FN Thomson Reuters Web of Science™
VR 1.0
PT J
AU Silbernagel, R
Burns, JD
Reed, DT
Hobbs, DT
Clearfield, A
AF Silbernagel, Rita
Burns, Jonathan D.
Reed, Donald T.
Hobbs, David T.
Clearfield, Abraham
TI Tetravalent metal phosphonate-phosphate hybrids as ion exchange
materials for the nuclear fuel cycle
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Silbernagel, Rita; Burns, Jonathan D.; Clearfield, Abraham] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA.
[Reed, Donald T.] Los Alamos Natl Lab Carlsbad Operat, Earth & Environm Sci Div, Carlsbad, NM 88220 USA.
[Hobbs, David T.] Savannah River Natl Lab, Aiken, SC USA.
EM Rita.Silbernagel@chem.tamu.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 107-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402446
ER
PT J
AU Silva, CM
Hunt, RD
Snead, LL
AF Silva, Chinthaka M.
Hunt, Rodney D.
Snead, Lance L.
TI Synthesis of uranium mononitride microspheres via higher uranium
nitrides
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Silva, Chinthaka M.; Hunt, Rodney D.; Snead, Lance L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
[Silva, Chinthaka M.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.
EM silvagw@ornl.gov
NR 0
TC 0
Z9 0
U1 1
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 110-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402449
ER
PT J
AU Simmonds, I
Ketring, A
Robertson, D
Venzie, J
Finck, M
AF Simmonds, Isaac
Ketring, Alan
Robertson, David
Venzie, J.
Finck, Martha
TI Attribution of Iridium-192 sources via QD-ICP-MS
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Simmonds, Isaac; Robertson, David] Univ Missouri, Dept Chem, Columbia, MO 65211 USA.
[Ketring, Alan] Univ Missouri, Univ Missouri Res Reactor, Columbia, MO 65211 USA.
[Venzie, J.] Savannah River Natl Lab, Aiken, SC 29803 USA.
[Finck, Martha] Idaho Natl Lab, Idaho Falls, ID USA.
EM idshxf@mail.missouri.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 29-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402373
ER
PT J
AU Sista, P
Ghosh, K
Balog, ERM
Martinez, JS
Rocha, RC
AF Sista, Prakash
Ghosh, Koushik
Balog, Eva R. M.
Martinez, Jennifer S.
Rocha, Reginaldo C.
TI Ligand-functionalized semiconducting polymers - towards integrated
metallopolymer assemblies
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sista, Prakash; Ghosh, Koushik; Balog, Eva R. M.; Martinez, Jennifer S.; Rocha, Reginaldo C.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, MPA CINT, Los Alamos, NM 87545 USA.
EM prakash@lanl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 537-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405652
ER
PT J
AU Skodje, RT
Davis, M
Kramer, Z
Li, WX
Bai, SR
Gu, XK
AF Skodje, Rex T.
Davis, Michael
Kramer, Zeb
Li, Weixue
Bai, Shirong
Gu, Xiang Kui
TI Sensitivity of chemical pathways in reactive networks
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Skodje, Rex T.; Kramer, Zeb; Bai, Shirong] Univ Colorado, Boulder, CO 80309 USA.
[Davis, Michael] Argonne Natl Lab, Div Chem Sci, Argonne, IL 60439 USA.
[Li, Weixue; Gu, Xiang Kui] Dalian Inst Chem Phys, Key State Inst Catalysis, Dalian, Peoples R China.
EM rex.skodje@colorado.edu
RI Gu, Xiangkui/H-3706-2014
NR 1
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 576-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105382
ER
PT J
AU Smith, JC
AF Smith, Jeremy C.
TI Progress and prospects in extreme scale supercomputing in biology,
bioenergy, and medicine
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Smith, Jeremy C.] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA.
EM cst@ornl.gov
RI smith, jeremy/B-7287-2012
OI smith, jeremy/0000-0002-2978-3227
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 226-BIOL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102123
ER
PT J
AU Smith, KE
Callahan, MP
Gerakines, PA
Dworkin, JP
House, CH
AF Smith, Karen E.
Callahan, Michael P.
Gerakines, Perry A.
Dworkin, Jason P.
House, Christopher H.
TI Investigation of pyridine carboxylic acids in CM2 carbonaceous
chondrites: Potential precursor molecules for ancient coenzymes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Smith, Karen E.; House, Christopher H.] Penn State Univ, Dept Geosci, University Pk, PA 16802 USA.
[Smith, Karen E.; House, Christopher H.] Penn State Univ, Penn State Astrobiol Res Ctr, University Pk, PA 16802 USA.
[Smith, Karen E.] Oak Ridge Associated Univ, NASA Goddard Space Flight Ctr, Oak Ridge, TN 37831 USA.
[Callahan, Michael P.; Gerakines, Perry A.; Dworkin, Jason P.] NASA Goddard Space Flight Ctr, Solar Syst Explorat Div, Greenbelt, MD 20771 USA.
EM karen.e.smith@nasa.gov
RI Dworkin, Jason/C-9417-2012
OI Dworkin, Jason/0000-0002-3961-8997
NR 0
TC 0
Z9 0
U1 1
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 120-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101571
ER
PT J
AU Smith, ZD
Sandoval, CW
Birdsell, SA
AF Smith, Zachary D.
Sandoval, Cynthia W.
Birdsell, Stephen A.
TI Assessment of service lives in polysiloxane foams using laboratory and
field data
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Smith, Zachary D.; Sandoval, Cynthia W.; Birdsell, Stephen A.] Los Alamos Natl Lab, Dept Polymers & Coatings, Los Alamos, NM 87545 USA.
EM zsmith@lanl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 641-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405753
ER
PT J
AU Snow, MS
Mann, NR
Snyder, DC
Clark, SB
AF Snow, Mathew S.
Mann, Nick R.
Snyder, Darin C.
Clark, Sue B.
TI Cs isotopic ratio measurements from environmental samples using thermal
ionization mass spectrometry: Applications to ultra-trace environmental
analyses and nuclear forensics
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Snow, Mathew S.; Mann, Nick R.; Snyder, Darin C.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Clark, Sue B.] Washington State Univ, Dept Chem, Pullman, WA 99163 USA.
EM mathew.snow@inl.gov
RI Snyder, Darin/B-6863-2017
OI Snyder, Darin/0000-0001-8104-4248
NR 0
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 116-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402455
ER
PT J
AU Snyder, RA
Reig, AJ
Butch, SE
Betzu, J
DeGrado, WF
Solomon, EI
AF Snyder, Rae Ana
Reig, Amanda J.
Butch, Susan E.
Betzu, Justine
DeGrado, William F.
Solomon, Edward I.
TI Structure and function studies of systematic perturbations on de novo
Due Ferri proteins: Insights into oxygen-dependent reactivity
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Snyder, Rae Ana; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
[Reig, Amanda J.; Butch, Susan E.; Betzu, Justine] Ursinus Coll, Dept Chem, Collegeville, PA 19460 USA.
[DeGrado, William F.] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94143 USA.
[Solomon, Edward I.] Stanford Univ, Stanford Linear Accelerator Ctr, Synchrotron Radiat Lightsource, Stanford, CA 94309 USA.
EM raeana@stanford.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 950-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401584
ER
PT J
AU Soled, SL
Miseo, S
Baumgartner, J
Guzman, J
Bolin, T
Meyer, R
AF Soled, Stuart L.
Miseo, Sal
Baumgartner, Joseph
Guzman, Javier
Bolin, Trudy
Meyer, Randall
TI Can nickel phosphides become viable hydroprocessing catalysts?
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Soled, Stuart L.; Miseo, Sal; Baumgartner, Joseph; Guzman, Javier] ExxonMobil Res & Engn Co, Corp Strateg Res, Annandale, NJ 08801 USA.
[Bolin, Trudy] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Meyer, Randall] Univ Illinois, Chicago, IL USA.
EM stu.soled@exxonmobil.com
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 96-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104821
ER
PT J
AU Sommer, SK
Zakharov, LN
Teat, SJ
Pluth, MD
AF Sommer, Samantha K.
Zakharov, Lev N.
Teat, Simon J.
Pluth, Michael D.
TI Design, synthesis, and characterization of hybrid metal-ligand
hydrogen-bonded (MLHB) supramolecular architectures
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sommer, Samantha K.; Zakharov, Lev N.; Pluth, Michael D.] Univ Oregon, Dept Chem & Biochem, Eugene, OR 97403 USA.
[Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
EM ssommer@uoregon.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 711-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403288
ER
PT J
AU Somorjai, GA
AF Somorjai, Gabor A.
TI Molecular catalysis science, nanoparticle synthesis, and instrument
development for characterization under reaction conditions: Conquering
catalytic complexity
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM somorjai@berkeley.edu
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 372-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165103800
ER
PT J
AU Somorjai, GA
AF Somorjai, Gabor A.
TI Atomic scale foundations of covalent and acid-base catalysis in reaction
selectivities and turnover rates
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM somorjai@berkeley.edu
NR 0
TC 0
Z9 0
U1 2
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 292-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102552
ER
PT J
AU Sonk, JA
Weston, RE
Barker, JR
AF Sonk, Jason A.
Weston, Ralph E.
Barker, John R.
TI Computed probability distributions for collisional energy and angular
momentum transfer between HONO and Ar in the gas phase
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sonk, Jason A.; Barker, John R.] Univ Michigan, Ann Arbor, MI 48198 USA.
[Weston, Ralph E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM jsonk@umich.edu
RI Barker, John/F-5904-2012
OI Barker, John/0000-0001-9248-2470
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 466-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404185
ER
PT J
AU Soong, Y
Howard, BH
Hedges, SW
Dilmore, RM
AF Soong, Yee
Howard, Bret H.
Hedges, Sheila W.
Dilmore, Robert M.
TI Potential impact of combustion contaminants in saline formation
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Soong, Yee; Howard, Bret H.; Hedges, Sheila W.; Dilmore, Robert M.] US DOE, NETL, Pittsburgh, PA 15236 USA.
EM soong@netl.doe.gov
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 314-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105151
ER
PT J
AU Soykal, II
Wang, H
Liang, CD
Schwartz, V
AF Soykal, Ibrahim Ilgaz
Wang, Hui
Liang, Chengdu
Schwartz, Viviane
TI Investigation of silica supported fullerene catalysts for oxidative
dehydrogenation of alkanes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Soykal, Ibrahim Ilgaz; Wang, Hui; Liang, Chengdu; Schwartz, Viviane] Oak Ridge Natl Lab, Ctr Nanophase Mat, Knoxville, TN 37831 USA.
EM soykalii@ornl.gov
NR 3
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 299-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105138
ER
PT J
AU Srivastava, S
Stevenson, N
AF Srivastava, Suresh
Stevenson, Nigel
TI Enabling personalized medicine: Simultaneous imaging and treatment with
tin-117m based radiopharmaceuticals
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Srivastava, Suresh] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA.
[Stevenson, Nigel] Clear Vasc Inc, The Woodlands, TX 77380 USA.
EM suresh@bnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 59-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402400
ER
PT J
AU Stacchiola, DJ
AF Stacchiola, Dario J.
TI In-situ studies on the water gas shift reaction: From planar to powder
catalysts
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stacchiola, Dario J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM djs@bnl.gov
NR 2
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 484-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105296
ER
PT J
AU Stacchiola, DJ
AF Stacchiola, Dario J.
TI Tuning the activity and stability of copper based catalysts with
reducible oxides
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stacchiola, Dario J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM djs@bnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 109-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165103552
ER
PT J
AU Stoyer, MA
AF Stoyer, Mark A.
TI Importance of service and education to Frank Kinard
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stoyer, Mark A.] LLNL, Div Phys, Livermore, CA 94550 USA.
EM mastoyer@llnl.gov
NR 3
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 41-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402384
ER
PT J
AU Stringfellow, WT
Domen, JK
Camarillo, MK
Sandelin, WL
Tinnacher, R
Jordan, P
Houseworth, J
Birkholzer, J
AF Stringfellow, William T.
Domen, Jeremy K.
Camarillo, Mary Kay
Sandelin, Whitney L.
Tinnacher, Ruth
Jordan, Preston
Houseworth, James
Birkholzer, Jens
TI Characterizing compounds used in hydraulic fracturing: A necessary step
for understanding environmental impacts
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stringfellow, William T.; Tinnacher, Ruth; Jordan, Preston; Houseworth, James; Birkholzer, Jens] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Domen, Jeremy K.; Camarillo, Mary Kay; Sandelin, Whitney L.] Univ Pacific, Stockton, CA 95211 USA.
EM wstringfellow@lbl.gov
RI Tinnacher, Ruth/I-4845-2015; Stringfellow, William/O-4389-2015; Jordan,
Preston/L-1587-2016; Birkholzer, Jens/C-6783-2011
OI Stringfellow, William/0000-0003-3189-5604; Jordan,
Preston/0000-0001-5853-9517; Birkholzer, Jens/0000-0002-7989-1912
NR 0
TC 0
Z9 0
U1 1
U2 8
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 448-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165106015
ER
PT J
AU Stuck, D
Head-Gordon, M
AF Stueck, David
Head-Gordon, Martin
TI Regularizing orbital optimized perturbation theory
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stueck, David; Head-Gordon, Martin] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM dstuck@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 454-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404173
ER
PT J
AU Stull, JA
Welch, CF
Lin, T
Edwards, SL
Hartung, VN
AF Stull, Jamie A.
Welch, Cindy F.
Lin, Terri
Edwards, Stephanie L.
Hartung, Vaughn N.
TI Stability of dendrimers in solution
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Stull, Jamie A.; Welch, Cindy F.; Lin, Terri; Edwards, Stephanie L.; Hartung, Vaughn N.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM jamie.stull@gmail.com
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 762-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406049
ER
PT J
AU Sullivan, RC
Ahern, A
Robinson, E
Saleh, R
Tkacik, D
Presto, A
Yokelson, R
Thornton, J
Saliba, G
Mazzolini, C
Sedlacek, A
Subramanian, R
Robinson, A
Donahue, N
AF Sullivan, Ryan C.
Ahern, Adam
Robinson, Ellis
Saleh, Rawad
Tkacik, Daniel
Presto, Albert
Yokelson, Robert
Thornton, Joel
Saliba, Georges
Mazzolini, Claudio
Sedlacek, Arthur
Subramanian, R.
Robinson, Allen
Donahue, Neil
TI Chemical evolution of combustion aerosol and its climate-forcing
properties
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sullivan, Ryan C.; Ahern, Adam; Robinson, Ellis; Saleh, Rawad; Tkacik, Daniel; Presto, Albert; Saliba, Georges; Subramanian, R.; Robinson, Allen; Donahue, Neil] Carnegie Mellon Univ, Ctr Atmospher Particle Studies, Pittsburgh, PA 15213 USA.
[Yokelson, Robert] Univ Montana, Dept Chem, Missolua, MT USA.
[Thornton, Joel; Mazzolini, Claudio] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA.
[Sedlacek, Arthur] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA.
EM rsullivan@cmu.edu
RI Yokelson, Robert/C-9971-2011; Tkacik, Daniel/G-5630-2011
OI Yokelson, Robert/0000-0002-8415-6808;
NR 0
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 323-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404047
ER
PT J
AU Sun, J
Balsara, NP
Zuckermann, R
AF Sun, Jing
Balsara, Nitash P.
Zuckermann, Ronald
TI Self-assembly and crystallization in sequence-specific peptoid diblock
copolymers
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sun, Jing; Zuckermann, Ronald] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94706 USA.
[Sun, Jing; Balsara, Nitash P.; Zuckermann, Ronald] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94706 USA.
[Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94706 USA.
[Balsara, Nitash P.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94706 USA.
EM jingsun@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 165-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405297
ER
PT J
AU Sun, J
Proulx, C
Olivier, G
Mannige, R
Haxton, T
Guo, L
Gertler, G
Connolly, M
Jun, JM
Su, J
Garcia, R
Yoo, S
Whitelam, S
Zuckermann, R
AF Sun, Jing
Proulx, Caroline
Olivier, Gloria
Mannige, Ranjan
Haxton, Tom
Guo, Li
Gertler, Golan
Connolly, Michael
Jun, Joo Myung
Su, Jessica
Garcia, Rita
Yoo, Stan
Whitelam, Steve
Zuckermann, Ronald
TI Folding and assembly of sequence-defined peptoid polymers
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sun, Jing; Proulx, Caroline; Olivier, Gloria; Mannige, Ranjan; Haxton, Tom; Guo, Li; Gertler, Golan; Connolly, Michael; Jun, Joo Myung; Su, Jessica; Garcia, Rita; Yoo, Stan; Whitelam, Steve; Zuckermann, Ronald] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
EM rnzuckermann@lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 54-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405190
ER
PT J
AU Sun, J
Zuckermann, R
AF Sun, Jing
Zuckermann, Ronald
TI Sequence-specific block copolypeptoids for battery applications
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sun, Jing; Zuckermann, Ronald] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM jingsun@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 75-AEI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165100070
ER
PT J
AU Sung, W
Wang, WJ
Anderson, NA
Ao, MQ
Vaknin, D
Kim, D
AF Sung, Woongmo
Wang, Wenjie
Anderson, Nathaniel A.
Ao, Mingqi
Vaknin, David
Kim, Doseok
TI Surface excess and structure of Gibbs monolayer of long-chain ionic
liquids
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Sung, Woongmo; Ao, Mingqi; Kim, Doseok] Sogang Univ, Dept Phys, Seoul 100611, South Korea.
[Wang, Wenjie; Anderson, Nathaniel A.; Vaknin, David] Ames Lab, Dept Phys, Ames, IA USA.
EM dandyswm@gmail.com
RI Vaknin, David/B-3302-2009
OI Vaknin, David/0000-0002-0899-9248
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 427-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404146
ER
PT J
AU Suseno, S
Kaiser, J
Tran, R
McCrory, CCL
Rittle, J
Yano, J
Agapie, T
AF Suseno, Sandy
Kaiser, Jens
Tran, Rosalie
McCrory, Charles C. L.
Rittle, Jonathan
Yano, Junko
Agapie, Theodor
TI Synthesis and characterization of a series of mixed transition metal
oxido cubanes (MMnO4)
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Suseno, Sandy; Kaiser, Jens; McCrory, Charles C. L.; Rittle, Jonathan; Agapie, Theodor] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.
[Tran, Rosalie; Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
EM ssueno@caltech.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 542-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401204
ER
PT J
AU Suseno, S
Kaiser, J
Tran, R
McCrory, CCL
Rittle, J
Yano, J
Agapie, T
AF Suseno, Sandy
Kaiser, Jens
Tran, Rosalie
McCrory, Charles C. L.
Rittle, Jonathan
Yano, Junko
Agapie, Theodor
TI Synthesis of mixed-metal transition metal oxido cubanes (MMn3O4) and
their potential as prescursors for water oxidation electrocatalysts
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Suseno, Sandy; Kaiser, Jens; McCrory, Charles C. L.; Rittle, Jonathan; Agapie, Theodor] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.
[Tran, Rosalie; Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
EM ssueno@caltech.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 361-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401028
ER
PT J
AU Svec, F
AF Svec, Frantisek
TI Recent progress in preparation of thin layers for TLC-MS separations
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Svec, Frantisek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
EM fsvec@lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 61-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101517
ER
PT J
AU Syed, A
Lesoine, MD
Bhattacharjee, U
Petrich, JW
Smith, EA
AF Syed, Aleem
Lesoine, Michael D.
Bhattacharjee, Ujjal
Petrich, Jacob W.
Smith, Emily A.
TI Sub-diffraction fluorescence lifetime imaging in cultured cells
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Syed, Aleem; Lesoine, Michael D.; Bhattacharjee, Ujjal; Petrich, Jacob W.; Smith, Emily A.] Iowa State Univ, Ames, IA 50010 USA.
[Syed, Aleem; Lesoine, Michael D.; Bhattacharjee, Ujjal; Petrich, Jacob W.; Smith, Emily A.] US DOE, Ames Lab, Ames, IA 50010 USA.
EM wrtaleem@iastate.edu
RI Petrich, Jacob/L-1005-2015
NR 0
TC 0
Z9 0
U1 1
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 363-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101798
ER
PT J
AU Szybist, JP
McLaughlin, S
Iyer, S
AF Szybist, James P.
McLaughlin, Samuel
Iyer, Suresh
TI Emissions and performance benchmarking of a prototype dimethyl
ether-fueled heavy-duty truck
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Szybist, James P.] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Knoxville, TN 37922 USA.
[McLaughlin, Samuel] Volvo Grp Trucks Technol, Adv Technol & Res, Hagerstown, MD 21742 USA.
[Iyer, Suresh] Penn State Univ, Larson Inst, University Pk, PA 16802 USA.
EM szybistjp@ornl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 40-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104770
ER
PT J
AU Tang, ZJ
Zawozdinski, T
AF Tang, Zhijiang
Zawozdinski, Thomas
TI Electrolyte equilibrium in ion exchange polymer
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tang, Zhijiang; Zawozdinski, Thomas] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA.
[Zawozdinski, Thomas] Oak Ridge Natl Lab, Phys Chem Mat Grp, Oak Ridge, TN 37831 USA.
[Zawozdinski, Thomas] King Abdulaziz Univ, Dept Chem, Jeddah, Saudi Arabia.
EM ztang1@utk.edu
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 380-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404740
ER
PT J
AU Taylor-Pashow, KML
Hobbs, DT
AF Taylor-Pashow, Kathryn M. L.
Hobbs, David T.
TI Large particle titanate sorbents for treatment of high level waste
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Taylor-Pashow, Kathryn M. L.; Hobbs, David T.] Savannah River Natl Lab, Aiken, SC 29808 USA.
EM Kathryn.Taylor-Pashow@srnl.doe.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 101-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402440
ER
PT J
AU Taylor-Pashow, KML
Fondeur, FF
White, TL
DiPrete, DP
Milliken, CE
AF Taylor-Pashow, Kathryn M. L.
Fondeur, Fernando F.
White, Thomas L.
DiPrete, David P.
Milliken, Charles E.
TI Development of analytical methods for determining suppressor
concentration in the MCU Next Generation Solvent (NGS)
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Taylor-Pashow, Kathryn M. L.; Fondeur, Fernando F.; White, Thomas L.; DiPrete, David P.; Milliken, Charles E.] Savannah River Natl Lab, Aiken, SC 29808 USA.
EM Kathryn.Taylor-Pashow@srnl.doe.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 194-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101643
ER
PT J
AU Tepavcevic, S
Zhou, DH
Johnson, C
Rajh, T
AF Tepavcevic, Sanja
Zhou, Dehua
Johnson, Christopher
Rajh, Tijana
TI Nanostructured V2O5/Sn Mg-ion full batteries
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tepavcevic, Sanja] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60643 USA.
[Rajh, Tijana] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA.
[Zhou, Dehua; Johnson, Christopher] Argonne Natl Lab, Lemont, IL 60439 USA.
EM sanja@anl.gov
NR 0
TC 0
Z9 0
U1 4
U2 8
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 325-ENFL
PG 2
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105162
ER
PT J
AU Thompson, CM
Somorjai, GA
AF Thompson, Christopher M.
Somorjai, Gabor A.
TI Monitoring metal oxygen coverage with sum-frequency generation: Studies
of surface oxygen coverage of platinum in liquid-phase heterogeneously
catalyzed ethanol oxidation
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Thompson, Christopher M.; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Thompson, Christopher M.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM chris.thompson@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 131-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102403
ER
PT J
AU Thompson, T
Wolfenstine, J
Allen, J
Johannes, M
Huq, A
Sakamoto, J
AF Thompson, Travis
Wolfenstine, Jeff
Allen, Jan
Johannes, Michelle
Huq, Ashfia
Sakamoto, Jeff
TI Tetragonal vs. cubic phase stability in Al - free Ta doped Li7La3Zr2O12
garnet Li ion solid electrolyte
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Thompson, Travis; Sakamoto, Jeff] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA.
[Wolfenstine, Jeff; Allen, Jan] Army Res Lab, RDRL SED C, Adelphi, MD 20783 USA.
[Johannes, Michelle] Naval Res Lab, Ctr Computat Mat Sci, Anacostia, VA USA.
[Huq, Ashfia] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN USA.
EM trthompson378@gmail.com
NR 0
TC 0
Z9 0
U1 2
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 561-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105368
ER
PT J
AU Thurmer, K
AF Thuermer, Konrad
TI Nucleation and growth of ice films on metal surfaces
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Thuermer, Konrad] Sandia Natl Labs, Livermore, CA 94550 USA.
EM kthurme@sandia.gov
RI Thurmer, Konrad/L-4699-2013
OI Thurmer, Konrad/0000-0002-3078-7372
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 487-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104024
ER
PT J
AU Tinnacher, RM
Holmboe, M
Davis, JA
Tournassat, C
Bourg, I
AF Tinnacher, Ruth M.
Holmboe, Michael
Davis, James A.
Tournassat, Christophe
Bourg, Ian
TI Impacts of pore structure and diffusion-accessible porosity for
calcium-bromide diffusion in sodium-montmorillonite
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tinnacher, Ruth M.; Davis, James A.; Bourg, Ian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Holmboe, Michael] Royal Inst Technol, Dept Theoret Phys, S-10044 Stockholm, Sweden.
[Tournassat, Christophe] Bur Rech Geol & Minieres, Water Environm & Ecotechnol Div, Orleans, France.
EM rmtinnacher@lbl.gov
RI Tinnacher, Ruth/I-4845-2015; Davis, James/G-2788-2015
NR 0
TC 0
Z9 0
U1 0
U2 5
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 37-GEOC
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400352
ER
PT J
AU Toberer, ES
Stevanovic, V
Ortiz, B
Yan, J
Lany, S
Zakutayev, A
Peng, HW
AF Toberer, Eric S.
Stevanovic, Vladan
Ortiz, Brenden
Yan, Jun
Lany, Stephan
Zakutayev, Andriy
Peng, Haowei
TI Computationally driven targeting of advanced thermoelectric materials
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Toberer, Eric S.; Stevanovic, Vladan; Ortiz, Brenden; Yan, Jun] Colorado Sch Mines, Golden, CO 80401 USA.
[Toberer, Eric S.; Stevanovic, Vladan; Lany, Stephan; Zakutayev, Andriy; Peng, Haowei] Natl Renewable Energy Lab, Golden, CO 80401 USA.
EM etoberer@mines.edu
NR 0
TC 0
Z9 0
U1 3
U2 7
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 505-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401167
ER
PT J
AU Toney, MF
AF Toney, Michael F.
TI In situ X-ray scattering and microscopy of energy materials processing
and operation
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Toney, Michael F.] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA.
EM mftoney@slac.stanford.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 610-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105410
ER
PT J
AU Tournassat, C
Bourg, IC
Steefel, CI
AF Tournassat, Christophe
Bourg, Ian C.
Steefel, Carl I.
TI Quantification of the breakdown of modified Gouy-Chapman model for 2:1
salt background electrolyte: A molecular dynamic study
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tournassat, Christophe] Bur Rech Geol & Minieres, Water Environm & Ecotechnol Div, Orleans, France.
[Bourg, Ian C.; Steefel, Carl I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
EM c.tournassat@brgm.fr
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 46-GEOC
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400361
ER
PT J
AU Trahey, L
Yang, ZZ
Thackeray, MM
AF Trahey, Lynn
Yang, Zhenzhen
Thackeray, Michael M.
TI Investigations of solid electrolyte interphase formation on
high-capacity Li-ion battery anodes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Trahey, Lynn; Yang, Zhenzhen; Thackeray, Michael M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
EM trahey@anl.gov
NR 0
TC 0
Z9 0
U1 1
U2 6
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 79-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104805
ER
PT J
AU Troiano, JM
Olenick, LL
Kuech, TR
Melby, E
Lohse, SE
Mensch, AC
Ehimiaghe, E
Walter, SR
Murphy, CJ
Orr, G
Hamers, RJ
Pedersen, JA
Geiger, FM
AF Troiano, Julianne M.
Olenick, Laura L.
Kuech, Thomas R.
Melby, Eric
Lohse, Samuel E.
Mensch, Arielle C.
Ehimiaghe, Eseohi
Walter, Stephanie R.
Murphy, Catherine J.
Orr, Galya
Hamers, Robert J.
Pedersen, Joel A.
Geiger, Franz M.
TI Nanoparticle interactions with supported lipid bilayers studied by
nonlinear optics
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Troiano, Julianne M.; Olenick, Laura L.; Ehimiaghe, Eseohi; Walter, Stephanie R.; Geiger, Franz M.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Kuech, Thomas R.; Melby, Eric; Pedersen, Joel A.] Univ Wisconsin, Environm Chem & Technol Program, Madison, WI 53706 USA.
[Lohse, Samuel E.; Murphy, Catherine J.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA.
[Mensch, Arielle C.; Hamers, Robert J.; Pedersen, Joel A.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA.
[Orr, Galya] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
EM juliannetroiano2016@u.northwestern.edu
NR 0
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 687-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104211
ER
PT J
AU Tsivion, E
Head-Gordon, M
AF Tsivion, Ehud
Head-Gordon, Martin
TI Increasing the hydrogen adsorption of MOFs: From principles to practice
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tsivion, Ehud; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Tsivion, Ehud] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
EM tsivion.ehud@gmail.com
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 20-AEI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165100019
ER
PT J
AU Tsutakawa, SE
Lafrance-Vanasse, J
Tainer, JA
AF Tsutakawa, Susan E.
Lafrance-Vanasse, Julien
Tainer, John A.
TI DNA and RNA repair nucleases sculpt DNA to measure twice, cut once
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Tsutakawa, Susan E.; Lafrance-Vanasse, Julien; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Tainer, John A.] Scripps Res Inst, Skaggs Inst Chem Biol, La Jolla, CA 92037 USA.
EM jatainer@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 140-TOXI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406290
ER
PT J
AU Udey, RN
Corzett, TH
Valdez, CA
Williams, AM
AF Udey, Ruth N.
Corzett, Todd H.
Valdez, Carlos A.
Williams, Audrey M.
TI Retrospective assessment of chemical warfare agent exposure in humans
using LC-HRMS
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Udey, Ruth N.; Corzett, Todd H.; Valdez, Carlos A.; Williams, Audrey M.] Lawrence Livermore Natl Lab, Forens Sci Ctr, Livermore, CA 94550 USA.
EM udey1@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 56-TOXI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406213
ER
PT J
AU Ung, H
Daemen, L
Morton, TH
AF Ung, Hou
Daemen, Luke
Morton, Thomas Hellman
TI Probing the i-motif using cytosine analogs
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Ung, Hou; Morton, Thomas Hellman] Univ Calif Riverside, Riverside, CA 92521 USA.
[Daemen, Luke] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM hung001@ucr.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 567-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403154
ER
PT J
AU Uribe, EC
Bruchet, A
Wall, TF
Shusterman, JA
Nitsche, H
AF Uribe, Eva C.
Bruchet, Anthony
Wall, Thomas F.
Shusterman, Jennifer A.
Nitsche, Heino
TI From the ACS Nuclear Chemistry Summer School to actinide chemistry at UC
Berkeley
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Uribe, Eva C.; Bruchet, Anthony; Wall, Thomas F.; Shusterman, Jennifer A.; Nitsche, Heino] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Nitsche, Heino] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.
EM eva.uribe@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 38-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402381
ER
PT J
AU Utschig, LM
AF Utschig, Lisa M.
TI Nature-driven photochemistry for solar fuel production
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Utschig, Lisa M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
EM utschig@anl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 13-PRES
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406102
ER
PT J
AU Vaddula, BR
Yalla, S
Gonzalez, MA
AF Vaddula, Buchi R.
Yalla, Swathi
Gonzalez, Michael A.
TI Multicomponent flow approach for the efficient and more sustainable
preparation of aminothiazole derivatives
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vaddula, Buchi R.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
[Yalla, Swathi; Gonzalez, Michael A.] US EPA, Natl Risk Management Lab, Cincinnati, OH 45268 USA.
EM reddy.buchi@epa.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 829-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400144
ER
PT J
AU Vaddula, BR
Anderson, L
Yalla, S
Gonzalez, M
AF Vaddula, Buchi Reddy
Anderson, Laura
Yalla, Swathi
Gonzalez, Michael
TI Rapid synthesis of a-hydroxy acids and N-alkyl amides in the
continuous-flow spinning tube-in-tube ( STT r) reactor
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Gonzalez, Michael] US EPA, Sustainable Technol Div, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA.
[Vaddula, Buchi Reddy] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
EM reddy.buchi@epa.gov
NR 0
TC 0
Z9 0
U1 1
U2 5
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 863-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403426
ER
PT J
AU Vaddula, BR
Yalla, S
Gonzalez, M
AF Vaddula, Buchi Reddy
Yalla, Swathi
Gonzalez, Michael
TI Efficient and more sustainable one-step continuous-flow multicomponent
synthesis of chromene derivatives
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Gonzalez, Michael] US EPA, Sustainable Technol Div, Natl Risk Management Res Lab, Cincinnati, OH 45220 USA.
[Vaddula, Buchi Reddy] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
EM reddy.buchi@epa.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 164-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402629
ER
PT J
AU Vaddula, BR
Yalla, S
Gonzalez, M
AF Vaddula, Buchi Reddy
Yalla, Swathi
Gonzalez, Michael
TI Rapid and benign approaches for addition and coupling reactions using
flow chemistry
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Gonzalez, Michael] US EPA, Sustainable Technol Div, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA.
[Vaddula, Buchi Reddy] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA.
EM reddy.buchi@epa.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 91-IEC
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400509
ER
PT J
AU Valdez, CA
Mayer, BP
Hok, S
AF Valdez, Carlos A.
Mayer, Brian P.
Hok, Saphon
TI Zinc-based catalysts for the destruction of organophosphorus-based
compounds
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Valdez, Carlos A.; Mayer, Brian P.; Hok, Saphon] Lawrence Livermore Natl Lab, Forens Sci Ctr, Livermore, CA 94551 USA.
EM valdez11@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 276-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400817
ER
PT J
AU Van Allsburg, KM
Anzenberg, E
Liu, WJ
Yano, J
Tilley, TD
AF Van Allsburg, Kurt M.
Anzenberg, Eitan
Liu, Wenjun
Yano, Junko
Tilley, T. Don
TI Materials for water oxidation prepared from Mn- and Co-oxo cubane
molecular precursors
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Van Allsburg, Kurt M.; Anzenberg, Eitan; Liu, Wenjun; Yano, Junko; Tilley, T. Don] Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.
[Van Allsburg, Kurt M.; Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Van Allsburg, Kurt M.; Anzenberg, Eitan; Liu, Wenjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
[Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
EM kvanallsburg@lbl.gov
NR 1
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 1026-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401655
ER
PT J
AU van Bibber, KA
Bernstein, LA
Bleuel, DL
Cerjan, C
Fortner, RJ
Gostic, J
Grant, PM
Gharibyan, N
Hagmann, CA
Henry, EA
Sayre, DB
Schneider, DHG
Shaughnessy, DA
Brown, JA
Daub, BH
Brickner, NM
Davis, PF
Goldblum, BL
Vujic, J
Firestone, RB
Rogers, AM
AF van Bibber, Karl A.
Bernstein, Lee A.
Bleuel, Darren L.
Cerjan, Charles
Fortner, Richard J.
Gostic, Julie
Grant, Patrick M.
Gharibyan, Narek
Hagmann, Christian A.
Henry, Eugene A.
Sayre, Daniel B.
Schneider, Dieter H. G.
Shaughnessy, Dawn A.
Brown, Joshua A.
Daub, Brian H.
Brickner, Nicholas M.
Davis, Paul F.
Goldblum, Bethany L.
Vujic, Jasmina
Firestone, Richard B.
Rogers, Andrew M.
TI High energy density nuclear physics at UC Berkeley, LLNL, and LBNL
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [van Bibber, Karl A.; Brown, Joshua A.; Daub, Brian H.; Brickner, Nicholas M.; Davis, Paul F.; Goldblum, Bethany L.; Vujic, Jasmina] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA.
[Bernstein, Lee A.; Bleuel, Darren L.; Cerjan, Charles; Fortner, Richard J.; Gostic, Julie; Grant, Patrick M.; Gharibyan, Narek; Hagmann, Christian A.; Henry, Eugene A.; Sayre, Daniel B.; Schneider, Dieter H. G.; Shaughnessy, Dawn A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Firestone, Richard B.; Rogers, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.
EM karl.van.bibber@berkeley.edu
NR 0
TC 0
Z9 0
U1 2
U2 6
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 3-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402347
ER
PT J
AU Vander Wal, MN
Lee, S
Chang, CJ
AF Vander Wal, Mark N.
Lee, Sumin
Chang, Christopher J.
TI Selective fluorescent sensors for imaging sodium signaling in living
cells
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vander Wal, Mark N.; Lee, Sumin; Chang, Christopher J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Vander Wal, Mark N.; Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
[Chang, Christopher J.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.
[Chang, Christopher J.] Howard Hughes Med Inst, Chevy Chase, MD USA.
EM mnvanderwal1@gmail.com
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 810-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403378
ER
PT J
AU Vardon, DR
Ferguson, GA
Strathmann, TJ
Beckham, GT
AF Vardon, Derek R.
Ferguson, Glen A.
Strathmann, Timothy J.
Beckham, Gregg T.
TI Integrated catalytic upgrading of muconic acid to adipic acid for
renewable nylon precursor production
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vardon, Derek R.; Strathmann, Timothy J.] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA.
[Vardon, Derek R.; Ferguson, Glen A.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA.
EM derek.vardon@nrel.gov
NR 0
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 208-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102475
ER
PT J
AU Veauthier, JM
AF Veauthier, Jacqueline M.
TI Synthesis and characterization of new nitrogen-rich metal complexes.
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Veauthier, Jacqueline M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM veauthier@lanl.gov
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 938-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401573
ER
PT J
AU Velsko, C
Cassata, W
Jedlovec, D
Tereshatov, E
Stoeffl, W
Yeamans, C
Shaughnessy, D
AF Velsko, Carol
Cassata, William
Jedlovec, Donald
Tereshatov, Evgeny
Stoeffl, Wolfgang
Yeamans, Charles
Shaughnessy, Dawn
TI Demonstrating capability for radiochemical analysis of gaseous samples
at NIF
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Velsko, Carol; Cassata, William; Stoeffl, Wolfgang; Shaughnessy, Dawn] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
[Tereshatov, Evgeny] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77840 USA.
[Jedlovec, Donald; Yeamans, Charles] Lawrence Livermore Natl Lab, NIF Directorate, Livermore, CA 94550 USA.
EM velsko1@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 21-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402365
ER
PT J
AU Vericella, JJ
Stolaroff, JK
Baker, SE
Duoss, EB
Spadaccini, CM
Lewis, JA
Aines, RD
AF Vericella, John J.
Stolaroff, Joshuah K.
Baker, Sarah E.
Duoss, Eric B.
Spadaccini, Christopher M.
Lewis, Jennifer A.
Aines, Roger D.
TI Carbon dioxide capture using microencapsulation of high concentration
capture media
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vericella, John J.; Duoss, Eric B.; Spadaccini, Christopher M.] Lawrence Livermore Natl Lab, Mat Engn Div, Livermore, CA 94551 USA.
[Baker, Sarah E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Stolaroff, Joshuah K.; Aines, Roger D.] Lawrence Livermore Natl Lab, Global Secur E Program, Livermore, CA 94551 USA.
[Lewis, Jennifer A.] Harvard Univ, Wyss Inst Biol Inspired Engn, Cambridge, MA 02138 USA.
[Lewis, Jennifer A.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA.
EM vericella1@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 252-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105099
ER
PT J
AU Villaluenga, I
Chen, X
Devaux, D
Hallinan, DT
Balsara, NP
AF Villaluenga, Irune
Chen, Xi
Devaux, Didier
Hallinan, Daniel T.
Balsara, Nitash P.
TI Nanoparticle-driven assembly of co-continuous block copolymer
electrolytes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Villaluenga, Irune; Devaux, Didier; Balsara, Nitash P.] Lawrence Berkeley Natl Lab, EETD, Berkeley, CA 94709 USA.
[Chen, Xi; Balsara, Nitash P.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Hallinan, Daniel T.] Florida State Univ, Florida A&M Univ, Tallahassee, FL 32306 USA.
[Balsara, Nitash P.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94709 USA.
EM ivillaluenga@lbl.gov
NR 2
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 552-PMSE
PG 2
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405041
ER
PT J
AU Visel, A
AF Visel, Axel
TI Introduction to the joint EMSL/JGI user program
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Visel, Axel] DOE Joint Genome Inst, Walnut Creek, CA 94598 USA.
EM avisel@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 159-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101608
ER
PT J
AU Viswanathan, H
AF Viswanathan, Hari
TI Discovery science of hydraulic fracturing: Innovative working fluids and
their interactions with rocks, fractures, and hydrocarbons
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Viswanathan, Hari] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM viswana@lanl.gov
NR 0
TC 0
Z9 0
U1 2
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 2-PRES
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406091
ER
PT J
AU Vjunov, A
Fulton, JL
Camaioni, DM
Derewinski, M
Lercher, JA
AF Vjunov, Aleksei
Fulton, John L.
Camaioni, Donald M.
Derewinski, Miroslaw
Lercher, Johannes A.
TI Development and application of Al EXAFS to characterize Al T-sites in
zeolite: Effect of hot liquid water treatment on the HBEA zeolite
framework
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vjunov, Aleksei; Fulton, John L.; Camaioni, Donald M.; Derewinski, Miroslaw; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Lercher, Johannes A.] TU Muenchen, Dept Chem, D-85747 Garching, Bavaria, Germany.
EM aleksei.vjunov@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 459-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105274
ER
PT J
AU Vjunov, A
Fulton, JL
Camaioni, DM
Derewinski, M
Lercher, JA
AF Vjunov, Aleksei
Fulton, John L.
Camaioni, Donald M.
Derewinski, Miroslaw
Lercher, Johannes A.
TI Biomass conversion: Impact of zeolite stability on aquoeus phase
catalysis
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Vjunov, Aleksei; Fulton, John L.; Camaioni, Donald M.; Derewinski, Miroslaw; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Lercher, Johannes A.] TU Muenchen, Dept Chem, D-85747 Garching, Bavaria, Germany.
EM aleksei.vjunov@pnnl.gov
NR 0
TC 0
Z9 0
U1 1
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 254-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102518
ER
PT J
AU Wang, HX
Cramer, SP
AF Wang, Hongxin
Cramer, Stephen P.
TI Iron specific nuclear resonant vibrational spectroscopy and practical
issues in studying iron enzymes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Hongxin; Cramer, Stephen P.] Univ Calif Davis, Davis, CA 95616 USA.
[Wang, Hongxin; Cramer, Stephen P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM hongxin@popper.lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 159-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403762
ER
PT J
AU Wang, HX
Cramer, S
Gee, LB
Scott, AD
Ogata, H
Kramer, T
Neese, F
Lubitz, W
Newton, W
Dapper, C
Lauterbach, L
Pelmentschikov, V
Yoda, Y
Tanaka, Y
AF Wang, Hongxin
Cramer, Stephen
Gee, Leland B.
Scott, Aubrey D.
Ogata, Hideaki
Kraemer, Tobias
Neese, Frank
Lubitz, Wolfgang
Newton, William
Dapper, Christie
Lauterbach, Lars
Pelmentschikov, Vladimir
Yoda, Yoshitaka
Tanaka, Yoshihito
TI Nuclear resonant vibrational spectroscopy in studying extremely weak
features in hydrogenases and nitrogenases
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Hongxin; Cramer, Stephen; Gee, Leland B.; Scott, Aubrey D.] Univ Calif Davis, Davis, CA 95616 USA.
[Wang, Hongxin; Cramer, Stephen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Ogata, Hideaki; Kraemer, Tobias; Neese, Frank; Lubitz, Wolfgang] Max Planck Inst Bioinorgan Chem, Mulheim, Germany.
[Lauterbach, Lars; Pelmentschikov, Vladimir] Tech Univ Berlin, Inst Chem, Berlin, Germany.
[Newton, William; Dapper, Christie] Virginia Tech Univ, Dept Chem & Biochem, Blacksburg, VA 24061 USA.
[Yoda, Yoshitaka; Tanaka, Yoshihito] SPring 8, Res & Utilizat Div, Kouto, Hyogo 6795198, Japan.
EM hongxin@popper.lbl.gov
RI Ogata, Hideaki/J-4975-2013
NR 0
TC 0
Z9 0
U1 1
U2 8
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 705-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401354
ER
PT J
AU Wang, H
Lu, Y
Liu, L
Alexoff, D
Kim, SW
Hooker, JM
Fowler, JS
Tonge, PJ
AF Wang, Hui
Lu, Yang
Liu, Li
Alexoff, David
Kim, Sung Won
Hooker, Jacob M.
Fowler, Joanna S.
Tonge, Peter J.
TI Radiosynthesis and biological evaluation of a novel Enoyl-ACP reductase
inhibitor for Staphylococcus aureus
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Hui; Lu, Yang; Liu, Li; Tonge, Peter J.] SUNY Stony Brook, Dept Chemsitry, Stony Brook, NY 11794 USA.
[Wang, Hui; Lu, Yang; Liu, Li; Tonge, Peter J.] Inst Chem Biol & Drug Discovery, Stony Brook, NY 11794 USA.
[Alexoff, David; Kim, Sung Won; Hooker, Jacob M.; Fowler, Joanna S.] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
EM hui.wang@stonybrook.edu
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 377-MEDI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402178
ER
PT J
AU Wang, J
AF Wang, Jun
TI X-ray nano-imaging application on energy materials
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Jun] Brookhaven Natl Lab, Upton, NY 11973 USA.
EM junwang@bnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 612-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105412
ER
PT J
AU Wang, LW
AF Wang, Lin-Wang
TI Ab initio calculations of charge transports in nanosystems
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM lwwang@lbl.gov
NR 6
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 468-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105282
ER
PT J
AU Wang, YY
Fan, F
Agapov, A
Saito, T
Yang, J
Yu, X
Hong, KL
Mays, J
Sokolov, A
AF Wang, Yangyang
Fan, Fei
Agapov, Alexander
Saito, Tomonori
Yang, Jun
Yu, Xiang
Hong, Kunlun
Mays, Jimmy
Sokolov, Alexei
TI Relationship between ionic transport and segmental relaxation in polymer
electrolytes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Yangyang; Fan, Fei; Agapov, Alexander; Mays, Jimmy; Sokolov, Alexei] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
[Saito, Tomonori; Yu, Xiang; Mays, Jimmy; Sokolov, Alexei] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[Yang, Jun; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM yywang@utk.edu
RI Hong, Kunlun/E-9787-2015; Saito, Tomonori/M-1735-2016
OI Hong, Kunlun/0000-0002-2852-5111; Saito, Tomonori/0000-0002-4536-7530
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 292-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405420
ER
PT J
AU Wang, Y
Ramasamy, K
AF Wang, Yong
Ramasamy, Karthikeyan
TI Biomass derived small oxygenates to fuel range hydrocarbons over HZSM-5
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Yong; Ramasamy, Karthikeyan] Pacific NW Natl Lab, Richland, WA 99354 USA.
[Wang, Yong] Washington State Univ, Pullman, WA 99164 USA.
EM yong.wang@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 258-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105105
ER
PT J
AU Wang, Y
Hong, YC
Hensley, AJR
Sun, JM
McEven, JS
AF Wang, Yong
Hong, Yongchun
Hensley, Alyssa J. R.
Sun, Junming
McEven, Jean-Sabin
TI Hydrodeoxygenation of phenolics via noble metal promoted Fe catalysts: A
combined experimental and theoretical investigation
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Yong; Hong, Yongchun; Hensley, Alyssa J. R.; Sun, Junming; McEven, Jean-Sabin] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA.
[Wang, Yong; Hong, Yongchun] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Hong, Yongchun] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[McEven, Jean-Sabin] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA.
EM wang42@wsu.edu
RI Sun, Junming/B-3019-2011
OI Sun, Junming/0000-0002-0071-9635
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 105-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102378
ER
PT J
AU Wang, ZM
Pan, DQ
Yin, ZX
Resch, TC
Wu, WS
AF Wang, Zheming
Pan, Duo-Qiang
Yin, Zhuo-Xin
Resch, Tom C.
Wu, Wangsuo
TI Time resolved laser fluorescence spectroscopic study of uranium(VI)
sorption on phlogopite: Effect of pH and temperature
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Zheming; Resch, Tom C.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
[Pan, Duo-Qiang; Yin, Zhuo-Xin; Wu, Wangsuo] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Gansu, Peoples R China.
EM zheming.wang@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 27-GEOC
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400343
ER
PT J
AU Wang, Z
Shen, JM
Akatay, C
Kung, MC
Stach, E
Kung, H
AF Wang, Zhen
Shen, Jingmei
Akatay, Cem
Kung, Mayfair C.
Stach, Eric
Kung, Harold
TI New methods of synthesis of gold nanoparticles
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Zhen; Shen, Jingmei; Kung, Mayfair C.; Kung, Harold] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL USA.
[Akatay, Cem; Stach, Eric] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
EM hkung@northwestern.edu
RI Stach, Eric/D-8545-2011
OI Stach, Eric/0000-0002-3366-2153
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 83-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102356
ER
PT J
AU Wang, ZH
Chen, YL
Battaglia, V
Liu, G
AF Wang, Zhihui
Chen, Yulin
Battaglia, Vincent
Liu, Gao
TI Improving the performance of lithium-sulfur batteries using conductive
polymer and micrometric sulfur powder
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wang, Zhihui; Chen, Yulin; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM zhwang@lbl.gov
NR 0
TC 0
Z9 0
U1 4
U2 9
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 266-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105111
ER
PT J
AU Weber, RS
AF Weber, Robert S.
TI Modeling the kinetics of deactivation of catalysts during the upgrading
of bio-oil
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Weber, Robert S.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
EM Robert.Weber@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 283-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105126
ER
PT J
AU Wei, ZW
Martinez, B
Zhou, HC
Palakurthi, S
Bashir, S
Liu, JB
AF Wei, Zhangwen
Martinez, Baldemar
Zhou, Hong-Cai
Palakurthi, Srinath
Bashir, Sajid
Liu, Jingbo
TI Investigation of nanostructured metal-organic frameworks used in cancer
research
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Martinez, Baldemar; Bashir, Sajid; Liu, Jingbo] Texas A&M Univ Kingsville, Kingsville, TX USA.
[Wei, Zhangwen; Zhou, Hong-Cai; Liu, Jingbo] Texas A&M Univ, College Stn, TX USA.
[Bashir, Sajid; Liu, Jingbo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Palakurthi, Srinath] Texas A&M Hlth Sci Ctr, Kingsville, TX 78363 USA.
EM jingbo.liu@tamuk.edu
RI Wei, Zhangwen/D-2536-2016
OI Wei, Zhangwen/0000-0002-8378-2479
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 429-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165103853
ER
PT J
AU Wen, YH
Liu, DM
AF Wen, Youhai
Liu, Danmin
TI Electrochemistry based phase-field modeling of metal oxidation kinetics
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wen, Youhai] Natl Energy Technol Lab, Albany, OR 97321 USA.
[Liu, Danmin] Beijing Univ Technol, Inst Microstruct & Property Adv Mat, Beijing, Peoples R China.
EM youhai.wen@netl.doe.gov
NR 0
TC 0
Z9 0
U1 7
U2 15
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 336-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105172
ER
PT J
AU White, MG
Nakayama, M
Yang, YX
Zhou, J
Liu, P
AF White, Michael G.
Nakayama, Miki
Yang, Yixiong
Zhou, Jia
Liu, Ping
TI Interfacial charge transfer and reactivity of supported metal oxide
nanoclusters
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [White, Michael G.; Nakayama, Miki; Zhou, Jia; Liu, Ping] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[White, Michael G.; Yang, Yixiong] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.
EM mgwhite@bnl.gov
NR 0
TC 0
Z9 0
U1 2
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 421-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165103845
ER
PT J
AU Whittemore, S
AF Whittemore, Sean
TI Kinetic and thermodynamic study of the catalytic reduction of imines by
a linked Lewis pair
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Whittemore, Sean] Pacific NW Natl Lab, Richland, WA 99352 USA.
EM sean.whittemore@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 19-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102295
ER
PT J
AU Wichner, SM
DeWitt, MA
Yildiz, A
Cohen, BE
AF Wichner, Sara M.
DeWitt, Mark A.
Yildiz, Ahmet
Cohen, Bruce E.
TI Small quantum dot probes for single-molecule studies of motor proteins
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wichner, Sara M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94705 USA.
[Yildiz, Ahmet] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94705 USA.
[Yildiz, Ahmet] Univ Calif Berkeley, Dept Mol Biol, Berkeley, CA 94705 USA.
[Cohen, Bruce E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[DeWitt, Mark A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA.
EM sarawichner@gmail.com
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 216-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403818
ER
PT J
AU Wiedner, SD
Anderson, LN
Sadler, NC
Chrisler, WB
Kodali, VK
Smith, RD
Wright, AT
AF Wiedner, Susan D.
Anderson, Lindsey N.
Sadler, Natalie C.
Chrisler, William B.
Kodali, Vamsi K.
Smith, Richard D.
Wright, Aaron T.
TI Organelle-specific activity-based protein profiling in live macrophage
cells revealed by super-resolution imaging and proteomics
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wiedner, Susan D.; Anderson, Lindsey N.; Sadler, Natalie C.; Chrisler, William B.; Kodali, Vamsi K.; Smith, Richard D.; Wright, Aaron T.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
EM natalie.sadler@pnnl.gov; aaron.wright@pnnl.gov
RI Smith, Richard/J-3664-2012; Anderson, Lindsey /S-6375-2016
OI Smith, Richard/0000-0002-2381-2349; Anderson, Lindsey
/0000-0002-8741-7823
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 72-BIOL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101879
ER
PT J
AU Wiegel, AA
Wilson, KR
Hinsberg, WD
Houle, FA
AF Wiegel, Aaron A.
Wilson, Kevin R.
Hinsberg, William D.
Houle, Frances A.
TI Using kinetics modeling to investigate the role of structure and phase
on the functionalization and fragmentation of hydrocarbons in the
heterogeneous oxidation by OH
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wiegel, Aaron A.; Wilson, Kevin R.; Houle, Frances A.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94702 USA.
[Hinsberg, William D.] Columbia Hill Tech Consulting, Fremont, CA 94539 USA.
EM aawiegel@lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 265-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403863
ER
PT J
AU Wills, AW
Helms, BA
AF Wills, Andrew W.
Helms, Brett A.
TI Beyond the jammed matter limit: Binary pore architectures for low-k
dielectric applications
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wills, Andrew W.; Helms, Brett A.] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94703 USA.
EM awwills@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 423-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404777
ER
PT J
AU Wilson, JJ
Radchenko, V
John, KD
Birnbaum, ER
AF Wilson, Justin J.
Radchenko, Valery
John, Kevin D.
Birnbaum, Eva R.
TI From halogenated porphyrins to actinium
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wilson, Justin J.; Radchenko, Valery; John, Kevin D.; Birnbaum, Eva R.] Los Alamos Natl Lab, Dept Chem, Los Alamos, NM 87545 USA.
EM eva@lanl.gov
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 342-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401009
ER
PT J
AU Wilson, KR
AF Wilson, Kevin R.
TI Multiphase chemistry of organic aerosols: The role of water, molecular
structure, and viscosity
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wilson, Kevin R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
EM krwilson@lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 260-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403858
ER
PT J
AU Winter, ND
Winter, NW
AF Winter, Nicolas D.
Winter, Nicholas W.
TI Molecular dynamics simulations of the ligand exchange reaction for the
aqueous beryllium(II) ion
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Winter, Nicolas D.] Dominican Univ, Dept Phys Sci, River Forest, IL 60305 USA.
[Winter, Nicholas W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Geophys, Berkeley, CA 94720 USA.
EM nwinter@dom.edu
NR 0
TC 0
Z9 0
U1 0
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 542-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404253
ER
PT J
AU Wood, BC
AF Wood, Brandon C.
TI Towards simulations of electrochemical interfaces in graphene-based
supercapacitors under realistic operating conditions
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wood, Brandon C.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA.
EM brandonwood@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 127-COMP
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104366
ER
PT J
AU Wright, A
Sadler, NC
Nandhikonda, P
Crowell, SR
Smith, RD
Corley, RA
AF Wright, Aaron
Sadler, Natalie C.
Nandhikonda, Premchendar
Crowell, Susan R.
Smith, Richard D.
Corley, Richard A.
TI Activity-based protein profiling of cytochrome P450 enzyme ontogeny in
the developing human fetus
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wright, Aaron; Sadler, Natalie C.; Nandhikonda, Premchendar; Crowell, Susan R.; Smith, Richard D.; Corley, Richard A.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
EM aaron.wright@pnnl.gov
RI Smith, Richard/J-3664-2012
OI Smith, Richard/0000-0002-2381-2349
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 134-TOXI
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167406284
ER
PT J
AU Wu, CH
Velasco-Velez, JJ
Fang, HT
Guo, JH
Salmeron, MB
AF Wu, Chenghao
Velasco-Velez, Juan J.
Fang, Haitao
Guo, Jinghua
Salmeron, Miquel B.
TI In-situ X-ray absorption spectroscopy study of metal/water interfaces
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wu, Chenghao] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Wu, Chenghao; Velasco-Velez, Juan J.; Fang, Haitao; Salmeron, Miquel B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Fang, Haitao] Harbin Inst Technol, Coll Mat Sci & Engn, Harbin 150001, Heilongjiang, Peoples R China.
[Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Salmeron, Miquel B.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
EM chenghaowu@lbl.gov
NR 0
TC 0
Z9 0
U1 1
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 117-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165103560
ER
PT J
AU Wu, MY
Yuan, W
Park, SJ
Battaglia, V
Liu, G
AF Wu, Mingyan
Yuan, Wen
Park, Sang-Jae
Battaglia, Vincent
Liu, Gao
TI Toward an ideal polymer binder design for high-capacity battery anodes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wu, Mingyan; Yuan, Wen; Park, Sang-Jae; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EETD, Berkeley, CA 94720 USA.
EM GLiu@lbl.gov
RI Yuan, Wen/G-7141-2015
OI Yuan, Wen/0000-0002-1812-9588
NR 0
TC 0
Z9 0
U1 3
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 540-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405030
ER
PT J
AU Wu, MY
Yuan, W
Park, SJ
Battaglia, VS
Liu, G
AF Wu, Mingyan
Yuan, Wen
Park, Sang-Jae
Battaglia, Vincent S.
Liu, Gao
TI In situ formed si nanoparticle network with micron-sized si particles
for lithium-ion battery anodes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wu, Mingyan; Yuan, Wen; Park, Sang-Jae; Battaglia, Vincent S.; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EETD, Berkeley, CA 94720 USA.
EM GLiu@lbl.gov
RI Yuan, Wen/G-7141-2015
OI Yuan, Wen/0000-0002-1812-9588
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 20-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104754
ER
PT J
AU Wu, QY
Cen, JJ
Zhao, Y
Su, D
Zhao, S
Shen, PC
Worner, W
White, M
Orlov, A
AF Wu, Qiyuan
Cen, Jiajie
Zhao, Yue
Su, Dong
Zhao, Shen
Shen, Peichuan
Worner, William
White, Michael
Orlov, Alexander
TI Developing novel light activated composite nanomaterials based on
perovskite structure for energy and environmental applications
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Wu, Qiyuan; Cen, Jiajie; Zhao, Yue; Zhao, Shen; Shen, Peichuan; White, Michael; Orlov, Alexander] SUNY Stony Brook, Stony Brook, NY 11794 USA.
[Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Worner, William] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA.
[White, Michael] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM qiyuan.wu@stonybrook.edu; jiajie.cen@stonybrook.edu;
yue.zhao.1@stonybrook.edu
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 686-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400013
ER
PT J
AU Wu, ZL
Mann, AK
Li, MJ
Overbury, SH
AF Wu, Zili
Mann, Amanda K.
Li, Meijun
Overbury, Steven H.
TI Understanding shape effect in catalysis: A case study of ceria
nanoshapes as catalyst and catalyst support
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM wuz1@ornl.gov
RI Overbury, Steven/C-5108-2016
OI Overbury, Steven/0000-0002-5137-3961
NR 0
TC 0
Z9 0
U1 0
U2 8
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 488-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105300
ER
PT J
AU Xantheas, SS
Miliordos, E
AF Xantheas, Sotiris S.
Miliordos, Evangelos
TI Efficient procedure for the numerical calculation of harmonic
vibrational frequencies based on internal coordinates: CCSD(T)
frequencies for (H2O)(n), n=2-8 and other aqueous complexes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xantheas, Sotiris S.; Miliordos, Evangelos] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
EM sotiris.xantheas@pnnl.gov
RI Xantheas, Sotiris/L-1239-2015
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 315-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404039
ER
PT J
AU Xiao, DJ
Bloch, ED
Mason, JA
Queen, WL
Hudson, MR
Brown, CM
Long, JR
AF Xiao, Dianne J.
Bloch, Eric D.
Mason, Jarad A.
Queen, Wendy L.
Hudson, Matthew R.
Brown, Craig M.
Long, Jeffrey R.
TI Hydrocarbon oxidations using iron metal-organic frameworks
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xiao, Dianne J.; Bloch, Eric D.; Mason, Jarad A.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Queen, Wendy L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Hudson, Matthew R.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA.
[Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA.
EM djxiao@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 437-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401100
ER
PT J
AU Xiao, J
AF Xiao, Jie
TI Graphene in Li-O-2 and Li-CFx batteries
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xiao, Jie] Pacific NW Natl Lab, Div Energy & Environm, Richland, WA 99352 USA.
EM jie.xiao@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 5
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 501-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105313
ER
PT J
AU Xiao, J
AF Xiao, Jie
TI Carbon in primary lithium air batteries
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
ID LI/AIR BATTERIES; ELECTRODE
C1 [Xiao, Jie] Pacific NW Natl Lab, Div Energy & Environm, Richland, WA 99352 USA.
EM jie.xiao@pnnl.gov
NR 5
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 491-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105303
ER
PT J
AU Xu, M
Kovarik, L
Arey, BW
Engelhard, MH
Ilton, ES
Perea, DE
Felmy, AR
Rosso, KM
Kerisit, S
AF Xu, Man
Kovarik, Libor
Arey, Bruce W.
Engelhard, Mark H.
Ilton, Eugene S.
Perea, Daniel E.
Felmy, Andrew R.
Rosso, Kevin M.
Kerisit, Sebastien
TI Heteroepitaxial growth of carbonates at calcite-water interfaces:
Effects of solution chemistry and crystal lattice mismatch
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xu, Man; Kovarik, Libor; Arey, Bruce W.; Engelhard, Mark H.; Ilton, Eugene S.; Perea, Daniel E.; Felmy, Andrew R.; Rosso, Kevin M.; Kerisit, Sebastien] Pacific NW Natl Lab, Richland, WA 99352 USA.
EM man.xu@pnnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 9-GEOC
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400326
ER
PT J
AU Xu, MZ
Mukarakate, C
Nimlos, M
Trewyn, BG
Richards, RM
AF Xu, Mengze
Mukarakate, Calvin
Nimlos, Mark
Trewyn, Brian G.
Richards, Ryan M.
TI Upgrading of biomass pyrolysis with sheet-like mesoporous MFI zeolite
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xu, Mengze; Trewyn, Brian G.; Richards, Ryan M.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA.
[Mukarakate, Calvin; Nimlos, Mark] Natl Renewable Energy Lab, Golden, CO 80401 USA.
EM mxu@mines.edu
RI Richards, Ryan/B-3513-2008
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 376-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105207
ER
PT J
AU Xu, T
AF Xu, Ting
TI Toward using protein/peptide as material building block
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Xu, Ting] Univ Calif Berkeley, Dept Mat Sci & Engn, Dept Chem, Berkeley, CA 94720 USA.
[Xu, Ting] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA.
EM tingxu@berkeley.edu
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 196-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105624
ER
PT J
AU Yaghi, OM
AF Yaghi, Omar M.
TI Multivariate metal-organic frameworks for carbon dioxide capture in the
presence of water
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Yaghi, Omar M.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA.
[Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM yaghi@berkeley.edu
NR 0
TC 0
Z9 0
U1 1
U2 8
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 375-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401040
ER
PT J
AU Yaghi, OM
AF Yaghi, Omar M.
TI High volumetric methane uptake in aluminum metal-organic frameworks
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA.
EM yaghi@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 49-ENFL
PG 2
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104777
ER
PT J
AU Yan, RX
Yan, PD
Sun, JW
AF Yan, Ruoxue
Yan, Peidong
Sun, Jianwei
TI Biomimic molysulfide co-catalyst for hydrogen photosynthesis
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yan, Ruoxue] Univ Calif Riverside, Dept Chem & Environm Engn, Riverside, CA 92521 USA.
[Yan, Ruoxue; Yan, Peidong; Sun, Jianwei] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Yan, Ruoxue; Yan, Peidong; Sun, Jianwei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Yan, Ruoxue] Univ Calif Riverside, Riverside, CA 92521 USA.
[Yan, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
EM rxyan@engr.ucr.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 23-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102299
ER
PT J
AU Yang, DL
Hubbard, KM
Henderson, KC
Devlin, DJ
Pacheco, RM
AF Yang, Dali
Hubbard, Kevin M.
Henderson, Kevin C.
Devlin, David J.
Pacheco, Robin M.
TI Thermal stability of NP, VCE, and its composites at isothermal and
non-isothermal conditions
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yang, Dali; Hubbard, Kevin M.; Henderson, Kevin C.; Devlin, David J.; Pacheco, Robin M.] Los Alamos Natl Lab, MST 7, Los Alamos, NM 87545 USA.
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 642-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405754
ER
PT J
AU Yang, PD
AF Yang, Peidong
TI Semiconductor nanowires for energy conversion
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yang, Peidong] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM p_yang@berkeley.edu
NR 0
TC 0
Z9 0
U1 2
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 286-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105128
ER
PT J
AU Yang, TR
Lin, HT
Wei, TY
Honda, H
Dai, M
AF Yang, Tairan
Lin, Hua-Tay
Wei, Tsao-Yi
Honda, Hiroshi
Dai, Meng
TI New functionalized tetracyanoquinodimethanes and precursors for
synthetic metals
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yang, Tairan] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada.
[Lin, Hua-Tay] Oak Ridge Natl Lab, Dept Mat Sci, Oak Ridge, TN 37831 USA.
[Wei, Tsao-Yi; Honda, Hiroshi; Dai, Meng] Northwestern Polytech Univ, Dept Bioengn, Fremont, CA 94539 USA.
EM yangtairan@gmail.com
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 724-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401372
ER
PT J
AU Yao, R
Laguisma, GAL
Osborn, D
Taatjes, C
Meloni, G
AF Yao, Rong
Laguisma, Gabrielle Anne L.
Osborn, David
Taatjes, Craig
Meloni, Giovanni
TI Low temperature oxidation of furfural using synchrotron photoionization
mass spectroscopy
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yao, Rong; Laguisma, Gabrielle Anne L.; Meloni, Giovanni] Univ San Francisco, Dept Chem, San Francisco, CA 94117 USA.
[Osborn, David; Taatjes, Craig] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA.
EM ryao4@usfca.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 537-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404248
ER
PT J
AU Yen, HJ
Tsai, HH
Kuo, CY
Nie, WY
Mohite, AD
Gupta, G
Wang, J
Wu, JH
Liou, GS
Wang, HL
AF Yen, Hung-Ju
Tsai, Hsinhan
Kuo, Cheng-Yu
Nie, Wanyi
Mohite, Aditya D.
Gupta, Gautam
Wang, Jian
Wu, Jia-Hao
Liou, Guey-Sheng
Wang, Hsing-Lin
TI Flexible nonvolatile polymer memory devices derived from donor-donor and
donor-acceptor conjugated polymers
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yen, Hung-Ju; Tsai, Hsinhan; Kuo, Cheng-Yu; Wang, Hsing-Lin] Los Alamos Natl Lab, Phys Chem & Appl Spect C PCS, Div Chem, Los Alamos, NM 87545 USA.
[Nie, Wanyi; Mohite, Aditya D.; Gupta, Gautam] Los Alamos Natl Lab, Mat Synth & Integrated Devices MPA 11, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
[Wang, Jian] Los Alamos Natl Lab, Mat Sci Radiat & Dynam MST 8, Mat Sci & Technol Div, Los Alamos, NM 87545 USA.
[Wu, Jia-Hao; Liou, Guey-Sheng] Natl Taiwan Univ, Inst Polymer Sci & Engn, Taipei 10764, Taiwan.
EM hjyen@lanl.gov
RI Wang, Jian/F-2669-2012
OI Wang, Jian/0000-0001-5130-300X
NR 3
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 392-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404752
ER
PT J
AU Yi, S
Houtz, EF
Harding, KC
Field, JA
Sedlak, DL
Alvarez-Cohen, L
AF Yi, Shan
Houtz, Erika F.
Harding, Katie C.
Field, Jennifer A.
Sedlak, David L.
Alvarez-Cohen, Lisa
TI Detection and identification of anaerobic biotransformation products of
polyfluorochemicals in aqueous film-forming foams
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yi, Shan; Houtz, Erika F.; Harding, Katie C.; Sedlak, David L.; Alvarez-Cohen, Lisa] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
[Field, Jennifer A.] Oregon State Univ, Dept Mol & Environm Toxicol, Corvallis, OR 97331 USA.
[Alvarez-Cohen, Lisa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
EM shan_yi@berkeley.edu
NR 0
TC 0
Z9 0
U1 1
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 861-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400174
ER
PT J
AU Yoo, S
Proulx, C
Zuckermann, RN
AF Yoo, Stan
Proulx, Caroline
Zuckermann, Ronald N.
TI Improved synthesis of peptoids with electron-deficient side chains and
their application in controlling chain conformation
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yoo, Stan; Proulx, Caroline; Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
EM SeungheeYoo@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 261-ORGN
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402725
ER
PT J
AU Younes, W
AF Younes, Walid
TI Nuclear fission inside astrophysical plasmas
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Younes, Walid] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
EM younes1@llnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 52-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402393
ER
PT J
AU Yu, CJ
Aubrey, ML
Wiers, BM
Keitz, BK
Long, JR
AF Yu, Chung Jui
Aubrey, Michael L.
Wiers, Brian M.
Keitz, Benjamin K.
Long, Jeffrey R.
TI Electrochemical cation insertion into metal-organic frameworks
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yu, Chung Jui; Aubrey, Michael L.; Wiers, Brian M.; Keitz, Benjamin K.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Mat Sci, Berkeley, CA 94720 USA.
EM raymond.yu@berkeley.edu
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 198-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400743
ER
PT J
AU Yuan, GB
Frei, H
AF Yuan, Guangbi
Frei, Heinz
TI Investigation of nanometer scale silica films as the robust proton
conducting, gas impermeable membrane for artificial photosynthesis
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yuan, Guangbi; Frei, Heinz] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
EM gbyuan@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 602-ENVR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165106156
ER
PT J
AU Yuca, N
Zhao, H
Dogdu, MF
Battaglia, VS
Liu, G
AF Yuca, Neslihan
Zhao, Hui
Dogdu, Murat Ferhat
Battaglia, Vincent S.
Liu, Gao
TI Effect of flexible polymer binders on electrochemical performance of
graphite negative electrode for lithium ion batteries
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yuca, Neslihan; Zhao, Hui; Battaglia, Vincent S.; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Yuca, Neslihan; Dogdu, Murat Ferhat] Istanbul Tech Univ, Energy Inst, Istanbul, Turkey.
EM huizhao@lbl.gov
NR 0
TC 0
Z9 0
U1 3
U2 3
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 542-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405032
ER
PT J
AU Yung, MM
Mukarakate, C
Engtrakul, C
Starace, A
AF Yung, Matthew M.
Mukarakate, Calvin
Engtrakul, Chaiwat
Starace, Anne
TI Upgrading biomass-derived pyrolysis vapors on catalysts of varying
acidity
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Yung, Matthew M.; Mukarakate, Calvin; Engtrakul, Chaiwat; Starace, Anne] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA.
EM matthew.yung@nrel.gov
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 137-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104860
ER
PT J
AU Zang, HD
Routh, PK
Cotlet, M
AF Zang, Huidong
Routh, Prahlad Kumar
Cotlet, Mircea
TI Regulating the intermittency of CdSe/ZnS quantum dots through controlled
charge transfer
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zang, Huidong; Routh, Prahlad Kumar; Cotlet, Mircea] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
EM hzang@bnl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 712-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104236
ER
PT J
AU Zavarin, M
Begg, JD
Zhao, PH
Boggs, MA
Joseph, C
Dai, ZR
Kersting, AB
AF Zavarin, Mavrik
Begg, James D.
Zhao, Pihong
Boggs, Mark A.
Joseph, Claudia
Dai, Zurong
Kersting, Annie B.
TI Colloid-facilitated Pu transport mechanisms at the Nevada National
Security Site: Linking field evidence, laboratory desorption kinetics,
and Pu desorption from glass alteration products
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zavarin, Mavrik; Begg, James D.; Zhao, Pihong; Boggs, Mark A.; Joseph, Claudia; Dai, Zurong; Kersting, Annie B.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Glenn T Seaborg Inst, Livermore, CA 64551 USA.
EM zavarin1@llnl.gov
NR 0
TC 0
Z9 0
U1 2
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 95-NUCL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167402435
ER
PT J
AU Zelenay, P
Chung, HT
Holby, EF
Taylor, CD
Wu, G
AF Zelenay, Piotr
Chung, Hoon T.
Holby, Edward F.
Taylor, Christopher D.
Wu, Gang
TI Carbon composite non-precious metal catalysts for oxygen reduction in
electrochemical energy conversion
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zelenay, Piotr; Chung, Hoon T.; Wu, Gang] Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
[Holby, Edward F.; Taylor, Christopher D.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA.
EM zelenay@lanl.gov
RI Wu, Gang/E-8536-2010; Chung, Hoon/A-7916-2012
OI Wu, Gang/0000-0003-4956-5208; Chung, Hoon/0000-0002-5367-9294
NR 0
TC 0
Z9 0
U1 2
U2 10
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 543-ENFL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165105351
ER
PT J
AU Zhang, BA
Azoulay, JD
Foster, ME
AF Zhang, Benjamin A.
Azoulay, Jason D.
Foster, Michael E.
TI Elucidation of features relevant to structural control and band gap
narrowing in donor acceptor copolymers using bridgehead imine
substituted cyclopentadithiophene derivatives
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhang, Benjamin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Zhang, Benjamin A.; Azoulay, Jason D.; Foster, Michael E.] Sandia Natl Labs, Dept Chem Mat, Livermore, CA 94551 USA.
EM bazhang@lbl.gov
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 447-POLY
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167405571
ER
PT J
AU Zhang, GH
Yi, H
Zhang, GT
Deng, Y
Bai, RP
Zhang, H
Krentz, T
Miller, JT
Kropf, AJ
Bunel, EE
Lei, AW
AF Zhang, Guanghui
Yi, Hong
Zhang, Guoting
Deng, Yi
Bai, Ruopeng
Zhang, Heng
Krentz, Timothy
Miller, Jeffrey T.
Kropf, A. Jeremy
Bunel, Emilio E.
Lei, Aiwen
TI Direct observation of reduction of Cu(II) to Cu(I) by terminal alkynes
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhang, Guanghui; Yi, Hong; Zhang, Guoting; Deng, Yi; Bai, Ruopeng; Zhang, Heng; Lei, Aiwen] Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China.
[Miller, Jeffrey T.; Kropf, A. Jeremy; Bunel, Emilio E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
EM guanghuizhang@whu.edu.cn
RI ID, MRCAT/G-7586-2011
NR 0
TC 0
Z9 0
U1 3
U2 10
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 162-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167400709
ER
PT J
AU Zhang, HF
Worton, DR
Shen, S
Wilson, KR
Goldstein, AH
AF Zhang, Haofei
Worton, David R.
Shen, Steve
Wilson, Kevin R.
Goldstein, Allen H.
TI Understanding the evolution of long-chain n-alkanes in the atmosphere
using gas chromatography-vacuum ultraviolet-mass spectrometry
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhang, Haofei; Worton, David R.; Goldstein, Allen H.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Zhang, Haofei; Wilson, Kevin R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
[Shen, Steve] Univ Calif Berk, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
[Goldstein, Allen H.] Univ Calif Berk, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
EM hfzhang@berkeley.edu
NR 0
TC 0
Z9 0
U1 1
U2 2
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 145-PHYS
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167403749
ER
PT J
AU Zhang, M
Frei, H
AF Zhang, Miao
Frei, Heinz
TI Direct observations of water oxidation intermediates on Co3O4
nanoparticle catalysts with time-resolved FTIR spectroscopy
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhang, Miao; Frei, Heinz] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
EM MZhang@lbl.gov
NR 1
TC 0
Z9 0
U1 1
U2 7
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 119-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102391
ER
PT J
AU Zhao, CQ
Hwang, SH
Buchholz, BA
Yang, J
Hammock, BD
Casida, JE
AF Zhao, Chunqing
Hwang, Sung Hee
Buchholz, Bruce A.
Yang, Jun
Hammock, Bruce D.
Casida, John E.
TI Determining the receptor target of tetramethylenedisulfotetramine
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhao, Chunqing; Casida, John E.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA.
[Hwang, Sung Hee; Yang, Jun; Hammock, Bruce D.] Univ Calif Davis, Dept Entomol & Nematol, Davis, CA 95616 USA.
[Buchholz, Bruce A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA.
EM buchholz2@llnl.gov
NR 0
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 145-ANYL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165101595
ER
PT J
AU Zheng, HM
AF Zheng, Haimei
TI Nanocrystal shape evolution during growth
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Zheng, Haimei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
EM hmzheng@lbl.gov
NR 2
TC 0
Z9 0
U1 1
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 409-INOR
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167401074
ER
PT J
AU Zheng, YL
Giordano, AJ
Cowan, SR
Fleming, SR
Shallcross, RC
Gliboff, M
Huang, YM
Ginger, DS
McGrath, DV
Armstrong, NR
Olson, DC
Marder, SR
Saavedra, SS
AF Zheng, Yilong
Giordano, Anthony J.
Cowan, Sara R.
Fleming, Sean R.
Shallcross, R. Clayton
Gliboff, Matthew
Huang, Yiming
Ginger, David S.
McGrath, Dominic V.
Armstrong, Neal R.
Olson, Dana C.
Marder, Seth R.
Saavedra, S. Scott
TI Surface modification of transparent conducting oxides with
functionalized perylene diimide dyes: Characterization of orientation,
charge-transfer kinetics, and related OPV performance
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zheng, Yilong; Fleming, Sean R.; Shallcross, R. Clayton; Huang, Yiming; McGrath, Dominic V.; Armstrong, Neal R.; Saavedra, S. Scott] Univ Arizona, Dept Chem & Biochem, Tucson, AZ 85721 USA.
[Giordano, Anthony J.; Marder, Seth R.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA.
[Giordano, Anthony J.; Marder, Seth R.] Georgia Inst Technol, Ctr Organ Photon & Elect, Atlanta, GA 30332 USA.
[Cowan, Sara R.; Olson, Dana C.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Gliboff, Matthew] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Ginger, David S.] Univ Washington, Dept Chem, Seattle, WA 98195 USA.
EM zhengyl@email.arizona.edu
RI Saavedra, Steven/K-6957-2014; Zhou, David/N-5367-2015
OI Saavedra, Steven/0000-0002-9946-2664;
NR 0
TC 0
Z9 0
U1 0
U2 4
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 473-COLL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165104010
ER
PT J
AU Zhong, MJ
Kim, EK
Nulwala, H
Star, A
Kowalewski, T
Matyjaszewski, K
AF Zhong, Mingjiang
Kim, Eun Kyung
Nulwala, Hunaid
Star, Alexander
Kowalewski, Tomasz
Matyjaszewski, Krzysztof
TI Block copolymers for rational design of nitrogen-enriched nanocarbons
suitable for sustainable energy applications
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhong, Mingjiang; Kim, Eun Kyung; Nulwala, Hunaid; Kowalewski, Tomasz; Matyjaszewski, Krzysztof] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA.
[Nulwala, Hunaid] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
[Star, Alexander] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA.
EM mj_zhong@mit.edu
RI Zhong, Mingjiang/F-3470-2011
OI Zhong, Mingjiang/0000-0001-7533-4708
NR 0
TC 0
Z9 0
U1 0
U2 0
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 8-PMSE
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404383
ER
PT J
AU Zhu, HY
Sigdel, A
Zhang, S
Su, D
Sun, SH
AF Zhu, Huiyuan
Sigdel, Aruna
Zhang, Sen
Su, Dong
Sun, Shouheng
TI Monodisperse MnAu nanoparticles and their phase segregation for high
sensitive H2O2 detection
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhu, Huiyuan; Sigdel, Aruna; Zhang, Sen; Sun, Shouheng] Brown Univ, Providence, RI 02912 USA.
[Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
EM huiyuan_zhu@brown.edu
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 313-CATL
PG 1
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8JN
UT WOS:000349165102568
ER
PT J
AU Zhu, X
Hu, J
Liu, HL
Dai, S
AF Zhu, Xiang
Hu, Jun
Liu, Honglai
Dai, Sheng
TI Task-specific porous organic polymer for high CO2/N-2 selectivity
SO ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Meeting Abstract
CT 248th National Meeting of the American-Chemical-Society (ACS)
CY AUG 10-14, 2014
CL San Francisco, CA
SP Amer Chem Soc
C1 [Zhu, Xiang; Hu, Jun; Liu, Honglai] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China.
[Zhu, Xiang; Hu, Jun; Liu, Honglai] E China Univ Sci & Technol, Dept Chem, Shanghai 200237, Peoples R China.
[Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Knoxville, TN 37831 USA.
EM zhuxiang.ecust@gmail.com
NR 0
TC 0
Z9 0
U1 0
U2 1
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0065-7727
J9 ABSTR PAP AM CHEM S
JI Abstr. Pap. Am. Chem. Soc.
PD AUG 10
PY 2014
VL 248
MA 456-PMSE
PG 2
WC Chemistry, Multidisciplinary
SC Chemistry
GA CA8KC
UT WOS:000349167404802
ER
PT J
AU Bodaghee, A
Tomsick, JA
Krivonos, R
Stern, D
Bauer, FE
Fornasini, FM
Barriere, N
Boggs, SE
Christensen, FE
Craig, WW
Gotthelf, EV
Hailey, CJ
Harrison, FA
Hong, J
Mori, K
Zhang, WW
AF Bodaghee, Arash
Tomsick, John A.
Krivonos, Roman
Stern, Daniel
Bauer, Franz E.
Fornasini, Francesca M.
Barriere, Nicolas
Boggs, Steven E.
Christensen, Finn E.
Craig, William W.
Gotthelf, Eric V.
Hailey, Charles J.
Harrison, Fiona A.
Hong, Jaesub
Mori, Kaya
Zhang, William W.
TI INITIAL RESULTS FROM NuSTAR OBSERVATIONS OF THE NORMA ARM
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE binaries: general; novae, cataclysmic variables; stars: neutron; X-rays:
binaries
ID MAGNETIC CATACLYSMIC VARIABLES; X-RAY SURVEY; GALACTIC-CENTER;
STAR-FORMATION; CATALOG; COMPLEX
AB Results are presented for an initial survey of the Norma Arm gathered with the focusing hard X-Ray Telescope NuSTAR. The survey covers 0.2 deg(2) of sky area in the 3-79 keV range with a minimum and maximum raw depth of 15 ks and 135 ks, respectively. Besides a bright black-hole X-ray binary in outburst (4U 1630-47) and a new X-ray transient (NuSTAR J163433-473841), NuSTAR locates three sources from the Chandra survey of this region whose spectra are extended above 10 keV for the first time: CXOU J163329.5-473332, CXOU J163350.9-474638, and CXOU J163355.1-473804. Imaging, timing, and spectral data from a broad X-ray range (0.3-79 keV) are analyzed and interpreted with the aim of classifying these objects. CXOU J163329.5-473332 is either a cataclysmic variable or a faint low-mass X-ray binary. CXOU J163350.9-474638 varies in intensity on year-long timescales, and with no multi-wavelength counterpart, it could be a distant X-ray binary or possibly a magnetar. CXOU J163355.1-473804 features a helium-like iron line at 6.7 keV and is classified as a nearby cataclysmic variable. Additional surveys are planned for the Norma Arm and Galactic Center, and those NuSTAR observations will benefit from the lessons learned during this pilot study.
C1 [Bodaghee, Arash; Tomsick, John A.; Krivonos, Roman; Barriere, Nicolas; Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.
[Bodaghee, Arash] Georgia Coll & State Univ, Milledgeville, GA 31061 USA.
[Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA.
[Bauer, Franz E.] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile.
[Bauer, Franz E.] Millennium Inst Astrophys, Santiago, Chile.
[Bauer, Franz E.] Space Sci Inst, Boulder, CO 80301 USA.
[Fornasini, Francesca M.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA.
[Christensen, Finn E.] Tech Univ Denmark, DTU Space, Natl Space Inst, DK-2800 Lyngby, Denmark.
[Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Gotthelf, Eric V.; Hailey, Charles J.; Mori, Kaya] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA.
[Harrison, Fiona A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA.
[Hong, Jaesub] Harvard Univ, Dept Astron, Cambridge, MA 02138 USA.
[Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
RP Bodaghee, A (reprint author), Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA.
RI Boggs, Steven/E-4170-2015
OI Boggs, Steven/0000-0001-9567-4224
FU NASA [NNG08FD60C]; National Science Foundation Graduate Research
Fellowship; BasalCATA [PFB-06/2007]; CONICYT-Chile [FONDECYT 1141218]
FX This work was supported under NASA Contract No. NNG08FD60C, and made use
of data from the NuSTAR mission, a project led by the California
Institute of Technology, managed by the Jet Propulsion Laboratory, and
funded by the National Aeronautics and Space Administration. We thank
the NuSTAR Operations, Software, and Calibration teams for support with
the execution and analysis of these observations. This research has made
use of the NuSTAR Data Analysis Software (NuSTAR-DAS) jointly developed
by the ASI Science Data Center (ASDC, Italy) and the California
Institute of Technology. This research has made use of: data obtained
from the High Energy Astrophysics Science Archive Research Center
(HEASARC) provided by NASA's Goddard Space Flight Center; NASA's
Astrophysics Data System Bibliographic Services; and the SIMBAD database
operated at CDS, Strasbourg, France. F. M. F. acknowledges support from
the National Science Foundation Graduate Research Fellowship. F. E. B.
acknowledges support from BasalCATA PFB-06/2007, CONICYT-Chile (FONDECYT
1141218 and "EMBIGGEN" Anillo ACT1101), and Project IC120009 "Millennium
Institute of Astrophysics (MAS)" of Iniciativa Cient ' ifica Milenio del
Ministerio de Economia, Fomento y Turismo.
NR 37
TC 3
Z9 3
U1 1
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
EI 1538-4357
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 10
PY 2014
VL 791
IS 1
AR 68
DI 10.1088/0004-637X/791/1
PG 10
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA AM2CY
UT WOS:000339657700068
ER
PT J
AU Degenaar, N
Medin, Z
Cumming, A
Wijnands, R
Wolff, MT
Cackett, EM
Miller, JM
Jonker, PG
Homan, J
Brown, EF
AF Degenaar, N.
Medin, Z.
Cumming, A.
Wijnands, R.
Wolff, M. T.
Cackett, E. M.
Miller, J. M.
Jonker, P. G.
Homan, J.
Brown, E. F.
TI PROBING THE CRUST OF THE NEUTRON STAR IN EXO 0748-676
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE accretion, accretion disks; binaries: eclipsing; stars: individual (EXO
0748-676); stars: neutron; X-rays: binaries
ID X-RAY TRANSIENT; PHOTON IMAGING CAMERA; COOLING LIGHT CURVES; BINARY MXB
1659-29; XMM-NEWTON; CEN X-4; QUIESCENT STATE; XTE J1701-462; KS
1731-260; TERZAN 5
AB X-ray observations of quiescent X-ray binaries have the potential to provide insight into the structure and the composition of neutron stars. EXO 0748-676 had been actively accreting for over 24 yr before its outburst ceased in late 2008. Subsequent X-ray monitoring revealed a gradual decay of the quiescent thermal emission that can be attributed to cooling of the accretion-heated neutron star crust. In this work, we report on new Chandra and Swift observations that extend the quiescent monitoring to similar or equal to 5 yr post-outburst. We find that the neutron star temperature remained at similar or equal to 117 eV between 2009 and 2011, but had decreased to similar or equal to 110 eV in 2013. This suggests that the crust has not fully cooled yet, which is supported by the lower temperature (similar or equal to 95 eV) measured similar or equal to 4 yr prior to the accretion phase in 1980. Comparing the data to thermal evolution simulations reveals that the apparent lack of cooling between 2009 and 2011 could possibly be a signature of convection driven by phase separation of light and heavy nuclei in the outer layers of the neutron star.
C1 [Degenaar, N.; Miller, J. M.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA.
[Medin, Z.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Cumming, A.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada.
[Wijnands, R.] Univ Amsterdam, Astron Inst Anton Pannekoek, NL-1090 GE Amsterdam, Netherlands.
[Wolff, M. T.] Naval Res Lab, Div Space Sci, Washington, DC 20375 USA.
[Cackett, E. M.] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48201 USA.
[Jonker, P. G.] SRON Netherlands Inst Space Res, SRON, NL-3584 CA Utrecht, Netherlands.
[Jonker, P. G.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA.
[Homan, J.] MIT Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA.
[Brown, E. F.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
RP Degenaar, N (reprint author), Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA.
EM degenaar@umich.edu
OI Brown, Edward/0000-0003-3806-5339
FU NASA through Hubble Postdoctoral Fellowship from the Space Telescope
Science Institute (STScI) [HST-HF-51287.01-A]; NASA through Chandra
award [GO3-14050X]; National Aeronautics and Space Administration (NASA)
[NAS8-03060, NAS 5-26555]; NSERC Discovery Grant; Office of Naval
Research
FX N.D. is supported by NASA through Hubble Postdoctoral Fellowship grant
number HST-HF-51287.01-A from the Space Telescope Science Institute
(STScI), which is operated by the Association of Universities for
Research in Astronomy, Incorporated, under the National Aeronautics and
Space Administration (NASA) contract NAS 5-26555. Support for this work
was provided by the NASA through Chandra award No. GO3-14050X issued by
the Chandra X-ray Observatory Center which is operated by the
Smithsonian Astrophysical Observatory for and on behalf of the NASA
under contract NAS8-03060. A.C. is supported by an NSERC Discovery Grant
and is an Associate Member of the CIFAR Cosmology and Gravity program.
M.T.W. is supported by the Office of Naval Research. The authors are
grateful to Neil Gehrels and the Swift planning team for approving and
scheduling the Swift TOO observations of EXO 0748-676. N.D., A.C., R.W.,
E.C., and E.B. acknowledge the hospitality of the International Space
Science Institute in Bern, Switzerland, where part of this work was
carried out. The authors are grateful to the anonymous referee and Joel
Fridriksson for very useful comments.
NR 78
TC 14
Z9 14
U1 1
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
EI 1538-4357
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 10
PY 2014
VL 791
IS 1
AR 47
DI 10.1088/0004-637X/791/1/47
PG 8
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA AM2CY
UT WOS:000339657700047
ER
PT J
AU Zhai, X
Li, H
Bellan, PM
Li, ST
AF Zhai, Xiang
Li, Hui
Bellan, Paul M.
Li, Shengtai
TI THREE-DIMENSIONAL MHD SIMULATION OF THE CALTECH PLASMA JET EXPERIMENT:
FIRST RESULTS
SO ASTROPHYSICAL JOURNAL
LA English
DT Article
DE galaxies: jets; ISM: jets and outflows; magnetohydrodynamics ( MHD);
methods: numerical
ID SCALE MAGNETIC-FIELDS; ACCRETION DISCS; YOUNG STARS; TOWER JETS; MODEL;
DISKS; COLLIMATION; ROTATION; OUTFLOWS; DRIVEN
AB Magnetic fields are believed to play an essential role in astrophysical jets with observations suggesting the presence of helical magnetic fields. Here, we present three-dimensional (3D) idealMHDsimulations of the Caltech plasma jet experiment using a magnetic tower scenario as the baseline model. Magnetic fields consist of an initially localized dipole-like poloidal component and a toroidal component that is continuously being injected into the domain. This flux injectionmimics the poloidal currents driven by the anode-cathode voltage drop in the experiment. The injected toroidal field stretches the poloidal fields to large distances, while forming a collimated jet along with several other key features. Detailed comparisons between 3D MHD simulations and experimental measurements provide a comprehensive description of the interplay among magnetic force, pressure, and flow effects. In particular, we delineate both the jet structure and the transition process that converts the injected magnetic energy to other forms. With suitably chosen parameters that are derived from experiments, the jet in the simulation agrees quantitatively with the experimental jet in terms of magnetic/kinetic/inertial energy, total poloidal current, voltage, jet radius, and jet propagation velocity. Specifically, the jet velocity in the simulation is proportional to the poloidal current divided by the square root of the jet density, in agreement with both the experiment and analytical theory. This work provides a new and quantitative method for relating experiments, numerical simulations, and astrophysical observation, and demonstrates the possibility of using terrestrial laboratory experiments to study astrophysical jets.
C1 [Zhai, Xiang; Bellan, Paul M.] CALTECH, Pasadena, CA 91125 USA.
[Li, Hui] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Li, Shengtai] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Zhai, X (reprint author), CALTECH, Pasadena, CA 91125 USA.
EM xzhai@caltech.edu; hli@lanl.gov; pbellan@caltech.edu; sli@lanl.gov
OI Zhai, Xiang/0000-0001-6155-091X; Li, Shengtai/0000-0002-4142-3080
FU NSF/DOE; LANL/LDRD; Institutional Computing Programs at LANL; DOE/Office
of Fusion Energy Science through CMSO
FX The experimental program at Caltech is supported by the NSF/DOE
Partnership in Plasma Science. H. L. is grateful to Stirling Colgate,
Ken Fowler, and Ellen Zweibel for discussions. H. L. and S. L. are
supported by the LANL/LDRD and Institutional Computing Programs at LANL
and by DOE/Office of Fusion Energy Science through CMSO.
NR 49
TC 6
Z9 6
U1 1
U2 14
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0004-637X
EI 1538-4357
J9 ASTROPHYS J
JI Astrophys. J.
PD AUG 10
PY 2014
VL 791
IS 1
AR 40
DI 10.1088/0004-637X/791/1/40
PG 22
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA AM2CY
UT WOS:000339657700040
ER
PT J
AU Moresco, P
Harris, TE
Jodoin, V
AF Moresco, P.
Harris, T. E.
Jodoin, V.
TI Vorticity generation by the instantaneous release of energy near a
reflective boundary
SO PHYSICAL REVIEW E
LA English
DT Article
ID SHOCK-BUBBLE INTERACTION; BLAST-WAVE; HOT CHANNELS; GAS; PROPAGATION;
INTERFACE; DYNAMICS; REFRACTION; IGNITION; SPHERE
AB The instantaneous release of energy in a localized area of a gas results in the formation of a low-density region and a series of shock and expansion waves. If this process occurs near a boundary, the shock reflections can interact with the density inhomogeneity, leading to the baroclinic generation of vorticity and the subsequent organization of the flow into several structures, including a vortex ring. By means of numerical simulations we illustrate the qualitative changes that occur in the pressure wave patterns and vorticity distribution as the distance from the area of energy release to the boundary is varied. Those changes are shown to be related to the combined effect of the shock waves that, respectively, initially move away and towards the center of the low-density region. In particular, we describe how for small enough offset distances the shocks internal to the inhomogeneity can make a substantial contribution to the vorticity field, influencing the circulation and characteristics of the resulting flow structures.
C1 [Moresco, P.; Harris, T. E.] AWE, Reading RG7 4PR, Berks, England.
[Jodoin, V.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Moresco, P (reprint author), AWE, Reading RG7 4PR, Berks, England.
FU US Department of Energy National Nuclear Security Administration's
Office of Technical Nuclear Forensics; US Department of Energy National
Nuclear Security Administration's Office of Defense Nuclear
Nonproliferation Research and Development
FX Partial support from the US Department of Energy National Nuclear
Security Administration's Offices of Technical Nuclear Forensics and
Defense Nuclear Nonproliferation Research and Development is gratefully
acknowledged.
NR 39
TC 0
Z9 0
U1 0
U2 2
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1539-3755
EI 1550-2376
J9 PHYS REV E
JI Phys. Rev. E
PD AUG 8
PY 2014
VL 90
IS 2
AR 023002
DI 10.1103/PhysRevE.90.023002
PG 12
WC Physics, Fluids & Plasmas; Physics, Mathematical
SC Physics
GA CB0GK
UT WOS:000349303700004
PM 25215815
ER
PT J
AU Barton, PT
Kemei, MC
Gaultois, MW
Moffitt, SL
Darago, LE
Seshadri, R
Suchomel, MR
Melot, BC
AF Barton, Phillip T.
Kemei, Moureen C.
Gaultois, Michael W.
Moffitt, Stephanie L.
Darago, Lucy E.
Seshadri, Ram
Suchomel, Matthew R.
Melot, Brent C.
TI Structural distortion below the Neel temperature in spinel GeCo2O4
SO PHYSICAL REVIEW B
LA English
DT Article
ID IRON-GERMANIUM SYSTEM; MAGNETIC-PROPERTIES; CRYSTAL-STRUCTURE; X-RAY;
TRANSITION; OXIDES; GENI2O4; PHASE
AB A structural phase transition from cubic Fd (3) over barm to tetragonal I4(1)/amd symmetry with c/a > 1 is observed at T-S = 16 K in spinel GeCo2O4 below the Neel temperature T-N = 21 K. Structural and magnetic ordering appear to be decoupled with the structural distortion occurring at 16 K while magnetic order occurs at 21 K as determined by magnetic susceptibility and heat capacity measurements. An elongation of CoO6 octahedra is observed in the tetragonal phase of GeCo2O4. We present the complete crystallographic description of GeCo2O4 in the tetragonal I4(1)/amd space group and discuss the possible origin of this distortion in the context of known structural transitions in magnetic spinels. GeCo2O4 exhibits magnetodielectric coupling below T-N. The related spinels GeFe2O4 and GeNi2O4 have also been examined for comparison. Structural transitions were not detected in either compound down to T approximate to 8 K. Magnetometry experiments reveal in GeFe2O4 a second antiferromagnetic transition, with T-N1 = 7.9 K and T-N2 = 6.2 K, that was previously unknown and that bears a similarity to the magnetism of GeNi2O4.
C1 [Barton, Phillip T.; Kemei, Moureen C.; Gaultois, Michael W.; Moffitt, Stephanie L.; Darago, Lucy E.; Seshadri, Ram] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA.
[Barton, Phillip T.; Kemei, Moureen C.; Gaultois, Michael W.; Moffitt, Stephanie L.; Darago, Lucy E.; Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA.
[Suchomel, Matthew R.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA.
[Melot, Brent C.] Univ So Calif, Dept Chem, Los Angeles, CA 90089 USA.
RP Barton, PT (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA.
EM kemei@mrl.ucsb.edu; seshadri@mrl.ucsb.edu
RI Seshadri, Ram/C-4205-2013; Gaultois, Michael/D-2867-2009; Barton,
Phillip/H-3847-2011; Melot, Brent/B-6456-2008;
OI Seshadri, Ram/0000-0001-5858-4027; Gaultois,
Michael/0000-0003-2172-2507; Melot, Brent/0000-0002-7078-8206; Darago,
Lucy/0000-0001-7515-5558
FU NSF [DMR 1105301]; Schlumberger Foundation; NSERC; International
Fulbright Science & Technology Award; MRSEC of the NSF [DMR 1121053]; US
Department of Energy, Office of Science [DE-AC02-06CH11357]; US
Department of Energy, Office of Basic Energy Sciences
[DE-AC02-06CH11357]
FX We thank Gavin Lawes for preliminary measurements on
GeCo2O4 and John Mitchell for helpful discussions.
We thank Christina Birkel for SPS. This project was supported by the NSF
through Grant No. DMR 1105301. P.T.B. was supported by the NSF Graduate
Research Fellowship Program. M.C.K. was supported by the Schlumberger
Foundation Faculty for the Future fellowship. M.W.G. was supported by a
NSERC Postgraduate Scholarship and an International Fulbright Science &
Technology Award. We acknowledge the use of the MRL Central Facilities,
which are supported by the MRSEC Program of the NSF under Grant No. DMR
1121053, a member of the NSF-funded Materials Research Facilities
Network (http://www.mrfn.org). Use of data from the 11-BM beamline at
the Advanced Photon Source was supported by the US Department of Energy,
Office of Science, Office of Basic Energy Sciences, under Contract No.
DE-AC02-06CH11357. Data were also collected on the ID31 beamline at the
European Synchrotron Radiation Facility (ESRF), Grenoble, France. We
thank Andy Fitch and Caroline Curfs for providing assistance in using
beamline ID31.
NR 46
TC 7
Z9 7
U1 7
U2 41
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 8
PY 2014
VL 90
IS 6
AR 064105
DI 10.1103/PhysRevB.90.064105
PG 7
WC Physics, Condensed Matter
SC Physics
GA AU6UJ
UT WOS:000345739300001
ER
PT J
AU Kraft, B
Tegetmeyer, HE
Sharma, R
Klotz, MG
Ferdelman, TG
Hettich, RL
Geelhoed, JS
Strous, M
AF Kraft, Beate
Tegetmeyer, Halina E.
Sharma, Ritin
Klotz, Martin G.
Ferdelman, Timothy G.
Hettich, Robert L.
Geelhoed, Jeanine S.
Strous, Marc
TI The environmental controls that govern the end product of bacterial
nitrate respiration
SO SCIENCE
LA English
DT Article
ID REDUCTION; SEDIMENTS; DENITRIFICATION; AMMONIFICATION; ANAMMOX
AB In the biogeochemical nitrogen cycle, microbial respiration processes compete for nitrate as an electron acceptor. Denitrification converts nitrate into nitrogenous gas and thus removes fixed nitrogen from the biosphere, whereas ammonification converts nitrate into ammonium, which is directly reusable by primary producers. We combined multiple parallel long-term incubations of marine microbial nitrate-respiring communities with isotope labeling and metagenomics to unravel how specific environmental conditions select for either process. Microbial generation time, supply of nitrite relative to nitrate, and the carbon/nitrogen ratio were identified as key environmental controls that determine whether nitrite will be reduced to nitrogenous gas or ammonium. Our results define the microbial ecophysiology of a biogeochemical feedback loop that is key to global change, eutrophication, and wastewater treatment.
C1 [Kraft, Beate; Tegetmeyer, Halina E.; Ferdelman, Timothy G.; Geelhoed, Jeanine S.; Strous, Marc] Max Planck Inst Marine Mikrobiol, D-28359 Bremen, Germany.
[Tegetmeyer, Halina E.; Strous, Marc] Univ Bielefeld, Ctr Biotechnol, Inst Genome Res & Syst Biol, D-33615 Bielefeld, Germany.
[Sharma, Ritin; Hettich, Robert L.] Univ Tennessee, UT ORNL Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA.
[Sharma, Ritin; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA.
[Klotz, Martin G.] Univ N Carolina, Dept Biol Sci, Charlotte, NC 28223 USA.
[Klotz, Martin G.] Xiamen Univ, State Key Lab Marine Environm Sci, Xiamen 361005, Peoples R China.
[Geelhoed, Jeanine S.] NIOZ Royal Netherlands Inst Sea Res, NL-4401 NT Yerseke, Netherlands.
[Strous, Marc] Univ Calgary, Dept Geosci, Calgary, AB T2N 1N4, Canada.
RP Strous, M (reprint author), Max Planck Inst Marine Mikrobiol, D-28359 Bremen, Germany.
EM mstrous@ucalgary.ca
RI Klotz, Martin/D-2091-2009; Hettich, Robert/N-1458-2016; Strous,
Marc/B-4064-2017;
OI Klotz, Martin/0000-0002-1783-375X; Hettich, Robert/0000-0001-7708-786X;
Strous, Marc/0000-0001-9600-3828; Kraft, Beate/0000-0003-0310-5206
FU European Research Council (ERC) [MASEM 242635]; ERC [StG 306933];
University of North Carolina at Charlotte; NSF [EF-0541797]; State Key
Laboratory of Marine Environmental Science at Xiamen University, China;
German Federal State Nordrhein-Westfalen; Max Planck Society
FX Supported by European Research Council (ERC) starting grant MASEM 242635
(M.S.); ERC grant StG 306933 (J.S.G.); research incentive funds from the
University of North Carolina at Charlotte, NSF grant EF-0541797, and a
distinguished fellowship at the State Key Laboratory of Marine
Environmental Science at Xiamen University, China (M.G.K.); the German
Federal State Nordrhein-Westfalen; and the Max Planck Society. We thank
I. Kattelmann and R. Vahrenhorst for their support in metagenomic
sequencing and analysis, and T. Hargesheimer for CARD-FISH analysis. Raw
sequencing data are publicly available under accession numbers
SAMN02566827-30, SAMN02592751, SAMN02584197-8
(http://trace.ncbi.nlm.nih.gov/Traces/sra), JDSF00000000, JDSG00000000,
and JDSH00000000 (www.ncbi.nlm.nih.gov/bioproject/231836).
NR 17
TC 49
Z9 51
U1 26
U2 270
PU AMER ASSOC ADVANCEMENT SCIENCE
PI WASHINGTON
PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA
SN 0036-8075
EI 1095-9203
J9 SCIENCE
JI Science
PD AUG 8
PY 2014
VL 345
IS 6197
BP 676
EP 679
DI 10.1126/science.1254070
PG 5
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM6GW
UT WOS:000339962800040
PM 25104387
ER
PT J
AU Kulshreshtha, PK
Maruyama, K
Kiani, S
Blackwell, J
Olynick, DL
Ashby, PD
AF Kulshreshtha, Prashant K.
Maruyama, Ken
Kiani, Sara
Blackwell, James
Olynick, Deirdre L.
Ashby, Paul D.
TI Harnessing entropic and enthalpic contributions to create a negative
tone chemically amplified molecular resist for high-resolution
lithography
SO NANOTECHNOLOGY
LA English
DT Article
DE EUV; cross linker; chemically amplified resist; high resolution; modulus
ID EXTREME-ULTRAVIOLET LITHOGRAPHY; NANOMETER LITHOGRAPHY; PATTERN
COLLAPSE; CYCLIC OLIGOMER; NORIA; POLYMERIZATION; DERIVATIVES; MECHANISM
AB Here we present a new resist design concept. By adding dilute cross-linkers to a chemically amplified molecular resist, we synergize entropic and enthalpic contributions to dissolution by harnessing both changes to molecular weight and changes in intermolecular bonding to create a system that outperforms resists that emphasize one contribution over the other. We study patterning performance, resist modulus, solubility kinetics and material redistribution as a function of cross-linker concentration. Cross-linking varies from dilute oligomerization to creating a highly networked system. The addition of small amounts of cross-linker improves resist performance by reducing material diffusion and redistribution during development and stiffening the features to avoid pattern collapse. The new dilute cross-linking system achieves the highest resolution of a sensitive molecular glass resist at 20 nm half-pitch and line-edge roughness (LER) of 4.3 nm and can inform new resist design towards patterned feature control at the molecular level.
C1 [Kulshreshtha, Prashant K.; Kiani, Sara; Olynick, Deirdre L.; Ashby, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Maruyama, Ken] JSR Micro INC, Sunnyvale, CA 94089 USA.
[Kiani, Sara] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Elect Microscopy, Berkeley, CA 94720 USA.
[Blackwell, James] Intel Corp, Components Res, Hillsboro, OR 97124 USA.
RP Kulshreshtha, PK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM dlolynick@lbl.gov; pdashby@lbl.gov
RI Foundry, Molecular/G-9968-2014
FU Intel Corporation; JSR Micro; US Department of Energy
[DE-AC02-05CH11231]
FX The authors are greatly indebted to Prof. Tadatomi Nishikubo, Kanagawa
University (Japan) for discussion about Noria and Dr Bill Hinsberg,
Columbia Hill Technical Consulting (USA) for helpful discussions and
suggestions related to this work and manuscript. We would like to thank
Miquel Salmeron for the use of his Bruker Icon AFM. We would also like
to thank Polina Babina, Pradeep Parera, Scott Dhuey, Erin Wood, Ed Wong
(Molecular Foundry), Weilun Chao (CXRO), Sergey Babin (aBeam Technology)
and EUV Beamline staff (Advanced Light Source) for their help and
discussions. This work was supported by the Intel Corporation (PK, PA,
DO and JB), JSR Micro (KM) and US Department of Energy through
experiments performed at the Molecular Foundry and Advanced Light Source
under Contract No. DE-AC02-05CH11231.
NR 43
TC 4
Z9 4
U1 2
U2 17
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0957-4484
EI 1361-6528
J9 NANOTECHNOLOGY
JI Nanotechnology
PD AUG 8
PY 2014
VL 25
IS 31
AR 315301
DI 10.1088/0957-4484/25/31/315301
PG 9
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA AL8KN
UT WOS:000339387500004
PM 25026410
ER
PT J
AU Piceno, YM
Reid, FC
Tom, LM
Conrad, ME
Bill, M
Hubbard, CG
Fouke, BW
Graff, CJ
Han, JB
Stringfellow, WT
Hanlon, JS
Hu, P
Hazen, TC
Andersen, GL
AF Piceno, Yvette M.
Reid, Francine C.
Tom, Lauren M.
Conrad, Mark E.
Bill, Markus
Hubbard, Christopher G.
Fouke, Bruce W.
Graff, Craig J.
Han, Jiabin
Stringfellow, William T.
Hanlon, Jeremy S.
Hu, Ping
Hazen, Terry C.
Andersen, Gary L.
TI Temperature and injection water source influence microbial community
structure in four Alaskan North Slope hydrocarbon reservoirs
SO FRONTIERS IN MICROBIOLOGY
LA English
DT Article
DE petroleum; reservoir; microbiology; phylochip; stable isotopes
ID SUBSURFACE OIL-RESERVOIRS; CRUDE-OIL; PETROLEUM RESERVOIRS; DEEP
SUBSURFACE; CLONE LIBRARY; SINGLE-CELL; BIODEGRADATION; SULFATE; FIELD;
SEA
AB A fundamental knowledge of microbial community structure in petroleum reservoirs can improve predictive modeling of these environments. We used hydrocarbon profiles, stable isotopes, and high-density DNA microarray analysis to characterize microbial communities in produced water from four Alaskan North Slope hydrocarbon reservoirs. Produced fluids from Schrader Bluff (24-27 degrees C), Kuparuk (47-70 degrees C), Sag River (80 degrees C), and lvishak (80-83 degrees C) reservoirs were collected, with paired soured/non-soured wells sampled from Kuparuk and lvishak. Chemical and stable isotope data suggested Schrader Bluff had substantial biogenic methane, whereas methane was mostly thermogenic in deeper reservoirs. Acetoclastic methanogens (Methanosaeta) were most prominent in Schrader Bluff samples, and the combined delta D and delta C-13 values of methane also indicated acetoclastic methanogenesis could be a primary route for biogenic methane. Conversely, hydrogenotrophic methanogens (e.g., Methanobacteriaceae) and sulfide-producing Archaeoglobus and Thermococcus were more prominent in Kuparuk samples. Sulfide-producing microbes were detected in all reservoirs, uncoupled from souring status (e.g., the non-soured Kuparuk samples had higher relative abundances of many sulfate-reducers compared to the soured sample, suggesting sulfate-reducers may be living fermentatively/syntrophically when sulfate is limited). Sulfate abundance via long-term seawater injection resulted in greater relative abundances of Desulfonauticus, Desulfomicrobium, and Desulfuromonas in the soured lvishak well compared to the non-soured well. In the non-soured lvishak sample, several taxa affiliated with Thermoanaerobacter and Halomonas predominated. Archaea were not detected in the deepest reservoirs. Functional group taxa differed in relative abundance among reservoirs, likely reflecting differing thermal and/or geochemical influences.
C1 [Piceno, Yvette M.; Reid, Francine C.; Tom, Lauren M.; Conrad, Mark E.; Bill, Markus; Hubbard, Christopher G.; Stringfellow, William T.; Hanlon, Jeremy S.; Hu, Ping; Andersen, Gary L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Piceno, Yvette M.; Reid, Francine C.; Tom, Lauren M.; Conrad, Mark E.; Bill, Markus; Hubbard, Christopher G.; Fouke, Bruce W.; Stringfellow, William T.; Hu, Ping; Andersen, Gary L.] Energy Biosci Inst, Berkeley, CA USA.
[Fouke, Bruce W.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA.
[Graff, Craig J.; Han, Jiabin] BP Explorat Co Ltd, Prod Chem, Anchorage, AK USA.
[Stringfellow, William T.; Hanlon, Jeremy S.] Univ Pacific, Ecol Engn Res Program, Stockton, CA 95211 USA.
[Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA.
RP Andersen, GL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Ecol, Ctr Environm Biotechnol, 1 Cyclotron Rd,MS 70A-3317, Berkeley, CA 94720 USA.
EM glandersen@lbl.gov
RI Tom, Lauren/E-9739-2015; Hu, Ping/G-2384-2015; Andersen,
Gary/G-2792-2015; Conrad, Mark/G-2767-2010; Hubbard,
Christopher/J-6150-2014; Stringfellow, William/O-4389-2015; Piceno,
Yvette/I-6738-2016; Bill, Markus/D-8478-2013; Hazen, Terry/C-1076-2012
OI Andersen, Gary/0000-0002-1618-9827; Hubbard,
Christopher/0000-0002-8217-8122; Stringfellow,
William/0000-0003-3189-5604; Piceno, Yvette/0000-0002-7915-4699; Bill,
Markus/0000-0001-7002-2174; Hazen, Terry/0000-0002-2536-9993
FU University of California at Berkeley, Energy Biosciences Institute under
its U.S. Department of Energy [DE-AC02-05CH11231]
FX We thank Sharon Borglin for the suggestion of adding salt to the
emulsified produced fluid sample to break the emulsion, allowing further
processing. We thank the reviewers for constructive comments and
suggestions. This work was supported by a subcontract from the
University of California at Berkeley, Energy Biosciences Institute to
Lawrence Berkeley National Laboratory under its U.S. Department of
Energy contract DE-AC02-05CH11231.
NR 73
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PU FRONTIERS RESEARCH FOUNDATION
PI LAUSANNE
PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND
SN 1664-302X
J9 FRONT MICROBIOL
JI Front. Microbiol.
PD AUG 7
PY 2014
VL 5
AR 409
DI 10.3389/fmicb.2014.00409
PG 13
WC Microbiology
SC Microbiology
GA AO7EW
UT WOS:000341515900001
PM 25147549
ER
PT J
AU Moseley, M
Allerman, A
Crawford, M
Wierer, JJ
Smith, M
Biedermann, L
AF Moseley, Michael
Allerman, Andrew
Crawford, Mary
Wierer, Jonathan J., Jr.
Smith, Michael
Biedermann, Laura
TI Electrical current leakage and open-core threading dislocations in
AlGaN-based deep ultraviolet light-emitting diodes
SO JOURNAL OF APPLIED PHYSICS
LA English
DT Article
ID REVERSE-BIAS LEAKAGE; MOLECULAR-BEAM EPITAXY; GAN SCHOTTKY DIODES; SCREW
DISLOCATIONS; FORCE MICROSCOPY; UV DEVICES; NANOPIPES; OPERATION;
NITRIDE; DENSITY
AB Electrical current transport through leakage paths in AlGaN-based deep ultraviolet (DUV) light-emitting diodes (LEDs) and their effect on LED performance are investigated. Open-core threading dislocations, or nanopipes, are found to conduct current through nominally insulating Al0.7Ga0.3N layers and limit the performance of DUV-LEDs. A defect-sensitive phosphoric acid etch reveals these open-core threading dislocations in the form of large, micron-scale hexagonal etch pits visible with optical microscopy, while closed-core screw-, edge-, and mixed-type threading dislocations are represented by smaller and more numerous nanometer-scale pits visible by atomic-force microscopy. The electrical and optical performances of DUV-LEDs fabricated on similar Si-doped Al0.7Ga0.3N templates are found to have a strong correlation to the density of these nanopipes, despite their small fraction (<0.1% in this study) of the total density of threading dislocations. (C) 2014 AIP Publishing LLC.
C1 [Moseley, Michael; Allerman, Andrew; Crawford, Mary; Wierer, Jonathan J., Jr.; Smith, Michael; Biedermann, Laura] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Moseley, M (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM mwmosel@sandia.gov
RI Wierer, Jonathan/G-1594-2013
OI Wierer, Jonathan/0000-0001-6971-4835
FU United States Department of Energy's National Nuclear Security
Administration [DE-AC04-94AL85000]
FX Sandia National Laboratories is a multi-program laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the United States Department of Energy's
National Nuclear Security Administration under Contract No.
DE-AC04-94AL85000.
NR 52
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U1 7
U2 57
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0021-8979
EI 1089-7550
J9 J APPL PHYS
JI J. Appl. Phys.
PD AUG 7
PY 2014
VL 116
IS 5
AR 053104
DI 10.1063/1.4891830
PG 7
WC Physics, Applied
SC Physics
GA AO2TM
UT WOS:000341178900004
ER
PT J
AU Perry, WL
Duque, ALH
AF Perry, William Lee
Duque, Amanda L. Higginbotham
TI Micro to mesoscale temperature gradients in microwave heated energetic
materials
SO JOURNAL OF APPLIED PHYSICS
LA English
DT Article
ID EXPLOSIVES; IGNITION; DECOMPOSITION
AB Temperature gradients will appear in any microwave-heated heterogeneous system where there is contrast in the complex permittivity of the constituent materials. The magnitude of the gradients depends on several factors that include the permittivity, thermal conductivity, length scale, and thermal diffusivity. In general, it is challenging to measure the absolute temperature accurately in a strong microwave field; the presence of large gradients can further complicate the interpretation of temperature measurements. These issues are especially important during the microwave heating of highly exothermic chemical reaction systems, such as those containing explosives or propellants. It was therefore the intent of this work to theoretically and numerically investigate the nature of microwave-induced thermal gradients in energetic systems over a wide range of length scales, primarily for the purpose of interpreting temperature measurement. (C) 2014 AIP Publishing LLC.
C1 [Perry, William Lee; Duque, Amanda L. Higginbotham] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Perry, WL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM wperry@lanl.gov
OI Duque, Amanda/0000-0002-2023-1389; Perry, William/0000-0003-1993-122X
FU Joint DoD-DOE Munitions Program
FX We appreciate the support of the Joint DoD-DOE Munitions Program. We
also appreciate many helpful discussions, and the insight of Dr. Bryan
Henson and Dr. Laura Smilowitz of Los Alamos National Laboratory,
LA-UR-14-23709.
NR 26
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0021-8979
EI 1089-7550
J9 J APPL PHYS
JI J. Appl. Phys.
PD AUG 7
PY 2014
VL 116
IS 5
AR 054911
DI 10.1063/1.4892391
PG 9
WC Physics, Applied
SC Physics
GA AO2TM
UT WOS:000341178900089
ER
PT J
AU Tringe, JW
Glascoe, EA
McClelland, MA
Greenwood, D
Chambers, RD
Springer, HK
Levie, HW
AF Tringe, J. W.
Glascoe, E. A.
McClelland, M. A.
Greenwood, D.
Chambers, R. D.
Springer, H. K.
Levie, H. W.
TI Pre-ignition confinement and deflagration violence in LX-10 and PBX 9501
SO JOURNAL OF APPLIED PHYSICS
LA English
DT Article
ID EXPLOSIVES; MODEL; SIMULATIONS; TRANSITION
AB In thermal explosions of the nitramine octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine (HMX)-based explosives LX-10 and PBX-9501, the pre-ignition spatial and temporal heating profile defines the ignition location. The ignition location then determines the extent of inertial confinement and the violence of the resulting deflagration. In this work, we present results of experiments in which similar to 23 g cylinders of LX-10 and PBX 9501 in thin-walled aluminum confinement vessels were subjected to identical heating profiles but which presented starkly different energy release signatures. Post-explosion LX-10 containment vessels were completely fragmented, while the PBX 9501 vessels were merely ruptured. Flash x-ray radiography images show that the initiation location for the LX-10 is a few mm farther from the end caps of the vessel relative to the initiation location of PBX 9501. This difference increases deflagration confinement for LX-10 at the time of ignition and extends the pressurization time during which the deflagration front propagates in the explosive. The variation in the initiation location, in turn, is determined by the thermal boundary conditions, which differ for these two explosives because of the larger coefficient of thermal expansion and greater thermal stability of the Viton binder in LX-10 relative to the estane and bis(2,2-dinitropropyl) acetal/formal binder of the PBX 9501. The thermal profile and initiation location were modeled for LX-10 using the hydrodynamics and structures code ALE3D; results indicate temperatures in the vicinity of the ignition location in excess of 274 degrees C near the time of ignition. The conductive burn rates for these two explosives, as determined by flash x-ray radiography, are comparable in the range 0.1-0.2 mm/mu s, somewhat faster than rates observed by strand burner experiments for explosives in the temperature range 150-180 degrees C and pressures up to 100 MPa. The thinnest-wall aluminum containment vessels presented here rupture at lower pressures, in the range 10 MPa, suggesting that moderately higher temperatures and pressures are present near the deflagration front. For these explosives, however the most important property for determining deflagration violence is the degree of inertial confinement. (C) 2014 AIP Publishing LLC.
C1 [Tringe, J. W.; Glascoe, E. A.; McClelland, M. A.; Greenwood, D.; Chambers, R. D.; Springer, H. K.; Levie, H. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Tringe, JW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM tringe2@llnl.gov
FU Joint DoD-DOE Munitions Technology Development Program; U.S. Department
of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]
FX We gratefully acknowledge helpful conversations with Jack Reaugh and
Kevin Vandersall of LLNL. We also thank Clark Souers at LLNL for
performing detonation simulations in ALE3D. This research was partially
supported by the Joint DoD-DOE Munitions Technology Development Program.
This work performed under the auspices of the U.S. Department of Energy
by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344.
NR 27
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PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0021-8979
EI 1089-7550
J9 J APPL PHYS
JI J. Appl. Phys.
PD AUG 7
PY 2014
VL 116
IS 5
AR 054903
DI 10.1063/1.4891994
PG 10
WC Physics, Applied
SC Physics
GA AO2TM
UT WOS:000341178900081
ER
PT J
AU Frischknecht, AL
Halligan, DO
Parks, ML
AF Frischknecht, Amalie L.
Halligan, Deaglan O.
Parks, Michael L.
TI Electrical double layers and differential capacitance in molten salts
from density functional theory
SO JOURNAL OF CHEMICAL PHYSICS
LA English
DT Article
ID FUNDAMENTAL-MEASURE-THEORY; FLUID-SOLID EQUILIBRIUM; HARD-SPHERE MODEL;
IONIC LIQUIDS; MONTE-CARLO; STATISTICAL-MECHANICS; PRIMITIVE MODEL;
DIMER MODEL; INTERFACE; ELECTROLYTE
AB Classical density functional theory (DFT) is used to calculate the structure of the electrical double layer and the differential capacitance of model molten salts. The DFT is shown to give good qualitative agreement with Monte Carlo simulations in the molten salt regime. The DFT is then applied to three common molten salts, KCl, LiCl, and LiKCl, modeled as charged hard spheres near a planar charged surface. The DFT predicts strong layering of the ions near the surface, with the oscillatory density profiles extending to larger distances for larger electrostatic interactions resulting from either lower temperature or lower dielectric constant. Overall the differential capacitance is found to be bell-shaped, in agreement with recent theories and simulations for ionic liquids and molten salts, but contrary to the results of the classical Gouy-Chapman theory. (C) 2014 AIP Publishing LLC.
C1 [Frischknecht, Amalie L.; Parks, Michael L.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Halligan, Deaglan O.] Purdue Univ, Dept Comp Sci, W Lafayette, IN 47907 USA.
RP Frischknecht, AL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM alfrisc@sandia.gov
RI Frischknecht, Amalie/N-1020-2014
OI Frischknecht, Amalie/0000-0003-2112-2587
FU NNSA Advanced Simulation and Computation (ASC) Program; Laboratory
Directed Research and Development (LDRD) program at Sandia National
Laboratories; DOE Office of Science Advanced Scientific Computing
Research (ASCR) Program; U.S. Department of Energy [DE-AC04-94AL85000]
FX We thank Professor S. Lamperski and Dr. J. Klos for sharing their MC
simulation data shown in Figs. 1-5. This work was supported by the NNSA
Advanced Simulation and Computation (ASC) Program and by the Laboratory
Directed Research and Development (LDRD) program at Sandia National
Laboratories (ALF). This work was also supported by the DOE Office of
Science Advanced Scientific Computing Research (ASCR) Program (D.O.H.
and M. L. P.). Sandia National Laboratories is a multiprogram laboratory
managed and operated by Sandia Corporation, a Lockheed-Martin Company,
for the U.S. Department of Energy under Contract No. DE-AC04-94AL85000.
NR 41
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0021-9606
EI 1089-7690
J9 J CHEM PHYS
JI J. Chem. Phys.
PD AUG 7
PY 2014
VL 141
IS 5
AR 054708
DI 10.1063/1.4891368
PG 11
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AN6OC
UT WOS:000340713100044
PM 25106601
ER
PT J
AU Wagner, AF
Dawes, R
Continetti, RE
Guo, H
AF Wagner, Albert F.
Dawes, Richard
Continetti, Robert E.
Guo, Hua
TI Theoretical/experimental comparison of deep tunneling decay of
quasi-bound H(D)OCO to H(D) + CO2
SO JOURNAL OF CHEMICAL PHYSICS
LA English
DT Article
ID POTENTIAL-ENERGY SURFACE; INFRARED-ABSORPTION SPECTRUM; HO PLUS CO;
TRANS-HOCO; QUANTUM DYNAMICS; STATE; CHEMISTRY; DISSOCIATION;
SPECTROSCOPY; CONSTANTS
AB The measured H(D)OCO survival fractions of the photoelectron-photofragment coincidence experiments by the Continetti group are qualitatively reproduced by tunneling calculations to H(D) + CO2 on several recent ab initio potential energy surfaces for the HOCO system. The tunneling calculations involve effective one-dimensional barriers based on steepest descent paths computed on each potential energy surface. The resulting tunneling probabilities are converted into H(D) OCO survival fractions using a model developed by the Continetti group in which every oscillation of the H(D)-OCO stretch provides an opportunity to tunnel. Four different potential energy surfaces are examined with the best qualitative agreement with experiment occurring for the PIP-NN surface based on UCCSD(T)-F12a/AVTZ electronic structure calculations and also a partial surface constructed for this study based on CASPT2/AVDZ electronic structure calculations. These two surfaces differ in barrier height by 1.6 kcal/mol but when matched at the saddle point have an almost identical shape along their reaction paths. The PIP surface is a less accurate fit to a smaller ab initio data set than that used for PIP-NN and its computed survival fractions are somewhat inferior to PIP-NN. The LTSH potential energy surface is the oldest surface examined and is qualitatively incompatible with experiment. This surface also has a small discontinuity that is easily repaired. On each surface, four different approximate tunneling methods are compared but only the small curvature tunneling method and the improved semiclassical transition state method produce useful results on all four surfaces. The results of these two methods are generally comparable and in qualitative agreement with experiment on the PIP-NN and CASPT2 surfaces. The original semiclassical transition state theory method produces qualitatively incorrect tunneling probabilities on all surfaces except the PIP. The Eckart tunneling method uses the least amount of information about the reaction path and produces too high a tunneling probability on PIP-NN surface, leading to survival fractions that peak at half their measured values. (C) 2014 AIP Publishing LLC.
C1 [Wagner, Albert F.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
[Dawes, Richard] Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA.
[Continetti, Robert E.] Univ Calif San Diego, Dept Chem & Biochem, San Diego, CA 92093 USA.
[Guo, Hua] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA.
RP Wagner, AF (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
EM wagner@anl.gov
RI Guo, Hua/J-2685-2014; Dawes, Richard/C-6344-2015;
OI Guo, Hua/0000-0001-9901-053X; Continetti, Robert/0000-0002-0685-4459
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences, Division of Chemical Sciences [DE-AC02-06CH11357,
DE-SC0010616, DE-FG03-98ER14879, DE-FG02-05ER15694]
FX This material is based upon work supported by the U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences, Division of
Chemical Sciences under Contract No. DE-AC02-06CH11357 (A. F. W.) and
Award Nos. DE-SC0010616 (R. D.), DE-FG03-98ER14879 (R. E. C.), and
DE-FG02-05ER15694 (H.G.).
NR 49
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0021-9606
EI 1089-7690
J9 J CHEM PHYS
JI J. Chem. Phys.
PD AUG 7
PY 2014
VL 141
IS 5
AR 054304
DI 10.1063/1.4891675
PG 13
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AN6OC
UT WOS:000340713100027
PM 25106584
ER
PT J
AU Chatrchyan, S
Khachatryan, V
Sirunyan, AM
Tumasyan, A
Adam, W
Bergauer, T
Dragicevic, M
Ero, J
Fabjan, C
Friedl, M
Fruhwirth, R
Ghete, VM
Hartl, C
Hormann, N
Hrubec, J
Jeitler, M
Kiesenhofer, W
Knunz, V
Krammer, M
Kratschmer, I
Liko, D
Mikulec, I
Rabady, D
Rahbaran, B
Rohringer, H
Schofbeck, R
Strauss, J
Taurok, A
Treberer-Treberspurg, W
Waltenberger, W
Wulz, CE
Mossolov, V
Shumeiko, N
Gonzalez, JS
Alderweireldt, S
Bansal, M
Bansal, S
Cornelis, T
De Wolf, EA
Janssen, X
Knutsson, A
Luyckx, S
Ochesanu, S
Roland, B
Rougny, R
Van Haevermaet, H
Van Mechelen, P
Van Remortel, N
Van Spilbeeck, A
Blekman, F
Blyweert, S
D'Hondt, J
Heracleous, N
Kalogeropoulos, A
Keaveney, J
Kim, TJ
Lowette, S
Maes, M
Olbrechts, A
Strom, D
Tavernier, S
Van Doninck, W
Van Mulders, P
Van Onsem, GP
Villella, I
Caillol, C
Clerbaux, B
De Lentdecker, G
Favart, L
Gay, APR
Leonard, A
Marage, PE
Mohammadi, A
Pernie, L
Reis, T
Seva, T
Thomas, L
Vander Velde, C
Vanlaer, P
Wang, J
Adler, V
Beernaert, K
Benucci, L
Cimmino, A
Costantini, S
Crucy, S
Dildick, S
Garcia, G
Klein, B
Lellouch, J
Mccartin, J
Rios, AAO
Ryckbosch, D
Diblen, SS
Sigamani, M
Strobbe, N
Thyssen, F
Tytgat, M
Walsh, S
Yazgan, E
Zaganidis, N
Basegmez, S
Beluffi, C
Bruno, G
Castello, R
Caudron, A
Ceard, L
Da Silveira, GG
Delaere, C
du Pree, T
Favart, D
Forthomme, L
Giammanco, A
Hollar, J
Jez, P
Komm, M
Lemaitre, V
Liao, J
Militaru, O
Nuttens, C
Pagano, D
Pin, A
Piotrzkowski, K
Popov, A
Quertenmont, L
Selvaggi, M
Marono, MV
Garcia, JMV
Beliy, N
Caebergs, T
Daubie, E
Hammad, GH
Alves, GA
Martins, MC
Martins, T
Pol, ME
Souza, MHG
Alda, WL
Carvalho, W
Chinellato, J
Custodio, A
Da Costa, EM
Damiao, DD
Martins, CD
De Souza, SF
Malbouisson, H
Malek, M
Figueiredo, DM
Mundim, L
Nogima, H
Da Silva, WLP
Santaolalla, J
Santoro, A
Sznajder, A
Manganote, EJT
Pereira, AV
Dias, FA
Tomei, TRFP
Novaes, SF
Padula, SS
Bernardes, CA
Gregores, EM
Mercadante, PG
Genchev, V
Iaydjiev, P
Marinov, A
Piperov, S
Rodozov, M
Sultanov, G
Vutova, M
Dimitrov, A
Glushkov, I
Hadjiiska, R
Kozhuharov, V
Litov, L
Pavlov, B
Petkov, P
Bian, JG
Chen, GM
Chen, HS
Chen, M
Du, R
Jiang, CH
Liang, D
Liang, S
Meng, X
Plestina, R
Tao, J
Wang, X
Wang, Z
Asawatangtrakuldee, C
Ban, Y
Guo, Y
Li, Q
Li, W
Liu, S
Mao, Y
Qian, SJ
Wang, D
Zhang, L
Zou, W
Avila, C
Sierra, LFC
Florez, C
Gomez, JP
Moreno, BG
Sanabria, JC
Godinovic, N
Lelas, D
Polic, D
Puljak, I
Antunovic, Z
Kovac, M
Brigljevic, V
Kadija, K
Luetic, J
Mekterovic, D
Morovic, S
Tikvica, L
Attikis, A
Mavromanolakis, G
Mousa, J
Nicolaou, C
Ptochos, F
Razis, PA
Finger, M
Finger, M
Assran, Y
Elgammal, S
Kamel, AE
Mahmoud, MA
Mahrous, A
Radi, A
Kadastik, M
Muntel, M
Murumaa, M
Raidal, M
Tiko, A
Eerola, P
Fedi, G
Voutilainen, M
Harkonen, J
Karimaki, V
Kinnunen, R
Kortelainen, MJ
Lampen, T
Lassila-Perini, K
Lehti, S
Linden, T
Luukka, P
Maenpaa, T
Peltola, T
Tuominen, E
Tuominiemi, J
Tuovinen, E
Wendland, L
Tuuva, T
Besancon, M
Couderc, F
Dejardin, M
Denegri, D
Fabbro, B
Faure, JL
Ferri, F
Ganjour, S
Givernaud, A
Gras, P
de Monchenault, GH
Jarry, P
Locci, E
Malcles, J
Nayak, A
Rander, J
Rosowsky, A
Titov, M
Baffioni, S
Beaudette, F
Busson, P
Charlot, C
Daci, N
Dahms, T
Dalchenko, M
Dobrzynski, L
Filipovic, N
Florent, A
de Cassagnac, RG
Mastrolorenzo, L
Mine, P
Mironov, C
Naranjo, IN
Nguyen, M
Ochando, C
Paganini, P
Sabes, D
Salerno, R
Sauvan, JB
Sirois, Y
Veelken, C
Yilmaz, Y
Zabi, A
Agram, JL
Andrea, J
Bloch, D
Brom, JM
Chabert, EC
Collard, C
Conte, E
Drouhin, F
Fontaine, JC
Gele, D
Goerlach, U
Goetzmann, C
Juillot, P
Le Bihan, AC
Van Hove, P
Gadrat, S
Beauceron, S
Beaupere, N
Boudoul, G
Brochet, S
Montoya, CAC
Chasserat, J
Chierici, R
Contardo, D
Depasse, P
El Mamouni, H
Fan, J
Fay, J
Gascon, S
Gouzevitch, M
Ille, B
Kurca, T
Lethuillier, M
Mirabito, L
Perries, S
Alvarez, JDR
Sgandurra, L
Sordini, V
Vander Donckt, M
Verdier, P
Viret, S
Xiao, H
Tsamalaidze, Z
Autermann, C
Beranek, S
Bontenackels, M
Calpas, B
Edelhoff, M
Feld, L
Hindrichs, O
Klein, K
Ostapchuk, A
Perieanu, A
Raupach, F
Sammet, J
Schael, S
Sprenger, D
Weber, H
Wittmer, B
Zhukov, V
Ata, M
Caudron, J
Dietz-Laursonn, E
Duchardt, D
Erdmann, M
Fischer, R
Guth, A
Hebbeker, T
Heidemann, C
Hoepfner, K
Klingebiel, D
Knutzen, S
Kreuzer, P
Merschmeyer, M
Meyer, A
Olschewski, M
Padeken, K
Papacz, P
Reithler, H
Schmitz, SA
Sonnenschein, L
Teyssier, D
Thuer, S
Weber, M
Cherepanov, V
Erdogan, Y
Flugge, G
Geenen, H
Geisler, M
Ahmad, WH
Hoehle, F
Kargoll, B
Kress, T
Kuessel, Y
Lingemann, J
Nowack, A
Nugent, IM
Perchalla, L
Pooth, O
Stahl, A
Asin, I
Bartosik, N
Behr, J
Behrenhoff, W
Behrens, U
Bell, AJ
Bergholz, M
Bethani, A
Borras, K
Burgmeier, A
Cakir, A
Calligaris, L
Campbell, A
Choudhury, S
Costanza, F
Pardos, CD
Dooling, S
Dorland, T
Eckerlin, G
Eckstein, D
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Borrello, L.
Carlsmith, D.
Cepeda, M.
Dasu, S.
Duric, S.
Friis, E.
Grothe, M.
Hall-Wilton, R.
Herndon, M.
Herve, A.
Klabbers, P.
Klukas, J.
Lanaro, A.
Lazaridis, C.
Levine, A.
Loveless, R.
Mohapatra, A.
Ojalvo, I.
Perry, T.
Pierro, G. A.
Polese, G.
Ross, I.
Sarangi, T.
Savin, A.
Smith, W. H.
Woods, N.
CA CMS Collaboration
TI Measurement of WZ and ZZ production in pp collisions at in final states
with b-tagged jets
SO EUROPEAN PHYSICAL JOURNAL C
LA English
DT Article
ID LHC
AB Measurements are reported of the WZ and ZZ production cross sections in proton-proton collisions at in final states where one Z boson decays to b-tagged jets. The other gauge boson, either W or Z, is detected through its leptonic decay (either , or , , or ). The results are based on data corresponding to an integrated luminosity of 18.9 fb collected with the CMS detector at the Large Hadron Collider. The measured cross sections, and , are consistent with next-to-leading order quantum chromodynamics calculations.
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[Blekman, F.; Blyweert, S.; D'Hondt, J.; Heracleous, N.; Kalogeropoulos, A.; Keaveney, J.; Kim, T. J.; Lowette, S.; Maes, M.; Olbrechts, A.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium.
[Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium.
[Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium.
[Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain La Neuve, Belgium.
[Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium.
[Alves, G. A.; Correa Martins Junior, M.; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil.
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[Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.
[Avila, C.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia.
[Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia.
[Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia.
[Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia.
[Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus.
[Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic.
[Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt.
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[Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland.
[Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland.
[Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland.
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[Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece.
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[Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary.
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[Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India.
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[Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India.
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[Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland.
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[Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy.
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[Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy.
[Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy.
[Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy.
[Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy.
[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Tropiano, A.] Univ Florence, Florence, Italy.
[Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy.
[Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy.
[Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy.
[Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy.
[Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy.
[Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy.
[Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy.
[Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy.
[Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy.
[Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy.
[Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy.
[Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy.
[Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy.
[Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy.
[Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy.
[Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy.
[Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy.
[Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy.
[Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy.
[Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy.
[Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy.
[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy.
[Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy.
[Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy.
[Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea.
[Kim, D. H.; Kim, G. N.; Kim, J. E.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea.
[Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea.
[Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea.
[Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea.
[Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea.
[Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania.
[Komaragiri, J. R.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia.
[Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico.
[Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico.
[Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico.
[Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico.
[Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand.
[Butler, P. H.; Doesburg, R.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand.
[Ahmad, A.; Ahmad, M.; Asghar, M. I.; Butt, J.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan.
[Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland.
[Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland.
[Bargassa, P.; Beiro Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal.
[Tsamalaidze, Z.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia.
[Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia.
[Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia.
[Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia.
[Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia.
[Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain.
[Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain.
[Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain.
[Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain.
[Genchev, V.; Iaydjiev, P.; Contardo, D.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Sharma, A.; Abdulsalam, A.; Mohanty, A. K.; Giordano, F.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Fiorendi, S.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Meola, S.; Galanti, M.; Galanti, M.; Palla, F.; Pelliccioni, M.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland.
[Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland.
[Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland.
[Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland.
[Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan.
[Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan.
[Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand.
[Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey.
[Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey.
[Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey.
[Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey.
[Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine.
[Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England.
[Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England.
[Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England.
[Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA.
[Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA.
[Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA.
[Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA.
[Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA.
[Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA.
[Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA.
[Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wurthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA.
[Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA.
[Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA.
[Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA.
[Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA.
[Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA.
[Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA.
[Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA.
[Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA.
[Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA.
[Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA.
[Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA.
[Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA.
[Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA.
[Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA.
[Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA.
[Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA.
[Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA.
[Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA.
[Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA.
[Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA.
[Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA.
[Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA.
[Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA.
[Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA.
[Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA.
[Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA.
[Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA.
[Parashar, N.] Purdue Univ Calumet, Hammond, LA USA.
[Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA.
[Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA.
[Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA.
[Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA.
[Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA.
[Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA.
[Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA.
[Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA.
[Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA.
[Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA.
[Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA.
[CMS Collaboration] CERN, Geneva, Switzerland.
[Jeitler, M.] Vienna Univ Technol, A-1040 Vienna, Austria.
[Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil.
[Assran, Y.] Suez Univ, Suez, Egypt.
[Elgammal, S.] British Univ Egypt, Cairo, Egypt.
[Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt.
[Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt.
[Mahrous, A.] Helwan Univ, Cairo, Egypt.
[Radi, A.] Zewail City Sci & Technol, Zewail, Egypt.
[Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France.
[Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany.
[Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary.
[Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India.
[Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka.
[Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran.
[Fahim, A.] Sharif Univ Technol, Tehran, Iran.
[Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran.
[Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy.
[Moon, C. S.] CNRS, IN2P3, Paris, France.
[Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico.
[Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia.
[Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy.
[Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy.
[Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland.
[Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey.
[Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey.
[Onengut, G.] Cag Univ, Mersin, Turkey.
[Sogut, K.] Mersin Univ, Mersin, Turkey.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia.
[Karapinar, G.] Izmir Inst Technol, Izmir, Turkey.
[Isildak, B.] Ozyegin Univ, Istanbul, Turkey.
[Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey.
[Ozkorucuklu, S.] Istanbul Univ, Fac Sci, Istanbul, Turkey.
[Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey.
[Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey.
[Brew, C.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England.
[Wasserbaech, S.] Utah Valley Univ, Orem, UT USA.
[Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey.
[Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey.
[Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar.
RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan, Armenia.
RI Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson,
Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi,
Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ,
James/P-3092-2014; vilar, rocio/P-8480-2014; Codispoti,
Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Cerrada,
Marcos/J-6934-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva,
Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Novaes,
Sergio/D-3532-2012; de la Cruz, Begona/K-7552-2014; Montanari,
Alessandro/J-2420-2012; Manganote, Edmilson/K-8251-2013; Scodellaro,
Luca/K-9091-2014; Lopez Virto, Amparo/K-9996-2014; Josa,
Isabel/K-5184-2014; Lokhtin, Igor/D-7004-2012; Gonzalez Caballero,
Isidro/E-7350-2010; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat
Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Ruiz, Alberto/E-4473-2011;
Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan,
Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Gulmez,
Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela
Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira,
Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad,
Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016;
Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Matorras,
Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae
Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin,
Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix,
Josep/G-5414-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Della
Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin,
Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Hernandez Calama,
Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya,
Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Lo Vetere,
Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin,
Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov,
Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir,
Altan/P-1024-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko,
Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal,
Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; Lazzizzera,
Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro,
Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev,
Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi,
Zoltan/A-5598-2009
OI Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023;
Ferguson, Thomas/0000-0001-5822-3731; Ragazzi,
Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ,
James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021;
Cerrada, Marcos/0000-0003-0112-1691; Dahms, Torsten/0000-0003-4274-5476;
Grandi, Claudio/0000-0001-5998-3070; Novaes, Sergio/0000-0003-0471-8549;
Montanari, Alessandro/0000-0003-2748-6373; Scodellaro,
Luca/0000-0002-4974-8330; Lopez Virto, Amparo/0000-0002-8707-5392;
Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo,
Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Ruiz,
Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301;
Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950;
Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre
David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626;
Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo
Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad,
Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie,
Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh,
Junghwan/0000-0002-1129-2083; Matorras, Francisco/0000-0003-4295-5668;
TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434;
Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao,
Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047;
Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Della Ricca,
Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226;
Dubinin, Mikhail/0000-0002-7766-7175; Hernandez Calama, Jose
Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462;
Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680;
Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli,
Tiziano/0000-0002-9746-4842; Chinellato, Jose
Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531;
Sen, Sercan/0000-0001-7325-1087; D'Alessandro,
Raffaello/0000-0001-7997-0306; Wulz,
Claudia-Elisabeth/0000-0001-9226-5812; Belyaev,
Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506;
Trocsanyi, Zoltan/0000-0002-2129-1279
FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq
(Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES
(Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS
(Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia);
ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP
(Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG
(Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India);
DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of
Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM
(Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico);
UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland);
NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom
(Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain);
CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei);
ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA
(Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR
(Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie
programme (European Union); European Research Council (European Union);
EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation;
Alexander von Humboldt Foundation; Belgian Federal Science Policy
Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans
l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap
en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports
(MEYS) of Czech Republic; Council of Science and Industrial Research,
India; Compagnia di San Paolo (Torino); HOMING PLUS programme of
Foundation for Polish Science; EU, Regional Development Fund; Thalis
programme; Aristeia programme; EU-ESF; Greek NSRF
FX We congratulate our colleagues in the CERN accelerator departments for
the excellent performance of the LHC and thank the technical and
administrative staffs at CERN and at other CMS institutes for their
contributions to the success of the CMS effort. In addition, we
gratefully acknowledge the computing centres and personnel of the
Worldwide LHC Computing Grid for delivering so effectively the computing
infrastructure essential to our analyses. Finally, we acknowledge the
enduring support for the construction and operation of the LHC and the
CMS detector provided by the following funding agencies: BMWF and FWF
(Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP
(Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS
(Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and
ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and
CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA
and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN
(Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM
(Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New
Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR
(Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and
CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei);
ThEPCenter, IPST, STAR and NSTDA Thailand); TUBITAK and TAEK (Turkey);
NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).
Individuals have received support from the Marie-Curie programme and the
European Research Council and EPLANET (European Union); the Leventis
Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt
Foundation; the Belgian Federal Science Policy Office; the Fonds pour la
Formation a la Recherche dans l'Industrie et dans l'Agriculture
(FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en
Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports
(MEYS) of Czech Republic; the Council of Science and Industrial
Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS
programme of Foundation for Polish Science, cofinanced by EU, Regional
Development Fund; and the Thalis and Aristeia programmes cofinanced by
EU-ESF and the Greek NSRF.
NR 43
TC 4
Z9 4
U1 7
U2 72
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1434-6044
EI 1434-6052
J9 EUR PHYS J C
JI Eur. Phys. J. C
PD AUG 7
PY 2014
VL 74
IS 8
AR 2973
DI 10.1140/epjc/s10052-014-2973-5
PG 22
WC Physics, Particles & Fields
SC Physics
GA AN3JV
UT WOS:000340484600001
ER
PT J
AU Kemper, TW
Larsen, RE
Gennett, T
AF Kemper, Travis W.
Larsen, Ross E.
Gennett, Thomas
TI Relationship between Molecular Structure and Electron Transfer in a
Polymeric Nitroxyl-Radical Energy Storage Material
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID RECHARGEABLE BATTERIES; FORCE-FIELD; CATHODES; SIMULATION; CHARGES;
SYSTEMS
AB In recent years, stable organic radical functional groups have been incorporated into a variety of polymeric materials for use as electrodes within energy storage devices, for example, batteries and capacitors. With the complex nature of the charge-transfer processes in a polymer matrix, the morphologies of the polymer films can have a significant impact on the redox behavior of the organic-based radical. To elucidate possible effects of packing on electron-transport mechanisms, theoretical modeling of the well-characterized cathode material poly(2,2,6,6-tetramethylpiperidinyloxy methacrylate) (PTMA) was conducted. Polymer morphologies were modeled using classical molecular dynamics simulations, and subsequently, the electronic-coupling matrix element between each radical site was calculated. Building on a previously derived treatment of diffusion in inhomogeneous materials, an expression for an effective electron diffusion length and an effective electron diffusion rate was derived in terms of an electronic-coupling-weighted radial distribution function. Two primary distances were found to contribute to the effective electron transfer length of 5.5 angstrom with a majority of the electron transfer, nearly 85%, occurring between radical sites on different polymer chains. Finally, we point out that this analysis of charge transfer using an electronic-coupling-weighted radial distribution function has application beyond the specific system addressed here and that it may prove useful more generally for simulating electron-transfer processes in disordered molecular materials.
C1 [Kemper, Travis W.; Larsen, Ross E.] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA.
[Gennett, Thomas] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA.
RP Kemper, TW (reprint author), Natl Renewable Energy Lab, Computat Sci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM Travis.Kemper@nrel.gov; Ross.Larsen@nrel.gov
RI Larsen, Ross/E-4225-2010
OI Larsen, Ross/0000-0002-2928-9835
FU U.S. Department of Energy, Office of Science, Basic Energy Sciences,
Materials Sciences and Engineering Division [DE-AC36-08GO28308];
Department of Energy's Office of Energy Efficiency and Renewable Energy
at the National Renewable Energy Laboratory
FX This work was supported by the U.S. Department of Energy, Office of
Science, Basic Energy Sciences, Materials Sciences and Engineering
Division under contract DE-AC36-08GO28308. The research was performed
using resources sponsored by the Department of Energy's Office of Energy
Efficiency and Renewable Energy, located at the National Renewable
Energy Laboratory.
NR 32
TC 16
Z9 16
U1 4
U2 39
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17213
EP 17220
DI 10.1021/jp501628z
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300005
ER
PT J
AU Davis, DJ
Lambert, TN
Vigil, JA
Rodriguez, MA
Brumbach, MT
Coker, EN
Limmer, SJ
AF Davis, Danae J.
Lambert, Timothy N.
Vigil, Julian A.
Rodriguez, Mark A.
Brumbach, Michael T.
Coker, Eric N.
Limmer, Steven J.
TI Role of Cu-Ion Doping in Cu-alpha-MnO2 Nanowire Electrocatalysts for the
Oxygen Reduction Reaction
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID NANOSTRUCTURED MANGANESE OXIDES; METAL-AIR BATTERIES; ELECTRODE
MATERIALS; HYBRID MATERIALS; ALKALINE-MEDIUM; ENERGY-STORAGE; REACTION
ORR; FUEL-CELLS; CATALYSTS; GRAPHENE
AB The role of Cu-ion doping in alpha-MnO2 electrocatalysts for the oxygen reduction reaction in alkaline electrolyte was investigated. Cu-doped alpha-MnO2 nanowires (Cu-alpha-MnO2) were prepared with varying amounts (up to similar to 3%) of Cu2+ using a hydrothermal method. The electrocatalytic data indicate that Cu-alpha-MnO2 nanowires have up to 74% higher terminal current densities, 2.5 times enhanced kinetic rate constants, and 66% lower charge transfer resistances that trend with Cu content, exceeding values attained by alpha-MnO2 alone. The observed improvement in catalytic behavior correlates with an increase in Mn3+ content at the surface of the Cu-alpha-MnO2 nanowires. The Mn3+/Mn4+ couple is the mediator for the rate-limiting redox-driven O-2/OH- exchange. O-2 adsorbs via an axial site (the e(g) orbital on the Mn3+ d(4) ion) at the surface or at edge defects of the nanowire, and the increase in covalent nature of the nanowire with Cu-ion doping leads to stabilization of O-2 adsorbates and faster rates of reduction. A smaller crystallite size (roughly half) for Cu-alpha-MnO2 leading to a higher density of (catalytic) edge defect sites was also observed. This work is applicable to other manganese oxide electrocatalysts and shows for the first time there is a correlation for manganese oxides between electrocatalytic activity for the oxygen reduction reaction (ORR) in alkaline electrolyte and an increase in Mn3+ character at the surface of the oxide.
C1 [Davis, Danae J.; Lambert, Timothy N.; Vigil, Julian A.] Sandia Natl Labs, Dept Mat Devices & Energy Technol, Albuquerque, NM 87185 USA.
[Rodriguez, Mark A.; Brumbach, Michael T.; Limmer, Steven J.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Coker, Eric N.] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87185 USA.
RP Lambert, TN (reprint author), Sandia Natl Labs, Dept Mat Devices & Energy Technol, POB 5800, Albuquerque, NM 87185 USA.
EM tnlambe@sandia.gov
FU Sandia National Laboratories [DE-AC04-94AL85000]
FX This work was supported by Sandia National Laboratories: Sandia is a
multiprogram laboratory operated by Sandia Corporation, a Lockheed
Martin Company, for the United States Department of Energy's National
Nuclear Security Administration under Contract DE-AC04-94AL85000.
NR 47
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17342
EP 17350
DI 10.1021/jp5039865
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300019
ER
PT J
AU Verdal, N
Udovic, TJ
Stavila, V
Tang, WS
Rush, JJ
Skripov, AV
AF Verdal, Nina
Udovic, Terrence J.
Stavila, Vitalie
Tang, Wan Si
Rush, John J.
Skripov, Alexander V.
TI Anion Reorientations in the Superionic Conducting Phase of Na2B12H12
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID SOLVENT-FREE SYNTHESIS; LI2B12H12; NA; DECOMPOSITION; DESORPTION;
SCATTERING; STABILITY; SYSTEM
AB Quasielastic neutron scattering (QENS) methods were used to characterize the reorientational dynamics of the dodecahydro-closo-dodecaborate (B12H122-) anions in the high-temperature, superionic conducting phase of Na2B12H12. The icosahedral anions in this disordered cubic phase were found to undergo rapid reorientational motions, on the order of 10(11) jumps s(-1) above 530 K, consistent with previous NMR measurements and neutron elastic-scattering fixed-window scans. QENS measurements as a function of the neutron momentum transfer suggest a reorientational mechanism dominated by small-angle jumps around a single axis. The results show a relatively low activation energy for reorientation of 259 meV (25 kJ mol(-1)).
C1 [Verdal, Nina; Udovic, Terrence J.; Tang, Wan Si; Rush, John J.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA.
[Verdal, Nina; Tang, Wan Si; Rush, John J.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA.
[Stavila, Vitalie] Sandia Natl Labs, Livermore, CA 94551 USA.
[Skripov, Alexander V.] Russian Acad Sci, Ural Branch, Inst Met Phys, Ekaterinburg 620990, Russia.
RP Verdal, N (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA.
RI Skripov, Alexander/K-4525-2013
OI Skripov, Alexander/0000-0002-0610-5538
FU DOE EERE [DE-EE0002978, DE-AI-01-05EE11104, DE-AC04-94AL85000]; Russian
Foundation for Basic Research [12-03-00078]; U.S. Civilian Research &
Development Foundation (CRDF Global) [RUP1-7076-EK-12]; National Science
Foundation [OISE-9531011, DMR-0944772]
FX This work was partially supported by the DOE EERE through Grant Nos.
DE-EE0002978, DE-AI-01-05EE11104, and DE-AC04-94AL85000 and by the
Russian Foundation for Basic Research under Grant No. 12-03-00078, the
U.S. Civilian Research & Development Foundation (CRDF Global) under
Award No. RUP1-7076-EK-12 and the National Science Foundation under
Cooperative Agreement No. OISE-9531011. This work utilized facilities
supported in part by the National Science Foundation under Agreement
DMR-0944772.
NR 27
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17483
EP 17489
DI 10.1021/jp506252c
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300034
ER
PT J
AU Masango, SS
Peng, LX
Marks, LD
Van Duyne, RP
Stair, PC
AF Masango, Sicelo S.
Peng, Lingxuan
Marks, Laurence D.
Van Duyne, Richard P.
Stair, Peter C.
TI Nucleation and Growth of Silver Nanoparticles by AB and ABC-Type Atomic
Layer Deposition
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID DIRECT PROPYLENE EPOXIDATION; ETHYLENE EPOXIDATION; METAL NANOPARTICLES;
DISTANCE-DEPENDENCE; SURFACE; CATALYSTS; NANOSTRUCTURES; MECHANISM;
FILMS; PARTICLES
AB In this work, we report synthesis strategies to produce Ag nanoparticles by AB-type and ABC-type atomic layer deposition (ALD) using trimethylphosphine-(hexafluoroacetylacetonato) silver(I) ((hfac)Ag(PMe3)) and formalin (AB-type) and (hfac)Ag(PMe3), trimethylaluminum, and H2O (ABC-type). In situ quartz crystal microbalance measurements reveal a Ag growth rate of 1-2 ng/cm(2)/cyde by ABC-type ALD at 110 degrees C and 2-10 ng/cm(2)/cyde for AB-type ALD at 170-200 degrees C. AB-type Ag ALD has a nucleation period before continuous linear growth that is shorter at 200 degrees C. Transmission electron microscopy reveals that AB-type Ag ALD particles have an average size of similar to 1.8 nrn after 10 cycles. ABC-type Ag ALD particles have an average size of similar to 2.2 run after 20 cycles. With increasing ALD cycles, ABC-type Ag ALD increases the metal loading while maintaining the particle size but AB-type Ag ALD results in the formation of bigger particles in addition to small particles. The ability to synthesize supported metal nanopartides with well-defined particle sizes and narrow size distributions makes ALD an attractive synthesis method compared to conventional wet chemistry techniques.
C1 [Masango, Sicelo S.; Van Duyne, Richard P.; Stair, Peter C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Masango, Sicelo S.; Van Duyne, Richard P.; Stair, Peter C.] Argonne Natl Lab, Inst Catalysis Energy Proc, Argonne, IL 60439 USA.
[Peng, Lingxuan; Marks, Laurence D.] Argonne Natl Lab, Dept Mat Sci & Engn, Argonne, IL 60439 USA.
RP Stair, PC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM pstair@northwestern.edu
RI Marks, Laurence/B-7527-2009
FU Northwestern University Institute for Catalysis in Energy Processes
(ICEP); US Department of Energy, Office of Basic Energy Science
[DE-FG02-03-ER15457]
FX The authors gratefully acknowledge financial support from the
Northwestern University Institute for Catalysis in Energy Processes
(ICEP). ICEP is funded through the US Department of Energy, Office of
Basic Energy Science (Award Number DE-FG02-03-ER15457).
NR 48
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U2 67
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17655
EP 17661
DI 10.1021/jp504067c
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300055
ER
PT J
AU Achtyl, JL
Vlassiouk, IV
Dai, S
Geiger, F
AF Achtyl, Jennifer L.
Vlassiouk, Ivan V.
Dai, Sheng
Geiger, Franz
TI Interactions of Organic Solvents at Graphene/alpha-Al2O3 and Graphene
Oxide/alpha-Al2O3 Interfaces Studied by Sum Frequency Generation
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID FUSED SILICA/AQUEOUS INTERFACES; DOWNSTREAM PLASMA TREATMENTS;
VIBRATIONAL SPECTROSCOPY; RAMAN-SPECTROSCOPY; IONIC LIQUID; EPITAXIAL
GRAPHENE; MONOLAYER GRAPHENE; ENVIRONMENTAL INTERFACES;
MOLECULAR-ORIENTATION; ATOMIC-STRUCTURE
AB The adsorption of 1-hexanol from cyclohexane-d(12) at single-layer graphene/alpha-Al2O3 interfaces was probed at mole percent values as low as 0.05 in the C H stretching region using vibrational sum frequency generation (SFG). The SFG spectra are indiscernible from those obtained in the absence of graphene, and from those obtained in the presence of graphene oxide films prepared via oxygen plasma treatment of pristine single-layer graphene. A Langmuir adsorption model yields observed free adsorption energies of -19.9(5) to -20.9(3) kJ/mol for the three interfaces. The results indicate that the molecular structure of the hexanol alkyl chain is subject to the same orientation distribution when graphene, oxidized or not, is present or absent at the alpha-Al2O3/cyclohexane-d(12) interface. Moreover, it appears that the adsorption of 1-hexanol in this binary mixture is driven by hexanol interactions with the underlying oxide support, and that a single layer of graphene does not influence the extent of this interaction, even when defects are introduced to it. Finally, our structural and quantitative thermodynamic data provide important benchmarks for theoretical calculations and atomistic simulations of liquid/graphene interfaces. We hypothesize that defects emerging in graphene during operation of any device application that relies on layered solvent/graphene/oxide interfaces have little impact on the interfacial structure or thermodynamics, at least for the binary mixture and over the range of defect densities probed in our studies.
C1 [Achtyl, Jennifer L.; Geiger, Franz] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Vlassiouk, Ivan V.] Oak Ridge Natl Lab, Measurement Sci & Syst Engn Div, Oak Ridge, TN 37931 USA.
[Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37931 USA.
[Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
RP Geiger, F (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.
EM geigerf@chem.northwestern.edu
RI Vlassiouk, Ivan/F-9587-2010; Dai, Sheng/K-8411-2015
OI Vlassiouk, Ivan/0000-0002-5494-0386; Dai, Sheng/0000-0002-8046-3931
FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an
Energy Frontier Research Center - U.S. Department of Energy, Office of
Science, and Office of Basic Energy Sciences; W. M. Keck Foundation,
Northwestern's Institute for Nanotechnology's NSF [EEC-0118025/003];
National Science Foundation; State of Illinois; Northwestern University
FX This work was supported by the Fluid Interface Reactions, Structures and
Transport (FIRST) Center, an Energy Frontier Research Center funded by
the U.S. Department of Energy, Office of Science, and Office of Basic
Energy Sciences. This work made use of the Keck-II facility (NUANCE
Center - Northwestern University), which has received support from the
W. M. Keck Foundation, Northwestern's Institute for Nanotechnology's
NSF-sponsored Nanoscale Science & Engineering Center (EEC-0118025/003),
both programs of the National Science Foundation, the State of Illinois,
and Northwestern University.
NR 110
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U2 67
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17745
EP 17755
DI 10.1021/jp5047547
PG 11
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300065
ER
PT J
AU Chen, DL
Wang, NW
Wang, FF
Xie, JW
Zhong, YJ
Zhu, WD
Johnson, JK
Krishna, R
AF Chen, De-Li
Wang, Ningwei
Wang, Fang-Fang
Xie, Jianwu
Zhong, Yijun
Zhu, Weidong
Johnson, J. Karl
Krishna, Rajamani
TI Utilizing the Gate-Opening Mechanism in ZIF-7 for Adsorption
Discrimination between N2O and CO2
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID INITIO MOLECULAR-DYNAMICS; METAL-ORGANIC FRAMEWORK; TOTAL-ENERGY
CALCULATIONS; WAVE BASIS-SET; NITROUS-OXIDE; SEPARATION; LIQUID;
SELECTIVITY; MIXTURES; CRYSTALS
AB N2O is a greenhouse gas with tremendous global warming potential, and more importantly it also causes ozone depletion; thus, the separation of N2O from industrial processes has gained significant attention. We have demonstrated that N2O can be selectively separated from CO2 using the zeolite imidazolate framework ZIF-7. The adsorption/desorption isotherms of both N2O and CO2 in ZIF-7 indicate the gate-opening mechanism of this material, and surprisingly, the threshold pressure for the gate opening with N2O is lower than that with CO2. Theoretical calculations indicate that both gas-host and gas-gas interaction energies for N2O are more favorable than those for CO2, giving rise to the difference in the threshold pressure between N2O and CO2 in ZIF-7. Breakthrough experiments for N2O/CO2 mixtures confirm that ZIF-7 is capable of separating N2O and CO2 mixtures under the optimized conditions, in reasonable agreement with simulation results, making it a promising material for industrial applications.
C1 [Chen, De-Li; Wang, Ningwei; Wang, Fang-Fang; Xie, Jianwu; Zhong, Yijun; Zhu, Weidong] Zhejiang Normal Univ, Inst Phys Chem, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China.
[Johnson, J. Karl] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA.
[Johnson, J. Karl] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
[Krishna, Rajamani] Univ Amsterdam, Vant Hoff Inst Mol Sci, NL-1098 XH Amsterdam, Netherlands.
RP Zhu, WD (reprint author), Zhejiang Normal Univ, Inst Phys Chem, Key Lab Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China.
EM weidongzhu@zjnu.cn; r.krishna@contact.uva.nl
RI Krishna, Rajamani/A-1098-2012; Chen, De-Li/H-6867-2012; Johnson,
Karl/E-9733-2013
OI Krishna, Rajamani/0000-0002-4784-8530; Johnson, Karl/0000-0002-3608-8003
FU National Natural Science Foundation of China [21036006, 21303165]
FX W.Z. and D.-L.C. gratefully acknowledge the support from the National
Natural Science Foundation of China (Grants 21036006 and 21303165).
Theoretical calculations were performed at the University of Pittsburgh
Center for Simulation and Modeling.
NR 45
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U1 9
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 17831
EP 17837
DI 10.1021/jp5056733
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300073
ER
PT J
AU Kovarik, L
Bowden, M
Genc, A
Szanyi, J
Peden, CHF
Kwak, JH
AF Kovarik, Libor
Bowden, Mark
Genc, Arda
Szanyi, Janos
Peden, Charles H. F.
Kwak, Ja Hun
TI Structure of delta-Alumina: Toward the Atomic Level Understanding of
Transition Alumina Phases
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID RIETVELD REFINEMENT SIMULATIONS; TOTAL-ENERGY CALCULATIONS; WAVE
BASIS-SET; GAMMA-ALUMINA; GAMMA-AL2O3; DFT; MODELS; SPINEL;
TRANSFORMATIONS; DIFFRACTION
AB Transition Al2O3 derived from thermal decomposition of AlOOH Boehmite have complex structures and to a large extent remain poorly understood. Here, we report a detailed atomic level analysis of beta-Al2O3 for the first time using a combination of high-angle annular dark field electron microscopy imaging, X-ray diffraction refinement, and density functional theory calculations. We show that the structure of delta-Al2O3 represents a complex structural intergrowth from two main crystallographic variants, which are identified as delta-Al2O3 and delta-Al2O3. The two main variants are fully structurally described, and in addition, we also derive their energy of formation. On the basis of comparison with other relevant transition Al2O3 phases, it is shown how energetic degeneracy leads to the structural disorder and complex intergrowths among several transition Al2O3. The results of the work have important implications for understanding thermodynamic stability and transformation processes in transition alumina.
C1 [Kovarik, Libor; Bowden, Mark] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[Szanyi, Janos; Peden, Charles H. F.; Kwak, Ja Hun] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Genc, Arda] FEI Co, Hillsboro, OR 97124 USA.
[Kwak, Ja Hun] UNIST, Sch Nanobiotechnol & Chem Engn, Ulsan 689798, South Korea.
RP Kovarik, L (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA.
EM libor.kovarik@pnnl.gov; jhkwak@unist.ac.kr
RI Kovarik, Libor/L-7139-2016
FU U.S. Department of Energy [DE-AC05-76RLO1830]; U.S. DOE, Office of Basic
Energy Sciences, Division of Chemical Sciences, Biosciences and
Geosciences; DOE's Office of Biological and Environmental Research
FX The research described in this paper is part of the Chemical Imaging
Initiative at Pacific Northwest National Laboratory (PNNL). It was
conducted under the Laboratory Directed Research and Development Program
at PNNL, a multiprogram national laboratory operated by Battelle
Memorial Institute for the U.S. Department of Energy under contract no.
DE-AC05-76RLO1830. C.H.F.P., J.S., and J.H.K. were supported by the U.S.
DOE, Office of Basic Energy Sciences, Division of Chemical Sciences,
Biosciences and Geosciences. The work was conducted in the William R.
Wiley Environmental Molecular Sciences Laboratory (EMSL), a national
scientific user facility sponsored by the DOE's Office of Biological and
Environmental Research and located at PNNL.
NR 43
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U1 2
U2 44
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 18051
EP 18058
DI 10.1021/jp500051j
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300098
ER
PT J
AU Jiang, WL
Kovarik, L
Zhu, ZH
Varga, T
Engelhard, MH
Bowden, ME
Nenoff, TM
Garino, TJ
AF Jiang, Weilin
Kovarik, Libor
Zhu, Zihua
Varga, Tamas
Engelhard, Mark H.
Bowden, Mark E.
Nenoff, Tina M.
Garino, Terry J.
TI Microstructure and Cs Behavior of Ba-Doped Aluminosilicate Pollucite
Irradiated with F+ Ions
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID HYDROTHERMAL SYNTHESIS; WASTE FORM; SRTIO3; IMMOBILIZATION;
RADIONUCLIDES; STORAGE; CESIUM; SR-90; O+
AB Radionuclide Cs-137 is one of the major fission products that dominate heat generation in spent fuels over the first 300 years. A durable waste form for Cs-137 that decays to Ba-137 is needed to minimize its environmental impact. Aluminosilicate pollucite CsAlSi2O6 is selected as a model waste form to study the decay-induced structural effects. Whereas Ba-containing precipitates are not present in charge-balanced Cs0.9Ba0.05AlSi2O6, they are found in Cs0.9Ba0.1AlSi2O6 and identified as monoclinic Ba2Si3O8. Pollucite is susceptible to electron-irradiation-induced amorphization. The threshold density of electronic energy deposition for amorphization was determined to be similar to 235 keV/nm(3). Pollucite can be readily amorphized under F+ ion irradiation at 673 K. A significant amount of Cs diffusion and release from the amorphized pollucite occurs during the irradiation. However, cesium is immobile in the crystalline structure under He+ ion irradiation at room temperature. The critical temperature for amorphization is not higher than 873 K under F+ ion irradiation. If kept at or above 873 K all the time, the pollucite structure is unlikely to be amorphized; Cs diffusion and release are improbable. A general discussion regarding pollucite as a potential waste form is provided in this report.
C1 [Jiang, Weilin; Kovarik, Libor; Zhu, Zihua; Varga, Tamas; Engelhard, Mark H.; Bowden, Mark E.] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Nenoff, Tina M.; Garino, Terry J.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Jiang, WL (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM weilin.jiang@pnnl.gov
RI Zhu, Zihua/K-7652-2012; Kovarik, Libor/L-7139-2016;
OI Engelhard, Mark/0000-0002-5543-0812; Jiang, Weilin/0000-0001-8302-8313
FU Nuclear Energy Research AMP; Development, U.S. Department of Energy;
U.S. DOE's Office of Biological and Environmental Research; U.S. DOE
[DE-AC05-76RL01830]; U.S. DOE/NE/FCRD-SWG; U.S. DOE's NNSA
[DE-AC04-94AL85000]
FX This work was supported by Nuclear Energy Research & Development, U.S.
Department of Energy. The research was performed using EMSL, a national
scientific user facility sponsored by the U.S. DOE's Office of
Biological and Environmental Research and located at Pacific Northwest
National Laboratory, a multidisciplinary national laboratory operated by
Battelle for the U.S. DOE under Contract DE-AC05-76RL01830. W.J. is
grateful to John Vienna and Joseph Ryan at PNNL for stimulating
discussions. T.M.N. and T.J.G. acknowledge support from the U.S.
DOE/NE/FCRD-SWG and thank David Rademacher and Clay Newton at SNL for
their assistance with sample preparation. Sandia National Laboratories
is a multiprogram laboratory managed and operated by Sandia Corp., a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
DOE's NNSA under Contract DE-AC04-94AL85000.
NR 30
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U1 1
U2 11
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 7
PY 2014
VL 118
IS 31
BP 18160
EP 18169
DI 10.1021/jp5045223
PG 10
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AM9SW
UT WOS:000340222300111
ER
PT J
AU Torres, D
Illas, F
Liu, P
AF Torres, Daniel
Illas, Francesc
Liu, Ping
TI Theoretical Study of Hydrogen Permeation through Mixed NiO-MgO Films
Supported on Mo(100): Role of the Oxide-Metal Interface
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID AUGMENTED-WAVE METHOD; ULTRATHIN FILMS; MOLECULAR-DYNAMICS; SURFACES;
DISSOCIATION; CATALYSTS; METHANE; WATER; NANOPARTICLES; DEFECTS
AB This work presents a periodic density functional study of the adsorption and permeation of atomic H on Ni-doped MgO oxide thin films supported on a Mo(100) surface. We find that the binding of atomic H is affected by the presence of a metallic support. The chemisorption energies increase considerably when the oxide film is supported. The H permeation through the NiO-MgO oxide was also studied. H migration through the unsupported NiO-MgO oxide is thermodynamically inhibited, while the presence of the metallic Mo makes permeation thermodynamically favored. We attribute the promoting effect to the different character of adsorbed H at the unsupported Ni-doped MgO oxide and at the oxide-Mo interface. In the former case, H forms hydroxyl groups, whereas in the latter case it appears as hydride due to the formation of strong metal-hydrogen bonds. These results illustrate the important role that the oxide metal interface could play in the mechanism for pure and mixed oxides reduction.
C1 [Torres, Daniel; Liu, Ping] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Illas, Francesc] Univ Barcelona, Dept Quim Fis, E-08028 Barcelona, Spain.
[Illas, Francesc] Univ Barcelona, Inst Quim Teor & Computac IQTCUB, E-08028 Barcelona, Spain.
RP Illas, F (reprint author), Univ Barcelona, Dept Quim Fis, E-08028 Barcelona, Spain.
EM francesc.illas@ub.edu
RI Illas, Francesc /C-8578-2011; COST, CM1104/I-8057-2015
OI Illas, Francesc /0000-0003-2104-6123;
FU Brookhaven National Laboratory (BNL) [DE-AC02-98CH10886]; US Department
of Energy, Office of Science; Spanish MINECO [FIS2008-02238,
CTQ2012-30751]; Generalitat de Catalunya [2009SGR1041, XRQTC]; ICREA
Academia award for excellence in research
FX This work was carried out at Brookhaven National Laboratory (BNL) under
Contract No. DE-AC02-98CH10886 with the US Department of Energy, Office
of Science. The calculations utilized resources at the BNL Center for
Functional Nanomaterials (CFN) and the Centre de Supercomputacio de
Catalunya (CESCA). Additional support from Spanish MINECO FIS2008-02238
and CTQ2012-30751 research grants and Generalitat de Catalunya grants
2009SGR1041 and XRQTC is accredited. F.I. acknowledges support from the
2009 ICREA Academia award for excellence in research. This work is also
a part of COST Actions CM1104.
NR 38
TC 2
Z9 2
U1 0
U2 22
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 7
PY 2014
VL 118
IS 31
BP 5756
EP 5761
DI 10.1021/jp408872x
PG 6
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AM9SY
UT WOS:000340222500004
PM 24446885
ER
PT J
AU Chellappa, RS
Dattelbaum, DM
Coe, JD
Velisavljevic, N
Stevens, LL
Liu, ZX
AF Chellappa, Raja S.
Dattelbaum, Dana M.
Coe, Joshua D.
Velisavljevic, Nenad
Stevens, Lewis L.
Liu, Zhenxian
TI Intermolecular Stabilization of 3,3 '-Diamino-4,4 '-azoxyfurazan (DAAF)
Compressed to 20 GPa
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID ENERGETIC MATERIALS; THERMAL-DECOMPOSITION; FURAZANS; DIFFRACTION; DFT
AB The room temperature stability of 3,3'-diamino-4,4'-azoxyfurazan (DAAF) has been investigated using synchrotron far-infrared, mid-infrared, Raman spectroscopy, and synchrotron X-ray diffraction (XRD) up to 20 GPa. The as-loaded DAAF samples exhibited subtle pressure-induced ordering phenomena (associated with positional disorder of the azoxy "O" atom) resulting in doubling of the a-axis, to form a superlattice similar to the low-temperature polymorph. Neither high pressure synchrotron XRD, nor high pressure infrared or Raman spectroscopies indicated the presence of structural phase transitions up to 20 GPa. Compression was accommodated in the unit cell by a reduction of the c-axis between the planar DAAF layers, distortion of the beta-angle of the monoclinic lattice, and an increase in intermolecular hydrogen bonding. Changes in the ring and -NH2 deformation modes and increased intermolecular hydrogen bonding interactions with compression suggest molecular reorganizations and electronic transitions at similar to 5 GPa and similar to 10 GPa that are accompanied by a shifting of the absorption band edge into the visible. A fourth-order Birch-Murnaghan fit to the room temperature isotherm afforded an estimate of the zero-pressure isothermal bulk modulus, K-0 = 12.4 +/- 0.6 GPa and its pressure derivative K-0' = 7.7 +/- 0.3.
C1 [Chellappa, Raja S.] Los Alamos Natl Lab, Lujan Ctr, Los Alamos, NM 87545 USA.
[Dattelbaum, Dana M.; Velisavljevic, Nenad; Stevens, Lewis L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Coe, Joshua D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Liu, Zhenxian] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA.
RP Chellappa, RS (reprint author), Los Alamos Natl Lab, Lujan Ctr, MS H805, Los Alamos, NM 87545 USA.
EM raja@lanl.gov; danadat@lanl.gov
FU Laboratory Directed Research and Development program; DOE-BES
[DE-AC02-06CH11357]; DOE-NNSA; NSF; W. M. Keck Foundation
FX Los Alamos National Laboratory is operated by LANS LLC for the
Department of Energy and NNSA. We thank Elizabeth Francois and David
Chavez of Los Alamos National Laboratory for providing the DAAF samples
for this investigation. The authors acknowledge funding from the
Laboratory Directed Research and Development program. We thank the
Carnegie-DOE Alliance Center for beam time, and Sector 16 beamline
scientists for their help with experimental measurements. HP-CAT is
supported by DOE-BES, DOE-NNSA, NSF, and the W. M. Keck Foundation. APS
is supported by DOE-BES under Contract No. DE-AC02-06CH11357.
NR 47
TC 2
Z9 3
U1 1
U2 15
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 7
PY 2014
VL 118
IS 31
BP 5969
EP 5982
DI 10.1021/jp504935g
PG 14
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AM9SY
UT WOS:000340222500027
PM 25011055
ER
PT J
AU Samet, M
Wang, XB
Kass, SR
AF Samet, Masoud
Wang, Xue-Bin
Kass, Steven R.
TI A Preorganized Hydrogen Bond Network and Its Effect on Anion Stability
SO JOURNAL OF PHYSICAL CHEMISTRY A
LA English
DT Article
ID PHOTOELECTRON-SPECTROSCOPY; DENSITY FUNCTIONALS; ELECTRON-AFFINITY;
ENZYME CATALYSIS; OXYANION HOLE; ACTIVE-SITE; BASIS-SETS; ENERGETICS;
RADICALS; THERMOCHEMISTRY
AB Rigid tricyclic locked in all axial 1,3,5-cydohexanetriol derivatives with 0-3 trifluoromethyl groups were synthesized and photoelectron spectra of their conjugate bases and chloride anion clusters are reported along with density functional computations. The resulting vertical and adiabatic detachment energies span 4.07-5.50 eV (VDE) and 3.75-5.00 (ADE) for the former ions and 5.60-6.23 eV (VDE) and 5.36-6.00 eV (ADE) for the latter species. These results provide measures of the anion stabilization due to the hydrogen bond network and inductive effects. The latter mechanism is found to be transmitted through space via hydrogen bonds, and the presence of three ring skeleton oxygen atoms and up to three trifluoromethyl groups enhance the ADEs by 1.61-2.88 eV for the conjugate bases and 1.01-1.60 eV for the chloride anion dusters. Computations indicate that the most favorable structures of the latter complexes have two hydrogen bonds to the chloride anion and one bifurcated interaction between the remote OH substituent and the two hydroxyl groups that directly bind to Cl-.
C1 [Samet, Masoud; Kass, Steven R.] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA.
[Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA.
RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA.
EM xuebin.wang@pnnl.gov; kass@umn.edu
FU National Science Foundation; Petroleum Research Fund; Division of
Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy
Sciences, U.S. Department of Energy (DOE); DOE's Office of Biological
and Environmental Research
FX Generous support from the National Science Foundation, the Petroleum
Research Fund administered by the American Chemical Society, and the
Minnesota Supercomputer Institute for Advanced Computational Research
are gratefully acknowledged. The photoelectron spectroscopy work was
supported by the Division of Chemical Sciences, Geosciences, and
Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy
(DOE), and was performed at the EMSL, a national scientific user
facility sponsored by DOE's Office of Biological and Environmental
Research and located at Pacific Northwest National Laboratory, which is
operated by Battelle for DOE.
NR 34
TC 5
Z9 5
U1 0
U2 11
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1089-5639
J9 J PHYS CHEM A
JI J. Phys. Chem. A
PD AUG 7
PY 2014
VL 118
IS 31
BP 5989
EP 5993
DI 10.1021/jp505308v
PG 5
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AM9SY
UT WOS:000340222500029
PM 25036443
ER
PT J
AU Ahmed, T
Haraldsen, JT
Zhu, JX
Balatsky, AV
AF Ahmed, Towfiq
Haraldsen, Jason T.
Zhu, Jian-Xin
Balatsky, Alexander V.
TI Next-Generation Epigenetic Detection Technique: Identifying Methylated
Cytosine Using Graphene Nanopore
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID DNA METHYLATION; ELECTRONIC TRANSPORT; TRANSLOCATION; CANCER; BASE;
NUCLEOTIDES; NUCLEOSIDES; MOLECULES
AB DNA methylation plays a pivotal role in the genetic evolution of both embryonic and adult cells. For adult somatic cells, the location and dynamics of methylation have been very precisely pinned down with the 5-cytosine markers on cytosine-phosphate-guanine (CpG) units. Unusual methylation on CpG islands is identified as one of the prime causes for silencing the tumor suppressant genes. Early detection of methylation changes can diagnose the potentially harmful oncogenic evolution of cells and provide promising guideline for cancer prevention. With this motivation, we propose a cytosine methylation detection technique. Our hypothesis is that electronic signatures of DNA acquired as a molecule translocates through a nanopore would be significantly different for methylated and nonmethylated bases. This difference in electronic fingerprints would allow for reliable real-time differentiation of methylated DNA. We calculate transport currents through a punctured graphene membrane while the cytosine and methylated cytosine translocate through the nanopore. We also calculate the transport properties for uracil and cyanocytosine for comparison. Our calculations of transmission, current, and tunneling conductance show distinct signatures in their spectrum for each molecular type. Thus, in this work, we provide a theoretical analysis that points to a viability of our hypothesis.
C1 [Ahmed, Towfiq; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
[Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA.
[Haraldsen, Jason T.] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22807 USA.
[Balatsky, Alexander V.] KTH Royal Inst Technol, Nord Inst Theoret Phys, S-10691 Stockholm, Sweden.
[Balatsky, Alexander V.] Stockholm Univ, S-10691 Stockholm, Sweden.
RP Ahmed, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM atowfiq@lanl.gov; avb@nordita.org
RI Haraldsen, Jason/B-9809-2012
OI Haraldsen, Jason/0000-0002-8641-5412
FU U.S. Department of Energy [DE-AC52-06NA25396]; U.S. DOE Office of Basic
Energy Sciences [VR 621-2012-2983, ERC 321031-DM]; Center for Integrated
Nanotechnologies
FX We are grateful to Los Alamos National Laboratory, an affirmative action
equal opportunity employer, operated by Los Alamos National Security,
LLC, for the National Nuclear Security Administration of the U.S.
Department of Energy under Contract DE-AC52-06NA25396. This work was
supported by the U.S. DOE Office of Basic Energy Sciences, by VR
621-2012-2983 and ERC 321031-DM, and, in part, by the Center for
Integrated Nanotechnologies, a U.S. DOE BES user facility.
NR 42
TC 9
Z9 9
U1 5
U2 41
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2601
EP 2607
DI 10.1021/jz501085e
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200019
PM 26277950
ER
PT J
AU Zhu, ZW
Barroo, C
Lichtenstein, L
Eren, B
Wu, CH
Mao, BH
de Bocarme, TV
Liu, Z
Kruse, N
Salmeron, M
Somorjai, GA
AF Zhu, Zhongwei
Barroo, Cedric
Lichtenstein, Leonid
Eren, Baran
Wu, Cheng Hao
Mao, Baohua
de Bocarme, Thierry Visart
Liu, Zhi
Kruse, Norbert
Salmeron, Miquel
Somorjai, Gabor A.
TI Influence of Step Geometry on the Reconstruction of Stepped Platinum
Surfaces under Coadsorption of Ethylene and CO
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID SCANNING-TUNNELING-MICROSCOPY; CARBON-MONOXIDE;
PHOTOELECTRON-SPECTROSCOPY; DEUTERIUM-EXCHANGE; STRUCTURAL-CHANGES;
OXYGEN REDUCTION; CRYSTAL-SURFACES; PT(111) SURFACE; MOLECULAR-BEAM;
WORK FUNCTION
AB We demonstrate the critical role of the specific atomic arrangement at step sites in the restructuring processes of low-coordinated surface atoms at high adsorbate coverage. By using high-pressure scanning tunneling microscopy (HP-STM) and ambient-pressure X-ray photoelectron spectroscopy (AP-XPS), we have investigated the reconstruction of Pt(332) (with (111)-oriented triangular steps) and Pt(557) surfaces (with (100)-oriented square steps) in the mixture of CO and C2H4 in the Torr pressure range at room temperature. CO creates Pt clusters at the step edges on both surfaces, although the dusters have different shapes and densities. A subsequent exposure to a similar partial pressure of C2H4 partially reverts the clusters on Pt(332). In contrast, the cluster structure is barely changed on Pt(557). These different reconstruction phenomena are attributed to the fact that the 3-fold (111)-step sites on Pt(332) allows for adsorption of ethylidyne-a strong adsorbate formed from ethylene-that does not form on the 4-fold (100)-step sites on Pt(557).
C1 [Zhu, Zhongwei; Wu, Cheng Hao; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Zhu, Zhongwei; Barroo, Cedric; Lichtenstein, Leonid; Eren, Baran; Wu, Cheng Hao; Salmeron, Miquel; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Mao, Baohua; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Barroo, Cedric; de Bocarme, Thierry Visart; Kruse, Norbert] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium.
[Liu, Zhi] ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai, Peoples R China.
[Kruse, Norbert] Washington State Univ, Dept Chem Engn & Bioengn, Pullman, WA 99163 USA.
RP Salmeron, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM mbsalmeron@lbl.gov; somorjai@berkeley.edu
RI Wu, Cheng Hao/C-9565-2014; Eren, Baran/A-9644-2013; Liu,
Zhi/B-3642-2009; Visart de Bocarme, Thierry/S-2824-2016;
OI Liu, Zhi/0000-0002-8973-6561; Visart de Bocarme,
Thierry/0000-0002-4041-7631; Barroo, Cedric/0000-0002-3085-4934
FU Office of Science, Office of Basic Energy Sciences, Materials Sciences
and Engineering Division, of the U.S. Department of Energy
[DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences,
of the U.S. Department of Energy [DE-AC02-05CH11231]; Fonds de la
Recherche Scientifique (F.R.S.-FNRS); Wallonie Bruxelles International
WBI [SUB/2011/17971]; Federation Wallonie-Bruxelles [BV12-15];
Wallonia-Brussels Federation (Action de Recherches Concertees) [AUWB
2010-2015/ULB15]; Humboldt Foundation of Germany; Early Postdoctoral
Mobility fellowship of the Swiss National Research Funds; National
Natural Science Foundation of China [11227902]
FX This work was supported by the Director, Office of Science, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division, of
the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The
Advanced Light Source is supported by the Director, Office of Science,
Office of Basic Energy Sciences, of the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231. C.B. gratefully thanks the Fonds de la
Recherche Scientifique (F.R.S.-FNRS) for the financial support (Ph.D.
grant), as well as Wallonie Bruxelles International WBI (SUB/2011/17971)
and the Federation Wallonie-Bruxelles (BV12-15) for the travel grants.
C.B. and T.V.d.B. thank the Wallonia-Brussels Federation (Action de
Recherches Concertees No. AUWB 2010-2015/ULB15). L.L. acknowledges the
support from the Humboldt Foundation of Germany. B.E. acknowledges
support from the Early Postdoctoral Mobility fellowship of the Swiss
National Research Funds. B.M. and Z.L. thank the support of National
Natural Science Foundation of China under Contract No. 11227902. We
acknowledge Prof. Jeong Young Park for his help on coating STM tips with
Au.
NR 44
TC 4
Z9 4
U1 2
U2 63
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2626
EP 2631
DI 10.1021/jz501341r
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200023
PM 26277954
ER
PT J
AU van der Poll, TS
Zhugayevych, A
Chertkov, E
Bakus, RC
Coughlin, JE
Teat, SJ
Bazan, GC
Tretiak, S
AF van der Poll, Thomas S.
Zhugayevych, Andriy
Chertkov, Eli
Bakus, Ronald C., II
Coughlin, Jessica E.
Teat, Simon J.
Bazan, Guillermo C.
Tretiak, Sergei
TI Polymorphism of Crystalline Molecular Donors for Solution-Processed
Organic Photovoltaics
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID THIN-FILM TRANSISTORS; CONJUGATED POLYMERS; SOLAR-CELLS; DEVICES;
CONFORMATIONS; TRANSPORT
AB Using ab initio calculations and classical molecular dynamics simulations coupled to complementary experimental characterization, four molecular semiconductors were investigated in vacuum, solution, and crystalline form. Independently, the molecules can be described as nearly isostructural, yet in crystalline form, two distinct crystal systems are observed with characteristic molecular geometries. The minor structural variations provide a platform to investigate the subtlety of simple substitutions, with particular focus on polymorphism and rotational isomerism. Resolved crystal structures offer an exact description of intermolecular ordering in the solid state. This enables evaluation of molecular binding energy in various crystallographic configurations to fully rationalize observed crystal packing on a basis of first-principle calculations of intermolecular interactions.
C1 [van der Poll, Thomas S.; Bakus, Ronald C., II; Coughlin, Jessica E.; Bazan, Guillermo C.] Univ Calif Santa Barbara, Ctr Polymers & Organ Solids, Dept Mat, Santa Barbara, CA 93106 USA.
[van der Poll, Thomas S.; Bakus, Ronald C., II; Coughlin, Jessica E.; Bazan, Guillermo C.] Univ Calif Santa Barbara, Ctr Polymers & Organ Solids, Dept Chem & Biochem, Santa Barbara, CA 93106 USA.
[Zhugayevych, Andriy; Chertkov, Eli; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA.
[Zhugayevych, Andriy; Chertkov, Eli; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
[Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
RP Bazan, GC (reprint author), Univ Calif Santa Barbara, Ctr Polymers & Organ Solids, Dept Mat, Santa Barbara, CA 93106 USA.
EM bazan@chem.ucsb.edu; serg@lanl.gov
RI Tretiak, Sergei/B-5556-2009; Bazan, Guillermo/B-7625-2014
OI Tretiak, Sergei/0000-0001-5547-3647;
FU Institute for Collaborative Biotechnologies through U.S. Army Research
Office [W911NF-09-0001]; U.S. Department of Energy; Laboratory Directed
Research and Development (LDRD) program at Los Alamos National
Laboratory (LANL); U.S. Department of Energy [DE-AC52-06NA25396]; Office
of Science, Office of Basic Energy Sciences, of the U.S. Department of
Energy [DE-AC02-05CH11231]
FX We acknowledge support from the Institute for Collaborative
Biotechnologies through grant W911NF-09-0001 from the U.S. Army Research
Office. This work was also partially supported the U.S. Department of
Energy and Laboratory Directed Research and Development (LDRD) program
at Los Alamos National Laboratory (LANL). LANL is operated by Los Alamos
National Security, LLC, for the National Nuclear Security Administration
of the U.S. Department of Energy under contract DE-AC52-06NA25396. The
Advanced Light Source is supported by the Director, Office of Science,
Office of Basic Energy Sciences, of the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231.
NR 39
TC 5
Z9 5
U1 3
U2 44
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2700
EP 2704
DI 10.1021/jz5012675
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200035
PM 26277966
ER
PT J
AU Zhai, DY
Wang, HH
Lau, KC
Gao, J
Redfern, PC
Kang, FY
Li, BH
Indacochea, E
Das, U
Sun, HH
Sun, HJ
Amine, K
Curtiss, LA
AF Zhai, Dengyun
Wang, Hsien-Hau
Lau, Kah Chun
Gao, Jing
Redfern, Paul C.
Kang, Feiyu
Li, Baohua
Indacochea, Ernesto
Das, Ujjal
Sun, Ho-Hyun
Sun, Ho-Jin
Amine, Khalil
Curtiss, Larry A.
TI Raman Evidence for Late Stage Disproportionation in a Li-O-2 Battery
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID LITHIUM-OXYGEN BATTERIES; LI2O2; ELECTROLYTE; MORPHOLOGY; STABILITY;
OXIDATION; GRAPHITE; KINETICS
AB Raman spectroscopy is used to characterize the composition of toroids formed in an aprotic Li-O-2 cell based on an activated carbon cathode. The trends in the Raman data as a function of discharge current density and charging cutoff voltage provide evidence that the toroids are made up of outer LiO2-like and inner Li2O2 regions, consistent with a disproportionation reaction occurring in the solid phase. The LiO2-like component is found to be associated with a new Raman peak identified in the carbon stretching region at similar to 1505 cm(-1), which appears only when the LiO2 peak at 1123 cm(-1) is present. The new peak is assigned to distortion of the graphitic ring stretching due to coupling with the LiO2-like component based on density functional calculations. These new results on the LiO2-like component from Raman spectroscopy provide evidence that a late stage disproportionation mechanism can occur during discharge and add new understanding to the complexities of possible processes occurring in Li-O-2 batteries.
C1 [Zhai, Dengyun; Redfern, Paul C.; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Wang, Hsien-Hau; Lau, Kah Chun; Das, Ujjal; Sun, Ho-Hyun; Sun, Ho-Jin; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Kang, Feiyu; Li, Baohua] Tsinghua Univ, Engn Lab Next Generat Power & Energy Storage Batt, Grad Sch Shenzhen, Shenzhen 518055, Peoples R China.
[Indacochea, Ernesto] Univ Illinois, Dept Civil & Mat Engn, Chicago, IL 60607 USA.
RP Curtiss, LA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM curtiss@anl.gov
RI Lau, Kah Chun/A-9348-2013
OI Lau, Kah Chun/0000-0002-4925-3397
FU U. S. Department of Energy, Office of Energy Efficiency and Renewable
Energy [DE-AC0206CH11357]
FX This work was supported by the U. S. Department of Energy under Contract
DE-AC0206CH11357, Office of Energy Efficiency and Renewable Energy. The
electron microscopy measurement was accomplished at the Electron
Microscopy Center for Materials Research at Argonne National Laboratory,
and part of the Raman measurements were performed at the Center for
Nanoscale Materials at Argonne National Laboratory. We acknowledge a
computer allocation on the CNM Carbon Cluster at Argonne National
Laboratory.
NR 23
TC 51
Z9 52
U1 4
U2 82
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2705
EP 2710
DI 10.1021/jz501323n
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200036
PM 26277967
ER
PT J
AU Yao, Y
Kanai, Y
Berkowitz, ML
AF Yao, Yi
Kanai, Yosuke
Berkowitz, Max L.
TI Role of Charge Transfer in Water Diffusivity in Aqueous Ionic Solutions
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID DENSITY-FUNCTIONAL THEORY; MOLECULAR-DYNAMICS SIMULATIONS; 1ST
PRINCIPLES SIMULATIONS; LIQUID WATER; ELECTRONIC-PROPERTIES;
SALT-SOLUTIONS; TEMPERATURE; ALGORITHMS; INTERFACE; CHEMISTRY
AB We performed molecular dynamics simulations on four types of systems containing ion and solvating water. Two systems contained a cation (Na+ or K+), and two other systems an anion (Cl- or I-). Classical molecular dynamics simulations were performed using three different force fields: a fixed charge force field, a polarizable force field that includes explicit polarization, and also a recently developed force field that includes polarization and charge transfer. These simulations were then compared to first-principles molecular dynamics simulations. While the first-principles simulations showed that the anions accelerated water translational diffusion, the cations slowed it down. In simulations with the classical force fields, only the force field that incorporates explicit charge transfer reproduced this ion-specific behavior. Additional simulations performed to understand the effect of charge transfer demonstrated that two competitive factors determine the behavior of water translational diffusion: the ions diminished charge accelerates water, while the net charge acquired by water either accelerates or slows down its dynamics. Our results show that charge transfer plays a crucial role in governing the water dynamics in aqueous ionic solutions.
C1 [Yao, Yi; Kanai, Yosuke; Berkowitz, Max L.] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA.
[Kanai, Yosuke] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA.
RP Kanai, Y (reprint author), Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA.
EM ykanai@unc.edu; maxb@unc.edu
RI Kanai, Yosuke/B-5554-2016
FU Petroleum Research Fund [52494-DNI6]; National Energy Research Computing
Center - Office of Science of the U.S. Department of Energy
[DE-AC02-05CH11231]; Office of Naval Research [N000141010096]
FX Y.K. and Y.Y. gratefully acknowledge support by the donors of the
Petroleum Research Fund, Grant 52494-DNI6 and National Energy Research
Computing Center, which is supported by the Office of Science of the
U.S. Department of Energy under Contract No. DE-AC02-05CH11231 for
computational resources. The work of M.L.B. and Y.Y. was also partially
supported by Grant N000141010096 from the Office of Naval Research. We
thank Prof. S. Rick (LSU) for useful discussions and for providing the
original code for our implementation of FQ-DCT model in the highly
parallel LAMMPS code. We also thank Dr. T. Ikeda (JAEA) for providing us
with the pseudopotential for iodide.
NR 64
TC 13
Z9 14
U1 4
U2 35
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2711
EP 2716
DI 10.1021/jz501238v
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200037
PM 26277968
ER
PT J
AU Tamblyn, I
Refaely-Abramson, S
Neaton, JB
Kronik, L
AF Tamblyn, Isaac
Refaely-Abramson, Sivan
Neaton, Jeffrey B.
Kronik, Leeor
TI Simultaneous Determination of Structures, Vibrations, and Frontier
Orbital Energies from a Self-Consistent Range-Separated Hybrid
Functional
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID PI-CONJUGATED OLIGOMERS; AB-INITIO CALCULATION; DENSITY FUNCTIONALS;
DERIVATIVE DISCONTINUITIES; ELECTRONIC EXCITATIONS; MOLECULAR-DYNAMICS;
RATIONAL DESIGN; EXCHANGE; GRADIENT; SPECTRA
AB A self-consistent optimally tuned range-separated hybrid density functional (scOT-RSH) approach is developed. It can simultaneously predict accurate geometries, vibrational modes, and frontier orbital energies. This is achieved by optimizing the range-separation parameter, gamma, to both satisfy the ionization energy theorem and minimize interatomic forces. We benchmark our approach against an established hybrid functional, B3LYP, using the G2 test set. scOT-RSH greatly improves the accuracy of occupied frontier orbital energies, with a mean absolute error (MAE) of only 0.2 eV relative to experimental ionization energies compared to 2.96 eV with B3LYP. Geometries do not change significantly compared to those obtained from B3LYP, with a bond length MAE of 0.012 angstrom compared to 0.008 angstrom for B3LYP, and a 6.5% MAE for zero-point energies, slightly larger than that of B3LYP (3.1%). scOT-RSH represents a new paradigm in which accurate geometries and ionization energies can be predicted simultaneously from a single functional approach.
C1 [Tamblyn, Isaac] Univ Ontario Inst Technol, Dept Phys, Oshawa, ON L1H 7K4, Canada.
[Refaely-Abramson, Sivan; Kronik, Leeor] Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel.
[Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Neaton, Jeffrey B.] Kavli Energy Nanosci Inst Berkeley, Berkeley, CA 94720 USA.
RP Tamblyn, I (reprint author), Univ Ontario Inst Technol, Dept Phys, Oshawa, ON L1H 7K4, Canada.
EM isaac.tamblyn@uoit.ca
RI Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014;
OI Neaton, Jeffrey/0000-0001-7585-6135; Tamblyn, Isaac/0000-0002-8146-6667
FU NSERC; Molecular Foundry; Israel Academy of Sciences and Humanities;
European Research Council; Israel Science Foundation; United States
Israel Binational Science Foundation; Helmsley Foundation; Wolfson
Foundation; Lise Meitner Minerva Center for Computational Chemistry; U.
S. Department of Energy, Office of Basic Energy Sciences, Division of
Materials Sciences and Engineering (Theory FWP) [DE-AC02-05CH11231];
Office of Science, Office of Basic Energy Sciences, of the US Department
of Energy
FX We thank Roi Baer (Hebrew University, Jerusalem) for illuminating
discussions. I.T. acknowledges support by NSERC and the Molecular
Foundry. S.R.A. acknowledges support by an Adams fellowship of the
Israel Academy of Sciences and Humanities. Work at the Weizmann
Institute was supported by the European Research Council, the Israel
Science Foundation, the United States Israel Binational Science
Foundation, the Helmsley Foundation, the Wolfson Foundation, and the
Lise Meitner Minerva Center for Computational Chemistry. J.B.N. was
supported by the U. S. Department of Energy, Office of Basic Energy
Sciences, Division of Materials Sciences and Engineering (Theory FWP)
under Contract No. DE-AC02-05CH11231. The work performed at the
Molecular Foundry was also supported by the Office of Science, Office of
Basic Energy Sciences, of the US Department of Energy. We thank the
National Energy Research Scientific Computing Center for computational
resources.
NR 83
TC 19
Z9 19
U1 1
U2 21
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2734
EP 2741
DI 10.1021/jz5010939
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200041
PM 26277972
ER
PT J
AU Siefermann, KR
Pemmaraju, CD
Neppl, S
Shavorskiy, A
Cordones, AA
Vura-Weis, J
Slaughter, DS
Sturm, FP
Weise, F
Bluhm, H
Strader, ML
Cho, H
Lin, MF
Bacellar, C
Khurmi, C
Guo, JH
Coslovich, G
Robinson, JS
Kaindl, RA
Schoenlein, RW
Belkacem, A
Neumark, DM
Leone, SR
Nordlund, D
Ogasawara, H
Krupin, O
Turner, JJ
Schlotter, WF
Holmes, MR
Messerschmidt, M
Minitti, MP
Gul, S
Zhang, JZ
Huse, N
Prendergast, D
Gessner, O
AF Siefermann, Katrin R.
Pemmaraju, Chaitanya D.
Neppl, Stefan
Shavorskiy, Andrey
Cordones, Amy A.
Vura-Weis, Josh
Slaughter, Daniel S.
Sturm, Felix P.
Weise, Fabian
Bluhm, Hendrik
Strader, Matthew L.
Cho, Hana
Lin, Ming-Fu
Bacellar, Camila
Khurmi, Champak
Guo, Jinghua
Coslovich, Giacomo
Robinson, Joseph S.
Kaindl, Robert A.
Schoenlein, Robert W.
Belkacem, Ali
Neumark, Daniel M.
Leone, Stephen R.
Nordlund, Dennis
Ogasawara, Hirohito
Krupin, Oleg
Turner, Joshua J.
Schlotter, William F.
Holmes, Michael R.
Messerschmidt, Marc
Minitti, Michael P.
Gul, Sheraz
Zhang, Jin Z.
Huse, Nils
Prendergast, David
Gessner, Oliver
TI Atomic-Scale Perspective of Ultrafast Charge Transfer at a
Dye-Semiconductor Interface
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID SENSITIZED SOLAR-CELLS; RAY-ABSORPTION-SPECTROSCOPY; COMPACT EFFECTIVE
POTENTIALS; ELECTRON-TRANSFER DYNAMICS; EXPONENT BASIS-SETS;
EXCITED-STATE; TIO2 FILMS; THIN-FILMS; ZNO; INJECTION
AB Understanding interfacial charge-transfer processes on the atomic level is crucial to support the rational design of energy-challenge relevant systems such as solar cells, batteries, and photocatalysts. A femtosecond time-resolved core-level photoelectron spectroscopy study is performed that probes the electronic structure of the interface between ruthenium-based N3 dye molecules and ZnO nanocrystals within the first picosecond after photoexcitation and from the unique perspective of the Ru reporter atom at the center of the dye. A transient chemical shift of the Ru 3d inner-shell photolines by (2.3 +/- 0.2) eV to higher binding energies is observed 500 fs after photoexcitation of the dye. The experimental results are interpreted with the aid of ab initio calculations using constrained density functional theory. Strong indications for the formation of an interfacial charge-transfer state are presented, providing direct insight into a transient electronic configuration that may limit the efficiency of photoinduced free charge-carrier generation.
C1 [Siefermann, Katrin R.; Neppl, Stefan; Slaughter, Daniel S.; Sturm, Felix P.; Weise, Fabian; Lin, Ming-Fu; Bacellar, Camila; Khurmi, Champak; Schoenlein, Robert W.; Belkacem, Ali; Neumark, Daniel M.; Leone, Stephen R.; Gessner, Oliver] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA.
[Pemmaraju, Chaitanya D.; Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Shavorskiy, Andrey; Bluhm, Hendrik; Strader, Matthew L.; Cho, Hana] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
[Cordones, Amy A.; Vura-Weis, Josh; Lin, Ming-Fu; Bacellar, Camila; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Coslovich, Giacomo; Robinson, Joseph S.; Kaindl, Robert A.; Schoenlein, Robert W.] Univ Calif Berkeley, Div Mat Sci, Berkeley, CA 94720 USA.
[Guo, Jinghua; Gul, Sheraz] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Robinson, Joseph S.; Krupin, Oleg; Turner, Joshua J.; Schlotter, William F.; Holmes, Michael R.; Messerschmidt, Marc; Minitti, Michael P.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
[Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Nordlund, Dennis; Ogasawara, Hirohito] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
[Krupin, Oleg] European XFEL GmbH, D-22761 Hamburg, Germany.
[Gul, Sheraz; Zhang, Jin Z.] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA.
[Huse, Nils] Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany.
[Huse, Nils] Max Planck Inst Struct & Dynam Matter, D-22761 Hamburg, Germany.
RP Gessner, O (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA.
EM ogessner@llbl.gov
RI Messerschmidt, Marc/F-3796-2010; PEMMARAJU, DAS/O-8153-2014; Nordlund,
Dennis/A-8902-2008; Foundry, Molecular/G-9968-2014; Ogasawara,
Hirohito/D-2105-2009; Neumark, Daniel/B-9551-2009; Huse,
Nils/A-5712-2017
OI Slaughter, Daniel/0000-0002-4621-4552; Messerschmidt,
Marc/0000-0002-8641-3302; PEMMARAJU, DAS/0000-0002-9016-7044; Nordlund,
Dennis/0000-0001-9524-6908; Ogasawara, Hirohito/0000-0001-5338-1079;
Neumark, Daniel/0000-0002-3762-9473; Huse, Nils/0000-0002-3281-7600
FU U.S. Department of Energy, Office of Basic Energy Sciences, Chemical
Sciences, Geosciences and Biosciences Division [DE-AC02-05CH11231];
Department of Energy Office of Science Early Career Research Program;
Alexander von Humboldt foundation; NSSEFF program of Department of
Defense; Basic Energy Sciences Division of the U.S. DOE
[DE-FG02-ER46232]; LCLS; Stanford University through Stanford Institute
for Materials Energy Sciences (SIMES); LBNL; University of Hamburg
through BMBF priority program FSP 301; Center for Free Electron Laser
Science (CFEL)
FX This work was supported by the U.S. Department of Energy, Office of
Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences
Division, through contract no. DE-AC02-05CH11231. O.G. was supported by
the Department of Energy Office of Science Early Career Research
Program. K.R.S. was supported by the Alexander von Humboldt foundation.
S.R.L. and J.V.-W. were supported by the NSSEFF program of the
Department of Defense. Ab initio modeling by C.D.P. and D.P. was
performed as part of a user project at The Molecular Foundry, Lawrence
Berkeley National Laboratory (LBNL) and using high-performance computing
resources of The Molecular Foundry and of the National Energy Research
Scientific Computing Center (NERSC) at LBNL. J.Z.Z. is grateful for
support by the Basic Energy Sciences Division of the U.S. DOE
(DE-FG02-ER46232). Portions of this research were carried out on the SXR
Instrument at the Linac Coherent Light Source (LCLS), a division of SLAC
National Accelerator Laboratory and an Office of Science user facility
operated by Stanford University for the U.S. Department of Energy. The
SXR Instrument is funded by a consortium whose membership includes the
LCLS, Stanford University through the Stanford Institute for Materials
Energy Sciences (SIMES), LBNL, University of Hamburg through the BMBF
priority program FSP 301, and the Center for Free Electron Laser Science
(CFEL). We appreciate the support received from T. Tyliszczak, M. P.
Hertlein, P. A. Heimann, A. R. Nilsson, and M. Beye as well as the staff
at LCLS and the Advanced Light Source (ALS) at LBNL.
NR 48
TC 28
Z9 28
U1 8
U2 95
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 7
PY 2014
VL 5
IS 15
BP 2753
EP 2759
DI 10.1021/jz501264x
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM9SV
UT WOS:000340222200044
PM 26277975
ER
PT J
AU Gupta, S
Chai, J
Cheng, J
D'Mello, R
Chance, MR
Fu, D
AF Gupta, Sayan
Chai, Jin
Cheng, Jie
D'Mello, Rhijuta
Chance, Mark R.
Fu, Dax
TI Visualizing the kinetic power stroke that drives proton-coupled zinc(II)
transport
SO NATURE
LA English
DT Article
ID MASS-SPECTROMETRY; METAL-BINDING; YIIP; SPECIFICITY; SELECTIVITY;
MECHANISM; DYNAMICS; VESICLES; FAMILY; FIEF
AB The proton gradient is a principal energy source for respiration-dependent active transport, but the structural mechanisms of proton-coupled transport processes are poorly understood. YiiP is a proton-coupled zinc transporter found in the cytoplasmic membrane of Escherichia coli. Its transport site receives protons from water molecules that gain access to its hydrophobic environment and transduces the energy of an inward proton gradient to drive Zn(II) efflux(1,2). This membrane protein is a well characterized member3- 7 of the family of cation diffusion facilitators that occurs at all phylogenetic levels(8-10). Here we show, using X-ray-mediated hydroxyl radical labelling of YiiP and mass spectrometry, that Zn( II) binding triggers a highly localized, all-or-nothing change of water accessibility to the transport site and an adjacent hydrophobic gate. Milli-secondtime-resolved dynamics reveal a concerted and reciprocal pattern of accessibility changes along a trans membrane helix, suggesting a rigid-body helical re-orientation linked to Zn( II) binding that triggers the closing of the hydrophobic gate. The gated water access to the transport site enables a stationary proton gradient to facilitate the conversion of zinc-binding energy to the kinetic power stroke of a vectorial zinc transport. The kinetic details provide energetic insights intoaproton-coupled active-transport reaction.
C1 [Gupta, Sayan; Cheng, Jie; D'Mello, Rhijuta] Case Western Reserve Univ, Ctr Synchrotron Biosci, Cleveland, OH 44109 USA.
[Gupta, Sayan; D'Mello, Rhijuta; Chance, Mark R.] Case Western Reserve Univ, Ctr Prote & Bioinformat, Cleveland, OH 44109 USA.
[Chai, Jin; Fu, Dax] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.
[Cheng, Jie; Fu, Dax] Johns Hopkins Sch Med, Dept Physiol, Baltimore, MD 21205 USA.
RP Fu, D (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.
EM mrc16@case.edu; dfu3@jhmi.edu
OI chai, jin/0000-0002-4760-5811
FU National Institutes of Health [R01GM065137]; Division of Chemical
Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences
of the US Department of Energy (DOE) [DE-AC02-98CH10886]; Physical
Biosciences Program, Office of Basic Energy Sciences of the DOE;
National Institute for Biomedical Imaging and Bioengineering
[P30-EB-09998, R01-EB-09688]; DOE [DE-AC02-98CH10886]
FX We dedicate this work to the memory of Peter C. Maloney, who read and
commented on a version of the manuscript. This work was supported in
part by the National Institutes of Health under grant R01GM065137(to
D.F.), the Division of Chemical Sciences, Geosciences, and Biosciences,
Office of Basic Energy Sciences of the US Department of Energy (DOE)
under contract DE-AC02-98CH10886 (to D.F.); D.F. is primarily supported
by the Physical Biosciences Program, Office of Basic Energy Sciences of
the DOE and the National Institute for Biomedical Imaging and
Bioengineering under grants P30-EB-09998 and R01-EB-09688 (to M.R.C.).
The National Synchrotron Light Source at Brookhaven National Laboratory
is supported by the DOE under contract DE-AC02-98CH10886.
NR 27
TC 24
Z9 24
U1 0
U2 41
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 0028-0836
EI 1476-4687
J9 NATURE
JI Nature
PD AUG 7
PY 2014
VL 512
IS 7512
BP 101
EP +
DI 10.1038/nature13382
PG 11
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM5NX
UT WOS:000339908000040
PM 25043033
ER
PT J
AU Kang, ZB
Ma, YQ
Qiu, JW
Sterman, G
AF Kang, Zhong-Bo
Ma, Yan-Qing
Qiu, Jian-Wei
Sterman, George
TI Heavy quarkonium production at collider energies: Factorization and
evolution
SO PHYSICAL REVIEW D
LA English
DT Article
ID HADRONIC PRODUCTION; J-PSI; PARTON DISTRIBUTION; POWER CORRECTIONS;
SMALL VALUES; SCATTERING; GLUON; DISTRIBUTIONS; ANNIHILATION; UPSILON
AB We present a perturbative QCD factorization formalism for inclusive production of heavy quarkonia of large transverse momentum, p(T) at collider energies, including both leading power (LP) and next-to-leading power (NLP) behavior in p(T). We demonstrate that both LP and NLP contributions can be factorized in terms of perturbativcly calculable short-distance partonic coefficient functions and universal nonperturbative fragmentation functions, and derive the evolution equations that are implied by the factorization. We identify projection operators for all channels of the factorized LP and NLP infrared safe short-distance partonic hard parts, and corresponding operator definitions of fragmentation functions. For the NLP, we focus on the contributions involving the production of a heavy quark pair, a necessary condition for producing a heavy quarkonium. We evaluate the first nontrivial order of evolution kernels for all relevant fragmentation functions, and discuss the role of NLP contributions.
C1 [Kang, Zhong-Bo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Ma, Yan-Qing; Qiu, Jian-Wei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
[Qiu, Jian-Wei; Sterman, George] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA.
[Qiu, Jian-Wei; Sterman, George] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA.
RP Kang, ZB (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM zkang@lanl.gov; yqma@bnl.gov; jqiu@bnl.gov;
sterman@insti.physics.sunysb.edu
RI Kang, Zhongbo/P-3645-2014
FU U.S. Department of Energy [DE-AC52-06NA25396, DE-AC02-98CH10886];
National Science Foundation [PHY-0969739, PHY-1316617]
FX We thank Geoff Bodwin, Eric Braaten, Sean Fleming, Adam Leibovich and
Tom Mehen for helpful discussions. This work was supported in part by
the U.S. Department of Energy under Contracts No. DE-AC52-06NA25396 and
No. DE-AC02-98CH10886, and the National Science Foundation under Grants
No. PHY-0969739 and No. PHY-1316617.
NR 63
TC 24
Z9 24
U1 0
U2 1
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0010
EI 2470-0029
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 7
PY 2014
VL 90
IS 3
AR 034006
DI 10.1103/PhysRcvD.90.034006
PG 37
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA AM6SN
UT WOS:000339995200002
ER
PT J
AU Hong, T
Chamlagain, B
Lin, WZ
Chuang, HJ
Pan, MH
Zhou, ZX
Xu, YQ
AF Hong, Tu
Chamlagain, Bhim
Lin, Wenzhi
Chuang, Hsun-Jen
Pan, Minghu
Zhou, Zhixian
Xu, Ya-Qiong
TI Polarized photocurrent response in black phosphorus field-effect
transistors
SO NANOSCALE
LA English
DT Article
ID SINGLE-LAYER MOS2; CARBON NANOTUBE TRANSISTORS; GRAPHENE TRANSISTORS;
ELECTRICAL-PROPERTIES; TRANSPORT; CRYSTALS; MOBILITY; HYSTERESIS;
CONTACTS
AB We investigate electrical transport and optoelectronic properties of field effect transistors (FETs) made from few-layer black phosphorus (BP) crystals down to a few nanometers. In particular, we explore the anisotropic nature and photocurrent generation mechanisms in BP FETs through spatial-, polarization-, gate-, and bias-dependent photocurrent measurements. Our results reveal that the photocurrent signals at BP-electrode junctions are mainly attributed to the photovoltaic effect in the off-state and photothermoelectric effect in the on-state, and their anisotropic feature primarily results from the directional-dependent absorption of BP crystals.
C1 [Hong, Tu; Xu, Ya-Qiong] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA.
[Chamlagain, Bhim; Chuang, Hsun-Jen; Zhou, Zhixian] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48201 USA.
[Lin, Wenzhi; Pan, Minghu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Xu, Ya-Qiong] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA.
RP Pan, MH (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM panm@ornl.gov; zxzhou@wayne.edu; yaqiong.xu@vanderbilt.edu
RI Xu, Yaqiong/D-8649-2012;
OI Chamlagain, Bhim/0000-0002-3412-8323
FU Office of Basic Energy Sciences, U.S. Department of Energy; National
Science Foundation [ECCS-1055852, CBET-1264982, ECCS-1128297,
DMR-1308436]
FX The BP FETs were fabricated at Wayne State University. Part of this
research (STM measurements) was conducted at the Center for Nanophase
Materials Sciences (CNMS), which is sponsored at Oak Ridge National
Laboratory by the Office of Basic Energy Sciences, U.S. Department of
Energy. This work was supported by the National Science Foundation
(ECCS-1055852 and CBET-1264982 to YX; ECCS-1128297 and DMR-1308436 to
ZZ).
NR 41
TC 103
Z9 103
U1 22
U2 180
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PD AUG 7
PY 2014
VL 6
IS 15
BP 8978
EP 8983
DI 10.1039/c4nr02164a
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM4YG
UT WOS:000339861500075
PM 24967826
ER
PT J
AU Agapov, RL
Boreyko, JB
Briggs, DP
Srijanto, BR
Retterer, ST
Collier, CP
Lavrik, NV
AF Agapov, Rebecca L.
Boreyko, Jonathan B.
Briggs, Dayrl P.
Srijanto, Bernadeta R.
Retterer, Scott T.
Collier, C. Patrick
Lavrik, Nickolay V.
TI Length scale of Leidenfrost ratchet switches droplet directionality
SO NANOSCALE
LA English
DT Article
ID SURFACES; NANOSTRUCTURES; MORPHOLOGIES; TEMPERATURE; ARRAYS; FILM
AB Arrays of tilted pillars with characteristic heights spanning from hundreds of nanometers to tens of micrometers were created using wafer level processing and used as Leidenfrost ratchets to control droplet directionality. Dynamic Leidenfrost droplets on the ratchets with nanoscale features were found to move in the direction of the pillar tilt while the opposite directionality was observed on the microscale ratchets. This remarkable switch in the droplet directionality can be explained by varying contributions from the two distinct mechanisms controlling droplet motion on Leidenfrost ratchets with nanoscale and microscale features. In particular, asymmetric wettability of dynamic Leidenfrost droplets upon initial impact appears to be the dominant mechanism determining their directionality on tilted nanoscale pillar arrays. By contrast, asymmetric wetting does not provide a strong enough driving force compared to the forces induced by asymmetric vapour flow on arrays of much taller tilted microscale pillars. Furthermore, asymmetric wetting plays a role only in the dynamic Leidenfrost regime, for instance when droplets repeatedly jump after their initial impact. The point of crossover between the two mechanisms coincides with the pillar heights comparable to the values of the thinnest vapor layers still capable of cushioning Leidenfrost droplets upon their initial impact. The proposed model of the length scale dependent interplay between the two mechanisms points to the previously unexplored ability to bias movement of dynamic Leidenfrost droplets and even switch their directionality.
C1 [Agapov, Rebecca L.; Boreyko, Jonathan B.; Briggs, Dayrl P.; Srijanto, Bernadeta R.; Retterer, Scott T.; Collier, C. Patrick; Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Boreyko, Jonathan B.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res, Knoxville, TN 37996 USA.
[Srijanto, Bernadeta R.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.
RP Lavrik, NV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
EM lavriknv@ornl.gov
RI Retterer, Scott/A-5256-2011; Lavrik, Nickolay/B-5268-2011; Srijanto,
Bernadeta/D-4213-2016; Collier, Charles/C-9206-2016
OI Retterer, Scott/0000-0001-8534-1979; Lavrik,
Nickolay/0000-0002-9543-5634; Srijanto, Bernadeta/0000-0002-1188-1267;
Collier, Charles/0000-0002-8198-793X
FU Oak Ridge National Laboratory by the Division of Scientific User
Facilities, U.S. Department of Energy
FX This research was conducted at the Center for Nanophase Materials
Sciences, which is sponsored at Oak Ridge National Laboratory by the
Division of Scientific User Facilities, U.S. Department of Energy.
NR 46
TC 8
Z9 8
U1 4
U2 49
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PD AUG 7
PY 2014
VL 6
IS 15
BP 9293
EP 9299
DI 10.1039/c4nr02362e
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AM4YG
UT WOS:000339861500113
PM 24986190
ER
PT J
AU Antropov, VP
Antonov, VN
Bekenov, LV
Kutepov, A
Kotliar, G
AF Antropov, V. P.
Antonov, V. N.
Bekenov, L. V.
Kutepov, A.
Kotliar, G.
TI Magnetic anisotropic effects and electronic correlations in MnBi
ferromagnet
SO PHYSICAL REVIEW B
LA English
DT Article
ID FULL-POTENTIAL CALCULATIONS; RANDOM-PHASE-APPROXIMATION; MAGNETOOPTICAL
PROPERTIES; THIN-FILMS; AB-INITIO; MAGNETOCRYSTALLINE ANISOTROPY;
INTERMETALLIC COMPOUND; LDA+U METHOD; BAND THEORY; BI
AB The electronic structure and numerous magnetic properties of MnBi magnetic systems are investigated using local spin density approximation (LSDA) with on-cite Coulomb correlations (LSDA+U) included. We show that the inclusion of Coulomb correlations provides a much better description of equilibrium magnetic moments on Mn atoms as well as the magnetic anisotropy energy behavior with temperature and magneto-optical effects. We found that the inversion of the anisotropic pairwise exchange interaction between Bi atoms is responsible for the observed spin reorientation transition at 90 K. This interaction appears as a result of strong spin orbit coupling on Bi atoms, large magnetic moments on Mn atoms, significant p-d hybridization between Mn and Bi atoms, and it depends strongly on lattice constants (anisotropic Bi-Bi exchange striction). A better agreement with the magneto-optical Kerr measurements at higher energies is obtained. We also present the detailed investigation of the Fermi surface, the de Haas-van Alphen effect, and the x-ray magnetic circular dichroism in MnBi.
C1 [Antropov, V. P.; Antonov, V. N.; Kutepov, A.] US DOE, Ames Lab, Ames, IA 50011 USA.
[Antonov, V. N.; Bekenov, L. V.] Inst Met Phys, UA-03142 Kiev, Ukraine.
[Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA.
RP Antropov, VP (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.
FU U.S. Department of Energy (DOE) ARPA-E [REACT 0472-1526]; Critical
Materials Institute; Energy Innovation Hub - US DOE; Office of Basic
Energy Science, Division of Materials Science and Engineering; Iowa
State University [DE-AC02-07CH11358]
FX This research is supported in part by the U.S. Department of Energy
(DOE) ARPA-E (REACT 0472-1526); the Critical Materials Institute, an
Energy Innovation Hub funded by the US DOE and by the Office of Basic
Energy Science, Division of Materials Science and Engineering. Ames
Laboratory is operated for the US DOE by Iowa State University under
Contract No. DE-AC02-07CH11358. V. P. A. is thankful to S. V. Antropov
for useful comments. V.N.A. gratefully acknowledges the hospitality at
Ames Laboratory during his stay there.
NR 97
TC 27
Z9 27
U1 10
U2 77
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 7
PY 2014
VL 90
IS 5
AR 054404
DI 10.1103/PhysRevB.90.054404
PG 18
WC Physics, Condensed Matter
SC Physics
GA AM6RH
UT WOS:000339991800003
ER
PT J
AU Laguta, VV
Buryi, M
Rosa, J
Savchenko, D
Hybler, J
Nikl, M
Zazubovich, S
Karner, T
Stanek, CR
McClellan, KJ
AF Laguta, V. V.
Buryi, M.
Rosa, J.
Savchenko, D.
Hybler, J.
Nikl, M.
Zazubovich, S.
Kaerner, T.
Stanek, C. R.
McClellan, K. J.
TI Electron and hole traps in yttrium orthosilicate single crystals: The
critical role of Si-unbound oxygen
SO PHYSICAL REVIEW B
LA English
DT Article
ID COMPLEX OXIDE SCINTILLATORS; SPIN-RESONANCE; RARE-EARTH; PARAMAGNETIC
RESONANCE; HYPERFINE-STRUCTURE; ALKALI HALIDES; LSO-CE; X-RAY; CENTERS;
LASER
AB We studied the processes of hole and electron trapping in yttrium orthosilicate Y2SiO5 single crystals using continuous wave and pulse electron spin resonance methods. We show that holes created by x-ray irradiation at low temperatures (T < 80 K) are preferably self-trapped at Si-unbound oxygen ions in the form of O- centers. Under irradiation at higher temperatures (200-290 K), the holes are trapped at the Si-unbound oxygen ions in the vicinity of perturbing defects such as yttrium vacancies and impurity ions forming a variety of O- centers with thermal stability up to room and higher temperatures. We have also found that under x-ray irradiation at T < 60 K, electrons are preferably trapped in the vicinity of Si-unbound oxygen ion vacancies and partly trapped also at Mo impurity ions in the form of F+ -type and Mo5+ centers, respectively. The trapped electrons are thermally released from the F+ centers at 75-90 K, thus giving rise to a thermally stimulated luminescence peak at these temperatures. We assume that this process is realized without excitation of the electrons to the conduction band. The spectroscopic parameters (g and hyperfine tensors) of all the investigated centers have been determined as well. Electron spin resonance measurements of electron and hole traps in the related compound lutetium orthosilicate (Lu2SiO5) are discussed as well.
C1 [Laguta, V. V.; Buryi, M.; Rosa, J.; Savchenko, D.; Hybler, J.; Nikl, M.] Inst Phys AS CR, Prague 16200, Czech Republic.
[Zazubovich, S.; Kaerner, T.] Univ Tartu, Inst Phys, EE-51014 Tartu, Estonia.
[Stanek, C. R.; McClellan, K. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Laguta, VV (reprint author), Inst Phys AS CR, Cukrovarnicka 10, Prague 16200, Czech Republic.
RI Buryi, Maksym/H-1176-2014; Savchenko, Dariya/D-8476-2012; Laguta,
Valentin/G-7302-2014
OI Savchenko, Dariya/0000-0002-0005-0732;
FU Czech Science Foundation [P204/12/0805]; use of facilities of the large
infrastructure SAFMAT project [CZ.2.13/3.1.00/22132]; Estonian Ministry
of Education and Research [IUT02-26]; Estonian Science Foundation [8678]
FX The authors gratefully acknowledge the financial support of the Czech
Science Foundation (Project No. P204/12/0805) and use of facilities of
the large infrastructure SAFMAT project CZ.2.13/3.1.00/22132. The work
was also supported by institutional research funding IUT02-26 of the
Estonian Ministry of Education and Research and the project of the
Estonian Science Foundation (No. 8678).
NR 51
TC 6
Z9 6
U1 4
U2 20
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 7
PY 2014
VL 90
IS 6
AR 064104
DI 10.1103/PhysRevB.90.064104
PG 12
WC Physics, Condensed Matter
SC Physics
GA AM6SE
UT WOS:000339994200003
ER
PT J
AU May, AF
McGuire, MA
Sales, BC
AF May, Andrew F.
McGuire, Michael A.
Sales, Brian C.
TI Effect of Eu magnetism on the electronic properties of the candidate
Dirac material EuMnBi2
SO PHYSICAL REVIEW B
LA English
DT Article
ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; SRMNBI2
AB The crystal structure and physical properties of the layered material EuMnBi2 have been characterized by measurements on single crystals. EuMnBi2 is isostructural with the Dirac material SrMnBi2 based on single-crystal x-ray diffraction, crystallizing in the I4/mmm space group (No. 139). Magnetic susceptibility measurements suggest antiferromagnetic (AFM) ordering of moments on divalent Eu ions near T-N = 22 K. For low fields, the ordered Eu moments are aligned along the c axis, and a spin flop is observed near 5.4 T at 5 K. The moment is not saturated in an applied field of 13 T at 5 K, which is uncommon for compounds containing Eu2+. The magnetic behavior suggests an anisotropy enhancement via interaction between Eu and the Mn moments that appear to be ordered antiferromagnetically below approximate to 310 K. A large increase in the magnetoresistance is observed across the spin flop, with absolute magnetoresistance reaching approximate to 650% at 5 K and 12 T. Hall effect measurements reveal a decrease in the carrier density belowT(N), which implies a manipulation of the Fermi surface by magnetism on the sites surrounding the Bi square nets that lead to Dirac cones in this family of materials.
C1 [May, Andrew F.; McGuire, Michael A.; Sales, Brian C.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP May, AF (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
EM mayaf@ornl.gov
RI McGuire, Michael/B-5453-2009; May, Andrew/E-5897-2011
OI McGuire, Michael/0000-0003-1762-9406; May, Andrew/0000-0003-0777-8539
FU US Department of Energy, Office of Basic Energy Sciences, Materials
Sciences and Engineering Division
FX This work was supported by the US Department of Energy, Office of Basic
Energy Sciences, Materials Sciences and Engineering Division. We thank
Radu Custelcean for assistance with single-crystal diffraction
measurements.
NR 27
TC 10
Z9 12
U1 10
U2 60
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 7
PY 2014
VL 90
IS 7
AR 075109
DI 10.1103/PhysRevB.90.075109
PG 7
WC Physics, Condensed Matter
SC Physics
GA AM6SG
UT WOS:000339994400001
ER
PT J
AU Parker, D
Idrobo, JC
Cantoni, C
Sefat, AS
AF Parker, D.
Idrobo, J. C.
Cantoni, C.
Sefat, A. S.
TI Evidence for superconductivity at T-c=12 K in oxygen-deficient
MoO2-delta and properties of molybdenum arsenide and oxide binaries
SO PHYSICAL REVIEW B
LA English
DT Article
ID ELECTRONIC-STRUCTURE; METALLIC ELEMENTS; PHASES
AB We find signatures of superconductivity at T-c = 12 K in a molybdenum arsenide sample containing similar to 4% of MoO2-delta impurity by weight. Below is a report on the electronic structure calculations, structures analyses, and thermodynamic and transport properties on Mo2As3, Mo5As4, and MoO2, in order to uncover the reasons for superconductivity for the sample that contains a mixture of these phases. The experimental and theoretical evidence suggest that superconductivity in the MoO2-delta phase is likely and may be caused by nesting- type fluctuations.
C1 [Parker, D.; Cantoni, C.; Sefat, A. S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
[Idrobo, J. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci Div, Oak Ridge, TN 37831 USA.
RP Parker, D (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RI Idrobo, Juan/H-4896-2015; Sefat, Athena/R-5457-2016
OI Idrobo, Juan/0000-0001-7483-9034; Sefat, Athena/0000-0002-5596-3504
FU Oak Ridge National Laboratory LDRD; Department of Energy, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division;
ORNL; Scientific User Facility Division, office of Basic Energy
Sciences, US Department of Energy
FX This work was supported by the Oak Ridge National Laboratory LDRD
funding program. A. S. also acknowledges support by the Department of
Energy, Office of Basic Energy Sciences, Materials Sciences and
Engineering Division. Part of this research was conducted at the Center
for Nanophase Materials Sciences User Facility (JCI), which is sponsored
at ORNL by the Scientific User Facility Division, office of Basic Energy
Sciences, US Department of Energy.
NR 23
TC 3
Z9 3
U1 2
U2 33
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 7
PY 2014
VL 90
IS 5
AR 054505
DI 10.1103/PhysRevB.90.054505
PG 7
WC Physics, Condensed Matter
SC Physics
GA AM6RH
UT WOS:000339991800006
ER
PT J
AU Sandilands, LJ
Reijnders, AA
Su, AH
Baydina, V
Xu, Z
Yang, A
Gu, G
Pedersen, T
Borondics, F
Burch, KS
AF Sandilands, L. J.
Reijnders, A. A.
Su, A. H.
Baydina, V.
Xu, Z.
Yang, A.
Gu, G.
Pedersen, T.
Borondics, F.
Burch, K. S.
TI Origin of the insulating state in exfoliated high-T-c two-dimensional
atomic crystals
SO PHYSICAL REVIEW B
LA English
DT Article
ID OPTICAL-PROPERTIES; ROOM-TEMPERATURE; THIN-FILMS; SUPERCONDUCTOR;
ELECTRODYNAMICS; SPECTROSCOPY; GRAPHENE; BI2SE3; PLANE
AB We present the results of an optical spectroscopic study of two- dimensional atomic crystals of the hightemperature superconductor Bi2Sr2CaCu2O8+delta. Our measurements reveal a pronounced suppression of the optical conductivity sigma(1)(omega) with thickness. Using an effective medium approximation, we interpret this in terms of an insulating surface layer. The surface layer explains the insulating behavior previously observed in exfoliated Bi2Sr2CaCu2O8+delta and has implications -for future studies and potential applications of these materials.
C1 [Sandilands, L. J.; Reijnders, A. A.; Su, A. H.; Baydina, V.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada.
[Xu, Z.; Yang, A.; Gu, G.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
[Pedersen, T.; Borondics, F.] Canadian Light Source, Saskatoon, SK S7N 2V3, Canada.
[Burch, K. S.] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA.
RP Sandilands, LJ (reprint author), Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada.
RI xu, zhijun/A-3264-2013; Borondics, Ferenc/A-7616-2008;
OI xu, zhijun/0000-0001-7486-2015; Borondics, Ferenc/0000-0001-9975-4301
FU Natural Sciences and Engineering Research Council of Canada; National
Research Council Canada; Canadian Institutes of Health Research;
Province of Saskatchewan; Western Economic Diversification Canada;
University of Saskatchewan; US DOE [DE-AC02-98CH10886]
FX The authors would like to acknowledge the input of Young-June Kim,
Andreea Lupascu, and Zhiqiang Li, and thank M. C. Goh for use of her
AFM. Research described in this work was performed at the Mid- IR
beamline of the Canadian Light Source, which is supported by the Natural
Sciences and Engineering Research Council of Canada, the National
Research Council Canada, the Canadian Institutes of Health Research, the
Province of Saskatchewan, Western Economic Diversification Canada, and
the University of Saskatchewan. Work at Brookhaven is supported by the
US DOE under Contract No. DE-AC02-98CH10886.
NR 33
TC 0
Z9 0
U1 0
U2 11
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 7
PY 2014
VL 90
IS 8
AR 081402
DI 10.1103/PhysRevB.90.081402
PG 5
WC Physics, Condensed Matter
SC Physics
GA AM6SI
UT WOS:000339994600002
ER
PT J
AU Kang, ZB
Vitev, I
Xing, HX
AF Kang, Zhong-Bo
Vitev, Ivan
Xing, Hongxi
TI Next-to-Leading-Order Forward Hadron Production in the Small-x Regime:
The Role of Rapidity Factorization
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID COLOR GLASS CONDENSATE; HIGH-ENERGY SCATTERING; COLLISIONS
AB Single inclusive hadron production at forward rapidity in high energy p + A collisions is an important probe of the high gluon density regime of QCD and the associated small-x formalism. We revisit an earlier one-loop calculation to illustrate the significance of the "rapidity factorization" approach in this regime. Such factorization separates the very small-x unintegrated gluon density evolution and leads to a new correction term to the physical cross section at one-loop level. Importantly, this rapidity factorization formalism remedies the previous unphysical negative next-to-leading-order contribution to the cross section. It is much more stable with respect to "rapidity" variation when compared to the leading-order calculation and provides improved agreement between theory and experiment in the forward rapidity region.
C1 [Kang, Zhong-Bo; Vitev, Ivan; Xing, Hongxi] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Xing, Hongxi] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.
RP Kang, ZB (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RI Kang, Zhongbo/P-3645-2014
FU U.S. Department of Energy, Office of Science; LDRD program at LANL
FX This research is supported by the U.S. Department of Energy, Office of
Science, and in part by the LDRD program at LANL.
NR 28
TC 13
Z9 13
U1 0
U2 2
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 7
PY 2014
VL 113
IS 6
AR 062002
DI 10.1103/PhysRevLett.113.062002
PG 5
WC Physics, Multidisciplinary
SC Physics
GA AM6SV
UT WOS:000339996100001
PM 25148318
ER
PT J
AU Masuda, S
Nakamura, K
del Campo, A
AF Masuda, Shumpei
Nakamura, Katsuhiro
del Campo, Adolfo
TI High-Fidelity Rapid Ground-State Loading of an Ultracold Gas into an
Optical Lattice
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID BOSE-EINSTEIN CONDENSATE; DYNAMICS; ADIABATICITY; SHORTCUTS; BILLIARDS;
TOOLBOX; PHYSICS
AB A protocol is proposed for the rapid coherent loading of a Bose-Einstein condensate into the ground state of an optical lattice, without residual excitation associated with the breakdown of adiabaticity. The driving potential required to assist the rapid loading is derived using the fast-forward technique, and generates the ground state in any desired short time. We propose an experimentally feasible loading scheme using a bichromatic lattice potential, which approximates the fast-forward driving potential with high fidelity.
C1 [Masuda, Shumpei] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA.
[Masuda, Shumpei] Tohoku Univ, Dept Phys, Sendai, Miyagi 980, Japan.
[Nakamura, Katsuhiro] Turin Polytech Univ Tashkent, Tashkent 100095, Uzbekistan.
[Nakamura, Katsuhiro] Osaka City Univ, Dept Appl Phys, Sumiyoshi Ku, Osaka 5588585, Japan.
[del Campo, Adolfo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[del Campo, Adolfo] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.
RP Masuda, S (reprint author), Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.
RI del Campo, Adolfo/B-8439-2009
OI del Campo, Adolfo/0000-0003-2219-2851
FU Japan Society for Promotion of Science; JSPS Postdoctoral Fellowships
for Research Abroad; U.S Department of Energy; LANL J. Robert
Oppenheimer Fellowship
FX It is a pleasure to acknowledge discussions with V. Ahufinger, R.
Onofrio, B. Rauer, and L. Tarruell. S. M. thanks Grants-in-Aid for
Centric Research of Japan Society for Promotion of Science and JSPS
Postdoctoral Fellowships for Research Abroad for its financial support.
This research is further supported by the U.S Department of Energy
through the LANL/LDRD Program and a LANL J. Robert Oppenheimer
Fellowship (A.D.).
NR 50
TC 22
Z9 22
U1 2
U2 17
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 7
PY 2014
VL 113
IS 6
AR 063003
DI 10.1103/PhysRevLett.113.063003
PG 5
WC Physics, Multidisciplinary
SC Physics
GA AM6SV
UT WOS:000339996100003
PM 25148323
ER
PT J
AU Yilmaz, T
Pletikosic, I
Weber, AP
Sadowski, JT
Gu, GD
Caruso, AN
Sinkovic, B
Valla, T
AF Yilmaz, T.
Pletikosic, I.
Weber, A. P.
Sadowski, J. T.
Gu, G. D.
Caruso, A. N.
Sinkovic, B.
Valla, T.
TI Absence of a Proximity Effect for a Thin-Films of a Bi2Se3 Topological
Insulator Grown on Top of a Bi2Sr2CaCu2O8+delta Cuprate Superconductor
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID BI2TE3; STATE
AB Proximity-induced superconductivity in a 3D topological insulator represents a new avenue for observing zero-energy Majorana fermions inside vortex cores. Relatively small gaps and low transition temperatures of conventional s-wave superconductors put hard constraints on these experiments. Significantly larger gaps and higher transition temperatures in cuprate superconductors might be an attractive alternative to considerably relax these constraints, but it is not clear whether the proximity effect would be effective in heterostructures involving cuprates and topological insulators. Here, we present angle-resolved photoemission studies of thin Bi2Se3 films grown in situ on optimally doped Bi2Sr2CaCu2O8+delta substrates that show the absence of proximity-induced gaps on the surfaces of Bi2Se3 films as thin as a 1.5 quintuple layer. These results suggest that the superconducting proximity effect between a cuprate superconductor and a topological insulator is strongly suppressed, likely due to a very short coherence length along the c axis, incompatible crystal and pairing symmetries at the interface, small size of the topological surface state's Fermi surface, and adverse effects of a strong spin-orbit coupling in the topological material.
C1 [Yilmaz, T.; Sinkovic, B.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA.
[Pletikosic, I.; Gu, G. D.; Valla, T.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
[Pletikosic, I.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA.
[Weber, A. P.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA.
[Sadowski, J. T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Caruso, A. N.] Univ Missouri, Dept Phys, Kansas City, MO 64110 USA.
RP Yilmaz, T (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA.
EM valla@bnl.gov
RI Pletikosic, Ivo/A-5683-2010; Weber, Andrew/G-8148-2016
OI Pletikosic, Ivo/0000-0003-4697-8912; Weber, Andrew/0000-0002-7636-2572
FU US Department of Energy, Office of Basic Energy Sciences
[DE-AC02-98CH10886]; ARO MURI program [W911NF-12-1-0461]
FX This work was supported by the US Department of Energy, Office of Basic
Energy Sciences, Contract No. DE-AC02-98CH10886, and the ARO MURI
program, Grant No. W911NF-12-1-0461.
NR 26
TC 12
Z9 12
U1 6
U2 59
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 7
PY 2014
VL 113
IS 6
AR 067003
DI 10.1103/PhysRevLett.113.067003
PG 5
WC Physics, Multidisciplinary
SC Physics
GA AM6SV
UT WOS:000339996100006
PM 25148345
ER
PT J
AU Zueva, EM
Herchel, R
Borshch, SA
Govor, EV
Sameera, WMC
McDonald, R
Singleton, J
Krzystek, J
Travnioek, Z
Sanakis, Y
McGrady, JE
Raptis, RG
AF Zueva, Ekaterina M.
Herchel, Radovan
Borshch, Serguei A.
Govor, Evgen V.
Sameera, W. M. C.
McDonald, Ross
Singleton, John
Krzystek, Jurek
Travnioek, Zdenek
Sanakis, Yiannis
McGrady, John E.
Raptis, Raphael G.
TI Double exchange in a mixed-valent octanuclear iron cluster,
[Fe-8(mu(4)-O)(4)(mu-4-Cl-pz)(12)Cl-4](-)
SO DALTON TRANSACTIONS
LA English
DT Article
ID MAGNETIC-PROPERTIES; ELECTRON DELOCALIZATION; VIBRONIC MODEL; COMPLEXES;
SYSTEMS; MOSSBAUER; PROTEINS; LOCALIZATION; RESONANCE; SPECTRA
AB A combination of SQUID and pulsed high-field magnetometry is used to probe the nature of mixed valency in an (FeFe7III)-Fe-II cluster. DFT-computed spin Hamiltonian parameters suggest that antiferromagnetic coupling dominates, and that electron transfer both between the four irons of the cubane core (t(1)) and between a cubane and three neighboring irons (t(2)) is significant. Simulations using the computed parameters are able to reproduce the key features of the measured effective magnetic moment, mu(eff)(T), over the 2 < T < 300 K temperature range. In contrast, the field dependence of the molar magnetization, M-mol, measured at 0.4 K is inconsistent with substantial electron transfer: only values of t(2) similar to 0 place the separation between ground and first excited states in the region indicated by experiment. The apparent quenching of the cubane-outer electron transfer at very low temperatures indicates that vibronic coupling generates one or more shallow minima on the adiabatic potential energy surfaces that serve to trap the itinerant electron in the cubane core.
C1 [Zueva, Ekaterina M.; Sameera, W. M. C.; McGrady, John E.] Univ Oxford, Inorgan Chem Lab, Dept Chem, Oxford OX1 3QR, England.
[Zueva, Ekaterina M.] Kazan Natl Res Technol Univ, Dept Inorgan Chem, Kazan 420015, Russia.
[Herchel, Radovan; Travnioek, Zdenek] Palacky Univ, Fac Sci, Dept Inorgan Chem, Reg Ctr Adv Technol & Mat, Olomouc, Czech Republic.
[Borshch, Serguei A.] Ecole Normale Super Lyon, UMR 5182, Chim Lab, F-69364 Lyon, France.
[Govor, Evgen V.; Raptis, Raphael G.] Univ Puerto Rico, Inst Funct Nanomat, Dept Chem, San Juan, PR 00936 USA.
[McDonald, Ross; Singleton, John] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA.
[Krzystek, Jurek] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA.
[Sanakis, Yiannis] NCRS Demokritos, Inst Mat Sci, Athens 15310, Greece.
RP McGrady, JE (reprint author), Univ Oxford, Inorgan Chem Lab, Dept Chem, S Parks Rd, Oxford OX1 3QR, England.
EM john.mcgrady@chem.ox.ac.uk
RI Raptis, Raphael/D-2833-2009; Herchel, Radovan/B-4339-2008
OI Raptis, Raphael/0000-0002-9522-0369; Herchel,
Radovan/0000-0001-8262-4666
FU EPSRC (UK) [EP/G002789/1]; National Science Foundation (USA)
[CHE-0822600]; Ministry of Education and Science (Russia) [8436];
Operational Program Research and Development for Innovations of the
Ministry of Education, Youth and Sports (Czech Republic)
[CZ.1.05/2.1.00/03.0058]; NSF [DMR 1157490]; State of Florida;
Department of Energy
FX Financial support from the EPSRC-EP/G002789/1 (UK), National Science
Foundation-CHE-0822600 (USA), the Ministry of Education and Science
project 8436 (Russia) and the Operational Program Research and
Development for Innovations CZ.1.05/2.1.00/03.0058 of the Ministry of
Education, Youth and Sports (Czech Republic) is gratefully acknowledged.
Part of this work was carried out at the National High Magnetic Field
Laboratory, which is funded by NSF (Cooperative Agreement DMR 1157490),
the State of Florida, and Department of Energy. RGR is grateful to the
NHMFL for the granting of instrument time to projects PO1587 and PO1965.
NR 45
TC 2
Z9 2
U1 5
U2 39
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 1477-9226
EI 1477-9234
J9 DALTON T
JI Dalton Trans.
PD AUG 7
PY 2014
VL 43
IS 29
BP 11269
EP 11276
DI 10.1039/c4dt00020j
PG 8
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA AL7IC
UT WOS:000339306400021
PM 24668287
ER
PT J
AU Holmes, DE
Giloteaux, L
Orellana, R
Williams, KH
Robbins, MJ
Lovley, DR
AF Holmes, Dawn E.
Giloteaux, Ludovic
Orellana, Roberto
Williams, Kenneth H.
Robbins, Mark J.
Lovley, Derek R.
TI Methane production from protozoan endosymbionts following stimulation of
microbial metabolism within subsurface sediments
SO FRONTIERS IN MICROBIOLOGY
LA English
DT Article
DE anaerobic protozoa; methanogenesis; in situ transcriptomics; uranium
bioremediation; endosymbiont
ID 16S RIBOSOMAL-RNA; URANIUM-CONTAMINATED GROUNDWATER;
POLYMERASE-CHAIN-REACTION; METHANOGENIC BACTERIA; PHYLOGENETIC ANALYSIS;
SULFATE REDUCERS; ARSENIC RELEASE; ORGANIC-MATTER; DISSIMILATORY
REDUCTION; ANAEROBIC PROTOZOA
AB Previous studies have suggested that protozoa prey on Fe(III)- and sulfate-reducing bacteria that are enriched when acetate is added to uranium contaminated subsurface sediments to stimulate U(VI) reduction. In order to determine whether protozoa continue to impact subsurface biogeochemistry after these acetate amendments have stopped, 18S rRNA and beta-tubulin sequences from this phase of an in situ uranium bioremediation field experiment were analyzed. Sequences most similar to Metopus species predominated, with the majority of sequences most closely related to M. palaeformis, a cilitated protozoan known to harbor methanogenic symbionts. Quantification of mcrA m RNA transcripts in the groundwater suggested that methanogens closely related to Metopus endosymbionts were metabolically active at this time. There was a strong correlation between the number of mcrA transcripts from the putative endosymbiotic methanogen and Metopus beta-tubulin m RNA transcripts during the course of the field experiment, suggesting that the activity of the methanogens was dependent upon the activity of the Metopus species. Addition of the eukaryotic inhibitors cyclohexamide and colchicine to laboratory incubations of acetate-amended subsurface sediments significantly inhibited methane production and there was a direct correlation between methane concentration and Metopus beta-tubulin and putative symbiont mcrA gene copies. These results suggest that, following the stimulation of subsurface microbial growth with acetate, protozoa harboring methanogenic endosymbionts become important members of the microbial community, feeding on moribund biomass and producing methane.
C1 [Holmes, Dawn E.; Giloteaux, Ludovic; Orellana, Roberto; Lovley, Derek R.] Univ Massachusetts, Dept Microbiol, Amherst, MA 01003 USA.
[Holmes, Dawn E.] Western New England Univ, Springfield, MA 01119 USA.
[Williams, Kenneth H.; Robbins, Mark J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Holmes, DE (reprint author), Western New England Univ, 1215 Wilbraham Rd, Springfield, MA 01119 USA.
EM dholmes@wne.edu
RI Williams, Kenneth/O-5181-2014; Giloteaux, Ludovic/L-6986-2015
OI Williams, Kenneth/0000-0002-3568-1155;
FU Office of Science (BER), U. S. Department of Energy [DE-SC0006790]
FX This research was supported by the Office of Science (BER), U. S.
Department of Energy, Award No. DE-SC0006790.
NR 65
TC 4
Z9 4
U1 2
U2 44
PU FRONTIERS RESEARCH FOUNDATION
PI LAUSANNE
PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND
SN 1664-302X
J9 FRONT MICROBIOL
JI Front. Microbiol.
PD AUG 6
PY 2014
VL 5
AR 366
DI 10.3389/fmicb.2014.00366
PG 9
WC Microbiology
SC Microbiology
GA AO7ED
UT WOS:000341514000001
PM 25147543
ER
PT J
AU Tsvelik, AM
AF Tsvelik, A. M.
TI Integrable Model with Parafermion Zero Energy Modes
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID TOPOLOGICAL QUANTUM COMPUTATION; CURRENT-ALGEBRA; 2 DIMENSIONS;
PERTURBATIONS; SYMMETRY; ANYONS
AB Parafermion zero energy modes are a vital element of fault-tolerant topological quantum computation. Although it is believed that such modes form on the border between topological and normal phases, this has been demonstrated only for Z(2) (Majorana) and Z(3) parafermions. I consider an integrable model of one-dimensional fermions where such a demonstration is possible for Z(N) parafermions with any N. The procedure is easily generalizable for more complicated symmetry groups.
C1 Brookhaven Natl Lab, Upton, NY 11973 USA.
RP Tsvelik, AM (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.
FU U.S. DOE [DE-AC02-98 CH 10886]
FX I am grateful to H. Frahm and R. Konik for valuable discussions and
interest in the work. The work was supported by the U.S. DOE under
Contract No. DE-AC02-98 CH 10886.
NR 27
TC 3
Z9 3
U1 0
U2 2
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 6
PY 2014
VL 113
IS 6
AR 066401
DI 10.1103/PhysRevLett.113.066401
PG 4
WC Physics, Multidisciplinary
SC Physics
GA AO4FJ
UT WOS:000341291300005
PM 25148341
ER
PT J
AU Cowan, SR
Schulz, P
Giordano, AJ
Garcia, A
MacLeod, BA
Marder, SR
Kahn, A
Ginley, DS
Ratcliff, EL
Olson, DC
AF Cowan, Sarah R.
Schulz, Philip
Giordano, Anthony J.
Garcia, Andres
MacLeod, Bradley A.
Marder, Seth R.
Kahn, Antoine
Ginley, David S.
Ratcliff, Erin L.
Olson, Dana C.
TI Chemically Controlled Reversible and Irreversible Extraction Barriers
Via Stable Interface Modification of Zinc Oxide Electron Collection
Layer in Polycarbazole-based Organic Solar Cells
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
ID OPEN-CIRCUIT VOLTAGE; INDIUM-TIN OXIDE; POWER-CONVERSION EFFICIENCY;
TITANIUM DIOXIDE; SURFACE; TANDEM; OXYGEN; ZNO; PERFORMANCE; ADSORPTION
AB A spin-cast method is presented for the formation of phosphonic acid functionalized small molecule layers on solution-processed ZnO substrates for use as electron collecting interlayers in organic photovoltaics. Phosphonic acid interlayers modify the ZnO work function and the charge carrier injection barrier at its interface, resulting in systematic control of V-OC in inverted bulk heterojunction solar cells. Surface modification is shown to moderate the need for UV light-soaking of the ZnO contact layers. Lifetime studies (30 days) indicate stable and improved OPV performance over the unmodified ZnO contact, which show significant increases in charge extraction barriers and series resistance. Results suggest that enhanced stability using small molecule modifiers is due to partial passivation of the oxide surface to molecular oxygen adsorption. Surface passivation while maintaining work function control of a selective interlayer can be employed to improve net efficiency and lifetime of organic photovoltaic devices. The modified cathode work function modulates V-OC via static energetic barriers and modulates contact conductivity by creating reversible and irreversible S-shape current-voltage characteristics as a result of kinetic barriers to charge transport.
C1 [Cowan, Sarah R.; Garcia, Andres; MacLeod, Bradley A.; Ginley, David S.; Olson, Dana C.] Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA.
[Schulz, Philip; Kahn, Antoine] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA.
[Giordano, Anthony J.; Marder, Seth R.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA.
[Giordano, Anthony J.; Marder, Seth R.] Georgia Inst Technol, Ctr Organ Photon & Elect, Atlanta, GA 30332 USA.
[Ratcliff, Erin L.] Univ Arizona, Dept Chem, Tucson, AZ 85721 USA.
RP Cowan, SR (reprint author), Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA.
EM Dana.Olson@nrel.gov
RI MacLeod, Bradley/F-5589-2013; Schulz, Philip/N-2295-2015
OI MacLeod, Bradley/0000-0001-5319-3051; Schulz, Philip/0000-0002-8177-0108
FU Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral
Research Fellowship through the SunShot Solar Energy Technologies
Program; Center for Interface Science: Solar Electric Materials, an
Energy Frontier Research Center - U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences [DE-SC0001084]
FX S.R.C. acknowledges funding from the Office of Energy Efficiency and
Renewable Energy (EERE) Postdoctoral Research Fellowship through the
SunShot Solar Energy Technologies Program. This work was supported as
part of the Center for Interface Science: Solar Electric Materials, an
Energy Frontier Research Center funded by the U.S. Department of Energy,
Office of Science, Office of Basic Energy Sciences under Award Number
DE-SC0001084. The authors acknowledge Mr. Skyler Jackson for work
function measurements on ITO.
NR 49
TC 34
Z9 34
U1 17
U2 95
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD AUG 6
PY 2014
VL 24
IS 29
BP 4671
EP 4680
DI 10.1002/adfm.201400158
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AN3CB
UT WOS:000340461400012
ER
PT J
AU Wang, JL
Yang, MY
Zhu, Y
Wang, L
Tomsia, AP
Mao, CB
AF Wang, Jianglin
Yang, Mingying
Zhu, Ye
Wang, Lin
Tomsia, Antoni P.
Mao, Chuanbin
TI Phage Nanofibers Induce Vascularized Osteogenesis in 3D Printed Bone
Scaffolds
SO ADVANCED MATERIALS
LA English
DT Article
ID MESENCHYMAL STEM-CELLS; INTEGRIN ALPHA(V)BETA(3); BIOLOGICAL NANOFIBERS;
IN-VIVO; ANGIOGENESIS; TISSUE; GROWTH; DELIVERY; DIFFERENTIATION;
MINERALIZATION
AB A virus-activated matrix is developed to overcome the challenge of forming vascularized bone tissue. It is generated by filling a 3D printed bioceramic scaffold with phage nanofibers displaying high-density RGD peptide. After it is seeded with mesenchymal stem cells (MSCs) and implanted into a bone defect, the phage nanofibers induce osteogenesis and angiogenesis by activating endothelialization and osteogenic differentiation of MSCs.
C1 [Wang, Jianglin; Zhu, Ye; Wang, Lin; Mao, Chuanbin] Univ Oklahoma, Dept Chem & Biochem, Stephenson Life Sci Res Ctr, Norman, OK 73019 USA.
[Yang, Mingying] Zhejiang Univ, Inst Appl Bioresource Res, Coll Anim Sci, Hangzhou 310058, Zhejiang, Peoples R China.
[Tomsia, Antoni P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Yang, MY (reprint author), Zhejiang Univ, Inst Appl Bioresource Res, Coll Anim Sci, Yuhangtang Rd 866, Hangzhou 310058, Zhejiang, Peoples R China.
EM yangm@zju.edu.cn; cbmao@ou.edu
RI WANG, JIANGLIN/L-5155-2015;
OI Mao, Chuanbin/0000-0002-8142-3659
FU National Institutes of Health [5R01DE015633, 5R01HL092526, 1R21EB015190,
4R03AR056848]; National Science Foundation [CBET-0854465, CMMI-1234957,
CBET-0854414, DMR-0847758]; Oklahoma Center for Adult Stem Cell Research
[434003]; Department of Defense Peer Reviewed Medical Research Program
[W81XWH-12-1-0384]; Oklahoma Center for the Advancement of Science and
Technology [070014, HR11-006]; National High Technology Research and
Development Program 863 [2013AA102507]; National Natural Science
Foundation of China [20804037, 21172194]; Zhejiang Provincial Natural
Science Foundation of China [LZ12C17001]; Projects of Zhejiang
Provincial Science and Technology Plans [2012C12910]; Silkworm Industry
Science and Technology Innovation Team [2011R50028]
FX We would like to thank the financial support from the National
Institutes of Health (5R01DE015633, 5R01HL092526, 1R21EB015190, and
4R03AR056848), the National Science Foundation (CBET-0854465,
CMMI-1234957, CBET-0854414, and DMR-0847758), the Oklahoma Center for
Adult Stem Cell Research (434003), Department of Defense Peer Reviewed
Medical Research Program (W81XWH-12-1-0384), and the Oklahoma Center for
the Advancement of Science and Technology (070014 and HR11-006). M.Y.
acknowledges the support of National High Technology Research and
Development Program 863 (2013AA102507), National Natural Science
Foundation of China (20804037 and 21172194), Zhejiang Provincial Natural
Science Foundation of China (LZ12C17001), Projects of Zhejiang
Provincial Science and Technology Plans (2012C12910), and Silkworm
Industry Science and Technology Innovation Team (2011R50028). We would
also like to thank Drs. Kun Ma and Yiyang Lin for their kind help during
the experiments.
NR 39
TC 47
Z9 47
U1 24
U2 206
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD AUG 6
PY 2014
VL 26
IS 29
BP 4961
EP 4966
DI 10.1002/adma.201400154
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA AN3PP
UT WOS:000340500700009
PM 24711251
ER
PT J
AU Book, AJ
Yennamalli, RM
Takasuka, TE
Currie, CR
Phillips, GN
Fox, BG
AF Book, Adam J.
Yennamalli, Ragothaman M.
Takasuka, Taichi E.
Currie, Cameron R.
Phillips, George N., Jr.
Fox, Brian G.
TI Evolution of substrate specificity in bacterial AA10 lytic
polysaccharide monooxygenases
SO BIOTECHNOLOGY FOR BIOFUELS
LA English
DT Article
DE Lytic polysaccharide monooxygenase; LPMO; Cellulase; Chitinase;
Streptomyces; AA9; AA10; Enzyme evolution; Biofuels
ID BAYESIAN PHYLOGENETIC INFERENCE; GLYCOSIDE HYDROLASE FAMILY; BINDING
PROTEIN CBP21; CELLOBIOSE DEHYDROGENASE; THERMOMONOSPORA-FUSCA;
DEGRADING ENZYMES; NEUROSPORA-CRASSA; CRYSTAL-STRUCTURE; PROVIDES
INSIGHT; ACTIVE-SITE
AB Background: Understanding the diversity of lignocellulose-degrading enzymes in nature will provide insights for the improvement of cellulolytic enzyme cocktails used in the biofuels industry. Two families of enzymes, fungal AA9 and bacterial AA10, have recently been characterized as crystalline cellulose or chitin-cleaving lytic polysaccharide monooxygenases (LPMOs). Here we analyze the sequences, structures, and evolution of LPMOs to understand the factors that may influence substrate specificity both within and between these enzyme families.
Results: Comparative analysis of sequences, solved structures, and homology models from AA9 and AA10 LPMO families demonstrated that, although these two LPMO families are highly conserved, structurally they have minimal sequence similarity outside the active site residues. Phylogenetic analysis of the AA10 family identified clades with putative chitinolytic and cellulolytic activities. Estimation of the rate of synonymous versus non-synonymous substitutions (dN/dS) within two major AA10 subclades showed distinct selective pressures between putative cellulolytic genes (subclade A) and CBP21-like chitinolytic genes (subclade D). Estimation of site-specific selection demonstrated that changes in the active sites were strongly negatively selected in all subclades. Furthermore, all codons in the subclade D had dN/dS values of less than 0.7, whereas codons in the cellulolytic subclade had dN/dS values of greater than 1.5. Positively selected codons were enriched at sites localized on the surface of the protein adjacent to the active site.
Conclusions: The structural similarity but absence of significant sequence similarity between AA9 and AA10 families suggests that these enzyme families share an ancient ancestral protein. Combined analysis of amino acid sites under Darwinian selection and structural homology modeling identified a subclade of AA10 with diversifying selection at different surfaces, potentially used for cellulose-binding and protein-protein interactions. Together, these data indicate that AA10 LPMOs are under selection to change their function, which may optimize cellulolytic activity. This work provides a phylogenetic basis for identifying and classifying additional cellulolytic or chitinolytic LPMOs.
C1 [Book, Adam J.; Takasuka, Taichi E.; Currie, Cameron R.; Phillips, George N., Jr.; Fox, Brian G.] Great Lakes Bioenergy Res Ctr, Dept Energy, Madison, WI 53726 USA.
[Book, Adam J.; Currie, Cameron R.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA.
[Yennamalli, Ragothaman M.; Takasuka, Taichi E.; Phillips, George N., Jr.; Fox, Brian G.] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA.
RP Fox, BG (reprint author), Great Lakes Bioenergy Res Ctr, Dept Energy, 1552 Univ Ave, Madison, WI 53726 USA.
EM bgfox@biochem.wisc.edu
FU Department of Energy Great Lakes Bioenergy Research Center (DOE BER
Office of Science) [DE-FC-02-07ER64494]; Department of Energy Bringing
Advanced Computational Techniques to Energy Research program (DOE
BACTER) [DE-FG02-04ER25627]; National Institute of Health Protein
Structure Initiative [U01 GM098248]; National Science Foundation GRAPE
[CMMI-0941013]
FX This work was funded by the Department of Energy Great Lakes Bioenergy
Research Center (DOE BER Office of Science DE-FC-02-07ER64494), the
Department of Energy Bringing Advanced Computational Techniques to
Energy Research program (DOE BACTER DE-FG02-04ER25627), the National
Institute of Health Protein Structure Initiative (U01 GM098248), and the
National Science Foundation GRAPE (CMMI-0941013).
NR 55
TC 15
Z9 15
U1 9
U2 54
PU BIOMED CENTRAL LTD
PI LONDON
PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND
SN 1754-6834
J9 BIOTECHNOL BIOFUELS
JI Biotechnol. Biofuels
PD AUG 6
PY 2014
VL 7
AR 109
DI 10.1186/1754-6834-7-109
PG 14
WC Biotechnology & Applied Microbiology; Energy & Fuels
SC Biotechnology & Applied Microbiology; Energy & Fuels
GA AN5KJ
UT WOS:000340629300001
PM 25161697
ER
PT J
AU Du, WX
Yang, GX
Wong, E
Deskins, NA
Frenkel, AI
Su, D
Teng, XW
AF Du, Wenxin
Yang, Guangxing
Wong, Emily
Deskins, N. Aaron
Frenkel, Anatoly I.
Su, Dong
Teng, Xiaowei
TI Platinum-Tin Oxide Core-Shell Catalysts for Efficient Electro-Oxidation
of Ethanol
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID PT-SN ELECTROCATALYSTS; IN-SITU; FUEL-CELLS; OXIDIZING ETHANOL;
CARBON-DIOXIDE; C-C; OXIDATION; METHANOL; DEMS; NANOPARTICLES
AB Platinum-tin (Pt/Sn) binary nanoparticles are active electrocatalysts for the ethanol oxidation reaction (EOR), but inactive for splitting the C-C bond of ethanol to CO2. Here we studied detailed structure properties of Pt/Sn catalysts for the EOR, especially CO2 generation in situ using a CO2 microelectrode. We found that composition and crystalline structure of the tin element played important roles in the CO2 generation: non-alloyed Pt-46-(SnO2)(54) core shell particles demonstrated a strong capability for C-C bond breaking of ethanol than pure Pt and intermetallic Pt/Sn, showing 4.1 times higher CO2 peak partial pressure generated from EOR than commercial Pt/C.
C1 [Du, Wenxin; Yang, Guangxing; Wong, Emily; Teng, Xiaowei] Univ New Hampshire, Dept Chem Engn, Durham, NH 03824 USA.
[Deskins, N. Aaron] Worcester Polytech Inst, Dept Chem Engn, Worcester, MA 01609 USA.
[Frenkel, Anatoly I.] Yeshiva Univ, Dept Phys, New York, NY 10016 USA.
[Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
RP Teng, XW (reprint author), Univ New Hampshire, Dept Chem Engn, Durham, NH 03824 USA.
EM xw.teng@unh.edu
RI Frenkel, Anatoly/D-3311-2011; Du, Wenxin/P-9195-2014; Deskins,
Nathaniel/H-3954-2012; Su, Dong/A-8233-2013
OI Frenkel, Anatoly/0000-0002-5451-1207; Su, Dong/0000-0002-1921-6683
FU National Science Foundation [CBET-1159662]; US Department of Energy
[DE-AC02-98CH10886]; Synchrotron Catalysis Consortium through the U.S.
Department of Energy grant [DE-FG02-05ER15688]; U.S. Department of
Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]
FX This material is based upon work supported by the National Science
Foundation (CBET-1159662) and the US Department of Energy
(DE-AC02-98CH10886). Use of the NSLS was supported by the U.S.
Department of Energy (DE-AC02-98CH10886). Beam lines X19A/X18B are
partly supported by Synchrotron Catalysis Consortium through the U.S.
Department of Energy grant (DE-FG02-05ER15688). TEM work was carried out
at the Center for Functional Nanomaterials at Brookhaven National
Laboratory supported by the U.S. Department of Energy, Office of Basic
Energy Sciences (DE-AC02-98CH10886).
NR 38
TC 45
Z9 45
U1 19
U2 173
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD AUG 6
PY 2014
VL 136
IS 31
BP 10862
EP 10865
DI 10.1021/ja505456w
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA AM7WQ
UT WOS:000340079800011
PM 25033229
ER
PT J
AU Xia, XH
Figueroa-Cosme, L
Tao, J
Peng, HC
Niu, GD
Zhu, YM
Xia, YN
AF Xia, Xiaohu
Figueroa-Cosme, Legna
Tao, Jing
Peng, Hsin-Chieh
Niu, Guangda
Zhu, Yimei
Xia, Younan
TI Facile Synthesis of Iridium Nanocrystals with Well-Controlled Facets
Using Seed-Mediated Growth
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID DEPENDENT CATALYTIC-ACTIVITY; OXYGEN REDUCTION REACTION; NOBLE-METAL
NANOCRYSTALS; HYDRAZINE DECOMPOSITION; PLATINUM NANOPARTICLES; PALLADIUM
NANOCRYSTALS; PD NANOCRYSTALS; CO OXIDATION; SHAPE; HYDROGENATION
AB Iridium nanoparticles have only been reported with roughly spherical shapes and sizes of 1-5 nm, making it impossible to investigate their facet-dependent catalytic properties. Here we report for the first time a simple method based on seed-mediated growth for the facile synthesis of Ir nanocrystals with well-controlled facets. The essence of this approach is to coat an ultrathin conformal shell of Ir on a Pd seed with a well-defined shape at a relatively high temperature to ensure fast surface diffusion. In this way, the facets on the initial Pd seed are faithfully replicated in the resultant Pd@Ir core shell nanocrystal. With 6 nm Pd cubes and octahedra encased by {100} and {111} facets, respectively, as the seeds, we have successfully generated Pd@Ir cubes and octahedra covered by Ir{100} and Ir{111} facets. The Pd@Ir cubes showed higher H-2 selectivity (31.8% vs 8.9%) toward the decomposition of hydrazine compared with Pd@Ir octahedra with roughly the same size.
C1 [Xia, Xiaohu; Niu, Guangda; Xia, Younan] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA.
[Xia, Xiaohu; Niu, Guangda; Xia, Younan] Emory Univ, Atlanta, GA 30332 USA.
[Figueroa-Cosme, Legna; Peng, Hsin-Chieh; Xia, Younan] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA.
[Tao, Jing; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.
RP Xia, YN (reprint author), Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA.
EM younan.xia@bme.gatech.edu
RI Xia, Younan/E-8499-2011; Xia, Xiaohu/H-4581-2015
FU NSF [DMR-1215034]; Georgia Institute of Technology; U.S. Department of
Energy, Office of Basic Energy Sciences, Materials Sciences and
Engineering Division [DE-AC02-98CH1088]
FX This work was supported in part by the NSF (DMR-1215034) and startup
funds from the Georgia Institute of Technology. Part of the electron
microscopy work at BNL was supported by the U.S. Department of Energy,
Office of Basic Energy Sciences, Materials Sciences and Engineering
Division, under Contract DE-AC02-98CH1088.
NR 37
TC 46
Z9 46
U1 18
U2 203
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD AUG 6
PY 2014
VL 136
IS 31
BP 10878
EP 10881
DI 10.1021/ja505716v
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA AM7WQ
UT WOS:000340079800015
PM 25058427
ER
PT J
AU Kim, W
Yuan, G
McClure, BA
Frei, H
AF Kim, Wooyul
Yuan, Guangbi
McClure, Beth Anne
Frei, Heinz
TI Light Induced Carbon Dioxide Reduction by Water at Binuclear ZrOCoII
Unit Coupled to Ir Oxide Nanocluster Catalyst
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID CHARGE-TRANSFER CHROMOPHORE; MESOPOROUS SILICA; ELECTRON-TRANSFER;
PHOTOCATALYTIC REDUCTION; HYDROGEN-PRODUCTION; ARTIFICIAL
PHOTOSYNTHESIS; CO2 REDUCTION; FERMI-LEVEL; OXIDATION; SEMICONDUCTOR
AB An all-inorganic polynuclear unit consisting of an oxo-bridged binuclear ZrOCoII group coupled to an iridium oxide nanocluster (IrOx) was assembled on an SBA-15 silica mesopore surface. A photodeposition method was developed that affords coupling of the IrOx water oxidation catalyst with the Co donor center. The approach consists of excitation of the ZrOCoII metal-to-metal charge-transfer (MMCT) chromophore with visible light in the presence of [Ir(acac)3] (acac: acetylacetonate) precursor followed by calcination under mild conditions, with each step monitored by optical and infrared spectroscopy. Illumination of the MMCT chromophore of the resulting ZrOCoII-IrOx units in the SBA-15 pores loaded with a mixture of (CO2)-C-13 and H2O vapor resulted in the formation of (CO)-C-13 and O-2 monitored by FT-IR and mass spectroscopy, respectively. Use of O-18 labeled water resulted in the formation of O-18(2) product. This is the first example of a closed photosynthetic cycle of carbon dioxide reduction by water using an all-inorganic polynuclear cluster featuring a molecularly defined light absorber. The observed activity implies successful competition of electron transfer between the IrOx catalyst cluster and the transient oxidized Co donor center with back electron transfer of the ZrOCo light absorber, and is further aided by the instant desorption of the CO and O-2 product from the silica pores.
C1 [Kim, Wooyul; Yuan, Guangbi; McClure, Beth Anne; Frei, Heinz] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
RP Frei, H (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
EM HMFrei@lbl.gov
RI Foundry, Molecular/G-9968-2014
FU Office of Science, Office of Basic Energy Sciences, Division of
Chemical, Geological and Biosciences of the U.S. Department of Energy
[DE-AC02-05CH11231]; National Center for Electron Microscopy, Lawrence
Berkeley National Laboratory; U.S. Department of Energy; National
Research Foundation of Korea (NRF) - Ministry of Education
[2012R1A6A3A03039210]
FX This work was supported by the Director, Office of Science, Office of
Basic Energy Sciences, Division of Chemical, Geological and Biosciences
of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.
The authors acknowledge the support of the National Center for Electron
Microscopy, Lawrence Berkeley National Laboratory, which is supported by
the U.S. Department of Energy. W.K. thankful for support from the Basic
Science Research Program through the National Research Foundation of
Korea (NRF) funded by the Ministry of Education (2012R1A6A3A03039210).
The authors thank Drs. Diana Cedeno and Wenjun Liu, Joint Center for
Artificial Photosynthesis at LBNL, for conducting XPS and NMR
measurements.
NR 72
TC 29
Z9 29
U1 8
U2 153
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD AUG 6
PY 2014
VL 136
IS 31
BP 11034
EP 11042
DI 10.1021/ja504753g
PG 9
WC Chemistry, Multidisciplinary
SC Chemistry
GA AM7WQ
UT WOS:000340079800039
PM 25033315
ER
PT J
AU Fang, L
Iyer, RG
Tan, GJ
West, DJ
Zhang, SB
Kanatzidis, MG
AF Fang, Lei
Iyer, Ratnasabapathy G.
Tan, Gangjian
West, Damien J.
Zhang, Shengbai
Kanatzidis, Mercouri G.
TI The New Phase [TI4Sb6Se10][Sn5Sb2Se14]: A Naturally Formed
Semiconducting Heterostructure with Two-Dimensional Conductance
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID AUGMENTED-WAVE METHOD; FERECRYSTALLINE COMPOUNDS; THERMOELECTRICS;
CRYSTALS; SUPERLATTICES; CONDUCTIVITY; PREDICTION; TRANSPORT; MERIT;
PBSE
AB We report on a new layered semiconductor TI8Sn10Sb16Se48 with an indirect band gap of 0.45 eV. The novel structure is made of alternating layers of SnSe2-type [Sn5Sb2Se14] and SnSe-type [TI4Sb6Se10]. The material exhibits two-dimensional (2D) electron variable range hopping at low temperatures, indicating an absence of interlayer coherency of the electronic state. Theoretical calculations unveil a 2D confinement for electrons in the [Sn5Sb2Se14] sheet and confirm the heterostructure nature. This unique electronic structure is attributed to the weak interlayer coupling and structure distortion in the electron-poor [TI4Sb6Se10] layer that energetically impedes electron propagation.
C1 [Fang, Lei; Iyer, Ratnasabapathy G.; Tan, Gangjian; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Iyer, Ratnasabapathy G.] Claflin Univ, Dept Chem, Orangeburg, SC 29118 USA.
[West, Damien J.; Zhang, Shengbai] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA.
[Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
EM m-kanatzidis@northwestern.edu
RI Tan, Gangjian/M-3509-2014; West, Damien/F-8616-2012; Zhang,
Shengbai/D-4885-2013
OI Tan, Gangjian/0000-0002-9087-4048; West, Damien/0000-0002-4970-3968;
Zhang, Shengbai/0000-0003-0833-5860
FU Defense Advanced Research Project Agency (DARPA) [N66001-12-1-4034]; NSF
[DMR-1104965]; US Department of Energy, Office of Science, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division
[DE-AC02-06CH11357]
FX The transport measurements were supported by the Defense Advanced
Research Project Agency (DARPA) (L.F., D.J.W., S.B.Z.) Award No.
N66001-12-1-4034. R.G.I. and G.T. were supported by NSF Grant
DMR-1104965. Research at Argonne was supported by the US Department of
Energy, Office of Science, Office of Basic Energy Sciences, Materials
Sciences and Engineering Division (Argonne Contract No.
DE-AC02-06CH11357).
NR 44
TC 4
Z9 4
U1 3
U2 53
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD AUG 6
PY 2014
VL 136
IS 31
BP 11079
EP 11084
DI 10.1021/ja505301y
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA AM7WQ
UT WOS:000340079800045
PM 25058471
ER
PT J
AU Kiriya, D
Chen, K
Ota, H
Lin, YJ
Zhao, PD
Yu, ZB
Ha, TJ
Javey, A
AF Kiriya, Daisuke
Chen, Kevin
Ota, Hiroki
Lin, Yongjing
Zhao, Peida
Yu, Zhibin
Ha, Tae-jun
Javey, Ali
TI Design of Surfactant-Substrate Interactions for Roll-to-Roll Assembly of
Carbon Nanotubes for Thin-Film Transistors
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID RADIOFREQUENCY APPLICATIONS; INTEGRATED-CIRCUITS; ELECTRONICS; SENSORS;
SOLUBILIZATION; DISPERSION; WATER; ADSORPTION; TRANSPARENT; SEPARATION
AB Controlled assembly of single-walled carbon nanotube (SWCNT) networks with high density and deposition rate is critical for many practical applications, including large-area electronics. In this regard, surfactant chemistry plays a critical role as it facilitates the substrate-nanotube interactions. Despite its importance, detailed understanding of the subject up until now has been lacking, especially toward tuning the controllability of SWCNT assembly for thin-film transistors. Here, we explore SWCNT assembly with steroid- and alkyl-based surfactants. While steroid-based surfactants yield highly dense nanotube thin films, alkyl surfactants are found to prohibit nanotube assembly. The latter is attributed to the formation of packed alkyl layers of residual surfactants on the substrate surface, which subsequently repel surfactant encapsulated SWCNTs. In addition, temperature is found to enhance the nanotube deposition rate and density. Using this knowledge, we demonstrate highly dense and rapid assembly with an effective SWCNT surface coverage of similar to 99% as characterized by capacitance voltage measurements. The scalability of the process is demonstrated through a roll-to-roll assembly of SWCNTs on plastic substrates for large-area thin-film transistors. The work presents an important process scheme for nanomanufacturing of SWCNT-based electronics.
C1 [Kiriya, Daisuke; Chen, Kevin; Ota, Hiroki; Lin, Yongjing; Zhao, Peida; Yu, Zhibin; Ha, Tae-jun; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Kiriya, Daisuke; Chen, Kevin; Ota, Hiroki; Lin, Yongjing; Zhao, Peida; Yu, Zhibin; Ha, Tae-jun; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA.
[Kiriya, Daisuke; Chen, Kevin; Ota, Hiroki; Lin, Yongjing; Zhao, Peida; Yu, Zhibin; Ha, Tae-jun; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Javey, A (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA.
EM ajavey@berkeley.edu
RI Javey, Ali/B-4818-2013
FU NSF NASCENT Center
FX This work was supported by NSF NASCENT Center.
NR 69
TC 24
Z9 24
U1 6
U2 61
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD AUG 6
PY 2014
VL 136
IS 31
BP 11188
EP 11194
DI 10.1021/ja506315j
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA AM7WQ
UT WOS:000340079800060
PM 25019509
ER
PT J
AU Marra, DM
Chambers, JQ
Higuchi, N
Trumbore, SE
Ribeiro, GHPM
dos Santos, J
Negron-Juarez, RI
Reu, B
Wirth, C
AF Marra, Daniel Magnabosco
Chambers, Jeffrey Q.
Higuchi, Niro
Trumbore, Susan E.
Ribeiro, Gabriel H. P. M.
dos Santos, Joaquim
Negron-Juarez, Robinson I.
Reu, Bjoern
Wirth, Christian
TI Large-Scale Wind Disturbances Promote Tree Diversity in a Central Amazon
Forest
SO PLOS ONE
LA English
DT Article
ID TROPICAL RAIN-FOREST; PHYLOGENY GROUP CLASSIFICATION;
BARRO-COLORADO-ISLAND; WOOD DENSITY; PUERTO-RICO; SPECIES-DIVERSITY;
FLOWERING PLANTS; GAP DISTURBANCES; LARGE BLOWDOWNS; HURRICANE HUGO
AB Canopy gaps created by wind-throw events, or blowdowns, create a complex mosaic of forest patches varying in disturbance intensity and recovery in the Central Amazon. Using field and remote sensing data, we investigated the shortterm (four-year) effects of large (>2000 m(2)) blowdown gaps created during a single storm event in January 2005 near Manaus, Brazil, to study (i) how forest structure and composition vary with disturbance gradients and (ii) whether tree diversity is promoted by niche differentiation related to wind-throw events at the landscape scale. In the forest area affected by the blowdown, tree mortality ranged from 0 to 70%, and was highest on plateaus and slopes. Less impacted areas in the region affected by the blowdown had overlapping characteristics with a nearby unaffected forest in tree density (583 +/- 46 trees ha(-1)) (mean +/- 699% Confidence Interval) and basal area (26.7 +/- 2.4 m(2) ha(-1)). Highly impacted areas had tree density and basal area as low as 120 trees ha(-1) and 14.9 m 2 ha(-1), respectively. In general, these structural measures correlated negatively with an index of tree mortality intensity derived from satellite imagery. Four years after the blowdown event, differences in size-distribution, fraction of resprouters, floristic composition and species diversity still correlated with disturbance measures such as tree mortality and gap size. Our results suggest that the gradients of wind disturbance intensity encompassed in large blowdown gaps (>2000 m(2)) promote tree diversity. Specialists for particular disturbance intensities existed along the entire gradient. The existence of species or genera taking an intermediate position between undisturbed and gap specialists led to a peak of rarefied richness and diversity at intermediate disturbance levels. A diverse set of species differing widely in requirements and recruitment strategies forms the initial post-disturbance cohort, thus lending a high resilience towards wind disturbances at the community level.
C1 [Marra, Daniel Magnabosco; Reu, Bjoern; Wirth, Christian] Univ Leipzig, D-04109 Leipzig, Germany.
[Marra, Daniel Magnabosco; Trumbore, Susan E.; Wirth, Christian] Max Planck Inst Biogeochem, BGC Prozesse, D-07745 Jena, Germany.
[Marra, Daniel Magnabosco; Chambers, Jeffrey Q.; Higuchi, Niro; Trumbore, Susan E.; Ribeiro, Gabriel H. P. M.; dos Santos, Joaquim] Inst Nacl de Pesquisas da Amazonia, Lab Manejo Florestal, Manaus, Amazonas, Brazil.
[Chambers, Jeffrey Q.] Univ Calif Berkeley, Dept Geog, Berkeley, CA 94720 USA.
[Chambers, Jeffrey Q.; Negron-Juarez, Robinson I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate Sci Dept, Berkeley, CA 94720 USA.
[Chambers, Jeffrey Q.; Negron-Juarez, Robinson I.] Tulane Univ, Dept Ecol & Evolutionary Biol, New Orleans, LA 70118 USA.
[Wirth, Christian] German Ctr Integrat Biodivers Res iDiv, Leipzig, Germany.
RP Marra, DM (reprint author), Univ Leipzig, D-04109 Leipzig, Germany.
EM daniel.marra@uni-leipzig.de
RI Chambers, Jeffrey/J-9021-2014; iDiv, Deutsches Zentrum/B-5164-2016;
Negron-Juarez, Robinson/I-6289-2016;
OI Chambers, Jeffrey/0000-0003-3983-7847; Ribeiro,
Gabriel/0000-0002-3343-3043
FU Brazilian Council for Scientific and Technological Development (CNPq);
National Aeronautics and Space Administration's Biodiversity Program
[08-BIODIV-10]; Max-Planck-Institute for Biogeochemistry (BGC-Processes,
Jena); Coordination for the Improvement of Higher Level Personal (CAPES)
FX This study was financed by the Brazilian Council for Scientific and
Technological Development (CNPq) [Projeto SAWI (Chamada Universal
MCTI/No 14/2012, Proc. 473357/2012-7) and INCT - Madeiras da Amazonia],
by the National Aeronautics and Space Administration's Biodiversity
Program (Project 08-BIODIV-10), and by the Max-Planck-Institute for
Biogeochemistry (BGC-Processes, Jena). The presented results are part of
the first author's PhD thesis, which incorporate data from his Master
thesis, undertaken at the INPA/CFT, with fellowship funded by the
Coordination for the Improvement of Higher Level Personal (CAPES). The
funders had no role in the study design, data collection and analysis,
decision to publish, or preparation of the manuscript.
NR 105
TC 9
Z9 9
U1 3
U2 51
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1932-6203
J9 PLOS ONE
JI PLoS One
PD AUG 6
PY 2014
VL 9
IS 8
AR e103711
DI 10.1371/journal.pone.0103711
PG 16
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM6SM
UT WOS:000339995100028
PM 25099118
ER
PT J
AU Vigneron, A
Cruaud, P
Roussel, EG
Pignet, P
Caprais, JC
Callac, N
Ciobanu, MC
Godfroy, A
Cragg, BA
Parkes, JR
Van Nostrand, JD
He, ZL
Zhou, JZ
Toffin, L
AF Vigneron, Adrien
Cruaud, Perrine
Roussel, Erwan G.
Pignet, Patricia
Caprais, Jean-Claude
Callac, Nolwenn
Ciobanu, Maria-Cristina
Godfroy, Anne
Cragg, Barry A.
Parkes, John R.
Van Nostrand, Joy D.
He, Zhili
Zhou, Jizhong
Toffin, Laurent
TI Phylogenetic and Functional Diversity of Microbial Communities
Associated with Subsurface Sediments of the Sonora Margin, Guaymas Basin
SO PLOS ONE
LA English
DT Article
ID DEEP SUBSEAFLOOR SEDIMENTS; MARINE-SEDIMENTS; SEA-FLOOR; ARCHAEAL
COMMUNITIES; GROWTH-RATE; GULF; RNA; CALIFORNIA; BIOSPHERE; NITROGEN
AB Subsurface sediments of the Sonora Margin (Guayma Basin), located in proximity of active cold seep sites were explored. The taxonomic and functional diversity of bacterial and archaeal communities were investigated from 1 to 10 meters below the seafloor. Microbial community structure and abundance and distribution of dominant populations were assessed using complementary molecular approaches (Ribosomal Intergenic Spacer Analysis, 16S rRNA libraries and quantitative PCR with an extensive primers set) and correlated to comprehensive geochemical data. Moreover the metabolic potentials and functional traits of the microbial community were also identified using the GeoChip functional gene microarray and metabolic rates. The active microbial community structure in the Sonora Margin sediments was related to deep subsurface ecosystems (Marine Benthic Groups B and D, Miscellaneous Crenarchaeotal Group, Chloroflexi and Candidate divisions) and remained relatively similar throughout the sediment section, despite defined biogeochemical gradients. However, relative abundances of bacterial and archaeal dominant lineages were significantly correlated with organic carbon quantity and origin. Consistently, metabolic pathways for the degradation and assimilation of this organic carbon as well as genetic potentials for the transformation of detrital organic matters, hydrocarbons and recalcitrant substrates were detected, suggesting that chemoorganotrophic microorganisms may dominate the microbial community of the Sonora Margin subsurface sediments.
C1 [Vigneron, Adrien; Cruaud, Perrine; Pignet, Patricia; Callac, Nolwenn; Godfroy, Anne; Toffin, Laurent] IFREMER, Lab Microbiol Environm Extremes, UMR6197, Plouzane, France.
[Vigneron, Adrien; Cruaud, Perrine; Pignet, Patricia; Callac, Nolwenn; Godfroy, Anne; Toffin, Laurent] Univ Bretagne Occidentale, Lab Microbiol Environm Extremes, UMR6197, Plouzane, France.
[Vigneron, Adrien; Cruaud, Perrine; Pignet, Patricia; Callac, Nolwenn; Godfroy, Anne; Toffin, Laurent] CNRS, Lab Microbiol Environm Extremes, UMR6197, Plouzane, France.
[Caprais, Jean-Claude] IFREMER, Lab Etud Environm Profonds, UMR6197, Plouzane, France.
[Callac, Nolwenn] Univ Brest, Domaines Ocean IUEM, UMR6538, Plouzane, France.
[Ciobanu, Maria-Cristina] IFREMER, Geosci Marines, Lab Environm Sedimentaires, Plouzane, France.
[Roussel, Erwan G.; Cragg, Barry A.; Parkes, John R.] Cardiff Univ, Sch Earth & Ocean Sci, Cardiff CF10 3AX, S Glam, Wales.
[Van Nostrand, Joy D.; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.
[Van Nostrand, Joy D.; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA.
[Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China.
[Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Vigneron, A (reprint author), IFREMER, Lab Microbiol Environm Extremes, UMR6197, Plouzane, France.
EM avignero@gmail.com
RI Cragg, Barry/D-2690-2009; Van Nostrand, Joy/F-1740-2016;
OI Van Nostrand, Joy/0000-0001-9548-6450; Roussel,
Erwan/0000-0002-8735-5597; Callac, Nolwenn/0000-0002-7578-3455
FU IFREMER; IFREMER PhD grant
FX The oceanographic cruise and this study was funded by IFREMER and a
IFREMER PhD grant. The funders had no role in study design, data
collection and analysis, decision to publish, or preparation of the
manuscript.
NR 65
TC 11
Z9 11
U1 5
U2 72
PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1932-6203
J9 PLOS ONE
JI PLoS One
PD AUG 6
PY 2014
VL 9
IS 8
AR e104427
DI 10.1371/journal.pone.0104427
PG 11
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM6SM
UT WOS:000339995100071
PM 25099369
ER
PT J
AU Li, XJ
Peng, ZL
Lei, H
Dao, M
Karniadakis, GE
AF Li, Xuejin
Peng, Zhangli
Lei, Huan
Dao, Ming
Karniadakis, George Em
TI Probing red blood cell mechanics, rheology and dynamics with a
two-component multi-scale model
SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL
AND ENGINEERING SCIENCES
LA English
DT Article
DE red blood cell; multi-scale modelling; dissipative particle dynamics
ID DISSIPATIVE PARTICLE DYNAMICS; SHEAR-FLOW; MESOSCOPIC SIMULATION;
LIPID-BILAYER; MEMBRANE; DEFORMATION; ERYTHROCYTE; VISCOSITY; VESICLES;
MOTION
AB This study is partially motivated by the validation of a new two-component multi-scale cell model we developed recently that treats the lipid bilayer and the cytoskeleton as two distinct components. Here, the whole cell model is validated and compared against several available experiments that examine red blood cell (RBC) mechanics, rheology and dynamics. First, we investigated RBC deformability in a microfluidic channel with a very small cross-sectional area and quantified the mechanical properties of the RBC membrane. Second, we simulated twisting torque cytometry and compared predicted rheological properties of the RBC membrane with experimental measurements. Finally, we modelled the tank-treading (TT) motion of a RBC in a shear flow and explored the effect of channel width variation on the TT frequency. We also investigated the effects of bilayer-cytoskeletal interactions on these experiments and our simulations clearly indicated that they play key roles in the determination of cell membrane mechanical, rheological and dynamical properties. These simulations serve as validation tests and moreover reveal the capabilities and limitations of the new whole cell model.
C1 [Li, Xuejin; Karniadakis, George Em] Brown Univ, Div Appl Math, Providence, RI 02912 USA.
[Peng, Zhangli; Dao, Ming] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.
[Lei, Huan] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99354 USA.
RP Karniadakis, GE (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA.
EM george_karniadakis@brown.edu
RI Dao, Ming/B-1602-2008; Li, Xuejin/B-8559-2009; Peng, Zhangli/N-7284-2016
OI Li, Xuejin/0000-0002-4446-2480;
FU National Institutes of Health (NIH) grant [U01HL114476]; new DOE
Collaboratory on Mathematics for Mesoscopic Modeling of Materials (CM4)
FX This work is supported by the National Institutes of Health (NIH) grant
no. U01HL114476 and the new DOE Collaboratory on Mathematics for
Mesoscopic Modeling of Materials (CM4).
NR 37
TC 15
Z9 15
U1 3
U2 36
PU ROYAL SOC
PI LONDON
PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND
SN 1364-503X
EI 1471-2962
J9 PHILOS T R SOC A
JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci.
PD AUG 6
PY 2014
VL 372
IS 2021
SI SI
AR 20130389
DI 10.1098/rsta.2013.0389
PG 17
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AL0VH
UT WOS:000338844500011
ER
PT J
AU Mahadevan, VS
Merzari, E
Tautges, T
Jain, R
Obabko, A
Smith, M
Fischer, P
AF Mahadevan, Vijay S.
Merzari, Elia
Tautges, Timothy
Jain, Rajeev
Obabko, Aleksandr
Smith, Michael
Fischer, Paul
TI High-resolution coupled physics solvers for analysing fine-scale nuclear
reactor design problems
SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL
AND ENGINEERING SCIENCES
LA English
DT Article
DE multi-physics; reactor analysis; code coupling
ID SPECTRAL ELEMENT SOLUTION; TIME-INTEGRATION METHODS; MULTIPHYSICS
SIMULATIONS; EQUATIONS; DIFFUSION; SYSTEMS
AB An integrated multi-physics simulation capability for the design and analysis of current and future nuclear reactor models is being investigated, to tightly couple neutron transport and thermal-hydraulics physics under the SHARP framework. Over several years, high-fidelity, validated monophysics solvers with proven scalability on petascale architectures have been developed independently. Based on a unified component-based architecture, these existing codes can be coupled with a mesh-data backplane and a flexible coupling-strategy-based driver suite to produce a viable tool for analysts. The goal of the SHARP framework is to perform fully resolved coupled physics analysis of a reactor on heterogeneous geometry, in order to reduce the overall numerical uncertainty while leveraging available computational resources. The coupling methodology and software interfaces of the framework are presented, along with verification studies on two representative fast sodium-cooled reactor demonstration problems to prove the usability of the SHARP framework.
C1 [Mahadevan, Vijay S.; Merzari, Elia; Tautges, Timothy; Jain, Rajeev; Obabko, Aleksandr; Smith, Michael; Fischer, Paul] Argonne Natl Lab, Argonne, IL 60439 USA.
RP Mahadevan, VS (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM mahadevan@anl.gov
OI Mahadevan, Vijay/0000-0002-3337-2607
FU Nuclear Energy Advanced Modeling and Simulation (NEAMS) programme of the
US Department of Energy Office of Nuclear Energy [DE-AC02-06CH11357]
FX This work was completed as part of the SHARP reactor performance and
safety code suite development project, which is funded under the
auspices of the Nuclear Energy Advanced Modeling and Simulation (NEAMS)
programme of the US Department of Energy Office of Nuclear Energy, under
contract DE-AC02-06CH11357.
NR 43
TC 5
Z9 5
U1 0
U2 4
PU ROYAL SOC
PI LONDON
PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND
SN 1364-503X
EI 1471-2962
J9 PHILOS T R SOC A
JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci.
PD AUG 6
PY 2014
VL 372
IS 2021
SI SI
AR 20130381
DI 10.1098/rsta.2013.0381
PG 22
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AL0VH
UT WOS:000338844500005
ER
PT J
AU Baquero-Ruiz, M
Charman, AE
Fajans, J
Little, A
Povilus, A
Robicheaux, F
Wurtele, JS
Zhmoginov, AI
AF Baquero-Ruiz, M.
Charman, A. E.
Fajans, J.
Little, A.
Povilus, A.
Robicheaux, F.
Wurtele, J. S.
Zhmoginov, A. I.
TI Using stochastic acceleration to place experimental limits on the charge
of antihydrogen
SO NEW JOURNAL OF PHYSICS
LA English
DT Article
DE antihydrogen; charge anomaly; CPT
ID AUTORESONANT NONSTATIONARY EXCITATION; TRAPPED ANTIHYDROGEN; MAGNETIC
TRAP; SPECTROSCOPY; CONFINEMENT; ANTIPROTON; POSITRONS; GRAVITY; ATOMS
AB Assuming hydrogen is charge neutral, CPT invariance demands that antihydrogen also be charge neutral. Quantum anomaly cancellation also demands that antihydrogen be charge neutral. Standard techniques based on measurements of macroscopic quantities of atoms cannot be used to measure the charge of antihydrogen. In this paper, we describe how the application of randomly oscillating electric fields to a sample of trapped antihydrogen atoms, a form of stochastic acceleration, can be used to place experimental limits on this charge.
C1 [Baquero-Ruiz, M.; Charman, A. E.; Fajans, J.; Little, A.; Povilus, A.; Wurtele, J. S.; Zhmoginov, A. I.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Fajans, J.; Wurtele, J. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Robicheaux, F.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA.
RP Baquero-Ruiz, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
RI wurtele, Jonathan/J-6278-2016; Fajans, Joel/J-6597-2016
OI wurtele, Jonathan/0000-0001-8401-0297; Fajans, Joel/0000-0002-4403-6027
FU DOE, (USA); NSF, (USA); LBNL-LDRD (USA); CNPq, (Brazil); FINEP/RENAFAE
(Brazil); ISF (Israel); FNU (Denmark); VR (Sweden); NSERC, (Canada);
NRC/TRIUMF, (Canada); AITF, (Canada); FQRNT (Canada); EPSRC; Royal
Society; Leverhulme Trust (UK)
FX This work was supported by the DOE, NSF, LBNL-LDRD (USA); the
experimental data were acquired by the ALPHA collaboration with
additional support from: CNPq, FINEP/RENAFAE (Brazil); ISF (Israel); FNU
(Denmark); VR (Sweden); NSERC, NRC/TRIUMF, AITF, FQRNT (Canada); and
EPSRC, the Royal Society and the Leverhulme Trust (UK). The ALPHA
collaboration is grateful for the efforts of the CERN AD team, without
which the experimental data could not have been collected. This article
constitutes part of the PhD work of MB-R.
NR 37
TC 2
Z9 2
U1 0
U2 4
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1367-2630
J9 NEW J PHYS
JI New J. Phys.
PD AUG 5
PY 2014
VL 16
AR 083013
DI 10.1088/1367-2630/16/8/083013
PG 13
WC Physics, Multidisciplinary
SC Physics
GA AP2QD
UT WOS:000341917800004
ER
PT J
AU Dobrescu, BA
Frugiuele, C
AF Dobrescu, Bogdan A.
Frugiuele, Claudia
TI Hidden GeV-Scale Interactions of Quarks
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID GAUGE BOSON; BARYON NUMBER; SEARCH; COLLISIONS; LEPTONS; DECAYS; TEV
AB We explore quark interactions mediated by new gauge bosons of masses in the 0.3-50 GeV range. A tight upper limit on the gauge coupling of light Z' bosons is imposed by the anomaly cancellation conditions in conjunction with collider bounds on new charged fermions. Limits from quarkonium decays are model dependent, while electroweak constraints are mild. We derive the limits for a Z' boson coupled to baryon number and then construct a Z' model with relaxed constraints, allowing quark couplings as large as 0.2 for a mass of a few GeV.
C1 [Dobrescu, Bogdan A.; Frugiuele, Claudia] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA.
RP Dobrescu, BA (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA.
NR 35
TC 17
Z9 17
U1 0
U2 3
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 5
PY 2014
VL 113
IS 6
AR 061801
DI 10.1103/PhysRevLett.113.061801
PG 5
WC Physics, Multidisciplinary
SC Physics
GA AO3XC
UT WOS:000341269600003
PM 25148315
ER
PT J
AU Martinez, E
Caro, A
Beyerlein, IJ
AF Martinez, Enrique
Caro, Alfredo
Beyerlein, Irene J.
TI Atomistic modeling of defect-induced plasticity in CuNb nanocomposites
SO PHYSICAL REVIEW B
LA English
DT Article
ID STACKING-FAULT TETRAHEDRA; PRIMARY DAMAGE; DISLOCATION DYNAMICS;
MOLECULAR-DYNAMICS; INFREQUENT EVENTS; RADIATION-DAMAGE; TIME-SCALE;
CASCADES; IRRADIATION; COMPOSITES
AB CuNb nanocomposites have proven stable under light-ion irradiation, although their response to heavy-ion bombardment and subsequent loading is still uncertain. In this paper we analyze the change in mechanical properties of model CuNb nanocomposites in vacancy supersaturated environments, mimicking certain effects introduced by heavy-ion irradiation. We have performed compression tests using molecular dynamics for different defect contents. The presence of defects substantially modifies the system response upon external loading. The dislocation nucleation mechanism changes with the interface atomic density. Stacking fault tetrahedra in the Cu layer may act as dislocation sources to lower significantly the yield stress and the same applies for voids present in the Nb layer. We have analyzed in detail the dislocation-interface interaction mechanisms under different conditions, showing how dislocations react with the misfit dislocations present at the interface to modify the atomic structure of the boundary, which suggests that the interface could be designed to optimize its defect healing properties. We conclude that heavy-ion irradiation softens the multilayer nanocomposites and that interfaces help in recovering these materials as they absorb the dislocations created from irradiation-induced defects.
C1 [Martinez, Enrique; Caro, Alfredo] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
[Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Martinez, E (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST 8, Los Alamos, NM 87545 USA.
EM enriquem@lanl.gov
OI Martinez Saez, Enrique/0000-0002-2690-2622
FU Center for Materials at Irradiation and Mechanical Extremes, an Energy
Frontier Research Center - U.S. Department of Energy at Los Alamos
National Laboratory [2008LANL1026]
FX The authors thank J. P. Hirth, M. J. Demkowicz, and A. Misra for
exciting discussions. The authors also gratefully acknowledge the
support from the Center for Materials at Irradiation and Mechanical
Extremes, an Energy Frontier Research Center funded by the U.S.
Department of Energy (Grant No. 2008LANL1026) at Los Alamos National
Laboratory. Parallel computations were performed on the Lobo machine at
the High Performance Computing clusters at Los Alamos National
Laboratory.
NR 33
TC 9
Z9 9
U1 3
U2 32
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 5
PY 2014
VL 90
IS 5
AR 054103
DI 10.1103/PhysRevB.90.054103
PG 9
WC Physics, Condensed Matter
SC Physics
GA AO3SN
UT WOS:000341256100002
ER
PT J
AU Velizhanin, KA
Shahbazyan, TV
AF Velizhanin, Kirill A.
Shahbazyan, Tigran V.
TI Exciton-plasmaritons in graphene/semiconductor structures
SO PHYSICAL REVIEW B
LA English
DT Article
ID RELAXATION-TIME APPROXIMATION; LINDHARD DIELECTRIC FUNCTION;
SURFACE-PLASMON POLARITONS; GRAPHENE PLASMONICS; SEMICONDUCTORS;
DEVICES; ENERGY
AB We study strong coupling between plasmons in monolayer charge-doped graphene and excitons in a narrow gap semiconductor quantum well separated from graphene by a potential barrier. We show that the Coulomb interaction between excitons and plasmons results in mixed states described by a Hamiltonian similar to that for exciton-polaritons and derive the exciton-plasmon coupling constant that depends on system parameters. We calculate numerically the Rabi splitting of exciton-plasmariton dispersion branches for several semiconductor materials and find that it can reach values of up to 50-100 meV.
C1 [Velizhanin, Kirill A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Shahbazyan, Tigran V.] Jackson State Univ, Dept Phys, Jackson, MS 39217 USA.
RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM kirill@lanl.gov; shahbazyan@jsums.edu
RI Velizhanin, Kirill/C-4835-2008
FU NNSA of the US DOE at LANL [DE AC52-06NA25396]; NSF [DMR-1206975]
FX The authors would like to thank G. Khodaparast for a helpful discussion.
Work at LANL was performed under the NNSA of the US DOE at LANL under
Contract No. DE AC52-06NA25396. Work at JSU was supported by the NSF
under Grant No. DMR-1206975.
NR 56
TC 4
Z9 4
U1 3
U2 27
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 5
PY 2014
VL 90
IS 8
AR 085403
DI 10.1103/PhysRevB.90.085403
PG 9
WC Physics, Condensed Matter
SC Physics
GA AO3SV
UT WOS:000341257100003
ER
PT J
AU Yan, L
Ollitrault, JY
Poskanzer, AM
AF Yan, Li
Ollitrault, Jean-Yves
Poskanzer, Arthur M.
TI Eccentricity distributions in nucleus-nucleus collisions
SO PHYSICAL REVIEW C
LA English
DT Article
ID ELLIPTIC FLOW; AU+AU COLLISIONS; FLUCTUATIONS; PARTICLES
AB We propose a new parametrization of the distribution of the initial eccentricity in a nucleus-nucleus collision at a fixed centrality, which we name the elliptic power distribution. It is a two-parameter distribution, where one of the parameters corresponds to the intrinsic eccentricity, while the other parameter controls the magnitude of eccentricity fluctuations. Unlike the previously used Bessel-Gaussian distribution, which becomes worse for more peripheral collisions, the new elliptic power distribution fits several Monte Carlo models of the initial state for all centralities.
C1 [Yan, Li; Ollitrault, Jean-Yves] IPhT Inst Phys Theor Saclay, CNRS, URA2306, F-91191 Gif Sur Yvette, France.
[Poskanzer, Arthur M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Yan, L (reprint author), IPhT Inst Phys Theor Saclay, CNRS, URA2306, F-91191 Gif Sur Yvette, France.
FU European Research Council under the Advanced Investigator
[ERC-AD-267258]; Office of Science, of the US Department of Energy
FX We thank Hiroshi Masui for carrying out the Monte Carlo Glauber
calculations which inspired this work, Bjorn Schenke for the IP-Glasma
results, C. Loizides for the new version of the PHOBOS Glauber, M. Luzum
and S. Voloshin for extensive discussions and suggestions. In
particular, we thank S. Voloshin for suggesting the name elliptic power,
and for useful comments on the manuscript. J.Y.O. thanks the MIT LNS for
hospitality. L.Y. is funded by the European Research Council under the
Advanced Investigator Grant No. ERC-AD-267258. A.M.P. was supported by
the Director, Office of Science, of the US Department of Energy.
NR 54
TC 14
Z9 14
U1 0
U2 2
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0556-2813
EI 1089-490X
J9 PHYS REV C
JI Phys. Rev. C
PD AUG 5
PY 2014
VL 90
IS 2
AR 024903
DI 10.1103/PhysRevC.90.024903
PG 9
WC Physics, Nuclear
SC Physics
GA AO3UF
UT WOS:000341260900002
ER
PT J
AU Davoudiasl, H
Lewis, IM
AF Davoudiasl, Hooman
Lewis, Ian M.
TI Right-handed neutrinos as the origin of the electroweak scale
SO PHYSICAL REVIEW D
LA English
DT Article
ID DARK-MATTER; SYMMETRY-BREAKING; STANDARD MODEL; HIGGS-BOSON; MECHANISM;
LHC
AB The insular nature of the Standard Model may be explained if the Higgs mass parameter is only sensitive to quantum corrections from physical states. Starting from a scale-free electroweak sector at tree level, we postulate that quantum effects of heavy right-handed neutrinos induce a mass term for a scalar weak doublet that contains the dark matter particle. In turn, below the scale of heavy neutrinos, the dark matter sector sets the scale of the Higgs potential. We show that this framework can lead to a Higgs mass that respects physical naturalness, while also providing a viable scalar dark matter candidate, realistic light neutrino masses, and the baryon asymmetry of the Universe via thermal leptogenesis. The proposed scenario can remain perturbative and stable up to the Planck scale, thereby accommodating simple extensions to include a high-scale (similar to 2 x 10(16) GeV) inflationary sector, implied by recent measurements. In that case, our model typically predicts that the dark matter scalar is close to 1 TeV in mass and could be accessible in near future direct detection experiments.
C1 [Davoudiasl, Hooman; Lewis, Ian M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
FU United States Department of Energy [DE-AC02-98CH10886]
FX We thank P. Meade and A. Strumia for discussions. This work was
supported in part by the United States Department of Energy under Grant
Contract No. DE-AC02-98CH10886.
NR 54
TC 31
Z9 31
U1 0
U2 1
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0010
EI 2470-0029
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 5
PY 2014
VL 90
IS 3
AR 033003
DI 10.1103/PhysRevD.90.033003
PG 10
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA AO3US
UT WOS:000341262400001
ER
PT J
AU Vogel, T
Li, YW
Wust, T
Landau, DP
AF Vogel, Thomas
Li, Ying Wai
Wuest, Thomas
Landau, David P.
TI Scalable replica-exchange framework for Wang-Landau sampling
SO PHYSICAL REVIEW E
LA English
DT Article
ID MONTE-CARLO METHOD; DENSITY-OF-STATES; PARALLEL IMPLEMENTATION;
PHASE-TRANSITIONS; POTTS-MODEL; RANDOM-WALK; FREE-ENERGY; SIMULATIONS;
ALGORITHM; PROTEINS
AB We investigate a generic, parallel replica-exchange framework for Monte Carlo simulations based on the Wang-Landau method. To demonstrate its advantages and general applicability for massively parallel simulations of complex systems, we apply it to lattice spin models, the self-assembly process in amphiphilic solutions, and the adsorption of molecules on surfaces. While of general current interest, the latter phenomena are challenging to study computationally because of multiple structural transitions occurring over a broad temperature range. We show how the parallel framework facilitates simulations of such processes and, without any loss of accuracy or precision, gives a significant speedup and allows for the study of much larger systems and much wider temperature ranges than possible with single-walker methods.
C1 [Vogel, Thomas; Landau, David P.] Univ Georgia, Ctr Simulat Phys, Athens, GA 30602 USA.
[Li, Ying Wai] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA.
[Wuest, Thomas] ETH, IT Serv, Sci IT Serv, CH-8092 Zurich, Switzerland.
RP Vogel, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM thomasvogel@physast.uga.edu
FU National Science Foundation [DMR-0810223, OCI-0904685]; Office of
Advanced Scientific Computing Research; U.S. Department of Energy;
UT-Battelle, LLC [De-AC05-00OR22725]; TACC under XSEDE [PHY130009]
FX This work has been supported by the National Science Foundation under
Grants No. DMR-0810223 and No. OCI-0904685. Y. W. Li was partly
sponsored by the Office of Advanced Scientific Computing Research; U.S.
Department of Energy. Part of the work was performed at the Oak Ridge
Leadership Computing Facility at ORNL, which is managed by UT-Battelle,
LLC under Contract No. De-AC05-00OR22725. Supercomputer time was
provided by TACC under XSEDE Grant No. PHY130009. LA-UR-13-29579
assigned.
NR 63
TC 16
Z9 16
U1 1
U2 14
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 2470-0045
EI 2470-0053
J9 PHYS REV E
JI Phys. Rev. E
PD AUG 5
PY 2014
VL 90
IS 2
AR 023302
DI 10.1103/PhysRevE.90.023302
PG 12
WC Physics, Fluids & Plasmas; Physics, Mathematical
SC Physics
GA AO3WA
UT WOS:000341266300008
PM 25215846
ER
PT J
AU He, HK
Averick, S
Roth, E
Luebke, D
Nulwala, H
Matyjaszewski, K
AF He, Hongkun
Averick, Saadyah
Roth, Elliot
Luebke, David
Nulwala, Hunaid
Matyjaszewski, Krzysztof
TI Clickable poly(ionic liquid)s for modification of glass and silicon
surfaces
SO POLYMER
LA English
DT Article
DE Poly(ionic liquid)s; ATRP; Click chemistry
ID TRANSFER RADICAL POLYMERIZATION; BLOCK-COPOLYMERS; POLY(ETHYLENE
GLYCOL); NITRENE CHEMISTRY; CARBON NANOTUBES; IONIC LIQUIDS; POLYMERS;
THIOL; BRUSHES; ATRP
AB Covalent attachment of poly(ionic liquid)s (PILs) by click chemistry on glass or silicon (Si) surfaces was performed. Poly[1-(4-vinylbenzyl)-3-butylimidazolium bis(trifluorcimethylsulfonyl)imide] (poly-VBBI+Tf2N-), and copolymers of polyVBBI(+)Tf(2)N(-) with fluorescein O-methacrylate were synthesized by conducting an atom transfer radical polymerization (ATRP) from initiators containing azide or thioacetate groups. The azide- and thiol-terminated PILs were then successfully grafted onto alkyne and alkene modified glass/Si wafers by thermal azide-alkyne cycloaddition and photoinitiated thiol-ene click reactions, respectively. The modified surfaces were characterized by contact angle measurements and ellipsometry. The fluorescent PIL functionalized surfaces showed strong fluorescence under UV irradiation. This procedure of tethering PILs to substrates also provides an easy way to change the surface hydrophilicity by replacing the anions in the grafted PILs. The present approach could be readily applied for surface modifications with other types of PILs or their copolymers to achieve different functionalities on various surfaces. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [He, Hongkun; Averick, Saadyah; Nulwala, Hunaid; Matyjaszewski, Krzysztof] Carnegie Mellon Univ, Dept Chem, Ctr Macromol Engn, Pittsburgh, PA 15213 USA.
[He, Hongkun; Roth, Elliot; Luebke, David; Nulwala, Hunaid; Matyjaszewski, Krzysztof] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
RP Nulwala, H (reprint author), Carnegie Mellon Univ, Dept Chem, Ctr Macromol Engn, 4400 Fifth Ave, Pittsburgh, PA 15213 USA.
EM hnulwala@andrew.cmu.edu; km3b@andrew.cmu.edu
RI He, Hongkun/B-4759-2011; Matyjaszewski, Krzysztof/A-2508-2008; Averick,
Saadyah/A-9999-2015;
OI He, Hongkun/0000-0002-7214-3313; Matyjaszewski,
Krzysztof/0000-0003-1960-3402; Nulwala, Hunaid/0000-0001-7481-3723
FU NSF support [CHE-1039870, DMR-0969301]; DoE support [ER-45998]; U.S.
Department of Energy's National Energy Technology Laboratory
[DE-FE0004000]
FX NSF support (CHE-1039870 and DMR-0969301) and DoE support (ER-45998) is
acknowledged. This technical effort was also performed in support of
U.S. Department of Energy's National Energy Technology Laboratory's
on-going research on CO2 capture under the contract
DE-FE0004000.
NR 89
TC 16
Z9 16
U1 13
U2 125
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0032-3861
EI 1873-2291
J9 POLYMER
JI Polymer
PD AUG 5
PY 2014
VL 55
IS 16
SI SI
BP 3330
EP 3338
DI 10.1016/j.polymer.2014.01.045
PG 9
WC Polymer Science
SC Polymer Science
GA AN7WS
UT WOS:000340812300007
ER
PT J
AU Brombosz, SM
Seifert, S
Firestone, MA
AF Brombosz, Scott M.
Seifert, Soenke
Firestone, Millicent A.
TI Patterning a pi-conjugated polyelectrolyte through sequential
polymerization of a bifunctional ionic liquid monomer
SO POLYMER
LA English
DT Article
DE pi-Conjugated polyelectrolyte; Ionic liquid; Sequential polymerization
ID OPTICAL-PROPERTIES; OXIDATIVE POLYMERIZATION; ORGANIC BIOELECTRONICS;
CARBON NANOTUBES; FILMS; COMPOSITES; POLYTHIOPHENE; MULTILAYERS;
DERIVATIVES; COMPLEXES
AB An electronically conductive polyelectrolyte is prepared by the sequential polymerization of a bifunctional imidazolium-based ionic liquid (IL) monomer, composed of a thienyl and vinyl containing cation paired with a tetrafluoroborate anion. In the first step, potentiodynamic electropolymerization of the thienyl moiety forms a cationic polyalkylthiophene that is soluble in select organic solvents. Cyclic voltammetry (CV) was used to determine the polymer p-doping potential (0.31 V) and the bipolaronic state (1.49 V). The polymer exhibits electrochromism, converting from red in the neutral state (lambda(max) = 443 nm) to dark blue in the polaronic state (lambda(max) = 819 nm). The solution-processable polymer can be cast into a film, masked and patterned by UV-initiated free radical polymerization of the vinyl moiety. Small-angle X-ray scattering (SAXS) revealed that the insoluble crosslinked polyalkylthiophene-polyvinylimidazolium adopts a lamellar structure with a lattice spacing of 3.3 nm. Four-probe d.c. conductivity measurements determined the de-doped electrical conductivity was 1.0 x 10(-2) S/cm. The results underscore the importance of the anion in controlling the polymerization of IL monomers. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Brombosz, Scott M.; Seifert, Soenke] Argonne Natl Lab, Argonne, IL 60439 USA.
[Firestone, Millicent A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
RP Firestone, MA (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663,MS K771, Los Alamos, NM 87545 USA.
EM firestone@lanl.gov
FU U.S. Department of Energy, Center for Integrated Nanotechnologies, at
Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National
Laboratories [DE-AC04-94AL85000]; Office of Basic Energy Sciences,
Division of Materials Sciences, U.S. Department of Energy
[DE-AC02-06CH11357]
FX This work was performed in part at the U.S. Department of Energy, Center
for Integrated Nanotechnologies, at Los Alamos National Laboratory
(Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract
DE-AC04-94AL85000). The efforts of SMB and SS were supported by the
Office of Basic Energy Sciences, Division of Materials Sciences, U.S.
Department of Energy under Contract No. DE-AC02-06CH11357 to the
UChicago, LLC.
NR 47
TC 9
Z9 9
U1 3
U2 46
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0032-3861
EI 1873-2291
J9 POLYMER
JI Polymer
PD AUG 5
PY 2014
VL 55
IS 16
SI SI
BP 3370
EP 3377
DI 10.1016/j.polymer.2014.04.049
PG 8
WC Polymer Science
SC Polymer Science
GA AN7WS
UT WOS:000340812300011
ER
PT J
AU Wang, YY
Fan, F
Agapov, AL
Saito, T
Yang, J
Yu, X
Hong, KL
Mays, J
Sokolov, AP
AF Wang, Yangyang
Fan, Fei
Agapov, Alexander L.
Saito, Tomonori
Yang, Jun
Yu, Xiang
Hong, Kunlun
Mays, Jimmy
Sokolov, Alexei P.
TI Examination of the fundamental relation between ionic transport and
segmental relaxation in polymer electrolytes
SO POLYMER
LA English
DT Article
DE Polymer electrolytes; Ionic transport; Decoupling
ID POLYCRYSTALLINE SOLID ELECTROLYTES; WALDEN PLOT ANALYSIS; DIELECTRIC
FRICTION; MICROPHASE SEPARATION; LITHIUM BATTERIES; MOLECULAR THEORY;
LIQUID-STATE; MOVING ION; CONDUCTIVITY; GLASSES
AB Replacing traditional liquid electrolytes by polymers will significantly improve electrical energy storage technologies. Despite significant advantages for applications in electrochemical devices, the use of solid polymer electrolytes is strongly limited by their poor ionic conductivity. The classical theory predicts that the ionic transport is dictated by the segmental motion of the polymer matrix. As a result, the low mobility of polymer segments is often regarded as the limiting factor for development of polymers with sufficiently high ionic conductivity. Here, we show that the ionic conductivity in many polymers can be strongly decoupled from their segmental dynamics, in terms of both temperature dependence and relative transport rate. Based on this principle, we developed several polymers with "superionic" conductivity. The observed fast ion transport suggests a fundamental difference between the ionic transport mechanisms in polymers and small molecules and provides a new paradigm for design of highly conductive polymer electrolytes. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Wang, Yangyang; Fan, Fei; Agapov, Alexander L.; Mays, Jimmy; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
[Saito, Tomonori; Yu, Xiang; Mays, Jimmy; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[Yang, Jun; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Wang, YY (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
EM yywang@utk.edu
RI Hong, Kunlun/E-9787-2015; Wang, Yangyang/A-5925-2010; Saito,
Tomonori/M-1735-2016
OI Hong, Kunlun/0000-0002-2852-5111; Wang, Yangyang/0000-0001-7042-9804;
Saito, Tomonori/0000-0002-4536-7530
FU Division of Materials Science and Engineering, U.S. Department of
Energy, Office of Basic Energy Sciences; NSF Polymer Program
[DMR-1104824]; Center for Nanophase Materials Sciences, at Oak Ridge
National Laboratory; Scientific User Facilities Division, Office of
Basic Energy Sciences, U.S. Department of Energy
FX The authors thank Dr. M. Nakanishi for providing the data of electrical
conductivity of the lithium chloride solution. T.S., J.M. and A.P.S.
acknowledge the financial support from the Division of Materials Science
and Engineering, U.S. Department of Energy, Office of Basic Energy
Sciences. The polymer synthesis was partly conducted at the Center for
Nanophase Materials Sciences, which is sponsored at Oak Ridge National
Laboratory by the Scientific User Facilities Division, Office of Basic
Energy Sciences, U.S. Department of Energy. F.F. thanks the NSF Polymer
Program (DMR-1104824) for funding.
NR 96
TC 22
Z9 22
U1 11
U2 75
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0032-3861
EI 1873-2291
J9 POLYMER
JI Polymer
PD AUG 5
PY 2014
VL 55
IS 16
SI SI
BP 4067
EP 4076
DI 10.1016/j.polymer.2014.06.085
PG 10
WC Polymer Science
SC Polymer Science
GA AN7WS
UT WOS:000340812300089
ER
PT J
AU Matsuda, Y
Fukatsu, A
Wang, YY
Miyamoto, K
Mays, JW
Tasaka, S
AF Matsuda, Yasuhiro
Fukatsu, Akinobu
Wang, Yangyang
Miyamoto, Kazuaki
Mays, Jimmy W.
Tasaka, Shigeru
TI Fabrication and characterization of poly(L-lactic acid) gels induced by
fibrous complex crystallization with solvents
SO POLYMER
LA English
DT Article
DE Poly(L-lactic acid); Complex crystal; Gelation
ID CRYSTAL-STRUCTURE; SYNDIOTACTIC POLYSTYRENE; INCLUSION-COMPOUNDS;
ALPHA-FORM; X-RAY; THERMOREVERSIBLE GELATION; INFRARED-SPECTROSCOPY;
CONFORMATION; MORPHOLOGY; BEHAVIOR
AB Complex crystal induced gelation of poly(L-lactic acid) (PLLA) solutions was studied for a series of solvents, including N,N-dimethylformamide (DMF). By cooling the solutions prepared at elevated temperatures, PLEA gels were produced in solvents that induced complex crystals (epsilon-crystals) with PLEA. Fibrous structure of PLEA in the gel with DMF was observed by polarizing optical microscopy, field emission electron microscopy, and atomic force microscopy. Upon heating, the crystal form of PLEA in the DMF gel changed from epsilon-crystal to alpha-crystal, the major crystal form in common untreated PLEA films, but the morphology and high elastic modulus of the gel remained until the alpha-crystal dissolved at higher temperature. In addition, a solvent exchanging method was developed, which allowed PLEA gels to be prepared in other useful solvents that do not induce epsilon-crystals without losing the morphology and mechanical properties. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Matsuda, Yasuhiro; Fukatsu, Akinobu; Miyamoto, Kazuaki; Tasaka, Shigeru] Shizuoka Univ, Dept Appl Chem & Biochem Engn, Naka Ku, Hamamatsu, Shizuoka, Japan.
[Wang, Yangyang; Mays, Jimmy W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
[Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.
RP Matsuda, Y (reprint author), Shizuoka Univ, Dept Appl Chem & Biochem Engn, Naka Ku, 3-5-1 Johoku, Hamamatsu, Shizuoka, Japan.
EM tymatud@ipc.shizuoka.ac.jp
RI Wang, Yangyang/A-5925-2010
OI Wang, Yangyang/0000-0001-7042-9804
FU US Department of Energy, Basic Energy Sciences, Division of Materials
Sciences and Engineering [ERKCC02]; Ministry of Education, Culture,
Science, Sports and Technology of Japan [26870245]
FX YYW and JWM acknowledge the financial support by the US Department of
Energy, Basic Energy Sciences, Division of Materials Sciences and
Engineering (ERKCC02).; This work is partially supported by a Grant-in
Aid for Young Scientists (B) (26870245) from the Ministry of Education,
Culture, Science, Sports and Technology of Japan.
NR 37
TC 4
Z9 4
U1 1
U2 17
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0032-3861
EI 1873-2291
J9 POLYMER
JI Polymer
PD AUG 5
PY 2014
VL 55
IS 16
SI SI
BP 4369
EP 4378
DI 10.1016/j.polymer.2014.06.086
PG 10
WC Polymer Science
SC Polymer Science
GA AN7WS
UT WOS:000340812300120
ER
PT J
AU Kesava, SV
Fei, ZP
Rimshaw, AD
Wang, C
Hexemer, A
Asbury, JB
Heeney, M
Gomez, ED
AF Kesava, Sameer Vajjala
Fei, Zhuping
Rimshaw, Adam D.
Wang, Cheng
Hexemer, Alexander
Asbury, John B.
Heeney, Martin
Gomez, Enrique D.
TI Domain Compositions and Fullerene Aggregation Govern Charge
Photogeneration in Polymer/Fullerene Solar Cells
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID X-RAY-SCATTERING; CONJUGATED-POLYMER BLENDS; SMALL-ANGLE; EXCITON
DIFFUSION; MORPHOLOGY; SEPARATION; EFFICIENCY; DISSOCIATION;
MISCIBILITY; PERFORMANCE
AB The complex microstructure of organic semiconductor mixtures continues to obscure the connection between the active layer morphology and photovoltaic device performance. For example, the ubiquitous presence of mixed phases in the active layer of polymer/fullerene solar cells creates multiple morphologically distinct interfaces which are capable of exciton dissociation or charge recombination. Here, it is shown that domain compositions and fullerene aggregation can strongly modulate charge photogeneration at ultrafast timescales through studies of a model system, mixtures of a low band-gap polymer, poly[(4,4'-bis(2-ethylhexyl) dithieno[3,2-b:2',3'-d] germole)-2,6-diyl-alt-(2,1,3-benzothia-diazole)-4,7-diyl], and [6,6]w-phenyl-C-71-butyric acid methyl ester. Structural characterization using energyfiltered transmission electron microscopy (EFTEM) and resonant soft X-ray scattering shows similar microstructures even with changes in the overall film composition. Composition maps generated from EFTEM, however, demonstrate that compositions of mixed domains vary significantly with overall film composition. Furthermore, the amount of polymer in the mixed domains is inversely correlated with device performance. Photoinduced absorption studies using ultrafast infrared spectroscopy demonstrate that polaron concentrations are highest when mixed domains contain the least polymer. Grazing-incidence X-ray scattering results show that larger fullerene coherence lengths are correlated to higher polaron yields. Thus, the purity of the mixed domains is critical for efficient charge photogeneration because purity modulates fullerene aggregation and electron delocalization.
C1 [Kesava, Sameer Vajjala; Gomez, Enrique D.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA.
[Fei, Zhuping; Heeney, Martin] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England.
[Fei, Zhuping; Heeney, Martin] Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England.
[Rimshaw, Adam D.; Asbury, John B.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA.
[Wang, Cheng; Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Gomez, Enrique D.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA.
RP Gomez, ED (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA.
EM edg12@psu.edu
RI Foundry, Molecular/G-9968-2014; Wang, Cheng/A-9815-2014;
OI Fei, Zhuping/0000-0002-2160-9136; Heeney, Martin/0000-0001-6879-5020
FU NSF [DMR-1056199]; National Science Foundation [CHE-0846241]; Office of
Naval Research [N00014-11-1-0239]; U.S. Department of Energy
[DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences,
of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-06CH11357]
FX Major funding for this work was provided by NSF under Grant No.
DMR-1056199. A.D.R. and J.B.A. gratefully acknowledge support for this
research from the National Science Foundation under Grant No.
CHE-0846241 and partial support from the Office of Naval Research under
Grant No. N00014-11-1-0239. The authors gratefully acknowledge the Penn
Regional Nanotechnology Facility, University of Pennsylvania and the
National Center for Electron Microscopy, Lawrence Berkeley National
Laboratory, which is supported by the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231 for TEM access. The authors also
acknowledge the Advanced Light Source, Lawrence Berkeley National
Laboratory, which is supported by the Director, Office of Science,
Office of Basic Energy Sciences, of the U.S. Department of Energy under
Contract No. DE-AC02-05CH11231 and Advanced Photon Source, Argonne
National Laboratory, which is supported by the U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences, under
Contract No. DE-AC02-06CH11357. The authors further thank Dr. Susan
Trolier-McKinstry and Dr. Janna Maranas for use of the spectroscopic
ellipsometer and differential scanning calorimeter, respectively.
NR 73
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Z9 34
U1 0
U2 69
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD AUG 5
PY 2014
VL 4
IS 11
AR 1400116
DI 10.1002/aenm.201400116
PG 10
WC Chemistry, Physical; Energy & Fuels; Materials Science,
Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AN3ZH
UT WOS:000340526900019
ER
PT J
AU Owczarczyk, ZR
Braunecker, WA
Oosterhout, SD
Kopidakis, N
Larsen, RE
Ginley, DS
Olson, DC
AF Owczarczyk, Zbyslaw R.
Braunecker, Wade A.
Oosterhout, Stefan D.
Kopidakis, Nikos
Larsen, Ross E.
Ginley, David S.
Olson, Dana C.
TI Cyclopenta[c]thiophene-4,6-dione-Based Copolymers as Organic
Photovoltaic Donor Materials
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID HETEROJUNCTION SOLAR-CELLS; CONJUGATED POLYMERS; MOLECULAR-WEIGHT;
MICROWAVE CONDUCTIVITY; CONVERSION EFFICIENCY; PERFORMANCE; CHARGE;
POLY(3-HEXYLTHIOPHENE); BLENDS; NANOPARTICLES
AB A class of "push-pull" conjugated copolymers based on cyclopenta[c] thiophene-4,6-dione (CTD) and benzodithiophene (BDT) is synthesized for application as an electron donor in organic photovoltaics (OPV). Given the diverse electronic and structural tunability of the CTD unit, specific CTD-containing copolymers are chosen with the aid of theoretical calculations from a broad array of potential candidate materials. Evaluation of the chosen materials as OPV absorbers includes characterization of the optical, electronic, and structural properties of the polymer films using UV-vis absorbance, photoluminescence, cyclic voltammetry, and X-ray diffraction techniques. In addition, the contactless time-resolved microwave conductivity (TRMC) technique is used to measure the photoconductance of polymer/fullerene blends. Excellent correlation between measured photoconductance and OPV device efficiency is demonstrated with these materials and TRMC is discussed as a tool for screening potential active layer materials for OPV devices.
C1 [Owczarczyk, Zbyslaw R.; Braunecker, Wade A.; Oosterhout, Stefan D.; Kopidakis, Nikos; Larsen, Ross E.; Ginley, David S.; Olson, Dana C.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Owczarczyk, ZR (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM zbyslaw.owczarczyk@nrel.gov; wade.braunecker@nrel.gov
RI Larsen, Ross/E-4225-2010; Kopidakis, Nikos/N-4777-2015
OI Larsen, Ross/0000-0002-2928-9835;
FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable
Energy Laboratory through the DOE SETP program
FX This work was supported by the U.S. Department of Energy under Contract
No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory
through the DOE SETP program.
NR 53
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Z9 7
U1 1
U2 35
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD AUG 5
PY 2014
VL 4
IS 11
AR 1301821
DI 10.1002/aenm.201301821
PG 9
WC Chemistry, Physical; Energy & Fuels; Materials Science,
Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AN3ZH
UT WOS:000340526900005
ER
PT J
AU Widjonarko, NE
Schulz, P
Parilla, PA
Perkins, CL
Ndione, PF
Sigdel, AK
Olson, DC
Ginley, DS
Kahn, A
Toney, MF
Berry, JJ
AF Widjonarko, N. Edwin
Schulz, Philip
Parilla, Philip A.
Perkins, Craig L.
Ndione, Paul F.
Sigdel, Ajaya K.
Olson, Dana C.
Ginley, David S.
Kahn, Antoine
Toney, Michael F.
Berry, Joseph J.
TI Impact of Hole Transport Layer Surface Properties on the Morphology of a
Polymer-Fullerene Bulk Heterojunction
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID ORGANIC SOLAR-CELLS; PHOTOVOLTAIC DEVICES; LOW-TEMPERATURE;
NICKEL-OXIDE; FREE-ENERGY; X-RAY; FILMS; THIN; CONTACT; BLENDS
AB Investigations on the impact of interfacial modification on organic optoelectronic device performance often attribute the improved device performance to the optoelectronic properties of the modifier. A critical assumption of such conclusions is that the organic active layer deposited on top of the modified surface (interface) remains unaltered. Here the validity of this assumption is investigated by examining the impact of substrate surface properties on the morphology of poly(3-hexylthiophene): 1-(3-methoxycarbonyl)-propyl-1-phenyl-[6,6]C-61 (P3HT: PCBM) bulk-heterojunction (BHJ). A set of four nickel oxide and poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PEDOT:PSS) hole transport layers (HTL) with contrasting surface properties and performance in organic photovoltaic (OPV) devices is studied. Differences in vertical composition variation and structural morphologies are observed across the samples, but only in the near-interface region of less than or similar to 20 nm. Near-interface differences in morphology are most closely correlated with surface polarity and surface roughness of the HTL. Surface polarity is more influenced by surface composition than surface roughness and crystal structure. These findings corroborate the previously mentioned conclusions that the differences in device performance observed in solar cells employing these HTLs are dominated by the electronic properties of the HTL/organic photoactive active layer interface and not by unintentional alteration in the BHJ active layer morphology.
C1 [Widjonarko, N. Edwin] Univ Colorado, Dept Phys, Boulder, CO 80309 USA.
[Widjonarko, N. Edwin; Parilla, Philip A.; Perkins, Craig L.; Ndione, Paul F.; Sigdel, Ajaya K.; Olson, Dana C.; Ginley, David S.; Berry, Joseph J.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Sigdel, Ajaya K.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA.
[Schulz, Philip; Kahn, Antoine] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA.
[Toney, Michael F.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA.
RP Widjonarko, NE (reprint author), Univ Colorado, Dept Phys, 390 UCB, Boulder, CO 80309 USA.
EM nicodemus.widjonarko@colorado.edu; joe.berry@nrel.gov
RI Schulz, Philip/N-2295-2015; Ndione, Paul/O-6152-2015
OI Schulz, Philip/0000-0002-8177-0108; Ndione, Paul/0000-0003-4444-2938
FU Center for Interface Science: Solar Electric Materials (CISSEM), an
Energy Frontier Research Center - U.S. Department of Energy, Office of
Science, Basic Energy Sciences, U.S. Department of Energy Award
[DE-SC0001084]; Center for Energy Efficent Materials (CEEM), an Energy
Frontier Research Center - U.S. Department of Energy, Office of Science,
Basic Energy Sciences, U.S. Department of Energy Award [DE-SC0001009];
DOE [DE-AC36-08GO28308]; National Renewable Energy Laboratory (NREL)
FX P.S., P.A.P., and C.L.P. contributed equally to this work. This paper
was based on research supported as part of the Center for Interface
Science: Solar Electric Materials (CISSEM), an Energy Frontier Research
Center funded by the U.S. Department of Energy, Office of Science, Basic
Energy Sciences, U.S. Department of Energy Award Number DE-SC0001084
(N.E.W., P.S., P.F.N., A.K.S., D.S.G., A.K.). also by the Center for
Energy Efficent Materials (CEEM), an Energy Frontier Research Center
funded by the U.S. Department of Energy, Office of Science, Basic Energy
Sciences, U.S. Department of Energy Award Number DE-SC0001009 (D.C.O.,
J.J.B.). P.A.P. and C.L.P. were supported by DOE Contract Number
DE-AC36-08GO28308 with the National Renewable Energy Laboratory (NREL).
Portions of this research were carried out at the Stanford Synchrotron
Radiation Light source, a national user facility operated by Stanford
University on behalf of the US Department of Energy, Office of Basic
Energy Sciences (M.F.T.). The authors gratefully acknowledge Prof.
Charles Rogers and Prof. Minhyea Lee of the University of Colorado, and
Dr. Jian V. Li of NREL for helpful discussions. Dr. Michele Olsen of
NREL has also provided significant comments during internal reviews.
NR 42
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Z9 9
U1 4
U2 70
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD AUG 5
PY 2014
VL 4
IS 11
AR 1301879
DI 10.1002/aenm.201301879
PG 10
WC Chemistry, Physical; Energy & Fuels; Materials Science,
Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AN3ZH
UT WOS:000340526900008
ER
PT J
AU Carpenter, TS
Kirshner, DA
Lau, EY
Wong, SE
Nilmeier, JP
Lightstone, FC
AF Carpenter, Timothy S.
Kirshner, Daniel A.
Lau, Edmond Y.
Wong, Sergio E.
Nilmeier, Jerome P.
Lightstone, Felice C.
TI A Method to Predict Blood-Brain Barrier Permeability of Drug-Like
Compounds Using Molecular Dynamics Simulations
SO BIOPHYSICAL JOURNAL
LA English
DT Article
ID NONSTEROIDAL ANTIINFLAMMATORY DRUGS; MEMBRANE LIQUID-CHROMATOGRAPHY;
IN-SILICO PREDICTION; PARTICLE MESH EWALD; LIPID-MEMBRANES;
PARTITION-COEFFICIENT; COMPUTER-SIMULATIONS; PERFUSION TECHNIQUE;
CORRELATION-ENERGY; PENETRATION
AB The blood-brain barrier (BBB) is formed by specialized tight junctions between endothelial cells that line brain capillaries to create a highly selective barrier between the brain and the rest of the body. A major problem to overcome in drug design is the ability of the compound in question to cross the BBB. Neuroactive drugs are required to cross the BBB to function. Conversely, drugs that target other parts of the body ideally should not cross the BBB to avoid possible psychotropic side effects. Thus, the task of predicting the BBB permeability of new compounds is of great importance. Two gold-standard experimental measures of BBB permeability are logBB (the concentration of drug in the brain divided by concentration in the blood) and logPS (permeability surface-area product). Both methods are time-consuming and expensive, and although logPS is considered the more informative measure, it is lower throughput and more resource intensive. With continual increases in computer power and improvements in molecular simulations, in silico methods may provide viable alternatives. Computational predictions of these two parameters for a sample of 12 small molecule compounds were performed. The potential of mean force for each compound through a 1,2-dioleoyl-sn-glycero-3-phosphocholine bilayer is determined by molecular dynamics simulations. This system setup is often used as a simple BBB mimetic. Additionally, one-dimensional position-dependent diffusion coefficients are calculated from the molecular dynamics trajectories. The diffusion coefficient is combined with the free energy landscape to calculate the effective permeability (P-eff) for each sample compound. The relative values of these permeabilities are compared to experimentally determined logBB and logPS values. Our computational predictions correlate remarkably well with both logBB (R-2 = 0.94) and logPS (R-2 = 0.90). Thus, we have demonstrated that this approach may have the potential to provide reliable, quantitatively predictive BBB permeability, using a relatively quick, inexpensive method.
C1 [Carpenter, Timothy S.; Kirshner, Daniel A.; Lau, Edmond Y.; Wong, Sergio E.; Nilmeier, Jerome P.; Lightstone, Felice C.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Biosci & Biotechnol Div, Livermore, CA 94550 USA.
RP Lightstone, FC (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Biosci & Biotechnol Div, Livermore, CA 94550 USA.
EM lightstone1@llnl.gov
FU Laboratory Directed Research and Development [12-SI-004]; U.S.
Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344, LLNL-JRNL-648046]
FX We thank Laboratory Directed Research and Development 12-SI-004 for
funding. This work performed under the auspices of the U.S. Department
of Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344. LLNL-JRNL-648046.
NR 102
TC 21
Z9 23
U1 3
U2 44
PU CELL PRESS
PI CAMBRIDGE
PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA
SN 0006-3495
EI 1542-0086
J9 BIOPHYS J
JI Biophys. J.
PD AUG 5
PY 2014
VL 107
IS 3
BP 630
EP 641
DI 10.1016/j.bpj.2014.06.024
PG 12
WC Biophysics
SC Biophysics
GA AM7AV
UT WOS:000340018000013
PM 25099802
ER
PT J
AU Dutilh, BE
Thompson, CC
Vicente, ACP
Marin, MA
Lee, C
Silva, GGZ
Schmieder, R
Andrade, BGN
Chimetto, L
Cuevas, D
Garza, DR
Okeke, IN
Aboderin, AO
Spangler, J
Ross, T
Dinsdale, EA
Thompson, FL
Harkins, TT
Edwards, RA
AF Dutilh, Bas E.
Thompson, Cristiane C.
Vicente, Ana C. P.
Marin, Michel A.
Lee, Clarence
Silva, Genivaldo G. Z.
Schmieder, Robert
Andrade, Bruno G. N.
Chimetto, Luciane
Cuevas, Daniel
Garza, Daniel R.
Okeke, Iruka N.
Aboderin, Aaron Oladipo
Spangler, Jessica
Ross, Tristen
Dinsdale, Elizabeth A.
Thompson, Fabiano L.
Harkins, Timothy T.
Edwards, Robert A.
TI Comparative genomics of 274 Vibrio cholerae genomes reveals mobile
functions structuring three niche dimensions
SO BMC GENOMICS
LA English
DT Article
DE Functional genomics; Mobile elements; Phages; Niche adaptation; Vibrio;
Genome evolution; Genotype-phenotype association; Random forest
ID RANDOM FORESTS; SEQUENCES; ALGORITHM; BACTERIA; STRAINS; PROJECT; SERVER
AB Background: Vibrio cholerae is a globally dispersed pathogen that has evolved with humans for centuries, but also includes non-pathogenic environmental strains. Here, we identify the genomic variability underlying this remarkable persistence across the three major niche dimensions space, time, and habitat.
Results: Taking an innovative approach of genome-wide association applicable to microbial genomes (GWAS-M), we classify 274 complete V. cholerae genomes by niche, including 39 newly sequenced for this study with the Ion Torrent DNA-sequencing platform. Niche metadata were collected for each strain and analyzed together with comprehensive annotations of genetic and genomic attributes, including point mutations (single-nucleotide polymorphisms, SNPs), protein families, functions and prophages.
Conclusions: Our analysis revealed that genomic variations, in particular mobile functions including phages, prophages, transposable elements, and plasmids underlie the metadata structuring in each of the three niche dimensions. This underscores the role of phages and mobile elements as the most rapidly evolving elements in bacterial genomes, creating local endemicity (space), leading to temporal divergence (time), and allowing the invasion of new habitats. Together, we take a data-driven approach for comparative functional genomics that exploits high-volume genome sequencing and annotation, in conjunction with novel statistical and machine learning analyses to identify connections between genotype and phenotype on a genome-wide scale.
C1 [Dutilh, Bas E.; Dinsdale, Elizabeth A.; Edwards, Robert A.] San Diego State Univ, Dept Biol, San Diego, CA 92182 USA.
[Dutilh, Bas E.; Silva, Genivaldo G. Z.; Schmieder, Robert; Cuevas, Daniel; Garza, Daniel R.; Edwards, Robert A.] San Diego State Univ, Dept Comp Sci, San Diego, CA 92182 USA.
[Dutilh, Bas E.] Radboud Univ Nijmegen, Med Ctr, Radboud Inst Mol Life Sci, Ctr Mol & Biomol Informat, NL-6525 ED Nijmegen, Netherlands.
[Dutilh, Bas E.; Chimetto, Luciane; Thompson, Fabiano L.; Edwards, Robert A.] Univ Fed Rio de Janeiro, Inst Biol, Dept Marine Biol, Rio De Janeiro, Brazil.
[Thompson, Cristiane C.; Vicente, Ana C. P.; Marin, Michel A.; Andrade, Bruno G. N.] Fiocruz MS, Inst Oswaldo Cruz, Lab Mol Genet Microorganisms, BR-21045900 Rio De Janeiro, Brazil.
[Silva, Genivaldo G. Z.; Schmieder, Robert; Edwards, Robert A.] San Diego State Univ, Computat Sci Res Ctr, San Diego, CA 92182 USA.
[Lee, Clarence; Cuevas, Daniel; Spangler, Jessica; Ross, Tristen; Harkins, Timothy T.] Life Technol Inc, Adv Applicat Grp, Beverly, MA USA.
[Okeke, Iruka N.] Haverford Coll, Dept Biol, Haverford, PA 19041 USA.
[Aboderin, Aaron Oladipo] Obafemi Awolowo Univ, Coll Hlth Sci, Dept Med Microbiol & Parasitol, Ife, Nigeria.
[Edwards, Robert A.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA.
RP Edwards, RA (reprint author), San Diego State Univ, Dept Biol, San Diego, CA 92182 USA.
EM redwards@sciences.sdsu.edu
RI Garza, Daniel Rios/A-1716-2016; Dutilh, Bas/B-9719-2011; Thompson,
Cristiane/I-5783-2016;
OI Garza, Daniel Rios/0000-0001-5956-6832; Dutilh, Bas/0000-0003-2329-7890;
Okeke, Iruka/0000-0002-1694-7587; Garza, Daniel/0000-0003-3865-2146;
Abanto Marin, Michel/0000-0001-9136-0041
FU Dutch Science foundation (NWO) Veni [016.111.075]; CAPES/BRASIL; CAPES;
CNPq; IOC-FIOCRUZ; NSF from the Division of Biological Infrastructure
[DBI: 0850356]; Division of Environmental Biology [DEB: 1046413];
Department of Education [P116M100007]; NSF TUES [1044453]
FX The authors thank Ankur Mutreja for sharing the most recent version of
the N16961 genome. BED is supported by the Dutch Science foundation
(NWO) Veni grant 016.111.075 and CAPES/BRASIL. ACPV, CCT, MAM and BNA
are supported by CAPES, CNPq and IOC-FIOCRUZ. RAE is supported by NSF
grants DBI: 0850356 from the Division of Biological Infrastructure and
DEB: 1046413 from the Division of Environmental Biology, and by grant
P116M100007 from the Department of Education. EAD is supported by NSF
TUES grant 1044453. We thank Anca Segall, Forest Rohwer, and Stanley
Maloy for thoughtful discussions and critical reviews of the manuscript.
NR 42
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U1 2
U2 23
PU BIOMED CENTRAL LTD
PI LONDON
PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND
SN 1471-2164
J9 BMC GENOMICS
JI BMC Genomics
PD AUG 5
PY 2014
VL 15
AR 654
DI 10.1186/1471-2164-15-654
PG 11
WC Biotechnology & Applied Microbiology; Genetics & Heredity
SC Biotechnology & Applied Microbiology; Genetics & Heredity
GA AN5PI
UT WOS:000340643300001
PM 25096633
ER
PT J
AU Eren, B
Marot, L
Steiner, R
de los Arcos, T
Duggelin, M
Mathys, D
Goldie, KN
Olivieri, V
Meyer, E
AF Eren, Baran
Marot, Laurent
Steiner, Roland
de los Arcos, Teresa
Dueggelin, Marcel
Mathys, Daniel
Goldie, Kenneth N.
Olivieri, Vesna
Meyer, Ernst
TI Carbon nanotube growth on AlN support: Comparison between Ni and Fe
chemical states and morphology
SO CHEMICAL PHYSICS LETTERS
LA English
DT Article
ID VAPOR-DEPOSITION; IRON; NANOPARTICLES; FILMS; MECHANISM; GRAPHENE;
NITRIDE; SPECTRA; PHASE
AB In this work, carbon nanotubes (CNTs) are grown from Ni and Fe nanoparticles supported on a rough AlN surface. Although, identical experimental parameters are used during dewetting (island formation) via thermal treatment, Ni particles appear metallic and larger, whereas Fe particles are smaller and slightly oxidized. This difference in the nanoparticle chemical state and morphology reflects to CNTs during catalytic chemical vapor deposition in terms of their CNT growth mode and size: tip-growth mode for Ni catalyst with CNT diameters of up to 40 nm, whereas base-growth mode for Fe with CNT diameters typically less than 10 nm are observed. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Eren, Baran; Marot, Laurent; Steiner, Roland; Meyer, Ernst] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland.
[Eren, Baran] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[de los Arcos, Teresa] Ruhr Univ Bochum, Res Dept Plasma, Inst Expt Phys 2, D-44780 Bochum, Germany.
[Dueggelin, Marcel; Mathys, Daniel; Olivieri, Vesna] Univ Basel, Ctr Microscopy, CH-4056 Basel, Switzerland.
[Goldie, Kenneth N.] Univ Basel, Biozentrum, Ctr Cellular Imaging & Nano Analyt, CH-4056 Basel, Switzerland.
RP Marot, L (reprint author), Univ Basel, Dept Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland.
EM laurent.marot@unibas.ch
RI Eren, Baran/A-9644-2013; Meyer, Ernst/L-3873-2016; Marot,
Laurent/A-5834-2008
OI Meyer, Ernst/0000-0001-6385-3412; Marot, Laurent/0000-0002-1529-9362
FU Swiss Federal Office of Energy; Federal Office for Education and
Science; Swiss National Foundation (SNF); Swiss Nanoscience Institute
(SNI); COST Action [MP1303]
FX The authors would like to thank the Swiss Federal Office of Energy and
the Federal Office for Education and Science for their financial
support. This work was also supported by the Swiss National Foundation
(SNF), the Swiss Nanoscience Institute (SNI) and the COST Action MP1303.
NR 36
TC 3
Z9 3
U1 5
U2 37
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0009-2614
EI 1873-4448
J9 CHEM PHYS LETT
JI Chem. Phys. Lett.
PD AUG 5
PY 2014
VL 609
BP 82
EP 87
DI 10.1016/j.cplett.2014.06.042
PG 6
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA AM9SJ
UT WOS:000340221000016
ER
PT J
AU Scown, CD
Gokhale, AA
Willems, PA
Horvath, A
McKone, TE
AF Scown, Corinne D.
Gokhale, Amit A.
Willems, Paul A.
Horvath, Arpad
McKone, Thomas E.
TI Role of Lignin in Reducing Life-Cycle Carbon Emissions, Water Use, and
Cost for United States Cellulosic Biofuels
SO ENVIRONMENTAL SCIENCE & TECHNOLOGY
LA English
DT Article
ID TECHNOECONOMIC ANALYSIS; ETHANOL-PRODUCTION; TRANSPORTATION;
BIOREFINERIES; PRETREATMENT; ELECTRICITY; ENERGY; FUELS
AB Cellulosic ethanol can achieve estimated greenhouse gas (GHG) emission reductions greater than 80% relative to gasoline, largely as a result of the combustion of lignin for process heat and electricity in biorefineries. Most studies assume lignin is combusted onsite, but exporting lignin to be cofired at coal power plants has the potential to substantially reduce biorefinery capital costs. We assess the life-cycle GHG emissions, water use, and capital costs associated with four representative biorefinery test cases. Each case is evaluated in the context of a U.S. national scenario in which corn stover, wheat straw, and Miscanthus are converted to 1.4 EJ (60 billion liters) of ethanol annually. Life-cycle GHG emissions range from 4.7 to 61 g CO2e/MJ of ethanol (compared with similar to 95 g CO2e/MJ of gasoline), depending on biorefinery configurations and marginal electricity sources. Exporting lignin can achieve GHG emission reductions comparable to onsite combustion in some cases, reduce life-cycle water consumption by up to 40%, and reduce combined heat and power-related capital costs by up to 63%. However, nearly 50% of current U.S. coal-fired power generating capacity is expected to be retired by 2050, which will limit the capacity for lignin cofiring and may double transportation distances between biorefineries and coal power plants.
C1 [Scown, Corinne D.; McKone, Thomas E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Gokhale, Amit A.; Willems, Paul A.] BP Corp North Amer Inc, Berkeley, CA 94704 USA.
[Horvath, Arpad] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA.
RP Scown, CD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM cdscown@lbl.gov
RI Scown, Corinne/D-1253-2013
FU Energy Biosciences Institute at the University of California, Berkeley;
U.S. Department of Energy [DE-AC03-76SF00098]
FX We wish to thank John Myers from the Department of Chemical Petroleum
Engineering at University of Wyoming for fruitful conversations
regarding modeling various power generation scenarios. Preparation of
this article was financially supported in part by the Energy Biosciences
Institute at the University of California, Berkeley. This work was
carried out in part at the Lawrence Berkeley National Laboratory, which
is operated for the U.S. Department of Energy under Contract Grant No.
DE-AC03-76SF00098.
NR 39
TC 5
Z9 5
U1 3
U2 34
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0013-936X
EI 1520-5851
J9 ENVIRON SCI TECHNOL
JI Environ. Sci. Technol.
PD AUG 5
PY 2014
VL 48
IS 15
SI SI
BP 8446
EP 8455
DI 10.1021/es5012753
PG 10
WC Engineering, Environmental; Environmental Sciences
SC Engineering; Environmental Sciences & Ecology
GA AM7WY
UT WOS:000340080600017
PM 24988448
ER
PT J
AU Cheah, S
Malone, SC
Feik, CJ
AF Cheah, Singfoong
Malone, Shealyn C.
Feik, Calvin J.
TI Speciation of Sulfur in Biochar Produced from Pyrolysis and Gasification
of Oak and Corn Stover
SO ENVIRONMENTAL SCIENCE & TECHNOLOGY
LA English
DT Article
ID RAY-ABSORPTION-SPECTROSCOPY; TRANSPORTATION FUELS; BIOMASS GASIFICATION;
COAL; SOIL; CATALYST; GAS; TRANSFORMATION; CHEMISTRY; IFEFFIT
AB The effects of feedstock type and biomass conversion conditions on the speciation of sulfur in biochars are not well-known. In this study, the sulfur content and speciation in biochars generated from pyrolysis and gasification of oak and corn stover were determined. We found the primary determinant of the total sulfur content of biomass to be the feedstock from which the biochar is generated, with oak and corn stover biochars containing 160 and 600-800 ppm sulfur, respectively. In contrast, for sulfur speciation, we found the primary determinant to be the temperature combined with the thermochemical conversion method. The speciation of sulfur in biochars was determined using X-ray absorption near-edge structure (XANES), ASTM method D2492, and scanning electron microscopy-energy-dispersive spectroscopy (SEM-EDS). Biochars produced under pyrolysis conditions at 500-600 degrees C contain sulfate, organosulfur, and sulfide. In some cases, the sulfate contents are up to 77-100%. Biochars produced in gasification conditions at 850 degrees C contain 73-100% organosulfur. The increase of the organosulfur content as the temperature of biochar production increases suggests a similar sulfur transformation mechanism as that in coal, where inorganic sulfur reacts with hydrocarbon and/or H-2 to form organosulfur when the coal is heated. EDS mapping of a biochar produced from corn stover pyrolysis shows individual sulfur-containing mineral particles in addition to the sulfur that is distributed throughout the organic matrix.
C1 [Cheah, Singfoong; Malone, Shealyn C.; Feik, Calvin J.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Cheah, S (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy,MS 3322, Golden, CO 80401 USA.
EM singfoong.cheah@nrel.gov
FU BioEnergy Technologies Office, U.S. Department of Energy (DOE)
[DE-AC36-08GO28308]; National Renewable Energy Laboratory; Science,
Technology, Engineering, and Mathematics Teacher and Researcher (STAR)
program - National Science Foundation; California State University; S.
D. Bechtel, Jr. Foundation; DOE Office of Biological and Environmental
Research; National Institutes of Health (NIH), National Institute of
General Medical Sciences (NIGMS) [P41GM103393]; National Center for
Research Resources (NCRR) [P41RR001209]
FX The authors thank Daniel Carpenter and Katherine Gaston at NREL for
their comments and discussion as well as three anonymous reviewers for
their constructive feedback and insights. The authors also gratefully
acknowledge the help of Dr. Ritimukta Sarangi and Dr. Erik Nelson of the
Stanford Synchrotron Radiation Laboratory (SSRL) during XANES data
collection. Funding for this research was provided by the BioEnergy
Technologies Office, U.S. Department of Energy (DOE), under contract
number DE-AC36-08GO28308, with the National Renewable Energy Laboratory.
Shealyn C. Malone's work at NREL was funded by the Science, Technology,
Engineering, and Mathematics Teacher and Researcher (STAR) program,
which is supported by the National Science Foundation, The California
State University, and the S. D. Bechtel, Jr. Foundation. Portions of
this research were carried out at SSRL a Directorate of SLAC National
Accelerator Laboratory and an Office of Science User Facility operated
for the U.S. Department of Energy Office of Science by Stanford
University. The SSRL Structural Molecular Biology Program is supported
by the DOE Office of Biological and Environmental Research and by the
National Institutes of Health (NIH), National Institute of General
Medical Sciences (NIGMS) (including P41GM103393), and National Center
for Research Resources (NCRR) (including P41RR001209). The contents of
this publication are solely the responsibility of the authors and do not
necessarily represent the official views of NIGMS, NCRR, or NIH.
NR 51
TC 15
Z9 15
U1 4
U2 75
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0013-936X
EI 1520-5851
J9 ENVIRON SCI TECHNOL
JI Environ. Sci. Technol.
PD AUG 5
PY 2014
VL 48
IS 15
SI SI
BP 8474
EP 8480
DI 10.1021/es500073r
PG 7
WC Engineering, Environmental; Environmental Sciences
SC Engineering; Environmental Sciences & Ecology
GA AM7WY
UT WOS:000340080600020
PM 25003702
ER
PT J
AU Lee, MS
McGrail, BP
Glezakou, VA
AF Lee, Mal-Soon
McGrail, B. Peter
Glezakou, Vassiliki-Alexandra
TI Microstructural Response of Variably Hydrated Ca-rich Montmorillonite to
Supercritical CO2
SO ENVIRONMENTAL SCIENCE & TECHNOLOGY
LA English
DT Article
ID X-RAY-DIFFRACTION; INITIO MOLECULAR-DYNAMICS; DENSITY-FUNCTIONAL THEORY;
CARBON-DIOXIDE; INFRARED-SPECTRA; NA-MONTMORILLONITE; WATER; SMECTITE;
CLUSTERS; IO
AB First-principles molecular dynamics simulations were carried out to explore the mechanistic and thermodynamic ramifications of the exposure of variably hydrated Ca-rich montmorillonites to supercritical CO2 and CO2-SO2 mixtures under geologic storage conditions. In sub- to single-hydrated systems (<= 1W), CO2 intercalation causes interlamellar expansion of 8-12%, while systems transitioning to 2W may undergo contraction (similar to 7%) or remain almost unchanged. When compared to similar to 2W hydration state, structural analysis of the <= 1W systems, reveals more Ca-CO2 contacts and partial transition to vertically confined CO2 molecules. Infrared spectra and projected vibrational frequency analysis imply that intercalated Ca-bound CO2 are vibrationally constrained and contribute to the higher frequencies of the asymmetric stretch band. Reduced intercalated H2O and CO2 (10(-6)-10(-7) cm(2)/s) indicate that Ca-montmorillonites in similar to 1W hydration states can be more efficient in capturing CO2. Simulations including SO2 imply that similar to 0.66 mmol SO2/g clay can be intercalated without other significant structural changes. SO2 is likely to divert H2O away from the cations, promoting Ca-CO2 interactions and CO2 capture by further reducing CO2 diffusion (10(-8) cm(2)/s). Vibrational bands at similar to 1267 or 1155 cm(-1) may be used to identify the chemical state (oxidation states +4 or +6, respectively) and the fate of sulfur contaminants.
C1 [Lee, Mal-Soon; McGrail, B. Peter; Glezakou, Vassiliki-Alexandra] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Glezakou, VA (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM Vanda.Glezakou@pnnl.gov
RI Lee, Mal-Soon/K-4161-2013
OI Lee, Mal-Soon/0000-0001-6851-177X
FU Office of Fossil Energy, U.S. Department of Energy; Department of
Energy's Office of Biological and Environmental Research; PNNL
Institutional Computing (PIC) program
FX We are infinitely grateful to Dr. R. Rousseau for insightful discussions
and a critical reading of the manuscript. The comments by Professor
Giammar and three expert reviewers were extremely beneficial and much
appreciated. This research would not have been possible without the
support of the Office of Fossil Energy, U.S. Department of Energy. A
portion of the research was performed using EMSL, a national scientific
user facility sponsored by the Department of Energy's Office of
Biological and Environmental Research, and PNNL Institutional Computing
(PIC) program, both located at Pacific Northwest National Laboratory. We
are particularly grateful to Dr. D. Baxter and Dr. T. Carlson for
facilitating timely access to computational resources.
NR 52
TC 14
Z9 14
U1 2
U2 51
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0013-936X
EI 1520-5851
J9 ENVIRON SCI TECHNOL
JI Environ. Sci. Technol.
PD AUG 5
PY 2014
VL 48
IS 15
SI SI
BP 8612
EP 8619
DI 10.1021/es5005889
PG 8
WC Engineering, Environmental; Environmental Sciences
SC Engineering; Environmental Sciences & Ecology
GA AM7WY
UT WOS:000340080600036
PM 24842544
ER
PT J
AU Tidwell, VC
Moreland, B
Zemlick, K
AF Tidwell, Vincent C.
Moreland, Barbie
Zemlick, Katie
TI Geographic Footprint of Electricity Use for Water Services in the
Western US
SO ENVIRONMENTAL SCIENCE & TECHNOLOGY
LA English
DT Article
AB A significant fraction of our nation's electricity use goes to lift, convey, and treat water, while the resulting expenditures on electricity represent a key budgetary consideration for water service providers. To improve understanding of the electricity-for-water interdependency, electricity used in providing water services is mapped at the regional, state and county level for the 17-conterminous states in the Western U.S. This study is unique in estimating electricity use for large-scale conveyance and agricultural pumping as well as mapping these electricity uses along with that for drinking and wastewater services at a state and county level. Results indicate that drinking and wastewater account for roughly 2% of total West-wide electricity use, while an additional 1.2% is consumed by large-scale conveyance projects and 2.6% is consumed by agricultural pumping. The percent of electricity used for water services varies strongly by state with some as high as 34%, while other states expend less than 1%. Every county in the West uses some electricity for water services; however, there is a large disparity in use ranging from 10 MWh/yr to 5.8 TWh/yr. These results support long-term transmission planning in the Western U.S. by characterizing an important component of the electric load.
C1 [Tidwell, Vincent C.; Moreland, Barbie; Zemlick, Katie] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Tidwell, VC (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM vctidwe@sandia.gov
FU U.S. Department of Energy's Office of Electricity Delivery and Energy
Reliability [M610000581]; U.S. Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX The authors acknowledge the very helpful comments of three anonymous
reviewers. The work described in this article was funded by the U.S.
Department of Energy's Office of Electricity Delivery and Energy
Reliability through the American Recovery and Reinvestment Act of 2009
under Contract No. M610000581. Sandia National Laboratories is a
multiprogram laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
Department of Energy's National Nuclear Security Administration under
contract DE-AC04-94AL85000.
NR 29
TC 2
Z9 2
U1 0
U2 12
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0013-936X
EI 1520-5851
J9 ENVIRON SCI TECHNOL
JI Environ. Sci. Technol.
PD AUG 5
PY 2014
VL 48
IS 15
SI SI
BP 8897
EP 8904
DI 10.1021/es5016845
PG 8
WC Engineering, Environmental; Environmental Sciences
SC Engineering; Environmental Sciences & Ecology
GA AM7WY
UT WOS:000340080600070
PM 24963828
ER
PT J
AU Kaplan, DI
Miller, TJ
Diprete, D
Powell, BA
AF Kaplan, Daniel I.
Miller, Todd J.
Diprete, David
Powell, Brian A.
TI Long-Term Radiostrontiunn Interactions and Transport through Sediment
SO ENVIRONMENTAL SCIENCE & TECHNOLOGY
LA English
DT Article
ID PLUTONIUM TRANSPORT; STRONTIUM; SOILS; RADIONUCLIDES; CESIUM; MODEL; IV
AB Radioactive strontium is one of the most common radiological contaminants in groundwater and soil. Objectives of this study were to (1) evaluate Sr transport through an 11-year-long field lysimeter study and (2) quantify secondary aging effects between Sr and sediment that may need to be considered for long-term transport modeling. Batch sorption/desorption tests were conducted with Sr-85, Sr-88, and Sr-90 using a sediment recovered from a field lysimeter containing a glass pellet amended with high-level nuclear waste for 24 years. Sr was largely reversibly and linearly sorbed. Sr-85 sorption coefficients (K-d, concentration ratios of solids/liquids) after a 23-day contact period were about the same as the Sr-90 desorption K-d values after a 24-year contact period: sorption K-d = 32.1 +/- 3.62 mL g(-1) and desorption K-d = 43.1 +/- 11.4 mL g(-1). Numerical modeling of the lysirneter Sr-90 depth profile indicated that a Kd value of 32 mL fit the data best. The Kd construct captured most of the data trends above and below the source term, except for immediately below the source where the model clearly overestimated Sr mobility. Sr-90 desorption tests suggested that the overestimated mobility may be attributed to a second, slower sorption reaction that occurs over a course of months to decades.
C1 [Kaplan, Daniel I.; Diprete, David] Savannah River Natl Lab, Aiken, SC 29803 USA.
[Miller, Todd J.; Powell, Brian A.] Clemson Univ, Clemson, SC 29634 USA.
RP Kaplan, DI (reprint author), Savannah River Natl Lab, Aiken, SC 29803 USA.
EM daniel.kaplan@srnl.doe.gov
RI Powell, Brian /C-7640-2011
OI Powell, Brian /0000-0003-0423-0180
FU Department of Energy's Subsurface Biogeochemistry Research program
within the Office of Science; U.S. Department of Energy
[DE-AC09-96SR18500]
FX Funding for this research was made possible by the Department of
Energy's Subsurface Biogeochemistry Research program within the Office
of Science. Work was conducted at Savannah River National Laboratory
under the U.S. Department of Energy Contract DE-AC09-96SR18500.
NR 32
TC 1
Z9 1
U1 1
U2 22
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0013-936X
EI 1520-5851
J9 ENVIRON SCI TECHNOL
JI Environ. Sci. Technol.
PD AUG 5
PY 2014
VL 48
IS 15
SI SI
BP 8919
EP 8925
DI 10.1021/es5021108
PG 7
WC Engineering, Environmental; Environmental Sciences
SC Engineering; Environmental Sciences & Ecology
GA AM7WY
UT WOS:000340080600073
PM 24960400
ER
PT J
AU Van Gough, D
Wheeler, JS
Cheng, SF
Stevens, MJ
Spoerke, ED
AF Van Gough, Dara
Wheeler, Jill S.
Cheng, Shengfeng
Stevens, Mark J.
Spoerke, Erik D.
TI Supramolecular Assembly of Asymmetric Self-Neutralizing Amphiphilic
Peptide Wedges
SO LANGMUIR
LA English
DT Article
ID SURFACTANT-LIKE PEPTIDES; SECONDARY STRUCTURE; NANOFIBERS; NANOTUBES;
NANOSTRUCTURES; PROTEIN; SCAFFOLDS
AB Mimicking the remarkable dynamic and multifunctional utility of biological nanofibers, such as microtubules, is a challenging and technologically attractive objective in synthetic supramolecular chemistry. Understanding the complex molecular interactions that govern the assembly of synthetic materials, such as peptides, is key to meeting this challenge. Using molecular dynamics simulations to guide molecular design, we explore here the self-assembly of structurally and functionally asymmetric wedge-shaped peptides. Supramolecular assembly into nanofiber gels or multilayered lamellar structures was determined by cooperative influences of hydrogen bonding, amphiphilicity (hydrophilic asymmetry), and the distribution of electrostatic charges on the aqueous self-assembly of asymmetric peptides. Molecular amphiphilicity and beta-sheet forming capacity were both identified as necessary, but not independently sufficient, to form supramolecular nanofibers. Imbalances in positive and negative charges prevented nanofiber assembly, while the asymmetric distribution of balanced charges within a peptide is believed to affect peptide conformation and subsequent self-assembly into either nanofibers or lamellar structures. Insights into cooperative molecular interactions and the effects of molecular asymmetry on assembly may aid the development of next-generation supramolecular nanomaterial assemblies.
C1 [Van Gough, Dara; Wheeler, Jill S.; Cheng, Shengfeng; Stevens, Mark J.; Spoerke, Erik D.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Spoerke, ED (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM edspoer@sandia.gov
OI Cheng, Shengfeng/0000-0002-6066-2968
FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Materials Sciences and Engineering [KC0203010]; US Department of
Energy's National Nuclear Security Administration [DE-AC04-94AL85000]
FX We gratefully acknowledge Bonnie McKenzie for performing scanning
electron microscopy analysis, Ana Trujillo for performing atomic force
microscopy, and Dr. Bruce Bunker for insightful discussions. This
research was supported by the U.S. Department of Energy, Office of Basic
Energy Sciences, Division of Materials Sciences and Engineering, Project
KC0203010. Sandia National Laboratories is a multiprogram laboratory
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Company, for the US Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000.
NR 37
TC 2
Z9 2
U1 0
U2 36
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0743-7463
J9 LANGMUIR
JI Langmuir
PD AUG 5
PY 2014
VL 30
IS 30
BP 9201
EP 9209
DI 10.1021/la501620g
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science,
Multidisciplinary
SC Chemistry; Materials Science
GA AM7WK
UT WOS:000340079200024
PM 25003982
ER
PT J
AU Tian, YY
Cui, WJ
Huang, MN
Robinson, H
Wan, YQ
Wang, YS
Ke, HM
AF Tian, Yuanyuan
Cui, Wenjun
Huang, Manna
Robinson, Howard
Wan, Yiqian
Wang, Yousheng
Ke, Hengming
TI Dual Specificity and Novel Structural Folding of Yeast
Phosphodiesterase-1 for Hydrolysis of Second Messengers Cyclic Adenosine
and Guanosine 3 ',5 '-Monophosphate
SO BIOCHEMISTRY
LA English
DT Article
ID AFFINITY CAMP-PHOSPHODIESTERASE; PROTEIN-KINASE-A; CANDIDA-ALBICANS;
SACCHAROMYCES-CEREVISIAE; NUCLEOTIDE PHOSPHODIESTERASE; BAKERS-YEAST;
INHIBITOR SELECTIVITY; SUBSTRATE-SPECIFICITY; AMP PHOSPHODIESTERASE;
STRESS RESPONSES
AB Cyclic nucleotide phosphodiesterases (PDEs) decompose second messengers cAMP and cGMP that play critical roles in many physiological processes. PDE1 of Saccharomyces cerevisiae has been subcloned and expressed in Escherichia coli. Recombinant yPDE1 has a Km of 110 mu M and a k(cat) of 16.9 s(-1) for cAMP and a Km of 105 mu M and a k(cat), of 11.8 s(-1) for cGMP. Thus, the specificity constant (k(cat)/K-M(cAMP))/(k(cat)/K-M(cGMP)) of 1.4 indicates a dual specificity of yPDE1 for hydrolysis of both cAMP and cGMP. The crystal structures of unliganded yPDE1 and its complex with GMP at 1.31 angstrom resolution reveal a new structural folding that is different from those of human PDEs but is partially similar to that of some other metalloenzymes such as metallo-beta-lactamase. In spite of their different structures and divalent metals, yPDE1 and human PDEs may share a common mechanism for hydrolysis of cAMP and CGMP.
C1 [Tian, Yuanyuan; Wang, Yousheng] Beijing Technol & Business Univ, Beijing Lab Food Qual & Safety, Beijing 100048, Peoples R China.
[Tian, Yuanyuan; Wang, Yousheng] Beijing Technol & Business Univ, Beijing Engn & Technol Res Ctr Food Addit, Beijing 100048, Peoples R China.
[Tian, Yuanyuan; Cui, Wenjun; Huang, Manna; Ke, Hengming] Univ N Carolina, Dept Biochem & Biophys, Chapel Hill, NC 27599 USA.
[Tian, Yuanyuan; Cui, Wenjun; Huang, Manna; Ke, Hengming] Univ N Carolina, Lineberger Comprehens Canc Ctr, Chapel Hill, NC 27599 USA.
[Huang, Manna; Wan, Yiqian] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China.
[Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.
RP Ke, HM (reprint author), Univ N Carolina, Dept Biochem & Biophys, Chapel Hill, NC 27599 USA.
EM wangys@th.btbu.edu.cn; hke@med.unc.edu
FU National Institutes of Health [GM59791]; National Natural Science
Foundation of China [31291944]; Offices of Biological and Environmental
Research and of Basic Energy Sciences of the U.S. Department of Energy;
National Center for Research Resources of the National Institutes of
Health
FX This work was supported in part by National Institutes of Health Grant
GM59791 to H.K, the National Natural Science Foundation of China
(31291944, to Y.W.), and the Offices of Biological and Environmental
Research and of Basic Energy Sciences of the U.S. Department of Energy
and the National Center for Research Resources of the National
Institutes of Health (H.R.).
NR 48
TC 2
Z9 2
U1 1
U2 16
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0006-2960
J9 BIOCHEMISTRY-US
JI Biochemistry
PD AUG 5
PY 2014
VL 53
IS 30
BP 4938
EP 4945
DI 10.1021/bi500406h
PG 8
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA AM7WH
UT WOS:000340078900008
PM 25050706
ER
PT J
AU Hawley, AK
Brewer, HM
Norbeck, AD
Pasa-Tolic, L
Hallam, SJ
AF Hawley, Alyse K.
Brewer, Heather M.
Norbeck, Angela D.
Pasa-Tolic, Ljiljana
Hallam, Steven J.
TI Metaproteomics reveals differential modes of metabolic coupling among
ubiquitous oxygen minimum zone microbes
SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF
AMERICA
LA English
DT Article
ID SUB-ARCTIC PACIFIC; CENTRAL BALTIC SEA; COMMUNITY STRUCTURE; OXIDIZING
BACTERIA; NITRITE OXIDATION; AMMONIA OXIDATION; CARBON FIXATION;
ORGANIC-CARBON; SULFUR CYCLE; DARK OCEAN
AB Marine oxygen minimum zones (OMZs) are intrinsic water column features arising from respiratory oxygen demand during organic matter degradation in stratified waters. Currently OMZs are expanding due to global climate change with resulting feedback on marine ecosystem function. Here we use metaproteomics to chart spatial and temporal patterns of gene expression along defined redox gradients in a seasonally stratified fjord to better understand microbial community responses to OMZ expansion. The expression of metabolic pathway components for nitrification, anaerobic ammonium oxidation (anammox), denitrification, and inorganic carbon fixation were differentially expressed across the redoxcline and covaried with distribution patterns of ubiquitous OMZ microbes including Thaumarchaeota, Nitrospina, Nitrospira, Planctomycetes, and SUP05/ARCTIC96BD-19 Gammaproteobacteria. Nitrification and inorganic carbon fixation pathways affiliated with Thaumarchaeota dominated dysoxic waters, and denitrification, sulfur oxidation, and inorganic carbon fixation pathways affiliated with the SUP05 group of nitrate-reducing sulfur oxidizers dominated suboxic and anoxic waters. Nitrifier nitrite oxidation and anammox pathways affiliated with Nirospina, Nitrospira, and Planctomycetes, respectively, also exhibited redox partitioning between dysoxic and suboxic waters. The numerical abundance of SUP05 proteins mediating inorganic carbon fixation under anoxic conditions suggests that SUP05 will become increasingly important in global ocean carbon and nutrient cycling as OMZs expand.
C1 [Hawley, Alyse K.; Hallam, Steven J.] Univ British Columbia, Dept Microbiol & Immunol, Vancouver, BC V6T 1Z3, Canada.
[Hallam, Steven J.] Univ British Columbia, Grad Program Bioinformat, Vancouver, BC V6T 1Z3, Canada.
[Hallam, Steven J.] Univ British Columbia, Genome Sci & Technol Training Program, Vancouver, BC V6T 1Z3, Canada.
[Brewer, Heather M.; Norbeck, Angela D.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Biol & Computat Sci Div, Richland, WA 99352 USA.
RP Hallam, SJ (reprint author), Univ British Columbia, Dept Microbiol & Immunol, Vancouver, BC V6T 1Z3, Canada.
EM shallam@mail.ubc.ca
FU US Department of Energy (DOE); Office of Science of US DOE
[DE-AC02-05CH11231]; Tula Foundation-funded Centre for Microbial
Diversity and Evolution; Natural Sciences and Engineering Research
Council of Canada; Canada Foundation for Innovation; Canadian Institute
for Advanced Research; US DOE's Office of Biological and Environmental
Research
FX We thank the crew aboard the MSV John Strickland for logistical support;
David Walsh, Olena Schevchuk, and Elena Zaikova for assistance with
sample collection; Jinshu Yang for assistance with sample preparation;
and Charles Howes for assistance with data analysis. We also thank Sean
Crowe and all members of the S.J.H. laboratory for helpful comments
along the way. We thank the Joint Genome Institute, including Sussanah
Tringe, Stephanie Malfatti, and Tijana Glavina del Rio, for technical
and project management assistance. This work was performed under the
auspices of the US Department of Energy (DOE) Joint Genome Institute
supported by the Office of Science of US DOE Contract DE-AC02-05CH11231,
the Tula Foundation-funded Centre for Microbial Diversity and Evolution,
the Natural Sciences and Engineering Research Council of Canada, the
Canada Foundation for Innovation, and the Canadian Institute for
Advanced Research through grants awarded to S. J. H. Metaproteomics
support came from the intramural research and development program of the
W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL). EMSL is
a national scientific user facility sponsored by the US DOE's Office of
Biological and Environmental Research and located at the Pacific
Northwest National Laboratory operated by Battelle for the US DOE.
NR 53
TC 26
Z9 26
U1 6
U2 108
PU NATL ACAD SCIENCES
PI WASHINGTON
PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA
SN 0027-8424
J9 P NATL ACAD SCI USA
JI Proc. Natl. Acad. Sci. U. S. A.
PD AUG 5
PY 2014
VL 111
IS 31
BP 11395
EP 11400
DI 10.1073/pnas.1322132111
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM4EZ
UT WOS:000339807200040
PM 25053816
ER
PT J
AU Rautengarten, C
Ebert, B
Moreno, I
Temple, H
Herter, T
Link, B
Donas-Cofre, D
Moreno, A
Saez-Aguayoc, S
Blanco, F
Mortimer, JC
Schultink, A
Reiter, WD
Dupree, P
Pauly, M
Heazlewood, JL
Scheller, HV
Orellana, A
AF Rautengarten, Carsten
Ebert, Berit
Moreno, Ignacio
Temple, Henry
Herter, Thomas
Link, Bruce
Donas-Cofre, Daniela
Moreno, Adrian
Saez-Aguayoc, Susana
Blanco, Francisca
Mortimer, Jennifer C.
Schultink, Alex
Reiter, Wolf-Dieter
Dupree, Paul
Pauly, Markus
Heazlewood, Joshua L.
Scheller, Henrik V.
Orellana, Ariel
TI The Golgi localized bifunctional UDP-rhamnose/UDP-galactose transporter
family of Arabidopsis
SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF
AMERICA
LA English
DT Article
DE membrane transport; proteoliposomes; glycan biosynthesis; galactan
ID NUCLEOTIDE-SUGAR TRANSPORTERS; CELL-WALL BIOSYNTHESIS; TANDEM
MASS-SPECTROMETRY; LIQUID-CHROMATOGRAPHY; MOLECULAR-CLONING; THALIANA;
IDENTIFICATION; ENZYME; PLANTS; GROWTH
AB Plant cells are surrounded by a cell wall that plays a key role in plant growth, structural integrity, and defense. The cell wall is a complex and diverse structure that is mainly composed of polysaccharides. The majority of noncellulosic cell wall polysaccharides are produced in the Golgi apparatus from nucleotide sugars that are predominantly synthesized in the cytosol. The transport of these nucleotide sugars from the cytosol into the Golgi lumen is a critical process for cell wall biosynthesis and is mediated by a family of nucleotide sugar transporters (NSTs). Numerous studies have sought to characterize substrate-specific transport by NSTs; however, the availability of certain substrates and a lack of robust methods have proven problematic. Consequently, we have developed a novel approach that combines reconstitution of NSTs into liposomes and the subsequent assessment of nucleotide sugar uptake by mass spectrometry. To address the limitation of substrate availability, we also developed a two-step reaction for the enzymatic synthesis of UDP-L-rhamnose (Rha) by expressing the two active domains of the Arabidopsis UDP-L-Rha synthase. The liposome approach and the newly synthesized substrates were used to analyze a clade of Arabidopsis NSTs, resulting in the identification and characterization of six bifunctional UDP-LRha/UDP-D-galactose (Gal) transporters (URGTs). Further analysis of loss-of-function and overexpression plants for two of these URGTs supported their roles in the transport of UDP-L-Rha and UDP-D-Gal for matrix polysaccharide biosynthesis.
C1 [Rautengarten, Carsten; Ebert, Berit; Herter, Thomas; Heazlewood, Joshua L.; Scheller, Henrik V.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94702 USA.
[Rautengarten, Carsten; Ebert, Berit; Herter, Thomas; Heazlewood, Joshua L.; Scheller, Henrik V.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94702 USA.
[Ebert, Berit] Univ Copenhagen, Fac Sci, Dept Plant & Environm Sci, DK-1871 Copenhagen C, Denmark.
[Moreno, Ignacio; Temple, Henry; Donas-Cofre, Daniela; Moreno, Adrian; Saez-Aguayoc, Susana; Blanco, Francisca; Orellana, Ariel] Univ Andres Bello, Fac Ciencias Biol, Ctr Biotecnol Vegetal, Santiago 8370146, Chile.
[Moreno, Ignacio; Temple, Henry; Donas-Cofre, Daniela; Moreno, Adrian; Saez-Aguayoc, Susana; Blanco, Francisca; Orellana, Ariel] Fondo Areas Prioritarias Ctr Genome Regulat, Santiago 8370146, Chile.
[Link, Bruce; Reiter, Wolf-Dieter] Univ Connecticut, Dept Mol & Cell Biol, Storrs, CT 06269 USA.
[Mortimer, Jennifer C.; Dupree, Paul] Univ Cambridge, Dept Biochem, Cambridge CB2 1QW, England.
[Schultink, Alex; Pauly, Markus; Scheller, Henrik V.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.
RP Scheller, HV (reprint author), Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94702 USA.
EM hscheller@lbl.gov; aorellana@unab.cl
RI Heazlewood, Joshua/A-2554-2008; Scheller, Henrik/A-8106-2008; Orellana,
Ariel/E-2166-2014; Ebert, Berit/F-1856-2016; Pauly, Markus/B-5895-2008
OI Mortimer, Jenny/0000-0001-6624-636X; Moreno, Adrian/0000-0001-5125-2927;
Heazlewood, Joshua/0000-0002-2080-3826; Donas-Cofre,
Daniela/0000-0001-7703-5613; Blanco, Maria/0000-0002-7497-9907;
Scheller, Henrik/0000-0002-6702-3560; Orellana,
Ariel/0000-0002-9243-808X; Ebert, Berit/0000-0002-6914-5473; Pauly,
Markus/0000-0002-3116-2198
FU US Department of Energy, Office of Science, Office of Biological and
Environmental Research [DE-AC02-05CH11231]; Division of Chemical
Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences
of the US Department of Energy [DE-FG02-08ER20203]; CONICYT; Fondo de
Areas Prioritarias-Centro de Regulacion del Genoma [15090007, PFB-16,
ICM-Millenium Nucleus P10-062-F, DI-365-13/R, Fondecyt 3140415];
Biotechnology and Biological Sciences Research Council [BB/G016240/1];
Fred E. Dickinson Chair funds; Danish Research Council for Strategic
Research; National Science Foundation-Research Coordination Network
[0090281]
FX This work was supported by the US Department of Energy, Office of
Science, Office of Biological and Environmental Research, through
Contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory
and the US Department of Energy. Funding for W.-D.R. was provided by the
Division of Chemical Sciences, Geosciences, and Biosciences, Office of
Basic Energy Sciences of the US Department of Energy through Grant
DE-FG02-08ER20203. This work was also supported by CONICYT fellowships
(I. M., H. T., and A. M.) and by Fondo de Areas Prioritarias-Centro de
Regulacion del Genoma-15090007, PFB-16, ICM-Millenium Nucleus P10-062-F,
DI-365-13/R, and Fondecyt 3140415 grants (to A.O.). J.C.M. was supported
by Biotechnology and Biological Sciences Research Council Grant
BB/G016240/1 (to P. D.). Both A. S. and M. P. were supported by Fred E.
Dickinson Chair funds. B. E. was supported in part by the Danish
Research Council for Strategic Research. The substrates obtained from
Carbosource Services were supported, in part, by National Science
Foundation-Research Coordination Network Grant 0090281.
NR 45
TC 23
Z9 23
U1 5
U2 48
PU NATL ACAD SCIENCES
PI WASHINGTON
PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA
SN 0027-8424
J9 P NATL ACAD SCI USA
JI Proc. Natl. Acad. Sci. U. S. A.
PD AUG 5
PY 2014
VL 111
IS 31
BP 11563
EP 11568
DI 10.1073/pnas.1406073111
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM4EZ
UT WOS:000339807200068
PM 25053812
ER
PT J
AU Heath, GA
O'Donoughue, P
Arent, DJ
Bazilian, M
AF Heath, Garvin A.
O'Donoughue, Patrick
Arent, Douglas J.
Bazilian, Morgan
TI Harmonization of initial estimates of shale gas life cycle greenhouse
gas emissions for electric power generation
SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF
AMERICA
LA English
DT Article
DE life cycle assessment; methane leakage; meta-analysis
ID NATURAL-GAS; METHANE LEAKAGE; COAL; FOOTPRINT
AB Recent technological advances in the recovery of unconventional natural gas, particularly shale gas, have served to dramatically increase domestic production and reserve estimates for the United States and internationally. This trend has led to lowered prices and increased scrutiny on production practices. Questions have been raised as to how greenhouse gas (GHG) emissions from the life cycle of shale gas production and use compares with that of conventionally produced natural gas or other fuel sources such as coal. Recent literature has come to different conclusions on this point, largely due to differing assumptions, comparison baselines, and system boundaries. Through a meta-analytical procedure we call harmonization, we develop robust, analytically consistent, and updated comparisons of estimates of life cycle GHG emissions for electricity produced from shale gas, conventionally produced natural gas, and coal. On a per-unit electrical output basis, harmonization reveals that median estimates of GHG emissions from shale gas-generated electricity are similar to those for conventional natural gas, with both approximately half that of the central tendency of coal. Sensitivity analysis on the harmonized estimates indicates that assumptions regarding liquids unloading and estimated ultimate recovery (EUR) of wells have the greatest influence on life cycle GHG emissions, whereby shale gas life cycle GHG emissions could approach the range of best-performing coal-fired generation under certain scenarios. Despite clarification of published estimates through harmonization, these initial assessments should be confirmed through methane emissions measurements at components and in the atmosphere and through better characterization of EUR and practices.
C1 [Heath, Garvin A.] Joint Inst Strateg Energy Anal, Golden, CO 80401 USA.
Strateg Energy Anal Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Heath, GA (reprint author), Joint Inst Strateg Energy Anal, Golden, CO 80401 USA.
EM garvin.heath@nrel.gov
FU Joint Institute for Strategic Energy Analysis; US Department of Energy,
Office of Energy Efficiency and Renewable Energy [DE-AC36-08-GO28308];
National Renewable Energy Laboratory
FX Funding to support this research was generously provided by the Joint
Institute for Strategic Energy Analysis. Funding for the foundational
research of the LCA Harmonization Project (www.nrel.gov/harmonization)
was provided by US Department of Energy, Office of Energy Efficiency and
Renewable Energy Contract DE-AC36-08-GO28308 with the National Renewable
Energy Laboratory.
NR 56
TC 25
Z9 25
U1 0
U2 32
PU NATL ACAD SCIENCES
PI WASHINGTON
PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA
SN 0027-8424
J9 P NATL ACAD SCI USA
JI Proc. Natl. Acad. Sci. U. S. A.
PD AUG 5
PY 2014
VL 111
IS 31
BP E3167
EP E3176
DI 10.1073/pnas.1309334111
PG 10
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM4EZ
UT WOS:000339807200001
PM 25049378
ER
PT J
AU Dziarmaga, J
Zurek, WH
AF Dziarmaga, Jacek
Zurek, Wojciech H.
TI Quench in the 1D Bose-Hubbard model: Topological defects and excitations
from the Kosterlitz-Thouless phase transition dynamics
SO SCIENTIFIC REPORTS
LA English
DT Article
ID SPONTANEOUS SYMMETRY-BREAKING; STRING FORMATION; COSMOLOGICAL
EXPERIMENTS; EINSTEIN CONDENSATE; VORTEX FORMATION; SUPERFLUID HE-3;
LIQUID-CRYSTALS; SYSTEMS; UNIVERSE; PIECES
AB Kibble-Zurek mechanism (KZM) uses critical scaling to predict density of topological defects and other excitations created in second order phase transitions. We point out that simply inserting asymptotic critical exponents deduced from the immediate vicinity of the critical point to obtain predictions can lead to results that are inconsistent with a more careful KZM analysis based on causality - on the comparison of the relaxation time of the order parameter with the "time distance'' from the critical point. As a result, scaling of quench-generated excitations with quench rates can exhibit behavior that is locally (i.e., in the neighborhood of any given quench rate) well approximated by the power law, but with exponents that depend on that rate, and that are quite different from the naive prediction based on the critical exponents relevant for asymptotically long quench times. Kosterlitz-Thouless scaling (that governs e.g. Mott insulator to superfluid transition in the Bose-Hubbard model in one dimension) is investigated as an example of this phenomenon.
C1 [Dziarmaga, Jacek] Uniwersytetu Jagiellonskiego, Inst Fizyki, PL-30059 Krakow, Poland.
[Zurek, Wojciech H.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Dziarmaga, J (reprint author), Uniwersytetu Jagiellonskiego, Inst Fizyki, Ul Reymonta 4, PL-30059 Krakow, Poland.
EM jacekdziarmaga@yahoo.com
FU Polish National Science Center (NCN) [DEC-2013/09/B/ST3/01603];
Department of Energy under the Los Alamos National Laboratory
FX This work was supported by the Polish National Science Center (NCN)
under Project DEC-2013/09/B/ST3/01603 and by Department of Energy under
the Los Alamos National Laboratory LDRD Program.
NR 59
TC 8
Z9 8
U1 3
U2 9
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2045-2322
J9 SCI REP-UK
JI Sci Rep
PD AUG 5
PY 2014
VL 4
AR 5950
DI 10.1038/srep05950
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM7GA
UT WOS:000340032000003
PM 25091996
ER
PT J
AU Mei, ZG
Stan, M
Yang, J
AF Mei, Zhi-Gang
Stan, Marius
Yang, Jiong
TI First-principles study of thermophysical properties of uranium dioxide
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Uranium dioxide; Thermophysical properties; First-principles
calculations
ID HEAT-CAPACITY; THERMAL-CONDUCTIVITY; NUCLEAR-FUELS; DYNAMICS; UO2
AB The structural and elastic properties, lattice dynamics and thermophysical properties of uranium dioxide (UO2) were studied by DFT based first-principles calculations. LDA+U method shows the overall best description of the lattice parameters and elastic constants of UO2 among all the DFT methods studied. The phonon dispersion relations of UO2 predicted by direct method agree with experimental results. Thermodynamic properties, including Gibbs energy, enthalpy, entropy and heat capacity, were evaluated under quasiharmonic approximation using the calculated phonon density of states. Good agreement with experiments is obtained up to 1000 K. Further improvement of heat capacity at high temperatures can be achieved by taking into account of thermal expansion. The calculated lattice thermal conductivity of UO2 shows that phonon scatterings by defects are critical at room temperature while three-phonon interactions dominate the phonon scattering at high temperatures. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Mei, Zhi-Gang; Stan, Marius] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA.
[Yang, Jiong] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.
RP Mei, ZG (reprint author), Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA.
EM zmei@anl.gov
RI Yang, Jiong/K-6330-2014; Mei, Zhi-Gang/D-3333-2012
OI Yang, Jiong/0000-0002-5862-5981; Mei, Zhi-Gang/0000-0002-4249-7532
FU US Department of Energy, Office of Science [DE-AC02-06CH11357]
FX This work was supported by the US Department of Energy, Office of
Science under Contract No. DE-AC02-06CH11357. First-principles
calculations were carried out on LCRC's high performance computing
cluster Fusion and CNM's high performance computing cluster Carbon. ZGM
thanks Boris Dorado for providing specific modules for the VASP code.
NR 36
TC 4
Z9 4
U1 2
U2 47
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
EI 1873-4669
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD AUG 5
PY 2014
VL 603
BP 282
EP 286
DI 10.1016/j.jallcom.2014.03.091
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA AG6CC
UT WOS:000335505100041
ER
PT J
AU Abdul-Jabbar, NM
Kalkan, B
Huang, GY
MacDowell, AA
Gronsky, R
Bourret-Courchesne, ED
Wirth, BD
AF Abdul-Jabbar, N. M.
Kalkan, B.
Huang, G. -Y.
MacDowell, A. A.
Gronsky, R.
Bourret-Courchesne, E. D.
Wirth, B. D.
TI The role of stoichiometric vacancy periodicity in pressure-induced
amorphization of the Ga2SeTe2 semiconductor alloy
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID PHASE-CHANGE MATERIALS; CRYSTAL-STRUCTURE; GA2TE3
AB We observe that pressure-induced amorphization of Ga2SeTe2 (a III-VI semiconductor) is directly influenced by the periodicity of its intrinsic defect structures. Specimens with periodic and semi-periodic two-dimensional vacancy structures become amorphous around 10-11 GPa in contrast to those with aperiodic structures, which amorphize around 7-8 GPa. The result is an instance of altering material phase-change properties via rearrangement of stoichiometric vacancies as opposed to adjusting their concentrations. Based on our experimental findings, we posit that periodic two-dimensional vacancy structures in Ga2SeTe2 provide an energetically preferred crystal lattice that is less prone to collapse under applied pressure. This is corroborated through first-principles electronic structure calculations, which demonstrate that the energy stability of III-VI structures under hydrostatic pressure is highly dependent on the configuration of intrinsic vacancies. (C) 2014 AIP Publishing LLC.
C1 [Abdul-Jabbar, N. M.; Wirth, B. D.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA.
[Abdul-Jabbar, N. M.; Bourret-Courchesne, E. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Kalkan, B.; MacDowell, A. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Huang, G. -Y.; Wirth, B. D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA.
[Gronsky, R.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
RP Abdul-Jabbar, NM (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA.
RI Wirth, Brian/O-4878-2015
OI Wirth, Brian/0000-0002-0395-0285
FU Nuclear Nonproliferation International Safeguards Graduate Fellowship
Program; National Nuclear Security Administration's Next Generation
Safeguards Initiative (NGSI); U.S. Department of Energy/NNSA/NA22;
Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
[DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences,
of the U.S. Department of Energy [DE-AC02-05CH11231]
FX The authors acknowledge C. A. Ramsey for experimental assistance and E.
C. Samulon and G. A. Bizarri for useful discussions. N.M.A. acknowledges
support from the Nuclear Nonproliferation International Safeguards
Graduate Fellowship Program sponsored by the National Nuclear Security
Administration's Next Generation Safeguards Initiative (NGSI). This work
was supported by the U.S. Department of Energy/NNSA/NA22 and carried out
at the Lawrence Berkeley National Laboratory under Contract No.
DE-AC02-05CH11231. Use of the Advanced Photon Source at Argonne National
Laboratory was supported by the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences, under Contract No.
DE-AC02-06CH11357. The Advanced Light Source is supported by the
Director, Office of Science, Office of Basic Energy Sciences, of the
U.S. Department of Energy under Contract No. DE-AC02-05CH11231.
NR 24
TC 2
Z9 2
U1 4
U2 16
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 051908
DI 10.1063/1.4892549
PG 5
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000027
ER
PT J
AU Cobaleda, CSF
Xiao, XY
Burckel, DB
Polsky, R
Huang, DN
Diez, E
Pan, W
AF Cobaleda, Cayetano S. F.
Xiao, Xiaoyin
Burckel, D. Bruce
Polsky, Ronen
Huang, Duanni
Diez, Enrique
Pan, W.
TI Superconducting properties in tantalum decorated three-dimensional
graphene and carbon structures
SO APPLIED PHYSICS LETTERS
LA English
DT Article
AB We present here the results on superconducting properties in tantalum thin films (100 nm thick) deposited on three-dimensional graphene (3DG) and carbon structures. A superconducting transition is observed in both composite thin films with a superconducting transition temperature of 1.2K and 1.0 K, respectively. We have further measured the magnetoresistance at various temperatures and differential resistance dV/dI at different magnetic fields in these two composite thin films. In both samples, a much large critical magnetic field (similar to 2 T) is observed and this critical magnetic field shows linear temperature dependence. Finally, an anomalously large cooling effect was observed in the differential resistance measurements in our 3DG-tantalum device when the sample turns superconducting. Our results may have important implications in flexible superconducting electronic device applications. (C) 2014 AIP Publishing LLC.
C1 [Cobaleda, Cayetano S. F.; Xiao, Xiaoyin; Burckel, D. Bruce; Polsky, Ronen; Huang, Duanni; Pan, W.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Cobaleda, Cayetano S. F.; Diez, Enrique] Univ Salamanca, Lab Bajas Temp, E-37008 Salamanca, Spain.
[Huang, Duanni] Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA.
RP Cobaleda, CSF (reprint author), Sandia Natl Labs, POB 5800,MS 1086, Albuquerque, NM 87185 USA.
EM ccobaleda@usal.es; wpan@sandia.gov
RI ENRIQUE, DIEZ/M-3691-2014
OI ENRIQUE, DIEZ/0000-0001-7964-4148
FU U.S. Department of Energy, Office of Science, Basic Energy Sciences,
Materials Sciences and Engineering Division; LDRD at Sandia; Spanish
MINECO [MAT2013-46308-C2-1-R, FPU-ap2009-2619, JCYL SA226U13]; United
States Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX This work was jointly supported by the U.S. Department of Energy, Office
of Science, Basic Energy Sciences, Materials Sciences and Engineering
Division (C. C., D. H., and W. P.) and by LDRD at Sandia (X. Y. X., D.
B. B., R. P., and W. P.), and also by the Spanish MINECO
MAT2013-46308-C2-1-R (C. C. and E. D.), FPU-ap2009-2619 (C. C.), and
JCYL SA226U13 (C. C. and E. D.). Sandia National Laboratories is a
multi-program laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the United
States Department of Energy's National Nuclear Security Administration
under contract DE-AC04-94AL85000.
NR 19
TC 0
Z9 0
U1 2
U2 21
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 053508
DI 10.1063/1.4892574
PG 4
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000096
ER
PT J
AU Du, Y
Zhang, KHL
Varga, T
Chambers, SA
AF Du, Y.
Zhang, K. H. L.
Varga, T.
Chambers, S. A.
TI Reflection high-energy electron diffraction beam-induced structural and
property changes on WO3 thin films
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID IN-SITU OBSERVATION; TUNGSTEN-OXIDE; TRANSPORT-PROPERTIES;
EPITAXIAL-GROWTH; X-RAY; SURFACE; ELECTROCHROMICS; PHOTOEMISSION;
SPECTROSCOPY; TRANSITION
AB Reduction of transition metal oxides can greatly change their physical and chemical properties. Using deposition of WO3 as a case study, we demonstrate that reflection high-energy electron diffraction (RHEED), a surface-sensitive tool widely used to monitor thin-film deposition processes, can significantly affect the cation valence and physical properties of the films through electron-beam induced sample reduction. The RHEED beam is found to increase film smoothness during epitaxial growth of WO3, as well as change the electronic properties of the film through preferential removal of surface oxygen. (C) 2014 AIP Publishing LLC.
C1 [Du, Y.; Varga, T.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[Zhang, K. H. L.; Chambers, S. A.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
RP Du, Y (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
EM yingge.du@pnnl.gov
FU Office of Basic Energy Sciences, Division of Materials Science and
Engineering [10122]; EMSL's Intramural Research and Capability
Development Program; Office of Biological and Environmental Research
FX A portion of the work was supported by the Office of Basic Energy
Sciences, Division of Materials Science and Engineering, under Award
10122. Y.D. gratefully acknowledges support by EMSL's Intramural
Research and Capability Development Program. The work was performed at
the W. R. Wiley Environmental Molecular Sciences Laboratory, a DOE User
Facility sponsored by the Office of Biological and Environmental
Research. The authors would like to thank Tiffany Kaspar and Tim Droubay
for many insightful discussions.
NR 41
TC 2
Z9 2
U1 6
U2 28
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 051606
DI 10.1063/1.4892810
PG 4
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000019
ER
PT J
AU Duenow, JN
Burst, JM
Albin, DS
Kuciauskas, D
Johnston, SW
Reedy, RC
Metzger, WK
AF Duenow, J. N.
Burst, J. M.
Albin, D. S.
Kuciauskas, D.
Johnston, S. W.
Reedy, R. C.
Metzger, W. K.
TI Single-crystal CdTe solar cells with V-oc greater than 900 mV
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID PHOTO-VOLTAIC PROPERTIES; VAPOR-PHASE EPITAXY; CADMIUM TELLURIDE;
SPRAY-PYROLYSIS; PHOTOVOLTAIC PROPERTIES; HETEROJUNCTIONS; JUNCTIONS;
CONTACTS; SURFACE; FILMS
AB We fabricated single-crystal CdTe photovoltaic devices in a heterojunction structure with an In-doped CdS window layer and ZnO/Al-doped ZnO front contact. By replacing the polycrystalline absorber layer of a CdTe solar cell with a single crystal, we were able to achieve open-circuit voltage (V-oc) as high as 929 mV. Simulations and measurements indicate that increased minority-carrier lifetime and carrier concentration can explain this high V-oc. Cu and Na both introduce transient effects in single-crystal CdTe similar to those observed in polycrystalline CdTe, suggesting that Group I dopants pose stability problems that are linked fundamentally to their defect chemistry in CdTe, regardless of the presence of grain boundaries. (C) 2014 AIP Publishing LLC.
C1 [Duenow, J. N.; Burst, J. M.; Albin, D. S.; Kuciauskas, D.; Johnston, S. W.; Reedy, R. C.; Metzger, W. K.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Duenow, JN (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM joel.duenow@nrel.gov
FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable
Energy Laboratory
FX The authors would like to thank Anna Duda and Clay M. DeHart for contact
depositions. This work was supported by the U.S. Department of Energy
under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy
Laboratory.
NR 37
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U1 3
U2 52
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 053903
DI 10.1063/1.4892401
PG 4
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000103
ER
PT J
AU Kiesow, KI
Dhuey, S
Habteyes, TG
AF Kiesow, Karissa I.
Dhuey, Scott
Habteyes, Terefe G.
TI Mapping near-field localization in plasmonic optical nanoantennas with
10 nm spatial resolution
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID ENHANCED RAMAN-SCATTERING; METAL NANOPARTICLE PAIRS; HOT-SPOTS;
MICROSCOPY; SIZE; SERS; RESONANCES; MOLECULES; ANTENNA; PROBE
AB Quantifying the near-field localization in plasmonic optical nanoantennas is fundamentally important to understand and optimize the design and fabrication of nanostructures for various applications. Here, the near-field localization in optical gap nanoantennas that are in resonance or near-resonance with 633 nm excitation wavelength is directly visualized in real space with 10 nm spatial resolutions, mapping the amplitude and phase characteristics of the in-plane and out-of-plane vector components selectively. While large field amplitude is observed in the gap for the in-plane component, the narrow gaps that are not resolved in the topographic image have been clearly observed in the optical images when the out-of-plane component is mapped, suggesting that the lateral optical resolution can surpass the radius of curvature of the probing tip. The effects of various structural parameters and metallic adhesion layer on the extent of field localization have been discussed, providing important insight in designing and fabricating plasmonic optical devices. (C) 2014 AIP Publishing LLC.
C1 [Kiesow, Karissa I.; Habteyes, Terefe G.] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA.
[Kiesow, Karissa I.; Habteyes, Terefe G.] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87131 USA.
[Dhuey, Scott] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
RP Kiesow, KI (reprint author), Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA.
RI Foundry, Molecular/G-9968-2014
FU Office of Science, Office of Basic Energy Sciences, of the U.S.
Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy
Office of Science by Los Alamos National Laboratory [DE-AC52-06NA25396];
Sandia National Laboratories [DE-AC04-94AL85000]
FX The fabrication of the nanostructures was performed as a user project at
the Molecular Foundry, Lawrence Berkeley National Laboratory, which was
supported by the Office of Science, Office of Basic Energy Sciences, of
the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. For
some of the samples, the evaporation of gold was carried out at the
Center for Integrated Nanotechnologies, an Office of Science User
Facility operated for the U.S. Department of Energy Office of Science by
Los Alamos National Laboratory (Contract No. DE-AC52-06NA25396) and
Sandia National Laboratories (Contract No. DE-AC04-94AL85000).
NR 36
TC 1
Z9 1
U1 1
U2 36
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 053105
DI 10.1063/1.4892577
PG 5
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000071
ER
PT J
AU Mickel, PR
Lohn, AJ
Marinella, MJ
AF Mickel, Patrick R.
Lohn, Andrew J.
Marinella, Matthew J.
TI Detection and characterization of multi-filament evolution during
resistive switching
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID ACCURATE EXPERIMENTAL-DETERMINATION; WEIBULL SHAPE FACTOR; INTRINSIC
BREAKDOWN; DIELECTRIC FILMS; MEMORIES
AB We report resistive switching data in TaOx memristors displaying signatures of multi-filament switching modes and present a technique which enables the characterization of the evolution of multiple filaments within a single device during switching, including their temperature, heat flow, conductivity, and time evolving areas. Using a geometrically defined equivalent circuit, we resolve the individual current/voltage values of each filament and demonstrate that the switching curves of each filament collapse onto a common curve determined by the analytical steady-state resistive switching solution for filamentary switching. Finally, we discuss operational modes which may limit the formation of additional conducting filaments, potentially leading to increased device endurance. (C) 2014 AIP Publishing LLC.
C1 [Mickel, Patrick R.; Lohn, Andrew J.; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Mickel, PR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
FU Sandia's Laboratory Directed Research and Development program; U.S.
Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX We would like to acknowledge James E. Stevens and the Sandia MESA Fab
for device fabrication. This work was funded by Sandia's Laboratory
Directed Research and Development program. Sandia National Laboratories
is a multi-program laboratory managed and operated by Sandia
Corporation, a wholly owned subsidiary of Lockheed Martin Corporation,
for the U.S. Department of Energy's National Nuclear Security
Administration under Contract DE-AC04-94AL85000.
NR 20
TC 3
Z9 3
U1 2
U2 39
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 053503
DI 10.1063/1.4892471
PG 4
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000091
ER
PT J
AU Odbadrakh, K
McNutt, NW
Nicholson, DM
Rios, O
Keffer, DJ
AF Odbadrakh, Khorgolkhuu
McNutt, N. W.
Nicholson, D. M.
Rios, O.
Keffer, D. J.
TI Lithium diffusion at Si-C interfaces in silicon-graphene composites
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID LI-ION BATTERIES; DENSITY-FUNCTIONAL THEORY; CRYSTALLINE SILICON;
ELECTROCHEMICAL PERFORMANCE; 1ST PRINCIPLES; ANODES; INTERCALATION;
ADSORPTION; LITHIATION; GRAPHITE
AB Models of intercalated Li and its diffusion in Si-Graphene interfaces are investigated using density functional theory. Results suggest that the presence of interfaces alters the energetics of Li binding and diffusion significantly compared to bare Si or Graphene surfaces. Our results show that cavities along reconstructed Si surface provide diffusion paths for Li. Diffusion barriers calculated along these cavities are significantly lower than penetration barriers to bulk Si. Interaction with Si surface results in graphene defects, creating Li diffusion paths that are confined along the cavities but have still lower barrier than in bulk Si. (C) 2014 AIP Publishing LLC.
C1 [Odbadrakh, Khorgolkhuu] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37830 USA.
[McNutt, N. W.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA.
[Nicholson, D. M.] Oak Ridge Natl Lab, Computat Sci & Math Div, Oak Ridge, TN 37830 USA.
[Nicholson, D. M.] Univ N Carolina, Dept Phys, Asheville, NC 28804 USA.
[Rios, O.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA.
[Keffer, D. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.
RP Odbadrakh, K (reprint author), Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37830 USA.
RI Rios, Orlando/E-6856-2017
OI Rios, Orlando/0000-0002-1814-7815
FU JDRD program at the University of Tennessee; Oak Ridge Associated
Universities High Performance Computing Program; Sustainable Energy
Education and Research Center of the University of Tennessee; National
Science Foundation [DGE-0801470]; NSF [OCI 07-11134.5]; Laboratory
Directed Research and Development Program of Oak Ridge National
Laboratory
FX K.O. was supported by a grant from the JDRD program at the University of
Tennessee. N.M. was supported by a grant from the Oak Ridge Associated
Universities High Performance Computing Program, by a grant from the
Sustainable Energy Education and Research Center of the University of
Tennessee and by a grant from the National Science Foundation
(DGE-0801470). This research project used resources of the National
Institute for Computational Sciences (NICS) supported by NSF under
Agreement No. OCI 07-11134.5. This research was also sponsored in part
by the Laboratory Directed Research and Development Program of Oak Ridge
National Laboratory, managed by UT-Battelle, LLC, for the U. S.
Department of Energy.
NR 41
TC 0
Z9 0
U1 8
U2 84
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 053906
DI 10.1063/1.4892829
PG 4
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000106
ER
PT J
AU Perret, E
Highland, MJ
Stephenson, GB
Streiffer, SK
Zapol, P
Fuoss, PH
Munkholm, A
Thompson, C
AF Perret, Edith
Highland, M. J.
Stephenson, G. B.
Streiffer, S. K.
Zapol, P.
Fuoss, P. H.
Munkholm, A.
Thompson, Carol
TI Real-time x-ray studies of crystal growth modes during metal-organic
vapor phase epitaxy of GaN on c- and m-plane single crystals
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID LIGHT-EMITTING-DIODES; SURFACE-STRUCTURE; DEPOSITION; SCATTERING;
ENVIRONMENT; SILICON
AB Non-polar orientations of III-nitride semiconductors have attracted significant interest due to their potential application in optoelectronic devices with enhanced efficiency. Using in situ surface x-ray scattering during metal-organic vapor phase epitaxy (MOVPE) of GaN on non-polar (m-plane) and polar (c-plane) orientations of single crystal substrates, we have observed the homoepitaxial growth modes as a function of temperature and growth rate. On the m-plane surface, we observe all three growth modes (step-flow, layer-by-layer, and three-dimensional) as conditions are varied. In contrast, the +c-plane surface exhibits a direct crossover between step-flow and 3D growth, with no layer-by-layer regime. The apparent activation energy of 2.8 +/- 0.2 eV observed for the growth rate at the layer-by-layer to step-flow boundary on the m-plane surface is consistent with those observed for MOVPE growth of other III-V compounds, indicating a large critical nucleus size for islands. (C) 2014 AIP Publishing LLC.
C1 [Perret, Edith; Highland, M. J.; Stephenson, G. B.; Zapol, P.; Fuoss, P. H.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Stephenson, G. B.; Streiffer, S. K.] Argonne Natl Lab, Photon Sci Directorate, Argonne, IL 60439 USA.
[Streiffer, S. K.] Argonne Natl Lab, Phys Sci & Engn Directorate, Argonne, IL 60439 USA.
[Munkholm, A.] AIXTRON Inc, Sunnyvale, CA 94089 USA.
[Thompson, Carol] Univ Illinois, Dept Phys, De Kalb, IL 60115 USA.
RP Highland, MJ (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM mhighland@anl.gov
RI Zapol, Peter/G-1810-2012;
OI Zapol, Peter/0000-0003-0570-9169; Thompson, Carol/0000-0003-3832-4855
FU U.S. Department of Energy, Office of Science, Basic Energy Sciences;
U.S. Department of Energy, Office of Science, Basic Energy Sciences,
Materials Sciences and Engineering Division
FX The authors would like to acknowledge all of those who have contributed
to the MOVPE facility at APS sector 12. GBS, SKS, and the use of the
Advanced Photon Source were supported by the U.S. Department of Energy,
Office of Science, Basic Energy Sciences. PZ, PHF, and CT were supported
by the U.S. Department of Energy, Office of Science, Basic Energy
Sciences, Materials Sciences and Engineering Division.
NR 19
TC 3
Z9 3
U1 3
U2 23
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 051602
DI 10.1063/1.4892349
PG 3
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000015
ER
PT J
AU Wong, AT
Beekman, C
Guo, H
Siemons, W
Gai, Z
Arenholz, E
Takamura, Y
Ward, TZ
AF Wong, A. T.
Beekman, C.
Guo, H.
Siemons, W.
Gai, Z.
Arenholz, E.
Takamura, Y.
Ward, T. Z.
TI Strain driven anisotropic magnetoresistance in antiferromagnetic
La0.4Sr0.6MnO3
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID PHASE-SEPARATED MANGANITE; THIN-FILMS; TRANSITIONS; DEVICES; FIELD
AB We investigate the effects of strain on antiferromagnetic (AFM) single crystal thin films of La1-xSrxMnO3 (x = 0.6). Nominally unstrained samples have strong magnetoresistance with anisotropic magnetoresistances (AMR) of up to 8%. Compressive strain suppresses magnetoresistance but generates AMR values of up to 63%. Tensile strain presents the only case of a metal-insulator transition and demonstrates a previously unreported AMR behavior. In all three cases, we find evidence of magnetic ordering and no indication of a global ferromagnetic phase transition. These behaviors are attributed to epitaxy induced changes in orbital occupation driving different magnetic ordering types. Our findings suggest that different AFM ordering types have a profound impact on the AMR magnitude and character. (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Wong, A. T.; Beekman, C.; Guo, H.; Siemons, W.; Ward, T. Z.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
[Wong, A. T.] Univ Tennessee, Knoxville, TN 37996 USA.
[Guo, H.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Gai, Z.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Takamura, Y.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA.
RP Ward, TZ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
EM wardtz@ornl.gov
RI Gai, Zheng/B-5327-2012; Ward, Thomas/I-6636-2016
OI Gai, Zheng/0000-0002-6099-4559; Ward, Thomas/0000-0002-1027-9186
FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences (BES),
Materials Sciences and Engineering Division; U.S. DOE [DE-SC0002136];
Scientific User Facilities Division, Office of BES, U.S. DOE; Office of
Science, Office of BES, of the U.S. DOE [DE-AC02-05CH11231]; National
Science Foundation [DMR 0747896]
FX This effort was supported by the U.S. Department of Energy (DOE), Office
of Basic Energy Sciences (BES), Materials Sciences and Engineering
Division, (T.Z.W., C.B., and W.S.) and under U.S. DOE grant DE-SC0002136
(A.W. and H.W.G.). Magnetization measurements (Z.G.) were conducted at
the Center for Nanophase Materials Sciences, which is sponsored at Oak
Ridge National Laboratory by the Scientific User Facilities Division,
Office of BES, U.S. DOE. The Advanced Light Source is supported by the
Direction, Office of Science, Office of BES, of the U.S. DOE under
Contract No. DE-AC02-05CH11231. Y.T. acknowledges the support of the
National Science Foundation Contract No. DMR 0747896.
NR 29
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Z9 5
U1 6
U2 47
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 052401
DI 10.1063/1.4892420
PG 5
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000040
ER
PT J
AU Zhu, GH
Wiederrecht, GP
Ling, C
Wu, ST
Banerjee, D
Yano, K
AF Zhu, Gaohua
Wiederrecht, Gary P.
Ling, Chen
Wu, Songtao
Banerjee, Debasish
Yano, Kazuhisa
TI Damping of coherent acoustic vibrations by nanosized pores in colloidal
hypersonic crystals
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID MESOPOROUS SILICA SPHERES; METAL NANOPARTICLES; GOLD NANOPARTICLES;
QUANTUM-WELLS; OSCILLATIONS; MODULATION; DYNAMICS; WAVES
AB We investigated the damping of the coherent acoustic vibrations in the presence of the nanosized pores in colloidal hypersonic crystals. The colloidal crystal samples are comprised of close-packed silica or monodisperse mesoporous silica spheres, where the mesoporous silica sphere contains radially aligned uniform nanosized pores. The decay of the acoustic vibrations was monitored by using ultrafast pump-probe spectroscopy. Two types of coherent acoustic modes are observed, the propagating bulk mode and the localized surface mode. Our studies show that porous structure could have different effects on different modes of vibrations. While the bulk mode is heavily damped due to the scattering from the nanosized pores, the surface mode is much less influenced. (C) 2014 AIP Publishing LLC.
C1 [Zhu, Gaohua; Ling, Chen; Wu, Songtao; Banerjee, Debasish; Yano, Kazuhisa] Toyota Res Inst North Amer, Mat Res Dept, Ann Arbor, MI 48105 USA.
[Wiederrecht, Gary P.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Yano, Kazuhisa] Toyota Cent Res & Dev Labs Inc, Inorgan Mat Lab, Nagakute, Aichi 4801192, Japan.
RP Zhu, GH (reprint author), Toyota Res Inst North Amer, Mat Res Dept, Ann Arbor, MI 48105 USA.
EM gaohua.zhu@tema.toyota.com; k-yano@mosk.tytlabs.co.jp
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]
FX Use of the Center for Nanoscale Materials was supported by the U.S.
Department of Energy, Office of Science, Office of Basic Energy
Sciences, under Contract No. DE-AC02-06CH11357.
NR 34
TC 0
Z9 0
U1 4
U2 18
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 051903
DI 10.1063/1.4892428
PG 5
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000022
ER
PT J
AU Zou, T
Dun, ZL
Cao, HB
Zhu, MZ
Coulter, D
Zhou, HD
Ke, XL
AF Zou, Tao
Dun, Zhiling
Cao, Huibo
Zhu, Mengze
Coulter, Daniel
Zhou, Haidong
Ke, Xianglin
TI Excess-hole induced high temperature polarized state and its correlation
with the multiferroicity in single crystalline DyMnO3
SO APPLIED PHYSICS LETTERS
LA English
DT Article
ID FERROELECTRICITY
AB Controlling the ferroelectricity and magnetism in multiferroic materials has been an important research topic. We report the formation of a highly polarized state in multiferroic DyMnO3 single crystals which develops well above the magnetic transition temperatures, and we attribute it to the thermally stimulated depolarization current effect of excess holes forming Mn4+ ions in the system. We also show that this high temperature polarized state intimately correlates with the lower temperature ferroelectric state that is induced by the incommensurate spiral magnetic order of Mn spins. This study demonstrates an efficient approach to tune the multiferroicity in the manganite system. (C) 2014 AIP Publishing LLC.
C1 [Zou, Tao; Zhu, Mengze; Coulter, Daniel; Ke, Xianglin] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
[Dun, Zhiling; Zhou, Haidong] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.
[Cao, Huibo] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA.
RP Ke, XL (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
EM ke@pa.msu.edu
RI Zou, Tao/A-1761-2013; Cao, Huibo/A-6835-2016; Dun, Zhiling/F-5617-2016;
Zhou, Haidong/O-4373-2016
OI Zou, Tao/0000-0002-6510-5749; Cao, Huibo/0000-0002-5970-4980; Dun,
Zhiling/0000-0001-6653-3051;
FU Michigan State University; NSF-DMR [DMR-1350002]; Scientific User
Facilities Division, Office of Basic Energy Sciences, U.S. Department of
Energy
FX X.K. acknowledges the support from the start-up funds at Michigan State
University. Z. L. Dun and H. D. Z. thank for the support from NSF-DMR
through Award DMR-1350002. Work at ORNL was sponsored by the Scientific
User Facilities Division, Office of Basic Energy Sciences, U.S.
Department of Energy. T. Z. appreciates the useful discussion with
Professor J. M. Liu.
NR 28
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Z9 6
U1 1
U2 19
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
EI 1077-3118
J9 APPL PHYS LETT
JI Appl. Phys. Lett.
PD AUG 4
PY 2014
VL 105
IS 5
AR 052906
DI 10.1063/1.4892470
PG 5
WC Physics, Applied
SC Physics
GA AO2LE
UT WOS:000341153000061
ER
PT J
AU Jiang, T
Xu, CF
Zuo, XB
Conticello, VP
AF Jiang, Tao
Xu, Chunfu
Zuo, Xiaobing
Conticello, Vincent P.
TI Structurally Homogeneous Nanosheets from Self-Assembly of a
Collagen-Mimetic Peptide
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE collagen-mimetic peptides; nanoarchitectonics; nanosheets;
self-assembly; structural homogeneity
ID TRIPLE-HELICAL STRUCTURES; CRYSTAL-STRUCTURE; MOLECULAR-STRUCTURE;
CONFORMATIONAL STABILITY; ANGSTROM RESOLUTION; MODEL PEPTIDE; GLY
SEQUENCE; 4-HYDROXYPROLINE; NANOARCHITECTONICS; 4-FLUOROPROLINE
AB A collagen-mimetic peptide, NSIII, has been designed with three sequential blocks having positive, neutral, and negative charges, respectively. The non-canonical imino acid, (2S, 4S)-4-aminoproline (amp), was used to specify the positive charges at the Xaa positions of (Xaa-Yaa-Gly) triads in the N-terminal domain of NSIII. Peptide NSIII underwent self-assembly from aqueous solution to form a highly homogeneous population of nanosheets. Two-dimensional crystalline sheets formed in which the length of the peptide defined the height of the sheets. These results contrasted with prior results on a similar multi-domain collagen-mimetic polypeptides in which the sheets had highly polydisperse distribution of sizes in the (x/y)- and (z)-dimensions. The structural differences between the two nanosheet assemblies were interpreted in terms of the relative stereoelectronic effects of the different aminoproline derivatives on the local triple helical conformation of the peptides.
C1 [Jiang, Tao; Xu, Chunfu; Conticello, Vincent P.] Emory Univ, Dept Chem, Atlanta, GA 30322 USA.
[Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA.
RP Conticello, VP (reprint author), Emory Univ, Dept Chem, 1515 Dickey Dr, Atlanta, GA 30322 USA.
EM vcontic@emory.edu
FU NSF [CHE-1012620]; U.S. D.O.E. Office of Basic Energy Sciences, Division
of Material Sciences [W-31-109-Eng-38]
FX V.P.C. acknowledges financial support from NSF grant CHE-1012620. This
work benefited from the use of the A.P.S. funded by U.S. D.O.E. Office
of Basic Energy Sciences, Division of Material Sciences, under contract
W-31-109-Eng-38. We thank Prof. Shuming Nie for use of the dynamic light
scattering instrument.
NR 37
TC 23
Z9 23
U1 7
U2 69
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD AUG 4
PY 2014
VL 53
IS 32
BP 8367
EP 8371
DI 10.1002/anie.201403780
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA AN3XT
UT WOS:000340522700016
PM 24961508
ER
PT J
AU Polinski, MJ
Pace, KA
Stritzinger, JT
Lin, J
Cross, JN
Cary, SK
Van Cleve, SM
Alekseev, EV
Albrecht-Schmitt, TE
AF Polinski, Matthew J.
Pace, Kristen A.
Stritzinger, Jared. T.
Lin, Jian
Cross, Justin N.
Cary, Samantha K.
Van Cleve, Shelley M.
Alekseev, Evgeny V.
Albrecht-Schmitt, Thomas E.
TI Chirality and Polarity in the f-Block Borates
M-4[B16O26(OH)(4)(H2O)(3)Cl-4] ( M = Sm, Eu, Gd, Pu, Am, Cm, and Cf)
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE actinides; americium; californium; curium; lanthanides; plutonium
ID ELECTRONIC ENERGY LEVELS; LANTHANIDE AQUO IONS; TRIVALENT ACTINIDE;
SPECTROSCOPIC PROPERTIES; SPECTRAL INTENSITIES; CRYSTAL-STRUCTURES;
SINGLE-CRYSTAL; SOLID-STATE; TH-CM; PLUTONIUM(III)
AB The reactions of trivalent lanthanides and actinides with molten boric acid in high chloride concentrations result in the formation of M-4[B16O26(OH)(4)(H2O)(3)Cl-4] (M = Sm, Eu, Gd, Pu, Am, Cm, Cf). This cubic structure type is remarkably complex and displays both chirality and polarity. The polymeric borate network forms helical features that are linked via two different types of nine-coordinate f-element environments. The f-f transitions are unusually intense and result in dark coloration of these compounds with actinides.
C1 [Polinski, Matthew J.; Pace, Kristen A.; Stritzinger, Jared. T.; Lin, Jian; Cross, Justin N.; Cary, Samantha K.; Albrecht-Schmitt, Thomas E.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA.
[Alekseev, Evgeny V.] Forschungszentrum Julich, Inst Energy & Climate Res IEK 6, D-52428 Julich, Germany.
[Alekseev, Evgeny V.] Univ Aachen, Inst Kristallog, Rhein Westfael TH, D-52066 Aachen, Germany.
[Van Cleve, Shelley M.] Oak Ridge Natl Lab, Nucl Mat Proc Grp, Oak Ridge, TN 37830 USA.
RP Albrecht-Schmitt, TE (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA.
OI Alekseev, Evgeny/0000-0002-4919-5211
FU Heavy Elements Chemistry Program, U.S. Department of Energy
[DE-FG02-13ER16414]
FX We are grateful for support provided by the Heavy Elements Chemistry
Program, U.S. Department of Energy, under Grant DE-FG02-13ER16414. The
249Cf was provided to Florida State University by the Isotope
Development and Production for Research and Applications Program through
the Radiochemical Engineering and Development Center at Oak Ridge
National Laboratory and was purchased by the Gregory R. Choppin Chair
Endowment. The 249Cf used in this research was supplied by
the United States Department of Energy Office of Science by the Isotope
Program in the Office of Nuclear Physics.
NR 49
TC 4
Z9 4
U1 3
U2 24
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
EI 1521-3765
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD AUG 4
PY 2014
VL 20
IS 32
BP 9892
EP 9896
DI 10.1002/chem.201403820
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA AN0ES
UT WOS:000340257000011
PM 25042434
ER
PT J
AU Sturzbecher-Hoehne, M
Kullgren, B
Jarvis, EE
An, DD
Abergel, RJ
AF Sturzbecher-Hoehne, Manuel
Kullgren, Birgitta
Jarvis, Erin E.
An, Dahlia D.
Abergel, Rebecca J.
TI Highly Luminescent and Stable Hydroxypyridinonate Complexes: A Step
Towards New Curium Decontamination Strategies
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE actinides; curium; energy transfer; luminescence; thermodynamics
ID RADIONUCLIDE DECORPORATION AGENTS; IN-VIVO; THERMODYNAMIC EVALUATION;
LANTHANIDE COMPLEXES; SEQUESTERING AGENTS; AQUEOUS-SOLUTION; LIGANDS;
CHELATION; 3,4,3-LI(1,2-HOPO); IONS
AB The photophysical properties, solution thermodynamics, and in vivo complex stabilities of Cm-III complexes formed with multidentate hydroxypyridinonate ligands, 3,4,3-LI(1,2-HOPO) and 5-LIO(Me-3,2-HOPO), are reported. Both chelators were investigated for their ability to act as antenna chromophores for Cm-III, leading to highly sensitized luminescence emission of the metal upon complexation, with long lifetimes (383 and 196 mu s for 3,4,3-LI(1,2-HOPO) and 5-LIO(Me-3,2-HOPO), respectively) and remarkable quantum yields (45% and 16%, respectively) in aqueous solution. The bright emission peaks were used to probe the electronic structure of the 5f complexes and gain insight into ligand field effects; they were also exploited to determine the high (and proton-independent) stabilities of the corresponding Cm-III complexes (log beta(110)=21.8(4) for 3,4,3-LI(1,2-HOPO) and log beta(120)=24.5(5) for 5-LIO(Me-3,2-HOPO)). The in vivo complex stability for both ligands was assessed by using Cm-248 as a tracer in a rodent model, which provided a direct comparison with the in vitro thermodynamic results and demonstrated the great potential of 3,4,3-LI(1,2-HOPO) as a therapeutic Cm-III decontamination agent.
C1 [Sturzbecher-Hoehne, Manuel; Kullgren, Birgitta; Jarvis, Erin E.; An, Dahlia D.; Abergel, Rebecca J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
RP Abergel, RJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.
EM rjabergel@lbl.gov
FU Office of Science, Office of Basic Energy Sciences, and the Division of
Chemical Sciences, Geosciences, and Biosciences of the U.S. Department
of Energy at LBNL [DE-AC02-05CH11231]; National Institutes of Health
through the U.S. Department of Energy [DE-AC02-05CH11231, RAI087604Z]
FX We thank Prof. Kenneth N. Raymond, Dr. Norman M. Edelstein, and Dr.
David K. Shuh for helpful discussions. Spectroscopic characterization of
Cm complexes and solution thermodynamic studies were supported by the
Director, Office of Science, Office of Basic Energy Sciences, and the
Division of Chemical Sciences, Geosciences, and Biosciences of the U.S.
Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. The
in vivo experiments were supported by the National Institutes of Health
(RAI087604Z) through the U.S. Department of Energy under Contract No.
DE-AC02-05CH11231.
NR 48
TC 9
Z9 9
U1 3
U2 24
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
EI 1521-3765
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD AUG 4
PY 2014
VL 20
IS 32
BP 9962
EP 9968
DI 10.1002/chem.201402103
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA AN0ES
UT WOS:000340257000021
PM 25043376
ER
PT J
AU Morrow, R
Freeland, JW
Woodward, PM
AF Morrow, Ryan
Freeland, John W.
Woodward, Patrick M.
TI Probing the Links between Structure and Magnetism in Sr2-xCaxFeOsO6
Double Perovskites
SO INORGANIC CHEMISTRY
LA English
DT Article
ID ORDERED DOUBLE-PEROVSKITE; CRYSTAL-STRUCTURE; TEMPERATURE; DIFFRACTION;
SR2FEOSO6; OSMIUM
AB synthesis, structure, and properties of the ordered double perovskites Sr2FeOsO6, Ca2FeOsO6, and SrCaFeOsO6 are reported. The latter two compounds have monoclinic P2(1)/n symmetry and a(-)a(-)b(+) tilting of the octahedra, while Sr2FeOsO6 is tetragonal with 14/m symmetry and a(0)a(0)c(-) tilting. Magnetic measurements indicate and neutron powder diffraction studies confirm that Ca2FeOsO6 is a ferrimagnet with a Curie temperature of 350 K. The ferrimagnetism is retained if half of the Ca2+ ions are replaced with larger Sr2+ ions to form SrCaFeOsO6 (Tc = 210 K). This substitution reduces the degree of octahedral tilting, but unlike most perovskites, the magnetic ordering temperature decreases as the Fe-O-Os bond angles approach a linear geometry. In contrast, Sr2FeOsO6 orders antiferromagnetically, as previously reported. X-ray absorption spectroscopy confirms the assignment of Fe(III) and Os(V) oxidation states for all three compounds. In these insulating double perovskites, the magnetic ground state is governed by a competition between the fourbond Fe-O-Os-O-Fe antiferromagnetic superexchange coupling of Fe(III) ions and the two-bond Fe-O-Os antiferromagnetic superexchange coupling between neighboring Fe(III) and Os(V) ions. When the Fe-O-Os bonds are linear, as they are in the c direction in Sr2FeOsO6, the four-bond coupling between Fe(III) ions prevails. The competition shifts in favor of antiferromagnetic coupling of Fe(III) and Os(V) as the Fe-O-Os bond angles bend in response to chemical pressure.
C1 [Morrow, Ryan; Woodward, Patrick M.] Ohio State Univ, Dept Chem & Biochem, Columbus, OH 43210 USA.
[Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Woodward, PM (reprint author), Ohio State Univ, Dept Chem & Biochem, Columbus, OH 43210 USA.
EM woodward@chemistry.ohio-state.edu
RI Morrow, Ryan/K-9668-2015
OI Morrow, Ryan/0000-0001-9986-3049
FU Materials World Network Grant - National Science Foundation
[DMR-1107637]; Center for Emergent Materials an NSF Materials Research
Science and Engineering Center [DMR-0820414]; U.S. Department of Energy,
Office of Basic Energy Sciences; U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX Support for this research was provided by a Materials World Network
Grant funded by the National Science Foundation (award no. DMR-1107637).
Partial support was supplied by the Center for Emergent Materials an NSF
Materials Research Science and Engineering Center (DMR-0820414). A
portion of this research was carried out at Oak Ridge National
Laboratory's Spallation Neutron Source, which is sponsored by the U.S.
Department of Energy, Office of Basic Energy Sciences. The authors thank
Ashfia Huq for assistance with the neutron diffraction experiments. Use
of the Advanced Photon Source was supported by the U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences, under
contract no. DE-AC02-06CH11357.
NR 34
TC 18
Z9 18
U1 6
U2 48
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 4
PY 2014
VL 53
IS 15
BP 7983
EP 7992
DI 10.1021/ic5006715
PG 10
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA AM6NR
UT WOS:000339982400025
PM 25025612
ER
PT J
AU Bacchi, M
Berggren, G
Niklas, J
Veinberg, E
Mara, MW
Shelby, ML
Poluektov, OG
Chen, LX
Tiede, DM
Cavazza, C
Field, MJ
Fontecave, M
Artero, V
AF Bacchi, Marine
Berggren, Gustav
Niklas, Jens
Veinberg, Elias
Mara, Michael W.
Shelby, Megan L.
Poluektov, Oleg G.
Chen, Lin X.
Tiede, David M.
Cavazza, Christine
Field, Martin J.
Fontecave, Marc
Artero, Vincent
TI Cobaloxime-Based Artificial Hydrogenases
SO INORGANIC CHEMISTRY
LA English
DT Article
ID PHOTOSYSTEM-I; MOLECULAR ELECTROCATALYSTS; ELECTRONIC-STRUCTURE;
FUNCTIONAL MODELS; OXYGEN CARRIERS; H-2 EVOLUTION; APO-MYOGLOBIN;
ACTIVE-SITES; PROTEIN; DESIGN
AB Cobaloximes are popular H-2 evolution molecular catalysts but have so far mainly been studied in nonaqueous conditions. We show here that they are also valuable for the design of artificial hydrogenases for application in neutral aqueous solutions and report on the preparation of two well-defined biohybrid species via the binding of two cobaloxime moieties, {Co(dmgH)(2)} and {Co(dmgBF(2))(2)} (dmgH(2) = dimethylglyoxime), to apo Sperm-whale myoglobin (SwMb). All spectroscopic data confirm that the cobaloxime moieties are inserted within the binding pocket of the SwMb protein and are coordinated to a histidine residue in the axial position of the cobalt complex, resulting in thermodynamically stable complexes. Quantum chemical/molecular mechanical docking calculations indicated a coordination preference for His93 over the other histidine residue (His64) present in the vicinity. Interestingly, the redox activity of the cobalt centers is retained in both biohybrids, which provides them with the catalytic activity for H-2 evolution near-neutral aqueous conditions. in
C1 [Bacchi, Marine; Berggren, Gustav; Cavazza, Christine; Fontecave, Marc; Artero, Vincent] Univ Grenoble Alpes, Lab Chem & Biol Met, CNRS, CEA, F-38000 Grenoble, France.
[Niklas, Jens; Poluektov, Oleg G.; Chen, Lin X.; Tiede, David M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Veinberg, Elias; Field, Martin J.] Univ Grenoble Alpes, CEA 5075, UMR CNRS, DYNAMO,DYNAMOP,Inst Biol Struct, F-38000 Grenoble, France.
[Mara, Michael W.; Shelby, Megan L.; Chen, Lin X.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
[Fontecave, Marc] Univ Paris 06, CNRS, Coll France, Lab Chim Proc Biol,UMR 8229, F-75005 Paris, France.
RP Artero, V (reprint author), Univ Grenoble Alpes, Lab Chem & Biol Met, CNRS, CEA, 17 Rue Martyrs, F-38000 Grenoble, France.
EM vincent.artero@cea.fr
RI berggren, gustav/H-8659-2013; Artero, Vincent/C-6853-2008; Niklas,
Jens/I-8598-2016
OI berggren, gustav/0000-0002-6717-6612; Artero,
Vincent/0000-0002-6148-8471; Niklas, Jens/0000-0002-6462-2680
FU French National Research Agency (ANR, NiFe-Cat project)
[ANR-10-BLAN-711,]; French National Research Agency (ANR, Labex program
ARCANE) [ANR-11-LABX-0003-01]; COST Action [CM1202 PERSPECT-H2O]; Life
Science Division of the CEA (Irtelis program); Life Science Division of
the CEA (DSV-Energy program); Bengt Lundqvist minnesfond; FORMAS
[213-2010-563]; Swedish Royal Academy of Sciences; Division of Chemical
Sciences, Biosciences, Office of Basic Energy Sciences of the U.S.
Department of Energy [DE-AC02-06CH11357]
FX The authors acknowledge partial support from the French National
Research Agency (ANR, NiFe-Cat project; Grant ANR-10-BLAN-711, and Labex
program ARCANE; Grant ANR-11-LABX-0003-01), the COST Action CM1202
PERSPECT-H2O, and the Life Science Division of the CEA
(Irtelis and 2011 DSV-Energy programs). G.B. gratefully acknowledges
support from Bengt Lundqvist minnesfond, FORMAS (Contract 213-2010-563),
and the Swedish Royal Academy of Sciences. Work at the Argonne National
Laboratory was supported by funding from the Division of Chemical
Sciences, Biosciences, Office of Basic Energy Sciences of the U.S.
Department of Energy through Grant DE-AC02-06CH11357. The authors thank
Sunshine Silver (Argonne National Laboratory) for ICP-AES measurements.
NR 91
TC 24
Z9 24
U1 8
U2 88
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
EI 1520-510X
J9 INORG CHEM
JI Inorg. Chem.
PD AUG 4
PY 2014
VL 53
IS 15
BP 8071
EP 8082
DI 10.1021/ic501014c
PG 12
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA AM6NR
UT WOS:000339982400035
PM 25029381
ER
PT J
AU Paley, JM
Messier, MD
Raja, R
Akgun, U
Asner, DM
Aydin, G
Baker, W
Barnes, PD
Bergfeld, T
Beverly, L
Bhatnagar, V
Choudhary, B
Dukes, EC
Duru, F
Feldman, GJ
Godley, A
Graf, N
Gronberg, J
Gulmez, E
Gunaydin, YO
Gustafson, HR
Hartouni, EP
Hanlet, P
Heffner, M
Kaplan, DM
Kamaev, O
Klay, J
Kumar, A
Lange, DJ
Lebedev, A
Ling, J
Longo, MJ
Lu, LC
Materniak, C
Mahajan, S
Meyer, H
Miller, DE
Mishra, SR
Nelson, K
Nigmanov, T
Norman, A
Onel, Y
Penzo, A
Peterson, RJ
Rajaram, D
Ratnikov, D
Rosenfeld, C
Rubin, H
Seun, S
Singh, A
Solomey, N
Soltz, RA
Torun, Y
Wilson, K
Wright, DM
Wu, QK
AF Paley, J. M.
Messier, M. D.
Raja, R.
Akgun, U.
Asner, D. M.
Aydin, G.
Baker, W.
Barnes, P. D., Jr.
Bergfeld, T.
Beverly, L.
Bhatnagar, V.
Choudhary, B.
Dukes, E. C.
Duru, F.
Feldman, G. J.
Godley, A.
Graf, N.
Gronberg, J.
Gulmez, E.
Gunaydin, Y. O.
Gustafson, H. R.
Hartouni, E. P.
Hanlet, P.
Heffner, M.
Kaplan, D. M.
Kamaev, O.
Klay, J.
Kumar, A.
Lange, D. J.
Lebedev, A.
Ling, J.
Longo, M. J.
Lu, L. C.
Materniak, C.
Mahajan, S.
Meyer, H.
Miller, D. E.
Mishra, S. R.
Nelson, K.
Nigmanov, T.
Norman, A.
Onel, Y.
Penzo, A.
Peterson, R. J.
Rajaram, D.
Ratnikov, D.
Rosenfeld, C.
Rubin, H.
Seun, S.
Singh, A.
Solomey, N.
Soltz, R. A.
Torun, Y.
Wilson, K.
Wright, D. M.
Wu, Q. K.
CA MIPP Collaboration
TI Measurement of charged pion production yields off the NuMI target
SO PHYSICAL REVIEW D
LA English
DT Article
ID COLLISIONS; DETECTOR
AB The fixed-target Main Injector Particle Production (MIPP) experiment, Fermilab E907, was designed to measure the production of hadrons from the collisions of hadrons of momenta ranging from 5 to 120 GeV/c on a variety of nuclei. These data will generally improve the simulation of particle detectors and predictions of particle beam fluxes at accelerators. The spectrometer momentum resolution is between 3% and 4%, and particle identification is performed for particles ranging between 0.3 and 80 GeV/c using dE/dx, time-of-flight, and Cherenkov radiation measurements. MIPP collected 1.42 x 10(6) events of 120 GeV Main Injector protons striking a target used in the Neutrinos at the Main Injector facility at Fermilab. The data have been analyzed and we present here charged pion yields per proton on target determined in bins of longitudinal and transverse momentum between 0.5 and 80 GeV/c, with combined statistical and systematic relative uncertainties between 5% and 10%.
C1 [Paley, J. M.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Akgun, U.] Coe Coll, Cedar Rapids, IA 52402 USA.
[Peterson, R. J.] Univ Colorado, Boulder, CO 80309 USA.
[Choudhary, B.] Univ Delhi, Delhi 110007, India.
[Raja, R.; Baker, W.; Beverly, L.; Norman, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Feldman, G. J.; Lebedev, A.; Seun, S.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA.
[Hanlet, P.; Kaplan, D. M.; Kamaev, O.; Rajaram, D.; Ratnikov, D.; Rubin, H.; Torun, Y.] IIT, Chicago, IL 60616 USA.
[Messier, M. D.; Graf, N.] Indiana Univ, Bloomington, IN 47403 USA.
[Akgun, U.; Aydin, G.; Duru, F.; Gulmez, E.; Gunaydin, Y. O.; Onel, Y.; Penzo, A.] Univ Iowa, Iowa City, IA 52242 USA.
[Asner, D. M.; Barnes, P. D., Jr.; Gronberg, J.; Hartouni, E. P.; Heffner, M.; Klay, J.; Lange, D. J.; Soltz, R. A.; Wright, D. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Gustafson, H. R.; Longo, M. J.; Nigmanov, T.; Rajaram, D.] Univ Michigan, Ann Arbor, MI 48109 USA.
[Bhatnagar, V.; Kumar, A.; Mahajan, S.; Singh, A.] Panjab Univ, Chandigarh 160014, India.
[Miller, D. E.] Purdue Univ, W Lafayette, IN 47907 USA.
[Bergfeld, T.; Godley, A.; Ling, J.; Mishra, S. R.; Rosenfeld, C.; Wilson, K.; Wu, Q. K.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA.
[Dukes, E. C.; Lu, L. C.; Materniak, C.; Nelson, K.; Norman, A.] Univ Virginia, Charlottesville, VA 22904 USA.
[Meyer, H.; Solomey, N.] Wichita State Univ, Wichita, KS 67260 USA.
[Gulmez, E.] Bogazici Univ, Istanbul, Turkey.
RP Paley, JM (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA.
RI Gulmez, Erhan/P-9518-2015; Ling, Jiajie/I-9173-2014;
OI Gulmez, Erhan/0000-0002-6353-518X; Ling, Jiajie/0000-0003-2982-0670;
Norman, Andrew/0000-0001-8572-956X; Torun, Yagmur/0000-0003-2336-6585
FU U.S. Department of Energy
FX This work was supported by the U.S. Department of Energy. We are
grateful to the staff of Fermilab, Lawrence Livermore National
Laboratory under Contract No. DE-AC52-07NA27344 and Argonne National
Laboratory for their contributions to this effort.
NR 11
TC 3
Z9 3
U1 0
U2 1
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1550-7998
EI 1550-2368
J9 PHYS REV D
JI Phys. Rev. D
PD AUG 4
PY 2014
VL 90
IS 3
AR 032001
DI 10.1103/PhysRevD.90.032001
PG 14
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA AM6UF
UT WOS:000340000000001
ER
PT J
AU Rusydi, A
Goos, A
Binder, S
Eich, A
Botril, K
Abbamonte, P
Yu, X
Breese, MBH
Eisaki, H
Fujimaki, Y
Uchida, S
Guerassimova, N
Treusch, R
Feldhaus, J
Reininger, R
Klein, MV
Rubhausen, M
AF Rusydi, A.
Goos, A.
Binder, S.
Eich, A.
Botril, K.
Abbamonte, P.
Yu, X.
Breese, M. B. H.
Eisaki, H.
Fujimaki, Y.
Uchida, S.
Guerassimova, N.
Treusch, R.
Feldhaus, J.
Reininger, R.
Klein, M. V.
Ruebhausen, M.
TI Electronic Screening-Enhanced Hole Pairing in Two-Leg Spin Ladders
Studied by High-Resolution Resonant Inelastic X-Ray Scattering at Cu M
Edges
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID RAMAN-SCATTERING; CORRELATED SYSTEMS; SR14CU24O41; EXCITATIONS;
SUPERCONDUCTORS; SPECTROSCOPY; LIGHT
AB We study the electronic screening mechanisms of the effective Coulomb on-site repulsion in hole-doped Sr14Cu24O41 compared to undoped La6Ca8Cu24O41 using polarization dependent high-resolution resonant inelastic x-ray scattering at Cu M edges. By measuring the energy of the effective Coulomb on-site repulsion and the spin excitations, we estimate superexchange and hopping matrix element energies along rungs and legs, respectively. Interestingly, hole doping locally screens the Coulomb on-site repulsion reducing it by as much as 25%. We suggest that the increased ratio of the electronic kinetic to the electronic correlation energy contributes to the local superexchange mediated pairing between holes.
C1 [Rusydi, A.; Goos, A.; Binder, S.; Eich, A.; Botril, K.; Ruebhausen, M.] Univ Hamburg, Inst Angew Phys, D-20355 Hamburg, Germany.
[Rusydi, A.; Goos, A.; Binder, S.; Eich, A.; Botril, K.; Ruebhausen, M.] Ctr Free Elect Laser Sci CFEL, D-22607 Hamburg, Germany.
[Rusydi, A.; Breese, M. B. H.; Ruebhausen, M.] Natl Univ Singapore, Dept Phys, NUSSNI NanoCore, Singapore 117542, Singapore.
[Rusydi, A.; Yu, X.; Breese, M. B. H.] Natl Univ Singapore, Singapore Synchrotron Light Sourc, Singapore 117603, Singapore.
[Abbamonte, P.; Klein, M. V.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA.
[Abbamonte, P.; Klein, M. V.] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA.
[Eisaki, H.] AIST, Nanoelect Res Inst, Tsukuba, Ibaraki 3058568, Japan.
[Fujimaki, Y.; Uchida, S.] Univ Tokyo, Dept Superconduct, Bunkyo Ku, Tokyo 113, Japan.
[Guerassimova, N.; Treusch, R.; Feldhaus, J.] DESY, D-22607 Hamburg, Germany.
[Reininger, R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Rusydi, A (reprint author), Univ Hamburg, Inst Angew Phys, Jungiusstr 11, D-20355 Hamburg, Germany.
EM phyandri@nus.edu.sg; michael.ruebhausen@desy.de
RI Treusch, Rolf/C-3935-2015; Breese, Mark/G-2068-2012; Rusydi,
Andrivo/I-1849-2016
FU BMBF [05K10GUD]; DFG [Ru 773/4-1, Ru 773/4-2]; Singapore National
Research Foundation [NRF-CRP 8-2011-06, NRF2008NRF-CRP002024]; MOE Tier
2 [MOE2010-T2-2-121]; FRC and NUS YIA
FX We would like to acknowledge technical support from Holger Weigelt,
Benjamin Schulz, Pelangi Saichu, Jason Lim, and Wong How Kwong, and
discussions with Dirk Manske, Wilfried Wurth, George Sawatzky, Jochen
Schneider, and Lance Cooper. We acknowledge financial support by BMBF
under 05K10GUD as well as DFG through Ru 773/4-1 & 4-2, and by Singapore
National Research Foundation under its Competitive Research Funding
(NRF-CRP 8-2011-06 and NRF2008NRF-CRP002024), MOE Tier 2
(MOE2010-T2-2-121), and FRC and NUS YIA.
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PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
EI 1079-7114
J9 PHYS REV LETT
JI Phys. Rev. Lett.
PD AUG 4
PY 2014
VL 113
IS 6
AR 067001
DI 10.1103/PhysRevLett.113.067001
PG 6
WC Physics, Multidisciplinary
SC Physics
GA AM7GW
UT WOS:000340034500009
PM 25148343
ER
PT J
AU Martinez, E
Hirth, JP
AF Martinez, Enrique
Hirth, John P.
TI Screw-dislocation constrictions in face-centered cubic crystals
SO PHYSICAL REVIEW B
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATION; CROSS-SLIP; THIN-FILM; COPPER;
DEFORMATION; NUCLEATION; PLASTICITY; GROWTH; METALS; NICKEL
AB We show, using molecular statics and dynamics simulations along with dislocation dynamics calculations, that the structure of a screw dislocation in a thin film or at a free surface for face-centered cubic Cu differs from that found in bulk. In agreement with earlier work, a screw dislocation at the surface is observed to dissociate in two different {111} planes, forming a constriction at the site where the glide plane changes. We analyze in detail the energetics of the structure and conclude that the constricted configuration is stable due to the long-range elastic interactions. We have also performed shear stress simulations and compared to bulk stress to understand how the constriction modifies the response of the dislocation to an applied load. We found that such constriction represents a strong pinning point, substantially increasing the yield stress required for the dislocation to glide. In contrast, the configuration provides a barrierless source for the dislocation to cross slip.
C1 [Martinez, Enrique] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
[Hirth, John P.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
RP Martinez, E (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST 8, Los Alamos, NM 87545 USA.
EM enriquem@lanl.gov
OI Martinez Saez, Enrique/0000-0002-2690-2622
FU Center for Materials at Irradiation and Mechanical Extremes, an Energy
Frontier Research Center - U.S. Department of Energy at Los Alamos
National Laboratory [2008LANL1026]
FX The authors gratefully acknowledge the support from the Center for
Materials at Irradiation and Mechanical Extremes, an Energy Frontier
Research Center funded by the U.S. Department of Energy (Award No.
2008LANL1026) at Los Alamos National Laboratory, as well as helpful
discussions with A. Caro. Parallel computations were performed on the
Lobo machine at the High Performance Computing clusters at Los Alamos
National Laboratory.
NR 36
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U2 32
PU AMER PHYSICAL SOC
PI COLLEGE PK
PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1098-0121
EI 1550-235X
J9 PHYS REV B
JI Phys. Rev. B
PD AUG 4
PY 2014
VL 90
IS 6
AR 064102
DI 10.1103/PhysRevB.90.064102
PG 6
WC Physics, Condensed Matter
SC Physics
GA AM6TO
UT WOS:000339998300002
ER
PT J
AU Cannon, WR
AF Cannon, William R.
TI Simulating Metabolism with Statistical Thermodynamics
SO PLOS ONE
LA English
DT Article
AB New methods are needed for large scale modeling of metabolism that predict metabolite levels and characterize the thermodynamics of individual reactions and pathways. Current approaches use either kinetic simulations, which are difficult to extend to large networks of reactions because of the need for rate constants, or flux-based methods, which have a large number of feasible solutions because they are unconstrained by the law of mass action. This report presents an alternative modeling approach based on statistical thermodynamics. The principles of this approach are demonstrated using a simple set of coupled reactions, and then the system is characterized with respect to the changes in energy, entropy, free energy, and entropy production. Finally, the physical and biochemical insights that this approach can provide for metabolism are demonstrated by application to the tricarboxylic acid (TCA) cycle of Escherichia coli. The reaction and pathway thermodynamics are evaluated and predictions are made regarding changes in concentration of TCA cycle intermediates due to 10-and 100-fold changes in the ratio of NAD+: NADH concentrations. Finally, the assumptions and caveats regarding the use of statistical thermodynamics to model non-equilibrium reactions are discussed.
C1 Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
RP Cannon, WR (reprint author), Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
EM William.cannon@pnnl.gov
RI Cannon, William/K-8411-2014
OI Cannon, William/0000-0003-3789-7889
FU Scientific Discovery through Advanced Computing (SciDAC) program, Office
of Advanced Scientific Computing Research (OASCR); Genomic Science
Program (GSP), Office of Biological and Environmental Research (OBER)
through a SciDAC award; U.S. Department of Energy [DE-AC06-76RLO]
FX This research was developed under the Laboratory Directed Research and
Development Program at Pacific Northwest National Laboratory. Initial
concepts were supported through joint funding from the Scientific
Discovery through Advanced Computing (SciDAC) program, Office of
Advanced Scientific Computing Research (OASCR) and the Genomic Science
Program (GSP), Office of Biological and Environmental Research (OBER),
through a SciDAC award to W. R. Cannon. PNNL is operated by Battelle for
the U.S. Department of Energy under Contract DE-AC06-76RLO. The funders
had no role in study design, data collection and analysis, decision to
publish, or preparation of the manuscript.
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PU PUBLIC LIBRARY SCIENCE
PI SAN FRANCISCO
PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA
SN 1932-6203
J9 PLOS ONE
JI PLoS One
PD AUG 4
PY 2014
VL 9
IS 8
AR e103582
DI 10.1371/journal.pone.0103582
PG 16
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AM4GX
UT WOS:000339812700033
PM 25089525
ER
PT J
AU Collier, SM
Ruark, MD
Oates, LG
Jokela, WE
Dell, CJ
AF Collier, Sarah M.
Ruark, Matthew D.
Oates, Lawrence G.
Jokela, William E.
Dell, Curtis J.
TI Measurement of Greenhouse Gas Flux from Agricultural Soils Using Static
Chambers
SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS
LA English
DT Article
DE Environmental Sciences; Issue 90; greenhouse gas; trace gas; gas flux;
static chamber; soil; field; agriculture; climate
ID NITROUS-OXIDE FLUXES; DIFFUSION-MODEL; ATMOSPHERE; EMISSIONS; METHANE
AB Measurement of greenhouse gas (GHG) fluxes between the soil and the atmosphere, in both managed and unmanaged ecosystems, is critical to understanding the biogeochemical drivers of climate change and to the development and evaluation of GHG mitigation strategies based on modulation of landscape management practices. The static chamber-based method described here is based on trapping gases emitted from the soil surface within a chamber and collecting samples from the chamber headspace at regular intervals for analysis by gas chromatography. Change in gas concentration over time is used to calculate flux. This method can be utilized to measure landscape-based flux of carbon dioxide, nitrous oxide, and methane, and to estimate differences between treatments or explore system dynamics over seasons or years. Infrastructure requirements are modest, but a comprehensive experimental design is essential. This method is easily deployed in the field, conforms to established guidelines, and produces data suitable to large-scale GHG emissions studies.
C1 [Collier, Sarah M.] Univ Wisconsin, Off Sustainabil, Madison, WI 53706 USA.
[Ruark, Matthew D.] Univ Wisconsin, Dept Soil Sci, Madison, WI 53706 USA.
[Oates, Lawrence G.] Univ Wisconsin, Dept Agron, Madison, WI 53706 USA.
[Oates, Lawrence G.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA.
[Jokela, William E.] USDA ARS, Dairy Forage Res Ctr, Washington, DC 20250 USA.
[Dell, Curtis J.] USDA ARS, Pasture Syst Watershed Management Res Unit, Washington, DC 20250 USA.
RP Dell, CJ (reprint author), USDA ARS, Pasture Syst Watershed Management Res Unit, Washington, DC 20250 USA.
EM curtis.dell@ars.usda.gov
OI Collier, Sarah/0000-0002-8834-5075; Oates, Lawrence/0000-0003-4829-7600
FU National Science Foundation [1215858]; US Department of Agriculture
[2013-68002-20525]; US Department of Energy Great Lakes Bioenergy
Research Center - DOE BER Office of Science [DE-FC02-07ER64494]; DOE OBP
Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830]
FX This material is based upon work supported by the National Science
Foundation under Grant Number 1215858, by the US Department of
Agriculture under Grant Number 2013-68002-20525, and by the US
Department of Energy Great Lakes Bioenergy Research Center - DOE BER
Office of Science (DE-FC02-07ER64494) and DOE OBP Office of Energy
Efficiency and Renewable Energy (DE-AC05-76RL01830). In-field video and
images were recorded at the Wisconsin Integrated Cropping System Trial
project of the University of Wisconsin-Madison. The authors are grateful
to Ryan Curtin for skillful videography and editing.
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PU JOURNAL OF VISUALIZED EXPERIMENTS
PI CAMBRIDGE
PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA
SN 1940-087X
J9 JOVE-J VIS EXP
JI J. Vis. Exp.
PD AUG
PY 2014
IS 90
AR e52110
DI 10.3791/52110
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA CB0EV
UT WOS:000349299200080
PM 25146426
ER
PT J
AU Rames, M
Yu, YD
Ren, G
AF Rames, Matthew
Yu, Yadong
Ren, Gang
TI Optimized Negative Staining: a High-throughput Protocol for Examining
Small and Asymmetric Protein Structure by Electron Microscopy
SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS
LA English
DT Article
DE Environmental Sciences; Issue 90; small and asymmetric protein
structure; electron microscopy; optimized negative staining
ID HIGH-DENSITY-LIPOPROTEINS; APOLIPOPROTEIN-A-I; LECITHIN-CHOLESTEROL
ACYLTRANSFERASE; MULTIPLE ISOMORPHOUS REPLACEMENT; ANOMALOUS DISPERSION
DATA; HEAVY-ATOM POSITIONS; LIPID-BINDING; CRYO-EM; SCATTERING FACTORS;
DIFFERENT SIZES
AB Structural determination of proteins is rather challenging for proteins with molecular masses between 40 - 200 kDa. Considering that more than half of natural proteins have a molecular mass between 40 - 200 kDa(1,2), a robust and high-throughput method with a nanometer resolution capability is needed. Negative staining (NS) electron microscopy (EM) is an easy, rapid, and qualitative approach which has frequently been used in research laboratories to examine protein structure and protein-protein interactions. Unfortunately, conventional NS protocols often generate structural artifacts on proteins, especially with lipoproteins that usually form presenting rouleaux artifacts. By using images of lipoproteins from cryo-electron microscopy (cryo-EM) as a standard, the key parameters in NS specimen preparation conditions were recently screened and reported as the optimized NS protocol (OpNS), a modified conventional NS protocol(3). Artifacts like rouleaux can be greatly limited by OpNS, additionally providing high contrast along with reasonably high#resolution (near 1 nm) images of small and asymmetric proteins. These high-resolution and high contrast images are even favorable for an individual protein (a single object, no average) 3D reconstruction, such as a 160 kDa antibody, through the method of electron tomography(4,5). Moreover, OpNS can be a high# throughput tool to examine hundreds of samples of small proteins. For example, the previously published mechanism of 53 kDa cholesteryl ester transfer protein (CETP) involved the screening and imaging of hundreds of samples(6). Considering cryo-EM rarely successfully images proteins less than 200 kDa has yet to publish any study involving screening over one hundred sample conditions, it is fair to call OpNS a high-throughput method for studying small proteins. Hopefully the OpNS protocol presented here can be a useful tool to push the boundaries of EM and accelerate EM studies into small protein structure, dynamics and mechanisms.
C1 [Rames, Matthew; Yu, Yadong; Ren, Gang] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
RP Ren, G (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
EM gren@lbl.gov
RI Foundry, Molecular/G-9968-2014; Chiang, Vincent, Ming-Hsien/D-4312-2016
OI Chiang, Vincent, Ming-Hsien/0000-0002-2029-7863
FU NHLBI NIH HHS [R01 HL115153, R01HL115153]; NIGMS NIH HHS [R01 GM104427,
R01GM104427]
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PU JOURNAL OF VISUALIZED EXPERIMENTS
PI CAMBRIDGE
PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA
SN 1940-087X
J9 JOVE-J VIS EXP
JI J. Vis. Exp.
PD AUG
PY 2014
IS 90
AR e51087
DI 10.3791/51087
PG 15
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA CB0EV
UT WOS:000349299200006
PM 25145703
ER
PT J
AU Tsai, WT
Hassan, A
Sarkar, P
Correa, J
Metlagel, Z
Jorgens, DM
Auer, M
AF Tsai, Wen-Ting
Hassan, Ahmed
Sarkar, Purbasha
Correa, Joaquin
Metlagel, Zoltan
Jorgens, Danielle M.
Auer, Manfred
TI From Voxels to Knowledge: A Practical Guide to the Segmentation of
Complex Electron Microscopy 3D-Data
SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS
LA English
DT Article
DE Bioengineering; Issue 90; 3D electron microscopy; feature extraction;
segmentation; image analysis; reconstruction; manual tracing;
thresholding
ID NOISE-REDUCTION; IMAGE-ANALYSIS; VISUALIZATION; CELLS
AB Modern 3D electron microscopy approaches have recently allowed unprecedented insight into the 3D ultrastructural organization of cells and tissues, enabling the visualization of large macromolecular machines, such as adhesion complexes, as well as higher-order structures, such as the cytoskeleton and cellular organelles in their respective cell and tissue context. Given the inherent complexity of cellular volumes, it is essential to first extract the features of interest in order to allow visualization, quantification, and therefore comprehension of their 3D organization. Each data set is defined by distinct characteristics, e.g., signal-to-noise ratio, crispness (sharpness) of the data, heterogeneity of its features, crowdedness of features, presence or absence of characteristic shapes that allow for easy identification, and the percentage of the entire volume that a specific region of interest occupies. All these characteristics need to be considered when deciding on which approach to take for segmentation.
The six different 3D ultrastructural data sets presented were obtained by three different imaging approaches: resin embedded stained electron tomography, focused ion beam-and serial block face-scanning electron microscopy (FIB-SEM, SBF-SEM) of mildly stained and heavily stained samples, respectively. For these data sets, four different segmentation approaches have been applied: (1) fully manual model building followed solely by visualization of the model, (2) manual tracing segmentation of the data followed by surface rendering, (3) semi-automated approaches followed by surface rendering, or (4) automated custom-designed segmentation algorithms followed by surface rendering and quantitative analysis. Depending on the combination of data set characteristics, it was found that typically one of these four categorical approaches outperforms the others, but depending on the exact sequence of criteria, more than one approach may be successful. Based on these data, we propose a triage scheme that categorizes both objective data set characteristics and subjective personal criteria for the analysis of the different data sets.
C1 [Tsai, Wen-Ting; Hassan, Ahmed; Correa, Joaquin; Metlagel, Zoltan; Jorgens, Danielle M.; Auer, Manfred] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
[Sarkar, Purbasha; Auer, Manfred] Lawrence Berkeley Natl Lab, Joint Bioenergy Inst, Phys Biosci Div, Berkeley, CA USA.
[Correa, Joaquin] Lawrence Berkeley Natl Lab, Natl Energy Res Sci Comp Ctr, Berkeley, CA USA.
RP Auer, M (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
EM mauer@lbl.gov
FU U.S. Department of Energy, Office of Science [DE-AC02-05CH11231]; U.S.
National Institutes of Health (NIH) [P01 GM051487]
FX Research was supported by the U.S. Department of Energy, Office of
Science under contract No. DE-AC02-05CH11231 [David Skinner], as well as
U.S. National Institutes of Health (NIH) grant No. P01 GM051487 [M.A.]
for the inner ear hair cell project and microscopy instrumentation use.
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PI CAMBRIDGE
PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA
SN 1940-087X
J9 JOVE-J VIS EXP
JI J. Vis. Exp.
PD AUG
PY 2014
IS 90
AR e51673
DI 10.3791/51673
PG 15
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA CB0EV
UT WOS:000349299200035
PM 25145678
ER
PT J
AU Yang, CR
Bland, W
Mellor-Crummey, J
Balaji, P
AF Yang, Chaoran
Bland, Wesley
Mellor-Crummey, John
Balaji, Pavan
TI Portable, MPI-Interoperable Coarray Fortran
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE Coarray Fortran; MPI; PGAS; Interoperability
AB The past decade has seen the advent of a number of parallel programming models such as Coarray Fortran (CAF), Unified Parallel C, X10, and Chapel. Despite the productivity gains promised by these models, most parallel scientific applications still rely on MPI as their data movement model. One reason for this trend is that it is hard for users to incrementally adopt these new programming models in existing MPI applications. Because each model use its own runtime system, they duplicate resources and are potentially error-prone. Such independent runtime systems were deemed necessary because MPI was considered insufficient in the past to play this role for these languages.
The recently released MPI-3, however, adds several new capabilities that now provide all of the functionality needed to act as a runtime, including a much more comprehensive one-sided communication framework. In this paper, we investigate how MPI-3 can form a runtime system for one example programming model, CAF, with a broader goal of enabling a single application to use both MPI and CAF with the highest level of interoperability.
C1 [Yang, Chaoran; Mellor-Crummey, John] Rice Univ, Dept Comp Sci, Houston, TX 77251 USA.
[Bland, Wesley; Balaji, Pavan] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA.
RP Yang, CR (reprint author), Rice Univ, Dept Comp Sci, Houston, TX 77251 USA.
EM chaoran@rice.edu; wbland@mcs.anl.gov; johnmc@rice.edu;
balaji@mcs.anl.gov
FU U.S. Department of Energy, Office of Science, Advanced Scientific
Computing Research [DE-AC02-06CH11357]
FX This work was supported by the U.S. Department of Energy, Office of
Science, Advanced Scientific Computing Research, under Contract
DE-AC02-06CH11357. We also thank Scott K. Warren and Dung X. Nguyen from
Rice Group for porting CGPOP to CAF 2.0 and allowing us to use it for
the evaluation of CAF-MPI.
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PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2014
VL 49
IS 8
BP 81
EP 92
DI 10.1145/2555243.2555270
PG 12
WC Computer Science, Software Engineering
SC Computer Science
GA CA8BS
UT WOS:000349142100008
ER
PT J
AU Leung, VJ
Bunde, DP
Ebbers, J
Feer, SP
Price, NW
Rhodes, ZD
Swank, M
AF Leung, Vitus J.
Bunde, David P.
Ebbers, Johnathan
Feer, Stefan P.
Price, Nickolas W.
Rhodes, Zachary D.
Swank, Matthew
TI Task Mapping Stencil Computations for Non-Contiguous Allocations
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE Task mapping; stencil communication pattern; non-contiguous allocation;
improved scalability
AB We examine task mapping algorithms for systems that allocate jobs non-contiguously. Several studies have shown that task placement affects job running time. We focus on jobs with a stencil communication pattern and use experiments on a Cray XE to evaluate novel task mapping algorithms as well as some adapted to this setting. This is done with the miniGhost miniApp which mimics the behavior of CTH, a shock physics application. Our strategies improve average and single-run times by as much as 28% and 36% over a baseline strategy, respectively.
C1 [Leung, Vitus J.] Sandia Natl Labs, Livermore, CA 94550 USA.
[Bunde, David P.; Ebbers, Johnathan; Feer, Stefan P.; Price, Nickolas W.; Rhodes, Zachary D.; Swank, Matthew] Knox Coll, Galesburg, IL USA.
[Rhodes, Zachary D.] Allstate Corp, Northbrook, IL USA.
RP Leung, VJ (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA.
EM vjleung@sandia.gov; dbunde@knox.edu; jebbers@knox.edu; sfeer@mmm.com;
nprice@knox.edu; rhodesz87@gmail.com; mswank@knox.edu
FU Sandia National Laboratories [899808]; Knox College; U.S. Department of
Energy's National Nuclear Security Administration [DE-AC04-94AL85000]
FX D.P. Bunde, J. Ebbers, S.P. Feer, N.W. Price, Z.D. Rhodes, and M. Swank
were partially supported by contract 899808 from Sandia National
Laboratories. Z.D. Rhodes also acknowledges support from a
Post-baccalaureate Fellowship from Knox College. Sandia National
Laboratories is a multiprogram laboratory managed and operated by Sandia
Corporation, a wholly owned subsidiary of Lockheed Martin Corporation,
for the U.S. Department of Energy's National Nuclear Security
Administration under contract DE-AC04-94AL85000.
NR 6
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PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2014
VL 49
IS 8
BP 377
EP 378
DI 10.1145/2555243.2555277
PG 2
WC Computer Science, Software Engineering
SC Computer Science
GA CA8BS
UT WOS:000349142100036
ER
PT J
AU Gomez, LB
Cappello, F
AF Gomez, Leonardo Bautista
Cappello, Franck
TI Detecting Silent Data Corruption through Data Dynamic Monitoring for
Scientific Applications
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE Fault Tolerance; Supercomputers; Silent Data Corruption; Soft Errors;
Bit Flips; Data Entropy
AB Parallel programming has become one of the best ways to express scientific models that simulate a wide range of natural phenomena. These complex parallel codes are deployed and executed on large-scale parallel computers, making them important tools for scientific discovery. As supercomputers get faster and larger, the increasing number of components is leading to higher failure rates. In particular, the miniaturization of electronic components is expected to lead to a dramatic rise in soft errors and data corruption. Moreover, soft errors can corrupt data silently and generate large inaccuracies or wrong results at the end of the computation. In this paper we propose a novel technique to detect silent data corruption based on data monitoring. Using this technique, an application can learn the normal dynamics of its datasets, allowing it to quickly spot anomalies. We evaluate our technique with synthetic benchmarks and we show that our technique can detect up to 50% of injected errors while incurring only negligible overhead.
C1 [Gomez, Leonardo Bautista; Cappello, Franck] Argonne Natl Lab, Argonne, IL 60439 USA.
RP Gomez, LB (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA.
OI Bautista-Gomez, Leonardo/0000-0002-0814-5779
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PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2014
VL 49
IS 8
BP 381
EP 382
DI 10.1145/2555243.2555279
PG 2
WC Computer Science, Software Engineering
SC Computer Science
GA CA8BS
UT WOS:000349142100038
ER
PT J
AU Isaacs, KE
Gamblin, T
Bhatele, A
Bremer, PT
Schulz, M
Hamann, B
AF Isaacs, Katherine E.
Gamblin, Todd
Bhatele, Abhinav
Bremer, Peer-Timo
Schulz, Martin
Hamann, Bernd
TI Extracting Logical Structure and Identifying Stragglers in Parallel
Execution Traces
SO ACM SIGPLAN NOTICES
LA English
DT Article
DE parallel execution trace; logical structure; visualization
AB We introduce a new approach to automatically extract an idealized logical structure from a parallel execution trace. We use this structure to define intuitive metrics such as the lateness of a process involved in a parallel execution. By analyzing and illustrating traces in terms of logical steps, we leverage a developer's understanding of the happened-before relations in a parallel program. This technique can uncover dependency chains, elucidate communication patterns, and highlight sources and propagation of delays, all of which may be obscured in a traditional trace visualization.
C1 [Isaacs, Katherine E.; Hamann, Bernd] Univ Calif Davis, Dept Comp Sci, Davis, CA 95616 USA.
[Gamblin, Todd; Bhatele, Abhinav; Bremer, Peer-Timo; Schulz, Martin] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA USA.
RP Isaacs, KE (reprint author), Univ Calif Davis, Dept Comp Sci, Davis, CA 95616 USA.
EM keisaacs@ucdavis.edu; tgamblin@llnl.gov; bhatele@llnl.gov;
ptbremer@llnl.gov; schulzm@llnl.gov; hamann@cs.ucdavis.edu
FU U.S. Department of Energy Office of Science Graduate Fellowship
[DE-AC05-06OR23100]; Lawrence Livermore National Laboratory
[DE-AC52-07NA27344, LLNL-ABS-647655]
FX This research is supported by the U.S. Department of Energy Office of
Science Graduate Fellowship administered by ORISE-ORAU under contract
DE-AC05-06OR23100 and by Lawrence Livermore National Laboratory under
contract DE-AC52-07NA27344 (LLNL-ABS-647655).
NR 5
TC 0
Z9 0
U1 0
U2 1
PU ASSOC COMPUTING MACHINERY
PI NEW YORK
PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA
SN 0362-1340
EI 1558-1160
J9 ACM SIGPLAN NOTICES
JI ACM Sigplan Not.
PD AUG
PY 2014
VL 49
IS 8
BP 397
EP 398
DI 10.1145/2555243.2555288
PG 2
WC Computer Science, Software Engineering
SC Computer Science
GA CA8BS
UT WOS:000349142100046
ER
PT J
AU Agar, JC
Mangalam, RVK
Damodaran, AR
Velarde, G
Karthik, J
Okatan, MB
Chen, ZH
Jesse, S
Balke, N
Kalinin, SV
Martin, LW
AF Agar, J. C.
Mangalam, R. V. K.
Damodaran, A. R.
Velarde, G.
Karthik, J.
Okatan, M. B.
Chen, Z. H.
Jesse, S.
Balke, N.
Kalinin, S. V.
Martin, L. W.
TI Tuning Susceptibility via Misfit Strain in Relaxed Morphotropic Phase
Boundary PbZr1-xTixO3 Epitaxial Thin Films
SO ADVANCED MATERIALS INTERFACES
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; ZIRCONATE-TITANATE FILMS; DOMAIN-WALL MOTION;
PIEZOELECTRIC PROPERTIES; DIELECTRIC PERMITTIVITY;
ELECTRICAL-PROPERTIES; PB(ZR,TI)O-3 FILMS; CERAMICS; DEPENDENCE;
THICKNESS
AB Epitaxial strain is a powerful tool to manipulate the properties of ferroelectric materials. But despite extensive work in this regard, few studies have explored the effect of epitaxial strain on PbZr0.52Ti0.48O3. Here we explore how epitaxial strain impacts the structure and properties of 75 nm thick films of the morphotropic phase boundary composition. Single-phase, fully epitaxial films are found to possess "relaxed" or nearly "relaxed" structures despite growth on a range of substrates. Subsequent studies of the dielectric and ferroelectric properties reveal films with low leakage currents facilitating the measurement of low-loss hysteresis loops down to measurement frequencies of 30 mHz and dielectric response at background dc bias fields as large as 850 kV/cm. Despite a seeming insensitivity of the crystal structure to the epitaxial strain, the polarization and switching characteristics are found to vary with substrate. The elastic constraint from the substrate produces residual strains that dramatically alter the electric-field response including quenching domain wall contributions to the dielectric permittivity and suppressing field-induced structural reorientation. These results demonstrate that substrate mediated epitaxial strain of PbZr0.52Ti0.48O3 is more complex than in conventional ferroelectrics with discretely defined phases, yet can have a marked effect on the material and its responses.
C1 [Agar, J. C.; Mangalam, R. V. K.; Damodaran, A. R.; Velarde, G.; Karthik, J.; Chen, Z. H.; Martin, L. W.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA.
[Agar, J. C.; Mangalam, R. V. K.; Damodaran, A. R.; Velarde, G.; Karthik, J.; Chen, Z. H.; Martin, L. W.] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA.
[Martin, L. W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Okatan, M. B.; Jesse, S.; Balke, N.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA.
RP Agar, JC (reprint author), Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA.
EM lwmartin@illinois.edu
RI Martin, Lane/H-2409-2011; Balke, Nina/Q-2505-2015; Kalinin,
Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Okatan, M.
Baris/E-1913-2016; Chen, Zuhuang/E-7131-2011
OI Martin, Lane/0000-0003-1889-2513; Balke, Nina/0000-0001-5865-5892;
Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483;
Okatan, M. Baris/0000-0002-9421-7846; Chen, Zuhuang/0000-0003-1912-6490
FU National Science Foundation [DMR-1149062, DMR-1124696]; Air Force Office
of Scientific Research (AFOSR) [AF FA 9550-11-1-0073]; Army Research
Office (ARO) [W911NF-10-1-0482]; Office of Naval Research (ONR)
[N00014-10-1-0525]
FX J. C. A. and L. W. M. would like to acknowledge support from the
National Science Foundation under grant DMR-1149062 and the Air Force
Office of Scientific Research (AFOSR) under grant AF FA 9550-11-1-0073.
R.V.K.M. and L.W.M. would like to acknowledge support from the National
Science Foundation under grant DMR-1124696. A.R.D. and L.W.M. would like
to acknowledge support from the Army Research Office (ARO) under grant
W911NF-10-1-0482. J.K. and L.W.M. would like to acknowledge support from
the Office of Naval Research (ONR) under grant N00014-10-1-0525.
NR 51
TC 3
Z9 3
U1 1
U2 19
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 2196-7350
J9 ADV MATER INTERFACES
JI Adv. Mater. Interfaces
PD AUG
PY 2014
VL 1
IS 5
AR 1400098
DI 10.1002/admi.201400098
PG 8
WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA AZ5TT
UT WOS:000348283700019
ER
PT J
AU Vandehey, NT
O'Neil, JP
AF Vandehey, Nicholas T.
O'Neil, James P.
TI Capturing [C-11]CO2 for use in aqueous applications
SO APPLIED RADIATION AND ISOTOPES
LA English
DT Article
DE [C-11]CO2; Carbon-11; Radiochemistry; Positron emission tomography;
Carbon capture; Ion exchange
ID EMISSION-TOMOGRAPHY
AB We present a simple method for trapping [C-11]CO2 gas and releasing it into a buffered solution using an ion-exchange cartridge. Sodium hydroxide cartridges captured >99% of [C-11]CO2 following NaOH activation. A sodium bicarbonate solution eluted >99% of trapped radioactivity. Trapping [C-11]CO2 directly in small volumes of several solutions was less effective than cartridge methods. The recommended methods allow for fast and simple production of highly concentrated carbon-11 containing aqueous solutions for use in filling phantoms, calibrating detectors, or (bio)geochemical experiments. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Vandehey, Nicholas T.; O'Neil, James P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Vandehey, NT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM ntvandehey@lbl.gov; jponei1@lbl.gov
OI Vandehey, Nicholas/0000-0003-0286-7532
FU Office of Science, Office of Biological and Environmental Research,
Biological Systems Science Division of the U.S. Department of Energy
[DE-AC02-05CH11231]
FX This work was supported by the Director, Office of Science, Office of
Biological and Environmental Research, Biological Systems Science
Division of the U.S. Department of Energy under Contract no.
DE-AC02-05CH11231.
NR 20
TC 4
Z9 4
U1 0
U2 5
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0969-8043
J9 APPL RADIAT ISOTOPES
JI Appl. Radiat. Isot.
PD AUG
PY 2014
VL 90
BP 74
EP 78
DI 10.1016/j.apradiso.2014.03.013
PG 5
WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology,
Nuclear Medicine & Medical Imaging
SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine &
Medical Imaging
GA AY5ER
UT WOS:000347596400011
PM 24705008
ER
PT J
AU Rennie, EA
Ebert, B
Miles, GP
Cahoon, RE
Christiansen, KM
Stonebloom, S
Khatab, H
Twell, D
Petzold, CJ
Adams, PD
Dupree, P
Heazlewood, JL
Cahoon, EB
Scheller, HV
AF Rennie, Emilie A.
Ebert, Berit
Miles, Godfrey P.
Cahoon, Rebecca E.
Christiansen, Katy M.
Stonebloom, Solomon
Khatab, Hoda
Twell, David
Petzold, Christopher J.
Adams, Paul D.
Dupree, Paul
Heazlewood, Joshua L.
Cahoon, Edgar B.
Scheller, Henrik Vibe
TI Identification of a Sphingolipid alpha-Glucuronosyltransferase That Is
Essential for Pollen Function in Arabidopsis
SO PLANT CELL
LA English
DT Article
ID TANDEM MASS-SPECTROMETRY; PROGRAMMED CELL-DEATH;
SACCHAROMYCES-CEREVISIAE; PLANT SPHINGOLIPIDS;
INOSITOLPHOSPHORYLCERAMIDE SYNTHASE; SERINE PALMITOYLTRANSFERASE;
TOBACCO-LEAVES; TUBE GROWTH; LIPID RAFTS; THALIANA
AB Glycosyl inositol phosphorylceramide (GIPC) sphingolipids are a major class of lipids in fungi, protozoans, and plants. GIPCs are abundant in the plasma membrane in plants, comprising around a quarter of the total lipids in these membranes. Plant GIPCs contain unique glycan decorations that include a conserved glucuronic acid (GlcA) residue and various additional sugars; however, no proteins responsible for glycosylating GIPCs have been identified to date. Here, we show that the Arabidopsis thaliana protein INOSITOL PHOSPHORYLCERAMIDE GLUCURONOSYLTRANSFERASE1 (IPUT1) transfers GlcA from UDP-GlcA to GIPCs. To demonstrate IPUT1 activity, we introduced the IPUT1 gene together with genes for a UDP-glucose dehydrogenase from Arabidopsis and a human UDP-GlcA transporter into a yeast mutant deficient in the endogenous inositol phosphorylceramide (IPC) mannosyltransferase. In this engineered yeast strain, IPUT1 transferred GlcA to IPC. Overexpression or silencing of IPUT1 in Nicotiana benthamiana resulted in an increase or a decrease, respectively, in IPC glucuronosyltransferase activity in vitro. Plants in which IPUT1 was silenced accumulated IPC, the immediate precursor, as well as ceramides and glucosylceramides. Plants overexpressing IPUT1 showed an increased content of GIPCs. Mutations in IPUT1 are not transmitted through pollen, indicating that these sphingolipids are essential in plants.
C1 [Rennie, Emilie A.; Ebert, Berit; Christiansen, Katy M.; Stonebloom, Solomon; Petzold, Christopher J.; Adams, Paul D.; Heazlewood, Joshua L.; Scheller, Henrik Vibe] Joint BioEnergy Inst, Emeryville, CA 94608 USA.
[Rennie, Emilie A.; Ebert, Berit; Christiansen, Katy M.; Stonebloom, Solomon; Petzold, Christopher J.; Adams, Paul D.; Heazlewood, Joshua L.; Scheller, Henrik Vibe] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
[Rennie, Emilie A.; Scheller, Henrik Vibe] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.
[Miles, Godfrey P.; Dupree, Paul] Univ Cambridge, Dept Biochem, Cambridge CB2 1QW, England.
[Cahoon, Rebecca E.; Khatab, Hoda; Cahoon, Edgar B.] Univ Nebraska, Ctr Plant Sci Innovat, Lincoln, NE 68588 USA.
[Cahoon, Rebecca E.; Khatab, Hoda; Cahoon, Edgar B.] Univ Nebraska, Dept Biochem, Lincoln, NE 68588 USA.
[Twell, David] Univ Leicester, Dept Biol, Leicester LE1 7RH, Leics, England.
[Adams, Paul D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.
RP Scheller, HV (reprint author), Joint BioEnergy Inst, Emeryville, CA 94608 USA.
EM hscheller@lbl.gov
RI Heazlewood, Joshua/A-2554-2008; Adams, Paul/A-1977-2013; Ebert,
Berit/F-1856-2016; Scheller, Henrik/A-8106-2008
OI Heazlewood, Joshua/0000-0002-2080-3826; Adams, Paul/0000-0001-9333-8219;
Ebert, Berit/0000-0002-6914-5473; Scheller, Henrik/0000-0002-6702-3560
FU U.S. Department of Energy, Office of Science, Office of Biological and
Environmental Research [DE-AC02-05CH11231]; National Science Foundation
Graduate Research Fellowship Program [DGE 1106400]; National Science
Foundation [MCB 115850]
FX We thank Sherry Chan for technical assistance and Tsan-Yiu Chiu for
providing vectors. This work was supported by the U.S. Department of
Energy, Office of Science, Office of Biological and Environmental
Research, through Contract DE-AC02-05CH11231 between Lawrence Berkeley
National Lab and the U.S. Department of Energy and by National Science
Foundation Graduate Research Fellowship Program Grant DGE 1106400
(E.A.R.) and National Science Foundation Grant MCB 115850 (E.B.C.).
NR 70
TC 13
Z9 14
U1 3
U2 21
PU AMER SOC PLANT BIOLOGISTS
PI ROCKVILLE
PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA
SN 1040-4651
EI 1532-298X
J9 PLANT CELL
JI Plant Cell
PD AUG
PY 2014
VL 26
IS 8
BP 3314
EP 3325
DI 10.1105/tpc.114.129171
PG 12
WC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
SC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
GA AU9MX
UT WOS:000345918600009
PM 25122154
ER
PT J
AU Boswell, R
Kaganovich, ID
AF Boswell, Rod
Kaganovich, Igor D.
TI Special issue on transport in B-fields in low-temperature plasmas
SO PLASMA SOURCES SCIENCE & TECHNOLOGY
LA English
DT Editorial Material
C1 [Boswell, Rod] Australian Natl Univ, Canberra, ACT, Australia.
[Kaganovich, Igor D.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Boswell, R (reprint author), Australian Natl Univ, Canberra, ACT, Australia.
NR 15
TC 0
Z9 0
U1 3
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0963-0252
EI 1361-6595
J9 PLASMA SOURCES SCI T
JI Plasma Sources Sci. Technol.
PD AUG
PY 2014
VL 23
IS 4
AR 040201
DI 10.1088/0963-0252/23/4/040201
PG 2
WC Physics, Fluids & Plasmas
SC Physics
GA AU7DR
UT WOS:000345761500001
ER
PT J
AU Griswold, ME
Raitses, Y
Fisch, NJ
AF Griswold, Martin E.
Raitses, Yevgeny
Fisch, Nathaniel J.
TI Cross-field plasma lens for focusing of the Hall thruster plume
SO PLASMA SOURCES SCIENCE & TECHNOLOGY
LA English
DT Article
DE Hall thruster; plasma lens; anomalous transport
ID ION-BEAMS
AB Hall thrusters produce neutralized ion beams with high current density because the acceleration takes place in quasi-neutral plasma and is not subject to space charge limitation. We tested an external plasma lens (PL) in front of the thruster as a means to focus the thruster plume. In the PL, the plasma is nearly collisionless, with non-magnetized flowing ions and magnetized electrons. Surprisingly, we observed anomalous electron cross-field transport, leading to large currents to the PL electrode and enhanced power loss.
C1 [Griswold, Martin E.; Raitses, Yevgeny; Fisch, Nathaniel J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Griswold, ME (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM martin.griswold@alumni.princeton.edu
FU US DOE [DE-AC02-09CH11466]; Air Force Office of Scientific Research; DOE
Fusion Energy Sciences Fellowship
FX This work was supported by the US DOE under Contract No
DE-AC02-09CH11466 and by the Air Force Office of Scientific Research.
MEG acknowledges the support of a DOE Fusion Energy Sciences Fellowship.
NR 19
TC 2
Z9 2
U1 4
U2 11
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0963-0252
EI 1361-6595
J9 PLASMA SOURCES SCI T
JI Plasma Sources Sci. Technol.
PD AUG
PY 2014
VL 23
IS 4
AR 044005
DI 10.1088/0963-0252/23/4/044005
PG 6
WC Physics, Fluids & Plasmas
SC Physics
GA AU7DR
UT WOS:000345761500008
ER
PT J
AU Appy, D
Lei, HP
Wang, CZ
Tringides, MC
Liu, DJ
Evans, JW
Thiel, PA
AF Appy, David
Lei, Huaping
Wang, Cai-Zhuang
Tringides, Michael C.
Liu, Da-Jiang
Evans, James W.
Thiel, Patricia A.
TI Transition metals on the (0001) surface of graphite: Fundamental aspects
of adsorption, diffusion, and morphology
SO PROGRESS IN SURFACE SCIENCE
LA English
DT Review
DE Graphite; Graphene; Transition metal; Nucleation; Adsorption; Diffusion
ID SCANNING-TUNNELING-MICROSCOPY; ORIENTED PYROLYTIC-GRAPHITE; ATOMIC-FORCE
MICROSCOPY; NANOMETER-SIZED PITS; GOLD CLUSTERS; NANOPARTICLE ARRAYS;
EQUILIBRIUM SHAPE; PROBE MICROSCOPY; MOLECULE CORRALS; DENDRITIC GROWTH
AB In this article, we review basic information about the interaction of transition metal atoms with the (0001) surface of graphite, especially fundamental phenomena related to growth. Those phenomena involve adatom-surface bonding, diffusion, morphology of metal clusters, interactions with steps and sputter-induced defects, condensation, and desorption. General traits emerge which have not been summarized previously. Some of these features are rather surprising when compared with metal-on-metal adsorption and growth. Opportunities for future work are pointed out. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Appy, David; Lei, Huaping; Wang, Cai-Zhuang; Tringides, Michael C.; Liu, Da-Jiang; Evans, James W.; Thiel, Patricia A.] Ames Lab, Ames, IA 50011 USA.
[Appy, David; Thiel, Patricia A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA.
[Lei, Huaping; Tringides, Michael C.; Evans, James W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.
[Thiel, Patricia A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA.
[Lei, Huaping] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China.
RP Thiel, PA (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
FU U.S. Department of Energy (USDOE), Office of Basic Energy Sciences,
Materials Sciences and Engineering Division; U.S. Department of Energy
(USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences,
Geosciences; Biosciences through the Ames Laboratory Chemical Physics
program; Ames Laboratory which is operated for the USDOE by Iowa State
University [DE-ACO207CH11358]; NSF [CHE-1111500]
FX Contributions by DA, HL, CZW, MCT, and PAT were supported by the U.S.
Department of Energy (USDOE), Office of Basic Energy Sciences, Materials
Sciences and Engineering Division through the Ames Laboratory Materials
Science program. Work by DJL was supported by the U.S. Department of
Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical
Sciences, Geosciences, and Biosciences through the Ames Laboratory
Chemical Physics program. The work was performed at Ames Laboratory
which is operated for the USDOE by Iowa State University under Contract
No. DE-ACO207CH11358. IWE's contribution was supported by NSF Grant
CHE-1111500.
NR 127
TC 11
Z9 11
U1 7
U2 55
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0079-6816
J9 PROG SURF SCI
JI Prog. Surf. Sci.
PD AUG-DEC
PY 2014
VL 89
IS 3-4
BP 219
EP 238
DI 10.1016/j.progsurf.2014.08.001
PG 20
WC Chemistry, Physical; Physics, Condensed Matter
SC Chemistry; Physics
GA AU6OD
UT WOS:000345721200001
ER
PT J
AU Chow, WW
Jahnke, F
Gies, C
AF Chow, Weng W.
Jahnke, Frank
Gies, Christopher
TI Emission properties of nanolasers during the transition to lasing
SO LIGHT-SCIENCE & APPLICATIONS
LA English
DT Review
DE nanolasers; optoelectronics; photon statistics; quantum light sources;
quantum optics; semiconductor quantum dots; thresholdless lasing
ID QUANTUM-DOT; PHASE-TRANSITION; OPTICAL MICROCAVITIES; MICROPILLAR
CAVITIES; LASER; DYNAMICS; ANALOGY; PHYSICS
AB This review addresses ongoing discussions involving nanolaser experiments, particularly those related to thresholdless lasing or few-emitter devices. A quantum-optical (quantum-mechanical active medium and radiation field) theory is used to examine the emission properties of nanolasers under different experimental configurations. The active medium is treated as inhomogeneously broadened semiconductor quantum dots embedded in a quantum well, where carriers are introduced via current injection. Comparisons are made between a conventional laser and a nanolaser with a spontaneous emission factor of unity, as well as a laser with only a few quantum dots providing the gain. It is found that the combined exploration of intensity, coherence time, photon autocorrelation function and carrier spectral hole burning can provide a unique and consistent picture of nanolasers in the new regimes of laser operation during the transition from thermal to coherent emission. Furthermore, by reducing the number of quantum dots in the optical cavity, a clear indication of non-classical photon statistics is observed before the single-quantum-dot limit is reached.
C1 [Chow, Weng W.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Jahnke, Frank; Gies, Christopher] Univ Bremen, Inst Theoret Phys, D-28334 Bremen, Germany.
RP Chow, WW (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM wwchow@sandia.gov
FU US Department of Energy, Office of Science, Office of Basic Energy
Sciences; Deutsche Forschungsgemeinschaft; [SFB787]
FX The present extension of the nanolaser model was developed at the Energy
Frontier Research Center for Solid-State Lighting Science, funded by the
US Department of Energy, Office of Science, Office of Basic Energy
Sciences. The application of this model to the specific cases of unity
spontaneous emission and the few-emitter limit was performed under
Sandia's LDRD program. FJ and CG acknowledge financial support from the
Deutsche Forschungsgemeinschaft. WWC is grateful for the hospitality of
the Technical University Berlin and travel support provided by SFB787.
FJ acknowledges the hospitality of the Sandia National Laboratories.
NR 45
TC 29
Z9 29
U1 3
U2 33
PU CHINESE ACAD SCIENCES, CHANGCHUN INST OPTICS FINE MECHANICS AND PHYSICS
PI CHANGCHUN
PA 3888, DONGNANHU ROAD, CHANGCHUN, 130033, PEOPLES R CHINA
SN 2047-7538
J9 LIGHT-SCI APPL
JI Light-Sci. Appl.
PD AUG
PY 2014
VL 3
AR e201
DI 10.1038/lsa.2014.82
PG 8
WC Optics
SC Optics
GA AT8MN
UT WOS:000345187400005
ER
PT J
AU Polyakov, A
Melli, M
Cantarella, G
Schwartzberg, A
Weber-Bargioni, A
Schuck, PJ
Cabrini, S
AF Polyakov, Aleksandr
Melli, Mauro
Cantarella, Giuseppe
Schwartzberg, Adam
Weber-Bargioni, Alexander
Schuck, P. James
Cabrini, Stefano
TI Coupling model for an extended-range plasmonic optical transformer
scanning probe
SO LIGHT-SCIENCE & APPLICATIONS
LA English
DT Article
DE optical transformer; plasmonic tip; plasmon coupling
ID SINGLE-MOLECULE FLUORESCENCE; DIFFRACTION LIMIT; SURFACE-PLASMONS;
MICROSCOPY; SPECTROSCOPY; NANOCAVITIES; LIGHT; GUIDE; TIPS
AB The expansion of nanoscale optics has generated a variety of scanning probe geometries that yield spatial resolution below 10 nm. In this work, we present a physical model for coupling far-field radiation to plasmonic modes on the surface of a scanning probe, and propose a scheme for extending the working distance of such a probe. In a subsurface application, an optical transformer at the tip of a probe can be coupled to a remote near-field antenna placed inside the sample at a distance away from the surface, expanding the effective working distance up to 100 nm.
C1 [Polyakov, Aleksandr; Melli, Mauro; Cantarella, Giuseppe; Schwartzberg, Adam; Weber-Bargioni, Alexander; Schuck, P. James; Cabrini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Polyakov, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 67-2206G, Berkeley, CA 94720 USA.
EM apolyakov@lbl.gov; scabrini@lbl.gov
RI Foundry, Molecular/G-9968-2014
FU Office of Science, Office of Basic Energy Sciences, Scientific User
Facilities Division of the US Department of Energy [DE-AC02-05CH11231]
FX This work was performed at the Molecular Foundry, Lawrence Berkeley
National Laboratory, and was supported by the Office of Science, Office
of Basic Energy Sciences, Scientific User Facilities Division of the US
Department of Energy under Contract No. DE-AC02-05CH11231.
NR 43
TC 4
Z9 4
U1 3
U2 10
PU CHINESE ACAD SCIENCES, CHANGCHUN INST OPTICS FINE MECHANICS AND PHYSICS
PI CHANGCHUN
PA 3888, DONGNANHU ROAD, CHANGCHUN, 130033, PEOPLES R CHINA
SN 2047-7538
J9 LIGHT-SCI APPL
JI Light-Sci. Appl.
PD AUG
PY 2014
VL 3
AR e195
DI 10.1038/lsa.2014.76
PG 6
WC Optics
SC Optics
GA AT8MN
UT WOS:000345187400002
ER
PT J
AU Goldman, AI
AF Goldman, Alan I.
TI Magnetism in icosahedral quasicrystals: current status and open
questions
SO SCIENCE AND TECHNOLOGY OF ADVANCED MATERIALS
LA English
DT Review
DE quasicrystals; rare earth magnetism; frustration; spin glass transition;
quantum critical behavior; magnetic ordering; neutron scattering
ID ZN-MG-HO; EARTH-METALS SYSTEMS; NEUTRON-SCATTERING; PENROSE LATTICE;
ANTIFERROMAGNETIC ORDER; ELECTRICAL-PROPERTIES; SPIN CORRELATIONS;
ATOMIC-STRUCTURE; ISING-MODEL; MN ALLOYS
AB Progress in our understanding of the magnetic properties of R-containing icosahedral quasicrystals (R = rare earth element) from over 20 years of experimental effort is reviewed. This includes the much studied R-Mg-Zn and R-Mg-Cd ternary systems, as well as several magnetic quasicrystals that have been discovered and investigated more recently including Sc-Fe-Zn, R-Ag-In, Yb-Au-Al, the recently synthesized R-Cd binary quasicrystals, and their periodic approximants. In many ways, the magnetic properties among these quasicrystals are very similar. However, differences are observed that suggest new experiments and promising directions for future research.
C1 [Goldman, Alan I.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.
Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.
RP Goldman, AI (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.
EM goldman@ameslab.gov
FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences,
Materials Science and Engineering Division; US DOE by Iowa State
University [DE-AC02-07CH11358]
FX I would like to acknowledge not only useful interactions, but also
delightful collaborations, over the past few years with Andreas
Kreyssig, Sergey Bud'ko, Tai Kong, Anton Jesche, Guillaume Beutier,
Takanobu Hiroto, Tsunetomo Yamada, Jong Woo Kim, Min Gyu Kim, Shibabrata
Nandi, Mandy Caudle, Mehmet Ramazanoglu, Kevin Dennis, Jens-Uwe Hoffman,
Claire Colin, Ian Fisher, Matthew Kramer, Patricia Thiel, Ryuji Tamura,
Mark de Boissieu and, especially, Paul Canfield. This work was supported
by the US Department of Energy (DOE), Office of Science, Basic Energy
Sciences, Materials Science and Engineering Division. The research was
performed at the Ames Laboratory, which is operated for the US DOE by
Iowa State University under contract # DE-AC02-07CH11358.
NR 107
TC 11
Z9 11
U1 7
U2 25
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND
SN 1468-6996
EI 1878-5514
J9 SCI TECHNOL ADV MAT
JI Sci. Technol. Adv. Mater.
PD AUG
PY 2014
VL 15
IS 4
AR 044801
DI 10.1088/1468-6996/15/4/044801
PG 15
WC Materials Science, Multidisciplinary
SC Materials Science
GA AT6CC
UT WOS:000345025400007
PM 27877699
ER
PT J
AU Gorton, I
AF Gorton, Ian
TI Cyberinfrastructures: Bridging the Divide between Scientific Research
and Software Engineering
SO COMPUTER
LA English
DT Article
AB Cyberinfrastructures-scientific research environments that span multiple institutions-require careful crafting and collaboration among domain specialists and software engineers, but several factors impede this collaboration. Recognizing five rules of thumb can help facilitate successful cyberinfrastructure creation and accelerate science in the disciplines they support.
C1 Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Gorton, I (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM igorton@sei.cmu.edu
NR 12
TC 1
Z9 1
U1 0
U2 0
PU IEEE COMPUTER SOC
PI LOS ALAMITOS
PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA
SN 0018-9162
EI 1558-0814
J9 COMPUTER
JI Computer
PD AUG
PY 2014
VL 47
IS 8
BP 48
EP 55
PG 8
WC Computer Science, Hardware & Architecture; Computer Science, Software
Engineering
SC Computer Science
GA AS8BW
UT WOS:000344476300018
ER
PT J
AU Denton, RE
Takahashi, K
Thomsen, MF
Borovsky, JE
Singer, HJ
Wang, Y
Goldstein, J
Brandt, PC
Reinisch, BW
AF Denton, R. E.
Takahashi, K.
Thomsen, M. F.
Borovsky, J. E.
Singer, H. J.
Wang, Y.
Goldstein, J.
Brandt, P. C.
Reinisch, B. W.
TI Evolution of mass density and O plus concentration at geostationary
orbit during storm and quiet events
SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS
LA English
DT Article
ID INNER MAGNETOSPHERE; ELECTRON-DENSITIES; OUTER PLASMASPHERE; POLAR-CAP;
ART.; FIELD; PLASMAPAUSE; IONS; IONOSPHERE; DYNAMICS
AB We investigated mass density rho(m) and O+ concentration eta(O+) = n(O+)/n(e) (where n(O+) and n(e) are the O+ and electron density, respectively) during two events, one active and one more quiet. We found rho(m) from observations of Alfven wave frequencies measured by the GOES, and we investigated composition by combining measurements of rho(m) with measurements of ion density n(MPA, i) from the Magnetospheric Plasma Analyzer (MPA) instrument on Los Alamos National Laboratory spacecraft or n(e) from the Radio Plasma Imager instrument on the Imager forMagnetopause-to-Aurora Global Exploration spacecraft. Using a simple assumption for the He+ density at solar maximum based on a statistical study, we found eta(O+) values ranging from near zero to close to unity. For geostationary spacecraft that corotate with the Earth, sudden changes in density for both rho(m) and n(e) often appear between dusk and midnight magnetic local time, especially when Kp is significantly above zero. This probably indicates that the bulk (total) ions have energy below a few keV and that the satellites are crossing from closed or previously closed to open drift paths. During long periods that are geomagnetically quiet, the mass density varies little, but ne gradually refills leading to a gradual change in composition from low-density plasma that is relatively cold and heavy (high-average ion mass M = rho(m)/n(e)) to high-density plasma that is relatively cold and light (low M) plasmasphere-like plasma. During active periods we observe a similar daily oscillation in plasma properties from the dayside to the nightside, with cold and light high-density plasma (more plasmasphere-like) on the dayside and hotter and more heavy low-density plasma (more plasma sheet-like) on the nightside. The value of ne is very dependent on whether it is measured inside or outside a plasmaspheric plume, while rho(m) is not. All of our results were found at solar maximum; previous results suggest that there will be much less O+ at solar minimum under all conditions.
C1 [Denton, R. E.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA.
[Takahashi, K.; Brandt, P. C.] Johns Hopkins Univ Appl Phys Lab, Laurel, MD USA.
[Thomsen, M. F.] Los Alamos Natl Lab, Los Alamos, NM USA.
[Borovsky, J. E.] Space Sci Inst, Boulder, CO USA.
[Singer, H. J.] Natl Ocean & Atmospher Adm Space Weather Predict, Boulder, CO USA.
[Wang, Y.] NASA Goddard Space Flight Ctr, Goddard Earth Sci & Technol Ctr, Greenbelt, MD USA.
[Wang, Y.] Univ Maryland Baltimore Cty, Baltimore, MD 21228 USA.
[Goldstein, J.] Southwest Res Inst, San Antonio, TX USA.
[Reinisch, B. W.] Univ Massachusetts Lowell, Space Sci Lab, Lowell, MA USA.
RP Denton, RE (reprint author), Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA.
EM richard.e.denton@dartmouth.edu
RI Brandt, Pontus/N-1218-2016
OI Brandt, Pontus/0000-0002-4644-0306
FU NSF [AGS-1105790, ATM-0855924]; NASA [NNX10AQ60G, NNX11AO59G]
FX Work at Dartmouth College was supported by NSF grant AGS-1105790 and
NASA grants NNX10AQ60G (Living with a Star Targeted Research
Plasmasphere focused science topic) and NNX11AO59G (Heliophysics Theory
Program). Work at the Applied Physics Laboratory was supported by NSF
grant ATM-0855924. We thank the reviewers for helpful comments.
Supplementary materials for this paper include GOES magnetometer data,
calculated Alfven frequencies and mass density, and IMAGE RPI electron
density. Most LANL MPA data used in this study are available at CDAWeb.
NR 44
TC 4
Z9 4
U1 1
U2 7
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 2169-9380
EI 2169-9402
J9 J GEOPHYS RES-SPACE
JI J. Geophys. Res-Space Phys.
PD AUG
PY 2014
VL 119
IS 8
DI 10.1002/2014JA019888
PG 15
WC Astronomy & Astrophysics
SC Astronomy & Astrophysics
GA AT3BJ
UT WOS:000344809600028
ER
PT J
AU Jha, PK
Churchfield, MJ
Moriarty, PJ
Schmitz, S
AF Jha, Pankaj K.
Churchfield, Matthew J.
Moriarty, Patrick J.
Schmitz, Sven
TI Guidelines for Volume Force Distributions Within Actuator Line Modeling
of Wind Turbines on Large-Eddy Simulation-Type Grids
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
ID STOKES COMPUTATIONS; WAKES
AB The objective of this work is to develop and test a set of general guidelines for choosing parameters to be used in the state-of-the-art actuator line method (ALM) for modeling wind turbine blades in computational fluid dynamics (CFD). The actuator line method is being increasingly used for the computation of wake interactions in large wind farms in which fully blade-resolving simulations are expensive and require complicated rotating meshes. The focus is on actuator line behavior using fairly isotropic grids of low aspect ratio typically used for large-eddy simulation (LES). Forces predicted along the actuator lines need to be projected onto the flow field as body forces, and this is commonly accomplished using a volumetric projection. In this study, particular attention is given to the spanwise distribution of the radius of this projection. A new method is proposed where the projection radius varies along the blade span following an elliptic distribution. The proposed guidelines for actuator line parameters are applied to the National Renewable Energy Laboratory's (NREL's) Phase VI rotor and the NREL 5-MW turbine. Results obtained are compared with available data and the blade-element code XTURB-PSU. It is found that the new criterion for the projection radius leads to improved prediction of blade tip loads for both blade designs.
C1 [Jha, Pankaj K.; Schmitz, Sven] Penn State Univ, Dept Aerosp Engn, University Pk, PA 16802 USA.
[Churchfield, Matthew J.; Moriarty, Patrick J.] Natl Wind Technol Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Jha, PK (reprint author), Penn State Univ, Dept Aerosp Engn, University Pk, PA 16802 USA.
FU Department of Energy as part of the "Cyber Wind Facility" project at The
Pennsylvania State University [DE-EE0005481]; NREL
FX This work was supported by the Department of Energy (DE-EE0005481) as
part of the "Cyber Wind Facility" project at The Pennsylvania State
University and in collaboration with NREL.
NR 51
TC 4
Z9 4
U1 2
U2 12
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2014
VL 136
IS 3
AR 031003
DI 10.1115/1.4026252
PG 11
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA AS8SN
UT WOS:000344518500003
ER
PT J
AU Ma, ZW
Glatzmaier, G
Mehos, M
AF Ma, Zhiwen
Glatzmaier, Greg
Mehos, Mark
TI Fluidized Bed Technology for Concentrating Solar Power With Thermal
Energy Storage
SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME
LA English
DT Article
DE concentrating solar power; thermal energy storage; fluidized bed; solid
particle
AB A generalized modeling method is introduced and used to evaluate thermal energy storage (TES) performance. The method describes TES performance metrics in terms of three efficiencies: first-law efficiency, second-law efficiency, and storage effectiveness. By capturing all efficiencies in a systematic way, various TES technologies can be compared on an equal footing before more detailed simulations of the components and concentrating solar power (CSP) system are performed. The generalized performance metrics are applied to the particle-TES concept in a novel CSP thermal system design. The CSP thermal system has an integrated particle receiver and fluidized-bed heat exchanger, which uses gas/solid two-phase flow as the heat-transfer fluid, and solid particles as the heat carrier and storage medium. The TES method can potentially achieve high temperatures (>800 degrees C) and high thermal efficiency economically.
C1 [Ma, Zhiwen; Glatzmaier, Greg; Mehos, Mark] Natl Renewable Energy Lab, Concentrating Solar Power Program, Golden, CO 80401 USA.
RP Ma, ZW (reprint author), Natl Renewable Energy Lab, Concentrating Solar Power Program, 15013 Denver West Pkwy,MS RSF033, Golden, CO 80401 USA.
EM zhiwen.ma@nrel.gov; Greg.Glatzmaier@nrel.gov; Mark.Mehos@nrel.gov
FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable
Energy Laboratory; U.S. Department of Energy, SunShot Initiative
[DE-EE0001586]
FX This work was supported by the U.S. Department of Energy under Contract
No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory.
The authors thank the funding support by the U.S. Department of Energy,
SunShot Initiative, under award number DE-EE0001586.
NR 23
TC 8
Z9 8
U1 1
U2 12
PU ASME
PI NEW YORK
PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA
SN 0199-6231
EI 1528-8986
J9 J SOL ENERG-T ASME
JI J. Sol. Energy Eng. Trans.-ASME
PD AUG
PY 2014
VL 136
IS 3
AR 031014
DI 10.1115/1.4027262
PG 9
WC Energy & Fuels; Engineering, Mechanical
SC Energy & Fuels; Engineering
GA AS8SN
UT WOS:000344518500014
ER
PT J
AU Shumpert, BL
Wolfe, AK
Bjornstad, DJ
Wang, S
Campa, MF
AF Shumpert, Barry L.
Wolfe, Amy K.
Bjornstad, David J.
Wang, Stephanie
Campa, Maria Fernanda
TI Specificity and Engagement: Increasing ELSI's Relevance to
Nano-Scientists
SO NANOETHICS
LA English
DT Article
DE Emerging technologies; Ethical, legal, and social issues; Nano-ELSI
literature; Nanoscience
AB Scholars studying the ethical, legal, and social issues (ELSI) associated with emerging technologies maintain the importance of considering these issues throughout the research and development cycle, even during the earliest stages of basic research. Embedding these considerations within the scientific process requires communication between ELSI scholars and the community of physical scientists who are conducting that basic research. We posit that this communication can be effective on a broad scale only if it links societal issues directly to characteristics of the emerging technology that are relevant to the physical and natural scientists involved in research and development. In this article, we examine nano-ELSI literature from 2003 to 2010 to discern the degree to which it makes these types of explicit connections. We find that, while the literature identifies a wide range of issues of societal concern, it generally does so in a non-specific manner. It neither links societal issues to particular forms or characteristics of widely divergent nanotechnologies nor to any of the many potential uses to which those nanotechnologies may be put. We believe that these kinds of specificity are essential to those engaged in nano-scale research. We also compare the literature-based findings to observations from interviews we conducted with nanoscientists and conclude that ELSI scholars should add technical- and application-related forms of specificity to their work and their writings to enhance effectiveness and impact in communicating with one important target audience-members of the nano-scale science community.
C1 [Shumpert, Barry L.; Wolfe, Amy K.; Bjornstad, David J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Wang, Stephanie] Oak Ridge Natl Lab Program, Oak Ridge, TN USA.
[Campa, Maria Fernanda] Univ Tennessee, Bredesen Ctr Interdisciplinary Res, Knoxville, TN USA.
[Campa, Maria Fernanda] Univ Tennessee, Grad Educ, Knoxville, TN USA.
RP Wolfe, AK (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA.
EM wolfeak@ornl.gov
FU U.S. Department of Energy, Office of Science, Office of Biological and
Environmental Research; U.S. Department of Energy [DE-AC05-00OR22725,
DE-AC05-06OR23100]; Oak Ridge Associated Universities
[DE-AC05-06OR23100]
FX This research was funded by the U.S. Department of Energy, Office of
Science, Office of Biological and Environmental Research.; This
manuscript has been authored by UT-Battelle, LLC, under Contract No.
DE-AC05-00OR22725 with the U.S. Department of Energy. The United States
Government retains and the publisher, by accepting the article for
publication, acknowledges that the United States Government retains a
non-exclusive, paid-up, irrevocable, world-wide license to publish or
reproduce the published form of this manuscript, or allow others to do
so, for United States Government purposes. This research was also
performed under two appointments to the Higher Education Research
Experiences (HERE) at the Oak Ridge National Laboratory (ORNL),
administered by the Oak Ridge Institute for Science and Education
(ORISE) under contract number DE-AC05-06OR23100 between the U.S.
Department of Energy and Oak Ridge Associated Universities.
NR 15
TC 1
Z9 1
U1 0
U2 4
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 1871-4757
EI 1871-4765
J9 NANOETHICS
JI NanoEthics
PD AUG
PY 2014
VL 8
IS 2
BP 193
EP 200
DI 10.1007/s11569-014-0194-x
PG 8
WC Ethics; History & Philosophy Of Science
SC Social Sciences - Other Topics; History & Philosophy of Science
GA AT2XC
UT WOS:000344796600007
ER
PT J
AU McGrath, S
Hodkinson, TR
Frohlich, A
Grant, J
Barth, S
AF McGrath, Sarah
Hodkinson, Trevor R.
Frohlich, Andreas
Grant, Jim
Barth, Susanne
TI Seasonal and genetic variations in water-soluble carbohydrates and other
quality traits in ecotypes and cultivars of perennial ryegrass (Lolium
perenne L.)
SO PLANT GENETIC RESOURCES-CHARACTERIZATION AND UTILIZATION
LA English
DT Article
DE carbohydrates; ecotypes; genetic resources; perennial ryegrass; protein
content; seasonal variation
ID NUTRITIVE-VALUE; IMPROVEMENT; GRASSES; AGRICULTURE; POPULATIONS;
METABOLISM; MORPHOLOGY; FRUCTAN; PROTEIN; MODEL
AB Phenotyping of genetic resources remains the bottleneck in the characterization of genetic resources, since the advent of modern next-generation sequencing technologies has made genotyping much more cost-and time-effective. This article reports on the phenotyping of agriculturally important traits in perennial ryegrass (Lolium perenne). In the present study, water-soluble carbohydrate (WSC), crude protein and dry matter contents were recorded for 1320 individuals, pooled into 132 samples from 33 perennial ryegrass ecotypes and cultivars at five different harvest time points across the 2004 growing season. While, in general, the cultivars had higher WSC contents than the ecotypes, individual ecotypes did show potential to be used in breeding programmes, as they had higher values than all other accessions at particular cutting time points. In correlation analyses, positive relationships were observed between dry matter and glucose contents both early and late in the growing season. Principal components analysis allowed the split either between cultivars and ecotypes or between tetraploid cultivars and the rest of the accessions at four of the five cutting time points. In the analysis of variance, cutting time was the most significant factor influencing the variation in traits.
C1 [McGrath, Sarah; Frohlich, Andreas; Barth, Susanne] TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland.
[McGrath, Sarah; Hodkinson, Trevor R.] Univ Dublin Trinity Coll, Sch Nat Sci, Dept Bot, Dublin 2, Ireland.
[Grant, Jim] TEAGASC, Operat Res Grp, Stat & Appl Phys Dept, Dublin 15, Ireland.
RP Barth, S (reprint author), TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland.
EM susanne.barth@teagasc.ie
RI Barth, Susanne/P-3366-2014; Hodkinson, Trevor/F-6850-2014
OI Barth, Susanne/0000-0002-4104-5964; Hodkinson,
Trevor/0000-0003-1384-7270
FU Teagasc and the Genetic Resources for Food and Agriculture Scheme of the
Irish Department of Agriculture, Fisheries and the Marine; Teagasc PhD
student fellowship; European Community
FX This project was financed by Teagasc and the Genetic Resources for Food
and Agriculture Scheme of the Irish Department of Agriculture, Fisheries
and the Marine. SMG received a Teagasc PhD student fellowship. The
authors are grateful to Monica Francioso, Simona Lamorte, Laura
Castelli, Jan Philip Jacobsen and Henry Skowski (all supported by the
European Community "Leonardo da Vinci" programme) and Adeline Airault
for their technical help in carbohydrate analysis.
NR 39
TC 0
Z9 0
U1 1
U2 19
PU CAMBRIDGE UNIV PRESS
PI CAMBRIDGE
PA EDINBURGH BLDG, SHAFTESBURY RD, CB2 8RU CAMBRIDGE, ENGLAND
SN 1479-2621
EI 1479-263X
J9 PLANT GENET RESOUR-C
JI Plant Genet. Resour.-Charact. Util.
PD AUG
PY 2014
VL 12
IS 2
BP 236
EP 247
DI 10.1017/S1479262113000567
PG 12
WC Plant Sciences; Genetics & Heredity
SC Plant Sciences; Genetics & Heredity
GA AS9DF
UT WOS:000344542700009
ER
PT J
AU Fent, KW
Eisenberg, J
Snawder, J
Sammons, D
Pleil, JD
Stiegel, MA
Mueller, C
Horn, GP
Dalton, J
AF Fent, Kenneth W.
Eisenberg, Judith
Snawder, John
Sammons, Deborah
Pleil, Joachim D.
Stiegel, Matthew A.
Mueller, Charles
Horn, Gavin P.
Dalton, James
TI Systemic Exposure to PAHs and Benzene in Firefighters Suppressing
Controlled Structure Fires
SO ANNALS OF OCCUPATIONAL HYGIENE
LA English
DT Article
DE aromatic hydrocarbons; benzene; biomarkers; dermal exposure; exhaled
breath; firefighters; PAHs; urine
ID POLYCYCLIC AROMATIC-HYDROCARBONS; ASPHALT PAVING WORKERS; ENVIRONMENTAL
EXPOSURE; DERMAL EXPOSURE; CANCER-RISK; ABSORPTION; BREATH; BIOMARKERS;
PENETRATION; EXHAUST
AB Turnout gear provides protection against dermal exposure to contaminants during firefighting; however, the level of protection is unknown. We explored the dermal contribution to the systemic dose of polycyclic aromatic hydrocarbons (PAHs) and other aromatic hydrocarbons in firefighters during suppression and overhaul of controlled structure burns. The study was organized into two rounds, three controlled burns per round, and five firefighters per burn. The firefighters wore new or laundered turnout gear tested before each burn to ensure lack of PAH contamination. To ensure that any increase in systemic PAH levels after the burn was the result of dermal rather than inhalation exposure, the firefighters did not remove their self-contained breathing apparatus until overhaul was completed and they were > 30 m upwind from the burn structure. Specimens were collected before and at intervals after the burn for biomarker analysis. Urine was analyzed for phenanthrene equivalents using enzyme-linked immunosorbent assay and a benzene metabolite (s-phenylmercapturic acid) using liquid chromatography/tandem mass spectrometry; both were adjusted by creatinine. Exhaled breath collected on thermal desorption tubes was analyzed for PAHs and other aromatic hydrocarbons using gas chromatography/mass spectrometry. We collected personal air samples during the burn and skin wipe samples (corn oil medium) on several body sites before and after the burn. The air and wipe samples were analyzed for PAHs using a liquid chromatography with photodiode array detection. We explored possible changes in external exposures or biomarkers over time and the relationships between these variables using non-parametric sign tests and Spearman tests, respectively. We found significantly elevated (P < 0.05) post-exposure breath concentrations of benzene compared with pre-exposure concentrations for both rounds. We also found significantly elevated post-exposure levels of PAHs on the neck compared with pre-exposure levels for round 1. We found statistically significant positive correlations between external exposures (i.e. personal air concentrations of PAHs) and biomarkers (i.e. change in urinary PAH metabolite levels in round 1 and change in breath concentrations of benzene in round 2). The results suggest that firefighters wearing full protective ensembles absorbed combustion products into their bodies. The PAHs most likely entered firefighters' bodies through their skin, with the neck being the primary site of exposure and absorption due to the lower level of dermal protection afforded by hoods. Aromatic hydrocarbons could have been absorbed dermally during firefighting or inhaled during the doffing of gear that was off-gassing contaminants.
C1 [Fent, Kenneth W.; Eisenberg, Judith; Mueller, Charles] NIOSH, Div Surveillance Hazard Evaluat & Field Studies, Cincinnati, OH 45226 USA.
[Snawder, John; Sammons, Deborah] NIOSH, Div Appl Res & Technol, Cincinnati, OH 45226 USA.
[Pleil, Joachim D.] US Environm Protect Agcy, Human Exposure & Atmospher Sci Div, Res Triangle Pk, NC 27709 USA.
[Stiegel, Matthew A.] Gillings Sch Global Publ, Oak Ridge Inst Sci & Educ, Chapel Hill, NC 27599 USA.
[Horn, Gavin P.] Univ Illinois, Illinois Fire Serv Inst, Champaign, IL 61820 USA.
[Dalton, James] Chicago Fire Dept, Training Div, Res & Dev Sect, Chicago, IL 60607 USA.
RP Fent, KW (reprint author), NIOSH, Div Surveillance Hazard Evaluat & Field Studies, 4676 Columbia Pkwy, Cincinnati, OH 45226 USA.
EM kfent@cdc.gov
OI Pleil, Joachim/0000-0001-8211-0796
FU National Institute for Occupational Safety and Health (NIOSH) by
National Occupational Research Agenda; NIOSH Human Subjects Review Board
FX National Institute for Occupational Safety and Health (NIOSH) by
intramural award under the National Occupational Research Agenda; NIOSH
Human Subjects Review Board.
NR 48
TC 10
Z9 11
U1 5
U2 35
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 0003-4878
EI 1475-3162
J9 ANN OCCUP HYG
JI Ann. Occup. Hyg.
PD AUG
PY 2014
VL 58
IS 7
BP 830
EP 845
DI 10.1093/annhyg/meu036
PG 16
WC Public, Environmental & Occupational Health; Toxicology
SC Public, Environmental & Occupational Health; Toxicology
GA AS4IY
UT WOS:000344239400004
PM 24906357
ER
PT J
AU Burkes, DE
Casella, AM
Buck, EC
Casella, AJ
Edwards, MK
MacFarlan, PJ
Pool, KN
Smith, FN
Steen, FH
AF Burkes, Douglas E.
Casella, Andrew M.
Buck, Edgar C.
Casella, Amanda J.
Edwards, Matthew K.
MacFarlan, Paul J.
Pool, Karl N.
Smith, Frances N.
Steen, Franciska H.
TI Development and Validation of Capabilities to Measure Thermal Properties
of Layered Monolithic U-Mo Alloy Plate-Type Fuel
SO INTERNATIONAL JOURNAL OF THERMOPHYSICS
LA English
DT Article
DE Multilayer; Nuclear fuel; Thermal conductivity; Uranium-molybdenum
ID ZR DIFFUSION BARRIER; WT.PERCENT-MO; PHYSICAL-PROPERTIES; TEMPERATURE
AB The uranium-molybdenum (U-Mo) alloy in a monolithic form has been proposed as one fuel design capable of converting some of the world's highest power research reactors from the use of high enriched uranium to low enriched uranium. One aspect of the fuel development and qualification process is to demonstrate appropriate understanding of the thermal-conductivity behavior of the fuel system as a function of temperature and expected irradiation conditions. The purpose of this paper is to verify functionality of equipment installed in hot cells for eventual measurements on irradiated uranium-molybdenum (U-Mo) monolithic fuel specimens, refine procedures to operate the equipment, and validate models to extract the desired thermal properties. The results presented here demonstrate the adequacy of the equipment, procedures, and models that have been developed for this purpose based on measurements conducted on surrogate depleted uranium-molybdenum (DU-Mo) alloy samples containing a Zr diffusion barrier and clad in aluminum alloy 6061 (AA6061). The results are in excellent agreement with thermal property data reported in the literature for similar U-Mo alloys as a function of temperature.
C1 [Burkes, Douglas E.; Casella, Andrew M.] Pacific NW Natl Lab, Engn & Anal Grp, Nucl Syst Design, Richland, WA 99352 USA.
[Buck, Edgar C.; Casella, Amanda J.; Edwards, Matthew K.; MacFarlan, Paul J.; Pool, Karl N.; Smith, Frances N.] Pacific NW Natl Lab, Nucl Chem & Engn Grp, Richland, WA 99352 USA.
[Steen, Franciska H.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Burkes, DE (reprint author), Pacific NW Natl Lab, Engn & Anal Grp, Nucl Syst Design, POB 999,MSIN K8-34, Richland, WA 99352 USA.
EM Douglas.Burkes@pnnl.gov
RI Buck, Edgar/N-7820-2013;
OI Buck, Edgar/0000-0001-5101-9084; Casella, Andrew/0000-0002-4053-6593
FU Global Threat Reduction Initiative [DE-AC05-76RL01830]
FX The authors wish to acknowledge Mr. Jason Schulthess, Mr. Adam Robinson,
Mr. Glenn Moore, Mr. Brady Mackowiak, Mr. Blair Park, Dr. Barry Rabin,
and Mrs. Susan Case from Idaho National Laboratory for the fabrication
of the surrogate plates and delivery of the surrogate mini-plates.
Installation of equipment into hot cells and the operations conducted in
hot cells are a large undertaking. The authors wish to acknowledge those
at Pacific Northwest National Laboratory who were involved in the
preparation of samples and performance of measurements, specifically Ms.
Nicole Green, Mr. Jake Bohlke, Mr. Jamin Trevino, Mr. Dustin Blundon,
Ms. Brittany Carman, Mr. Jason Cartwright, Mr. Jeffrey Chenault, Mr.
Steve Halstead, Mr. Eric Hanson, Mr. Kevin Heaton, Mr. Robert Orton, Mr.
Stan Owsley, Mr. Ben Palma, Mr. Mario Pereira, Mr. Bruce Slonecker, Mr.
Timothy Smith, Mr. Randy Thornhill, and Mr. Patrick Valdez. Finally, the
authors wish to acknowledge the sponsor, the Global Threat Reduction
Initiative, for the opportunity to conduct this work under Contract
DE-AC05-76RL01830.
NR 32
TC 3
Z9 3
U1 0
U2 4
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 0195-928X
EI 1572-9567
J9 INT J THERMOPHYS
JI Int. J. Thermophys.
PD AUG
PY 2014
VL 35
IS 8
BP 1476
EP 1500
DI 10.1007/s10765-014-1683-4
PG 25
WC Thermodynamics; Chemistry, Physical; Mechanics; Physics, Applied
SC Thermodynamics; Chemistry; Mechanics; Physics
GA AR9WB
UT WOS:000343925800005
ER
PT J
AU Hathcock, CD
Fair, JM
AF Hathcock, Charles D.
Fair, Jeanne M.
TI HAZARDS TO BIRDS FROM OPEN METAL PIPES
SO WESTERN NORTH AMERICAN NATURALIST
LA English
DT Article
AB There are reports of open polyvinyl chloride (PVC) pipes causing bird deaths in the western United States (Brattstrom 1995). Here, we document cases of open bollards and open pipes on gates causing bird deaths in northern New Mexico. At Los Alamos National Laboratory (LANL), a 10,240-ha site, over 100 uncapped 10.16 cm diameter protective bollard posts were examined, and 27% of the open bollards contained dead birds. A total of 88 open pipes used as gate posts, with diameters of 8.89 cm or 10.16 cm, were examined, and 11% contained dead birds. We conducted a preliminary assessment of open pipes on gates along a highway on federal land north of LANL, and 14% of the open pipes contained dead birds. This gate configuration, with open pipes anchoring the gate on either side, is very common in the western United States. In all cases, Western Bluebirds (Sialia mexicana) composed the majority of the identifiable birds we discovered. Based on these preliminary findings, the number of bird deaths from this source is potentially very large and should be a concern in bird conservation and management.
C1 [Hathcock, Charles D.; Fair, Jeanne M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Hathcock, CD (reprint author), Los Alamos Natl Lab, Box 1663,Mailstop J978, Los Alamos, NM 87545 USA.
EM hathcock@lanl.gov
FU Environmental Protection Division through Los Alamos National Security,
LLC, operator of the Los Alamos National Laboratory [DEAC52-06NA25396]
FX We thank M. Alexander, P Gallagher, S. Terp, J. Payne, D. Keller, H.
Mahowald, K. Schoenberg, M. Musgrave, A. Smith, B. Lechel, A. Jacobs, L.
Martinez, and P Maestas. This research was funded by the Environmental
Protection Division through Los Alamos National Security, LLC, operator
of the Los Alamos National Laboratory under Contract No.
DEAC52-06NA25396 for the National Nuclear Security Administration of the
U.S. Department of Energy.
NR 6
TC 2
Z9 2
U1 1
U2 7
PU BRIGHAM YOUNG UNIV
PI PROVO
PA 290 LIFE SCIENCE MUSEUM, PROVO, UT 84602 USA
SN 1527-0904
EI 1944-8341
J9 WEST N AM NATURALIST
JI West. North Am. Naturalist
PD AUG
PY 2014
VL 74
IS 2
BP 228
EP 230
PG 3
WC Biodiversity Conservation; Ecology
SC Biodiversity & Conservation; Environmental Sciences & Ecology
GA AS7BW
UT WOS:000344413500009
ER
PT J
AU Fleetwood, D
Brown, D
Girard, S
Gouker, P
Gerardin, S
Quinn, H
Barnaby, H
AF Fleetwood, Dan
Brown, Dennis
Girard, Sylvain
Gouker, Pascale
Gerardin, Simone
Quinn, Heather
Barnaby, Hugh
TI SELECTED PAPERS FROM THE 2013 RADIATION AND ITS EFFECTS ON COMPONENTS
AND SYSTEMS (RADECS) CONFERENCE, Oxford, UK, September 23-27, 2013
Comments by the Editors
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Editorial Material
C1 [Fleetwood, Dan] Vanderbilt Univ, Nashville, TN 37235 USA.
[Girard, Sylvain] Univ St Etienne, St Etienne, France.
[Gouker, Pascale] MIT Lincoln Lab, Cambridge, MD USA.
[Gerardin, Simone] Univ Padua, I-35100 Padua, Italy.
[Quinn, Heather] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Barnaby, Hugh] Arizona State Univ, Tempe, AZ 85287 USA.
RP Fleetwood, D (reprint author), Vanderbilt Univ, Nashville, TN 37235 USA.
NR 0
TC 0
Z9 0
U1 0
U2 0
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 1507
EP 1507
DI 10.1109/TNS.2014.2344371
PN 1
PG 1
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9WT
UT WOS:000343928100002
ER
PT J
AU Javanainen, A
Ferlet-Cavrois, V
Bosser, A
Jaatinen, J
Kettunen, H
Muschitiello, M
Pintacuda, F
Rossi, M
Schwank, JR
Shaneyfelt, MR
Virtanen, A
AF Javanainen, Arto
Ferlet-Cavrois, Veronique
Bosser, Alexandre
Jaatinen, Jukka
Kettunen, Heikki
Muschitiello, Michele
Pintacuda, Francesco
Rossi, Mikko
Schwank, James R.
Shaneyfelt, Marty R.
Virtanen, Ari
TI SEGR in SiO2-Si3N4 Stacks
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article; Proceedings Paper
CT European Conference on Radiation and its Effects on Components and
Systems (RADECS)
CY SEP 23-27, 2013
CL Oxford, ENGLAND
SP Synergy Hlth plc, RADECS Assoc, IEEE, Nucl & Plasma Sci Soc, AWE, Intersil, Peregrine Semicond
DE Modeling; MOS; semi-empirical; Si3N4; SiO2; Single Event Gate Rupture
(SEGR)
ID EVENT GATE RUPTURE; BREAKDOWN; SILICON
AB This paper presents experimental Single Event Gate Rupture (SEGR) data for Metal-Insulator-Semiconductor (MIS) devices, where the gate dielectrics are made of stacked SiO2-Si3N4 structures. A semi-empirical model for predicting the critical gate voltage in these structures under heavy-ion exposure is first proposed. Then interrelationship between SEGR cross-section and heavy-ion induced energy deposition probability in thin dielectric layers is discussed. Qualitative connection between the energy deposition in the dielectric and the SEGR is proposed.
C1 [Javanainen, Arto; Bosser, Alexandre; Jaatinen, Jukka; Kettunen, Heikki; Rossi, Mikko; Virtanen, Ari] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland.
[Ferlet-Cavrois, Veronique; Muschitiello, Michele] European Space Agcy, Estec, NL-2200 AG Noordwijk, Netherlands.
[Pintacuda, Francesco] STMicroelectronics Srl, I-95121 Catania, Italy.
[Schwank, James R.; Shaneyfelt, Marty R.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Javanainen, A (reprint author), Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland.
EM arto.javanainen@jyu.fi
RI Javanainen, Arto/P-6355-2016
OI Javanainen, Arto/0000-0001-7906-3669
NR 11
TC 3
Z9 3
U1 0
U2 2
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 1902
EP 1908
DI 10.1109/TNS.2014.2303493
PN 1
PG 7
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9WT
UT WOS:000343928100057
ER
PT J
AU Rempe, JL
Knudson, DL
AF Rempe, Joy L.
Knudson, Darrell L.
TI Instrumentation Performance During the TMI-2 Accident
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Accident instrumentation; Three Mile Island Unit 2
AB The accident at the Three Mile Island Unit 2 (TMI-2) reactor provided a unique opportunity to evaluate sensors exposed to severe accident conditions. The loss of coolant and the hydrogen combustion that occurred during this accident exposed instrumentation to harsh conditions, including direct radiation, radioactive contamination, and high humidity with elevated temperatures and pressures. As part of a program initiated by the Department of Energy Office of Nuclear Energy (DOE-NE), a review was completed to gain insights from prior TMI-2 sensor survivability and data qualification efforts. This new effort focused upon a set of sensors that provided critical data to TMI-2 operators for assessing the condition of the plant and the effects of mitigating actions taken by these operators. In addition, the effort considered sensors providing data required for subsequent accident simulations. Over 100 references related to instrumentation performance and post-accident evaluations of TMI-2 sensors and measurements were reviewed. Insights gained from this review are summarized within this paper. As noted within this paper, several techniques were invoked in the TMI-2 post-accident program to evaluate sensor survivability status and data qualification, including comparisons with data from other sensors, analytical calculations, laboratory testing, and comparisons with sensors subjected to similar conditions in large-scale integral tests and with sensors that were similar in design but more easily removed from the TMI-2 plant for evaluations. Conclusions from this review provide important insights related to sensor survivability and enhancement options for improving sensor performance. In addition, this paper provides recommendations related to sensor survivability and the data evaluation process that could be implemented in upcoming Fukushima Daiichi recovery efforts.
C1 [Rempe, Joy L.; Knudson, Darrell L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Rempe, JL (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA.
EM joy.rempe@inl.gov
OI Rempe, Joy/0000-0001-5527-3549
FU U.S. Department of Energy, Office of Nuclear Energy, Science, and
Technology, under DOE-NE Idaho Operations Office [DE AC07 05ID14517]
FX This work was supported by the U.S. Department of Energy, Office of
Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations
Office Contract DE AC07 05ID14517.
NR 9
TC 1
Z9 1
U1 1
U2 7
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 1963
EP 1970
DI 10.1109/TNS.2013.2293350
PN 2
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400002
ER
PT J
AU Rempe, JL
Knudson, DL
Daw, JE
Unruh, TC
Chase, BM
Davis, KL
Palmer, AJ
Schley, RS
AF Rempe, J. L.
Knudson, D. L.
Daw, J. E.
Unruh, T. C.
Chase, B. M.
Davis, K. L.
Palmer, A. J.
Schley, R. S.
TI Advanced In-Pile Instrumentation for Materials Testing Reactors
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE In-pile detectors; radiation resistant sensors
ID THERMAL-CONDUCTIVITY MEASUREMENT; NUCLEAR-FUELS; IRRADIATION;
THERMOCOUPLES
AB The U.S. Department of Energy sponsors the Advanced Test Reactor (ATR) National Scientific User Facility (NSUF) program to promote U.S. research in nuclear science and technology. By attracting new research users - universities, laboratories, and industry - the ATR NSUF facilitates basic and applied nuclear research and development, advancing U.S. energy security needs. A key component of the ATR NSUF effort is to design, develop, and deploy new in-pile instrumentation techniques that are capable of providing real-time measurements of key parameters during irradiation. This paper describes the strategy developed by the Idaho National Laboratory (INL) for identifying instrumentation needed for ATR irradiation tests and the program initiated to obtain these sensors. New sensors developed from this effort are identified, and the progress of other development efforts is summarized. As reported in this paper, INL researchers are currently involved in several tasks to deploy real-time length and flux detection sensors, and efforts have been initiated to develop a crack growth test rig. Tasks evaluating 'advanced' technologies, such as fiber-optics based length detection and ultrasonic thermometers, are also underway. In addition, specialized sensors for real-time detection of temperature and thermal conductivity are not only being provided to NSUF reactors, but are also being provided to several international test reactors.
C1 [Rempe, J. L.; Knudson, D. L.; Daw, J. E.; Unruh, T. C.; Chase, B. M.; Davis, K. L.; Palmer, A. J.; Schley, R. S.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Rempe, JL (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA.
EM Joy.Rempe@inl.gov
RI Schley, Robert/B-9124-2017;
OI Schley, Robert/0000-0001-8907-6535; Rempe, Joy/0000-0001-5527-3549
FU U.S. Department of Energy, Office of Nuclear Energy, Science, and
Technology, under DOE-NE Idaho Operations Office [DE AC07 05ID14517]
FX This research was supported by the U.S. Department of Energy, Office of
Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations
Office Contract DE AC07 05ID14517.
NR 22
TC 0
Z9 0
U1 0
U2 6
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 1984
EP 1994
DI 10.1109/TNS.2014.2335616
PN 2
PG 11
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400005
ER
PT J
AU Vaccaro, S
Hu, J
Svedkauskaite, J
Smejkal, A
Schwalbach, P
De Baere, P
Gauld, IC
AF Vaccaro, S.
Hu, J.
Svedkauskaite, J.
Smejkal, A.
Schwalbach, P.
De Baere, P.
Gauld, I. C.
TI A New Approach to Fork Measurements Data Analysis by RADAR-CRISP and
ORIGEN Integration
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Depletion modelling; fork detector measurements; nuclear safeguards;
spent fuel verification
ID SCALE
AB Currently, in the EU, activities related to storage of spent fuel are constantly increasing. This is particularly true in Finland and Sweden, where final geological repository sites are planned to be operational in 2023 and 2026 respectively, but also in several other countries where fuel is moved from wet ponds to dry storage (Germany, Belgium, Spain, Czech Republic, Bulgaria). The required verification activities present a considerable challenge to the EURATOM Safeguards authority. Both EURATOM and IAEA safeguards need to know the contents of the storage casks and keep continuity of knowledge of the spent fuel. A frequently-used tool for the verification of the nuclear material during loading is the Fork detector for gross gamma and neutron counting. The data acquisition applications RADAR (Remote Acquisition of Data and Review) and CRISP (Central RADAR Inspection Support Package), developed by EURATOM, are used to acquire safeguards measurement data and to analyse them in order to verify the declarations of the nuclear plant operators. Under the framework of the U. S. DOE-EURATOM agreement on nuclear safeguards and security, a module for automated analysis of spent fuel measurement data using the ORIGEN (Oak Ridge Isotope GENeration) code, part of the SCALE nuclear systems modelling and simulation package, has been integrated into CRISP. Measurement data are collected in an unattended mode by RADAR and then processed by CRISP, which outputs, for each fuel assembly, the measured gamma and neutron count rates. In parallel, ORIGEN performs burn-up calculations based on operator declarations previously entered into CRISP and calculates the expected neutron and gamma count rates for each assembly. These calculations use detector response functions, developed using Monte Carlo modelling, to account for the detection probabilities of both neutron and photon particles that originate in each fuel pin. Finally, CRISP correlates and compares the expected (calculated) gamma and neutron signals with the measured values. The comparison is presented to the inspector to help draw safeguards conclusions. This paper will show initial case studies of in-field applications of the CRISP-ORIGEN approach for safeguards inspection activities during the loading of a spent fuel cask.
C1 [Vaccaro, S.; Svedkauskaite, J.; Smejkal, A.; Schwalbach, P.; De Baere, P.] Commiss European Communities, Directorate Gen Energy, L-2310 Luxembourg, Luxembourg.
[Hu, J.; Gauld, I. C.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA.
RP Vaccaro, S (reprint author), Commiss European Communities, Directorate Gen Energy, L-2310 Luxembourg, Luxembourg.
EM stefano.vaccaro@ec.eu-ropa.eu
OI Gauld, Ian/0000-0002-3893-7515
FU U.S. Department of Energy NNSA under the U.S.-Euratom cooperation
agreement
FX This work was supported in part by the U.S. Department of Energy NNSA
under the U.S.-Euratom cooperation agreement.
NR 16
TC 2
Z9 2
U1 1
U2 4
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2161
EP 2168
DI 10.1109/TNS.2014.2320604
PN 2
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400030
ER
PT J
AU LaFleur, AM
Croft, S
Mayer, RL
Swinhoe, MT
Mayo, DR
Sapp, BA
AF LaFleur, Adrienne M.
Croft, Stephen
Mayer, Richard L.
Swinhoe, Martyn T.
Mayo, Douglas R.
Sapp, Benjamin A.
TI Traceable Determination of the Absolute Neutron Emission Yields of UO2F2
Working Reference Materials
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Holdup; nondestructive assay; nuclear safeguards; uranium enrichment
AB The nuclear material contained in the process equipment of a uranium enrichment plant (referred to as holdup) is an important component of the overall nuclear material inventory for the plant. Accurate quantification and verification of holdup is needed to improve international safeguards and nuclear material accountancy. This is also needed for criticality safety and waste disposition. Passive neutron and gamma-ray nondestructive assay (NDA) methods are used to measure the holdup in process equipment. A key advantage of neutron measurements is that neutrons are highly penetrating and can be measured through thick walled equipment. The dominant source of neutrons in the UO2F2 holdup is from the F-19(alpha,n)Na-22 reaction resulting from U-234 alpha decay when uranium is enriched. There is a considerable spread between different historic determinations of the F-19(alpha,n) yield from uranium which limits the accuracy of modeling and the calibration of NDA instruments. Furthermore, the compound form and presence of water also significantly affects the neutron emission rate from the holdup. This paper describes a series of experimental measurements performed at Los Alamos National Laboratory (LANL) to determine the absolute neutron emission yield from 10 different UO2F2 working reference materials (WRMs) fabricated at the Portsmouth Gaseous Diffusion Plant (PGDP). The Mini Epithermal Neutron Multiplicity Counter (Mini ENMC) and a NIST certified neutron source were used for these measurements. The high efficiency and short die-away time of the Mini ENMC provides the high measurement precision needed to certify the neutron emission yield. The experiment was designed to achieve sub 1% accuracy in the net counting rate on each item and to provide assurance that important factors such as instrument stability, item placement and background were well understood. The traceable neutron yields measured from the WRMs were used to determine a more accurate neutron yield for the UO2F2 material. The results were compared to historical neutron emission rates. The F(alpha,n) data obtained from these measurements directly supports nuclear safeguards for NDA of uranium holdup and provides a more accurate calibration for new and existing NDA detector systems.
C1 [LaFleur, Adrienne M.; Swinhoe, Martyn T.; Mayo, Douglas R.; Sapp, Benjamin A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Croft, Stephen] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Mayer, Richard L.] DOE Portsmouth Paducah Project Off, Piketon, OH 45661 USA.
RP LaFleur, AM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM alafleur@lanl.gov; crofts@ornl.gov; Richard.Mayer@lex.doe.gov;
swinhoe@lanl.gov; mayo@lanl.gov; bsapp@lanl.gov
FU Department of Energy National Nuclear Security Administration (NNSA)
Office of Nonproliferation and International Security
FX This work was supported by the Department of Energy National Nuclear
Security Administration (NNSA) Office of Nonproliferation and
International Security.
NR 23
TC 0
Z9 0
U1 0
U2 1
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2182
EP 2188
DI 10.1109/TNS.2013.2284435
PN 2
PG 7
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400033
ER
PT J
AU Chapelle, A
Authier, N
Casoli, P
Richard, B
Myers, W
Hutchinson, J
Sood, A
Rooney, B
AF Chapelle, Amaury
Authier, Nicolas
Casoli, Pierre
Richard, Benoit
Myers, Will
Hutchinson, Jesson
Sood, Avneet
Rooney, Brian
TI Joint Neutron Noise Measurements on Metallic Reactor Caliban
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Bare reactor; Caliban; Feynman method; Hage-Cifarelli; Hansen-Dowdy;
helium 3; kinetic parameters; neutron noise; Rossi method;
subcriticality; uncertainties
AB The aim of the experiments concerning neutron noise measurements presented in this article is to provide robust experimental subcritical data. These measurements will make possible to compare measured parameters to simulated ones. The results of these measurements must therefore be very accurate, with controlled uncertainties. To determine the relative contribution of uncertainties to the final result, a table presents the prompt multiplication estimated by a French team and a U. S. team. The different sources of uncertainties are then explored, by a sensitivity analysis, separated in three categories, linked to the experimental configuration, to the detection process and finally to the analysis process. These experiments improve the safety task of reactivity control far from criticality, with static methods, and the knowledge of the behaviour of a subcritical reactor.
C1 [Chapelle, Amaury] EAMEA, F-50100 Cherbourg, France.
[Authier, Nicolas; Casoli, Pierre] CEA, F-21120 Valduc, France.
[Richard, Benoit] CEA, F-50100 Cherbourg, France.
[Myers, Will; Hutchinson, Jesson; Sood, Avneet; Rooney, Brian] LANL, Los Alamos, NM 87545 USA.
RP Chapelle, A (reprint author), EAMEA, F-50100 Cherbourg, France.
EM amaury.chapelle@eamea.fr
NR 8
TC 0
Z9 0
U1 2
U2 4
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2262
EP 2270
DI 10.1109/TNS.2014.2320853
PN 2
PG 9
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400045
ER
PT J
AU Daw, J
Tittmann, B
Reinhardt, B
Kohse, G
Ramuhalli, P
Montgomery, R
Chien, HT
Villard, JF
Palmer, J
Rempe, J
AF Daw, J.
Tittmann, B.
Reinhardt, B.
Kohse, G.
Ramuhalli, P.
Montgomery, R.
Chien, H. -T.
Villard, J. -F.
Palmer, J.
Rempe, J.
TI Irradiation Testing of Ultrasonic Transducers
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE In-pile instrumentation; magnetostriction; material and test reactors;
piezoelectricity; ultrasonic transducers
ID RADIATION-DAMAGE; VELOCITY
AB Ultrasonic technologies offer the potential for high accuracy and resolution in-pile measurement of numerous parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of ultrasonic technologies to provide enhanced sensors for in-pile instrumentation during irradiation testing. For example, the ability of single, small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. Other efforts include an ultrasonic technique to detect morphology changes (such as crack initiation and growth) and acoustic techniques to evaluate fission gas composition and pressure. These efforts are limited by the lack of existing knowledge of ultrasonic transducer material survivability under irradiation conditions. To address this need, the Pennsylvania State University (PSU) was awarded an Advanced Test Reactor National Scientific User Facility (ATR NSUF) project to evaluate promising magnetostrictive and piezoelectric transducer performance in the Massachusetts Institute of Technology Research Reactor (MITR) up to a fast fluence of at least 10(21) n/cm(2) (E > 0.1 MeV). This test will be an instrumented lead test; and real-time transducer performance data will be collected along with temperature and neutron and gamma flux data. By characterizing magnetostrictive and piezoelectric transducer survivability during irradiation, test results will enable the development of novel radiation tolerant ultrasonic sensors for use in Material and Test Reactors (MTRs). The current work bridges the gap between proven out-of-pile ultrasonic techniques and in-pile deployment of ultrasonic sensors by acquiring the data necessary to demonstrate the performance of ultrasonic transducers.
C1 [Daw, J.; Palmer, J.; Rempe, J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Tittmann, B.; Reinhardt, B.] Penn State Univ, University Pk, PA 16802 USA.
[Kohse, G.] MIT, Cambridge, MA 02139 USA.
[Ramuhalli, P.; Montgomery, R.] Pacific NW Natl Lab, Richland, WA 99354 USA.
[Chien, H. -T.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Villard, J. -F.] Commissariat Energie Atom & Energies Alternat, Ctr Etud Cadarache, F-13108 St Paul Les Durance, France.
RP Daw, J (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA.
EM Joshua.Daw@inl.gov
OI Rempe, Joy/0000-0001-5527-3549; Ramuhalli, Pradeep/0000-0001-6372-1743
FU U.S. Department of Energy, Office of Nuclear Energy, Science, and
Technology, under DOE-NE Idaho Operations Office [DE AC07 05ID14517]
FX This work was supported by the U.S. Department of Energy, Office of
Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations
Office Contract DE AC07 05ID14517.
NR 22
TC 2
Z9 2
U1 1
U2 18
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2279
EP 2284
DI 10.1109/TNS.2014.2335613
PN 2
PG 6
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XF
UT WOS:000343929400047
ER
PT J
AU Mendoza, E
Cano-Ott, D
Koi, T
Guerrero, C
AF Mendoza, Emilio
Cano-Ott, Daniel
Koi, Tatsumi
Guerrero, Carlos
CA GEANT4 Collaboration
TI New Standard Evaluated Neutron Cross Section Libraries for the GEANT4
Code and First Verification
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE GEANT; Monte Carlo simulation; neutrons; radiation detectors; simulation
ID NUCLEAR-SCIENCE
AB The Monte Carlo simulation of the interaction of neutrons with matter relies on evaluated nuclear data libraries and models. The evaluated libraries are compilations of measured physical parameters (such as cross sections) combined with predictions of nuclear model calculations which have been adjusted to reproduce the experimental data. The results obtained from the simulations depend largely on the accuracy of the underlying nuclear data used, and thus it is important to have access to the nuclear data libraries available, either of general use or compiled for specific applications, and to perform exhaustive validations which cover the wide scope of application of the simulation code. In this paper we describe the work performed in order to extend the capabilities of the GEANT4 toolkit for the simulation of the interaction of neutrons with matter at neutron energies up to 20 MeV and a first verification of the results obtained. Such a work is of relevance for applications as diverse as the simulation of a neutron detector, an entire particle physics experiment, a fission or fusion nuclear reactor, a neutron shielding or a hadron therapy cancer treatment facility.
C1 [Mendoza, Emilio; Cano-Ott, Daniel] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid 208040, Spain.
[Koi, Tatsumi] Stanford Linear Accelerator Ctr, Stanford, CA 94309 USA.
[Guerrero, Carlos] CERN, CH-1211 Geneva, Switzerland.
RP Mendoza, E (reprint author), Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid 208040, Spain.
EM emilio.mendoza@ciemat.es; daniel.cano@ciemat.es;
tatsumi.koi@slac.stanford.edu; carlos.guerrero@cern.ch
RI Mendoza Cembranos, Emilio/K-5789-2014; Cano Ott, Daniel/K-4945-2014
OI Mendoza Cembranos, Emilio/0000-0002-2843-1801; Cano Ott,
Daniel/0000-0002-9568-7508
FU Spanish national company for radioactive waste ENRESA through
CIEMAT-ENRESA; Spanish Plan Nacional de I+D+i de Fisica de Particulas
[FPA2008-04972-C03-01]; Spanish Ministerio de Ciencia e Innovacion
through CONSOLIDER CSD [2007-00042]; European Union [262010]
FX This work was supported in part by the Spanish national company for
radioactive waste ENRESA, through the CIEMAT-ENRESA agreements on
"Transmutacion de residuos radiactivos de alta actividad," the Spanish
Plan Nacional de I+D+i de Fisica de Particulas (project
FPA2008-04972-C03-01), the Spanish Ministerio de Ciencia e Innovacion
through the CONSOLIDER CSD 2007-00042 project, and in part by the
European Union's Seventh Framework Programme under grant agreement
262010 (ENSAR).
NR 16
TC 13
Z9 13
U1 1
U2 9
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2357
EP 2364
DI 10.1109/TNS.2014.2335538
PN 3
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XI
UT WOS:000343929900007
ER
PT J
AU Hoover, AS
Winkler, R
Rabin, MW
Bennett, DA
Doriese, WB
Fowler, JW
Hayes-Wehle, J
Horansky, RD
Reintsema, CD
Schmidt, DR
Vale, LR
Ullom, JN
Schaffer, K
AF Hoover, Andrew S.
Winkler, Ryan
Rabin, Michael W.
Bennett, Douglas A.
Doriese, William B.
Fowler, Joseph W.
Hayes-Wehle, James
Horansky, Robert D.
Reintsema, Carl D.
Schmidt, Dan R.
Vale, Leila R.
Ullom, Joel N.
Schaffer, Kathryn
TI Uncertainty of Plutonium Isotopic Measurements with Microcalorimeter and
High-Purity Germanium Detectors
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Gamma-ray detectors; measurement uncertainty; spectroscopy;
superconducting photodetectors
ID GAMMA-RAY SPECTROSCOPY; PHOTON MASS ATTENUATION; X-RAY; COEFFICIENTS
AB The nondestructive assay (NDA) of plutonium-bearing materials using gamma-ray spectroscopy supports global nuclear nonproliferation and safeguards efforts. High-purity germanium (HPGe) detectors have been used for this application for decades, but the uncertainty limit remains around 1% relative error for measured isotope ratios, an order of magnitude larger than destructive assay. To lower NDA uncertainty limits, we are pursuing new measurement technology using superconducting microcalorimeter detectors, and assessing the sources of current uncertainty limits. We compare results from analysis of plutonium isotopic standards using HPGe and microcalorimeter detectors, and find lower random error for the microcalorimeter data. Uncertainties in the reference values of constants of nature contribute to the total measurement error. For one particular set of constants, the gamma-ray energies, we find that microcalorimeter analysis is much less sensitive (more than a factor of ten) to the uncertainty in nuclear data than HPGe.
C1 [Hoover, Andrew S.; Winkler, Ryan; Rabin, Michael W.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
[Bennett, Douglas A.; Doriese, William B.; Fowler, Joseph W.; Hayes-Wehle, James; Horansky, Robert D.; Reintsema, Carl D.; Schmidt, Dan R.; Vale, Leila R.; Ullom, Joel N.] NIST, Boulder, CO 80305 USA.
[Schaffer, Kathryn] Sch Art Inst Chicago, Chicago, IL 60603 USA.
RP Hoover, AS (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA.
FU U.S. Department of Energy Office of Nuclear Energy
FX This work was supported by the U.S. Department of Energy Office of
Nuclear Energy.
NR 26
TC 1
Z9 1
U1 0
U2 5
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2365
EP 2372
DI 10.1109/TNS.2014.2332275
PN 3
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XI
UT WOS:000343929900008
ER
PT J
AU Ayaz-Maierhafer, B
Zhang, X
Hayward, JP
Bell, ZW
Laubach, MA
AF Ayaz-Maierhafer, B.
Zhang, X.
Hayward, J. P.
Bell, Z. W.
Laubach, M. A.
TI Investigation of Active Background From Photofission in Depleted Uranium
Using Cherenkov Detectors and Gamma Ray Time-of-Flight Analysis
SO IEEE TRANSACTIONS ON NUCLEAR SCIENCE
LA English
DT Article
DE Cherenkov radiation; glass detectors; photo-fission
ID GLASS DETECTORS; BREMSSTRAHLUNG; INTERROGATION; RESOLUTION; ENERGY
AB Prompt gammas from induced fission could potentially be a valuable fission signature to use for detection of special nuclear materials like highly enriched uranium. Detectability requires an understanding of both signal and background, and the background from highly enriched uranium can be understood using depleted uranium as a surrogate. In order to study the prompt gamma active backgrounds from special nuclear materials induced through photofission, a combination of measurements using the Idaho Accelerator Center 44 MeV Electron Linear Accelerator and Monte CarloN-Particle simulations were used. In this paper, we discuss the prompt, time-gated glass Cherenkov detector response to gamma emissions resulting from short pulse 6, 10, and 25 MeV bremsstrahlung beams incident on a depleted uranium target. Considering any threshold used with the Cherenkov detectors, the prompt gamma signal from depleted uranium is buried in the active background from the interrogating photon source. This paper describes the contributions to this prominent prompt active background observed in our measurements.
C1 [Ayaz-Maierhafer, B.; Zhang, X.; Hayward, J. P.; Laubach, M. A.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA.
[Bell, Z. W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Ayaz-Maierhafer, B (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA.
EM bi1@ornl.gov
OI Bell, Zane/0000-0003-1115-8674
FU [1-09-1-0052]
FX This work was supported by Grant 1-09-1-0052.
NR 22
TC 2
Z9 2
U1 0
U2 6
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0018-9499
EI 1558-1578
J9 IEEE T NUCL SCI
JI IEEE Trans. Nucl. Sci.
PD AUG
PY 2014
VL 61
IS 4
BP 2402
EP 2409
DI 10.1109/TNS.2014.2332273
PN 3
PG 8
WC Engineering, Electrical & Electronic; Nuclear Science & Technology
SC Engineering; Nuclear Science & Technology
GA AR9XI
UT WOS:000343929900013
ER
PT J
AU Feld, GK
Frank, M
AF Feld, Geoffrey K.
Frank, Matthias
TI Enabling membrane protein structure and dynamics with X-ray free
electron lasers
SO CURRENT OPINION IN STRUCTURAL BIOLOGY
LA English
DT Article
ID SERIAL FEMTOSECOND CRYSTALLOGRAPHY; ROOM-TEMPERATURE;
ACETYLCHOLINE-RECEPTOR; COUPLED RECEPTORS; PHOTOSYSTEM-II;
NANOCRYSTALLOGRAPHY; DIFFRACTION; CRYSTALLIZATION; RESOLUTION;
OPPORTUNITIES
AB Determining the three-dimensional structures and dynamics of membrane proteins remains one of the great challenges of modern biology. The recent availability of X-ray free electron laser (XFEL) light sources has opened the door to a new and revolutionary approach to performing X-ray analysis of these important biomolecules. Recent advances in sample delivery, data reduction, and phasing have enabled the high-resolution structural probing of membrane proteins at room temperature. While considerable challenges remain, the recent developments described in this review may ultimately provide structural biologists with powerful tools for obtaining unprecedented atomic-scale and dynamic visualization of membrane proteins at near-physiological conditions.
C1 [Feld, Geoffrey K.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
[Frank, Matthias] Lawrence Livermore Natl Lab, Div Phys, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
RP Frank, M (reprint author), Lawrence Livermore Natl Lab, Div Phys, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
EM frank1@llnl.gov
RI Frank, Matthias/O-9055-2014
FU LLNL Lab-Directed Research and Development (LDRD) Project [012-ERD-031];
U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]
FX The authors thank Dr. Brent W. Segelke of Lawrence Livermore National
Laboratory (LLNL) for valuable commentary and suggestions, Dr. Bill
Pedrini of the Paul Scherrer Institute for contributing the diffraction
image in Figure 3, and Ryan W. Chen of LLNL's Technical Information
Department for helping to produce Figure 1. This work was supported by
LLNL Lab-Directed Research and Development (LDRD) Project 012-ERD-031
(to M.F.), and was performed under the auspices of the U.S. Department
of Energy by Lawrence Livermore National Laboratory under contract
DE-AC52-07NA27344.
NR 55
TC 12
Z9 12
U1 1
U2 22
PU CURRENT BIOLOGY LTD
PI LONDON
PA 84 THEOBALDS RD, LONDON WC1X 8RR, ENGLAND
SN 0959-440X
EI 1879-033X
J9 CURR OPIN STRUC BIOL
JI Curr. Opin. Struct. Biol.
PD AUG
PY 2014
VL 27
BP 69
EP 78
DI 10.1016/j.sbi.2014.05.002
PG 10
WC Biochemistry & Molecular Biology; Cell Biology
SC Biochemistry & Molecular Biology; Cell Biology
GA AR6JG
UT WOS:000343689300012
PM 24930119
ER
PT J
AU Holliday, VT
Surovell, T
Meltzer, DJ
Grayson, DK
Boslough, M
AF Holliday, Vance T.
Surovell, Todd
Meltzer, David J.
Grayson, Donald K.
Boslough, Mark
TI The Younger Dryas impact hypothesis: a cosmic catastrophe
SO JOURNAL OF QUATERNARY SCIENCE
LA English
DT Review
DE Clovis; extinction; extraterrestrial impact; Younger Dryas; Younger
Dryas impact hypothesis
ID SOUTHERN HIGH-PLAINS; NORTH-AMERICAN PALEOINDIANS; BEARS ARCTODUS-SIMUS;
EXTRATERRESTRIAL IMPACT; MURRAY SPRINGS; NEW-MEXICO; PLEISTOCENE
EXTINCTIONS; OKLAHOMA PANHANDLE; HUMAN RESPONSES; CLIMATE-CHANGE
AB In this paper we review the evidence for the Younger Dryas impact hypothesis (YDIH), which proposes that at similar to 12.9k cal a BP North America, South America, Europe and the Middle East were subjected to some sort of extraterrestrial event. This purported event is proposed as a catastrophic process responsible for: terminal Pleistocene environmental changes (onset of YD cooling, continent-scale wildfires); extinction of late Pleistocene mammals; and demise of the Clovis 'culture' in North America, the earliest well-documented, continent-scale settlement of the region. The basic physics in the YDIH is not in accord with the physics of impacts nor the basic laws of physics. No YD boundary (YDB) crater, craters or other direct indicators of an impact are known. Age control is weak to nonexistent at 26 of the 29 localities claimed to have evidence for the YDIH. Attempts to reproduce the results of physical and geochemical analyses used to support the YDIH have failed or show that many indicators are not unique to an impact nor to similar to 12.9k cal a BP. The depositional environments of purported indicators at most sites tend to concentrate particulate matter and probably created many 'YDB zones'. Geomorphic, stratigraphic and fire records show no evidence of any sort of catastrophic changes in the environment at or immediately following the YDB. Late Pleistocene extinctions varied in time and across space. Archeological data provide no indication of population decline, demographic collapse or major adaptive shifts at or just after similar to 12.9 ka. The data and the hypotheses generated by YDIH proponents are contradictory, inconsistent and incoherent. Copyright (C) 2014 John Wiley & Sons, Ltd.
C1 [Holliday, Vance T.] Univ Arizona, Sch Anthropol, Tucson, AZ 85721 USA.
[Surovell, Todd] Univ Wyoming, Dept Anthropol, Laramie, WY 82071 USA.
[Meltzer, David J.] So Methodist Univ, Dept Anthropol, Dallas, TX 75275 USA.
[Grayson, Donald K.] Univ Washington, Seattle, WA 98195 USA.
[Boslough, Mark] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Holliday, VT (reprint author), Univ Arizona, Sch Anthropol, Tucson, AZ 85721 USA.
EM vthollid@email.arizona.edu
OI Meltzer, David/0000-0001-8084-9802
NR 145
TC 7
Z9 8
U1 9
U2 54
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0267-8179
EI 1099-1417
J9 J QUATERNARY SCI
JI J. Quat. Sci.
PD AUG
PY 2014
VL 29
IS 6
BP 515
EP 530
DI 10.1002/jqs.2724
PG 16
WC Geography, Physical; Geosciences, Multidisciplinary
SC Physical Geography; Geology
GA AS0YR
UT WOS:000344003200002
ER
PT J
AU Aad, G
Abbott, B
Abdallah, J
Khalek, SA
Abdinov, O
Aben, R
Abi, B
Abolins, M
AbouZeid, OS
Abramowicz, H
Abreu, H
Abreu, R
Abulaitia, Y
Acharya, BS
Adamczyk, L
Adams, DL
Adelman, J
Adomeit, S
Adye, T
Agatonovic-Jovin, T
Aguilar-Saavedra, JA
Agustoni, M
Ahlen, SP
Ahmad, A
Ahmadov, F
Aielli, G
Aring;kesson, TPA
Akimoto, G
Akimov, AV
Alberghi, GL
Albert, J
Albrand, S
Verzini, MJA
Aleksa, M
Aleksandrov, IN
Alexa, C
Alexander, G
Alexandre, G
Alexopoulos, T
Alhroob, M
Alimonti, G
Alio, L
Alison, J
Allbrooke, BMM
Allison, LJ
Allport, PP
Allwood-Spiers, SE
Almond, J
Aloisio, A
Alonso, A
Alonso, F
Alpigiani, C
Altheimer, A
Gonzalez, BA
Alviggi, MG
Amako, K
Coutinho, YA
Amelung, C
Amidei, D
Dos Santos, SPA
Amorim, A
Amoroso, S
Amram, N
Amundsen, G
Anastopoulos, C
Ancu, LS
Andari, N
Andeen, T
Anders, CF
Anders, G
Anderson, KJ
Andreazza, A
Andrei, V
Anduaga, XS
Angelidakis, S
Angelozzi, I
Anger, P
Angerami, A
Anghinolfi, F
Anisenkov, AV
Anjos, N
Annovi, A
Antonaki, A
Antonelli, M
Antonov, A
Antos, J
Anulli, F
Aoki, M
Bella, LA
Apolle, R
Arabidze, G
Aracena, I
Arai, Y
Araque, JP
Arce, ATH
Arguin, JF
Argyropoulos, S
Arik, M
Armbruster, AJ
Arnaez, O
Arnal, V
Arnold, H
Arslan, O
Artamonov, A
Artoni, G
Asai, S
Asbah, N
Ashkenazi, A
Ask, S
Aring;sman, B
Asquith, L
Assamagan, K
Astalos, R
Atkinson, M
Atlay, NB
Auerbach, B
Augsten, K
Aurousseau, M
Avolio, G
Azuelos, G
Azuma, Y
Baak, MA
Bacci, C
Bachacou, H
Bachas, K
Backes, M
Backhaus, M
Mayes, JB
Badescu, E
Bagiacchi, P
Bagnaia, P
Bai, Y
Bain, T
Baines, JT
Baker, OK
Baker, S
Balek, P
Balli, F
Banas, E
Banerjee, S
Banfi, D
Bangert, A
Bannoura, AAE
Bansal, V
Bansil, HS
Barak, L
Baranov, SP
Barberio, EL
Barberis, D
Barbero, M
Barillari, T
Barisonzi, M
Barklow, T
Barlow, N
Barnett, BM
Barnett, RM
Barnovska, Z
Baroncelli, A
Barone, G
Barr, AJ
Barreiro, F
da Costa, JBG
Bartoldus, R
Barton, AE
Bartos, P
Bartsch, V
Bassalat, A
Basye, A
Bates, RL
Batkova, L
Batley, JR
Battistin, M
Bauer, F
Bawa, HS
Beau, T
Beauchemin, PH
Beccherle, R
Bechtle, P
Beck, HP
Becker, K
Becker, S
Beckingham, M
Becot, C
Beddall, AJ
Beddall, A
Bedikian, S
Bednyakov, VA
Bee, CP
Beemster, LJ
Beermann, TA
Begel, M
Behr, K
Belanger-Champagne, C
Bell, PJ
Bell, WH
Bella, G
Bellagamba, L
Bellerive, A
Bellomo, M
Belloni, A
Belotskiy, K
Beltramello, O
Benary, O
Benchekroun, D
Bendtz, K
Benekos, N
Benhammou, Y
Noccioli, EB
Garcia, JAB
Benjamin, DP
Bensinger, JR
Benslama, K
Bentvelsen, S
Berge, D
Kuutmann, EB
Berger, N
Berghaus, F
Berglund, E
Beringer, J
Bernabeu, J
Bernard, C
Bernat, P
Bernius, C
Bernlochner, FU
Berry, T
Berta, P
Bertella, C
Bertolucci, F
Besana, MI
Besjes, GJ
Bessidskaia, O
Besson, N
Betancourt, C
Bethke, S
Bhimji, W
Bianchi, RM
Bianchini, L
Bianco, M
Biebel, O
Bieniek, SP
Bierwagen, K
Biesiada, J
Bigliettia, M
De Mendizabal, JB
Bilokon, H
Bindi, M
Binet, S
Bingul, A
Bini, C
Black, CW
Black, JE
Black, KM
Blackburn, D
Blair, RE
Blanchard, JB
Blazek, T
Bloch, I
Blocker, C
Blum, W
Blumenschein, U
Bobbink, GJ
Bobrovnikov, VS
Bocchetta, SS
Bocci, A
Boddy, CR
Boehler, M
Boek, J
Boek, TT
Bogaerts, JA
Bogdanchikov, AG
Bogouch, A
Bohm, C
Bohm, J
Boisvert, V
Bold, T
Boldea, V
Boldyrev, AS
Bomben, M
Bona, M
Boonekamp, M
Borisov, A
Borissov, G
Borri, M
Borroni, S
Bortfeldt, J
Bortolotto, V
Bos, K
Boscherini, D
Bosman, M
Boterenbrood, H
Boudreau, J
Bouffard, J
Bouhova-Thacker, EV
Boumediene, D
Bourdarios, C
Bousson, N
Boutouil, S
Boveia, A
Boyd, J
Boyko, IR
Bozovic-Jelisavcic, I
Bracinik, J
Branchini, P
Brandt, A
Brandt, G
Brandt, O
Bratzler, U
Brau, B
Brau, JE
Braun, HM
Brazzale, SF
Brelier, B
Brendlinger, K
Brennan, AJ
Brenner, R
Bressler, S
Bristow, K
Bristow, TM
Britton, D
Brochu, FM
Brock, I
Brock, R
Bromberg, C
Bronner, J
Brooijmans, G
Brooks, T
Brooks, WK
Brosamer, J
Brost, E
Brown, G
Brown, J
de Renstrom, PAB
Bruncko, D
Bruneliere, R
Brunet, S
Bruni, A
Bruni, G
Bruschi, M
Bryngemark, L
Buanes, T
Buat, Q
Bucci, F
Buchholz, P
Buckingham, RM
Buckley, AG
Buda, SI
Budagov, IA
Buehrer, F
Bugge, L
Bugge, MK
Bulekov, O
Bundock, AC
Burckhart, H
Burdin, S
Burghgrave, B
Burke, S
Burmeister, I
Busato, E
Buscher, D
Buscher, V
Bussey, P
Buszello, CP
Butler, B
Butler, JM
Butt, AI
Buttar, CM
Butterworth, JM
Butti, P
Buttinger, W
Buzatu, A
Byszewski, M
Urban, SC
Caforio, D
Cakir, O
Calafiura, P
Calandri, A
Calderini, G
Calfayan, P
Calkins, R
Caloba, LP
Calvet, D
Calvet, S
Toro, RC
Camarda, S
Cameron, D
Caminada, LM
Armadans, RC
Campana, S
Campanelli, M
Campoverde, A
Canale, V
Canepa, A
Cantero, J
Cantrill, R
Cao, T
Garrido, MDMC
Caprini, I
Caprini, M
Capua, M
Caputo, R
Cardarelli, R
Carli, T
Carlino, G
Carminati, L
Caron, S
Carquin, E
Carrillo-Montoya, GD
Carter, AA
Carter, JR
Carvalho, J
Casadei, D
Casado, MP
Castaneda-Miranda, E
Castelli, A
Gimenez, VC
Castro, NF
Catastini, P
Catinaccio, A
Catmore, JR
Cattai, A
Cattani, G
Caughron, S
Cavaliere, V
Cavalli, D
Cavalli-Sforza, M
Cavasinni, V
Ceradini, F
Cerio, B
Cerny, K
Cerqueira, AS
Cerri, A
Cerrito, L
Cerutti, F
Cerv, M
Cervelli, A
Cetin, SA
Chafaq, A
Chakraborty, D
Chalupkova, I
Chan, K
Chang, P
Chapleau, B
Chapman, JD
Charfeddine, D
Charlton, DG
Chau, CC
Barajas, CAC
Cheatham, S
Chegwidden, A
Chekanov, S
Chekulaev, SV
Chelkov, GA
Chelstowska, MA
Chen, C
Chen, H
Chen, K
Chen, L
Chen, S
Chen, X
Chen, Y
Cheng, HC
Cheng, Y
Cheplakov, A
El Moursli, RC
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Zhemchugov, A.
Zhong, J.
Zhou, B.
Zhou, L.
Zhou, N.
Zhu, C. G.
Zhu, H.
Zhu, J.
Zhu, Y.
Zhuang, X.
Zibell, A.
Zieminska, D.
Zimine, N. I.
Zimmermann, C.
Zimmermann, R.
Zimmermann, S.
Zimmermann, S.
Zinonos, Z.
Ziolkowski, M.
Zobernig, G.
Zoccoli, A.
zur Nedden, M.
Zurzolo, G.
Zutshi, V.
Zwalinski, L.
CA ATLAS Collboration
TI Operation and performance of the ATLAS semiconductor tracker
SO JOURNAL OF INSTRUMENTATION
LA English
DT Article
DE Solid state detectors; Charge transport and multiplication in solid
media; Particle tracking detectors (Solid-state detectors); Detector
modelling and simulations I (interaction of radiation with matter,
interaction of photons with matter, interaction of hadrons with matter,
etc)
ID PROTON CROSS-SECTION; ROOT-S=7 TEV; DETECTOR; LHC; MODULES; SILICON;
SYSTEM; MONITOR; SINGLE; CHARGE
AB The semiconductor tracker is a silicon microstrip detector forming part of the inner tracking system of the ATLAS experiment at the LHC. The operation and performance of the semiconductor tracker during the first years of LHC running are described. More than 99% of the detector modules were operational during this period, with an average intrinsic hit efficiency of (99.74 +/- 0.04)%. The evolution of the noise occupancy is discussed, and measurements of the Lorentz angle, delta-ray production and energy loss presented. The alignment of the detector is found to be stable at the few-micron level over long periods of time. Radiation damage measurements, which include the evolution of detector leakage currents, are found to be consistent with predictions and are used in the verification of radiation background simulations.
C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia.
[Bouffard, J.; Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA.
[Butt, A. I.; Chan, K.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada.
[Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey.
[Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey.
[Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey.
[Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey.
[Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France.
[Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] Univ Savoie, Annecy Le Vieux, France.
[Asquith, L.; Auerbach, B.; Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; Goshaw, A. T.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Ferrando, B. M. Salvachua; Stanek, R. W.; van Gemmeren, P.; Vaniachine, A.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.
[Cheu, E.; Johns, K. A.; Kaushik, V.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Toggerson, B.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA.
[Brandt, A.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Maeno, M.; Nilsson, P.; Ozturk, N.; Pravahan, R.; Sosebee, M.; Spurlock, B.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA.
[Angelidakis, S.; Antonaki, A.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece.
[Alexopoulos, T.; Byszewski, M.; Dris, M.; Gazis, E. N.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece.
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[Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain.
[Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain.
[Dimitrievska, A.; Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia.
[Agatonovic-Jovin, T.; Bozovic-Jelisavcic, I.; Cirkovic, P.; Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia.
[Buanes, T.; Dale, O.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Martin dit Latour, B.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway.
[Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Hasib, A.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Joseph, J.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA.
[Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Joseph, J.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Kuutmann, E. Bergeaas; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany.
[Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland.
[Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland.
[Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England.
[Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey.
[Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey.
[Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey.
[Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Conta, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Dondero, P.; Fabbri, L.; Ferrari, R.; Franchini, M.; Fraternali, M.; Gabrielli, A.; Gaudio, G.; Giacobbe, B.; Grafstrom, P.; Livan, M.; Massa, I.; Mengarelli, A.; Negri, A.; Negrini, M.; Piccinini, M.; Polesello, G.; Polini, A.; Rebuzzi, D. M.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Vercesi, V.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy.
[Alberghi, G. L.; Caforio, D.; Conta, C.; De Castro, S.; Di Sipio, R.; Dondero, P.; Fabbri, L.; Franchini, M.; Fraternali, M.; Gabrielli, A.; Grafstrom, P.; Livan, M.; Massa, I.; Mengarelli, A.; Negri, A.; Piccinini, M.; Rebuzzi, D. M.; Rimoldi, A.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy.
[Bruni, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey.
[Arslan, O.; Bechtle, P.; Bellerive, A.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutt, F.; Stillings, J. A.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany.
[Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA.
[Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA.
[Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil.
[Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil.
[do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil.
[Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil.
[Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.
[Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoice, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania.
[Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania.
[Darlea, G. L.] Univ Politeh Bucharest, Bucharest, Romania.
[Chitan, A.] West Univ Timisoara, Timisoara, Romania.
[Silva, M. L. Gonzalez; Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina.
[Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Goodrick, M. J.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Shaw, R. S.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England.
[Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada.
[Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Uhrssen, M. D.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland.
[Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA.
[Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile.
[Brooks, W. K.; Kuleshov, S.; Petridis, A.; Pezo, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile.
[Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China.
[Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Songb, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China.
[Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China.
[Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China.
[Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France.
[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Li, Y.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France.
[Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA.
[Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark.
[Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy.
[Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy.
[Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland.
[Kuhl, A.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland.
[Banas, E.; Bruckman de Renstrom, P. A.; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland.
[Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA.
[Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA.
[Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Goncalves Pinto Firmino Da Costa, J.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany.
[Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; O'Neil, D. C.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany.
[Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany.
[Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA.
[Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland.
[Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy.
[Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany.
[Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Bilbao De Mendizabal, J.; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Perinia, L.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland.
[Barberis, D.; Darbo, G.; Favaret, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettinia, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy.
[Barberis, D.; Favaret, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy.
[Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia.
[Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia.
[Uren, M. D.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany.
[Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland.
[Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany.
[Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France.
[McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA.
[Barreiro Guimaraes da Costa, J.; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA.
[Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Kugel, A.; Laier, H.; Lang, V. S.; Meier, K.; Poddar, S.; Scharfa, V.; Schultz-Coulon, H. -C.; Stamen, R.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany.
[Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany.
[Colombo, T.; Kretz, M.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany.
[Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan.
[Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Lukas, W.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
[Franz, S.; Jussel, P.; Kneringer, E.; Nagai, K.; Pieron, J. P.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria.
[Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA.
[Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA.
[Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia.
[Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan.
[Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan.
[Takashima, R.] Kyoto Univ, Kyoto 612, Japan.
[Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan.
[Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis Plata, La Plata, Buenos Aires, Argentina.
[Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina.
[Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England.
[Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy.
[Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy.
[Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England.
[Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia.
[Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Univ Ljubljana, Ljubljana, Slovenia.
[Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England.
[Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England.
[Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Warren, M.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England.
Louisiana Tech Univ, Ruston, LA 71270 USA.
[Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France.
[Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, CNRS, IN2P3, Paris, France.
[Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Pater, J. R.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden.
[Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain.
[Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Konig, S.; Kopke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meade, A.; Meyer, C.; Moreno, D.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany.
[Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Peters, R. F. Y.; Price, D.; Qin, Y.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England.
[Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France.
[Bellomo, M.; Brau, B.; Chen, L.; Colon, G.; Dallapiccola, C.; Gao, J.; Liu, K.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] CNRS, IN2P3, Marseille, France.
[Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA.
[Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada.
[Barberio, E. L.; Brennan, A. J.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia.
[Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.
[Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.
[Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Univ Milan, INFN Sez Milano, Milan, Italy.
[Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy.
[Bogouch, A.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus.
[Harkusha, S.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus.
[Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA.
[Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada.
[Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia.
[Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia.
[Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia.
[Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnov, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany.
[Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany.
[Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan.
[Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan.
[Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy.
[Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy.
[Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA.
[Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands.
[Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands.
[Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands.
[Burghgrave, B.; Calkins, R.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA.
[Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia.
[Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA.
[Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA.
[Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan.
[Abbott, B.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA.
[Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA.
[Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palack Univ, RCPTM, Olomouc, Czech Republic.
[Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA.
[Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Chakraborty, D.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France.
[Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Chakraborty, D.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France.
[Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan.
[Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oslo, Dept Phys, Oslo, Norway.
[Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Conventi, F.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Della Pietra, M.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England.
[Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, I-27100 Pavia, Italy.
[Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy.
[Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA.
[Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia.
[Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.] Univ Pisa, INFN Sez Pisa, Pisa, Italy.
[Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy.
[Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA.
[Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal.
[Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal.
[Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Maio, A.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal.
[Gomes, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal.
[Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal.
[Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain.
[Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain.
[Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal.
[Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic.
[Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic.
[Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Kubik, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic.
[Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia.
[Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Petridou, C.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England.
[Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada.
[Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan.
[Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzania, S.; Nisati, A.; Pasqualucci, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN Sez Roma, I-00185 Rome, Italy.
[Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzania, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy.
[Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy.
[Aielli, G.; Cattani, G.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy.
[Bacci, C.; Baroncelli, A.; Bigliettia, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petruccia, F.; Stanescu, C.; Trovatelli, M.] Univ Roma Tre, INFN Sez Roma Tre, Rome, Italy.
[Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petruccia, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy.
[Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco.
[Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco.
[El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Oujda, Morocco.
[El Moursli, R. Cherkaoui; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco.
[Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, Inst Rech Lois Fondament Univers, DSM IRFU, Gif Sur Yvette, France.
[Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA.
[Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA.
[Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Takeshita, T.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England.
[Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan.
[Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany.
[Buat, Q.; Dawe, E.; Godfrey, J.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada.
[Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Petrolo, E.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA.
[Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia.
[Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia.
[Hamilton, A.; Vickey, T.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa.
[Aurousseau, M.; Castaneda-Miranda, E.; Connellb, S. H.; Yacoobb, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa.
[Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Garcia, B. R. Mellado; Ruan, X.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa.
[Abulaitia, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden.
[Abulaitia, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden.
[Consorti, V.; Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden.
[Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA.
[Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA.
[Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England.
[Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Savedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
[Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan.
[Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel.
[Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Astalos, R.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel.
[Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan.
[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan.
[Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan.
[Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan.
[AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada.
[Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada.
[Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada.
[Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan.
[Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA.
[Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia.
[Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA.
[Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy.
[Acharya, B. S.; Alhroob, M.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy.
[Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy.
[Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA.
[Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden.
[Bernabeu, J.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Argos, C. Garcia; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Miano; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain.
[Bernabeu, J.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Argos, C. Garcia; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Miano; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Aom Mol & Nucl, Valencia, Spain.
[Bernabeu, J.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Argos, C. Garcia; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Miano; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain.
[Bernabeu, J.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Argos, C. Garcia; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Miano; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain.
[Bernabeu, J.; Urban, S. Cabrera; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Argos, C. Garcia; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; March, L.; Marti-Garcia, S.; Moya, M. Miano; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain.
[Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada.
[Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hill, E.; Jeske, C.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada.
[Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England.
[Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan.
[Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel.
[Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA.
[Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany.
[Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany.
[Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA.
[Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France.
[Acharya, B. S.] Kings Coll London, Dept Phys, London, England.
[Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan.
[Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA.
[Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy.
[Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia.
[Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece.
[Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain.
[Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan.
[Korol, A. A.; Maximov, D. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia.
[Conventi, F.; Della Pietra, M.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China.
[Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan.
[Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India.
[Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia.
[Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary.
[Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy.
[Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA.
[Smirnov, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia.
[Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany.
[Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.
[Yacoobb, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa.
RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.
RI Grinstein, Sebastian/N-3988-2014; Li, Liang/O-1107-2015; Fullana
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Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia,
Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira,
Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin,
Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi,
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Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko,
Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev,
Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin,
Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Gutierrez,
Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan,
Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou,
Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Villa,
Mauro/C-9883-2009; Joergensen, Morten/E-6847-2015; Riu,
Imma/L-7385-2014; Bernabeu, Jose/H-6708-2015; Della Pietra,
Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci,
Fabrizio/G-8348-2012; Di Domenico, Antonio/G-6301-2011; Wemans,
Andre/A-6738-2012; Nemecek, Stanislav/G-5931-2014; Staroba,
Pavel/G-8850-2014; Lokajicek, Milos/G-7800-2014; Gabrielli,
Alessandro/H-4931-2012; Moraes, Arthur/F-6478-2010; Castro,
Nuno/D-5260-2011; Boyko, Igor/J-3659-2013; Warburton,
Andreas/N-8028-2013; Brooks, William/C-8636-2013; Lei,
Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009;
OI Gray, Heather/0000-0002-5293-4716; Mincer, Allen/0000-0002-6307-1418;
Grinstein, Sebastian/0000-0002-6460-8694; Cristinziani,
Markus/0000-0003-3893-9171; Chromek-Burckhart,
Doris/0000-0003-4243-3288; Qian, Jianming/0000-0003-4813-8167; Haas,
Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Li,
Liang/0000-0001-6411-6107; Garcia-Argos, Carlos/0000-0001-8348-4693;
Troncon, Clara/0000-0002-7997-8524; Fullana Torregrosa,
Esteban/0000-0003-3082-621X; Dell'Asta, Lidia/0000-0002-9601-4225; Chen,
Hucheng/0000-0002-9936-0115; Sawyer, Lee/0000-0001-8295-0605; Juste,
Aurelio/0000-0002-1558-3291; Begel, Michael/0000-0002-1634-4399; Vari,
Riccardo/0000-0002-2814-1337; Nisati, Aleandro/0000-0002-5080-2293;
Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia,
Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620;
Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399;
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Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz,
Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar
Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton,
Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes
Milosavljevic, Marija/0000-0003-4477-9733; Perrino,
Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495;
Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy,
Alexander/0000-0002-8902-1793; Negrini, Matteo/0000-0003-0101-6963;
Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo,
Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348;
Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov,
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Jose/0000-0002-0296-9988; Della Pietra, Massimo/0000-0003-4446-3368;
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Doyle, Anthony/0000-0001-6322-6195; Smirnov, Sergei/0000-0002-6778-073X;
Belanger-Champagne, Camille/0000-0003-2368-2617; Beck, Hans
Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401;
Veneziano, Stefano/0000-0002-2598-2659; Vazquez Schroeder,
Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Walsh,
Brian/0000-0003-1689-2309; Filthaut, Frank/0000-0003-3338-2247; Terzo,
Stefano/0000-0003-3388-3906; Pina, Joao /0000-0001-8959-5044; Hays,
Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271;
Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031;
Wang, Kuhan/0000-0002-6151-0034; Grohsjean,
Alexander/0000-0003-0748-8494; La Rosa, Alessandro/0000-0001-6291-2142
FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF,
Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil;
NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS,
China; MOST, China; NSFC, China; COL-CIENCIAS, Colombia; MSMT CR, Czech
Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark;
DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union;
ERC, European Union; NSRF, European Union; IN2P3-CNRS, France;
CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF,
Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF,
Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel;
Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST,
Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway;
MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA,
Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia;
MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa;
MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER,
Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Geneva,
Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal
Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United
States of America; NSF, United States of America
FX We thank CERN for the very successful operation of the LHC, as well as
the support staff from our institutions without whom ATLAS could not be
operated efficiently.; We acknowledge the support of ANPCyT, Argentina;
YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS,
Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI,
Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COL-CIENCIAS,
Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and
Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union;
IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and
AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF,
I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan;
CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and
NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia
and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia;
ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and
Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva,
Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and
Leverhulme Trust, United Kingdom; DOE and NSF, United States of America.
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PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1748-0221
J9 J INSTRUM
JI J. Instrum.
PD AUG
PY 2014
VL 9
AR UNSP P08009
DI 10.1088/1748-0221/9/08/P08009
PG 73
WC Instruments & Instrumentation
SC Instruments & Instrumentation
GA AP2TJ
UT WOS:000341927600037
ER
PT J
AU Chiang, A
Dreger, DS
Ford, SR
Walter, WR
AF Chiang, Andrea
Dreger, Douglas S.
Ford, Sean R.
Walter, William R.
TI Source Characterization of Underground Explosions from Combined Regional
Moment Tensor and First-Motion Analysis
SO BULLETIN OF THE SEISMOLOGICAL SOCIETY OF AMERICA
LA English
DT Article
ID JOINT VERIFICATION EXPERIMENT; NUCLEAR-EXPLOSIONS; TECTONIC RELEASE;
CRANDALL CANYON; SURFACE-WAVES; INVERSIONS; EVENT; UTAH
AB In this study, we investigate the 14 September 1988 U.S.-Soviet Joint Verification Experiment nuclear test at the Semipalatinsk test site in eastern Kazakhstan and two nuclear explosions conducted less than 10 years later at the Chinese Lop Nor test site. These events were very sparsely recorded by stations located within 1600 km, and in each case only three or four stations were available in the regional distance range. We have utilized a regional distance seismic waveform method fitting long-period, complete, three-component waveforms jointly with first-motion observations from regional stations and teleseismic arrays. The combination of long-period waveforms and first-motion observations provides a unique discrimination of these sparsely recorded events in the context of the Hudson et al. (1989) source-type diagram. We demonstrate through a series of jackknife tests and sensitivity analyses that the source type of the explosions is well constrained. One event, a 1996 Lop Nor shaft explosion, displays large Love waves and possibly reversed Rayleigh waves at one station, indicative of a large F-factor. We show the combination of long-period waveforms and P-wave first motions are able to discriminate this event as explosion-like and distinct from earthquakes and collapses. We further demonstrate the behavior of network sensitivity solutions for models of tectonic release and spall-based tensile damage over a range of F-factors and K-factors.
C1 [Chiang, Andrea; Dreger, Douglas S.] Berkeley Seismol Lab, Berkeley, CA 94720 USA.
[Ford, Sean R.; Walter, William R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Chiang, A (reprint author), Berkeley Seismol Lab, 215 McCone Hall, Berkeley, CA 94720 USA.
EM achiang@seismo.berkeley.edu
RI Walter, William/C-2351-2013; Chiang, Andrea/I-9577-2016; Ford,
Sean/F-9191-2011
OI Walter, William/0000-0002-0331-0616; Chiang, Andrea/0000-0001-8513-4363;
Ford, Sean/0000-0002-0376-5792
FU Air Force Research Laboratory [FA9453-10-C-0263]
FX The authors thank the two anonymous reviewers and associate editor for
their comments. We acknowledge funding from the Air Force Research
Laboratory, Contract Number FA9453-10-C-0263, which supports this
research. We thank Seung Hoon Yoo for his 1D Earth model inversion code
and the parallelization of the Network Sensitivity Solutions.
NR 29
TC 4
Z9 4
U1 2
U2 8
PU SEISMOLOGICAL SOC AMER
PI ALBANY
PA 400 EVELYN AVE, SUITE 201, ALBANY, CA 94706-1375 USA
SN 0037-1106
EI 1943-3573
J9 B SEISMOL SOC AM
JI Bull. Seismol. Soc. Amer.
PD AUG
PY 2014
VL 104
IS 4
BP 1587
EP 1600
DI 10.1785/0120130228
PG 14
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA AR0CQ
UT WOS:000343233600001
ER
PT J
AU Patton, HJ
Pabian, FV
AF Patton, Howard J.
Pabian, Frank V.
TI Comment on "Advanced Seismic Analyses of the Source Characteristics of
the 2006 and 2009 North Korean Nuclear Tests" by J. R. Murphy, J. L.
Stevens, B. C. Kohl, and T. J. Bennett
SO BULLETIN OF THE SEISMOLOGICAL SOCIETY OF AMERICA
LA English
DT Editorial Material
ID HIGH-PRECISION LOCATION; TEST-SITE; EXPLOSIONS; YIELD
C1 [Patton, Howard J.; Pabian, Frank V.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Patton, HJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
NR 35
TC 3
Z9 3
U1 0
U2 5
PU SEISMOLOGICAL SOC AMER
PI ALBANY
PA 400 EVELYN AVE, SUITE 201, ALBANY, CA 94706-1375 USA
SN 0037-1106
EI 1943-3573
J9 B SEISMOL SOC AM
JI Bull. Seismol. Soc. Amer.
PD AUG
PY 2014
VL 104
IS 4
BP 2104
EP 2110
DI 10.1785/0120130262
PG 7
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA AR0CQ
UT WOS:000343233600039
ER
PT J
AU Nichols, GP
Cragle, DL
Benitez, JG
AF Nichols, Gregory P.
Cragle, Donna L.
Benitez, John G.
TI Medical Screening After a Coal Fly Ash Spill in Roane County, Tennessee
SO DISASTER MEDICINE AND PUBLIC HEALTH PREPAREDNESS
LA English
DT Article
DE coal fly ash; disaster management; medical screening; medical
toxicology; Kingston Fossil Plant
ID AMERICAN; INFECTION; PULMONARY
AB Objective: To assess the health of community residents following a coal fly ash spill at the Tennessee Valley Authority Kingston Fossil Plant in Harriman, Tennessee, on December 22, 2008.
Methods: A uniform health assessment was developed by epidemiologists at Oak Ridge Associated Universities and medical toxicologists at Vanderbilt University Medical Center. Residents who believed that their health may have been affected by the coal fly ash spill were invited to participate in the medical screening program.
Results: Among the 214 individuals who participated in the screening program, the most commonly reported symptoms were related to upper airway irritation. No evidence of heavy metal toxicity was found.
Conclusions: This is the first report, to our knowledge, regarding the comprehensive health evaluation of a community after a coal fly ash spill. Because this evaluation was voluntary, the majority of residents screened represented those with a high percentage of symptoms and concerns about the potential for toxic exposure. Based on known toxicity of the constituents present in the coal fly ash, health complaints did not appear to be related to the fly ash. This screening model could be used to assess immediate or baseline toxicity concerns after other disasters.
C1 [Nichols, Gregory P.; Cragle, Donna L.] Oak Ridge Associated Univ, Occupat Exposure & Worker Hlth Programs, Oak Ridge, TN USA.
[Benitez, John G.] Vanderbilt Univ, Med Ctr, Tennessee Poison Ctr, Nashville, TN USA.
RP Nichols, GP (reprint author), ORAU Occupat Exposure & Worker Hlth Programs, POB 117 MS 23, Oak Ridge, TN 37831 USA.
EM Gregory.Nichols@orau.org
OI Benitez, John/0000-0002-2047-6204
FU Tennessee Valley Authority (TVA)
FX Funding for this medical screening was provided by the Tennessee Valley
Authority (TVA).
NR 27
TC 0
Z9 0
U1 0
U2 4
PU CAMBRIDGE UNIV PRESS
PI NEW YORK
PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA
SN 1935-7893
EI 1938-744X
J9 DISASTER MED PUBLIC
JI Dis. Med. Public Health Prep.
PD AUG
PY 2014
VL 8
IS 4
BP 341
EP 348
DI 10.1017/dmp.2014.60
PG 8
WC Public, Environmental & Occupational Health
SC Public, Environmental & Occupational Health
GA AQ9UM
UT WOS:000343202100012
PM 25058814
ER
PT J
AU Zelinski, ME
Henderson, J
Smith, M
AF Zelinski, Michael E.
Henderson, John
Smith, Milton
TI Use of Landsat 5 for Change Detection at 1998 Indian and Pakistani
Nuclear Test Sites
SO IEEE JOURNAL OF SELECTED TOPICS IN APPLIED EARTH OBSERVATIONS AND REMOTE
SENSING
LA English
DT Article
DE Comprehensive Nuclear Test-Ban Treaty (CTBT); covariance matrix Landsat
5; Mahalanobis distance; multispectral change detection
AB An underground nuclear explosion (UNE) can generate a shock wave that lofts surface material, resulting in surface changes that might be detectable. The Comprehensive Nuclear Test-Ban Treaty (CTBT) allows ground and airborne spectral and thermal imaging to help locate such events. Landsat 5 data on the 1998 Indian and Pakistani tests are used here to demonstrate that there are detectable changes in surface features which might be used to localize an underground nuclear test and to develop change detection techniques specific to the use of satellite data to support a CTBT on-site inspection. Landsat 5 has been active for over 20 years providing repeat coverage of the Earth's surface every 16 days. Most locations have Landsat data available for a variety of dates, allowing for statistical analysis of the data to understand temporal trends and data variability on a pixel-by-pixel basis. Given the right conditions, these usual patterns of change (such as seasonal changes or weathering) can be discerned from unusual patterns of change, such as features relating to a UNE. This paper extends known change detection techniques to a temporal series of data and shows that multispectral change detection can be used to help localize a UNE.
C1 [Zelinski, Michael E.; Smith, Milton] Lawrence Livermore Natl Lab, Pass Remote Sensing Grp, Livermore, CA 94550 USA.
[Henderson, John] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Zelinski, ME (reprint author), Lawrence Livermore Natl Lab, Pass Remote Sensing Grp, Livermore, CA 94550 USA.
EM zelinski1@llnl.gov
NR 20
TC 1
Z9 1
U1 2
U2 4
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1939-1404
EI 2151-1535
J9 IEEE J-STARS
JI IEEE J. Sel. Top. Appl. Earth Observ. Remote Sens.
PD AUG
PY 2014
VL 7
IS 8
BP 3453
EP 3460
DI 10.1109/JSTARS.2013.2294322
PG 8
WC Engineering, Electrical & Electronic; Geography, Physical; Remote
Sensing; Imaging Science & Photographic Technology
SC Engineering; Physical Geography; Remote Sensing; Imaging Science &
Photographic Technology
GA AQ8DZ
UT WOS:000343055200024
ER
PT J
AU Ryutov, DD
Cohen, RH
Farmer, WA
Rognlien, TD
Umansky, MV
AF Ryutov, D. D.
Cohen, R. H.
Farmer, W. A.
Rognlien, T. D.
Umansky, M. V.
TI The 'churning mode' of plasma convection in the tokamak divertor region
SO PHYSICA SCRIPTA
LA English
DT Article; Proceedings Paper
CT 4th Italian-Pakistani Workshop on Relativistic Astrophysics
CY FEB, 2013
CL Islamabad, PAKISTAN
DE tokamak; divertor; convection; turbulence
AB The churning mode can arise in a toroidally-symmetric plasma where it causes convection in the vicinity of the poloidal magnetic field null. The mode is driven by the toroidal curvature of magnetic field lines coupled with a pressure gradient. The toroidal equilibrium conditions cannot be satisfied easily in the virtual absence of the poloidal field (PF)-hence the onset of this mode, which 'churns' the plasma around the PF null without perturbing the strong toroidal field. We find the conditions under which this mode can be excited in magnetic configurations with first-, second-, and third-order PF nulls (i.e., in the geometry of standard, snowflake and cloverleaf divertors). The size of the affected zone in second- and third-order-null divertors is much larger than in a standard first-order-null divertor. The proposed phenomenological theory allows one to evaluate observable characteristics of the mode, in particular the frequency and amplitude of the PF perturbations. The mode spreads the tokamak heat exhaust between multiple divertor legs and may lead to a broadening of the plasma width in each leg. The mode causes much more intense plasma convection in the poloidal plane than the classical plasma drifts.
C1 [Ryutov, D. D.; Cohen, R. H.; Farmer, W. A.; Rognlien, T. D.; Umansky, M. V.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
RP Ryutov, DD (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
EM ryutov1@llnl.gov
FU US Department of Energy [DE-AC52-07NA27344]
FX This work was performed under the auspices of the US Department of
Energy by Lawrence Livermore National Security, LLC, Lawrence Livermore
National Laboratory, under Contract DE-AC52-07NA27344.
NR 24
TC 8
Z9 8
U1 0
U2 6
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0031-8949
EI 1402-4896
J9 PHYS SCRIPTA
JI Phys. Scr.
PD AUG
PY 2014
VL 89
IS 8
AR 088002
DI 10.1088/0031-8949/89/8/088002
PG 10
WC Physics, Multidisciplinary
SC Physics
GA AR0WT
UT WOS:000343295000041
ER
PT J
AU Muniz, RA
Kato, Y
Batista, CD
AF Muniz, Rodrigo A.
Kato, Yasuyuki
Batista, Cristian D.
TI Generalized spin-wave theory: Application to the bilinear-biquadratic
model
SO PROGRESS OF THEORETICAL AND EXPERIMENTAL PHYSICS
LA English
DT Article
ID CEB6; ANTIFERROMAGNETS; TRANSITION; SYSTEMS; PHASE
AB We present a mathematical framework for the multi-boson approach that has been used several times for treating spin systems. We demonstrate that the multi-boson approach corresponds to a generalization of the traditional spin-wave theory from SU(2) to SU(N), where N is the number of states of the local degree of freedom. Low-energy excitations are waves of the local order parameter that fluctuates in the SU(N) space of unitary transformations of the local spin states, instead of the SU(2) space of local spin rotations. Since the generators of the SU(N) group can be represented as bilinear forms in N-flavored bosons, the low-energy modes of the generalized spin-wave theory (GSWT) are described with N - 1 different bosons, which provide a more accurate description of low-energy excitations even for the usual ferromagnetic and antiferromagnetic phases. The generalization enables the treatment of quantum spin systems whose ground states exhibit multipolar ordering as well as the detection of instabilities of magnetically ordered states (dipolar ordering) towards higher multipolar orderings. We illustrate the advantages of the GSWT by applying it to a bilinear-biquadratic model of arbitrary spin S on hypercubic lattices, and then analyzing the spectrum of dipolar phases in order to find their instabilities. In contrast to the known results for S = 1when the biquadratic termin the Hamiltonian is negative, we find that there is no nematic phase between the ferromagnetic or antiferromagnetic orderings for S > 1.
C1 [Muniz, Rodrigo A.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada.
[Muniz, Rodrigo A.] Univ Toronto, Inst Opt Sci, Toronto, ON M5S 1A7, Canada.
[Muniz, Rodrigo A.] Univ Fed Rio Grande do Norte, Int Inst Phys, BR-59078400 Natal, RN, Brazil.
[Kato, Yasuyuki; Batista, Cristian D.] Los Alamos Natl Lab, Div Theoret, T4 & CNLS, Los Alamos, NM 87545 USA.
[Kato, Yasuyuki] RIKEN, CEMS, Wako, Saitama 3510198, Japan.
RP Muniz, RA (reprint author), Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada.
EM yasuyuki.kato@riken.jp
RI Batista, Cristian/J-8008-2016
FU US DOE [DE-AC52-06NA25396]; NSF [PHY-1066293]; CNPq (Brazil); JSPS
KAKENHI [26800199]
FX We thank A. V. Chubukov for stimulating discussions. Work at the LANL
was performed under the auspices of the US DOE Contract No.
DE-AC52-06NA25396 through the LDRD program. This material is based upon
work supported in part by the NSF under Grant No. PHY-1066293 and the
hospitality of the Aspen Center for Physics. R. M. also thanks CNPq
(Brazil) for financial support. Y.K. acknowledges support from JSPS
KAKENHI Grants No. 26800199.
NR 30
TC 3
Z9 3
U1 1
U2 8
PU OXFORD UNIV PRESS INC
PI CARY
PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA
SN 2050-3911
J9 PROG THEOR EXP PHYS
JI Prog. Theor. Exp. Phys.
PD AUG
PY 2014
IS 8
AR 083I01
DI 10.1093/ptep/ptu109
PG 16
WC Physics, Multidisciplinary; Physics, Particles & Fields
SC Physics
GA AQ7GJ
UT WOS:000342980300010
ER
PT J
AU Greenwood, DM
Gentle, JP
Myers, KS
Davison, PJ
West, IJ
Bush, JW
Ingram, GL
Troffaes, MCM
AF Greenwood, David M.
Gentle, Jake P.
Myers, Kurt S.
Davison, Peter J.
West, Isaac J.
Bush, Jason W.
Ingram, Grant L.
Troffaes, Matthias C. M.
TI A Comparison of Real-Time Thermal Rating Systems in the U.S. and the
U.K.
SO IEEE TRANSACTIONS ON POWER DELIVERY
LA English
DT Article
DE Fluid dynamics; power system planning; power transmission
AB Real-time thermal rating is a smart-grid technology that allows the rating of electrical conductors to be increased based on local weather conditions. Overhead lines are conventionally given a conservative, constant seasonal rating based on seasonal and regional worst case scenarios rather than actual, say, local hourly weather predictions. This paper provides a report of two pioneering schemes-one in the U.S. and one in the U.K.-where real-time thermal ratings have been applied. Thereby, we demonstrate that observing the local weather conditions in real time leads to additional capacity and safer operation. Second, we critically compare both approaches and discuss their limitations. In doing so, we arrive at novel insights which will inform and improve future real-time thermal rating projects.
C1 [Greenwood, David M.; Davison, Peter J.] Newcastle Univ, Sch Elect & Elect Engn, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England.
[Gentle, Jake P.; Myers, Kurt S.; West, Isaac J.; Bush, Jason W.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Ingram, Grant L.] Univ Durham, Sch Engn & Comp Sci, Durham DH1 3LE, England.
[Troffaes, Matthias C. M.] Univ Durham, Dept Math Sci, Durham DH1 3LE, England.
RP Greenwood, DM (reprint author), Newcastle Univ, Sch Elect & Elect Engn, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England.
EM d.m.greenwood2@ncl.ac.uk; Jake.Gentle@inl.gov; g.l.ingram@durham.ac.uk;
Matthias.troffaes@dur.ac.uk
OI Troffaes, Matthias/0000-0002-1294-600X
FU U.S. Department of Energy Wind Power Technology Office; Idaho National
Laboratory; Durham Energy Institute; EPSRC [EP/J501323/1]
FX This work was supported in part by the U.S. Department of Energy Wind
Power Technology Office under contract with Idaho National Laboratory,
in part by the Durham Energy Institute, and in part by EPSRC under Grant
EP/J501323/1. Paper no. TPWRD-00609-2013.
NR 23
TC 16
Z9 16
U1 1
U2 6
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-8977
EI 1937-4208
J9 IEEE T POWER DELIVER
JI IEEE Trans. Power Deliv.
PD AUG
PY 2014
VL 29
IS 4
BP 1849
EP 1858
DI 10.1109/TPWRD.2014.2299068
PG 10
WC Engineering, Electrical & Electronic
SC Engineering
GA AQ6JO
UT WOS:000342917700038
ER
PT J
AU Hong, L
Petridis, L
Smith, JC
AF Hong, Liang
Petridis, Loukas
Smith, Jeremy C.
TI Biomolecular Structure and Dynamics with Neutrons: The View from
Simulation
SO ISRAEL JOURNAL OF CHEMISTRY
LA English
DT Review
DE hydration; lignocellulose; molecular dynamics; neutron scattering;
proteins
ID PROTEIN VIBRATIONAL DYNAMICS; STRONGLY-DENATURED PROTEIN; METHYL-GROUP
DYNAMICS; ENZYME-ACTIVITY; SCATTERING ANALYSIS; CONFIGURATIONAL
DISTRIBUTION; TEMPERATURE-DEPENDENCE; COMPUTER-SIMULATION; GLOBULAR
PROTEIN; NORMAL-MODE
AB The characterization of the structure and internal dynamics of biomolecules is essential to understanding their biological function. Neutron scattering probes similar time- and length-scales to molecular dynamics simulation. Hence, simulation models of biomolecules have become invaluable in the interpretation of experimental neutron data. Here, we report on advances in the application of simulation in developing neutron scattering to investigate internal protein motions and, as an example of industrial relevance, in the derivation of physical models of use in biofuel renewable energy research.
C1 [Hong, Liang; Petridis, Loukas; Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA.
[Hong, Liang; Petridis, Loukas; Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Mol & Cellular Biol, Knoxville, TN USA.
RP Smith, JC (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, POB 2008, Oak Ridge, TN 37831 USA.
EM smithjc@ornl.gov
RI smith, jeremy/B-7287-2012; Petridis, Loukas/B-3457-2009; hong,
liang/D-5647-2012
OI smith, jeremy/0000-0002-2978-3227; Petridis, Loukas/0000-0001-8569-060X;
FU Genomic Science Program Office of Biological and Environmental Research
U.S. Department of Energy [FWP ERKP752]; DOE EpsCOR; ASCR (SciDAC); DFG;
National Science Foundation
FX JCS is privileged to have been able to be a part of Martin Karplus'
highly competent, dynamic and creative research group in Harvard in the
1980s. Part of this research was funded by the Genomic Science Program
Office of Biological and Environmental Research U.S. Department of
Energy FWP ERKP752, DOE EpsCOR, ASCR (SciDAC), DFG and the National
Science Foundation.
NR 58
TC 1
Z9 1
U1 4
U2 11
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0021-2148
EI 1869-5868
J9 ISR J CHEM
JI Isr. J. Chem.
PD AUG
PY 2014
VL 54
IS 8-9
SI SI
BP 1264
EP 1273
DI 10.1002/ijch.201300137
PG 10
WC Chemistry, Multidisciplinary
SC Chemistry
GA AQ4UY
UT WOS:000342796500021
ER
PT J
AU Satyal, S
Joglekar, PV
Shastry, K
Kalaskar, S
Dong, Q
Hulbert, SL
Bartynski, RA
Weiss, AH
AF Satyal, S.
Joglekar, P. V.
Shastry, K.
Kalaskar, S.
Dong, Q.
Hulbert, S. L.
Bartynski, R. A.
Weiss, A. H.
TI Measurement of the background in Auger-photoemission coincidence spectra
(APECS) associated with inelastic or multi-electron valence, band
photoemission processes
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Electron spectroscopy; Coincidence spectroscopy; Auger photoelectron;
Background elimination; Low energy tail (LET)
ID SPECTROSCOPY APECS; EMISSION; RADIATION; SOLIDS
AB Auger photoelectron coincidence spectroscopy (APECS), in which the Auger spectra are measured in coincidence with the core level photoelectron, is capable of pulling difficult to observe low energy Auger peaks out of a large background due mostly to inelastically scattered valence band (VB) photoelectrons. However the APECS method alone cannot eliminate the background due to valence band photoemission processes in which the initial photon energy is shared by two or more electrons and one of the electrons is in the energy range of the core level photoemission peak. Here we describe an experimental method to determine the contributions from these background processes and apply this method in the case of copper M3VV Auger spectrum obtained in coincidence with the 3p(3/2) photoemission peak. A beam of 200 eV photons was incident on a Cu(1 0 0) sample and a series of coincidence measurements were performed using a spectrometer equipped with two cylindrical mirror analyzers (CMAs). One CMA was set at series of fixed energies that ranged between the energy of the core and the VB peaks. The other CMA was scanned over a range corresponding to electrons leaving the surface between 0 eV and 70 eV. The set of measured spectra were then fit to a parameterized function which was extrapolated to determine the background in the APECS spectra due to multi-electron and inelastic VB photoemission processes. The extrapolated background was subtracted from the APECS spectrum to obtain the spectrum of electrons emitted solely as the result of the Auger process. A comparison of the coincidence spectrum with the same spectrum with background removed shows that in the case of Cu M3VV the background due to the inelastic scattering of VB electrons is negligible in the region of the Auger peak but is more than half the total signal down in the low energy tail of the Auger peak. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Satyal, S.; Joglekar, P. V.; Shastry, K.; Kalaskar, S.; Weiss, A. H.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA.
[Dong, Q.; Hulbert, S. L.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA.
[Bartynski, R. A.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA.
RP Weiss, AH (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA.
EM weiss@uta.edu
FU Department of Physics, University of Texas at Arlington; NSF [DMR
0907679, 1213727]; U.S. Department of Energy, Office of Science, Office
of Basic Energy Sciences [DE-AC02-98CH10886]
FX The authors would like to thank the Department of Physics, University of
Texas at Arlington for financial support and the referees of this paper
for their comments and suggestions. This research was sponsored in part
by the NSF DMR 0907679 and NSF Award Number: 1213727. Use of the
National Synchrotron Light Source, Brookhaven National Laboratory, was
supported by the U.S. Department of Energy, Office of Science, Office of
Basic Energy Sciences, under Contract No. DE-AC02-98CH10886.
NR 18
TC 1
Z9 1
U1 2
U2 8
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2014
VL 195
BP 66
EP 70
DI 10.1016/j.elspec.2014.05.010
PG 5
WC Spectroscopy
SC Spectroscopy
GA AQ5TZ
UT WOS:000342872800010
ER
PT J
AU Fero, A
Smallwood, CL
Affeldt, G
Lanzara, A
AF Fero, A.
Smallwood, C. L.
Affeldt, G.
Lanzara, A.
TI Impact of work function induced electric fields on laser-based
angle-resolved photoemission spectroscopy
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Electric fields; ARPES; Photoemission; Laser; Spectroscopy; Work
function
ID SUPERCONDUCTORS
AB We examine the effects of the electric fields caused by the difference in work function between a sample and its surroundings in laser-based angle-resolved photoemission spectroscopy (laser ARPES) experiments. To simulate these effects we created several samples and surrounding puck geometries using Simian 8.0 modeling software, and found that in most cases the system can be approximated by a circular sample mounted on an infinite conducting plane. Experimental measurements of the cuprate superconductor Bi2Sr2CaCu2O8+delta mounted on copper, aluminum, and graphite pucks confirmed the model's accuracy. Both the model and experimental data showed that work-function-induced fields have a significant effect on the outgoing trajectories of electrons for kinetic energies up to six times the work function difference between the sample and the puck. However, with the exception of effects very close to the sample edge, all electric field effects can be taken into account using linear corrections. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Fero, A.; Smallwood, C. L.; Affeldt, G.; Lanzara, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Fero, A.; Smallwood, C. L.; Affeldt, G.; Lanzara, A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
RP Fero, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM allie.fero@gmail.com
RI Smallwood, Christopher/D-4925-2011
OI Smallwood, Christopher/0000-0002-4103-8748
FU Berkeley Lab's program on Quantum Materials - U.S. Department of Energy,
Office of Science, Office of Basic Energy Sciences, Materials Sciences
and Engineering Division [DE-AC02-05CH11231]; Innovation Seed Fund in
Energy and Climate Research at the University of California
FX We thank W.T. Zhang and T.L. Miller for useful discussions, H. Eisaki
for growing the samples, and C. Jozwiak for feedback and input on the
SimIon simulation. This work was supported by Berkeley Lab's program on
Quantum Materials, funded by the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences, Materials Sciences and
Engineering Division, under Contract No. DE-AC02-05CH11231. A. F. was
partially supported by the Innovation Seed Fund in Energy and Climate
Research at the University of California (Berkeley, CA).
NR 27
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2014
VL 195
BP 237
EP 243
DI 10.1016/j.elspec.2014.01.008
PG 7
WC Spectroscopy
SC Spectroscopy
GA AQ5TZ
UT WOS:000342872800034
ER
PT J
AU Sobota, JA
Yang, SL
Leuenberger, D
Kemper, AF
Analytis, JG
Fisher, IR
Kirchmann, PS
Devereaux, TP
Shen, ZX
AF Sobota, J. A.
Yang, S. -L.
Leuenberger, D.
Kemper, A. F.
Analytis, J. G.
Fisher, I. R.
Kirchmann, P. S.
Devereaux, T. P.
Shen, Z. -X.
TI Ultrafast electron dynamics in the topological insulator Bi2Se3 studied
by time-resolved photoemission spectroscopy
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Topological insulator; Time- and angle-resolved photoemission;
Two-photon photoemission; Electron-phonon scattering
ID SINGLE DIRAC CONE; 2-PHOTON PHOTOEMISSION; SURFACE; BI2TE3; SB2TE3;
STATES
AB We characterize the topological insulator Bi2Se3 using time- and angle-resolved photoemission spectroscopy. By employing two-photon photoemission, a complete picture of the unoccupied electronic structure from the Fermi level up to the vacuum level is obtained. We demonstrate that the unoccupied states host a second Dirac surface state which can be resonantly excited by 1.5 eV photons. We then study the ultrafast relaxation processes following optical excitation. We find that they culminate in a persistent non-equilibrium population of the first Dirac surface state, which is maintained by a metastable population of the bulk conduction band. Finally, we perform a temperature-dependent study of the electron-phonon scattering processes in the conduction band, and find the unexpected result that their rates decrease with increasing sample temperature. We develop a model of phonon emission and absorption from a population of electrons, and show that this counter-intuitive trend is the natural consequence of fundamental electron-phonon scattering processes. This analysis serves as an important reminder that the decay rates extracted by time-resolved photoemission are not in general equal to single electron scattering rates, but include contributions from filling and emptying processes from a continuum of states. Published by Elsevier B.V.
C1 [Sobota, J. A.; Yang, S. -L.; Leuenberger, D.; Fisher, I. R.; Kirchmann, P. S.; Devereaux, T. P.; Shen, Z. -X.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA.
[Sobota, J. A.; Yang, S. -L.; Leuenberger, D.; Fisher, I. R.; Devereaux, T. P.; Shen, Z. -X.] Stanford Univ, Dept Appl Phys, Geballe Lab Adv Mat, Stanford, CA 94305 USA.
[Sobota, J. A.; Yang, S. -L.; Shen, Z. -X.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA.
[Kemper, A. F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Analytis, J. G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
RP Kirchmann, PS (reprint author), SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.
EM kirchman@stanford.edu; zxshen@stanford.edu
RI Kemper, Alexander/F-8243-2016; Kirchmann, Patrick/C-1195-2008;
OI Kemper, Alexander/0000-0002-5426-5181; Kirchmann,
Patrick/0000-0002-4835-0654; Yang, Shuolong/0000-0002-8200-9898
FU Department of Energy, Office of Basic Energy Sciences, Division of
Materials Science [DE-AC02-76SF00515]; Stanford Graduate Fellowship;
Alexander-von-Humboldt Foundation; M. Wolf; Laboratory Directed Research
and Development Program of Lawrence Berkeley National Laboratory under
the U.S. Department of Energy [DE-AC02-05CH11231]
FX We thank M. Sentef for valuable discussions. This work is supported by
the Department of Energy, Office of Basic Energy Sciences, Division of
Materials Science under contract DE-AC02-76SF00515. J. A. S. and S.-L.
Y. acknowledge support by the Stanford Graduate Fellowship. P. S. K.
acknowledges support by the Alexander-von-Humboldt Foundation through a
Feodor-Lynen fellowship and continuous support by M. Wolf. A. F. K. is
supported by the Laboratory Directed Research and Development Program of
Lawrence Berkeley National Laboratory under the U.S. Department of
Energy contract number DE-AC02-05CH11231.
NR 47
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U1 9
U2 45
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2014
VL 195
BP 249
EP 257
DI 10.1016/j.elspec.2014.01.005
PG 9
WC Spectroscopy
SC Spectroscopy
GA AQ5TZ
UT WOS:000342872800036
ER
PT J
AU Fadley, CS
Nemsak, S
AF Fadley, Charles S.
Nemsak, Slavomir
TI Some future perspectives in soft- and hard- X-ray photoemission
SO JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA
LA English
DT Article
DE Photoemission; X-ray photoemission; Hard X-ray photoemission;
Photoelectron diffraction; Hard X-ray photoelectron diffraction;
Photoelectron holography; Ambient pressure photoemission; Angle-resolved
photoemission; ARPES; HARPES; XPS; XPD; HXPD; HXPS; HAXPES; PH; Standing
wave photoemission; Synchrotron radiation; Spintronics
ID ANGLE-RESOLVED PHOTOEMISSION; BULK ELECTRONIC-STRUCTURE;
PHOTOELECTRON-SPECTROSCOPY; STANDING-WAVE; DIFFRACTION PATTERNS;
HOLOGRAPHIC IMAGES; ANGULAR RESOLUTION; AUGER-ELECTRON; ATOMIC IMAGES;
VALENCE BANDS
AB We discuss several recent developments in photoemission, with comments on their perspectives for the future. These include an adequate allowance for differential cross section effects in core- and valence-angular distributions, as well as more accurate one-step modeling of angle-resolved photoemission (ARPES); the use of higher photon energies from the soft- to hard- X-ray regime to permit probing bulk electronic structure and buried layers and interfaces; extending ARPES into the soft- and hard- X-ray regimes; tailoring the X-ray wave field through X-ray optical effects including standing waves, total reflection, and tuning through resonances; using standing-wave excitation to provide much enhanced depth sensitivity in studying solid/gas and solid/liquid interfaces; and applying photoelectron holography to time-resolved studies of molecular reactions and dissociation. Specific application examples include a magnetic semiconductor, multilayer structures of complex metal oxides, a thin water solution on a metal oxide surface, and a halo-substituted benzene molecule. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Fadley, Charles S.; Nemsak, Slavomir] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
[Fadley, Charles S.; Nemsak, Slavomir] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Fadley, CS (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA.
EM fadley@physics.ucdavis.edu
FU Office of Science, Office of Basic Energy Sciences, Materials Sciences
and Engineering Division, of the U.S. Department of Energy through the
Materials Sciences Division of the Lawrence Berkeley National Laboratory
(LBNL) [DE-AC02-05CH11231]; Army Research Office MURI
[W911-NF-09-1-0398]; Julich Research Center, Peter Grunberg Institute
[PGI-6]; LABEX-PALM APTCOM Project of the Triangle de Physique (Paris)
FX This work has been supported by the Director, Office of Science, Office
of Basic Energy Sciences, Materials Sciences and Engineering Division,
of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231,
through the Materials Sciences Division of the Lawrence Berkeley
National Laboratory (LBNL). Additional support has come from Army
Research Office MURI grant W911-NF-09-1-0398, in particular for the
GTO/STO study; the Julich Research Center, Peter Grunberg Institute
(PGI-6); and from the LABEX-PALM APTCOM Project of the Triangle de
Physique (Paris). We are also grateful to various co-authors and staff
scientists who have provided excellent assistance with measurements at
the Advanced Light Source, SPring-8, the Swiss Light Source, Soleil, and
Petra III.
NR 72
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U1 6
U2 57
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0368-2048
EI 1873-2526
J9 J ELECTRON SPECTROSC
JI J. Electron Spectrosc. Relat. Phenom.
PD AUG
PY 2014
VL 195
BP 409
EP 422
DI 10.1016/j.elspec.2014.06.004
PG 14
WC Spectroscopy
SC Spectroscopy
GA AQ5TZ
UT WOS:000342872800057
ER
PT J
AU Pasha, MFK
Yeasmin, D
Kao, SC
Hadjerioua, B
Wei, YX
Smith, BT
AF Pasha, M. Fayzul K.
Yeasmin, Dilruba
Kao, Shih-Chieh
Hadjerioua, Boualem
Wei, Yaxing
Smith, Brennan T.
TI Stream-Reach Identification for New Run-of-River Hydropower Development
through a Merit Matrix-Based Geospatial Algorithm
SO JOURNAL OF WATER RESOURCES PLANNING AND MANAGEMENT
LA English
DT Article
DE Hydropower resource assessment; New hydropower development; Stream-reach
selection; Flood elevation
ID OPTIMIZATION; SYSTEMS; ENERGY
AB Even after a century of development, the total hydropower potential from undeveloped rivers is still considered to be abundant in the United States. However, unlike evaluating hydropower potential at existing hydropower plants or nonpowered dams, locating a feasible new hydropower plant involves many unknowns; hence, the total undeveloped potential is harder to quantify. In light of the rapid development of multiple national geospatial data sets for topography, hydrology, and environmental characteristics, a merit matrix-based geospatial algorithm is proposed to identify possible hydropower stream reaches for future development. These hydropower stream reaches-sections of natural streams with suitable head, flow, and slope for possible future development-are identified and compared by using three different scenarios. A case study was conducted in the Alabama-Coosa-Tallapoosa and Apalachicola-Chattahoochee-Flint hydrologic subregions. It was found that a merit matrix-based algorithm, which is based on the product of hydraulic head, annual mean flow, and average channel slope, can effectively identify stream reaches with high power density and small surface inundation. These identified stream reaches can then be evaluated for their potential environmental impact, land development cost, and other competing water usage in detailed feasibility studies. Given that the selected data sets are available nationally (at least within the conterminous U. S.), the proposed methodology will have wide applicability across the country. (C) 2014 American Society of Civil Engineers.
C1 [Pasha, M. Fayzul K.] Calif State Univ Fresno, Dept Civil & Geomat Engn, Fresno, CA 93740 USA.
[Yeasmin, Dilruba; Kao, Shih-Chieh; Wei, Yaxing] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
[Hadjerioua, Boualem; Smith, Brennan T.] Oak Ridge Natl Lab, Div Environm Sci, Energy Water Ecosyst Engn Grp, Oak Ridge, TN 37831 USA.
RP Pasha, MFK (reprint author), Calif State Univ Fresno, Dept Civil & Geomat Engn, 2320 E San Ramon Ave M-S EE94, Fresno, CA 93740 USA.
EM mpasha@csufresno.edu
RI Kao, Shih-Chieh/B-9428-2012
OI Kao, Shih-Chieh/0000-0002-3207-5328
FU US Department of Energy's Office of Energy Efficiency and Renewable
Energy, Wind and Water Power Technologies Program; California State
University-Fresno; US Department of Energy [DE-AC05-00OR22725]; United
States government
FX This research was sponsored by the US Department of Energy's Office of
Energy Efficiency and Renewable Energy, Wind and Water Power
Technologies Program. Support from California State University-Fresno is
also acknowledged. This paper was co-authored by employees of Oak Ridge
National Laboratory, managed by UT Battelle, LLC, under contract
DE-AC05-00OR22725 with the US Department of Energy. Accordingly, the
publisher, by accepting the article for publication, acknowledges that
the United States government retains a nonexclusive, paid-up,
irrevocable, worldwide license to publish or reproduce the published
form of this manuscript, or allow others to do so, for United States
government purposes.
NR 29
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U2 7
PU ASCE-AMER SOC CIVIL ENGINEERS
PI RESTON
PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA
SN 0733-9496
EI 1943-5452
J9 J WATER RES PLAN MAN
JI J. Water Resour. Plan. Manage.-ASCE
PD AUG
PY 2014
VL 140
IS 8
AR 04014016
DI 10.1061/(ASCE)WR.1943-5452.0000429
PG 11
WC Engineering, Civil; Water Resources
SC Engineering; Water Resources
GA AQ5HF
UT WOS:000342837700009
ER
PT J
AU Chen, X
Heidbrink, WW
Kramer, GJ
Van Zeeland, MA
Pace, DC
Petty, CC
Fisher, RK
Nazikian, R
Zeng, L
Austin, ME
Grierson, BA
Podesta, M
AF Chen, X.
Heidbrink, W. W.
Kramer, G. J.
Van Zeeland, M. A.
Pace, D. C.
Petty, C. C.
Fisher, R. K.
Nazikian, R.
Zeng, L.
Austin, M. E.
Grierson, B. A.
Podesta, M.
TI Enhanced localized energetic ion losses resulting from first-orbit
linear and non-linear interactions with Alfven eigenmodes in DIII-D
SO PHYSICS OF PLASMAS
LA English
DT Article
ID DIGITAL BISPECTRAL ANALYSIS; D TOKAMAK; TOROIDAL PLASMAS; DRIVEN; SHEAR;
INSTABILITIES; DISCHARGES; OPERATION; PROFILE; CODE
AB Two key insights into interactions between Alfven eigenmodes (AEs) and energetic particles in the plasma core are gained from measurements and modeling of first-orbit beam-ion loss in DIII-D. First, the neutral beam-ion first-orbit losses are enhanced by AEs and a single AE can cause large fast-ion displacement. The coherent losses are from born trapped full energy beam-ions being non-resonantly scattered by AEs onto loss orbits within their first poloidal transit, The loss amplitudes scale linearly with the mode amplitude but the slope is different for different modes. The radial displacement of fast-ions by individual AEs can be directly inferred from the measurements. Second, oscillations in the beam-ion first-or-bit losses are observed at the sum, difference, and harmonic frequencies of two independent AEs. These oscillations are not plasma modes and are absent in magnetic, density', and temperature fluctuations. The origin of the non-linearity as a wave-particle coupling is confirmed through hi-coherence analysis, which is clearly observed because the coherences are preserved by the first-orbit loss mechanism. An analytic model and full orbit simulations show that the non-linear features seen in the loss signal can be explained by' a non-linear interaction between the fast ions and the two independent AEs. (C) 2014 AIP Publishing LLC.
C1 [Chen, X.; Heidbrink, W. W.] Univ Calif Irvine, Irvine, CA 92697 USA.
[Chen, X.; Van Zeeland, M. A.; Pace, D. C.; Petty, C. C.; Fisher, R. K.] Gen Atom Co, San Diego, CA 92186 USA.
[Kramer, G. J.; Nazikian, R.; Grierson, B. A.; Podesta, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Zeng, L.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA.
[Austin, M. E.] Univ Texas Austin, Austin, TX 78712 USA.
RP Chen, X (reprint author), Univ Calif Irvine, Irvine, CA 92697 USA.
FU U.S. Department of Energy [DE-FG03-94ER54271, DEACO5-060R23100,
SC-G903402, DE-FG02-99-ER54522, DE-ACO2-09CH11466, DE-FCO2-04ER54698,
DE-FG02-08ER54984, SCG903402, DE-FG03-97ER54415]
FX This work was supported by the U.S. Department of Energy under
DE-FG03-94ER54271, DEACO5-060R23100, SC-G903402, DE-FG02-99-ER54522,
DE-ACO2-09CH11466, DE-FCO2-04ER54698, DE-FG02-08ER54984, SCG903402, and
DE-FG03-97ER54415. The authors thank the DIII-D Team for their support,
especially, the physics operator Dr. T. H. Osborne and Dr. A. W. Hyatt;
and thank Dr. N. J. Commaux, Dr. J. M. Hanson, Dr. G. R. McKee, Dr. T.
Rhodes, Dr. B. J. Tobias. and Dr. Z. Yan. DIII-D data shown in this
paper can be obtained in digital format by following the links at
https://fusion.gat.com/global/D3D_DMP.
NR 47
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U1 1
U2 7
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082503
DI 10.1063/1.4891442
PG 9
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600031
ER
PT J
AU Johns, HM
Mancini, RC
Hakel, P
Nagayama, T
Smalyuk, VA
Regan, SP
Delettrez, J
AF Johns, H. M.
Mancini, R. C.
Hakel, P.
Nagayama, T.
Smalyuk, V. A.
Regan, S. P.
Delettrez, J.
TI Compressed shell conditions extracted from spectroscopic analysis of Ti
K-shell absorption spectra with evaluation of line self-emission
SO PHYSICS OF PLASMAS
LA English
DT Article
ID OMEGA LASER SYSTEM; PUSHER CONDITIONS; IMPLOSIONS; PLASMAS; MODULATIONS;
PERFORMANCE; PROFILES; PHASE
AB Ti-doped tracer layers embedded in the shell at varying distances from the fuel-shell interface serve as a spectroscopic diagnostic for direct-drive experiments conducted at OMEGA. Detailed modeling of Ti K-shell absorption spectra produced in the tracer layer considers n = 1-2 transitions in F-through Li-like Ti ions in the 4400-4800 eV range, both including and excluding line self-emission. Testing the model on synthetic spectra generated from 1-D LILAC hydrodynamic simulations reveals that the model including self-emission best reproduces the simulation, while the model excluding self-emission overestimates electron temperature T-e and density N-e to a higher degree for layers closer to the core. The prediction of the simulation that the magnitude of T-e and duration of Ti absorption will be strongly tied to the distance of the layer from the core is consistent with the idea that regions of the shell close to the core are more significantly heated by thermal transport out of the hot dense core, but more distant regions are less affected by it. The simulation predicts more time variation in the observed Te, Ne conditions in the compressed shell than is observed in the experiment, analysis of which reveals conditions remain in the range T-e = 400-600 eV and Ne = 3.0-10.0 x 10(24) cm(-3) for all but the most distant Ti-doped layer, with error bars similar to 5% T-e value and similar to 10% N-e on average. The T-e, N-e conditions of the simulation lead to a greater degree of ionization for zones close to the core than occurs experimentally, and less ionization for zones far from the core. (C) 2014 AIP Publishing LLC.
C1 [Johns, H. M.; Mancini, R. C.; Hakel, P.; Nagayama, T.] Univ Nevada, Dept Phys, Reno, NV 89557 USA.
[Smalyuk, V. A.; Regan, S. P.; Delettrez, J.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA.
RP Johns, HM (reprint author), Los Alamos Natl Lab, TA-3 Bldg 1400 Casa Grande Dr, Los Alamos, NM 87545 USA.
FU LLE [416232-G]; DOE [DE-NA0002267]
FX This work was supported by LLE contract 416232-G and DOE grant
DE-NA0002267.
NR 29
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U1 1
U2 9
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082711
DI 10.1063/1.4892554
PG 12
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600055
ER
PT J
AU Kaye, SM
Guttenfelder, W
Bell, RE
Gerhardt, SP
LeBlanc, BP
Maingi, R
AF Kaye, S. M.
Guttenfelder, W.
Bell, R. E.
Gerhardt, S. P.
LeBlanc, B. P.
Maingi, R.
TI Reduced model prediction of electron temperature profiles in
microtearing-dominated National Spherical Torus eXperiment plasmas
SO PHYSICS OF PLASMAS
LA English
DT Article
ID HEAT-TRANSPORT; CONFINEMENT; EQUILIBRIUM; TURBULENCE
AB A representative H-mode discharge from the National Spherical Torus eXperiment is studied in detail to utilize it as a basis for a time-evolving prediction of the electron temperature profile using an appropriate reduced transport model. The time evolution of characteristic plasma variables such as beta(e), nu(*)(e), the MHD alpha parameter, and the gradient scale lengths of T-e, T-i, and n(e) were examined as a prelude to performing linear gyrokinetic calculations to determine the fastest growing micro instability at various times and locations throughout the discharge. The inferences from the parameter evolutions and the linear stability calculations were consistent. Early in the discharge, when beta(e) and nu(*)(e) were relatively low, ballooning parity modes were dominant. As time progressed and both beta(e) and nu(*)(e) increased, microtearing became the dominant low-k(theta) mode, especially in the outer half of the plasma. There are instances in time and radius, however, where other modes, at higher-k(theta), may, in addition to microtearing, be important for driving electron transport. Given these results, the Rebut-Lallia-Watkins (RLW) electron thermal diffusivity model, which is based on microtearing-induced transport, was used to predict the time-evolving electron temperature across most of the profile. The results indicate that RLW does a good job of predicting Te for times and locations where microtearing was determined to be important, but not as well when microtearing was predicted to be stable or subdominant. (C) 2014 AIP Publishing LLC.
C1 [Kaye, S. M.; Guttenfelder, W.; Bell, R. E.; Gerhardt, S. P.; LeBlanc, B. P.; Maingi, R.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
RP Kaye, SM (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM skaye@pppl.gov
FU U.S. Department of Energy [DE-AC02-09CH11466]
FX This work has been supported by U.S. Department of Energy Contract
DE-AC02-09CH11466.
NR 35
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PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082510
DI 10.1063/1.4893135
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600038
ER
PT J
AU Mikkelsen, DR
Tanaka, K
Nunami, M
Watanabe, TH
Sugama, H
Yoshinuma, M
Ida, K
Suzuki, Y
Goto, M
Morita, S
Wieland, B
Yamada, I
Yasuhara, R
Tokuzawa, T
Akiyama, T
Pablant, NA
AF Mikkelsen, D. R.
Tanaka, K.
Nunami, M.
Watanabe, T. -H.
Sugama, H.
Yoshinuma, M.
Ida, K.
Suzuki, Y.
Goto, M.
Morita, S.
Wieland, B.
Yamada, I.
Yasuhara, R.
Tokuzawa, T.
Akiyama, T.
Pablant, N. A.
TI Quasilinear carbon transport in an impurity hole plasma in LHD
SO PHYSICS OF PLASMAS
LA English
DT Article
ID LARGE HELICAL DEVICE; ELECTRON HEAT-TRANSPORT; TOKAMAK; TURBULENCE;
SPECTROSCOPY; SIMULATIONS
AB Comprehensive electrostatic gyrokinetic linear stability calculations for ion-scale microinstabilities in an LHD plasma with an ion-internal transport barrier (ITB) and carbon "impurity hole" are used to make quasilinear estimates of particle flux to explore whether microturbulence can explain the observed outward carbon fluxes that flow "up" the impurity density gradient. The ion temperature is not stationary in the ion-ITB phase of the simulated discharge, during which the core carbon density decreases continuously. To fully sample these varying conditions, the calculations are carried out at three radial locations and four times. The plasma parameter inputs are based on experimentally measured profiles of electron and ion temperature, as well as electron and carbon density. The spectroscopic line-average ratio of hydrogen and helium densities is used to set the density of these species. Three ion species (H, He, C) and the electrons are treated kinetically, including collisions. Electron instability drive does enhance the growth rate significantly, but the most unstable modes have characteristics of ion temperature gradient modes in all cases. As the carbon density gradient is scanned between the measured value and zero, the quasilinear carbon flux is invariably inward when the carbon density profile is hollow, so turbulent transport due to the instabilities considered here does not explain the observed outward flux of impurities in impurity hole plasmas. The stiffness of the quasilinear ion heat flux is found to be 1.7-2.3, which is lower than several estimates in tokamaks. (C) 2014 AIP Publishing LLC.
C1 [Mikkelsen, D. R.; Pablant, N. A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Tanaka, K.; Nunami, M.; Sugama, H.; Yoshinuma, M.; Ida, K.; Suzuki, Y.; Goto, M.; Morita, S.; Wieland, B.; Yamada, I.; Yasuhara, R.; Tokuzawa, T.; Akiyama, T.] Natl Inst Fus Sci, Toki, Gifu 5095292, Japan.
[Watanabe, T. -H.] Nagoya Univ, Dept Phys, Chikusa Ku, Nagoya, Aichi 4648602, Japan.
RP Mikkelsen, DR (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.
EM dmikkelsen@pppl.gov
RI Ida, Katsumi/E-4731-2016;
OI Ida, Katsumi/0000-0002-0585-4561; Hideo, Sugama/0000-0001-5444-1758
FU U.S. Department of Energy [DE-AC02-76CH03073]; Office of Science of the
U.S. Department of Energy [DE-AC02-05CH11231]
FX We thank M. Yokoyama for TASK3D analysis, and C. D. Beidler, G. W.
Hammett, and P. Xanthopoulos for helpful discussions. This work has been
done under the collaboration research of National Institute for Fusion
Science. It is a pleasure to acknowledge cooperation and discussions
with Professor K. Komori, Professor O. Kaneko, and Professor H. Yamada
of National Institute for Fusion Science. This work was supported by
U.S. Department of Energy Contract No DE-AC02-76CH03073. This research
used resources of the National Energy Research Scientific Computing
Center (NERSC), which is supported by the Office of Science of the U.S.
Department of Energy under Contract No. DE-AC02-05CH11231. Use of
parallel computer clusters at PPPL is also gratefully acknowledged.
NR 55
TC 9
Z9 9
U1 0
U2 5
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082302
DI 10.1063/1.4890973
PG 14
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600023
ER
PT J
AU Shahzad, M
Tallents, GJ
Steel, AB
Hobbs, L
Hoarty, DJ
Dunn, J
AF Shahzad, M.
Tallents, G. J.
Steel, A. B.
Hobbs, L.
Hoarty, D. J.
Dunn, J.
TI Electron temperature and density characterization using L-shell
spectroscopy of laser irradiated buried iron layer targets
SO PHYSICS OF PLASMAS
LA English
DT Article
ID PLASMA; PULSES; HOT; SPECTRA
AB Uniform high density plasmas of different materials with properties relevant to the interior of stars and to inertial fusion can be created by laser irradiation of targets containing a buried layer of the material. Buried layer targets also enable the diagnosis of hot and thermal electron, x-ray and ion heating of targets. In this paper, L-emission spectroscopy from an iron layer (thickness 77 nm) encased in an otherwise plastic target (of thickness 240 nm-1.36 mu m on the laser side) is irradiated by 0.53 mu m wavelength, 2 ps duration laser pulses at irradiances of 10(17)-10(18) Wcm(-2). The relative iron L-emission from Li-like Fe XXIV to Ne-like Fe XVII is used to diagnose the plasma conditions of temperature and density in the iron layer. As the upper quantum states of the L-emission lines are in local thermodynamic equilibrium, line intensity ratios depend on both electron temperature and density, which-we show-enables the simultaneous measurement of both electron temperature and density by considering several line intensity ratios. We also show that hot electron target heating and the value of thermal flux limited heat conduction can be evaluated from the relative intensity of iron lines. (C) 2014 AIP Publishing LLC.
C1 [Shahzad, M.; Tallents, G. J.] Univ York, York Plasma Inst, York YO10 5DQ, N Yorkshire, England.
[Steel, A. B.; Dunn, J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Hobbs, L.; Hoarty, D. J.] Atom Weap Estab, Reading RG7 4PR, Berks, England.
RP Shahzad, M (reprint author), Univ York, York Plasma Inst, York YO10 5DQ, N Yorkshire, England.
FU UK Atomic Weapons Establishment; Engineering and Physical Sciences
Research Council
FX We would like to acknowledge the staff at LLNL, especially Jim Hunter
and Jim Moody. Additionally, we acknowledge Dr. J. Pasley and Professor
N. C. Woolsey for access to HYADES Cascade Applied Sciences Inc. and
PRISM Computational Sciences Inc codes. Author M. Shahzad acknowledges
funding from the UK Atomic Weapons Establishment and Engineering and
Physical Sciences Research Council.
NR 21
TC 2
Z9 2
U1 0
U2 5
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082702
DI 10.1063/1.4892263
PG 5
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600047
ER
PT J
AU Yu, EP
Velikovich, AL
Maron, Y
AF Yu, Edmund P.
Velikovich, A. L.
Maron, Y.
TI Application of one-dimensional stagnation solutions to three-dimensional
simulation of compact wire array in absence of radiation
SO PHYSICS OF PLASMAS
LA English
DT Article
ID Z-PINCH IMPLOSIONS; SELF-SIMILAR OSCILLATIONS; K-SHELL RADIATION;
DENSITY Z-PINCHES; X-RAY-EMISSION; ENERGY DEPOSITION; ATOMIC-NUMBER;
PLASMA; PHYSICS; GENERATION
AB We investigate the stagnation phase of a three-dimensional (3D), magnetohydrodynamic simulation of a compact, tungsten wire-array Z pinch, under the simplifying assumption of negligible radiative loss. In particular, we address the ability of one-dimensional (1D) analytic theory to describe the time evolution of spatially averaged plasma properties from 3D simulation. The complex fluid flows exhibited in the stagnated plasma are beyond the scope of 1D theory and result in centrifugal force as well as enhanced thermal transport. Despite these complications, a 1D homogeneous (i.e., shockless) stagnation solution can capture the increase of on-axis density and pressure during the initial formation of stagnated plasma. Later, when the stagnated plasma expands outward into the imploding plasma, a 1D shock solution describes the decrease of on-axis density and pressure, as well as the growth of the shock accretion region. (C) 2014 AIP Publishing LLC.
C1 [Yu, Edmund P.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Velikovich, A. L.] Naval Res Lab, Div Plasma Phys, Washington, DC 20375 USA.
[Maron, Y.] Weizmann Inst Sci, IL-76100 Rehovot, Israel.
RP Yu, EP (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM epyu@sandia.gov
NR 77
TC 2
Z9 2
U1 1
U2 5
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD AUG
PY 2014
VL 21
IS 8
AR 082703
DI 10.1063/1.4891844
PG 22
WC Physics, Fluids & Plasmas
SC Physics
GA AQ4IZ
UT WOS:000342760600048
ER
PT J
AU Bionta, MR
Hartmann, N
Weaver, M
French, D
Nicholson, DJ
Cryan, JP
Glownia, JM
Baker, K
Bostedt, C
Chollet, M
Ding, Y
Fritz, DM
Fry, AR
Kane, DJ
Krzywinski, J
Lemke, HT
Messerschmidt, M
Schorb, S
Zhu, D
White, WE
Coffee, RN
AF Bionta, M. R.
Hartmann, N.
Weaver, M.
French, D.
Nicholson, D. J.
Cryan, J. P.
Glownia, J. M.
Baker, K.
Bostedt, C.
Chollet, M.
Ding, Y.
Fritz, D. M.
Fry, A. R.
Kane, D. J.
Krzywinski, J.
Lemke, H. T.
Messerschmidt, M.
Schorb, S.
Zhu, D.
White, W. E.
Coffee, R. N.
TI Spectral encoding method for measuring the relative arrival time between
x-ray/optical pulses
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID FREE-ELECTRON LASER; RAY
AB The advent of few femtosecond x-ray light sources brings promise of x-ray/optical pump-probe experiments that can measure chemical and structural changes in the 10-100 fs time regime. Widely distributed timing systems used at x-ray Free-Electron Laser facilities are typically limited to above 50 fs fwhm jitter in active x-ray/optical synchronization. The approach of single-shot timing measurements is used to sort results in the event processing stage. This has seen wide use to accommodate the insufficient precision of active stabilization schemes. In this article, we review the current technique for "measure-and-sort" at the Linac Coherent Light Source at the SLAC National Accelerator Laboratory. The relative arrival time between an x-ray pulse and an optical pulse is measured near the experimental interaction region as a spectrally encoded cross-correlation signal. The cross-correlation provides a time-stamp for filter-and-sort algorithms used for real-time sorting. Sub-10 fs rms resolution is common in this technique, placing timing precision at the same scale as the duration of the shortest achievable x-ray pulses. (C) 2014 AIP Publishing LLC.
C1 [Bionta, M. R.] Univ Toulouse, UPS, Lab Collis Agregats Reactivite, IRSAMC, F-31062 Toulouse, France.
[Bionta, M. R.] CNRS, UMR 5589, F-31062 Toulouse, France.
[Bionta, M. R.; Hartmann, N.; Weaver, M.; French, D.; Nicholson, D. J.; Cryan, J. P.; Glownia, J. M.; Bostedt, C.; Chollet, M.; Ding, Y.; Fritz, D. M.; Fry, A. R.; Krzywinski, J.; Lemke, H. T.; Messerschmidt, M.; Schorb, S.; Zhu, D.; White, W. E.; Coffee, R. N.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
[Hartmann, N.] Univ Bern, Inst Appl Phys, CH-3012 Bern, Switzerland.
[Nicholson, D. J.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA.
[Cryan, J. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Baker, K.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
[Kane, D. J.] Mesa Photon LLC, Santa Fe, NM 87505 USA.
[Coffee, R. N.] SLAC Natl Accelerator Lab, PULSE Inst Ultrafast Energy Sci, Menlo Pk, CA 94025 USA.
RP Bionta, MR (reprint author), Univ Toulouse, UPS, Lab Collis Agregats Reactivite, IRSAMC, F-31062 Toulouse, France.
EM mina.bionta@irsamc.ups-tlse.fr; coffee@slac.stanford.edu
RI Messerschmidt, Marc/F-3796-2010; Lemke, Henrik Till/N-7419-2016
OI Messerschmidt, Marc/0000-0002-8641-3302; Lemke, Henrik
Till/0000-0003-1577-8643
FU U.S. Department of Energy Office of Science
FX This research was carried out at the Linac Coherent Light Source (LCLS)
at the SLAC National Accelerator Laboratory. LCLS is an Office of
Science User Facility funded under the auspices of the U.S. Department
of Energy Office of Science operated by Stanford University.
NR 35
TC 15
Z9 15
U1 1
U2 14
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083116
DI 10.1063/1.4893657
PG 10
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500017
PM 25173255
ER
PT J
AU Covo, MK
AF Covo, Michel Kireeff
TI Measurement of axial injection displacement with trim coil current
unbalance
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
AB The Dee probe used for measuring internal radial beam intensity shows large losses inside the radius of 20 cm of the 88 in. cyclotron. The current of the top and bottom innermost trim coil 1 is unbalanced to study effects of the axial injection displacement. A beam profile monitor images the ion beam bunches, turn by turn. The experimental bunch center of mass position is compared with calculations of the magnetic mirror effect displacement and shows good agreement. (C) 2014 AIP Publishing LLC.
C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Covo, MK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM mkireeffcovo@lbl.gov
FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics
[DE-AC02-05CH11231]
FX The author would like to thank Damon Todd and Markus Strohmeier for
fruitful comments. This material is based upon work supported by the
U.S. Department of Energy, Office of Science, Office of Nuclear Physics
under Award Number DE-AC02-05CH11231.
NR 5
TC 0
Z9 0
U1 1
U2 2
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 085113
DI 10.1063/1.4892463
PG 3
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500080
ER
PT J
AU Danly, CR
Merrill, FE
Barlow, D
Mariam, FG
AF Danly, C. R.
Merrill, F. E.
Barlow, D.
Mariam, F. G.
TI Nonuniform radiation damage in permanent magnet quadrupoles
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID RADIOGRAPHY
AB We present data that indicate nonuniform magnetization loss due to radiation damage in neodymiumiron- boron Halbach-style permanent magnet quadrupoles. The proton radiography (pRad) facility at Los Alamos uses permanent-magnet quadrupoles for magnifying lenses, and a system recently commissioned at GSI-Darmsdadt uses permanent magnets for its primary lenses. Large fluences of spallation neutrons can be produced in close proximity to these magnets when the proton beam is, intentionally or unintentionally, directed into the tungsten beam collimators; imaging experiments at LANL's pRad have shown image degradation with these magnetic lenses at proton beam doses lower than those expected to cause damage through radiation-induced reduction of the quadrupole strength alone. We have observed preferential degradation in portions of the permanent magnet quadrupole where the field intensity is highest, resulting in increased high-order multipole components. (C) 2014 AIP Publishing LLC.
C1 [Danly, C. R.; Merrill, F. E.; Barlow, D.; Mariam, F. G.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
RP Danly, CR (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA.
OI Merrill, Frank/0000-0003-0603-735X
NR 13
TC 5
Z9 5
U1 0
U2 3
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083305
DI 10.1063/1.4892803
PG 5
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500022
PM 25173260
ER
PT J
AU Frantti, J
Fujioka, Y
Zhang, J
Zhu, J
Vogel, SC
Zhao, Y
AF Frantti, J.
Fujioka, Y.
Zhang, J.
Zhu, J.
Vogel, S. C.
Zhao, Y.
TI Microstrain in tetragonal lead-zirconate-titanate: The effect of
pressure on the ionic displacements
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID NEUTRON-DIFFRACTION; PBTIO3; PHASE; PEROVSKITES; DIFFRACTOMETER;
CERAMICS; EQUATION; HIPPO; STATE; GPA
AB Piezoelectric materials respond to external stimuli by adjusting atomic positions. In solid-solutions, the changes occurring in atomic scale are very complex since the short-and long-range order are different. Standard methods used in diffraction data analysis fail to model the short-range order accurately. Pressure-induced cation displacements in ferroelectric Pb(Zr0.45Ti0.55)O-3 perovskite oxide are modeled by starting from a short-range order. We show that the model gives the average structure correctly and properly describes the local structure. The origin of the microstrain in lead zirconate titanate is the spatially varying Zr and Ti concentration and atomic distances, which is taken into account in the simulation. High-pressure neutron powder diffraction and simulation techniques are applied for the determination of atomic positions and bond-valences as a function of pressure. Under hydrostatic pressure, the material loses its piezoelectric properties far before the transition to the cubic phase takes place. The total cation valence +6 is preserved up to 3.31 GPa by compensating the increasing B-cation valence by decreasing Pb-displacement from the high-symmetry position. At 3.31 GPa, Pb-displacement is zero and the material is no more ferroelectric. This is also the pressure at which the Pb-valence is minimized. The average structure is still tetragonal. The model for microstrain predicts that the transition occurs over a finite pressure range: Pb-displacements are spatially varying and follow the distribution of Zr and Ti ions. (C) 2014 AIP Publishing LLC.
C1 [Frantti, J.; Fujioka, Y.] Finnish Res & Engn, Helsinki 00180, Finland.
[Zhang, J.; Zhu, J.; Vogel, S. C.; Zhao, Y.] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA.
RP Frantti, J (reprint author), Finnish Res & Engn, Jaalaranta 9 B 42, Helsinki 00180, Finland.
EM Johannes.Frantti@fre.fi
OI Zhang, Jianzhong/0000-0001-5508-1782; Vogel, Sven C./0000-0003-2049-0361
NR 33
TC 3
Z9 3
U1 3
U2 13
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083901
DI 10.1063/1.4891458
PG 7
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500040
PM 25173278
ER
PT J
AU Grapes, MD
LaGrange, T
Friedman, LH
Reed, BW
Campbell, GH
Weihs, TP
LaVan, DA
AF Grapes, Michael D.
LaGrange, Thomas
Friedman, Lawrence H.
Reed, Bryan W.
Campbell, Geoffrey H.
Weihs, Timothy P.
LaVan, David A.
TI Combining nanocalorimetry and dynamic transmission electron microscopy
for in situ characterization of materials processes under rapid heating
and cooling
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID THIN-FILMS; ULTRATHIN FILMS; ALLOY; PURE; DTEM
AB Nanocalorimetry is a chip-based thermal analysis technique capable of analyzing endothermic and exothermic reactions at very high heating and cooling rates. Here, we couple a nanocalorimeter with an extremely fast in situ microstructural characterization tool to identify the physical origin of rapid enthalpic signals. More specifically, we describe the development of a system to enable in situ nanocalorimetry experiments in the dynamic transmission electron microscope (DTEM), a time-resolved TEM capable of generating images and electron diffraction patterns with exposure times of 30 ns-500 ns. The full experimental system consists of a modified nanocalorimeter sensor, a custom-built in situ nanocalorimetry holder, a data acquisition system, and the DTEM itself, and is capable of thermodynamic and microstructural characterization of reactions over a range of heating rates (102 K/s-105 K/s) accessible by conventional (DC) nanocalorimetry. To establish its ability to capture synchronized calorimetric and microstructural data during rapid transformations, this work describes measurements on the melting of an aluminum thin film. We were able to identify the phase transformation in both the nanocalorimetry traces and in electron diffraction patterns taken by the DTEM. Potential applications for the newly developed system are described and future system improvements are discussed. (C) 2014 AIP Publishing LLC.
C1 [Grapes, Michael D.; Weihs, Timothy P.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA.
[Grapes, Michael D.; Friedman, Lawrence H.; LaVan, David A.] NIST, Mat Measurement Sci Div, Mat Measurement Lab, Gaithersburg, MD 20899 USA.
[LaGrange, Thomas; Reed, Bryan W.; Campbell, Geoffrey H.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA.
RP Grapes, MD (reprint author), Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA.
EM mgrapes1@jhu.edu; weihs@jhu.edu; david.lavan@nist.gov
RI Weihs, Timothy/A-3313-2010; Friedman, Lawrence/G-5650-2011
OI Friedman, Lawrence/0000-0003-2416-9903
FU National Institute of Standards and Technology (NIST) [70NANB9H9146];
National Science Foundation (NSF) [DMR-1308966]; (U.S.) Department of
Energy (DOE) by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; U.S. Department of Energy, Office of Basic Energy
Sciences, Division of Materials Science and Engineering [FWP SCW0974]
FX The authors are grateful to Chris Amigo for design guidance and
machining of the holder and to Bernadette Cannon for her help
calibrating nanocalorimeter sensors during her time as a NIST Summer
Undergraduate Research Fellowship (SURF) student. M. D. G. and T. P. W.
were supported in part by National Institute of Standards and Technology
(NIST) Grant No. 70NANB9H9146 and in part by National Science Foundation
(NSF) Grant No. DMR-1308966. Nanocalorimeter fabrication was performed
at the NIST Center for Nanoscale Science and Technology. The work
presented in this article conducted at the LLNL DTEM facility was
performed under the auspices of the (U.S.) Department of Energy (DOE) by
Lawrence Livermore National Laboratory under Contract No.
DE-AC52-07NA27344. The DTEM experiments conducted at LLNL and effort of
T. L., B. W. R., and G. H. C. were supported by the U.S. Department of
Energy, Office of Basic Energy Sciences, Division of Materials Science
and Engineering under FWP SCW0974. Certain commercial equipment,
instruments, or materials are identified in this document. Such
identification does not imply recommendation or endorsement by the
National Institute of Standards and Technology, nor does it imply that
the products identified are necessarily the best available for the
purpose. Since the completion of this work, T. L. and B. W. R. have
become employees at Integrated Dynamic Electron Solutions, Inc., a
startup company marketing time-resolved electron microscope technology.
NR 34
TC 3
Z9 3
U1 8
U2 37
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 084902
DI 10.1063/1.4892537
PG 12
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500060
PM 25173298
ER
PT J
AU Haboub, A
Bale, HA
Nasiatka, JR
Cox, BN
Marshall, DB
Ritchie, RO
MacDowell, AA
AF Haboub, Abdel
Bale, Hrishikesh A.
Nasiatka, James R.
Cox, Brian N.
Marshall, David B.
Ritchie, Robert O.
MacDowell, Alastair A.
TI Tensile testing of materials at high temperatures above 1700 degrees C
with in situ synchrotron X-ray micro-tomography
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID CERAMIC-MATRIX COMPOSITES; COMPUTED-TOMOGRAPHY; K FURNACE;
MICROTOMOGRAPHY; DAMAGE
AB A compact ultrahigh temperature tensile testing instrument has been designed and fabricated for in situ x-ray micro-tomography using synchrotron radiation at the Advanced Light Source, Lawrence Berkeley National Laboratory. It allows for real time x-ray micro-tomographic imaging of test materials under mechanical load at temperatures up to 2300 degrees C in controlled environments (vacuum or controlled gas flow). Sample heating is by six infrared halogen lamps with ellipsoidal reflectors arranged in a confocal configuration, which generates an approximately spherical zone of high heat flux approximately 5 mm in diameter. Samples are held between grips connected to a motorized stage that loads the samples in tension or compression with forces up to 2.2 kN. The heating chamber and loading system are water-cooled for thermal stability. The entire instrument is mounted on a rotation stage that allows stepwise recording of radiographs over an angular range of 180 degrees. A thin circumferential (360 degrees) aluminum window in the wall of the heating chamber allows the x-rays to pass through the chamber and the sample over the full angular range. The performance of the instrument has been demonstrated by characterizing the evolution of 3D damage mechanisms in ceramic composite materials under tensile loading at 1750 degrees C. (C) 2014 AIP Publishing LLC.
C1 [Haboub, Abdel; Nasiatka, James R.; Ritchie, Robert O.; MacDowell, Alastair A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Bale, Hrishikesh A.; Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Cox, Brian N.; Marshall, David B.] Teledyne Sci Co, Thousand Oaks, CA 91360 USA.
RP Ritchie, RO (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM roritchie@lbl.gov
RI Ritchie, Robert/A-8066-2008
OI Ritchie, Robert/0000-0002-0501-6998
FU U.S. Air Force Office of Scientific Research (AFOSR); National
Aeronautics and Space Administration (NASA) under the National
Hypersonics Science Center for Materials and Structures (AFOSR)
[FA9550-09-1-0477]; Office of Science, Office of Basic Energy Sciences,
of the U.S. Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the U.S. Air Force Office of Scientific
Research (AFOSR) (Dr. Ali Sayir) and National Aeronautics and Space
Administration (NASA) ( Dr. Anthony Calomino) under the National
Hypersonics Science Center for Materials and Structures (AFOSR Prime
Contract No. FA9550-09-1-0477 to Teledyne Scientific with sub-contract
to the University of California, Berkeley). We are grateful for use of
the x-ray micro-tomography beamline (8.3.2) at the Advanced Light
Source, which is supported by the Director, Office of Science, Office of
Basic Energy Sciences, of the U.S. Department of Energy under Contract
No. DE-AC02-05CH11231.
NR 31
TC 4
Z9 4
U1 4
U2 42
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083702
DI 10.1063/1.4892437
PG 13
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500033
PM 25173271
ER
PT J
AU Jones, MC
Ampleford, DJ
Cuneo, ME
Hohlfelder, R
Jennings, CA
Johnson, DW
Jones, B
Lopez, MR
MacArthur, J
Mills, JA
Preston, T
Rochau, GA
Savage, M
Spencer, D
Sinars, DB
Porter, JL
AF Jones, M. C.
Ampleford, D. J.
Cuneo, M. E.
Hohlfelder, R.
Jennings, C. A.
Johnson, D. W.
Jones, B.
Lopez, M. R.
MacArthur, J.
Mills, J. A.
Preston, T.
Rochau, G. A.
Savage, M.
Spencer, D.
Sinars, D. B.
Porter, J. L.
TI X-ray power and yield measurements at the refurbished Z machine
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID Z-PINCH EXPERIMENTS; Z-ACCELERATOR; ARRAY; DETECTORS; FLUENCE
AB Advancements have been made in the diagnostic techniques to measure accurately the total radiated x-ray yield and power from z-pinch implosion experiments at the Z machine with high accuracy. The Z machine is capable of outputting 2 MJ and 330 TW of x-ray yield and power, and accurately measuring these quantities is imperative. We will describe work over the past several years which include the development of new diagnostics, improvements to existing diagnostics, and implementation of automated data analysis routines. A set of experiments on the Z machine were conducted in which the load and machine configuration were held constant. During this shot series, it was observed that the total z-pinch x-ray emission power determined from the two common techniques for inferring the x-ray power, a Kimfol filtered x-ray diode diagnostic and the total power and energy diagnostic, gave 449 TW and 323 TW, respectively. Our analysis shows the latter to be the more accurate interpretation. More broadly, the comparison demonstrates the necessity to consider spectral response and field of view when inferring x-ray powers from z-pinch sources. (C) 2014 AIP Publishing LLC.
C1 [Jones, M. C.; Ampleford, D. J.; Cuneo, M. E.; Hohlfelder, R.; Jennings, C. A.; Johnson, D. W.; Jones, B.; Lopez, M. R.; MacArthur, J.; Mills, J. A.; Preston, T.; Rochau, G. A.; Savage, M.; Spencer, D.; Sinars, D. B.; Porter, J. L.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Jones, MC (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM micjone@sandia.gov
FU U.S. Department of Energy's National Nuclear Security Administration
[DEAC04-94AL85000]
FX The authors would like to thank the entire Z Operation Team, who make
this work possible. Sandia National Laboratories is a multiprogram
laboratory managed and operated by Sandia Corporation, a wholly owned
subsidiary of Lockheed Martin Corporation, for the U.S. Department of
Energy's National Nuclear Security Administration under Contract No.
DEAC04-94AL85000.
NR 35
TC 20
Z9 22
U1 0
U2 6
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083501
DI 10.1063/1.4891316
PG 11
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500025
PM 25173263
ER
PT J
AU King, JD
Strait, EJ
Boivin, RL
Taussig, D
Watkins, MG
Hanson, JM
Logan, NC
Paz-Soldan, C
Pace, DC
Shiraki, D
Lanctot, MJ
La Haye, RJ
Lao, LL
Battaglia, DJ
Sontag, AC
Haskey, SR
Bak, JG
AF King, J. D.
Strait, E. J.
Boivin, R. L.
Taussig, D.
Watkins, M. G.
Hanson, J. M.
Logan, N. C.
Paz-Soldan, C.
Pace, D. C.
Shiraki, D.
Lanctot, M. J.
La Haye, R. J.
Lao, L. L.
Battaglia, D. J.
Sontag, A. C.
Haskey, S. R.
Bak, J. G.
TI An upgrade of the magnetic diagnostic system of the DIII-D tokamak for
non-axisymmetric measurements
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID SPECTROSCOPY; MODE
AB The DIII-D tokamak magnetic diagnostic system [E. J. Strait, Rev. Sci. Instrum. 77, 023502 (2006)] has been upgraded to significantly expand the measurement of the plasma response to intrinsic and applied non-axisymmetric "3D" fields. The placement and design of 101 additional sensors allow resolution of toroidal mode numbers 1 <= n <= 3, and poloidal wavelengths smaller than MARS-F, IPEC, and VMEC magnetohydrodynamic model predictions. Small 3D perturbations, relative to the equilibrium field (10(-5) < delta B/B-0 < 10(-4)), require sub-millimeter fabrication and installation tolerances. This high precision is achieved using electrical discharge machined components, and alignment techniques employing rotary laser levels and a coordinate measurement machine. A 16-bit data acquisition system is used in conjunction with analog signal-processing to recover non-axisymmetric perturbations. Co-located radial and poloidal field measurements allow up to 14.2 cm spatial resolution of poloidal structures (plasma poloidal circumference is similar to 500 cm). The function of the new system is verified by comparing the rotating tearing mode structure, measured by 14 BP fluctuation sensors, with that measured by the upgraded BR saddle loop sensors after the mode locks to the vessel wall. The result is a nearly identical 2/1 helical eigenstructure in both cases. (C) 2014 AIP Publishing LLC.
C1 [King, J. D.; Paz-Soldan, C.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA.
[Strait, E. J.; Boivin, R. L.; Taussig, D.; Watkins, M. G.; Pace, D. C.; Lanctot, M. J.; La Haye, R. J.; Lao, L. L.] Gen Atom, San Diego, CA 92186 USA.
[Hanson, J. M.; Shiraki, D.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
[Logan, N. C.; Battaglia, D. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Sontag, A. C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Haskey, S. R.] Australia Natl Univ, Res Sch Phys Sci & Engn, Plasma Res Lab, Canberra, ACT 0200, Australia.
[Bak, J. G.] Natl Fus Res Ctr, Div Res & Dev, Taejon, South Korea.
RP King, JD (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA.
RI Haskey, Shaun/M-1469-2015; Lanctot, Matthew J/O-4979-2016
OI Haskey, Shaun/0000-0002-9978-6597; Lanctot, Matthew
J/0000-0002-7396-3372
FU U.S. Department of Energy, Office of Science, Office of Fusion Energy
Sciences [DE-FC02-04ER54698, DE-AC05-06OR23100, DE-AC02-09CH11466,
DE-AC05-00OR22725]; AINSE Ltd.
FX This material is based upon work supported by the U.S. Department of
Energy, Office of Science, Office of Fusion Energy Sciences, using the
DIII-D National Fusion Facility, a DOE Office of Science user facility,
under Awards DE-FC02-04ER54698, DE-AC05-06OR23100, DE-AC02-09CH11466,
DE-AC02-09CH11466, and DE-AC05-00OR22725. DIII-D data shown in this
paper can be obtained in digital format by following the links at
https://fusion.gat.com/global/D3D. The authors are very grateful to the
whole DIII-D team. The authors would like to give a special thanks to J.
Kulchar and D. Ayala for their enormous fabrication efforts. Additional
gratitude is also due to the operations staff of DIII-D, who went the
extra mile to see this project succeed, namely: R. L. Lee, P. L. Taylor,
A. G. Kellman, C. J. Murphy, B. Scoville, B. Brown, R. Tompkins, J.
Burchett, E. Gonzales, D. Kellman, D. Piglowski, W. Carrig, and D.
Whitaker. Also, thanks to D. Eldon for his graphics expertise. S. R.
Haskey wishes to thank AINSE Ltd. for providing financial assistance.
NR 27
TC 18
Z9 18
U1 0
U2 5
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083503
DI 10.1063/1.4891817
PG 8
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500027
PM 25173265
ER
PT J
AU Oks, E
Shandrikov, M
Salvadori, C
Brown, I
AF Oks, Efim
Shandrikov, Maxim
Salvadori, Cecilia
Brown, Ian
TI Low-energy dc ion source for low operating pressure
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID FILMS
AB We report on an experimental study of an ion source based on a Penning discharge with a cold hollow cathode in crossed electric and magnetic fields. The minimum vacuum chamber operating pressure was 3 x 10(-5) Torr for argon and 5 x 10(-5) Torr for hydrogen. The use of a hollow cathode allowed decreasing the discharge operating voltage down to 350 V at a discharge current of similar to 100 mA. At a discharge current of 100 mA and beam accelerating voltage of 2 kV, the ion current was 2.5 mA for argon and 8 mA for hydrogen, and the ion beam on-axis current density 170 and 450 mu A/cm(2), respectively. The current-voltage characteristics of the discharge and the radial ion beam current density distribution were measured. The influence of pressure on the discharge parameters and their time stability was investigated. (C) 2014 AIP Publishing LLC.
C1 [Oks, Efim; Shandrikov, Maxim] Russian Acad Sci, Inst High Current Elect, Tomsk 634055, Russia.
[Oks, Efim] State Univ Control Syst & Radioelect, Tomsk 634050, Russia.
[Salvadori, Cecilia] Univ Sao Paulo, Inst Phys, BR-05315970 Sao Paulo, Brazil.
[Brown, Ian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Oks, E (reprint author), Russian Acad Sci, Inst High Current Elect, Akademichesky Ave 2-3, Tomsk 634055, Russia.
EM oks@opee.hcei.tsc.ru
RI Salvadori, Maria Cecilia/A-9379-2013; Shandrikov, Maxim/R-2148-2016;
OI Oks, Efim/0000-0002-9323-0686
FU Russian Science Foundation [14-49-00001]
FX The work was supported by the Russian Science Foundation, program for
international research group, Project No. 14-49-00001.
NR 9
TC 1
Z9 1
U1 1
U2 13
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 083502
DI 10.1063/1.4891697
PG 4
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500026
PM 25173264
ER
PT J
AU Seol, Y
Choi, JH
Dai, S
AF Seol, Yongkoo
Choi, Jeong-Hoon
Dai, Sheng
TI Multi-property characterization chamber for geophysical-hydrological
investigations of hydrate bearing sediments
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID STRATIGRAPHIC TEST WELL; ALASKA NORTH SLOPE; METHANE-HYDRATE;
PHYSICAL-PROPERTIES; SAND; PERMEABILITY; DISSOCIATION; DEFORMATION;
STRENGTH
AB With the increase in the interest of producing natural gas from methane hydrates as well as potential risks of massive hydrate dissociation in the context of global warming, studies have recently shifted from pure hydrate crystals to hydrates in sediments. Such a research focus shift requires a series of innovative laboratory devices that are capable of investigating various properties of hydrate-bearing sediments (HBS). This study introduces a newly developed high pressure testing chamber, i.e., multi-property characterization chamber (MPCC), that allows simultaneous investigation of a series of fundamental properties of HBS, including small-strain stiffness (i.e., P- and S-waves), shear strength, large-strain deformation, stress-volume responses, and permeability. The peripheral coolant circulation system of the MPCC permits stable and accurate temperature control, while the core holder body, made of aluminum, enables X-ray computer tomography scanning to be easily employed for structural and morphological characterization of specimens. Samples of hydrate-bearing sediments are held within a rubber sleeve inside the chamber. The thick sleeve is more durable and versatile than thin membranes while also being much softer than oedometer-type chambers that are incapable of enabling flow tests. Bias introduced by the rubber sleeve during large deformation tests are also calibrated both theoretically and experimentally. This system provides insight into full characterization of hydrate-bearing sediments in the laboratory, as well as pressure core technology in the field.
C1 [Seol, Yongkoo; Choi, Jeong-Hoon; Dai, Sheng] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
RP Seol, Y (reprint author), US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
EM Yongkoo.Seol@netl.doe.gov
RI Dai, Sheng/A-1691-2015;
OI Dai, Sheng/0000-0003-0221-3993
FU Oak Ridge Institute for Science and Education (ORISE) fellowship - NETL,
(U.S.) Department of Energy (DOE)
FX We thank Karl Jarvis (URS) for technical support and Richard Baker
(NETL) for discussions. J.-H. Choi and S. Dai are supported via the Oak
Ridge Institute for Science and Education (ORISE) fellowship granted by
NETL, (U.S.) Department of Energy (DOE).
NR 46
TC 3
Z9 3
U1 0
U2 10
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 084501
DI 10.1063/1.4892995
PG 8
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500050
PM 25173288
ER
PT J
AU Smither, RK
AF Smither, Robert K.
TI Invited Review Article: Development of crystal lenses for energetic
photons
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Review
ID X-RAY PROPAGATION; DISTORTED CRYSTALS; PENDELLOSUNG FRINGES; GAMMA-RAYS;
DIFFRACTION EFFICIENCY; GRADIENT CRYSTALS; SINGLE-CRYSTALS;
IMAGING-SYSTEM; LAUE GEOMETRY; BENT-CRYSTAL
AB This paper follows the development of crystal diffraction lenses designed to focus energetic photons. It begins with the search for a solution to the astrophysics problem of how to detect weak astrophysics sources of gamma rays and x-rays. This led to the basic designs for a lens and to the understanding of basic limitations of lens design. The discussion of the development of crystal diffraction lenses is divided into two parts: lenses using crystals with mosaic structure, and lenses that use crystals with curved crystal planes. This second group divides into two sub-groups: (1) Curved crystals that are used to increase the acceptance angle of the diffraction of a monochromatic beam and to increase the energy bandwidth of the diffraction. (2) Curved crystals used to focus gamma ray beams. The paper describes how these two types of crystals affect the design of the corresponding crystal lenses in different fields: astrophysics, medical imaging, detection of weak, distant, gamma-ray sources, etc. The designs of crystal lenses for these applications are given in enough detail to allow the reader to design a lens for his own application. (C) 2014 AIP Publishing LLC.
C1 Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Smither, RK (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
FU U.S. Department of Energy, BES-Materials Science [W-31-109-Eng-38]
FX The author wishes to thank Bernard Hamermesh for introducing him to the
art of crystal diffraction, Art Namenson for his assistance in many
cutting-edge experiments in crystal diffraction, and Niels Lund for his
encouragement and many interesting suggestions and advice. Thanks are
due to Armando Travelli for his support through the Argonne Treaty
Verification program, Larry Greenwood and Charles Roche for their
assistance in the construction of partial crystal lenses early in the
Treaty Verification program, and Patricia Fernandez, Tim Graber, Mohamed
Faiz, and Antje Kohnle for their assistance in constructing the first
full size Treaty Verification lens. The author would like to thank Peter
von Ballmoos and Jerry Skinner from CESR in Toulouse, France for
organizing the European collaboration that flew a crystal diffraction
telescope on two balloon flights to detect x-rays from the Crab nebula,
and Antje Kohnle, Juan Naya, Francis Albernhe, G. Vedrenne, and the
members of the European collaboration for their support and assistance
in these balloon flight experiments. The author would like to thank
Dante Roa for his assistance in building the first medical imaging
crystal diffraction lens at Argonne and Khaliefeh Abu Seleem, Mark Beno,
Charles Kurtz, and Ali Khounsary for their assistance in performing
experiments with bent crystals. Ali Paugys assisted in all of the above
mentioned activities and in the construction of the 50 m test facility
for the Treaty Verification lens and the two test stands used to conduct
the crystal diffraction experiments at the Argonne National Laboratory.
This work was supported by the U.S. Department of Energy, BES-Materials
Science, under Contract No. W-31-109-Eng-38.
NR 59
TC 3
Z9 3
U1 0
U2 3
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 081101
DI 10.1063/1.4893585
PG 35
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500001
PM 25173239
ER
PT J
AU Stone, MB
Niedziela, JL
Loguillo, MJ
Overbay, MA
Abernathy, DL
AF Stone, M. B.
Niedziela, J. L.
Loguillo, M. J.
Overbay, M. A.
Abernathy, D. L.
TI A radial collimator for a time-of-flight neutron spectrometer
SO REVIEW OF SCIENTIFIC INSTRUMENTS
LA English
DT Article
ID DIFFRACTION; SCATTERING; DIFFRACTOMETER; DETECTORS; STRESS
AB We have engineered and installed a radial collimator for use in the scattered beam of a neutron time-of-flight spectrometer at a spallation neutron source. The radial collimator may be used with both thermal and epithermal neutrons, reducing the detected scattering intensity due to material outside of the sample region substantially. The collimator is located inside of the sample chamber of the instrument, which routinely cycles between atmospheric conditions and cryogenic vacuum. The oscillation and support mechanism of the collimator allow it to be removed from use without breaking vacuum. We describe here the design and characterization of this radial collimator. (C) 2014 AIP Publishing LLC.
C1 [Stone, M. B.; Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Sci Div, Oak Ridge, TN 37831 USA.
[Niedziela, J. L.; Loguillo, M. J.; Overbay, M. A.] Oak Ridge Natl Lab, Instrument & Source Div, Oak Ridge, TN 37831 USA.
RP Stone, MB (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Sci Div, Oak Ridge, TN 37831 USA.
RI Stone, Matthew/G-3275-2011; Abernathy, Douglas/A-3038-2012; BL18,
ARCS/A-3000-2012
OI Stone, Matthew/0000-0001-7884-9715; Abernathy,
Douglas/0000-0002-3533-003X;
FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.
S. Department of Energy
FX We gratefully acknowledge the contributions of other support groups from
within the Neutron Sciences Directorate at ORNL including the Instrument
Data Acquisition and Controls group, especially A. A. Parizzi and G. C.
Greene, the Instrumentation Projects and Development group especially M.
Harvey, W. S. Keener, and G. Q. Rennich, the Vacuum Systems group
especially J. P. Price and C. M. Stone, the Mechanical Shop especially
G. L. Beets and W. Smith, the Instrument Development and Target Support
group especially B. J. Cagley, J. A. Groff, and R. Morgan, and the
Instrument Support group especially G. Brackett, W. Dawkins, D. Engle,
and S. Vasquez. We acknowledge helpful discussions with E. Iverson of
the Neutronics Analysis group. We thank JJ-Xray for their final design
and production of the radial collimator as well as Keller Technology
Corporation for their manufacturing of the elevator and oscillator
parts. For supplying information for the collimator comparison table we
thank B. Winn and G. Ehlers from the Spallation Neutron Source, D. Yu
from ANSTO, S. Rols from The Institut Laue Langevin, J. Embs from the
Paul Scherrer Institut, and C. M. Brown and J. R. D. Copley from the
NIST Center for Neutron Research. The research at Oak Ridge National
Laboratory's Spallation Neutron Source was sponsored by the Scientific
User Facilities Division, Office of Basic Energy Sciences, U. S.
Department of Energy.
NR 22
TC 5
Z9 5
U1 1
U2 13
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0034-6748
EI 1089-7623
J9 REV SCI INSTRUM
JI Rev. Sci. Instrum.
PD AUG
PY 2014
VL 85
IS 8
AR 085101
DI 10.1063/1.4891302
PG 9
WC Instruments & Instrumentation; Physics, Applied
SC Instruments & Instrumentation; Physics
GA AQ6IH
UT WOS:000342913500068
PM 25173306
ER
PT J
AU Oostrom, M
Truex, MJ
Wietsma, TW
Tartakovsky, GD
AF Oostrom, M.
Truex, M. J.
Wietsma, T. W.
Tartakovsky, G. D.
TI Pore-Water Extraction from Unsaturated Porous Media: Intermediate-Scale
Laboratory
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID VADOSE ZONE; HYDRAULIC CONDUCTIVITY; SOLUTE TRANSPORT; SOILS;
LYSIMETERS; COLLECTION; SIMULATION; SAMPLERS; MODEL
AB As a remedial approach, vacuum-induced pore-water extraction offers the possibility of contaminant and water removal from the vadose zone, which may be beneficial in reducing the flux of vadose zone contaminants to groundwater. Vadose zone water extraction is being considered at the Hanford Site in Washington State as a means to remove technetium-99 contamination from low permeability sediments with relatively high water contents. A series of intermediate-scale laboratory experiments have been conducted to improve the fundamental understanding and to recognize the limitations of the technique. Column experiments were designed to investigate the relations between imposed suctions, water saturations, and water extraction. Flow cell experiments were conducted to investigate the effects of high-permeability layers and near-well compaction on pore-water extraction efficiency. Results show that water extraction from unsaturated systems can be achieved in low permeability sediments, provided that the initial water saturations are relatively high. The presence of a high-permeability layer decreased the yield, and compaction near the well screen had a limited effect on overall performance. In all experiments, large pressure gradients were observed near the extraction screen. Minimum requirements for water extraction include an imposed suction larger than the initial sediment capillary pressure in combination with a fully saturated seepage-face boundary. A numerical multiphase simulator with a coupled seepage-face boundary condition was used to simulate the experiments. Reasonable matches were obtained between measured and simulated results for both water extraction and capillary pressures, suggesting that numerical simulations may be used as a design tool for field-scale applications of pore-water extraction.
C1 [Oostrom, M.; Truex, M. J.; Tartakovsky, G. D.] Pacific NW Natl Lab, Div Energy & Environm, Richland, WA 99354 USA.
[Wietsma, T. W.] Pacific NW Natl Lab, Dept Environm Mol Sci Lab, Richland, WA 99354 USA.
RP Oostrom, M (reprint author), Pacific NW Natl Lab, Div Energy & Environm, POB 999,MS K9-33, Richland, WA 99354 USA.
EM mart.oostrom@pnnl.gov
FU USDOE [DE-AC06-76RLO 1830]; U.S. Department of Energy, Richland
Operations Office; USDOE's Office of Biological and Environmental
Research
FX Pacific Northwest National Laboratory is operated by the Battelle
Memorial Institute for the USDOE under Contract DE-AC06-76RLO 1830. This
effort was part of the Deep Vadose Zone-Applied Field Research
Initiative at Pacific Northwest National Laboratory. Funding for this
work was provided by the U.S. Department of Energy, Richland Operations
Office. The intermediate-scale experiments were performed in the
Environmental Molecular Sciences Laboratory (EMSL), a national
scientific user facility sponsored by the USDOE's Office of Biological
and Environmental Research and located at PNNL. Scientists interested in
conducting experimental work in the EMSL are encouraged to contact M.
Oostrom (mart.oostrom@pnnl.gov).
NR 33
TC 1
Z9 1
U1 3
U2 21
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD AUG
PY 2014
VL 13
IS 8
DI 10.2136/vzj2014.04.0044
PG 13
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA AQ9HT
UT WOS:000343162100004
ER
PT J
AU Mizutani, U
Sato, H
Inukai, M
Zijlstra, ES
Lin, Q
Corbett, JD
Miller, GJ
AF Mizutani, U.
Sato, H.
Inukai, M.
Zijlstra, E. S.
Lin, Q.
Corbett, J. D.
Miller, G. J.
TI Fermi Surface-Brillouin Zone Interactions in 2/1-2/1-2/1 Bergman-Type
Approximant Na27Au27Ga31
SO ACTA PHYSICA POLONICA A
LA English
DT Article; Proceedings Paper
CT 12th International Conference on Quasicrystals (ICQ12)
CY SEP 01-06, 2013
CL Krakow, POLAND
ID ROTHERY STABILIZATION MECHANISM; ELECTRON-CONCENTRATION RULE; E/A
DETERMINATION; INTERMETALLIC COMPOUNDS; METAL ELEMENTS; QUASI-CRYSTAL;
AL; ZN
AB The X-ray diffraction studies on a newly synthesized Na26Au25Ga29 single crystal revealed the formation of a single phase 2/1-2/1-2/1 Bergman-type approximant and the presence of Au/Ga mixed occupancies in its unit cell containing 680 atoms. The structure model of the 2/1-2/1-2/1 approximant with composition Na27Au27Ga31 was constructed by eliminating the chemical disorder with a minimum sacrifice of composition displacement. The full potential linearized augmented plane wave electronic structure calculations with subsequent full potential linearized augmented plane wave-Fourier analysis were performed for the 2/1-2/1-2/1 approximant Na27Au27Ga31 with space group Pa (3) over bar. The square of the Fermi diameter (2kF)(2), electrons per atom ratio e/a and the critical reciprocal lattice vector vertical bar G vertical bar(2) are determined. A shallow pseudogap at the Fermi level was interpreted as originating from interference of electrons having (2kF)(2) = 109.2 +/- 1.0 with sets of lattice planes with vertical bar G vertical bar(2)s centered at 108. The effective e/a value for the compound is found to be 1.76 in good agreement with 1.73 derived from a composition average of (e/a)Na = 1.0, (e/a)Au = 1.0 and (e/a)Ga = 3.0.
C1 [Mizutani, U.] Nagoya Ind Sci Res Inst, Chikusa Ku, Nagoya, Aichi 4640819, Japan.
[Sato, H.] Aichi Univ Educ, Kariya, Aichi 4488542, Japan.
[Inukai, M.] Nagoya Inst Technol, Dept Frontier Mat, Showa Ku, Nagoya, Aichi 4668555, Japan.
[Zijlstra, E. S.] Univ Kassel, D-34132 Kassel, Germany.
[Lin, Q.; Corbett, J. D.; Miller, G. J.] US DOE, Ames Lab, Washington, DC 20585 USA.
[Lin, Q.; Corbett, J. D.; Miller, G. J.] Iowa State Univ, Dept Chem, Ames, IA USA.
RP Mizutani, U (reprint author), Nagoya Ind Sci Res Inst, Chikusa Ku, 1-13 Yotsuya Dori, Nagoya, Aichi 4640819, Japan.
EM uichiro@xa3.so-net.ne.jp
NR 11
TC 3
Z9 3
U1 0
U2 4
PU POLISH ACAD SCIENCES INST PHYSICS
PI WARSAW
PA AL LOTNIKOW 32-46, PL-02-668 WARSAW, POLAND
SN 0587-4246
EI 1898-794X
J9 ACTA PHYS POL A
JI Acta Phys. Pol. A
PD AUG
PY 2014
VL 126
IS 2
BP 535
EP 538
PG 4
WC Physics, Multidisciplinary
SC Physics
GA AQ1ME
UT WOS:000342544700029
ER
PT J
AU Unal, B
Evans, JW
Thiel, PA
AF Uenal, B.
Evans, J. W.
Thiel, P. A.
TI Temperature Dependence of Ag Film Roughening during Deposition on
Quasicrystal and Approximant Surfaces
SO ACTA PHYSICA POLONICA A
LA English
DT Article; Proceedings Paper
CT 12th International Conference on Quasicrystals (ICQ12)
CY SEP 01-06, 2013
CL Krakow, POLAND
ID MOLECULAR-BEAM EPITAXY; GROWTH; HOMOEPITAXY; ROUGHNESS; ISLANDS
AB The temperature (T) dependence of roughening as assessed by scanning tunneling microscopy is compared for growth of Ag films on an 5-fold icosahedral Al-Pd-Mn quasicrystal surface and on an xi'-approximant. Growth on the quasicrystal corresponds to a version of the Volmer Weber growth, but modified by quantum size effects, and also by kinetic smoothening at low T and low coverages (theta). Growth on the approximant corresponds to a version of the Stranski Krastanov growth modified by kinetic roughening at low T and low theta. For larger theta, i.e., for thicker films, distinct behavior is observed.
C1 [Uenal, B.; Evans, J. W.; Thiel, P. A.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
[Uenal, B.; Thiel, P. A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA.
[Evans, J. W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.
[Thiel, P. A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA.
RP Thiel, PA (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
EM pthiel@iastate.edu
NR 22
TC 0
Z9 0
U1 1
U2 5
PU POLISH ACAD SCIENCES INST PHYSICS
PI WARSAW
PA AL LOTNIKOW 32-46, PL-02-668 WARSAW, POLAND
SN 0587-4246
EI 1898-794X
J9 ACTA PHYS POL A
JI Acta Phys. Pol. A
PD AUG
PY 2014
VL 126
IS 2
BP 608
EP 612
PG 5
WC Physics, Multidisciplinary
SC Physics
GA AQ1ME
UT WOS:000342544700047
ER
PT J
AU Clague, DA
Dreyer, BM
Paduan, JB
Martin, JF
Caress, DW
Gill, JB
Kelley, DS
Thomas, H
Portner, RA
Delaney, JR
Guilderson, TP
McGann, ML
AF Clague, David. A.
Dreyer, Brian M.
Paduan, Jennifer B.
Martin, Julie F.
Caress, David W.
Gill, James B.
Kelley, Deborah S.
Thomas, Hans
Portner, Ryan A.
Delaney, John R.
Guilderson, Thomas P.
McGann, Mary L.
TI Eruptive and tectonic history of the Endeavour Segment, Juan de Fuca
Ridge, based on AUV mapping data and lava flow ages
SO GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS
LA English
DT Article
DE Juan de Fuca Ridge; Endeavour Segment; high-resolution bathymetry; lava
flow ages; tectonic; magmatic history
ID EAST PACIFIC RISE; RA-226 TH-230 DISEQUILIBRIUM; SEISMIC LAYER 2A;
OCEANIC-CRUST; HYDROTHERMAL SYSTEM; SULFIDE DEPOSITS; MIDOCEAN RIDGES;
AXIAL SEAMOUNT; RIFT-VALLEY; TIME-SCALE
AB High-resolution bathymetric surveys from autonomous underwater vehicles ABE and D. Allan B. were merged to create a coregistered map of 71.7 km(2) of the Endeavour Segment of the Juan de Fuca Ridge. Radiocarbon dating of foraminifera in cores from three dives of remotely operated vehicle Doc Ricketts provide minimum eruption ages for 40 lava flows that are combined with the bathymetric data to outline the eruptive and tectonic history. The ages range from Modern to 10,700 marine-calibrated years before present (yr BP). During a robust magmatic phase from >10,700 yr BP to approximate to 4300 yr BP, flows erupted from an axial high and many flowed >5 km down the flanks; some partly buried adjacent valleys. Axial magma chambers (AMCs) may have been wider than today to supply dike intrusions over a 2 km wide axial zone. Summit Seamount formed by approximate to 4770 yr BP and was subsequently dismembered during a period of extension with little volcanism starting approximate to 4300 yr BP. This tectonic phase with only rare volcanic eruptions lasted until approximate to 2300 yr BP and may have resulted in near-solidification of the AMCs. The axial graben formed by crustal extension during this period of low magmatic activity. Infrequent eruptions occurred on the flanks between 2620-1760 yr BP and within the axial graben since approximate to 1750 yr BP. This most recent phase of limited volcanic and intense hydrothermal activity that began approximate to 2300 yr BP defines a hydrothermal phase of ridge development that coincides with the present-day 1 km wide AMCs and overlying hydrothermal vent fields.
C1 [Clague, David. A.; Dreyer, Brian M.; Paduan, Jennifer B.; Martin, Julie F.; Caress, David W.; Thomas, Hans; Portner, Ryan A.] Monterey Bay Aquarium Res Inst, Moss Landing, CA 95039 USA.
[Dreyer, Brian M.; Gill, James B.; Guilderson, Thomas P.] Univ Calif Santa Cruz, Inst Marine Sci, Santa Cruz, CA 95064 USA.
[Kelley, Deborah S.; Delaney, John R.] Univ Washington, Sch Oceanog, Seattle, WA 98195 USA.
[Portner, Ryan A.] Brown Univ, Providence, RI 02912 USA.
[Guilderson, Thomas P.] LLNL, Ctr Accelerator Mass Spectrometry, Livermore, CA USA.
[McGann, Mary L.] US Geol Survey, Menlo Pk, CA 94025 USA.
RP Clague, DA (reprint author), Monterey Bay Aquarium Res Inst, Moss Landing, CA 95039 USA.
EM clague@mbari.org
OI Caress, David/0000-0002-6596-9133
FU NSF [OCE 0732611, OCE 1043274, OCE 0623161, 1061176, OCE 1043403]; David
and Lucile Packard Foundation; U.S. Department of Energy by Lawrence
Livermore National Laboratory [DE-AC52-07NA27344]
FX We thank the captains and crews of the R/V Western Flyer, R/V Zephyr,
R/V Thompson, and R/V Atlantis, and the skillful pilots of the ROV Doc
Ricketts, HOV ALVIN, and the AUV D. Allan B. and ABE teams. Without
their skill and professionalism at sea, neither the high-resolution
mapping data nor the 46 cores could have been collected and this study
could not have been completed. Andrew Burleigh, John Jamieson, Linda
Kunhz, Amy Lange, Sean Scott, and Kevin Werts assisted at sea during the
ROV dives and postdive sample curation at sea, including the cores
reported here. Marilena Calarco assisted at sea during the collection of
D. Allan B. data in 2008. Jim Holden, funded by NSF grant OCE 0732611,
kindly provided ship time to launch and recover the AUV during his 2008
cruise, including expenditure of a precious ALVIN dive to recover the
wayward AUV D. Allan B. Suzanne Carbotte kindly shared her latest AMC
depths and patiently educated the first author about MCS data and
interpretations. The AUV D. Allan B. surveys, ROV Doc Ricketts dives,
and salary and laboratory support to D. A. C., B. M. D., J.B.P., J.F.M.,
D. W. C., R. A. P., and H. T. were supported by a grant from the David
and Lucile Packard Foundation to MBARI. Additional support to process
and combine the AUV ABE survey data with that from the AUV D. Allan B
was provided to D. A. C. and D. W. C. under NSF grant OCE 1043274.
J.B.G. and B. M. D. were supported under NSF grants OCE 0623161 and
1061176. D. S. K. was supported under NSF grant OCE 1043403. The ABE
surveys were collected as part of a joint project between the University
of Washington, the W. M. Keck Foundation, and NEPTUNE Canada. We also
thank Dana Yoerger for his development and support of the ABE missions.
The 14C dating was performed under the auspices of the U.S.
Department of Energy by Lawrence Livermore National Laboratory under
Contract DE-AC52-07NA27344. The bathymetric swath data and grids are
available through the RIDGE Portal at Lamont Doherty Geological
Observatory.
NR 76
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PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 1525-2027
J9 GEOCHEM GEOPHY GEOSY
JI Geochem. Geophys. Geosyst.
PD AUG
PY 2014
VL 15
IS 8
BP 3364
EP 3391
DI 10.1002/2014GC005415
PG 28
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA AQ3KY
UT WOS:000342693400016
ER
PT J
AU Gangodagamage, C
Rowland, JC
Hubbard, SS
Brumby, SP
Liljedahl, AK
Wainwright, H
Wilson, CJ
Altmann, GL
Dafflon, B
Peterson, J
Ulrich, C
Tweedie, CE
Wullschleger, SD
AF Gangodagamage, Chandana
Rowland, Joel C.
Hubbard, Susan S.
Brumby, Steven P.
Liljedahl, Anna K.
Wainwright, Haruko
Wilson, Cathy J.
Altmann, Garrett L.
Dafflon, Baptiste
Peterson, John
Ulrich, Craig
Tweedie, Craig E.
Wullschleger, Stan D.
TI Extrapolating active layer thickness measurements across Arctic
polygonal terrain using LiDAR and NDVI data sets
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE active layer thickness; thaw depth; frozen ground; ice wedge polygons;
barrow; Alaska; eco-hydro-geo-thermal regimes
ID NORTH-CENTRAL ALASKA; KUPARUK RIVER-BASIN; CLIMATE-CHANGE; GROUND
TEMPERATURES; MODEL PERFORMANCE; MACKENZIE DELTA; PERMAFROST; USA;
TERRITORIES; VARIABILITY
AB Landscape attributes that vary with microtopography, such as active layer thickness (ALT), are labor intensive and difficult to document effectively through in situ methods at kilometer spatial extents, thus rendering remotely sensed methods desirable. Spatially explicit estimates of ALT can provide critically needed data for parameterization, initialization, and evaluation of Arctic terrestrial models. In this work, we demonstrate a new approach using high-resolution remotely sensed data for estimating centimeter-scale ALT in a 5 km(2) area of ice-wedge polygon terrain in Barrow, Alaska. We use a simple regression-based, machine learning data-fusion algorithm that uses topographic and spectral metrics derived from multisensor data (LiDAR and WorldView-2) to estimate ALT (2 m spatial resolution) across the study area. Comparison of the ALT estimates with ground-based measurements, indicates the accuracy (r(2)=0.76, RMSE 4.4 cm) of the approach. While it is generally accepted that broad climatic variability associated with increasing air temperature will govern the regional averages of ALT, consistent with prior studies, our findings using high-resolution LiDAR and WorldView-2 data, show that smaller-scale variability in ALT is controlled by local eco-hydro-geomorphic factors. This work demonstrates a path forward for mapping ALT at high spatial resolution and across sufficiently large regions for improved understanding and predictions of coupled dynamics among permafrost, hydrology, and land-surface processes from readily available remote sensing data.
Key Points
First effort to map the ALT using fine resolution remotely sensed data A blended methodology incorporating RS data and statistical manipulation Smaller-scale ALT is controlled by eco-hydro-geo variables
C1 [Gangodagamage, Chandana; Rowland, Joel C.; Brumby, Steven P.; Wilson, Cathy J.; Altmann, Garrett L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Hubbard, Susan S.; Wainwright, Haruko; Dafflon, Baptiste; Peterson, John; Ulrich, Craig] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Liljedahl, Anna K.] Univ Alaska Fairbanks, Water & Environm Res Ctr, Fairbanks, AK USA.
[Liljedahl, Anna K.] Univ Alaska Fairbanks, Int Arctic Res Ctr, Fairbanks, AK USA.
[Tweedie, Craig E.] Univ Texas El Paso, Dept Biol Sci, El Paso, TX 79968 USA.
[Wullschleger, Stan D.] Oak Ridge Natl Lab, Oak Ridge, TN USA.
RP Gangodagamage, C (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM chhandana@gmail.com
RI Wainwright, Haruko/A-5670-2015; Dafflon, Baptiste/G-2441-2015; Hubbard,
Susan/E-9508-2010; Wullschleger, Stan/B-8297-2012;
OI Wainwright, Haruko/0000-0002-2140-6072; Wullschleger,
Stan/0000-0002-9869-0446; Gangodagamage, Chandana/0000-0001-6511-1711
FU Next-Generation Ecosystem Experiments Arctic (NGEE-Arctic) project -
Office of Science, Office of Biological and Environmental Research of
the U.S. Department of Energy [DE-AC02-05CH11231]
FX This project was funded by the Next-Generation Ecosystem Experiments
Arctic (NGEE-Arctic) project, which is supported by the Director, Office
of Science, Office of Biological and Environmental Research of the U.S.
Department of Energy under contract DE-AC02-05CH11231. Authors would
like to thanks the three anonymous reviewers for their helpful comments.
Helpful discussions with Jacques Cloutier from Aero-Metric, Inc.
Anchorage, AK are greatly appreciated.
NR 83
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PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
EI 1944-7973
J9 WATER RESOUR RES
JI Water Resour. Res.
PD AUG
PY 2014
VL 50
IS 8
BP 6339
EP 6357
DI 10.1002/2013WR014283
PG 19
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA AQ2QJ
UT WOS:000342632300005
ER
PT J
AU Stein, CA
Cerrone, A
Ozturk, T
Lee, S
Kenesei, P
Tucker, H
Pokharel, R
Lind, J
Hefferan, C
Suter, RM
Ingraffea, AR
Rollett, AD
AF Stein, Clayton A.
Cerrone, Albert
Ozturk, Tugce
Lee, Sukbin
Kenesei, Peter
Tucker, Harris
Pokharel, Reeju
Lind, Jonathan
Hefferan, Christopher
Suter, Robert M.
Ingraffea, Anthony R.
Rollett, Anthony D.
TI Fatigue crack initiation, slip localization and twin boundaries in a
nickel-based superalloy
SO CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE
LA English
DT Review
DE LSHR; Fatigue; Slip accumulation; Coherent Sigma 3; Crack initiation;
Superalloy
ID GRAIN-SIZE; ROOM-TEMPERATURE; NUMERICAL-METHOD; NIMONIC PE16; COPPER;
MICROSTRUCTURE; COMPOSITES; MICROSCOPY; TEXTURE; TEM
AB The study of fatigue in metals, and fatigue initiation specifically, lends itself to analysis via an emerging set of characterization and modeling tools that describe polycrystals on the meso- or microstructural length scale. These include three-dimensional characterization techniques, elastic anisotropic and visco-plastic stress models, new approaches to the statistical description of stress and strain distributions, synthetic microstructure modeling, and improved tools for manipulating the large datasets generated. A specific example of analysis in both 2D and 3D of fatigue cracks in a nickel-based superalloy is given where all the cracks are effectively coincident with coherent twin boundaries. A spectral method is used to analyze the stress state based on a fully anisotropic elastic calculation. The results indicate that, although a high resolved shear stress is associated with the locations of the observed cracks, the length of the trace of the twin boundary is more strongly correlated with crack formation. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Stein, Clayton A.; Ozturk, Tugce; Tucker, Harris; Pokharel, Reeju; Rollett, Anthony D.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA.
[Cerrone, Albert; Ingraffea, Anthony R.] Cornell Univ, Sch Civil & Environm Engn, Ithaca, NY 14853 USA.
[Lee, Sukbin] UNIST, Sch Mech & Adv Mat Engn, Ulsan, South Korea.
[Kenesei, Peter] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Pokharel, Reeju] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
[Lind, Jonathan; Hefferan, Christopher; Suter, Robert M.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA.
[Lind, Jonathan] RJ Lee Grp, Monroeville, PA 15146 USA.
[Hefferan, Christopher] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Stein, CA (reprint author), Carnegie Mellon Univ, Dept Mat Sci & Engn, 5000 Forbes Ave, Pittsburgh, PA 15213 USA.
EM claystein@cmu.edu; arc247@cornell.edu; tozturk@andrew.cmu.edu;
sukbinlee@unist.ac.kr; kenesei@aps.anl.gov; reeju@lanl.gov;
lind.jf@gmail.com; chefferan@gmail.com; suter@andrew.cmu.edu;
ari1@comell.edu; rollett@cmu.edu
RI Suter, Robert/P-2541-2014; Rollett, Anthony/A-4096-2012; LEE,
SUKBIN/A-4936-2012; Ozturk, Tugce/E-9317-2016
OI Suter, Robert/0000-0002-0651-0437; Rollett, Anthony/0000-0003-4445-2191;
Ozturk, Tugce/0000-0001-5040-5821
FU AFOSR Discovery Challenge Thrust Grant [FA9550-10-1-0213]; National
Science Foundation [DMR080072]; U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX This project was supported by an AFOSR Discovery Challenge Thrust Grant
#FA9550-10-1-0213. This Research was also supported in part by the
National Science Foundation through XSEDE resources provided by Texas
Advanced Computing Center under Grant No. DMR080072. Materials and
testing were performed at the Air Force Research Laboratory at
Wright-Patterson Air Force Base in Dayton, Ohio, courtesy of Drs. R.
John and S. Jha. Use of the Advanced Photon Source was supported by the
U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences, under contract No. DE-AC02-06CH11357. Orientation maps were
reconstructed using IceNine, a software implementation of Li and Suter
[41] developed by S.F. Li. Dr. R. Lebensohn at the Los Alamos National
Laboratory is thanked for the use of his spectral method code.
NR 58
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U1 10
U2 53
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-0286
EI 1879-0348
J9 CURR OPIN SOLID ST M
JI Curr. Opin. Solid State Mat. Sci.
PD AUG
PY 2014
VL 18
IS 4
SI SI
BP 244
EP 252
DI 10.1016/j.cossms.2014.06.001
PG 9
WC Materials Science, Multidisciplinary; Physics, Applied; Physics,
Condensed Matter
SC Materials Science; Physics
GA AP7PW
UT WOS:000342270200009
ER
PT J
AU Meng, JY
Endo, T
AF Meng, Jiayuan
Endo, Toshio
TI Special Issue on Applications for the Heterogeneous Computing Era
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Editorial Material
C1 [Meng, Jiayuan] Argonne Natl Lab, Leadership Comp Facil Div, Argonne, IL 60439 USA.
[Endo, Toshio] Tokyo Inst Technol, Global Sci Informat & Comp Ctr GSIC, Tokyo, Japan.
RP Meng, JY (reprint author), Argonne Natl Lab, Leadership Comp Facil Div, Argonne, IL 60439 USA.
EM jmeng@alcf.anl.gov; endo@is.titech.ac.jp
NR 0
TC 0
Z9 0
U1 1
U2 1
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2014
VL 28
IS 3
SI SI
BP 253
EP 254
DI 10.1177/1094342014527657
PG 2
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA AP9GS
UT WOS:000342387600001
ER
PT J
AU You, Y
Fu, HH
Song, SL
Dehnavi, MM
Gan, L
Huang, XM
Yang, GW
AF You, Yang
Fu, Haohuan
Song, Shuaiwen Leon
Dehnavi, Maryam Mehri
Gan, Lin
Huang, Xiaomeng
Yang, Guangwen
TI Evaluating multi-core and many-core architectures through accelerating
the three-dimensional Lax-Wendroff correction stencil
SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS
LA English
DT Article
DE Complex stencil; 3D wave forward modeling; Kepler GPU; Intel Xeon Phi;
optimization techniques; performance power analysis
ID WAVE-PROPAGATION; HIGH-ORDER; GPU; PROCESSORS; POWER; CARDS
AB Wave propagation forward modeling is a widely used computational method in oil and gas exploration. The iterative stencil loops in such problems have broad applications in scientific computing. However, executing such loops can be highly time-consuming, which greatly limits their performance and power efficiency. In this paper, we accelerate the forward-modeling technique on the latest multi-core and many-core architectures such as Intel (R) Sandy Bridge CPUs, NVIDIA Fermi C2070 GPUs, NVIDIA Kepler K20X GPUs, and the Intel (R) Xeon Phi co-processor. For the GPU platforms, we propose two parallel strategies to explore the performance optimization opportunities for our stencil kernels. For Sandy Bridge CPUs and MIC, we also employ various optimization techniques in order to achieve the best performance. Although our stencil with 114 component variables poses several great challenges for performance optimization, and the low stencil ratio between computation and memory access is too inefficient to fully take advantage of our evaluated architectures, we manage to achieve performance efficiencies ranging from 4.730% to 20.02% of the theoretical peak. We also conduct cross-platform performance and power analysis (focusing on Kepler GPU and MIC) and the results could serve as insights for users selecting the most suitable accelerators for their targeted applications.
C1 [You, Yang; Fu, Haohuan; Gan, Lin; Huang, Xiaomeng; Yang, Guangwen] Tsinghua Univ, Dept Comp Sci & Technol, Beijing 100084, Peoples R China.
[Song, Shuaiwen Leon] Pacific NW Natl Lab, Performance Anal Lab, Richland, WA 99352 USA.
[Dehnavi, Maryam Mehri] MIT, Comp Sci & Artificial Intelligence Lab, Cambridge, MA 02139 USA.
[Fu, Haohuan; Gan, Lin; Huang, Xiaomeng; Yang, Guangwen] Tsinghua Univ, Key Lab Earth Syst Modeling, Minist Educ, Beijing 100084, Peoples R China.
RP You, Y (reprint author), Tsinghua Univ, Dept Comp Sci & Technol, FIT 3-126, Beijing 100084, Peoples R China.
EM you-y12@mails.tsinghua.edu.cn
FU National Natural Science Foundation of China [61303003, 41374113];
National High-tech R&D (863) Program of China [2013AA01A208]
FX This work was supported in part by the National Natural Science
Foundation of China (grant numbers 61303003 and 41374113) and the
National High-tech R&D (863) Program of China (grant number
2013AA01A208).
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U1 1
U2 8
PU SAGE PUBLICATIONS LTD
PI LONDON
PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND
SN 1094-3420
EI 1741-2846
J9 INT J HIGH PERFORM C
JI Int. J. High Perform. Comput. Appl.
PD AUG
PY 2014
VL 28
IS 3
SI SI
BP 301
EP 318
DI 10.1177/1094342014524807
PG 18
WC Computer Science, Hardware & Architecture; Computer Science,
Interdisciplinary Applications; Computer Science, Theory & Methods
SC Computer Science
GA AP9GS
UT WOS:000342387600005
ER
PT J
AU Schroeder, U
Yurchuk, E
Muller, J
Martin, D
Schenk, T
Polakowski, P
Adelmann, C
Popovici, MI
Kalinin, SV
Mikolajick, T
AF Schroeder, Uwe
Yurchuk, Ekaterina
Mueller, Johannes
Martin, Dominik
Schenk, Tony
Polakowski, Patrick
Adelmann, Christoph
Popovici, Mihaela I.
Kalinin, Sergei V.
Mikolajick, Thomas
TI Impact of different dopants on the switching properties of ferroelectric
hafniumoxide
SO JAPANESE JOURNAL OF APPLIED PHYSICS
LA English
DT Article
ID FENAND FLASH MEMORY; CAPACITORS; LOGIC; FILMS; HFO2
AB The wake-up behavior of ferroelectric thin film capacitors based on doped hafnium oxide dielectrics in TiN-based metal-insulator-metal-structures is reported. After field cycling a remanent polarization up to 40 mu C/cm(2) and a high coercive field of about 1 MV/cm was observed. Doping of HfO2 by different dopants with a crystal radius ranging from 54 pm (Si) to 132 pm (Sr) was evaluated. In all cases, an improved polarization-voltage hysteresis after wake-up cycling is visible. For smaller dopant atoms like Si and Al stronger pinching of the polarization hysteresis appeared with increasing dopant concentration and proved to be stable during cycling. (C) 2014 The Japan Society of Applied Physics
C1 [Schroeder, Uwe; Yurchuk, Ekaterina; Martin, Dominik; Schenk, Tony; Mikolajick, Thomas] NaMLab gGmbH, D-01187 Dresden, Germany.
[Mueller, Johannes; Polakowski, Patrick] Fraunhofer IPMS CNT, D-01099 Dresden, Germany.
[Adelmann, Christoph; Popovici, Mihaela I.] Imec, B-3001 Leuven, Belgium.
[Mikolajick, Thomas] Tech Univ Dresden, IHM, D-01187 Dresden, Germany.
[Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Schroeder, U (reprint author), NaMLab gGmbH, Noethnitzer Str 64, D-01187 Dresden, Germany.
EM Uwe.Schroeder@namlab.com
RI Mikolajick, Thomas/F-8427-2011; Kalinin, Sergei/I-9096-2012;
OI Mikolajick, Thomas/0000-0003-3814-0378; Kalinin,
Sergei/0000-0001-5354-6152; Adelmann, Christoph/0000-0002-4831-3159
FU European Fund for Regional Development; Free State of Saxony (Heiko/Cool
Memory project)
FX The authors acknowledge T. Boscke and D. Brauhaus for their initial work
on ferroelectric HfO2, and S. Muller, and T. Schlosser for
sample preparation and characterization. This work was financially
supported by the European Fund for Regional Development and the Free
State of Saxony (Heiko/Cool Memory project).
NR 30
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U1 10
U2 63
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 0021-4922
EI 1347-4065
J9 JPN J APPL PHYS
JI Jpn. J. Appl. Phys.
PD AUG
PY 2014
VL 53
IS 8
SI 1
BP 85
EP 89
DI 10.7567/JJAP.53.08LE02
PG 5
WC Physics, Applied
SC Physics
GA AQ1EC
UT WOS:000342523700018
ER
PT J
AU Humble, TS
Sadlier, RJ
AF Humble, Travis S.
Sadlier, Ronald J.
TI Software-defined quantum communication systems
SO OPTICAL ENGINEERING
LA English
DT Article
DE quantum communication; software-defined systems; quantum networks;
quantum engineering; software engineering
ID QKD SYSTEM; RECONCILIATION; CHANNELS; STATES; FPGA
AB Quantum communication (QC) systems harness modern physics through state-of-the-art optical engineering to provide revolutionary capabilities. An important concern for QC engineering is designing and prototyping these systems to evaluate the proposed capabilities. We apply the paradigm of software-defined communication for engineering QC systems to facilitate rapid prototyping and prototype comparisons. We detail how to decompose QC terminals into functional layers defining hardware, software, and middleware concerns, and we describe how each layer behaves. Using the superdense coding protocol as an example, we describe implementations of both the transmitter and receiver, and we present results from numerical simulations of the behavior. We conclude that the software-defined QC provides a robust framework in which to explore the large design space offered by this new regime of communication. (C) 2014 Society of Photo-Optical Instrumentation Engineers (SPIE)
C1 [Humble, Travis S.; Sadlier, Ronald J.] Oak Ridge Natl Lab, Quantum Comp Inst, Oak Ridge, TN 37831 USA.
[Humble, Travis S.] Univ Tennessee, Bredesen Ctr, Knoxville, TN 37996 USA.
[Sadlier, Ronald J.] Univ Rhode Isl, Kingston, RI 02881 USA.
RP Humble, TS (reprint author), Oak Ridge Natl Lab, Quantum Comp Inst, MS 6015,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.
EM humblets@ornl.gov
OI Sadlier, Ronald/0000-0003-2922-1125
FU Department of Energy Science Undergraduate Laboratory Internships (SULI)
program; U.S. Government [DE-AC05-00OR22725]
FX T. S. H. thanks Henry Humble for comments regarding the SDQC design in
Sec. 2, Toby Flynn and Laura Ann Anderson for help evaluating the Zynq
middleware, and Ali Ismail for initial efforts in defining the
middleware interface. R. J. S. thanks the Department of Energy Science
Undergraduate Laboratory Internships (SULI) program for support. This
work was supported by the Defense Threat Reduction Agency. This
manuscript has been authored by a contractor of the U.S. Government
under Contract No. DE-AC05-00OR22725.
NR 29
TC 5
Z9 5
U1 4
U2 33
PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS
PI BELLINGHAM
PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA
SN 0091-3286
EI 1560-2303
J9 OPT ENG
JI Opt. Eng.
PD AUG
PY 2014
VL 53
IS 8
AR 086103
DI 10.1117/1.OE.53.8.086103
PG 8
WC Optics
SC Optics
GA AO2YT
UT WOS:000341195300038
ER
PT J
AU Yashchuk, VV
Ty