental Health (NIMH): 5R01 MH094698 and P50 MH096890. B.A.G. gratefully acknowledges funding from the following NIH grants: R21MH102679 and RO1GM110174. Support for accelerator mass spectrometry analyses was provided by NIH 8P41GM103483. This work was performed, in part, under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contracts DE-AC52-07NA27344 and LLNL-JRNL-653296. NR 22 TC 29 Z9 29 U1 4 U2 19 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0896-6273 EI 1097-4199 J9 NEURON JI Neuron PD JUL 1 PY 2015 VL 87 IS 1 BP 77 EP 94 DI 10.1016/j.neuron.2015.06.014 PG 18 WC Neurosciences SC Neurosciences & Neurology GA CQ9ZQ UT WOS:000360977400010 PM 26139371 ER PT J AU Bucksbaum, PH Berrah, N AF Bucksbaum, Philip H. Berrah, Nora TI BRIGHTER AND FASTER The promise and challenge of the x-ray free-electron laser SO PHYSICS TODAY LA English DT Article ID DYNAMICS C1 [Bucksbaum, Philip H.] Stanford Univ, Nat Sci, Stanford, CA 94305 USA. [Bucksbaum, Philip H.] SLAC, Stanford, CA USA. [Berrah, Nora] Univ Connecticut, Dept Phys, Storrs, CT USA. RP Bucksbaum, PH (reprint author), Stanford Univ, Nat Sci, Stanford, CA 94305 USA. NR 16 TC 2 Z9 2 U1 4 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0031-9228 EI 1945-0699 J9 PHYS TODAY JI Phys. Today PD JUL PY 2015 VL 68 IS 7 BP 26 EP 32 DI 10.1063/PT.3.2845 PG 7 WC Physics, Multidisciplinary SC Physics GA CQ9HO UT WOS:000360924700015 ER PT J AU Fowler, TK Ryutov, D AF Fowler, T. Kenneth Ryutov, Dmitri TI Richard Freeman Post obituary SO PHYSICS TODAY LA English DT Biographical-Item C1 [Fowler, T. Kenneth] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Ryutov, Dmitri] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Fowler, TK (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. NR 1 TC 1 Z9 1 U1 1 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0031-9228 EI 1945-0699 J9 PHYS TODAY JI Phys. Today PD JUL PY 2015 VL 68 IS 7 BP 56 EP + PG 2 WC Physics, Multidisciplinary SC Physics GA CQ9HO UT WOS:000360924700020 ER PT J AU Field, RV Grigoriu, M Emery, JM AF Field, R. V., Jr. Grigoriu, M. Emery, J. M. TI On the efficacy of stochastic collocation, stochastic Galerkin, and stochastic reduced order models for solving stochastic problems SO PROBABILISTIC ENGINEERING MECHANICS LA English DT Article DE Approximation theory; Monte Carlo simulation; Random variables and fields; Stochastic differential equations; Uncertainty propagation ID PARTIAL-DIFFERENTIAL-EQUATIONS; RANDOM INPUT DATA; APPROXIMATIONS AB The stochastic collocation (SC) and stochastic Galerkin (SG) methods are two well-established and successful approaches for solving general stochastic problems. A recently developed method based on stochastic reduced order models (SROMs) can also be used. Herein we provide a comparison of the three methods for some numerical examples; our evaluation only holds for the examples considered in the paper. The purpose of the comparisons is not to criticize the SC or SG methods, which have proven very useful for a broad range of applications, nor is it to provide overall ratings of these methods as compared to the SROM method. Rather, our objectives are to present the SROM method as an alternative approach to solving stochastic problems and provide information on the computational effort required by the implementation of each method, while simultaneously assessing their performance for a collection of specific problems. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Field, R. V., Jr.; Emery, J. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Grigoriu, M.] Cornell Univ, Ithaca, NY 14853 USA. RP Field, RV (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rvfield@sandia.gov; mdg12@cornell.edu; jmemery@sandia.gov OI Emery, John /0000-0001-6671-4952 NR 21 TC 3 Z9 3 U1 0 U2 1 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0266-8920 EI 1878-4275 J9 PROBABILIST ENG MECH JI Probab. Eng. Eng. Mech. PD JUL PY 2015 VL 41 BP 60 EP 72 DI 10.1016/j.probengmech.2015.05.002 PG 13 WC Engineering, Mechanical; Mechanics; Statistics & Probability SC Engineering; Mechanics; Mathematics GA CQ9RO UT WOS:000360952900006 ER PT J AU Shen, TM Ye, LY Turrioni, D Li, P AF Shen, Tengming Ye, Liyang Turrioni, Daniele Li, Pei TI High-field quench behavior and dependence of hot spot temperature on quench detection voltage threshold in a Bi2Sr2CaCu2Ox coil SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE Bi-2212 magnet; quench detection; quench protection; quench behavior; superconducting magnets ID WIRES; MAGNET; PROTECTION; STABILITY AB Small insert solenoids have been built using a multifilamentary Ag/Bi2Sr2CaCu2Ox round wire insulated with a mullite sleeve (similar to 100 mu m in thickness) and characterized in background fields to explore the quench behaviors and limits of Bi2Sr2CaCu2Ox superconducting magnets, with an emphasis on assessing the impact of slow normal zone propagation on quench detection. Using heaters of various lengths to initiate a small normal zone, a coil was quenched safely more than 70 times without degradation, with the maximum coil temperature reaching 280 K. Coils withstood a resistive voltage of tens of mV for seconds without quenching, showing the high stability of these coils and suggesting that the quench detection voltage should be greater than 50 mV in order not to falsely trigger protection. The hot spot temperature for the resistive voltage of the normal zone to reach 100 mV increased from similar to 40-similar to 80 K while increasing the operating wire current density J(o) from 89 A mm(-2) to 354 A mm(-2), whereas for the voltage to reach 1 V, it increased from similar to 60-similar to 140 K. This shows the increasing negative impact of slow normal zone propagation on quench detection with increasing Jo and the need to limit the quench detection voltage to <1 V. These measurements, coupled with an analytical quench model, were used to assess the impact of the maximum allowable detection voltage and temperature upon quench detection on the quench protection, assuming a limit of the hot spot temperature to <300 K. C1 [Shen, Tengming; Ye, Liyang; Turrioni, Daniele; Li, Pei] Fermilab Natl Accelerator Lab, Magnet Syst Dept, Batavia, IL 60510 USA. [Ye, Liyang] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. RP Shen, TM (reprint author), Fermilab Natl Accelerator Lab, Magnet Syst Dept, POB 500, Batavia, IL 60510 USA. EM tshen@fnal.gov FU Office of High Energy Physics at the U S Department of Energy (DOE) through the Fermi Research Alliance [DE-AC02-07CH11359] FX This work was supported by the Office of High Energy Physics at the U S Department of Energy (DOE) through the Fermi Research Alliance (DE-AC02-07CH11359) and an Early Career Award to T S We would like to thank Xiaorong Wang with Lawrence Berkeley National Laboratory for useful discussion and reading the manuscript. NR 40 TC 6 Z9 6 U1 1 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD JUL PY 2015 VL 28 IS 7 AR 075014 DI 10.1088/0953-2048/28/7/075014 PG 11 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CQ9JH UT WOS:000360930000022 ER PT J AU Sung, ZH Dzyuba, A Lee, PJ Larbalestier, DC Cooley, LD AF Sung, Z-H Dzyuba, A. Lee, P. J. Larbalestier, D. C. Cooley, L. D. TI Evidence of incomplete annealing at 800 degrees C and the effects of 120 degrees C baking on the crystal orientation and the surface superconducting properties of cold-worked and chemically polished Nb SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE superconducting radio frequency; niobium; surface superconductivity; ac susceptibility; cold-work deformation ID NIOBIUM; CAVITIES; HYDROGEN; DIFFRACTION; TANTALUM; PAIR AB High-purity niobium rods were cold-worked by wire-drawing, followed by various combinations of chemical polishing and high-vacuum baking at 120 degrees C or annealing at 800 degrees C in order to better understand changes to the surface superconducting properties resulting from typical superconducting radio-frequency cavity processing. AC susceptibility measurements revealed an enhanced upper transition T-c at similar to 9.3-9.4 K in all samples that was stable through all annealing steps, a value significantly above the accepted Tc of 9.23 K for pure annealed niobium. Corresponding elevations were seen in the critical fields, the ratio of the surface critical field H-c3 to the bulk upper critical field H-c2 rising to 2.3, well above the Ginzburg-Landau value of 1.695. Orientation imaging revealed an extensive dislocation rich sub-grain structure in the as-drawn rods, a small reduction of the surface strain after baking at 120 degrees C, and a substantial but incomplete recrystallization near the surface after annealing at 800 degrees C. We interpret these changes in surface superconducting and structural properties to extensive changes in the near-surface interstitial contamination produced by baking and annealing and to synergistic interactions between H and surface O introduced during electropolishing and buffered chemical polishing. C1 [Sung, Z-H; Lee, P. J.; Larbalestier, D. C.] Natl High Magnet Field Lab, Ctr Appl Superconduct, Tallahassee, FL 32310 USA. [Dzyuba, A.; Cooley, L. D.] Fermilab Natl Accelerator Lab, Superconducting Mat Dept, Tech Div, Batavia, IL 60510 USA. [Dzyuba, A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. RP Sung, ZH (reprint author), Natl High Magnet Field Lab, Ctr Appl Superconduct, Tallahassee, FL 32310 USA. EM zsung@asc.magnet.fsu.edu RI Larbalestier, David/B-2277-2008; OI Larbalestier, David/0000-0001-7098-7208; Lee, Peter/0000-0002-8849-8995 FU US DOE [DE-SC0009960]; FNAL, Fermi Research Alliance [DE-AC02-07CH11359]; United States Department of Energy; National Science Foundation [DMR-1157490] FX This work was supported by the US DOE under awards DE-SC0009960 and FNAL, Fermi Research Alliance, DE-AC02-07CH11359 with the United States Department of Energy. The National High Magnetic Field Laboratory is supported in part by the National Science Foundation Cooperative Agreement DMR-1157490. The authors would like to thank W Starch for Nb wire-drawing in the Applied Superconductivity Center, National High Magnetic Field Laboratory, Florida State University. NR 56 TC 4 Z9 4 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD JUL PY 2015 VL 28 IS 7 AR 075003 DI 10.1088/0953-2048/28/7/075003 PG 12 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CQ9JH UT WOS:000360930000011 ER PT J AU Sanchez, JL Cooper, MJ Myers, CA Cummings, JF Vest, KG Russell, KL Sanchez, JL Hiser, MJ Gaydos, CA AF Sanchez, Jose L. Cooper, Michael J. Myers, Christopher A. Cummings, James F. Vest, Kelly G. Russell, Kevin L. Sanchez, Joyce L. Hiser, Michelle J. Gaydos, Charlotte A. TI Respiratory Infections in the US Military: Recent Experience and Control SO CLINICAL MICROBIOLOGY REVIEWS LA English DT Review ID INFLUENZA-A H1N1; COMMUNITY-ACQUIRED PNEUMONIA; HEALTH-CARE WORKERS; REAL-TIME PCR; DEPARTMENT-OF-DEFENSE; BACTEREMIC PNEUMOCOCCAL PNEUMONIA; IMMUNIZATION PRACTICES ACIP; DRUG-RESISTANT TUBERCULOSIS; RANDOMIZED CONTROLLED-TRIAL; SYNCYTIAL VIRUS-INFECTION AB This comprehensive review outlines the impact of military-relevant respiratory infections, with special attention to recruit training environments, influenza pandemics in 1918 to 1919 and 2009 to 2010, and peacetime operations and conflicts in the past 25 years. Outbreaks and epidemiologic investigations of viral and bacterial infections among high-risk groups are presented, including (i) experience by recruits at training centers, (ii) impact on advanced trainees in special settings, (iii) morbidity sustained by shipboard personnel at sea, and (iv) experience of deployed personnel. Utilizing a pathogen-by-pathogen approach, we examine (i) epidemiology, (ii) impact in terms of morbidity and operational readiness, (iii) clinical presentation and outbreak potential, (iv) diagnostic modalities, (v) treatment approaches, and (vi) vaccine and other control measures. We also outline military-specific initiatives in (i) surveillance, (ii) vaccine development and policy, (iii) novel influenza and coronavirus diagnostic test development and surveillance methods, (iv) influenza virus transmission and severity prediction modeling efforts, and (v) evaluation and implementation of nonvaccine, nonpharmacologic interventions. C1 [Sanchez, Jose L.; Cooper, Michael J.; Cummings, James F.; Vest, Kelly G.; Russell, Kevin L.; Hiser, Michelle J.] Armed Forces Hlth Surveillance Ctr, Silver Spring, MD 20910 USA. [Myers, Christopher A.] Naval Hlth Res Ctr, San Diego, CA USA. [Sanchez, Joyce L.] Mayo Clin, Div Gen Internal Med, Rochester, MN USA. [Hiser, Michelle J.] US Army Publ Hlth Command, Oak Ridge Inst Sci & Educ, Postgrad Res Participat Program, Aberdeen, MD USA. [Gaydos, Charlotte A.] Johns Hopkins Univ, Div Infect Dis, Int STD Resp & Biothreat Res Lab, Baltimore, MD USA. RP Sanchez, JL (reprint author), Armed Forces Hlth Surveillance Ctr, Silver Spring, MD 20910 USA. EM jose.l.sanchez76.ctr@mail.mil FU Global Emerging Infections Surveillance and Response Division at the Armed Forces Health Surveillance Center FX Michelle J. Hiser's work in collating routine surveillance data, reports, and publications included in this project was partially supported by an appointment to the Postgraduate Research Participation Program administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and USAPHC. This work was funded by the Global Emerging Infections Surveillance and Response Division at the Armed Forces Health Surveillance Center. NR 703 TC 6 Z9 6 U1 6 U2 28 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0893-8512 EI 1098-6618 J9 CLIN MICROBIOL REV JI Clin. Microbiol. Rev. PD JUL PY 2015 VL 28 IS 3 BP 743 EP 800 DI 10.1128/CMR.00039-14 PG 58 WC Microbiology SC Microbiology GA CQ3IH UT WOS:000360495000008 PM 26085551 ER PT J AU Thompson-Paul, AM Wei, SC Mattson, CL Robertson, M Hernandez-Romieu, AC Bell, TK Skarbinski, J AF Thompson-Paul, Angela M. Wei, Stanley C. Mattson, Christine L. Robertson, McKaylee Hernandez-Romieu, Alfonso C. Bell, Tanvir K. Skarbinski, Jacek TI Obesity Among HIV-Infected Adults Receiving Medical Care in the United States: Data From the Cross-Sectional Medical Monitoring Project and National Health and Nutrition Examination Survey SO MEDICINE LA English DT Article ID BODY-MASS INDEX; ANTIRETROVIRAL THERAPY; GENERAL-POPULATION; WEIGHT-GAIN; MORTALITY; COHORT; PREVALENCE; DISEASE; RISK; DEATH AB Our objective was to compare obesity prevalence among human immunodeficiency virus (HIV)-infected adults receiving care and the U.S. general population and identify obesity correlates among HIV-infected men and women. Cross-sectional data was collected in 2009 to 2010 from 2 nationally representative surveys: Medical Monitoring Project (MMP) and National Health and Nutrition Examination Survey (NHANES). Weighted prevalence estimates of obesity, defined as body mass index >= 30.0 kg/m(2), were compared using prevalence ratios (PR, 95% confidence interval [CI]). Correlates of obesity in HIV-infected adults were examined using multivariable logistic regression. Demographic characteristics of the 4006 HIV-infected adults in MMP differed from the 5657 adults from the general U.S. population in NHANES, including more men (73.2% in MMP versus 49.4% in NHANES, respectively), black or African Americans (41.5% versus 11.6%), persons with annual incomes <$20,000 (64.5% versus 21.9%), and homosexuals or bisexuals (50.9% versus 3.9%). HIV-infected men were less likely to be obese (PR 0.5, CI 0.5-0.6) and HIV-infected women were more likely to be obese (PR1.2, CI 1.1-1.3) compared with men and women in the general population, respectively. Among HIV-infected women, younger age was associated with obesity (60 years). Among HIV-infected men, correlates of obesity included black or African American race/ethnicity, annual income >$20,000 and <$50,000, heterosexual orientation, and geometric mean CD4+ T-lymphocyte cell count >200 cells/mu L. Obesity is common, affecting 2 in 5 HIV-infected women and 1 in 5 HIV-infected men. Correlates of obesity differ for HIV-infected men and women; therefore, different strategies may be needed for the prevention and treatment. C1 [Thompson-Paul, Angela M.; Wei, Stanley C.; Mattson, Christine L.; Robertson, McKaylee; Hernandez-Romieu, Alfonso C.; Skarbinski, Jacek] Ctr Dis Control & Prevent, Div HIV AIDS Prevent, Atlanta, GA USA. [Thompson-Paul, Angela M.] Ctr Dis Control & Prevent, Epidem Intelligence Serv, Atlanta, GA USA. [Thompson-Paul, Angela M.; Wei, Stanley C.] US PHS, Rockville, MD USA. [Robertson, McKaylee] Emory Univ, Rollins Sch Publ Hlth, Oak Ridge Inst Sci & Educ, Atlanta, GA 30322 USA. [Hernandez-Romieu, Alfonso C.] Emory Univ, Rollins Sch Publ Hlth, Dept Epidemiol, Atlanta, GA 30322 USA. [Bell, Tanvir K.] Univ Texas Med Sch Houston, Dept Internal Med, Div Infect Dis, Houston, TX USA. RP Skarbinski, J (reprint author), CDC OID NCHHSTP, Div HIV AIDS Prevent, 1600 Clifton Rd NE,Mail Stop E-46, Atlanta, GA 30329 USA. EM jskarbinski@cdc.gov FU CDC; [PS09-937] FX The CDC provides funds to all states and the District of Columbia, through a Cooperative Agreement (PS09-937), to conduct the HIV surveillance used in this study and to selected areas to conduct the MMP, and provides technical assistance to all funded areas. NR 56 TC 5 Z9 5 U1 2 U2 2 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0025-7974 EI 1536-5964 J9 MEDICINE JI Medicine (Baltimore) PD JUL PY 2015 VL 94 IS 27 AR e1081 DI 10.1097/MD.0000000000001081 PG 10 WC Medicine, General & Internal SC General & Internal Medicine GA CQ8SP UT WOS:000360879100001 PM 26166086 ER PT J AU Aquila, A Barty, A Bostedt, C Boutet, S Carini, G dePonte, D Drell, P Doniach, S Downing, KH Earnest, T Elmlund, H Elser, V Guhr, M Hajdu, J Hastings, J Hau-Riege, SP Huang, Z Lattman, EE Maia, FRNC Marchesini, S Ourmazd, A Pellegrini, C Santra, R Schlichting, I Schroer, C Spence, JCH Vartanyants, IA Wakatsuki, S Weis, WI Williams, GJ AF Aquila, A. Barty, A. Bostedt, C. Boutet, S. Carini, G. dePonte, D. Drell, P. Doniach, S. Downing, K. H. Earnest, T. Elmlund, H. Elser, V. Guehr, M. Hajdu, J. Hastings, J. Hau-Riege, S. P. Huang, Z. Lattman, E. E. Maia, F. R. N. C. Marchesini, S. Ourmazd, A. Pellegrini, C. Santra, R. Schlichting, I. Schroer, C. Spence, J. C. H. Vartanyants, I. A. Wakatsuki, S. Weis, W. I. Williams, G. J. TI The linac coherent light source single particle imaging road map SO STRUCTURAL DYNAMICS LA English DT Article ID X-RAY LASER; FREE-ELECTRON LASER; IN-FLIGHT AB Intense femtosecond x-ray pulses from free-electron laser sources allow the imaging of individual particles in a single shot. Early experiments at the Linac Coherent Light Source (LCLS) have led to rapid progress in the field and, so far, coherent diffractive images have been recorded from biological specimens, aerosols, and quantum systems with a few-tens-of-nanometers resolution. In March 2014, LCLS held a workshop to discuss the scientific and technical challenges for reaching the ultimate goal of atomic resolution with single-shot coherent diffractive imaging. This paper summarizes the workshop findings and presents the roadmap toward reaching atomic resolution, 3D imaging at free-electron laser sources. (C) 2015 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Aquila, A.; Bostedt, C.; Boutet, S.; Carini, G.; dePonte, D.; Drell, P.; Doniach, S.; Elser, V.; Hastings, J.; Huang, Z.; Pellegrini, C.; Wakatsuki, S.; Williams, G. J.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Aquila, A.; Hajdu, J.] European XFEL GmbH, D-22671 Hamburg, Germany. [Barty, A.; Santra, R.] DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany. [Drell, P.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Drell, P.; Doniach, S.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Downing, K. H.; Maia, F. R. N. C.; Marchesini, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Earnest, T.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China. [Earnest, T.] ShanghaiTech Univ, Shanghai 201210, Peoples R China. [Elmlund, H.] Monash Univ, Dept Biochem Mol Biol, Clayton, Vic 3800, Australia. [Elmlund, H.] ARC Ctr Excellence Adv Mol Imaging, Clayton, Vic 3800, Australia. [Elser, V.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Guehr, M.] SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. [Hajdu, J.; Maia, F. R. N. C.] Uppsala Univ, Dept Cell & Mol Biol, Lab Mol Biophys, S-75124 Uppsala, Sweden. [Hau-Riege, S. P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lattman, E. E.] SUNY Buffalo, BioXFEL Ctr, Buffalo, NY 14203 USA. [Lattman, E. E.] SUNY Buffalo, Dept Biol Struct, Buffalo, NY 14203 USA. [Lattman, E. E.] Hauptman Woodward Inst, Buffalo, NY 14203 USA. [Ourmazd, A.] Univ Wisconsin, Dept Phys, Milwaukee, WI 53211 USA. [Pellegrini, C.] UCLA, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Santra, R.] Univ Hamburg, Dept Phys, D-20355 Hamburg, Germany. [Schlichting, I.] Max Planck Inst Med Res, D-69120 Heidelberg, Germany. [Schroer, C.; Vartanyants, I. A.] DESY, D-22607 Hamburg, Germany. [Spence, J. C. H.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Vartanyants, I. A.] Moscow Engn Phys Inst, Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Wakatsuki, S.; Weis, W. I.] Stanford Univ, Sch Med, Stanford, CA 94305 USA. [Williams, G. J.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Bostedt, C (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM bostedt@slac.stanford.edu RI Santra, Robin/E-8332-2014; Barty, Anton/K-5137-2014 OI Santra, Robin/0000-0002-1442-9815; Barty, Anton/0000-0003-4751-2727 FU U.S. National Science Foundation [STC 1231306]; PULSE Institute at SLAC National Accelerator Laboratory - U.S. DOE Office of Basic Energy Sciences [DE-AC02-76SF00515]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-FG02-09ER16114]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Helmholtz Association; BMBF [05K2012]; Hamburg Ministry of Science and Research; Swedish Research Councils; Swedish Foundation for Strategic Research; Knut and Alice Wallenberg Foundation; European Research Council; Rontgen-Angstrom cluster; Monash University FX The Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. This work was: supported by the U.S. National Science Foundation under Award No. STC 1231306; supported through the PULSE Institute at SLAC National Accelerator Laboratory funded by the U.S. DOE Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515; was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-FG02-09ER16114; performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344; supported by The Helmholtz Association and BMBF Grant No. 05K2012 and the Hamburg Ministry of Science and Research; supported by the Swedish Research Councils, the Swedish Foundation for Strategic Research, the Knut and Alice Wallenberg Foundation, the European Research Council, and the Rontgen-Angstrom cluster. H.E. was supported by funds from Monash University. NR 28 TC 21 Z9 22 U1 5 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD JUL PY 2015 VL 2 IS 4 AR 041701 DI 10.1063/1.4918726 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ5MQ UT WOS:000360649200003 PM 26798801 ER PT J AU Coughlan, HD Darmanin, C Phillips, NW Hofmann, F Clark, JN Harder, RJ Vine, DJ Abbey, B AF Coughlan, H. D. Darmanin, C. Phillips, N. W. Hofmann, F. Clark, J. N. Harder, R. J. Vine, D. J. Abbey, B. TI Radiation damage in a micron-sized protein crystal studied via reciprocal space mapping and Bragg coherent diffractive imaging SO STRUCTURAL DYNAMICS LA English DT Article ID MACROMOLECULAR CRYSTALS; X-RAYS; CRYSTALLOGRAPHY; LYSOZYME; CRYOCRYSTALLOGRAPHY; TOMOGRAPHY; TOPOGRAPHY; RESOLUTION; NANOSCALE AB For laboratory and synchrotron based X-ray sources, radiation damage has posed a significant barrier to obtaining high-resolution structural data from biological macromolecules. The problem is particularly acute for micron-sized crystals where the weaker signal often necessitates the use of higher intensity beams to obtain the relevant data. Here, we employ a combination of techniques, including Bragg coherent diffractive imaging to characterise the radiation induced damage in a micron-sized protein crystal over time. The approach we adopt here could help screen for potential protein crystal candidates for measurement at X-ray free election laser sources. (C) 2015 Author(s). C1 [Coughlan, H. D.; Darmanin, C.; Phillips, N. W.; Abbey, B.] La Trobe Univ, Dept Chem & Phys, Australian Res Council Ctr Excellence Adv Mol Ima, Melbourne, Vic 3086, Australia. [Coughlan, H. D.; Phillips, N. W.] CSIRO Mfg Flagship, Parkville, Vic 3052, Australia. [Hofmann, F.] Univ Oxford, Dept Engn Sci, Oxford OX1 3PJ, England. [Clark, J. N.] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. [Clark, J. N.] Deutsch Elektronensynchrotron DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany. [Harder, R. J.; Vine, D. J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Abbey, B.] Melbourne Ctr Nanofabricat, Melbourne, Vic 3168, Australia. RP Darmanin, C (reprint author), La Trobe Univ, Dept Chem & Phys, Australian Res Council Ctr Excellence Adv Mol Ima, Melbourne, Vic 3086, Australia. EM C.Darmanin@latrobe.edu.au; B.Abbey@latrobe.edu.au RI Abbey, Brian/D-3274-2011; OI Abbey, Brian/0000-0001-6504-0503; Phillips, Nicholas/0000-0002-9742-7937 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; CSIRO Materials Science and Engineering Capability Development Fund; Volkswagen Foundation FX The software implementation of the phase retrieval algorithms used in this work was developed by J. N. Clark. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Part of this research was undertaken on the MX1 and MX2 beamlines at the Australian Synchrotron, Victoria, Australia. With the help and expertise of Eugeniu Balaur, this work was also performed in part at the Melbourne Centre for Nanofabrication (MCN) in the Victorian Node of the Australian National Fabrication Facility (ANFF). This work was partly funded by the CSIRO Materials Science and Engineering Capability Development Fund. The work was carried out in collaboration with the ARC centre of excellence in Coherent X-ray Science and the ARC centre of excellence in Advanced Molecular Imaging. J. N. Clark gratefully acknowledges financial support from the Volkswagen Foundation. NR 43 TC 5 Z9 5 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD JUL PY 2015 VL 2 IS 4 AR 041704 DI 10.1063/1.4919641 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ5MQ UT WOS:000360649200006 PM 26798804 ER PT J AU Dao, EH Sierra, RG Laksmono, H Lemke, HT Alonso-Mori, R Coey, A Larsen, K Baxter, EL Cohen, AE Soltis, SM DeMirci, H AF Dao, E. Han Sierra, Raymond G. Laksmono, Hartawan Lemke, Henrik T. Alonso-Mori, Roberto Coey, Aaron Larsen, Kevin Baxter, Elizabeth L. Cohen, Aina E. Soltis, S. Michael DeMirci, Hasan TI Goniometer-based femtosecond X-ray diffraction of mutant 30S ribosomal subunit crystals SO STRUCTURAL DYNAMICS LA English DT Article ID FREE-ELECTRON LASERS; PHOTOSYSTEM-II; MACROMOLECULAR CRYSTALLOGRAPHY; THERMUS-THERMOPHILUS; PROTEIN CRYSTALS; ROOM-TEMPERATURE; RADIATION-DAMAGE; DATA-COLLECTION; SOFTWARE; PULSES AB In this work, we collected radiation-damage-free data from a set of cryo-cooled crystals for a novel 30S ribosomal subunit mutant using goniometer-based femtosecond crystallography. Crystal quality assessment for these samples was conducted at the X-ray Pump Probe end-station of the Linac Coherent Light Source (LCLS) using recently introduced goniometer-based instrumentation. These 30S subunit crystals were genetically engineered to omit a 26-residue protein, Thx, which is present in the wild-type Thermus thermophilus 30S ribosomal subunit. We are primarily interested in elucidating the contribution of this ribosomal protein to the overall 30S subunit structure. To assess the viability of this study, femtosecond X-ray diffraction patterns from these crystals were recorded at the LCLS during a protein crystal screening beam time. During our data collection, we successfully observed diffraction from these difficult-to-grow 30S ribosomal subunit crystals. Most of our crystals were found to diffract to low resolution, while one crystal diffracted to 3.2 angstrom resolution. These data suggest the feasibility of pursuing high-resolution data collection as well as the need to improve sample preparation and handling in order to collect a complete radiation-damage-free data set using an X-ray Free Electron Laser. (C) 2015 Author(s). C1 [Dao, E. Han; Sierra, Raymond G.; Laksmono, Hartawan; DeMirci, Hasan] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. [Lemke, Henrik T.; Alonso-Mori, Roberto] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. [Coey, Aaron; Larsen, Kevin] Stanford Univ, Sch Med, Biophys Program, Stanford, CA 94305 USA. [Baxter, Elizabeth L.; Cohen, Aina E.; Soltis, S. Michael; DeMirci, Hasan] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. RP DeMirci, H (reprint author), SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. EM Hasan_DeMirci@Stanford.edu RI Lemke, Henrik Till/N-7419-2016 OI Lemke, Henrik Till/0000-0003-1577-8643 FU Office of Basic Energy Sciences (BES) through the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences; Department of Energy through the SLAC Laboratory Directed Research and Development Program; Stanford University Dean of Research; joint Stanford ChEM-H and SLAC National Accelerator Laboratory seed grant program. FX The authors thank Dr. Steven Gregory and Dr. Albert E. Dahlberg for the T. thermophilus Delta Thx 30S mutant strain. Portions of this research were carried out at the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory. LCLS is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. The LCLS was acknowledged for beam time access under Experiment No. xppe8814. E.H.D., H.L., R.G.S., and H.D. acknowledge the support of the Office of Basic Energy Sciences (BES) through the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, and the Department of Energy through the SLAC Laboratory Directed Research and Development Program. E.H.D. acknowledges financial support from the Stanford University Dean of Research. H.D. and S.M.S. acknowledge support from the joint Stanford ChEM-H and SLAC National Accelerator Laboratory seed grant program. H.D. also acknowledges valuable discussions with Aiko Takeuchi, Kenji Dursuncan, and Emi Satunaz. NR 47 TC 1 Z9 1 U1 2 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD JUL PY 2015 VL 2 IS 4 AR 041706 DI 10.1063/1.4919407 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ5MQ UT WOS:000360649200008 PM 26798805 ER PT J AU Ibrahim, M Chatterjee, R Hellmich, J Tran, R Bommer, M Yachandra, VK Yano, J Kern, J Zouni, A AF Ibrahim, Mohamed Chatterjee, Ruchira Hellmich, Julia Tran, Rosalie Bommer, Martin Yachandra, Vittal K. Yano, Junko Kern, Jan Zouni, Athina TI Improvements in serial femtosecond crystallography of photosystem II by optimizing crystal uniformity using microseeding procedures SO STRUCTURAL DYNAMICS LA English DT Article ID THERMOSYNECHOCOCCUS-ELONGATUS; ROOM-TEMPERATURE; RESOLUTION; PROTEIN; CRYSTALLIZATION; CYANOBACTERIAL; DIFFRACTION; MECHANISM AB In photosynthesis, photosystem II (PSII) is the multi-subunit membrane protein complex that catalyzes photo-oxidation of water into dioxygen through the oxygen evolving complex (OEC). To understand the water oxidation reaction, it is important to get structural information about the transient and intermediate states of the OEC in the dimeric PSII core complex (dPSIIcc). In recent times, femtosecond X-ray pulses from the free electron laser (XFEL) are being used to obtain X-ray diffraction (XRD) data of dPSIIcc microcrystals at room temperature that are free of radiation damage. In our experiments at the XFEL, we used an electrospun liquid microjet setup that requires microcrystals less than 40 mu m in size. In this study, we explored various microseeding techniques to get a high yield of monodisperse uniform-sized microcrystals. Monodisperse microcrystals of dPSIIcc of uniform size were a key to improve the stability of the jet and the quality of XRD data obtained at the XFEL. This was evident by an improvement of the quality of the datasets obtained, from 6.5 angstrom, using crystals grown without the micro seeding approach, to 4.5 angstrom using crystals generated with the new method. (C) 2015 Author(s). C1 [Ibrahim, Mohamed; Hellmich, Julia; Bommer, Martin; Zouni, Athina] Humboldt Univ, Inst Biol, D-10099 Berlin, Germany. [Ibrahim, Mohamed; Hellmich, Julia; Zouni, Athina] Tech Univ Berlin, Max Volmer Lab Biophys Chem, D-10623 Berlin, Germany. [Chatterjee, Ruchira; Tran, Rosalie; Yachandra, Vittal K.; Yano, Junko; Kern, Jan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kern, Jan] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. RP Ibrahim, M (reprint author), Humboldt Univ, Inst Biol, D-10099 Berlin, Germany. EM jyano@lbl.gov; jfkern@lbl.gov; athina.zouni@hu-berlin.de FU NIH Grant [GM055302]; Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB) of the Department of Energy (DOE) [DE-AC02-05CH11231]; DFG-Cluster of Excellence "UniCat" [Sfb1078] FX This work was supported by NIH Grant No. GM055302 (V.K.Y) for PSII biochemistry, structure, and mechanism; the Director, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB) of the Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 (J.Y. and V.K.Y) for X-ray methodology and instrumentation. The DFG-Cluster of Excellence "UniCat" coordinated by the Technische Universitat Berlin and Sfb1078, TP A5 (A.Z., M.I., and M.B.); the Alexander von Humboldt Foundation (J.K.); and the Human Frontiers Science Project Award No. RGP0063/2013 (J.Y. and A.Z.). We thank the staff at LCLS/SLAC and the staff at ALS (BL5.0.2) and BESSY for support of synchrotron experiments. Portions of this research were carried out at the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory. LCLS is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. We thank I. Seuffert and D. DiFiore (Sfb1078, project A5) for their excellent technical assistance. NR 30 TC 6 Z9 6 U1 1 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD JUL PY 2015 VL 2 IS 4 AR 041705 DI 10.1063/1.4919741 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CQ5MQ UT WOS:000360649200007 ER PT J AU Angyal, A Ilyas, Z Hadadi, E Johnston, J Ariaans, M Kraus, R Wilson, H Bauer, R Rader, D Francis, S Kiss-Toth, E AF Angyal, A. Ilyas, Z. Hadadi, E. Johnston, J. Ariaans, M. Kraus, R. Wilson, H. Bauer, R. Rader, D. Francis, S. Kiss-Toth, E. TI DOES MYELOID EXPRESSION OF TRIB1 REGULATE PLASMA LIPID LEVELS? SO ATHEROSCLEROSIS LA English DT Meeting Abstract CT 83rd Congress of the European-Atherosclerosis-Society (EAS) CY MAR 22-25, 2015 CL Glasgow, SCOTLAND SP European Atherosclerosis Soc C1 [Angyal, A.; Ilyas, Z.; Hadadi, E.; Johnston, J.; Ariaans, M.; Wilson, H.; Francis, S.; Kiss-Toth, E.] Univ Sheffield, Cardiovasc Dept, Sheffield, S Yorkshire, England. [Kraus, R.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA USA. [Bauer, R.; Rader, D.] Univ Penn, Cardiovasc Inst, Philadelphia, PA 19104 USA. [Bauer, R.; Rader, D.] Univ Penn, Inst Translat Med & Therapeut, Philadelphia, PA 19104 USA. RI Kiss-Toth, Endre/A-8596-2014 OI Kiss-Toth, Endre/0000-0003-4406-4017 NR 0 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0021-9150 EI 1879-1484 J9 ATHEROSCLEROSIS JI Atherosclerosis PD JUL PY 2015 VL 241 IS 1 MA EAS-0387 BP E34 EP E34 PG 1 WC Cardiac & Cardiovascular Systems; Peripheral Vascular Disease SC Cardiovascular System & Cardiology GA CP7WS UT WOS:000360100600105 ER PT J AU Li, T Wang, L Ku, X Guell, BM Lovas, T Shaddix, CR AF Li, Tian Wang, Liang Ku, Xiaoke Guell, Berta Matas Lovas, Terese Shaddix, Christopher R. TI Experimental and Modeling Study of the Effect of Torrefaction on the Rapid Devolatilization of Biomass SO ENERGY & FUELS LA English DT Article; Proceedings Paper CT 2nd International Conference Biogas Science CY 2014 CL Vienna, AUSTRIA ID COAL DEVOLATILIZATION; PYROLYSIS CONDITIONS; HEATING RATE; KINETICS; PARTICLE; WOOD; PREDICTIONS; COMBUSTION; FLASHCHAIN; REACTOR AB In the present work, experimental and computational fluid dynamics (CFD) approaches were proposed and applied to assess rapid devolatilization behaviors of four types of biomass (forest residue, torrefied forest residue, Norwegian spruce, and torrefied Norwegian spruce). Biomass particles were subjected to devolatilization experiments at 1073 and 1473 K in a drop-tube reactor. Torrefaction was found to have consistent effects on the size reduction of studied biomass. In addition, similar behaviors of char fragmentation were observed for tested torrefied biomass after rapid devolatilization at 1473 K. Mass loss during devolatilization of biomass was highly dependent on heating condition. Both rates and extents of devolatilization of biomass were increased at elevated temperatures and heating rates. In comparison with raw feedstock, high char yields were realized with the torrefied biomass after devolatilization experiments. Evolution of elemental composition of studied biomass was found to be insensitive to tested conditions. However, organic composition of char was strongly affected by elemental composition of fuel, thus also influenced by torrefaction. CFD simulation showed that sizes of fuel particles had decisive effects on residence time of them in the reactor, especially particles with diameter larger than 355 mu m. Particle temperature, in contrast, depended on both particle diameter and particle density. A modified two-competing-rates devolatilization model was also presented in the present work. On the basis of experimental data, one optimal set of kinetic parameters was obtained following a proposed procedure. The model predicted well the mass loss of all tested fuel and the evolution of each organic element in char at all operation conditions. C1 [Li, Tian; Ku, Xiaoke; Lovas, Terese] Norwegian Univ Sci & Technol, Dept Energy & Proc Engn, N-7491 Trondheim, Norway. [Wang, Liang; Guell, Berta Matas] SINTEF Energy Res, N-7465 Trondheim, Norway. [Shaddix, Christopher R.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. RP Li, T (reprint author), Norwegian Univ Sci & Technol, Dept Energy & Proc Engn, Kolbjorn Hejes Vei 1b, N-7491 Trondheim, Norway. EM tian.li@ntnu.no OI Li, Tian/0000-0002-4248-8396; Wang, Liang/0000-0002-1458-7653 FU Research Council of Norway; Sandia Laboratory's Directed Research and Development (LDRD) program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was carried out within the GasBio project, funded by Research Council of Norway and industry partners. Support was also provided through Sandia Laboratory's Directed Research and Development (LDRD) program. We thank Manfred Geier for his assistance with the experiments at Sandia. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 34 TC 5 Z9 5 U1 3 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD JUL PY 2015 VL 29 IS 7 BP 4328 EP 4338 DI 10.1021/acs.energyfuels.5b00348 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CP6VS UT WOS:000360026900036 ER PT J AU Engebretson, MJ Posch, JL Wygant, JR Kletzing, CA Lessard, MR Huang, CL Spence, HE Smith, CW Singer, HJ Omura, Y Horne, RB Reeves, GD Baker, DN Gkioulidou, M Oksavik, K Mann, IR Raita, T Shiokawa, K AF Engebretson, M. J. Posch, J. L. Wygant, J. R. Kletzing, C. A. Lessard, M. R. Huang, C. -L. Spence, H. E. Smith, C. W. Singer, H. J. Omura, Y. Horne, R. B. Reeves, G. D. Baker, D. N. Gkioulidou, M. Oksavik, K. Mann, I. R. Raita, T. Shiokawa, K. TI Van Allen probes, NOAA, GOES, and ground observations of an intense EMIC wave event extending over 12 h in magnetic local time SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE EMIC waves; radiation belts; magnetospheric compressions ID ION-CYCLOTRON WAVES; RELATIVISTIC ELECTRON-PRECIPITATION; SUBAURORAL PROTON PRECIPITATION; PITCH-ANGLE SCATTERING; EQUATORIAL MAGNETOSPHERE; ENERGETIC PARTICLE; GEOMAGNETIC STORMS; RADIATION BELTS; PULSATIONS; EMISSIONS AB Although most studies of the effects of electromagnetic ion cyclotron (EMIC) waves on Earth's outer radiation belt have focused on events in the afternoon sector in the outer plasmasphere or plume region, strong magnetospheric compressions provide an additional stimulus for EMIC wave generation across a large range of local times and L shells. We present here observations of the effects of a wave event on 23 February 2014 that extended over 8h in UT and over 12h in local time, stimulated by a gradual 4h rise and subsequent sharp increases in solar wind pressure. Large-amplitude linearly polarized hydrogen band EMIC waves (up to 25nT p-p) appeared for over 4h at both Van Allen Probes, from late morning through local noon, when these spacecraft were outside the plasmapause, with densities similar to 5-20cm(-3). Waves were also observed by ground-based induction magnetometers in Antarctica (near dawn), Finland (near local noon), Russia (in the afternoon), and in Canada (from dusk to midnight). Ten passes of NOAA-POES and METOP satellites near the northern foot point of the Van Allen Probes observed 30-80keV subauroral proton precipitation, often over extended L shell ranges; other passes identified a narrow L shell region of precipitation over Canada. Observations of relativistic electrons by the Van Allen Probes showed that the fluxes of more field-aligned and more energetic radiation belt electrons were reduced in response to both the emission over Canada and the more spatially extended emission associated with the compression, confirming the effectiveness of EMIC-induced loss processes for this event. C1 [Engebretson, M. J.; Posch, J. L.] Augsburg Coll, Dept Phys, Minneapolis, MN 55454 USA. [Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Lessard, M. R.; Huang, C. -L.; Spence, H. E.; Smith, C. W.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Singer, H. J.] NOAA, Boulder, CO USA. [Omura, Y.] Kyoto Univ, Res Inst Sustainable Humanosphere, Kyoto, Japan. [Horne, R. B.] British Antarctic Survey, Cambridge CB3 0ET, England. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Boulder, CO 80309 USA. [Gkioulidou, M.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. [Oksavik, K.] Univ Bergen, Birkeland Ctr Space Sci, Dept Phys & Technol, Bergen, Norway. [Oksavik, K.] Univ Ctr Svalbard, Longyearbyen, Norway. [Mann, I. R.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Mann, I. R.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Raita, T.] Univ Oulu, Sodankyla Geophys Observ, Sodankyla, Finland. [Shiokawa, K.] Nagoya Univ, STELAB, Toyokawa, Japan. RP Engebretson, MJ (reprint author), Augsburg Coll, Dept Phys, Minneapolis, MN 55454 USA. EM engebret@augsburg.edu RI Reeves, Geoffrey/E-8101-2011; Gkioulidou, Matina/G-9009-2015; Omura, Yoshiharu/P-8565-2014; OI Reeves, Geoffrey/0000-0002-7985-8098; Gkioulidou, Matina/0000-0001-9979-2164; Omura, Yoshiharu/0000-0002-6683-3940; Horne, Richard/0000-0002-0412-6407; Kletzing, Craig/0000-0002-4136-3348; Oksavik, Kjellmar/0000-0003-4312-6992 FU NSF [ANT-1142045, PLR-1341493, ANT-1141987, PLR-1341677]; Van Allen Probes mission; NASA [NAS5-01072]; Research Council of Norway [223252, 212014] FX This research was supported by NSF grants ANT-1142045 and PLR-1341493 to Augsburg College and NSF grants ANT-1141987 and PLR-1341677 to the University of New Hampshire. Work performed by M.J.E. at NASA/GSFC was supported by the Van Allen Probes mission. Van Allen Probes research at the University of Minnesota, University of Iowa, University of New Hampshire, and Los Alamos National Laboratory was supported by NASA prime contract NAS5-01072 to The Johns Hopkins University Applied Physics Laboratory. Work performed by K.O. at the University of Bergen was supported by the Research Council of Norway under contracts 223252 and 212014. We thank David Sibeck, Brian Anderson, Shrikanth Kanekal, Sasha Ukhorskiy, Yuri Shprits, Viacheslav Pilipenko, Finn Soraas, and Barry Mauk for helpful comments The Halley research station in Antarctica is operated by the British Antarctic Survey. We thank R.A. Rakhmatulin for providing Mondy induction magnetometer data, we thank the referees for their helpful comments, and we gratefully acknowledge use of NASA/GSFC's Space Physics Data Facility's OMNIWeb, SSCweb, and CDAWeb data. NR 76 TC 24 Z9 24 U1 3 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2015 VL 120 IS 7 BP 5465 EP 5488 DI 10.1002/2015JA021227 PG 24 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ1TF UT WOS:000360381400018 ER PT J AU Allen, RC Zhang, JC Kistler, LM Spence, HE Lin, RL Klecker, B Dunlop, MW Andre, M Jordanova, VK AF Allen, R. C. Zhang, J. -C. Kistler, L. M. Spence, H. E. Lin, R. -L. Klecker, B. Dunlop, M. W. Andre, M. Jordanova, V. K. TI A statistical study of EMIC waves observed by Cluster: 1. Wave properties SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE magnetosphere; EMIC waves; Cluster; Shabansky orbits ID ION-CYCLOTRON WAVES; 1-2 MAGNETIC PULSATIONS; DAWN-DUSK ASYMMETRY; EQUATORIAL MAGNETOSPHERE; GLOBAL CHARACTERISTICS; EARTHS MAGNETOSPHERE; SOURCE REGION; HEAVY-IONS; INSTABILITY; MODEL AB Electromagnetic ion cyclotron (EMIC) waves are an important mechanism for particle energization and losses inside the magnetosphere. In order to better understand the effects of these waves on particle dynamics, detailed information about the occurrence rate, wave power, ellipticity, normal angle, energy propagation angle distributions, and local plasma parameters are required. Previous statistical studies have used in situ observations to investigate the distribution of these parameters in the magnetic local time versus L-shell (MLT-L) frame within a limited magnetic latitude (MLAT) range. In this study, we present a statistical analysis of EMIC wave properties using 10years (2001-2010) of data from Cluster, totaling 25,431min of wave activity. Due to the polar orbit of Cluster, we are able to investigate EMIC waves at all MLATs and MLTs. This allows us to further investigate the MLAT dependence of various wave properties inside different MLT sectors and further explore the effects of Shabansky orbits on EMIC wave generation and propagation. The statistical analysis is presented in two papers. This paper focuses on the wave occurrence distribution as well as the distribution of wave properties. The companion paper focuses on local plasma parameters during wave observations as well as wave generation proxies. C1 [Allen, R. C.; Zhang, J. -C.; Kistler, L. M.; Spence, H. E.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Lin, R. -L.] Chinese Acad Sci, Natl Space Sci Ctr, Beijing, Peoples R China. [Klecker, B.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Dunlop, M. W.] Rutherford Appleton Lab, Div Space Sci, Harwell, Oxon, England. [Andre, M.] Swedish Inst Space Phys IRF, Uppsala, Sweden. [Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Allen, RC (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. EM robert.allen@swri.edu RI Allen, Robert/F-5187-2011 OI Jordanova, Vania/0000-0003-0475-8743; Allen, Robert/0000-0003-2079-5683 FU NASA [NNX11AO82G, NNX11AB65G]; RBSP-ECT - JHU/APL Contract under NASA's Prime Contract [967399, NAS5-01072] FX NASA supported work at UNH under grants NNX11AO82G and NNX11AB65G. This work was also supported by RBSP-ECT funding provided by JHU/APL Contract 967399 under NASA's Prime Contract NAS5-01072. The authors thank the Cluster team for their data and software. C. Torrence and G. Compo at University of Colorado and the THEMIS Science Support Team supplied IDL routines for the polarization and normal angle analysis, which are available at URL: http://themis.ssl.berkeley.edu/software.shtml. N. A. Tsyganenko of University of St.-Petersburg in the Russian Federation and H. Korth of JHU/APL provided the Tsyganenko magnetic field model and the IDL/Geopack module. Solar wind plasma/IMF data, Dst, and Kp indices were obtained from the GSFC/SPDF OMNIWeb interface at URL: http://omniweb.gsfc.nasa.gov. The authors would also like to thank the Cluster instrument teams (FGM and EFW) along with the Cluster Science Archive URL: http://www.cosmos.esa.int/web/csa. Finally, we would like to thank UCLA for the website on statistical analysis methods URL: http://statistics.ats.ucla.edu/stat/mult_pkg/whatstat/. NR 71 TC 24 Z9 24 U1 1 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2015 VL 120 IS 7 BP 5574 EP 5592 DI 10.1002/2015JA021333 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ1TF UT WOS:000360381400024 ER PT J AU Damiano, PA Johnson, JR Chaston, CC AF Damiano, P. A. Johnson, J. R. Chaston, C. C. TI Ion temperature effects on magnetotail Alfven wave propagation and electron energization SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE electron acceleration; kinetic Alfven waves; kinetic simulations; magnetosphere-ionosphere coupling; ion gyroradius effects ID PLASMA SHEET; SMALL-SCALE; MAGNETOSPHERIC PLASMA; AURORAL ELECTRONS; R-E; ACCELERATION; SIMULATIONS; DISPERSION AB A new 2-D self-consistent hybrid gyrofluid-kinetic electron model in dipolar coordinates is presented and used to simulate dispersive-scale Alfven wave pulse propagation from the equator to the ionosphere along an L = 10 magnetic field line. The model is an extension of the hybrid MHD-kinetic electron model that incorporates ion Larmor radius corrections via the kinetic fluid model of Cheng and Johnson (1999). It is found that consideration of a realistic ion to electron temperature ratio decreases the propagation time of the wave from the plasma sheet to the ionosphere by several seconds relative to a (i)=0 case (which also implies shorter timing for a substorm onset signal) and leads to significant dispersion of wave energy perpendicular to the ambient magnetic field. Additionally, ion temperature effects reduce the parallel current and electron energization all along the field line for the same magnitude perpendicular electric field perturbation. C1 [Damiano, P. A.; Johnson, J. R.] Princeton Univ, Princeton Plasma Phys Lab, Princeton Ctr Heliophys, Princeton, NJ 08543 USA. [Chaston, C. C.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Chaston, C. C.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. RP Damiano, PA (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton Ctr Heliophys, POB 451, Princeton, NJ 08543 USA. EM pdamiano@pppl.gov FU NASA [NNH11AR071, NNX14AM27G, NNH14AY20I, NNX13XAE12G, NNX15AJ01G]; NSF [AGS1203299]; Australian Research Council [FT110100316]; U.S. Department of Energy [DE-AC02-09CH11466]; CISL project [UPR10002] FX The authors thank the referees for many comments which significantly improved the manuscript. P.A.D. also acknowledges useful discussions with Will Fox regarding nonlinear trapping effects. The authors acknowledge support from NASA grants (NNH11AR071, NNX14AM27G, NNH14AY20I, NNX13XAE12G, and NNX15AJ01G) and NSF grant (AGS1203299). C. Chaston also acknowledges support from Australian Research Council grant FT110100316. This manuscript was authored by Princeton University under contract DE-AC02-09CH11466 with the U.S. Department of Energy. This work was facilitated by the Max-Planck/Princeton Center for Plasma Physics. The numerical data used in the figures may be obtained by contacting the corresponding author. Computing resources were provided by the Princeton Plasma Physics Laboratory and the National Center for Atmospheric Research (under CISL project UPR10002). NR 41 TC 3 Z9 3 U1 0 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2015 VL 120 IS 7 BP 5623 EP 5632 DI 10.1002/2015JA021074 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ1TF UT WOS:000360381400028 ER PT J AU Claudepierre, SG O'Brien, TP Blake, JB Fennell, JF Roeder, JL Clemmons, JH Looper, MD Mazur, JE Mulligan, TM Spence, HE Reeves, GD Friedel, RHW Henderson, MG Larsen, BA AF Claudepierre, S. G. O'Brien, T. P. Blake, J. B. Fennell, J. F. Roeder, J. L. Clemmons, J. H. Looper, M. D. Mazur, J. E. Mulligan, T. M. Spence, H. E. Reeves, G. D. Friedel, R. H. W. Henderson, M. G. Larsen, B. A. TI A background correction algorithm for Van Allen Probes MagEIS electron flux measurements SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE radiation belt; inner radiation belt; background contamination; spacecraft engineering; outer radiation belt; particle measurements ID RELATIVISTIC ELECTRONS; RADIATION BELT; SLOT REGION; ENVIRONMENT; PARTICLE; MODEL AB We describe an automated computer algorithm designed to remove background contamination from the Van Allen Probes Magnetic Electron Ion Spectrometer (MagEIS) electron flux measurements. We provide a detailed description of the algorithm with illustrative examples from on-orbit data. We find two primary sources of background contamination in the MagEIS electron data: inner zone protons and bremsstrahlung X-rays generated by energetic electrons interacting with the spacecraft material. Bremsstrahlung X-rays primarily produce contamination in the lower energy MagEIS electron channels (approximate to 30-500keV) and in regions of geospace where multi-MeV electrons are present. Inner zone protons produce contamination in all MagEIS energy channels at roughly L < 2.5. The background-corrected MagEIS electron data produce a more accurate measurement of the electron radiation belts, as most earlier measurements suffer from unquantifiable and uncorrectable contamination in this harsh region of the near-Earth space environment. These background-corrected data will also be useful for spacecraft engineering purposes, providing ground truth for the near-Earth electron environment and informing the next generation of spacecraft design models (e.g., AE9). C1 [Claudepierre, S. G.; O'Brien, T. P.; Blake, J. B.; Fennell, J. F.; Roeder, J. L.; Clemmons, J. H.; Looper, M. D.; Mazur, J. E.; Mulligan, T. M.] Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.; Friedel, R. H. W.; Henderson, M. G.; Larsen, B. A.] Los Alamos Natl Lab, Space & Atmospher Sci Grp, Los Alamos, NM USA. RP Claudepierre, SG (reprint author), Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. EM seth@aero.org RI Reeves, Geoffrey/E-8101-2011; Henderson, Michael/A-3948-2011; Claudepierre, Seth/A-6109-2012; OI Reeves, Geoffrey/0000-0002-7985-8098; Henderson, Michael/0000-0003-4975-9029; Clemmons, James/0000-0002-5298-5222 FU RBSP-ECT - JHU/APL contract under NASA [967399, NAS5-01072]; NASA [NNX10AK93G]; U.S. Department of Energy; NASA Van Allen Probes mission FX This work was supported by RBSP-ECT funding provided by JHU/APL contract 967399 under NASA's prime contract NAS5-01072. Work at JHU/APL was supported by NASA grant NNX10AK93G. Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy, with support from the NASA Van Allen Probes mission. All of the level 2+ Van Allen Probes data used in this manuscript are in the public domain and accessible from the Van Allen Probes Science Gateway (www.rbsp-ect.lanl.gov/data_pub/). Level 1 MagEIS histogram data can be made available by contacting the lead author (S.G.C.). One author (S.G.C.) would like to thank Jeremy Faden and all of the developers of Autoplot. NR 24 TC 13 Z9 13 U1 1 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2015 VL 120 IS 7 BP 5703 EP 5727 DI 10.1002/2015JA021171 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ1TF UT WOS:000360381400035 ER PT J AU Lay, EH Shao, XM Kendrick, AK Carrano, CS AF Lay, Erin H. Shao, Xuan-Min Kendrick, Alexander K. Carrano, Charles S. TI Ionospheric acoustic and gravity waves associated with midlatitude thunderstorms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE ionosphere; thunderstorms; acoustic waves; gravity waves; troposphere; ionosphere coupling ID TOTAL ELECTRON-CONTENT; SEVERE WEATHER; DISTURBANCES; INFRASOUND; CONVECTION; RESPONSES; SPRITES AB Acoustic waves with periods of 2-4min and gravity waves with periods of 6-16min have been detected at ionospheric heights (250-350km) using GPS total electron content measurements. The area disturbed by these waves and the wave amplitudes have been associated with underlying thunderstorm activity. A statistical study comparing Next Generation Weather Radar thunderstorm measurements with ionospheric acoustic and gravity waves in the midlatitude U.S. Great Plains region was performed for the time period of May-July 2005. An increase of ionospheric acoustic wave disturbed area and amplitude is primarily associated with large thunderstorms (mesoscale convective systems). Ionospheric gravity wave disturbed area and amplitude scale with thunderstorm activity, with even small storms (i.e., individual storm cells) producing an increase of gravity waves. C1 [Lay, Erin H.; Shao, Xuan-Min; Kendrick, Alexander K.] Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM 87545 USA. [Carrano, Charles S.] Boston Coll, Inst Sci Res, Boston, MA USA. RP Lay, EH (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM 87545 USA. EM elay@lanl.gov OI Kendrick, Alexander/0000-0002-0472-2575; Lay, Erin/0000-0002-1310-9035 FU Los Alamos National Laboratory's Laboratory Directed Research and Development (LDRD) project [20130737ECR] FX This research was supported by the Los Alamos National Laboratory's Laboratory Directed Research and Development (LDRD) project 20130737ECR. Ground-based GPS receiver data used in this study were downloaded from http://geodesy.noaa.gov/CORS/. NEXRAD radar data were downloaded from http://www.roc.noaa.gov/WSR88D/. Los Alamos Sferic Array data used in the analysis can be released through official Los Alamos National Laboratory's release policy after a request is made to authors E.H.L. or X.-M.S. NR 28 TC 3 Z9 3 U1 1 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2015 VL 120 IS 7 BP 6010 EP 6020 DI 10.1002/2015JA021334 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ1TF UT WOS:000360381400057 ER PT J AU Mittal, S Vetter, JS AF Mittal, Sparsh Vetter, Jeffrey S. TI A Survey of CPU-GPU Heterogeneous Computing Techniques SO ACM COMPUTING SURVEYS LA English DT Article DE Experimentation; Management; Measurement; Performance; Analysis; CPU-GPU heterogeneous/hybrid/collaborative computing; workload division/partitioning; dynamic/static load balancing; pipelining; programming frameworks; fused CPU-GPU chip ID MULTI-GPU; SYSTEMS; MODEL; ARCHITECTURES; COMPUTATION; SIMULATIONS; PERFORMANCE; EXECUTION; TIME; IMPLEMENTATION AB As both CPUs and GPUs become employed in a wide range of applications, it has been acknowledged that both of these Processing Units (PUs) have their unique features and strengths and hence, CPU-GPU collaboration is inevitable to achieve high-performance computing. This has motivated a significant amount of research on heterogeneous computing techniques, along with the design of CPU-GPU fused chips and petascale heterogeneous supercomputers. In this article, we survey Heterogeneous Computing Techniques (HCTs) such as workload partitioning that enable utilizing both CPUs and GPUs to improve performance and/or energy efficiency. We review heterogeneous computing approaches at runtime, algorithm, programming, compiler, and application levels. Further, we review both discrete and fused CPU-GPU systems and discuss benchmark suites designed for evaluating Heterogeneous Computing Systems (HCSs). We believe that this article will provide insights into the workings and scope of applications of HCTs to researchers and motivate them to further harness the computational powers of CPUs and GPUs to achieve the goal of exascale performance. C1 [Mittal, Sparsh; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Vetter, Jeffrey S.] Georgia Tech, Atlanta, GA USA. RP Mittal, S (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,Bldg 5100,MS-6173, Oak Ridge, TN 37830 USA. EM mittals@ornl.gov; vetter@ornl.gov FU U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research FX Support for this work was provided by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research. NR 190 TC 4 Z9 4 U1 2 U2 15 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0360-0300 EI 1557-7341 J9 ACM COMPUT SURV JI ACM Comput. Surv. PD JUL PY 2015 VL 47 IS 4 AR 69 DI 10.1145/2788396 PG 35 WC Computer Science, Theory & Methods SC Computer Science GA CP6NY UT WOS:000360005500015 ER PT J AU Hegerl, GC Black, E Allan, RP Ingram, WJ Polson, D Trenberth, KE Chadwick, RS Arkin, PA Sarojini, BB Becker, A Dai, AG Durack, PJ Easterling, D Fowler, HJ Kendon, EJ Huffman, GJ Liu, CL Marsh, R New, M Osborn, TJ Skliris, N Stott, PA Vidale, PL Wijffels, SE Wilcox, LJ Willett, KM Zhang, XB AF Hegerl, Gabriele C. Black, Emily Allan, Richard P. Ingram, William J. Polson, Debbie Trenberth, Kevin E. Chadwick, Robin S. Arkin, Phillip A. Sarojini, Beena Balan Becker, Andreas Dai, Aiguo Durack, Paul J. Easterling, David Fowler, Hayley J. Kendon, Elizabeth J. Huffman, George J. Liu, Chunlei Marsh, Robert New, Mark Osborn, Timothy J. Skliris, Nikolaos Stott, Peter A. Vidale, Pier-Luigi Wijffels, Susan E. Wilcox, Laura J. Willett, Kate M. Zhang, Xuebin TI CHALLENGES IN QUANTIFYING CHANGES IN THE GLOBAL WATER CYCLE SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID EXPLAINING EXTREME EVENTS; CLIMATE-CHANGE; PRECIPITATION EXTREMES; ANTHROPOGENIC AEROSOLS; TROPICAL PRECIPITATION; HYDROLOGICAL CYCLE; SURFACE HUMIDITY; INTENSE PRECIPITATION; REGIONAL PERSPECTIVE; NORTHERN-HEMISPHERE C1 [Hegerl, Gabriele C.; Polson, Debbie] Univ Edinburgh, Sch GeoSci, Grant Inst, Edinburgh EH8 9YL, Midlothian, Scotland. [Black, Emily; Allan, Richard P.; Sarojini, Beena Balan; Liu, Chunlei; Vidale, Pier-Luigi; Wilcox, Laura J.] Univ Reading, Dept Meteorol, Natl Ctr Atmospher Sci Climate, Reading, Berks, England. [Ingram, William J.; Chadwick, Robin S.; Kendon, Elizabeth J.; Stott, Peter A.; Willett, Kate M.] Hadley Ctr, Met Off, Exeter, Devon, England. [Ingram, William J.] Univ Oxford, Dept Phys, Oxford, England. [Trenberth, Kevin E.; Dai, Aiguo] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Arkin, Phillip A.] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. [Becker, Andreas] Deutsch Wetterdienst, Offenbach, Germany. [Dai, Aiguo] SUNY Albany, Dept Atmospher & Environm Sci, Albany, NY 12222 USA. [Durack, Paul J.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA USA. [Durack, Paul J.; Wijffels, Susan E.] CSIRO, Hobart, Tas, Australia. [Easterling, David] NOAA, Natl Climat Data Ctr, Asheville, NC USA. [Fowler, Hayley J.] Newcastle Univ, Sch Civil Engn & Geosci, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Huffman, George J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Marsh, Robert; Skliris, Nikolaos] Univ Southampton, Ocean & Earth Sci, Southampton, Hants, England. [New, Mark] Univ Cape Town, ZA-7700 Cape Town, South Africa. [Osborn, Timothy J.] Univ E Anglia, Sch Environm Sci, Climat Res Unit, Norwich NR4 7TJ, Norfolk, England. [Zhang, Xuebin] Environm Canada, Div Climate Res, Toronto, ON, Canada. RP Hegerl, GC (reprint author), Grant Inst, GeoSci, Kings Bldg,James Hutton Rd, Edinburgh EH9 3FE, Midlothian, Scotland. EM gabi.hegerl@ed.ac.uk RI Trenberth, Kevin/A-5683-2012; Allan, Richard/B-5782-2008; Dai, Aiguo/D-3487-2009; New, Mark/A-7684-2008; Huffman, George/F-4494-2014; Durack, Paul/A-8758-2010; Stott, Peter/N-1228-2016; OI Trenberth, Kevin/0000-0002-1445-1000; Allan, Richard/0000-0003-0264-9447; Fowler, Hayley/0000-0001-8848-3606; New, Mark/0000-0001-6082-8879; Huffman, George/0000-0003-3858-8308; Durack, Paul/0000-0003-2835-1438; Stott, Peter/0000-0003-4853-7686; Vidale, Pier Luigi/0000-0002-1800-8460; Marsh, Robert/0000-0002-1051-8749 FU U.K. Natural Environment Research Council (NERC) [NE/I006672/1]; DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; Lawrence Livermore National Laboratory - U.S. Department of Energy [DE-AC52-07NA27344]; NERC [NE/I00680X/1]; NCAS; NASA [NNX11AG69G]; PAGODA project of the Changing Water Cycle programme of NERC [NE/I006672/1]; ERC [EC320691]; NSF [AGS-1353740]; Wolfson Foundation; Royal Society as Royal Society Wolfson Research Merit Award [WM140025, WM130060]; European Research Council (TITAN) [ERC-2012-AdG 320691]; CONVEX project of the Changing Water Cycle programme of NERC [NE/I006680/1]; European Research Council FX We thank several anonymous reviewers for their helpful and perceptive suggestions. The workshop that formed the basis for this paper was funded by the U.K. Natural Environment Research Council (NERC Grant NE/I006672/1). We thank Eleanor Blyth and David Parker for comments. Robin Chadwick, Kate Willett, William Ingram, Lizzie Kendon, and Peter Stott were supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). Paul Durack is supported by the Lawrence Livermore National Laboratory that is funded by the U.S. Department of Energy under Contract DE-AC52-07NA27344, and William Ingram is partly supported by NERC Grant NE/I00680X/1. Gabi Hegerl and Richard Allan are partly supported by NCAS. Kevin Trenberth is supported by NASA Grant NNX11AG69G. P. L. Vidale, R. P. Allan, B. Balan Sarojini, C. Liu, E. Black, P. Stott, G. Hegerl, D. Polson, R. Marsh, N. Skliris, and Laura Wilcox are supported by the PAGODA project of the Changing Water Cycle programme of NERC under Grant NE/I006672/1. G. Hegerl and D. Polson are supported by the ERC Grant EC320691. A. Dai acknowledges the support of NSF Grant AGS-1353740. H. J. Fowler and G. Hegerl are funded by the Wolfson Foundation and the Royal Society as Royal Society Wolfson Research Merit Award (WM140025 and WM130060, respectively) holders. G. Hegerl is further supported by the European Research Council (TITAN, ERC-2012-AdG 320691). H. J. Fowler is supported by the CONVEX project of the Changing Water Cycle programme of NERC under Grant NE/I006680/1 and European Research Council funded INTENSE (ERC-2013-CoG). NR 164 TC 16 Z9 16 U1 14 U2 62 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 EI 1520-0477 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD JUL PY 2015 VL 96 IS 7 BP 1097 EP 1115 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CP4LX UT WOS:000359854600004 ER PT J AU Pelletier, JD Murray, AB Pierce, JL Bierman, PR Breshears, DD Crosby, BT Ellis, M Foufoula-Georgiou, E Heimsath, AM Houser, C Lancaster, N Marani, M Merritts, DJ Moore, LJ Pederson, JL Poulos, MJ Rittenour, TM Rowland, JC Ruggiero, P Ward, DJ Wickert, AD Yager, EM AF Pelletier, Jon D. Murray, A. Brad Pierce, Jennifer L. Bierman, Paul R. Breshears, David D. Crosby, Benjamin T. Ellis, Michael Foufoula-Georgiou, Efi Heimsath, Arjun M. Houser, Chris Lancaster, Nick Marani, Marco Merritts, Dorothy J. Moore, Laura J. Pederson, Joel L. Poulos, Michael J. Rittenour, Tammy M. Rowland, Joel C. Ruggiero, Peter Ward, Dylan J. Wickert, Andrew D. Yager, Elowyn M. TI Forecasting the response of Earth's surface to future climatic and land use changes: A review of methods and research needs SO EARTHS FUTURE LA English DT Review DE global change; Earth-surface processes; forecasting ID SEA-LEVEL RISE; LAST GLACIAL MAXIMUM; SOUTHWESTERN UNITED-STATES; LANDSCAPE EVOLUTION MODEL; BEDROCK RIVER INCISION; CANADIAN ARCTIC ARCHIPELAGO; YELLOWSTONE-NATIONAL-PARK; STRATH-TERRACE FORMATION; FLUVIAL THERMAL EROSION; UPPER MISSISSIPPI RIVER AB In the future, Earth will be warmer, precipitation events will be more extreme, global mean sea level will rise, and many arid and semiarid regions will be drier. Human modifications of landscapes will also occur at an accelerated rate as developed areas increase in size and population density. We now have gridded global forecasts, being continually improved, of the climatic and land use changes (C&LUC) that are likely to occur in the coming decades. However, besides a few exceptions, consensus forecasts do not exist for how these C&LUC will likely impact Earth-surface processes and hazards. In some cases, we have the tools to forecast the geomorphic responses to likely future C&LUC. Fully exploiting these models and utilizing these tools will require close collaboration among Earth-surface scientists and Earth-system modelers. This paper assesses the state-of-the-art tools and data that are being used or could be used to forecast changes in the state of Earth's surface as a result of likely future C&LUC. We also propose strategies for filling key knowledge gaps, emphasizing where additional basic research and/or collaboration across disciplines are necessary. The main body of the paper addresses cross-cutting issues, including the importance of nonlinear/threshold-dominated interactions among topography, vegetation, and sediment transport, as well as the importance of alternate stable states and extreme, rare events for understanding and forecasting Earth-surface response to C&LUC. Five supplements delve into different scales or process zones (global-scale assessments and fluvial, aeolian, glacial/periglacial, and coastal process zones) in detail. C1 [Pelletier, Jon D.] Univ Arizona, Dept Geosci, Tucson, AZ 85721 USA. [Murray, A. Brad; Marani, Marco] Duke Univ, Nicholas Sch Environm, Div Earth & Ocean Sci, Durham, NC 27708 USA. [Pierce, Jennifer L.; Poulos, Michael J.] Boise State Univ, Dept Geosci, Boise, ID 83725 USA. [Bierman, Paul R.] Univ Vermont, Dept Geol, Burlington, VT USA. [Breshears, David D.] Univ Arizona, Sch Nat Resources & Environm, Tucson, AZ USA. [Crosby, Benjamin T.] Idaho State Univ, Dept Geosci, Pocatello, ID 83209 USA. [Ellis, Michael] British Geol Survey, Ctr Environm Sci, Nottingham NG12 5GG, England. [Foufoula-Georgiou, Efi] Univ Minnesota, St Anthony Falls Lab, Dept Civil Engn, Minneapolis, MN USA. [Heimsath, Arjun M.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA. [Houser, Chris] Texas A&M Univ, Dept Geog, College Stn, TX USA. [Lancaster, Nick] Univ Nevada, Desert Res Inst, Reno, NV 89506 USA. [Marani, Marco] Duke Univ, Dept Civil & Environm Engn, Durham, NC 27706 USA. [Marani, Marco] Univ Padua, Dept Civil Architectural & Environm Engn, Padua, Italy. [Merritts, Dorothy J.] Franklin & Marshall Coll, Dept Earth & Environm, Lancaster, PA 17604 USA. [Moore, Laura J.] Univ N Carolina, Dept Geol Sci, Chapel Hill, NC USA. [Pederson, Joel L.; Rittenour, Tammy M.] Utah State Univ, Dept Geol, Logan, UT 84322 USA. [Rowland, Joel C.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Ruggiero, Peter] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. [Ward, Dylan J.] Univ Cincinnati, Dept Geol, Cincinnati, OH USA. [Wickert, Andrew D.] Univ Colorado, Dept Geol Sci, Boulder, CO 80309 USA. [Yager, Elowyn M.] Univ Idaho, Dept Civil Engn, Boise, ID USA. RP Pelletier, JD (reprint author), Univ Arizona, Dept Geosci, Tucson, AZ 85721 USA. EM jdpellet@email.arizona.edu RI Marani, Marco/F-9451-2016; OI Marani, Marco/0000-0002-1493-6913; Ruggiero, Peter/0000-0001-7425-9953 FU NSF Geomorphology and Land-Use Dynamics program [1250358] FX We wish to thank the NSF Geomorphology and Land-Use Dynamics program and its manager Paul Cutler for supporting this effort intellectually and financially through award #1250358. We also thank the many members of the broader Working Group on Predicting Landscape Response to Climatic and Land-Use Changes that commented on drafts of the manuscript at http://geomorphicprediction.geo.arizona.edu/. Data used to make any of the figures can be obtained upon request from J.D.P. NR 634 TC 12 Z9 12 U1 18 U2 77 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2328-4277 J9 EARTHS FUTURE JI Earth Future PD JUL PY 2015 VL 3 IS 7 BP 220 EP 251 DI 10.1002/2014EF000290 PG 32 WC Environmental Sciences; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Geology; Meteorology & Atmospheric Sciences GA CP5DT UT WOS:000359902200002 ER PT J AU Wang, JL Kotamarthi, VR AF Wang, Jiali Kotamarthi, Veerabhadra R. TI High-resolution dynamically downscaled projections of precipitation in the mid and late 21st century over North America SO EARTHS FUTURE LA English DT Article DE high-resolution; dynamic downscaling; precipitation; projection; North America ID REGIONAL CLIMATE-CHANGE; CONTIGUOUS UNITED-STATES; GCM BIAS CORRECTIONS; PART I; SURFACE-TEMPERATURE; MODEL SIMULATION; EXTREMES INDEXES; AIR-QUALITY; FUTURE; REANALYSIS AB This study performs high-spatial-resolution (12km) Weather Research and Forecasting (WRF) simulations over a very large domain (7200kmx6180km, covering much of North America) to explore changes in mean and extreme precipitation in the mid and late 21st century under Representative Concentration Pathways 4.5 (RCP 4.5) and 8.5 (RCP 8.5). We evaluate WRF model performance for a historical simulation and future projections, applying the Community Climate System Model version 4 (CCSM4) as initial and boundary conditions with and without a bias correction. WRF simulations using boundary and initial conditions from both versions of CCSM4 show smaller biases versus evaluation data sets than does CCSM4 over western North America. WRF simulations also improve spatial details of precipitation over much of North America. However, driving the WRF with the bias-corrected CCSM4 does not always reduce the bias. WRF-projected changes in precipitation include decreasing intensity over the southwestern United States, increasing intensity over the eastern United Sates and most of Canada, and an increase in the number of days with heavy precipitation over much of North America. Projected precipitation changes are more evident in the late 21st century than the mid 21st century, and they are more evident under RCP 8.5 than under RCP 4.5 in the late 21st century. Uncertainties in the projected changes in precipitation due to different warming scenarios are non-negligible. Differences in summer precipitation changes between WRF and CCSM4 are significant over most of the United States. C1 [Wang, Jiali; Kotamarthi, Veerabhadra R.] Argonne Natl Lab, Environm Sci Div, Argonne, IL 60439 USA. RP Wang, JL (reprint author), Argonne Natl Lab, Environm Sci Div, Argonne, IL 60439 USA. EM jialiwang@anl.gov FU U.S. Department of Energy (DOE) [RC-2242, DE-AC02-06CH11357] FX This work is supported under a military interdepartmental purchase request from the Strategic Environmental Research and Development Program, RC-2242, through U.S. Department of Energy (DOE) contract DE-AC02-06CH11357. The PRISM data are available at http://www.prism.oregonstate.edu/. The NARR data (in NetCDF format) are provided by the NOAA-ESRL Physical Sciences Division, Boulder, Colorado, at http://www.esrl.noaa.gov/psd/. The CCSM4 data are downloaded from https://www.earthsystemgrid.org/home.htm. Computational resources are provided by the DOE-supported Argonne Leadership Computing Facility and the National Energy Research Scientific Computing Center. All the model outputs generated in this study will be available online. We are in the process of setting up access to the data archive. NR 86 TC 3 Z9 3 U1 4 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2328-4277 J9 EARTHS FUTURE JI Earth Future PD JUL PY 2015 VL 3 IS 7 BP 268 EP 288 DI 10.1002/2015EF000304 PG 21 WC Environmental Sciences; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Geology; Meteorology & Atmospheric Sciences GA CP5DT UT WOS:000359902200004 ER PT J AU Wise, M Hodson, EL Mignone, BK Clarke, L Waldhoff, S Luckow, P AF Wise, Marshall Hodson, Elke L. Mignone, Bryan K. Clarke, Leon Waldhoff, Stephanie Luckow, Patrick TI An approach to computing marginal land use change carbon intensities for bioenergy in policy applications SO ENERGY ECONOMICS LA English DT Article DE Bioenergy crops; Land use change; Carbon intensity; Integrated assessment modeling ID GREENHOUSE-GAS EMISSIONS; ENERGY; CROPLANDS; ETHANOL AB Accurately characterizing the emissions implications of bioenergy is increasingly important to the design of regional and global greenhouse gas mitigation policies. Market-based policies, in particular, often use information about carbon intensity to adjust relative deployment incentives for different energy sources. However, the carbon intensity of bioenergy is difficult to quantify because carbon emissions can occur when land use changes to expand production of bioenergy crops rather than simply when the fuel is consumed as for fossil fuels. Using a long-term, integrated assessment model, this paper develops an approach for computing the carbon intensity of bioenergy production that isolates the marginal impact of increasing production of a specific bioenergy crop in a specific region, taking into account economic competition among land uses. We explore several factors that affect emissions intensity and explain these results in the context of previous studies that use different approaches. Among the factors explored, our results suggest that the carbon intensity of bioenergy production from land use change (LUC) differs by a factor of two depending on the region in which the bioenergy crop is grown in the United States. Assumptions about international land use policies (such as those related to forest protection) and crop yields also significantly impact carbon intensity. Finally, we develop and demonstrate a generalized method for considering the varying time profile of LUC emissions from bioenergy production, taking into account the time path of future carbon prices, the discount rate and the time horizon. When evaluated in the context of power sector applications, we found electricity from bioenergy crops to be less carbon-intensive than conventional coal-fired electricity generation and often less carbon-intensive than natural-gas fired generation. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wise, Marshall; Clarke, Leon; Waldhoff, Stephanie; Luckow, Patrick] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Hodson, Elke L.; Mignone, Bryan K.] US DOE, Off Climate & Environm Anal, Washington, DC 20585 USA. RP Wise, M (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM Marshall.Wise@pnnl.gov FU U.S. Department of Energy (DOE) Office of Climate and Environmental Analysis [DE-AC05-76RL01830] FX The PNNL authors are grateful for research support provided by the U.S. Department of Energy (DOE) Office of Climate and Environmental Analysis under prime contract DE-AC05-76RL01830. The authors thank Liwayway Adkins, Aaron Bergman, and Kate Calvin for helpful comments on the manuscript. This work does not reflect the official views or policies of the United States Government or any agency thereof, including the funding entities. NR 39 TC 1 Z9 2 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0140-9883 EI 1873-6181 J9 ENERG ECON JI Energy Econ. PD JUL PY 2015 VL 50 BP 337 EP 347 DI 10.1016/j.eneco.2015.05.009 PG 11 WC Economics SC Business & Economics GA CP4TZ UT WOS:000359876800032 ER PT J AU Gunduz, A Morita, H Rossi, PJ Allen, WL Alterman, RL Bronte-Stewart, H Butson, CR Charles, D Deckers, S de Hemptinne, C DeLong, M Dougherty, D Ellrich, J Foote, KD Giordano, J Goodman, W Greenberg, BD Greene, D Gross, R Judy, JW Karst, E Kent, A Kopell, B Lang, A Lozano, A Lungu, C Lyon, KE Machado, A Martens, H McIntyre, C Min, HK Neimat, J Ostrem, J Pannu, S Ponce, F Pouratian, N Reymers, D Schrock, L Sheth, S Shih, L Stanslaski, S Steinke, GK Stypulkowski, P Troster, AI Verhagen, L Walker, H Okun, MS AF Gunduz, Aysegul Morita, Hokuto Rossi, P. Justin Allen, William L. Alterman, Ron L. Bronte-Stewart, Helen Butson, Christopher R. Charles, David Deckers, Sjaak de Hemptinne, Coralie DeLong, Mahlon Dougherty, Darin Ellrich, Jens Foote, Kelly D. Giordano, James Goodman, Wayne Greenberg, Benjamin D. Greene, David Gross, Robert Judy, Jack W. Karst, Edward Kent, Alexander Kopell, Brian Lang, Anthony Lozano, Andres Lungu, Codrin Lyon, Kelly E. Machado, Andre Martens, Hubert McIntyre, Cameron Min, Hoon-Ki Neimat, Joseph Ostrem, Jill Pannu, Sat Ponce, Francisco Pouratian, Nader Reymers, Donnie Schrock, Lauren Sheth, Sameer Shih, Ludy Stanslaski, Scott Steinke, G. Karl Stypulkowski, Paul Troester, Alexander I. Verhagen, Leo Walker, Harrison Okun, Michael S. TI Proceedings of the Second Annual Deep Brain Stimulation Think Tank: What's in the Pipeline SO INTERNATIONAL JOURNAL OF NEUROSCIENCE LA English DT Review DE deep brain stimulation; Movement disorders; Neuroethics; Electrophysiology; neurotechnology ID HIGH-FREQUENCY STIMULATION; HUMAN SUBTHALAMIC NUCLEUS; SHORT-LATENCY ACTIVATION; PRIMARY MOTOR CORTEX; PARKINSONS-DISEASE; NONMOTOR SYMPTOMS; GLOBUS-PALLIDUS; THALAMIC SEGMENTATION; CLINICAL ARTICLE; BOLD ACTIVATION AB The proceedings of the 2nd Annual Deep Brain Stimulation Think Tank summarize the most contemporary clinical, electrophysiological, and computational work on DBS for the treatment of neurological and neuropsychiatric disease and represent the insights of a unique multidisciplinary ensemble of expert neurologists, neurosurgeons, neuropsychologists, psychiatrists, scientists, engineers and members of industry. Presentations and discussions covered a broad range of topics, including advocacy for DBS, improving clinical outcomes, innovations in computational models of DBS, understanding of the neurophysiology of Parkinson's disease (PD) and Tourette syndrome (TS) and evolving sensor and device technologies. C1 [Gunduz, Aysegul; Morita, Hokuto; Rossi, P. Justin; Allen, William L.; Foote, Kelly D.; Judy, Jack W.; Okun, Michael S.] Univ Florida, Gainesville, FL USA. [Alterman, Ron L.; Shih, Ludy] Beth Israel Deaconess Med Ctr, Boston, MA 02215 USA. [Bronte-Stewart, Helen] Stanford Univ, Stanford, CA 94305 USA. [Butson, Christopher R.; Schrock, Lauren] Univ Utah, Salt Lake City, UT USA. [Charles, David; Neimat, Joseph] Vanderbilt Univ, Nashville, TN 37235 USA. [Deckers, Sjaak; Ellrich, Jens; Martens, Hubert] Sapiens Steering Brain Stimulat, Eindhoven, Netherlands. [de Hemptinne, Coralie; Ostrem, Jill] Univ Calif San Francisco, San Francisco, CA 94143 USA. [DeLong, Mahlon; Gross, Robert] Emory Univ, Atlanta, GA 30322 USA. [Dougherty, Darin] Massachusetts Gen Hosp, Boston, MA 02114 USA. [Giordano, James] Georgetown Univ, Med Ctr, Washington, DC 20007 USA. [Goodman, Wayne; Kopell, Brian] Mt Sinai Hosp, New York, NY 10029 USA. [Greenberg, Benjamin D.] Brown Univ, Providence, RI 02912 USA. [Greene, David] Neuropace Univ, Mountain View, CA USA. [Karst, Edward] St Jude Med, Sylmar, CA USA. [Kent, Alexander] St Jude Med, Sunnyvale, CA USA. [Lang, Anthony; Lozano, Andres] Univ Toronto, Toronto, ON, Canada. [Lungu, Codrin] NIH, Bethesda, MD 20892 USA. [Lyon, Kelly E.] Univ Kansas, Med Ctr, Kansas City, KS 66103 USA. [Machado, Andre] Cleveland Clin, Cleveland, OH 44106 USA. [McIntyre, Cameron] Case Western Reserve Univ, Cleveland, OH 44106 USA. [Min, Hoon-Ki] Mayo Clin, Rochester, MN USA. [Pannu, Sat] Lawrence Livermore Natl Lab, Livermore, CA USA. [Ponce, Francisco; Troester, Alexander I.] Barrow Neurol Inst, Phoenix, AZ 85013 USA. [Pouratian, Nader] Univ Calif Los Angeles, Los Angeles, CA USA. [Reymers, Donnie] Funct Neuromodulat Ltd, Toronto, ON, Canada. [Sheth, Sameer] Columbia Univ, New York, NY USA. [Stanslaski, Scott; Stypulkowski, Paul] Medtronic, Minneapolis, MN USA. [Steinke, G. Karl] Boston Sci Neuromodulat, Valencia, CA USA. [Verhagen, Leo] Rush Univ, Med Ctr, Chicago, IL 60612 USA. [Walker, Harrison] Univ Alabama Birmingham, Birmingham, AL USA. RP Okun, MS (reprint author), Univ Florida, Dept Neurol, Gainesville, FL 32611 USA. EM okun@neurology.ufl.edu RI Gunduz, Aysegul/Q-2336-2016; OI Okun, Michael/0000-0002-6247-9358 FU Medtronic, Inc.; Allergan; Ipsen; Merz; Medtronic; Alliance for Patient Access for education or consulting services; Cyberonics; Eli Lilly; Roche; St. Jude; Boston Scientific; Neuropace; Brain Canada; Canadian Institutes of Health Research; Edmond J Safra Philanthropic Foundation; Michael J. Fox Foundation; Ontario Brain Institute; National Parkinson Foundation; Parkinson Society Canada; Tourette Syndrome Association; W. Garfield Weston Foundation; MRI Interventions; St Jude Medical; Glaxo Smith Kone; NIH; NPF; Parkinson Alliance; Smallwood Foundation; Bachmann-Strauss Foundation; UP Foundation FX AG: Grant support from Medtronic, Inc.; HK: None; PJR: None; WLA: None; RLA: Consultant for Medtronic, Inc.; HB-S: None; CRB: Consultant for St Jude Medical, Boston Scientific; IP related to DBS; DC: Vanderbilt receives income from grants or contracts from Allergan, Ipsen, Merz and Medtronic for research led by DC; DC receives income from Allergan, Ipsen, Medtronic and, the Alliance for Patient Access for education or consulting services; SD: Employee and shareholder of Sapiens Steering Brain Stimulation GmbH (Medtronic Eindhoven Design Center); CDH: None; MDL: None; DD: Grant support from Medtronic, Cyberonics, Eli Lilly, Roche, Honoraria from Medtronic, Insys, Johnson & Johnson; JE: Chief Medical Officer at Sapiens Steering Brain Stimulation GmbH; KDF: Grant support from Medtronic, St. Jude, Boston Scientific, Neuropace; Consultant for Medtronic, Neuropace; JG: None; WG: None; BDG: None; DG: Employee of Neuropace; RG: None; JJ: None; EK. Employee of St. Jude Medical; AK: Employee of St. Jude Medical; BK. Consultant for Medtronic, St Jude Neuromodulation, MRI Interventions; ALang: Consultant for Abbvie, Allon Therapeutics, Avanir Pharmaceuticals, Biogen Idec, Boerhinger-Ingelheim, Ceregene, Lilly, Medtronic, Merck, Novartis, NeuroPhage Pharmaceuticals, Teva, UCB; Honoraria from Medtronic, Teva, UCB, AbbVie; Grant support from Brain Canada, Canadian Institutes of Health Research, Edmond J Safra Philanthropic Foundation, Michael J. Fox Foundation, the Ontario Brain Institute, National Parkinson Foundation, Parkinson Society Canada, Tourette Syndrome Association, W. Garfield Weston Foundation; Publishing royalties from Saunders, Wiley-Blackwell, Johns Hopkins Press, Cambridge University Press; ALozano: Consultant for Medtronic, St Jude and Boston Scientific, Co-Founder of Functional Neuromodulation; CL: None; KL: Consultant for Medtronic, St. Jude Medical; AM: IP in Enspire, ATI, Cardionomics, Grant support from Medtronic, Inc., Consultant for Functional Neuromodulation, Spinal Modulation; HM: Employee and shareholder of Sapiens Steering Brain Stimulation GmbH (Medtronic Eindhoven Design Center); CM: IP in Boston Scientific Neuromodulation; Consultant for Boston Scientific Neuromodulation; Shareholder in Autonomic Technologies, Inc., Cardionomics, Inc., Neuros Medical, Inc., Surgical Information Sciences, Inc.; BM: None; HKM: None; JN: Grant support from Medtronic, Inc.; Consultant for Medtronic, Inc., Montens Inc.; JO: Grant support from Boston Scientific, MRI Interventions, St Jude Medical, Medtronic; SP: None; FP: Consultant for Medtronic, Inc; NP: None; DR: Employee of Neuromodulation, Inc; LSchrock: Site PI for the Boston Scientific INTREPID DBS trial; SSheth: None; LShih: None; SStanslanski: Employee of Medtronic, Inc.; GKS: Employee of Boston Scientific Neuromodulation; PS: Employee of Medtronic, Inc.; AT: Consultant for St Jude Medical, Boston Scientific, Theravance, Teva; Grant support from Glaxo Smith Kone, Speaker for Medtronic; Royalties from Oxford University Press; LV: None; HW: None; MSO: Consultant for National Parkinson Foundation; Grant support from NIH, NPF, Michael J. Fox Foundation, Parkinson Alliance, Smallwood Foundation, Bachmann-Strauss Foundation, Tourette Syndrome Association, UP Foundation. NR 79 TC 5 Z9 5 U1 2 U2 19 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0020-7454 EI 1563-5279 J9 INT J NEUROSCI JI Int. J. Neurosci. PD JUL PY 2015 VL 125 IS 7 BP 475 EP 485 DI 10.3109/00207454.2014.999268 PG 11 WC Neurosciences SC Neurosciences & Neurology GA CP4WV UT WOS:000359884200001 PM 25526555 ER PT J AU Xu, XF Elias, DA Graham, DE Phelps, TJ Carroll, SL Wullschleger, SD Thornton, PE AF Xu, Xiaofeng Elias, Dwayne A. Graham, David E. Phelps, Tommy J. Carroll, Sue L. Wullschleger, Stan D. Thornton, Peter E. TI A microbial functional group-based module for simulating methane production and consumption: Application to an incubated permafrost soil SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article DE carbon dioxide; methane; methanogen; methanotroph; microbial functional group ID TEMPERATURE SENSITIVITY; TERRESTRIAL ECOSYSTEMS; BIOGEOCHEMISTRY MODEL; ANAEROBIC OXIDATION; NATURAL WETLANDS; CARBON RELEASE; NORTH-AMERICA; TRACE GASES; METHANOGENESIS; FLUXES AB Accurately estimating methane (CH4) flux in terrestrial ecosystems is critically important for investigating and predicting biogeochemistry-climate feedbacks. Improved simulations of CH4 flux require explicit representations of the microbial processes that account for CH4 dynamics. A microbial functional group-based module was developed, building on the decomposition subroutine of the Community Land Model 4.5. This module considers four key mechanisms for CH4 production and consumption: methanogenesis from acetate or from single-carbon compounds and CH4 oxidation using molecular oxygen or other inorganic electron acceptors. Four microbial functional groups perform these processes: acetoclastic methanogens, hydrogenotrophic methanogens, aerobic methanotrophs, and anaerobic methanotrophs. This module was used to simulate dynamics of carbon dioxide (CO2) and CH4 concentrations from an incubation experiment with permafrost soils. The results show that the model captures the dynamics of CO2 and CH4 concentrations in microcosms with top soils, mineral layer soils, and permafrost soils under natural and saturated moisture conditions and three temperature conditions of -2 degrees C, 3 degrees C, and 5 degrees C (R-2>0.67; P<0.001). The biases for modeled results are less than 30% across the soil samples and moisture and temperature conditions. Sensitivity analysis confirmed the importance of acetic acid's direct contribution as substrate and indirect effects through pH feedback on CO2 and CH4 production and consumption. This study suggests that representing the microbial mechanisms is critical for modeling CH4 production and consumption; it is urgent to incorporate microbial mechanisms into Earth system models for better predicting trace gas dynamics and the behavior of the climate system. C1 [Xu, Xiaofeng; Elias, Dwayne A.; Wullschleger, Stan D.; Thornton, Peter E.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Xu, Xiaofeng; Elias, Dwayne A.; Wullschleger, Stan D.; Thornton, Peter E.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Elias, Dwayne A.; Graham, David E.; Phelps, Tommy J.; Carroll, Sue L.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. RP Xu, XF (reprint author), Univ Texas El Paso, Dept Biol Sci, El Paso, TX 79968 USA. EM xxu2@utep.edu; thorntonpe@ornl.gov RI Graham, David/F-8578-2010; Thornton, Peter/B-9145-2012; Xu, Xiaofeng/B-2391-2008; Wullschleger, Stan/B-8297-2012 OI Graham, David/0000-0001-8968-7344; Thornton, Peter/0000-0002-4759-5158; Xu, Xiaofeng/0000-0002-6553-6514; Wullschleger, Stan/0000-0002-9869-0446 FU Laboratory Directed Research and Development program at ORNL; U.S. Department of Energy [DE-AC05-00OR22725] FX We are grateful for Guoping Tang and Fengming Yuan at Oak Ridge National Laboratory (ORNL) for their comments on an early version of the manuscript. Special thanks to Anna Wagner and Mark Beede, USACE Cold Regions Research and Engineering Laboratory (CRREL), Fairbanks, AK, for collecting soil samples. Three anonymous reviewers, Dennis Baldocchi, and Miguel Goni made valuable comments which significantly improve the manuscript. This research was sponsored in part by the Laboratory Directed Research and Development program at ORNL. Additional support for model development was provided by the Next-Generation Ecosystem Experiments (NGEE-Arctic) project, which is supported by the Office of Biological and Environmental Research in the U.S. Department of Energy, Office of Science. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. The data used in this study will be available upon request. NR 89 TC 6 Z9 6 U1 8 U2 49 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD JUL PY 2015 VL 120 IS 7 BP 1315 EP 1333 DI 10.1002/2015JG002935 PG 19 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA CP4QU UT WOS:000359868200009 ER PT J AU Lee, T Oh, T Yang, S Shin, J Hwang, S Kim, CY Kim, H Shim, H Shim, JE Ronald, PC Lee, I AF Lee, Tak Oh, Taeyun Yang, Sunmo Shin, Junha Hwang, Sohyun Kim, Chan Yeong Kim, Hyojin Shim, Hongseok Shim, Jung Eun Ronald, Pamela C. Lee, Insuk TI RiceNet v2: an improved network prioritization server for rice genes SO NUCLEIC ACIDS RESEARCH LA English DT Article ID GENOMICS DATA SETS; SACCHAROMYCES-CEREVISIAE; DATABASE; INFORMATION; DISSECTION; GENETICS; SEQUENCE; PLANTS; TOOL; V3 AB Rice is the most important staple food crop and a model grass for studies of bioenergy crops. We previously published a genome-scale functional network server called RiceNet, constructed by integrating diverse genomics data and demonstrated the use of the network in genetic dissection of rice biotic stress responses and its usefulness for other grass species. Since the initial construction of the network, there has been a significant increase in the amount of publicly available rice genomics data. Here, we present an updated network prioritization server for Oryza sativa ssp. japonica, RiceNet v2 (http://www.inetbio.org/ricenet), which provides a network of 25 765 genes (70.1% of the coding genome) and 1 775 000 co-functional links. Ricenet v2 also provides two complementary methods for network prioritization based on: (i) network direct neighborhood and (ii) context-associated hubs. RiceNet v2 can use genes of the related subspecies O. sativa ssp. indica and the reference plant Arabidopsis for versatility in generating hypotheses. We demonstrate that RiceNet v2 effectively identifies candidate genes involved in rice root/shoot development and defense responses, demonstrating its usefulness for the grass research community. C1 [Lee, Tak; Yang, Sunmo; Shin, Junha; Hwang, Sohyun; Kim, Chan Yeong; Kim, Hyojin; Shim, Hongseok; Shim, Jung Eun; Lee, Insuk] Yonsei Univ, Coll Life Sci & Biotechnol, Dept Biotechnol, Seoul 120749, South Korea. [Oh, Taeyun; Ronald, Pamela C.] Joint Bioenergy Inst, Emeryville, CA USA. [Oh, Taeyun; Ronald, Pamela C.] Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA. [Oh, Taeyun; Ronald, Pamela C.] Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. RP Lee, I (reprint author), Yonsei Univ, Coll Life Sci & Biotechnol, Dept Biotechnol, Seoul 120749, South Korea. EM pcronald@ucdavis.edu; insuklee@yonsei.ac.kr FU National Research Foundation of Korea [2010-0017649, 2012M3A9B4028641, 2012M3A9C7050151]; Joint BioEnergy Institute; Office of Science, Office of Biological and Environmental Research, U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy Systems Biology Knowledgebase [KBase] FX National Research Foundation of Korea [2010-0017649, 2012M3A9B4028641, 2012M3A9C7050151] to I.L.; The Joint BioEnergy Institute, the Office of Science, Office of Biological and Environmental Research, U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy Systems Biology Knowledgebase [KBase] to P.C.R. Funding for open access charge: National Research Foundation of Korea [2010-0017649]. NR 27 TC 9 Z9 9 U1 2 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 1 PY 2015 VL 43 IS W1 BP W122 EP W127 DI 10.1093/nar/gkv253 PG 6 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP3IP UT WOS:000359772700019 PM 25813048 ER PT J AU Sahraeian, SM Luo, KR Brenner, SE AF Sahraeian, Sayed M. Luo, Kevin R. Brenner, Steven E. TI SIFTER search: a web server for accurate phylogeny-based protein function prediction SO NUCLEIC ACIDS RESEARCH LA English DT Article ID HETEROGENEOUS DATA SOURCES; GENE-FUNCTION; INTERACTION NETWORKS; ANNOTATION; FAMILIES; ONTOLOGY; TOOL AB We are awash in proteins discovered through high-throughput sequencing projects. As only a minuscule fraction of these have been experimentally characterized, computational methods are widely used for automated annotation. Here, we introduce a user-friendly web interface for accurate protein function prediction using the SIFTER algorithm. SIFTER is a state-of-the-art sequence-based gene molecular function prediction algorithm that uses a statistical model of function evolution to incorporate annotations throughout the phylogenetic tree. Due to the resources needed by the SIFTER algorithm, running SIFTER locally is not trivial for most users, especially for large-scale problems. The SIFTER web server thus provides access to precomputed predictions on 16 863 537 proteins from 232 403 species. Users can explore SIFTER predictions with queries for proteins, species, functions, and homologs of sequences not in the precomputed prediction set. The SIFTER web server is accessible at http://sifter.berkeley.edu/ and the source code can be downloaded. C1 [Sahraeian, Sayed M.; Brenner, Steven E.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Luo, Kevin R.; Brenner, Steven E.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Brenner, Steven E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Brenner, SE (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM brenner@compbio.berkeley.edu RI Brenner, Steven/A-8729-2008 OI Brenner, Steven/0000-0001-7559-6185 FU U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231]; NIH [R01 GM071749] FX This material by ENIGMA-Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231]. This work was a Technology Development effort for ENIGMA. This work was also supported by grant NIH R01 GM071749. Funding for open access charge: U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231]. NR 35 TC 2 Z9 3 U1 1 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 1 PY 2015 VL 43 IS W1 BP W141 EP W147 DI 10.1093/nar/gkv461 PG 7 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP3IP UT WOS:000359772700022 PM 25979264 ER PT J AU Smedley, D Haider, S Durinck, S Pandini, L Provero, P Allen, J Arnaiz, O Awedh, MH Baldock, R Barbiera, G Bardou, P Beck, T Blake, A Bonierbale, M Brookes, AJ Bucci, G Buetti, I Burge, S Cabau, C Carlson, JW Chelala, C Chrysostomou, C Cittaro, D Collin, O Cordova, R Cutts, RJ Dassi, E Di Genova, A Djari, A Esposito, A Estrella, H Eyras, E Fernandez-Banet, J Forbes, S Free, RC Fujisawa, T Gadaleta, E Garcia-Manteiga, JM Goodstein, D Gray, K Guerra-Assuncao, JA Haggarty, B Han, DJ Han, BW Harris, T Harshbarger, J Hastings, RK Hayes, RD Hoede, C Hu, S Hu, ZL Hutchins, L Kan, ZY Kawaji, H Keliet, A Kerhornou, A Kim, S Kinsella, R Klopp, C Kong, L Lawson, D Lazarevic, D Lee, JH Letellier, T Li, CY Lio, P Liu, CJ Luo, J Maass, A Mariette, J Maurel, T Merella, S Mohamed, AM Moreews, F Nabihoudine, I Ndegwa, N Noirot, C Perez-Llamas, C Primig, M Quattrone, A Quesneville, H Rambaldi, D Reecy, J Riba, M Rosanoff, S Saddiq, AA Salas, E Sallou, O Shepherd, R Simon, R Sperling, L Spooner, W Staines, DM Steinbach, D Stone, K Stupka, E Teague, JW Ullah, AZD Wang, J Ware, D Wong-Erasmus, M Youens-Clark, K Zadissa, A Zhang, SJ Kasprzyk, A AF Smedley, Damian Haider, Syed Durinck, Steffen Pandini, Luca Provero, Paolo Allen, James Arnaiz, Olivier Awedh, Mohammad Hamza Baldock, Richard Barbiera, Giulia Bardou, Philippe Beck, Tim Blake, Andrew Bonierbale, Merideth Brookes, Anthony J. Bucci, Gabriele Buetti, Iwan Burge, Sarah Cabau, Cedric Carlson, Joseph W. Chelala, Claude Chrysostomou, Charalambos Cittaro, Davide Collin, Olivier Cordova, Raul Cutts, Rosalind J. Dassi, Erik Di Genova, Alex Djari, Anis Esposito, Anthony Estrella, Heather Eyras, Eduardo Fernandez-Banet, Julio Forbes, Simon Free, Robert C. Fujisawa, Takatomo Gadaleta, Emanuela Garcia-Manteiga, Jose M. Goodstein, David Gray, Kristian Guerra-Assuncao, JoseE Afonso Haggarty, Bernard Han, Dong-Jin Han, Byung Woo Harris, Todd Harshbarger, Jayson Hastings, Robert K. Hayes, Richard D. Hoede, Claire Hu, Shen Hu, Zhi-Liang Hutchins, Lucie Kan, Zhengyan Kawaji, Hideya Keliet, Aminah Kerhornou, Arnaud Kim, Sunghoon Kinsella, Rhoda Klopp, Christophe Kong, Lei Lawson, Daniel Lazarevic, Dejan Lee, Ji-Hyun Letellier, Thomas Li, Chuan-Yun Lio, Pietro Liu, Chu-Jun Luo, Jie Maass, Alejandro Mariette, Jerome Maurel, Thomas Merella, Stefania Mohamed, Azza Mostafa Moreews, Francois Nabihoudine, Ibounyamine Ndegwa, Nelson Noirot, Celine Perez-Llamas, Cristian Primig, Michael Quattrone, Alessandro Quesneville, Hadi Rambaldi, Davide Reecy, James Riba, Michela Rosanoff, Steven Saddiq, Amna Ali Salas, Elisa Sallou, Olivier Shepherd, Rebecca Simon, Reinhard Sperling, Linda Spooner, William Staines, Daniel M. Steinbach, Delphine Stone, Kevin Stupka, Elia Teague, Jon W. Ullah, Abu Z. Dayem Wang, Jun Ware, Doreen Wong-Erasmus, Marie Youens-Clark, Ken Zadissa, Amonida Zhang, Shi-Jian Kasprzyk, Arek TI The BioMart community portal: an innovative alternative to large, centralized data repositories SO NUCLEIC ACIDS RESEARCH LA English DT Article ID BIOLOGICAL DATA; BIOINFORMATICS; GENOMICS; ACCESS; BIOCONDUCTOR; RESOURCE; PLATFORM AB The BioMart Community Portal (www.biomart.org) is a community-driven effort to provide a unified interface to biomedical databases that are distributed worldwide. The portal provides access to numerous database projects supported by 30 scientific organizations. It includes over 800 different biological datasets spanning genomics, proteomics, model organisms, cancer data, ontology information and more. All resources available through the portal are independently administered and funded by their host organizations. The BioMart data federation technology provides a unified interface to all the available data. The latest version of the portal comes with many new databases that have been created by our ever-growing community. It also comes with better support and extensibility for data analysis and visualization tools. A new addition to our toolbox, the enrichment analysis tool is now accessible through graphical and web service interface. The BioMart community portal averages over one million requests per day. Building on this level of service and the wealth of information that has become available, the BioMart Community Portal has introduced a new, more scalable and cheaper alternative to the large data stores maintained by specialized organizations. C1 [Smedley, Damian; Forbes, Simon; Shepherd, Rebecca; Teague, Jon W.] Wellcome Trust Sanger Inst, Hinxton CB10 1SD, England. [Haider, Syed] Univ Oxford, Weatherall Inst Mol Med, Oxford OX3 9DS, England. [Durinck, Steffen] Genentech Inc, San Francisco, CA 94080 USA. [Pandini, Luca; Provero, Paolo; Barbiera, Giulia; Bucci, Gabriele; Buetti, Iwan; Cittaro, Davide; Garcia-Manteiga, Jose M.; Lazarevic, Dejan; Merella, Stefania; Rambaldi, Davide; Riba, Michela; Stupka, Elia; Kasprzyk, Arek] Ist Sci San Raffaele, Ctr Translat Genom & Bioinformat, I-20132 Milan, Italy. [Provero, Paolo] Univ Turin, Dept Mol Biotechnol & Hlth Sci, Turin, Italy. [Allen, James; Burge, Sarah; Kerhornou, Arnaud; Kinsella, Rhoda; Luo, Jie; Maurel, Thomas; Rosanoff, Steven; Staines, Daniel M.; Zadissa, Amonida] European Bioinformat Inst, European Mol Biol Lab, Cambridge CB10 1SD, England. [Arnaiz, Olivier; Sperling, Linda] Univ Paris 11, CNRS, CEA, I2BC, F-91198 Gif Sur Yvette, France. [Awedh, Mohammad Hamza] King Abdulaziz Univ, Fac Engn, Dept Elect & Comp Engn, Jeddah 21413, Saudi Arabia. [Baldock, Richard; Haggarty, Bernard] Western Gen Hosp, Inst Genet & Mol Med, MRC Human Genet Unit, Edinburgh EH4 2XU, Midlothian, Scotland. [Bardou, Philippe; Cabau, Cedric] Sigenae, INRA, Castanet Tolosan, France. [Beck, Tim; Brookes, Anthony J.; Chrysostomou, Charalambos; Free, Robert C.; Hastings, Robert K.] Univ Leicester, Dept Genet, Leicester LE1 7RH, Leics, England. [Blake, Andrew] MRC Harwell, Didcot OX11 0RD, Oxon, England. [Bonierbale, Merideth; Cordova, Raul; Salas, Elisa; Simon, Reinhard] CIP, Lima 1558, Peru. [Carlson, Joseph W.; Goodstein, David; Hayes, Richard D.] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [Chelala, Claude; Cutts, Rosalind J.; Gadaleta, Emanuela; Guerra-Assuncao, JoseE Afonso; Ullah, Abu Z. Dayem] Queen Mary Univ London, Barts Canc Inst, Ctr Mol Oncol, London EC1M 6BQ, England. [Collin, Olivier; Sallou, Olivier] INRIA, IRISA, F-35042 Rennes, France. [Dassi, Erik; Quattrone, Alessandro] Univ Trento, Ctr Integrat Biol, Lab Translat Genom, Trento, Italy. [Di Genova, Alex; Maass, Alejandro] Univ Chile, Ctr Math Modeling, Beauchef 851, Chile. [Di Genova, Alex; Maass, Alejandro] Univ Chile, Ctr Genome Regulat, Beauchef 851, Chile. [Djari, Anis; Hoede, Claire; Klopp, Christophe; Mariette, Jerome; Nabihoudine, Ibounyamine; Noirot, Celine] INRA, Plate Forme Bioinformat Genotoul Math & Informat, F-31326 Castanet Tolosan, France. [Esposito, Anthony; Estrella, Heather; Fernandez-Banet, Julio; Kan, Zhengyan] Pfizer, Oncol Computat Biol, La Jolla, CA USA. [Eyras, Eduardo] Passeig Lluis Co, Catalan Inst Res & Adv Studies ICREA, E-08010 Barcelona, Spain. [Eyras, Eduardo; Perez-Llamas, Cristian] Univ Pompeu Fabra, E-08003 Barcelona, Spain. [Fujisawa, Takatomo] Kasuza DNA Res Inst, Chiba 2920818, Japan. [Gray, Kristian] European Bioinformat Inst EMBL EBI, HUGO Gene Nomenclature Comm HGNC, Hinxton CB10 1SD, England. [Han, Dong-Jin; Kim, Sunghoon; Lee, Ji-Hyun] Seoul Natl Univ, Coll Pharm, Med Bioconvergence Res Ctr, Seoul 151742, South Korea. [Han, Dong-Jin; Kim, Sunghoon] Seoul Natl Univ, Dept Mol Med & Biopharmaceut Sci, Seoul 151742, South Korea. [Han, Byung Woo; Lee, Ji-Hyun] Seoul Natl Univ, Coll Pharm, Res Inst Pharmaceut Sci, Seoul 151742, South Korea. [Han, Byung Woo; Lee, Ji-Hyun] Seoul Natl Univ, Informat Ctr Biopharmacol Network, Suwon 443270, South Korea. [Harris, Todd] Ontario Inst Canc Res, Toronto, ON M5G 0A3, Canada. [Harshbarger, Jayson; Kawaji, Hideya] RIKEN Ctr Life Sci Technol CLST, DGT, Yokohama, Kanagawa 2300045, Japan. [Hu, Shen] Univ Calif Los Angeles, Sch Dent, Los Angeles, CA 90095 USA. [Hu, Shen] Univ Calif Los Angeles, Dent Res Inst, Los Angeles, CA 90095 USA. [Hu, Zhi-Liang; Reecy, James] Iowa State Univ, Iowa City, IA USA. [Hutchins, Lucie; Stone, Kevin] Jackson Lab, Mouse Genom Informat Grp, Bar Harbor, ME 04609 USA. [Kawaji, Hideya] RIKEN Prevent Med & Diag Innovat Program, Wako, Saitama 3510198, Japan. [Keliet, Aminah; Letellier, Thomas; Quesneville, Hadi; Steinbach, Delphine] INRA URGI Ctr Versailles, F-78026 Versailles, France. [Kong, Lei; Wang, Jun] Peking Univ, Coll Life Sci, State Key Lab Prot & Plant Gene Res, Ctr Bioinformat, Beijing 100871, Peoples R China. [Lawson, Daniel] European Bioinformat Inst, VectorBase, Hinxton CB10 1SD, England. [Li, Chuan-Yun; Liu, Chu-Jun; Zhang, Shi-Jian] Peking Univ, Inst Mol Med, Beijing 100871, Peoples R China. [Lio, Pietro] Univ Cambridge, Comp Lab, Cambridge CB3 0FD, England. [Maass, Alejandro] Univ Chile, Dept Engn Math, Santiago, Chile. [Mohamed, Azza Mostafa] King Abdulaziz Univ, Fac Sci Girls, Dept Biochem, Jeddah 21413, Saudi Arabia. [Ndegwa, Nelson] Karolinska Inst, Dept Med Epidemiol & Biostat, S-17177 Stockholm, Sweden. [Primig, Michael] Univ Rennes 1, Inserm IRSET U1085, F-35042 Rennes, France. [Saddiq, Amna Ali] King Abdulaziz Univ, Fac Sci Girls, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Spooner, William; Ware, Doreen; Youens-Clark, Ken] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Spooner, William] Eagle Genom Ltd, Cambridge CB22 3AT, England. [Wong-Erasmus, Marie] Human Longev Inc, San Diego, CA 92121 USA. [Kasprzyk, Arek] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah, Saudi Arabia. RP Kasprzyk, A (reprint author), Ist Sci San Raffaele, Ctr Translat Genom & Bioinformat, Via Olgettina 58, I-20132 Milan, Italy. EM Arek.Kasprzyk@gmail.com RI mohamed, azza/I-5066-2012; primig, michael/G-3175-2013; Eyras, Eduardo/L-1053-2014; Kawaji, Hideya/N-5116-2015; Awedh, Mohammad/P-7168-2014; Maass, Alejandro/D-5848-2012; Gasull, Martina/A-6630-2013; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017; Allen, James/B-2457-2009; OI Rosanoff, Steven/0000-0002-4216-4674; Maurel, Thomas/0000-0003-0247-3971; Quattrone, Alessandro/0000-0003-3333-7630; Eyras, Eduardo/0000-0003-0793-6218; Kawaji, Hideya/0000-0002-0575-0308; Awedh, Mohammad/0000-0002-7055-010X; Maass, Alejandro/0000-0002-7038-4527; Allen, James/0000-0002-3894-4854; Christophe, KLOPP/0000-0001-7126-5477; chelala, claude/0000-0002-2488-0669; Cittaro, Davide/0000-0003-0384-3700; Lawson, Daniel/0000-0001-7765-983X; Hastings, Robert/0000-0001-8703-127X; Staines, Daniel/0000-0002-7564-9125; Dassi, Erik/0000-0003-4487-0449; Guerra-Assuncao, Jose Afonso/0000-0001-6593-403X; Collin, Olivier/0000-0002-8959-8402; Baldock, Richard/0000-0003-0332-6877; Fernandez Banet, Julio/0000-0003-0901-1286; Sperling, Linda/0000-0002-7772-4774 FU Wellcome Trust [077012/Z/05/Z, WT095908, WT098051]; Spanish Government [BIO2011-23920, CSD2009-00080]; Sandra Ibarra Foundation for Cancer [FSI2013]; Breast Cancer Campaign Tissue Bank [09TBBAR]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Global Frontier Project - Ministry of Science, ICT and Future Planning through National Research Foundation of Korea [NRF-2013M3A6A4043695]; Agence National de la Recherche [ANR-10-BLAN-1122, ANR-12-BSV6-0017-03, ANR-14-CE10-0005-03]; Centre National de la Recherche Scientifique; Center for Genome Regulation [SalmonDB] [Fondap-1509007]; Center for Mathematical Modelling [Basal-PFB 03]; European Molecular Biology Laboratory; Japanese Ministry of Education, Culture, Sports, Science and Technology [FANTOM5 BioMart]; Deanship of Scientific Research (DSR) King Abdulaziz University [96-130-35-HiCi]; King Abdulaziz University FX The BioMart Community Portal is a collaborative, community effort and as such it is the product of the efforts of dozens of different groups and organizations. The individual data sources that the portal comprises are funded separately and independently. In particular: Wellcome Trust [077012/Z/05/Z to COSMIC mart]; Spanish Government [BIO2011-23920 and CSD2009-00080 to BioMart database of the Regulatory Genomics group at Pompeu Fabra University]; Sandra Ibarra Foundation for Cancer [FSI2013]; Breast Cancer Campaign Tissue Bank [09TBBAR to BCCTB bioinformatics portal]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231 to Phytozome]; Global Frontier Project (to i-Pharm research) funded by the Ministry of Science, ICT and Future Planning through the National Research Foundation of Korea (NRF-2013M3A6A4043695); Agence National de la Recherche [ANR-10-BLAN-1122, ANR-12-BSV6-0017-03, ANR-14-CE10-0005-03 to ParameciumDB and cilDB]; Centre National de la Recherche Scientifique; Center for Genome Regulation [SalmonDB; Fondap-1509007 to A.M. and A.D.G.]; Center for Mathematical Modelling [Basal-PFB 03 to A.M. and A.D.G.]; Wellcome Trust (WT095908 and WT098051 to R.K., T.M. and A.Z.); European Molecular Biology Laboratory; Japanese Ministry of Education, Culture, Sports, Science and Technology [FANTOM5 BioMart; for RIKEN OSC and RIKEN PMI to Yoshihide Hayashizaki, and for RIKEN CLST]. Deanship of Scientific Research (DSR) King Abdulaziz University (96-130-35-HiCi to M.H.A., A.M.M., A.A.S. and A.K.). Funding for open access charge: King Abdulaziz University. NR 53 TC 69 Z9 69 U1 6 U2 29 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 1 PY 2015 VL 43 IS W1 BP W589 EP W598 DI 10.1093/nar/gkv350 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP3IP UT WOS:000359772700095 PM 25897122 ER PT J AU Yoon, H Macke, J West, AP Foley, B Bjorkman, PJ Korber, B Yusim, K AF Yoon, Hyejin Macke, Jennifer West, Anthony P., Jr. Foley, Brian Bjorkman, Pamela J. Korber, Bette Yusim, Karina TI CATNAP: a tool to compile, analyze and tally neutralizing antibody panels SO NUCLEIC ACIDS RESEARCH LA English DT Article ID HIV-1 GP120; SEQUENCE-ANALYSIS; VIRAL STRAINS; BINDING-SITE; CD4 BINDING; BROAD; EPITOPE; POTENT; DOMAIN; GLYCOPROTEIN AB CATNAP (Compile, Analyze and Tally NAb Panels) is a new web server at Los Alamos HIV Database, created to respond to the newest advances in HIV neutralizing antibody research. It is a comprehensive platform focusing on neutralizing antibody potencies in conjunction with viral sequences. CATNAP integrates neutralization and sequence data from published studies, and allows users to analyze that data for each HIV Envelope protein sequence position and each antibody. The tool has multiple data retrieval and analysis options. As input, the user can pick specific antibodies and viruses, choose a panel from a published study, or supply their own data. The output superimposes neutralization panel data, virus epidemiological data, and viral protein sequence alignments on one page, and provides further information and analyses. The user can highlight alignment positions, or select antibody contact residues and view position-specific information from the HIV databases. The tool calculates tallies of amino acids and N-linked glycosylation motifs, counts of antibody-sensitive and -resistant viruses in conjunction with each amino acid or N-glycosylation motif, and performs Fisher's exact test to detect potential positive or negative amino acid associations for the selected antibody. Website name: CATNAP (Compile, Analyze and Tally NAb Panels). Website address: http://hiv.lanl.gov/catnap. C1 [Yoon, Hyejin; Macke, Jennifer; Foley, Brian; Korber, Bette; Yusim, Karina] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [West, Anthony P., Jr.; Bjorkman, Pamela J.] CALTECH, Pasadena, CA 91125 USA. RP Yusim, K (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87544 USA. EM kyusim@lanl.gov OI Foley, Brian/0000-0002-1086-0296 FU National Institutes of Health (NIH) [AGRAAI1200700101000, HIVRAD P01 AI100148]; Bill & Melinda Gates Foundation [1032144, 1040753]; NIH through Los Alamos National Laboratory [AGRAAI1200700101000] FX National Institutes of Health (NIH) [contract AGRAAI1200700101000 HIV/SIV, Database and Analysis Unit (B.T.K., H.Y., J.M., B.F., K.Y.) and grant HIVRAD P01 AI100148 (P.J.B., A.P.W.)]; Bill & Melinda Gates Foundation [Collaboration for AIDS Vaccine Discovery, grant 1032144 (B.T.K., H.Y.) and grant 1040753 (P.J.B., A.P.W.)]. Funding for open access charge: NIH contract AGRAAI1200700101000 through Los Alamos National Laboratory. NR 31 TC 4 Z9 4 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 1 PY 2015 VL 43 IS W1 BP W213 EP W219 DI 10.1093/nar/gkv404 PG 7 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP3IP UT WOS:000359772700033 PM 26044712 ER PT J AU Birch, GC Griffin, JC AF Birch, Gabriel C. Griffin, John C. TI Sinusoidal Siemens star spatial frequency response measurement errors due to misidentified target centers SO OPTICAL ENGINEERING LA English DT Article DE spatial frequency response; modulation transfer function; resolution; image quality evaluation; Siemens star AB Numerous methods are available to measure the spatial frequency response (SFR) of an optical system. A recent change to the ISO 12233 photography resolution standard includes a sinusoidal Siemens star test target. We take the sinusoidal Siemens star proposed by the ISO 12233 standard, measure system SFR, and perform an analysis of errors induced by incorrectly identifying the center of a test target. We show a closed-form solution for the radial profile intensity measurement given an incorrectly determined center and describe how this error reduces the measured SFR of the system. Using the closed-form solution, we propose a two-step process by which test target centers are corrected and the measured SFR is restored to the nominal, correctly centered values. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. C1 [Birch, Gabriel C.; Griffin, John C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Birch, GC (reprint author), Sandia Natl Labs, POB 5800 MS 0781, Albuquerque, NM 87185 USA. EM gcbirch@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000. SAND2015-3823 J] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. SAND2015-3823 J. NR 12 TC 1 Z9 1 U1 0 U2 4 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 0091-3286 EI 1560-2303 J9 OPT ENG JI Opt. Eng. PD JUL PY 2015 VL 54 IS 7 AR 074104 DI 10.1117/1.OE.54.7.074104 PG 8 WC Optics SC Optics GA CP3ZZ UT WOS:000359823100021 ER PT J AU Denisov, DS AF Denisov, D. S. TI Future Particle-Physics Projects in the United States SO PHYSICS OF ATOMIC NUCLEI LA English DT Article AB Basic proposals of experiments aimed at precision measurements of Standard Model parameters and at searches for new particles, including dark-matter particles, are described along with future experimental projects considered by American Physical Society at the meeting in the summer of 2013 and intended for implementation within the next ten to twenty years. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Denisov, DS (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM denisovd@fnal.gov NR 1 TC 0 Z9 0 U1 0 U2 0 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 1063-7788 EI 1562-692X J9 PHYS ATOM NUCL+ JI Phys. Atom. Nuclei PD JUL PY 2015 VL 78 IS 5 BP 586 EP 590 DI 10.1134/S1063778815050038 PG 5 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CP7MQ UT WOS:000360072700007 ER PT J AU Lovelace, E Wagoner, J MacDonald, J Bammler, T Kim, YM Robertson, BJ Metz, T Farin, F Oberlies, NH Polyak, S AF Lovelace, E. Wagoner, J. MacDonald, J. Bammler, T. Kim, Y. M. Robertson, B. J. Metz, T. Farin, F. Oberlies, N. H. Polyak, S. TI Silymarin suppresses cellular inflammation by inducing reparative stress signaling SO PLANTA MEDICA LA English DT Meeting Abstract CT Annual Meeting of the American-Society-of-Pharmacognosy CY JUL 25-29, 2015 CL CO SP Amer Soc Pharmacognosy C1 [Lovelace, E.; Wagoner, J.; Polyak, S.] Univ Washington, Dept Lab Med, Seattle, WA 98104 USA. [MacDonald, J.; Bammler, T.; Farin, F.] Univ Washington, Dept Environm & Occupat Hlth Sci, Seattle, WA 98104 USA. [Kim, Y. M.; Robertson, B. J.; Metz, T.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. [Oberlies, N. H.] Univ N Carolina, Dept Chem & Biochem, Greensboro, NC 27412 USA. RI Kim, Young-Mo/D-3282-2009 OI Kim, Young-Mo/0000-0002-8972-7593 NR 0 TC 0 Z9 0 U1 0 U2 2 PU GEORG THIEME VERLAG KG PI STUTTGART PA RUDIGERSTR 14, D-70469 STUTTGART, GERMANY SN 0032-0943 EI 1439-0221 J9 PLANTA MED JI Planta Med. PD JUL PY 2015 VL 81 IS 11 MA PE14 BP 884 EP 884 PG 1 WC Plant Sciences; Chemistry, Medicinal; Integrative & Complementary Medicine; Pharmacology & Pharmacy SC Plant Sciences; Pharmacology & Pharmacy; Integrative & Complementary Medicine GA CP6AP UT WOS:000359967000138 ER PT J AU Lohman, JR Joachimiak, A Phillips, GN Shen, B AF Lohman, J. R. Joachimiak, A. Phillips, G. N., Jr. Shen, B. TI Structural and evolutionary relationships of ketosynthase domains from modular polyketide synthases SO PLANTA MEDICA LA English DT Meeting Abstract CT Annual Meeting of the American-Society-of-Pharmacognosy CY JUL 25-29, 2015 CL CO SP Amer Soc Pharmacognosy C1 [Lohman, J. R.] Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. [Joachimiak, A.] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Joachimiak, A.] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. [Phillips, G. N., Jr.] Rice Univ, Dept Biochem & Cell Biol, Houston, TX 77251 USA. [Shen, B.] Scripps Res Inst, Dept Chem, Jupiter, FL 33458 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU GEORG THIEME VERLAG KG PI STUTTGART PA RUDIGERSTR 14, D-70469 STUTTGART, GERMANY SN 0032-0943 EI 1439-0221 J9 PLANTA MED JI Planta Med. PD JUL PY 2015 VL 81 IS 11 MA PF5 BP 886 EP 886 PG 1 WC Plant Sciences; Chemistry, Medicinal; Integrative & Complementary Medicine; Pharmacology & Pharmacy SC Plant Sciences; Pharmacology & Pharmacy; Integrative & Complementary Medicine GA CP6AP UT WOS:000359967000147 ER PT J AU Sica, VP Raja, HA El-Elimat, T Kertesz, V Van Berke, GJ Pearce, CJ Oberlies, NH AF Sica, V. P. Raja, H. A. El-Elimat, T. Kertesz, V Van Berke, G. J. Pearce, C. J. Oberlies, N. H. TI Profiling fungal cultures in situ via the droplet-LMJ-SSP coupled with UPLC-PDA-HRMS-MS/MS SO PLANTA MEDICA LA English DT Meeting Abstract CT Annual Meeting of the American-Society-of-Pharmacognosy CY JUL 25-29, 2015 CL CO SP Amer Soc Pharmacognosy C1 [Sica, V. P.; Raja, H. A.; El-Elimat, T.; Oberlies, N. H.] Univ N Carolina, Dept Chem & Biochem, Greensboro, NC 27402 USA. [Kertesz, V; Van Berke, G. J.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. [Pearce, C. J.] Mycosynthetix Inc, Hillsborough, NC 27278 USA. RI Kertesz, Vilmos/M-8357-2016 OI Kertesz, Vilmos/0000-0003-0186-5797 NR 0 TC 0 Z9 0 U1 0 U2 0 PU GEORG THIEME VERLAG KG PI STUTTGART PA RUDIGERSTR 14, D-70469 STUTTGART, GERMANY SN 0032-0943 EI 1439-0221 J9 PLANTA MED JI Planta Med. PD JUL PY 2015 VL 81 IS 11 MA PR1 BP 915 EP 915 PG 1 WC Plant Sciences; Chemistry, Medicinal; Integrative & Complementary Medicine; Pharmacology & Pharmacy SC Plant Sciences; Pharmacology & Pharmacy; Integrative & Complementary Medicine GA CP6AP UT WOS:000359967000285 ER PT J AU Lovelace, ES Kline, T Olivas, K Wagoner, J Oberlies, NH Combet, C Anderson, LN Smith, RD Wright, AT Polyak, SJ AF Lovelace, E. S. Kline, T. Olivas, K. Wagoner, J. Oberlies, N. H. Combet, C. Anderson, L. N. Smith, R. D. Wright, A. T. Polyak, S. J. TI Identification of cellular protein targets of silymarin-derived flavonolignans SO PLANTA MEDICA LA English DT Meeting Abstract CT Annual Meeting of the American-Society-of-Pharmacognosy CY JUL 25-29, 2015 CL CO SP Amer Soc Pharmacognosy C1 [Lovelace, E. S.; Wagoner, J.; Polyak, S. J.] Univ Washington, Dept Lab Med, Seattle, WA 98104 USA. [Kline, T.; Olivas, K.; Polyak, S. J.] Univ Washington, Dept Microbiol, Seattle, WA 98104 USA. [Polyak, S. J.] Univ Washington, Dept Global Hlth, Seattle, WA 98104 USA. [Oberlies, N. H.] Univ N Carolina, Dept Chem, Greensboro, NC 27412 USA. [Combet, C.] INSERM, F-69008 Lyon, France. [Anderson, L. N.; Smith, R. D.; Wright, A. T.] Pacific NW Natl Lab, Richland, WA 99354 USA. RI Smith, Richard/J-3664-2012; Anderson, Lindsey /S-6375-2016 OI Smith, Richard/0000-0002-2381-2349; Anderson, Lindsey /0000-0002-8741-7823 NR 0 TC 0 Z9 0 U1 0 U2 2 PU GEORG THIEME VERLAG KG PI STUTTGART PA RUDIGERSTR 14, D-70469 STUTTGART, GERMANY SN 0032-0943 EI 1439-0221 J9 PLANTA MED JI Planta Med. PD JUL PY 2015 VL 81 IS 11 MA PX79 BP 946 EP 946 PG 1 WC Plant Sciences; Chemistry, Medicinal; Integrative & Complementary Medicine; Pharmacology & Pharmacy SC Plant Sciences; Pharmacology & Pharmacy; Integrative & Complementary Medicine GA CP6AP UT WOS:000359967000437 ER PT J AU Lu, ZM Vesselinov, VV AF Lu, Zhiming Vesselinov, Velimir V. TI Analytical sensitivity analysis of transient groundwater flow in a bounded model domain using the adjoint method SO WATER RESOURCES RESEARCH LA English DT Article DE sensitivity analysis; adjoint method; analytical solutions; transient flow ID TRAVEL-TIME PROBABILITIES; VARIABLY SATURATED FLOW; PUMPING TESTS; INVERSE PROBLEM; PARAMETER-IDENTIFICATION; HYDRAULIC TOMOGRAPHY; UNCONFINED AQUIFERS; NONUNIFORM AQUIFERS; POROUS-MEDIA; CONTAMINANT AB Sensitivity analyses are an important component of any modeling exercise. We have developed an analytical methodology based on the adjoint method to compute sensitivities of a state variable (hydraulic head) to model parameters (hydraulic conductivity and storage coefficient) for transient groundwater flow in a confined and randomly heterogeneous aquifer under ambient and pumping conditions. For a special case of two-dimensional rectangular domains, these sensitivities are represented in terms of the problem configuration (the domain size, boundary configuration, medium properties, pumping schedules and rates, and observation locations and times), and there is no need to actually solve the adjoint equations. As an example, we present analyses of the obtained solution for typical groundwater flow conditions. Analytical solutions allow us to calculate sensitivities efficiently, which can be useful for model-based analyses such as parameter estimation, data-worth evaluation, and optimal experimental design related to sampling frequency and locations of observation wells. The analytical approach is not limited to groundwater applications but can be extended to any other mathematical problem with similar governing equations and under similar conceptual conditions. C1 [Lu, Zhiming; Vesselinov, Velimir V.] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87544 USA. RP Lu, ZM (reprint author), Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, MS T003, Los Alamos, NM 87544 USA. EM zhiming@lanl.gov RI Vesselinov, Velimir/P-4724-2016; OI Vesselinov, Velimir/0000-0002-6222-0530; Lu, Zhiming/0000-0001-5800-3368 FU Environmental Programs Directorate of the Los Alamos National Laboratory FX This research was funded by the Environmental Programs Directorate of the Los Alamos National Laboratory. The data to support this paper are available, and can be obtained by contacting Zhiming Lu at zhiming@lanl.gov. The authors wish to thank the associated editor and three anonymous reviewers for comments that substantially improved the manuscript. The authors are grateful to Daniel O'Malley for his thorough review on the paper. NR 37 TC 0 Z9 0 U1 3 U2 13 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD JUL PY 2015 VL 51 IS 7 BP 5060 EP 5080 DI 10.1002/2014WR016819 PG 21 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA CP7PM UT WOS:000360080200010 ER PT J AU Rodriguez, JA AF Rodriguez, Jose A. TI Accessible atomic structures from sub-micron protein crystals SO ACTA CRYSTALLOGRAPHICA A-FOUNDATION AND ADVANCES LA English DT Editorial Material DE MicroED; nanocrystals; electron diffraction ID FREE-ELECTRON LASER; FEMTOSECOND CRYSTALLOGRAPHY; DIFFRACTION DATA; MODEL C1 Univ Calif Los Angeles, Dept Biol Chem, DOE Inst Genom & Prote, Los Angeles, CA 90024 USA. RP Rodriguez, JA (reprint author), Univ Calif Los Angeles, Dept Biol Chem, DOE Inst Genom & Prote, Los Angeles, CA 90024 USA. NR 24 TC 0 Z9 0 U1 3 U2 4 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2053-2733 J9 ACTA CRYSTALLOGR A JI Acta Crystallogr. Sect. A PD JUL PY 2015 VL 71 BP 351 EP 352 DI 10.1107/S2053273315012206 PN 4 PG 2 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CO5NF UT WOS:000359205100001 PM 26131893 ER PT J AU Granlund, L Billinge, SJL Duxbury, PM AF Granlund, L. Billinge, S. J. L. Duxbury, P. M. TI Algorithm for systematic peak extraction from atomic pair distribution functions SO ACTA CRYSTALLOGRAPHICA A-FOUNDATION AND ADVANCES LA English DT Article DE pair distribution function; peak extraction; model selection; Akaike information criterion; computer program ID AKAIKES INFORMATION CRITERION; SMALL-ANGLE SCATTERING; RADIAL-DISTRIBUTION FUNCTION; AB-INITIO DETERMINATION; MODEL SELECTION; POWDER DIFFRACTION; CRYSTAL-STRUCTURE; METALLIC GLASSES; NANOPARTICLES; REFINEMENT AB The study presents an algorithm, ParSCAPE, for model-independent extraction of peak positions and intensities from atomic pair distribution functions (PDFs). It provides a statistically motivated method for determining parsimony of extracted peak models using the information-theoretic Akaike information criterion (AIC) applied to plausible models generated within an iterative framework of clustering and chi-square fitting. All parameters the algorithm uses are in principle known or estimable from experiment, though careful judgment must be applied when estimating the PDF baseline of nanostructured materials. ParSCAPE has been implemented in the Python program SrMise. Algorithm performance is examined on synchrotron X-ray PDFs of 16 bulk crystals and two nanoparticles using AIC-based multimodeling techniques, and particularly the impact of experimental uncertainties on extracted models. It is quite resistant to misidentification of spurious peaks coming from noise and termination effects, even in the absence of a constraining structural model. Structure solution from automatically extracted peaks using the Liga algorithm is demonstrated for 14 crystals and for C-60. Special attention is given to the information content of the PDF, theory and practice of the AIC, as well as the algorithm's limitations. C1 [Granlund, L.; Duxbury, P. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Billinge, S. J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Billinge, S. J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Granlund, L (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM luke.r.granlund@gmail.com; sb2896@columbia.edu FU Center of Research Excellence in Complex Materials at Michigan State University; US Department of Energy, Office of Basic Energy Sciences (DOE-BES) at Brookhaven National Laboratory [DE-AC02-98CH10886]; US DOE-BES [W-31-109-Eng-38] FX We thank Dr Chris Farrow and Dr Pavol Juhas for productive conversations, particularly regarding the PDF baseline and uncertainties. We gratefully acknowledge the preceding as well as Dr Saurabh Gujarathi, Dr Peng Tian, Max Terban and Soham Banerjee for help testing SrMise. We appreciate the efforts of Dr Emil Bozin, Dr Ahmad Masadeh and Dr Douglas Robinson for assistance with the X-ray measurements at the Advanced Photon Source, Argonne National Laboratory (APS, ANL). We thank Dr Christos Malliakas for providing the NaCl, PbTe nanoparticle and ZnS wurtzite samples, as well as Professor Harry Dorn for the C60 sample. Work at MSU was supported by the Center of Research Excellence in Complex Materials at Michigan State University. Work in the Billinge group was supported by the US Department of Energy, Office of Basic Energy Sciences (DOE-BES), as the complex modeling laboratory directed research and development grant at Brookhaven National Laboratory through contract DE-AC02-98CH10886. The Advanced Photon Source is supported by the US DOE-BES under contract No. W-31-109-Eng-38. NR 78 TC 3 Z9 3 U1 5 U2 30 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2053-2733 J9 ACTA CRYSTALLOGR A JI Acta Crystallogr. Sect. A PD JUL PY 2015 VL 71 BP 392 EP 409 DI 10.1107/S2053273315005276 PN 4 PG 18 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CO5NF UT WOS:000359205100006 PM 26131896 ER PT J AU Yan, LH Wu, RT Bao, DL Ren, JH Zhang, YF Zhang, HG Huang, L Wang, YL Du, SX Huan, Q Gao, HJ AF Yan Ling-Hao Wu Rong-Ting Bao De-Liang Ren Jun-Hai Zhang Yan-Fang Zhang Hai-Gang Huang Li Wang Ye-Liang Du Shi-Xuan Huan Qing Gao Hong-Jun TI Adsorption behavior of Fe atoms on a naphthalocyanine monolayer on Ag(111) surface SO CHINESE PHYSICS B LA English DT Article DE naphthalocyanine; Fe atoms; Ag(111) surface; adsorption behavior ID SCANNING-TUNNELING-MICROSCOPY; METAL-FREE NAPHTHALOCYANINE; SUBMONOLAYER COVERAGE; MAGNETIC-ANISOTROPY; IRON PHTHALOCYANINE; AU(111) SURFACE; SPECTROSCOPY; MOLECULES; NANOSTRUCTURES; CLUSTERS AB Adsorption behavior of Fe atoms on a metal-free naphthalocyanine (H(2)Nc) monolayer on Ag(111) surface at room temperature has been investigated using scanning tunneling microscopy combined with density functional theory (DFT) based calculations. We found that the Fe atoms were adsorbed on the centers of H(2)Nc molecules and formed Fe-H(2)Nc complexes at low coverage. DFT calculations show that Fe sited in the center of the molecule is the most stable configuration, in good agreement with the experimental observations. After an Fe-H(2)Nc complex monolayer was formed, the extra Fe atoms self-assembled to Fe clusters of uniform size and adsorbed dispersively at the interstitial positions of Fe-H(2)Nc complex monolayer. Therefore, the H(2)Nc monolayer grown on Ag(111) could be a good template to grow dispersed magnetic metal atoms and clusters at room temperature for further investigation of their magnetism-related properties. C1 [Yan Ling-Hao; Wu Rong-Ting; Ren Jun-Hai; Zhang Yan-Fang; Huang Li; Wang Ye-Liang; Du Shi-Xuan; Huan Qing; Gao Hong-Jun] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. [Bao De-Liang; Wang Ye-Liang; Du Shi-Xuan; Huan Qing; Gao Hong-Jun] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Zhang Hai-Gang] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Du, SX (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. EM sxdu@iphy.ac.cn; huanq@iphy.ac.cn RI Du, Shixuan/K-7145-2012; WANG, Yeliang/D-9643-2012 OI Du, Shixuan/0000-0001-9323-1307; FU National Natural Science Foundation of China [61390501, 51325204, 11204361]; National Basic Research Program of China [2011CB808401, 2011CB921702]; National Key Scientific Instrument and Equipment Development Project of China [2013YQ1203451]; National Supercomputing Center in Tianjin, China; Chinese Academy of Sciences FX Project supported by the National Natural Science Foundation of China (Grant Nos. 61390501, 51325204, and 11204361), the National Basic Research Program of China (Grant Nos. 2011CB808401 and 2011CB921702), the National Key Scientific Instrument and Equipment Development Project of China (Grant No. 2013YQ1203451), the National Supercomputing Center in Tianjin, China, and the Chinese Academy of Sciences. NR 48 TC 1 Z9 1 U1 3 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1674-1056 EI 1741-4199 J9 CHINESE PHYS B JI Chin. Phys. B PD JUL PY 2015 VL 24 IS 7 AR 076802 DI 10.1088/1674-1056/24/7/076802 PG 5 WC Physics, Multidisciplinary SC Physics GA CP1UU UT WOS:000359662600057 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalosa, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D 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Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamada, M. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yanush, S. Yao, L. Yao, W-M. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yurkewicz, A. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena in final states with an energetic jet and large missing transverse momentum in pp collisions at root s=8 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DYNAMICAL SUPERSYMMETRY BREAKING; HIGGS-BOSON PRODUCTION; CARLO EVENT GENERATOR; E(+)E(-) COLLISIONS; HADRON COLLIDERS; DARK-MATTER; SUPERGAUGE TRANSFORMATIONS; ELECTROWEAK CORRECTIONS; CROSS-SECTION; SINGLE-PHOTON AB Results of a search for new phenomena in final states with an energetic jet and large missing transverse momentum are reported. The search uses 20.3 fb(-1) of root s = 8 TeV data collected in 2012 with the ATLAS detector at the LHC. Events are required to have at least one jet with pT > 120 GeV and no leptons. Nine signal regions are considered with increasing missing transverse momentum requirements between E-T(miss) > 150 GeV and E-T(miss) > 700 GeV. Good agreement is observed between the number of events in data and Standard Model expectations. The results are translated into exclusion limits on models with either large extra spatial dimensions, pair production of weakly interacting dark matter candidates, or production of very light gravitinos in a gauge-mediated supersymmetric model. In addition, limits on the production of an invisibly decaying Higgs-like boson leading to similar topologies in the final state are presented. C1 [ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Alfred, Dept Phys, Albany, NY USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. 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A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duerssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Messina, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; TenKate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Krizka, K.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Fac Fis, Santiago 22, Chile. [Brooks, W. K.; Kuleshov, S.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Coll Cosenza, Lab Nazl Frascati, Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Experimentelle Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Wall, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvilib, A.; Khubua, J.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E-E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Glonti, G. L.; Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto 606, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Dept Phys, Jozef Stefan Inst, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cerio, B. C.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Kpke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, B I Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, P N Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Kishimoto, T.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] M V Lomonosov Moscow State Univ, D V skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Iengo, P.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Arik, M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Cetin, S. A.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Ideal, E.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Ideal, E.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Beresford, L.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Saraiva, J. G.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Carvalho, J.; Galhardo, B.; Gomes, A.; Maioa, A.; Maneira, J.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Carvalho, J.; Muino, P. Conde; de Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maioa, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Galhardo, B.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maioa, A.; Pina, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Hasegawa, S.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. 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C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Ceradini, F.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univ, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S-C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalosa, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Annovi, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Jeanty, L.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sin, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.] Techn Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Diamond, M.; Ilic, N.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] INFN Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Cerny, K.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzaez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzaez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzaez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzaez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzaez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kwan, T.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Hellman, S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astronomie, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maetig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Gkougkousis, E. L.; Guest, D.; Henrichs, A.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. Kings Coll London, Dept Phys, London, England. 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[Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI la rotonda, laura/B-4028-2016; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Livan, Michele/D-7531-2012; Shmeleva, Alevtina/M-6199-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013 OI la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Livan, Michele/0000-0002-5877-0062; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRCand Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society; DOE and NSF, United States of America; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRCand Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 138 TC 46 Z9 46 U1 16 U2 77 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 1 PY 2015 VL 75 IS 7 AR 299 DI 10.1140/epjc/s10052-015-3517-3 PG 43 WC Physics, Particles & Fields SC Physics GA CL7AZ UT WOS:000357123400003 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-Conde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, G Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, M Martins, TD Herrera, CM Pol, ME Teles, PR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, J Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, J Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T 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CA CMS Collaboration TI Distributions of topological observables in inclusive three- and four-jet events in pp collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SPIN CORRELATIONS; Z0 DECAYS; QCD; FRAGMENTATION; SIMULATION; JETS AB This paper presents distributions of topological observables in inclusive three- and four-jet events produced in pp collisions at a centre-of-mass energy of 7 TeV with a data sample collected by the CMS experiment corresponding to a luminosity of 5.1 fb(-1). The distributions are corrected for detector effects, and compared with several event generators based on two- and multi-parton matrix elements at leading order. Among the considered calculations, MadGraph interfaced with PYTHIA6 displays the overall best agreement with data. C1 [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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[Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Kamel, A. Ellithi; Mahmoud, M. A.; Radi, A.] Arab Republ Egypt, Egyptian Network High Energy Phys, Acad Sci Res & Technol, Cairo, Egypt. [Giammanco, A.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. 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C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Gadrat, S.] CNRS IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Bouvier, E.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Edelhoff, M.; Feld, L.; Heister, A.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Raupach, F.; Sammet, J.; Schael, S.; Schulte, F.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behr, J.; Behrens, U.; Bell, A. J.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, L.; Kruecker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Ron, E.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Anagnostou, G.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Debrecen Univ Med, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Sirolia, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Sirolia, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Nazl Frascati Lab, I-00044 Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Biasotto, M.; Dall'Osso, M.; Dorigo, T.; Galanti, M.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Ventura, S.; Zotto, P.; Zucchetta, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Biasotto, M.; Dorigo, T.; Galanti, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.; Margoni, M.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Broccolo, G.; Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.; Verdini, P. G.] Univ Pisa, Pisa, Italy. [Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, T. A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Chonju, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, L.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Vinca Inst Nucl Sci, Belgrade 11001, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Paolucci, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, P.; Casasso, S.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; Moon, D. H.; O'Brien, C.; Gonzalez, L. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kennyiii, R. P.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Malik, S.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Biasotto, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Kaya, M.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A& M Univ Qatar, Doha, Qatar. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; ciocci, maria agnese /I-2153-2015; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Dremin, Igor/K-8053-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Rovelli, Tiziano/K-4432-2015 OI Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Ghezzi, Alessio/0000-0002-8184-7953; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Di Matteo, Leonardo/0000-0001-6698-1735; Boccali, Tommaso/0000-0002-9930-9299; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Montanari, Alessandro/0000-0003-2748-6373; Rovelli, Tiziano/0000-0002-9746-4842 FU European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET(European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 37 TC 0 Z9 0 U1 9 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 1 PY 2015 VL 75 IS 7 AR 302 DI 10.1140/epjc/s10052-015-3491-9 PG 26 WC Physics, Particles & Fields SC Physics GA CL7AZ UT WOS:000357123400006 ER PT J AU Sabne, A Sakdhnagool, P Lee, S Vetter, JS AF Sabne, Amit Sakdhnagool, Putt Lee, Seyong Vetter, Jeffrey S. TI UNDERSTANDING PORTABILITY OF A HIGH-LEVEL PROGRAMMING MODEL ON CONTEMPORARY HETEROGENEOUS ARCHITECTURES SO IEEE MICRO LA English DT Article AB HeteroIR is a high-level, architecture-independent intermediate representation for mapping high-level programming models to heterogeneous architectures. The authors present a compiler approach that translates OpenACC programs into HeteroIR and accelerator kernels to obtain OpenACC functional portability. They evaluate the performance portability obtained by OpenACC and study the effects of compiler optimizations and OpenACC program settings on various architectures to provide insights into the achieved performance portability. C1 [Sabne, Amit; Sakdhnagool, Putt] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Lee, Seyong] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN USA. [Vetter, Jeffrey S.] Oak Ridge Natl Lab, Future Technol Grp, Oak Ridge, TN USA. RP Sabne, A (reprint author), Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. EM asabne@purdue.edu; psakdhna@purdue.edu; lees2@ornl.gov; vetter@ornl.gov FU US Department of Energy [DE-AC05-00OR22725]; Office of Advanced Scientific Computing Research in the DoE FX This manuscript has been authored by Oak Ridge National Laboratory, which is managed by UT-Battelle under contract no. DE-AC05-00OR22725 with the US Department of Energy. The US government retains, and the publisher, by accepting the article for publication, acknowledges that the US government retains, a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. The DoE will provide public access to these results of federally sponsored research in accordance with the DoE Public Access Plan (http://energy.gov/downloads/doe-public-accessplan). This research is sponsored by the Office of Advanced Scientific Computing Research in the DoE. NR 9 TC 1 Z9 1 U1 0 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1732 EI 1937-4143 J9 IEEE MICRO JI IEEE Micro PD JUL-AUG PY 2015 VL 35 IS 4 BP 48 EP 58 PG 11 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA CP0VN UT WOS:000359594300007 ER PT J AU Sakaguchi, K Leung, LR Zhao, C Yang, Q Lu, J Hagos, S Rauscher, SA Dong, L Ringler, TD Lauritzen, PH AF Sakaguchi, Koichi Leung, L. Ruby Zhao, Chun Yang, Qing Lu, Jian Hagos, Samson Rauscher, Sara A. Dong, Li Ringler, Todd D. Lauritzen, Peter H. TI Exploring a Multiresolution Approach Using AMIP Simulations SO JOURNAL OF CLIMATE LA English DT Review ID COMMUNITY-ATMOSPHERIC-MODEL; REGIONAL CLIMATE-CHANGE; LOW-LEVEL JET; SOUTHERN-HEMISPHERE WINTER; GENERAL-CIRCULATION MODEL; DYNAMICAL CORE; AQUAPLANET SIMULATIONS; PRECIPITATION EXTREMES; HORIZONTAL RESOLUTION; GLOBAL PRECIPITATION AB This study presents a diagnosis of a multiresolution approach using the Model for Prediction Across Scales-Atmosphere (MPAS-A) for simulating regional climate. Four Atmospheric Model Intercomparison Project (AMIP) experiments were conducted for 1999-2009. In the first two experiments, MPAS-A was configured using global quasi-uniform grids at 120- and 30-km grid spacing. In the other two experiments, MPAS-A was configured using variable-resolution (VR) mesh with local refinement at 30 km over North America and South America and embedded in a quasi-uniform domain at 120 km elsewhere. Precipitation and related fields in the four simulations are examined to determine how well the VRs reproduce the features simulated by the globally high-resolution model in the refined domain. In previous analyses of idealized aquaplanet simulations, characteristics of the global high-resolution simulation in moist processes developed only near the boundary of the refined region. In contrast, AMIP simulations with VR grids can reproduce high-resolution characteristics across the refined domain, particularly in South America. This finding indicates the importance of finely resolved lower boundary forcings such as topography and surface heterogeneity for regional climate and demonstrates the ability of the MPAS-A VR to replicate the large-scale moisture transport as simulated in the quasi-uniform high-resolution model. Upscale effects from the high-resolution regions on a large-scale circulation outside the refined domain are observed, but the effects are mainly limited to northeastern Asia during the warm season. Together, the results support the multiresolution approach as a computationally efficient and physically consistent method for modeling regional climate. C1 [Sakaguchi, Koichi; Leung, L. Ruby; Zhao, Chun; Yang, Qing; Lu, Jian; Hagos, Samson] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Rauscher, Sara A.] Univ Delaware, Dept Geog, Newark, DE USA. [Dong, Li] Auburn Univ, Sch Forestry & Wildlife Sci, Auburn, AL 36849 USA. [Ringler, Todd D.] Los Alamos Natl Lab, Climate Ocean & Sea Ice Modeling Grp, Div Theoret, Los Alamos, NM USA. [Lauritzen, Peter H.] Natl Ctr Atmospher Res, Climate & Global Dynam Lab, Boulder, CO 80307 USA. RP Leung, LR (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, 902 Battelle Blvd, Richland, WA 99352 USA. EM ruby.leung@pnnl.gov RI Yang, Qing/H-3275-2011; Zhao, Chun/A-2581-2012 OI Yang, Qing/0000-0003-2067-5999; Zhao, Chun/0000-0003-4693-7213 FU U.S. Department of Energy (DOE) Office of Science Biological and Environmental Research; Office of Science [DE-AC02-05CH11231]; National Science Foundation; DOE by Battelle Memorial Institute [DE-AC05-76RL01830] FX This study was supported by the U.S. Department of Energy (DOE) Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling program. The research used computational resources from the National Energy Research Scientific Computing Center (NERSC), a DOE User Facility supported by the Office of Science under Contract DE-AC02-05CH11231. Additional computational resources were provided by the Pacific Northwest National Laboratory (PNNL) Institutional Computing program. The FV-CAM4 data were provided by the Earth system grid data portal from the National Center for Atmospheric Research (NCAR), which is supported by grants from the National Science Foundation. The authors wish to thank Dr. Travis O'Brien of Lawrence Berkeley National Laboratory for facilitating the use of the model data archive at NERSC. We also thank Drs. Jin-Ho Yoon, Matus Martini, Phil Rasch, and Hailong Wang for their insights provided through discussions. The thorough review and constructive comments by two anonymous reviewers are also greatly appreciated. PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. NR 119 TC 6 Z9 6 U1 2 U2 10 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD JUL PY 2015 VL 28 IS 14 BP 5549 EP 5574 DI 10.1175/JCLI-D-14-00729.1 PG 26 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CP1LR UT WOS:000359637800004 ER PT J AU Yang, B Zhang, YC Qian, Y Wu, TW Huang, AN Fang, YJ AF Yang, Ben Zhang, Yaocun Qian, Yun Wu, Tongwen Huang, Anning Fang, Yongjie TI Parametric Sensitivity Analysis for the Asian Summer Monsoon Precipitation Simulation in the Beijing Climate Center AGCM, Version 2.1 SO JOURNAL OF CLIMATE LA English DT Article ID CONVECTIVE PARAMETERIZATION SCHEME; GENERAL-CIRCULATION MODELS; SEA-SURFACE TEMPERATURE; TROPICAL INDIAN-OCEAN; INTERANNUAL VARIABILITY; EAST-ASIA; EL-NINO; WESTERN PACIFIC; UNCERTAINTY QUANTIFICATION; CUMULUS PARAMETERIZATION AB In this study, the authors apply an efficient sampling approach and conduct a large number of simulations to explore the sensitivity of the simulated Asian summer monsoon (ASM) precipitation, including the climatological state and interannual variability, to eight parameters related to the cloud and precipitation processes in the Beijing Climate Center AGCM, version 2.1 (BCC_AGCM2.1). The results herein show that BCC_AGCM2.1 has large biases in simulating the ASM precipitation. The precipitation efficiency and evaporation coefficient for deep convection are the most sensitive parameters in simulating the ASM precipitation. With optimal parameter values, the simulated precipitation climatology could be remarkably improved, including increased precipitation over the equatorial Indian Ocean, suppressed precipitation over the Philippine Sea, and more realistic mei-yu distribution over eastern China. The ASM precipitation interannual variability is further analyzed, with a focus on the ENSO impacts. It is shown that simulations with better ASM precipitation climatology can also produce more realistic precipitation anomalies during El Nino-decaying summer. In the low-skill experiments for precipitation climatology, the ENSO-induced precipitation anomalies are most significant over continents (vs over ocean in observations) in the South Asian monsoon region. More realistic results are derived from the higher-skill experiments with stronger anomalies over the Indian Ocean and weaker anomalies over India and the western Pacific Ocean, favoring more evident easterly anomalies forced by the tropical Indian Ocean warming and stronger Indian Ocean-western Pacific teleconnection as observed. The model results reveal a strong connection between the simulated ASM precipitation climatological state and interannual variability in BCC_AGCM2.1 when key parameters are perturbed. C1 [Yang, Ben; Zhang, Yaocun; Huang, Anning] Nanjing Univ, Sch Atmospher Sci, Nanjing 210023, Jiangsu, Peoples R China. [Yang, Ben; Zhang, Yaocun; Huang, Anning] Jiangsu Collaborat Innovat Ctr Climate Change, Nanjing, Jiangsu, Peoples R China. [Qian, Yun] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Wu, Tongwen; Fang, Yongjie] China Meteorol Adm, Natl Climate Ctr, Beijing Climate Ctr, Beijing, Peoples R China. RP Zhang, YC (reprint author), Nanjing Univ, Sch Atmospher Sci, 163 Xianlin Ave, Nanjing 210023, Jiangsu, Peoples R China. EM yczhang@nju.edu.cn RI qian, yun/E-1845-2011; Yang, Ben/O-8548-2015 FU National Natural Science Foundation of China [41305084, 41475092]; Fundamental Research Funds for the Central Universities [20620140049]; Special Program for China Meteorology Trade [GYHY201306020]; Jiangsu Collaborative Innovation Center for Climate Change; U.S. Department of Energy's (DOE) Office of Science; DOE by Battelle Memorial Institute [DE-AC05-76RL01830] FX The authors acknowledge the editor and three anonymous reviewers for the careful review and constructive comments, and Xiaoge Xin and Jie Zhang of the Beijing Climate Center for help in model configurations. This work is jointly supported by the National Natural Science Foundation of China (41305084 and 41475092), the Fundamental Research Funds for the Central Universities (20620140049), the Special Program for China Meteorology Trade (GYHY201306020), and the Jiangsu Collaborative Innovation Center for Climate Change. The contribution of Yun Qian in this study is supported by the U.S. Department of Energy's (DOE) Office of Science as part of the Regional and Global Climate Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under Contract DE-AC05-76RL01830. NR 98 TC 4 Z9 4 U1 5 U2 15 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD JUL PY 2015 VL 28 IS 14 BP 5622 EP 5644 DI 10.1175/JCLI-D-14-00655.1 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CP1LR UT WOS:000359637800008 ER PT J AU Simas-Rodrigues, C Villela, HDM Martins, AP Marques, LG Colepicolo, P Tonon, AP AF Simas-Rodrigues, Cntia Villela, Helena D. M. Martins, Aline P. Marques, Luiza G. Colepicolo, Pio Tonon, Angela P. TI Microalgae for economic applications: advantages and perspectives for bioethanol SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Review DE Biochemical effects; bioethanol; biofuels; environmental impacts; genetic manipulation; microalgae ID ADP-GLUCOSE PYROPHOSPHORYLASE; CHLORELLA-VULGARIS BEIJERINCK; CHLAMYDOMONAS-REINHARDTII BIOMASS; CHLOROPHYLL ANTENNA SIZE; ETHANOL-PRODUCTION; ZYMOMONAS-MOBILIS; BIOFUEL PRODUCTION; GREEN-ALGA; FERMENTATIVE METABOLISM; BIODIESEL PRODUCTION AB Renewable energy has attracted significant interest in recent years as a result of sustainability, environmental impact, and socio-economic considerations. Given existing technological knowledge and based on projections relating to biofuels derived from microalgae, microalgal feedstock is considered to be one of the most important renewable energy sources potentially available for industrial production. Therefore, this review examines microalgal bioethanol technology, which converts biomass from microalgae to fuel, the chemical processes involved, and possible ways of increasing the bioethanol yield, such as abiotic factors and genetic manipulation of fermenting organisms. C1 [Simas-Rodrigues, Cntia; Villela, Helena D. M.; Martins, Aline P.; Marques, Luiza G.; Colepicolo, Pio] Univ Sao Paulo, Inst Quim, Dept Bioquim, BR-05508000 Sao Paulo, Brazil. [Tonon, Angela P.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Tonon, AP (reprint author), Los Alamos Natl Lab, Biosci Div, POB M888, Los Alamos, NM 87545 USA. EM angptpnon@gmail.com RI Tonon, Angela/H-3546-2012; Martins, Aline/H-7951-2012 OI Martins, Aline/0000-0003-4847-7580 FU Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Foundation for Research Support of the State of Sao Paulo) [11/16072-5, 10/50193-1, 04/11459-5]; FAPESP [11/16072-5, 10/50193-1, 04/11459-5]; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (National Counsel of Technological and Scientific Development, CNPq) [142168/2009-2] FX This work was supported by Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Foundation for Research Support of the State of Sao Paulo, or FAPESP) [projects 11/16072-5, 10/50193-1 and 04/11459-5] and Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (National Counsel of Technological and Scientific Development, CNPq) [project 142168/2009-2]. NR 140 TC 6 Z9 6 U1 1 U2 45 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4097 EP 4108 DI 10.1093/jxb/erv130 PG 12 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900002 PM 25873683 ER PT J AU Cushman, JC Davis, SC Yang, XH Borland, AM AF Cushman, John C. Davis, Sarah C. Yang, Xiaohan Borland, Anne M. TI Development and use of bioenergy feedstocks for semi-arid and arid lands SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Review DE Agave; arid lands; bioenergy feedstocks; ethanol; Opuntia; renewable energy; semi-arid lands ID OPUNTIA-FICUS-INDICA; CRASSULACEAN ACID METABOLISM; CACTUS PEAR OPUNTIA; ENVIRONMENTAL PRODUCTIVITY INDEXES; AGAVE-TEQUILANA WEBER; NET CO2 UPTAKE; ETHANOL-PRODUCTION; WATER FOOTPRINT; LIGNOCELLULOSIC BIOFUELS; KLUYVEROMYCES-MARXIANUS AB Global climate change is predicted to increase heat, drought, and soil-drying conditions, and thereby increase crop sensitivity to water vapour pressure deficit, resulting in productivity losses. Increasing competition between agricultural freshwater use and municipal or industrial uses suggest that crops with greater heat and drought durability and greater water-use efficiency will be crucial for sustainable biomass production systems in the future. Agave (Agavaceae) and Opuntia (Cactaceae) represent highly water-use efficient bioenergy crops that could diversify bioenergy feedstock supply yet preserve or expand feedstock production into semi-arid, abandoned, or degraded agricultural lands, and reclaim drylands. Agave and Opuntia are crassulacean acid metabolism species that can achieve high water-use efficiencies and grow in water-limited areas with insufficient precipitation to support traditional C-3 or C-4 bioenergy crops. Both Agave and Opuntia have the potential to produce above-ground biomass rivalling that of C-3 and C-4 crops under optimal growing conditions. The low lignin and high amorphous cellulose contents of Agave and Opuntia lignocellulosic biomass will be less recalcitrant to deconstruction than traditional feedstocks, as confirmed by pretreatments that improve saccharification of Agave. Refined environmental productivity indices and geographical information systems modelling have provided estimates of Agave and Opuntia biomass productivity and terrestrial sequestration of atmospheric CO2; however, the accuracy of such modelling efforts can be improved through the expansion of field trials in diverse geographical settings. Lastly, life cycle analysis indicates that Agave would have productivity, life cycle energy, and greenhouse gas balances comparable or superior to those of traditional bioenergy feedstocks, but would be far more water-use efficient. C1 [Cushman, John C.] Univ Nevada, Dept Biochem & Mol Biol, MS330, Reno, NV 89557 USA. [Davis, Sarah C.] Ohio Univ, Voinovich Sch Leadership & Publ Affairs, Athens, OH 45701 USA. [Davis, Sarah C.] Ohio Univ, Dept Environm & Plant Biol, Athens, OH 45701 USA. [Yang, Xiaohan; Borland, Anne M.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Borland, Anne M.] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Cushman, JC (reprint author), Univ Nevada, Dept Biochem & Mol Biol, MS330, Reno, NV 89557 USA. EM jcushman@unr.edu RI Yang, Xiaohan/A-6975-2011 OI Yang, Xiaohan/0000-0001-5207-4210 FU Department of Energy (DOE), Office of Science, Genomic Science Program [DE-SC0008834]; Nevada Agricultural Experiment Station [NAES-00377, NAES-00380]; US DOE [DE-AC05-00OR22725] FX This review is based on work supported by the Department of Energy (DOE), Office of Science, Genomic Science Program under Award Number DE-SC0008834. Additional support from the Nevada Agricultural Experiment Station under projects NAES-00377 and NAES-00380 is acknowledged. The contents of this review are solely the responsibility of the authors and do not necessarily represent the official views of the DOE. The authors wish to Mary Ann Cushman for critical review and clarifying comments on the manuscript and Lori Kunder (Kunder Design Studio) for assistance with figure preparation. Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the US DOE under Contract Number DE-AC05-00OR22725. NR 171 TC 7 Z9 7 U1 8 U2 39 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4177 EP 4193 DI 10.1093/jxb/erv087 PG 17 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900008 PM 25873672 ER PT J AU Pattathil, S Hahn, MG Dale, BE Chundawat, SPS AF Pattathil, Sivakumar Hahn, Michael G. Dale, Bruce E. Chundawat, Shishir P. S. TI Insights into plant cell wall structure, architecture, and integrity using glycome profiling of native and AFEX (TM)-pre-treated biomass SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE AFEX; biofuels; cell walls; glycome profiling; plant biomass; recalcitrance ID FIBER EXPANSION AFEX; LIGNOCELLULOSIC BIOMASS; ENZYMATIC DIGESTIBILITY; MONOCLONAL-ANTIBODIES; PRETREATMENT; RECALCITRANCE; HEMICELLULOSE; CELLULOSE; BIOFUELS; ENZYMES AB Cell walls, which constitute the bulk of plant biomass, vary considerably in their structure, composition, and architecture. Studies on plant cell walls can be conducted on both native and pre-treated plant biomass samples, allowing an enhanced understanding of these structural and compositional variations. Here glycome profiling was employed to determine the relative abundance of matrix polysaccharides in several phylogenetically distinct native and pre-treated plant biomasses. Eight distinct biomass types belonging to four different subgroups (i.e. monocot grasses, woody dicots, herbaceous dicots, and softwoods) were subjected to various regimes of AFEX (TM) (ammonia fiber expansion) pre-treatment [AFEX is a trademark of MBI, Lansing (http://www.mbi.org)]. This approach allowed detailed analysis of close to 200 cell wall glycan epitopes and their relative extractability using a high-throughput platform. In general, irrespective of the phylogenetic origin, AFEX (TM) pre-treatment appeared to cause loosening and improved accessibility of various xylan epitope subclasses in most plant biomass materials studied. For most biomass types analysed, such loosening was also evident for other major non-cellulosic components including subclasses of pectin and xyloglucan epitopes. The studies also demonstrate that AFEX (TM) pre-treatment significantly reduced cell wall recalcitrance among diverse phylogenies (except softwoods) by inducing structural modifications to polysaccharides that were not detectable by conventional gross composition analyses. It was found that monitoring changes in cell wall glycan compositions and their relative extractability for untreated and pre-treated plant biomass can provide an improved understanding of variations in structure and composition of plant cell walls and delineate the role(s) of matrix polysaccharides in cell wall recalcitrance. C1 [Pattathil, Sivakumar; Hahn, Michael G.] Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. [Pattathil, Sivakumar; Hahn, Michael G.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Dale, Bruce E.; Chundawat, Shishir P. S.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. RP Pattathil, S (reprint author), Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. EM siva@ccrc.uga.edu; shishir.chundawat@rutgers.edu FU Office of Biological and Environmental Research, Office of Science, US Department of Energy [DE-AC05-00OR22725]; National Science Foundation Plant Genome Program [DBI-0421683, IOS-0923992]; Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-FC02-07ER64494]; National Science Foundation [1236120] FX The glycome profiling analyses were supported by the BioEnergy Science Center administered by Oak Ridge National Laboratory and funded by Grant DE-AC05-00OR22725 from the Office of Biological and Environmental Research, Office of Science, US Department of Energy. The generation of the CCRC series of plant cell wall glycan-directed monoclonal antibodies used in this work was supported by the National Science Foundation Plant Genome Program (DBI-0421683 and IOS-0923992). Biomass pre-treatment and composition analyses were supported by the DOE Great Lakes Bioenergy Research Center (supported by the Department of Energy, Office of Science, Office of Biological and Environmental Research, through Cooperative Agreement DE-FC02-07ER64494 between The Board of Regents of the University of Wisconsin System and the Department of Energy). SPSC acknowledges partial support from the National Science Foundation Grant #1236120 (CBET-Energy for Sustainability) and would like to thank all members of the Dale lab for their enthusiastic and timely support. We also thank the GLBRC Cell Wall Analytical Facility (Cliff Foster) for conducting biomass composition analyses. We thank Professor Jonathan Walton (Michigan State University), Professor Art Ragauskas (Georgia Institute of Technology), and Professor Jack Saddler (University of British Columbia) for providing the goldenrod, loblolly pine, and Douglas fir biomass samples. We thank Ms Maria J Soto, a graduate student in our laboratory, for critically reading the manuscript. Special thanks to Novozymes for their generous gift of enzymes. NR 58 TC 10 Z9 11 U1 7 U2 39 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4279 EP 4294 DI 10.1093/jxb/erv107 PG 16 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900015 PM 25911738 ER PT J AU Li, MY Heckwolf, M Crowe, JD Williams, DL Magee, TD Kaeppler, SM de Leon, N Hodge, DB AF Li, Muyang Heckwolf, Marlies Crowe, Jacob D. Williams, Daniel L. Magee, Timothy D. Kaeppler, Shawn M. de Leon, Natalia Hodge, David B. TI Cell-wall properties contributing to improved deconstruction by alkaline pre-treatment and enzymatic hydrolysis in diverse maize (Zea mays L.) lines SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE Biofuels; cell-wall recalcitrance; enzymatic hydrolysis; maize; plant cell-wall characterization; pre-treatment ID FORAGE QUALITY VARIATION; NEUTRAL DETERGENT FIBER; IN-VITRO DIGESTIBILITY; 3 PERENNIAL GRASSES; CORN STOVER; BIOMASS RECALCITRANCE; STRUCTURAL FEATURES; CELLULOSIC ETHANOL; DOWN-REGULATION; SUGAR RELEASE AB A maize (Zea mays L. subsp. mays) diversity panel consisting of 26 maize lines exhibiting a wide range of cell-wall properties and responses to hydrolysis by cellulolytic enzymes was employed to investigate the relationship between cell-wall properties, cell-wall responses to mild NaOH pre-treatment, and enzymatic hydrolysis yields. Enzymatic hydrolysis of the cellulose in the untreated maize was found to be positively correlated with the water retention value, which is a measure of cell-wall susceptibility to swelling. It was also positively correlated with the lignin syringyl/guaiacyl ratio and negatively correlated with the initial cell-wall lignin, xylan, acetate, and p-coumaric acid (pCA) content, as well as pCA released from the cell wall by pre-treatment. The hydrolysis yield following pre-treatment exhibited statistically significant negative correlations to the lignin content after pre-treatment and positive correlations to the solubilized ferulic acid and pCA. Several unanticipated results were observed, including a positive correlation between initial lignin and acetate content, lack of correlation between acetate content and initial xylan content, and negative correlation between each of these three variables to the hydrolysis yields for untreated maize. Another surprising result was that pCA release was negatively correlated with hydrolysis yields for untreated maize and, along with ferulic acid release, was positively correlated with the pre-treated maize hydrolysis yields. This indicates that these properties that may negatively contribute to the recalcitrance in untreated cell walls may positively contribute to their deconstruction by alkaline pre-treatment. C1 [Li, Muyang; Hodge, David B.] Michigan State Univ, Dept Biosyst & Agr Engn, E Lansing, MI 48824 USA. [Li, Muyang; Heckwolf, Marlies; Williams, Daniel L.; Kaeppler, Shawn M.; de Leon, Natalia; Hodge, David B.] DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53703 USA. [Crowe, Jacob D.; Williams, Daniel L.; Magee, Timothy D.; Hodge, David B.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Kaeppler, Shawn M.; de Leon, Natalia] Univ Wisconsin, Dept Agron, Madison, WI 53706 USA. [Hodge, David B.] Lulea Univ Technol, Div Sustainable Proc Engn, S-97187 Lulea, Sweden. RP Hodge, DB (reprint author), Michigan State Univ, Dept Biosyst & Agr Engn, E Lansing, MI 48824 USA. EM hodgeda@msu.edu OI Kaeppler, Shawn/0000-0002-5964-1668 FU US Department of Energy Great Lakes Bioenergy Research Center [DOE BER Office of Science DE-FC02-07ER64494]; US National Science Foundation [NSF CBET 1336622]; US Department of Energy, Office of Science [DE-FOA-0000995]; US Department of Energy, Office of Basic Energy Sciences (BES) [DE-FOA-0000995]; US Department of Energy, Office of Biological and Environmental Research (BER) [DE-FOA-0000995] FX The authors would like to acknowledge Robert Sykes (NREL) for generously performing py-MBMS analysis on the samples. This work was supported by the US Department of Energy Great Lakes Bioenergy Research Center (grant no. DOE BER Office of Science DE-FC02-07ER64494). ML and JDC were supported in part by a grant from the US National Science Foundation (grant no. NSF CBET 1336622). David Hodge is grateful for support by a travel award from the US Department of Energy, Office of Science, Office of Basic Energy Sciences (BES) and the Office of Biological and Environmental Research (BER), DE-FOA-0000995. NR 73 TC 2 Z9 2 U1 4 U2 22 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4305 EP 4315 DI 10.1093/jxb/erv016 PG 11 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900017 PM 25871649 ER PT J AU Cass, CL Peraldi, A Dowd, PF Mottiar, Y Santoro, N Karlen, SD Bukhman, YV Foster, CE Thrower, N Bruno, LC Moskvin, OV Johnson, ET Willhoit, ME Phutane, M Ralph, J Mansfield, SD Nicholson, P Sedbrook, JC AF Cass, Cynthia L. Peraldi, Antoine Dowd, Patrick F. Mottiar, Yaseen Santoro, Nicholas Karlen, Steven D. Bukhman, Yury V. Foster, Cliff E. Thrower, Nick Bruno, Laura C. Moskvin, Oleg V. Johnson, Eric T. Willhoit, Megan E. Phutane, Megha Ralph, John Mansfield, Shawn D. Nicholson, Paul Sedbrook, John C. TI Effects of PHENYLALANINE AMMONIA LYASE (PAL) knockdown on cell wall composition, biomass digestibility, and biotic and abiotic stress responses in Brachypodium SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE Bioenergy; ferulic acid; Fusarium; grass; herbivory; lignin; phenylpropanoid; saccharification; tyrosine ammonia lyase; ultraviolet light ID CINNAMYL ALCOHOL-DEHYDROGENASE; FUSARIUM-GRAMINEARUM; ARABIDOPSIS-THALIANA; SACCHARIFICATION EFFICIENCY; SPODOPTERA-FRUGIPERDA; LIGNIN BIOSYNTHESIS; DISEASE RESISTANCE; ETHANOL-PRODUCTION; INSECT RESISTANCE; GENE-EXPRESSION AB The phenylpropanoid pathway in plants synthesizes a variety of structural and defence compounds, and is an important target in efforts to reduce cell wall lignin for improved biomass conversion to biofuels. Little is known concerning the trade-offs in grasses when perturbing the function of the first gene family in the pathway, PHENYLALANINE AMMONIA LYASE (PAL). Therefore, PAL isoforms in the model grass Brachypodium distachyon were targeted, by RNA interference (RNAi), and large reductions (up to 85%) in stem tissue transcript abundance for two of the eight putative BdPAL genes were identified. The cell walls of stems of BdPAL-knockdown plants had reductions of 43% in lignin and 57% in cell wall-bound ferulate, and a nearly 2-fold increase in the amounts of polysaccharide-derived carbohydrates released by thermochemical and hydrolytic enzymic partial digestion. PAL-knockdown plants exhibited delayed development and reduced root growth, along with increased susceptibilities to the fungal pathogens Fusarium culmorum and Magnaporthe oryzae. Surprisingly, these plants generally had wild-type (WT) resistances to caterpillar herbivory, drought, and ultraviolet light. RNA sequencing analyses revealed that the expression of genes associated with stress responses including ethylene biosynthesis and signalling were significantly altered in PAL knocked-down plants under non-challenging conditions. These data reveal that, although an attenuation of the phenylpropanoid pathway increases carbohydrate availability for biofuel, it can adversely affect plant growth and disease resistance to fungal pathogens. The data identify notable differences between the stress responses of these monocot pal mutants versus Arabidopsis (a dicot) pal mutants and provide insights into the challenges that may arise when deploying phenylpropanoid pathway-altered bioenergy crops. C1 [Cass, Cynthia L.; Willhoit, Megan E.; Phutane, Megha; Sedbrook, John C.] Illinois State Univ, Sch Biol Sci, Normal, IL 61790 USA. [Cass, Cynthia L.; Mottiar, Yaseen; Karlen, Steven D.; Bukhman, Yury V.; Moskvin, Oleg V.; Willhoit, Megan E.; Phutane, Megha; Ralph, John; Mansfield, Shawn D.; Sedbrook, John C.] US DOE, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Peraldi, Antoine; Bruno, Laura C.; Nicholson, Paul] John Innes Ctr, Dept Crop Genet, Norwich NR4 7UH, Norfolk, England. [Dowd, Patrick F.; Johnson, Eric T.] ARS, USDA, Natl Ctr Agr Utilizat Res, Crop Bioprotect Res Unit, Peoria, IL 61604 USA. [Mottiar, Yaseen; Mansfield, Shawn D.] Univ British Columbia, Dept Wood Sci, Vancouver, BC V6T 1Z4, Canada. [Santoro, Nicholas; Foster, Cliff E.; Thrower, Nick] Michigan State Univ, US Dept Energy, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Ralph, John] Univ Wisconsin, Wisconsin Energy Inst, Dept Biochem, Madison, WI 53706 USA. RP Sedbrook, JC (reprint author), Illinois State Univ, Sch Biol Sci, Normal, IL 61790 USA. EM jcsedbr@ilstu.edu FU US Department of Energy Great Lakes Bioenergy Research Center (Department of Energy, Biological and Environmental Research, Office of Science) [DE-FC02-07ER64494]; USDA Agricultural Research Service CRIS projects [3620-42000-041-00D] FX We thank Mark Doehring, David Lee, and Stephen Lutgen for technical assistance, and John Vogel for providing the BdPAL1 cDNA clone. We also thank Bruce Dien, Jim Webb, John Vogel, Craig Gatto, and Alejandro Rooney for valuable discussions. This work was supported by the US Department of Energy Great Lakes Bioenergy Research Center (Department of Energy, Biological and Environmental Research, Office of Science grant no. DE-FC02-07ER64494) and USDA Agricultural Research Service CRIS projects 3620-42000-041-00D. Mention of trade names or commercial products in this article is solely for the purpose of providing specific information and does not imply recommendation or endorsement by the US Department of Agriculture. USDA is an equal opportunity provider and employer. NR 95 TC 13 Z9 14 U1 7 U2 41 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4317 EP 4335 DI 10.1093/jxb/erv269 PG 19 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900018 PM 26093023 ER PT J AU Lara-Chavez, A Lowman, S Kim, S Tang, YH Zhang, JY Udvardi, M Nowak, J Flinn, B Mei, CS AF Lara-Chavez, Alejandra Lowman, Scott Kim, Seonhwa Tang, Yuhong Zhang, Jiyi Udvardi, Michael Nowak, Jerzy Flinn, Barry Mei, Chuansheng TI Global gene expression profiling of two switchgrass cultivars following inoculation with Burkholderia phytofirmans strain PsJN SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE Beneficial bacterial endophyte; Burkholderia phytofirmans strain PsJN; gene expression profiling; genotypic specificity; growth promotion; Panicum virgatum L. ID PANICUM VIRGATUM L.; VITIS-VINIFERA L.; RICE ORYZA-SATIVA; PLANT-GROWTH; ENDOPHYTIC COLONIZATION; TRANSCRIPTION FACTORS; SALICYLIC-ACID; ABIOTIC STRESS; BACTERIAL ENDOPHYTE; SIGNALING NETWORKS AB Improvement and year-to-year stabilization of biomass yields are primary objectives for the development of a low-input switchgrass feedstock production system using microbial endophytes. An earlier investigation of the effect of Burkholderia phytofirmans strain PsJN on switchgrass germplasm demonstrated differential responses between genotypes. PsJN inoculation of cv. Alamo (lowland ecotype) increased the plant root system, shoot length, and biomass yields, whereas it had no beneficial effect on cv. Cave-in-Rock (upland ecotype). To understand the gene networks governing plant growth promotion responses triggered by PsJN, the gene expression profiles were analysed in these two hosts, following seedling inoculation. The Affymetrix platform switchgrass expressed sequence tag (EST) microarray chip representing 122 972 probe sets, developed by the DOE BioEnergy Science Center, was employed to assess transcript abundance at 0.5, 2, 4, and 8 DAI (days after PsJN inoculation). Approximately 20 000 switchgrass probe sets showed significant responses in either cultivar. Switchgrass identifiers were used to map 19 421 genes in MapMan software. There were apparent differences in gene expression profiling between responsive and non-responsive cultivars after PsJN inoculation. Overall, there were 14 984 and 9691 genes affected by PsJN inoculation in Alamo and Cave-in-Rock, respectively. Of these, 394 are annotated as pathogenesis-related genes. In the responsive cv. Alamo, 68 pathogenesis-related genes were affected, compared with only 10 in the non-responsive cv. Cave-in-Rock. At the very early stage at 0.5 DAI, both cultivars exhibited similar recognition and defence responses, such as genes in signalling and proteolysis, after which the defence reaction in the responsive cv. Alamo became weaker while it was sustained in non-responsive cv. Cave-in-Rock. C1 [Lara-Chavez, Alejandra; Lowman, Scott; Kim, Seonhwa; Flinn, Barry; Mei, Chuansheng] Inst Adv Learning & Res, Inst Sustainable & Renewable Resources, Danville, VA 24540 USA. [Lowman, Scott; Nowak, Jerzy; Flinn, Barry; Mei, Chuansheng] Virginia Polytech Inst & State Univ, Dept Hort, Blacksburg, VA 24601 USA. [Flinn, Barry; Mei, Chuansheng] Virginia Polytech Inst & State Univ, Dept Forest Resources & Environm Conservat, Blacksburg, VA 24601 USA. [Tang, Yuhong; Zhang, Jiyi; Udvardi, Michael] Samuel Roberts Noble Fdn Inc, Div Plant Biol, Ardmore, OK 73401 USA. [Tang, Yuhong; Zhang, Jiyi; Udvardi, Michael] US DOE, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Mei, CS (reprint author), Inst Adv Learning & Res, Inst Sustainable & Renewable Resources, Danville, VA 24540 USA. EM chuansheng.mei@ialr.org FU Office of Science (BER), US Department of Energy for Plant Feedstock Genomics for Bioenergy Program [DE-SC0004951] FX This work was funded by the Office of Science (BER), US Department of Energy for Plant Feedstock Genomics for Bioenergy Program (DE-SC0004951). NR 85 TC 2 Z9 2 U1 7 U2 25 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2015 VL 66 IS 14 SI SI BP 4337 EP 4350 DI 10.1093/jxb/erv096 PG 14 WC Plant Sciences SC Plant Sciences GA CP2CU UT WOS:000359685900019 PM 25788737 ER PT J AU Du Frane, WL Stern, LA Constable, S Weitemeyer, KA Smith, MM Roberts, JJ AF Du Frane, Wyatt L. Stern, Laura A. Constable, Steven Weitemeyer, Karen A. Smith, Megan M. Roberts, Jeffery J. TI Electrical properties of methane hydrate plus sediment mixtures SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE gas hydrates; electrical conductivity; methane; ice; ionic impurities; controlled source electromagnetics ID GAS HYDRATE; POLYCRYSTALLINE OLIVINE; ELECTROMAGNETIC SURVEY; MARINE-SEDIMENTS; NATURAL-GAS; SEA-FLOOR; WATER; ICE; PERMEABILITY; TEMPERATURE AB Knowledge of the electrical properties of multicomponent systems with gas hydrate, sediments, and pore water is needed to help relate electromagnetic (EM) measurements to specific gas hydrate concentration and distribution patterns in nature. Toward this goal, we built a pressure cell capable of measuring in situ electrical properties of multicomponent systems such that the effects of individual components and mixing relations can be assessed. We first established the temperature-dependent electrical conductivity (sigma) of pure, single-phase methane hydrate to be similar to 5 orders of magnitude lower than seawater, a substantial contrast that can help differentiate hydrate deposits from significantly more conductive water-saturated sediments in EM field surveys. Here we report sigma measurements of two-component systems in which methane hydrate is mixed with variable amounts of quartz sand or glass beads. Sand by itself has low sigma but is found to increase the overall sigma of mixtures with well-connected methane hydrate. Alternatively, the overall sigma decreases when sand concentrations are high enough to cause gas hydrate to be poorly connected, indicating that hydrate grains provide the primary conduction path. Our measurements suggest that impurities from sand induce chemical interactions and/or doping effects that result in higher electrical conductivity with lower temperature dependence. These results can be used in the modeling of massive or two-phase gas-hydrate-bearing systems devoid of conductive pore water. Further experiments that include a free water phase are the necessary next steps toward developing complex models relevant to most natural systems. C1 [Du Frane, Wyatt L.; Smith, Megan M.; Roberts, Jeffery J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Stern, Laura A.] US Geol Survey, Menlo Pk, CA 94025 USA. [Constable, Steven; Weitemeyer, Karen A.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Weitemeyer, Karen A.] Univ Southampton, Natl Oceanog Ctr Southampton, Southampton, Hants, England. RP Du Frane, WL (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM Wyatt.DuFrane@asu.edu RI Constable, Steven/B-8959-2008 FU DOE [DE-NT0005668]; USGS Gas Hydrate Project [DE-NT0006147]; DOE's Methane Hydrate RD Program [DE-NT0006147]; [DE-AC52-07NA27344] FX The authors thank S. Roberts (LLNL) for assisting with ion chromatography measurements; W. Durham (MIT) for providing the OK#1 sand used in this study; J. Pinkston, S. Kirby, D. Lockner, W. Waite, and A. Hunt (U. S. Geological Survey) for their helpful discussions, advice, and reviews; and J. Lemire (Scripps Institution of Oceanography) for the help with the cell fabrication and design. Data supporting Figures 3-5 are available in the supporting information. Support for this work was provided by DOE contract DE-NT0005668 awarded to S. Constable (SIO) and Interagency Agreement DE-NT0006147 between the USGS Gas Hydrate Project and the DOE's Methane Hydrate R&D Program. Prepared by LLNL under contract DE-AC52-07NA27344. The use of trade, product, industry, or firm names in this report is for descriptive purposes only and does not constitute endorsement by the U. S. Geological Survey or the U. S. Government. NR 44 TC 1 Z9 1 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD JUL PY 2015 VL 120 IS 7 BP 4773 EP 4783 DI 10.1002/2015JB011940 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CP2ZN UT WOS:000359746700007 ER PT J AU Lei, QH Latham, JP Tsang, CF Xiang, JS Lang, P AF Lei, Qinghua Latham, John-Paul Tsang, Chin-Fu Xiang, Jiansheng Lang, Philipp TI A new approach to upscaling fracture network models while preserving geostatistical and geomechanical characteristics SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE Scaling; Fractures; Random walk; Geomechanical constraints; Permeability; Flow structure ID STRESS-DEPENDENT PERMEABILITY; SCALING RELATIONS; LENGTH DISTRIBUTION; CRYSTALLINE ROCKS; DEFORMATION BANDS; DISPLACEMENT; FAULTS; CONNECTIVITY; APERTURE; SYSTEMS AB A new approach to upscaling two-dimensional fracture network models is proposed for preserving geostatistical and geomechanical characteristics of a smaller-scale source fracture pattern. First, the scaling properties of an outcrop system are examined in terms of spatial organization, lengths, connectivity, and normal/shear displacements using fractal geometry and power law relations. The fracture pattern is observed to be nonfractal with the fractal dimension D approximate to 2, while its length distribution tends to follow a power law with the exponent 2 formaldehyde > acetaldehyde even though acetaldehyde yields were 10-fold greater than formaldehyde and acrolein. C1 [Corley, Richard A.; Kabilan, Senthil; Kuprat, Andrew P.; Jacob, Richard E.; Minard, Kevin R.; Teeguarden, Justin G.; Timchalk, Charles; Einstein, Daniel R.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Carson, James P.] Univ Texas Austin, Texas Adv Comp Ctr, Austin, TX 78758 USA. [Pipavath, Sudhakar] Univ Washington, Radiol, Seattle, WA 98195 USA. [Glenny, Robb] Univ Washington, Div Pulm & Crit Care Med, Seattle, WA 98195 USA. RP Corley, RA (reprint author), Pacific NW Natl Lab, Div Biol Sci, 902 Battelle Blvd,POB 999,MSIN J4-02, Richland, WA 99352 USA. EM rick.corley@pnnl.gov FU National Heart, Lung, and Blood Institute of the National Institutes of Health [R01 HL073598]; Reynolds Tobacco Co. [56296] FX National Heart, Lung, and Blood Institute of the National Institutes of Health (R01 HL073598). R.J. Reynolds Tobacco Co. under a separate contract with Battelle (Project 56296 to R.A.C., S.K., A.P.K., D.R.E., and C.T.) and published previously (Corley et al., 2012). NR 70 TC 5 Z9 5 U1 2 U2 11 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1096-6080 EI 1096-0929 J9 TOXICOL SCI JI Toxicol. Sci. PD JUL PY 2015 VL 146 IS 1 BP 65 EP 88 DI 10.1093/toxsci/kfv071 PG 24 WC Toxicology SC Toxicology GA CP1IH UT WOS:000359629000007 PM 25858911 ER PT J AU Tilton, SC Siddens, LK Krueger, SK Larkin, AJ Lohr, CV Williams, DE Baird, WM Waters, KM AF Tilton, Susan C. Siddens, Lisbeth K. Krueger, Sharon K. Larkin, Andrew J. Loehr, Christiane V. Williams, David E. Baird, William M. Waters, Katrina M. TI Mechanism-Based Classification of PAH Mixtures to Predict Carcinogenic Potential SO TOXICOLOGICAL SCIENCES LA English DT Article DE polycyclic aromatic hydrocarbons; toxicogenomics; modeling; skin cancer; mixtures ID POLYCYCLIC AROMATIC-HYDROCARBONS; GENE-EXPRESSION; COMPLEX-MIXTURES; MICROARRAY DATA; RISK-ASSESSMENT; C57BL/6 MICE; VARIANCE; MOUSE; TCDD; SKIN AB We have previously shown that relative potency factors and DNA adduct measurements are inadequate for predicting carcinogenicity of certain polycyclic aromatic hydrocarbons (PAHs) and PAH mixtures, particularly those that function through alternate pathways or exhibit greater promotional activity compared to benzo[a] pyrene (BaP). Therefore, we developed a pathway-based approach for classification of tumor outcome after dermal exposure to PAH/mixtures. FVB/N mice were exposed to dibenzo[def, p] chrysene (DBC), BaP, or environmental PAH mixtures (Mix 1-3) following a 2-stage initiation/promotion skin tumor protocol. Resulting tumor incidence could be categorized by carcinogenic potency as DBC>> BaP = Mix2 = Mix3> Mix1 = Control, based on statistical significance. Gene expression profiles measured in skin of mice collected 12h post-initiation were compared with tumor outcome for identification of short-term bioactivity profiles. A Bayesian integration model was utilized to identify biological pathways predictive of PAH carcinogenic potential during initiation. Integration of probability matrices from four enriched pathways (P<. 05) for DNA damage, apoptosis, response to chemical stimulus, and interferon gamma signaling resulted in the highest classification accuracy with leave-one-out cross validation. This pathway-driven approach was successfully utilized to distinguish early regulatory events during initiation prognostic for tumor outcome and provides proof-of-concept for using short-term initiation studies to classify carcinogenic potential of environmental PAH mixtures. These data further provide a 'source-to-outcome' model that could be used to predict PAH interactions during tumorigenesis and provide an example of how mode-of-action-based risk assessment could be employed for environmental PAH mixtures. C1 [Tilton, Susan C.; Siddens, Lisbeth K.; Krueger, Sharon K.; Larkin, Andrew J.; Williams, David E.; Baird, William M.; Waters, Katrina M.] Oregon State Univ, Superfund Res Ctr, Corvallis, OR 97331 USA. [Tilton, Susan C.; Siddens, Lisbeth K.; Larkin, Andrew J.; Williams, David E.; Baird, William M.] Oregon State Univ, Environm & Mol Toxicol Dept, Corvallis, OR 97331 USA. [Krueger, Sharon K.; Williams, David E.] Oregon State Univ, Linus Pauling Inst, Corvallis, OR 97331 USA. [Loehr, Christiane V.] Oregon State Univ, Coll Vet Med, Corvallis, OR 97331 USA. [Waters, Katrina M.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Tilton, SC (reprint author), Oregon State Univ, Environm & Mol Toxicol Dept, Corvallis, OR 97331 USA. EM susan.tilton@oregonstate.edu FU National Institute of Environmental Health Sciences [P42 ES016465]; ARRA Supplement to Promote Diversity in Health Research [P42 ES016465-S1, P01 CA90890] FX National Institute of Environmental Health Sciences grants P42 ES016465, ARRA Supplement to Promote Diversity in Health Research P42 ES016465-S1 and P01 CA90890. NR 25 TC 5 Z9 5 U1 1 U2 17 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1096-6080 EI 1096-0929 J9 TOXICOL SCI JI Toxicol. Sci. PD JUL PY 2015 VL 146 IS 1 BP 135 EP 145 DI 10.1093/toxsci/kfv080 PG 11 WC Toxicology SC Toxicology GA CP1IH UT WOS:000359629000012 PM 25908611 ER PT J AU Van Bonn, W LaPointe, A Gibbons, SM Frazier, A Hampton-Marcell, J Gilbert, J AF Van Bonn, William LaPointe, Allen Gibbons, Sean M. Frazier, Angel Hampton-Marcell, Jarrad Gilbert, Jack TI Aquarium microbiome response to ninety-percent system water change: Clues to microbiome management SO ZOO BIOLOGY LA English DT Article DE aquatic microbes; aquarium life support; veterinary; dysbiosis; fish health ID HYGIENE HYPOTHESIS; ENVIRONMENT AB The bacterial community composition and structure of water from an established teleost fish system was examined before, during and after a major water change to explore the impact of such a water-change disturbance on the stability of the aquarium water microbiome. The diversity and evenness of the bacterial community significantly increased following the 90% water replacement. While the change in bacterial community structure was significant, it was slight, and was also weakly correlated with changes in physicochemical parameters. Interestingly there was a significant shift in the correlative network relationships between operational taxonomic units from before to after the water replacement. We suggest this shift in network structure is due to the turnover of many taxa during the course of water replacement. These observations will inform future studies into manipulation of the microbiome by changing system environmental parameter values to optimize resident animal health. Zoo Biol. 34:360-367, 2015. (c) 2015 Wiley Periodicals Inc. C1 [Van Bonn, William; LaPointe, Allen] John G Shedd Aquarium, A Watson Armour III Ctr Anim Hlth & Welf, Chicago, IL 60605 USA. [Gibbons, Sean M.; Gilbert, Jack] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. [Gibbons, Sean M.; Frazier, Angel; Hampton-Marcell, Jarrad; Gilbert, Jack] Argonne Natl Lab, Biosci Div, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Hampton-Marcell, Jarrad; Gilbert, Jack] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gilbert, Jack] Univ Chicago, Dept Surg, Chicago, IL 60637 USA. [Gilbert, Jack] Marine Biol Lab, Woods Hole, MA 02543 USA. [Gilbert, Jack] Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310058, Zhejiang, Peoples R China. RP Van Bonn, W (reprint author), John G Shedd Aquarium, A Watson Armour III Ctr Anim Hlth & Welf, 1200 South Lake Shore Dr, Chicago, IL 60605 USA. EM bvanbonn@sheddaquarium.org FU EPA STAR Graduate Fellowship FX We are grateful to Mr. James Clark, aquarist responsible for study system, Ms. Caryn Svienty, Ms. Julie Nagler and Ms. Jennifer Bozych for water sample collection and processing. We thank Ms. Lei Zhao for assistance with statistical analyses. The authors confirm no conflict of interest involved in this work product. Sean Gibbons was supported by an EPA STAR Graduate Fellowship. NR 15 TC 0 Z9 0 U1 2 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0733-3188 EI 1098-2361 J9 ZOO BIOL JI Zoo Biol. PD JUL-AUG PY 2015 VL 34 IS 4 BP 360 EP 367 DI 10.1002/zoo.21220 PG 8 WC Veterinary Sciences; Zoology SC Veterinary Sciences; Zoology GA CO7SQ UT WOS:000359362500009 PM 26031788 ER PT J AU Uphoff, H AF Uphoff, Heidi TI Reading the Comments: Likers, Haters, and Manipulators at the Bottom of the Web SO LIBRARY JOURNAL LA English DT Book Review C1 [Uphoff, Heidi] Los Alamos Natl Lab, Los Alamos, NM USA. RP Uphoff, H (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. NR 1 TC 0 Z9 0 U1 1 U2 1 PU REED BUSINESS INFORMATION PI NEW YORK PA 360 PARK AVENUE SOUTH, NEW YORK, NY 10010 USA SN 0363-0277 J9 LIBR J JI Libr. J. PD JUL PY 2015 VL 140 IS 12 BP 109 EP 109 PG 1 WC Information Science & Library Science SC Information Science & Library Science GA CM7BJ UT WOS:000357845100273 ER PT J AU Li, JR Ross, SS Liu, Y Liu, YX Wang, KH Chen, HY Liu, FT Laurence, TA Liu, GY AF Li, Jie-Ren Ross, Shailise S. Liu, Yang Liu, Ying X. Wang, Kang-hsin Chen, Huan-Yuan Liu, Fu-Tong Laurence, Ted A. Liu, Gang-yu TI Engineered Nanostructures of Haptens Lead to Unexpected Formation of Membrane Nanotubes Connecting Rat Basophilic Leukemia Cells SO ACS NANO LA English DT Article DE membrane nanotubes; rat basophilic leukemia (RBL) cells; mast cells; atomic force microscopy (AFM); scanning electron microscopy (SEM); haptens; particle lithography ID FC-EPSILON-RI; ATOMIC-FORCE MICROSCOPY; ENDOTHELIAL PROGENITOR CELLS; MAST-CELLS; TUNNELING NANOTUBES; INTERCELLULAR TRANSPORTATION; PARTICLE LITHOGRAPHY; NEGATIVE REGULATION; ALLERGIC RESPONSES; LIPID-BILAYERS AB A recent finding reports that co-stimulation of the high-affinity immunoglobulin E (IgE) receptor (Fc epsilon RI) and the chemokine receptor 1 (CCR1) triggered formation of membrane nanotubes among bone-marrow-derived mast cells. The co-stimulation was attained using corresponding ligands: IgE binding antigen and macrophage inflammatory protein 1 alpha (MIP1 alpha), respectively. However, this approach failed to trigger formation of nanotubes among rat basophilic leukemia (RBL) cells due to the lack of CCR1 on the cell surface (Int. Immunol 2010,22 (2), 113-128). RBL cells are frequently used as a model for mast cells and are best known for antibody-mediated activation via Fc epsilon RI. This work reports the successful formation of membrane nanotubes among RBLs using only one stimulus, a hapten of 2,4-dinitrophenyl (DNP) molecules, which are presented as nanostructures with our designed spatial arrangements. This observation underlines the significance of the local presentation of ligands in the context of impacting the cellular signaling cascades. In the case of RBL, certain DNP nanostructures suppress antigen-induced degranulation and facilitate the rearrangement of the cytoskeleton to form nanotubes. These results demonstrate an important scientific concept; engineered nanostructures enable cellular signaling cascades, where current technologies encounter great difficulties. More importantly, nanotechnology offers a new platform to selectively activate and/or inhibit desired cellular signaling cascades. C1 [Li, Jie-Ren; Ross, Shailise S.; Liu, Yang; Liu, Ying X.; Wang, Kang-hsin; Liu, Gang-yu] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Chen, Huan-Yuan; Liu, Fu-Tong] Univ Calif Davis, Sch Med, Dept Dermatol, Sacramento, CA 95817 USA. [Chen, Huan-Yuan; Liu, Fu-Tong] Acad Sinica, Inst Biomed Sci, Taipei, Taiwan. [Laurence, Ted A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Liu, GY (reprint author), Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. EM gyliu@ucdavis.edu FU National Institutes of Health [1R21CA176850-01]; Gordon and Betty Moore Foundation; Alfred P. Sloan Foundation Minority Ph.D. Scholarship; UCD-LLNL Joint Graduate Mentorship Award FX We would like to thank Mr. Alan Hicklin at the UC Davis' Keck Spectral Imaging Facility for his technical assistance, and Ms. Susan Stagner for her help in the preparation of the manuscript. This work was supported by National Institutes of Health (1R21CA176850-01) and the Gordon and Betty Moore Foundation. S.S.R. is a recipient of the Alfred P. Sloan Foundation Minority Ph.D. Scholarship. Y.L. is supported by a UCD-LLNL Joint Graduate Mentorship Award. NR 78 TC 3 Z9 3 U1 9 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 6738 EP 6746 DI 10.1021/acsnano.5b02270 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200010 PM 26057701 ER PT J AU Brubaker, CE Velluto, D Demurtas, D Phelps, EA Hubbell, JA AF Brubaker, Carrie E. Velluto, Diana Demurtas, Davide Phelps, Edward A. Hubbell, Jeffrey A. TI Crystalline Oligo(ethylene sulfide) Domains Define Highly Stable Supramolecular Block Copolymer Assemblies SO ACS NANO LA English DT Article DE polymer; self-assembly; nanoparticle; micelle; cylindrical micelle; hydrogel ID POLY(PROPYLENE SULFIDE); POLY(ETHYLENE GLYCOL); IMAGE-ANALYSIS; MICELLES; POLYMERS; NANOPARTICLES; DELIVERY; CORE; MORPHOLOGIES; MICROSCOPY AB With proper control over copolymer design and solvation conditions, self-assembled materials display impressive morphological variety that encompasses nanoscale colloids as well as bulk three-dimensional architectures. Here we take advantage of both hydrophobicity and crystallinity to mediate supramolecular self-assembly of spherical micellar, linear fibrillar, or hydrogel structures by a family of highly asymmetric poly(ethylene glycol)-b-oligo(ethylene sulfide) (PEG-OES) copolymers. Assembly structural polymorphism was achieved with modification of PEG-OES topology (linear versus multiarm) and with precise, monomer-by-monomer control of DES length. Notably, all three morphologies were accessed utilizing OES oligomers with degrees of polymerization as short as three. These exceptionally small assembly forming blocks represent the first application of ethylene sulfide oligomers in supramolecular materials. While the assemblies demonstrated robust aqueous stability over time, oxidation by hydrogen peroxide progressively converted ethylene sulfide residues to increasingly hydrophilic and amorphous sulfoxides and sulfones, causing morphological changes and permanent disassembly. We utilized complementary microscopic and spectroscopic techniques to confirm this chemical stimulus-responsive behavior in self-assembled PEG-OES colloidal dispersions and physical gels. In addition to inherent stimulus-responsive behavior, fibrillar assemblies demonstrated biologically relevant molecular delivery, as confirmed by the dose-dependent activation of murine bone marrow-derived dendritic cells following fibril-mediated delivery of the immunological adjuvant monophosphoryl lipid A. In physical gels composed of either linear or multiarm PEG-DES precursors, rheologic analysis also identified mechanical stimuli-responsive shear thinning behavior. Thanks to the facile preparation, user-defined morphology, aqueous stability, carrier functionality, and stimuli-responsive behaviors of PEG-OES supramolecular assemblies, our findings support a future role for these materials as injectable or implantable biomaterials. C1 [Brubaker, Carrie E.; Velluto, Diana; Phelps, Edward A.; Hubbell, Jeffrey A.] Ecole Polytech Fed Lausanne, Sch Life Sci, Inst Bioengn, CH-1015 Lausanne, Switzerland. [Demurtas, Davide] Ecole Polytech Fed Lausanne, Sch Basic Sci, Interdisciplinary Ctr Electron Microscopy, CH-1015 Lausanne, Switzerland. [Hubbell, Jeffrey A.] Ecole Polytech Fed Lausanne, Sch Basic Sci, Inst Chem Sci & Engn, CH-1015 Lausanne, Switzerland. [Hubbell, Jeffrey A.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Hubbell, Jeffrey A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Hubbell, JA (reprint author), Ecole Polytech Fed Lausanne, Sch Life Sci, Inst Bioengn, CH-1015 Lausanne, Switzerland. EM jeffrey.hubbell@epfl.ch RI Phelps, Edward/Q-1302-2016 OI Phelps, Edward/0000-0001-8666-805X FU ERC; Whitaker Foundation/IIE FX This work was supported by ERC Advanced Grant Nanolmmune, under the Seventh Framework Programme (J.A.H) and by the Whitaker Foundation/IIE (C.E.B). We gratefully recognize F. Spiga for technical assistance with SPR acquisition, and F. Sordo and T. Nardi for rheometer access. 1H NMR spectroscopy was performed in the EPFL Institute of Chemical Sciences and Engineering. The EPFL Molecular and Hybrid Materials Characterization Center and J. Morisod are recognized for DSC access and training. Confocal microscopy was acquired in the EPFL BioImaging and Optics Platform. We thank C. Card and D. S. Wilson for editorial feedback during manuscript preparation. NR 49 TC 6 Z9 6 U1 11 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 6872 EP 6881 DI 10.1021/acsnano.5b02937 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200024 PM 26125494 ER PT J AU Voros, M Galli, G Zimanyi, GT AF Voeroes, Marton Galli, Giulia Zimanyi, Gergely T. TI Colloidal Nanoparticles for Intermediate Band Solar Cells SO ACS NANO LA English DT Article DE nanocrystal; nanoparticle solid; intermediate band; solar cell; density functional theory; doping; absorption ID CDSE QUANTUM DOTS; DENSITY-FUNCTIONAL THEORY; AB-INITIO CALCULATIONS; AUGMENTED-WAVE METHOD; SEMICONDUCTOR NANOCRYSTALS; CARRIER MULTIPLICATION; EDGE ENERGIES; THIN-FILMS; EFFICIENCY; CHARGE AB The Intermediate Band (IB) solar cell concept is a promising idea to transcend the Shockley-Queisser limit. Using the results of first-principles calculations, we propose that colloidal nanoparticles (CNPs) are a viable and efficient platform for the implementation of the IB solar cell concept. We focused on CdSe CNPs and we showed that intragap states present in the isolated CNPs with reconstructed surfaces combine to form an IB in arrays of CNPs, which is well separated from the valence and conduction band edges. We demonstrated that optical transitions to and from the IB are active. We also showed that the IB can be electron doped in a solution, e.g., by decamethylcobaltocene, thus activating an IB-induced absorption process. Our results, together with the recent report of a nearly 10% efficient CNP solar cell, indicate that colloidal nanoparticle intermediate band solar cells are a promising platform to overcome the Shockley-Queisser limit. C1 [Voeroes, Marton; Zimanyi, Gergely T.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Voeroes, Marton; Galli, Giulia] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Galli, Giulia] Argonne Natl Lab, Lemont, IL 60439 USA. RP Voros, M (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. EM vormar@gmail.com; gagalli@uchicago.edu; zimanyi@physics.ucdavis.edu OI Voros, Marton/0000-0003-1321-9207 FU NSF [DMR-1035468]; National Energy Research Scientific Computing Center (NERSC) through NISE; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center (EFRC) - US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) FX The authors thank A. Marti, A. Nozik, J. Krich, S. Hubbard, A. Freundlich, J. Skone, T. Szilvasi for useful discussions and N. Brawand for rendering the nanoparticle solid image. M.V. thanks A. Csuhai for inspiring discussions. This research was supported by the NSF Solar Collaborative under DMR-1035468. This research used resources of the National Energy Research Scientific Computing Center (NERSC) through the NISE project Larnint. NERSC is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors also acknowledge support from the Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center (EFRC) funded by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES). NR 96 TC 3 Z9 3 U1 9 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 6882 EP 6890 DI 10.1021/acsnano.5b00332 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200025 PM 26042468 ER PT J AU Johnson, PE Muttil, P MacKenzie, D Carnes, EC Pelowitz, J Mara, NA Mook, WM Jett, SD Dunphy, DR Timmins, GS Brinker, CJ AF Johnson, Patrick E. Muttil, Pavan MacKenzie, Debra Carnes, Eric C. Pelowitz, Jennifer Mara, Nathan A. Mook, William M. Jett, Stephen D. Dunphy, Darren R. Timmins, Graham S. Brinker, C. Jeffrey TI Spray-Dried Multiscale Nano-biocomposites Containing Living Cells SO ACS NANO LA English DT Article DE viable-but-not-culturable cells; biopreservation; bacterial persistence; cellular; encapsulation; sol-gel; spray drying; evaporation-induced self-assembly ID NONCULTURABLE STATE; DRUG-DELIVERY; PARTICLES; SILICA; BACTERIA; NANOPARTICLES; AEROSOL; PROTEIN; ATP; NANOINDENTATION AB Three-dimensional encapsulation of cells within nanostructured silica gels or matrices enables applications as diverse as biosensors, microbial fuel cells, artificial organs, and vaccines; it also allows the study of individual cell behaviors. Recent progress has improved the performance and flexibility of cellular encapsulation, yet there remains a need for robust scalable processes. Here, we report a spray-drying process enabling the large-scale production of functional nano-biocomposites (NBCs) containing living cells within ordered 3D lipid-silica nanostructures. The spray-drying process is demonstrated to work with multiple cell types and results in dry powders exhibiting a unique combination of properties including highly ordered 3D nanostructure, extended lipid fluidity, tunable macromorphologies and aerodynamic diameters, and unexpectedly high physical strength. Nanoindentation of the encasing nanostructure revealed a Young's modulus and hardness of 13 and 1.4 GPa, respectively. We hypothesized this high strength would prevent cell growth and force bacteria into viable but not culturable (VBNC) states. In concordance with the VBNC state, cellular ATP levels remained elevated even over eight months. However, their ability to undergo resuscitation and enter growth phase greatly decreased with time in the VBNC state. A quantitative method of determining resuscitation frequencies was developed and showed that, after 36 weeks in a NBC-induced VBNC, less than 1 in 10 000 cells underwent resuscitation. The NBC platform production of large quantities of VBNC cells is of interest for research in bacterial persistence and screening of drugs targeting such cells. NBCs may also enable long-term preservation of living cells for applications in cell-based sensing and the packaging and delivery of live-cell vaccines. C1 [Johnson, Patrick E.] Univ New Mexico, Dept Nanosci & Microsyst Engn, Ctr Microengineered Mat, Albuquerque, NM 87106 USA. [Muttil, Pavan; MacKenzie, Debra; Timmins, Graham S.] Univ New Mexico, Dept Pharmaceut Sci, Ctr Microengineered Mat, Albuquerque, NM 87106 USA. [Jett, Stephen D.] Univ New Mexico, Dept Cell Biol & Physiol, Ctr Microengineered Mat, Albuquerque, NM 87106 USA. [Johnson, Patrick E.; Dunphy, Darren R.; Brinker, C. Jeffrey] Univ New Mexico, Dept Chem & Biol Engn, Ctr Microengineered Mat, Albuquerque, NM 87106 USA. [Mara, Nathan A.; Mook, William M.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Mara, Nathan A.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Carnes, Eric C.; Pelowitz, Jennifer; Brinker, C. Jeffrey] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87185 USA. RP Timmins, GS (reprint author), Univ New Mexico, Dept Pharmaceut Sci, Ctr Microengineered Mat, Albuquerque, NM 87106 USA. EM gtimmins@salud.unm.edu; cjbrink@sandia.gov RI Mara, Nathan/J-4509-2014 FU University of New Mexico; Cancer Center Fluorescence Microscopy Shared Resource; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Sandia National Laboratory LDRD program; NSF IGERT program; Air Force Office of Scientific Research [FA9550-14-1-0066]; U.S. Department of Energy [DE-AC52-06NA25396]; NIH/NIAID [AI081015, 081090] FX We would like to thank Y. B. Jiang for help with TEM sample preparation. Fluorescence images in this paper were generated in the University of New Mexico & Cancer Center Fluorescence Microscopy Shared Resource funded as detailed at http://hsc.unm.edu/crtc/microscopy/acknowledgements.html. C.J.B. and E.C. acknowledge support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, and the Sandia National Laboratory LDRD program. P.E.J. and J.P. acknowledge support from the NSF IGERT program and the Air Force Office of Scientific Research under grant no. FA9550-14-1-0066. Nanoindentation studies were performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. G.S.T. acknowledges support from NIH/NIAID AI081015 and 081090. C.J.B. and E.C.C. acknowledge support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division for support of self-assembly of lipid-silica nanocomposites, and the Sandia National Laboratory LDRD program for support of studies of cellular function. We thank Patrick Fleig for preparing the aerosol samples shown in Supplemental Figure 2. TEM Data were generated in the UNM Electron Microscopy Shared Facility supported by the University of New Mexico Health Sciences Center and the University of New Mexico Cancer Center. NR 66 TC 6 Z9 6 U1 11 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 6961 EP 6977 DI 10.1021/acsnano.5b01139 PG 17 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200033 PM 26083188 ER PT J AU Zhang, JB Chernomordik, BD Crisp, RW Kroupa, DM Luther, JM Miller, EM Gao, JB Beard, MC AF Zhang, Jianbing Chernomordik, Boris D. Crisp, Ryan W. Kroupa, Daniel M. Luther, Joseph M. Miller, Elisa M. Gao, Jianbo Beard, Matthew C. TI Preparation of Cd/Pb Chalcogenide Heterostructured Janus Particles via Controllable Cation Exchange SO ACS NANO LA English DT Article DE quantum dots; heterostructures; cation-exchange reactions; synthesis; lead chalcogenide ID DOT SOLAR-CELLS; QUANTUM DOTS; CORE/SHELL NANOCRYSTALS; COLLOIDAL NANOCRYSTALS; SULFIDE NANOCRYSTALS; INFRARED-EMISSION; ION-EXCHANGE; II-VI; PBSE; NANORODS AB We developed a strategy for producing quasi-spherical nanocrystals of anisotropic heterostructures of Cd/Pb chalcogenides. The nanostructures are fabricated via a controlled cation exchange reaction where the Cd2+ cation is exchanged for the Pb2+ cation. The cation exchange reaction is thermally activated and can be controlled by adjusting the reaction temperature or time. We characterized the particles using TEM, XPS, PL, and absorption spectroscopy. With complete exchange, high quality Pb-chalcogenide quantum dots are produced. In addition to Cd2+, we also find suitable conditions for the exchange of Zn2+ cations for Pb2+ cations. The cation exchange is anisotropic starting at one edge of the nanocrystals and proceeds along the (111) direction producing a sharp interface at a (111) crystallographic plane. Instead of spherical core/shell structures, we produced and studied quasi-spherical CdS/PbS and CdSe/PbSe Janus-type heterostructures. Nontrivial PL behavior was observed from the CdS(e)/PbS(e) heterostructures as the Pb:Cd ratio is increased. C1 [Zhang, Jianbing] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Hubei, Peoples R China. [Zhang, Jianbing; Chernomordik, Boris D.; Crisp, Ryan W.; Kroupa, Daniel M.; Luther, Joseph M.; Miller, Elisa M.; Beard, Matthew C.] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Crisp, Ryan W.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Kroupa, Daniel M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Gao, Jianbo] Los Alamos Natl Lab, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. RP Beard, MC (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. EM matt.beard@nrel.gov OI BEARD, MATTHEW/0000-0002-2711-1355 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences; DOE [DE-AC36-08G028308]; National Natural Science Foundation of China [51302096]; Fundamental Research Funds of Wuhan City [2013060501010163]; NREL Director's Postdoctoral Fellowship FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences. J.M.L, J.G., B.D.C. J.Z., and M.C.B acknowledge the Energy Frontier Research Centers program within the Center for Advanced Solar Photophysics, D.M.K. acknowledges support from the solar photochemistry program. DOE funding was provided to NREL through contract DE-AC36-08G028308. E.M.M. was supported an NREL Director's Postdoctoral Fellowship. J.Z. acknowledges partial support of the National Natural Science Foundation of China (No. 51302096) and the Fundamental Research Funds of Wuhan City (No. 2013060501010163). NR 52 TC 13 Z9 13 U1 23 U2 83 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 7151 EP 7163 DI 10.1021/acsnano.5b01859 PG 13 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200052 PM 26161785 ER PT J AU Agar, JC Damodaran, AR Velarde, GA Pandya, S Mangalam, RVK Martin, LW AF Agar, Joshua C. Damodaran, Anoop R. Velarde, Gabriel A. Pandya, Shishir Mangalam, R. V. K. Martin, Lane W. TI Complex Evolution of Built-in Potential in Compositionally-Graded PbZr1-xTixO3 Thin Films SO ACS NANO LA English DT Article DE ferroelectrics; PbZr1-xTixO3; thin films; compositionally-graded heterostructures; permittivity ID MISFIT RELAXATION MECHANISMS; ZIRCONATE-TITANATE CERAMICS; FERROELECTRIC PROPERTIES; DOMAIN CONFIGURATIONS; ELECTRIC POLARIZATION; FLEXOELECTRICITY; BEHAVIOR; ENERGY; PIEZOELECTRICITY; NANOGENERATORS AB Epitaxial strain has been widely used to tune crystal and domain structures in ferroelectric thin films. New avenues of strain engineering based on varying the composition at the nanometer scale have been shown to generate symmetry breaking and large strain gradients culminating in large built-in potentials. In this work, we develop routes to deterministically control these builtin potentials by exploiting the interplay between strain gradients, strain accommodation, and domain formation in compositionally graded PbZr1-xTi3O3 heterostructures. We demonstrate that variations in the nature of the compositional gradient and heterostructure thickness can be used to control both the crystal and domain structures and give rise to nonintuitive evolution of the built-in potential, which does not scale directly with the magnitude of the strain gradient as would be expected. Instead, large built-in potentials are observed in compositionally-graded heterostructures that contain (1) compositional gradients that traverse chemistries associated with structural phase boundaries (such as the morphotropic phase boundary) and (2) ferroelastic domain structures. In turn, the built-in potential is observed to be dependent on a combination of flexoelectric effects (i.e., polarization strain gradient coupling), chemical-gradient effects (i.e., polarization chemical potential gradient coupling), and local inhomogeneities (in structure or chemistry) that enhance strain (and/or chemical potential) gradients such as areas with nonlinear lattice parameter variation with chemistry or near ferroelastic domain boundaries. Regardless of origin, large built-in potentials act to suppress the dielectric permittivity, while having minimal impact on the magnitude of the polarization, which is important for the optimization of these materials for a range of nanoapplications from vibrational energy harvesting to thermal energy conversion and beyond. C1 [Agar, Joshua C.; Damodaran, Anoop R.; Pandya, Shishir; Mangalam, R. V. K.; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Agar, Joshua C.; Velarde, Gabriel A.; Martin, Lane W.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Martin, LW (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM lwmartin@berkeley.edu RI Martin, Lane/H-2409-2011 OI Martin, Lane/0000-0003-1889-2513 FU National Science Foundation [DMR-1451219, ENG-1434147]; Army Research Office [W911NF-14-1-0104] FX J.C.A. and L.W.M. acknowledge support from the National Science Foundation under grant number DMR-1451219. A.R.D. and S.P. acknowledge the support of the Army Research Office under grant number W911NF-14-1-0104. R.V.K.M: acknowledges support from the National Science Foundation under grant ENG-1434147. NR 67 TC 9 Z9 9 U1 6 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 7332 EP 7342 DI 10.1021/acsnano.5b02289 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200070 PM 26125636 ER PT J AU Sun, XH Jiang, KZ Zhang, N Guo, SJ Huang, XQ AF Sun, Xiuhui Jiang, Kezhu Zhang, Nan Guo, Shaojun Huang, Xiaoqing TI Crystalline Control of {111} Bounded Pt3Cu Nanocrystals: Multiply-Twinned Pt3Cu Icosahedra with Enhanced Electrocatalytic Properties SO ACS NANO LA English DT Article DE Platinum; copper; icosahedron; twin defect; electrocatalyst ID OXYGEN REDUCTION REACTION; ALLOY NANOPARTICLES; DEFECT CHEMISTRY; SOLID-STATE; METAL; PD; EVOLUTION; CATALYSIS; TRANSPORT; NANOCUBES AB Despite that different facets have distinct catalytic behavior, the important role of twin defects on enhancing the catalytic performance of metallic nanocrystals is largely unrevealed. The key challenge in demonstrating the importance of twin defects for catalysis is the extreme difficulties in creating nanostructures with the same exposed facets but tunable twin defects that are suitable for catalytic investigations. Herein, we show an efficient synthetic strategy to selectively synthesize {111}-terminated Pt3Cu nanocrystals with controllable crystalline features. Two distinct {111}-bounded shapes, namely, multiply-twinned Pt3Cu icosahedra and single-crystalline Pt3Cu octahedra, are successfully prepared by simply changing the types of Cu precursors with the other growth parameters unchanged. Electrocatalytic studies show that the {111}-terminated Pt3Cu nanocrystals exhibit the very interesting crystalline nature-dependent electrocatalytic activities toward both the oxygen reduction reaction (ORR) and methanol oxidation reaction (MOR) with multiply-twinned Pt3Cu icosahedra demonstrating enhanced electrocatalytic activities compared to the single-crystalline Pt3Cu octahedra due to their additional yet important effect of twin defect. As a result, under the multiple tuning conditions (alloy, shape, and twin effects), the multiply-twinned Pt3Cu icosahedra exhibit much enhanced electrocatalytic activities in both ORR and MOR with respect to the Pt black. The present work highlights the importance of twin defects in enhancing electrocatalytic activities of metallic nanocrystals. C1 [Sun, Xiuhui; Jiang, Kezhu; Zhang, Nan; Huang, Xiaoqing] Soochow Univ, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Jiangsu, Peoples R China. [Guo, Shaojun] Los Alamos Natl Lab, Phys Chem & Appl Spect, Los Alamos, NM 87545 USA. RP Guo, SJ (reprint author), Los Alamos Natl Lab, Phys Chem & Appl Spect, POB 1663, Los Alamos, NM 87545 USA. EM shaojun.guo.nano@gmail.com; hxq006@suda.edu.cn RI Guo, Shaojun/A-8449-2011 OI Guo, Shaojun/0000-0002-5941-414X FU Soochow University; Young Thousand Talented Program FX This work was financially supported by the start-up funding from Soochow University and Young Thousand Talented Program. NR 43 TC 28 Z9 28 U1 34 U2 164 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2015 VL 9 IS 7 BP 7634 EP 7640 DI 10.1021/acsnano.5b02986 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CO0EP UT WOS:000358823200100 PM 26172056 ER PT J AU Bi, S He, ZR Chen, JH Li, DW AF Bi, Sheng He, Zhengran Chen, Jihua Li, Dawen TI Solution-grown small-molecule organic semiconductor with enhanced crystal alignment and areal coverage for organic thin film transistors SO AIP ADVANCES LA English DT Article ID FIELD-EFFECT TRANSISTORS; HIGH-PERFORMANCE; SINGLE-CRYSTALS; PHOTOPHYSICAL PROPERTIES; CONJUGATED POLYMERS; SOLAR-CELLS; DIKETOPYRROLOPYRROLE; PENTACENE; MOBILITY; PHOTOVOLTAICS AB Drop casting of small-molecule organic semiconductors typically forms crystals with random orientation and poor areal coverage, which leads to significant performance variations of organic thin-film transistors (OTFTs). In this study, we utilize the controlled evaporative self-assembly (CESA) method combined with binary solvent system to control the crystal growth. A small-molecule organic semiconductor, 2,5-Di-(2-ethylhexyl)-3,6-bis(5 ''-n-hexyl-2,2',5',2 '']terthiophen-5-yl)-pyrrolo[3,4-c]pyrrole-1,4-dione (SMDPPEH), is used as an example to demonstrate the effectiveness of our approach. By optimizing the double solvent ratios, well-aligned SMDPPEH crystals with significantly improved areal coverage were achieved. As a result, the SMDPPEH based OTFTs exhibit a mobility of 1.6 x 10(-2) cm(2)/Vs, which is the highest mobility from SMDPPEH ever reported. (C) 2015 Author(s). C1 [Bi, Sheng; He, Zhengran; Li, Dawen] Univ Alabama, Dept Elect & Comp Engn, Ctr Mat Informat Technol, Tuscaloosa, AL 35487 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Li, DW (reprint author), Univ Alabama, Dept Elect & Comp Engn, Ctr Mat Informat Technol, Tuscaloosa, AL 35487 USA. EM dawenl@eng.ua.edu RI Chen, Jihua/F-1417-2011; He, Zhengran/A-9898-2017 OI Chen, Jihua/0000-0001-6879-5936; FU National Science Foundation [ECCS-1151140]; University of Alabama FX This work was supported by National Science Foundation (ECCS-1151140) and Research Stimulation Program at The University of Alabama. A portion of experimental design and analysis was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 38 TC 3 Z9 3 U1 3 U2 33 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2015 VL 5 IS 7 AR 077170 DI 10.1063/1.4927577 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CO1NQ UT WOS:000358922500070 ER PT J AU Kim, JS Kim, SY Kim, DH Ott, RT Kim, HG Lee, MH AF Kim, J. S. Kim, S. Y. Kim, D. H. Ott, R. T. Kim, H. G. Lee, M. H. TI Effect of hydrothermal condition on the formation of multi-component oxides of Ni-based metallic glass under high temperature water near the critical point SO AIP ADVANCES LA English DT Article ID SUPERCRITICAL WATER; SURFACE-AREA; NANOPARTICLES; CRYSTALLIZATION; COMPOSITES AB The specific feature of multi-component oxides synthesized by hydrothermal process under high temperature (633 K) and highly pressurized water (18.9 MPa) near critical point. Effects of hydrothermal processing duration times 24 hours and 72 hours, respectively, on the oxide formation of the Ni59Zr20Ti16Si2Sn3 metallic glass synthesized by powder metallurgy process were characterized by X-ray diffractometer, differential scanning calorimeter along with the particle size, morphology and crystalline phase of the oxides. The crystallization of the needle-shape NiTiO3, ZrTiO4 and ZrSnO4 ternary oxide phases observed on the surface of metallic glass at below glass transition temperature and the morphology of oxide phases changed to plate-shape around 2 mu m in diameter by the increase processing time. This hydrothermal processing in subcritical water provides accelerated dense metal oxide crystals due to the reaction medium being at higher pressure than conventional oxidation processing. (C) 2015 Author(s). C1 [Kim, J. S.; Lee, M. H.] Iljin Global Co Ltd, Headquarters Bearing Div, Seoul 135875, South Korea. [Kim, S. Y.] Korea Inst Ind Technol, Rare Met R&D Grp, Inchon 406840, South Korea. [Kim, D. H.] Yonsei Univ, Ctr Noncrystalline Mat, Seoul 120749, South Korea. [Ott, R. T.] US DOE, Div Mat & Engn, Ames Lab, Ames, IA 50011 USA. [Kim, H. G.] Korea Atom Energy Inst, LWR Fuel Technol Div, Taejon 305600, South Korea. RP Lee, MH (reprint author), Iljin Global Co Ltd, Headquarters Bearing Div, Seoul 135875, South Korea. EM mhlee1@kitech.re.kr OI KIM, SONGYi/0000-0001-5185-2279; LEE, MIN HA/0000-0001-6006-0628 FU Industrial Technology Innovation Program - Ministry of Trade, Industry and Energy (MOTIE); Korea Institute of Technology Evaluation and Planning (KETEP) FX This work was supported by the Industrial Technology Innovation Program funded by the Ministry of Trade, Industry and Energy (MOTIE) and Korea Institute of Technology Evaluation and Planning (KETEP). NR 14 TC 1 Z9 1 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2015 VL 5 IS 7 AR 077132 DI 10.1063/1.4926972 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CO1NQ UT WOS:000358922500032 ER PT J AU Li, Y Xu, B Hu, SY Li, YL Li, QL Liu, W AF Li, Yi Xu, Ben Hu, Shenyang Li, Yulan Li, Qiulin Liu, Wei TI Simulation of magnetic hysteresis loops and magnetic Barkhausen noise of alpha-iron containing nonmagnetic particles SO AIP ADVANCES LA English DT Article ID PRESSURE-VESSEL STEELS; MONTE-CARLO-SIMULATION; FERROMAGNETIC MATERIALS; RADIATION-DAMAGE; RPV STEELS; IRRADIATION; EMBRITTLEMENT; PARAMETERS; CLUSTERS; MODEL AB The magnetic hysteresis loops and Barkhausen noise of a single alpha-iron with nonmagnetic particles are simulated to investigate into the magnetic hardening due to Cu-rich precipitates in irradiated reactor pressure vessel (RPV) steels. Phase field method basing Landau-Lifshitz-Gilbert (LLG) equation is used for this simulation. The results show that the presence of the nonmagnetic particle could result in magnetic hardening by making the nucleation of reversed domains difficult. The coercive field is found to increase, while the intensity of Barkhausen noise voltage is decreased when the nonmagnetic particle is introduced. Simulations demonstrate the impact of nucleation field of reversed domains on the magnetization reversal behavior and the magnetic properties. (C) 2015 Author(s). C1 [Li, Yi; Xu, Ben; Li, Qiulin; Liu, Wei] Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China. [Li, Yi; Li, Qiulin; Liu, Wei] Tsinghua Univ, Grad Sch Shenzhen, Shenzhen 518055, Peoples R China. [Hu, Shenyang; Li, Yulan] Pacific NW Natl Lab, Energy Mat Div, Richland, WA 99352 USA. RP Liu, W (reprint author), Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China. EM liuw@mail.tsinghua.edu.cn NR 28 TC 1 Z9 1 U1 8 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2015 VL 5 IS 7 AR 077168 DI 10.1063/1.4927548 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CO1NQ UT WOS:000358922500068 ER PT J AU Smartt, SJ Valenti, S Fraser, M Inserra, C Young, DR Sullivan, M Pastorello, A Benetti, S Gal-Yam, A Knapic, C Molinaro, M Smareglia, R Smith, KW Taubenberger, S Yaron, O Anderson, JP Ashall, C Balland, C Baltay, C Barbarino, C Bauer, FE Baumont, S Bersier, D Blagorodnova, N Bongard, S Botticella, MT Bufano, F Bulla, M Cappellaro, E Campbell, H Cellier-Holzem, F Chen, TW Childress, MJ Clocchiatti, A Contreras, C Dall'Ora, M Danziger, J de Jaeger, T De Cia, A Della Valle, M Dennefeld, M Elias-Rosa, N Elman, N Feindt, U Fleury, M Gall, E Gonzalez-Gaitan, S Galbany, L Garoffolo, AM Greggio, L Guillou, LL Hachinger, S Hadjiyska, E Hage, PE Hillebrandt, W Hodgkin, S Hsiao, EY James, PA Jerkstrand, A Kangas, T Kankare, E Kotak, R Kromer, M Kuncarayakti, H Leloudas, G Lundqvist, P Lyman, JD Hook, IM Maguire, K Manulis, I Margheim, SJ Mattila, S Maund, JR Mazzali, PA McCrum, M McKinnon, R Moreno-Raya, ME Nicholl, M Nugent, P Pain, R Pignata, G Phillips, MM Polshaw, J Pumo, ML Rabinowitz, D Reilly, E Romero-Canizales, C Scalzo, R Schmidt, B Schulze, S Sim, S Sollerman, J Taddia, F Tartaglia, L Terreran, G Tomasella, L Turatto, M Walker, E Walton, NA Wyrzykowski, L Yuan, F Zampieri, L AF Smartt, S. J. Valenti, S. Fraser, M. Inserra, C. Young, D. R. Sullivan, M. Pastorello, A. Benetti, S. Gal-Yam, A. Knapic, C. Molinaro, M. Smareglia, R. Smith, K. W. Taubenberger, S. Yaron, O. Anderson, J. P. Ashall, C. Balland, C. Baltay, C. Barbarino, C. Bauer, F. E. Baumont, S. Bersier, D. Blagorodnova, N. Bongard, S. Botticella, M. T. Bufano, F. Bulla, M. Cappellaro, E. Campbell, H. Cellier-Holzem, F. Chen, T. -W. Childress, M. J. Clocchiatti, A. Contreras, C. Dall'Ora, M. Danziger, J. de Jaeger, T. De Cia, A. Della Valle, M. Dennefeld, M. Elias-Rosa, N. Elman, N. Feindt, U. Fleury, M. Gall, E. Gonzalez-Gaitan, S. Galbany, L. Morales Garoffolo, A. Greggio, L. Guillou, L. L. Hachinger, S. Hadjiyska, E. Hage, P. E. Hillebrandt, W. Hodgkin, S. Hsiao, E. Y. James, P. A. Jerkstrand, A. Kangas, T. Kankare, E. Kotak, R. Kromer, M. Kuncarayakti, H. Leloudas, G. Lundqvist, P. Lyman, J. D. Hook, I. M. Maguire, K. Manulis, I. Margheim, S. J. Mattila, S. Maund, J. R. Mazzali, P. A. McCrum, M. McKinnon, R. Moreno-Raya, M. E. Nicholl, M. Nugent, P. Pain, R. Pignata, G. Phillips, M. M. Polshaw, J. Pumo, M. L. Rabinowitz, D. Reilly, E. Romero-Canizales, C. Scalzo, R. Schmidt, B. Schulze, S. Sim, S. Sollerman, J. Taddia, F. Tartaglia, L. Terreran, G. Tomasella, L. Turatto, M. Walker, E. Walton, N. A. Wyrzykowski, L. Yuan, F. Zampieri, L. TI PESSTO: survey description and products from the first data release by the Public ESO Spectroscopic Survey of Transient Objects SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE instrumentation: spectrographs; methods: data analysis; techniques: spectroscopic; surveys; supernovae: general ID OBSERVATORY SUPERNOVA SEARCH; DIGITAL SKY SURVEY; PAN-STARRS 1; CORE-COLLAPSE; IA SUPERNOVAE; ULTRALUMINOUS SUPERNOVAE; SUPERLUMINOUS SUPERNOVAE; IC SUPERNOVAE; MASSIVE STAR; NO EVIDENCE AB Context. The Public European Southern Observatory Spectroscopic Survey of Transient Objects (PESSTO) began as a public spectroscopic survey in April 2012. PESSTO classifies transients from publicly available sources and wide-field surveys, and selects science targets for detailed spectroscopic and photometric follow-up. PESSTO runs for nine months of the year, January - April and August - December inclusive, and typically has allocations of 10 nights per month. Aims. We describe the data reduction strategy and data products that are publicly available through the ESO archive as the Spectroscopic Survey data release 1 (SSDR1). Methods. PESSTO uses the New Technology Telescope with the instruments EFOSC2 and SOFI to provide optical and NIR spectroscopy and imaging. We target supernovae and optical transients brighter than 20.5(m) for classification. Science targets are selected for follow-up based on the PESSTO science goal of extending knowledge of the extremes of the supernova population. We use standard EFOSC2 set-ups providing spectra with resolutions of 13-18 angstrom between 3345-9995 angstrom. A subset of the brighter science targets are selected for SOFI spectroscopy with the blue and red grisms (0.935-2.53 mu m and resolutions 23-33 angstrom) and imaging with broadband JHK(s) filters. Results. This first data release (SSDR1) contains flux calibrated spectra from the first year (April 2012-2013). A total of 221 confirmed supernovae were classified, and we released calibrated optical spectra and classifications publicly within 24 h of the data being taken (via WISeREP). The data in SSDR1 replace those released spectra. They have more reliable and quantifiable flux calibrations, correction for telluric absorption, and are made available in standard ESO Phase 3 formats. We estimate the absolute accuracy of the flux calibrations for EFOSC2 across the whole survey in SSDR1 to be typically similar to 15%, although a number of spectra will have less reliable absolute flux calibration because of weather and slit losses. Acquisition images for each spectrum are available which, in principle, can allow the user to refine the absolute flux calibration. The standard NIR reduction process does not produce high accuracy absolute spectrophotometry but synthetic photometry with accompanying JHK(s) imaging can improve this. Whenever possible, reduced SOFI images are provided to allow this. Conclusions. Future data releases will focus on improving the automated flux calibration of the data products. The rapid turnaround between discovery and classification and access to reliable pipeline processed data products has allowed early science papers in the first few months of the survey. C1 [Smartt, S. J.; Inserra, C.; Young, D. R.; Smith, K. W.; Bulla, M.; Chen, T. -W.; Gall, E.; Jerkstrand, A.; Kankare, E.; Kotak, R.; Maund, J. R.; McCrum, M.; Nicholl, M.; Polshaw, J.; Reilly, E.; Sim, S.; Terreran, G.] Queens Univ Belfast, Sch Math & Phys, Astrophys Res Ctr, Belfast BT7 1NN, Antrim, North Ireland. [Valenti, S.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Fraser, M.; Blagorodnova, N.; Campbell, H.; Hodgkin, S.; Walton, N. A.; Wyrzykowski, L.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Fraser, M.; Blagorodnova, N.; Campbell, H.; Hodgkin, S.; Walton, N. A.; Wyrzykowski, L.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Sullivan, M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Pastorello, A.; Benetti, S.; Cappellaro, E.; Elias-Rosa, N.; Greggio, L.; Hachinger, S.; Pumo, M. L.; Tartaglia, L.; Terreran, G.; Tomasella, L.; Turatto, M.; Zampieri, L.] INAF Osservatorio Astron Padova, I-35122 Padua, Italy. [Gal-Yam, A.; Yaron, O.; De Cia, A.; Leloudas, G.; Manulis, I.] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Knapic, C.; Molinaro, M.; Smareglia, R.; Danziger, J.] INAF Osservatorio Astron Trieste, I-34143 Trieste, Italy. 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EM s.smartt@qub.ac.uk RI Jerkstrand, Anders/K-9648-2015; Galbany, Lluis/A-8963-2017; Elias-Rosa, Nancy/D-3759-2014; OI Sullivan, Mark/0000-0001-9053-4820; Dall'Ora, Massimo/0000-0001-8209-0449; James, Philip/0000-0003-4131-5183; Schulze, Steve/0000-0001-6797-1889; Cappellaro, Enrico/0000-0001-5008-8619; Turatto, Massimo/0000-0002-9719-3157; Jerkstrand, Anders/0000-0001-8005-4030; Galbany, Lluis/0000-0002-1296-6887; Elias-Rosa, Nancy/0000-0002-1381-9125; Knapic, Cristina/0000-0002-4752-6777; Greggio, Laura/0000-0003-2634-4875; Molinaro, Marco/0000-0001-5028-6041; Benetti, Stefano/0000-0002-3256-0016; Smareglia, Riccardo/0000-0001-9363-3007; lina, tomasella/0000-0002-3697-2616; Zampieri, Luca/0000-0002-6516-1329; Sollerman, Jesper/0000-0003-1546-6615; Chen, Ting-Wan/0000-0002-1066-6098; Maund, Justyn/0000-0003-0733-7215; Della Valle, Massimo/0000-0003-3142-5020; Schmidt, Brian/0000-0001-6589-1287; Inserra, Cosimo/0000-0002-3968-4409; Fraser, Morgan/0000-0003-2191-1674; Scalzo, Richard/0000-0003-3740-1214; Kotak, Rubina/0000-0001-5455-3653 FU European Organisation for Astronomical Research in the Southern Hemisphere, Chile as part of PESSTO, (the Public ESO Spectroscopic Survey for Transient Objects Survey) ESO programme [188.D-3003, 191.D-0935.]; European Research Council under the European Union [291222]; STFC [ST/I001123/1, ST/L000709/1]; Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO) [CE110001020]; Royal Society; EU/FP7-ERC [615929, 307260]; European Union FP7 programme through ERC [320360]; PRIN-INAF; project Transient Universe: from ESO Large; CONICYT-Chile; Basal-CATA [PFB-06/2007]; FONDECYT [1141218, 3140534]; PCCI [130074]; ALMA-CONICYT [31100004]; "EMBIGGEN" Anillo [ACT1101]; Millennium Institute of Astrophysics (MAS) of the Iniciativa Cientifica Milenio del Ministerio de Economia, Fomento y Turismo [IC120009]; Quantum Universe' I-Core programme by the Israeli Committee for planning and budgeting; ISF; Weizmann-UK; Kimmel award; European Union [267251]; Ministry of Economy, Development, and Tourisms Millennium Science Initiative [IC12009]; CONICYT through FONDECYT [3130680, 3140563, 3140566] FX This work is based on observations collected at the European Organisation for Astronomical Research in the Southern Hemisphere, Chile as part of PESSTO, (the Public ESO Spectroscopic Survey for Transient Objects Survey) ESO programme 188.D-3003, 191.D-0935. Research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement No. [291222] (PI : S. J. Smartt) and STFC grants ST/I001123/1 and ST/L000709/1. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. M.J.C. acknowledges funding from the Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO), through project number CE110001020 MS acknowledges support from the Royal Society and EU/FP7-ERC grant No. [615929]. MF acknowledges support by the European Union FP7 programme through ERC grant number 320360. S.B., E.C., A.P., L.T. and M.T. are partially supported by the PRIN-INAF 2011 with the project Transient Universe: from ESO Large to PESSTO. We acknowledge CONICYT-Chile grants, Basal-CATA PFB-06/2007 (FEB), FONDECYT 1141218 (FEB) and 3140534 (SS), PCCI 130074 (FEB, SS), ALMA-CONICYT 31100004 (FEB, CRC), "EMBIGGEN" Anillo ACT1101 (FEB), Project IC120009 "Millennium Institute of Astrophysics (MAS) of the Iniciativa Cientifica Milenio del Ministerio de Economia, Fomento y Turismo (FEB, SS, CRC). A.G.-Y. is supported by the EU/FP7-ERC grant No. [307260], The Quantum Universe' I-Core programme by the Israeli Committee for planning and budgeting and the ISF, the Weizmann-UK making connections programme, and the Kimmel award. NER acknowledges support from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement No. 267251 "Astronomy Fellowships in Italy" (AstroFIt). Support for LG, SG and HK is provided by the Ministry of Economy, Development, and Tourisms Millennium Science Initiative through grant IC12009, awarded to The Millennium Institute of Astrophysics, MAS. L.G., S.G. and H.K. acknowledge support by CONICYT through FONDECYT grants 3130680 and 3140563, 3140566 NR 78 TC 30 Z9 30 U1 2 U2 8 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD JUL PY 2015 VL 579 AR A40 DI 10.1051/0004-6361/201425237 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO0XL UT WOS:000358877100052 ER PT J AU Alam, S Albareti, FD Prieto, CA Anders, F Anderson, SF Anderton, T Andrews, BH Armengaud, E Aubourg, E Bailey, S Basu, S Bautista, JE Beaton, RL Beers, TC Bender, CF Berlind, AA Beutler, F Bhardwaj, V Bird, JC Bizyaev, D Blake, CH Blanton, MR Blomqvist, M Bochanski, JJ Bolton, AS Bovy, J Bradley, AS Brandt, WN Brauer, DE Brinkmann, J Brown, PJ Brownstein, JR Burden, A Burtin, E Busca, NG Cai, Z Capozzi, D Rosell, AC Carr, MA Carrera, R Chambers, KC Chaplin, WJ Chen, YC Chiappini, C Chojnowski, SD Chuang, CH Clerc, N Comparat, J Covey, K Croft, RAC Cuesta, AJ Cunha, K da Costa, LN Da Rio, N Davenport, JRA Dawson, KS De Lee, N Delubac, T Deshpande, R Dhital, S Dutra-Ferreira, L Dwelly, T Ealet, A Ebelke, GL Edmondson, EM Eisenstein, DJ Ellsworth, T Elsworth, Y Epstein, CR Eracleous, M Escoffier, S Esposito, M Evans, ML Fan, XH Fernandez-Alvar, E Feuillet, D Ak, NF Finley, H Finoguenov, A Flaherty, K Fleming, SW Font-Ribera, A Foster, J Frinchaboy, PM Galbraith-Frew, JG Garcia, RA Garcia-Hernandez, DA Perez, AEG Gaulme, P Ge, J Genova-Santos, R Georgakakis, A Ghezzi, L Gillespie, BA Girardi, L Goddard, D Gontcho, SGA Hernandez, JIG Grebel, EK Green, PJ Grieb, JN Grieves, N Gunn, JE Guo, H Harding, P Hasselquist, S Hawley, SL Hayden, M Hearty, FR Hekker, S Ho, S Hogg, DW Holley-Bockelmann, K Holtzman, JA Honscheid, K Huber, D Huehnerhoff, J Ivans, II Jiang, LH Johnson, JA Kinemuchi, K Kirkby, D Kitaura, F Klaene, MA Knapp, GR Kneib, JP Koenig, XP Lam, CR Lan, TW Lang, DT Laurent, P Le Goff, JM Leauthaud, A Lee, KG Lee, YS Licquia, TC Liu, J Long, DC Lopez-Corredoira, M Lorenzo-Oliveira, D Lucatello, S Lundgren, B Lupton, RH Mack, CE Mahadevan, S Maia, MAG Majewski, SR Malanushenko, E Malanushenko, V Manchado, A Manera, M Mao, QQ Maraston, C Marchwinski, RC Margala, D Martell, SL Martig, M Masters, KL Mathur, S McBride, CK McGehee, PM McGreer, ID McMahon, RG Menard, B Menzel, ML Merloni, A Meszaros, S Miller, AA Miralda-Escude, J Miyatake, H Montero-Dorta, AD More, S Morganson, E Morice-Atkinson, X Morrison, HL Mosser, B Muna, D Myers, AD Nandra, K Newman, JA Neyrinck, M Nguyen, DC Nichol, RC Nidever, DL Noterdaeme, P Nuza, SE O'Connell, JE O'Connell, RW O'Connell, R Ogando, RLC Olmstead, MD Oravetz, AE Oravetz, DJ Osumi, K Owen, R Padgett, DL Padmanabhan, N Paegert, M Palanque-Delabrouille, N Pan, KK Parejko, JK Paris, I Park, C Pattarakijwanich, P Pellejero-Ibanez, M Pepper, J Percival, WJ Perez-Fournon, I Perez-Rafols, I Petitjean, P Pieri, MM Pinsonneault, MH de Mello, GFP Prada, F Prakash, A Price-Whelan, AM Protopapas, P Raddick, MJ Rahman, M Reid, BA Rich, J Rix, HW Robin, AC Rockosi, CM Rodrigues, TS Rodriguez-Torres, S Roe, NA Ross, AJ Ross, NP Rossi, G Ruan, JJ Rubino-Martin, JA Rykoff, ES Salazar-Albornoz, S Salvato, M Samushia, L Sanchez, AG Santiago, B Sayres, C Schiavon, RP Schlegel, DJ Schmidt, SJ Schneider, DP Schultheis, M Schwope, AD Scoccola, CG Scott, C Sellgren, K Seo, HJ Serenelli, A Shane, N Shen, Y Shetrone, M Shu, YP Aguirre, VS Sivarani, T Skrutskie, MF Slosar, A Smith, VV Sobreira, F Souto, D Stassun, KG Steinmetz, M Stello, D Strauss, MA Streblyanska, A Suzuki, N Swanson, MEC Tan, JC Tayar, J Terrien, RC Thakar, AR Thomas, D Thomas, N Thompson, BA Tinker, JL Tojeiro, R Troup, NW Vargas-Magana, M Vazquez, JA Verde, L Viel, M Vogt, NP Wake, DA Wang, J Weaver, BA Weinberg, DH Weiner, BJ White, M Wilson, JC Wisniewski, JP Wood-Vasey, WM Yeche, C York, DG Zakamska, NL Zamora, O Zasowski, G Zehavi, I Zhao, GB Zheng, Z Zhou, X Zhou, ZM Zou, H Zhu, GT AF Alam, Shadab Albareti, Franco D. Allende Prieto, Carlos Anders, F. Anderson, Scott F. Anderton, Timothy Andrews, Brett H. Armengaud, Eric Aubourg, Eric Bailey, Stephen Basu, Sarbani Bautista, Julian E. Beaton, Rachael L. Beers, Timothy C. Bender, Chad F. Berlind, Andreas A. Beutler, Florian Bhardwaj, Vaishali Bird, Jonathan C. Bizyaev, Dmitry Blake, Cullen H. Blanton, Michael R. Blomqvist, Michael Bochanski, John J. Bolton, Adam S. Bovy, Jo Bradley, A. Shelden Brandt, W. N. Brauer, D. E. Brinkmann, J. Brown, Peter J. Brownstein, Joel R. Burden, Angela Burtin, Etienne Busca, Nicolas G. Cai, Zheng Capozzi, Diego Rosell, Aurelio Carnero Carr, Michael A. Carrera, Ricardo Chambers, K. C. Chaplin, William James Chen, Yen-Chi Chiappini, Cristina Chojnowski, S. Drew Chuang, Chia-Hsun Clerc, Nicolas Comparat, Johan Covey, Kevin Croft, Rupert A. C. Cuesta, Antonio J. Cunha, Katia da Costa, Luiz N. Da Rio, Nicola Davenport, James R. A. Dawson, Kyle S. De Lee, Nathan Delubac, Timothee Deshpande, Rohit Dhital, Saurav Dutra-Ferreira, Leticia Dwelly, Tom Ealet, Anne Ebelke, Garrett L. Edmondson, Edward M. Eisenstein, Daniel J. Ellsworth, Tristan Elsworth, Yvonne Epstein, Courtney R. Eracleous, Michael Escoffier, Stephanie Esposito, Massimiliano Evans, Michael L. Fan, Xiaohui Fernandez-Alvar, Emma Feuillet, Diane Ak, Nurten Filiz Finley, Hayley Finoguenov, Alexis Flaherty, Kevin Fleming, Scott W. Font-Ribera, Andreu Foster, Jonathan Frinchaboy, Peter M. Galbraith-Frew, J. G. Garcia, Rafael A. Garcia-Hernandez, D. A. Garcia Perez, Ana E. Gaulme, Patrick Ge, Jian Genova-Santos, R. Georgakakis, A. Ghezzi, Luan Gillespie, Bruce A. Girardi, Leo Goddard, Daniel Gontcho, Satya Gontcho A. Gonzalez Hernandez, Jonay I. Grebel, Eva K. Green, Paul J. Grieb, Jan Niklas Grieves, Nolan Gunn, James E. Guo, Hong Harding, Paul Hasselquist, Sten Hawley, Suzanne L. Hayden, Michael Hearty, Fred R. Hekker, Saskia Ho, Shirley Hogg, David W. Holley-Bockelmann, Kelly Holtzman, Jon A. Honscheid, Klaus Huber, Daniel Huehnerhoff, Joseph Ivans, Inese I. Jiang, Linhua Johnson, Jennifer A. Kinemuchi, Karen Kirkby, David Kitaura, Francisco Klaene, Mark A. Knapp, Gillian R. Kneib, Jean-Paul Koenig, Xavier P. Lam, Charles R. Lan, Ting-Wen Lang, Dustin Laurent, Pierre Le Goff, Jean-Marc Leauthaud, Alexie Lee, Khee-Gan Lee, Young Sun Licquia, Timothy C. Liu, Jian Long, Daniel C. Lopez-Corredoira, Martin Lorenzo-Oliveira, Diego Lucatello, Sara Lundgren, Britt Lupton, Robert H. Mack, Claude E., III Mahadevan, Suvrath Maia, Marcio A. G. Majewski, Steven R. Malanushenko, Elena Malanushenko, Viktor Manchado, A. Manera, Marc Mao, Qingqing Maraston, Claudia Marchwinski, Robert C. Margala, Daniel Martell, Sarah L. Martig, Marie Masters, Karen L. Mathur, Savita McBride, Cameron K. McGehee, Peregrine M. McGreer, Ian D. McMahon, Richard G. Menard, Brice Menzel, Marie-Luise Merloni, Andrea Meszaros, Szabolcs Miller, Adam A. Miralda-Escude, Jordi Miyatake, Hironao Montero-Dorta, Antonio D. More, Surhud Morganson, Eric Morice-Atkinson, Xan Morrison, Heather L. Mosser, Benoit Muna, Demitri Myers, Adam D. Nandra, Kirpal Newman, Jeffrey A. Neyrinck, Mark Nguyen, Duy Cuong Nichol, Robert C. Nidever, David L. Noterdaeme, Pasquier Nuza, Sebastian E. O'Connell, Julia E. O'Connell, Robert W. O'Connell, Ross Ogando, Ricardo L. C. Olmstead, Matthew D. Oravetz, Audrey E. Oravetz, Daniel J. Osumi, Keisuke Owen, Russell Padgett, Deborah L. Padmanabhan, Nikhil Paegert, Martin Palanque-Delabrouille, Nathalie Pan, Kaike Parejko, John K. Paris, Isabelle Park, Changbom Pattarakijwanich, Petchara Pellejero-Ibanez, M. Pepper, Joshua Percival, Will J. Perez-Fournon, Ismael Perez-Rafols, Ignasi Petitjean, Patrick Pieri, Matthew M. Pinsonneault, Marc H. Porto de Mello, Gustavo F. Prada, Francisco Prakash, Abhishek Price-Whelan, Adrian M. Protopapas, Pavlos Raddick, M. Jordan Rahman, Mubdi Reid, Beth A. Rich, James Rix, Hans-Walter Robin, Annie C. Rockosi, Constance M. Rodrigues, Thaise S. Rodriguez-Torres, Sergio Roe, Natalie A. Ross, Ashley J. Ross, Nicholas P. Rossi, Graziano Ruan, John J. Rubino-Martin, J. A. Rykoff, Eli S. Salazar-Albornoz, Salvador Salvato, Mara Samushia, Lado Sanchez, Ariel G. Santiago, Basilio Sayres, Conor Schiavon, Ricardo P. Schlegel, David J. Schmidt, Sarah J. Schneider, Donald P. Schultheis, Mathias Schwope, Axel D. Scoccola, C. G. Scott, Caroline Sellgren, Kris Seo, Hee-Jong Serenelli, Aldo Shane, Neville Shen, Yue Shetrone, Matthew Shu, Yiping Aguirre, V. Silva Sivarani, Thirupathi Skrutskie, M. F. Slosar, Anze Smith, Verne V. Sobreira, Flavia Souto, Diogo Stassun, Keivan G. Steinmetz, Matthias Stello, Dennis Strauss, Michael A. Streblyanska, Alina Suzuki, Nao Swanson, Molly E. C. Tan, Jonathan C. Tayar, Jamie Terrien, Ryan C. Thakar, Aniruddha R. Thomas, Daniel Thomas, Neil Thompson, Benjamin A. Tinker, Jeremy L. Tojeiro, Rita Troup, Nicholas W. Vargas-Magana, Mariana Vazquez, Jose A. Verde, Licia Viel, Matteo Vogt, Nicole P. Wake, David A. Wang, Ji Weaver, Benjamin A. Weinberg, David H. Weiner, Benjamin J. White, Martin Wilson, John C. Wisniewski, John P. Wood-Vasey, W. M. Yeche, Christophe York, Donald G. Zakamska, Nadia L. Zamora, O. Zasowski, Gail Zehavi, Idit Zhao, Gong-Bo Zheng, Zheng Zhou, Xu Zhou, Zhimin Zou, Hu Zhu, Guangtun TI THE ELEVENTH AND TWELFTH DATA RELEASES OF THE SLOAN DIGITAL SKY SURVEY: FINAL DATA FROM SDSS-III SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE atlases; catalogs; surveys ID OSCILLATION SPECTROSCOPIC SURVEY; GALACTIC EVOLUTION EXPERIMENT; BARYON ACOUSTIC-OSCILLATIONS; LOW-MASS STELLAR; 1ST DATA RELEASE; SOLAR-LIKE STARS; FIXED-DELAY INTERFEROMETRY; CATALOG ARCHIVE SERVER; BROWN DWARF CANDIDATE; MAIN-SEQUENCE STARS AB The third generation of the Sloan Digital Sky Survey (SDSS-III) took data from 2008 to 2014 using the original SDSS wide-field imager, the original and an upgraded multi-object fiber-fed optical spectrograph, a new near-infrared high-resolution spectrograph, and a novel optical interferometer. All of the data from SDSS-III are now made public. In particular, this paper describes Data Release 11 (DR11) including all data acquired through 2013 July, and Data Release 12 (DR12) adding data acquired through 2014 July (including all data included in previous data releases), marking the end of SDSS-III observing. Relative to our previous public release (DR10), DR12 adds one million new spectra of galaxies and quasars from the Baryon Oscillation Spectroscopic Survey (BOSS) over an additional 3000 deg(2) of sky, more than triples the number of H-band spectra of stars as part of the Apache Point Observatory (APO) Galactic Evolution Experiment (APOGEE), and includes repeated accurate radial velocity measurements of 5500 stars from the Multi-object APO Radial Velocity Exoplanet Large-area Survey (MARVELS). The APOGEE outputs now include the measured abundances of 15 different elements for each star. In total, SDSS-III added 5200 deg(2) of ugriz imaging; 155,520 spectra of 138,099 stars as part of the Sloan Exploration of Galactic Understanding and Evolution 2 (SEGUE-2) survey; 2,497,484 BOSS spectra of 1,372,737 galaxies, 294,512 quasars, and 247,216 stars over 9376 deg(2); 618,080 APOGEE spectra of 156,593 stars; and 197,040 MARVELS spectra of 5513 stars. Since its first light in 1998, SDSS has imaged over 1/3 of the Celestial sphere in five bands and obtained over five million astronomical spectra. C1 [Alam, Shadab; Croft, Rupert A. C.; Ho, Shirley; Lang, Dustin; O'Connell, Ross; Osumi, Keisuke; Vargas-Magana, Mariana] Carnegie Mellon Univ, Dept Phys, McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA. [Albareti, Franco D.; Chuang, Chia-Hsun; Comparat, Johan; Prada, Francisco; Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Inst Fis Teor, UAM CSIC, E-28049 Madrid, Spain. [Allende Prieto, Carlos; Carrera, Ricardo; Esposito, Massimiliano; Fernandez-Alvar, Emma; Garcia-Hernandez, D. A.; Garcia Perez, Ana E.; Genova-Santos, R.; Gonzalez Hernandez, Jonay I.; Lopez-Corredoira, Martin; Manchado, A.; Pellejero-Ibanez, M.; Perez-Fournon, Ismael; Rubino-Martin, J. A.; Scoccola, C. G.; Streblyanska, Alina; Zamora, O.] IAC, E-38200 Tenerife, Spain. [Allende Prieto, Carlos; Carrera, Ricardo; Esposito, Massimiliano; Fernandez-Alvar, Emma; Garcia-Hernandez, D. A.; Garcia Perez, Ana E.; Genova-Santos, R.; Gonzalez Hernandez, Jonay I.; Lopez-Corredoira, Martin; Manchado, A.; Pellejero-Ibanez, M.; Perez-Fournon, Ismael; Rubino-Martin, J. A.; Scoccola, C. G.; Streblyanska, Alina; Zamora, O.] Univ La Laguna, Dept Astrofis, E-38206 Tenerife, Spain. [Anders, F.; Brauer, D. E.; Chiappini, Cristina; Kitaura, Francisco; Mack, Claude E., III; Nuza, Sebastian E.; Schwope, Axel D.; Steinmetz, Matthias] Leibniz Inst Astrophys Potsdam AIP, D-14482 Potsdam, Germany. [Anderson, Scott F.; Bhardwaj, Vaishali; Bochanski, John J.; Davenport, James R. A.; Eracleous, Michael; Evans, Michael L.; Hawley, Suzanne L.; Owen, Russell; Ruan, John J.; Sayres, Conor] Univ Washington, Dept Astron, Seattle, WA 98195 USA. [Anderton, Timothy; Bolton, Adam S.; Brownstein, Joel R.; Dawson, Kyle S.; Ellsworth, Tristan; Galbraith-Frew, J. G.; Guo, Hong; Ivans, Inese I.; Montero-Dorta, Antonio D.; Olmstead, Matthew D.; Shu, Yiping; Zheng, Zheng] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Andrews, Brett H.; Epstein, Courtney R.; Johnson, Jennifer A.; Muna, Demitri; Pinsonneault, Marc H.; Schmidt, Sarah J.; Sellgren, Kris; Tayar, Jamie; Weinberg, David H.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Andrews, Brett H.; Licquia, Timothy C.; Newman, Jeffrey A.; Prakash, Abhishek; Wood-Vasey, W. M.] Univ Pittsburgh, Dept Phys & Astron, PITT PACC, Pittsburgh, PA 15260 USA. [Armengaud, Eric; Burtin, Etienne; Laurent, Pierre; Le Goff, Jean-Marc; Palanque-Delabrouille, Nathalie; Rich, James; Rossi, Graziano; Yeche, Christophe] CEA, Ctr Saclay, Irfu SPP, F-91191 Gif Sur Yvette, France. [Aubourg, Eric; Bautista, Julian E.; Busca, Nicolas G.] Univ Paris Diderot, Sorbonne Paris Cite, Observ Paris, APC,CNRS IN2P3,CEA IRFU, F-75205 Paris, France. [Bailey, Stephen; Beutler, Florian; Bhardwaj, Vaishali; Font-Ribera, Andreu; Reid, Beth A.; Roe, Natalie A.; Schlegel, David J.; White, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Basu, Sarbani; Koenig, Xavier P.; Wang, Ji] Yale Univ, Dept Astron, New Haven, CT 06520 USA. [Beaton, Rachael L.; Ebelke, Garrett L.; Garcia Perez, Ana E.; Lam, Charles R.; Majewski, Steven R.; O'Connell, Robert W.; Shane, Neville; Skrutskie, M. F.; Troup, Nicholas W.; Wilson, John C.] Univ Virginia, Dept Astron, Charlottesville, VA 22904 USA. [Beaton, Rachael L.; Shen, Yue] Observ Carnegie Inst Washington, Pasadena, CA 91101 USA. [Beers, Timothy C.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Beers, Timothy C.] Univ Notre Dame, JINA Ctr Evolut Elements, Notre Dame, IN 46556 USA. [Bender, Chad F.; Brandt, W. N.; Deshpande, Rohit; Eracleous, Michael; Ak, Nurten Filiz; Hearty, Fred R.; Mahadevan, Suvrath; Marchwinski, Robert C.; Schneider, Donald P.; Terrien, Ryan C.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Bender, Chad F.; Deshpande, Rohit; Mahadevan, Suvrath; Marchwinski, Robert C.; Terrien, Ryan C.] Penn State Univ, Ctr Exoplanets & Habitable Worlds, Davey Lab 525, University Pk, PA 16802 USA. [Berlind, Andreas A.; Bird, Jonathan C.; Holley-Bockelmann, Kelly; Mack, Claude E., III; Mao, Qingqing; Paegert, Martin; Pepper, Joshua; Stassun, Keivan G.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Bizyaev, Dmitry; Bradley, A. Shelden; Brinkmann, J.; Gaulme, Patrick; Huehnerhoff, Joseph; Kinemuchi, Karen; Klaene, Mark A.; Long, Daniel C.; Malanushenko, Elena; Malanushenko, Viktor; Oravetz, Audrey E.; Oravetz, Daniel J.; Pan, Kaike] Apache Point Observ, Sunspot, NM 88349 USA. [Bizyaev, Dmitry; Chojnowski, S. Drew; Feuillet, Diane; Hasselquist, Sten; Hayden, Michael; Holtzman, Jon A.; Kinemuchi, Karen; Long, Daniel C.; Malanushenko, Elena; Malanushenko, Viktor; Oravetz, Audrey E.; Vogt, Nicole P.] New Mexico State Univ, Dept Astron, Las Cruces, NM 88003 USA. [Bizyaev, Dmitry] Moscow MV Lomonosov State Univ, Sternberg Astron Inst, Moscow 119992, Russia. [Blake, Cullen H.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Blanton, Michael R.; Hogg, David W.; Tinker, Jeremy L.; Weaver, Benjamin A.] NYU, Dept Phys, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [Blomqvist, Michael; Kirkby, David; Margala, Daniel] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. 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[Busca, Nicolas G.; Rosell, Aurelio Carnero; Chiappini, Cristina; da Costa, Luiz N.; Dutra-Ferreira, Leticia; Girardi, Leo; Lorenzo-Oliveira, Diego; Maia, Marcio A. G.; Ogando, Ricardo L. C.; Porto de Mello, Gustavo F.; Rodrigues, Thaise S.; Santiago, Basilio; Sobreira, Flavia] Lab Interinstituc & Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Cai, Zheng; Cunha, Katia; Fan, Xiaohui; McGreer, Ian D.; Weiner, Benjamin J.] Steward Observ, Tucson, AZ 85721 USA. [Carr, Michael A.; Gunn, James E.; Knapp, Gillian R.; Lupton, Robert H.; Miyatake, Hironao; Pattarakijwanich, Petchara; Strauss, Michael A.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Chambers, K. C.] Univ Hawaii, Inst Astron, Honolulu, HI 96822 USA. [Chaplin, William James; Elsworth, Yvonne] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Chaplin, William James; Elsworth, Yvonne; Hekker, Saskia; Huber, Daniel; Aguirre, V. Silva; Stello, Dennis] Aarhus Univ, Dept Phys & Astron, SAC, DK-8000 Aarhus C, Denmark. [Chen, Yen-Chi] Carnegie Mellon Univ, Dept Stat, Bruce & Astrid McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA. [Clerc, Nicolas; Dwelly, Tom; Georgakakis, A.; Grieb, Jan Niklas; Menzel, Marie-Luise; Merloni, Andrea; Nandra, Kirpal; Salazar-Albornoz, Salvador; Salvato, Mara; Sanchez, Ariel G.] Max Planck Inst Extraterr Phys, D-85741 Garching, Germany. [Covey, Kevin] Lowell Observ, Flagstaff, AZ 86001 USA. [Covey, Kevin] Western Washington Univ, Dept Phys & Astron, Bellingham, WA 98225 USA. [Cuesta, Antonio J.; Gontcho, Satya Gontcho A.; Miralda-Escude, Jordi; Perez-Rafols, Ignasi; Verde, Licia] Univ Barcelona, Inst Ciencies Cosmos, IEEC, E-08028 Barcelona, Spain. [Cuesta, Antonio J.; Foster, Jonathan; Padmanabhan, Nikhil] Yale Univ, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. 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C.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Eracleous, Michael] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Ak, Nurten Filiz] Erciyes Univ, Dept Astron & Space Sci, Fac Sci, TR-38039 Kayseri, Turkey. [Finley, Hayley; Noterdaeme, Pasquier; Petitjean, Patrick] UPMC, Inst Astrophys Paris, CNRS, UMR7095, F-75014 Paris, France. [Finoguenov, Alexis] Univ Helsinki, Dept Phys, FI-00140 Helsinki, Finland. [Flaherty, Kevin] Wesleyan Univ, Van Vleck Observ, Dept Astron, Middletown, CT 06459 USA. [Fleming, Scott W.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Fleming, Scott W.] Comp Sci Corp, Baltimore, MD 21218 USA. [Frinchaboy, Peter M.; O'Connell, Julia E.; Thompson, Benjamin A.] Texas Christian Univ, Dept Phys & Astron, Ft Worth, TX 76129 USA. [Garcia, Rafael A.] Univ Paris Diderot, Lab AIM, Ctr Saclay, CEA DSM,CNRS,IRFU SAp, F-91191 Gif Sur Yvette, France. [Gillespie, Bruce A.; Lan, Ting-Wen; Menard, Brice; Neyrinck, Mark; Raddick, M. Jordan; Rahman, Mubdi; Thakar, Aniruddha R.; Zakamska, Nadia L.; Zasowski, Gail; Zhu, Guangtun] Johns Hopkins Univ, Ctr Astrophys Sci, Dept Phys & Astron, Baltimore, MD 21218 USA. [Girardi, Leo; Lucatello, Sara; Rodrigues, Thaise S.] INAF, Osservatorio Astron Padova, I-35122 Padua, Italy. [Grebel, Eva K.] Heidelberg Univ, Zentrum Astron, Astron Rech Inst, D-69120 Heidelberg, Germany. [Harding, Paul; Morrison, Heather L.; Zehavi, Idit] Case Western Reserve Univ, Dept Astron, Cleveland, OH 44106 USA. [Hekker, Saskia] Max Planck Inst Sonnensystemforsch, D-37077 Gottingen, Germany. [Honscheid, Klaus] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Honscheid, Klaus; Johnson, Jennifer A.; Ross, Ashley J.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Huber, Daniel; Stello, Dennis] Univ Sydney, Sch Phys, Sydney Inst Astron SIfA, Sydney, NSW 2006, Australia. [Huber, Daniel] SETI Inst, Mountain View, CA 94043 USA. [Jiang, Linhua; Shen, Yue] Peking Univ, Kavli Inst Astron & Astrophys, Beijing 100871, Peoples R China. [Kneib, Jean-Paul] Univ Provence, CNRS, Lab Astrophys Marseille, F-13388 Marseille 13, France. [Leauthaud, Alexie; Menard, Brice; Miyatake, Hironao; More, Surhud; Suzuki, Nao] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys Math Univ Kavli IPMU, WPI, Kashiwa, Chiba 2778583, Japan. [Lee, Khee-Gan; Martig, Marie; Rix, Hans-Walter] Max Planck Inst Astron, D-69117 Heidelberg, Germany. [Lee, Young Sun] Chungnam Natl Univ, Dept Astron & Space Sci, Taejon 305764, South Korea. [Lundgren, Britt; Wake, David A.] Univ Wisconsin, Dept Astron, Madison, WI 53703 USA. [Manera, Marc] UCL, London WC1E 6BT, England. [Martell, Sarah L.] Univ New S Wales, Sch Phys, Sydney, NSW 2052, Australia. [Mathur, Savita] Space Sci Inst, Boulder, CO 80301 USA. [McGehee, Peregrine M.] CALTECH, IPAC, Pasadena, CA 91125 USA. [McMahon, Richard G.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [McMahon, Richard G.] Univ Cambridge, Kavli Inst Cosmol, Cambridge CB3 0HA, England. [Meszaros, Szabolcs] ELTE Gothard Astrophys Observ, H-9704 Szombathely, Hungary. [Miller, Adam A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Miller, Adam A.] CALTECH, Dept Astron, Pasadena, CA 91125 USA. [Miralda-Escude, Jordi; Verde, Licia] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Mosser, Benoit] Univ Paris 07, Univ Paris 06, Observ Paris, LESIA,UMR 8109, F-92195 Meudon, France. [Myers, Adam D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Nguyen, Duy Cuong] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Nidever, David L.] Univ Michigan, Dept Astron, Ann Arbor, MI 48104 USA. [Olmstead, Matthew D.] Kings Coll, Dept Chem & Phys, Wilkes Barre, PA 18711 USA. [Padgett, Deborah L.] NASA GSFC, Greenbelt, MD USA. [Parejko, John K.] Yale Univ, Dept Phys, New Haven, CT USA. [Paris, Isabelle; Viel, Matteo] INAF, Osservatorio Astron Trieste, I-34131 Trieste, Italy. [Park, Changbom] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea. [Pepper, Joshua] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. [Perez-Rafols, Ignasi] Univ Barcelona, Fac Fis, Dept Astron & Meteorol, E-08028 Barcelona, Spain. [Pieri, Matthew M.] Aix Marseille Univ, A MIDEX, CNRS, LAM UMR 7326, F-13388 Marseille 13, France. [Prada, Francisco; Rodriguez-Torres, Sergio] Campus Int Excellence UAM CSIC, E-28049 Madrid, Spain. [Prada, Francisco] CSIC, Inst Astrofis Andalucia, E-18080 Granada, Spain. [Price-Whelan, Adrian M.] Columbia Univ, Dept Astron, New York, NY 10027 USA. [Protopapas, Pavlos] Harvard Univ, SEAS, Inst Appl Computat Sci, Cambridge, MA 02138 USA. [Reid, Beth A.; White, Martin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Robin, Annie C.] Univ Franche Comte, Inst Utinam, UMR CNRS 6213, OSU Theta, F-25010 Besancon, France. [Rockosi, Constance M.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Rodrigues, Thaise S.] Univ Padua, Dipartimento Fis & Astron, I-35122 Padua, Italy. [Ross, Nicholas P.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Rossi, Graziano] Sejong Univ, Dept Astron & Space Sci, Seoul 143747, South Korea. [Rykoff, Eli S.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Salazar-Albornoz, Salvador] Univ Sternwarte, D-81679 Munich, Germany. [Salvato, Mara] Cluster Excellence, D-85748 Garching, Germany. [Samushia, Lado] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA. [Samushia, Lado] Ilia State Univ, Natl Abastumani Astrophys Observ, GE-1060 Tbilisi, Rep of Georgia. [Santiago, Basilio] Univ Fed Rio Grande do Sul, Inst Fis, BR-91501970 Porto Alegre, RS, Brazil. [Schiavon, Ricardo P.] Gemini Observ, Hilo, HI 96720 USA. [Schiavon, Ricardo P.] Liverpool John Moores Univ, Astrophys Res Inst, Liverpool L3 5RF, Merseyside, England. [Schultheis, Mathias] Univ Nice Sophia Antipolis, CNRS, Observ Cote dAzur, Lab Lagrange, F-06304 Nice 4, France. [Seo, Hee-Jong] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Serenelli, Aldo] CSIC IEEC, Inst Ciencias Espacio, Fac Ciencias, E-08193 Bellaterra, Spain. [Shetrone, Matthew] Univ Texas Austin, Hobby Eberly Telescope, McDonald Observatory, TX 79734 USA. [Sivarani, Thirupathi] Indian Inst Astrophys, Bangalore 560034, Karnataka, India. [Slosar, Anze; Vazquez, Jose A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Smith, Verne V.] Natl Opt Astron Observ, Tucson, AZ USA. [Sobreira, Flavia] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Stassun, Keivan G.] Fisk Univ, Dept Phys, Nashville, TN 37208 USA. [Terrien, Ryan C.] Penn State Univ, Penn State Astrobiol Res Ctr, University Pk, PA 16802 USA. [Thomas, Daniel] South East Phys Network, SEPnet, Southampton, Hants, England. [Tojeiro, Rita] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Verde, Licia] Univ Oslo, Inst Theoret Astrophys, NO-0315 Oslo, Norway. [Viel, Matteo] Ist Nazl Fis Nucl, I-34127 Trieste, Italy. [Wake, David A.] Open Univ, Dept Phys Sci, Milton Keynes MK7 6AA, Bucks, England. [Wisniewski, John P.] Univ Oklahoma, HL Dodge Dept Phys & Astron, Norman, OK 73019 USA. [York, Donald G.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [York, Donald G.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Zhao, Gong-Bo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. [Zhou, Xu; Zhou, Zhimin; Zou, Hu] Chinese Acad Sci, Key Lab Opt Astron, Natl Astron Observ, Beijing 100012, Peoples R China. RP Wood-Vasey, WM (reprint author), Univ Pittsburgh, Dept Phys & Astron, PITT PACC, 3941 OHara St, Pittsburgh, PA 15260 USA. RI Ogando, Ricardo/A-1747-2010; White, Martin/I-3880-2015; Brandt, William/N-2844-2015; Meszaros, Szabolcs/N-2287-2014; Georgakakis, Antonis/K-4457-2013; Mao, Qingqing/E-2043-2016; Sobreira, Flavia/F-4168-2015; Jiang, Linhua/H-5485-2016; Croft, Rupert/N-8707-2014; EPFL, Physics/O-6514-2016; Carrera, Ricardo/K-8760-2014; OI Covey, Kevin/0000-0001-6914-7797; Davenport, James/0000-0002-0637-835X; Georgakakis, Antonis/0000-0002-3514-2442; Garcia, Rafael/0000-0002-8854-3776; Serenelli, Aldo/0000-0001-6359-2769; Chambers, Kenneth /0000-0001-6965-7789; Pepper, Joshua/0000-0002-3827-8417; Beaton, Rachael/0000-0002-1691-8217; Kirkby, David/0000-0002-8828-5463; Viel, Matteo/0000-0002-2642-5707; Schmidt, Sarah/0000-0002-7224-7702; Zhu, Guangtun/0000-0002-7574-8078; Beutler, Florian/0000-0003-0467-5438; Shane, Neville/0000-0003-1024-7739; Finley, Hayley/0000-0002-1216-8914; Cuesta Vazquez, Antonio Jose/0000-0002-4153-9470; Fleming, Scott/0000-0003-0556-027X; /0000-0002-1891-3794; Verde, Licia/0000-0003-2601-8770; Martig, Marie/0000-0001-5454-1492; McMahon, Richard/0000-0001-8447-8869; Hogg, David/0000-0003-2866-9403; Ogando, Ricardo/0000-0003-2120-1154; White, Martin/0000-0001-9912-5070; Brandt, William/0000-0002-0167-2453; Meszaros, Szabolcs/0000-0001-8237-5209; Escoffier, Stephanie/0000-0002-2847-7498; Mao, Qingqing/0000-0001-6001-6723; Sobreira, Flavia/0000-0002-7822-0658; Jiang, Linhua/0000-0003-4176-6486; Croft, Rupert/0000-0003-0697-2583; Carrera, Ricardo/0000-0001-6143-8151; Rahman, Mubdi/0000-0003-1842-6096 NR 157 TC 340 Z9 341 U1 15 U2 53 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD JUL PY 2015 VL 219 IS 1 AR 12 DI 10.1088/0067-0049/219/1/12 PG 27 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO0RE UT WOS:000358858900012 ER PT J AU Walker, ES Baltay, C Campillay, A Citrenbaum, C Contreras, C Ellman, N Feindt, U Gonzalez, C Graham, ML Hadjiyska, E Hsiao, EY Krisciunas, K McKinnon, R Ment, K Morrell, N Nugent, P Phillips, MM Rabinowitz, D Rostami, S Seron, J Stritzinger, M Sullivan, M Tucker, BE AF Walker, E. S. Baltay, C. Campillay, A. Citrenbaum, C. Contreras, C. Ellman, N. Feindt, U. Gonzalez, C. Graham, M. L. Hadjiyska, E. Hsiao, E. Y. Krisciunas, K. McKinnon, R. Ment, K. Morrell, N. Nugent, P. Phillips, M. M. Rabinowitz, D. Rostami, S. Seron, J. Stritzinger, M. Sullivan, M. Tucker, B. E. TI FIRST RESULTS FROM THE La Silla-QUEST SUPERNOVA SURVEY AND THE CARNEGIE SUPERNOVA PROJECT SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE dark energy; supernovae: general; surveys ID HUBBLE-SPACE-TELESCOPE; BARYON ACOUSTIC-OSCILLATIONS; DARK-ENERGY CONSTRAINTS; PHOTOMETRY DATA RELEASE; IA SUPERNOVAE; SKY SURVEY; DUST EXTINCTION; LEGACY SURVEY; LIGHT CURVES; REDSHIFT AB The La Silla/QUEST Variability Survey (LSQ) and the Carnegie Supernova Project (CSP II) are collaborating to discover and obtain photometric light curves for a large sample of low-redshift (z < 0.1) Type Ia supernovae (SNe Ia). The supernovae are discovered in the LSQ survey using the 1 m ESO Schmidt telescope at the La Silla Observatory with the 10 square degree QUEST camera. The follow-up photometric observations are carried out using the 1 m Swope telescope and the 2.5 m du Pont telescopes at the Las Campanas Observatory. This paper describes the survey, discusses the methods of analyzing the data, and presents the light curves for the first 31 SNe Ia obtained in the survey. The SALT 2.4 supernova light-curve fitter was used to analyze the photometric data, and the Hubble diagram for this first sample is presented. The measurement errors for these supernovae averaged 4%, and their intrinsic spread was 14%. C1 [Walker, E. S.; Baltay, C.; Citrenbaum, C.; Ellman, N.; Hadjiyska, E.; Ment, K.; Morrell, N.; Rostami, S.; Seron, J.] Yale Univ, Dept Phys, New Haven, CT 06511 USA. [Campillay, A.; Contreras, C.; Gonzalez, C.; Morrell, N.; Phillips, M. M.; Seron, J.] Carnegie Inst Sci, Las Campanas Observ, La Serena, Chile. [Feindt, U.] Univ Bonn, Inst Phys, HU Berlin & Phys Inst, D-53113 Bonn, Germany. [Contreras, C.; Hsiao, E. Y.; Stritzinger, M.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Krisciunas, K.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Nugent, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Graham, M. L.; Nugent, P.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Sullivan, M.] Univ Southampton, Dept Astron, Southampton SO1 BJ, Hants, England. [Tucker, B. E.] Australian Natl Univ, Sch Astron & Astrophys, Acton, ACT 2601, Australia. RP Walker, ES (reprint author), Yale Univ, Dept Phys, 217 Prospect St, New Haven, CT 06511 USA. OI Sullivan, Mark/0000-0001-9053-4820; stritzinger, maximilian/0000-0002-5571-1833 FU Office of Science of the US Department of Energy [DE-FG02-92ER40704]; Provosts Office at Yale; NSF [AST-0306969, AST-0908886, AST-0607438, AST-1008343]; Danish Agency for Science and Technology and Innovation through a Sapere Aude Level 2 grant FX We thank the staff at Yale University, the Carnegie Observatory, and the La Silla and Las Campanas observatories whose efforts made this supernova survey possible. The Yale group thanks the Office of Science of the US Department of Energy, grant No. DE-FG02-92ER40704 and the Provosts Office at Yale for their support. The C.S.P. acknowledges NSF funding under grants AST-0306969, AST-0908886, AST-0607438, and AST-1008343, and support provided by the Danish Agency for Science and Technology and Innovation through a Sapere Aude Level 2 grant. NR 52 TC 3 Z9 3 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD JUL PY 2015 VL 219 IS 1 AR 13 DI 10.1088/0067-0049/219/1/13 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO0RE UT WOS:000358858900013 ER PT J AU Smith, NMG Mlcochova, P Watters, SA Aasa-Chapman, MMI Rabin, N Moore, S Edwards, SG Garson, JA Grant, PR Ferns, RB Kashuba, A Mayor, NP Schellekens, J Marsh, SGE McMichael, AJ Perelson, AS Pillay, D Goonetilleke, N Gupta, RK AF Smith, Nicola M. G. Mlcochova, Petra Watters, Sarah A. Aasa-Chapman, Marlene M. I. Rabin, Neil Moore, Sally Edwards, Simon G. Garson, Jeremy A. Grant, Paul R. Ferns, R. Bridget Kashuba, Angela Mayor, Neema P. Schellekens, Jennifer Marsh, Steven G. E. McMichael, Andrew J. Perelson, Alan S. Pillay, Deenan Goonetilleke, Nilu Gupta, Ravindra K. TI Proof-of-Principle for Immune Control of Global HIV-1 Reactivation In Vivo SO CLINICAL INFECTIOUS DISEASES LA English DT Article DE elite control; HIV; cure; CD8; myeloablation ID HUMAN-IMMUNODEFICIENCY-VIRUS; T-CELL RESPONSES; VIRAL REPLICATION; INFECTION; ESCAPE; HLA; TRANSPLANTATION; LYMPHOCYTES; MUTATIONS; DEPLETION AB Background. Emerging data relating to human immunodeficiency virus type 1 (HIV-1) cure suggest that vaccination to stimulate the host immune response, particularly cytotoxic cells, may be critical to clearing of reactivated HIV-1-infected cells. However, evidence for this approach in humans is lacking, and parameters required for a vaccine are unknown because opportunities to study HIV-1 reactivation are rare. Methods. We present observations from a HIV-1 elite controller, not treated with combination antiretroviral therapy, who experienced viral reactivation following treatment for myeloma with melphalan and autologous stem cell transplantation. Mathematical modeling was performed using a standard viral dynamic model. Enzyme-linked immunospot, intracellular cytokine staining, and tetramer staining were performed on peripheral blood mononuclear cells; in vitro CD8 T-cell-mediated control of virion production by autologous CD4 T cells was quantified; and neutralizing antibody titers were measured. Results. Viral rebound was measured at 28 000 copies/mL on day 13 post-transplant before rapid decay to < 50 copies/mL in 2 distinct phases with t(1/2) of 0.71 days and 4.1 days. These kinetics were consistent with an expansion of cytotoxic effector cells and killing of productively infected CD4 T cells. Following transplantation, innate immune cells, including natural killer cells, recovered with virus rebound. However, most striking was the expansion of highly functional HIV-1-specific cytotoxic CD8 T cells, at numbers consistent with those applied in modeling, as virus control was regained. Conclusions. These observations provide evidence that the human immune response is capable of controlling coordinated global HIV-1 reactivation, remarkably with potency equivalent to combination antiretroviral therapy. These data will inform design of vaccines for use in HIV-1 curative interventions. C1 [Smith, Nicola M. G.; McMichael, Andrew J.; Goonetilleke, Nilu] Univ Oxford, Nuffield Dept Med, Oxford OX1 2JD, England. [Mlcochova, Petra; Watters, Sarah A.; Aasa-Chapman, Marlene M. I.; Garson, Jeremy A.; Ferns, R. Bridget; Pillay, Deenan; Gupta, Ravindra K.] UCL, Div Infect & Immun, Dept Infect, London WC1E 6BT, England. [Rabin, Neil; Moore, Sally; Grant, Paul R.] Univ Coll London Hosp Natl Hlth Serv NHS Fdn Trus, London, England. [Edwards, Simon G.] Cent & North West London NHS Fdn Trust, Mortimer Market Ctr, London, England. [Kashuba, Angela] Univ N Carolina, Eshelman Sch Pharm, Div Pharmacotherapy & Expt Therapeut, Chapel Hill, NC 27515 USA. [Mayor, Neema P.; Schellekens, Jennifer; Marsh, Steven G. E.] Royal Free Hosp, Anthony Nolan Res Inst, London, England. [Mayor, Neema P.; Schellekens, Jennifer; Marsh, Steven G. E.] UCL, Inst Canc, London WC1E 6BT, England. [Perelson, Alan S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Pillay, Deenan] Univ KwaZulu Natal, Africa Ctr Hlth & Populat Sci, Durban, South Africa. [Goonetilleke, Nilu] Univ N Carolina, Dept Microbiol & Immunol, Chapel Hill, NC 27515 USA. RP Gupta, RK (reprint author), UCL, Div Infect & Immun, London WC1E 6BT, England. EM ravindra.gupta@ucl.ac.uk OI Pillay, Dorsamy/0000-0003-3640-2573 FU Wellcome Trust [WT093722MA]; European Community under project Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN) [223131]; National Institutes for Health Research University College London Hospitals Biomedical Research Centre; National Institutes of Health [AI028433, OD011095]; McMichael Trust Fund at Oxford University; Creative and Novel Ideas in HIV research award [AI0227763]; Medical Research Council FX This work was supported by the Wellcome Trust Fellowship to R. K. G. (WT093722MA) and the European Community's Seventh Framework Programme (FP7/2007-2013) under the project Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN; 223131). We also acknowledge support from the National Institutes for Health Research University College London Hospitals Biomedical Research Centre and National Institutes of Health for A. S. P. (AI028433 and OD011095). N. G. was supported by the McMichael Trust Fund at Oxford University and a Creative and Novel Ideas in HIV research award (AI0227763); N. M. G. S. and A. J. M. were supported by the Medical Research Council. NR 35 TC 5 Z9 5 U1 1 U2 8 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1058-4838 EI 1537-6591 J9 CLIN INFECT DIS JI Clin. Infect. Dis. PD JUL 1 PY 2015 VL 61 IS 1 BP 120 EP 128 DI 10.1093/cid/civ219 PG 9 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA CO7EX UT WOS:000359323500019 PM 25778749 ER PT J AU Spotts, R Chumbley, LS Ekstrand, L Zhang, S Kreiser, J AF Spotts, Ryan Chumbley, L. Scott Ekstrand, Laura Zhang, Song Kreiser, James TI Angular Determination of Toolmarks Using a Computer-Generated Virtual Tool SO JOURNAL OF FORENSIC SCIENCES LA English DT Article DE forensic science; statistical comparison; computer simulation; algorithm; toolmark; virtual toolmark ID VALIDATION; MARKS AB A blind study to determine whether virtual toolmarks created using a computer could be used to identify and characterize angle of incidence of physical toolmarks was conducted. Six sequentially manufactured screwdriver tips and one random screwdriver were used to create toolmarks at various angles. An apparatus controlled tool angle. Resultant toolmarks were randomly coded and sent to the researchers, who scanned both tips and toolmarks using an optical profilometer to obtain 3D topography data. Developed software was used to create virtual marks based on the tool topography data. Virtual marks generated at angles from 30 to 85 degrees (5 degrees increments) were compared to physical toolmarks using a statistical algorithm. Twenty of twenty toolmarks were correctly identified by the algorithm. On average, the algorithm misidentified the correct angle of incidence by -6.12 degrees. This study presents the results, their significance, and offers reasons for the average angular misidentification. C1 [Spotts, Ryan; Chumbley, L. Scott; Ekstrand, Laura; Zhang, Song] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Kreiser, James] Illinois State Police, Springfield, IL 62712 USA. RP Chumbley, LS (reprint author), Iowa State Univ, Dept Mat Sci & Engn, 214 Wilhelm Hall, Ames, IA 50010 USA. EM chumbley@iastate.edu RI Zhang, Song/C-5294-2012 OI Zhang, Song/0000-0001-8452-4837 FU National Institute of Justice; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358]; National Institute of Justice [2011-DNR-0230] FX Supported by the National Institute of Justice and the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under contract number DE-AC02-07CH11358. Funding was provided by award number 2011-DNR-0230 from the National Institute of Justice. NR 12 TC 1 Z9 1 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-1198 EI 1556-4029 J9 J FORENSIC SCI JI J. Forensic Sci. PD JUL PY 2015 VL 60 IS 4 BP 878 EP 884 DI 10.1111/1556-4029.12759 PG 7 WC Medicine, Legal SC Legal Medicine GA CO6JL UT WOS:000359262900006 PM 25929523 ER PT J AU Christov, IC Jordan, PM AF Christov, Ivan C. Jordan, P. M. TI Corrections to Morse and Ingard's variational-based treatment of weakly-nonlinear acoustics in lossless gases (L) (1968) SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA LA English DT Article C1 [Christov, Ivan C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Christov, Ivan C.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Jordan, P. M.] US Naval Res Lab, Acoust Div, Stennis Space Ctr, MS 39529 USA. RP Christov, IC (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM pedro.jordan@nrlssc.navy.mil RI Christov, Ivan/B-9418-2008 OI Christov, Ivan/0000-0001-8531-0531 NR 6 TC 1 Z9 1 U1 1 U2 5 PU ACOUSTICAL SOC AMER AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0001-4966 EI 1520-8524 J9 J ACOUST SOC AM JI J. Acoust. Soc. Am. PD JUL PY 2015 VL 138 IS 1 BP 361 EP 362 DI 10.1121/1.4922951 PG 2 WC Acoustics; Audiology & Speech-Language Pathology SC Acoustics; Audiology & Speech-Language Pathology GA CO1QB UT WOS:000358929000056 PM 26233035 ER PT J AU Sturtevant, BT Pantea, C Sinha, DN AF Sturtevant, Blake T. Pantea, Cristian Sinha, Dipen N. TI The acoustic nonlinearity parameter in Fluorinert up to 381K and 13.8MPa SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA LA English DT Article ID FLUIDS AB This work reports on the determination of the acoustic nonlinearity parameter, B/A, from measured sound speed data, in Fluorinert FC-43 at temperatures up to 381K and pressures up to 13.8MPa using the thermodynamic method. Sound speed was measured using Swept Frequency Acoustic Interferometry at 11 pressures between ambient and 13.8MPa along 6 isotherms between ambient and 381K. Second-order least-squares polynomial fits of measured sound speeds were used to determine temperature and pressure dependence. A room temperature B/A - 11.7 was determined and this parameter was found to increase by a factor of 2.5 over the temperature/pressure range investigated. (C) 2015 Acoustical Society of America C1 [Sturtevant, Blake T.; Pantea, Cristian; Sinha, Dipen N.] Los Alamos Natl Lab, Mat Phys & Applicat, Los Alamos, NM 87545 USA. RP Sturtevant, BT (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat, POB 1663, Los Alamos, NM 87545 USA. EM bsturtev@lanl.gov; pantea@lanl.gov; sinha@lanl.gov RI Pantea, Cristian/D-4108-2009; OI Pantea, Cristian/0000-0002-0805-8923; Sinha, Dipen/0000-0002-3606-7907 FU U.S. Department of Energy Geothermal Technologies Program FX This work was supported by the U.S. Department of Energy Geothermal Technologies Program. NR 11 TC 2 Z9 2 U1 0 U2 3 PU ACOUSTICAL SOC AMER AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0001-4966 EI 1520-8524 J9 J ACOUST SOC AM JI J. Acoust. Soc. Am. PD JUL PY 2015 VL 138 IS 1 BP EL31 EP EL35 DI 10.1121/1.4922537 PG 5 WC Acoustics; Audiology & Speech-Language Pathology SC Acoustics; Audiology & Speech-Language Pathology GA CO1QB UT WOS:000358929000006 PM 26233057 ER PT J AU Chang, C Cameron, P Elliott, J Perelson, A Roche, M Dantanarayana, A Solomon, A Naranbhai, V Tenakoon, S Hoh, R McMahon, J Sikaris, K Hartogensis, W Bacchetti, P Hecht, F Lifson, J Deeks, S Lewin, S AF Chang, Christina Cameron, Paul Elliott, Julian Perelson, Alan Roche, Michael Dantanarayana, Ashanti Solomon, Ajantha Naranbhai, Vivek Tenakoon, Surekha Hoh, Rebecca McMahon, James Sikaris, Ken Hartogensis, Wendy Bacchetti, Peter Hecht, Frederick Lifson, Jeffrey Deeks, Steve Lewin, Sharon TI Time-associated changes in cell-associated HIV RNA in HIV-infected subjects on suppressive antiretroviral therapy - implications for clinical trials of cure interventions SO JOURNAL OF THE INTERNATIONAL AIDS SOCIETY LA English DT Meeting Abstract C1 [Chang, Christina; Cameron, Paul; Roche, Michael; Dantanarayana, Ashanti; Solomon, Ajantha; Tenakoon, Surekha; Lewin, Sharon] Univ Melbourne, Doherty Inst, Melbourne, Vic, Australia. [Chang, Christina; Cameron, Paul; Elliott, Julian; McMahon, James; Lewin, Sharon] Alfred Hosp, Dept Infect Dis, Melbourne, Vic, Australia. [Perelson, Alan] Los Alamos Natl Lab, Los Alamos, NM USA. [Naranbhai, Vivek] Univ Oxford, Dept Med, Oxford, England. [Hoh, Rebecca; Deeks, Steve] Univ Calif San Francisco, Sch Med, San Francisco, CA USA. [Sikaris, Ken] Dept Pathol, Melbourne, Vic, Australia. [Hartogensis, Wendy; Bacchetti, Peter] Univ Calif San Francisco, Div Biostat, San Francisco, CA 94143 USA. [Hecht, Frederick] Univ Calif San Francisco, Ctr Integrat Med, San Francisco, CA 94143 USA. [Lifson, Jeffrey] NCI, Natl Lab Canc Res, Frederick, MD 21701 USA. EM christina.chang@unimelb.edu.au NR 0 TC 0 Z9 0 U1 0 U2 8 PU INT AIDS SOCIETY PI GENEVA PA AVENUE DE FRANCE 23, GENEVA, 1202, SWITZERLAND SN 1758-2652 J9 J INT AIDS SOC JI J. Int. AIDS Soc. PD JUL PY 2015 VL 18 SU 4 MA MOAA0106LB DI 10.7448/IAS.18.5.20567 PG 1 WC Immunology; Infectious Diseases SC Immunology; Infectious Diseases GA CN8FS UT WOS:000358675700007 ER PT J AU Viljoen, K Wendoh, J Karaoz, U Brodie, E Mulder, N Botha, G Kidzeru, E Butcher, J Gray, C Rosenthal, K Abimiku, A Cameron, B Stintzi, A Jaspan, H AF Viljoen, Katie Wendoh, Jerome Karaoz, Ulas Brodie, Eoin Mulder, Nicola Botha, Gerrit Kidzeru, Elvis Butcher, James Gray, Clive Rosenthal, Ken Abimiku, Alash'le Cameron, Bill Stintzi, Alain Jaspan, Heather TI HIV-exposure, gut microbiome, and vaccine responses in South African infants SO JOURNAL OF THE INTERNATIONAL AIDS SOCIETY LA English DT Meeting Abstract C1 [Viljoen, Katie; Wendoh, Jerome; Kidzeru, Elvis; Gray, Clive; Jaspan, Heather] Univ Cape Town, Inst Infect Dis & Mol Med, Clin Sci Lab, Cape Town, South Africa. [Karaoz, Ulas; Brodie, Eoin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Mulder, Nicola; Botha, Gerrit] Univ Cape Town, Inst Infect Dis & Mol Med, ZA-7925 Cape Town, South Africa. [Butcher, James; Stintzi, Alain] Ottawa Inst Syst Biol, Ottawa, ON, Canada. [Rosenthal, Ken] McMaster Univ, Inst Mol Med & Hlth, Hamilton, ON, Canada. [Abimiku, Alash'le] Inst Human Virol, Baltimore, MD USA. [Cameron, Bill] Ottawa Hosp Res Inst, Ottawa, ON, Canada. [Jaspan, Heather] Seattle Childrens Res Inst, Seattle, WA USA. [Jaspan, Heather] Univ Washington, Dept Pediat, Global Hlth, Seattle, WA 98195 USA. EM hbjaspan@gmail.com RI Brodie, Eoin/A-7853-2008 OI Brodie, Eoin/0000-0002-8453-8435 NR 0 TC 0 Z9 0 U1 0 U2 4 PU INT AIDS SOCIETY PI GENEVA PA AVENUE DE FRANCE 23, GENEVA, 1202, SWITZERLAND SN 1758-2652 J9 J INT AIDS SOC JI J. Int. AIDS Soc. PD JUL PY 2015 VL 18 SU 4 MA MOAA0205 DI 10.7448/IAS.18.5.20327 PG 1 WC Immunology; Infectious Diseases SC Immunology; Infectious Diseases GA CN8FS UT WOS:000358675700011 ER PT J AU Belianinov, A He, Q Kravchenko, M Jesse, S Borisevich, A Kalinin, SV AF Belianinov, Alex He, Qian Kravchenko, Mikhail Jesse, Stephen Borisevich, Albina Kalinin, Sergei V. TI Identification of phases, symmetries and defects through local crystallography SO NATURE COMMUNICATIONS LA English DT Article ID PROPANE AMMOXIDATION; ELECTRON-MICROSCOPY; OXIDE CATALYSTS; REAL SPACE; POLARIZATION; M1 AB Advances in electron and probe microscopies allow 10 pm or higher precision in measurements of atomic positions. This level of fidelity is sufficient to correlate the length (and hence energy) of bonds, as well as bond angles to functional properties of materials. Traditionally, this relied on mapping locally measured parameters to macroscopic variables, for example, average unit cell. This description effectively ignores the information contained in the microscopic degrees of freedom available in a high-resolution image. Here we introduce an approach for local analysis of material structure based on statistical analysis of individual atomic neighbourhoods. Clustering and multivariate algorithms such as principal component analysis explore the connectivity of lattice and bond structure, as well as identify minute structural distortions, thus allowing for chemical description and identification of phases. This analysis lays the framework for building image genomes and structure-property libraries, based on conjoining structural and spectral realms through local atomic behaviour. C1 [Belianinov, Alex; Kravchenko, Mikhail; Jesse, Stephen; Borisevich, Albina; Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Belianinov, Alex; Kravchenko, Mikhail; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [He, Qian; Borisevich, Albina] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Belianinov, A (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. EM belianinova@ornl.gov; albinab@ornl.gov; sergei2@ornl.gov RI Borisevich, Albina/B-1624-2009; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; He, Qian/J-1277-2014 OI Borisevich, Albina/0000-0002-3953-8460; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Research for A. Bel., Q. H., M. K., A. Bor., S. V. K., was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Research for SJ was sponsored by Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 39 TC 10 Z9 10 U1 1 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7801 DI 10.1038/ncomms8801 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0RN UT WOS:000358860100003 PM 26190623 ER PT J AU Busch, DJ Houser, JR Hayden, CC Sherman, MB Lafer, EM Stachowiak, JC AF Busch, David J. Houser, Justin R. Hayden, Carl C. Sherman, Michael B. Lafer, Eileen M. Stachowiak, Jeanne C. TI Intrinsically disordered proteins drive membrane curvature SO NATURE COMMUNICATIONS LA English DT Article ID CLATHRIN-MEDIATED ENDOCYTOSIS; SYNAPTIC VESICLE SIZE; COATED VESICLES; DYNAMIC INTERACTIONS; TRIPLET PROTEINS; AP180; CARGO; DIFFUSION; COMPLEX; DOMAIN AB Assembly of highly curved membrane structures is essential to cellular physiology. The prevailing view has been that proteins with curvature-promoting structural motifs, such as wedge-like amphipathic helices and crescent-shaped BAR domains, are required for bending membranes. Here we report that intrinsically disordered domains of the endocytic adaptor proteins, Epsin1 and AP180 are highly potent drivers of membrane curvature. This result is unexpected since intrinsically disordered domains lack a well-defined three-dimensional structure. However, in vitro measurements of membrane curvature and protein diffusivity demonstrate that the large hydrodynamic radii of these domains generate steric pressure that drives membrane bending. When disordered adaptor domains are expressed as transmembrane cargo in mammalian cells, they are excluded from clathrin-coated pits. We propose that a balance of steric pressure on the two surfaces of the membrane drives this exclusion. These results provide quantitative evidence for the influence of steric pressure on the content and assembly of curved cellular membrane structures. C1 [Busch, David J.; Houser, Justin R.; Hayden, Carl C.; Stachowiak, Jeanne C.] Univ Texas Austin, Dept Biomed Engn, Austin, TX 78712 USA. [Hayden, Carl C.] Sandia Natl Labs, Livermore, CA 94550 USA. [Sherman, Michael B.] Univ Texas Med Branch, Dept Biochem & Mol Biol, Galveston, TX 77555 USA. [Lafer, Eileen M.] Univ Texas Hlth Sci Ctr San Antonio, Dept Biochem, UTHSCSA Biochem 415B, San Antonio, TX 78229 USA. [Lafer, Eileen M.] Univ Texas Hlth Sci Ctr San Antonio, Ctr Biomed Neurosci, UTHSCSA Biochem 415B, San Antonio, TX 78229 USA. [Stachowiak, Jeanne C.] Univ Texas Austin, Inst Cellular & Mol Biol, Keeton, TX 78712 USA. RP Stachowiak, JC (reprint author), Univ Texas Austin, Dept Biomed Engn, 107 W Dean Keeton, Austin, TX 78712 USA. EM jcstach@austin.utexas.edu FU National Institutes of Health [1R01GM112065, NIH-NS029051]; University of Texas at Austin FX J.C.S. acknowledges support from the National Institutes of Health (1R01GM112065 to Stachowiak in support of Busch, Houser, and Hayden) as well as startup funding from The University of Texas at Austin. E.M.L. acknowledges support from the National Institutes of Health (NIH-NS029051 to Lafer). We thank Dr Ernst Ungewickell (Hannover Medical School) for providing the Epsin1 CTD and AP180 CTD plasmids, Dr Thomas Kirchhausen (Harvard Medical School) for providing a transferrin receptor plasmid and Dr Anthony Brown (Ohio State University) for making the neurofilament-M plasmid available through Addgene. We thank Dr Dwight Romanovicz and the ICMB Microscopy Facility at UT Austin for assistance with electron microscopy. We thank Dr Allen Liu (University of Michigan) and Dr Sandra Schmid (UT Southwestern Medical School) for providing the RPE cell line stably expressing mCherry-labelled CLC used in this study, as well as for helpful advice using the clathrin pit detection software, freely provided by the lab of Dr Gaudenz Danuser (Harvard Medical School). We thank Dr Terry O'Halloran (UT Austin) for feedback on this project, as well as undergraduate researchers Jerin Jose, Saad Jafri and Brian Li for assistance with preliminary experiments. NR 62 TC 20 Z9 20 U1 12 U2 39 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7875 DI 10.1038/ncomms8875 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0SH UT WOS:000358862100002 PM 26204806 ER PT J AU Cecchini, NM Steffes, K Schlappi, MR Gifford, AN Greenberg, JT AF Cecchini, Nicolas M. Steffes, Kevin Schlaeppi, Michael R. Gifford, Andrew N. Greenberg, Jean T. TI Arabidopsis AZI1 family proteins mediate signal mobilization for systemic defence priming SO NATURE COMMUNICATIONS LA English DT Article ID LIPID-TRANSFER PROTEINS; MEMBRANE CONTACT SITES; ACQUIRED-RESISTANCE; METHYL SALICYLATE; AZELAIC-ACID; ENDOPLASMIC-RETICULUM; PSEUDOMONAS-SYRINGAE; FREEZING TOLERANCE; SECRETORY PATHWAY; GENE-EXPRESSION AB Priming is a major mechanism behind the immunological 'memory' observed during two key plant systemic defences: systemic acquired resistance (SAR) and induced systemic resistance (ISR). Lipid-derived azelaic acid (AZA) is a mobile priming signal. Here, we show that the lipid transfer protein (LTP)-like AZI1 and its closest paralog EARLI1 are necessary for SAR, ISR and the systemic movement and uptake of AZA in Arabidopsis. Imaging and fractionation studies indicate that AZI1 and EARLI1 localize to expected places for lipid exchange/movement to occur. These are the ER/plasmodesmata, chloroplast outer envelopes and membrane contact sites between them. Furthermore, these LTP-like proteins form complexes and act at the site of SAR establishment. The plastid targeting of AZI1 and AZI1 paralogs occurs through a mechanism that may enable/facilitate their roles in signal mobilization. C1 [Cecchini, Nicolas M.; Steffes, Kevin; Greenberg, Jean T.] Univ Chicago, Dept Mol Genet & Cell Biol, Chicago, IL 60637 USA. [Schlaeppi, Michael R.] Marquette Univ, Dept Biol Sci, Milwaukee, WI 53233 USA. [Gifford, Andrew N.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Greenberg, JT (reprint author), Univ Chicago, Dept Mol Genet & Cell Biol, 929 East 57th St,GCIS Room W519P, Chicago, IL 60637 USA. EM jgreenbe@uchicago.edu OI Greenberg, Jean/0000-0002-7213-7618; Cecchini, Nicolas/0000-0002-2894-7744 FU NSF grant [IOS 0957963]; Genomic Science Program (Science Focus Area 'Plant: Microbe Interfaces'), U.S. Department of Energy, Office of Science, Biological and Environmental Research [DE-AC05-00OR22725]; U.S. Department of Agriculture [2001-35100-10688] FX This research was mainly supported by NSF grant IOS 0957963 to J.T.G. A.N.G.'s contribution was supported by the Genomic Science Program (Science Focus Area 'Plant: Microbe Interfaces'), U.S. Department of Energy, Office of Science, Biological and Environmental Research under the contract DE-AC05-00OR22725. M.R.S.'s contribution was supported by NRI Competitive Grant No. 2001-35100-10688 from the U.S. Department of Agriculture. NR 70 TC 8 Z9 9 U1 7 U2 48 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7658 DI 10.1038/ncomms8658 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QW UT WOS:000358858100002 PM 26203923 ER PT J AU Kendrick, BK Hazra, J Balakrishnan, N AF Kendrick, B. K. Hazra, Jisha Balakrishnan, N. TI The geometric phase controls ultracold chemistry SO NATURE COMMUNICATIONS LA English DT Article ID QUANTUM REACTIVE SCATTERING; STATE TRANSITION-PROBABILITIES; HYDROGEN-EXCHANGE REACTION; POTENTIAL-ENERGY SURFACES; CONICAL INTERSECTION; H+O-2 SCATTERING; MOLECULES; DYNAMICS; HO2; RECOMBINATION AB The geometric phase is shown to control the outcome of an ultracold chemical reaction. The control is a direct consequence of the sign change on the interference term between two scattering pathways (direct and looping), which contribute to the reactive collision process in the presence of a conical intersection (point of degeneracy between two Born-Oppenheimer electronic potential energy surfaces). The unique properties of the ultracold energy regime lead to an effective quantization of the scattering phase shift enabling maximum constructive or destructive interference between the two pathways. By taking the O + OH -> H + O-2 reaction as an illustrative example, it is shown that inclusion of the geometric phase modifies ultracold reaction rates by nearly two orders of magnitude. Interesting experimental control possibilities include the application of external electric and magnetic fields that might be used to exploit the geometric phase effect reported here and experimentally switch on or off the reactivity. C1 [Kendrick, B. K.] Los Alamos Natl Lab, Theoret Div T 1, Los Alamos, NM 87545 USA. [Hazra, Jisha; Balakrishnan, N.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. RP Kendrick, BK (reprint author), Los Alamos Natl Lab, Theoret Div T 1, MS B221, Los Alamos, NM 87545 USA. EM bkendric@lanl.gov FU US Department of Energy under Laboratory Directed Research and Development Program at Los Alamos National Laboratory [20140309ER]; National Security Administration of the US Department of Energy [DE-AC52-06NA25396]; Army Research Office, MURI [W911NF-12-1-0476]; National Science Foundation [PHY-1205838] FX We acknowledge G.B. Pradhan for his initial exploratory calculations of the GP effect on the O + OH reaction. B.K.K. acknowledges that part of this work was carried out under the auspices of the US Department of Energy under Project No. 20140309ER of the Laboratory Directed Research and Development Program at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. The UNLV team acknowledges support from the Army Research Office, MURI grant No. W911NF-12-1-0476 and the National Science Foundation, grant No. PHY-1205838. NR 52 TC 14 Z9 14 U1 5 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7918 DI 10.1038/ncomms8918 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0TC UT WOS:000358864700001 PM 26224326 ER PT J AU Mahjouri-Samani, M Lin, MW Wang, K Lupini, AR Lee, J Basile, L Boulesbaa, A Rouleau, CM Puretzky, AA Ivanov, IN Xiao, K Yoon, M Geohegan, DB AF Mahjouri-Samani, Masoud Lin, Ming-Wei Wang, Kai Lupini, Andrew R. Lee, Jaekwang Basile, Leonardo Boulesbaa, Abdelaziz Rouleau, Christopher M. Puretzky, Alexander A. Ivanov, Ilia N. Xiao, Kai Yoon, Mina Geohegan, David B. TI Patterned arrays of lateral heterojunctions within monolayer two-dimensional semiconductors SO NATURE COMMUNICATIONS LA English DT Article ID PULSED-LASER DEPOSITION; LAYER MOS2; MOLYBDENUM-DISULFIDE; SINGLE-LAYER; GROWTH; NANOSHEETS; HETEROSTRUCTURES; TRANSISTORS; GRAPHENE AB The formation of semiconductor heterojunctions and their high-density integration are foundations of modern electronics and optoelectronics. To enable two-dimensional crystalline semiconductors as building blocks in next-generation electronics, developing methods to deterministically form lateral heterojunctions is crucial. Here we demonstrate an approach for the formation of lithographically patterned arrays of lateral semiconducting heterojunctions within a single two-dimensional crystal. Electron beam lithography is used to pattern MoSe2 monolayer crystals with SiO2, and the exposed locations are selectively and totally converted to MoS2 using pulsed laser vaporization of sulfur to form MoSe2/MoS2 heterojunctions in predefined patterns. The junctions and conversion process are studied by Raman and photoluminescence spectroscopy, atomically resolved scanning transmission electron microscopy and device characterization. This demonstration of lateral heterojunction arrays within a monolayer crystal is an essential step for the integration of two-dimensional semiconductor building blocks with different electronic and optoelectronic properties for high-density, ultrathin devices. C1 [Mahjouri-Samani, Masoud; Lin, Ming-Wei; Wang, Kai; Lee, Jaekwang; Basile, Leonardo; Boulesbaa, Abdelaziz; Rouleau, Christopher M.; Puretzky, Alexander A.; Ivanov, Ilia N.; Xiao, Kai; Yoon, Mina; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Lupini, Andrew R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Basile, Leonardo] Escuela Politec Nacl, Dept Fis, Quito 170525, Ecuador. RP Mahjouri-Samani, M (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM mahjourisamm@ornl.gov; geohegandb@ornl.gov RI Wang, Kai/H-4361-2011; Mahjouri-Samani, Masoud/Q-2239-2015; Rouleau, Christopher/Q-2737-2015; Yoon, Mina/A-1965-2016; Puretzky, Alexander/B-5567-2016; Boulesbaa, Abdelaziz/J-3314-2016; Geohegan, David/D-3599-2013; OI ivanov, ilia/0000-0002-6726-2502; Wang, Kai/0000-0002-6405-7837; Mahjouri-Samani, Masoud/0000-0002-6080-7450; Rouleau, Christopher/0000-0002-5488-3537; Yoon, Mina/0000-0002-1317-3301; Puretzky, Alexander/0000-0002-9996-4429; Boulesbaa, Abdelaziz/0000-0003-4519-4403; Geohegan, David/0000-0003-0273-3139; Lin, Ming-Wei/0000-0001-8150-5585 FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division; National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT) FX Synthesis science including crystal growth, in situ plume diagnostics, TEM analysis, SEM and AFM studies and conversion technique development (M.M.-S., K.W., J.L., A.R.L., K.X., D.B.G., C.M.R., A.A.P. and M.Y.) was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and performed in part as a user project at the Center for Nanophase Materials Sciences, which is a DOE Office of the Science User Facility. Characterization science at Center for Nanophase Materials Sciences (CNMS) including optical characterization and lithography techniques (M.-W.L., A.B. and I.N.I.) was supported by the Scientific User Facilities Division. L.B. was supported by the National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT). NR 28 TC 21 Z9 21 U1 20 U2 116 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7749 DI 10.1038/ncomms8749 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0RA UT WOS:000358858500055 PM 26198727 ER PT J AU Mairoser, T Mundy, JA Melville, A Hodash, D Cueva, P Held, R Glavic, A Schubert, J Muller, DA Schlom, DG Schmehl, A AF Mairoser, Thomas Mundy, Julia A. Melville, Alexander Hodash, Daniel Cueva, Paul Held, Rainer Glavic, Artur Schubert, Juergen Muller, David A. Schlom, Darrell G. Schmehl, Andreas TI High-quality EuO thin films the easy way via topotactic transformation SO NATURE COMMUNICATIONS LA English DT Article ID CRYSTAL-STRUCTURE; LOW-TEMPERATURE; SOLID-STATE; OXIDE-FILMS; PEROVSKITE; REDUCTION; EUROPIUM; IRON; DEPOSITION; METALS AB Epitaxy is widely employed to create highly oriented crystalline films. A less appreciated, but nonetheless powerful means of creating such films is via topotactic transformation, in which a chemical reaction transforms a single crystal of one phase into a single crystal of a different phase, which inherits its orientation from the original crystal. Topotactic reactions may be applied to epitactic films to substitute, add or remove ions to yield epitactic films of different phases. Here we exploit a topotactic reduction reaction to provide a non-ultra-high vacuum (UHV) means of growing highly oriented single crystalline thin films of the easily over-oxidized half-metallic semiconductor europium monoxide (EuO) with a perfection rivalling that of the best films of the same material grown by molecular-beam epitaxy or UHV pulsed-laser deposition. As the technique only requires high-vacuum deposition equipment, it has the potential to drastically improve the accessibility of high-quality single crystalline films of EuO as well as other difficult-to-synthesize compounds. C1 [Mairoser, Thomas; Schmehl, Andreas] Univ Augsburg, Zentrum Elekt Korrelat & Magnetismus, D-86159 Augsburg, Germany. [Mundy, Julia A.; Cueva, Paul; Muller, David A.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Melville, Alexander; Hodash, Daniel; Held, Rainer; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Glavic, Artur] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Schubert, Juergen] Peter Grunberg Inst, Res Ctr Julich, PGI IT 9, D-52425 Julich, Germany. [Muller, David A.; Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Schlom, DG (reprint author), Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. EM schlom@cornell.edu RI Glavic, Artur/B-3453-2015; OI Glavic, Artur/0000-0003-4951-235X; Schubert, Jurgen/0000-0003-0185-6794 FU DFG [TRR 80]; EC (oxIDes); AFOSR [FA9550-10-1-0123]; National Science Foundation Materials Research Science and Engineering Centers (MRSEC) programme [DMR-1120296]; NSF [IMR-0417392]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0002334]; Army Research Office; National Science Foundation; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The work in Augsburg was supported by the DFG (TRR 80) and the EC (oxIDes). The work at Cornell was supported by the AFOSR (Grant No. FA9550-10-1-0123). This work made use of the electron microscopy facility of the Cornell Center for Materials Research (CCMR) with support from the National Science Foundation Materials Research Science and Engineering Centers (MRSEC) programme (DMR-1120296) and NSF IMR-0417392. EELS acquisition and analysis by P.C. and D.A.M. supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Award No. DE-SC0002334. J.A.M. acknowledges financial support from the Army Research Office in the form of a National Defense Science and Engineering Graduate Fellowship and from the National Science Foundation in the form of a graduate research fellowship. The X-ray reflectivity part of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 50 TC 6 Z9 6 U1 12 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7716 DI 10.1038/ncomms8716 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0RA UT WOS:000358858500022 PM 26177710 ER PT J AU Svanidze, E Wang, JKK Besara, T Liu, L Huang, Q Siegrist, T Frandsen, B Lynn, JW Nevidomskyy, AH Gamza, MB Aronson, MC Uemura, YJ Morosan, E AF Svanidze, E. Wang, Jiakui K. Besara, T. Liu, L. Huang, Q. Siegrist, T. Frandsen, B. Lynn, J. W. Nevidomskyy, Andriy H. Gamza, Monika B. Aronson, M. C. Uemura, Y. J. Morosan, E. TI An itinerant antiferromagnetic metal without magnetic constituents SO NATURE COMMUNICATIONS LA English DT Article ID ELECTRON FERROMAGNETISM; SPIN FLUCTUATIONS; TRANSITIONS; POINTS AB The origin of magnetism in metals has been traditionally discussed in two diametrically opposite limits: itinerant and local moments. Surprisingly, there are very few known examples of materials that are close to the itinerant limit, and their properties are not universally understood. In the case of the two such examples discovered several decades ago, the itinerant ferromagnets ZrZn2 and Sc3In, the understanding of their magnetic ground states draws on the existence of 3d electrons subject to strong spin fluctuations. Similarly, in Cr, an elemental itinerant antiferromagnet with a spin density wave ground state, its 3d electron character has been deemed crucial to it being magnetic. Here, we report evidence for an itinerant antiferromagnetic metal with no magnetic constituents: TiAu. Antiferromagnetic order occurs below a Neel temperature of 36 K, about an order of magnitude smaller than in Cr, rendering the spin fluctuations in TiAu more important at low temperatures. This itinerant antiferromagnet challenges the currently limited understanding of weak itinerant antiferromagnetism, while providing insights into the effects of spin fluctuations in itinerant-electron systems. C1 [Svanidze, E.; Wang, Jiakui K.; Nevidomskyy, Andriy H.; Morosan, E.] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Besara, T.; Siegrist, T.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA. [Liu, L.; Frandsen, B.; Uemura, Y. J.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Huang, Q.; Lynn, J. W.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Gamza, Monika B.; Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Morosan, E (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM emorosan@rice.edu RI Besara, Tiglet/M-7969-2014; OI Besara, Tiglet/0000-0002-2143-2254; Nevidomskyy, Andriy/0000-0002-8684-7979 FU NSF [DMR 0847681, DMR-1105961, OISE-0968226, DMR-1436095]; AFOSR MURI; Welch Foundation [C-1818]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-SC0008832]; National Science Foundation [DMR-1157490]; State of Florida; REIMEI project from JAEA, Japan; Friends of Todai Inc. Foundation FX We would like to thank M.B. Maple, P. Dai, M. Foster, S. Kivelson, Z. Deng, T. Munsie, T. Medina, and G. Luke for assistance and discussions. The work at Rice University was supported by NSF DMR 0847681 (E.M. and E.S.), AFOSR MURI (J.K.W.) and the Welch Foundation grant C-1818 (A.H.N.). Work at Brookhaven National Laboratory (M.B.G. and M.C.A.) was carried out under the auspices of the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH1886. T.B. and T.S. are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Award #DE-SC0008832. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490 and the State of Florida. Work at Columbia and TRIUMF (L.L., B.F. and Y.J.U.) is supported by NSF grants DMR-1105961, OISE-0968226 (PIRE) and DMR-1436095 (DMREF), REIMEI project from JAEA, Japan, and the Friends of Todai Inc. Foundation. The identification of any commercial product or trade name does not imply endorsement or recommendation by the National Institute of Standards and Technology. NR 32 TC 2 Z9 2 U1 9 U2 47 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7701 DI 10.1038/ncomms8701 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0RA UT WOS:000358858500007 PM 26166042 ER PT J AU Wolf, O Campione, S Benz, A Ravikumar, AP Liu, S Luk, TS Kadlec, EA Shaner, EA Klem, JF Sinclair, MB Brener, I AF Wolf, Omri Campione, Salvatore Benz, Alexander Ravikumar, Arvind P. Liu, Sheng Luk, Ting S. Kadlec, Emil A. Shaner, Eric A. Klem, John F. Sinclair, Michael B. Brener, Igal TI Phased-array sources based on nonlinear metamaterial nanocavities SO NATURE COMMUNICATIONS LA English DT Article ID INTERSUBBAND TRANSITIONS; LIGHT; METASURFACES; REFRACTION; PATCHES AB Coherent superposition of light from subwavelength sources is an attractive prospect for the manipulation of the direction, shape and polarization of optical beams. This phenomenon constitutes the basis of phased arrays, commonly used at microwave and radio frequencies. Here we propose a new concept for phased-array sources at infrared frequencies based on metamaterial nanocavities coupled to a highly nonlinear semiconductor heterostructure. Optical pumping of the nanocavity induces a localized, phase-locked, nonlinear resonant polarization that acts as a source feed for a higher-order resonance of the nanocavity. Varying the nanocavity design enables the production of beams with arbitrary shape and polarization. As an example, we demonstrate two second harmonic phased-array sources that perform two optical functions at the second harmonic wavelength (similar to 5 mu m): a beam splitter and a polarizing beam splitter. Proper design of the nanocavity and nonlinear heterostructure will enable such phased arrays to span most of the infrared spectrum. C1 [Wolf, Omri; Campione, Salvatore; Benz, Alexander; Liu, Sheng; Luk, Ting S.; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Wolf, Omri; Campione, Salvatore; Benz, Alexander; Liu, Sheng; Luk, Ting S.; Kadlec, Emil A.; Shaner, Eric A.; Klem, John F.; Sinclair, Michael B.; Brener, Igal] Sandia Natl Labs, Div Sci & Technol, Albuquerque, NM 87185 USA. [Ravikumar, Arvind P.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. RP Wolf, O (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM owolf@sandia.gov; ibrener@sandia.gov RI Ravikumar, Arvind/L-1580-2016; OI Campione, Salvatore/0000-0003-4655-5485; Ravikumar, Arvind/0000-0001-8385-6573 FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US DOE's National Nuclear Security Administration [DE-AC04-94AL85000] FX O.W. would like to acknowledge Mr Caner Guclu, University of California Irvine, for his assistance in the far field calculations, Dr Xuedan Ma, Sandia National Laboratories, for her assistance with SEM imaging and Dr Naama Wald for assistance in graphical designs of figures in this manuscript. This work was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering and performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the US DOE Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US DOE's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 24 TC 30 Z9 30 U1 7 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7667 DI 10.1038/ncomms8667 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QW UT WOS:000358858100011 PM 26126879 ER PT J AU Yi, M Liu, ZK Zhang, Y Yu, R Zhu, JX Lee, JJ Moore, RG Schmitt, FT Li, W Riggs, SC Chu, JH Lv, B Hu, J Hashimoto, M Mo, SK Hussain, Z Mao, ZQ Chu, CW Fisher, IR Si, Q Shen, ZX Lu, DH AF Yi, M. Liu, Z-K Zhang, Y. Yu, R. Zhu, J. -X. Lee, J. J. Moore, R. G. Schmitt, F. T. Li, W. Riggs, S. C. Chu, J. -H. Lv, B. Hu, J. Hashimoto, M. Mo, S. -K. Hussain, Z. Mao, Z. Q. Chu, C. W. Fisher, I. R. Si, Q. Shen, Z. -X. Lu, D. H. TI Observation of universal strong orbital-dependent correlation effects in iron chalcogenides SO NATURE COMMUNICATIONS LA English DT Article ID ELECTRONIC-STRUCTURE; T-C; SUPERCONDUCTIVITY; FESE; TRANSITION; INSULATOR; PNICTIDES; ORIGIN; FILMS; GAP AB Establishing the appropriate theoretical framework for unconventional superconductivity in the iron-based materials requires correct understanding of both the electron correlation strength and the role of Fermi surfaces. This fundamental issue becomes especially relevant with the discovery of the iron chalcogenide superconductors. Here, we use angle-resolved photoemission spectroscopy to measure three representative iron chalcogenides, FeTe0.56Se0.44, monolayer FeSe grown on SrTiO3 and K0.76Fe1.72Se2. We show that these superconductors are all strongly correlated, with an orbital-selective strong renormalization in the d(xy) bands despite having drastically different Fermi surface topologies. Furthermore, raising temperature brings all three compounds from a metallic state to a phase where the dxy orbital loses all spectral weight while other orbitals remain itinerant. These observations establish that iron chalcogenides display universal orbital-selective strong correlations that are insensitive to the Fermi surface topology, and are close to an orbital-selective Mott phase, hence placing strong constraints for theoretical understanding of iron-based superconductors. C1 [Yi, M.; Liu, Z-K; Zhang, Y.; Lee, J. J.; Moore, R. G.; Schmitt, F. T.; Li, W.; Riggs, S. C.; Chu, J. -H.; Fisher, I. R.; Shen, Z. -X.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Yi, M.; Liu, Z-K; Zhang, Y.; Lee, J. J.; Moore, R. G.; Schmitt, F. T.; Li, W.; Riggs, S. C.; Chu, J. -H.; Fisher, I. R.; Shen, Z. -X.] Stanford Univ, Menlo Pk, CA 94025 USA. [Yi, M.; Liu, Z-K; Lee, J. J.; Riggs, S. C.; Fisher, I. R.; Shen, Z. -X.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Yi, M.; Liu, Z-K; Lee, J. J.; Riggs, S. C.; Fisher, I. R.; Shen, Z. -X.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Yi, M.; Liu, Z-K; Lee, J. J.; Riggs, S. C.; Fisher, I. R.; Shen, Z. -X.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Zhang, Y.; Mo, S. -K.; Hussain, Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Yu, R.] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Yu, R.; Si, Q.] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Zhu, J. -X.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Lv, B.; Chu, C. W.] Univ Houston, Texas Ctr Superconduct, Dept Phys, Houston, TX 77204 USA. [Hu, J.; Mao, Z. Q.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. [Hashimoto, M.; Lu, D. H.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Shen, ZX (reprint author), Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM zxshen@stanford.edu; dhlu@slac.stanford.edu RI Mo, Sung-Kwan/F-3489-2013; Hu, Jin/C-4141-2014; Yu, Rong/H-3355-2016 OI Mo, Sung-Kwan/0000-0003-0711-8514; Hu, Jin/0000-0003-0080-4239; FU US DOE, Office of Basic Energy Science, Division of Materials Science and Engineering [DE-AC02-76SF00515]; NSF Grant [DMR-1309531]; Robert A. Welch Foundation [C-1411]; National Science Foundation of China [11374361]; Fundamental Research Funds for the Central Universities; Research Funds of Remnin University of China; NSF [DMR-1205469]; U.S. DOE Office of Basic Energy Sciences FX ARPES experiments were performed at the Stanford Synchrotron Radiation Lightsource and the Advanced Light Source, which are both operated by the Office of Basic Energy Sciences, U.S. Department of Energy. The Stanford work is supported by the US DOE, Office of Basic Energy Science, Division of Materials Science and Engineering, under award number DE-AC02-76SF00515. The work at Rice is supported by NSF Grant DMR-1309531 and the Robert A. Welch Foundation Grant No. C-1411. The work at Renmin University is supported by the National Science Foundation of China Grant number 11374361, and the Fundamental Research Funds for the Central Universities and the Research Funds of Remnin University of China. The work at Tulane is supported by the NSF under grant DMR-1205469. The work at Los Alamos was supported by the U.S. DOE Office of Basic Energy Sciences. NR 41 TC 27 Z9 27 U1 9 U2 51 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7777 DI 10.1038/ncomms8777 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0RL UT WOS:000358859800003 PM 26204461 ER PT J AU Firestone, RB AF Firestone, R. B. TI Nuclear Data Sheets for A=21 SO NUCLEAR DATA SHEETS LA English DT Article ID THERMAL-NEUTRON CAPTURE; DELAYED-PROTON-DECAY; FIRST EXCITED STATES; DRIP-LINE NUCLEI; ENERGY-LEVELS; BETA-DECAY; MAGNETIC-MOMENT; LIGHT-NUCLEI; RICH NUCLEI; LIFETIME MEASUREMENTS AB This evaluation of A=21 has been updated from previous evaluations published in 2004Fi10,1998En04, 1990En08, and 1978En02. Coverage includes properties of adopted levels and gamma-rays, decay-scheme data (energies, intensities and placement of radiations), and cross reference entries. The following tables continue the tradition of showing the systematic relationships between levels in A=21. Much of the new data in this evaluations were taken directly from the xundl database, compiled under the direction of Balraj Singh, McMaster University. The evaluator is particularly appreciative of the efforts of the xundl compilers. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Firestone, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Ms 88r0192,1 Cyclotron Rd, Berkeley, CA 94720 USA. NR 144 TC 1 Z9 1 U1 1 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD JUL-AUG PY 2015 VL 127 BP 1 EP 68 DI 10.1016/j.nds.2015.07.001 PG 68 WC Physics, Nuclear SC Physics GA CO0BE UT WOS:000358814300001 ER PT J AU Basunia, MS AF Basunia, M. Shamsuzzoha TI Nuclear Data Sheets for A=22 SO NUCLEAR DATA SHEETS LA English DT Article ID HIGH-SPIN STATES; NEUTRON-RICH NUCLEI; RECOIL-DISTANCE METHOD; DOPPLER-SHIFT ATTENUATION; BEAM GAMMA-SPECTROSCOPY; HALF-LIFE MEASUREMENTS; LOW-ENERGY RESONANCES; RESOLUTION ION-BEAM; SD-SHELL NUCLEI; ROTATIONAL BAND-STRUCTURE AB Evaluated spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented for C-22, N-22, O-22, F-22, Ne-22, Na-22, Mg-22, Al-22, and Si-22. This evaluation for A=22 supersedes the earlier one by R. B. Firestone (2005Fi16). C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Basunia, MS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, MS 88R0192,1 Cyclotron Rd, Berkeley, CA 94720 USA. FU Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231] FX This work was supported by Office of Basic Energy Sciences, US Department of Energy, under contract DE-AC02-05CH11231. NR 325 TC 2 Z9 2 U1 1 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD JUL-AUG PY 2015 VL 127 BP 69 EP 190 DI 10.1016/j.nds.2015.07.002 PG 122 WC Physics, Nuclear SC Physics GA CO0BE UT WOS:000358814300002 ER PT J AU Browne, E Tuli, JK AF Browne, E. Tuli, J. K. TI Nuclear Data Sheets for A=238 SO NUCLEAR DATA SHEETS LA English DT Article ID DOUBLE-BETA-DECAY; EVEN-EVEN NUCLEI; SPONTANEOUSLY-FISSIONING ISOMERS; CAPTURE CROSS-SECTION; INELASTIC NEUTRON-SCATTERING; U-238 SPONTANEOUS-FISSION; ATOMIC MASS EVALUATION; RICH ISOTOPE TH-238; HIGH-SPIN STATES; MACROSCOPIC-MICROSCOPIC APPROACH C1 [Browne, E.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Lawrence Berkeley Natl Lab, Upton, NY 11973 USA. [Tuli, J. K.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Browne, E (reprint author), Brookhaven Natl Lab, Natl Nucl Data Ctr, Lawrence Berkeley Natl Lab, Upton, NY 11973 USA. FU Office of Nuclear Physics, Office of Science, US Department of Energy [DE-AC02-98CH10946] FX Research sponsored by Office of Nuclear Physics, Office of Science, US Department of Energy, under contract DE-AC02-98CH10946. NR 666 TC 3 Z9 3 U1 2 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD JUL-AUG PY 2015 VL 127 BP 191 EP 332 DI 10.1016/j.nds.2015.07.003 PG 142 WC Physics, Nuclear SC Physics GA CO0BE UT WOS:000358814300003 ER PT J AU Hu, Y Dera, P Zhuravlev, K AF Hu, Yi Dera, Przemyslaw Zhuravlev, Kirill TI Single-crystal diffraction and Raman spectroscopy of hedenbergite up to 33 GPa SO PHYSICS AND CHEMISTRY OF MINERALS LA English DT Article DE Hedenbergite; Diopside; Pyroxenes; High pressure; Synchrotron single-crystal X-ray diffraction; Mantle; Subduction zone ID MEMBER THERMODYNAMIC PROPERTIES; METASTABLE OLIVINE WEDGE; PHASE-TRANSFORMATION; SUBDUCTING SLABS; TRANSITION ZONE; GARNET; POLYHEDRA; PYROXENES; MINERALS; MANTLE AB Pyroxenes are important minerals in Earth's upper mantle and subducting plate. Here, we report results of high-pressure single-crystal X-ray diffraction and Raman spectroscopy experiments conducted on natural Ca, Fe pyroxene hedenbergite up to similar to 33 GPa in diamond anvil cell. Unit cell parameters a, b, c, beta and V, as well as bond lengths of hedenbergite are reported within the studied pressure range. Cell parameters exhibit continuous decrease on compression. Axial compressibilities of a, b and c are calculated to be 1.7(2), 4.9(5) and 2.13(9) x 10(-3) GPa(-1), respectively. Bulk modulus and its pressure derivative are determined to be 131(4) GPa and 3.8(3) by fitting thirdorder Birch-Murnaghan equation of state. Compression mechanism is dominated by polyhedral and bond compression trends typical of clinopyroxenes. In general, shorter bonds show lower compressibility, and SiO4, the smallest polyhedron, shows the lowest compressibility. Angle and elongation distortions are reported for the three types of polyhedra at high pressure. Thirteen vibrational modes are observed with Raman spectroscopy up to similar to 33 GPa. All observed mode frequencies increase as pressure increases. C1 [Hu, Yi] Univ Hawaii Manoa, Sch Ocean & Earth Sci & Technol, Dept Geol & Geophys, Honolulu, HI 96822 USA. [Dera, Przemyslaw] Univ Hawaii Manoa, Sch Ocean & Earth Sci & Technol, Hawaii Inst Geophys & Planetol, Honolulu, HI 96822 USA. [Zhuravlev, Kirill] Univ Chicago, Ctr Adv Radiat Sources, Argonne Natl Lab, Argonne, IL 60439 USA. RP Hu, Y (reprint author), Univ Hawaii Manoa, Sch Ocean & Earth Sci & Technol, Dept Geol & Geophys, 1680 East West Rd,POST Bldg, Honolulu, HI 96822 USA. EM yihu@hawaii.edu FU National Science Foundation Division of Earth Sciences Geophysics [1344942]; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-Geosciences [DE-FG02-94ER14466]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Carnegie-DOE Alliance Center FX The project was supported by the National Science Foundation Division of Earth Sciences Geophysics Grant No. 1344942. Portions of this work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), and Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We would also like to thank Carnegie-DOE Alliance Center for support through Academic Partner subcontract to PD and Prof. R. T. Downs at the University of Arizona for kindly providing the samples from RRUFF collections. We would like to thank the two reviewers, Diego Gatta and Jennifer Kung for helpful comments. NR 38 TC 2 Z9 2 U1 3 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0342-1791 EI 1432-2021 J9 PHYS CHEM MINER JI Phys. Chem. Miner. PD JUL PY 2015 VL 42 IS 7 BP 595 EP 608 DI 10.1007/s00269-015-0747-8 PG 14 WC Materials Science, Multidisciplinary; Mineralogy SC Materials Science; Mineralogy GA CO1UE UT WOS:000358940200007 ER PT J AU Bose, A Woo, KM Nora, R Betti, R AF Bose, A. Woo, K. M. Nora, R. Betti, R. TI Hydrodynamic scaling of the deceleration-phase Rayleigh-Taylor instability SO PHYSICS OF PLASMAS LA English DT Article ID INERTIAL CONFINEMENT FUSION; DIRECT-DRIVE; IMPLOSIONS AB The scaling of the deceleration phase of inertial fusion direct-drive implosions is investigated for OMEGA and National Ignition Facility (NIF)-size targets. It is shown that the deceleration-phase Rayleigh-Taylor instability (RTI) does not scale hydro-equivalently with implosion size. This is because ablative stabilization resulting from thermal conduction and radiation transport in a spherically converging geometry is different on the two scales. As a consequence, NIF-scale implosions show lower hot-spot density and mass ablation velocity, allowing for higher RTI growth. On the contrary, stabilization resulting from density-gradient enhancement, caused by reabsorption of radiation emitted from the hot spot, is higher on NIF implosions. Since the RTI mitigation related to thermal conduction and radiation transport scale oppositely with implosion size, the degradation of implosion performance caused by the deceleration RTI is similar for NIF and OMEGA targets. It is found that a minimum threshold for the no-alpha Lawson ignition parameter of chi(Omega) approximate to 0.2 at the OMEGA scale is required to demonstrate hydro-equivalent ignition at the NIF scale for symmetric direct-drive implosions. (C) 2015 AIP Publishing LLC. C1 [Bose, A.; Woo, K. M.; Betti, R.] Univ Rochester, Dept Phys, Laser Energet Lab, Rochester, NY 14623 USA. [Bose, A.; Woo, K. M.; Betti, R.] Univ Rochester, Fus Sci Ctr, Rochester, NY 14623 USA. [Nora, R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Bose, A (reprint author), Univ Rochester, Dept Phys, Laser Energet Lab, 250 East River Rd, Rochester, NY 14623 USA. EM abos@lle.rochester.edu FU U.S. Department of Energy [DE-FC02-04ER54789, DE-NA0001944]; New York State Energy Research Development Authority; University of Rochester; Office of Fusion Energy Sciences FX The authors thank Dr. K. Anderson, Dr. J. Delettrez, and Dr. R. Epstein from the Laboratory of Laser Energetics, and Professor D. Shvarts from Ben-Gurion University of the Negev, for many useful discussions. This work has been supported by the U.S. Department of Energy under Cooperative Agreement Nos. DE-FC02-04ER54789 (Fusion Science Center supported by the Office of Fusion Energy Sciences) and DE-NA0001944 (National Nuclear Security Administration), the New York State Energy Research Development Authority, and the University of Rochester. The support of DOE does not constitute an endorsement by DOE of the views expressed in this article. NR 31 TC 2 Z9 2 U1 3 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 072702 DI 10.1063/1.4923438 PG 12 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600040 ER PT J AU Daniels, J van Tilborg, J Gonsalves, AJ Schroeder, CB Benedetti, C Esarey, E Leemans, WP AF Daniels, J. van Tilborg, J. Gonsalves, A. J. Schroeder, C. B. Benedetti, C. Esarey, E. Leemans, W. P. TI Plasma density diagnostic for capillary-discharge based plasma channels SO PHYSICS OF PLASMAS LA English DT Article ID LASER-PULSES; ACCELERATORS AB The plasma density in discharged laser guiding structures, of order 10(18) cm(-3), is critical to laser-plasma accelerators. Here, we demonstrate a technique that uses spectral interferometry to measure the on-axis laser group velocity (and thus density) in cm-scale cylindrical hydrogen-discharge plasma channels by using laser pulses with a Gaussian transverse profile. Experimental density retrieval over a range of capillary parameters (density, length, and diameter) is presented. The accuracy (of order 8 x 10(16) cm(-3)) and shot-to-shot stability (of order 2 x 10(16) cm(-3)) of the diagnostic are discussed. (C) 2015 AIP Publishing LLC. C1 [Daniels, J.; van Tilborg, J.; Gonsalves, A. J.; Schroeder, C. B.; Benedetti, C.; Esarey, E.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Daniels, J.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. RP van Tilborg, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM jvantilborg@lbl.gov RI Daniels, Joost/N-2378-2015; OI Daniels, Joost/0000-0002-9480-6077; Schroeder, Carl/0000-0002-9610-0166 FU U.S. Department of Energy, Office of Science, Office of High Energy Physics [DE-AC02-05CH11231] FX The authors acknowledge contributions by F. Mollica and the invaluable support from Scientific, Technical, and Administrative Staff at Lawrence Berkeley National Laboratory. This work was supported by the U.S. Department of Energy, Office of Science, Office of High Energy Physics, under Contract No. DE-AC02-05CH11231. NR 16 TC 1 Z9 1 U1 2 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 073112 DI 10.1063/1.4926825 PG 6 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600058 ER PT J AU King, JD Strait, EJ Lazerson, SA Ferraro, NM Logan, NC Haskey, SR Park, JK Hanson, JM Lanctot, MJ Liu, YQ Nazikian, R Okabayashi, M Paz-Soldan, C Shiraki, D Turnbull, AD AF King, J. D. Strait, E. J. Lazerson, S. A. Ferraro, N. M. Logan, N. C. Haskey, S. R. Park, J. -K. Hanson, J. M. Lanctot, M. J. Liu, Yueqiang Nazikian, R. Okabayashi, M. Paz-Soldan, C. Shiraki, D. Turnbull, A. D. TI Experimental tests of linear and nonlinear three-dimensional equilibrium models in DIII-D SO PHYSICS OF PLASMAS LA English DT Article ID RESISTIVE WALL MODE; ENERGY PRINCIPLE; BOOZER MODEL; D TOKAMAK; HIGH-BETA; COLLISIONALITY REGIME; PLASMAS; STABILITY; CONFINEMENT; PERTURBATIONS AB DIII-D experiments using new detailed magnetic diagnostics show that linear, ideal magnetohydrodynamics (MHD) theory quantitatively describes the magnetic structure (as measured externally) of three-dimensional (3D) equilibria resulting from applied fields with toroidal mode number n = 1, while a nonlinear solution to ideal MHD force balance, using the VMEC code, requires the inclusion of n >= 1 to achieve similar agreement. These tests are carried out near ITER baseline parameters, providing a validated basis on which to exploit 3D fields for plasma control development. Scans of the applied poloidal spectrum and edge safety factor confirm that low-pressure, n = 1 non-axisymmetric tokamak equilibria are determined by a single, dominant, stable eigenmode. However, at higher beta, near the ideal kink mode stability limit in the absence of a conducting wall, the qualitative features of the 3D structure are observed to vary in a way that is not captured by ideal MHD. (C) 2015 AIP Publishing LLC. C1 [King, J. D.] Oak Ridge Inst Sci Educ, Oak Ridge, TN 37830 USA. [King, J. D.; Strait, E. J.; Ferraro, N. M.; Lanctot, M. J.; Paz-Soldan, C.; Turnbull, A. D.] Gen Atom, San Diego, CA 92816 USA. [Lazerson, S. A.; Logan, N. C.; Park, J. -K.; Nazikian, R.; Okabayashi, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Haskey, S. R.] Australian Natl Univ, Res Sch Phys Sci & Engn, Plasma Res Lab, Canberra, ACT 0200, Australia. [Hanson, J. M.] Columbia Univ, New York, NY 10027 USA. [Liu, Yueqiang] Culham Sci Ctr, Culham Ctr Fusion Energy, Abingdon OX14 3DB, Oxon, England. [Shiraki, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP King, JD (reprint author), Oak Ridge Inst Sci Educ, Oak Ridge, TN 37830 USA. EM kingjd@fusion.gat.com RI Lazerson, Samuel/E-4816-2014; Lanctot, Matthew J/O-4979-2016 OI Lazerson, Samuel/0000-0001-8002-0121; Lanctot, Matthew J/0000-0002-7396-3372 FU U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FC02-04ER54698, DE-AC05-06OR23100, DE-AC02-09CH11466, DE-FG02-04ER54761, DE-AC05-00OR22725] FX This material is based upon work supported in part by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under Award Nos. DE-FC02-04ER54698, DE-AC05-06OR23100, DE-AC02-09CH11466, DE-FG02-04ER54761, and DE-AC05-00OR22725. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. The authors wish to thank R. J. Buttery for encouraging concurrent benchmarking of all codes tested. We also express gratitude to A. H. Reiman for fruitful validation discussions. NR 65 TC 13 Z9 13 U1 0 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 072501 DI 10.1063/1.4923017 PG 9 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600027 ER PT J AU Montgomery, DS Albright, BJ Barnak, DH Chang, PY Davies, JR Fiksel, G Froula, DH Kline, JL MacDonald, MJ Sefkow, AB Yin, L Betti, R AF Montgomery, D. S. Albright, B. J. Barnak, D. H. Chang, P. Y. Davies, J. R. Fiksel, G. Froula, D. H. Kline, J. L. MacDonald, M. J. Sefkow, A. B. Yin, L. Betti, R. TI Use of external magnetic fields in hohlraum plasmas to improve laser-coupling (vol 22, 010703, 2015) SO PHYSICS OF PLASMAS LA English DT Correction C1 [Montgomery, D. S.; Albright, B. J.; Kline, J. L.; Yin, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Barnak, D. H.; Chang, P. Y.; Davies, J. R.; Fiksel, G.; Froula, D. H.; Betti, R.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [MacDonald, M. J.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [MacDonald, M. J.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sefkow, A. B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Montgomery, DS (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. NR 1 TC 1 Z9 1 U1 1 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 079901 DI 10.1063/1.4926815 PG 1 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600086 ER PT J AU Si, JH Colgate, SA Sonnenfeld, RG Nornberg, MD Li, H Colgate, AS Westpfahl, DJ Romero, VD Martinic, J AF Si, Jiahe Colgate, Stirling A. Sonnenfeld, Richard G. Nornberg, Mark D. Li, Hui Colgate, Arthur S. Westpfahl, David J., Jr. Romero, Van D. Martinic, Joe TI Suppression of turbulent resistivity in turbulent Couette flow SO PHYSICS OF PLASMAS LA English DT Article ID SHEAR-DRIVEN TURBULENCE; RIGA DYNAMO EXPERIMENT; ALPHA-OMEGA-DYNAMO; MAGNETIC-FIELD; ROTATING CYLINDERS; REYNOLDS-NUMBER; TAYLOR FLOW; AGN DISKS; TRANSPORT; CONDUCTIVITY AB Turbulent transport in rapidly rotating shear flow very efficiently transports angular momentum, a critical feature of instabilities responsible both for the dynamics of accretion disks and the turbulent power dissipation in a centrifuge. Turbulent mixing can efficiently transport other quantities like heat and even magnetic flux by enhanced diffusion. This enhancement is particularly evident in homogeneous, isotropic turbulent flows of liquid metals. In the New Mexico dynamo experiment, the effective resistivity is measured using both differential rotation and pulsed magnetic field decay to demonstrate that at very high Reynolds number rotating shear flow can be described entirely by mean flow induction with very little contribution from correlated velocity fluctuations. (C) 2015 AIP Publishing LLC. C1 [Si, Jiahe; Sonnenfeld, Richard G.; Colgate, Arthur S.; Westpfahl, David J., Jr.; Romero, Van D.; Martinic, Joe] New Mexico Inst Min & Technol, Socorro, NM 87801 USA. [Colgate, Stirling A.; Li, Hui] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Nornberg, Mark D.] Univ Wisconsin, Madison, WI 53706 USA. RP Si, JH (reprint author), New Mexico Inst Min & Technol, Socorro, NM 87801 USA. EM jsi@nmt.edu OI Westpfahl, David/0000-0001-8865-1817; Si, Jiahe/0000-0002-1683-2093; Sonnenfeld, Richard/0000-0003-0364-850X; Nornberg, Mark/0000-0003-1786-4190 FU NSF [1102444]; LANL; NM-Tech; LANL/LDRD program; DoE/OFES through CMSO; New Mexico Tech office of RED; Colgate family; CMSO [PHY 08-21899] FX We gratefully acknowledge the funding over the years by NSF (Grant No. 1102444), and LANL via a cooperative arrangement with NM-Tech. We offer heartfelt thanks to National Instruments for providing much of the data acquisition system. S.A.C. and H.L. also acknowledge the support by the LANL/LDRD program and DoE/OFES through CMSO. J.S. expresses thanks to the New Mexico Tech office of R&ED for bridging funds between grants. Several members of the Colgate family and other private investors have contributed funds and we are deeply appreciative of their commitment to this project. M.D.N. acknowledges the support from CMSO PHY 08-21899 covering his time for this project. NR 46 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 072304 DI 10.1063/1.4926582 PG 10 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600023 ER PT J AU Smalyuk, VA Weber, SV Casey, DT Clark, DS Field, JE Haan, SW Hammel, BA Hamza, AV Hoover, DE Landen, OL Nikroo, A Robey, HF Weber, CR AF Smalyuk, V. A. Weber, S. V. Casey, D. T. Clark, D. S. Field, J. E. Haan, S. W. Hammel, B. A. Hamza, A. V. Hoover, D. E. Landen, O. L. Nikroo, A. Robey, H. F. Weber, C. R. TI Hydrodynamic instability growth of three-dimensional, "native-roughness" modulations in x-ray driven, spherical implosions at the National Ignition Facility SO PHYSICS OF PLASMAS LA English DT Article AB Hydrodynamic instability growth experiments with three-dimensional (3-D) surface-roughness modulations were performed on plastic (CH) shell spherical implosions at the National Ignition Facility (NIF) [E. M. Campbell, R. Cauble, and B. A. Remington, AIP Conf. Proc. 429, 3 (1998)]. The initial capsule outer-surface roughness was similar to the standard specifications ("native roughness") used in a majority of implosions on NIF. The experiments included instability growth measurements of the perturbations seeded by the thin membranes (or tents) used to hold the capsules inside the hohlraums. In addition, initial modulations included two divots used as spatial fiducials to determine the convergence in the experiments and to check the accuracy of 3D simulations in calculating growth of known initial perturbations. The instability growth measurements were performed using x-ray, through-foil radiography of one side of the imploding shell, based on time-resolved pinhole imaging. Averaging over 30 similar images significantly increases the signal-to-noise ratio, making possible a comparison with 3-D simulations. At a convergence ratio of similar to 3, the measured tent and divot modulations were close to those predicted by 3-D simulations (within similar to 15%-20%), while measured 3-D, broadband modulations were similar to 3-4 times larger than those simulated based on the growth of the known imposed initial surface modulations. In addition, some of the measured 3-D features in x-ray radiographs did not resemble those characterized on the outer capsule surface before the experiments. One of the hypotheses to explain the results is based on the increased instability amplitudes due to modulations of the oxygen content in the bulk of the capsule. As the target assembly and handling procedures involve exposure to UV light, this can increase the uptake of the oxygen into the capsule, with irregularities in the oxygen seeding hydrodynamic instabilities. These new experimental results have prompted looking for ways to reduce UV light exposure during target fabrication. (C) 2015 AIP Publishing LLC. C1 [Smalyuk, V. A.; Weber, S. V.; Casey, D. T.; Clark, D. S.; Field, J. E.; Haan, S. W.; Hammel, B. A.; Hamza, A. V.; Landen, O. L.; Robey, H. F.; Weber, C. R.] Lawrence Livermore Natl Lab, NIF Directorate, Livermore, CA 94550 USA. [Hoover, D. E.; Nikroo, A.] Gen Atom, San Diego, CA 92186 USA. RP Smalyuk, VA (reprint author), Lawrence Livermore Natl Lab, NIF Directorate, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 40 TC 14 Z9 14 U1 0 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 072704 DI 10.1063/1.4926591 PG 10 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600042 ER PT J AU Swadling, GF Lebedev, SV Harvey-Thompson, AJ Rozmus, W Burdiak, G Suttle, L Patankar, S Smith, RA Bennett, M Hall, GN Suzuki-Vidal, F Bland, S Yuan, J AF Swadling, G. F. Lebedev, S. V. Harvey-Thompson, A. J. Rozmus, W. Burdiak, G. Suttle, L. Patankar, S. Smith, R. A. Bennett, M. Hall, G. N. Suzuki-Vidal, F. Bland, S. Yuan, J. TI Interpenetration and deflection phenomena in collisions between supersonic, magnetized, tungsten plasma flows diagnosed using high resolution optical Thomson scattering SO PHYSICS OF PLASMAS LA English DT Article ID Z-PINCH EXPERIMENTS; FIELD; JETS AB An optical Thomson scattering diagnostic has been used to investigate collisions between supersonic, magnetized plasma flows, in particular the transition from collisionless to collisional interaction dynamics. These flows were produced using tungsten wire array z-pinches, driven by the 1.4 MA 240 ns Magpie generator at Imperial College London. Measurements of the collective-mode Thomson scattering ion-feature clearly indicate that the ablation flows are interpenetrating at 100 ns (after current start), and this interpenetration continues until at least 140 ns. The Thomson spectrum at 150 ns shows a clear change in the dynamics of the stream interactions, transitioning towards a collisional, shock-like interaction of the streams near the axis. The Thomson scattering data also provide indirect evidence of the presence of a significant toroidal magnetic field embedded in the "precursor" plasma near the axis of the array over the period 100-140 ns; these observations are in agreement with previous measurements [Swadling et al., Phys. Rev. Lett. 113, 035003 (2014)]. The Thomson scattering measurements at 150 ns suggest that this magnetic field must collapse at around the time the dense precursor column begins to form. (C) 2015 AIP Publishing LLC. C1 [Swadling, G. F.; Lebedev, S. V.; Burdiak, G.; Bland, S.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. [Harvey-Thompson, A. J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Rozmus, W.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2J1, Canada. [Yuan, J.] CAE, Inst Fluid Phys, Key Lab Pulsed Power, Mianyang 621900, Peoples R China. RP Swadling, GF (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. RI Swadling, George/S-5980-2016 OI Swadling, George/0000-0001-8370-8837 FU EPSRC by DOE [EP/G001324/1, DE-F03-02NA00057, DE-SC-0001063]; Sandia National Laboratories FX This work was supported in part by EPSRC Grant No. EP/G001324/1 by DOE cooperative Agreement Nos. DE-F03-02NA00057 and DE-SC-0001063 and by Sandia National Laboratories. NR 40 TC 2 Z9 2 U1 1 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2015 VL 22 IS 7 AR 072706 DI 10.1063/1.4926579 PG 17 WC Physics, Fluids & Plasmas SC Physics GA CO1RT UT WOS:000358933600044 ER PT J AU Matmon, A Hidy, AJ Vainer, S Crouvi, O Fink, D Erel, Y Horwitz, LK Chazan, M AF Matmon, Ari Hidy, Alan J. Vainer, Shlomy Crouvi, Onn Fink, David Erel, Yigal Horwitz, Liora K. Chazan, Michael CA ASTER Team TI New chronology for the southern Kalahari Group sediments with implications for sediment-cycle dynamics and early hominin occupation SO QUATERNARY RESEARCH LA English DT Article DE Kalahari Group; Cosmogenic isotope burial dating; Sedimentary cycles ID NUCLIDE PRODUCTION-RATES; COSMOGENIC NUCLIDES; CENTRAL-AFRICA; DRAINAGE EVOLUTION; WONDERWERK CAVE; MANGANESE FIELD; NAMIB DESERT; ENVIRONMENTAL-CHANGE; LANDSCAPE EVOLUTION; AMS STANDARDS AB Kalahari Group sediments accumulated in the Kalahari basin, which started forming during the breakup of Gondwana in the early Cretaceous. These sediments cover an extensive part of southern Africa and form a low-relief landscape. Current models assume that the Kalahari Group accumulated throughout the entire Cenozoic. However, chronology has been restricted to early-middle Cenozoic biostratigraphic correlations and to OSL dating of only the past similar to 300 ka. We present a new chronological framework that reveals a dynamic nature of sedimentation in the southern Kalahari. Cosmogenic burial ages obtained from a 55 m section of Kalahari Group sediments from the Mamatwan Mine, southern Kalahari, indicate that the majority of deposition at this location occurred rapidly at 1-1.2 Ma. This Pleistocene sequence overlies the Archaean basement, forming a significant hiatus that permits the possibility of many Phanerozoic cycles of deposition and erosion no longer preserved in the sedimentary record. Our data also establish the existence of a shallow early-middle Pleistocene water body that persisted for >450 ka prior to this rapid period of deposition. Evidence from neighboring archeological excavations in southern Africa suggests an association of high-density hominin occupation with this water body. (C) 2015 University of Washington. Published by Elsevier Inc. All rights reserved. C1 [Matmon, Ari; Hidy, Alan J.; Vainer, Shlomy; Erel, Yigal] Hebrew Univ Jerusalem, Fredy & Nadine Herrmann Inst Earth Sci, IL-91904 Jerusalem, Israel. [Hidy, Alan J.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. [Crouvi, Onn] Geol Survey Israel, IL-95501 Jerusalem, Israel. [Fink, David] Australian Nucl Sci & Technol Org, Menai, NSW 2234, Australia. [Horwitz, Liora K.] Hebrew Univ Jerusalem, Fac Life Sci, Natl Nat Hist Collect, IL-91904 Jerusalem, Israel. [Chazan, Michael] Univ Toronto, Dept Anthropol, Toronto, ON M5S 2S2, Canada. RP Matmon, A (reprint author), Hebrew Univ Jerusalem, Fredy & Nadine Herrmann Inst Earth Sci, Edmond J Safra Campus, IL-91904 Jerusalem, Israel. EM arimatmon@mail.huji.ac.il RI fink, David/A-9518-2012 FU Canadian Social Sciences and Humanities Research Council (SSHRC) [LLNL-JRNL-657937] FX We thank the Mamatwan Mine management and geologist, especially, P. Markram, G. van der Bank, D. Spies, A. Ntalo, and Dr. L. Jacobson for their assistance during fieldwork. We thank P. Bierman and an anonymous reviewer for their very constructive reviews. This project was partially funded by a grant from the Canadian Social Sciences and Humanities Research Council (SSHRC) awarded to M. Chazan. This is LLNL-JRNL-657937. NR 120 TC 1 Z9 1 U1 4 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0033-5894 EI 1096-0287 J9 QUATERNARY RES JI Quat. Res. PD JUL PY 2015 VL 84 IS 1 BP 118 EP 132 DI 10.1016/j.yqres.2015.04.009 PG 15 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA CO0CE UT WOS:000358816900011 ER PT J AU Simpson, JT Hunter, SR Aytug, T AF Simpson, John T. Hunter, Scott R. Aytug, Tolga TI Superhydrophobic materials and coatings: a review SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE superhydrophobic; volumetric; superhydrophilic; oleophobic; desalination; anti-biofouling; anti-corrosion ID SURFACES; LITHOGRAPHY; NANOSTRUCTURES; WETTABILITY; FABRICATION; WATER AB Over the past few years, the scientific community, as well as the world's coatings industry has seen the introduction of oxide/polymer-based superhydrophobic surfaces and coatings with exceptional water repellency. Online videos have caught the public's imagination by showing people walking through mud puddles without getting their tennis shoes wet or muddy, and water literally flying off coated surfaces. This article attempts to explain the basics of this behavior and to discuss and explain the latest superhydrophobic technological breakthroughs. Since superhydrophobic surfaces and coatings can fundamentally change how water interacts with surfaces, and the fact that earth is a water world, it can legitimately be said that this technology has the potential to literally change the world. C1 [Simpson, John T.] Univ Tennessee, Knoxville, TN 37996 USA. [Hunter, Scott R.; Aytug, Tolga] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Simpson, JT (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM jsimpso4@utk.edu; huntersr@ornl.gov; aytugt@ornl.gov FU DARPA; USMC, Forrest Pilgrim; SOCOM; US Army; DOE FX I would like to thank the following associates, collaborators, and funding agencies:; My research team and supportive management while at Oak Ridge National Lab; Dr B D'Urso; Dr D Hill; Dr J Wadsworth; My research team and supportive management at University of Tennessee; S McNeany; Dr R Benson; Dr E Drumm; F Tompkins; Funding Agencies for our superhydrophobic technology research; DARPA-Leo Christodoulou; USMC-Matthew Koch, Forrest Pilgrim; SOCOM-Shawn Martin; US Army-Picatinny Arsenal; DOE-EERE; ORNL's superhydrophobic technology licensees; Dry Surface Coatings, LLC-Stewart Kennedy; United Protective Technologies-Brent Barbee, Marty Efird Lowes Corp. NR 53 TC 22 Z9 23 U1 41 U2 202 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD JUL PY 2015 VL 78 IS 8 AR 086501 DI 10.1088/0034-4885/78/8/086501 PG 14 WC Physics, Multidisciplinary SC Physics GA CO0RW UT WOS:000358861000003 PM 26181655 ER PT J AU Kletetschka, G Hruba, J AF Kletetschka, Gunther Hruba, Jolana TI Dissolved Gases and Ice Fracturing During the Freezing of a Multicellular Organism: Lessons from Tardigrades SO BIORESEARCH OPEN ACCESS LA English DT Article DE cryopreservation; cryptobiosis; DNA damage; extracellular damage; survival ID NEMATODE PANAGROLAIMUS-DAVIDI; EUTARDIGRADE RICHTERSIUS-CORONIFER; ANTARCTIC NEMATODE; CRYOPROTECTIVE DEHYDRATION; COLD TOLERANCE; ANHYDROBIOTIC TARDIGRADES; MILNESIUM-TARDIGRADUM; RADIATION TOLERANCE; BELGICA-ANTARCTICA; IONIZING-RADIATION AB Three issues are critical for successful cryopreservation of multicellular material: gases dissolved in liquid, thermal conductivity of the tissue, and localization of microstructures. Here we show that heat distribution is controlled by the gas amount dissolved in liquids and that when changing the liquid into solid, the dissolved gases either form bubbles due to the absence of space in the lattice of solids and/or are migrated toward the concentrated salt and sugar solution at the cost of amount of heat required to be removed to complete a solid-state transition. These factors affect the heat distribution in the organs to be cryopreserved. We show that the gas concentration issue controls fracturing of ice when freezing. There are volumetric changes not only when changing the liquid into solid (volume increases) but also reduction of the volume when reaching lower temperatures (volume decreases). We discuss these issues parallel with observations of the cryosurvivability of multicellular organisms, tardigrades, and discuss their analogy for cryopreservation of large organs. C1 [Kletetschka, Gunther; Hruba, Jolana] Charles Univ Prague, Fac Sci, Prague 12843 2, Czech Republic. [Kletetschka, Gunther] Acad Sci Czech Republic, Inst Geol, Vvi, Prague, Czech Republic. [Kletetschka, Gunther] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Kletetschka, G (reprint author), Charles Univ Prague, Fac Sci, Albertov 6, Prague 12843 2, Czech Republic. EM kletetschka@gmail.com RI Kletetschka, Gunther/C-9996-2011 OI Kletetschka, Gunther/0000-0002-0645-9037 NR 68 TC 0 Z9 0 U1 6 U2 27 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 2164-7844 EI 2164-7860 J9 BIORESEARCH OPEN ACC JI BioResearch Open Access PD JUL PY 2015 VL 4 IS 1 BP 209 EP 217 DI 10.1089/biores.2015.0008 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CL9QD UT WOS:000357312300020 PM 26309797 ER PT J AU ElSohly, AM Francis, MB AF ElSohly, Adel M. Francis, Matthew B. TI Development of Oxidative Coupling Strategies for Site-Selective Protein Modification SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID SURFACE MODIFICATION; O-AMINOPHENOLS; CROSS-LINKING; BIOCONJUGATION; CHEMISTRY; BACTERIOPHAGE-MS2; ANILINES; CELLS; DNA; INTEGRATION AB CONSPECTUS: As the need to prepare ever more complex but well-defined materials has increased, a similar need for reliable synthetic strategies to access them has arisen. Accordingly, recent years have seen a steep increase in the development of reactions that can proceed under mild conditions, in aqueous environments, and with low concentrations of reactants. To enable the preparation of well-defined biomolecular materials with novel functional properties, our laboratory has a continuing interest in developing new bioconjugation reactions. A particular area of focus has been the development of oxidative reactions to perform rapid site- and chemoselective couplings of electron rich aromatic species with both unnatural and canonical amino acid residues. This Account details the evolution of oxidative coupling reactions in our laboratory, from initial concepts to highly efficient reactions, focusing on the practical aspects of performing and developing reactions of this type. We begin by discussing our rationale for choosing an oxidative coupling approach to bioconjugation, highlighting many of the benefits that such strategies provide. In addition, we discuss the general workflow we have adopted to discover protein modification reactions directly in aqueous media with biologically relevant substrates. We then review our early explorations of periodate-mediated oxidative couplings between primary anilines and p-phenylenediamine substrates, highlighting the most important lessons that were garnered from these studies. Key mechanistic insights allowed us to develop second-generation reactions between anilines and anisidine derivatives. In addition, we summarize the methods we have used for the introduction of aniline groups onto protein substrates for modification. The development of an efficient and chemoselective coupling of anisidine derivatives with tyrosine residues in the presence of ceric ammonium nitrate is next described. Here, our logic and workflow are used to highlight the challenges and opportunities associated with the optimization of site-selective chemistries that target native amino acids. We close by discussing the most recent reports from our laboratory that have capitalized on the unique reactivity of o-iminoquinone derivatives. We discuss the various oxidants and conditions that can be used to generate these reactive intermediates from appropriate precursors, as well as the product distributions that result. We also describe our work to determine the nature of iminoquinone reactivity with proteins and peptides bearing free N-terminal amino groups. Through this discussion, we hope to facilitate the use of oxidative approaches to protein bioconjugation, as well as inspire the discovery of new reactions for the site-selective modification of biomolecular targets. C1 [ElSohly, Adel M.; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Francis, Matthew B.] Lawrence Berkeley Natl Labs, Mol Foundry, Berkeley, CA 94720 USA. RP Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mbfrancis@berkeley.edu FU NIH [R01 GM072700]; DOD Breast Cancer Research Program [BC061995]; DOD BCRP postdoctoral fellowship [W81XWH-14-0400] FX The development of these reactive strategies was generously supported by the NIH (Grant R01 GM072700) and the DOD Breast Cancer Research Program (Grant BC061995). A.M.E. was supported by a DOD BCRP postdoctoral fellowship (Grant W81XWH-14-0400). The authors thank Dr. Allie Obermeyer and Dr. Kristen Seim for very helpful discussions. NR 40 TC 6 Z9 7 U1 12 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JUL PY 2015 VL 48 IS 7 BP 1971 EP 1978 DI 10.1021/acs.accounts.5b00139 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PJ UT WOS:000358556400021 PM 26057118 ER PT J AU Bullock, RM Helm, ML AF Bullock, R. Morris Helm, Monte L. TI Molecular Electrocatalysts for Oxidation of Hydrogen Using Earth-Abundant Metals: Shoving Protons Around with Proton Relays SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID COUPLED ELECTRON-TRANSFER; PENDANT AMINES; HETEROLYTIC CLEAVAGE; H-2 OXIDATION; COORDINATION SPHERES; TRANSITION-METALS; ACTIVE-SITE; FUEL-CELLS; COMPLEXES; NICKEL AB Sustainable, carbon-neutral energy is needed to supplant the worldwide reliance on fossil fuels in order to address the persistent problem of increasing emissions of CO2. Solar and wind energy are intermittent, highlighting the need to develop energy storage on a huge scale. Electrocatalysts provide a way to convert between electrical energy generated by renewable energy sources and chemical energy in the form of chemical bonds. Oxidation of hydrogen to give two electrons and two protons is carried out in fuel cells, but the typical catalyst is platinum, a precious metal of low earth abundance and high cost. In nature, hydrogenases based on iron or iron/nickel reversibly oxidize hydrogen with remarkable efficiencies and rates. Functional models of these enzymes have been synthesized with the goal of achieving electrocatalytic H-2 oxidation using inexpensive, earth-abundant metals along with a key feature identified in the [FeFe]-hydrogenase: an amine base positioned near the metal. The diphosphine ligands (P2NR)-N-R'2 (1,5-diaza-3,7-diphosphacyclooctane with alkyl or aryl groups on the P and N atoms) are used as ligands in Ni, Fe, and Mn complexes. The pendant amines facilitate binding and heterolytic cleavage of H-2, placing the hydride on the metal and the proton on the amine. The pendant amines also serve as proton relays, accelerating intramolecular and intermolecular proton transfers. Electrochemical oxidations and deprotonations by an exogeneous amine base lead to catalytic cycles for oxidation of H-2 (1 atm) at room temperature for catalysts derived from [Ni((P2NR)-N-Cy'(2))(2)](2+), (CpC6Fe)-Fe-F5((P2N2Bn)-N-tBu)H, and MnH((P2N2Bn)-N-Ph)(bppm)(CO) [bppm = (PAr2F)(2)CH2]. In the oxidation of H-2 catalyzed by [Ni((P2NR)-N-Cy'(2))(2)](2+), the initial product observed experimentally is a Ni(0) complex in which two of the pendant amines are protonated. Two different pathways can occur from this intermediate; deprotonation followed by oxidation occurs with a lower overpotential than the alternate pathway involving oxidation followed by deprotonation. The Mn cation [Mn(PPh2N2Bn)(bppm)(CO)](+) mediates the rapid (>10(4) s(-1) at -95 degrees C), reversible heterolytic cleavage of H-2. Obtaining the optimal benefit of pendant amines incorporated into the ligand requires that the pendant amine be properly positioned to interact with a M-H or M(H-2) bond. In addition, ligands are ideally selected such that the hydride-acceptor ability of the metal and the basicity of a pendant are tuned to give low barriers for heterolytic cleavage of the HH bond and subsequent proton transfer reactions. Using these principles allows the rational design of electrocatalysts for H-2 oxidation using earth-abundant metals. C1 [Bullock, R. Morris; Helm, Monte L.] Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. RP Bullock, RM (reprint author), Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, POB 999,K2-12, Richland, WA 99352 USA. EM morris.bullock@pnnl.gov RI Bullock, R. Morris/L-6802-2016 OI Bullock, R. Morris/0000-0001-6306-4851 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX We thank Dan DuBois for many helpful discussions and our co-workers for their dedicated efforts that produced the results described here. This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. NR 52 TC 28 Z9 28 U1 16 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JUL PY 2015 VL 48 IS 7 BP 2017 EP 2026 DI 10.1021/acs.accounts.5b00069 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PJ UT WOS:000358556400025 PM 26079983 ER PT J AU Zee, DZ Chantarojsiri, T Long, JR Chang, CJ AF Zee, David Z. Chantarojsiri, Teera Long, Jeffrey R. Chang, Christopher J. TI Metal-Polypyridyl Catalysts for Electro- and Photochemical Reduction of Water to Hydrogen SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID MOLECULAR COBALT COMPLEX; 2ND COORDINATION SPHERE; MOLYBDENUM-OXO CATALYST; H-2 EVOLUTION; ELECTROCATALYTIC REDUCTION; GENERATING HYDROGEN; OXIDATIVE ADDITION; FUNCTIONAL MODELS; AQUEOUS-SOLUTION; MOS2 AB Climate change, rising global energy demand, and energy security concerns motivate research into alternative, sustainable energy sources. In principle, solar energy can meet the worlds energy needs, but the intermittent nature of solar illumination means that it is temporally and spatially separated from its consumption. Developing systems that promote solar-to-fuel conversion, such as via reduction of protons to hydrogen, could bridge this production-consumption gap, but this effort requires invention of catalysts that are cheap, robust, and efficient and that use earth-abundant elements. In this context, catalysts that utilize water as both an earth-abundant, environmentally benign substrate and a solvent for proton reduction are highly desirable. This Account summarizes our studies of molecular metal-polypyridyl catalysts for electrochemical and photochemical reduction of protons to hydrogen. Inspired by concept transfer from biological and materials catalysts, these scaffolds are remarkably resistant to decomposition in water, with fast and selective electrocatalytic and photocatalytic conversions that are sustainable for several days. Their modular nature offers a broad range of opportunities for tuning reactivity by molecular design, including altering ancillary ligand electronics, denticity, and/or incorporating redox-active elements. Our first-generation complex, [(PY4)Co(CH3CN)(2)](2+), catalyzes the reduction of protons from a strong organic acid to hydrogen in 50% water. Subsequent investigations with the pentapyridyl ligand PY5Me(2) furnished molybdenum and cobalt complexes capable of catalyzing the reduction of water in fully aqueous electrolyte with 100% Faradaic efficiency. Of particular note, the complex [(PY5Me(2))MoO](2+) possesses extremely high activity and durability in neutral water, with turnover frequencies at least 8500 mol of H-2 per mole of catalyst per hour and turnover numbers over 600 000 mol of H-2 per mole of catalyst over 3 days at an overpotential of 1.0 V, without apparent loss in activity. Replacing the oxo moiety with a disulfide affords [(PY5Me(2))MoS2](2+), which bears a molecular MoS2 triangle that structurally and functionally mimics bulk molybdenum disulfide, improving the catalytic activity for water reduction. In water buffered to pH 3, catalysis by [(PY5Me(2))MoS2](2+) onsets at 400 mV of overpotential, whereas [(PY5Me(2))MoO](2+) requires an additional 300 mV of driving force to operate at the same current density. Metalation of the PY5Me(2) ligand with an appropriate Co(ii) source also furnishes electrocatalysts that are active in water. Importantly, the onset of catalysis by the [(PY5Me(2))Co(H2O)](2+) series is anodically shifted by introducing electron-withdrawing functional groups on the ligand. With the [(bpy2PYMe)Co(CF3SO3)](1+) system, we showed that introducing a redox-active moiety can facilitate the electro- and photochemical reduction of protons from weak acids such as acetic acid or water. Using a high-throughput photochemical reactor, we examined the structure-reactivity relationship of a series of cobalt(ii) complexes. Taken together, these findings set the stage for the broader application of polypyridyl systems to catalysis under environmentally benign aqueous conditions. C1 [Zee, David Z.; Chantarojsiri, Teera; Long, Jeffrey R.; Chang, Christopher J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu; chrischang@berkeley.edu FU DOE/LBNL [101528-002]; Center for Artificial Photosynthesis, a DOE Energy Innovation Hub through Office of Science of the U.S. Department of Energy [DE-SC0004993]; DPST scholarship from Thai government; National Science Foundation FX Our work in sustainable energy catalysis is funded by DOE/LBNL Grant 101528-002 (T.C. and C.J.C.) and the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy award DE-SC0004993 (D.Z.Z. and J.R.L.). T.C. is supported by a DPST scholarship from the Thai government. D.Z.Z. thanks the National Science Foundation for a Graduate Research Fellowship. C.J.C. is an Investigator with the Howard Hughes Medical Institute. NR 71 TC 35 Z9 35 U1 36 U2 160 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JUL PY 2015 VL 48 IS 7 BP 2027 EP 2036 DI 10.1021/acs.accounts.5b00082 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PJ UT WOS:000358556400026 PM 26101803 ER PT J AU Hanson, SK Baker, RT AF Hanson, Susan K. Baker, R. Tom TI Knocking on Wood: Base Metal Complexes as Catalysts for Selective Oxidation of Lignin Models and Extracts SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID AEROBIC ALCOHOL OXIDATION; O BOND-CLEAVAGE; MOLECULAR-OXYGEN ACTIVATION; NITROXYL RADICALS; VANADIUM CATALYST; VERATRYL ALCOHOL; AQUEOUS-MEDIA; IONIC LIQUID; COPPER; MECHANISM AB CONSPECTUS: This work began as part of a biomass conversion catalysis project with UC Santa Barbara funded by the first NSF Chemical Bonding Center, CATSB. Recognizing that catalytic aerobic oxidation of diol C-C bonds could potentially be used to break down lignocellulose, we began to synthesize oxovanadiurn complexes and explore their fundamental reactivity. Of course there were theories regarding the oxidation mechanism, but our mechanistic studies soon revealed a number of surprises of the type that keep all chemists coming back to the bench! We realized that these reactions were also exciting in that they actually used the oxygen-on-every-carbon property of biomass-derived molecules to control the selectivity of the oxidation. When we found that these oxovanadium complexes tended to convert sugars predominantly to formic acid and carbon dioxide, we replaced one of the OH groups with an ether and entered the dark world of lignin chemistry. In this Account, we summarize results from our collaboration and from our individual labs. In particular, we show that oxidation selectivity (C-C vs C-O bond cleavage) of lignin models using air and vanadium complexes depends on the ancillary ligands, the reaction solvent, and the substrate structure (i.e., phenolic vs non-phenolic). Selected vanadium complexes in the presence of added base serve as effective alcohol oxidation catalysts via a novel base-assisted dehydrogenation pathway. In contrast, copper catalysts effect direct C-C bond cleavage of these lignin models, presumably through a radical pathway. The most active vanadium catalyst exhibits unique activity for the depolymerization of organosolv lignin. After Weckhuysen's excellent 2010 review on lignin valorization, the number of catalysis studies and approaches on both lignin models and extracts has expanded rapidly. Today we are seeing new start-ups and lignin production facilities sprouting up across the globe as we all work to prove wrong the old pulp and paper chemist's adage: you can make anything from lignin except money! C1 [Hanson, Susan K.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Baker, R. Tom] Univ Ottawa, Dept Chem, Ottawa, ON K1N 6N5, Canada. [Baker, R. Tom] Univ Ottawa, Ctr Catalysis Res & Innovat, Ottawa, ON K1N 6N5, Canada. RP Hanson, SK (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM skhanson@lanl.gov; rbaker@uottawa.ca FU NSERC Biomaterials and Chemicals strategic research network (Lignoworks); Los Alamos National Laboratory LDRD [20100160ER]; NSF Center for Enabling New Technologies through Catalysis FX R.T.B. thanks the NSERC Biomaterials and Chemicals strategic research network (Lignoworks) for support of this work and the Canada Foundation for Innovation, Ontario Ministry of Economic Development and Innovation, Canada Research Chairs and the University of Ottawa for providing essential infrastructure. S.K.H. thanks Los Alamos National Laboratory LDRD (20100160ER) and the NSF Center for Enabling New Technologies through Catalysis for funding. NR 56 TC 23 Z9 25 U1 28 U2 172 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JUL PY 2015 VL 48 IS 7 BP 2037 EP 2048 DI 10.1021/acs.accounts.5b00104 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PJ UT WOS:000358556400027 PM 26151603 ER PT J AU Stacchiola, DJ AF Stacchiola, Dario J. TI Tuning the Properties of Copper-Based Catalysts Based on Molecular in Situ Studies of Model Systems SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID WATER-GAS SHIFT; SCANNING-TUNNELING-MICROSCOPY; RAY PHOTOELECTRON-SPECTROSCOPY; INFRARED REFLECTION-ABSORPTION; CARBON-MONOXIDE OXIDATION; MIXED-METAL OXIDE; SURFACE SCIENCE; METHANOL SYNTHESIS; REACTION-KINETICS; NANOMETER LEVEL AB Studying catalytic processes at the molecular level is extremely challenging, due to the structural and chemical complexity of the materials used as catalysts and the presence of reactants and products in the reactors environment. The most common materials used on catalysts are transition metals and their oxides. The importance of multifunctional active sites at metal/oxide interfaces has been long recognized, but a molecular picture of them based on experimental observations is only recently emerging. The initial approach to interrogate the surface chemistry of catalysts at the molecular level consisted of studying metal single crystals as models for reactive metal centers, moving later to single crystal or well-defined thin film oxides. The natural next iteration consisted in the deposition of metal nanoparticles on well-defined oxide substrates. Metal nanoparticles contain undercoordinated sites, which are more reactive. It is also possible to create architectures where oxide nanoparticles are deposited on top of metal single crystals, denominated inverse catalysts, leading in this case to a high concentration of reactive cationic sites in direct contact with the underlying fully coordinated metal atoms. Using a second oxide as a support (host), a multifunctional configuration can be built in which both metal and oxide nanoparticles are located in close proximity. Our recent studies on copper-based catalysts are presented here as an example of the application of these complementary model systems, starting from the creation of undercoordinated sites on Cu(111) and Cu2O(111) surfaces, continuing with the formation of mixed-metal copper oxides, the synthesis of ceria nanoparticles on Cu(111) and the codeposition of Cu and ceria nanoparticles on TiO2(110). Catalysts have traditionally been characterized before or after reactions and analyzed based on static representations of surface structures. It is shown here how dynamic changes on a catalysts chemical state and morphology can be followed during a reaction by a combination of in situ microscopy and spectroscopy. In addition to determining the active phase of a catalyst by in situ methods, the presence of weakly adsorbed surface species or intermediates generated only in the presence of reactants can be detected, allowing in turn the comparison of experimental results with first principle modeling of specific reaction mechanisms. Three reactions are used to exemplify the approach: CO oxidation (CO + 1/2O(2) -> CO2), water gas shift reaction (WGSR) (CO + H2O -> CO2 + H-2), and methanol synthesis (CO2 + 3H(2) -> CH3OH + H2O). During CO oxidation, the full conversion of Cu-0 to Cu2+ deactivates an initially outstanding catalyst. This can be remedied by the formation of a TiCuOx mixed-oxide that protects the presence of active partially oxidized Cu+ cations. It is also shown that for the WGSR a switch occurs in the reaction mechanism, going from a redox process on Cu(111) to a more efficient associative pathway at the interface of ceria nanoparticles deposited on Cu(111). Similarly, the activation of CO2 at the ceria/Cu(111) interface allows its facile hydrogenation to methanol. Our combined studies emphasize the need of searching for optimal metal/oxide interfaces, where multifunctional sites can lead to new efficient catalytic reaction pathways. C1 Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Stacchiola, DJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RI Stacchiola, Dario/B-1918-2009 OI Stacchiola, Dario/0000-0001-5494-3205 FU U.S. Department of Energy, Office of Basic Energy Science [DE-SC0012704] FX All the work presented here has been carried out in the framework of the Catalysis group research program at Brookhaven National Laboratory. The author is deeply grateful of the close collaboration with Jose Rodriguez, Ping Liu, Sanjaya Senanayake, and all the students and postdocs from the Catalysis Group, who together with our external collaborators are responsible for the experiments presented here. The work at BNL was financed by the U.S. Department of Energy, Office of Basic Energy Science (DE-SC0012704). NR 42 TC 9 Z9 9 U1 27 U2 136 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JUL PY 2015 VL 48 IS 7 BP 2151 EP 2158 DI 10.1021/acs.accounts.5b00200 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PJ UT WOS:000358556400039 PM 26103058 ER PT J AU Fix, MB Smith, JA Tucker, DL Wester, W Annis, J AF Fix, M. B. Smith, J. A. Tucker, D. L. Wester, W. Annis, J. TI Discovery of a new blue quasar: SDSS J022218.03-062511.1 SO ASTRONOMISCHE NACHRICHTEN LA English DT Article DE quasars: individual: (SDSS J022218.03-062511.1); techniques: spectroscopic ID DIGITAL-SKY-SURVEY; DATA RELEASE; TARGET SELECTION; LUMINOSITY FUNCTION; WHITE-DWARFS; CATALOG; EVOLUTION; GALAXIES; EXPLORER; MISSION AB We report the discovery of a bright blue quasar: SDSS J022218.03-062511.1. This object was discovered spectroscopically while searching for hot white dwarfs that may be used as calibration sources for large sky surveys such as the Dark Energy Survey or the Large Synoptic Survey Telescope project. We present the calibrated spectrum, spectral line shifts and report a redshift of z = 0.521 +/- 0.0015 and a rest-frame g-band luminosity of 8.71x10(11) L-circle dot. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Fix, M. B.; Smith, J. A.] Austin Peay State Univ, Dept Phys & Astron, Clarksville, TN 37044 USA. [Tucker, D. L.; Wester, W.; Annis, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Smith, JA (reprint author), Austin Peay State Univ, Dept Phys & Astron, Clarksville, TN 37044 USA. EM smithj@apsu.edu OI Smith, J. Allyn/0000-0002-6261-4601; Tucker, Douglas/0000-0001-7211-5729 FU Department of Energy Visiting Faculty Program; Fermilab Center for Particle Astrophysics; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; National Aeronautics and Space Administration; NASA [NAS5-98034] FX Partial support for MBF and JAS was provided by the Department of Energy Visiting Faculty Program run by the Department of Energy Office of Science. Additional support came from the Fermilab Center for Particle Astrophysics. Based on observations obtained with the Apache Point Observatory 3.5-meter telescope, which is owned and operated by the Astrophysical Research Consortium. DIStools is used for spectral reductions at Apache Point and was developed by Gordon Richards while at the University of Chicago.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; This publication makes use of data products from the Two Micron All Sky Survey, which is a joint project of the University of Massachusetts and the Infrared Processing and Analysis Center/California Institute of Technology, funded by the National Aeronautics and Space Administration and the National Science Foundation.; This research has made use of the NASA/IPAC Extragalactic Database (NED), which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. This research made use of data from the GALEX mission. GALEX is a NASA small explorer, launched in 2003 April. It is operated for NASA by Caltech under NASA contract NAS5-98034. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory California Institute of Technology, funded by the National Aeronautics and Space Administration. The TOPCAT software package10 was used in much of the plotting and analysis in this work. NR 32 TC 0 Z9 0 U1 0 U2 1 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0004-6337 EI 1521-3994 J9 ASTRON NACHR JI Astro. Nachr. PD JUL PY 2015 VL 336 IS 6 BP 614 EP 618 DI 10.1002/asna.201512173 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CN8TG UT WOS:000358715500009 ER PT J AU Aartsen, MG Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Baker, M Beatty, JJ Tjus, JB Becker, KH BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bos, F Bose, D Boser, S Botner, O Brayeur, L Bretz, HP Brown, AM Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Christy, B Clark, K Classen, L Clevermann, F Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC Dumm, JP Dunkman, M Eagan, R Eberhardt, B Ehrhardt, T Eichmann, B Eisch, J Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Frantzen, K Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Gier, D Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grant, D Gretskov, P Groh, JC Gross, A Ha, C Haack, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Hebecker, D Heereman, D Heinen, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huang, F Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Jacobsen, J Japaridze, GS Jero, K Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Koob, A Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larsen, DT Larson, MJ Lesiak-Bzdak, M Leuermann, M Lunemann, J Madsen, J Maggi, G Mahn, KBM Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Meures, T Miarecki, S Middell, E Middlemas, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Olivas, A Omairat, A O'Murchadha, A Palczewski, T Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Radel, L Rameez, M Rawlins, K Redl, P Rees, I Reimann, R Relich, M Resconi, E Rhode, W Richman, M Riedel, B Robertson, S Rodrigues, JP Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sander, HG Sandroos, J Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Tamburro, A Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S van Eijndhoven, N Vandenbroucke, J van Santen, J Vanheule, S Vehring, M Voge, M Vraeghe, M Walck, C Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zoll, M AF Aartsen, M. G. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Baker, M. Beatty, J. J. Tjus, J. Becker Becker, K. -H. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bos, F. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. -P. Brown, A. M. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Clevermann, F. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. Dumm, J. P. Dunkman, M. Eagan, R. Eberhardt, B. Ehrhardt, T. Eichmann, B. Eisch, J. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Frantzen, K. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Gier, D. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Hebecker, D. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huang, F. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Jacobsen, J. Japaridze, G. S. Jero, K. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larsen, D. T. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Meures, T. Miarecki, S. Middell, E. Middlemas, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Rees, I. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Riedel, B. Robertson, S. Rodrigues, J. P. Rongen, M. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sander, H. -G. Sandroos, J. Santander, M. Sarkar, S. Schatto, K. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Sestayo, Y. Seunarine, S. Shanidze, R. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Tamburro, A. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Vandenbroucke, J. van Santen, J. Vanheule, S. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallraff, M. Weaver, Ch. Wellons, M. Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zoll, M. CA IceCube Collaboration TI SEARCHES FOR TIME-DEPENDENT NEUTRINO SOURCES WITH ICECUBE DATA FROM 2008 TO 2012 SO ASTROPHYSICAL JOURNAL LA English DT Article DE astroparticle physics; binaries: general; BL Lacertae objects: general; galaxies: active; neutrinos; X-rays: binaries ID GAMMA-RAY EMISSION; ACTIVE GALACTIC NUCLEI; LS I+61-DEGREES-303; PROTON BLAZAR; LAC OBJECTS; COSMIC-RAYS; ACCELERATION; TEV; MODEL; 1ES-1959+650 AB In this paper searches for flaring astrophysical neutrino sources and sources with periodic emission with the IceCube neutrino telescope are presented. In contrast to time-integrated searches, where steady emission is assumed, the analyses presented here look for a time-dependent signal of neutrinos using the information from the neutrino arrival times to enhance the discovery potential. A search was performed for correlations between neutrino arrival times and directions, as well as neutrino emission following time-dependent light curves, sporadic emission, or periodicities of candidate sources. These include active galactic nuclei, soft gamma-ray repeaters, supernova remnants hosting pulsars, microquasars, and X-ray binaries. The work presented here updates and extends previously published results to a longer period that covers 4 years. of data from 2008 April 5 to 2012 May 16, including the first year of operation of the completed 86 string detector. The analyses did not find any significant time-dependent point sources of neutrinos, and the results were used to set upper limits on the neutrino flux from source candidates. C1 [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Whelan, B. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Kowalski, M.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N. L.; Terliuk, A.; Usner, M.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Adams, J.; Brown, A. M.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Aguilar, J. A.; Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Ahlers, M.; Arguelles, C.; Baker, M.; BenZvi, S.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Larsen, D. T.; McNally, F.; Middlemas, E.; Morse, R.; Rees, I.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; Baker, M.; BenZvi, S.; Chirkin, D.; Christov, A.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Larsen, D. T.; McNally, F.; Middlemas, E.; Morse, R.; Rees, I.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Ahrens, M.; Bohm, C.; Christov, A.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Ahrens, M.; Bohm, C.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Altmann, D.; Classen, L.; Kappes, A.; Tselengidou, M.] Univ Erlangen Nurnberg, Erlangen Ctr Astroparticle Phys, D-91058 Erlangen, Germany. [Anderson, T.; Arlen, T. C.; Christov, A.; Cowen, D. F.; Dunkman, M.; Eagan, R.; Groh, J. C.; Huang, F.; Keivani, A.; Lanfranchi, J. L.; Quinnan, M.; Smith, M. W. E.; Stanisha, N. A.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Archinger, M.; Baum, V.; Boeser, S.; Christov, A.; Eberhardt, B.; Ehrhardt, T.; Keivani, A.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Christov, A.; Gier, D.; Gretskov, P.; Haack, C.; Hallen, P.; Heinen, D.; Hellwig, D.; Keivani, A.; Koob, A.; Leuermann, M.; Paul, L.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schoenen, S.; Schukraft, A.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Inst Phys, D-52056 Aachen, Germany. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Christov, A.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Tjus, J. Becker; Bos, F.; Eichmann, B.; Fedynitch, A.; Kroll, M.; Saba, S. M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Becker, K. -H.; Bindig, D.; Christov, A.; Fischer-Wasels, T.; Helbing, K.; Hickford, S.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.] Univ Gesamthsch Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Berley, D.; Blaufuss, E.; Cheung, E.; Christov, A.; Christy, B.; Felde, J.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Keivani, A.; Maunu, R.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Bernhard, A.; Christov, A.; Coenders, S.; Gross, A.; Jurkovic, M.; Keivani, A.; Krings, K.; Olivas, A.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85748 Garching, Germany. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Boersma, D. J.; Botner, O.; Euler, S.; Hallgren, A.; Strom, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Bose, D.; In, S.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; de Wasseige, G.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Buzinsky, N.; Grant, D.; Kopper, C.; Nowicki, S. C.; Riedel, B.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [Clark, K.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [de Andre, J. P. A. M.; DeYoung, T.; Hignight, J.; Mahn, K. B. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Koskinen, D. J.; Larson, M. J.; Medici, M.; Sandroos, J.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Kurahashi, N.; Meures, T.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Aartsen, MG (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. RI Maruyama, Reina/A-1064-2013; Koskinen, David/G-3236-2014; Tjus, Julia/G-8145-2012; Beatty, James/D-9310-2011; Sarkar, Subir/G-5978-2011; Wiebusch, Christopher/G-6490-2012; OI Dembinski, Hans/0000-0003-3337-3850; Arguelles Delgado, Carlos/0000-0003-4186-4182; Maruyama, Reina/0000-0003-2794-512X; Koskinen, David/0000-0002-0514-5917; Beatty, James/0000-0003-0481-4952; Sarkar, Subir/0000-0002-3542-858X; Wiebusch, Christopher/0000-0002-6418-3008; Schukraft, Anne/0000-0002-9112-5479; Groh, John/0000-0001-9880-3634; Larsen, Dag Toppe/0000-0002-9898-2174; Perez de los Heros, Carlos/0000-0002-2084-5866; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Strotjohann, Nora Linn/0000-0002-4667-6730 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; WestGrid and Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 63 TC 6 Z9 6 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 46 DI 10.1088/0004-637X/807/1/46 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200046 ER PT J AU An, HJ Archibald, RF Hascoet, R Kaspi, VM Beloborodov, AM Archibald, AM Beardmore, A Boggs, SE Christensen, FE Craig, WW Gehrels, N Hailey, CJ Harrison, FA Kennea, J Kouveliotou, C Stern, D Younes, G Zhang, WW AF An, Hongjun Archibald, Robert F. Hascoet, Romain Kaspi, Victoria M. Beloborodov, Andrei M. Archibald, Anne M. Beardmore, Andy Boggs, Steven E. Christensen, Finn E. Craig, William W. Gehrels, Niel Hailey, Charles J. Harrison, Fiona A. Kennea, Jamie Kouveliotou, Chryssa Stern, Daniel Younes, George Zhang, William W. TI DEEP NuSTAR AND SWIFT MONITORING OBSERVATIONS OF THE MAGNETAR 1E 1841-045 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: individual (1E 1841-045); stars: magnetars; stars: neutron; X-rays: bursts ID X-RAY PULSARS; SOFT GAMMA-REPEATERS; NEUTRON-STARS; KES 73; 4U 0142+61; SPIN-DOWN; EMISSION; BURSTS; OUTBURST; RXTE AB We report on a 350 ks NuSTAR observation of the magnetar 1E 1841-045 taken in 2013 September. During the observation, NuSTAR detected six bursts of short duration, with T-90 less than or similar to 1 s. An elevated level of emission tail is detected after the brightest burst, persisting for similar to 1 ks. The emission showed a power-law decay with a temporal index of 0.5 before returning to the persistent emission level. The long observation also provided detailed phase-resolved spectra of the persistent X-ray emission of the source. By comparing the persistent spectrum with that previously reported, we find that the source hard-band emission has been stable for over approximately 10 yr. The persistent hard-X-ray emission is well fitted by a coronal outflow model, where e(+/-) pairs in the magnetosphere upscatter thermal X-rays. Our fit of phase-resolved spectra allowed us to estimate the angle between the rotational and magnetic dipole axes of the magnetar, alpha(mag) = 0.25, the twisted magnetic flux, 2.5 x 10(26) G cm(2), and the power released in the twisted magnetosphere, L-j = 6 x 10(36) erg s(-1). Assuming this model for the hard-X-ray spectrum, the soft-X-ray component is well fit by a two-blackbody model, with the hotter blackbody consistent with the footprint of the twisted magnetic field lines on the star. We also report on the 3 yr. Swift monitoring observations obtained since 2011 July. The soft-X-ray spectrum remained stable during this period, and the timing behavior was noisy, with large timing residuals. C1 [An, Hongjun; Archibald, Robert F.; Kaspi, Victoria M.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [An, Hongjun] Stanford Univ, Dept Phys, KIPAC, Stanford, CA 94305 USA. [Hascoet, Romain; Beloborodov, Andrei M.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Archibald, Anne M.] ASTRON, Netherlands Inst Radio Astron, NL-7990 AA Dwingeloo, Netherlands. [Beardmore, Andy] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gehrels, Niel] NASA, Astrophys Sci Div, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Harrison, Fiona A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Kennea, Jamie] Penn State Univ, Dept Astron & Astrophys, Lab 525, University Pk, PA 16802 USA. [Kouveliotou, Chryssa; Younes, George] NASA, Space Sci Off, Marshall Space Flight Ctr, Huntsville, AL 35812 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP An, HJ (reprint author), McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; An, Hongjun/0000-0002-6389-9012; Archibald, Anne/0000-0003-0638-3340; Archibald, Robert/0000-0002-4017-8837 FU NASA [NNG08FD60C, NAS5-00147, NNX13AI34G]; National Aeronautics and Space Administration; Kavli Institute for Particle Astrophysics and Cosmology; NSERC; FQRNT Centre de Recherche Astrophysique du Quebec; R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Research (CIFAR); Canada Research Chairs Program; Lorne Trottier Chair in Astrophysics and Cosmology FX This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). H.A. acknowledges support provided by the NASA sponsored Fermi Contract NAS5-00147 and by Kavli Institute for Particle Astrophysics and Cosmology. V.M.K. acknowledges support from an NSERC Discovery Grant and Accelerator Supplement, the FQRNT Centre de Recherche Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Research (CIFAR), the Canada Research Chairs Program, and the Lorne Trottier Chair in Astrophysics and Cosmology. A.M.B. acknowledges the support by NASA grant NNX13AI34G. NR 57 TC 6 Z9 6 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 93 DI 10.1088/0004-637X/807/1/93 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200093 ER PT J AU Bechtol, K Drlica-Wagner, A Balbinot, E Pieres, A Simon, JD Yanny, B Santiago, B Wechsler, RH Frieman, J Walker, AR Williams, P Rozo, E Rykoff, ES Queiroz, A Luque, E Benoit-Levy, A Tucker, D Sevilla, I Gruendl, RA da Costa, LN Neto, AF Maia, MAG Abbott, T Allam, S Armstrong, R Bauer, AH Bernstein, GM Bernstein, RA Bertin, E Brooks, D Buckley-Geer, E Burke, DL Rosell, AC Castander, FJ Covarrubias, R D'Andrea, CB DePoy, DL Desai, S Diehl, HT Eifler, TF Estrada, J Evrard, AE Fernandez, E Finley, DA Flaugher, B Gaztanaga, E Gerdes, D Girardi, L Gladders, M Gruen, D Gutierrez, G Hao, J Honscheid, K Jain, B James, D Kent, S Kron, R Kuehn, K Kuropatkin, N Lahav, O Li, TS Lin, H Makler, M March, M Marshall, J Martini, P Merritt, KW Miller, C Miquel, R Mohr, J Neilsen, E Nichol, R Nord, B Ogando, R Peoples, J Petravick, D Plazas, AA Romer, AK Roodman, A Sako, M Sanchez, E Scarpine, V Schubnell, M Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Wester, W Zuntz, J AF Bechtol, K. Drlica-Wagner, A. Balbinot, E. Pieres, A. Simon, J. D. Yanny, B. Santiago, B. Wechsler, R. H. Frieman, J. Walker, A. R. Williams, P. Rozo, E. Rykoff, E. S. Queiroz, A. Luque, E. Benoit-Levy, A. Tucker, D. Sevilla, I. Gruendl, R. A. da Costa, L. N. Fausti Neto, A. Maia, M. A. G. Abbott, T. Allam, S. Armstrong, R. Bauer, A. H. Bernstein, G. M. Bernstein, R. A. Bertin, E. Brooks, D. Buckley-Geer, E. Burke, D. L. Carnero Rosell, A. Castander, F. J. Covarrubias, R. D'Andrea, C. B. DePoy, D. L. Desai, S. Diehl, H. T. Eifler, T. F. Estrada, J. Evrard, A. E. Fernandez, E. Finley, D. A. Flaugher, B. Gaztanaga, E. Gerdes, D. Girardi, L. Gladders, M. Gruen, D. Gutierrez, G. Hao, J. Honscheid, K. Jain, B. James, D. Kent, S. Kron, R. Kuehn, K. Kuropatkin, N. Lahav, O. Li, T. S. Lin, H. Makler, M. March, M. Marshall, J. Martini, P. Merritt, K. W. Miller, C. Miquel, R. Mohr, J. Neilsen, E. Nichol, R. Nord, B. Ogando, R. Peoples, J. Petravick, D. Plazas, A. A. Romer, A. K. Roodman, A. Sako, M. Sanchez, E. Scarpine, V. Schubnell, M. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Wester, W. Zuntz, J. CA DES Collaboration TI EIGHT NEW MILKY WAY COMPANIONS DISCOVERED IN FIRST-YEAR DARK ENERGY SURVEY DATA SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: dwarf; Local Group ID DWARF SPHEROIDAL GALAXIES; ULTRA-FAINT SATELLITES; STAR-FORMATION HISTORY; DIGITAL SKY SURVEY; GLOBULAR-CLUSTERS; LOCAL GROUP; URSA-MAJOR; STRUCTURAL-PROPERTIES; SPECTROSCOPIC SURVEY; STELLAR POPULATIONS AB We report the discovery of eight new Milky Way companions in similar to 1800 deg(2) of optical imaging data collected during the first year of the Dark Energy Survey (DES). Each system is identified as a statistically significant over-density of individual stars consistent with the expected isochrone and luminosity function of an old and metal-poor stellar population. The objects span a wide range of absolute magnitudes (M-V from -2.2 to -7.4 mag), physical sizes (10-170 pc), and heliocentric distances (30-330 kpc). Based on the low surface brightnesses, large physical sizes, and/or large Galactocentric distances of these objects, several are likely to be new ultra-faint satellite galaxies of the Milky Way and/or Magellanic Clouds. We introduce a likelihood-based algorithm to search for and characterize stellar over-densities, as well as identify stars with high satellite membership probabilities. We also present completeness estimates for detecting ultra-faint galaxies of varying luminosities, sizes, and heliocentric distances in the first-year DES data. C1 [Bechtol, K.; Frieman, J.; Williams, P.; Gladders, M.; Kron, R.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Drlica-Wagner, A.; Yanny, B.; Frieman, J.; Tucker, D.; Allam, S.; Buckley-Geer, E.; Diehl, H. T.; Estrada, J.; Finley, D. A.; Flaugher, B.; Gutierrez, G.; Hao, J.; Kent, S.; Kuropatkin, N.; Lin, H.; Merritt, K. W.; Neilsen, E.; Nord, B.; Peoples, J.; Scarpine, V.; Soares-Santos, M.; Sobreira, F.; Wester, W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Balbinot, E.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Balbinot, E.; Pieres, A.; Santiago, B.; Queiroz, A.; Luque, E.; da Costa, L. N.; Fausti Neto, A.; Maia, M. A. G.; Carnero Rosell, A.; Ogando, R.; Sobreira, F.] Lab Interinst eAstron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Pieres, A.; Santiago, B.; Queiroz, A.; Luque, E.] Univ Fed Rio Grande do Sul, Inst Fis, BR-91501970 Porto Alegre, RS, Brazil. [Simon, J. D.; Bernstein, R. A.] Carnegie Observ, Pasadena, CA 91101 USA. [Wechsler, R. H.; Roodman, A.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Wechsler, R. H.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Wechsler, R. H.; Rozo, E.; Rykoff, E. S.; Burke, D. L.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Walker, A. R.; Abbott, T.; James, D.; Roodman, A.; Smith, R. C.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, La Serena, Chile. [Rozo, E.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Benoit-Levy, A.; Brooks, D.; Lahav, O.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Sevilla, I.; Gruendl, R. A.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Sevilla, I.; Sanchez, E.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Gruendl, R. A.; Covarrubias, R.; Petravick, D.; Swanson, M. E. C.] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [da Costa, L. N.; Maia, M. A. G.; Carnero Rosell, A.; Girardi, L.; Ogando, R.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Allam, S.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Armstrong, R.; Bernstein, G. M.; Eifler, T. F.; Jain, B.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bauer, A. H.; Castander, F. J.; Gaztanaga, E.] Fac Ciencies, IEEC CSIC, Inst Ciencies Espai, E-08193 Bellaterra, Barcelona, Spain. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Bertin, E.] Inst Astrophys Paris, CNRS, UMR 7095, F-75014 Paris, France. [D'Andrea, C. B.; Nichol, R.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [DePoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Mohr, J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Desai, S.] Excellence Cluster Universe, D-85748 Garching, Germany. [Eifler, T. F.; Plazas, A. A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Evrard, A. E.; Gerdes, D.; Miller, C.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Fernandez, E.; Gladders, M.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Fernandez, E.; Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Gruen, D.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Honscheid, K.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Honscheid, K.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Kuehn, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Makler, M.] Ctr Brasileiro Pesquisas Fis, ICRA, BR-22290180 Rio De Janeiro, RJ, Brazil. [Martini, P.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Miller, C.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Plazas, A. A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Romer, A. K.] Univ Sussex, Ctr Astron, Brighton BN1 9QH, E Sussex, England. [Thaler, J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Oxford M13 9PL, England. RP Bechtol, K (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. EM bechtol@kicp.uchicago.edu; kadrlica@fnal.gov RI Ogando, Ricardo/A-1747-2010; Makler, Martin/G-2639-2012; Sanchez, Eusebio/H-5228-2015; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Gaztanaga, Enrique/L-4894-2014; Balbinot, Eduardo/E-8019-2015; OI Ogando, Ricardo/0000-0003-2120-1154; Makler, Martin/0000-0003-2206-2651; Sanchez, Eusebio/0000-0002-9646-8198; Sobreira, Flavia/0000-0002-7822-0658; Fernandez, Enrique/0000-0002-6405-9488; Gaztanaga, Enrique/0000-0001-9632-0815; Balbinot, Eduardo/0000-0002-1322-3153; Suchyta, Eric/0000-0002-7047-9358; Tucker, Douglas/0000-0001-7211-5729 FU National Science Foundation [1138766, AST-1138766]; PAPDRJ CAPES/FAPERJ Fellowship; DOE grant [DE-AC02-98CH10886]; JPL; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Union; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; University of Edinburgh; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Ludwig-Maximilians Universitat Munchen; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory, Stanford University; University of Sussex; Texas AM University; Lawrence Berkeley National Laboratory FX We thank Sergey Koposov and collaborators for sending a copy of their submitted paper with their nine discoveries, and Helmut Jerjen for pointing out the association between Kim 2 and DES J2108.8-5109. Marla Geha provided useful comments on the presentation of these results. K.B. and A.D.W. thank Beth Willman for advice regarding the search for ultra-faint galaxies. A.D.W. thanks Ellen Bechtol for her generous hospitality during the preparation of this manuscript. We acknowledge helpful suggestions from the anonymous referee. This work made use of computational resources at the SLAC National Accelerator Laboratory and University of Chicago Research Computing Center. This material is based upon work supported by the National Science Foundation under Grant Number (1138766). A.C.R. acknowledges financial support provided by the PAPDRJ CAPES/FAPERJ Fellowship. A.A.P. was supported by DOE grant DE-AC02-98CH10886 and by JPL, run by Caltech under a contract for NASA. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. NR 102 TC 108 Z9 108 U1 3 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 50 DI 10.1088/0004-637X/807/1/50 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200050 ER PT J AU Fu, W Lubow, SH Martin, RG AF Fu, Wen Lubow, Stephen H. Martin, Rebecca G. TI THE KOZAI-LIDOV MECHANISM IN HYDRODYNAMICAL DISKS. II. EFFECTS OF BINARY AND DISK PARAMETERS SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; binaries: general; hydrodynamics; planets and satellites: formation ID HIERARCHICAL 3-BODY SYSTEMS; SUPERMASSIVE BLACK-HOLES; ECCENTRIC ASTROPHYSICAL DISCS; DIFFERENTIALLY ROTATING-DISKS; WARPED ACCRETION DISCS; X-RAY BINARIES; 16 CYGNI B; PLANETARY ORBITS; STELLAR SPIN; STAR SYSTEMS AB Martin et al. showed that a substantially misaligned accretion disk around one component of a binary system can undergo global damped Kozai-Lidov (KL) oscillations. During these oscillations, the inclination and eccentricity of the disk are periodically exchanged. However, the robustness of this mechanism and its dependence on the system parameters were unexplored. In this paper, we use three-dimensional hydrodynamical simulations to analyze how various binary and disk parameters affect the KL mechanism in hydrodynamical disks. The simulations include the effect of gas pressure and viscosity, but ignore the effects of disk self-gravity. We describe results for different numerical resolutions, binary mass ratios and orbital eccentricities, initial disk sizes, initial disk surface density profiles, disk sound speeds, and disk viscosities. We show that the KL mechanism can operate for a wide range of binary-disk parameters. We discuss the applications of our results to astrophysical disks in various accreting systems. C1 [Fu, Wen] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Fu, Wen] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lubow, Stephen H.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Martin, Rebecca G.] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. RP Fu, W (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM wf5@rice.edu FU NASA [NNX11AK61G]; institutional computing program at Los Alamos National Laboratory FX W.F. and S.H.L. acknowledge support from NASA grant NNX11AK61G. Computing resources supporting this work were provided by the institutional computing program at Los Alamos National Laboratory. We thank Daniel Price for providing the PHANTOM code for SPH simulations and SPLASH code (Price 2007) for data analysis and the rendering of figures. NR 81 TC 6 Z9 6 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 75 DI 10.1088/0004-637X/807/1/75 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200075 ER PT J AU Gelfand, JD Slane, PO Temim, T AF Gelfand, Joseph D. Slane, Patrick O. Temim, Tea TI THE PROPERTIES OF THE PROGENITOR SUPERNOVA, PULSAR WIND, AND NEUTRON STAR INSIDE PWN G54.1+0.3 SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: individual objects (PWN G54.1+0.3); ISM: supernova remnants; pulsars: individual (PSR J1930+1852); X-rays: individual (PWN G54.1+0.3) ID RELATIVISTIC COLLISIONLESS SHOCKS; PAIR PRODUCTION MULTIPLICITIES; GALACTIC ABUNDANCE GRADIENT; REMNANT G54.1+0.3; NEBULA G54.1+0.3; CRAB-NEBULA; SPECTRAL EVOLUTION; ACCRETION SHOCK; RADIO-EMISSION; SIGMA-PROBLEM AB The evolution of a pulsar wind nebula (PWN) inside a supernova remnant (SNR) is sensitive to the properties of the central neutron star, pulsar wind, progenitor supernova, and interstellar medium. These properties are both difficult to measure directly and critical for understanding the formation of neutron stars and their interaction with the surrounding medium. In this paper, we determine these properties for PWN G54.1+0.3 by fitting its observed properties with a model for the dynamical and radiative evolution of a PWN inside an SNR. Our modeling suggests that the progenitor of G54.1+0.3 was an isolated similar to 15-20 M-circle dot star which exploded inside a massive star cluster, creating a neutron star initially spinning with a period of P-0 similar to 30-80 ms. We also find that greater than or similar to 99.9% of the pulsar's rotational energy is injected into the PWN as relativistic electrons and positrons whose energy spectrum is well characterized by a broken power law. Finally, we propose future observations which can both test the validity of this model and better determine the properties of this source-in particular, its distance and the initial spin period of the central pulsar. C1 [Gelfand, Joseph D.] NYU Abu Dhabi, New York, NY 10276 USA. [Slane, Patrick O.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Temim, Tea] NASA, Goddard Space Flight Ctr, Observat Cosmol Lab, Greenbelt, MD 20771 USA. [Gelfand, Joseph D.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [Temim, Tea] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. RP Gelfand, JD (reprint author), NYU Abu Dhabi, POB 903, New York, NY 10276 USA. EM jg168@nyu.edu OI Gelfand, Joseph/0000-0003-4679-1058; Temim, Tea/0000-0001-7380-3144 FU NASA [RSA 1479542] FX Support for this work was provided by NASA through an award issued by JPL/Caltech (RSA 1479542). J.D.G. will like to thank Erin Sheldon for the IDL code used in the MCMC fits, Kaisey Mandel and David Hogg for useful discussions concerning MCMC fitting, Ester Aliu for information regarding the GeV spectrum, and Roger Chevalier, Vikram Dwarkadas, Daniel Patnaude, and Lorenzo Sironi for useful advice. NR 56 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 30 DI 10.1088/0004-637X/807/1/30 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200030 ER PT J AU Hayashida, M Nalewajko, K Madejski, GM Sikora, M Itoh, R Ajello, M Blandford, RD Buson, S Chiang, J Fukazawa, Y Furniss, AK Urry, CM Hasan, I Harrison, FA Alexander, DM Balokovic, M Barret, D Boggs, SE Christensen, FE Craig, WW Forster, K Giommi, P Grefenstette, B Hailey, C Hornstrup, A Kitaguchi, T Koglin, JE Madsen, KK Mao, PH Miyasaka, H Mori, K Perri, M Pivovaroff, MJ Puccetti, S Rana, V Stern, D Tagliaferri, G Westergaard, NJ Zhang, WW Zoglauer, A Gurwell, MA Uemura, M Akitaya, H Kawabata, KS Kawaguchi, K Kanda, Y Moritani, Y Takaki, K Ui, T Yoshida, M Agarwal, A Gupta, AC AF Hayashida, M. Nalewajko, K. Madejski, G. M. Sikora, M. Itoh, R. Ajello, M. Blandford, R. D. Buson, S. Chiang, J. Fukazawa, Y. Furniss, A. K. Urry, C. M. Hasan, I. Harrison, F. A. Alexander, D. M. Balokovic, M. Barret, D. Boggs, S. E. Christensen, F. E. Craig, W. W. Forster, K. Giommi, P. Grefenstette, B. Hailey, C. Hornstrup, A. Kitaguchi, T. Koglin, J. E. Madsen, K. K. Mao, P. H. Miyasaka, H. Mori, K. Perri, M. Pivovaroff, M. J. Puccetti, S. Rana, V. Stern, D. Tagliaferri, G. Westergaard, N. J. Zhang, W. W. Zoglauer, A. Gurwell, M. A. Uemura, M. Akitaya, H. Kawabata, K. S. Kawaguchi, K. Kanda, Y. Moritani, Y. Takaki, K. Ui, T. Yoshida, M. Agarwal, A. Gupta, A. C. TI RAPID VARIABILITY OF BLAZAR 3C 279 DURING FLARING STATES IN 2013-2014 WITH JOINT FERMI-LAT, NuSTAR, SWIFT, AND GROUND-BASED MULTI-WAVELENGTH OBSERVATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: jets; gamma rays: galaxies; quasars: individual (3C 279); radiation mechanisms: non-thermal; X-rays: galaxies ID ACTIVE GALACTIC NUCLEI; LARGE-AREA TELESCOPE; EXTRAGALACTIC RADIO-SOURCES; ENERGY GAMMA-RADIATION; LUMINOUS BLAZARS; PKS 1510-089; MAGNETIC RECONNECTION; RELATIVISTIC JET; BRIGHT BLAZARS; QUASAR 3C-279 AB We report the results of a multiband observing campaign on the famous blazar 3C 279 conducted during a phase of increased activity from 2013 December to 2014 April, including first observations of it with NuSTAR. The gamma-ray emission of the source measured by Fermi-LAT showed multiple distinct flares reaching the highest flux level measured in this object since the beginning of the Fermi mission, with F(E > 100 MeV) of 10(-5) photons cm(-2) s(-1), and with a flux-doubling time scale as short as 2 hr. The gamma-ray spectrum during one of the flares was very hard, with an index of Gamma(gamma) = 1.7 +/- 0.1, which is rarely seen in flat-spectrum radio quasars. The lack of concurrent optical variability implies a very high Compton dominance parameter L-gamma/L-syn > 300. Two 1 day NuSTAR observations with accompanying Swift pointings were separated by 2 weeks, probing different levels of source activity. While the 0.5 - 70 keV X-ray spectrum obtained during the first pointing, and fitted jointly with Swift-XRT is well-described by a simple power law, the second joint observation showed an unusual spectral structure: the spectrum softens by Delta Gamma(X) similar or equal to 0.4 at similar to 4 keV. Modeling the broadband spectral energy distribution during this flare with the standard synchrotron plus inverse-Compton model requires: (1) the location of the gamma-ray emitting region is comparable with the broad-line region radius, (2) a very hard electron energy distribution index p similar or equal to 1, (3) total jet power significantly exceeding the accretion-disk luminosity L-j/L-d greater than or similar to 10, and (4) extremely low jet magnetization with L-B/L-j less than or similar to 10(-4). We also find that single-zone models that match the observed gamma-ray and optical spectra cannot satisfactorily explain the production of X-ray emission. C1 [Hayashida, M.] Univ Tokyo, Inst Cosm Ray Res, Kashiwa, Chiba 2778582, Japan. [Nalewajko, K.; Madejski, G. M.; Blandford, R. D.; Chiang, J.; Furniss, A. K.; Koglin, J. E.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Dept Phys, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Nalewajko, K.; Madejski, G. M.; Blandford, R. D.; Chiang, J.; Furniss, A. K.; Koglin, J. E.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Sikora, M.] Nicolaus Copernicus Astron Ctr, PL-00716 Warsaw, Poland. [Itoh, R.; Fukazawa, Y.; Kawaguchi, K.; Kanda, Y.; Takaki, K.; Ui, T.] Hiroshima Univ, Dept Phys Sci, Higashihiroshima, Hiroshima 7398526, Japan. [Ajello, M.] Clemson Univ, Dept Phys & Astron, Kinard Lab Phys, Clemson, SC 29634 USA. [Buson, S.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Buson, S.] Univ Padua, Dipartimento Fis & Astron G Galilei, I-35131 Padua, Italy. [Urry, C. M.; Hasan, I.] Yale Univ, Yale Ctr Astron & Astrophys, Dept Phys, New Haven, CT 06520 USA. [Harrison, F. A.; Balokovic, M.; Forster, K.; Grefenstette, B.; Madsen, K. K.; Mao, P. H.; Miyasaka, H.; Rana, V.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Alexander, D. M.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Barret, D.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Barret, D.; Craig, W. W.] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Boggs, S. E.; Zoglauer, A.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.; Hornstrup, A.; Westergaard, N. J.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, W. W.; Pivovaroff, M. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Giommi, P.; Perri, M.; Puccetti, S.] ASI Sci Data Ctr, D-52425 Rome, Italy. [Hailey, C.; Mori, K.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Kitaguchi, T.] Hiroshima Univ, Grad Sch Sci, Core Res Energet Universe, Higashihiroshima, Hiroshima 7398526, Japan. [Perri, M.; Puccetti, S.] INAF, Osservatorio Astron Roma, I-00040 Monte Porzio Catone, Italy. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Tagliaferri, G.] INAF, Osservatorio Astron Brera, I-23807 Merate, Italy. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Gurwell, M. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Uemura, M.; Akitaya, H.; Kawabata, K. S.; Moritani, Y.; Yoshida, M.] Hiroshima Univ, Hiroshima Astrophys Sci Ctr, Higashihiroshima, Hiroshima 7398526, Japan. [Agarwal, A.; Gupta, A. C.] Aryabhatta Res Inst Observat Sci ARIES, Naini Tal 263002, India. RP Hayashida, M (reprint author), Univ Tokyo, Inst Cosm Ray Res, 5-1-5 Kashiwanoha, Kashiwa, Chiba 2778582, Japan. EM mahaya@icrr.u-tokyo.ac.jp; knalew@stanford.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Perri, Matteo/0000-0003-3613-4409; giommi, paolo/0000-0002-2265-5003; Puccetti, Simonetta/0000-0002-2734-7835; Rana, Vikram/0000-0003-1703-8796; Urry, Meg/0000-0002-0745-9792; Ajello, Marco/0000-0002-6584-1703 FU NASA [NNG08FD60C, NAS8-03060]; NASA through Einstein Postdoctoral Fellowship - Chandra X-ray Center [PF3-140130]; NASA Headquarters under the NASA earth and Space Science Fellowship Program [NNX14AQ07H]; Smithsonian Institution; Academia Sinica FX This work was partially supported under the NASA contract no. NNG08FD60C, and made use of observations from the NuSTAR mission, a project led by California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. We thank the NuSTAR Operations, Software, and Calibration teams for support of the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This research has made use of the XRT Data Analysis Software (XRTDAS) developed under the responsibility of the ASI Science Data Center (ASDC), Italy. The Submillimeter Array is a joint project between the Smithsonian Astrophysical Observatory and the Academia Sinica Institute of Astronomy and Astrophysics and is funded by the Smithsonian Institution and the Academia Sinica.; K.N. was supported by NASA through Einstein Postdoctoral Fellowship grant number PF3-140130 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. M.B. acknowledges support from NASA Headquarters under the NASA earth and Space Science Fellowship Program, grant NNX14AQ07H. NR 81 TC 33 Z9 33 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 79 DI 10.1088/0004-637X/807/1/79 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200079 ER PT J AU Law, CJ Bower, GC Burke-Spolaor, S Butler, B Lawrence, E Lazio, TJW Mattmann, CA Rupen, M Siemion, A VanderWiel, S AF Law, Casey J. Bower, Geoffrey C. Burke-Spolaor, Sarah Butler, Bryan Lawrence, Earl Lazio, T. Joseph W. Mattmann, Chris A. Rupen, Michael Siemion, Andrew VanderWiel, Scott TI A MILLISECOND INTERFEROMETRIC SEARCH FOR FAST RADIO BURSTS WITH THE VERY LARGE ARRAY SO ASTROPHYSICAL JOURNAL LA English DT Article DE instrumentation: interferometers; intergalactic medium; pulsars: general; radio continuum: general; surveys ID GAMMA-RAY BURSTS; COSMOLOGICAL DISTANCES; TRANSIENT DETECTION; MISSING BARYONS; PULSAR SURVEY; SCINTILLATION; DISCOVERIES; REDSHIFT; MERGERS AB We report on the first millisecond timescale radio interferometric search for the new class of transient known as fast radio bursts (FRBs). We used the Very Large Array (VLA) for a 166 hr, millisecond imaging campaign to detect and precisely localize an FRB. We observed at 1.4 GHz and produced visibilities with 5 ms time resolution over 256 MHz of bandwidth. Dedispersed images were searched for transients with dispersion measures from 0 to 3000 pc cm(-3). No transients were detected in observations of high Galactic latitude fields taken from 2013 September though 2014 October. Observations of a known pulsar show that images typically had a thermal-noise limited sensitivity of 120 mJy beam(-1) (8 sigma; Stokes I) in 5 ms and could detect and localize transients over a wide field of view. Our nondetection limits the FRB rate to less than 7 x 10(4) sky(-1) day(-1) (95% confidence) above a fluence limit of 1.5 Jy ms. The VLA rate limit is consistent with past estimates when published flux limits are recalculated with a homogeneous definition that includes effects of primary beam attenuation, dispersion, pulse width, and sky brightness. This calculation revises the FRB rate downward by a factor of 2, giving the VLA observations a roughly 50% chance of detecting a typical FRB, assuming a pulse width of 3 ms. A 95% confidence constraint would require 600 hr of similar VLA observing. Our survey also limits the repetition rate of an FRB to 2 times less than any known repeating millisecond radio transient. C1 [Law, Casey J.; Siemion, Andrew] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Law, Casey J.; Siemion, Andrew] Univ Calif Berkeley, Radio Astron Lab, Berkeley, CA 94720 USA. [Bower, Geoffrey C.] Acad Sinica, Inst Astron & Astrophys, Hilo, HI 96720 USA. [Burke-Spolaor, Sarah; Lazio, T. Joseph W.; Mattmann, Chris A.] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. [Burke-Spolaor, Sarah; Butler, Bryan] Natl Radio Astron Observ, Socorro, NM 87801 USA. [Lawrence, Earl; VanderWiel, Scott] Los Alamos Natl Lab, Los Alamos, NM USA. [Rupen, Michael] NRC Herzberg, Penticton, BC, Canada. RP Law, CJ (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. OI Law, Casey/0000-0002-4119-9963 FU University of California Office of the President under Lab Fees Research Program Award [237863]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the VLA staff, particularly Martin Pokorny, Ken Sowinski, Vivek Dhawan, James Robnett, and Joan Wrobel, for working tirelessly to support this challenging observing mode. Peter Williams contributed with wide-ranging Python expertise. This project was supported by the University of California Office of the President under Lab Fees Research Program Award 237863. The National Radio Astronomy Observatory is a facility of the National Science Foundation operated under cooperative agreement by Associated Universities, Inc. Part of this research was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 43 TC 23 Z9 23 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 16 DI 10.1088/0004-637X/807/1/16 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200016 ER PT J AU Ryan, BR Dolence, JC Gammie, CF AF Ryan, B. R. Dolence, J. C. Gammie, C. F. TI bhlight: GENERAL RELATIVISTIC RADIATION MAGNETOHYDRODYNAMICS WITH MONTE CARLO TRANSPORT SO ASTROPHYSICAL JOURNAL LA English DT Article DE black hole physics; methods: numerical; relativistic processes ID 2-COMPONENT ACCRETION FLOW; SUPER-EDDINGTON ACCRETION; BLACK-HOLE; SPHERICAL ACCRETION; OPTICALLY THICK; M1 CLOSURE; DISKS; HYDRODYNAMICS; SIMULATION; CODE AB We present bhlight, a numerical scheme for solving the equations of general relativistic radiation magnetohydrodynamics using a direct Monte Carlo solution of the frequency-dependent radiative transport equation. bhlight is designed to evolve black hole accretion flows at intermediate accretion rate, in the regime between the classical radiatively efficient disk and the radiatively inefficient accretion flow (RIAF), in which global radiative effects play a sub-dominant but non-negligible role in disk dynamics. We describe the governing equations, numerical method, idiosyncrasies of our implementation, and a suite of test and convergence results. We also describe example applications to radiative Bondi accretion and to a slowly accreting Kerr black hole in axisymmetry. C1 [Ryan, B. R.; Gammie, C. F.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Dolence, J. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Gammie, C. F.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. RP Ryan, BR (reprint author), Univ Illinois, Dept Astron, 1110 W Green St, Urbana, IL 61801 USA. OI Gammie, Charles /0000-0001-7451-8935; Dolence, Joshua/0000-0003-4353-8751 FU NSF [AST 13-33612]; NASA [NNX10AD03G]; Romano Professorial Scholarship; National Science Foundation [OCI-0725070, ACI-1238993]; state of Illinois FX This work was supported by NSF grant AST 13-33612 and NASA grant NNX10AD03G, by a NASA GSRP fellowship to J.C.D, an Illinois Distinguished Fellowship to B.R.R, a Metropolis Fellowship to J.C.D, and a Romano Professorial Scholarship to C.F.G. We thank B. Farris, C. Roedig, and particularly M. Chandra and S. Shapiro for discussions, as well as J. Stone, E. Quataert, and all the members of the horizon collaboration (horizon.astro.illinois.edu). We also thank the anonymous referee for a very useful report. A portion of the analytic results presented here were obtained using the SageMath software package running on SageMathCloud (https://cloud.sagemath.com). A portion of the numerical results presented here were obtained on Princeton's tiger cluster. This research is part of the Blue Waters sustained-petascale computing project, which is supported by the National Science Foundation (awards OCI-0725070 and ACI-1238993) and the state of Illinois. Blue Waters is a joint effort of the University of Illinois at Urbana-Champaign and its National Center for Supercomputing Applications. NR 53 TC 6 Z9 6 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 31 DI 10.1088/0004-637X/807/1/31 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200031 ER PT J AU Schneider, MD Hogg, DW Marshall, PJ Dawson, WA Meyers, J Bard, DJ Lang, D AF Schneider, Michael D. Hogg, David W. Marshall, Philip J. Dawson, William A. Meyers, Joshua Bard, Deborah J. Lang, Dustin TI HIERARCHICAL PROBABILISTIC INFERENCE OF COSMIC SHEAR SO ASTROPHYSICAL JOURNAL LA English DT Article DE catalogs; cosmology: observations; gravitational lensing: weak; methods: data analysis; methods: statistical; surveys ID DIRICHLET PROCESS MIXTURE; WEAK-LENSING SURVEYS; GALAXY SHAPE MEASUREMENT; NONPARAMETRIC PROBLEMS; BAYESIAN-INFERENCE; MODELS; CONSTRAINTS; CFHTLENS; DISTRIBUTIONS; REQUIREMENTS AB Point estimators for the shearing of galaxy images induced by gravitational lensing involve a complex inverse problem in the presence of noise, pixelization, and model uncertainties. We present a probabilistic forward modeling approach to gravitational lensing inference that has the potential to mitigate the biased inferences in most common point estimators and is practical for upcoming lensing surveys. The first part of our statistical framework requires specification of a likelihood function for the pixel data in an imaging survey given parameterized models for the galaxies in the images. We derive the lensing shear posterior by marginalizing over all intrinsic galaxy properties that contribute to the pixel data (i.e., not limited to galaxy ellipticities) and learn the distributions for the intrinsic galaxy properties via hierarchical inference with a suitably flexible conditional probabilitiy distribution specification. We use importance sampling to separate the modeling of small imaging areas from the global shear inference, thereby rendering our algorithm computationally tractable for large surveys. With simple numerical examples we demonstrate the improvements in accuracy from our importance sampling approach, as well as the significance of the conditional distribution specification for the intrinsic galaxy properties when the data are generated from an unknown number of distinct galaxy populations with different morphological characteristics. C1 [Schneider, Michael D.; Dawson, William A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Schneider, Michael D.] Univ Calif Davis, Davis, CA 95616 USA. [Hogg, David W.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [Marshall, Philip J.; Bard, Deborah J.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Meyers, Joshua] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94035 USA. [Lang, Dustin] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. RP Schneider, MD (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM schneider42@llnl.gov OI Schneider, Michael/0000-0002-8505-7094; Hogg, David/0000-0003-2866-9403 FU U.S. Department of Energy [DE-AC52-07NA27344]; NSF [IIS-1124794]; Moore-Sloan Data Science Environment at NYU FX We thank Dominique Boutigny for several technical reviews of this work and for contributions to our GREAT3 challenge submissions based on these methods. We thank Bob Armstrong, Gary Bernstein, Jim Bosch, and Erin Sheldon for helpful conversations. We also thank the GREAT3 gravitational lensing community challenge team for motivating much of this work and providing valuable feedback on the implementation of our algorithms. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. D.W.H. was partially supported by the NSF (grant IIS-1124794) and the Moore-Sloan Data Science Environment at NYU. NR 64 TC 9 Z9 9 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 AR 87 DI 10.1088/0004-637X/807/1/87 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200087 ER PT J AU Zingale, M Malone, CM Nonaka, A Almgren, AS Bell, JB AF Zingale, M. Malone, C. M. Nonaka, A. Almgren, A. S. Bell, J. B. TI COMPARISONS OF TWO- AND THREE-DIMENSIONAL CONVECTION IN TYPE I X-RAY BURSTS SO ASTROPHYSICAL JOURNAL LA English DT Article DE convection; hydrodynamics; methods: numerical; stars: neutron; X-rays: bursts ID HYPERBOLIC CONSERVATION-LAWS; ACCRETING NEUTRON-STARS; EQUATION-OF-STATE; 2-DIMENSIONAL TURBULENCE; SUPERNOVAE; SIMULATIONS; ENERGY; APPROXIMATION; HYDRODYNAMICS; CONSISTENCY AB We perform the first detailed three-dimensional simulation of low Mach number convection preceding runaway thermonuclear ignition in a mixed H/He X-ray burst. Our simulations include a moderate-sized, approximate network that captures hydrogen and helium burning up through rp-process breakout. We look at the difference between two- and three-dimensional convective fields, including the details of the turbulent convection. C1 [Zingale, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Malone, C. M.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [Nonaka, A.; Almgren, A. S.; Bell, J. B.] Los Alamos Natl Lab, XCP 1, Los Alamos, NM 87545 USA. [Nonaka, A.; Almgren, A. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. RP Zingale, M (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. EM michael.zingale@stonybrook.edu OI Malone, Chris/0000-0002-4045-7932; Zingale, Michael/0000-0001-8401-030X FU DOE/Office of Nuclear Physics grants [DE-FG02-06ER41448, DE-FG02-87ER40317]; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Applied Mathematics Program of the DOE Office of Advance Scientific Computing Research under U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231, DE-AC05-00OR22725] FX We thank Frank Timmes for making his equation of state publicly available. The work at Stony Brook was supported by DOE/Office of Nuclear Physics grants Nos. DE-FG02-06ER41448 and DE-FG02-87ER40317 to Stony Brook. Work at LANL was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The work at LBNL was supported by the Applied Mathematics Program of the DOE Office of Advance Scientific Computing Research under U.S. Department of Energy under contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 41 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2015 VL 807 IS 1 DI 10.1088/0004-637X/807/1/60 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO1VX UT WOS:000358945200060 ER PT J AU Naumann, S Schwanenberg, D Karimanzira, D Fan, F Allen, C AF Naumann, Steffi Schwanenberg, Dirk Karimanzira, Divas Fan, Fernando Allen, Christopher TI Short-term management of hydropower reservoirs under meteorological uncertainty by means of multi-stage optimization SO AT-AUTOMATISIERUNGSTECHNIK LA English DT Article DE Hydropower; short-term management; multi-stage stochastic optimization AB Uncertainty in meteorology, market volatility and balancing requirements for introducing renewable energy resources into the power grid, environmental obligations require robust management of non-intermittent energy sources such as hydropower. In this paper, a probalistic management system is shown and its performance is discussed in relation to the deterministic one. In the system, scenario trees enable to setup a multi-stage stochastic optimization approach as the mathematical formulation of the short-term system management. The Federal Columbia River Power System (FCRPS), managed by the Bonneville Power Administration, the US Army Corps of Engineers and the Bureau of Reclamation, serves as a large-scale test case for the application of the management system and proves that the stochastic approach is feasible and verify the operational applicability within a real-time environment. C1 [Naumann, Steffi; Karimanzira, Divas] Fraunhofer IOSB AST, Ilmenau, Germany. [Schwanenberg, Dirk] Deltares, Dept Operat Water Management, Delft, Netherlands. [Fan, Fernando] Univ Fed Rio Grande do Sul, Inst Pesquisas Hidraul, Porto Alegre, RS, Brazil. [Allen, Christopher] Bonneville Power Adm, US Dept Energy, Portland, OR USA. RP Karimanzira, D (reprint author), Fraunhofer IOSB AST, Ilmenau, Germany. EM divas.karimanzira@iosb-ast.fraunhofer.de FU BPA [259, 2013-1517]; CEMIG, Deltares and Fraunhofer IOSB-AST FX This research is supported by the BPA (TI ProjectNr. 259, Application 2013-1517), CEMIG, Deltares and Fraunhofer IOSB-AST. Thanks to all colleagues who are involved in the Project. NR 21 TC 0 Z9 0 U1 1 U2 2 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0178-2312 J9 AT-AUTOM JI AT-Autom. PD JUL PY 2015 VL 63 IS 7 SI SI BP 535 EP 542 DI 10.1515/auto-2014-1168 PG 8 WC Automation & Control Systems SC Automation & Control Systems GA CN9OV UT WOS:000358779600006 ER PT J AU Villeneuve, S Rabinovici, GD Cohn-Sheehy, BI Madison, C Ayakta, N Ghosh, PM La Joie, R Arthur-Bentil, SK Vogel, JW Marks, SM Lehmann, M Rosen, HJ Reed, B Olichney, J Boxer, AL Miller, BL Borys, E Jin, LW Huang, EJ Grinberg, LT DeCarli, C Seeley, WW Jagust, W AF Villeneuve, Sylvia Rabinovici, Gil D. Cohn-Sheehy, Brendan I. Madison, Cindee Ayakta, Nagehan Ghosh, Pia M. La Joie, Renaud Arthur-Bentil, Samia Kate Vogel, Jacob W. Marks, Shawn M. Lehmann, Manja Rosen, Howard J. Reed, Bruce Olichney, John Boxer, Adam L. Miller, Bruce L. Borys, Ewa Jin, Lee-Way Huang, Eric J. Grinberg, Lea T. DeCarli, Charles Seeley, William W. Jagust, William TI Existing Pittsburgh Compound-B positron emission tomography thresholds are too high: statistical and pathological evaluation SO BRAIN LA English DT Article DE Alzheimer's disease; dementia; biomarkers; neurodegeneration; beta-amyloid ID MILD COGNITIVE IMPAIRMENT; ALZHEIMERS ASSOCIATION WORKGROUPS; AMYLOID-BETA DEPOSITION; NATIONAL INSTITUTE; NEUROPATHOLOGIC ASSESSMENT; DIAGNOSTIC-CRITERIA; FUNCTIONAL CONNECTIVITY; FRONTOTEMPORAL DEMENTIA; HYPOTHETICAL MODEL; DYNAMIC BIOMARKERS AB Arnyloid-beta, a hallmark or Alzheimer's disease, begins accumulating up to two decades before me onset of dementia, and can be detected in vivo applying amyloid-beta positron emission tomography tracers such as carbon-11-labelled Pittsburgh compound-B A variety of threshold,: have been applied in the literature to define Pittsburgh compound-B positron emission tomography positivity, but the ability of these thresholds to detect early amyloid-beta deposition is unknown, and validation studies comparing Pittsburgh compound-B thresholds to post-mortem amyloid burden are lacking. In this study we first derived threshold for amyloid positron emission tomography positivity using Pittsburgh compound-B positron emission tomography in 154 cognitively normal older adult,: with four complementary approaches: (i) reference values from a young control group aged between 2(1 and 31 years; jii) a Gaussian mixture model that assigned each subject a probability of being amyloid-p-positive or amyloid-beta-negative based on Pittsburgh compound-B index uptake; (iii) a k-means cluster approach that clustered subject,: into amyloid-p-positive or amyloid-p-negative based on Pittsburgh compound-B uptake in different brain regions (features); and (iv) an iterative voxel-based analysis that further explored the spatial pattern of early amyloid-beta positron emission tomography signal. Next, we tested the, sensitivity and specificity of the derived thresholds in 50 individuals who underwent Pittsburgh compound-B positron emission tomography during life and brain autopsy mean time positron emission tomography to autopsy 3.1 +/- 1.8 years). Am bid autopsy was classified using Consortium to Establish a Registry for Alzheimer's Disease (CERAD) criteria, unadjusted for age. The analytic approaches yielded low thresholds standard uptake value ratio(low) = 1.21, distribution volume ratio(low) = 1.08) that represent the earliest detectable Pittsburgh compound-B signal, as well as high thresholds (standard uptake value ratio(high) = 1.40, distribution volume ratio(high) = 1.20) that are more conservative in defining Pittsburgh compound-B positron emission tomography positivity. In voxel-wise contrasts, elevated Pittsburgh compound-B retention was first noted in the medial frontal cortex, then the precuneus, lateral frontal and parietal lobes, and finally the lateral temporal lobe. When compared to post-mortem amyloid burden, tow proposed thresholds were more sensitive than high thresholds (sensitivities: distribution volume ratio(low) 81.0% standard uptake value ratio(low) 83.3%; distribution volume ratio(high) 61.9%, standard uptake value ratio(high) 62.5%) for GERM moderate-to-frequent neuritic plaques, with similar specificity (distribution volume ratio(low) 95.8%; standard uptake value ratio: distribution volume ratio(high), and standard uptake value ratio(high) 100.0%). A receiver operator characteristic analysis identified optimal distribution volume ratio (1.06) and standard uptake value ratio;1.20) thresholds that were nearly identical to the a prior distribution volume ratio(low) and standard uptake value ratio(low). In summary, We found that frequently applied thresholds for Pittsburgh compound-B positivity (typically at or above distribution volume ratio(high) and standard uptake value ratio(high)) are overly stringent in defining amyloid positivity. Lower thresholds in this study resulted in higher sensitivity while not comprimising specificity. C1 [Villeneuve, Sylvia; Rabinovici, Gil D.; Cohn-Sheehy, Brendan I.; Madison, Cindee; Ayakta, Nagehan; Ghosh, Pia M.; La Joie, Renaud; Arthur-Bentil, Samia Kate; Vogel, Jacob W.; Marks, Shawn M.; Lehmann, Manja; Jagust, William] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Rabinovici, Gil D.; Cohn-Sheehy, Brendan I.; Ghosh, Pia M.; Arthur-Bentil, Samia Kate; Jagust, William] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rabinovici, Gil D.; Cohn-Sheehy, Brendan I.; Ayakta, Nagehan; Ghosh, Pia M.; Lehmann, Manja; Rosen, Howard J.; Boxer, Adam L.; Miller, Bruce L.; Grinberg, Lea T.; Seeley, William W.] Univ Calif San Francisco, Dept Neurol, Memory & Aging Ctr, San Francisco, CA USA. [Reed, Bruce; Olichney, John; DeCarli, Charles] Univ Calif Davis, Sch Med, Dept Neurol, Davis, CA 95616 USA. [Reed, Bruce] Vet Affairs Northern Calif Hlth Care Syst, Martinez, CA USA. [Borys, Ewa] Loyola Univ Chicago, Stritch Sch Med, Dept Pathol, Chicago, IL USA. [Jin, Lee-Way] Univ Calif Davis, Dept Pathol & Lab Med, Davis, CA 95616 USA. [Huang, Eric J.; Grinberg, Lea T.; Seeley, William W.] Univ Calif San Francisco, Dept Pathol, San Francisco, CA 94140 USA. RP Villeneuve, S (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 132 Barker Hall,MC 3190, Berkeley, CA 94720 USA. EM villeneuve.sylvia@gmail.com OI Huang, Eric/0000-0002-5381-3801; Marks, Shawn/0000-0001-9884-8461; La Joie, Renaud/0000-0003-2581-8100 FU National Institute on Aging [K23-AG031861, R01-AG045611, P01-AG1972403, P50-AG023501, R01-AG032306, K24-AG045333, P01-AG12435, P30-AG10129, R01-AG021028, R01-AG031563, R01AG038791, R01-AG034570]; Consortium for Frontotemporal Dementia Research; Tau Consortium; John Douglas French Alzheimer's Foundation; State of California Department of Health Services Alzheimer's Disease Research Center of California [04-33516]; Hellman Family Foundation; Canadian Institutes of Health Research FX This work was supported by National Institute on Aging grants K23-AG031861 and R01-AG045611 to G.D.R., P01-AG1972403 to B.LM. and W.W.S, P50-AG023501 to B.L.M., G.D.R and W.W.S., R01-AG032306 and K24-AG045333 to H.J.R, P01-AG12435, P30-AG10129, R01-AG021028 and R01-AG031563 to C.D., R01-AG031563 to B.R.; R01AG038791 to A.L.B., R01-AG034570 to WJJ; the Consortium for Frontotemporal Dementia Research to B.L.M. and W.W.S; the Tau Consortium to W.W.S., G.D.R and W.J.J.; John Douglas French Alzheimer's Foundation to G.D.R. and B.L.M.; State of California Department of Health Services Alzheimer's Disease Research Center of California grant 04-33516 to B.L.M; Hellman Family Foundation award to G.D.R.; and Canadian Institutes of Health Research post-doctoral fellowship to S.V. NR 64 TC 21 Z9 21 U1 0 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0006-8950 EI 1460-2156 J9 BRAIN JI Brain PD JUL 1 PY 2015 VL 138 BP 2020 EP 2033 DI 10.1093/brain/awv112 PN 7 PG 14 WC Clinical Neurology; Neurosciences SC Neurosciences & Neurology GA CN6HY UT WOS:000358536600030 PM 25953778 ER PT J AU Weston, DJ Rogers, A Tschaplinski, TJ Gunter, LE Jawdy, SA Engle, NL Heady, LE Tuskan, GA Wullschleger, SD AF Weston, David J. Rogers, Alistair Tschaplinski, Timothy J. Gunter, Lee E. Jawdy, Sara A. Engle, Nancy L. Heady, Lindsey E. Tuskan, Gerald A. Wullschleger, Stan D. TI Scaling nitrogen and carbon interactions: what are the consequences of biological buffering? SO ECOLOGY AND EVOLUTION LA English DT Article DE Buffering; carbon; ecological genomics; networks; nitrogen; robustness; scaling ID NITRATE REDUCTASE; ARABIDOPSIS-THALIANA; DUPLICATE GENES; CO2 ENRICHMENT; DIFFERENTIAL EXPRESSION; FUNCTIONAL COMPENSATION; DIOXIDE CONCENTRATION; NETWORK STRUCTURE; PLANT CARBON; GLYCINE-MAX AB Understanding the consequences of elevated CO2 (eCO(2); 800ppm) on terrestrial ecosystems is a central theme in global change biology, but relatively little is known about how altered plant C and N metabolism influences higher levels of biological organization. Here, we investigate the consequences of C and N interactions by genetically modifying the N-assimilation pathway in Arabidopsis and initiating growth chamber and mesocosm competition studies at current CO2 (cCO(2); 400ppm) and eCO(2) over multiple generations. Using a suite of ecological, physiological, and molecular genomic tools, we show that a single-gene mutant of a key enzyme (nia2) elicited a highly orchestrated buffering response starting with a fivefold increase in the expression of a gene paralog (nia1) and a 63% increase in the expression of gene network module enriched for N-assimilation genes. The genetic perturbation reduced amino acids, protein, and TCA-cycle intermediate concentrations in the nia2 mutant compared to the wild-type, while eCO(2) mainly increased carbohydrate concentrations. The mutant had reduced net photosynthetic rates due to a 27% decrease in carboxylation capacity and an 18% decrease in electron transport rates. The expression of these buffering mechanisms resulted in a penalty that negatively correlated with fitness and population dynamics yet showed only minor alterations in our estimates of population function, including total per unit area biomass, ground cover, and leaf area index. This study provides insight into the consequences of buffering mechanisms that occur post-genetic perturbations in the N pathway and the associated outcomes these buffering systems have on plant populations relative to eCO(2). C1 [Weston, David J.; Tschaplinski, Timothy J.; Gunter, Lee E.; Jawdy, Sara A.; Engle, Nancy L.; Tuskan, Gerald A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Rogers, Alistair; Heady, Lindsey E.] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Wullschleger, Stan D.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Weston, DJ (reprint author), Oak Ridge Natl Lab, Biosci Div, POB 2008 MS-6407, Oak Ridge, TN 37831 USA. EM westondj@ornl.gov RI Rogers, Alistair/E-1177-2011; Gunter, Lee/L-3480-2016; Wullschleger, Stan/B-8297-2012; Tuskan, Gerald/A-6225-2011; OI Rogers, Alistair/0000-0001-9262-7430; Gunter, Lee/0000-0003-1211-7532; Wullschleger, Stan/0000-0002-9869-0446; Tuskan, Gerald/0000-0003-0106-1289; Tschaplinski, Timothy/0000-0002-9540-6622; Engle, Nancy/0000-0003-0290-7987 FU U.S. Department of Energy, Office of Science, Office of the Biological and Environmental Research through the Terrestrial Ecosystem Sciences (TES) Program; DOE [DE-AC05-00OR22725]; Brookhaven National Laboratory [DE-AC02-98CHI0886] FX This research was funded by the U.S. Department of Energy, Office of Science, Office of the Biological and Environmental Research through the Terrestrial Ecosystem Sciences (TES) Program. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the DOE under contract DE-AC05-00OR22725 and Brookhaven National Laboratory under contract No. DE-AC02-98CHI0886. NR 63 TC 1 Z9 1 U1 1 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2045-7758 J9 ECOL EVOL JI Ecol. Evol. PD JUL PY 2015 VL 5 IS 14 BP 2839 EP 2850 DI 10.1002/ece3.1565 PG 12 WC Ecology; Evolutionary Biology SC Environmental Sciences & Ecology; Evolutionary Biology GA CN5EN UT WOS:000358452700008 PM 26306170 ER PT J AU Boeckmann, B Marcet-Houben, M Rees, JA Forslund, K Huerta-Cepas, J Muffato, M Yilmaz, P Xenarios, I Bork, P Lewis, SE Gabaldon, T AF Boeckmann, Brigitte Marcet-Houben, Marina Rees, Jonathan A. Forslund, Kristoffer Huerta-Cepas, Jaime Muffato, Matthieu Yilmaz, Pelin Xenarios, Ioannis Bork, Peer Lewis, Suzanna E. Gabaldon, Toni CA Quest Orthologs Species Tree TI Quest for Orthologs Entails Quest for Tree of Life: In Search of the Gene Stream SO GENOME BIOLOGY AND EVOLUTION LA English DT Article DE Tree of Life; species tree; gene tree support ID GENOME; PHYLOGENY; EVOLUTION; RECONSTRUCTION; EUKARYOTES; RESOLUTION; POSITIONS; ANIMALS; DOMAIN; RNA AB Quest for Orthologs (QfO) is a community effort with the goal to improve and benchmark orthology predictions. As quality assessment assumes prior knowledge on species phylogenies, we investigated the congruency between existing species trees by comparing the relationships of 147 QfO reference organisms from six Tree of Life (ToL)/species tree projects: The National Center for Biotechnology Information (NCBI) taxonomy, Opentree of Life, the sequenced species/species ToL, the 16S ribosomal RNA (rRNA) database, and trees published by Ciccarelli et al. (Ciccarelli FD, et al. 2006. Toward automatic reconstruction of a highly resolved tree of life. Science 311:1283-1287) and by Huerta-Cepas et al. (Huerta-Cepas J, Marcet-Houben M, Gabaldon T. 2014. A nested phylogenetic reconstruction approach provides scalable resolution in the eukaryotic Tree Of Life. PeerJ PrePrints 2: 223) Our study reveals that each species tree suggests a different phylogeny: 87 of the 146 (60%) possible splits of a dichotomous and rooted tree are congruent, while all other splits are incongruent in at least one of the species trees. Topological differences are observed not only at deep speciation events, but also within younger clades, such as Hominidae, Rodentia, Laurasiatheria, or rosids. The evolutionary relationships of 27 archaea and bacteria are highly inconsistent. By assessing 458,108 gene trees from 65 genomes, we show that consistent species topologies are more often supported by gene phylogenies than contradicting ones. The largest concordant species tree includes 77 of the QfO reference organisms at the most. Results are summarized in the form of a consensus ToL (http://swisstree.vital-it.ch/species_tree) that can serve different benchmarking purposes. C1 [Boeckmann, Brigitte; Xenarios, Ioannis] Swiss Prot, Swiss Inst Bioinformat, Geneva, Switzerland. [Marcet-Houben, Marina; Gabaldon, Toni] Ctr Genom Regulat, Bioinformat & Genom, Barcelona, Spain. [Marcet-Houben, Marina; Gabaldon, Toni] Univ Pompeu Fabra, Barcelona, Spain. [Rees, Jonathan A.] Duke Univ, US Natl Evolutionary Synth Ctr, Durham, NC USA. [Forslund, Kristoffer; Huerta-Cepas, Jaime; Bork, Peer] European Mol Biol Lab, Struct & Computat Biol Unit, D-69012 Heidelberg, Germany. [Muffato, Matthieu] European Bioinformat Inst, European Mol Biol Lab, Hinxton, England. [Yilmaz, Pelin] Max Planck Inst Marine Microbiol, Microbial Genom & Bioinformat Res Grp, Bremen, Germany. [Xenarios, Ioannis] Swiss Inst Bioinformat, Vital IT, Lausanne, Switzerland. [Xenarios, Ioannis] Univ Lausanne, Ctr Integrat Genom, Lausanne, Switzerland. [Bork, Peer] Univ Heidelberg Hosp, Germany Mol Med Partnership Unit, Heidelberg, Germany. [Bork, Peer] European Mol Biol Lab, D-69012 Heidelberg, Germany. [Bork, Peer] Max Delbruck Ctr Mol Med, Berlin, Germany. [Lewis, Suzanna E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Gabaldon, Toni] Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. RP Boeckmann, B (reprint author), Swiss Prot, Swiss Inst Bioinformat, Geneva, Switzerland. EM brigitte.boeckmann@isb-sib.ch RI Bork, Peer/F-1813-2013; OI Yilmaz, Pelin/0000-0003-4724-323X; Forslund, Kristoffer/0000-0003-4285-6993; Bork, Peer/0000-0002-2627-833X; Lewis, Suzanna/0000-0002-8343-612X; Gabaldon, Toni/0000-0003-0019-1735; Muffato, Matthieu/0000-0002-7860-3560 FU Swiss Federal Government through the Federal Office of Education and Science; Swiss Institute of Bioinformatics; Spanish ministry of Economy and Competitiveness [BIO2012-37161]; Qatar National Research Fund [NPRP 5-298-3-086]; European Research Council under the European Union [ERC-2012-StG-310325]; Wellcome Trust [WT095908]; European Molecular Biology Laboratory FX The authors wish to thank Vivienne Baillie Gerritsen for proofreading. This work was supported by the Swiss Federal Government through the Federal Office of Education and Science (B.B.). Funding for open access charge: Swiss Institute of Bioinformatics. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. T.G. group research is funded in part by a grant from the Spanish ministry of Economy and Competitiveness (BIO2012-37161), a Grant from the Qatar National Research Fund (NPRP 5-298-3-086), and a grant from the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013)/ERC (grant agreement no. ERC-2012-StG-310325). M.M. acknowledges support from the Wellcome Trust (grant number WT095908) and the European Molecular Biology Laboratory. NR 60 TC 3 Z9 3 U1 2 U2 15 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1759-6653 J9 GENOME BIOL EVOL JI Genome Biol. Evol. PD JUL PY 2015 VL 7 IS 7 BP 1988 EP 1999 DI 10.1093/gbe/evv121 PG 12 WC Evolutionary Biology; Genetics & Heredity SC Evolutionary Biology; Genetics & Heredity GA CN9WF UT WOS:000358800500012 PM 26133389 ER PT J AU Campbell, BD Samsel, F AF Campbell, Bruce D. Samsel, Francesca TI Murmurations: Drawing Together Art, Visualization, and Physical Phenomena SO IEEE COMPUTER GRAPHICS AND APPLICATIONS LA English DT Editorial Material C1 [Campbell, Bruce D.] Rhode Isl Sch Design, Providence, RI 02903 USA. [Samsel, Francesca] Univ Texas Austin, Ctr Agile Technol, Austin, TX 78712 USA. [Samsel, Francesca] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Campbell, BD (reprint author), Rhode Isl Sch Design, Providence, RI 02903 USA. EM bcampbel01@risd.edu; figs@cat.utexas.edu NR 4 TC 0 Z9 0 U1 1 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1716 EI 1558-1756 J9 IEEE COMPUT GRAPH JI IEEE Comput. Graph. Appl. PD JUL-AUG PY 2015 VL 35 IS 4 BP 8 EP 12 PG 5 WC Computer Science, Software Engineering SC Computer Science GA CN5WB UT WOS:000358501400003 ER PT J AU Norman, M Larkin, J Vose, A Evans, K AF Norman, Matthew Larkin, Jeffrey Vose, Aaron Evans, Katherine TI A case study of CUDA FORTRAN and OpenACC for an atmospheric climate kernel SO JOURNAL OF COMPUTATIONAL SCIENCE LA English DT Article; Proceedings Paper CT 15th Annual International Conference on Computational Science (ICCS) CY JUN 01-03, 2015 CL Reykjavik Univ, Reykjavik, ICELAND SP Elsevier, Univ Amsterdam, NTU Singapore, Univ Tennessee HO Reykjavik Univ DE OpenACC; Climate; CUDA; GPU; HPC ID SIMULATED CLIMATE; VERTICAL RESOLUTION; MODEL AB The porting of a key kernel in the tracer advection routines of the Community Atmosphere Model Spectral Element (CAM-SE) to use Graphics Processing Units (GPUs) using OpenACC is considered in comparison to an existing CUDA FORTRAN port. The development of the OpenACC kernel for GPUs was substantially simpler than that of the CUDA port. Also, OpenACC performance was about 1.5 x slower than the optimized CUDA version. Particular focus is given to compiler maturity regarding OpenACC implementation for modern FORTRAN, and it is found that the Cray implementation is currently more mature than the PGI implementation. Still, for the case that ran successfully on PGI, the PGI OpenACC runtime was slightly faster than Cray. The results show encouraging performance for OpenACC implementation compared to CUDA while also exposing some issues that may be necessary before the implementations are suitable for porting all of CAM-SE. Most notable are that GPU shared memory should be used by future OpenACC implementations and that derived type support should be expanded. (C) 2015 Published by Elsevier B.V. C1 [Norman, Matthew; Evans, Katherine] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Larkin, Jeffrey] Nvidia, Santa Clara, CA USA. [Vose, Aaron] Cray Seattle, Seattle, WA USA. RP Norman, M (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM normanmr@ornl.gov; jlarkin@nvidia.com; avose@cray.com; evanskj@ornl.gov OI Evans, Katherine/0000-0001-8174-6450 FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This research used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 14 TC 2 Z9 2 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-7503 J9 J COMPUT SCI-NETH JI J. Comput. Sci. PD JUL PY 2015 VL 9 SI SI BP 1 EP 6 DI 10.1016/j.jocs.2015.04.022 PG 6 WC Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA CN7PZ UT WOS:000358627800002 ER PT J AU Randles, A Draeger, EW Bailey, PE AF Randles, Amanda Draeger, Erik W. Bailey, Peter E. TI Massively parallel simulations of hemodynamics in the primary large arteries of the human vasculature SO JOURNAL OF COMPUTATIONAL SCIENCE LA English DT Article; Proceedings Paper CT 15th Annual International Conference on Computational Science (ICCS) CY JUN 01-03, 2015 CL Reykjavik Univ, Reykjavik, ICELAND SP Elsevier, Univ Amsterdam, NTU Singapore, Univ Tennessee HO Reykjavik Univ DE Lattice Boltzmann; Computational fluid dynamics; High performance computing; Patient-specific hemodynamics; Strong scaling ID BLOOD-FLOW; MODEL; DYNAMICS; NETWORK AB We present a computational model of three-dimensional and unsteady hemodynamics within the primary large arteries in the human on 1,572,864 cores of the IBM Blue Gene/Q Models of large regions of the circulatory system are needed to study the impact of local factors on global hemodynamics and to inform next generation drug delivery mechanisms. The HARVEY code successfully addresses key challenges that can hinder effective solution of image-based hemodynamics on contemporary supercomputers, such as limited memory capacity and bandwidth, flexible load balancing, and scalability. This work is the first demonstration of large fluid dynamics simulations of the aortofemoral region of the circulatory system at resolutions as small as 10 mu m. Published by Elsevier B.V. C1 [Randles, Amanda; Draeger, Erik W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bailey, Peter E.] Univ Arizona, Tucson, AZ USA. RP Randles, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM randles2@llnl.gov; draeger1@llnl.gov; pbailey@cs.arizona.edu FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors would like to thank Liam Krauss at LLNL for visualization and analysis work, and the staff at Livermore Computing for system support. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 33 TC 0 Z9 0 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-7503 J9 J COMPUT SCI-NETH JI J. Comput. Sci. PD JUL PY 2015 VL 9 SI SI BP 70 EP 75 DI 10.1016/j.jocs.2015.04.003 PG 6 WC Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA CN7PZ UT WOS:000358627800013 ER PT J AU Johnson, BM AF Johnson, B. M. TI Buoyancy instability of homologous implosions SO JOURNAL OF FLUID MECHANICS LA English DT Article DE compressible flows; instability; sonoluminescence ID INERTIAL CONFINEMENT FUSION; PERTURBATIONS; COLLAPSE; GROWTH; BUBBLE AB I consider the hydrodynamic stability of imploding ideal gases as an idealized model for inertial confinement fusion capsules, sonoluminescent bubbles and the gravitational collapse of astrophysical gases. For oblate modes (short-wavelength incompressive modes elongated in the direction of the mean flow), a second-order ordinary differential equation is derived that can be used to assess the stability of any timedependent flow with planar, cylindrical or spherical symmetry. Upon further restricting the analysis to homologous flows, it is shown that a monatomic gas is governed by the Schwarzschild criterion for buoyant stability. Under buoyantly unstable conditions, both entropy and vorticity fluctuations experience power-law growth in time, with a growth rate that depends upon mean flow gradients and, in the absence of dissipative effects, is independent of mode number. If the flow accelerates throughout the implosion, oblate modes amplify by a factor (2C)(vertical bar N0 vertical bar ti), where C is the convergence ratio of the implosion, N-0 is the initial buoyancy frequency and t(i) is the implosion time scale. If, instead, the implosion consists of a coasting phase followed by stagnation, oblate modes amplify by a factor exp (pi vertical bar N-0 vertical bar t(s)), where N-0 is the buoyancy frequency at stagnation and t(s) is the stagnation time scale. Even under stable conditions, vorticity fluctuations grow due to the conservation of angular momentum as the gas is compressed. For non-monatomic gases, this additional growth due to compression results in weak oscillatory growth under conditions that would otherwise be buoyantly stable; this over-stability is consistent with the conservation of wave action in the fluid frame. The above analytical results are verified by evolving the complete set of linear equations as an initial value problem, and it is demonstrated that oblate modes are the fastest-growing modes and that high mode numbers are required to reach this limit (Legendre mode l greater than or similar to 100 for spherical flows). Finally, comparisons are made with a Lagrangian hydrodynamics code, and it is found that a numerical resolution of similar to 30 zones per wavelength is required to capture these solutions accurately. This translates to an angular resolution of similar to(12/l)degrees, or less than or similar to 0.1 degrees to resolve the fastest-growing modes. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Johnson, BM (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM johnson359@llnl.gov FU Lawrence Livermore National Security, LLC (LLNS) [DE-AC52-07NA27344] FX I thank D. Clark, O. Hurricane, K. Mikaelian, O. Schilling and the referees for their comments. This work was performed under the auspices of Lawrence Livermore National Security, LLC (LLNS) under contract number DE-AC52-07NA27344. NR 29 TC 0 Z9 0 U1 1 U2 5 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0022-1120 EI 1469-7645 J9 J FLUID MECH JI J. Fluid Mech. PD JUL PY 2015 VL 774 AR R4 DI 10.1017/jfm.2015.309 PG 12 WC Mechanics; Physics, Fluids & Plasmas SC Mechanics; Physics GA CN8SQ UT WOS:000358713400004 ER PT J AU Asel, TJ Gao, HT Heinl, TJ Adkins, D Woodward, PM Hoffman, J Bhattacharya, A Brillson, LJ AF Asel, Thaddeus J. Gao, Hantian Heinl, Tyler J. Adkins, Drew Woodward, Patrick M. Hoffman, Jason Bhattacharya, Anand Brillson, Leonard J. TI Near-nanoscale-resolved energy band structure of LaNiO3/La2/3Sr1/3MnO3/SrTiO3 heterostructures and their interfaces SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID SUPERLATTICES; SPECTROSCOPY; LUMINESCENCE; DEFECTS; CASINO; SRTIO3 AB Depth-resolved cathodoluminescence spectroscopy (DRCLS) studies of LNO/LSMO/STO interfaces display an ability to detect optical transitions between orbital-derived energy levels with filled states near the Fermi level of ultrathin complex oxides and to detect changes in the electronic structure at their interfaces on a near-nanometer scale. A differential form of DRCLS (DDRCLS) provides a unique capability to measure electronic features at buried interfaces of ultrathin complex oxide films. DDRCLS measurements demonstrate the abruptness of LNO/LSMO interfaces but atomic layer distortions and altered optical emissions at the LSMO/STO heterojunction. The capability to probe electronic structure at buried complex oxide interfaces with enhanced depth resolution can reveal changes in energy levels within nanometers of interfaces, band alignments across interfaces, and the possible effect of local defects on these energy levels. (C) 2015 American Vacuum Society. C1 [Asel, Thaddeus J.; Gao, Hantian; Brillson, Leonard J.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Heinl, Tyler J.; Brillson, Leonard J.] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [Adkins, Drew; Woodward, Patrick M.] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA. [Hoffman, Jason; Bhattacharya, Anand] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Asel, TJ (reprint author), Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. EM asel.3@osu.edu RI Bhattacharya, Anand/G-1645-2011 OI Bhattacharya, Anand/0000-0002-6839-6860 FU NSF MRSEC [DMR-1420451]; NSF [DMR-1305193]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy, Office of Basic Energy Science, Materials Science Division FX This work supported by NSF MRSEC Grant No. DMR-1420451 (Charles Ying) and NSF Grant No. DMR-1305193 (Charles Ying and Haiyan Wang). Work at Argonne National Laboratory, including the use of the Center for Nanoscale Materials and Advanced Photon Source, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. J.D.H. and A.B. acknowledge support from Department of Energy, Office of Basic Energy Science, Materials Science Division. NR 29 TC 1 Z9 1 U1 7 U2 22 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD JUL PY 2015 VL 33 IS 4 AR 04E103 DI 10.1116/1.4922270 PG 5 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA CN8GB UT WOS:000358676700003 ER PT J AU Douglas, EA Sheng, JJ Verley, JC Carroll, MS AF Douglas, Erica A. Sheng, Josephine J. Verley, Jason C. Carroll, Malcolm S. TI Argon-germane in situ plasma clean for reduced temperature Ge on Si epitaxy by high density plasma chemical vapor deposition SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID SILICON HOMOEPITAXIAL GROWTH; RESONANCE HYDROGEN PLASMA; HIGH-QUALITY GE; THIN-FILMS; PHOTODETECTORS; OXYGEN AB Demand for integration of near infrared optoelectronic functionality with silicon complementary metal oxide semiconductor (CMOS) technology has for many years motivated the investigation of low temperature germanium on silicon deposition processes. This work describes the development of a high density plasma chemical vapor deposition process that uses a low temperature (<460 degrees C) in situ germane/argon plasma surface preparation step for epitaxial growth of germanium on silicon. It is shown that the germane/argon plasma treatment sufficiently removes SiOx and carbon at the surface to enable germanium epitaxy. The use of this surface preparation step demonstrates an alternative way to produce germanium epitaxy at reduced temperatures, a key enabler for increased flexibility of integration with CMOS back-end-of-line fabrication. (C) 2015 American Vacuum Society. C1 [Douglas, Erica A.; Sheng, Josephine J.; Verley, Jason C.; Carroll, Malcolm S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Sheng, Josephine J.] Univ New Mexico, Dept Elect Engn, Albuquerque, NM 87185 USA. RP Douglas, EA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM edougla@sandia.gov RI Verley, Jason/C-2026-2008 OI Verley, Jason/0000-0003-2184-677X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 34 TC 1 Z9 1 U1 1 U2 6 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD JUL PY 2015 VL 33 IS 4 AR 041202 DI 10.1116/1.4921590 PG 7 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA CN8GB UT WOS:000358676700011 ER PT J AU Hwang, YH Dong, C Hsieh, YL Zhu, WD Ahn, S Ren, F Pearton, SJ Kravchenko, II AF Hwang, Ya-Hsi Dong, Chen Hsieh, Yue-Ling Zhu, Weidi Ahn, Shihyun Ren, Fan Pearton, Stephen J. Kravchenko, Ivan I. TI Improvement of drain breakdown voltage with a back-side gate on AlGaN/GaN high electron mobility transistors SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID FIELD-EFFECT TRANSISTOR; MODULATING PLATE; OPERATION AB The effect of a back gate on the dc performance of AlGaN/GaN high electron mobility transistor was investigated. The back gate was fabricated directly under the device active area by etching off the Si substrate, AlN nucleation layer, and graded AlGaN transition layer and depositing Ni/Au-based gate metal on the exposed GaN buffer layer. The reverse bias gate leakage current decreased from 3.9 x 10(-5) to 1.2 x 10(-5) mA/mm by applying -10V at the back gate. Because of the suppression of gate leakage current by the back gate, the drain on/off ratio improved from 1.8 x 10(5) to 1.2 x 10(6) and the subthreshold swing from 204 to 137 mV/dec. Moreover, the drain breakdown voltage could be improved by 40% when the back gate was biased at -25 V. (C) 2015 American Vacuum Society. C1 [Hwang, Ya-Hsi; Dong, Chen; Hsieh, Yue-Ling; Zhu, Weidi; Ahn, Shihyun; Ren, Fan] Univ Florida, Dept Chem Engn, Gainesville, FL 32611 USA. [Pearton, Stephen J.] Univ Florida, Mat Sci & Engn, Gainesville, FL 32611 USA. [Kravchenko, Ivan I.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Hwang, YH (reprint author), Univ Florida, Dept Chem Engn, Gainesville, FL 32611 USA. EM fren@che.ufl.edu RI Kravchenko, Ivan/K-3022-2015 OI Kravchenko, Ivan/0000-0003-4999-5822 FU U.S. DOD HDTRA [1-11-1-0020]; NSF [ECCS-1445720] FX The work performed at UF was supported by an U.S. DOD HDTRA Grant No. 1-11-1-0020 monitored by James Reed and a NSF Grant No. ECCS-1445720 monitored by Mahmoud Fallahi. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 20 TC 0 Z9 0 U1 2 U2 13 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD JUL PY 2015 VL 33 IS 4 AR 042201 DI 10.1116/1.4922022 PG 4 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA CN8GB UT WOS:000358676700024 ER PT J AU Xiao, ZG Kisslinger, K AF Xiao, Zhigang Kisslinger, Kim TI Electron-beam-evaporated thin films of hafnium dioxide for fabricating electronic devices SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID ATOMIC LAYER DEPOSITION; INTEGRATED-CIRCUITS; OXIDE; DIELECTRICS; TRANSISTORS; PRECURSORS; OZONE AB Thin films of hafnium dioxide (HfO2) are widely used as the gate oxide in fabricating integrated circuits because of their high dielectric constants. In this paper, the authors report the growth of thin films of HfO2 using e-beam evaporation, and the fabrication of complementary metal-oxide semiconductor (CMOS) integrated circuits using this HfO2 thin film as the gate oxide. The authors analyzed the thin films using high-resolution transmission electron microscopy and electron diffraction, thereby demonstrating that the e-beam-evaporation-grown HfO2 film has a polycrystalline structure and forms an excellent interface with silicon. Accordingly, the authors fabricated 31-stage CMOS ring oscillator to test the quality of the HfO2 thin film as the gate oxide, and obtained excellent rail-to-rail oscillation waveforms from it, denoting that the HfO2 thin film functioned very well as the gate oxide. (C) 2015 American Vacuum Society. C1 [Xiao, Zhigang] Alabama A&M Univ, Dept Elect Engn, Normal, AL 35762 USA. [Kisslinger, Kim] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Xiao, ZG (reprint author), Alabama A&M Univ, Dept Elect Engn, Normal, AL 35762 USA. EM zhigang.xiao@aamu.edu RI Kisslinger, Kim/F-4485-2014 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC00112704]; National Science Foundation [ECCS-1229312, EPS-0814103] FX Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC00112704. The research is supported by National Science Foundation under Grant Nos. ECCS-1229312 and EPS-0814103. The authors gratefully thank Avril D. Woodhead for editing the manuscript. NR 15 TC 0 Z9 0 U1 3 U2 10 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD JUL PY 2015 VL 33 IS 4 AR 042001 DI 10.1116/1.4922627 PG 4 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA CN8GB UT WOS:000358676700022 ER PT J AU Haushalter, RW Groff, D Deutsch, S The, L Chavkin, TA Brunner, SF Katz, L Keasling, JD AF Haushalter, Robert W. Groff, Dan Deutsch, Samuel The, Lionadi Chavkin, Ted A. Brunner, Simon F. Katz, Leonard Keasling, Jay D. TI Development of an orthogonal fatty acid biosynthesis system in E. coli for oleochemical production SO METABOLIC ENGINEERING LA English DT Article DE Fatty alcohols; Methyl ketones; Fatty acid synthase; Synthetic biology ID ENGINEERED ESCHERICHIA-COLI; ALCOHOL PRODUCTION; ACYL-COA; REDUCTASE; THIOESTERASE; INHIBITION; SYNTHASES; CHEMICALS; BIOFUELS; PATHWAY AB Here we report recombinant expression and activity of several type I fatty acid synthases that can function in parallel with the native Escherichia colt fatty acid synthase. Corynebacterium glutamicum FAS1A was the most active in E. coli and this fatty acid synthase was leveraged to produce oleochemicals including fatty alcohols and methyl ketones. Coexpression of FAS1A with the ACP/CoA-reductase Maciu2220 from Marinobacter aquaeolei shifted the chain length distribution of fatty alcohols produced. Coexpression of FAS1A with FadM, FadB, and an acyl-CoA-oxidase from Micrococcus luteus resulted in the production of methyl ketones, although at a lower level than cells using the native FAS. This work, to our knowledge, is the first example of in vivo function of a heterologous fatty acid synthase in E. coli. Using FAS1 enzymes for oleochemical production have several potential advantages, and further optimization of this system could lead to strains with more efficient conversion to desired products. Finally, functional expression of these large enzyme complexes in E coli will enable their study without culturing the native organisms. Published by Elsevier Inc. On behalf of International Metabolic Engineering Society. C1 [Haushalter, Robert W.; Groff, Dan; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Haushalter, Robert W.; Groff, Dan; Deutsch, Samuel; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Deutsch, Samuel] Joint Genome Inst, Walnut Creek, CA 94598 USA. [The, Lionadi; Chavkin, Ted A.; Brunner, Simon F.; Katz, Leonard; Keasling, Jay D.] Univ Calif Berkeley, Inst QB3, Emeryville, CA 94608 USA. [Katz, Leonard; Keasling, Jay D.] Univ Calif Berkeley, Synthet Biol Engn Res Ctr, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Joint BioEnergy Inst, 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA. EM jdkeasling@lbl.gov OI Brunner, Simon/0000-0002-5935-6189 FU Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U. S. Department of Energy [DE-AC02-05CH11231] FX We thank Dr. Ee-Been Goh for supplying plasmids and guidance for the methyl ketone experiments. This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U. S. Department of Energy Office of Science, Office of Biological and Environmental Research, through Contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U. S. Department of Energy. NR 22 TC 11 Z9 12 U1 8 U2 43 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 EI 1096-7184 J9 METAB ENG JI Metab. Eng. PD JUL PY 2015 VL 30 BP 1 EP 6 DI 10.1016/j.ymben.2015.04.003 PG 6 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA CN4UD UT WOS:000358424800001 PM 25887638 ER PT J AU Lee, TC Xiong, W Paddock, T Carrieri, D Chang, IF Chiu, HF Ungerer, J Juo, SHH Maness, PC Yu, JP AF Lee, Tai-Chi Xiong, Wei Paddock, Troy Carrieri, Damian Chang, Ing-Feng Chiu, Hui-Fen Ungerer, Justin Juo, Suh-Hang Hank Maness, Pin-Ching Yu, Jianping TI Engineered xylose utilization enhances bio-products productivity in the cyanobacterium Synechocystis sp PCC 6803 SO METABOLIC ENGINEERING LA English DT Article DE Cyanobacteria; Isotopic tracing; Photomixotrophic growth; Xylose utilization ID CHROMATOGRAPHY-MASS SPECTROMETRY; ACTIVATED HETEROTROPHIC GROWTH; ZYMOMONAS-MOBILIS; GLYCOGEN-STORAGE; GENETIC-ANALYSIS; CARBON-DIOXIDE; ORGANIC-ACIDS; METABOLISM; PATHWAY; FERMENTATION AB Hydrolysis of plant biomass generates a mixture of simple sugars that is particularly rich in glucose and xylose. Fermentation of the released sugars emits CO2 as byproduct due to metabolic inefficiencies. Therefore, the ability of a microbe to simultaneously convert biomass sugars and photosynthetically fix CO2 into target products is very desirable. In this work, the cyanobacterium, Synechocystis 6803, was engineered to grow on xylose in addition to glucose. Both the xylA (xylose isomerase) and xylB (xylulokinase) genes from Escherichia coli were required to confer xylose utilization, but a xylose-specific transporter was not required. Introduction of xylAB into an ethylene-producing strain increased the rate of ethylene production in the presence of xylose. Additionally, introduction of xylAB into a glycogensynthesis mutant enhanced production of keto acids. Isotopic tracer studies found that nearly half of the carbon in the excreted keto acids was derived from the engineered xylose metabolism, while the remainder was derived from CO2 fixation. (C) 2015 International Metabolic Engineering Society. Published by Elsevier Inc. All rights reserved. C1 [Lee, Tai-Chi; Xiong, Wei; Paddock, Troy; Carrieri, Damian; Ungerer, Justin; Maness, Pin-Ching; Yu, Jianping] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO USA. [Chang, Ing-Feng] Natl Taiwan Univ, Inst Plant Biol, Taipei 10764, Taiwan. [Chiu, Hui-Fen] Kaohsiung Med Univ, Inst Pharmacol, Kaohsiung, Taiwan. [Juo, Suh-Hang Hank] Kaohsiung Med Univ, Dept Genome Med, Kaohsiung, Taiwan. RP Juo, SHH (reprint author), Kaohsiung Med Univ, Dept Genome Med, Kaohsiung, Taiwan. EM hjuo@kmu.edu.tw; Pinching.Maness@nrel.gov; Jianping.Yu@nrel.gov RI Juo, Suh-Hang/C-9545-2009; OI CHANG, ING-FENG/0000-0003-0237-1246 FU National Science Council in Taiwan [100-2911-1-037-503]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office; BioEnergy Technologies Office; NREL Director's Postdoc Fellowship FX This work was supported by a Dragon-Gate grant (to TCL, IFC, NEC, SHJ) from National Science Council (project no. 100-2911-1-037-503) (renamed Ministry of Science and Technology as of March 2014) in Taiwan. It was also supported in part by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office (to PCM), BioEnergy Technologies Office (to JY), and NREL Director's Postdoc Fellowship (to WX). The authors acknowledge helpful discussion and technical assistance from Drs. Min Zhang, Yat-Chen Chou, Maria Ghirardi, Michael Seibert, Melissa Cano, and Carrie Eckert, all from NREL. NR 50 TC 10 Z9 10 U1 1 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 EI 1096-7184 J9 METAB ENG JI Metab. Eng. PD JUL PY 2015 VL 30 BP 179 EP 189 DI 10.1016/j.ymben.2015.06.002 PG 11 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA CN4UD UT WOS:000358424800019 PM 26079651 ER PT J AU Ceja-Navarro, JA Vega, FE Karaoz, U Hao, Z Jenkins, S Lim, HC Kosina, P Infante, F Northen, TR Brodie, EL AF Ceja-Navarro, Javier A. Vega, Fernando E. Karaoz, Ulas Hao, Zhao Jenkins, Stefan Lim, Hsiao Chien Kosina, Petr Infante, Francisco Northen, Trent R. Brodie, Eoin L. TI Gut microbiota mediate caffeine detoxification in the primary insect pest of coffee SO NATURE COMMUNICATIONS LA English DT Article ID HYPOTHENEMUS-HAMPEI COLEOPTERA; BERRY BORER; SEQUENCE ALIGNMENT; NITROGEN-FIXATION; PURINE ALKALOIDS; TOBACCO PLANTS; GENE; BACTERIA; METHYLXANTHINES; SCOLYTIDAE AB The coffee berry borer (Hypothenemus hampei) is the most devastating insect pest of coffee worldwide with its infestations decreasing crop yield by up to 80%. Caffeine is an alkaloid that can be toxic to insects and is hypothesized to act as a defence mechanism to inhibit herbivory. Here we show that caffeine is degraded in the gut of H. hampei, and that experimental inactivation of the gut microbiota eliminates this activity. We demonstrate that gut microbiota in H. hampei specimens from seven major coffee-producing countries and laboratory-reared colonies share a core of microorganisms. Globally ubiquitous members of the gut microbiota, including prominent Pseudomonas species, subsist on caffeine as a sole source of carbon and nitrogen. Pseudomonas caffeine demethylase genes are expressed in vivo in the gut of H. hampei, and re-inoculation of antibiotic-treated insects with an isolated Pseudomonas strain reinstates caffeine-degradation ability confirming their key role. C1 [Ceja-Navarro, Javier A.; Karaoz, Ulas; Hao, Zhao; Lim, Hsiao Chien; Brodie, Eoin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Ecol, Berkeley, CA 94720 USA. [Vega, Fernando E.] USDA ARS, Sustainable Perennial Crops Lab, Beltsville, MD 20705 USA. [Jenkins, Stefan; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Genome Dynam Dept, Berkeley, CA 94720 USA. [Kosina, Petr] Int Maize & Wheat Improvement Ctr CIMMYT, El Batan 56130, Texcoco, Mexico. [Infante, Francisco] El Colegio Frontera ECOSUR, Tapachula 30700, Chiapas, Mexico. [Brodie, Eoin L.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Ceja-Navarro, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Ecol, Berkeley, CA 94720 USA. EM jcnavarro@lbl.gov; Fernando.Vega@ars.usda.gov; elbrodie@lbl.gov RI Brodie, Eoin/A-7853-2008; Hao, Zhao/G-2391-2015; Ceja-Navarro, Javier/A-1731-2013; Karaoz, Ulas/J-7093-2014; OI Brodie, Eoin/0000-0002-8453-8435; Hao, Zhao/0000-0003-0677-8529; Ceja-Navarro, Javier/0000-0002-2954-3477; Northen, Trent/0000-0001-8404-3259; Vega, Fernando E./0000-0001-8103-5640; Kosina, Petr/0000-0002-8805-0306; Infante, Francisco/0000-0002-7419-7606 FU United States Department of Agriculture Agricultural Research Service; Laboratory Directed Research and Development programme at the Lawrence Berkeley National Laboratory under United States Department of Energy [DE-AC02-05CH11231]; 'Consejo Nacional de Ciencia y Tecnologia' (CONACyT, Mexico); Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under US Department of Energy [DE-AC02-05CH1121231] FX This work was funded by the United States Department of Agriculture Agricultural Research Service, and part of this work was funded by the Laboratory Directed Research and Development programme at the Lawrence Berkeley National Laboratory under United States Department of Energy contract number DE-AC02-05CH11231. J.A.C.-N. was supported in part by a grant from 'Consejo Nacional de Ciencia y Tecnologia' (CONACyT, Mexico) and the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under US Department of Energy Contract DE-AC02-05CH1121231. We are very grateful to S. Wiryadiputra (Indonesia), P.K. Vinod Kumar (India), A. Ramirez (Puerto Rico), PePe Miranda (Hawaii) and J. Jaramillo (Kenya) for providing specimens used in this study. We thank Susan Lynch for comments on this manuscript, Hoi-Ying Holman for advice on FTIR analyses, and Clark Santee for laboratory assistance. NR 54 TC 17 Z9 17 U1 13 U2 56 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7618 DI 10.1038/ncomms8618 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QM UT WOS:000358857000011 PM 26173063 ER PT J AU Gao, MR Chan, MKY Sun, YG AF Gao, Min-Rui Chan, Maria K. Y. Sun, Yugang TI Edge-terminated molybdenum disulfide with a 9.4-angstrom interlayer spacing for electrochemical hydrogen production SO NATURE COMMUNICATIONS LA English DT Article ID MOS2 ULTRATHIN NANOSHEETS; EVOLUTION REACTION; ELECTROCATALYTIC MATERIALS; CATALYTIC-ACTIVITY; EFFICIENT; SULFIDES; NANOPARTICLES; PERFORMANCE; GRAPHENE; SITES AB Layered molybdenum disulfide has demonstrated great promise as a low-cost alternative to platinum-based catalysts for electrochemical hydrogen production from water. Research effort on this material has focused mainly on synthesizing highly nanostructured molybdenum disulfide that allows the exposure of a large fraction of active edge sites. Here we report a promising microwave-assisted strategy for the synthesis of narrow molybdenum disulfide nanosheets with edge-terminated structure and a significantly expanded interlayer spacing, which exhibit striking kinetic metrics with onset potential of -103mV, Tafel slope of 49mV per decade and exchange current density of 9.62 X 10(-3) mAcm(-2), performing among the best of current molybdenum disulfide catalysts. Besides benefits from the edge-terminated structure, the expanded interlayer distance with modified electronic structure is also responsible for the observed catalytic improvement, which suggests a potential way to design newly advanced molybdenum disulfide catalysts through modulating the interlayer distance. C1 [Gao, Min-Rui; Chan, Maria K. Y.; Sun, Yugang] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Sun, YG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ygsun@anl.gov RI Sun, Yugang /A-3683-2010 OI Sun, Yugang /0000-0001-6351-6977 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 49 TC 62 Z9 62 U1 27 U2 172 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7493 DI 10.1038/ncomms8493 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0MD UT WOS:000358844700002 PM 26138031 ER PT J AU Perea, DE Arslan, I Liu, J Ristanovic, Z Kovarik, L Arey, BW Lercher, JA Bare, SR Weckhuysen, BM AF Perea, Daniel E. Arslan, Ilke Liu, Jia Ristanovic, Zoran Kovarik, Libor Arey, Bruce W. Lercher, Johannes A. Bare, Simon R. Weckhuysen, Bert M. TI Determining the location and nearest neighbours of aluminium in zeolites with atom probe tomography SO NATURE COMMUNICATIONS LA English DT Article ID MQ MAS NMR; ZSM-5 CRYSTALS; LOCAL-STRUCTURE; AL-27 MAS; ALK-EDGE; T-SITES; COORDINATION; ACIDITY; SPECTROSCOPY; BETA AB Zeolite catalysis is determined by a combination of pore architecture and Bronsted acidity. As Bronsted acid sites are formed by the substitution of AlO4 for SiO4 tetrahedra, it is of utmost importance to have information on the number as well as the location and neighbouring sites of framework aluminium. Unfortunately, such detailed information has not yet been obtained, mainly due to the lack of suitable characterization methods. Here we report, using the powerful atomic-scale analysis technique known as atom probe tomography, the quantitative spatial distribution of individual aluminium atoms, including their three-dimensional extent of segregation. Using a nearest-neighbour statistical analysis, we precisely determine the short-range distribution of aluminium over the different T-sites and determine the most probable Al-Al neighbouring distance within parent and steamed ZSM-5 crystals, as well as assess the long-range redistribution of aluminium upon zeolite steaming. C1 [Perea, Daniel E.; Liu, Jia; Kovarik, Libor; Arey, Bruce W.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Arslan, Ilke; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Ristanovic, Zoran; Weckhuysen, Bert M.] Univ Utrecht, Fac Sci, Debye Inst Nanomat Sci, NL-3584 CG Utrecht, Netherlands. [Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85748 Garching, Germany. [Bare, Simon R.] Honeywell Co, UOP LLC, Lincolnshire, IL 60016 USA. RP Bare, SR (reprint author), Honeywell Co, UOP LLC, 25 E Algonquin Rd Des Plaines, Lincolnshire, IL 60016 USA. EM simon.bare@honeywell.com; b.m.weckhuysen@uu.nl RI Perea, Daniel/A-5345-2010; Institute (DINS), Debye/G-7730-2014; Weckhuysen, Bert/D-3742-2009; Kovarik, Libor/L-7139-2016; OI Weckhuysen, Bert/0000-0001-5245-1426; Bare, Simon/0000-0002-4932-0342 FU LDRD programme at PNNL; U.S. Department of Energy [DE-AC05-76RL01830]; Netherlands Organisation for Scientific Research (NWO) Gravitation Program (Netherlands Center for Multiscale Catalytic Energy Conversion, MCEC); TOP NWO-CW Grant; European Research Council (ERC) Advanced Grant [321140]; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX The APT experiments in this study were performed under a science theme user proposal at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. I. A. acknowledges support through the LDRD programme at PNNL. PNNL is operated by Battelle for the U.S. Department of Energy under contract DE-AC05-76RL01830. B.M.W. acknowledges financial support from the Netherlands Organisation for Scientific Research (NWO) Gravitation Program (Netherlands Center for Multiscale Catalytic Energy Conversion, MCEC) and a TOP NWO-CW Grant, as well as a European Research Council (ERC) Advanced Grant (321140). We acknowledge Machteld Mertens (ExxonMobil) for making the zeolite ZSM-5 crystals. NR 47 TC 12 Z9 13 U1 15 U2 92 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7589 DI 10.1038/ncomms8589 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QB UT WOS:000358855900002 PM 26133270 ER PT J AU Streubel, R Kronast, F Fischer, P Parkinson, D Schmidt, OG Makarov, D AF Streubel, Robert Kronast, Florian Fischer, Peter Parkinson, Dula Schmidt, Oliver G. Makarov, Denys TI Retrieving spin textures on curved magnetic thin films with full-field soft X-ray microscopies SO NATURE COMMUNICATIONS LA English DT Article ID ROLLED-UP NANOMEMBRANES; ELECTRON TOMOGRAPHY; CO/PT MULTILAYERS; DOMAIN-WALL; HOLOGRAPHY; NANOTUBES; MICROSTRUCTURE; ARRAYS AB X-ray tomography is a well-established technique to characterize 3D structures in material sciences and biology; its magnetic analogue-magnetic X-ray tomography-is yet to be developed. Here we demonstrate the visualization and reconstruction of magnetic domain structures in a 3D curved magnetic thin films with tubular shape by means of full-field soft X-ray microscopies. The 3D arrangement of the magnetization is retrieved from a set of 2D projections by analysing the evolution of the magnetic contrast with varying projection angle. Using reconstruction algorithms to analyse the angular evolution of 2D projections provides quantitative information about domain patterns and magnetic coupling phenomena between windings of azimuthally and radially magnetized tubular objects. The present approach represents a first milestone towards visualizing magnetization textures of 3D curved thin films with virtually arbitrary shape. C1 [Streubel, Robert; Schmidt, Oliver G.; Makarov, Denys] IFW Dresden, Inst Integrat Nanosci, D-01069 Dresden, Germany. [Kronast, Florian] Helmholtz Zentrum Berlin Mat & Energie GmbH, D-12489 Berlin, Germany. [Fischer, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. [Fischer, Peter] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Parkinson, Dula] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Schmidt, Oliver G.] TU Chemnitz, Mat Syst Nanoelect, D-09107 Chemnitz, Germany. RP Streubel, R (reprint author), IFW Dresden, Inst Integrat Nanosci, D-01069 Dresden, Germany. EM r.streubel@ifw-dresden.de; d.makarov@ifw-dresden.de RI Makarov, Denys/G-1025-2011; Streubel, Robert/D-9686-2012; Fischer, Peter/A-3020-2010 OI Fischer, Peter/0000-0002-9824-9343 FU German Science Foundation (DFG) [MA 5144/2-1]; DFG Research Group [FOR1713]; European Research Council under European Union's Seventh Framework programme (FP7/2007 2013)/ERC grant [n.306277]; Future and Emerging Technologies (FET) programme [618083]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05-CH11231]; Leading Foreign Research Institute Recruitment Program through the National Research Foundation (NRF) of Korea - Ministry of Education, Science and Technology (MEST) [2012K1A4A3053565] FX We thank Irina Fiering (IFW Dresden) for metal deposition, Professor Joshua Deutsch (UC Santa Cruz) for fruitful discussions on the magnetization reconstruction algorithm and Professor Rudolf Schafer (IFW Dresden) for access to the Kerr microscope. This work is financed via the German Science Foundation (DFG) grant MA 5144/2-1 and DFG Research Group FOR1713, the European Research Council under European Union's Seventh Framework programme (FP7/2007 2013)/ERC grant agreement n.306277 and the Future and Emerging Technologies (FET) programme under FET-Open grant number 618083. We thank HZB for the allocation of synchrotron radiation beamtime. P.F. acknowledges support by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231 and by the Leading Foreign Research Institute Recruitment Program (Grant No. 2012K1A4A3053565) through the National Research Foundation (NRF) of Korea funded by the Ministry of Education, Science and Technology (MEST). NR 64 TC 10 Z9 10 U1 7 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7612 DI 10.1038/ncomms8612 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QM UT WOS:000358857000005 PM 26139445 ER PT J AU Wang, X Choi, SI Roling, LT Luo, M Ma, C Zhang, L Chi, MF Liu, JY Xie, ZX Herron, JA Mavrikakis, M Xia, YN AF Wang, Xue Choi, Sang-Il Roling, Luke T. Luo, Ming Ma, Cheng Zhang, Lei Chi, Miaofang Liu, Jingyue Xie, Zhaoxiong Herron, Jeffrey A. Mavrikakis, Manos Xia, Younan TI Palladium-platinum core-shell icosahedra with substantially enhanced activity and durability towards oxygen reduction SO NATURE COMMUNICATIONS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BY-LAYER DEPOSITION; FUEL-CELL CATHODE; MONOLAYER ELECTROCATALYSTS; CATALYTIC-ACTIVITY; ALLOY CATALYSTS; BASIS-SET; NANOPARTICLES; NANOCRYSTALS AB Conformal deposition of platinum as ultrathin shells on facet-controlled palladium nanocrystals offers a great opportunity to enhance the catalytic performance while reducing its loading. Here we report such a system based on palladium icosahedra. Owing to lateral confinement imposed by twin boundaries and thus vertical relaxation only, the platinum overlayers evolve into a corrugated structure under compressive strain. For the core-shell nanocrystals with an average of 2.7 platinum overlayers, their specific and platinum mass activities towards oxygen reduction are enhanced by eight- and sevenfold, respectively, relative to a commercial catalyst. Density functional theory calculations indicate that the enhancement can be attributed to the weakened binding of hydroxyl to the compressed platinum surface supported on palladium. After 10,000 testing cycles, the mass activity of the core-shell nanocrystals is still four times higher than the commercial catalyst. These results demonstrate an effective approach to the development of electrocatalysts with greatly enhanced activity and durability. C1 [Wang, Xue; Choi, Sang-Il; Luo, Ming; Zhang, Lei; Xia, Younan] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. [Wang, Xue; Choi, Sang-Il; Luo, Ming; Zhang, Lei; Xia, Younan] Emory Univ, Atlanta, GA 30332 USA. [Wang, Xue; Zhang, Lei; Xie, Zhaoxiong] Xiamen Univ, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Fujian, Peoples R China. [Wang, Xue; Zhang, Lei; Xie, Zhaoxiong] Xiamen Univ, Dept Chem, Xiamen 361005, Fujian, Peoples R China. [Roling, Luke T.; Herron, Jeffrey A.; Mavrikakis, Manos] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Ma, Cheng; Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Liu, Jingyue] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Xia, Younan] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Xia, Younan] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. RP Mavrikakis, M (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. EM emavrikakis@wisc.edu; younan.xia@bme.gatech.edu RI Ma, Cheng/C-9120-2014; Xie, Zhaoxiong/G-3416-2010; Roling, Luke/B-8793-2015; Mavrikakis, Manos/D-5702-2012; Xia, Younan/E-8499-2011; Zhang, Lei/N-7527-2015; Chi, Miaofang/Q-2489-2015; Wang, Xue/D-4488-2012 OI Roling, Luke/0000-0001-9742-2573; Mavrikakis, Manos/0000-0002-5293-5356; Chi, Miaofang/0000-0003-0764-1567; Wang, Xue/0000-0002-6298-1858 FU Georgia Institute of Technology; DOE-BES (Office of Chemical Scienses) [DE-FG02-05ER15731]; China Scholarship Council; ORNL's Center for Nanophase Materials Sciences; Arizona State University; DOE Office of Biological and Environmental Research at PNNL; DOE [DE-AC02-06CH11357, DE-AC02-05CH11231] FX The syntheses were supported by start-up funds from the Georgia Institute of Technology (to Y.X.) while the computations were supported by DOE-BES (Office of Chemical Scienses, grant DE-FG02-05ER15731, to M.M.). As visiting students, X.W., M.L. and L.Z. were also partially supported by the China Scholarship Council. Part of the electron microscopy work was performed through a user project supported by the ORNL's Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. J.L. gratefully acknowledges the support by Arizona State University and the use of facilities in the John M. Cowley Center for High Resolution Electron Microscopy at Arizona State University. The calculations were performed at supercomputing centres located at EMSL (which is sponsored by the DOE Office of Biological and Environmental Research at PNNL), CNM (supported by DOE contract DE-AC02-06CH11357 to ANL) and NERSC (supported by DOE contract DE-AC02-05CH11231 to LBL). NR 49 TC 76 Z9 77 U1 60 U2 282 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2015 VL 6 AR 7594 DI 10.1038/ncomms8594 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0QD UT WOS:000358856100001 PM 26133469 ER PT J AU Fiedler, JD Lanzatella, C Okada, M Jenkins, J Schmutz, J Tobias, CM AF Fiedler, Jason D. Lanzatella, Christina Okada, Miki Jenkins, Jerry Schmutz, Jeremy Tobias, Christian M. TI High-Density Single Nucleotide Polymorphism Linkage Maps of Lowland Switchgrass using Genotyping-by-Sequencing SO PLANT GENOME LA English DT Article ID PANICUM-VIRGATUM L.; SEGREGATION DISTORTION; SELF-INCOMPATIBILITY; MOLECULAR MARKERS; SNP DISCOVERY; CONSTRUCTION; PLANTS; POPULATIONS; SOFTWARE; HERITABILITY AB Switchgrass (Panicum virgatum L.) is a warm-season perennial grass with promising potential as a bioenergy crop in the United States. However, the lack of genomic resources has slowed the development of plant lines with optimal characteristics for sustainable feedstock production. We generated high-density single nucleotide polymorphism (SNP) linkage maps using a reduced-representation sequencing approach by genotyping 231 F-1 progeny of a cross between two parents of lowland ecotype from the cultivars Kanlow and Alamo. Over 350 million reads were generated and aligned, which enabled identification and ordering of 4611 high-quality SNPs. The total lengths of the resulting framework maps were 1770 cM for the Kanlow parent and 2059 cM for the Alamo parent. These maps show collinearity with maps generated with polymerase chain reaction (PCR)-based simple-sequence repeat (SSR) markers, and new SNP markers were identified in previously unpopulated regions of the genome. Transmission segregation distortion affected all linkage groups (LGs) to differing degrees, and ordering of distorted markers high-lighted several regions of unequal inheritance. Framework maps were adversely affected by the addition of distorted markers with varying severity, but distorted maps were of higher marker density and provided additional information for analysis. Alignment of these linkage maps with a draft version of the switchgrass genome assembly demonstrated high levels of collinearity and provides greater confidence in the validity of both resources. This methodology has proven to be a rapid and cost-effective way to generate high-quality linkage maps of an outcrossing species. C1 [Fiedler, Jason D.; Lanzatella, Christina; Tobias, Christian M.] USDA ARS, Western Reg Res Ctr, Albany, CA 94710 USA. [Okada, Miki] Univ Calif Davis, Davis, CA 95616 USA. [Jenkins, Jerry; Schmutz, Jeremy] HudsonAlpha Genome Sequencing Ctr, Huntsville, AL USA. [Jenkins, Jerry; Schmutz, Jeremy] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. RP Tobias, CM (reprint author), USDA ARS, Western Reg Res Ctr, 800 Buchanan St, Albany, CA 94710 USA. EM christian.tobias@ars.usda.gov RI Tobias, Christian/B-6602-2009; Schmutz, Jeremy/N-3173-2013 OI Tobias, Christian/0000-0002-7881-750X; Schmutz, Jeremy/0000-0001-8062-9172 FU USDA-ARS [CRIS 9235-21000-017-00D]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the USDA-ARS, CRIS 9235-21000-017-00D, National Program 301, Plant Genetic Resources, Genomics and Genetic Improvement. The work conducted by the US Department of Energy Joint Genome Institute was supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. The draft genome sequence data were produced by the US Department of Energy Joint Genome Institute. The USDA-ARS is an equal opportunity/affirmative action employer, and all agency services are available without discrimination. Mention of commercial products and organizations in this manuscript is solely to provide specific information. It does not constitute endorsement by USDA-ARS over other products and organizations not mentioned. NR 81 TC 3 Z9 3 U1 5 U2 20 PU CROP SCIENCE SOC AMER PI MADISON PA 677 S SEGOE ROAD, MADISON, WI 53711 USA SN 1940-3372 J9 PLANT GENOME-US JI Plant Genome PD JUL PY 2015 VL 8 IS 2 DI 10.3835/plantgenome2014.10.0065 PG 14 WC Plant Sciences; Genetics & Heredity SC Plant Sciences; Genetics & Heredity GA CN5BJ UT WOS:000358444200011 ER PT J AU Serba, DD Uppalapati, SR Mukherjee, S Krom, N Tang, YH Mysore, KS Saha, MC AF Serba, Desalegn D. Uppalapati, Srinivasa Rao Mukherjee, Shreyartha Krom, Nick Tang, Yuhong Mysore, Kirankumar S. Saha, Malay C. TI Transcriptome Profiling of Rust Resistance in Switchgrass Using RNA-Seq Analysis SO PLANT GENOME LA English DT Article ID PANICUM-VIRGATUM L.; LIPID-TRANSFER PROTEINS; PROGRAMMED CELL-DEATH; GENE-EXPRESSION ATLAS; PLANT IMMUNE-SYSTEM; PUCCINIA-EMACULATA; 1ST REPORT; ARABIDOPSIS; DEFENSE; ALIGNMENT AB Switchgrass rust caused by Puccinia emaculata is a major limiting factor for switchgrass (Panicum virgatum L.) production, especially in monoculture. Natural populations of switchgrass displayed diverse reactions to P. emaculata when evaluated in an Ardmore, OK, field. To identify the differentially expressed genes during the rust infection process and the mechanisms of switchgrass rust resistance, transcriptome analysis using RNA-Seq was conducted in two pseudo-F 1 parents ('PV281' and 'NFGA472'), and three moderately resistant and three susceptible progenies selected from a three-generation, four-founder switchgrass population (K5 x A4) x (AP13 x VS16). On average, 23.5 million reads per sample (leaf tissue was collected at 0, 24, and 60 h post-inoculation (hpi)) were obtained from paired-end (2 x 100 bp) sequencing on the Illumina HiSeq2000 platform. Mapping of the RNA-Seq reads to the switchgrass reference genome (AP13 ver. 1.1 assembly) constructed a total of 84,209 transcripts from 98,007 gene loci among all of the samples. Further analysis revealed that host defense- related genes, including the nucleotide binding site-leucinerich repeat domain containing disease resistance gene analogs, play an important role in resistance to rust infection. Rust-induced gene (RIG) transcripts inherited across generations were identified. The rust-resistant gene transcripts can be a valuable resource for developing molecular markers for rust resistance. Furthermore, the rust-resistant genotypes and gene transcripts identified in this study can expedite rust-resistant cultivar development in switchgrass. C1 [Serba, Desalegn D.; Saha, Malay C.] Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA. [Uppalapati, Srinivasa Rao; Tang, Yuhong; Mysore, Kirankumar S.] Samuel Roberts Noble Fdn Inc, Div Plant Biol, Ardmore, OK 73401 USA. [Mukherjee, Shreyartha; Krom, Nick] Samuel Roberts Noble Fdn Inc, Comp Serv, Ardmore, OK 73401 USA. [Uppalapati, Srinivasa Rao] Dupont Pioneer, Dupont Knowledge Ctr, Hyderabad 500078, Telangana, India. [Serba, Desalegn D.; Tang, Yuhong; Saha, Malay C.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Dept Energy, Oak Ridge, TN 37831 USA. RP Saha, MC (reprint author), Samuel Roberts Noble Fdn Inc, Forage Improvement Div, 2510 Sam Noble Pkwy, Ardmore, OK 73401 USA. EM mcsaha@noble.org FU Department of Energy (DOE); United States Department of Agriculture; BioEnergy Science Center, a U.S. DOE Bioenergy Research Center; Office of Biological and Environmental Research in the DOE Office of Science; National Science Foundation's Experimental Program to Stimulate Competitive Research [EPS-0814361] FX The three-generation, four founder population was developed with funds provided by the Department of Energy (DOE) and United States Department of Agriculture. This research work was partially funded by the BioEnergy Science Center, a U.S. DOE Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science, and the National Science Foundation's Experimental Program to Stimulate Competitive Research (EPS-0814361). The authors thank Stacy Allen of the Genomics and Microarray Core Facility of The Samuel Roberts Noble Foundation for RNA-Seq data generation. We are also thankful to Jackie Kelley for her grammatical editing of the manuscript. Mention of commercial products and companies in this manuscript is solely to provide specific information and does not constitute endorsement by any part herein. NR 74 TC 2 Z9 2 U1 5 U2 21 PU CROP SCIENCE SOC AMER PI MADISON PA 677 S SEGOE ROAD, MADISON, WI 53711 USA SN 1940-3372 J9 PLANT GENOME-US JI Plant Genome PD JUL PY 2015 VL 8 IS 2 DI 10.3835/plantgenome2014.10.0075 PG 12 WC Plant Sciences; Genetics & Heredity SC Plant Sciences; Genetics & Heredity GA CN5BJ UT WOS:000358444200016 ER PT J AU Shi, ZW Bechtel, HA Berweger, S Sun, YH Zeng, B Jin, CH Chang, H Martin, MC Raschke, MB Wang, F AF Shi, Zhiwen Bechtel, Hans A. Berweger, Samuel Sun, Yinghui Zeng, Bo Jin, Chenhao Chang, Henry Martin, Michael C. Raschke, Markus B. Wang, Feng TI Amplitude- and Phase-Resolved Nanospectral Imaging of Phonon Polaritons in Hexagonal Boron Nitride SO ACS PHOTONICS LA English DT Article DE phonon polariton; boron nitride; near-field spectroscopy; synchrotron infrared nanospectroscopy (SINS) ID NEAR-FIELD MICROSCOPY; INFRARED-ABSORPTION; GRAPHENE PLASMONS; DIRAC FERMIONS; LIGHT; HETEROSTRUCTURES; SUPERLATTICES; NANOPARTICLES; SCATTERING; PRESSURE AB Phonon polaritons are quasiparticles resulting from strong coupling of photons with optical phonons. Excitation and control of these quasiparticles in 2D materials offer the opportunity to confine and transport light at the nanoscale. Here, we image the phonon polariton (PhP) spectral response in thin hexagonal boron nitride (hBN) crystals as a representative 2D material using amplitude- and phase-resolved scattering scanning near-field optical microscopy (s-SNOM) using broadband mid-IR synchrotron radiation. The large spectral bandwidth enables the simultaneous measurement of both out-of-plane (780 cm(-1)) and in-plane (1370 cm(-1)) hBN phonon modes. In contrast to the strong in-plane mode, the out-of-plane PhP mode response is weak Measurements of the PhP wavelength reveal a proportional dependence on sample thickness for thin hBN flakes, which can be understood by a general model describing two-dimensional polariton excitation in ultrathin materials. C1 [Shi, Zhiwen; Sun, Yinghui; Zeng, Bo; Jin, Chenhao; Chang, Henry; Wang, Feng] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bechtel, Hans A.; Martin, Michael C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. [Wang, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Berweger, Samuel] NIST, Boulder, CO 80305 USA. [Berweger, Samuel; Raschke, Markus B.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Berweger, Samuel; Raschke, Markus B.] Univ Colorado, Dept Chem, Boulder, CO 80309 USA. [Berweger, Samuel; Raschke, Markus B.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Wang, Feng] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Wang, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Wang, F (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM markus.raschke@colorado.edu; fengwang76@berkeley.edu RI Shi, Zhiwen/C-4945-2013; Raschke, Markus/F-8023-2013; Sun, Yinghui/I-5947-2016; wang, Feng/I-5727-2015 OI Shi, Zhiwen/0000-0002-3928-2960; FU Office of Naval Research [N00014-13-1-0464]; David and Lucile Packard fellowship; Office of Biological and Environmental Research, through the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-12ER46893] FX Sample preparation and optical measurements in this work were mainly supported by the Office of Naval Research (award N00014-13-1-0464). F.W. acknowledges support from a David and Lucile Packard fellowship. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, and the BSISB is supported by the Office of Biological and Environmental Research, all through the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. M.R. acknowledges supported by the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award No. DE-FG02-12ER46893. Mention of commercial products is for informational purposes only; it does not imply NIST's recommendation or endorsement. NR 34 TC 12 Z9 12 U1 6 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2330-4022 J9 ACS PHOTONICS JI ACS Photonics PD JUL PY 2015 VL 2 IS 7 BP 790 EP 796 DI 10.1021/acsphotonics.5b00007 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics; Physics, Applied; Physics, Condensed Matter SC Science & Technology - Other Topics; Materials Science; Optics; Physics GA CN1OC UT WOS:000358188300002 ER PT J AU Majewski, J Andre, S Jones, E Chi, E Gabius, HJ AF Majewski, J. Andre, S. Jones, E. Chi, E. Gabius, H. -J. TI X-ray reflectivity and grazing incidence diffraction studies of interaction between human adhesion/growth-regulatory galectin-1 and DPPE-GM1 lipid monolayer at an air/water interface SO BIOCHEMISTRY-MOSCOW LA English DT Article DE agglutinin; Bragg peaks; ganglioside; lectin; X-ray diffraction/reflectivity ID AMPHIPHILIC JANUS GLYCODENDRIMERS; PANCREATIC-CARCINOMA MODEL; NEUROBLASTOMA-CELL-GROWTH; GM1 GANGLIOSIDE; LECTIN GALECTIN-1; BINDING-PROTEINS; SUGAR CODE; CARBOHYDRATE SPECIFICITY; BACTERIAL TOXINS; SURFACE BINDING AB The specific interaction of ganglioside GM1 with the homodimeric (prototype) endogenous lectin galectin-1 triggers growth regulation in tumor and activated effector T cells. This proven biorelevance directed interest to studying association of the lectin to a model surface, i.e. a 1,2-dihexadecanoyl-sn-glycero-3-phosphoethanolamine/ganglioside GM1 (80: 20 mol%) monolayer, at a bioeffective concentration. Surface expansion by the lectin insertion was detected at a surface pressure of 20 mN/m. On combining the methods of grazing incidence X-ray diffraction and X-ray reflectivity, a transient decrease in lipid-ordered phase of the monolayer was observed. The measured electron density distribution indicated that galectin-1 is oriented with its long axis in the surface plane, ideal for cis-crosslinking. The data reveal a conspicuous difference to the way the pentameric lectin part of the cholera toxin, another GM1-specific lectin, is bound to the monolayer. They also encourage further efforts to monitor effects of structurally different members of the galectin family such as the functionally antagonistic chimera-type galectin-3. C1 [Majewski, J.] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM USA. [Andre, S.; Gabius, H. -J.] Univ Munich, Fac Vet Med, Inst Physiol Chem, D-80539 Munich, Germany. [Jones, E.; Chi, E.] Univ New Mexico, Dept Chem & Biol Engn, Ctr Biomed Engn, Albuquerque, NM 87131 USA. RP Gabius, HJ (reprint author), Univ Munich, Fac Vet Med, Inst Physiol Chem, Vet Str 13, D-80539 Munich, Germany. EM gabius@tiph.vetmed.uni-muenchen.de OI Andre, Sabine/0000-0003-0850-0432; Gabius, Hans-Joachim/0000-0003-3467-3900 FU US Department of Energy [W-7405-ENG-36]; Oakridge Associated Universities Ralph E. Powe Junior Faculty Enhancement Award; EC [317297] FX The Los Alamos Neutron Science Center at the Los Alamos National Laboratory is funded by the US Department of Energy under contract W-7405-ENG-36. EYC and EJ would like to acknowledge funding from Oakridge Associated Universities Ralph E. Powe Junior Faculty Enhancement Award and the University of New Mexico Research Allocation Committee for supporting the X-ray scattering experiments. We would also like to acknowledge EC funding (GLYCOPHARM, contract No. 317297), HASYLAB for beam time, Dr. B. Struth for help with the reflectivity and grazing incidence diffraction experiments, and Drs. J. Domingo-Ekark and B. Friday for inspiring discussions. NR 80 TC 6 Z9 6 U1 1 U2 5 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 0006-2979 EI 0320-9725 J9 BIOCHEMISTRY-MOSCOW+ JI Biochem.-Moscow PD JUL PY 2015 VL 80 IS 7 BP 943 EP 956 DI 10.1134/S0006297915070135 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CN2KJ UT WOS:000358249500013 PM 26542007 ER PT J AU Wood, CE Hester, SD Chorley, BN Carswell, G George, MH Ward, W Vallanat, B Ren, HZ Fisher, A Lake, AD Okerberg, CV Gaillard, ET Moore, TM Deangelo, AB AF Wood, Charles E. Hester, Susan D. Chorley, Brian N. Carswell, Gleta George, Michael H. Ward, William Vallanat, Beena Ren, Hongzu Fisher, Anna Lake, April D. Okerberg, Carlin V. Gaillard, Elias T. Moore, Tanya M. Deangelo, Anthony B. TI Latent carcinogenicity of early-life exposure to dichloroacetic acid in mice SO CARCINOGENESIS LA English DT Article ID GLUTATHIONE TRANSFERASE-ZETA; MALE B6C3F(1) MOUSE; DOSE-RESPONSE; HEPATOCELLULAR-CARCINOMA; TRICHLOROACETIC-ACID; DRINKING-WATER; LIVER-TUMORS; CANCER-RISK; IN-UTERO; DISEASE AB This study demonstrates latent carcinogenic effects of the metabolic programming agent dichloroacetic acid following transient exposure in mice. Our findings highlight the potential for early-life postnatal changes in cell metabolism to alter cancer risk later in life.Environmental exposures occurring early in life may have an important influence on cancer risk later in life. Here, we investigated carryover effects of dichloroacetic acid (DCA), a small molecule analog of pyruvate with metabolic programming properties, on age-related incidence of liver cancer. The study followed a stop-exposure/promotion design in which 4-week-old male and female B6C3F1 mice received the following treatments: deionized water alone (dH(2)O, control); dH(2)O with 0.06% phenobarbital (PB), a mouse liver tumor promoter; or DCA (1.0, 2.0 or 3.5g/l) for 10 weeks followed by dH(2)O or PB (n = 20-30/group/sex). Pathology and molecular assessments were performed at 98 weeks of age. In the absence of PB, early-life exposure to DCA increased the incidence and number of hepatocellular tumors in male and female mice compared with controls. Significant dose trends were observed in both sexes. At the high dose level, 10 weeks of prior DCA treatment induced comparable effects (a parts per thousand yen85% tumor incidence and number) to those seen after continuous lifetime exposure. Prior DCA treatment did not enhance or inhibit the carcinogenic effects of PB, induce persistent liver cytotoxicity or preneoplastic changes on histopathology or alter DNA sequence variant profiles within liver tumors compared with controls. Distinct changes in liver messenger RNA and micro RNA profiles associated with prior DCA treatment were not apparent at 98 weeks. Our findings demonstrate that early-life exposure to DCA may be as carcinogenic as life-long exposures, potentially via epigenetic-mediated effects related to cellular metabolism. C1 [Wood, Charles E.; Hester, Susan D.; Chorley, Brian N.; Carswell, Gleta; George, Michael H.; Ward, William; Vallanat, Beena; Ren, Hongzu; Fisher, Anna; Lake, April D.; Moore, Tanya M.; Deangelo, Anthony B.] US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC 27711 USA. [Lake, April D.] Univ N Carolina, Curriculum Toxicol, Chapel Hill, NC 27713 USA. [Lake, April D.] US EPA, Oak Ridge Inst Sci & Educ ORISE, Res Triangle Pk, NC 27711 USA. [Okerberg, Carlin V.; Gaillard, Elias T.] Expt Pathol Labs, Morrisville, NC 27560 USA. RP Wood, CE (reprint author), US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC 27711 USA. EM wood.charles@epa.gov FU U.S. EPA Office of Research and Development FX The U.S. EPA Office of Research and Development. NR 53 TC 1 Z9 1 U1 3 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0143-3334 EI 1460-2180 J9 CARCINOGENESIS JI Carcinogenesis PD JUL PY 2015 VL 36 IS 7 BP 782 EP 791 DI 10.1093/carcin/bgv057 PG 10 WC Oncology SC Oncology GA CN1JN UT WOS:000358175700009 PM 25913432 ER PT J AU Jiang, N Tran, H AF Jiang, Nan Hoang Tran TI Analysis of a Stabilized CNLF Method with Fast Slow Wave Splittings for Flow Problems SO COMPUTATIONAL METHODS IN APPLIED MATHEMATICS LA English DT Article DE CNLF; NSE; Stabilization; Fast-Slow Wave Splitting ID NAVIER-STOKES EQUATIONS; TIME DISCRETIZATION; EVOLUTION-EQUATIONS; NUMERICAL-ANALYSIS; APPROXIMATION; REGULARIZATION; IMPLICIT; EXPLICIT; FILTER AB In this work, we study Crank-Nicolson leap-frog (CNLF) methods with fast-slow wave splittings for Navier-Stokes equations (NSE) with a rotation/Coriolis force term, which is a simplification of geophysical flows. We propose a new stabilized CNLF method where the added stabilization completely removes the method's CFL time step condition. A comprehensive stability and error analysis is given. We also prove that for Oseen equations with the rotation term, the unstable mode (for which u(n+1) + u(n-1) equivalent to 0) of CNLF is asymptotically stable. Numerical results are provided to verify the stability and the convergence of the methods. C1 [Jiang, Nan] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. [Hoang Tran] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Jiang, N (reprint author), Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. EM njiang@fsu.edu; tranha@ornl.gov OI Jiang, Nan/0000-0002-1080-258X FU NSF [DMS 1216465]; AFOSR [FA 9550-12-1-0191] FX The authors were partially supported by NSF grant DMS 1216465 and AFOSR grant FA 9550-12-1-0191. NR 37 TC 0 Z9 0 U1 1 U2 1 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 1609-4840 EI 1609-9389 J9 COMPUT METH APPL MAT JI Comput. Methods Appl. Math. PD JUL PY 2015 VL 15 IS 3 BP 307 EP 330 DI 10.1515/cmam-2015-0010 PG 24 WC Mathematics, Applied SC Mathematics GA CN3KJ UT WOS:000358324700005 ER PT J AU GopiReddy, LR Tolbert, LM Ozpineci, B Pinto, JOP AF GopiReddy, Lakshmi Reddy Tolbert, Leon M. Ozpineci, Burak Pinto, Joao O. P. TI Rainflow Algorithm-Based Lifetime Estimation of Power Semiconductors in Utility Applications SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS LA English DT Article DE Cycle counting; lifetime estimation; power semiconductor reliability; rainflow algorithms; STATCOM ID DEVICE RELIABILITY; PREDICTION; SYSTEMS; TEMPERATURE; TOPOLOGIES; MODULES; IGBT AB Rainflow algorithms are one of the popular counting methods used in fatigue and failure analysis in conjunction with semiconductor lifetime estimation models. However, the rain-flow algorithm used in power semiconductor reliability does not consider the time-dependent mean temperature calculation. The equivalent temperature calculation proposed by Nagode et al. is applied to semiconductor lifetime estimation in this paper. A month-long arc furnace load profile is used as a test profile to estimate temperatures in insulated-gate bipolar transistors (IGBTs) in a STATCOM for reactive compensation of load. The degradation in the life of the IGBT power device is predicted based on time-dependent temperature calculation. C1 [GopiReddy, Lakshmi Reddy; Tolbert, Leon M.; Ozpineci, Burak] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Tolbert, Leon M.; Ozpineci, Burak] Oak Ridge Natl Lab, Power Elect & Elect Machinery Res Grp PEEMRG, Knoxville, TN 37932 USA. [Pinto, Joao O. P.] Univ Fed Mato Grosso do Sul, Dept Elect Engn, BR-79070900 Campo Grande, Brazil. RP GopiReddy, LR (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. EM lgopired@utk.edu; tolbert@utk.edu; burak@ornl.gov; joaonofre@gmail.com OI Ozpineci, Burak/0000-0002-1672-3348; Tolbert, Leon/0000-0002-7285-609X FU U.S. Department of Energy; Engineering Research Center Program of the National Science Foundation and DOE under NSF [EEC-1041877]; CURENT Industry Partnership Program FX Paper 2014-PEDCC-0495.R1, presented at the 2014 IEEE Applied Power Electronics Conference and Exposition, Fort Worth, TX, USA, March 16-20, and approved for publication in the IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS by the Power Electronic Devices and Components Committee of the IEEE Industry Applications Society. This work was supported in part by the U.S. Department of Energy. This work made use of Engineering Research Center Shared Facilities supported by the Engineering Research Center Program of the National Science Foundation and DOE under NSF Award Number EEC-1041877 and the CURENT Industry Partnership Program. NR 32 TC 5 Z9 5 U1 3 U2 18 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0093-9994 EI 1939-9367 J9 IEEE T IND APPL JI IEEE Trans. Ind. Appl. PD JUL-AUG PY 2015 VL 51 IS 4 BP 3368 EP 3375 DI 10.1109/TIA.2015.2407055 PG 8 WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic SC Engineering GA CN2MN UT WOS:000358255700068 ER PT J AU Berdnikov, VV Somov, SV Pentchev, L AF Berdnikov, V. V. Somov, S. V. Pentchev, L. TI Use of cluster counting technique for particle identification in a drift chamber with the cathode strip readout SO INSTRUMENTS AND EXPERIMENTAL TECHNIQUES LA English DT Article ID IONIZATION AB The possibility of using the clusters counting technique for particle identification in a drift chamber with the cathode strip readout is experimentally investigated. Results of counting of primary ionization clusters on a relativistic particle track, as well as results of computer simulation of pion, kaon, and proton identification in the momentum range of 1-8 GeV/c, are presented. C1 [Berdnikov, V. V.; Somov, S. V.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Pentchev, L.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Berdnikov, VV (reprint author), Natl Res Nucl Univ MEPhI, Kashirskoe Sh 31, Moscow 115409, Russia. EM vvberdnikov@gmail.com FU Jefferson Science Associates, LLC; United States Department of Energy [DOE_AC05_06OR23177] FX This work was performed by the National Research Nuclear University MEPhI in collaboration with the Thomas Jefferson Accelerator Facility as a part of the GlueX experiment and was supported by the Jefferson Science Associates, LLC, which performs the work of the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under US DOE contract no. DOE_AC05_06OR23177. NR 5 TC 1 Z9 1 U1 0 U2 2 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 0020-4412 EI 1608-3180 J9 INSTRUM EXP TECH+ JI Instrum. Exp. Tech. PD JUL PY 2015 VL 58 IS 4 BP 473 EP 477 DI 10.1134/S0020441215030185 PG 5 WC Engineering, Multidisciplinary; Instruments & Instrumentation SC Engineering; Instruments & Instrumentation GA CN4FB UT WOS:000358384700004 ER PT J AU Soniat, M Rogers, DM Rempe, SB AF Soniat, Marielle Rogers, David M. Rempe, Susan B. TI Dispersion- and Exchange-Corrected Density Functional Theory for Sodium Ion Hydration SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID INITIO MOLECULAR-DYNAMICS; QUASI-CHEMICAL THEORY; BASIS-SET LIMIT; AB-INITIO; COUPLED-CLUSTER; WATER CLUSTERS; LIQUID WATER; FREE-ENERGY; AQUEOUS-SOLUTIONS; HYDROGEN GAS AB A challenge in density functional theory is developing functionals that simultaneously describe intermolecular electron correlation and electron delocalization. Recent exchange-correlation functionals address those two issues by adding corrections important at long ranges: an atom-centered pairwise dispersion term to account for correlation and a modified long-range component of the electron exchange term to correct for delocalization. Here we investigate how those corrections influence the accuracy of binding free energy predictions for sodium-water clusters. We find that the dual-corrected omega B97X-D functional gives cluster binding energies closest to high-level ab initio methods (CCSD(T)). Binding energy decomposition shows that the omega B97X-D functional predicts the smallest ion water (pairwise) interaction energy and larger multibody contributions for a four-water cluster than most other functionals a trend consistent with CCSD(T) results. Also, omega B97X-D produces the smallest amounts of charge transfer and the least polarizable waters of the density functionals studied, which mimics the lower polarizability of CCSD. When compared with experimental binding tree energies, however, the exchange-corrected CAM-B3LYP functional performs best (error <1 kcal/mol), possibly because of its parametrization to experimental formation enthalpies. For clusters containing more than four waters, "split-shell" coordination must be considered to obtain accurate free energies in comparison with experiment. C1 [Soniat, Marielle] Univ New Orleans, Dept Chem, New Orleans, LA 70148 USA. [Rogers, David M.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Engn Sci, Albuquerque, NM 87123 USA. [Rogers, David M.] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. RP Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Engn Sci, Albuquerque, NM 87123 USA. EM slrempe@sandia.gov FU State of Louisiana Board of Regents; National Science Foundation under the NSF EPSCoR [EPS-1003897]; University of South Florida Research Foundation; National Science Foundation [PHYS-1066293]; U.S. Department of Energy [DE-AC04-94AL8500] FX M.S. gratefully acknowledges support from the State of Louisiana Board of Regents and the National Science Foundation under the NSF EPSCoR Cooperative Agreement No. EPS-1003897. D.M.R. acknowledges support from the University of South Florida Research Foundation. D.M.R. and S.B.R. acknowledge Sandia's LDRD program. This work was also supported in part by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL8500. NR 123 TC 7 Z9 7 U1 13 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD JUL PY 2015 VL 11 IS 7 BP 2958 EP 2967 DI 10.1021/acs.jctc.5b00357 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN0LJ UT WOS:000358104800007 PM 26575733 ER PT J AU Bereau, T Andrienko, D von Lilienfeld, OA AF Bereau, Tristan Andrienko, Denis von Lilienfeld, O. Anatole TI Transferable Atomic Multipole Machine Learning Models for Small Organic Molecules SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID INTERMOLECULAR INTERACTION ENERGIES; DENSITY-FUNCTIONAL THEORY; FORCE-FIELD; NONCOVALENT INTERACTIONS; COMPLEXES; DYNAMICS; DATABASE; KERNEL; ELECTROSTATICS; SIMULATIONS AB Accurate representation of the molecular electrostatic potential, which is often expanded in distributed multipole moments, is crucial for an efficient evaluation of intermolecular interactions. Here we introduce a machine learning model for multipole coefficients of atom types H, C, O, N, S, F, and Cl in any molecular conformation. The model is trained on quantum-chemical results for atoms in varying chemical environments drawn from thousands of organic molecules. Multipoles in systems with neutral, cationic, and anionic molecular charge states are treated with individual models. The models' predictive accuracy and applicability are illustrated by evaluating intermolecular interaction energies of nearly 1,000 dimers and the cohesive energy of the benzene crystal. C1 [Bereau, Tristan; Andrienko, Denis] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. [von Lilienfeld, O. Anatole] Univ Basel, Inst Phys Chem, CH-4056 Basel, Switzerland. [von Lilienfeld, O. Anatole] Univ Basel, Natl Ctr Computat Design & Discovery Novel Mat, Dept Chem, CH-4056 Basel, Switzerland. [von Lilienfeld, O. Anatole] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. RP Bereau, T (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany. EM bereau@mpip-mainz.mpg.de; anatole.vonlilienfeld@unibas.ch RI MPIP, Theory/I-9884-2014; von Lilienfeld, O. Anatole/D-8529-2011; Andrienko, Denis/B-7721-2008; Bereau, Tristan/G-4987-2010 OI Andrienko, Denis/0000-0002-1541-1377; Bereau, Tristan/0000-0001-9945-1271 FU Swiss National Science Foundation [PP00P2_138932]; Office of Science of the U.S. Department of Energy (DOE) [DE-AC02-06CH11357] FX O.A.v.L. acknowledges funding from the Swiss National Science Foundation (Grant No. PP00P2_138932). This research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy (DOE) under Contract DE-AC02-06CH11357. NR 56 TC 4 Z9 4 U1 9 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD JUL PY 2015 VL 11 IS 7 BP 3225 EP 3233 DI 10.1021/acs.jctc.5b00301 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN0LJ UT WOS:000358104800033 PM 26575759 ER PT J AU Moore, B Sun, HT Govind, N Kowalski, K Autschbach, J AF Moore, Barry, II Sun, Haitao Govind, Niranjan Kowalski, Karol Autschbach, Jochen TI Charge-Transfer Versus Charge-Transfer-Like Excitations Revisited SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID DENSITY-FUNCTIONAL THEORY; TRANSFER EXCITED-STATES; COUPLED-CLUSTER METHOD; FRONTIER ORBITAL ENERGIES; CYANINE DYES; BASIS-SETS; ELECTRONIC EXCITATION; DELOCALIZATION ERROR; OPTICAL-PROPERTIES; TRANSFER CHARACTER AB Criteria to assess charge-transfer (CT) and CT-like character of electronic excitations are examined. Time-dependent density functional theory (TDDFT) calculations with non-hybrid, hybrid, and tuned long-range corrected (LC) functionals are compared with coupledcluster (CC) benchmarks. The test set comprises an organic CT complex, two push pull donor acceptor chromophores, a cyanine dye, and several polycyclic aromatic hydrocarbons. Proper CT is easily identified. Excitations with significant density changes upon excitation within regions of close spatial proximity can also be diagnosed. For such excitations, the use of LC functionals in TDDFT sometimes leads to dramatic improvements of the singlet energies, similar to proper CT. It is shown that such CT-like excitations do not have the characteristics of physical charge transfer, and improvements with LC functionals may not be obtained for the right reasons. The TDDFT triplet excitation energies are underestimated for all systems, often severely. For the CT-like candidates, the singlet triplet (SIT) separation changes from negative with a non-hybrid functional to positive with a tuned LC functional. For the cyanine, the S/T separation is systematically too large with TDDFT, leading to better error compensation for the singlet energy with a non-hybrid functional. C1 [Moore, Barry, II; Sun, Haitao; Autschbach, Jochen] SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. [Sun, Haitao] E China Normal Univ, Dept Phys, State Key Lab Precis Spect, Shanghai 200062, Peoples R China. [Govind, Niranjan; Kowalski, Karol] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Autschbach, J (reprint author), SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. EM jochena@buffalo.edu RI Sun, Haitao/O-8894-2016; Autschbach, Jochen/S-5472-2016 OI Autschbach, Jochen/0000-0001-9392-877X FU National Science Foundation [CHE-1265833]; China Scholarship Council; U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program [DE-SC0008666]; Department of Energy's Office of Biological and Environmental Research FX J.A. and B.M.II acknowledge support by the National Science Foundation, Grant No. CHE-1265833. J.A. thanks Prof. L. Kronik for constructive discussions on the topic of CT. H.S. is grateful for financial support by the China Scholarship Council. N.G. acknowledges support from the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program, under Award No. DE-SC0008666 for the analytical TDDFT excited-state gradients developments in NWChem. We thank the Center for Computational Research at the Univ. at Buffalo for providing and hosting computational resources. A portion of the calculations were performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory. NR 91 TC 16 Z9 16 U1 7 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD JUL PY 2015 VL 11 IS 7 BP 3305 EP 3320 DI 10.1021/acs.jctc.5b00335 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN0LJ UT WOS:000358104800040 PM 26575765 ER PT J AU Aradi, B Niklasson, AMN Frauenheim, T AF Aradi, Balint Niklasson, Anders M. N. Frauenheim, Thomas TI Extended Lagrangian Density Functional Tight-Binding Molecular Dynamics for Molecules and Solids SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID SIMULATIONS; INTEGRATORS AB A computationally fast quantum mechanical molecular dynamics scheme using an extended Lagrangian density functional tight-binding formulation has been developed and implemented in the DFTB+ electronic structure program package for simulations of solids and molecular systems. The scheme combines the computational speed of self-consistent density functional tight-binding theory with the efficiency and long-term accuracy of extended Lagrangian Born-Oppenheimer molecular dynamics. For systems without self-consistent charge instabilities, only a single diagonalization or construction of the single-particle density matrix is required in each time step. The molecular dynamics simulation scheme can be applied to a broad range of problems in materials science, chemistry, and biology. C1 [Aradi, Balint; Frauenheim, Thomas] Univ Bremen, Bremen Ctr Computat Mat Sci, D-28359 Bremen, Germany. [Niklasson, Anders M. N.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Aradi, B (reprint author), Univ Bremen, Bremen Ctr Computat Mat Sci, Fallturm 1, D-28359 Bremen, Germany. EM aradi@uni-bremen.de FU United States Department of Energy (U.S. DOE), Office of Basic Energy Sciences (FWP) [LANL2014E8AN] FX A.M.N.N. acknowledges support by the United States Department of Energy (U.S. DOE), Office of Basic Energy Sciences (FWP no. LANL2014E8AN). NR 38 TC 2 Z9 2 U1 4 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD JUL PY 2015 VL 11 IS 7 BP 3357 EP 3363 DI 10.1021/acs.jctc.5b00324 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN0LJ UT WOS:000358104800044 PM 26575769 ER PT J AU Fernandez-Rodriguez, J Toby, B van Veenendaal, M AF Fernandez-Rodriguez, Javier Toby, Brian van Veenendaal, Michel TI Xclaim: A graphical interface for the calculation of core-hole spectroscopies SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA LA English DT Article DE X-ray absorption spectroscopy; X-ray photoemission; Crystal field; Strongly correlated materials ID X-RAY-ABSORPTION; TRANSITION-METAL COMPOUNDS; ELECTRONIC-STRUCTURE; CIRCULAR-DICHROISM; CRYSTAL-FIELD; BRANCHING RATIO; 3D; PHOTOEMISSION; SPECTRA; DIHALIDES AB Xclaim (X-ray core level atomic multiplets) is a graphical interface for the calculation of core-hole spectroscopy and ground state properties within a charge-transfer multiplet model taking into account a many-body Hamiltonian with Coulomb, spin-orbit, crystal-field, and hybridization interactions. Using Coulomb and spin-orbit parameters calculated in the Hartree-Fock limit and ligand field parameters (crystal-field, hybridization and charge-transfer energy) the program calculates X-ray absorption spectroscopy (XAS), X-ray photoemission spectroscopy (XPS), photoemission spectroscopy (PES) and inverse photoemission (IPES). The program runs on Linux, Windows and MacOS platforms. (C) 2015 Elsevier B.V. All rights reserved. C1 [Fernandez-Rodriguez, Javier; van Veenendaal, Michel] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Fernandez-Rodriguez, Javier; Toby, Brian; van Veenendaal, Michel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Fernandez-Rodriguez, J (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. EM toby@anl.gov; veenendaal@niu.edu RI Toby, Brian/F-3176-2013 OI Toby, Brian/0000-0001-8793-8285 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-03ER46097]; Computational Materials Science Network (CMSCN) [DE-FG02-08ER46540, DE-SC0007091]; NIU Institute for Nanoscience, Engineering, and Technology; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We are thankful to D. Haskel, U. Staub, and J.A. Blanco for useful discussions. The periodic table was adapted from Robert Von Dreele's program pyFprime [47]. This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-03ER46097, the time-dependent X-ray spectroscopy collaboration as part of the Computational Materials Science Network (CMSCN) under Grants DE-FG02-08ER46540 and DE-SC0007091, and NIU Institute for Nanoscience, Engineering, and Technology. Work at Argonne National Laboratory was supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 43 TC 3 Z9 3 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0368-2048 EI 1873-2526 J9 J ELECTRON SPECTROSC JI J. Electron Spectrosc. Relat. Phenom. PD JUL PY 2015 VL 202 BP 81 EP 88 DI 10.1016/j.elspec.2015.03.010 PG 8 WC Spectroscopy SC Spectroscopy GA CM7VM UT WOS:000357904600014 ER PT J AU Zhao, L Klopf, JM Reece, CE Kelley, MJ AF Zhao, L. Klopf, J. M. Reece, C. E. Kelley, M. J. TI Laser polishing for topography management of accelerator cavity surfaces SO MATERIALWISSENSCHAFT UND WERKSTOFFTECHNIK LA English DT Article DE Laser polishing; topography; cavity surfaces AB Improved energy efficiency and reduced cost are greatly desired for advanced particle accelerators. Progress toward these goals can be made by atomically-smoothing the interior surface of the niobium superconducting radiofrequency (SRF) accelerator cavities at the heart of these machines. Laser polishing offers a green alternative to the present aggressive chemical processes. We found parameters suitable for polishing niobium in all surface conditions that are expected for cavity production. Careful measurement of the resulting surface chemistry revealed a modest thinning of the surface oxide layer, but no contamination. C1 [Zhao, L.; Klopf, J. M.; Kelley, M. J.] Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23187 USA. [Zhao, L.; Reece, C. E.; Kelley, M. J.] Jefferson Lab, Newport News, VA 23606 USA. RP Kelley, MJ (reprint author), Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23187 USA. EM mkelley@jlab.org FU Office of High Energy Physics of the U.S. Department of Energy [SC0007907]; U.S. DOE [DE-AC05-06OR23177] FX Liang Zhao is grateful for support by the Office of High Energy Physics of the U.S. Department of Energy under grant SC0007907 to the College of William & Mary. The experiment was conducted at Jefferson Lab. Partly authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. The U.S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce this manuscript for U.S. Government purposes. Thanks to staff at the College of William and Mary characterization lab, especially Olga Trofimova for the AFM images. We thank Fred Stevie and Chuanzhen Zhou of North Carolina State University and Jay Tuggle of Virginia Tech for their assistance with materials characterization. NR 19 TC 1 Z9 1 U1 3 U2 10 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0933-5137 EI 1521-4052 J9 MATERIALWISS WERKST JI Materialwiss. Werkstofftech. PD JUL PY 2015 VL 46 IS 7 BP 675 EP 685 DI 10.1002/mawe.201500323 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA CN2KD UT WOS:000358248900003 ER PT J AU Ye, B Rest, J Kim, YS Hofman, G Dionne, B AF Ye, Bei Rest, Jeff Kim, Yeon Soo Hofman, Gerard Dionne, Benoit TI DART ANALYSIS OF IRRADIATION BEHAVIOR OF U-Mo/Al DISPERSION FUELS SO NUCLEAR TECHNOLOGY LA English DT Article DE irradiation behavior modeling; U-Mo/Al dispersion fuel; irradiation-induced swelling ID MO ALLOY; LOW-TEMPERATURE; AL MATRIX; ALUMINUM; PRODUCT; GROWTH AB DART (Dispersion Analysis Research Tool) is a computational code developed for integrated simulation of the irradiation behavior of aluminum dispersion fuels used in research reactors. The DART computational code uses a mechanistic fission gas behavior model and a set of up-to-date empirical correlations to simulate the fuel morphology change as a function of burnup. Integrating a thermal calculation subroutine enables fuel material properties to be updated at each time step. This paper describes the primary physical models that form the basis of the DART computational code. A baseline validation was performed through the modeling of several U-Mo/Al mini-plate tests (RERTR-6, 7, and 9) in the Advanced Test Reactor (ATR). A demonstration problem is also presented through the calculation of fuel plate swelling and constituent volume fractions in full-sized plates from the AFIP-1 test in ATR. C1 [Ye, Bei; Rest, Jeff; Kim, Yeon Soo; Hofman, Gerard; Dionne, Benoit] Argonne Natl Lab, Argonne, IL 60439 USA. RP Ye, B (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA. EM bye@anl.gov FU U.S. Department of Energy, Office of Global Threat Reduction [NA-21]; UChicago Argonne, LLC [DE-AC-02-06CH11357]; U.S. Department of Energy [DE-AC-02-06CH11357] FX The authors would like to acknowledge D. Wachs and A. Robinson from INL for PIE data. The physics data from the AFIP-1 test was made available by G. Chang, M. Lillo, and D. M. Perez from INL, which is appreciated. This work was supported by the U.S. Department of Energy, Office of Global Threat Reduction (NA-21), National Nuclear Security Administration, under contract DE-AC-02-06CH11357 between UChicago Argonne, LLC, and the U.S. Department of Energy. NR 39 TC 2 Z9 2 U1 1 U2 4 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD JUL PY 2015 VL 191 IS 1 BP 27 EP 40 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CN0LF UT WOS:000358104400003 ER PT J AU Davis, KL Knudson, DL Rempe, JL Crepeau, JC Solstad, S AF Davis, K. L. Knudson, D. L. Rempe, J. L. Crepeau, J. C. Solstad, S. TI DESIGN AND LABORATORY EVALUATION OF FUTURE ELONGATION AND DIAMETER MEASUREMENTS AT THE ADVANCED TEST REACTOR SO NUCLEAR TECHNOLOGY LA English DT Article DE in-pile deformation; measurement instrumentation AB New materials are being considered for fuel, cladding, and structures in next-generation and existing nuclear reactors. Such materials can undergo significant dimensional and physical changes during high-temperature irradiation. To accurately predict these changes, real-time data must be obtained under prototypic irradiation conditions for model development and validation. To provide these data, programs such as the Advanced Test Reactor (ATR) National Scientific Users Facility (NSUF) have funded researchers at the Idaho National Laboratory (INL) High Temperature Test Laboratory (HTTL) to develop several instrumented test rigs to obtain data in real time from specimens irradiated in well-controlled pressurized water reactor (PWR) coolant conditions in ATR. This technical note reports the status of INL efforts to develop and evaluate prototype test rigs that rely on linear variable differential transformers (LVDTs) in laboratory settings. Although similar LVDT-based test rigs have been deployed in lower-flux materials testing reactors (MTRs), this effort is unique because it relies on robust LVDTs that can withstand higher temperatures and higher fluxes than often found in other MTR irradiations. Specifically, the test rigs are designed for detecting changes in the length and diameter of specimens irradiated in ATR PWR loops. Once implemented, these test rigs will provide ATR users with unique capabilities that are sorely needed to obtain measurements such as elongation caused by thermal expansion and/or creep loading and diameter changes associated with fuel and cladding swelling, pellet-cladding interaction, and crud buildup. C1 [Davis, K. L.; Knudson, D. L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Rempe, J. L.] Rempe & Associates LLC, Idaho Falls, ID 83404 USA. [Crepeau, J. C.] Univ Idaho, Dept Mech Engn, Moscow, ID 83844 USA. [Solstad, S.] Inst Energy Technol, N-1777 Halden, Norway. RP Davis, KL (reprint author), Idaho Natl Lab, POB 1625,Mail Stop 3531, Idaho Falls, ID 83415 USA. EM Kurt.Davis@inl.gov OI Rempe, Joy/0000-0001-5527-3549 FU DOE-NE under Idaho Operations Office contract [DE AC07 05ID14517] FX This work was supported by the DOE-NE under Idaho Operations Office contract DE AC07 05ID14517. NR 19 TC 0 Z9 0 U1 2 U2 2 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD JUL PY 2015 VL 191 IS 1 BP 92 EP 105 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CN0LF UT WOS:000358104400007 ER PT J AU Millsap, DW Cournoyer, ME Landsberger, S Tesmer, J Wang, Y AF Millsap, D. W. Cournoyer, M. E. Landsberger, S. Tesmer, J. Wang, Y. TI DEGRADATION OF NYLON 6,6 FIRE-SUPPRESSION CASING FROM PLUTONIUM GLOVE BOXES UNDER ALPHA AND NEUTRON IRRADIATION SO NUCLEAR TECHNOLOGY LA English DT Article DE alpha ion beam; glove box; nylon 6,6 AB Nylon 6,6 tensile specimens, conforming to the casing for self-contained fire extinguisher systems, have been irradiated using both an accelerator He++ ion beam and a 5-Ci PuBe neutron source to model the radiation damage these systems would likely incur over a lifetime of operation within glove boxes. Following irradiation, these samples were mechanically tested using standard practices as described in ASTM D638. The results of the He++ study indicate that the tensile strength of the nylon specimens undergoes some slight (<10%) degradation while other properties of the samples, such as elongation and tangent modulus, appear to fluctuate with increasing dose levels. The He++-irradiated specimens also have a noticeable level of discoloration corresponding to increasing levels of dose. The neutron-irradiated samples show a higher degree of mechanical degradation than the He++-irradiated samples. C1 [Millsap, D. W.; Landsberger, S.] Univ Texas Austin, Nucl Engn Teaching Lab, Austin, TX 78712 USA. [Cournoyer, M. E.; Tesmer, J.; Wang, Y.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Millsap, DW (reprint author), Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd, Austin, TX 78712 USA. EM s.landsberger@mail.utexas.edu FU U.S. Department of Energy through LANL; Nuclear Materials Technology Division; Ion Beam Materials Laboratory of LANL FX This work was financially supported by the U.S. Department of Energy through LANL and was conducted at the University of Texas at Austin. The authors would like to thank the personnel at the Nuclear Engineering Teaching Laboratory at the University of Texas's Pickle Research Campus. Special thanks are also given to the personnel at the Nuclear Materials Technology Division and the Ion Beam Materials Laboratory of LANL for their support throughout the completion of this research. NR 11 TC 0 Z9 0 U1 0 U2 0 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD JUL PY 2015 VL 191 IS 1 BP 106 EP 112 PG 7 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CN0LF UT WOS:000358104400008 ER PT J AU Leander, R Lenhart, S Protopopescu, V AF Leander, Rachel Lenhart, Suzanne Protopopescu, Vladimir TI Optimal control of continuous systems with impulse controls SO OPTIMAL CONTROL APPLICATIONS & METHODS LA English DT Article DE continuous systems; impulse control; discrete time optimal control ID COMPARTMENT MODELS AB Impulse control problems, in which a continuously evolving state is modified by discrete control actions, have applications in epidemiology, medicine, and ecology. In this paper, we present a simple method for solving impulse control problems for systems of differential equations. In particular, we show how impulse control problems can be reformulated and solved as discrete optimal control problems. The method is illustrated with two examples. Published 2014. This article has been contributed to by US Government employees and their work is in the public domain in the USA. C1 [Leander, Rachel] Middle Tennessee State Univ, Dept Math Sci, Murfreesboro, TN 37132 USA. [Lenhart, Suzanne] Univ Tennessee, Dept Math, Knoxville, TN 37996 USA. [Protopopescu, Vladimir] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN USA. RP Leander, R (reprint author), Middle Tennessee State Univ, Dept Math Sci, Murfreesboro, TN 37132 USA. EM rleander@mbi.osu.edu FU National Science Foundation [0931642]; National Institute for Mathematical and Biological Synthesis - National Science Foundation; US Department of Homeland Security; US Department of Agriculture through NSF [EF-0832858]; University of Tennessee; University of Tennessee Center for Business and Economic Research; US Department of Energy [DE-AC05-00OR22725] FX Leander's work is supported by the National Science Foundation under Agreement No. 0931642. Lenhart's work is partially supported by the National Institute for Mathematical and Biological Synthesis, sponsored by the National Science Foundation, the US Department of Homeland Security, and the US Department of Agriculture through NSF Award EF-0832858, with additional support from The University of Tennessee. Lenhart is also partially supported by the University of Tennessee Center for Business and Economic Research. The Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the US Department of Energy under contract DE-AC05-00OR22725. NR 20 TC 0 Z9 0 U1 1 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0143-2087 EI 1099-1514 J9 OPTIM CONTR APPL MET JI Optim. Control Appl. Methods PD JUL-AUG PY 2015 VL 36 IS 4 BP 535 EP 549 DI 10.1002/oca.2128 PG 15 WC Automation & Control Systems; Operations Research & Management Science; Mathematics, Applied SC Automation & Control Systems; Operations Research & Management Science; Mathematics GA CN1HD UT WOS:000358168400009 ER PT J AU Burr, T Hamada, MS AF Burr, T. Hamada, M. S. TI A Multiplicative Model for Gauge R & R Studies SO QUALITY AND RELIABILITY ENGINEERING INTERNATIONAL LA English DT Article DE Bayesian; repeatability; reproducibility AB We introduce a multiplicative measurement error model and analyze a gauge R & R study with the new model using data from a sample exchange program. Some aspects of designing a gauge R & R study are considered. Also, we analyze data from a factorial experiment where the measurement error arises from the new model using a simultaneous analysis of experimental and gauge R & R study data. WinBUGS code for these analyses is provided. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Burr, T.; Hamada, M. S.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. RP Hamada, MS (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663, Los Alamos, NM 87545 USA. EM hamada@lanl.gov NR 11 TC 1 Z9 1 U1 2 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0748-8017 EI 1099-1638 J9 QUAL RELIAB ENG INT JI Qual. Reliab. Eng. Int. PD JUL PY 2015 VL 31 IS 5 BP 801 EP 809 DI 10.1002/qre.1638 PG 9 WC Engineering, Multidisciplinary; Engineering, Industrial; Operations Research & Management Science SC Engineering; Operations Research & Management Science GA CN4XJ UT WOS:000358433500008 ER PT J AU Kristo, MJ Keegan, E Colella, M Williams, R Lindvall, R Eppich, G Roberts, S Borg, L Gaffney, A Plaue, J Knight, K Loi, E Hotchkis, M Moody, K Singleton, M Robel, M Hutcheon, I AF Kristo, Michael Joseph Keegan, Elizabeth Colella, Michael Williams, Ross Lindvall, Rachel Eppich, Gary Roberts, Sarah Borg, Lars Gaffney, Amy Plaue, Jonathan Knight, Kim Loi, Elaine Hotchkis, Michael Moody, Kenton Singleton, Michael Robel, Martin Hutcheon, Ian TI Nuclear forensic analysis of uranium oxide powders interdicted in Victoria, Australia SO RADIOCHIMICA ACTA LA English DT Article DE Nuclear forensics; origin assessment; scanning electron microscopy (SEM); X-ray diffraction; inductively coupled plasma mass spectrometry; depleted uranium ID MULTICOMPONENT ISOTOPE SEPARATION; WATERS AB Nuclear forensic analysis was conducted on two uranium samples confiscated during a police investigation in Victoria, Australia. The first sample, designated NSR-F-270409-1, was a depleted uranium powder of moderate purity (similar to 1000 mu g/g total elemental impurities). The chemical form of the uranium was a compound similar to K-2(UO2)(3)O-4 center dot 4H(2)O. While aliquoting NSR-F-270409-1 for analysis, the body and head of a Tineid moth was discovered in the sample. The second sample, designated NSRF-270409-2, was also a depleted uranium powder. It was of reasonably high purity (similar to 380 mu g/g total elemental impurities). The chemical form of the uranium was primarily UO3 center dot 2H(2)O, with minor phases of U3O8 and UO2. While aliquoting NSR-F-270409-2 for analysis, a metal staple of unknown origin was discovered in the sample. The presence of U-236 and U-232 in both samples indicates that the uranium feed stocks for these samples experienced a neutron flux at some point in their history. The reactor burn-up calculated from the isotopic composition of the uranium is consistent with that of spent fuel from natural uranium (NU) fueled Pu production. These nuclear forensic conclusions allow us to categorically exclude Australia as the origin of the material and greatly reduce the number of candidate sources. C1 [Kristo, Michael Joseph; Williams, Ross; Lindvall, Rachel; Eppich, Gary; Roberts, Sarah; Borg, Lars; Gaffney, Amy; Plaue, Jonathan; Knight, Kim; Moody, Kenton; Singleton, Michael; Robel, Martin; Hutcheon, Ian] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Keegan, Elizabeth; Colella, Michael; Loi, Elaine; Hotchkis, Michael] Australian Nucl Sci & Technol Org, Kirrawee, NSW 2232, Australia. RP Kristo, MJ (reprint author), Lawrence Livermore Natl Lab, POB 808,L-186, Livermore, CA 94551 USA. EM kristo2@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344]; Department of Energy/National Nuclear Security Administration Office of Nuclear Controls [NA-242]; Department of Energy/National Nuclear Security Administration Office of Nuclear Noncompliance Verification [NA-243] FX Lawrence Livermore National Laboratory performed this work under the auspices of the U.S. Department of Energy under Contract DE-AC52-07NA27344. Funding for this work was provided by the Department of Energy/National Nuclear Security Administration Office of Nuclear Controls (NA-242) and utilized capabilities developed with funding from Department of Energy/National Nuclear Security Administration Office of Nuclear Noncompliance Verification (NA-243). NR 26 TC 2 Z9 2 U1 5 U2 37 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PD JUL PY 2015 VL 103 IS 7 BP 487 EP 500 DI 10.1515/ract-2014-2363 PG 14 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA CN3UW UT WOS:000358354100003 ER PT J AU Rhee, H Tucker, MT Whittington, WR Horstemeyer, MF Lim, H AF Rhee, Hongjoo Tucker, Matthew T. Whittington, Wilburn R. Horstemeyer, Mark F. Lim, Hyeona TI Structure-property responses of bio-inspired synthetic foams at low and high strain rates SO SCIENCE AND ENGINEERING OF COMPOSITE MATERIALS LA English DT Article DE aluminum foams; low and high strain rate mechanical response; structure-property relations; turtle shell ID COMPRESSIVE BEHAVIOR; ALUMINUM FOAM; MECHANICAL-PROPERTIES; TEMPERATURE; METAL AB Various aluminum foams were fabricated with a structure comparable to the Terrapene carolina (box turtle) shell hierarchy as a synthetic means of attaining the lightweight, yet impact-resistive, nature of the biological counterpart. Each foam was constructed from a single aluminum alloy but with different morphologies and foam densities. By borrowing from the sophistication of biological design, the aluminum foams were shown to exhibit robust mechanical performance. High strain rate experimentation, via split Hopkinson pressure bar, was utilized to reveal the strain rate sensitivity of the foams as well as a metric to compare impact performance. The structure-property relations, necessary for accurate material modeling, were also characterized by way of optical microscopy, scanning electron microscopy, energy dispersive X-ray spectroscopy, and nanoindentation tests. The robust varying mechanical performance was attributed to the biologically inspired materials design. C1 [Rhee, Hongjoo; Whittington, Wilburn R.; Horstemeyer, Mark F.] Mississippi State Univ, Ctr Adv Vehicular Syst, Mississippi State, MS 39762 USA. [Rhee, Hongjoo; Whittington, Wilburn R.; Horstemeyer, Mark F.] Mississippi State Univ, Dept Mech Engn, Mississippi State, MS 39762 USA. [Tucker, Matthew T.] Los Alamos Natl Lab, MST Grp 8, Los Alamos, NM 87545 USA. [Lim, Hyeona] Mississippi State Univ, Dept Math & Stat, Mississippi State, MS 39762 USA. RP Rhee, H (reprint author), Mississippi State Univ, Ctr Adv Vehicular Syst, Mississippi State, MS 39762 USA. EM hrhee@cavs.msstate.edu OI Horstemeyer, Mark/0000-0003-4230-0063 FU Center for Advanced Vehicular Systems at Mississippi State University under grant CAVS Initiatives [190000-060803-021000]; U.S. Department of Army (DOD) [TCN07173 07121203] FX The authors would like to acknowledge-the financial supports for this work from the Center for Advanced Vehicular Systems at Mississippi State University under grant CAVS Initiatives 190000-060803-021000 and the U.S. Department of Army (DOD) through grant TCN07173 07121203. They also thank Cymat Technologies, Ltd. for providing samples. NR 24 TC 0 Z9 0 U1 2 U2 10 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0792-1233 EI 2191-0359 J9 SCI ENG COMPOS MATER JI Sci. Eng. Compos. Mater. PD JUL PY 2015 VL 22 IS 4 BP 365 EP 373 DI 10.1515/secm-2013-0238 PG 9 WC Materials Science, Composites SC Materials Science GA CN3LF UT WOS:000358327000003 ER PT J AU Thimmaiah, S Miller, GJ AF Thimmaiah, Srinivasa Miller, Gordon J. TI Influence of Valence Electron Concentration on Laves Phases: Structures and Phase Stability of Pseudo-Binary MgZn2-xPdx SO ZEITSCHRIFT FUR ANORGANISCHE UND ALLGEMEINE CHEMIE LA English DT Article DE Laves phase; X-ray diffraction; Single crystal diffraction; Structure determination; Electronic structure ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; MG-CU-NI; STACKING VARIANTS; HYDROGEN STORAGE; CRYSTAL-STRUCTURES; ALLOY SYSTEMS; PART II; METALS AB A series of pseudo-binary compounds MgZn2-xPdx (0.15 x 1.0) were synthesized and structurally characterized to understand the role of valence electron concentration (vec) on the prototype Laves phase MgZn2 with Pd-substitution. Three distinctive phase regions were observed with respect to Pd content, all exhibiting fundamental Laves phase structures: 0.1 x 0.3 (MgNi2-type, hP24; MgZn1.80Pd0.20(2)), 0.4 x 0.6 (MgCu2-type, cF24; MgZn1.59Pd0.41(2)), and 0.62 x 0.8 (MgZn2-type, hP12: MgZn1.37Pd0.63(2)). Refinements from single-crystal X-ray diffraction indicated nearly statistical distributions of Pd and Zn atoms among the majority atom sites in these structures. Interestingly, the MgZn2-type structure re-emerges in MgZn2-xPdx at x approximate to 0.7 with the refined composition MgZn1.37(2)Pd0.63 and a c/a ratio of 1.59 compared to 1.64 for binary MgZn2. Electronic structure calculations on a model MgZn1.25Pd0.75 yielded a density of states (DOS) curve showing enhancement of a pseudogap at the Fermi level as a result of electronic stabilization due to the Pd addition. Moreover, integrated crystal orbital Hamilton population (ICOHP) values show significant increases of orbital interactions for (Zn,Pd)-(Zn,Pd) atom pairs within the majority atom substructure, i.e., within the Kagome nets as well as between a Kagome net and an apical site, from binary MgZn2 to the ternary MgZn1.25Pd0.75. Multi-centered bonding is evident from electron localization function (ELF) plots for MgZn1.25Pd0.75, an outcome which is in accordance with analysis of other Laves phases(.> {100}. The underlying surface-structure sensitivity can be attributed to the variation in low-coordinate surface cerium cations between {110} and {100} facets. To further enhance light absorption, Au nanoparticles (NPs) are deposited on CeO2 NRs to form Au/CeO2 plasmonic nanocomposites, which dramatically promotes the photoreactivity that is Au particle size- and excitation light wavelength-dependent. The mechanisms responsible for the enhancement of photocatalytic activity are discussed, highlighting the crucial role of photoexcited charge carrier transfer. C1 [Lei, Wanying; Zhang, Tingting; Liu, Gang; Liu, Minghua] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China. [Gu, Lin] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Liu, Ping; Rodriguez, Jose A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Liu, G (reprint author), Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China. EM liug@nanoctr.cn; liuminghua@nanoctr.cn RI Gu, Lin/D-9631-2011; Zhang, Tingting/N-9698-2015 OI Gu, Lin/0000-0002-7504-031X; FU National Natural Science Foundation of China [51272048] FX We gratefully acknowledge the financial support of this work from National Natural Science Foundation of China (51272048). NR 39 TC 18 Z9 18 U1 15 U2 125 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD JUL PY 2015 VL 5 IS 7 BP 4385 EP 4393 DI 10.1021/acscatal.5b00620 PG 9 WC Chemistry, Physical SC Chemistry GA CM4AO UT WOS:000357626800058 ER PT J AU Pelzer, AW Sturgeon, MR Yanez, AJ Chupka, G O'Brien, MH Katahira, R Cortright, RD Woods, L Beckham, GT Broadbelt, LJ AF Pelzer, Adam W. Sturgeon, Matthew R. Yanez, Abraham J. Chupka, Gina O'Brien, Marykate H. Katahira, Rui Cortright, Randy D. Woods, Liz Beckham, Gregg T. Broadbelt, Linda J. TI Acidolysis of alpha-O-4 Aryl-Ether Bonds in Lignin Model Compounds: A Modeling and Experimental Study SO ACS SUSTAINABLE CHEMISTRY & ENGINEERING LA English DT Article DE Density functional theory; Microkinetic modeling; alpha-O-4; Ether bond ID BENZYL PHENYL ETHER; MOLECULAR-WEIGHT PHENOLS; ACID DEGRADATION; AQUEOUS ACID; BIOFUEL PRODUCTION; ORGANIC-CHEMISTRY; HYDROLYSIS; CLEAVAGE; BIOMASS; WATER AB Lignocellulosic biomass offers a vast, renewable resource for the sustainable production of fuels and chemicals. To date, a commonly employed approach to depolymerize the polysaccharides in plant cell walls employs mineral acids, and upgrading strategies for the resulting sugars are under intense development. Although the behavior of cellulose and hemicellulose is reasonably well characterized, a more thorough understanding of lignin depolymerization mechanisms in acid environments is necessary to predict the fate of lignin under such conditions and ultimately to potentially make lignin a viable feedstock. To this end, dilute acid hydrolysis experiments were performed on two lignin model compounds containing the alpha-O-4 ether linkage at two temperatures concomitant with dilute acid pretreatment. Both primary and secondary products were tracked over time, giving insight into the reaction kinetics. The only difference between the two model compounds was the presence or absence of a methyl group on the alpha-carbon, with the former being typical of native lignin. It was found that methylation of the alpha-carbon increases the rate of reaction by an order of magnitude. Density functional theory calculations were performed on a proposed mechanism initiated by a nucleophilic attack on the alpha-carbon by water with a commensurate protonation of the ether oxygen. The values for the thermodynamics and kinetics derived from these calculations were used as the basis for a microkinetic model of the reaction. Results from this model are in good agreement with the experimental kinetic data for both lignin model compounds and provide useful insight into the primary pathways of alpha-O-4 scission reactions in acid-catalyzed lignin depolymerization. The distribution of primary and secondary products is interpreted as a function of two barriers of formation exhibiting opposite trends upon methylation of the alpha-carbon (one barrier is lowered while the other is increased). Such insights will be needed to construct a comprehensive model of how lignin behaves in a common deconstruction approach. C1 [Sturgeon, Matthew R.; Chupka, Gina; O'Brien, Marykate H.; Katahira, Rui; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Adv Biofuels Consortium, Golden, CO 80401 USA. [Sturgeon, Matthew R.; Chupka, Gina; O'Brien, Marykate H.; Katahira, Rui; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Cortright, Randy D.; Woods, Liz] Virent Inc, Madison, WI 53704 USA. [Pelzer, Adam W.; Yanez, Abraham J.; Broadbelt, Linda J.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. RP Pelzer, AW (reprint author), Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. EM adam.pelzer@northwestern.edu; gregg.beckham@nrel.gov; broadbelt@northwestern.edu RI Broadbelt, Linda/B-7640-2009 FU National Science Foundation [CHE-1314063]; National Advanced Biofuels Consortium - DOE BioEnergy Technologies Office through American Recovery and Reinvestment Act Funds; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy [DE-EE0005006]; Virent, Inc. FX Work performed by A.W.P. was supported by the National Science Foundation under Grant No. CHE-1314063. We acknowledge funding from the National Advanced Biofuels Consortium, which was funded by the DOE BioEnergy Technologies Office through American Recovery and Reinvestment Act Funds. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also acknowledge support from the Department of Energy Grant No. DE-EE0005006 and Virent, Inc. NR 63 TC 5 Z9 5 U1 1 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2168-0485 J9 ACS SUSTAIN CHEM ENG JI ACS Sustain. Chem. Eng. PD JUL PY 2015 VL 3 IS 7 BP 1339 EP 1347 DI 10.1021/acssuschemeng.5b00070 PG 9 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Chemical SC Chemistry; Science & Technology - Other Topics; Engineering GA CM5EE UT WOS:000357708800011 ER PT J AU Karp, EM Resch, MG Donohoe, BS Ciesielski, PN O'Brien, MH Nill, JE Mittal, A Biddy, MJ Beckham, GT AF Karp, Eric M. Resch, Michael G. Donohoe, Bryon S. Ciesielski, Peter N. O'Brien, Marykate H. Nill, Jennifer E. Mittal, Ashutosh Biddy, Mary J. Beckham, Gregg T. TI Alkaline Pretreatment of Switchgrass SO ACS SUSTAINABLE CHEMISTRY & ENGINEERING LA English DT Article DE Biofuels; Lignin valorization; Enzymatic hydrolysis; Lignocellulose; Pulping ID DILUTE-ACID PRETREATMENT; CLEAN FRACTIONATION PRETREATMENT; SODIUM-HYDROXIDE PRETREATMENT; COMPARATIVE SUGAR RECOVERY; IONIC LIQUID PRETREATMENT; SODA-AQ DELIGNIFICATION; FIBER EXPLOSION AFEX; CORN STOVER; ENZYMATIC-HYDROLYSIS; CELL-WALL AB Alkaline pretreatment using sodium hydroxide offers a means to extract lignin and acetate from lignocellulosic biomass, in turn enabling higher enzymatic digestibility of the remaining polysaccharides and production of a lignin-enriched stream for potential valorization. Key criteria for alkaline pretreatment processes, which are important for commercial feasibility, include the minimization of carbohydrate loss during pretreatment and the ability to capture carbon lost to the liquor stream, much of which will be feedstock dependent. Here, we present a comprehensive study of alkaline pretreatment of switchgrass over NaOH loadings from 35 to 140 mg NaOH/g dry switchgrass and with a constant charge of 0.2% anthraquinone for pretreatment temperatures between 100 and 160 degrees C for 30 min. Full compositional analysis of the pretreated solids are reported as a function of pretreatment severity, along with the yields of each biomass component present in the process streams generated during pretreatment (pretreated solid, liquor, and wash fraction). The pretreated solids are further characterized through crystallinity measurements and electron microscopy. Additionally, enzymatic digestions of the residual solids are performed over a range of enzyme loadings for varying pretreatment severities. These results are compared to our recent work with alkaline pretreatment of corn stover using the ratio of lignin fractionation to carbohydrate retention (in the solids after pretreatment), which highlights the greater recalcitrance of switchgrass relative to corn stover. Specifically, compared to corn stover, switchgrass requires approximately twice the NaOH loading to achieve identical delignification and high enzymatic digestibility. From this work, the optimal pretreatment conditions for switchgrass are suggested to be 154 mg NaOH/g dry switchgrass at 130 degrees C for 30 min at temperature. The results from these bench-scale experiments will serve as a guide to scale up processes for the optimization of lignin removal while minimizing carbohydrate loss during alkaline pretreatment. C1 [Karp, Eric M.; Resch, Michael G.; O'Brien, Marykate H.; Nill, Jennifer E.; Biddy, Mary J.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Donohoe, Bryon S.; Ciesielski, Peter N.; Mittal, Ashutosh] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. RP Beckham, GT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM gregg.beckham@nrel.gov OI Nill, Jennifer/0000-0002-9274-4650 FU U.S. Department of Energy BioEnergy Technologies Office; U.S. Government FX The authors thank the U.S. Department of Energy BioEnergy Technologies Office for funding this work. We also thank J. B. Sluiter for helpful discussions. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 73 TC 16 Z9 16 U1 4 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2168-0485 J9 ACS SUSTAIN CHEM ENG JI ACS Sustain. Chem. Eng. PD JUL PY 2015 VL 3 IS 7 BP 1479 EP 1491 DI 10.1021/acssuschemeng.5b00201 PG 13 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Chemical SC Chemistry; Science & Technology - Other Topics; Engineering GA CM5EE UT WOS:000357708800027 ER PT J AU Malinska, M Dauter, M Kowiel, M Jaskolski, M Dauter, Z AF Malinska, Maura Dauter, Miroslawa Kowiel, Marcin Jaskolski, Mariusz Dauter, Zbigniew TI Protonation and geometry of histidine rings SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE imidazole; histidine protonation; hydrogen bond; X-ray crystal structure; stereochemical restraints ID CAMBRIDGE STRUCTURAL DATABASE; CRYSTAL-STRUCTURES; STRUCTURE REFINEMENT; PROTEINS; RESOLUTION; RESTRAINTS; PARAMETERS; ACCURATE; STATE; BOND AB The presence of H atoms connected to either or both of the two N atoms of the imidazole moiety in a histidine residue affects the geometry of the five-membered ring. Analysis of the imidazole moieties found in histidine residues of atomic resolution protein crystal structures in the Protein Data Bank (PDB), and in small-molecule structures retrieved from the Cambridge Structural Database (CSD), identified characteristic patterns of bond lengths and angles related to the protonation state of the imidazole moiety. Using discriminant analysis, two functions could be defined, corresponding to linear combinations of the four most sensitive stereochemical parameters, two bond lengths (ND1-CE1 and CE1-NE2) and two endocyclic angles (-ND1- and -NE2-), that uniquely identify the protonation states of all imidazole moieties in the CSD and can be used to predict which N atom(s) of the histidine side chains in protein structures are protonated. Updated geometrical restraint target values are proposed for differently protonated histidine side chains for use in macromolecular refinement. C1 [Malinska, Maura; Dauter, Zbigniew] NCI, Synchrotron Radiat Res Sect, MCL, Argonne Natl Lab, Argonne, IL 60439 USA. [Dauter, Miroslawa] Leidos Biomedical Res Inc, Basic Sci Program, Argonne Natl Lab, Argonne, IL 60439 USA. [Kowiel, Marcin] Poznan Univ Med Sci, Dept Organ Chem, Poznan, Poland. [Jaskolski, Mariusz] Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, PL-60780 Poznan, Poland. [Jaskolski, Mariusz] Polish Acad Sci, Inst Bioorgan Chem, Ctr Biocrystallog Res, Poznan, Poland. RP Dauter, Z (reprint author), NCI, Synchrotron Radiat Res Sect, MCL, Argonne Natl Lab, Argonne, IL 60439 USA. EM dauter@anl.gov OI Malinska, Maura/0000-0002-7138-7041 FU Intramural Research Program of the National Cancer Institute, Center for Cancer Research; Federal funds from the National Cancer Institute, National Institutes of Health [HHSN261200800E]; National Science Center [2013/10/M/NZ1/00251]; Polish Ministry of Science and Higher Education through the 'Mobility Plus' program FX This project was supported in part by the Intramural Research Program of the National Cancer Institute, Center for Cancer Research and with Federal funds from the National Cancer Institute, National Institutes of Health (Contract No. HHSN261200800E). The content of this publication does not necessarily reflect the views or policies of the US Department of Health and Human Services, nor does mention of trade names, commercial products, or organizations imply endorsement by the US Government. The collaboration of MJ and ZD was supported in part by a grant (2013/10/M/NZ1/00251) from the National Science Center. MM acknowledges the Polish Ministry of Science and Higher Education for financial support through the 'Mobility Plus' program. NR 31 TC 2 Z9 2 U1 2 U2 19 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD JUL PY 2015 VL 71 BP 1444 EP 1454 DI 10.1107/S1399004715007816 PN 7 PG 11 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA CM6VQ UT WOS:000357829500004 PM 26143916 ER PT J AU Carlin, JL Liu, C Newberg, HJ Beers, TC Chen, L Deng, LC Guhathakurta, P Hou, JL Hou, YH Lepine, S Li, GW Luo, AL Smith, MC Wu, Y Yang, M Yanny, B Zhang, HT Zheng, Z AF Carlin, Jeffrey L. Liu, Chao Newberg, Heidi Jo Beers, Timothy C. Chen, Li Deng, Licai Guhathakurta, Puragra Hou, Jinliang Hou, Yonghui Lepine, Sebastien Li, Guangwei Luo, A-Li Smith, Martin C. Wu, Yue Yang, Ming Yanny, Brian Zhang, Haotong Zheng, Zheng TI ESTIMATION OF DISTANCES TO STARS WITH STELLAR PARAMETERS FROM LAMOST SO ASTRONOMICAL JOURNAL LA English DT Article DE Galaxy: stellar content; Galaxy: structure; stars: distances; surveys ID VELOCITY EXPERIMENT RAVE; DATA RELEASE; THEORETICAL ISOCHRONES; TELESCOPE LAMOST; NSTARS PROJECT; PILOT SURVEY; MILKY-WAY; EVOLUTION; CATALOG; SAMPLE AB We present a method to estimate distances to stars with spectroscopically derived stellar parameters. The technique is a Bayesian approach with likelihood estimated via comparison of measured parameters to a grid of stellar isochrones, and returns a posterior probability density function for each star's absolute magnitude. This technique is tailored specifically to data from the Large Sky Area Multi-object Fiber Spectroscopic Telescope (LAMOST) survey. Because LAMOST obtains roughly 3000 stellar spectra simultaneously within each similar to 5 degrees diameter "plate" that is observed, we can use the stellar parameters of the observed stars to account for the stellar luminosity function and target selection effects. This removes biasing assumptions about the underlying populations, both due to predictions of the luminosity function from stellar evolution modeling, and from Galactic models of stellar populations along each line of sight. Using calibration data of stars with known distances and stellar parameters, we show that our method recovers distances for most stars within similar to 20%, but with some systematic overestimation of distances to halo giants. We apply our code to the LAMOST database, and show that the current precision of LAMOST stellar parameters permits measurements of distances with similar to 40% error bars. This precision should improve as the LAMOST data pipelines continue to be refined. C1 [Carlin, Jeffrey L.; Newberg, Heidi Jo] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Carlin, Jeffrey L.] Earlham Coll, Dept Phys & Astron, Richmond, IN 47374 USA. [Liu, Chao; Deng, Licai; Li, Guangwei; Luo, A-Li; Wu, Yue; Yang, Ming; Zhang, Haotong] Chinese Acad Sci, Key Lab Opt Astron, Natl Astron Observ, Beijing 100012, Peoples R China. [Beers, Timothy C.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Beers, Timothy C.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Chen, Li; Hou, Yonghui; Smith, Martin C.] Shanghai Astron Observ, Shanghai 200030, Peoples R China. [Guhathakurta, Puragra] Univ Calif Santa Cruz, Dept Astron & Astrophys, UCO Lick Observ, Santa Cruz, CA 95064 USA. [Hou, Jinliang] Chinese Acad Sci, Nanjing Inst Astron Opt & Technol, Natl Astron Observ, Nanjing 210042, Peoples R China. [Lepine, Sebastien] Georgia State Univ, Dept Phys & Astron, Atlanta, GA 30303 USA. [Yanny, Brian] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Zheng, Zheng] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. RP Carlin, JL (reprint author), Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. EM jeffreylcarlin@gmail.com RI Yang, Ming/G-5128-2015; OI Yang, Ming/0000-0001-8247-4936; Carlin, Jeffrey/0000-0002-3936-9628; Newberg, Heidi/0000-0001-8348-0983; Guhathakurta, Puragra/0000-0001-8867-4234; Liu, Chao/0000-0002-1802-6917 FU U.S. National Science Foundation [AST 09-37523, AST 14-09421]; Strategic Priority Research Program "The Emergence of Cosmological Structures" of the Chinese Academy of Sciences [XDB09000000]; National Key Basic Research Program of China [2014CB845700]; National Science Foundation of China [11373032, 11333003, 11403056]; Physics Frontiers Center/Joint Institute for Nuclear Astrophysics (JINA) - U.S. National Science Foundation [PHY 08-22648]; Physics Frontier Center/JINA Center for the Evolution of the Elements (JINA-CEE) - U.S. National Science Foundation [PHY 14-30152]; National Development and Reform Commission; National Aeronautics and Space Administration; National Science Foundation FX We thank the anonymous referee for careful and thoughtful comments. This work was supported by the U.S. National Science Foundation under grants AST 09-37523 and AST 14-09421. C. L. also acknowledges the Strategic Priority Research Program "The Emergence of Cosmological Structures" of the Chinese Academy of Sciences, grant No. XDB09000000, the National Key Basic Research Program of China, grants No. 2014CB845700, and the National Science Foundation of China, grants No. 11373032 and 11333003. T. C. B. acknowledges partial support from grant PHY 08-22648: Physics Frontiers Center/Joint Institute for Nuclear Astrophysics (JINA), and PHY 14-30152; Physics Frontier Center/JINA Center for the Evolution of the Elements (JINA-CEE), awarded by the U.S. National Science Foundation. W. Y. appreciates support from the National Science Foundation of China, grant No. 11403056. Guoshoujing Telescope (the Large Sky Area Multi-object Fiber Spectroscopic Telescope LAMOST) is a National Major Scientific Project built by the Chinese Academy of Sciences. Funding for the project has been provided by the National Development and Reform Commission. LAMOST is operated and managed by the National Astronomical Observatories, Chinese Academy of Sciences. This publication makes use of data products from the 2MASS, which is a joint project of the University of Massachusetts and the Infrared Processing and Analysis Center/California Institute of Technology, funded by the National Aeronautics and Space Administration and the National Science Foundation. NR 43 TC 6 Z9 6 U1 2 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-6256 EI 1538-3881 J9 ASTRON J JI Astron. J. PD JUL PY 2015 VL 150 IS 1 AR 4 DI 10.1088/0004-6256/150/1/4 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CM5QU UT WOS:000357744400004 ER PT J AU Wang, SYS Huang, WR Yoon, JH AF Wang, Shih-Yu Simon Huang, Wan-Ru Yoon, Jin-Ho TI The North American winter 'dipole' and extremes activity: a CMIP5 assessment SO ATMOSPHERIC SCIENCE LETTERS LA English DT Article DE California drought; dipole; west Pacific warming; ENSO precursor ID EL-NINO; ARCTIC AMPLIFICATION; HEAT WAVES; CIRCULATION; PACIFIC; MODEL; ENSO; SIMULATIONS; OCEAN; TELECONNECTIONS AB The 2013-2014 winter in North America brought intense drought in the West and severe cold in the East. The circulation anomalies were characterized as a dipole: an amplified upper-level ridge over the West Coast and a deepened trough over the central-eastern United States. A previous study using a single model has linked the dipole to the El Nino precursor and found that this link has strengthened in recent years. Here, 17 models from the Coupled Model Intercomparison Project Phase 5 are used to examine the dipole activity. Most models capture the dipole and its association with El Nino precursor and project this association to strengthen. C1 [Wang, Shih-Yu Simon] Utah State Univ, Dept Plants Soils & Climate, Utah Climate Ctr, Logan, UT 84322 USA. [Huang, Wan-Ru] Natl Taiwan Normal Univ, Dept Earth Sci, Taipei, Taiwan. [Yoon, Jin-Ho] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wang, SYS (reprint author), Utah State Univ, Dept Plants Soils & Climate, Utah Climate Ctr, 4820 Old Main Hill, Logan, UT 84322 USA. EM simon.wang@usu.edu RI YOON, JIN-HO/A-1672-2009; Huang, Wan-Ru/G-7272-2014 OI YOON, JIN-HO/0000-0002-4939-8078; Huang, Wan-Ru/0000-0002-2171-4075 FU Utah Agricultural Experiment Station; Office of Science of the US Department of Energy (DOE) as part of the Earth System Modeling program; Ministry of Science and Technology of Taiwan under MOST [103-2111-M-003-001, 103-2621-M-492-001]; [NNX13AC37G]; [WaterSMART R13AC80039] FX This research was supported by grants NNX13AC37G and WaterSMART R13AC80039, and the Utah Agricultural Experiment Station. Jin-Ho Yoon was supported by the Office of Science of the US Department of Energy (DOE) as part of the Earth System Modeling program. Wan-Ru Huang was supported by the Ministry of Science and Technology of Taiwan under MOST 103-2111-M-003-001 and MOST 103-2621-M-492-001. NR 28 TC 13 Z9 13 U1 3 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1530-261X J9 ATMOS SCI LETT JI Atmos. Sci. Lett. PD JUL-SEP PY 2015 VL 16 IS 3 BP 338 EP 345 DI 10.1002/asl2.565 PG 8 WC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences SC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences GA CM9HW UT WOS:000358020000023 ER PT J AU Kim, S Dale, BE AF Kim, Seungdo Dale, Bruce E. TI All biomass is local: The cost, volume produced, and global warming impact of cellulosic biofuels depend strongly on logistics and local conditions SO BIOFUELS BIOPRODUCTS & BIOREFINING-BIOFPR LA English DT Article DE biorefinery; cellulosic ethanol; feedstock supply cluster; global warming impact; minimum ethanol selling price; supply chain ID ETHANOL SUPPLY CHAIN; OPTIMIZATION MODEL; CORN STOVER; SWITCHGRASS; MANAGEMENT; DESIGN AB Current models of cellulosic biofuel systems require that the delivered price of the cellulosic biomass feedstock be kept low. Thus the predicted biorefinery size is relatively small, limiting potential economies of scale. However, it is actually the ultimate selling price of the biofuel that largely determines market penetration. We relaxed the constraint of low delivered feedstock price and explored the resulting effects on biofuel price, biofuel volume produced, and global warming impact (GWI). Feedstock price greatly affects the feedstock supply chains that may develop. Increased feedstock price does not affect the final ethanol selling price very much, but higher feedstock prices greatly increase the amount of ethanol produced. Farmers will supply much more cellulosic biomass at higher feedstock prices, leading to shorter transportation distances with reduced transportation costs and enabling larger biorefineries with improved economies of scale, thereby reducing the ethanol selling price. The cellulosic feedstock supply chain systems were studied as a function of feedstock prices by determining potential feedstock supply clusters and the maximum capacity of cellulosic biorefineries across the United States. Supply clusters were determined by minimizing costs associated with ethanol production. The analysis is based on county-level cellulosic feedstock production data projected in the US Billion-Ton Update report. Each biomass supply cluster is unique in terms of local and regional characteristics (e.g. area, feedstock types), biorefinery capacity, ethanol selling price, and GWI. Very large-scale biorefineries (>= 20 000 dry Mg day(-1)) may be feasible in some regions. (C) 2015 Society of Chemical Industry and John Wiley & Sons, Ltd C1 [Kim, Seungdo; Dale, Bruce E.] Michigan State Univ, Lansing, MI USA. RP Dale, BE (reprint author), Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, 3815 Technol Blvd, Lansing, MI 48910 USA. EM bdale@egr.msu.edu FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; DOE OBP Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830]; AgBioResearch; USDA National Institute of Food and Agriculture FX This work was funded in part by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494) and DOE OBP Office of Energy Efficiency and Renewable Energy (DE-AC05-76RL01830). This project was also supported by AgBioResearch and the USDA National Institute of Food and Agriculture. NR 23 TC 5 Z9 5 U1 2 U2 15 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1932-104X EI 1932-1031 J9 BIOFUEL BIOPROD BIOR JI Biofuels Bioprod. Biorefining PD JUL-AUG PY 2015 VL 9 IS 4 BP 422 EP 434 DI 10.1002/bbb.1554 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CM8RJ UT WOS:000357969400018 ER PT J AU Dale, VH Efroymson, RA Kline, KL Davitt, MS AF Dale, Virginia H. Efroymson, Rebecca A. Kline, Keith L. Davitt, Marcia S. TI A framework for selecting indicators of bioenergy sustainability SO BIOFUELS BIOPRODUCTS & BIOREFINING-BIOFPR LA English DT Review DE best management practices; bioenergy; biomass; criteria; indicators; sustainability ID ECOLOGICAL INDICATORS; BIOFUELS; CONSERVATION; MANAGEMENT; CRITERIA; SCIENCE; POLICY; EMISSIONS; SYSTEMS; IMPACT AB A framework for selecting and evaluating indicators of bioenergy sustainability is presented. This framework is designed to facilitate decision-making about which indicators are useful for assessing sustainability of bioenergy systems and supporting their deployment. Efforts to develop sustainability indicators in the United States and Europe are reviewed. The first steps of the framework for indicator selection are defining the sustainability goals and other goals for a bioenergy project or program, gaining an understanding of the context, and identifying the values of stakeholders. From the goals, context, and stakeholders, the objectives for analysis and criteria for indicator selection can be developed. The user of the framework identifies and ranks indicators, applies them in an assessment, and then evaluates their effectiveness, while identifying gaps that prevent goals from being met, assessing lessons learned, and moving toward best practices. The framework approach emphasizes that the selection of appropriate criteria and indicators is driven by the specific purpose of an analysis. Realistic goals and measures of bioenergy sustainability can be developed systematically with the help of the framework presented here. (C) 2015 Society of Chemical Industry and John Wiley & Sons, Ltd C1 [Dale, Virginia H.; Efroymson, Rebecca A.; Kline, Keith L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Davitt, Marcia S.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. RP Dale, VH (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Ctr BioEnergy Sustainabil & Climate Change Sci In, Oak Ridge, TN 37831 USA. EM dalevh@ornl.gov OI Kline, Keith/0000-0003-2294-1170; Efroymson, Rebecca/0000-0002-3190-880X FU US Department of Energy (DOE) under Bioenergy Technologies Office; UT-Battelle, LLC, for DOE [DE-AC05-00OR22725] FX This research was supported by the US Department of Energy (DOE) under the Bioenergy Technologies Office. Oak Ridge National Laboratory is managed by the UT-Battelle, LLC, for DOE under contract DE-AC05-00OR22725. The authors thank FM O'Hara, Jr., for his review and Erica Atkin for editing the manuscript. Comments by Amy Wolfe on an earlier draft are also appreciated. NR 47 TC 5 Z9 6 U1 5 U2 17 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1932-104X EI 1932-1031 J9 BIOFUEL BIOPROD BIOR JI Biofuels Bioprod. Biorefining PD JUL-AUG PY 2015 VL 9 IS 4 BP 435 EP 446 DI 10.1002/bbb.1562 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CM8RJ UT WOS:000357969400019 ER PT J AU Chan-Thaw, CE Villa, A Wang, D Dal Santo, V Biroli, AO Veith, GM Thomas, A Prati, L AF Chan-Thaw, Carine E. Villa, Alberto Wang, Di Dal Santo, Vladimiro Biroli, Alessio Orbelli Veith, Gabriel M. Thomas, Arne Prati, Laura TI PdHx Entrapped in a Covalent Triazine Framework Modulates Selectivity in Glycerol Oxidation SO CHEMCATCHEM LA English DT Article DE cleavage reactions; heterogeneous catalysis; nitrogen heterocycles; oxidation; palladium ID PALLADIUM NANOPARTICLES; IONOTHERMAL SYNTHESIS; AEROBIC OXIDATION; MOLECULAR-OXYGEN; PHASE OXIDATION; SUPPORTED GOLD; CATALYSTS; ALCOHOLS; HYDROGENATION; POLYMERS AB Pd nanoparticles within a nitrogen-containing covalent triazine framework (CTF) material are investigated to understand if the highly tunable CTF chemistry mediates the catalytic properties of the Pd nanoparticles. Surprisingly, our results demonstrate that the CTF stabilizes the formation of 2.6nm PdHx particles within the pores. These confined PdHx particles are very active for the liquid-phase oxidation of glycerol and promote CC cleavage, probably connected with the enhanced insitu formation of H2O2. During recycling tests, the confined particles are transformed progressively to very stable Pd-0 particles. This stability has been attributed mainly to a confinement effect as nanoparticles trapped outside the pores lose activity rapidly. These results indicate that there is a potential to tune CTF chemistry to modify the chemistry of the catalytic metals significantly. C1 [Chan-Thaw, Carine E.; Villa, Alberto; Prati, Laura] Univ Milan, Dept Chem, I-20133 Milan, Italy. [Wang, Di] Karlsruhe Inst Technol, Inst Nanotechnol & Karlsruhe Nano Micro Facil, Eggenstein Leopoldshafen, Germany. [Dal Santo, Vladimiro; Biroli, Alessio Orbelli] CNR Ist Sci & Tecnol Mol, I-20133 Milan, Italy. [Veith, Gabriel M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Thomas, Arne] Tech Univ Berlin, Dept Chem, Funct Mat, D-10623 Berlin, Germany. RP Prati, L (reprint author), Univ Milan, Dept Chem, Via Golgi 19, I-20133 Milan, Italy. EM laura.prati@unimi.it RI Chan-Thaw, Carine /O-9785-2014; Thomas, Arne/A-2178-2016; Villa, Alberto/H-7355-2013; Prati, Laura/Q-3970-2016 OI Chan-Thaw, Carine /0000-0002-7330-9629; Thomas, Arne/0000-0002-2130-4930; Villa, Alberto/0000-0001-8656-6256; Prati, Laura/0000-0002-8227-9505 FU UniCat cluster of excellence (Unifying Concepts in Catalysis, Berlin); U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Karlsruhe Nano Micro Facility (KNMF) FX We thank Phisan Katekomol for the preparation of the support. Financial support by the UniCat cluster of excellence (Unifying Concepts in Catalysis, Berlin) is gratefully acknowledged. A portion of this research was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (GMV). TEM characterization was performed at KIT and sponsored by Karlsruhe Nano Micro Facility (KNMF). NR 32 TC 4 Z9 4 U1 6 U2 51 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1867-3880 EI 1867-3899 J9 CHEMCATCHEM JI ChemCatChem PD JUL PY 2015 VL 7 IS 14 BP 2149 EP 2154 DI 10.1002/cctc.201500055 PG 6 WC Chemistry, Physical SC Chemistry GA CM8OV UT WOS:000357962400019 ER PT J AU Liu, XP Aranda, MAG Chen, B Wang, PM Harder, R Robinson, I AF Liu, Xianping Aranda, Miguel A. G. Chen, Bo Wang, Peiming Harder, Ross Robinson, Ian TI In Situ Bragg Coherent Diffraction Imaging Study of a Cement Phase Microcrystal during Hydration SO CRYSTAL GROWTH & DESIGN LA English DT Article ID CALCIUM ALUMINATE CEMENTS; GRAIN-BOUNDARIES; RAY; DEFORMATION; KINETICS; CAAL2O4; STRAIN AB Results of Bragg coherent diffraction imaging (BCDI) confirm that ion migration and consumption occur during hydration of calcium monoaluminate (CA). The chemical phase transformation promotes the hydration process and the formation of new hydrates. There is a potential for the formation of hydrates near where the active ions accumulate. BCDI has been used to study the in situ hydration process of CA over a 3 day period. The evolution of three-dimensional (3D) Bragg diffraction electron density, the Bragg density, and strain fields present on the nanoscale within the crystal was measured and visualized. Initial Bragg densities and strains in CA crystal derived from sintering evolve into various degrees during hydration. The variation of Bragg density within the crystal is attributed to the change of the degree of crystal ordering, which could occur through ion transfer during hydration. The observed strain, coming from the interfacial mismatch effect between high Bragg density and low Bragg density parts in the crystal, remained throughout the experiment. The first Bragg density change during the hydration process is due to a big loss of Bragg density as seen in the image amplitude but not its phase. This work provides new evidence supporting the through-solution reaction mechanism of CA. C1 [Liu, Xianping; Chen, Bo; Wang, Peiming; Robinson, Ian] Tongji Univ, Sch Mat Sci & Engn, Shanghai 201804, Peoples R China. [Liu, Xianping; Wang, Peiming] Tongji Univ, Minist Educ, Key Lab Adv Civil Engn Mat, Shanghai 201804, Peoples R China. [Aranda, Miguel A. G.] Univ Malaga, Dept Quim Inorgan Crystalog & Mineral, E-29071 Malaga, Spain. [Aranda, Miguel A. G.] ALBA Synchrotron, E-08290 Barcelona, Spain. [Chen, Bo; Robinson, Ian] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Chen, Bo; Robinson, Ian] Rutherford Appleton Lab, Didcot OX11 0FA, Oxon, England. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Liu, XP (reprint author), Tongji Univ, Sch Mat Sci & Engn, Shanghai 201804, Peoples R China. EM lxp@tongji.edu.cn; i.robinson@ucl.ac.uk RI Aranda, Miguel A.G./D-4614-2009 OI Aranda, Miguel A.G./0000-0001-7708-3578 FU National Science Foundation [DMR-9724294]; National Natural Science Foundation of China [51102181]; Tongji University, China; EPSRC [EP/I022562/1]; BBSRC Professorial Fellowship; State Scholarship Fund of China; U.S. Department of Energy [DE-AC02-06CH11357]; FEDER; [MAT2010-16213] FX We acknowledge the use of the Advanced Photon Source, which is operated by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. The BCDI instrumentation at the Advanced Photon Source beamline 34-ID-C was built with a National Science Foundation grant DMR-9724294. The work was supported by National Natural Science Foundation of China (Project 51102181) and the grant "Materials Nanostructure" from Tongji University, China. The work at UMA was funded by MAT2010-16213 research grant (Spain) which is cofunded by FEDER. Ian Robinson is supported by EPSRC grant EP/I022562/1 and a BBSRC Professorial Fellowship. Xianping Liu is supported by the State Scholarship Fund of China. NR 28 TC 2 Z9 2 U1 3 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 EI 1528-7505 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD JUL PY 2015 VL 15 IS 7 BP 3087 EP 3091 DI 10.1021/cg5013389 PG 5 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA CM1IY UT WOS:000357435800001 ER PT J AU Kaiser, A Sokolov, A Aranson, IS Lowen, H AF Kaiser, A. Sokolov, A. Aranson, I. S. Loewen, H. TI Motion of two micro-wedges in a turbulent bacterial bath SO EUROPEAN PHYSICAL JOURNAL-SPECIAL TOPICS LA English DT Article ID SWIMMING BACTERIA; COLLECTIVE MOTION; ACTIVE COLLOIDS; PHASE-BEHAVIOR; SPERM CELLS; HYDRODYNAMICS; MACROMOLECULES; PARTICLES; DYNAMICS; MICROCHANNELS AB The motion of a pair of micro-wedges ("carriers") in a turbulent bacterial bath is explored using computer simulations with explicit modeling of the bacteria and experiments. The orientation of the two micro-wedges is fixed by an external magnetic field but the translational coordinates can move freely as induced by the bacterial bath. As a result, two carriers of same orientation move such that their mutual distance decreases, while they drift apart for an anti-parallel orientation. Eventually the two carriers stack on each other with no intervening bacteria exhibiting a stable dynamical mode where the two micro-wedges follow each other with the same velocity. These findings are in qualitative agreement with experiment on two micro-wedges in a bacterial bath. Our results provide insight into understanding self-assembly of many micro-wedges in an active bath. C1 [Kaiser, A.; Loewen, H.] Univ Dusseldorf, Inst Theoret Phys Weiche Mat 2, D-40225 Dusseldorf, Germany. [Sokolov, A.; Aranson, I. S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Kaiser, A (reprint author), Univ Dusseldorf, Inst Theoret Phys Weiche Mat 2, Univ Str 1, D-40225 Dusseldorf, Germany. RI Kaiser, Andreas/K-2166-2012; Lowen, Hartmut/K-9999-2016 OI Lowen, Hartmut/0000-0001-5376-8062 FU ERC Advanced Grant INTERCOCOS [267499]; German Science Foundation (DFG); U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division FX A. K. was supported by the ERC Advanced Grant INTERCOCOS (Grant No. 267499) and H. L. by the science priority program SPP 1726 of the German Science Foundation (DFG). Work by A. S. and I. S. A. was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division. NR 82 TC 5 Z9 5 U1 3 U2 16 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1951-6355 EI 1951-6401 J9 EUR PHYS J-SPEC TOP JI Eur. Phys. J.-Spec. Top. PD JUL PY 2015 VL 224 IS 7 BP 1275 EP 1286 DI 10.1140/epjst/e2015-02459-x PG 12 WC Physics, Multidisciplinary SC Physics GA CN1IS UT WOS:000358173000009 ER PT J AU Absar, SM Preston, BL AF Absar, Syeda Mariya Preston, Benjamin L. TI Extending the Shared Socioeconomic Pathways for sub-national impacts, adaptation, and vulnerability studies SO GLOBAL ENVIRONMENTAL CHANGE-HUMAN AND POLICY DIMENSIONS LA English DT Article DE Socioeconomic scenarios; Shared Socioeconomic Pathways; Climate change; Vulnerability; Adaptive capacity ID GLOBAL ENVIRONMENTAL-CHANGE; CLIMATE-CHANGE; MULTISCALE NARRATIVES; INTEGRATED ASSESSMENT; SCENARIO DEVELOPMENT; IA PERSPECTIVE; EUROPE; WATER; ASSESSMENTS; TECHNOLOGY AB The exploration of alternative socioeconomic futures is an important aspect of understanding the potential consequences of climate change. While socioeconomic scenarios are common and, at times essential, tools for the impacts, adaptation and vulnerability and integrated assessment modeling research communities, their approaches to scenario development have historically been quite distinct. However, increasing convergence of impacts, adaptation and vulnerability and integrated assessment modeling research in terms of scales of analysis suggests there may be value in the development of a common framework for socioeconomic scenarios. The Shared Socioeconomic Pathways represents an opportunity for the development of such a common framework. However, the scales at which these global storylines have been developed are largely incommensurate with the sub-national scales at which impacts, adaptation and vulnerability and, increasingly, integrated assessment modeling studies are conducted. The objective of this study was to develop sub-national and sectoral extensions of the global SSP storylines in order to identify future socioeconomic challenges for adaptation for the U.S. Southeast. A set of nested qualitative socioeconomic storyline elements, integrated storylines, and accompanying quantitative indicators were developed through an application of the Factor-Actor-Sector framework. In addition to revealing challenges and opportunities associated with the use of the SSPs as a basis for more refined scenario development, this study generated sub-national storyline elements and storylines that can subsequently be used to explore the implications of alternative sub-national socioeconomic futures for the assessment of climate change impacts and adaptation. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Absar, Syeda Mariya] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Absar, SM (reprint author), Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. EM absarsm@ornl.gov OI Preston, Benjamin/0000-0002-7966-2386 FU U.S. Department of Energy, Office of Science, Biological and Environment Research, Integrated Assessment Program [ERKP719]; U.S. Department of Energy [DE-ACO5-000R22725]; DOE Public Access Plan FX This research was sponsored by the U.S. Department of Energy, Office of Science, Biological and Environment Research, Integrated Assessment Program under project ERKP719. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-ACO5-000R22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). The authors acknowledge the constructive comments of Kristie L. Ebi and Kasper Kok on prior drafts of this manuscript. NR 104 TC 5 Z9 5 U1 2 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-3780 EI 1872-9495 J9 GLOBAL ENVIRON CHANG JI Glob. Environ. Change-Human Policy Dimens. PD JUL PY 2015 VL 33 BP 83 EP 96 DI 10.1016/j.gloenvcha.2015.04.004 PG 14 WC Environmental Sciences; Environmental Studies; Geography SC Environmental Sciences & Ecology; Geography GA CM7UV UT WOS:000357902900008 ER PT J AU Gernaat, DEHJ Calvin, K Lucas, PL Luderer, G Otto, SAC Rao, S Strefler, J van Vuuren, DP AF Gernaat, David E. H. J. Calvin, Katherine Lucas, Paul L. Luderer, Gunnar Otto, Sander A. C. Rao, Shilpa Strefler, Jessica van Vuuren, Detlef P. TI Understanding the contribution of non-carbon dioxide gases in deep mitigation scenarios SO GLOBAL ENVIRONMENTAL CHANGE-HUMAN AND POLICY DIMENSIONS LA English DT Article DE Non-CO2 emissions; Deep mitigation scenarios; Climate policy strategies; Methane (CH4); Nitrous oxide (N2O); Fluorinated gasses (F-gas) ID GREENHOUSE GASES; CLIMATE POLICY; EMISSIONS; METHANE; TARGETS; COSTS AB In 2010, the combined emissions of methane (CH4), nitrous oxide (N2O) and the fluorinated gasses (F-gas) accounted for 20-30% of Kyoto emissions and about 30% of radiative forcing. Current scenario studies conclude that in order to reach deep climate targets (radiative forcing of 2.8 W/m(2)) in 2100, carbon dioxide (CO2) emissions will need to be reduced to zero or negative. However, studies indicated that non-CO2 emissions seem to be have less mitigation potential. To support effective climate policy strategies, an in-depth assessment was made of non-CO2 greenhouse gas emission and their sources in achieving an ambitious climate target. Emission scenarios were assessed that had been produced by six integrated assessments models, which contributed to the scenario database for the fifth IPCC report. All model scenarios reduced emissions from energy-related sectors, largely resulting from structural changes and end-of-pipe abatement technologies. However, emission reductions were much less in the agricultural sectors. Furthermore, there were considerable differences in abatement potential between the model scenarios, and most notably in the agricultural sectors. The paper shows that better exploration of long-term abatement potential of non-CO2 emissions is critical for the feasibility of deep climate targets. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gernaat, David E. H. J.; Otto, Sander A. C.; van Vuuren, Detlef P.] Univ Utrecht, Copernicus Inst Sustainable Dev, NL-3584 CS Utrecht, Netherlands. [Gernaat, David E. H. J.; Lucas, Paul L.; van Vuuren, Detlef P.] PBL Netherlands Environm Assessment Agcy, NL-3720 BA Bilthoven, Netherlands. [Calvin, Katherine] Pacific NW Natl Lab, Joint Global Change Res Inst, Richland, WA 99352 USA. [Calvin, Katherine] Univ Maryland, College Pk, MD USA. [Rao, Shilpa] IIASA, A-2361 Laxenburg, Austria. [Luderer, Gunnar; Strefler, Jessica] Potsdam Inst Climate Impact Res PIK, D-14412 Potsdam, Germany. RP Gernaat, DEHJ (reprint author), Univ Utrecht, Copernicus Inst Sustainable Dev, Heidelberglaan 2, NL-3584 CS Utrecht, Netherlands. EM d.e.h.j.gemaat@uu.nl; katherine.calvin@pnnl.gov; paul.lucas@pbl.nl; luderer@pik-potsdam.de; a.a.c.otto@uu.nl; rao@iiasa.ac.at; strefler@pik-potsdam.de; detlef.vanvuuren@pbl.nl RI Luderer, Gunnar/G-2967-2012; van Vuuren, Detlef/A-4764-2009; Strefler, Jessica/O-7556-2015; OI van Vuuren, Detlef/0000-0003-0398-2831; Gernaat, David/0000-0003-4994-1453; Lucas, Paul/0000-0003-0292-7830 FU European Union Seventh Framework Programme FP7 (LIMITS) [282846] FX The research leading to these results has received funding from the European Union Seventh Framework Programme FP7/2007-2013 under grant agreement no 282846 (LIMITS). NR 48 TC 5 Z9 5 U1 2 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-3780 EI 1872-9495 J9 GLOBAL ENVIRON CHANG JI Glob. Environ. Change-Human Policy Dimens. PD JUL PY 2015 VL 33 BP 142 EP 153 DI 10.1016/j.gloenvcha.2015.04.010 PG 12 WC Environmental Sciences; Environmental Studies; Geography SC Environmental Sciences & Ecology; Geography GA CM7UV UT WOS:000357902900013 ER PT J AU Lawal, KA Stone, DA Aina, T Rye, C Abiodun, BJ AF Lawal, Kamoru A. Stone, Daithi A. Aina, Tolu Rye, Cameron Abiodun, Babatunde J. TI Trends in the potential spread of seasonal climate simulations over South Africa SO INTERNATIONAL JOURNAL OF CLIMATOLOGY LA English DT Review DE ensemble spread; HadRM3P; seasonal climate simulations; South Africa; predictability; trend ID MODEL INTERCOMPARISON PROJECT; PROBABILITY SKILL SCORES; REGIONAL COUPLED MODEL; ATMOSPHERIC PREDICTABILITY; INTERANNUAL VARIABILITY; ENSEMBLE SIMULATIONS; FORECASTS; RAINFALL; PRECIPITATION; UNCERTAINTY AB This study assesses the existence and importance of trends in the spread of South African climate simulations covering 50 years of a large initial-condition ensemble from a dynamical atmospheric model. It quantifies ensemble spread using two contrasting measures-standard deviation and 10-90th percentile range. The study then evaluates and examines the characteristics of long-term trends in the ensemble spread in relation to trends in the ensemble mean and in the observational record, by considering the skill of the monthly mean precipitation and near surface air temperature simulations. Results provide evidence that variations in ensemble spreads generated by the atmospheric model used in this study reflect fundamental properties of atmospheric variability in the real climate system. We find significant long-term trends in the measures of spread, with a general coastal-inland gradient, suggesting the possibility of existence of interannual variations in the potential range of seasonal climate simulations over South Africa. We also find robust relationships between trends in the observational record, in the simulated ensemble means and in measures of the simulated ensemble spread. Irrespective of the direction of trends, the correspondence of higher model skill when trends in the ensemble spread are larger suggests that the skill produced by a dynamical modelling system may not be independent of the model ability to capture the real atmospheric trends in whatever the model is simulating or forecasting. Therefore, based on historical data, further understanding of how potential predictability is changing has the prospect to improve the interpretation of current estimates of simulation skill. C1 [Lawal, Kamoru A.; Abiodun, Babatunde J.] Univ Cape Town, Climate Syst Anal Grp, Dept Environm & Geog Sci, ZA-7701 Cape Town, South Africa. [Stone, Daithi A.] Lawrence Berkeley Natl Lab, Computat Chem Mat & Climate Grp, Berkeley, CA USA. [Aina, Tolu] Univ Oxford, Oxford E Res Ctr, Oxford OX1 2JD, England. [Rye, Cameron] Univ Oxford, Atmospher Ocean & Planetary Phys, Oxford OX1 2JD, England. RP Lawal, KA (reprint author), Univ Cape Town, Climate Syst Anal Grp, Dept Environm & Geog Sci, ZA-7701 Cape Town, South Africa. EM lawal@csag.uct.ac.za OI Stone, Daithi/0000-0002-2518-100X FU South African Water Research Commission (WRC) [K5/2067/1]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research's Regional and Global Climate Modelling Program [DE-AC02-05CH11231]; Microsoft Research FX The authors would like to thank the many volunteers who generously ran the weather@home/SAF model simulations on their personal computers. We acknowledge invaluable advice from Bruce Hewitson, Willem Landman, Geoff Pegram, Francisco Doblas-Reyes and Omar Bellprat; technical assistance on the weather@home/SAF project from the CPDN team at the University of Oxford; Chris Forest and Chuck Pavolski at Pennsylvania State University; the PRECIS team at the UK Met Office; and Phillip Mukwena. KAL was funded by a grant from the South African Water Research Commission (WRC - Project K5/2067/1). DAS was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research's Regional and Global Climate Modelling Program under contract number DE-AC02-05CH11231. The weather@home/SAF project was developed with support from Microsoft Research. NR 58 TC 0 Z9 0 U1 1 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0899-8418 EI 1097-0088 J9 INT J CLIMATOL JI Int. J. Climatol. PD JUL PY 2015 VL 35 IS 9 BP 2193 EP 2209 DI 10.1002/joc.4234 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CM7RO UT WOS:000357894100001 ER PT J AU Shupe, MD Turner, DD Zwink, A Thieman, MM Mlawer, EJ Shippert, T AF Shupe, Matthew D. Turner, David D. Zwink, Alexander Thieman, Mandana M. Mlawer, Eli J. Shippert, Timothy TI Deriving Arctic Cloud Microphysics at Barrow, Alaska: Algorithms, Results, and Radiative Closure SO JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY LA English DT Article ID ANGULAR-DISTRIBUTION MODELS; GROUND-BASED OBSERVATIONS; ENERGY SYSTEM INSTRUMENT; MIXED-PHASE CLOUDS; STRATUS CLOUD; TERRA SATELLITE; FLUX ESTIMATION; DOPPLER RADAR; ATMOSPHERE; SURFACE AB Cloud phase and microphysical properties control the radiative effects of clouds in the climate system and are therefore crucial to characterize in a variety of conditions and locations. An Arctic-specific, ground-based, multisensor cloud retrieval system is described here and applied to 2 yr of observations from Barrow, Alaska. Over these 2 yr, clouds occurred 75% of the time, with cloud ice and liquid each occurring nearly 60% of the time. Liquid water occurred at least 25% of the time, even in winter, and existed up to heights of 8 km. The vertically integrated mass of liquid was typically larger than that of ice. While it is generally difficult to evaluate the overall uncertainty of a comprehensive cloud retrieval system of this type, radiative flux closure analyses were performed in which flux calculations using the derived microphysical properties were compared with measurements at the surface and the top of the atmosphere. Radiative closure biases were generally smaller for cloudy scenes relative to clear skies, while the variability of flux closure results was only moderately larger than under clear skies. The best closure at the surface was obtained for liquid-containing clouds. Radiative closure results were compared with those based on a similar, yet simpler, cloud retrieval system. These comparisons demonstrated the importance of accurate cloud-phase and cloud-type classification, and specifically the identification of liquid water, for determining radiative fluxes. Enhanced retrievals of liquid water path for thin clouds were also shown to improve radiative flux calculations. C1 [Shupe, Matthew D.] Cooperat Inst Res Environm Sci, Boulder, CO USA. [Shupe, Matthew D.] NOAA Earth Syst Res Lab, Norman, OK USA. [Turner, David D.] NOAA Natl Severe Storms Lab, Norman, OK USA. [Zwink, Alexander] Univ Oklahoma, Norman, OK 73019 USA. [Thieman, Mandana M.] Sci Syst & Applicat Inc, Hampton, VA USA. [Mlawer, Eli J.] Atmospher & Environm Res, Lexington, MA USA. [Shippert, Timothy] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Shupe, MD (reprint author), R PSD3,325 Broadway, Boulder, CO 80305 USA. EM matthew.shupe@noaa.gov RI Shupe, Matthew/F-8754-2011 OI Shupe, Matthew/0000-0002-0973-9982 FU Office of Science (BER), U.S. Department of Energy [DE-SC0011918, DE-SC0008830, DE-SC0000991, DE-FG01-06ER64167] FX This research was supported by the Office of Science (BER), U.S. Department of Energy, Grants DE-SC0011918, DE-SC0008830, DE-SC0000991, and DE-FG01-06ER64167. Ground-based datasets were obtained from the ARM data archive (www.archive.arm.gov). Connor Flynn provided the MPL dataset. The CERES satellite data were subsected from the full CERES Terra and/or Aqua Edition 3A Single Scanner Footprint dataset, obtained from the NASA Langley Research Center Atmospheric Science Data Center (https://eosweb.larc.nasa.gov/order-data) and described online (http://ceres.larc.nasa.gov/documents/DPC/DPC_current/pdfs/DPC_SSF-Ed3_R 5V2.pdf). NR 42 TC 2 Z9 2 U1 0 U2 15 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 1558-8424 EI 1558-8432 J9 J APPL METEOROL CLIM JI J. Appl. Meteorol. Climatol. PD JUL PY 2015 VL 54 IS 7 BP 1675 EP 1689 DI 10.1175/JAMC-D-15-0054.1 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CM9AT UT WOS:000357998100019 ER PT J AU Teplitsky, E Joshi, K Ericson, DL Scalia, A Mullen, JD Sweet, RM Soares, AS AF Teplitsky, Ella Joshi, Karan Ericson, Daniel L. Scalia, Alexander Mullen, Jeffrey D. Sweet, Robert M. Soares, Alexei S. TI High throughput screening using acoustic droplet ejection to combin