FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Badosa, J Calbo, J Mckenzie, R Liley, B Gonzalez, JA Forgan, B Long, CN AF Badosa, Jordi Calbo, Josep Mckenzie, Richard Liley, Ben Gonzalez, Josep-Abel Forgan, Bruce Long, Charles N. TI Two Methods for Retrieving UV Index for All Cloud Conditions from Sky Imager Products or Total SW Radiation Measurements SO PHOTOCHEMISTRY AND PHOTOBIOLOGY LA English DT Article ID CLEAR SKIES; IRRADIANCE; OZONE; MIDLATITUDES; VARIABILITY; ULTRAVIOLET; ATMOSPHERE; NORTHERN; TRENDS; SITES AB Cloud effects on UV Index (UVI) and total solar radiation (TR) as a function of cloud cover and sunny conditions (from sky images) as well as of solar zenith angle (SZA) are assessed. These analyses are undertaken for a southern-hemisphere mid-latitude site where a 10-years dataset is available. It is confirmed that clouds reduce TR more than UV, in particular for obscured Sun conditions, low cloud fraction (<60%) and large SZA (>60 degrees). Similarly, local short-time enhancement effects are stronger for TR than for UV, mainly for visible Sun conditions, large cloud fraction and large SZA. Two methods to estimate UVI are developed: (1) from sky imaging cloud cover and sunny conditions, and (2) from TR measurements. Both methods may be used in practical applications, although Method 2 shows overall the best performance, as TR allows considering cloud optical properties. The mean absolute (relative) differences of Method 2 estimations with respect to measured values are 0.17 UVI units (6.7%, for 1 min data) and 0.79 Standard Erythemal Dose (SED) units (3.9%, for daily integrations). Method 1 shows less accurate results but it is still suitable to estimate UVI: mean absolute differences are 0.37 UVI units (15%) and 1.6 SED (8.0%). C1 [Badosa, Jordi] Ecole Polytech, LMD, Palaiseau, France. [Calbo, Josep; Gonzalez, Josep-Abel] UdG, Dept Fis, Girona, Spain. [Mckenzie, Richard; Liley, Ben] Natl Inst Water & Atmospher Res NIWA, Lauder, New Zealand. [Forgan, Bruce] BoM, Melbourne, Vic, Australia. [Long, Charles N.] PNNL, Richland, WA USA. RP Calbo, J (reprint author), UdG, Dept Fis, Girona, Spain. EM josep.calbo@udg.edu RI Calbo, Josep/K-2462-2014; OI Calbo, Josep/0000-0002-9374-0790; Liley, Ben/0000-0002-8844-7928 FU Ministry of Economy and Competitiveness project NUCLIEREX [CGL 2007-62664/CLI]; Ministry of Economy and Competitiveness project NUCLIERSOL [CGL 2010-18546]; Spanish Complementary Action [PCI2006-A7-0604]; Office of Science of the U.S. Department of Energy as part of the Atmospheric Systems Research Program FX We acknowledge the support in the data analyses from Michael Kotkamp (NIWA, Lauder, New Zealand). This study has been partly financed by the Spanish Ministry of Science and Innovation (currently Ministry of Economy and Competitiveness) projects NUCLIEREX (CGL 2007-62664/CLI) and NUCLIERSOL (CGL 2010-18546). Also, the Spanish Complementary Action PCI2006-A7-0604 allowed travelling Dr. J. Calbo and Dr. R. L. McKenzie to compile the data and to initiate the study. Dr. Long acknowledges support from the Office of Science of the U.S. Department of Energy as part of the Atmospheric Systems Research Program. NR 37 TC 2 Z9 2 U1 0 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0031-8655 EI 1751-1097 J9 PHOTOCHEM PHOTOBIOL JI Photochem. Photobiol. PD JUL-AUG PY 2014 VL 90 IS 4 BP 941 EP 951 DI 10.1111/php.12272 PG 11 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AL4IM UT WOS:000339096400027 PM 24645969 ER PT J AU Matmon, A Fink, D Davis, M Niedermann, S Rood, D Frumkin, A AF Matmon, A. Fink, D. Davis, M. Niedermann, S. Rood, D. Frumkin, A. TI Unraveling rift margin evolution and escarpment development ages along the Dead Sea fault using cosmogenic burial ages SO QUATERNARY RESEARCH LA English DT Article DE Sedom Lagoon; Amora Lake; Cosmogenic burial dating; Dead Sea fault ID BE-10 HALF-LIFE; RED-SEA; LANDSCAPE EVOLUTION; SEDOM DIAPIR; HISTORIC EARTHQUAKES; TERRESTRIAL ROCKS; PLATE KINEMATICS; NORTHERN ISRAEL; YAMMOUNEH FAULT; DRAINAGE-BASIN AB The Dead Sea fault (DSF) is one of the most active plate boundaries in the world. Understanding the Quaternary history and sediments of the DSF requires investigation into the Neogene development of this plate boundary. DSF lateral motion preceded significant extension and rift morphology by -10 Ma. Sediments of the Sedom Formation, dated here between 5.0 0.5 Ma and 6.2 +/- 451 Ma, yielded extremely lowl Be concentrations and 26A1 is absent. These reflect the antiquity of the sediments, deposited in the Sedom Lagoon, which evolved in a subdued landscape and was connected to the Mediterranean Sea. The base of the overlying Amora Formation, deposited in the terminal Amora Lake which developed under increasing relief that promoted escarpment incision, was dated at 3.311 Ma. Burial ages of fluvial sediments within caves (3.4 +/- 0.2 Ma and 3.6 +/- 0.4 Ma) represent the timing of initial incision. Initial DSF topography coincides with the earliest Red Sea MORB's and the East Anatolian fault initiation. These suggest a change in the relative Arabian-African plate motion. This change introduced the rifting component to the DSF followed by a significant subsidence, margin uplift, and a reorganization of relief and drainage pattern in the region resulting in the topographic framework observed today. (C) 2014 University of Washington. Published by Elsevier Inc. All rights reserved. C1 [Matmon, A.; Davis, M.] Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. [Fink, D.] Australian Nucl Sci & Technol Org, Menai, NSW 2234, Australia. [Niedermann, S.] Helmholtz Zentrum Potsdam, Deutsch GeoForschungsZentrum, D-14473 Potsdam, Germany. [Rood, D.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. [Frumkin, A.] Hebrew Univ Jerusalem, Dept Geog, IL-91905 Jerusalem, Israel. RP Matmon, A (reprint author), Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. EM arimatmon@mail.huji.ac.il RI fink, David/A-9518-2012; OI Niedermann, Samuel/0000-0003-1626-5284 FU ISF-Bikura [362/06]; Hebrew University Ring internal grant FX This study was supported by the ISF-Bikura grant 362/06 and Hebrew University Ring internal grant. We thank Roi Porat and Uri Davidovich who noted to us the potential significance of the Masada cave sediments to the rift margin evolution. NR 117 TC 8 Z9 8 U1 0 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0033-5894 EI 1096-0287 J9 QUATERNARY RES JI Quat. Res. PD JUL PY 2014 VL 82 IS 1 BP 281 EP 295 DI 10.1016/j.ygres.2014.04.008 PG 15 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA AL4XP UT WOS:000339138400027 ER PT J AU Kim, YJ Karaulanov, T Matlashov, AN Newman, S Urbaitis, A Volegov, P Yoder, J Espy, MA AF Kim, Y. J. Karaulanov, T. Matlashov, A. N. Newman, S. Urbaitis, A. Volegov, P. Yoder, J. Espy, M. A. TI Polarization enhancement technique for nuclear quadrupole resonance detection SO SOLID STATE NUCLEAR MAGNETIC RESONANCE LA English DT Article DE Nuclear quadrupole resonance (NQR); Nitrogen-14; Polarization enhancement NQR; Ammonium nitrate ID N-14 NQR SIGNAL; RELAXATION MEASUREMENTS; SODIUM-NITRITE; EXPLOSIVES; DRUGS; T1 AB We demonstrate a dramatic increase in the signal-to-noise ratio (SNR) of a nuclear quadrupole resonance (NQR) signal by using a polarization enhancement technique. By first applying a static magnetic field to pre-polarize one spin subsystem of a material, and then allowing that net polarization to be transferred to the quadrupole subsystem, we increased the SNR of a sample of ammonium nitrate by one-order of magnitude. Published by Elsevier Inc. C1 [Kim, Y. J.; Karaulanov, T.; Matlashov, A. N.; Newman, S.; Urbaitis, A.; Volegov, P.; Yoder, J.; Espy, M. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Kim, YJ (reprint author), Los Alamos Natl Lab, POB 1663,MS-D454, Los Alamos, NM 87545 USA. EM youngjin@lanl.gov OI Urbaitis, Algis/0000-0002-8626-5987 FU Los Alamos National Laboratory LDRD office [201202187ER] FX The authors are grateful for helpful discussions with Dr. Michael Malone. This work was supported by the Los Alamos National Laboratory LDRD office through Grant 201202187ER. NR 26 TC 1 Z9 1 U1 0 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0926-2040 EI 1527-3326 J9 SOLID STATE NUCL MAG JI Solid State Nucl. Magn. Reson. PD JUL-SEP PY 2014 VL 61-62 BP 35 EP 38 DI 10.1016/j.ssnmr.2014.05.002 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical; Physics, Condensed Matter; Spectroscopy SC Chemistry; Physics; Spectroscopy GA AL7HT UT WOS:000339305500006 PM 24882748 ER PT J AU Luo, ZP Dauter, M Dauter, Z AF Luo, Zhipu Dauter, Miroslawa Dauter, Zbigniew TI Phosphates in the Z-DNA dodecamer are flexible, but their P-SAD signal is sufficient for structure solution SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY LA English DT Article ID HANDED Z-DNA; X-RAY-DIFFRACTION; SINGLE-CRYSTAL STRUCTURE; 1.0-A ATOMIC RESOLUTION; PURE-SPERMINE FORM; DOUBLE-HELICAL DNA; BASE-PAIRS; MOLECULAR-STRUCTURE; ANGSTROM RESOLUTION; MINOR-GROOVE AB A large number of Z-DNA hexamer duplex structures and a few oligomers of different lengths are available, but here the first crystal structure of the d(CGCGCGCGCGCG)(2) dodecameric duplex is presented. Two synchrotron data sets were collected; one was used to solve the structure by the single-wavelength anomalous dispersion (SAD) approach based on the anomalous signal of P atoms, the other set, extending to an ultrahigh resolution of 0.75 angstrom, served to refine the atomic model to an R factor of 12.2% and an R-free of 13.4%. The structure consists of parallel duplexes arranged into practically infinitely long helices packed in a hexagonal fashion, analogous to all other known structures of Z-DNA oligomers. However, the dodecamer molecule shows a high level of flexibility, especially of the backbone phosphate groups, with six out of 11 phosphates modeled in double orientations corresponding to the two previously observed Z-DNA conformations: Z(I), with the phosphate groups inclined towards the inside of the helix, and Z(II), with the phosphate groups rotated towards the outside of the helix. C1 [Luo, Zhipu; Dauter, Zbigniew] NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne Natl Lab, Argonne, IL 60439 USA. [Dauter, Miroslawa] Argonne Natl Lab, Leidos Biomed Res Inc, Basic Res Program, Argonne, IL 60439 USA. RP Dauter, Z (reprint author), NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne Natl Lab, Argonne, IL 60439 USA. EM dauter@anl.gov RI Luo, Zhipu/P-9168-2014 FU NIH, National Cancer Institute, Center for Cancer Research; National Cancer Institute, National Institutes of Health [NO1-CO-12400]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38] FX This project was supported in part by the Intramural Research Program of the NIH, National Cancer Institute, Center for Cancer Research and with Federal funds from the National Cancer Institute, National Institutes of Health (Contract No. NO1-CO-12400). Diffraction data were collected at the NE-CAT beamline 24-ID and SER-CAT beamline 22-ID at the Advanced Photon Source, Argonne National Laboratory. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. W-31-109-Eng-38. NR 83 TC 9 Z9 9 U1 0 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1399-0047 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Biol. Crystallogr. PD JUL PY 2014 VL 70 BP 1790 EP 1800 DI 10.1107/S1399004714004684 PN 7 PG 11 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA AL1WM UT WOS:000338917000001 PM 25004957 ER PT J AU Dufek, EJ Lister, TE Stone, SG AF Dufek, Eric J. Lister, Tedd E. Stone, Simon G. TI Sampling dynamics for pressurized electrochemical cells SO JOURNAL OF APPLIED ELECTROCHEMISTRY LA English DT Article DE CO2; Electroreduction; Pressurized electrolysis; Syngas ID CARBON-DIOXIDE; CO2 REDUCTION; METAL-ELECTRODES; ELECTROLYTES; TEMPERATURE; PERFORMANCE; SELECTIVITY; OPERATION; DESIGN; II. AB A model describing the gas distribution within a constant pressure electrolysis system and how the distribution impacts electrochemical efficiencies is presented. The primary system of interest is the generation of syngas (CO and H-2) associated with the co-electrolysis of H2O and CO2. The model developed for this system takes into account the primary process variables of operation including total system pressure, applied current, and the in-flow of reactant gases. From these, and the chemical equilibria within the system, the impact on electrochemically generated gases is presented. Comparison of predicted and measured faradaic efficiency of an electrode's processes reveals significant disagreement under certain conditions. Methods to minimize and account for the discrepancy are presented with the goal of being able to discern, in a real-time manner, degradation of electrode performance. Comparison of the model to experimental data shows a strong correlation between the two with slight variation in experimental data, which is attributed to reversible system dynamics such as wetting of the gas diffusion electrode used as the cell cathode. C1 [Dufek, Eric J.; Lister, Tedd E.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Stone, Simon G.] Giner Inc, Newton, MA 02466 USA. RP Dufek, EJ (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM eric.dufek@inl.gov RI Dufek, Eric/B-8847-2017 OI Dufek, Eric/0000-0003-4802-1997 FU INL Laboratory Directed Research and Development (LDRD) Program under DOE Idaho Operations Office; U.S. Department of Energy [DE-AC07-05ID14517] FX Work supported through the INL Laboratory Directed Research and Development (LDRD) Program under DOE Idaho Operations Office. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 23 TC 0 Z9 0 U1 0 U2 11 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0021-891X EI 1572-8838 J9 J APPL ELECTROCHEM JI J. Appl. Electrochem. PD JUL PY 2014 VL 44 IS 7 BP 849 EP 855 DI 10.1007/s10800-014-0693-z PG 7 WC Electrochemistry SC Electrochemistry GA AK9QM UT WOS:000338761700010 ER PT J AU Philippov, A Tchekhovskoy, A Li, JG AF Philippov, Alexander Tchekhovskoy, Alexander Li, Jason G. TI Time evolution of pulsar obliquity angle from 3D simulations of magnetospheres SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE stars: magnetic field; stars: neutron; pulsars: general; stars: rotation ID FORCE-FREE MAGNETOSPHERE; MAGNETIC-FIELD; NEUTRON-STAR; MAGNETOHYDRODYNAMIC SIMULATIONS; NUMERICAL SCHEME; RADIO PULSARS; BLACK-HOLES; ALIGNMENT; POPULATION; PRECESSION AB The rotational period of isolated pulsars increases over time due to the extraction of angular momentum by electromagnetic torques. These torques also change the obliquity angle alpha between the magnetic and rotational axes. Although actual pulsar magnetospheres are plasma filled, the time evolution of alpha has mostly been studied for vacuum pulsar magnetospheres. In this work, we self-consistently account for the plasma effects for the first time by analysing the results of time-dependent 3D force-free and magnetohydrodynamic simulations of pulsar magnetospheres. We show that if a neutron star is spherically symmetric and is embedded with a dipolar magnetic moment, the pulsar evolves so as to minimize its spin-down luminosity: both vacuum and plasma-filled pulsars evolve towards the aligned configuration (alpha = 0). However, they approach the alignment in qualitatively different ways. Vacuum pulsars come into alignment exponentially fast, with alpha proportional to exp (-t/tau) and tau similar to spin-down time-scale. In contrast, we find that plasma-filled pulsars align much more slowly, with alpha proportional to (t/tau)(-1/2). We argue that the slow time evolution of obliquity of plasma-filled pulsars can potentially resolve several observational puzzles, including the origin of normal pulsars with periods of similar to 1 s, the evidence that oblique pulsars come into alignment over a time-scale of similar to 10(7) yr, and the observed deficit, relative to an isotropic obliquity distribution, of pulsars showing interpulse emission. C1 [Philippov, Alexander; Li, Jason G.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. RP Philippov, A (reprint author), Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. EM philippo@astro.princeton.edu FU Princeton Center for Theoretical Science; NASA [PF3-140115] FX We thank J. Arons, L. Arzamasskiy, V.S. Beskin, R. Blandford, C.-A. Faucher-Giguere, P. Goldreich, A. Jessner, R. Narayan, A. Spitkovsky, T. Tauris, D. Uzdensky and J. Zrake for insightful discussions. AT was supported by a Princeton Center for Theoretical Science Fellowship and by NASA through the Einstein Fellowship Program, grant PF3-140115. The simulations presented in this article used computational resources supported by the PICSciE-OIT High Performance Computing Center and Visualization Laboratory, and by XSEDE allocation TG-AST100040 on NICS Kraken and Nautilus and TACC Lonestar, Longhorn and Ranch. NR 41 TC 21 Z9 22 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 1 PY 2014 VL 441 IS 3 BP 1879 EP 1887 DI 10.1093/mnras/stu591 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK9RE UT WOS:000338763600003 ER PT J AU Chen, XH Chatterjee, R Zhang, HC Pohl, M Fossati, G Bottcher, M Bailyn, CD Bonning, EW Buxton, M Coppi, P Isler, J Maraschi, L Urry, M AF Chen, Xuhui Chatterjee, Ritaban Zhang, Haocheng Pohl, Martin Fossati, Giovanni Boettcher, Markus Bailyn, Charles D. Bonning, Erin W. Buxton, Michelle Coppi, Paolo Isler, Jedidah Maraschi, Laura Urry, Meg TI Magnetic field amplification and flat spectrum radio quasars SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE radiation mechanisms: non-thermal; galaxies: active; galaxies: jets; quasars: individual: PKS 0208-512 ID ACTIVE GALACTIC NUCLEI; TIME-DEPENDENT SIMULATIONS; RAPID NONTHERMAL FLARES; SELF-COMPTON MODEL; ENERGY-DISTRIBUTIONS; EXTERNAL COMPTON; PKS 1510-089; MULTIWAVELENGTH VARIABILITY; TURBULENT AMPLIFICATION; RELATIVISTIC SHOCK AB We perform time-dependent, spatially resolved simulations of blazar emission to evaluate several flaring scenarios related to magnetic-field amplification and enhanced particle acceleration. The code explicitly accounts for light-travel-time effects and is applied to flares observed in the flat spectrum radio quasar (FSRQ) PKS 0208-512, which show optical/gamma-ray correlation at some times, but orphan optical flares at other times. Changes in both the magnetic field and the particle acceleration efficiency are explored as causes of flares. Generally, external Compton (EC) emission appears to describe the available data better than a synchrotron self-Compton (SSC) scenario, and in particular orphan optical flares are difficult to produce in the SSC framework. X-ray soft-excesses, gamma-ray spectral hardening, and the detections at very high energies of certain FSRQs during flares find natural explanations in the EC scenario with particle acceleration change. Likewise, optical flares with/without gamma-ray counterparts can be explained by different allocations of energy between the magnetization and particle acceleration, which may be related to the orientation of the magnetic field relative to the jet flow. We also calculate the degree of linear polarization and polarization angle as a function of time for a jet with helical magnetic field. Tightening of the magnetic helix immediately downstream of the jet perturbations, where flares occur, can be sufficient to explain the increases in the degree of polarization and a rotation by a parts per thousand yen180A degrees of the observed polarization angle, if light-travel-time effects are properly considered. C1 [Chen, Xuhui; Pohl, Martin] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, Xuhui; Pohl, Martin] DESY, D-15738 Zeuthen, Germany. [Chatterjee, Ritaban] Presidency Univ, Dept Phys, Kolkata 700073, W Bengal, India. [Zhang, Haocheng; Boettcher, Markus] Ohio Univ, Inst Astrophys, Dept Phys & Astron, Athens, OH 45701 USA. [Zhang, Haocheng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Fossati, Giovanni] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Boettcher, Markus] North West Univ, Ctr Space Res, ZA-2520 Potchefstroom, South Africa. [Bailyn, Charles D.; Buxton, Michelle; Coppi, Paolo; Isler, Jedidah] Yale Univ, Dept Astron, New Haven, CT 06520 USA. [Bonning, Erin W.] Emory Univ, Dept Phys, Atlanta, GA 30322 USA. [Maraschi, Laura] INAFOsservatorio Astron Brera, I-20100 Milan, Italy. [Urry, Meg] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Urry, Meg] Yale Univ, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. RP Chen, XH (reprint author), Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. EM chenxuhui.phys@gmail.com OI Urry, Meg/0000-0002-0745-9792 FU Helmholtz Alliance for Astroparticle Physics HAP - Initiative and Networking Fund of the Helmholtz Association; NASA [NNX12AP20G, NNX12AE43G]; LANL/LDRD programme; DoE/Office of Fusion Energy Science through CMSO; Department of Science and Technology of South Africa; South African Research Chair Initiative of the National Research Foundation FX The authors thank A. Barnacka for useful discussions. XC and MP acknowledge support by the Helmholtz Alliance for Astroparticle Physics HAP funded by the Initiative and Networking Fund of the Helmholtz Association. HZ acknowledges supports by NASA through Fermi Guest Investigator Grant no. NNX12AP20G, and by the LANL/LDRD programme and by DoE/Office of Fusion Energy Science through CMSO. GF acknowledges support by NASA grant NNX12AE43G. MB acknowledges support through the South African Research Chair Initiative of the National Research Foundation and the Department of Science and Technology of South Africa. NR 51 TC 10 Z9 10 U1 0 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 1 PY 2014 VL 441 IS 3 BP 2188 EP 2199 DI 10.1093/mnras/stu713 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK9RE UT WOS:000338763600028 ER PT J AU Pasqualini, D Bassi, AM AF Pasqualini, D. Bassi, A. M. TI Oil shale and climate policy in the shift to a low carbon and more resilient economy SO TECHNOLOGICAL FORECASTING AND SOCIAL CHANGE LA English DT Article DE Climate policy; Oil shale; Integrated modeling; Energy development impacts; Unconventional fossil fuels ID ENERGY; GAS AB Policy makers worldwide are recently debating options to implement an effective climate policy that would put a cap on green house gas emissions. At the same time, investors are carefully evaluating the profitability of unconventional fossil fuels such as shale oil. To enhance the understanding of the impacts of a climate policy such as the American Clean Energy and Security Act of 2009, on oil shale production - and vice versa - we have customized an integrated assessment model, the Climate and Energy Assessment for Resiliency model for Unconventional Fossil Fuels to the U.S. Western Energy Corridor. Our analysis indicates that while the bill would increase the production cost of oil shale, the industry remains highly profitable in the longer-term, generating a potential profit of about $10 to $16 billion per year by 2040 at 2.5 million barrels per day. These results suggest that the oil shale industry may comfortably face the enactment of a carbon policy, albeit with some caveats. Furthermore, while its potential economic impact on non-compliant industries may be severe, it would generate mounting profits for those achieving energy efficiency gains, thereby increasing the profitability of energy efficiency investments. Published by Elsevier Inc. C1 [Pasqualini, D.] Los Alamos Natl Lab, Div Los Alamos D, Los Alamos, NM 87545 USA. [Bassi, A. M.] Millennium Inst, Arlington, VA 22201 USA. RP Pasqualini, D (reprint author), Los Alamos Natl Lab, Div Los Alamos D, Los Alamos, NM 87545 USA. EM dmp@lanl.gov NR 22 TC 0 Z9 0 U1 3 U2 14 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0040-1625 EI 1873-5509 J9 TECHNOL FORECAST SOC JI Technol. Forecast. Soc. Chang. PD JUL PY 2014 VL 86 BP 168 EP 176 DI 10.1016/j.techfore.2013.08.018 PG 9 WC Business; Planning & Development SC Business & Economics; Public Administration GA AL0JO UT WOS:000338813400015 ER PT J AU Zhi, MJ Yang, F Meng, FK Li, MQ Manivannan, A Wu, NQ AF Zhi, Mingjia Yang, Feng Meng, Fanke Li, Minqi Manivannan, Ayyakkannu Wu, Nianqiang TI Effects of Pore Structure on Performance of An Activated-Carbon Supercapacitor Electrode Recycled from Scrap Waste Tires SO ACS SUSTAINABLE CHEMISTRY & ENGINEERING LA English DT Article DE Activated carbon; Waste tire; Supercapacitor; Electrode; Porous material ID DOUBLE-LAYER CAPACITANCE; COAL-TAR PITCH; ENERGY-STORAGE; KOH ACTIVATION; POROUS CARBONS; TEMPLATE; BLACK AB It is important to address the challenges posed with the ever-increasing demand for energy supply and environmental sustainability. Activated carbon, which is the common material for commercial supercapadtor electrodes, is currently derived from petroleum-based precursors. This paper presents an effective synthetic method that utilizes waste tires as the precursor to prepare the activated carbon electrodes by the pyrolysis and chemical activation processes. Adjusting the activation parameters can tailor multiple physical properties of the resulting activated carbon, which in turns tunes the performance of the activated carbon electrode. Statistical multiple linear regression and stepwise regression methods are employed to investigate the dependence of the specific capacitance and the rate capability upon the physical properties (such as porosity) of the activated carbon electrode. The specific capacitance of activated carbon electrode is controlled by the micropore volume but independent of the mesopores volume. The rate capability is dominated by the mesopore/micropore volume ratio instead of the absolute value of mesopore volume. C1 [Zhi, Mingjia] Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China. [Zhi, Mingjia; Meng, Fanke; Manivannan, Ayyakkannu; Wu, Nianqiang] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Yang, Feng; Li, Minqi] W Virginia Univ, Ind & Management Syst Engn Dept, Morgantown, WV 26506 USA. [Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Wu, NQ (reprint author), W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. EM nick.wu@mail.wvu.edu RI Meng, Fanke /F-3978-2010; Zhi, Mingjia/A-6866-2010; Wu, Nianqiang/B-9798-2015; Meng, Fanke/D-7395-2017 OI Zhi, Mingjia/0000-0002-4291-0809; Wu, Nianqiang/0000-0002-8888-2444; Meng, Fanke/0000-0001-7961-4248 FU NSF [CMMI-1068131] FX F.Y. is grateful for partial support by NSF grant (CMMI-1068131). The use of the WVU Shared Facility is appreciated. The authors thank Mr. J. Bright, S. Hao, and P. Zheng for their assistance with XPS, Raman, and FTIR analysis. NR 32 TC 45 Z9 47 U1 18 U2 119 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2168-0485 J9 ACS SUSTAIN CHEM ENG JI ACS Sustain. Chem. Eng. PD JUL PY 2014 VL 2 IS 7 BP 1592 EP 1598 DI 10.1021/sc500336h PG 7 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Chemical SC Chemistry; Science & Technology - Other Topics; Engineering GA AK9LK UT WOS:000338748400008 ER PT J AU Danalis, A Luszczek, P Marin, G Vetter, JS Dongarra, J AF Danalis, Anthony Luszczek, Piotr Marin, Gabriel Vetter, Jeffrey S. Dongarra, Jack TI BlackjackBench: Portable Hardware Characterization with Automated Results' Analysis SO COMPUTER JOURNAL LA English DT Article DE micro-benchmarks; hardware characterization; statistical analysis ID PERFORMANCE; CACHE; ACCURATE; SOFTWARE AB DARPA's AACE project aimed to develop Architecture Aware Compiler Environments. Such a compiler automatically characterizes the targeted hardware and optimizes the application codes accordingly. We present the BlackjackBench suite, a collection of portable micro-benchmarks that automate system characterization, plus statistical analysis techniques for interpreting the results. The BlackjackBench benchmarks discover the effective sizes and speeds of the hardware environment rather than the often unattainable peak values. We aim at hardware characteristics that can be observed by running executables generated by existing compilers from standard C codes. We characterize the memory hierarchy, including cache sharing and non-uniform memory access characteristics of the system, properties of the processing cores affecting the instruction execution speed and the length of the operating system scheduler time slot. We show how these features of modern multicores can be discovered programmatically. We also show how the features could potentially interfere with each other resulting in incorrect interpretation of the results, and how established classification and statistical analysis techniques can reduce experimental noise and aid automatic interpretation of results. We show how effective hardware metrics from our probes allow guided tuning of computational kernels that outperform an autotuning library further tuned by the hardware vendor. C1 [Danalis, Anthony; Luszczek, Piotr; Dongarra, Jack] Univ Tennessee, Knoxville, TN 37996 USA. [Marin, Gabriel; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Luszczek, P (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM luszczek@eecs.utk.edu NR 23 TC 0 Z9 0 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0010-4620 EI 1460-2067 J9 COMPUT J JI Comput. J. PD JUL PY 2014 VL 57 IS 7 BP 1002 EP 1016 DI 10.1093/comjnl/bxt057 PG 15 WC Computer Science, Hardware & Architecture; Computer Science, Information Systems; Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA AK8AG UT WOS:000338648900005 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglionia, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Balek, P Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, AK Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Behera, PK Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S 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Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brown, G Brown, H de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buescher, V Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Capasso, L Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, B Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP 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CA ATLAS Collaboration TI The differential production cross section of the phi(1020) meson in root s=7 TeV pp collisions measured with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID FRAGMENTATION AB A measurement is presented of the phi x BR(phi -> K+ K-) production cross section at root s = 7 TeV using pp collision data corresponding to an integrated luminosity of 383 mu b(-1), collected with the ATLAS experiment at the LHC. Selection of phi(1020) mesons is based on the identification of charged kaons by their energy loss in the pixel detector. The differential cross section is measured as a function of the transverse momentum, pT, phi, and rapidity, y(phi), of the phi(1020) meson in the fiducial region 500 < pT,phi < 1200MeV, vertical bar y phi| < 0.8, kaon p(T), (K) > 230 MeV and kaon momentum p(K) < 800 MeV. 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[Bertin, A.; Bindi, M.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Grafstrom, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartmento Fis, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Schaepe, S.; Schmieden, K.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Subramaniam, R.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Garzon, G. Otero Y.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Lacey, J.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Chavez Barajas, C. A.; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Henriques Correia, A. M.; Hervas, L.; Hoecker, A.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Roda Dos Santos, D.; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Pino, S. A. Olivares; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wu, Y.; Xu, C.; Xu, L.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Perez Reale, V.; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; Bruckman de Renstrom, P. A.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Goncalves Pinto Firmino Da Costa, J.; Grahn, K. -J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Jimenez Belenguer, M.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Goncalves Pinto Firmino Da Costa, J.; Grahn, K. -J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Jimenez Belenguer, M.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Cerutti, F.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Ferretto Parodi, A.; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Ferretto Parodi, A.; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; Ferreira de Lima, D. E.; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M. -L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M. -L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M. -L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Barreiro Guimares da Costa, J.; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Lopez Mateos, D.; Martinez Outschoorn, V.; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Panduro Vazquez, J. G.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Robertson, S. H.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M. -A.; Klemetti, M.; Mc Donald, J.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Alvarez Gonzalez, B.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Baranov, S. P.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; Rocha de Lima, J. G.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; Van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lorenzo Martinez, N.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lorenzo Martinez, N.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Di Donato, C.; Dressnandt, N.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarriab, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarriab, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Munio, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Manjarres Ramos, J. A.; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.] Commissariat Energie Atom, CEA Saclay, Inst Rech Lois Fondamentales Univers, DSM IRFU, Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Cuhadar Donszelmann, T.; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellmanab, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellmanab, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Abramowicz, H.; Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Perez Codina, E.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Benitez Garcia, J. A.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Farrell, S.; Gough Eschrich, I.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Milan, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. 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J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. 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[Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Dobson, E.] UCL, Dept Phys & Astron, London, England. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, S.] Aix Marseille Univ, CPPM, Marseille, France. [Li, S.] CNRS IN2P3, Marseille, France. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Meng, Z.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Mountricha, E.; Xu, C.] Commissariat Energie Atom, CEA Saclay, Inst Rech Lois Fondamentales Univers, DSM IRFU, Gif Sur Yvette, France. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Ruan, X.] Univ Paris 11, LAL, Orsay, France. [Ruan, X.] CNRS IN2P3, Orsay, France. [Spousta, M.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Tsionou, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wu, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Zhang, D.] Acad Sinica, Inst Phys, Taipei, Taiwan. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Moorhead, Gareth/B-6634-2009; Bosman, Martine/J-9917-2014; Fazio, Salvatore /G-5156-2010; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Warburton, Andreas/N-8028-2013; Kuday, Sinan/C-8528-2014; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Peleganchuk, Sergey/J-6722-2014; Ferrando, James/A-9192-2012; Santamarina Rios, Cibran/K-4686-2014; Alexa, Calin/F-6345-2010; Kuleshov, Sergey/D-9940-2013; Lokajicek, Milos/G-7800-2014; Castro, Nuno/D-5260-2011; Staroba, Pavel/G-8850-2014; Doyle, Anthony/C-5889-2009; de Groot, Nicolo/A-2675-2009; Wemans, Andre/A-6738-2012; Nemecek, Stanislav/G-5931-2014; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Samset, Bjorn H./B-9248-2012; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Canelli, Florencia/O-9693-2016; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015 OI Moorhead, Gareth/0000-0002-9299-9549; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Kuday, Sinan/0000-0002-0116-5494; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Peleganchuk, Sergey/0000-0003-0907-7592; Ferrando, James/0000-0002-1007-7816; Santamarina Rios, Cibran/0000-0002-9810-1816; Kuleshov, Sergey/0000-0002-3065-326X; Castro, Nuno/0000-0001-8491-4376; Doyle, Anthony/0000-0001-6322-6195; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Samset, Bjorn H./0000-0001-8013-1833; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Canelli, Florencia/0000-0001-6361-2117; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; MOST; NSFC, China; COLCIEN-CIAS, Colombia; MSMT CR; MPO CR; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT; NSRF, Greece; ISF; MINERVA; GIF; DIP; Benoziyo Center, Israel; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, The Netherlands; BRF; RCN, Norway; MNiSW, Poland; GRICES; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC; Wallenberg Foundation, Sweden; SER; SNSF; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC; Royal Society; Leverhulme Trust, United Kingdom; DOE; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIEN-CIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, The Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (The Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 24 TC 4 Z9 4 U1 9 U2 111 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 1 PY 2014 VL 74 IS 7 AR 2895 DI 10.1140/epjc/s10052-014-2895-2 PG 21 WC Physics, Particles & Fields SC Physics GA AK9AG UT WOS:000338719300001 ER PT J AU Parks, DA Tittmann, BR AF Parks, David A. Tittmann, Bernhard R. TI Radiation Tolerance of Piezoelectric Bulk Single-Crystal Aluminum Nitride SO IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL LA English DT Article ID NEUTRON-IRRADIATION; AMORPHIZATION; CERAMICS; REACTOR; DAMAGE AB For practical use in harsh radiation environments, we pose selection criteria for piezoelectric materials for non-destructive evaluation (NDE) and material characterization. Using these criteria, piezoelectric aluminum nitride is shown to be an excellent candidate. The results of tests on an aluminum-nitride-based transducer operating in a nuclear reactor are also presented. We demonstrate the tolerance of single-crystal piezoelectric aluminum nitride after fast and thermal neutron fluences of 1.85 x 10(18) neutron/cm(2) and 5.8 x 10(18) neutron/cm(2), respectively, and a gamma dose of 26.8 MGy. The radiation hardness of AlN is most evident from the unaltered piezoelectric coefficient d(33), which measured 5.5 pC/N after a fast and thermal neutron exposure in a nuclear reactor core for over 120 MWh, in agreement with the published literature value. The results offer potential for improving reactor safety and furthering the understanding of radiation effects on materials by enabling structural health monitoring and NDE in spite of the high levels of radiation and high temperatures, which are known to destroy typical commercial ultrasonic transducers. C1 [Parks, David A.] Idaho Natl Lab, NDE Phys Dept, Idaho Falls, ID 83402 USA. [Tittmann, Bernhard R.] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16802 USA. RP Parks, DA (reprint author), Idaho Natl Lab, NDE Phys Dept, Idaho Falls, ID 83402 USA. EM brt4@psu.edu NR 23 TC 10 Z9 10 U1 3 U2 28 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-3010 EI 1525-8955 J9 IEEE T ULTRASON FERR JI IEEE Trans. Ultrason. Ferroelectr. Freq. Control PD JUL PY 2014 VL 61 IS 7 BP 1216 EP 1222 DI 10.1109/TUFFC.2014.3020 PG 7 WC Acoustics; Engineering, Electrical & Electronic SC Acoustics; Engineering GA AK8GM UT WOS:000338665500014 PM 24960710 ER PT J AU Eberhart, CJ Lineberry, DM Frederick, RA Kastengren, AL AF Eberhart, Chad J. Lineberry, David M. Frederick, Robert A., Jr. Kastengren, Alan L. TI Mechanistic Assessment of Swirl Coaxial Injection by Quantitative X-Ray Radiography SO JOURNAL OF PROPULSION AND POWER LA English DT Article ID DYNAMICS; SPRAYS AB Detailed x-ray radiographic experiments were conducted to evaluate the time-averaged spray characteristics of a liquid rocket swirl injector. Sprays issued from a single liquid-centered swirl coaxial element - with and without coannular gas flow - were exposed to focused, monochromatic x rays produced by a synchrotron light source. Two-dimensional attenuation data are presented at various axial stations and reveal both projected mass distribution of liquid in the injector near field and mass-weighted axial velocity integrated over time. Measurements describing spray morphology are also inferred from the x-ray data and compared with those measured through objective image processing of visible light imagery. The gas flow is observed to reduce spray cone angle up to 50% and increase liquid film thickness up to 20% in the near field. Measurements compare well with those extracted from imagery of the pressure-swirl spray; however, the x-ray technique is more robust in resolving liquid film thickness for the optically dense swirl coaxial spray. C1 [Eberhart, Chad J.; Frederick, Robert A., Jr.] Univ Alabama, Dept Mech & Aerosp Engn, Huntsville, AL 35899 USA. [Lineberry, David M.] Univ Alabama, Prop Res Ctr, Huntsville, AL 35899 USA. [Kastengren, Alan L.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Eberhart, CJ (reprint author), Univ Alabama, Dept Mech & Aerosp Engn, S225 Technol Hall, Huntsville, AL 35899 USA. FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-O6CH11375] FX The authors would like to thank Alex Schumaker, Malissa Lightfoot, and Steve Danczyk of the U.S. Air Force Research Laboratory for facilitating the opportunity to conduct the x-ray radiographic portion of this work, for productive discussion, and for guidance with data processing. The authors would also like to thank Chris Powell of Argonne National Laboratory, Daniel Duke of Monash University, and William Miller of Kettering University for assistance with collection of the x-ray radiography data. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-O6CH11375. This research was conducted under the University of Alabama in Huntsville's Wernher von Braun Propulsion Fellowship. NR 29 TC 2 Z9 2 U1 0 U2 2 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0748-4658 EI 1533-3876 J9 J PROPUL POWER JI J. Propul. Power PD JUL-AUG PY 2014 VL 30 IS 4 BP 1070 EP 1079 DI 10.2514/1.B35007 PG 10 WC Engineering, Aerospace SC Engineering GA AK9DD UT WOS:000338726800020 ER PT J AU Liu, XW Dekker, LJM Wu, S Vanduijn, MM Luider, TM Tolic, N Kou, Q Dvorkin, M Alexandrova, S Vyatkina, K Pasa-Tolic, L Pevzner, PA AF Liu, Xiaowen Dekker, Lennard J. M. Wu, Si Vanduijn, Martijn M. Luider, Theo M. Tolic, Nikola Kou, Qiang Dvorkin, Mikhail Alexandrova, Sonya Vyatkina, Kira Pasa-Tolic, Ljiljana Pevzner, Pavel A. TI De Novo Protein Sequencing by Combining Top-Down and Bottom-Up Tandem Mass Spectra SO JOURNAL OF PROTEOME RESEARCH LA English DT Article ID MONOCLONAL-ANTIBODIES; SPECTROMETRY; IDENTIFICATION; PEPTIDES; PROTEOMICS; DATABASE; MIXTURES; MS/MS AB There are two approaches for de novo protein sequencing: Edman degradation and mass spectrometry (MS). Existing MS-based methods characterize a novel protein by assembling tandem mass spectra of overlapping peptides generated from multiple proteolytic digestions of the protein. Because each tandem mass spectrum covers only a short peptide of the target protein, the key to high coverage protein sequencing is to find spectral pairs from overlapping peptides in order to assemble tandem mass spectra to long ones. However, overlapping regions of peptides may be too short to be confidently identified. High-resolution mass spectrometers have become accessible to many laboratories. These mass spectrometers are capable of analyzing molecules of large mass values, boosting the development of top-down MS. Top-down tandem mass spectra cover whole proteins. However, top-down tandem mass spectra, even combined, rarely provide full ion fragmentation coverage of a protein. We propose an algorithm, TBNovo, for de novo protein sequencing by combining top-down and bottom-up MS. In TBNovo, a top-down tandem mass spectrum is utilized as a scaffold, and bottom-up tandem mass spectra are aligned to the scaffold to increase sequence coverage. Experiments on data sets of two proteins showed that TBNovo achieved high sequence coverage and high sequence accuracy. C1 [Liu, Xiaowen; Kou, Qiang] Indiana Univ Purdue Univ, Dept BioHlth Informat, Indianapolis, IN 46202 USA. [Liu, Xiaowen] Indiana Univ Sch Med, Ctr Computat Biol & Bioinformat, Indianapolis, IN 46202 USA. [Dekker, Lennard J. M.; Vanduijn, Martijn M.; Luider, Theo M.] Erasmus MC, Dept Neurol, NL-3000 CA Rotterdam, Netherlands. [Wu, Si; Tolic, Nikola; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Dvorkin, Mikhail; Alexandrova, Sonya; Vyatkina, Kira] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg 194021, Russia. [Pevzner, Pavel A.] Univ Calif San Diego, Dept Comp Sci & Engn, San Diego, CA 92093 USA. RP Liu, XW (reprint author), Indiana Univ Purdue Univ, Dept BioHlth Informat, 535 West Michigan St,IT 475, Indianapolis, IN 46202 USA. EM xwliu@iupui.edu; ppevzner@cs.ucsd.edu OI van Duijn, Martijn/0000-0002-6654-994X FU Indiana University-Purdue University Indianapolis; Netherlands Organization for Scientific Research (NWO), Zenith grant [93511034]; DOE [DE-AC05-76RLO1830]; Government of the Russian Federation [11.G34.31.0018] FX This work was supported by a startup fund provided by Indiana University-Purdue University Indianapolis. L.J.M.D. and M.M.V. are financially supported by The Netherlands Organization for Scientific Research (NWO), Zenith grant no. 93511034. Portions of this work were performed in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a Department of Energy, Biological and Environmental Research (DOE BER) national scientific user facility located on the campus of Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is a multiprogram national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RLO1830. M.D., S.A, K.V., and P.A.P. were partially supported by the Government of the Russian Federation (grant 11.G34.31.0018). NR 33 TC 17 Z9 17 U1 4 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1535-3893 EI 1535-3907 J9 J PROTEOME RES JI J. Proteome Res. PD JUL PY 2014 VL 13 IS 7 BP 3241 EP 3248 DI 10.1021/pr401300m PG 8 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA AK8QP UT WOS:000338693400011 PM 24874765 ER PT J AU Aryal, UK Callister, SJ McMahon, BH McCue, LA Brown, J Stockel, J Liberton, M Mishra, S Zhang, XH Nicora, CD Angel, TE Koppenaal, DW Smith, RD Pakrasi, HB Sherman, LA AF Aryal, Uma K. Callister, Stephen J. McMahon, Benjamin H. McCue, Lee-Ann Brown, Joseph Stoeckel, Jana Liberton, Michelle Mishra, Sujata Zhang, Xiaohui Nicora, Carrie D. Angel, Thomas E. Koppenaal, David W. Smith, Richard D. Pakrasi, Himadri B. Sherman, Louis A. TI Proteomic Profiles of Five Strains of Oxygenic Photosynthetic Cyanobacteria of the Genus Cyanothece SO JOURNAL OF PROTEOME RESEARCH LA English DT Article DE Cyanobacteria; Cyanothece; orthologues; photosynthesis; N-2 fixation; H-2 production; proteome ID MULTIPLE SEQUENCE ALIGNMENT; LIGHT-DARK; ATCC 51142; PHOTOSYSTEM-I; GENOME; MASS; ATCC-51142; STRATEGY; CULTURES; SPECTRA AB Members of the cyanobacterial genus Cyanothece exhibit considerable variation in physiological and biochemical characteristics. The comparative assessment of the genomes and the proteomes has the potential to provide insights on differences among Cyanothece strains. By applying Sequedex, an annotation-independent method for ascribing gene functions, we confirmed significant species-specific differences of functional genes in different Cyanothece strains, particularly in Cyanothece PCC7425. Using a shotgun proteomics approach based on prefractionation and tandem mass spectrometry, we detected similar to 28-48% of the theoretical Cyanothece proteome, depending on the strain. The expression of a total of 642 orthologous proteins was observed in all five Cyanothece strains. These shared orthologous proteins showed considerable correlations in their abundances across different Cyanothece strains. Functional classification indicated that the majority of proteins involved in central metabolic functions such as amino acid, carbohydrate, protein, and RNA metabolism, photosynthesis, respiration, and stress responses were observed to a greater extent in the core proteome, whereas proteins involved in membrane transport, iron acquisition, regulatory functions, flagellar motility, and chemotaxis were observed to a greater extent in the unique proteome. Considerable differences were evident across different Cyanothece strains. Notably, the analysis of Cyanothece PCC7425, which showed the highest number of unique proteins (682), provided direct evidence of evolutionary differences in this strain. We conclude that Cyanothece PCC7425 diverged significantly from the other Cyanothece strains or evolved from a different lineage. C1 [Aryal, Uma K.; Callister, Stephen J.; McCue, Lee-Ann; Brown, Joseph; Nicora, Carrie D.; Angel, Thomas E.; Koppenaal, David W.; Smith, Richard D.] Pacific NW Natl Lab, Richland, WA 99352 USA. [McMahon, Benjamin H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Stoeckel, Jana; Liberton, Michelle; Pakrasi, Himadri B.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Mishra, Sujata; Zhang, Xiaohui; Sherman, Louis A.] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. [Angel, Thomas E.] Kinemed Inc, Emeryville, CA 94608 USA. [Stoeckel, Jana] MOgene Green Chem LC, St Louis, MO 63132 USA. RP Sherman, LA (reprint author), Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. EM lsherman@purdue.edu RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; McCue, Lee Ann/0000-0003-4456-517X FU DOE [DE-AC05-76RL01830]; Pan-omics program; DOE Genomics GTL program [DE 09-19 PO 2905402N]; Office of Science (BER), U.S. Department of Energy FX This work was part of a Membrane Biology Scientific Grand Challenge (MBGC) project at the W.R. Wiley Environmental Molecular Science Laboratory (EMSL). The Environmental Molecular Sciences Laboratory is a U.S. Department of Energy (DOE) Office of Biological and Environmental Research national scientific user facility on the Pacific Northwest National Laboratory (PNNL) campus. PNNL is a multiprogram national laboratory operated by Battelle for the DOE under contract DE-AC05-76RL01830. This work was supported in part by the Pan-omics program and a grant from the DOE Genomics GTL program (DE 09-19 PO 2905402N) and by funding from the Office of Science (BER), U.S. Department of Energy to Drs. Pakrasi and Sherman. NR 45 TC 4 Z9 5 U1 3 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1535-3893 EI 1535-3907 J9 J PROTEOME RES JI J. Proteome Res. PD JUL PY 2014 VL 13 IS 7 BP 3262 EP 3276 DI 10.1021/pr5000889 PG 15 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA AK8QP UT WOS:000338693400013 PM 24846609 ER PT J AU Wu, GA Prochnik, S Jenkins, J Salse, J Hellsten, U Murat, F Perrier, X Ruiz, M Scalabrin, S Terol, J Takita, MA Labadie, K Poulain, J Couloux, A Jabbari, K Cattonaro, F Del Fabbro, C Pinosio, S Zuccolo, A Chapman, J Grimwood, J Tadeo, FR Estornell, LH Munoz-Sanz, JV Ibanez, V Herrero-Ortega, A Aleza, P Perez-Perez, J Ramon, D Brunel, D Luro, F Chen, CX Farmerie, WG Desany, B Kodira, C Mohiuddin, M Harkins, T Fredrikson, K Burns, P Lomsadze, A Borodovsky, M Reforgiato, G Freitas-Astua, J Quetier, F Navarro, L Roose, M Wincker, P Schmutz, J Morgante, M Machado, MA Talon, M Jaillon, O Ollitrault, P Gmitter, F Rokhsar, D AF Wu, G. Albert Prochnik, Simon Jenkins, Jerry Salse, Jerome Hellsten, Uffe Murat, Florent Perrier, Xavier Ruiz, Manuel Scalabrin, Simone Terol, Javier Takita, Marco Aurelio Labadie, Karine Poulain, Julie Couloux, Arnaud Jabbari, Kamel Cattonaro, Federica Del Fabbro, Cristian Pinosio, Sara Zuccolo, Andrea Chapman, Jarrod Grimwood, Jane Tadeo, Francisco R. Estornell, Leandro H. Munoz-Sanz, Juan V. Ibanez, Victoria Herrero-Ortega, Amparo Aleza, Pablo Perez-Perez, Julian Ramon, Daniel Brunel, Dominique Luro, Francois Chen, Chunxian Farmerie, William G. Desany, Brian Kodira, Chinnappa Mohiuddin, Mohammed Harkins, Tim Fredrikson, Karin Burns, Paul Lomsadze, Alexandre Borodovsky, Mark Reforgiato, Giuseppe Freitas-Astua, Juliana Quetier, Francis Navarro, Luis Roose, Mikeal Wincker, Patrick Schmutz, Jeremy Morgante, Michele Machado, Marcos Antonio Talon, Manuel Jaillon, Olivier Ollitrault, Patrick Gmitter, Frederick Rokhsar, Daniel TI Sequencing of diverse mandarin, pummelo and orange genomes reveals complex history of admixture during citrus domestication SO NATURE BIOTECHNOLOGY LA English DT Article ID SINENSIS L. OSBECK; HORT. EX TAN.; MOLECULAR MARKERS; ORIGIN; CLEMENTINA; RUTACEAE; ORGANIZATION; EVOLUTION; SSRS; MAP AB Cultivated citrus are selections from, or hybrids of, wild progenitor species whose identities and contributions to citrus domestication remain controversial. Here we sequence and compare citrus genomes-a high-quality reference haploid clementine genome and mandarin, pummelo, sweet-orange and sour-orange genomes- and show that cultivated types derive from two progenitor species. Although cultivated pummelos represent selections from one progenitor species, Citrus maxima, cultivated mandarins are introgressions of C. maxima into the ancestral mandarin species Citrus reticulata. The most widely cultivated citrus, sweet orange, is the offspring of previously admixed individuals, but sour orange is an F1 hybrid of pure C. maxima and C. reticulata parents, thus implying that wild mandarins were part of the early breeding germplasm. A Chinese wild 'mandarin' diverges substantially from C. reticulata, thus suggesting the possibility of other unrecognized wild citrus species. Understanding citrus phylogeny through genome analysis clarifies taxonomic relationships and facilitates sequence-directed genetic improvement. C1 [Wu, G. Albert; Prochnik, Simon; Hellsten, Uffe; Chapman, Jarrod; Rokhsar, Daniel] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Jenkins, Jerry; Grimwood, Jane; Schmutz, Jeremy] HudsonAlpha Biotechnol Inst, Huntsville, AL USA. [Salse, Jerome; Murat, Florent] UBA, INRA, UMR Genet Diversite Ecophysiol Cereales GDEC 1095, Clermont Ferrand, France. [Perrier, Xavier; Ruiz, Manuel; Ollitrault, Patrick] Ctr Cooperat Int Rech Agronom Dev CIRAD, UMR Arneliorat Genet & Adaptat Plantes Mediterran, Montpellier, France. [Scalabrin, Simone; Cattonaro, Federica; Del Fabbro, Cristian; Pinosio, Sara; Zuccolo, Andrea; Morgante, Michele] Ist Genom Applicata, Udine, Italy. [Terol, Javier; Tadeo, Francisco R.; Estornell, Leandro H.; Munoz-Sanz, Juan V.; Ibanez, Victoria; Herrero-Ortega, Amparo; Talon, Manuel] IVIA, Ctr Genom, Valencia, Spain. [Takita, Marco Aurelio; Freitas-Astua, Juliana; Machado, Marcos Antonio] Inst Agron IAC, Ctr Citricultura Sylvio Moreira, Cordeiropolis, Brazil. [Labadie, Karine; Poulain, Julie; Couloux, Arnaud; Jabbari, Kamel; Brunel, Dominique; Quetier, Francis; Wincker, Patrick; Jaillon, Olivier] Genoscope, CEA, IG, Evry, France. [Zuccolo, Andrea] Scuola Super Sant Anna, Inst Life Sci, Pisa, Italy. [Aleza, Pablo; Navarro, Luis] Inst Valenciano Invest Agr, Ctr Protecc Vegetal & Biotecnol, E-46113 Moncada, Spain. [Perez-Perez, Julian; Ramon, Daniel] Lifesequencing, Valencia, Spain. [Perez-Perez, Julian] Secugen, Madrid, Spain. [Brunel, Dominique] INRA, US Etude Polymorphisme Genomes Vegetaux EPGV 1279, Evry, France. [Luro, Francois] INRA Genete & Ecophysiol Qualite Agrumes GEQA, San Giuliano, France. [Chen, Chunxian; Gmitter, Frederick] Univ Florida, CREC, IFAS, Lake Alfred, FL USA. [Farmerie, William G.] Univ Florida, Interdisciplinary Ctr Biotechnol Res, Gainesville, FL USA. [Desany, Brian; Kodira, Chinnappa; Mohiuddin, Mohammed; Harkins, Tim; Fredrikson, Karin] Roche, Life Sci 454, Branford, CT USA. [Burns, Paul; Lomsadze, Alexandre; Borodovsky, Mark] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. [Burns, Paul; Lomsadze, Alexandre; Borodovsky, Mark] Georgia Inst Technol, Sch Computat Sci & Engn, Atlanta, GA 30332 USA. [Borodovsky, Mark] Moscow Inst Phys & Technol, Dept Biol & Med Phys, Dolgoprudnyi, Russia. [Reforgiato, Giuseppe] Consiglio Ric & Sperimentaz Agr CRA ACM, Acireale, Italy. [Freitas-Astua, Juliana] Embrapa Cassava & Fruits, Cruz Das Almas, Brazil. [Quetier, Francis; Wincker, Patrick; Jaillon, Olivier] Univ Evry, Dept Biol, Evry, France. [Roose, Mikeal] Univ Calif Riverside, Dept Bot & Plant Sci, Riverside, CA 92521 USA. [Wincker, Patrick; Jaillon, Olivier] CNRS, Evry, France. [Morgante, Michele] Univ Udine, Dept Agr & Environm Sci, I-33100 Udine, Italy. [Rokhsar, Daniel] Univ Calif Berkeley, Div Genet Genom & Dev, Berkeley, CA 94720 USA. RP Rokhsar, D (reprint author), US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. EM fgmitter@ufl.edu; dsrokhsar@gmail.com RI Del Fabbro, Cristian/C-5523-2014; Navarro, Luis/D-1001-2012; Aleza, Pablo/M-3710-2014; Tadeo, Francisco/C-8977-2014; Terol, Javier/H-6401-2013; Talon, Manuel/C-8540-2014; Freitas-Astua, Juliana/C-5833-2013 OI Del Fabbro, Cristian/0000-0001-8189-6192; Navarro, Luis/0000-0001-5163-5960; MUNOZ-SANZ, JUAN VICENTE/0000-0002-6752-7398; Aleza, Pablo/0000-0002-8936-1448; Tadeo, Francisco/0000-0002-5839-4255; Terol, Javier/0000-0003-3345-0078; Talon, Manuel/0000-0003-4291-9333; Freitas-Astua, Juliana/0000-0002-0506-6880 FU National Science and Technology Institute of Genomics for Citrus Breeding, Brazil [FAPESP 08/57909-2, CNPq 573848/08-4]; Brazilian Agricultural Research Corporation (Embrapa); Embrapa-Monsanto Agreement; Agence Nationale de la Recherche (ANR) [CITRUSSEQ PCS-08-GENO]; program ANR Blanc-PAGE [ANR-2011-BSV6-00801]; US National Institutes of Health [HG00783]; Generalitat Valenciana, Spain [PrometeoII/2013/008]; Ministry of Economy and Innovation-Fondo Europeo de Desarrollo Regional (FEDER), Spain [AGL2011-26490]; Conselleria de Agricultura, Pesca, Alimentacion y Agua from the Generalitat Valenciana; Ministerio de Economia e Innovacion [PSE-060000-2009-8, IPT-010000-2010-43]; Citruseq-Citrusgenn consortium company (Anecoop S. Coop., Eurosemillas S.A.); Citruseq-Citrusgenn consortium company (Fundacion Ruralcaja Valencia); Citruseq-Citrusgenn consortium company (GCM Variedades Vegetales A.I.E.); Citruseq-Citrusgenn consortium company ( Investigacion Citricola Castellon S.A.); Citruseq-Citrusgenn consortium company (Source Citrus Genesis-Special New Fruit Licensing, Ltd.); Florida Citrus Production Research Advisory Council (FCPRAC); Florida Department of Agriculture and Consumer Services [013646]; Florida Department of Citrus (FDOC); Citrus Research and Development Foundation [71]; Ministero delle Politiche Agricole Alimentari e Forestali, Project Citrustart; Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Programma Operativo Nazionale 'Ricerca e Competitivita', Project IT-Citrus Genomics [PON_01623]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge the following support: National Science and Technology Institute of Genomics for Citrus Breeding, Brazil, grants FAPESP 08/57909-2 and CNPq 573848/08-4, and Brazilian Agricultural Research Corporation (Embrapa) (M. A. T. and M. A. M.) and Embrapa-Monsanto Agreement (J.F.-A.); Agence Nationale de la Recherche (ANR) grant CITRUSSEQ PCS-08-GENO (O.J., X. P., M. Ruiz, P.O., F. L., D. B. and K.J.) and program ANR Blanc-PAGE, ref. ANR-2011-BSV6-00801 (J. Salse and F. M.); US National Institutes of Health grant HG00783 (M. B., P. B. and A. L.); Generalitat Valenciana, Spain grant PrometeoII/2013/008 and Ministry of Economy and Innovation-Fondo Europeo de Desarrollo Regional (FEDER), Spain, grant AGL2011-26490 (P. A. and L.N.); Conselleria de Agricultura, Pesca, Alimentacion y Agua from the Generalitat Valenciana (J. P.-P. and D. Ramon); Ministerio de Economia e Innovacion grants PSE-060000-2009-8 and IPT-010000-2010-43 and Citruseq-Citrusgenn consortium companies (Anecoop S. Coop., Eurosemillas S.A., Fundacion Ruralcaja Valencia, GCM Variedades Vegetales A.I.E., Investigacion Citricola Castellon S.A. and Source Citrus Genesis-Special New Fruit Licensing, Ltd.) (J. T., F. R. T., L. H. E., J.V.M.-S., V. I., A.H.-O. and M. T.); Florida Citrus Production Research Advisory Council (FCPRAC), Florida Department of Agriculture and Consumer Services grant no. 013646, Florida Department of Citrus (FDOC) and Citrus Research and Development Foundation grant no. 71, on behalf of the Florida citrus growers (F. G., C. C. and W. G. F.); Ministero delle Politiche Agricole Alimentari e Forestali, Project Citrustart and Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Programma Operativo Nazionale 'Ricerca e Competitivita' 2007-2013, Project IT-Citrus Genomics PON_01623 (M. Morgante, S. S., F. C., C. D. F., S. Pinozio and A.Z.). Pineapple Ridge sweet-orange sequencing was performed by 454 Life Sciences, a Roche company. The work conducted by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 37 TC 97 Z9 99 U1 10 U2 96 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1087-0156 EI 1546-1696 J9 NAT BIOTECHNOL JI Nat. Biotechnol. PD JUL PY 2014 VL 32 IS 7 BP 656 EP + DI 10.1038/nbt.2906 PG 8 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AK8VE UT WOS:000338705900031 PM 24908277 ER PT J AU Meinecke, J Doyle, HW Miniati, F Bell, AR Bingham, R Crowston, R Drake, RP Fatenejad, M Koenig, M Kuramitsu, Y Kuranz, CC Lamb, DQ Lee, D MacDonald, MJ Murphy, CD Park, HS Pelka, A Ravasio, A Sakawa, Y Schekochihin, AA Scopatz, A Tzeferacos, P Wan, WC Woolsey, NC Yurchak, R Reville, B Gregori, G AF Meinecke, J. Doyle, H. W. Miniati, F. Bell, A. R. Bingham, R. Crowston, R. Drake, R. P. Fatenejad, M. Koenig, M. Kuramitsu, Y. Kuranz, C. C. Lamb, D. Q. Lee, D. MacDonald, M. J. Murphy, C. D. Park, H-S. Pelka, A. Ravasio, A. Sakawa, Y. Schekochihin, A. A. Scopatz, A. Tzeferacos, P. Wan, W. C. Woolsey, N. C. Yurchak, R. Reville, B. Gregori, G. TI Turbulent amplification of magnetic fields in laboratory laser-produced shock waves SO NATURE PHYSICS LA English DT Article ID REMNANT CASSIOPEIA-A; SUPERNOVA REMNANT; PROPER MOTIONS; X-RAY; EMISSION; HYDRODYNAMICS; ACCELERATION; SIMULATION; EJECTA; SHELL AB X-ray(1-3) and radio(4-6) observations of the supernova remnant Cassiopeia A reveal the presence of magnetic fields about 100 times stronger than those in the surrounding interstellar medium. Field coincident with the outer shock probably arises through a nonlinear feedback process involving cosmic rays(2,7,8). The origin of the large magnetic field in the interior of the remnant is less clear but it is presumably stretched and amplified by turbulent motions. Turbulence may be generated by hydrodynamic instability at the contact discontinuity between the supernova ejecta and the circumstellar gas(9). However, optical observations of Cassiopeia A indicate that the ejecta are interacting with a highly inhomogeneous, dense circumstellar cloud bank formed before the supernova explosion(10-12). Herewe investigate the possibility that turbulent amplification is induced when the outer shock overtakes dense clumps in the ambient medium(13-15). We report laboratory experiments that indicate the magnetic field is amplified when the shock interacts with a plastic grid. We show that our experimental results can explain the observed synchrotron emission in the interior of the remnant. The experiment also provides a laboratory example of magnetic field amplification by turbulence in plasmas, a physical process thought to occur in many astrophysical phenomena. C1 [Meinecke, J.; Doyle, H. W.; Bell, A. R.; Fatenejad, M.; Schekochihin, A. A.; Tzeferacos, P.; Reville, B.; Gregori, G.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Miniati, F.] ETH, Dept Phys, CH-8093 Zurich, Switzerland. [Bingham, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bingham, R.] Univ Strathclyde, Dept Phys, Glasgow G4 0NG, Lanark, Scotland. [Crowston, R.; Woolsey, N. C.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Drake, R. P.; Kuranz, C. C.; MacDonald, M. J.; Wan, W. C.] Univ Michigan, Ann Arbor, MI 48103 USA. [Fatenejad, M.; Lamb, D. Q.; Lee, D.; Scopatz, A.; Tzeferacos, P.; Gregori, G.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Koenig, M.; Pelka, A.; Ravasio, A.; Yurchak, R.] Univ Paris 06, Ecole Polytech, CNRS CEA, Lab Utilisat Lasers Intenses,UMR7605, F-91128 Palaiseau, France. [Kuramitsu, Y.; Sakawa, Y.] Osaka Univ, Inst Laser Engn, Suita, Osaka 5650871, Japan. [Murphy, C. D.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH8 9YL, Midlothian, Scotland. [Park, H-S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Reville, B.] Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland. RP Meinecke, J (reprint author), Univ Oxford, Dept Phys, Parks Rd, Oxford OX1 3PU, England. EM jena.meinecke@physics.ox.ac.uk; g.gregori1@physics.ox.ac.uk RI Sakawa, Youichi/J-5707-2016; Drake, R Paul/I-9218-2012; OI Sakawa, Youichi/0000-0003-4165-1048; Drake, R Paul/0000-0002-5450-9844; MacDonald, Michael/0000-0002-6295-6978 FU European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC [256973, 247039]; LASERLAB-EUROPE [284464]; US Department of Energy [B591485]; USDOE [DE-NA0001840] FX We thank the Vulcan technical team at the Central Laser Facility of the Rutherford Appleton Laboratory for their support during the experiments; in particular, R. Clarke, M. Notley and R. Heathcote. A. R. B. acknowledges valuable discussions with H. Li (Los Alamos National Laboratory). The research leading to these results has received financial support from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreements no. 256973 and 247039, LASERLAB-EUROPE grant agreement No. 284464, the US Department of Energy under Contract No. B591485 to Lawrence Livermore National Laboratory, and FieldWork Proposal No. 57789 to Argonne National Laboratory. Partial support from the Science and Technology Facilities Council and the Engineering and Physical Sciences Research Council of the United Kingdom (Grant No. EP/G007187/1) is also acknowledged. The work of R. P. D., C. C. K., M. J. M. andW. C. W. was supported by the USDOE under grant DE-NA0001840. NR 30 TC 18 Z9 18 U1 1 U2 49 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1745-2473 EI 1745-2481 J9 NAT PHYS JI Nat. Phys. PD JUL PY 2014 VL 10 IS 7 BP 520 EP 524 DI 10.1038/NPHYS2978 PG 5 WC Physics, Multidisciplinary SC Physics GA AL0UT UT WOS:000338843100020 ER PT J AU Childs, KL Nandety, A Hirsch, CN Gongora-Castillo, E Schmutz, J Kaeppler, SM Casler, MD Buell, CR AF Childs, Kevin L. Nandety, Aruna Hirsch, Candice N. Gongora-Castillo, Elsa Schmutz, Jeremy Kaeppler, Shawn M. Casler, Michael D. Buell, C. Robin TI Generation of Transcript Assemblies and Identification of Single Nucleotide Polymorphisms from Seven Lowland and Upland Cultivars of Switchgrass SO PLANT GENOME LA English DT Article ID GENOME-WIDE ASSOCIATION; PANICUM-VIRGATUM L.; EXPRESSED SEQUENCE TAGS; NUCLEAR-DNA CONTENT; INFERRING PHYLOGENY; GENETIC DIVERSITY; RNA-SEQ; MAIZE; MARKERS; POPULATIONS AB Switchgrass is a North American perennial prairie species that has been used as a rangeland and forage crop and has recently been targeted as a potential biofuel feedstock species. Switchgrass, which occurs as tetraploid and octoploid forms, is classified into lowland or upland ecotypes that differ in growth phenotypes and adaptation to distinct habitats. Using RNA-sequencing (RNA-seq) reads derived from crown, young shoot, and leaf tissues, we generated sequence data from seven switchgrass cultivars, three lowland and four upland, to enable comparative analyses between switchgrass cultivars and to identify single nucleotide polymorphisms (SNPs) for use in breeding and genetic analysis. We also generated individual transcript assemblies for each of the cultivars. Transcript data indicate that subgenomes of octoploid switchgrass are not substantially different from subgenomes of tetraploids as expected for an autopolyploid origin of switchgrass octoploids. Using RNA-seq reads aligned to the switchgrass Release 0 AP13 reference genome, we identified 1,305,976 high-confidence SNPs. Of these SNPs, 438,464 were unique to lowland cultivars, but only 12,002 were found in all lowlands. Conversely, 723,678 SNPs were unique to upland cultivars, with only 34,665 observed in all uplands. Comparison of our high-confidence transcriptome-derived SNPs with SNPs previously identified in a genotyping-by-sequencing (GBS) study of an association panel revealed limited overlap between the two methods, highlighting the utility of transcriptome-based SNP discovery in augmenting genome diversity polymorphism datasets. The transcript and SNP data described here provide a useful resource for switchgrass gene annotation and marker-based analyses of the switchgrass genome. C1 [Childs, Kevin L.; Hirsch, Candice N.; Buell, C. Robin] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Childs, Kevin L.; Hirsch, Candice N.; Gongora-Castillo, Elsa; Buell, C. Robin] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Nandety, Aruna; Kaeppler, Shawn M.; Casler, Michael D.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Nandety, Aruna; Kaeppler, Shawn M.] Univ Wisconsin, Dept Agron, Madison, WI 53706 USA. [Schmutz, Jeremy] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL 35806 USA. [Casler, Michael D.] USDA ARS, US Dairy Forage Res Ctr, Madison, WI 53706 USA. RP Childs, KL (reprint author), Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. EM kchilds@plantbiology.msu.edu RI Childs, Kevin/C-9513-2014; Gongora, Elsa/R-8854-2016; OI Childs, Kevin/0000-0002-3680-062X; Gongora, Elsa/0000-0001-6327-6993; Kaeppler, Shawn/0000-0002-5964-1668 FU Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494] FX This work was funded by the Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 81 TC 1 Z9 1 U1 1 U2 30 PU CROP SCIENCE SOC AMER PI MADISON PA 677 S SEGOE ROAD, MADISON, WI 53711 USA SN 1940-3372 J9 PLANT GENOME-US JI Plant Genome PD JUL PY 2014 VL 7 IS 2 DI 10.3835/plantgenome2013.12.0041 PG 13 WC Plant Sciences; Genetics & Heredity SC Plant Sciences; Genetics & Heredity GA AL0RP UT WOS:000338834700006 ER PT J AU Cloet, IC Roberts, CD AF Cloet, Ian C. Roberts, Craig D. TI Explanation and prediction of observables using continuum strong QCD SO PROGRESS IN PARTICLE AND NUCLEAR PHYSICS LA English DT Review DE Confinement; Dynamical chiral symmetry breaking; Dyson-Schwinger equations; Hadron physics; In-hadron condensates; Parton distributions ID DYSON-SCHWINGER EQUATIONS; ELECTROMAGNETIC FORM-FACTORS; DEEP-INELASTIC-SCATTERING; CHIRAL-SYMMETRY-BREAKING; QUARK-DIQUARK MODEL; VIRTUAL COMPTON-SCATTERING; JONA-LASINIO MODEL; ANOMALOUS MAGNETIC-MOMENT; MONTE-CARLO CALCULATIONS; PION LOOP CONTRIBUTION AB The last five years have brought considerable progress in the study of the bound-state problem in continuum quantum field theory. We highlight a subset of that progress; viz., that made within the context of Dyson-Schwinger equation analyses of cold, sparse hadrons. Our focus is primarily on advances in the reliable computation, explanation and prediction of quantities that are truly measurable; but we also review aspects of a new paradigm that has condensates contained within hadrons, and explain that the asymptotic form of parton distribution amplitudes and functions are practically unreachable with terrestrial facilities. Given the pace of expansion in experiment and improvement in theory, it appears possible that the next five years will bring profound growth in our store of knowledge about hadrons and nuclei. (C) 2014 Elsevier B.V. All rights reserved. C1 [Cloet, Ian C.; Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM cdroberts@anl.gov FU Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX We acknowledge valuable input from A. Bashir, W. Bentz, S.J. Brodsky, L. Chang, C. Chen, B. El-Bennich, R. Gothe, R.J. Holt, Y.-x. Liu, V. Mokeev, M. Pitschmann, S.-x. Qin, H.L.L. Roberts, J. Segovia, S.M. Schmidt, R. Shrock, P.C. Tandy, A.W. Thomas, K.-I. Wang and D.J. Wilson. This work was supported by Department of Energy, Office of Nuclear Physics, contract no. DE-AC02-06CH11357. NR 499 TC 94 Z9 94 U1 0 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0146-6410 EI 1873-2224 J9 PROG PART NUCL PHYS JI Prog. Part. Nucl. Phys. PD JUL PY 2014 VL 77 BP 1 EP 69 DI 10.1016/j.ppnp.2014.02.001 PG 69 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK7KW UT WOS:000338608200001 ER PT J AU Roland, G Safarik, K Steinberg, P AF Roland, G. Safarik, K. Steinberg, P. TI Heavy-ion collisions at the LHC SO PROGRESS IN PARTICLE AND NUCLEAR PHYSICS LA English DT Review DE Heavy-ion collisions; Quark-gluon plasma; Quantum chromo-dynamics; LHC ID PB-PB COLLISIONS; QUARK-GLUON PLASMA; NUCLEUS-NUCLEUS COLLISIONS; TRANSVERSE-MOMENTUM DEPENDENCE; CHARGED-PARTICLE PRODUCTION; COLOR GLASS CONDENSATE; LEAD-LEAD COLLISIONS; LEE-YANG ZEROS; ROOT-S(NN)=2.76 TEV; ANISOTROPIC FLOW AB A new era in the study of high-energy nuclear collisions began when the CERN Large Hadron Collider (LHC) provided the first collisions of lead nuclei in late 2010. In the first three years of operation the ALICE, ATLAS and CMS experiments each collected Pb-Pb data samples of more than 50 mu b(-1) at 3 root S-NN = 2.76 TeV, exceeding the previously studied collision energies by more than an order of magnitude. These data have provided new insights into the properties of QCD matter under extreme conditions, with extensive measurements of soft particle production and newly accessible hard probes of the hot and dense medium. In this review, we provide a comprehensive overview of the results obtained in heavy-ion collisions at the LHC so far, with particular emphasis on the complementary nature of the observations by the three experiments. In particular, the combination of ALICE's strengths at hadron identification, the strengths of ATLAS and CMS to make precise measurements of high pr probes, and the resourceful measurements of collective flow by all of the experiments have provided a rich and diverse dataset in only a few years. While the basic paradigm established at RHIC - that of a hot, dense medium that flows with a viscosity to shear-entropy ratio near the predicted lower bound, and which degrades the energy of probes, such as jets, heavy-flavours and J/psi - is confirmed at the LHC, the new data suggest many new avenues for extracting its properties in detail. (C) 2014 Elsevier B.V. All rights reserved. C1 [Roland, G.] MIT, Cambridge, MA 02139 USA. [Safarik, K.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Steinberg, P.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Safarik, K (reprint author), CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. EM Karel.Safarik@cern.ch NR 277 TC 8 Z9 8 U1 1 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0146-6410 EI 1873-2224 J9 PROG PART NUCL PHYS JI Prog. Part. Nucl. Phys. PD JUL PY 2014 VL 77 BP 70 EP 127 DI 10.1016/j.ppnp.2014.05.001 PG 58 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK7KW UT WOS:000338608200002 ER PT J AU Rodney, SA Riess, AG Strolger, LG Dahlen, T Graur, O Casertano, S Dickinson, ME Ferguson, HC Garnavich, P Hayden, B Jha, SW Jones, DO Kirshner, RP Koekemoer, AM McCully, C Mobasher, B Patel, B Weiner, BJ Cenko, SB Clubb, KI Cooper, M Filippenko, AV Frederiksen, TF Hjorth, J Leibundgut, B Matheson, T Nayyeri, H Penner, K Trump, J Silverman, JM Vivian, U Bostroem, KA Challis, P Rajan, A Wolff, S Faber, SM Grogin, NA Kocevski, D AF Rodney, Steven A. Riess, Adam G. Strolger, Louis-Gregory Dahlen, Tomas Graur, Or Casertano, Stefano Dickinson, Mark E. Ferguson, Henry C. Garnavich, Peter Hayden, Brian Jha, Saurabh W. Jones, David O. Kirshner, Robert P. Koekemoer, Anton M. McCully, Curtis Mobasher, Bahram Patel, Brandon Weiner, Benjamin J. Cenko, S. Bradley Clubb, Kelsey I. Cooper, Michael Filippenko, Alexei V. Frederiksen, Teddy F. Hjorth, Jens Leibundgut, Bruno Matheson, Thomas Nayyeri, Hooshang Penner, Kyle Trump, Jonathan Silverman, Jeffrey M. Vivian, U. Bostroem, K. Azalee Challis, Peter Rajan, Abhijith Wolff, Schuyler Faber, S. M. Grogin, Norman A. Kocevski, Dale TI TYPE Ia SUPERNOVA RATE MEASUREMENTS TO REDSHIFT 2.5 FROM CANDELS: SEARCHING FOR PROMPT EXPLOSIONS IN THE EARLY UNIVERSE SO ASTRONOMICAL JOURNAL LA English DT Article DE infrared: general; supernovae: general; surveys ID CORE-COLLAPSE SUPERNOVAE; DELAY-TIME DISTRIBUTION; ORIGINS DEEP SURVEY; DIGITAL SKY SURVEY; EXTRAGALACTIC LEGACY SURVEY; TELESCOPE ADVANCED CAMERA; GOODS-SOUTH FIELD; GAMMA-RAY BURSTS; II-P SUPERNOVAE; STAR-FORMATION AB dThe Cosmic Assembly Near-infrared Deep Extragalactic Legacy Survey (CANDELS) was a multi-cycle treasury program on the Hubble Space Telescope (HST) that surveyed a total area of -0.25 deg2 with -900 HST orbits spread across five fields over three years. Within these survey images we discovered 65 supernovae (SNe) of all types, out to z 2.5. We classify -24 of these as Type Ia SNe (SNe Ia) based on host galaxy redshifts and SN photometry (supplemented by grism spectroscopy of six SNe). Here we present a measurement of the volumetric SN Ia rate as a function of redshift, reaching for the first time beyond z =- 2 and putting new constraints on SN Ia progenitor models. Our highest redshift bin includes detections of SNe that exploded when the universe was only -3 Gyr old and near the peak of the cosmic star formation history. This gives the CANDELS high redshift sample unique leverage for evaluating the fraction of SNe Ia that explode promptly after formation (<500 Myr). Combining the CANDELS rates with all available SN Ia rate measurements in the literature we find that this prompt SN Ia fraction is fp = 0.53st=sg.Zc6', consistent with a delay time distribution that follows a simple t-1 power law for all times t > 40 Myr. However, mild tension is apparent between ground-based low-z surveys and space-based high-z surveys. In both CANDELS and the sister HST program CLASH (Cluster Lensing And Supernova Survey with Hubble), we find a low rate of SNe Ia at z > 1. This could be a hint that prompt progenitors are in fact relatively rare, accounting for only 20% of all SN Ia explosions-though further analysis and larger samples will be needed to examine that suggestion. Key words: infrared: general - supernovae: C1 [Rodney, Steven A.; Riess, Adam G.; Graur, Or; Jones, David O.; Wolff, Schuyler] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Riess, Adam G.; Strolger, Louis-Gregory; Dahlen, Tomas; Casertano, Stefano; Ferguson, Henry C.; Koekemoer, Anton M.; Bostroem, K. Azalee; Grogin, Norman A.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Graur, Or] Tel Aviv Univ, Dept Astrophys, IL-69978 Tel Aviv, Israel. [Graur, Or] Amer Museum Nat Hist, Dept Astrophys, New York, NY 10024 USA. [Dickinson, Mark E.; Matheson, Thomas] Natl Opt Astron Observ, Tucson, AZ 85719 USA. [Garnavich, Peter] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Hayden, Brian] EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Jha, Saurabh W.; McCully, Curtis; Patel, Brandon] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Kirshner, Robert P.; Challis, Peter] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Mobasher, Bahram; Nayyeri, Hooshang; Vivian, U.] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. [Weiner, Benjamin J.; Penner, Kyle] Univ Arizona, Dept Astron, Tucson, AZ 85721 USA. [Cenko, S. Bradley] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Cenko, S. Bradley] Univ Maryland, Joint Space Sci Inst, College Pk, MD 20742 USA. [Clubb, Kelsey I.; Filippenko, Alexei V.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Cooper, Michael] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Frederiksen, Teddy F.; Hjorth, Jens] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, DK-2100 Copenhagen, Denmark. [Leibundgut, Bruno] European So Observ, Garching, Germany. [Leibundgut, Bruno] Tech Univ Munich, D-80290 Munich, Germany. [Trump, Jonathan] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Silverman, Jeffrey M.] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [Rajan, Abhijith] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Faber, S. M.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 92064 USA. [Kocevski, Dale] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. RP Rodney, SA (reprint author), Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. RI Hjorth, Jens/M-5787-2014; OI Hjorth, Jens/0000-0002-4571-2306; Graur, Or/0000-0002-4391-6137; Koekemoer, Anton/0000-0002-6610-2048 NR 117 TC 28 Z9 28 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-6256 EI 1538-3881 J9 ASTRON J JI Astron. J. PD JUL PY 2014 VL 148 IS 1 AR 13 DI 10.1088/0004-6256/148/1/13 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK4PF UT WOS:000338405900013 ER PT J AU Schenck, DE Datta, A Burns, JO Skillman, S AF Schenck, David E. Datta, Abhirup Burns, Jack O. Skillman, Sam TI X-RAY OBSERVATIONS OF COMPLEX TEMPERATURE STRUCTURE IN THE COOL-CORE CLUSTER A85 SO ASTRONOMICAL JOURNAL LA English DT Article DE galaxies: clusters: individual (Abell 85); shock waves; X-rays: galaxies: clusters ID GALAXY CLUSTERS; XMM-NEWTON; RADIO RELICS; SHOCK-WAVES; CHANDRA OBSERVATIONS; RICH CLUSTER; COSMIC-RAYS; SIMULATIONS; ABELL-85; VIEW AB X-ray observations were used to examine the complex temperature structure of A85, a cool-core galaxy cluster. Temperature features can provide evidence of merging events which shock heat the intracluster gas. Temperature maps were made from both Chandra and XMM-Newton observations. The combination of a new, long-exposure XMM observation and an improved temperature map binning technique produced the highest fidelity temperature maps of A85 to date. Hot regions were detected near the subclusters to the south and southwest in both the Chandra and XMM temperature maps. The presence of these structures implies A85 is not relaxed. The hot regions may indicate the presence of shocks. The Mach numbers were estimated to be similar to 1.9 at the locations of the hot spots. Observational effects will tend to systematically reduce temperature jumps, so the measured Mach numbers are likely underestimated. Neither temperature map showed evidence for a shock in the vicinity of the presumed radio relic near the southwest subcluster. However, the presence of a weak shock cannot be ruled out. There was tension between the temperatures measured by the two instruments. C1 [Schenck, David E.; Datta, Abhirup; Burns, Jack O.] Univ Colorado, Dept Astrophys & Planetary Sci, Ctr Astrophys & Space Astron, Boulder, CO 80309 USA. [Skillman, Sam] SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. RP Schenck, DE (reprint author), Univ Colorado, Dept Astrophys & Planetary Sci, Ctr Astrophys & Space Astron, Boulder, CO 80309 USA. FU NSF [AST-1106437]; DOE Computational Science Graduate Fellowship [DE-FG02-97ER25308] FX The authors thank Eric Hallman, Maxim Markevitch, Alexey Vikhlinin, Scott Randall, Steve Allen, and Norbert Werner for taking the time to discuss data reduction and for general advice on interpretation. We also thank the referee for valuable input. This work was funded by NSF grant AST-1106437 to J.B. S.W.S. was partially supported by a DOE Computational Science Graduate Fellowship under grant No. DE-FG02-97ER25308. NR 39 TC 7 Z9 7 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-6256 EI 1538-3881 J9 ASTRON J JI Astron. J. PD JUL PY 2014 VL 148 IS 1 AR 23 DI 10.1088/0004-6256/148/1/23 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK4PF UT WOS:000338405900023 ER PT J AU Li, YL Li, SY Zhang, TJ Li, TP AF Li, Yun-Long Li, Shi-Yu Zhang, Tong-Jie Li, Ti-Pei TI MODEL-INDEPENDENT DETERMINATION OF CURVATURE PARAMETER USING H(z) AND D-A (z) DATA PAIRS FROM BAO MEASUREMENTS SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE cosmological parameters; cosmology: observations ID EXPANSION RATE; GALAXIES; GROWTH; Z=0.57; SAMPLE AB We present a model-independent determination of the curvature parameter Omega(k) using the Hubble parameter H(z) and the angular diameter distance D-A(z) from recent baryon acoustic oscillation (BAO) measurements. Each H(z) and D-A(z) pair from a BAO measurement can constrain a curvature parameter. The accuracy of the curvature measurement improves with increased redshift of H(z) and D-A(z) data. By using the H(z) and D-A(z) pair derived from a BAO Lyman a forest measurement at z = 2.36, the Omega(k) is confined to be -0.05 +/- 0.06, which is consistent with the curvature of -0.037(-0.042) (+0.044) constrained by the nine year Wilkinson Microwave Anisotropy Probe data only. Considering future BAOmeasurements, at least one order of magnitude improvement of this curvature measurement can be expected. C1 [Li, Yun-Long; Li, Ti-Pei] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Li, Shi-Yu; Zhang, Tong-Jie] Beijing Normal Univ, Dept Astron, Beijing 100875, Peoples R China. [Zhang, Tong-Jie] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Zhang, Tong-Jie] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Zhang, Tong-Jie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Li, Ti-Pei] Chinese Acad Sci, Inst High Energy Phys, Key Lab Particle Astrophys, Beijing 100049, Peoples R China. RP Li, YL (reprint author), Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. EM tjzhang@bnu.edu.cn OI Li, Yun-Long/0000-0003-3931-0084 FU National Science Foundation of China [11033003, 11173006]; Ministry of Science and Technology National Basic Science program (project 973) [2012CB821804] FX This work is supported by the National Science Foundation of China (grant No. 11033003), the National Science Foundation of China (grant No. 11173006), and the Ministry of Science and Technology National Basic Science program (project 973) under grant No. 2012CB821804. NR 22 TC 9 Z9 9 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUL 1 PY 2014 VL 789 IS 1 AR L15 DI 10.1088/2041-8205/789/1/L15 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK6UR UT WOS:000338563300015 ER PT J AU Zhang, XJ Li, H Li, ST Lin, DNC AF Zhang, Xiaojia Li, Hui Li, Shengtai Lin, Douglas N. C. TI RESONANCES OF MULTIPLE EXOPLANETS AND IMPLICATIONS FOR THEIR FORMATION SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE planet-disk interactions; planetary systems; protoplanetary disks ID MEAN MOTION RESONANCES; I PLANETARY MIGRATION; ORBITAL RESONANCES; TORQUE FORMULA; SUPER-EARTHS; SYSTEMS; DISK; PROTOPLANETS; DYNAMICS; CANDIDATES AB Among similar to 160 of the multiple exoplanetary systems confirmed, about 30% of them have neighboring pairs with a period ratio <= 2. A significant fraction of these pairs are around mean motion resonance (MMR), and, more interestingly, peak around 2:1 and 3:2, with a clear absence of more closely packed MMRs with period ratios less than 4: 3, regardless of planet masses. Here, we report numerical simulations demonstrating that such MMR behavior places important constraints on the disk evolution stage out of which the observed planets formed. Multiple massive planets (with mass >= 0.8 M-Jup) tend to end up with a 2:1 MMR mostly independent of the disk masses, but low-mass planets (with mass <= 30 M-circle plus) can have MMRs larger than 4:3 only when the disk mass is quite small, suggesting that the observed dynamical architecture of most low-mass-planet pairs was established late in the disk evolution stage, just before it was dispersed completely. C1 [Zhang, Xiaojia; Lin, Douglas N. C.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Li, Hui; Li, Shengtai] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lin, Douglas N. C.] Tsinghua Univ, Inst Adv Studies, Beijing 100084, Peoples R China. RP Zhang, XJ (reprint author), Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. EM xzhang47@ucsc.edu OI Zhang, Xiaojia/0000-0002-6612-5127; Li, Shengtai/0000-0002-4142-3080 FU LDRD program; IGPP of Los Alamos National Laboratory; UC-fee program of University of California FX We thank the referee, Frederic Rasio, for helpful comments that improved the manuscript. We acknowledge support from the LDRD program and IGPP of Los Alamos National Laboratory. H.L. and D.N.C.L. also acknowledge support from the UC-fee program of University of California. Simulations were carried out using the Institutional Computing resources at LANL. NR 40 TC 8 Z9 8 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUL 1 PY 2014 VL 789 IS 1 AR L23 DI 10.1088/2041-8205/789/1/L23 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK6UR UT WOS:000338563300023 ER PT J AU Hoover, AN Tumuluru, JS Teymouri, F Moore, J Gresham, G AF Hoover, Amber N. Tumuluru, Jaya Shankar Teymouri, Farzaneh Moore, Janette Gresham, Garold TI Effect of pelleting process variables on physical properties and sugar yields of ammonia fiber expansion pretreated corn stover SO BIORESOURCE TECHNOLOGY LA English DT Article DE Pelletization; Densification; Ammonia fiber expansion (AFEX); Corn stover; Enzymatic hydrolysis ID ENZYMATIC-HYDROLYSIS; BIOMASS DENSIFICATION; RICE STRAW; BIOFUELS; QUALITY; AFEX AB Pelletization process variables, including grind size (4, 6 mm), die speed (40, 50, 60 Hz), and preheating (none, 70 degrees C), were evaluated to understand their effect on pellet quality attributes and sugar yields of ammonia fiber expansion (AFEX) pretreated biomass. The bulk density of the pelletized AFEX corn stover was three to six times greater compared to untreated and AFEX-treated corn stover. Also, the durability of the pelletized AFEX corn stover was >97.5% for all pelletization conditions studied except for preheated pellets. Die speed had no effect on enzymatic hydrolysis sugar yields of pellets. Pellets produced with preheating or a larger grind size (6 mm) had similar or lower sugar yields. Pellets generated with 4 mm AFEX-treated corn stover, a 60 Hz die speed, and no preheating resulted in pellets with similar or greater density, durability, and sugar yields compared to other pelletization conditions. (C) 2014 Battelle Energy Alliance, LLC, contract manager for Idaho National Laboratory. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/3.0/). C1 [Hoover, Amber N.; Tumuluru, Jaya Shankar; Gresham, Garold] Idaho Natl Lab, Biofuels & Renewable Energy Technol, Idaho Falls, ID 83415 USA. [Teymouri, Farzaneh; Moore, Janette] MBI Int, Lansing, MI 48910 USA. RP Hoover, AN (reprint author), Idaho Natl Lab, ESL IF 685,MS 3570,1765 N Yellowstone Hwy, Idaho Falls, ID 83401 USA. EM amber.hoover@inl.gov; jayashankar.tumuluru@inl.gov; teymouri@mbi.org; moore@mbi.org; garold.gresham@inl.gov RI Hoover, Amber/B-8373-2017 OI Hoover, Amber/0000-0001-8584-3995 FU US Department of Energy under Department of Energy Idaho Operations Office [DE-AC07-05ID14517] FX The authors would like to thank Chandra Nielson and Josh Videto from MBI for performing the AFEX pretreatment and the following INL colleagues for their assistance: Ian Bonner, Cynthia Breckenridge, Debra Bruhn, Karen Delezene-Briggs, Craig Conner, Rachel Emerson, Jeffrey Lacey, Sabrina Morgan, Manunya Phanphanich, Allison Ray, Tammy Trowbridge, and Neal Yancey. This research was supported by the US Department of Energy under Department of Energy Idaho Operations Office Contract No. DE-AC07-05ID14517. NR 35 TC 22 Z9 23 U1 2 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD JUL PY 2014 VL 164 BP 128 EP 135 DI 10.1016/j.biortech.2014.02.005 PG 8 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AK8WX UT WOS:000338710500019 PM 24844167 ER PT J AU Sapi, A Thompson, C Wang, HL Michalak, WD Ralston, WT Alayoglu, S Somorjai, GA AF Sapi, Andras Thompson, Chris Wang, Hailiang Michalak, William D. Ralston, Walter T. Alayoglu, Selim Somorjai, Gabor A. TI Recovery of Pt Surfaces for Ethylene Hydrogenation-Based Active Site Determination SO CATALYSIS LETTERS LA English DT Article DE Heterogeneous catalysis; Ethylene hydrogenation; Platinum; Catalyst pretreatment ID SUM-FREQUENCY GENERATION; OXYGEN REDUCTION REACTION; SINGLE-CRYSTAL SURFACES; PLATINUM NANOPARTICLES; VIBRATIONAL SPECTROSCOPY; METHANOL OXIDATION; CATALYTIC-REACTIONS; IN-SITU; 7 NM; PT(111) AB The effect of pretreatment (O-2 or H-2) and catalyst history was investigated through room temperature ethylene hydrogenation reaction over several types of platinum based nanoparticle systems: 1.6 nm Pt/TTAB, 4.1 nm Pt/PVP (with and without UV treatment), 4.1 nm Pt with a silica shell, and e-beam evaporated Pt thin films were tested. The H-2 pretreatment resulted in the absence of activity. However, Pt active sites for the ethylene hydrogenation reaction were recovered after an O-2 pretreatment irrespective of the catalyst history, regardless of the particle size nor the presence, absence or type of capping agent. The calculation of the average TOF resulted in 10.13 +/- A 3.27. This value correlates well with data from the literature. Thus, the ethylene hydrogenation reaction can be used to determine available sites of Pt catalysts if the reaction is following an O-2 pretreatment. . C1 [Sapi, Andras; Thompson, Chris; Wang, Hailiang; Michalak, William D.; Ralston, Walter T.; Alayoglu, Selim; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Sapi, Andras; Thompson, Chris; Wang, Hailiang; Michalak, William D.; Ralston, Walter T.; Alayoglu, Selim; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Sapi, Andras; Thompson, Chris; Wang, Hailiang; Michalak, William D.; Ralston, Walter T.; Alayoglu, Selim; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu RI Sapi, Andras/G-3527-2015 OI Sapi, Andras/0000-0001-6557-0731 FU Office of Basic Energy Sciences, Material Sciences and Engineering Division U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported the Director, Office of Basic Energy Sciences, Material Sciences and Engineering Division U.S. Department of Energy, under Contract DE-AC02-05CH11231. NR 31 TC 4 Z9 4 U1 2 U2 41 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1011-372X EI 1572-879X J9 CATAL LETT JI Catal. Lett. PD JUL PY 2014 VL 144 IS 7 BP 1151 EP 1158 DI 10.1007/s10562-014-1272-y PG 8 WC Chemistry, Physical SC Chemistry GA AK8CA UT WOS:000338653600007 ER PT J AU Moeller, SL Parvaz, MA Shumay, E Wu, SLN Beebe-Wang, N Konova, AB Misyrlis, M Alia-Klein, N Goldstein, RZ AF Moeller, Scott. L. Parvaz, Muhammad A. Shumay, Elena Wu, Salina Beebe-Wang, Nicasia Konova, Anna B. Misyrlis, Michail Alia-Klein, Nelly Goldstein, Rita Z. TI Monoamine polygenic liability in health and cocaine dependence: Imaging genetics study of aversive processing and associations with depression symptomatology SO DRUG AND ALCOHOL DEPENDENCE LA English DT Article DE Cocaine addiction; Imaging genetics; Depression; comorbidity; 5-HTTLPR; MAOA; Event-related potentials ID SEROTONIN TRANSPORTER GENE; TRYPTOPHAN DEPLETION; NEURAL RESPONSES; BIASED ATTENTION; PROMOTER REGION; POPULATION STRATIFICATION; 5-HTTLPR POLYMORPHISM; MOTIVATED ATTENTION; EMOTION REGULATION; PREFRONTAL CORTEX AB Background: Gene polymorphisms that affect serotonin signaling modulate reactivity to salient stimuli and risk for emotional disturbances. Here, we hypothesized that these serotonin genes, which have been primarily explored in depressive disorders, could also have important implications for drug addiction, with the potential to reveal important insights into drug symptomatology, severity, and/or possible sequelae such as dysphoria. Methods: Using an imaging genetics approach, the current study tested in 62 cocaine abusers and 57 healthy controls the separate and combined effects of variations in the serotonin transporter (5-HTTLPR) and monoamine oxidase A (MAOA) genes on processing of aversive information. Reactivity to standardized unpleasant images was indexed by a psychophysiological marker of stimulus salience (i.e., the late positive potential (LPP) component of the event-related potential) during passive picture viewing. Depressive symptomatology was assessed with the Beck Depression Inventory (BDI). Results: Results showed that, independent of diagnosis, the highest unpleasant LPPs emerged in individuals with MAOA-Low and at least one 'Short' allele of 5-HTTLPR. Uniquely in the cocaine participants with these two risk variants, higher unpleasant LPPs correlated with higher BDI scores. Conclusions: Taken together, these results suggest that a multilocus genetic composite of monoamine signaling relates to depression symptomatology through brain function associated with the experience of negative emotions. This research lays the groundwork for future studies that can investigate clinical outcomes and/or pharmacogenetic therapies in drug addiction and potentially other psychopathologies of emotion dysregulation. (C) 2014 Elsevier Ireland Ltd. All rights reserved. C1 [Moeller, Scott. L.; Parvaz, Muhammad A.; Konova, Anna B.; Misyrlis, Michail; Alia-Klein, Nelly; Goldstein, Rita Z.] Icahn Sch Med Mt Sinai, Dept Psychiat, New York, NY 10029 USA. [Moeller, Scott. L.; Parvaz, Muhammad A.; Konova, Anna B.; Misyrlis, Michail; Alia-Klein, Nelly; Goldstein, Rita Z.] Icahn Sch Med Mt Sinai, Dept Neurosci, New York, NY 10029 USA. [Shumay, Elena; Wu, Salina; Beebe-Wang, Nicasia] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Konova, Anna B.] SUNY Stony Brook, Dept Psychol, Stony Brook, NY 11794 USA. [Misyrlis, Michail] SUNY Stony Brook, Dept Comp Sci, Stony Brook, NY 11794 USA. RP Goldstein, RZ (reprint author), One Gustave L Levy Pl,Box 1230, New York, NY 10029 USA. EM rita.goldstein@mssm.edu RI Moeller, Scott/L-5549-2016; OI Moeller, Scott/0000-0002-4449-0844; Parvaz, Muhammad/0000-0002-2671-2327 FU National Institute on Drug Abuse [1R01DA023579, 1F32DA030017-01, 1F32DA033088-01] FX This study was supported by grants from the National Institute on Drug Abuse: 1R01DA023579 (RZG), 1F32DA030017-01 (SJM), and 1F32DA033088-01 (MAP). NIDA had no further role in study design; in the collection, analysis and interpretation of data; in the writing of the report; or in the decision to submit the paper for publication. NR 75 TC 2 Z9 2 U1 0 U2 8 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0376-8716 EI 1879-0046 J9 DRUG ALCOHOL DEPEN JI Drug Alcohol Depend. PD JUL 1 PY 2014 VL 140 BP 17 EP 24 DI 10.1016/j.drugalcdep.2014.04.019 PG 8 WC Substance Abuse; Psychiatry SC Substance Abuse; Psychiatry GA AK7PD UT WOS:000338619300003 PM 24837582 ER PT J AU Dale, BE Anderson, JE Brown, RC Csonka, S Dale, VH Herwick, G Jackson, RD Jordan, N Kaffka, S Kline, KL Lynd, LR Malmstrom, C Ong, RG Richard, TL Taylor, C Wang, MQ AF Dale, Bruce E. Anderson, James E. Brown, Robert C. Csonka, Steven Dale, Virginia H. Herwick, Gary Jackson, Randall D. Jordan, Nicholas Kaffka, Stephen Kline, Keith L. Lynd, Lee R. Malmstrom, Carolyn Ong, Rebecca G. Richard, Tom L. Taylor, Caroline Wang, Michael Q. TI Take a Closer Look: Biofuels Can Support Environmental, Economic and Social Goals SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Editorial Material ID ENERGY C1 [Dale, Bruce E.; Malmstrom, Carolyn; Ong, Rebecca G.] Michigan State Univ, E Lansing, MI 48824 USA. [Dale, Bruce E.; Jackson, Randall D.; Ong, Rebecca G.] Great Lakes Bioenergy Res Ctr, Madison, WI 53703 USA. [Anderson, James E.] Ford Motor Co, Dearborn, MI 48126 USA. [Brown, Robert C.] Iowa State Univ, Ames, IA 50011 USA. [Csonka, Steven] Commercial Aviat Alternat Fuels Initiat, Lebanon, OH 45036 USA. [Dale, Virginia H.; Kline, Keith L.] Oak Ridge Natl Lab, Oak Ridge, TN 37849 USA. [Herwick, Gary] Transportat Fuels Consulting, Milford, MI 48380 USA. [Jackson, Randall D.] Univ Wisconsin, Madison, WI 53706 USA. [Jordan, Nicholas] Univ Minnesota, Minneapolis, MN 55455 USA. [Kaffka, Stephen] Univ Calif Davis, Davis, CA 95616 USA. [Lynd, Lee R.] Dartmouth Coll, Hanover, NH 03755 USA. [Richard, Tom L.] Penn State Univ, State Coll, PA 16801 USA. [Taylor, Caroline] Energy Biosci Inst, Berkeley, CA 94704 USA. [Wang, Michael Q.] Argonne Natl Lab, Lemont, IL 60439 USA. RP Dale, BE (reprint author), Michigan State Univ, E Lansing, MI 48824 USA. EM bdale@egr.msu.edu OI Kline, Keith/0000-0003-2294-1170; Ong, Rebecca/0000-0001-5020-646X NR 11 TC 22 Z9 23 U1 5 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7200 EP 7203 DI 10.1021/es5025433 PG 4 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700002 PM 24934084 ER PT J AU Molins, S Trebotich, D Yang, L Ajo-Franklin, JB Ligocki, TJ Shen, CP Steefel, CI AF Molins, Sergi Trebotich, David Yang, Li Ajo-Franklin, Jonathan B. Ligocki, Terry J. Shen, Chaopeng Steefel, Carl I. TI Pore-Scale Controls on Calcite Dissolution Rates from Flow-through Laboratory and Numerical Experiments SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CARBONATE PRECIPITATION; REACTIVE TRANSPORT; KINETICS; CO2 AB A combination of experimental, imaging, and modeling techniques were applied to investigate the pore-scale transport and surface reaction controls on calcite dissolution under elevated pCO(2) conditions. The laboratory experiment consisted of the injection of a solution at 4 bar pCO(2) into a capillary tube packed with crushed calcite. A high resolution pore-scale numerical model was used to simulate the experiment based on a computational domain consisting of reactive calcite, pore space, and the capillary wall constructed from volumetric X-ray microtomography images. Simulated pore-scale effluent concentrations were higher than those measured by a factor of 1.8, with the largest component of the discrepancy related to uncertainties in the reaction rate model and its parameters. However, part of the discrepancy was apparently due to mass transport limitations to reactive surfaces, which were most pronounced near the inlet where larger diffusive boundary layers formed around grains and in slow-flowing pore spaces that exchanged mass by diffusion with fast flow paths. Although minor, the difference between pore- and continuum-scale results due to transport controls was discernible with the highly accurate methods employed and is expected to be more significant where heterogeneity is greater, as in natural subsurface materials. C1 [Molins, Sergi; Yang, Li; Ajo-Franklin, Jonathan B.; Steefel, Carl I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Trebotich, David; Ligocki, Terry J.; Shen, Chaopeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Molins, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM smolins@lbl.gov RI Molins, Sergi/A-9097-2012; Steefel, Carl/B-7758-2010; YANG, LI/F-9392-2010; Ajo-Franklin, Jonathan/G-7169-2015; OI Molins, Sergi/0000-0001-7675-3218; Ajo-Franklin, Jonathan/0000-0002-6666-4702; Shen, Chaopeng/0000-0002-0685-1901 FU Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and the Office of Advanced Scientific Computing Research [DE-AC02-05CH11231]; U.S. DOE Office of Science [DE-AC02-05CH11231]; U.S. DOE Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231] FX This material is based upon work supported as part of the Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and the Office of Advanced Scientific Computing Research (D.T., T.L., and C.S.), under contract number DE-AC02-05CH11231. This research also used resources of the National Energy Research Scientific Computing Center, supported by the U.S. DOE Office of Science (DE-AC02-05CH11231). XCMT imaging was performed with the assistance of Alastair MacDowell and Dula Parkinson at the Advanced Light Source, Beamline 8.3.2, supported by the U.S. DOE Office of Science, Office of Basic Energy Sciences (DE-AC02-05CH11231). The work presented in this manuscript has greatly benefitted from discussion of the results with members of the Center. NR 36 TC 24 Z9 25 U1 2 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7453 EP 7460 DI 10.1021/es5013438 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700033 PM 24865463 ER PT J AU Gaspar, FW Castorina, R Maddalena, RL Nishioka, MG McKone, TE Bradman, A AF Gaspar, Fraser W. Castorina, Rosemary Maddalena, Randy L. Nishioka, Marcia G. McKone, Thomas E. Bradman, Asa TI Phthalate Exposure and Risk Assessment in California Child Care Facilities SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID EXPERT PANEL REPORT; ENDOCRINE-DISRUPTING COMPOUNDS; IN-HOUSE DUST; DI(2-ETHYLHEXYL) PHTHALATE; DEVELOPMENTAL TOXICITY; HUMAN-REPRODUCTION; INDOOR AIR; NTP CENTER; PRESCHOOL-CHILDREN; DANISH CHILDREN AB Approximately 13 million U.S. children less than 6 years old spend some time in early childhood education (ECE) facilities where they may be exposed to potentially harmful chemicals during critical periods of development. We measured five phthalate esters in indoor dust (n = 39) and indoor and outdoor air (n = 40 and 14, respectively) at ECE facilities in Northern California. Dust and airborne concentrations were used to perform a probabilistic health risk assessment to compare estimated exposures with risk levels established for chemicals causing reproductive toxicity and cancer under California's Proposition 65. Di(2-ethylhexyl) phthalate (DEHP) and butyl benzyl phthalate (BBzP) were the dominant phthalates present in floor dust (medians = 172.2 and 46.8 mu g/g, respectively), and dibutyl phthalate (DBP), diethyl phthalate (DEP), and diisobutyl phthalate (DIBP) were the dominant phthalates in indoor air (medians = 0.52, 0.21, and 0.10 mu g/m(3), respectively). The risk assessment results indicate that 82-89% of children in California ECE had DBP exposure estimates exceeding reproductive health benchmarks. Further, 8-11% of children less than 2 years old had DEHP exposure estimates exceeding cancer benchmarks. This is the largest study to measure phthalate exposure in U.S. ECE facilities and findings indicate wide phthalate contamination and potential risk to developing children. C1 [Gaspar, Fraser W.; Castorina, Rosemary; McKone, Thomas E.; Bradman, Asa] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA. [Maddalena, Randy L.; McKone, Thomas E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Nishioka, Marcia G.] Battelle Mem Inst, Columbus, OH 43201 USA. RP Bradman, A (reprint author), 1995 Univ Ave,Suite 265, Berkeley, CA 94704 USA. EM ABradman@berkeley.edu OI Gaspar, Fraser/0000-0002-0782-5721 FU California Air Resource Board [08305] FX We thank the ECE programs that participated in this study. We thank Dr. Martha Sandy of the Office of Environmental Health Hazard Assessment (OEHHA) for reviewing risk evaluation methods and approaches to incorporate age-specific sensitivity factors when evaluating OEHHA NSRLs and MADLs. We also thank Dr. William Nazaroff for advice on strategies to measure air exchange rates. We thank individuals at the Community Child Care Council of Alameda County and Monterey County Child Care Resource and Referral for help with participant recruitment. Finally, we thank the anonymous reviewers of this manuscript for their insightful comments. This research was supported by the California Air Resource Board, Agreement 08305. NR 74 TC 23 Z9 24 U1 5 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7593 EP 7601 DI 10.1021/es501189t PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700050 PM 24870214 ER PT J AU Elgowainy, A Han, J Cai, H Wang, M Forman, GS DiVita, VB AF Elgowainy, Amgad Han, Jeongwoo Cai, Hao Wang, Michael Forman, Grant S. DiVita, Vincent B. TI Energy Efficiency and Greenhouse Gas Emission Intensity of Petroleum Products at US Refineries SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article AB This paper describes the development of (1) a formula correlating the variation in overall refinery energy efficiency with crude quality, refinery complexity, and product slate; and (2) a methodology for calculating energy and greenhouse gas (GHG) emission intensities and processing fuel shares of major U.S. refinery products. Overall refinery energy efficiency is the ratio of the energy present in all product streams divided by the energy in all input streams. Using linear programming (LP) modeling of the various refinery processing units, we analyzed 43 refineries that process 70% of total crude input to U.S. refineries and cover the largest four Petroleum Administration for Defense District (PADD) regions (I, II, III, V). Based on the allocation of process energy among products at the process unit level, the weighted-average product-specific energy efficiencies (and ranges) are estimated to be 88.6% (86.2%-91.2%) for gasoline, 90.9% (84.8%-94.5%) for diesel, 95.3% (93.0%-97.5%) for jet fuel, 94.5% (91.6%-96.2%) for residual fuel oil (RFO), and 90.8% (88.0%-94.3%) for liquefied petroleum gas (LPG). The corresponding weighted-average, production GHG emission intensities (and ranges) (in grams of carbon dioxide-equivalent (CO2e) per megajoule (MJ)) are estimated to be 7.8 (6.2-9.8) for gasoline, 4.9 (2.7-9.9) for diesel, 2.3 (0.9-4.4) for jet fuel, 3.4 (1.5-6.9) for RFO, and 6.6 (4.3-9.2) for LPG. The findings of this study are key components of the life-cycle assessment of GHG emissions associated with various petroleum fuels; such assessment is the centerpiece of legislation developed and promulgated by government agencies in the United States and abroad to reduce GHG emissions and abate global warming. C1 [Elgowainy, Amgad; Han, Jeongwoo; Cai, Hao; Wang, Michael] Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, Argonne, IL 60439 USA. [Forman, Grant S.] Sasol Synfuels Int, Houston, TX 77079 USA. [DiVita, Vincent B.] Jacobs Consultancy Inc, Houston, TX 77072 USA. RP Forman, GS (reprint author), Sasol Synfuels Int, 900 Threadneedle,Suite 100, Houston, TX 77079 USA. EM aelgowainy@anl.gov RI Cai, Hao/A-1975-2016 FU Bioenergy Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357]; Vehicle Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX This research effort by Argonne National Laboratory was supported by the Bioenergy Technologies Office and the Vehicle Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy under Contract DE-AC02-06CH11357. NR 19 TC 22 Z9 22 U1 2 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7612 EP 7624 DI 10.1021/es5010347 PG 13 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700052 PM 24869918 ER PT J AU Forman, GS Divita, VB Han, J Cai, H Elgowainy, A Wang, M AF Forman, Grant S. Divita, Vincent B. Han, Jeongwoo Cai, Hao Elgowainy, Amgad Wang, Michael TI US Refinery Efficiency: Impacts Analysis and Implications for Fuel Carbon Policy Implementation SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ENERGY AB In the next two decades, the U.S. refining industry will face significant changes resulting from a rapidly evolving domestic petroleum energy landscape. The rapid influx of domestically sourced tight light oil and relative demand shifts for gasoline and diesel will impose challenges on the ability of the U.S. refining industry to satisfy both demand and quality requirements. This study uses results from Linear Programming (LP) modeling data to examine the potential impacts of these changes on refinery, process unit, and product-specific efficiencies, focusing on current baseline efficiency values across 43 existing large U.S. refineries that are operating today. These results suggest that refinery and product-specific efficiency values are sensitive to crude quality, seasonal and regional factors, and refinery configuration and complexity, which are determined by final fuel specification requirements. Additional processing of domestically sourced tight light oil could marginally increase refinery efficiency, but these benefits could be offset by crude rebalancing. The dynamic relationship between efficiency and key parameters such as crude API gravity, sulfur content, heavy products, residual upgrading, and complexity are key to understanding possible future changes in refinery efficiency. Relative to gasoline, the efficiency of diesel production is highly variable, and is influenced by the number and severity of units required to produce diesel. To respond to future demand requirements, refiners will need to reduce the gasoline/diesel (G/D) production ratio, which will likely result in greater volumes of diesel being produced through less efficient pathways resulting in reduced efficiency, particularly on the marginal barrel of diesel. This decline in diesel efficiency could be offset by blending of Gas to Liquids (GTL) diesel, which could allow refiners to uplift intermediate fuel streams into more efficient diesel production pathways, thereby allowing for the efficient production of incremental barrels of diesel without added capital investment for the refiner. Given the current wide range of refinery carbon intensity values of baseline transportation fuels in LCA models, this study has shown that the determination of refinery, unit, and product efficiency values requires careful consideration in the context of specific transportation fuel GHG policy objectives. C1 [Forman, Grant S.] Sasol Synfuels Int, Houston, TX 77079 USA. [Divita, Vincent B.] Jacobs Consultancy Inc, Houston, TX 77072 USA. [Han, Jeongwoo; Cai, Hao; Elgowainy, Amgad; Wang, Michael] Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, Argonne, IL 60439 USA. RP Forman, GS (reprint author), Sasol Synfuels Int, 900 Threadneedle,Suite 100, Houston, TX 77079 USA. EM grant.forman@us.sasol.com RI Cai, Hao/A-1975-2016 FU Biomass Energy Technology Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357]; Vehicle Technology Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX We gratefully acknowledge the support of Sasol Synfuels International and Jacobs Consultancy by providing data and giving permission to publish this manuscript. This research effort by Argonne National Laboratory was supported by the Biomass Energy Technology Office and the Vehicle Technology Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy under Contract DE-AC02-06CH11357. NR 34 TC 7 Z9 7 U1 0 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7625 EP 7633 DI 10.1021/es501035a PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700053 PM 24870020 ER PT J AU Sun, RY Sonke, JE Heimburger, LE Belkin, HE Liu, GJ Shome, D Cukrowska, E Liousse, C Pokrovsky, OS Streets, DG AF Sun, Ruoyu Sonke, Jeroen E. Heimbuerger, Lars-Eric Belkin, Harvey E. Liu, Guijian Shome, Debasish Cukrowska, Ewa Liousse, Catherine Pokrovsky, Oleg S. Streets, David G. TI Mercury Stable Isotope Signatures of World Coal Deposits and Historical Coal Combustion Emissions SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID MASS-INDEPENDENT FRACTIONATION; FIRED POWER-PLANTS; ATMOSPHERE; CHINA; HG AB Mercury (Hg) emissions from coal combustion contribute approximately half of anthropogenic Hg emissions to the atmosphere. With the implementation of the first legally binding UNEP treaty aimed at reducing anthropogenic Hg emissions, the identification and traceability of Hg emissions from different countries/regions are critically important. Here, we present a comprehensive world coal Hg stable isotope database including 108 new coal samples from major coal-producing deposits in South Africa, China, Europe, India, Indonesia, Mongolia, former USSR, and the U.S. A 4.7 parts per thousand range in delta Hg-202 (-3.9 to 0.8 parts per thousand) and a 1 parts per thousand range in Delta Hg-199 (-0.6 to 0.4 parts per thousand) are observed. Fourteen (p < 0.05) to 17 (p < 0.1) of the 28 pairwise comparisons between eight global regions are statistically distinguishable on the basis of delta Hg-202, Delta Hg-199 or both, highlighting the potential application of Hg isotope signatures to coal Hg emissions tracing. A revised coal combustion Hg isotope fractionation model is presented, and suggests that gaseous elemental coal Hg emissions are enriched in the heavier Hg isotopes relative to oxidized forms of emitted Hg. The model explains to first order the published delta Hg-202 observations on near-field Hg deposition from a power plant and global scale atmospheric gaseous Hg. Yet, model uncertainties appear too large at present to permit straightforward Hg isotope source identification of atmospheric forms of Hg. Finally, global historical (1850-2008) coal Hg isotope emission curves were modeled and indicate modern-day mean delta Hg-202 and Delta Hg-199 values for bulk coal emissions of -1.2 +/- 0.5 parts per thousand (1SD) and 0.05 +/- 0.06 parts per thousand (1SD). C1 [Sun, Ruoyu; Sonke, Jeroen E.; Heimbuerger, Lars-Eric; Pokrovsky, Oleg S.] Univ Toulouse, Observ Midi Pyrenees, Lab Geosci Environm Toulouse, CNRS,IRD, F-31400 Toulouse, France. [Sun, Ruoyu; Liu, Guijian] Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China. [Belkin, Harvey E.] US Geol Survey, Natl Ctr 956, Reston, VA 20192 USA. [Shome, Debasish] Jadavpur Univ, Dept Geol, Kolkata 700032, India. [Cukrowska, Ewa] Univ Witwatersrand, Sch Chem, Inst Mol Sci, ZA-2050 Johannesburg, South Africa. [Liousse, Catherine] Univ Toulouse, Observ Midi Pyrenees, Lab Aerol Toulouse, CNRS, F-31400 Toulouse, France. [Pokrovsky, Oleg S.] Tomsk State Univ, BIOGEOCLIM Lab, Tomsk 634050, Russia. [Streets, David G.] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Sun, RY (reprint author), Univ Toulouse, Observ Midi Pyrenees, Lab Geosci Environm Toulouse, CNRS,IRD, 14 Ave Edouard Belin, F-31400 Toulouse, France. EM roysun1986@gmail.com; sonke@get.obs-mip.fr RI Liu, Guijian/M-9597-2014; 若愚, 孙/F-3823-2010; OI 若愚, 孙/0000-0001-7261-8377; Heimburger, Lars-Eric/0000-0003-0632-5183; Belkin, Harvey/0000-0001-7879-6529 FU French Agence Nationale de Recherche [ANR-09-JCJC-0035-01]; European Research Council [ERC-2010-StG_20091028]; Midi-Pyrenees Observatory BQR grant; Chinese Scholarship Council; Fundamental Research Funds for the Central Universities [WK2080000062]; National Basic Research Program of China (973 Program) [2014CB238903]; National Natural Science Foundation of China [41173032, 41373110]; Tomsk State University [14.B25.31.0001] FX This work is supported by research grants ANR-09-JCJC-0035-01 from the French Agence Nationale de Recherche and ERC-2010-StG_20091028 from the European Research Council to JES, and a Midi-Pyrenees Observatory BQR grant to CL and JES. RS thank Chinese Scholarship Council for his PhD scholarship and support by the Fundamental Research Funds for the Central Universities (WK2080000062). GL acknowledges support from the National Basic Research Program of China (973 Program, 2014CB238903) and the National Natural Science Foundation of China (No. 41173032 and 41373110). Partial support from grant No. 14.B25.31.0001 of Tomsk State University is also acknowledged. We thank Reshmi Das for help with coal from India, Andrey Bychkov and Boris Pokrovsky for some coal samples from the USSR, Clinton Scott for help with USGS coal samples and Jerome Chmeleff for maintaining the OMP Neptune. We thank Nicholas Geboy and three anonymous reviewers for thoughtful comments. Any use of trade, product, or firm names is for descriptive purposes only and does not imply endorsement by the United States government. NR 39 TC 26 Z9 31 U1 9 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 1 PY 2014 VL 48 IS 13 BP 7660 EP 7668 DI 10.1021/es501208a PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AK5TG UT WOS:000338488700057 PM 24905585 ER PT J AU Clausen, H Nudelman, E Hakomori, SI AF Clausen, Henrik Nudelman, Edward Hakomori, Sen-itiroh TI Obituary: Steven Bruce Levery (1949-2014) SO GLYCOCONJUGATE JOURNAL LA English DT Biographical-Item C1 [Clausen, Henrik; Nudelman, Edward] Univ Copenhagen, Dept Cellular & Mol Med, Copenhagen, Denmark. [Hakomori, Sen-itiroh] Univ Washington, Pacific Northwest Res Inst, Div Biomembrane Res, Seattle, WA 98195 USA. [Hakomori, Sen-itiroh] Univ Washington, Dept Pathobiol, Seattle, WA 98195 USA. [Hakomori, Sen-itiroh] Univ Washington, Dept Global Hlth, Seattle, WA 98195 USA. RP Clausen, H (reprint author), Univ Copenhagen, Dept Cellular & Mol Med, Copenhagen, Denmark. EM hclau@sund.ku.dk; edward.nudelman@yahoo.com; hakomori@u.washington.edu NR 1 TC 0 Z9 0 U1 1 U2 4 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0282-0080 EI 1573-4986 J9 GLYCOCONJUGATE J JI Glycoconjugate J. PD JUL PY 2014 VL 31 IS 5 BP 339 EP 340 DI 10.1007/s10719-014-9531-0 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AK7XO UT WOS:000338641200002 PM 25105190 ER PT J AU Liu, ZK Jiang, J Zhou, B Wang, ZJ Zhang, Y Weng, HM Prabhakaran, D Mo, SK Peng, H Dudin, P Kim, T Hoesch, M Fang, Z Dai, X Shen, ZX Feng, DL Hussain, Z Chen, YL AF Liu, Z. K. Jiang, J. Zhou, B. Wang, Z. J. Zhang, Y. Weng, H. M. Prabhakaran, D. Mo, S-K. Peng, H. Dudin, P. Kim, T. Hoesch, M. Fang, Z. Dai, X. Shen, Z. X. Feng, D. L. Hussain, Z. Chen, Y. L. TI A stable three-dimensional topological Dirac semimetal Cd3As2 SO NATURE MATERIALS LA English DT Article ID INSULATORS; SUPERCONDUCTORS; PHASE AB Three-dimensional (3D) topological Dirac semimetals (TDSs) are a recently proposed state of quantum matter(1-6) that have attracted increasing attention in physics and materials science. A 3D TDS is not only a bulk analogue of graphene; it also exhibits non-trivial topology in its electronic structure that shares similarities with topological insulators. Moreover, a TDS can potentially be driven into other exotic phases (such as Weyl semimetals(1,7), axion insulators(1,4) and topological superconductors(8,9)), making it a unique parent compound for the study of these states and the phase transitions between them. Here, by performing angle-resolved photoemission spectroscopy, we directly observe a pair of 3D Dirac fermions in Cd3As2, proving that it is a model 3D TDS. Compared with other 3D TDSs, for example, beta-cristobalite BiO2 (ref. 3) and Na3Bi (refs 4,5), Cd3As2 is stable and has much higher Fermi velocities. Furthermore, by in situ doping we have been able to tune its Fermi energy, making it a flexible platform for exploring exotic physical phenomena. C1 [Liu, Z. K.; Zhang, Y.; Shen, Z. X.; Chen, Y. L.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Jiang, J.; Zhou, B.; Prabhakaran, D.; Peng, H.; Chen, Y. L.] Univ Oxford, Clarendon Lab, Phys Dept, Oxford OX1 3PU, England. [Jiang, J.; Feng, D. L.] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Jiang, J.; Feng, D. L.] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China. [Zhou, B.; Zhang, Y.; Mo, S-K.; Hussain, Z.; Chen, Y. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Wang, Z. J.; Weng, H. M.; Fang, Z.; Dai, X.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Wang, Z. J.; Weng, H. M.; Fang, Z.; Dai, X.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Dudin, P.; Kim, T.; Hoesch, M.; Chen, Y. L.] Diamond Light Source, Didcot OX11 0DE, Oxon, England. RP Chen, YL (reprint author), Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM Yulin.Chen@physics.ox.ac.uk RI Zhang, Yi/J-9025-2013; Peng, Han/I-4944-2013; Weng, Hongming/F-2948-2011; Dai, Xi/C-4236-2008; Mo, Sung-Kwan/F-3489-2013; Wang, Zhijun/O-8015-2014; Fang, Zhong/D-4132-2009 OI Zhang, Yi/0000-0003-1204-8717; Weng, Hongming/0000-0001-8021-9413; Dai, Xi/0000-0003-0538-1829; Mo, Sung-Kwan/0000-0003-0711-8514; Wang, Zhijun/0000-0003-2169-8068; FU EPSRC (UK) [EP/K04074X/1]; DARPA (US) MESO project [N66001-11-1-4105]; Department of Energy, Office of Basic Energy Science [DE-AC02-76SF00515, DE-AC02-05CH11231]; NSF of China; National Basic Research Program of China; International Science and Technology Cooperation Program of China; National Basic Research Program of China [2012CB921402]; China Scholarship Council FX Y.L.C. and B.Z. acknowledge the support from the EPSRC (UK) grant EP/K04074X/1 and a DARPA (US) MESO project (no. N66001-11-1-4105). Z.K.L. and Z.X.S. acknowledge support from the Department of Energy, Office of Basic Energy Science (contract DE-AC02-76SF00515). The Advanced Light Source is operated by the Department of Energy, Office of Basic Energy Science (contract DE-AC02-05CH11231). Z.F., X.D. and H.M.W. acknowledge the support by the NSF of China, the National Basic Research Program of China, and the International Science and Technology Cooperation Program of China. J.J. and D.L.F. acknowledge the support by the NSF of China, the National Basic Research Program of China under grant no. 2012CB921402. J.J. acknowledges the support from the China Scholarship Council. NR 30 TC 266 Z9 268 U1 53 U2 370 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD JUL PY 2014 VL 13 IS 7 BP 677 EP 681 DI 10.1038/NMAT3990 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AK5QY UT WOS:000338482300013 PM 24859642 ER PT J AU Mefford, JT Hardin, WG Dai, S Johnston, KP Stevenson, KJ AF Mefford, J. Tyler Hardin, William G. Dai, Sheng Johnston, Keith P. Stevenson, Keith J. TI Anion charge storage through oxygen intercalation in LaMnO3 perovskite pseudocapacitor electrodes SO NATURE MATERIALS LA English DT Article ID ELECTROCHEMICAL ENERGY-STORAGE; REDUCTION ACTIVITY; ELECTROCATALYSTS; SUPERCAPACITORS; NANOPARTICLES; PRINCIPLES; BATTERIES; EVOLUTION; SURFACES; BEHAVIOR AB Perovskite oxides have attracted significant attention as energy conversion materials for metal-air battery and solid-oxide fuel-cell electrodes owing to their unique physical and electronic properties. Amongst these unique properties is the structural stability of the cation array in perovskites that can accommodate mobile oxygen ions under electrical polarization. Despite oxygen ion mobility and vacancies having been shown to play an important role in catalysis, their role in charge storage has yet to be explored. Herein we investigate the mechanism of oxygen-vacancy-mediated redox pseudocapacitance for a nanostructured lanthanum-based perovskite, LaMnO3. This is the first example of anion-based intercalation pseudocapacitance as well as the first time oxygen intercalation has been exploited for fast energy storage. Whereas previous pseudocapacitor and rechargeable battery charge storage studies have focused on cation intercalation, the anion-based mechanism presented here offers a new paradigm for electrochemical energy storage. C1 [Mefford, J. Tyler; Stevenson, Keith J.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Hardin, William G.; Johnston, Keith P.; Stevenson, Keith J.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Dai, Sheng] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Johnston, Keith P.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Johnston, Keith P.; Stevenson, Keith J.] Univ Texas Austin, Ctr Electrochem, Austin, TX 78712 USA. RP Johnston, KP (reprint author), Univ Texas Austin, Texas Mat Inst, 1 Univ Stn, Austin, TX 78712 USA. EM kpj@che.utexas.edu; stevenson@cm.utexas.edu RI Dai, Sheng/K-8411-2015 OI Dai, Sheng/0000-0002-8046-3931 FU R. A. Welch Foundation [F-1529, F-1319]; Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - US Department of Energy, Office of Science; Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - US Department of Energy, Office of Basic Energy Sciences FX Financial support for this work was provided by the R. A. Welch Foundation (grants F-1529 and F-1319). S.D. was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, and Office of Basic Energy Sciences. NR 37 TC 72 Z9 73 U1 38 U2 313 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD JUL PY 2014 VL 13 IS 7 BP 726 EP 732 DI 10.1038/NMAT4000 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AK5QY UT WOS:000338482300021 PM 24880729 ER PT J AU McAndrews, HJ Thomsen, MF Arridge, CS Jackman, CM Wilson, RJ Henderson, MG Tokar, RL Khurana, KK Sittler, EC Coates, AJ Dougherty, MK AF McAndrews, H. J. Thomsen, M. F. Arridge, C. S. Jackman, C. M. Wilson, R. J. Henderson, M. G. Tokar, R. L. Khurana, K. K. Sittler, E. C. Coates, A. J. Dougherty, M. K. TI Plasma in Saturn's nightside magnetosphere and the implications for global circulation (vol 57, pg 1714, 2009) SO PLANETARY AND SPACE SCIENCE LA English DT Correction C1 [Thomsen, M. F.; Tokar, R. L.] Planetary Sci Inst, Tucson, AZ 85719 USA. [Arridge, C. S.; Coates, A. J.] Univ Coll London, Mullard Space Sci Lab, Dorking RH5 6NT, Surrey, England. [Arridge, C. S.; Coates, A. J.] UCL Birkbeck, Ctr Planetary Sci, London WC1E 6BT, England. [Jackman, C. M.] Univ Southampton, Dept Phys & Astron, Southampton SO17 1BJ, Hants, England. [Wilson, R. J.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80303 USA. [Henderson, M. G.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Khurana, K. K.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90095 USA. [Sittler, E. C.] NASA, Heliophys Sci Div, Geospace Phys Lab, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Dougherty, M. K.] Univ London Imperial Coll Sci Technol & Med, Space & Atmospher Phys Grp, London SW7 2BW, England. RP Thomsen, MF (reprint author), Planetary Sci Inst, Tucson, AZ 85719 USA. EM mthomsen@psi.edu RI Wilson, Rob/C-2689-2009; Arridge, Christopher/A-2894-2009; Coates, Andrew/C-2396-2008; Henderson, Michael/A-3948-2011 OI Wilson, Rob/0000-0001-9276-2368; Arridge, Christopher/0000-0002-0431-6526; Coates, Andrew/0000-0002-6185-3125; Henderson, Michael/0000-0003-4975-9029 NR 1 TC 4 Z9 4 U1 0 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0032-0633 J9 PLANET SPACE SCI JI Planet Space Sci. PD JUL PY 2014 VL 97 BP 86 EP 87 DI 10.1016/j.pss.2014.05.011 PG 2 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK7OS UT WOS:000338618200009 ER PT J AU Lin, F Montano, M Tian, CX Ji, YZ Nordlund, D Weng, TC Moore, RG Gillaspie, DT Jones, KM Dillon, AC Richards, RM Engtrakul, C AF Lin, Feng Montano, Manuel Tian, Chixia Ji, Yazhou Nordlund, Dennis Weng, Tsu-Chien Moore, Rob G. Gillaspie, Dane T. Jones, Kim M. Dillon, Anne C. Richards, Ryan M. Engtrakul, Chaiwat TI Electrochromic performance of nanocomposite nickel oxide counter electrodes containing lithium and zirconium SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article; Proceedings Paper CT 10th International Meeting on Electrochromism (IME) CY AUG 12-16, 2012 CL Holland, MI SP Sage Electrochrom, Pleotint LLC, Gentex Corp DE Nickel oxide; Nanocomposite; Oxidation state; Electrochromic; Li stoichiometry ID ULTRASONIC SPRAY DEPOSITION; RAY ABSORPTION-SPECTROSCOPY; THIN-FILMS; DEVICES; NI; WINDOWS; AL AB Nickel oxide materials are suitable for counter electrodes in complementary electrochromic devices. The state-of-the-art nickel oxide counter electrode materials are typically prepared with multiple additives to enhance peformance. Herein, nanocomposite nickel oxide counter electrodes were fabricated via RF magnetron co-sputtering from Ni-Zr alloy and Li2O ceramic targets. The as-deposited nanocomposite counter electrodes were characterized with inductively coupled plasma mass spectrometry (ICP-MS), scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HRTEM), X-ray diffraction (XRD), and X-ray absorption spectroscopy (XAS). It was found that the stoichiometry, crystal structure and electronic structure of the nickel oxide-based materials could be readily tuned by varying the Li2O sputter deposition power level. Comprehensive electrochromic evaluation demonstrated that the performance of the nickel oxide-based materials was dependent on the overall Li stoichiometry. Overall, the nanocomposite nickel oxide counter electrode containing lithium and zirconium synthesized with a Li2O deposition power of 45 W exhibited the optimal performance with an optical modulation of 71% and coloration efficiency of 30 cm(2)/C at 670 nm in Li-ion electrolyte. (C) 2014 Elsevier B.V. All rights reserved. C1 [Lin, Feng; Gillaspie, Dane T.; Jones, Kim M.; Dillon, Anne C.; Engtrakul, Chaiwat] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Lin, Feng; Ji, Yazhou; Richards, Ryan M.] Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. [Montano, Manuel; Tian, Chixia; Richards, Ryan M.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Nordlund, Dennis; Weng, Tsu-Chien] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Moore, Rob G.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. RP Engtrakul, C (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM chaiwat.engtrakul@nrel.gov RI Nordlund, Dennis/A-8902-2008; Richards, Ryan/B-3513-2008 OI Nordlund, Dennis/0000-0001-9524-6908; NR 26 TC 4 Z9 4 U1 2 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD JUL PY 2014 VL 126 SI SI BP 206 EP 212 DI 10.1016/j.solmat.2013.11.023 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AK4LB UT WOS:000338395100030 ER PT J AU Pehlivan, IB Marsal, R Pehlivan, E Runnerstrom, EL Milliron, DJ Granqvist, CG Niklasson, GA AF Pehlivan, Ilknur Bayrak Marsal, Roser Pehlivan, Esat Runnerstrom, Evan L. Milliron, Delia J. Granqvist, Claes G. Niklasson, Gunnar A. TI Electrochromic devices with polymer electrolytes functionalized by SiO2 and In2O3:Sn nanoparticles: Rapid coloring/bleaching dynamics and strong near-infrared absorption SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article; Proceedings Paper CT 10th International Meeting on Electrochromism (IME) CY AUG 12-16, 2012 CL Holland, MI SP Sage Electrochrom, Pleotint LLC, Gentex Corp DE Smart windows; Polymer electrolytes; Nanoparticles; Coloring/bleaching dynamics; Near-infrared absorption ID TUNGSTEN-OXIDE; OPTICAL-PROPERTIES; ION CONDUCTION; SMART WINDOWS; NICKEL-OXIDE; THIN-FILMS AB We studied the optical properties and coloring/bleaching dynamics of electrochromic devices based on tungsten oxide and nickel oxide and incorporating polymer electrolytes functionalized by adding about one percent of nanoparticles of SiO2 (fumed silica) or In2O3:Sn. SiO2 improved the coloring/bleaching dynamics and In2O3:Sn quenched the near-infrared transmittance. Both of these effects can be important in electrochromic smart windows, and our results point at the advantage of a polymer laminated construction over a monolithic one. (C) 2013 Elsevier B.V. All rights reserved. C1 [Pehlivan, Ilknur Bayrak; Granqvist, Claes G.; Niklasson, Gunnar A.] Uppsala Univ, Angstrom Lab, Dept Engn Sci, SE-75121 Uppsala, Sweden. [Marsal, Roser; Pehlivan, Esat] ChromoGenics AB, SE-75323 Uppsala, Sweden. [Runnerstrom, Evan L.; Milliron, Delia J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Runnerstrom, Evan L.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Pehlivan, IB (reprint author), Uppsala Univ, Angstrom Lab, Dept Engn Sci, POB 534, SE-75121 Uppsala, Sweden. EM ilknur.pehlivan@angstrom.uu.se RI Foundry, Molecular/G-9968-2014; Milliron, Delia/D-6002-2012; OI Niklasson, Gunnar/0000-0002-8279-5163 NR 28 TC 10 Z9 10 U1 5 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD JUL PY 2014 VL 126 SI SI BP 241 EP 247 DI 10.1016/j.solmat.2013.06.010 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AK4LB UT WOS:000338395100035 ER PT J AU Kronewitter, SR Slysz, GW Marginean, I Hagler, CD LaMarche, BL Zhao, R Harris, MY Monroe, ME Polyukh, CA Crowell, KL Fillmore, TL Carlson, TS Camp, DG Moore, RJ Payne, SH Anderson, GA Smith, RD AF Kronewitter, Scott R. Slysz, Gordon W. Marginean, Ioan Hagler, Clay D. LaMarche, Brian L. Zhao, Rui Harris, Myanna Y. Monroe, Matthew E. Polyukh, Christina A. Crowell, Kevin L. Fillmore, Thomas L. Carlson, Timothy S. Camp, David G., II Moore, Ronald J. Payne, Samuel H. Anderson, Gordon A. Smith, Richard D. TI GlyQ-IQ: Glycomics Quintavariate-Informed Quantification with High-Performance Computing and GlycoGrid 4D Visualization SO ANALYTICAL CHEMISTRY LA English DT Article ID MASS-SPECTROMETRY DATA; ELECTROSPRAY-IONIZATION; ANNOTATION; MS; SOFTWARE; SPECTRA; FRAGMENTATION; GLYCOSYLATION; HETEROGENEITY; GLYCANS AB Glycomics quintavariate-informed quantification (GlyQIQ) is a biologically guided glycomics analysis tool for identifying N-glycans in liquid chromatography-mass spectrometry (LC-MS) data. Glycomics LC-MS data sets have convoluted extracted ion chromatograms that are challenging to deconvolve with existing software tools. LC deconvolution into constituent pieces is critical in glycomics data sets because chromatographic peaks correspond to different intact glycan structural isomers. The biological targeted analysis approach offers several key advantages to traditional LC-MS data processing. A priori glycan information about the individual target's elemental composition allows for improved sensitivity by utilizing the exact isotope profile information to focus chromatogram generation and LC peak fitting on the isotopic species having the highest intensity. Glycan target annotation utilizes glycan family relationships and in source fragmentation in addition to high specificity feature LC-MS detection to improve the specificity of the analysis. The GlyQ-IQ software was developed in this work and evaluated in the context of profiling the N-glycan compositions from human serum LC-MS data sets. A case study is presented to demonstrate how GlyQ-IQ identifies and removes confounding chromatographic peaks from high mannose glycan isomers from human blood serum. In addition, GlyQ-IQ was used to generate a broad human serum N-glycan profile from a high resolution nanoelectrospray-liquid chromatography tandem mass spectrometry (nESI-LC-MS/MS) data set. A total of 156 glycan compositions and 640 glycan isomers were detected from a single sample. Over 99% of the GlyQ-IQ glycan-feature assignments passed manual validation and are backed with high-resolution mass spectra. C1 [Kronewitter, Scott R.; Slysz, Gordon W.; Marginean, Ioan; Hagler, Clay D.; LaMarche, Brian L.; Zhao, Rui; Harris, Myanna Y.; Monroe, Matthew E.; Polyukh, Christina A.; Crowell, Kevin L.; Fillmore, Thomas L.; Carlson, Timothy S.; Camp, David G., II; Moore, Ronald J.; Payne, Samuel H.; Anderson, Gordon A.; Smith, Richard D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Smith, RD (reprint author), Pacific NW Natl Lab, Div Biol Sci, POB 999, Richland, WA 99352 USA. EM rds@pnnl.gov RI Marginean, Ioan/A-4183-2008; Smith, Richard/J-3664-2012; OI Marginean, Ioan/0000-0002-6693-0361; Smith, Richard/0000-0002-2381-2349; Payne, Samuel/0000-0002-8351-1994 FU U.S. DOE office of Biological and Environmental Research Pan-omics project of the Genome Sciences Program; NIH GMS [P41 GM103493-11]; Microsoft Windows Azure Cloud Deployment; DOE [DE-AC05-76RLO 1830] FX Portions of this work were supported by the U.S. DOE office of Biological and Environmental Research Pan-omics project of the Genome Sciences Program, as well as by the NIH GMS Grant P41 GM103493-11. Work was performed in the EMSL, a DOE-BER national scientific user facility PNNL. High-performance computing research was performed using PNNL Institutional Computing at Pacific Northwest National Laboratory. The Microsoft Azure Research was made possible by a Windows Azure Research Pass Grant. We also acknowledge Daniel Fay and Wen-ming Ye from Microsoft Research (http://azure4research.com, Redmond, WA), Magnus Martensson from Martensson Consulting (Malmo, Sweden), and Alan Smith from Active Solutions (Stockholm, Sweden) for their expertise and support with the Microsoft Windows Azure Cloud Deployment. PNNL is a multiprogram national laboratory operated by Battelle Memorial Institute for the DOE under Contract DE-AC05-76RLO 1830. NR 26 TC 4 Z9 4 U1 0 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 1 PY 2014 VL 86 IS 13 BP 6268 EP 6276 DI 10.1021/ac501492f PG 9 WC Chemistry, Analytical SC Chemistry GA AK5TH UT WOS:000338488800017 PM 24881670 ER PT J AU Kelly, RT Wang, CC Rausch, SJ Lee, CS Tang, KQ AF Kelly, Ryan T. Wang, Chenchen Rausch, Sarah J. Lee, Cheng S. Tang, Keqi TI Pneumatic Microvalve-Based Hydrodynamic Sample Injection for High-Throughput, Quantitative Zone Electrophoresis in Capillaries SO ANALYTICAL CHEMISTRY LA English DT Article ID SINGLE-CELL ANALYSIS; MICROCHIP ELECTROPHORESIS; MASS-SPECTROMETRY; MICROFLUIDIC DEVICES; FLOW; SENSITIVITY; INTERFACE; DESIGN; CHIP AB A hybrid microchip/capillary electrophoresis (CE) system was developed to allow unbiased and lossless sample loading and high-throughput repeated injections. This new hybrid CE system consists of a poly(dimethylsiloxane) (PDMS) microchip sample injector featuring a pneumatic microvalve that separates a sample introduction channel from a short sample loading channel, and a fused-silica capillary separation column that connects seamlessly to the sample loading channel. The sample introduction channel is pressurized such that when the pneumatic microvalve opens briefly, a variable-volume sample plug is introduced into the loading channel. A high voltage for CE separation is continuously applied across the loading channel and the fused-silica capillary separation column. Analytes are rapidly separated in the fused-silica capillary, and following separation, high-sensitivity MS detection is accomplished via a sheathless CE/ESI-MS interface. The performance evaluation of the complete CE/ESI-MS platform demonstrated that reproducible sample injection with well controlled sample plug volumes could be achieved by using the PDMS microchip injector. The absence of band broadening from microchip to capillary indicated a minimum dead volume at the junction. The capabilities of the new CE/ESI-MS platform in performing high-throughput and quantitative sample analyses were demonstrated by the repeated sample injection without interrupting an ongoing separation and a linear dependence of the total analyte ion abundance on the sample plug volume using a mixture of peptide standards. The separation efficiency of the new platform was also evaluated systematically at different sample injection times, flow rates, and CE separation voltages. C1 [Kelly, Ryan T.; Rausch, Sarah J.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Tang, Keqi] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Wang, Chenchen; Lee, Cheng S.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. RP Kelly, RT (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM ryan.kelly@pnnl.gov RI wang, chenchen/B-5838-2015; Kelly, Ryan/B-2999-2008 OI Kelly, Ryan/0000-0002-3339-4443 FU NIH National Cancer Institute [1R33CA155252, R21 CA143177]; Department of Energy's Office of Biological and Environmental Research FX We thank Brandon Kelly for assistance with microfluidic device fabrication. The research described in this paper was conducted under the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL), a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy, and grants from the NIH National Cancer Institute (1R33CA155252 and R21 CA143177). The research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. NR 34 TC 8 Z9 8 U1 3 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 1 PY 2014 VL 86 IS 13 BP 6723 EP 6729 DI 10.1021/ac501910p PG 7 WC Chemistry, Analytical SC Chemistry GA AK5TH UT WOS:000338488800077 PM 24865952 ER PT J AU Xu, ZJ AF Xu, Zhijie TI A stochastic analysis of steady and transient heat conduction in random media using a homogenization approach SO APPLIED MATHEMATICAL MODELLING LA English DT Article DE Stochastic; Heat conduction; Homogenization; Random field; Uncertainty ID FINITE-ELEMENT-ANALYSIS; HETEROGENEOUS MATERIALS AB We present a new stochastic analysis for steady and transient one-dimensional heat conduction problem based on the homogenization approach. Thermal conductivity is assumed to be a random field K consisting of random variables of a total number N. Both steady and transient solutions Tare expressed in terms of the homogenized solution (T) over tilde and its spatial derivatives T(x,t) = (T) over tilde + Sigma L-infinity(n=1)n(x)partial derivative(n)(T) over tilde/partial derivative x(n), where homogenized solution (T) over tilde is obtained by solving the homogenized equation with effective thermal conductivity. Both mean and variance of stochastic solutions can be obtained analytically for K field consisting of independent identically distributed (i.i.d) random variables. The mean and variance of T are shown to be dependent only on the mean and variance of these i.i.d variables, not the particular form of probability distribution function of i.i.d variables. Variance of temperature field T can be separated into two contributions: the ensemble contribution (through the homogenized temperature (T) over tilde); and the configurational contribution (through the random variable L-n(x)). The configurational contribution is shown to be proportional to the local gradient of (T) over tilde. Large uncertainty of T field was found at locations with large gradient of (T) over tilde due to the significant configurational contributions at these locations. Numerical simulations were implemented based on a direct Monte Carlo method and good agreement is obtained between numerical Monte Carlo results and the proposed stochastic analysis. (C) 2013 Elsevier Inc. All rights reserved. C1 [Xu, Zhijie] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Xu, ZJ (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Computat Math Grp, Richland, WA 99352 USA. EM zhijiexu@hotmail.com RI Xu, Zhijie/A-1627-2009 OI Xu, Zhijie/0000-0003-0459-4531 NR 16 TC 1 Z9 1 U1 2 U2 11 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0307-904X EI 1872-8480 J9 APPL MATH MODEL JI Appl. Math. Model. PD JUL 1 PY 2014 VL 38 IS 13 BP 3233 EP 3243 DI 10.1016/j.apm.2013.11.044 PG 11 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA AK1MT UT WOS:000338179900014 ER PT J AU Riquelme, F Northrup, P Ruvalcaba-Sil, JL Stojanoff, V Siddons, DP Alvarado-Ortega, J AF Riquelme, Francisco Northrup, Paul Luis Ruvalcaba-Sil, Jose Stojanoff, Vivian Siddons, D. Peter Alvarado-Ortega, Jesus TI Insights into molecular chemistry of Chiapas amber using infrared-light microscopy, PIXE/RBS, and sulfur K-edge XANES spectroscopy SO APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING LA English DT Article ID HUMIC SUBSTANCES; ORGANIC-MATTER; SPECIATION; MEXICO; CLASSIFICATION; SOIL; SAMPLES; ORIGIN AB Chiapas amber is a natural occurring fossil resin structurally composed of long macromolecule chains with semicrystalline phases associated with both fossil and polymerization process. The most conspicuous characteristic of this fossil polymer is that it preserves ancient organic inclusions. In the present work, PIXE/RBS spectrometry (particle-induced X-ray emission/Rutherford backscattering) were combined with complementary K-edge XANES spectroscopy (X-ray absorption near-edge structure) to identify the amount of sulfur in Chiapas amber. Initially, the amber samples were examined using infrared reflected photomicrography. Amber is transparent to infrared light and so embedded plants and animals are easily visible, showing them in extraordinary detail, as if they were immersed in a water-like solution. The PIXE/RBS data show that the proportion of sulfur in amber is significantly higher than that found in recently formed resins, consistent with the biogeochemical process that transforms the resin into amber during long-term burial in geological deposits. The sulfur K-edge XANES spectra from amber confirm the sulfur abundance and reveal sulfur species in the reduced and intermediate oxidation states in amber. Almost no oxidized sulfur was found, whereas the recent resins show mostly oxidized sulfur fractions. This indicates that labile oxidized sulfur decays during fossilization and resin maturation must occur under conditions of oxygen depletion. The implications of the presence of sulfur in amber for organic preservation is also discussed here. Sulfur compounds work as a polymer additive that promotes intense resin solidification. This restricts the early oxidant-specific biodegradation of the embedded biomatter and, over geological time, provides greater stability against chemical changes. C1 [Riquelme, Francisco; Luis Ruvalcaba-Sil, Jose] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 20364, DF, Mexico. [Northrup, Paul] SUNY Stony Brook, Dept Geosci, Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY USA. [Stojanoff, Vivian; Siddons, D. Peter] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Alvarado-Ortega, Jesus] Univ Nacl Autonoma Mexico, Inst Geol, Mexico City 04510, DF, Mexico. RP Riquelme, F (reprint author), Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 20364, DF, Mexico. EM riquelme.fc@gmail.com OI Ruvalcaba-Sil, Jose Luis/0000-0003-1431-3019 FU CONACYT [131944 MOVIL II]; UNAM-PAPIIT [IN106011, IN403210] FX We thank Karim Lopez, Francisco Jaimes, and Mauricio Escobar, for their technical support during the experimental runs at the Pelletron Accelerator Laboratory, IF-UNAM. We also thank Dr. Lauro Bucio from IF-UNAM, for the valuable comments that enriched the manuscript discussion. We thank Biol. Gerardo Carbot and Biol. Marco A. Coutino, from the Museo de Paleontologia 'Eliseo Palacios Aguilera', Chiapas, they facilitated the holotype of H. allendis and sample T2. The editor and referees provided useful suggestions that improved the manuscript. This research is part of the PhD-granting program in Biological Sciences at the UNAM, financially supported by CONACYT, also partially supported by UNAM-PAPIIT IN106011 and IN403210 grants, as well as CONACYT 131944 MOVIL II endowment. NR 47 TC 9 Z9 9 U1 2 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0947-8396 EI 1432-0630 J9 APPL PHYS A-MATER JI Appl. Phys. A-Mater. Sci. Process. PD JUL PY 2014 VL 116 IS 1 BP 97 EP 109 DI 10.1007/s00339-013-8185-2 PG 13 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AK1YC UT WOS:000338214300014 ER PT J AU Webster, KD Ng, WP Fletcher, DA AF Webster, Kevin D. Ng, Win Pin Fletcher, Daniel A. TI Tensional Homeostasis in Single Fibroblasts SO BIOPHYSICAL JOURNAL LA English DT Article ID ACTIN-FILAMENTS; CELLULAR STIFFNESS; MECHANICAL FORCE; ALPHA-ACTININ; LIVING CELLS; DYNAMICS; STRESS; MECHANOTRANSDUCTION; MECHANOBIOLOGY; CONTRACTILITY AB Adherent cells generate forces through acto-myosin contraction to move, change shape, and sense the mechanical properties of their environment. They are thought to maintain defined levels of tension with their surroundings despite mechanical perturbations that could change tension, a concept known as tensional homeostasis. Misregulation of tensional homeostasis has been proposed to drive disorganization of tissues and promote progression of diseases such as cancer. However, whether tensional homeostasis operates at the single cell level is unclear. Here, we directly test the ability of single fibroblast cells to regulate tension when subjected to mechanical displacements in the absence of changes to spread area or substrate elasticity. We use a feedback-controlled atomic force microscope to measure and modulate forces and displacements of individual contracting cells as they spread on a fibronectin-patterned atomic-force microscope cantilever and coverslip. We find that the cells reach a steady-state contraction force and height that is insensitive to stiffness changes as they fill the micro-patterned areas. Rather than maintaining a constant tension, the fibroblasts altered their contraction force in response to mechanical displacement in a strain-rate-dependent manner, leading to a new and stable steady-state force and height. This' response is influenced by overexpression of the actin crosslinker alpha-actinin, and rheology measurements reveal that changes in cell elasticity are also strain- rate-dependent. Our finding of tensional buffering, rather than homeostasis, allows cells to transition between different tensional states depending on how they are displaced, permitting distinct responses to slow deformations during tissue growth and rapid deformations associated with injury. C1 [Webster, Kevin D.; Fletcher, Daniel A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Webster, Kevin D.; Ng, Win Pin; Fletcher, Daniel A.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Ng, Win Pin; Fletcher, Daniel A.] Univ Calif Berkeley Univ Calif San Francisco Grad, Berkeley, CA USA. [Fletcher, Daniel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Fletcher, DA (reprint author), Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. EM fletch@berkeley.edu FU National Science Foundation Biomechanics & Mechanobiology program [1235569]; National Institutes of Health Bay Area Physical Sciences Oncology Center FX This work was supported by the National Science Foundation Biomechanics & Mechanobiology program (grant No. 1235569) and the National Institutes of Health Bay Area Physical Sciences Oncology Center. NR 53 TC 14 Z9 14 U1 1 U2 14 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JUL 1 PY 2014 VL 107 IS 1 BP 146 EP 155 DI 10.1016/j.bpj.2014.04.051 PG 10 WC Biophysics SC Biophysics GA AK4RK UT WOS:000338411600018 PM 24988349 ER PT J AU Alam, TM Liao, ZL Zakharov, LN Nyman, M AF Alam, Todd M. Liao, Zuolei Zakharov, Lev N. Nyman, May TI Solid-State Dynamics of Uranyl Polyoxometalates SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE ion-exchange; polyoxometalate; proton MAS NMR; solid-state NMR; uranyl ID DIAMAGNETIC URANIUM-COMPOUNDS; SHIELDING CALCULATIONS; PEROXIDE NANOCAPSULES; PERIODIC-TABLE; METAL; NMR; NANOPARTICLES; NANOCLUSTERS; MONOLAYER; CATIONS AB Understanding fundamental uranyl polyoxometalate (POM) chemistry in solution and the solid state is the first step to defining its future role in the development of new actinide materials and separation processes that are vital to every step of the nuclear fuel cycle. Many solid-state geometries of uranyl POMs have been described, but we are only beginning to understand their chemical behavior, which thus far includes the role of templates in their self-assembly, and the dynamics of encapsulated species in solution. This study provides unprecedented detail into the exchange dynamics of the encapsulated species in the solid state through Magic Angle Spinning Nuclear Magnetic Resonance (MAS NMR) spectroscopy. Although it was previously recognized that capsule-like molybdate and uranyl POMs exchange encapsulated species when dissolved in water, analogous exchange in the solid state has not been documented, or even considered. Here, we observe the extremely high rate of transport of Li+ and aqua species across the uranyl shell in the solid state, a process that is affected by both temperature and pore blocking by larger species. These results highlight the untapped potential of emergent f-block element materials and vesicle-like POMs. C1 [Alam, Todd M.] Sandia Natl Labs, Dept Elect Opt & Nanostruct Mat, Albuquerque, NM 87185 USA. [Liao, Zuolei; Zakharov, Lev N.; Nyman, May] Oregon State Univ, Frontier Res Ctr, Dept Chem & Mat Sci Actinides, Corvallis, OR 97331 USA. RP Alam, TM (reprint author), Sandia Natl Labs, Dept Elect Opt & Nanostruct Mat, POB 5800, Albuquerque, NM 87185 USA. EM tmalam@sandia.gov; May.Nyman@oregonstate.edu FU Materials Science of Actinides, an Energy Frontier Research Center - Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001089]; U. S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported as part of the Materials Science of Actinides, an Energy Frontier Research Center funded by the Department of Energy, Office of Science, Office of Basic Energy Sciences under award number DE-SC0001089. The NMR component of the work (T.M.A.) was performed at Sandia National Laboratories, which is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin company, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 24 TC 8 Z9 8 U1 6 U2 46 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUL 1 PY 2014 VL 20 IS 27 BP 8302 EP 8307 DI 10.1002/chem.201402351 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AJ9HO UT WOS:000338019300011 PM 24889825 ER PT J AU Chylek, P Dubey, MK Lesins, G Li, JN Hengartner, N AF Chylek, Petr Dubey, Manvendra K. Lesins, Glen Li, Jiangnan Hengartner, Nicolas TI Imprint of the Atlantic multi-decadal oscillation and Pacific decadal oscillation on southwestern US climate: past, present, and future SO CLIMATE DYNAMICS LA English DT Article ID SURFACE AIR-TEMPERATURE; NORTH-ATLANTIC; MULTIDECADAL OSCILLATION; THERMOHALINE CIRCULATION; 21ST-CENTURY DROUGHT; VARIABILITY; MODEL; HOLOCENE; AMERICA; SYSTEM AB The surface air temperature increase in the southwestern United States was much larger during the last few decades than the increase in the global mean. While the global temperature increased by about 0.5 A degrees C from 1975 to 2000, the southwestern US temperature increased by about 2 A degrees C. If such an enhanced warming persisted for the next few decades, the southwestern US would suffer devastating consequences. To identify major drivers of southwestern climate change we perform a multiple-linear regression of the past 100 years of the southwestern US temperature and precipitation. We find that in the early twentieth century the warming was dominated by a positive phase of the Atlantic multi-decadal oscillation (AMO) with minor contributions from increasing solar irradiance and concentration of greenhouse gases. The late twentieth century warming was about equally influenced by increasing concentration of atmospheric greenhouse gases (GHGs) and a positive phase of the AMO. The current southwestern US drought is associated with a near maximum AMO index occurring nearly simultaneously with a minimum in the Pacific decadal oscillation (PDO) index. A similar situation occurred in mid-1950s when precipitation reached its minimum within the instrumental records. If future atmospheric concentrations of GHGs increase according to the IPCC scenarios (Solomon et al. in Climate change 2007: working group I. The Physical Science Basis, Cambridge, 996 pp, 2007), climate models project a fast rate of southwestern warming accompanied by devastating droughts (Seager et al. in Science 316:1181-1184, 2007; Williams et al. in Nat Clim Chang, 2012). However, the current climate models have not been able to predict the behavior of the AMO and PDO indices. The regression model does support the climate models (CMIP3 and CMIP5 AOGCMs) projections of a much warmer and drier southwestern US only if the AMO changes its 1,000 years cyclic behavior and instead continues to rise close to its 1975-2000 rate. If the AMO continues its quasi-cyclic behavior the US SW temperature should remain stable and the precipitation should significantly increase during the next few decades. C1 [Chylek, Petr; Dubey, Manvendra K.; Hengartner, Nicolas] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lesins, Glen] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS, Canada. [Li, Jiangnan] Environm Canada, Canadian Ctr Climate Modeling & Anal, Victoria, BC, Canada. RP Chylek, P (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM chylek@lanl.gov RI Dubey, Manvendra/E-3949-2010; Li, Jiangnan/J-6262-2016 OI Dubey, Manvendra/0000-0002-3492-790X; FU Los Alamos National Laboratory Institute of Geophysics, Planetary Physics, and Signatures [LA-UR-12-25073] FX Reported research (LA-UR-12-25073) was supported in part by the Los Alamos National Laboratory Institute of Geophysics, Planetary Physics, and Signatures. NR 59 TC 14 Z9 14 U1 6 U2 56 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0930-7575 EI 1432-0894 J9 CLIM DYNAM JI Clim. Dyn. PD JUL PY 2014 VL 43 IS 1-2 BP 119 EP 129 DI 10.1007/s00382-013-1933-3 PG 11 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3PS UT WOS:000338337700008 ER PT J AU MacMartin, DG Kravitz, B Keith, DW Jarvis, A AF MacMartin, Douglas G. Kravitz, Ben Keith, David W. Jarvis, Andrew TI Dynamics of the coupled human-climate system resulting from closed-loop control of solar geoengineering SO CLIMATE DYNAMICS LA English DT Article DE Geoengineering; Solar radiation management; Dynamics; Feedback; Control ID CONTROL PERSPECTIVE; MODEL; OCEAN AB If solar radiation management (SRM) were ever implemented, feedback of the observed climate state might be used to adjust the radiative forcing of SRM in order to compensate for uncertainty in either the forcing or the climate response. Feedback might also compensate for unexpected changes in the system, e.g. a nonlinear change in climate sensitivity. However, in addition to the intended response to greenhouse-gas induced changes, the use of feedback would also result in a geoengineering response to natural climate variability. We use a box-diffusion dynamic model of the climate system to understand how changing the properties of the feedback control affect the emergent dynamics of this coupled human-climate system, and evaluate these predictions using the HadCM3L general circulation model. In particular, some amplification of natural variability is unavoidable; any time delay (e.g., to average out natural variability, or due to decision-making) exacerbates this amplification, with oscillatory behavior possible if there is a desire for rapid correction (high feedback gain). This is a challenge for policy as a delayed response is needed for decision making. Conversely, the need for feedback to compensate for uncertainty, combined with a desire to avoid excessive amplification of natural variability, results in a limit on how rapidly SRM could respond to changes in the observed state of the climate system. C1 [MacMartin, Douglas G.] CALTECH, Pasadena, CA 91125 USA. [Kravitz, Ben] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Keith, David W.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Keith, David W.] Harvard Univ, Kennedy Sch Govt, Cambridge, MA 02138 USA. [Jarvis, Andrew] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England. RP MacMartin, DG (reprint author), CALTECH, 1200 E Calif Blvd,M-C 107-81, Pasadena, CA 91125 USA. EM macmardg@cds.caltech.edu RI Kravitz, Ben/P-7925-2014; MacMartin, Douglas/A-6333-2016 OI Kravitz, Ben/0000-0001-6318-1150; MacMartin, Douglas/0000-0003-1987-9417 FU Fund for Innovative Climate and Energy Research; U S. Department of Energy by Battelle Memorial Institute [DE-AC05-76RLO1830] FX Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research. The Pacific Northwest National Laboratory is operated for the U S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RLO1830. Peter Thompson of Systems Technology Inc. provided assistance with the content of Appendix 2. NR 33 TC 17 Z9 17 U1 2 U2 20 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0930-7575 EI 1432-0894 J9 CLIM DYNAM JI Clim. Dyn. PD JUL PY 2014 VL 43 IS 1-2 BP 243 EP 258 DI 10.1007/s00382-013-1822-9 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AK3PS UT WOS:000338337700016 ER PT J AU He, L Cornelius, CJ Perahia, D AF He, Lliin Cornelius, Chris J. Perahia, Dvora TI Water dynamics within a highly rigid sulfonated polyphenylene SO EUROPEAN POLYMER JOURNAL LA English DT Article DE Water molecules; Polyphenylene ionomers; Pulse field gradient (PFG) NMR; FFIR ID STUDYING TRANSLATIONAL DIFFUSION; POLYMER-ELECTROLYTE MEMBRANES; NUCLEAR-MAGNETIC-RESONANCE; FUEL-CELLS; FIELD GRADIENT; IONOMER MEMBRANES; TRANSPORT; NAFION; ION; MECHANISMS AB Complex water molecule interactions within the confined environments of a sulfonated polyphenylene (sPP) ionomer were studied using H-1 nuclear magnetic resonance (NMR), and Fourier transform infrared (FTIR) spectroscopy. Multiple water environments were observed due to variations in hydrophilicity created by its structure, and chemical composition. Confined water properties are strongly dependent upon water content, degree of ionization, and temperature. Increasing the degree of sulfonation (DS) results in the creation of more water states and sites. The chemical shifts of water depend upon its environment with a smaller dependence on temperature. Confined water relaxation time T-1 is than significantly lower bulk water and increases with temperature. Pulse field gradient (PFG) NMR studies reveals that water self-diffusion coefficients increase with. Water molecules diffuse faster in sPP than Nafion, which implies that diffusion is facilitated by bundled hydrophilic pathways. Time-dependent FTIR reveals that bound water evaporates slower than unbound water during drying, which illustrates the difference of bulk and confined water within sPP ionomers. Hindered water evaporation is due to a reduction in the degrees of freedom for ion containing domains and mass transfer limitations at interfacial boundaries between hydrophobic and hydrophilic domains. (C) 2014 Elsevier Ltd. All rights reserved. C1 [He, Lliin] Oak Ridge Natl Lab, Neutron Scattering Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Cornelius, Chris J.] Univ Nebraska, Dept Chem & Biomol Engn, Lincoln, NE 68588 USA. [He, Lliin; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. RP Perahia, D (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. EM ccornelius2@unl.edu; dperahi@clemson.edu OI He, Lilin/0000-0002-9560-8101 FU DOE [DE-FG02-12ER46843]; Sharp Corporation FX The authors gratefully acknowledge financial support from DOE Grant No. DE-FG02-12ER46843, and support from Sharp Corporation. NR 34 TC 1 Z9 1 U1 4 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0014-3057 EI 1873-1945 J9 EUR POLYM J JI Eur. Polym. J. PD JUL PY 2014 VL 56 BP 168 EP 173 DI 10.1016/j.eurpolymj.2014.03.035 PG 6 WC Polymer Science SC Polymer Science GA AK4JW UT WOS:000338392000016 ER PT J AU Arthur, RK Ma, LJ Slattery, M Spokony, RF Ostapenko, A Negre, N White, KP AF Arthur, Robert K. Ma, Lijia Slattery, Matthew Spokony, Rebecca F. Ostapenko, Alexander Negre, Nicolas White, Kevin P. TI Evolution of H3K27me3-marked chromatin is linked to gene expression evolution and to patterns of gene duplication and diversification SO GENOME RESEARCH LA English DT Article ID TRANSCRIPTION FACTOR-BINDING; FUNCTIONAL-ORGANIZATION; HISTONE MODIFICATIONS; DROSOPHILA GENOME; DIVERGENCE; CONSERVATION; POLYCOMB; SEQUENCES; PROTEINS; INSIGHTS AB Histone modifications are critical for the regulation of gene expression, cell type specification, and differentiation. However, evolutionary patterns of key modifications that regulate gene expression in differentiating organisms have not been examined. Here we mapped the genomic locations of the repressive mark histone 3 lysine 27 trimethylation (H3K27me3) in four species of Drosophila, and compared these patterns to those in C. elegans. We found that patterns of H3K27me3 are highly conserved across species, but conservation is substantially weaker among duplicated genes. We further discovered that retropositions are associated with greater evolutionary changes in H3K27me3 and gene expression than tandem duplications, indicating that local chromatin constraints influence duplicated gene evolution. These changes are also associated with concomitant evolution of gene expression. Our findings reveal the strong conservation of genomic architecture governed by an epigenetic mark across distantly related species and the importance of gene duplication in generating novel H3K27me3 profiles. C1 [Arthur, Robert K.; White, Kevin P.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Arthur, Robert K.; Ma, Lijia; Slattery, Matthew; Spokony, Rebecca F.; Ostapenko, Alexander; Negre, Nicolas; White, Kevin P.] Univ Chicago, Inst Genom & Syst Biol, Chicago, IL 60637 USA. [Arthur, Robert K.; Ma, Lijia; Slattery, Matthew; Spokony, Rebecca F.; Ostapenko, Alexander; Negre, Nicolas; White, Kevin P.] Argonne Natl Lab, Chicago, IL 60637 USA. [Ma, Lijia; Slattery, Matthew; Spokony, Rebecca F.; Ostapenko, Alexander; Negre, Nicolas; White, Kevin P.] Univ Chicago, Dept Human Genet, Chicago, IL 60637 USA. [Slattery, Matthew] Univ Minnesota, Sch Med, Dept Biomed Sci, Duluth, MN 55455 USA. [Spokony, Rebecca F.] CUNY, Baruch Coll, Dept Nat Sci, New York, NY 10010 USA. [Negre, Nicolas] Univ Montpellier 2, F-34095 Montpellier, France. [Negre, Nicolas] INRA, DGIMI, UMR1333, F-34095 Montpellier, France. RP White, KP (reprint author), Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. EM kpwhite@uchicago.edu OI Negre, Nicolas/0000-0001-9727-3416 FU NIH [U01HG004264, T32GM007197]; NSF FX The modENCODE Project was supported by NIH grant U01HG004264 awarded to K. P. W. R. K. A. was supported by an NSF Graduate Research Fellowship and an NIH training grant (T32GM007197). We thank Jason Lieb and his laboratory for use of the C. elegans H3K27me3 ChIP-seq data. We are grateful to Benjamin Krinsky and Manyuan Long for interesting discussions on gene duplication. We thank Kacy Gordon, Aashish Jha, and Xiaochun Ni for helpful comments and critical review of our manuscript. We are indebted to many members of the White and Ruvinsky laboratories for useful criticism, wonderful discussions, and technical help. Finally, we appreciate the comments of three anonymous reviewers whose feedback greatly improved the paper. NR 54 TC 5 Z9 5 U1 0 U2 13 PU COLD SPRING HARBOR LAB PRESS, PUBLICATIONS DEPT PI COLD SPRING HARBOR PA 1 BUNGTOWN RD, COLD SPRING HARBOR, NY 11724 USA SN 1088-9051 EI 1549-5469 J9 GENOME RES JI Genome Res. PD JUL PY 2014 VL 24 IS 7 BP 1115 EP 1124 DI 10.1101/gr.162008.113 PG 10 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity GA AK1OS UT WOS:000338185000006 PM 24985914 ER PT J AU Chen, ZX Sturgill, D Qu, JX Jiang, HY Park, S Boley, N Suzuki, AM Fletcher, AR Plachetzki, DC FitzGerald, PC Artieri, CG Atallah, J Barmina, O Brown, JB Blankenburg, KP Clough, E Dasgupta, A Gubbala, S Han, Y Jayaseelan, JC Kalra, D Kim, YA Kovar, CL Lee, SL Li, MM Malley, JD Malone, JH Mathew, T Mattiuzzo, NR Munidasa, M Muzny, DM Ongeri, F Perales, L Przytycka, TM Pu, LL Robinson, G Thornton, RL Saada, N Scherer, SE Smith, HE Vinson, C Warner, CB Worley, KC Wu, YQ Zou, XY Cherbas, P Kellis, M Eisen, MB Piano, F Kionte, K Fitch, DH Sternberg, PW Cutter, AD Duff, MO Hoskins, RA Graveley, BR Gibbs, RA Bickel, PJ Kopp, A Carninci, P Celniker, SE Oliver, B Richards, S AF Chen, Zhen-Xia Sturgill, David Qu, Jiaxin Jiang, Huaiyang Park, Soo Boley, Nathan Suzuki, Ana Maria Fletcher, Anthony R. Plachetzki, David C. FitzGerald, Peter C. Artieri, Carlo G. Atallah, Joel Barmina, Olga Brown, James B. Blankenburg, Kerstin P. Clough, Emily Dasgupta, Abhijit Gubbala, Sai Han, Yi Jayaseelan, Joy C. Kalra, Divya Kim, Yoo-Ah Kovar, Christie L. Lee, Sandra L. Li, Mingmei Malley, James D. Malone, John H. Mathew, Tittu Mattiuzzo, Nicolas R. Munidasa, Mala Muzny, Donna M. Ongeri, Fiona Perales, Lora Przytycka, Teresa M. Pu, Ling-Ling Robinson, Garrett Thornton, Rebecca L. Saada, Nehad Scherer, Steven E. Smith, Harold E. Vinson, Charles Warner, Crystal B. Worley, Kim C. Wu, Yuan-Qing Zou, Xiaoyan Cherbas, Peter Kellis, Manolis Eisen, Michael B. Piano, Fabio Kionte, Karin Fitch, David H. Sternberg, Paul W. Cutter, Asher D. Duff, Michael O. Hoskins, Roger A. Graveley, Brenton R. Gibbs, Richard A. Bickel, Peter J. Kopp, Artyom Carninci, Piero Celniker, Susan E. Oliver, Brian Richards, Stephen TI Comparative validation of the D. melanogaster modENCODE transcriptome annotation SO GENOME RESEARCH LA English DT Article ID DROSOPHILA-MELANOGASTER; GENE-EXPRESSION; HUMAN GENOME; JUNK DNA; EVOLUTIONARY DYNAMICS; RNA-POLYMERASE; CAP-ANALYSIS; START SITE; ENCODE; SEQUENCE AB Accurate gene model annotation of reference genomes is critical for making them useful. The modENCODE project has improved the D. melanogaster genome annotation by using deep and diverse high-throughput data. Since transcriptional activity that has been evolutionarily conserved is likely to have an advantageous function, we have performed large-scale interspecific comparisons to increase confidence in predicted annotations. To support comparative genomics, we filled in divergence gaps in the Drosophila phylogeny by generating draft genomes for eight new species. For comparative transcriptome analysis, we generated mRNA expression profiles on 81 samples from multiple tissues and developmental stages of 15 Drosophila species, and we performed cap analysis of gene expression in D. melanogaster and D. pseudoobscura. We also describe conservation of four distinct core promoter structures composed of combinations of elements at three positions. Overall, each type of genomic feature shows a characteristic divergence rate relative to neutral models, highlighting the value of multispecies alignment in annotating a target genome that should prove useful in the annotation of other high priority genomes, especially human and other mammalian genomes that are rich in noncoding sequences. We report that the vast majority of elements in the annotation are evolutionarily conserved, indicating that the annotation will be an important springboard for functional genetic testing by the Drosophila community. C1 [Chen, Zhen-Xia; Sturgill, David; Artieri, Carlo G.; Clough, Emily; Malone, John H.; Mattiuzzo, Nicolas R.; Smith, Harold E.; Oliver, Brian] NIDDK, NIH, Bethesda, MD 20892 USA. [Qu, Jiaxin; Jiang, Huaiyang; Blankenburg, Kerstin P.; Gubbala, Sai; Han, Yi; Jayaseelan, Joy C.; Kalra, Divya; Kovar, Christie L.; Lee, Sandra L.; Li, Mingmei; Mathew, Tittu; Munidasa, Mala; Muzny, Donna M.; Ongeri, Fiona; Perales, Lora; Pu, Ling-Ling; Thornton, Rebecca L.; Saada, Nehad; Scherer, Steven E.; Warner, Crystal B.; Worley, Kim C.; Wu, Yuan-Qing; Zou, Xiaoyan; Gibbs, Richard A.; Richards, Stephen] Baylor Coll Med, Human Genome Sequencing Ctr, Houston, TX 77030 USA. [Park, Soo; Hoskins, Roger A.; Celniker, Susan E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Div Life Sci, Berkeley, CA 94720 USA. [Boley, Nathan; Brown, James B.; Robinson, Garrett; Bickel, Peter J.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Suzuki, Ana Maria; Carninci, Piero] RIKEN Omics Sci Ctr, Technol Dev Grp, Yokohama, Kanagawa 2300045, Japan. [Suzuki, Ana Maria; Carninci, Piero] RIKEN Ctr Life Sci Technol, Div Genom Technol, Yokohama, Kanagawa 2300045, Japan. [Fletcher, Anthony R.; Malley, James D.] NIH, Div Computat Biosci, Ctr Informat Technol, Bethesda, MD 20814 USA. [Plachetzki, David C.; Atallah, Joel; Barmina, Olga; Kopp, Artyom] Univ Calif Davis, Dept Ecol & Evolut, Davis, CA 95616 USA. [FitzGerald, Peter C.; Vinson, Charles] NCI, NIH, Bethesda, MD 20892 USA. [Dasgupta, Abhijit] NIAMSD, Clin Trials & Outcomes Branch, NIH, Bethesda, MD 20892 USA. [Kim, Yoo-Ah; Przytycka, Teresa M.] NIH, Natl Ctr Biotechnol Informat, Natl Lib Med, Bethesda, MD 20892 USA. [Cherbas, Peter] Indiana Univ, Dept Biol, Bloomington, IN 47405 USA. [Kellis, Manolis] MIT, Comp Sci & Artificial Intelligence Lab, Cambridge, MA 02139 USA. [Eisen, Michael B.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Piano, Fabio; Kionte, Karin; Fitch, David H.] New York Univ, Dept Biol, New York, NY 10003 USA. [Sternberg, Paul W.] CALTECH, HHMI, Pasadena, CA 91125 USA. [Sternberg, Paul W.] CALTECH, Div Biol, Pasadena, CA 91125 USA. [Cutter, Asher D.] Univ Toronto, Dept Ecol & Evolutionary Biol, Toronto, ON M5S 3B2, Canada. [Duff, Michael O.; Graveley, Brenton R.] Univ Connecticut, Inst Syst Genom, Dept Genet & Dev Biol, Ctr Hlth, Farmington, CT 06030 USA. RP Oliver, B (reprint author), NIDDK, NIH, Bethesda, MD 20892 USA. EM briano@helix.nih.gov RI Cutter, Asher/A-5647-2009; Carninci, Piero/K-1568-2014; Kalra, Divya/N-5453-2014; JAYASEELAN, JOY CHRISTINA/F-9824-2015; Brown, James/H-2971-2015; OI Carninci, Piero/0000-0001-7202-7243; JAYASEELAN, JOY CHRISTINA/0000-0002-7759-0139; Graveley, Brenton/0000-0001-5777-5892 FU Intramural Research Programs of the National Institutes of Health, NIDDK [DK015600-18]; extramural National Institutes of Health program [1ROIGM082843, U01HB004271] FX We thank modENCODE and laboratory members for discussion. This research was supported by the Intramural Research Programs of the National Institutes of Health, NIDDK (DK015600-18 to B.O.) and by the extramural National Institutes of Health program (1ROIGM082843 to A. K.; U01HB004271 to S. E. C.). This study utilized the high-performance computational capabilities of the Biowulf Linux cluster at the National Institutes of Health, Bethesda, Maryland (http://biowulf.nih.gov). NR 65 TC 33 Z9 33 U1 1 U2 18 PU COLD SPRING HARBOR LAB PRESS, PUBLICATIONS DEPT PI COLD SPRING HARBOR PA 1 BUNGTOWN RD, COLD SPRING HARBOR, NY 11724 USA SN 1088-9051 EI 1549-5469 J9 GENOME RES JI Genome Res. PD JUL PY 2014 VL 24 IS 7 BP 1209 EP 1223 DI 10.1101/gr.159384.113 PG 15 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity GA AK1OS UT WOS:000338185000014 PM 24985915 ER PT J AU Lin, F Fardad, M Jovanovic, MR AF Lin, Fu Fardad, Makan Jovanovic, Mihailo R. TI Algorithms for Leader Selection in Stochastically Forced Consensus Networks SO IEEE TRANSACTIONS ON AUTOMATIC CONTROL LA English DT Article DE Alternating direction method of multipliers (ADMMs); consensus networks; convex optimization; convex relaxations; greedy algorithm; leader selection; performance bounds; semidefinite programming (SDP); sensor selection; variance amplification ID SEMIDEFINITE RELAXATION; RELATIVE MEASUREMENTS; MULTIAGENT SYSTEMS; AVERAGE CONSENSUS; GRAPH; CONTROLLABILITY; OPTIMIZATION; PERFORMANCE; COHERENCE AB We are interested in assigning a pre-specified number of nodes as leaders in order to minimize the mean-square deviation from consensus in stochastically forced networks. This problem arises in several applications including control of vehicular formations and localization in sensor networks. For networks with leaders subject to noise, we show that the Boolean constraints (which indicate whether a node is a leader) are the only source of nonconvexity. By relaxing these constraints to their convex hull we obtain a lower bound on the global optimal value. We also use a simple but efficient greedy algorithm to identify leaders and to compute an upper bound. For networks with leaders that perfectly follow their desired trajectories, we identify an additional source of nonconvexity in the form of a rank constraint. Removal of the rank constraint and relaxation of the Boolean constraints yields a semidefinite program for which we develop a customized algorithm well-suited for large networks. Several examples ranging from regular lattices to random graphs are provided to illustrate the effectiveness of the developed algorithms. C1 [Lin, Fu] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Fardad, Makan] Syracuse Univ, Dept Elect Engn & Comp Sci, Syracuse, NY 13244 USA. [Jovanovic, Mihailo R.] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. RP Lin, F (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM fulin@mcs.anl.gov; makan@syr.edu; mihailo@umn.edu FU National Science Foundation under CAREER [CMMI-06-44793, CMMI-09-27720, CMMI-0927509] FX This work was supported by the National Science Foundation under CAREER Award CMMI-06-44793 and under awards CMMI-09-27720 and CMMI-0927509. Recommended by Associate Editor D. Bauso. NR 53 TC 32 Z9 32 U1 3 U2 19 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9286 EI 1558-2523 J9 IEEE T AUTOMAT CONTR JI IEEE Trans. Autom. Control PD JUL PY 2014 VL 59 IS 7 BP 1789 EP 1802 DI 10.1109/TAC.2014.2314223 PG 14 WC Automation & Control Systems; Engineering, Electrical & Electronic SC Automation & Control Systems; Engineering GA AK3VO UT WOS:000338353300008 ER PT J AU Schneider, KP Weaver, TF AF Schneider, K. P. Weaver, T. F. TI A Method for Evaluating Volt-VAR Optimization Field Demonstrations SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Distribution system analysis; power system control; voltage control; voltage optimization ID REDUCTION CVR AB In a regulated business environment, a utility must be able to validate that deployed technologies provide quantifiable benefits to the end-use customers. While there are well established procedures for determining the benefits derived from the deployment of traditional technologies, the same procedures do not exist for many emerging technologies. Volt-VAR Optimization is an example of an emerging technology that is being deployed across the nation without a standardized method for determining system performance and benefits. This paper will present a method for the evaluation, and quantification of benefits, for field deployments of Volt-VAR Optimization technologies. In addition to presenting the methodology, the paper will present a summary of results, and observations, from two separate Volt-VAR Optimization field evaluations using the presented method. C1 [Schneider, K. P.] Pacific NW Natl Lab, Battelle Seattle Res Ctr, Seattle, WA 98109 USA. [Weaver, T. F.] Amer Elect Power Co, Columbus, OH 43201 USA. RP Schneider, KP (reprint author), Pacific NW Natl Lab, Battelle Seattle Res Ctr, Seattle, WA 98109 USA. EM kevin.schneider@pnnl.gov; tfweaver@aep.com FU U.S. Department of Energy [DE-AC06-76RL01830] FX This work was supported by Battelle for the U.S. Department of Energy under Contract DE-AC06-76RL01830. NR 18 TC 11 Z9 11 U1 0 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD JUL PY 2014 VL 5 IS 4 BP 1696 EP 1703 DI 10.1109/TSG.2014.2308872 PG 8 WC Engineering, Electrical & Electronic SC Engineering GA AK1QS UT WOS:000338191200016 ER PT J AU Su, WC Wang, JH Roh, J AF Su, Wencong Wang, Jianhui Roh, Jaehyung TI Stochastic Energy Scheduling in Microgrids With Intermittent Renewable Energy Resources SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Microgrid; plug-in electric vehicle (PEV); renewable energy; smart grid; stochastic programming ID WIND POWER; DEMAND RESPONSE; UNIT COMMITMENT; MANAGEMENT; SYSTEMS AB Renewable energy resources such as wind and solar are an important component of a microgrid. However, the inherent intermittency and variability of such resources complicates microgrid operations. Meanwhile, more controllable loads (e.g., plug-in electric vehicles), distributed generators (e.g., micro gas turbines and diesel generators), and distributed energy storage devices (e.g., battery banks) are being integrated into the microgrid operation. To address the operational challenges associated with these technologies and energy resources, this paper formulates a stochastic problem for microgrid energy scheduling. The proposed problem formulation minimizes the expected operational cost of the microgrid and power losses while accommodating the intermittent nature of renewable energy resources. Case studies are performed on a modified IEEE 37-bus test feeder. The simulation results demonstrate the effectiveness and accuracy of the proposed stochastic microgrid energy scheduling model. C1 [Su, Wencong] Univ Michigan, Dept Elect & Comp Engn, Dearborn, MI 48128 USA. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. [Roh, Jaehyung] Konkuk Univ, Dept Elect Engn, Seoul, South Korea. RP Su, WC (reprint author), Univ Michigan, Dept Elect & Comp Engn, Dearborn, MI 48128 USA. EM wencong@umich.edu; jianhui.wang@anl.gov; jhroh@konkuk.ac.kr FU U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; KETEP [2001T100100424] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U. S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government.; Jaehyung Roh's work is sponsored by KETEP(2001T100100424). NR 31 TC 64 Z9 67 U1 9 U2 49 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD JUL PY 2014 VL 5 IS 4 BP 1876 EP 1883 DI 10.1109/TSG.2013.2280645 PG 8 WC Engineering, Electrical & Electronic SC Engineering GA AK1QS UT WOS:000338191200034 ER PT J AU Goddard, G Klose, J Backhaus, S AF Goddard, Gary Klose, Joseph Backhaus, Scott TI Model Development and Identification for Fast Demand Response in Commercial HVAC Systems SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Demand response (DR) ID LOADS AB Large commercial HVAC systems are attractive targets for fast demand response (DR) applications, e.g., integrating time-intermittent renewable generation. By leveraging the communications in the building automation system (BAS) already present in most buildings, large commercial HVAC systems provide easier access to a large controllable resource than aggregating a large number of small residential loads. However, large commercial HVAC systems are complex with many variables, many end point controllers, and several internal control loops that interact with each other. In addition, the existing fleet of large commercial buildings is diverse with many different HVAC configurations and BAS architectures. Capturing these buildings as DR resources requires a method to greatly reduce the complexity of the HVAC DR control and is general and flexible enough that it can be easily deployed across the diverse fleet of existing buildings. We create such a DR control by developing a system model that uses a single state variable instead of the several hundred variables in a commercial HVAC system. The model includes a small number of system parameters, and we demonstrate how their values can be determined via system identification measurements. Finally, we test our model on a large commercial HVAC system to investigate its control performance. C1 [Goddard, Gary; Klose, Joseph] Los Alamos Natl Los Alamos, Util & Infrastruct Div, Los Alamos, NM 87544 USA. [Backhaus, Scott] Los Alamos Natl Lab, MPA Div, Los Alamos, NM 87545 USA. RP Goddard, G (reprint author), Los Alamos Natl Los Alamos, Util & Infrastruct Div, Los Alamos, NM 87544 USA. EM goddard@lanl.gov; klose@lanl.gov; backhaus@lanl.gov OI Backhaus, Scott/0000-0002-0344-6791 FU Microgrid Program of the Office of Electricity within the U.S. Department of Energy FX This work was supported by the Microgrid Program of the Office of Electricity within the U.S. Department of Energy. NR 14 TC 13 Z9 13 U1 1 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD JUL PY 2014 VL 5 IS 4 BP 2084 EP 2092 DI 10.1109/TSG.2014.2312430 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA AK1QS UT WOS:000338191200056 ER PT J AU Thrash, JC Temperton, B Swan, BK Landry, ZC Woyke, T DeLong, EF Stepanauskas, R Giovannoni, SJ AF Thrash, J. Cameron Temperton, Ben Swan, Brandon K. Landry, Zachary C. Woyke, Tanja DeLong, Edward F. Stepanauskas, Ramunas Giovannoni, Stephan J. TI Single-cell enabled comparative genomics of a deep ocean SAR11 bathytype SO ISME JOURNAL LA English DT Article DE bathytype; ecotype; metagenomics; SAR11; single-cell genomics; deep ocean ID MULTIPLE SEQUENCE ALIGNMENT; RIBOSOMAL-RNA GENES; MICROBIAL ASSEMBLAGES; METAGENOMIC ANALYSIS; PROTEIN EVOLUTION; MESOPELAGIC ZONE; SARGASSO SEA; LIFE-STYLES; ATLANTIC; BACTERIA AB Bacterioplankton of the SAR11 clade are the most abundant microorganisms in marine systems, usually representing 25% or more of the total bacterial cells in seawater worldwide. SAR11 is divided into subclades with distinct spatiotemporal distributions (ecotypes), some of which appear to be specific to deep water. Here we examine the genomic basis for deep ocean distribution of one SAR11 bathytype (depth-specific ecotype), subclade Ic. Four single-cell Ic genomes, with estimated completeness of 55%-86%, were isolated from 770m at station ALOHA and compared with eight SAR11 surface genomes and metagenomic datasets. Subclade Ic genomes dominated metagenomic fragment recruitment below the euphotic zone. They had similar COG distributions, high local synteny and shared a large number (69%) of orthologous clusters with SAR11 surface genomes, yet were distinct at the 16S rRNA gene and amino-acid level, and formed a separate, monophyletic group in phylogenetic trees. Subclade Ic genomes were enriched in genes associated with membrane/cell wall/envelope biosynthesis and showed evidence of unique phage defenses. The majority of subclade Ic-specfic genes were hypothetical, and some were highly abundant in deep ocean metagenomic data, potentially masking mechanisms for niche differentiation. However, the evidence suggests these organisms have a similar metabolism to their surface counterparts, and that subclade Ic adaptations to the deep ocean do not involve large variations in gene content, but rather more subtle differences previously observed deep ocean genomic data, like preferential amino-acid substitutions, larger coding regions among SAR11 clade orthologs, larger intergenic regions and larger estimated average genome size. C1 [Thrash, J. Cameron; Temperton, Ben; Landry, Zachary C.; Giovannoni, Stephan J.] Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA. [Thrash, J. Cameron] Louisiana State Univ, Dept Biol Sci, Baton Rouge, LA 70803 USA. [Swan, Brandon K.; Stepanauskas, Ramunas] Bigelow Lab Ocean Sci, East Boothbay, ME USA. [Woyke, Tanja] DOE Joint Genome Inst, Walnut Creek, CA USA. [DeLong, Edward F.] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA. [DeLong, Edward F.] Ctr Microbial Ecol Res & Educ, Honolulu, HI USA. RP Thrash, JC (reprint author), Louisiana State Univ, Dept Biol Sci, Baton Rouge, LA 70803 USA. EM thrashc@lsu.edu OI Thrash, Cameron/0000-0003-0896-9986; Stepanauskas, Ramunas/0000-0003-4458-3108 FU Gordon and Betty Moore Foundation; US Department of Energy Joint Genome Institute (JGI) Community Supported Program [2011-387]; National Science Foundation (NSF) Science and Technology Center [EF0424599]; NSF [EF-826924, OCE-821374, OCE-1232982, DBI-1003269]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Gordon and Betty Moore Foundation (SJG and EFD), the US Department of Energy Joint Genome Institute (JGI) Community Supported Program grant 2011-387 (RS, BKS, EFD, SJG), National Science Foundation (NSF) Science and Technology Center Award EF0424599 (EFD), NSF awards EF-826924 (RS), OCE-821374 (RS) and OCE-1232982 (RS and BKS), and is based on work supported by the NSF under Award no. DBI-1003269 (JCT). Sequencing was conducted by JGI and supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. We thank Christopher M Sullivan and the Oregon State University Center for Genome Research and Biocomputing, as well as the Louisiana State University Center for Computation and Technology for vital computational resources. We also thank Kelly C Wrighton and Laura A Hug for critical discussions about single-cell genomics, metagenomics and metabolic reconstruction. NR 79 TC 17 Z9 18 U1 5 U2 30 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD JUL PY 2014 VL 8 IS 7 BP 1440 EP 1451 DI 10.1038/ismej.2013.243 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AK1XZ UT WOS:000338213900009 PM 24451205 ER PT J AU Wrighton, KC Castelle, CJ Wilkins, MJ Hug, LA Sharon, I Thomas, BC Handley, KM Mullin, SW Nicora, CD Singh, A Lipton, MS Long, PE Williams, KH Banfield, JF AF Wrighton, Kelly C. Castelle, Cindy J. Wilkins, Michael J. Hug, Laura A. Sharon, Itai Thomas, Brian C. Handley, Kim M. Mullin, Sean W. Nicora, Carrie D. Singh, Andrea Lipton, Mary S. Long, Philip E. Williams, Kenneth H. Banfield, Jillian F. TI Metabolic interdependencies between phylogenetically novel fermenters and respiratory organisms in an unconfined aquifer SO ISME JOURNAL LA English DT Article DE metagenomics; proteomics; candidate phylum; hydrogenase; fermentation; sulfate reduction; microbial diversity ID GENOME SEQUENCE; SP-NOV; DESULFOTALEA-PSYCHROPHILA; MICROBIAL COMMUNITIES; REDUCING BACTERIA; ELEMENTAL SULFUR; GENE DIVERSITY; OXIDATION; REDUCTION; SEDIMENT AB Fermentation-based metabolism is an important ecosystem function often associated with environments rich in organic carbon, such as wetlands, sewage sludge and the mammalian gut. The diversity of microorganisms and pathways involved in carbon and hydrogen cycling in sediments and aquifers and the impacts of these processes on other biogeochemical cycles remain poorly understood. Here we used metagenomics and proteomics to characterize microbial communities sampled from an aquifer adjacent to the Colorado River at Rifle, CO, USA, and document interlinked microbial roles in geochemical cycling. The organic carbon content in the aquifer was elevated via acetate amendment of the groundwater occurring over 2 successive years. Samples were collected at three time points, with the objective of extensive genome recovery to enable metabolic reconstruction of the community. Fermentative community members include organisms from a new phylum, Melainabacteria, most closely related to Cyanobacteria, phylogenetically novel members of the Chloroflexi and Bacteroidales, as well as candidate phyla genomes (OD1, BD1-5, SR1, WWE3, ACD58, TM6, PER and OP11). These organisms have the capacity to produce hydrogen, acetate, formate, ethanol, butyrate and lactate, activities supported by proteomic data. The diversity and expression of hydrogenases suggests the importance of hydrogen metabolism in the subsurface. Our proteogenomic data further indicate the consumption of fermentation intermediates by Proteobacteria can be coupled to nitrate, sulfate and iron reduction. Thus, fermentation carried out by previously unknown members of sediment microbial communities may be an important driver of nitrogen, hydrogen, sulfur, carbon and iron cycling. C1 [Wrighton, Kelly C.; Wilkins, Michael J.] Ohio State Univ, Dept Microbiol, Columbus, OH 43210 USA. [Castelle, Cindy J.; Hug, Laura A.; Sharon, Itai; Thomas, Brian C.; Mullin, Sean W.; Singh, Andrea; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Wilkins, Michael J.] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. [Handley, Kim M.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Nicora, Carrie D.; Lipton, Mary S.; Banfield, Jillian F.] Pacific NW Natl Lab, Dept Energy, Dept Biol Sci, Richland, WA 99352 USA. [Long, Philip E.; Williams, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Energy, Berkeley, CA 94720 USA. RP Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Dept Environm Sci Policy & Management, 369 McCone Hall, Berkeley, CA 94720 USA. EM jbanfield@berkeley.edu RI Williams, Kenneth/O-5181-2014; Wilkins, Michael/A-9358-2013; Long, Philip/F-5728-2013; Lipton, Mary/H-3913-2012; OI Williams, Kenneth/0000-0002-3568-1155; Long, Philip/0000-0003-4152-5682; Sharon, Itai/0000-0003-0705-2316; Handley, Kim/0000-0003-0531-3009 FU Integrated Field Research Challenge Site (IFRC) at Rifle, Colorado; US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This material is based upon work supported through the Integrated Field Research Challenge Site (IFRC) at Rifle, Colorado, the US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research funded the work under contract DE-AC02-05CH11231 (Lawrence Berkeley National Laboratory; operated by the University of California). NR 56 TC 47 Z9 47 U1 10 U2 75 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD JUL PY 2014 VL 8 IS 7 BP 1452 EP 1463 DI 10.1038/ismej.2013.249 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AK1XZ UT WOS:000338213900010 PM 24621521 ER PT J AU Mason, OU Scott, NM Gonzalez, A Robbins-Pianka, A Baelum, J Kimbrel, J Bouskill, NJ Prestat, E Borglin, S Joyner, DC Fortney, JL Jurelevicius, D Stringfellow, WT Alvarez-Cohen, L Hazen, TC Knight, R Gilbert, JA Jansson, JK AF Mason, Olivia U. Scott, Nicole M. Gonzalez, Antonio Robbins-Pianka, Adam Baelum, Jacob Kimbrel, Jeffrey Bouskill, Nicholas J. Prestat, Emmanuel Borglin, Sharon Joyner, Dominique C. Fortney, Julian L. Jurelevicius, Diogo Stringfellow, William T. Alvarez-Cohen, Lisa Hazen, Terry C. Knight, Rob Gilbert, Jack A. Jansson, Janet K. TI Metagenomics reveals sediment microbial community response to Deepwater Horizon oil spill SO ISME JOURNAL LA English DT Article DE DWH oil spill; hydrocarbons; iTag/Metagenomics; microbial community structure; sediments ID GULF-OF-MEXICO; DEGRADING BACTERIA; SEQUENCES; DIVERSITY; TAXONOMY; METHANE; GROWTH AB The Deepwater Horizon (DWH) oil spill in the spring of 2010 resulted in an input of similar to 4.1 million barrels of oil to the Gulf of Mexico; >22% of this oil is unaccounted for, with unknown environmental consequences. Here we investigated the impact of oil deposition on microbial communities in surface sediments collected at 64 sites by targeted sequencing of 16S rRNA genes, shotgun metagenomic sequencing of 14 of these samples and mineralization experiments using C-14-labeled model substrates. The 16S rRNA gene data indicated that the most heavily oil-impacted sediments were enriched in an uncultured Gammaproteobacterium and a Colwellia species, both of which were highly similar to sequences in the DWH deep-sea hydrocarbon plume. The primary drivers in structuring the microbial community were nitrogen and hydrocarbons. Annotation of unassembled metagenomic data revealed the most abundant hydrocarbon degradation pathway encoded genes involved in degrading aliphatic and simple aromatics via butane monooxygenase. The activity of key hydrocarbon degradation pathways by sediment microbes was confirmed by determining the mineralization of C-14-labeled model substrates in the following order: propylene glycol, dodecane, toluene and phenanthrene. Further, analysis of metagenomic sequence data revealed an increase in abundance of genes involved in denitrification pathways in samples that exceeded the Environmental Protection Agency (EPA)'s benchmarks for polycyclic aromatic hydrocarbons (PAHs) compared with those that did not. Importantly, these data demonstrate that the indigenous sediment microbiota contributed an important ecosystem service for remediation of oil in the Gulf. However, PAHs were more recalcitrant to degradation, and their persistence could have deleterious impacts on the sediment ecosystem. C1 [Mason, Olivia U.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Mason, Olivia U.; Baelum, Jacob; Kimbrel, Jeffrey; Bouskill, Nicholas J.; Prestat, Emmanuel; Borglin, Sharon; Joyner, Dominique C.; Fortney, Julian L.; Jurelevicius, Diogo; Stringfellow, William T.; Alvarez-Cohen, Lisa; Hazen, Terry C.; Jansson, Janet K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Scott, Nicole M.; Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL USA. [Scott, Nicole M.; Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gonzalez, Antonio] Univ Colorado, Biofrontiers Inst, Boulder, CO 80309 USA. [Robbins-Pianka, Adam] Univ Colorado, Dept Comp Sci, Boulder, CO 80309 USA. [Baelum, Jacob] Tech Univ Denmark, Ctr Biol Sequence Anal, DK-2800 Lyngby, Denmark. [Kimbrel, Jeffrey; Jansson, Janet K.] Joint Bioenergy Inst JBEI, Deconstruct Div, Emeryville, CA USA. [Joyner, Dominique C.; Fortney, Julian L.; Hazen, Terry C.] Univ Tennessee, Civil & Environm Engn Dept, Knoxville, TN USA. [Jurelevicius, Diogo] Univ Fed Rio de Janeiro, Lab Genet Microbiana, Inst Microbiol Paulo de Goes, Rio De Janeiro, Brazil. [Stringfellow, William T.] Univ Pacific, Sch Engn & Comp Sci, Ecol Engn Res Program, Stockton, CA 95211 USA. [Alvarez-Cohen, Lisa] Univ Calif Berkeley, Civil & Environm Engn Dept, Berkeley, CA 94720 USA. [Hazen, Terry C.] Oak Ridge Natl Lab, Div Biol Sci, Oak Ridge, TN USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. [Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Jansson, Janet K.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Mason, OU (reprint author), Florida State Univ, Dept Earth Ocean & Atmospher Sci, Room 307 OSB,117 North Woodward Ave, Tallahassee, FL 32306 USA. EM omason@fsu.edu; jrjansson@lbl.gov RI Balum, Jacob/I-2353-2013; Stringfellow, William/O-4389-2015; Bouskill, Nick/G-2390-2015; Borglin, Sharon/I-1013-2016; Knight, Rob/D-1299-2010; Hazen, Terry/C-1076-2012 OI Balum, Jacob/0000-0002-1022-6586; Stringfellow, William/0000-0003-3189-5604; Hazen, Terry/0000-0002-2536-9993 FU University of California at Berkeley, Energy Biosciences Institute (EBI) [DE-AC02-05CH11231]; Interdisciplinary Quantitative (IQ Biology) program at the Biofrontiers Institute, University of Colorado, Boulder; NSF IGERT [1144807]; National Institutes of Health; Howard Hughes Medical Institute FX This work was supported by a subcontract from the University of California at Berkeley, Energy Biosciences Institute (EBI) to Lawrence Berkeley National Laboratory under its U.S. Department of Energy contract DE-AC02-05CH11231. In addition, we acknowledge support from the Interdisciplinary Quantitative (IQ Biology) program at the Biofrontiers Institute, University of Colorado, Boulder, NSF IGERT grant number 1144807, by the National Institutes of Health, and by the Howard Hughes Medical Institute. We are thankful for the help of Yvette Piceno and Francine Reid with sampling and sample sectioning. We thank Theresa Pollard for handling shipping, ordering and transportation of supplies and people to and from the field. We also thank the captain and crew of the R/V Gyre. NR 39 TC 52 Z9 53 U1 21 U2 201 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD JUL PY 2014 VL 8 IS 7 BP 1464 EP 1475 DI 10.1038/ismej.2013.254 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AK1XZ UT WOS:000338213900011 PM 24451203 ER PT J AU Shilova, IN Robidart, JC Tripp, HJ Turk-Kubo, K Wawrik, B Post, AF Thompson, AW Ward, B Hollibaugh, JT Millard, A Ostrowski, M Scanlan, DJ Paerl, RW Stuart, R Zehr, JP AF Shilova, Irina N. Robidart, Julie C. Tripp, H. James Turk-Kubo, Kendra Wawrik, Boris Post, Anton F. Thompson, Anne W. Ward, Bess Hollibaugh, James T. Millard, Andy Ostrowski, Martin Scanlan, David J. Paerl, Ryan W. Stuart, Rhona Zehr, Jonathan P. TI A microarray for assessing transcription from pelagic marine microbial taxa SO ISME JOURNAL LA English DT Article DE marine; microbial; microarray; transcription; molecular ID FUNCTIONAL GENE MICROARRAY; PACIFIC SUBTROPICAL GYRE; HIGH-THROUGHPUT TOOL; NITROGEN-FIXATION; OPEN-OCEAN; OLIGONUCLEOTIDE MICROARRAY; COMMUNITY COMPOSITION; RED-SEA; PROCHLOROCOCCUS ECOTYPES; TEMPORAL VARIABILITY AB Metagenomic approaches have revealed unprecedented genetic diversity within microbial communities across vast expanses of the world's oceans. Linking this genetic diversity with key metabolic and cellular activities of microbial assemblages is a fundamental challenge. Here we report on a collaborative effort to design MicroTOOLs (Microbiological Targets for Ocean Observing Laboratories), a high-density oligonucleotide microarray that targets functional genes of diverse taxa in pelagic and coastal marine microbial communities. MicroTOOLs integrates nucleotide sequence information from disparate data types: genomes, PCR-amplicons, metagenomes, and metatranscriptomes. It targets 19 400 unique sequences over 145 different genes that are relevant to stress responses and microbial metabolism across the three domains of life and viruses. MicroTOOLs was used in a proof-of-concept experiment that compared the functional responses of microbial communities following Fe and P enrichments of surface water samples from the North Pacific Subtropical Gyre. We detected transcription of 68% of the gene targets across major taxonomic groups, and the pattern of transcription indicated relief from Fe limitation and transition to N limitation in some taxa. Prochlorococcus (eHLI), Synechococcus (sub-cluster 5.3) and Alphaproteobacteria SAR11 clade (HIMB59) showed the strongest responses to the Fe enrichment. In addition, members of uncharacterized lineages also responded. The MicroTOOLs microarray provides a robust tool for comprehensive characterization of major functional groups of microbes in the open ocean, and the design can be easily amended for specific environments and research questions. C1 [Shilova, Irina N.; Robidart, Julie C.; Turk-Kubo, Kendra; Zehr, Jonathan P.] Univ Calif Santa Cruz, Dept Ocean Sci, Santa Cruz, CA 95064 USA. [Tripp, H. James] DOE Joint Genome Inst, Walnut Creek, CA USA. [Wawrik, Boris] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Post, Anton F.] Marine Biol Lab, Woods Hole, MA 02543 USA. [Thompson, Anne W.] BD Biosci, Adv Cytometry Grp, Seattle, WA USA. [Ward, Bess] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Hollibaugh, James T.] Univ Georgia, Dept Marine Sci, Athens, GA 30602 USA. [Millard, Andy; Ostrowski, Martin; Scanlan, David J.] Univ Warwick, Dept Marine Microbiol, Coventry CV4 7AL, W Midlands, England. [Paerl, Ryan W.] Univ Calif San Diego, Marine Biol Res Div, San Diego, CA 92103 USA. [Stuart, Rhona] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Shilova, IN (reprint author), Univ Calif Santa Cruz, Dept Ocean Sci, 1156 High St, Santa Cruz, CA 95064 USA. EM iirina@ucsc.edu RI Zehr, Jonathan/B-3513-2014; Paerl, Ryan/E-7380-2015; Scanlan, David/G-4080-2016 OI Zehr, Jonathan/0000-0002-5691-5408; Paerl, Ryan/0000-0003-1237-9882; Scanlan, David/0000-0003-3093-4245 FU Gordon and Betty Moore Foundation (the MEGAMER facility); Gordon and Betty Moore Foundation Marine Investigator grant; NSF Center for Microbial Oceanography (C-MORE) [NSF EF0424599]; Moore foundation FX This work resulted from two workshops, and the design of the microarray was partially supported by the Gordon and Betty Moore Foundation (the MEGAMER facility), by a Gordon and Betty Moore Foundation Marine Investigator grant (JPZ) and by the NSF Center for Microbial Oceanography (C-MORE, NSF EF0424599). We thank all the participants of the October 2010 MicroTOOLs workshop sponsored by the Moore foundation. Particularly, we thank those who provided sequences for the design of microarray: Mahdi Belcaid, Dreux Chappell, Jackie Collier, Chris Francis, Scott Gifford, Jana Grote, Bethany Jenkins, Julie LaRoche, Pia Moisander, Annika Mosier, Micaela Parker, Holly Simon, Mariya Smit, Jody Wright, and Louie Wurch. We thank Shulei Sun and the team at CAMERA for support during microarray design. We also thank the Hawaii Ocean Time-series (HOT) program and C-MORE, specifically the captain and crew of R/V Kilo Moana and chief scientist of KM1016 cruise, Matt Church, for their expertise and for providing the opportunity and support for conducting experiments at sea. We thank Philip Heller and Jonathan Magasin for developing Java scripts for the microarray design and for computational support during the MicroTOOLs workshop in October 2010. Finally, we thank Nicole Pereira for help in running the incubation experiment, Sasha Tozzi for FRRF measurements, Rob Tibshirani for a consultation on microarray data normalization and analysis and the JPZ laboratory members for constructive discussions. NR 116 TC 8 Z9 8 U1 4 U2 36 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD JUL PY 2014 VL 8 IS 7 BP 1476 EP 1491 DI 10.1038/ismej.2014.1 PG 16 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AK1XZ UT WOS:000338213900012 PM 24477198 ER PT J AU Mueller, RC Paula, FS Mirza, BS Rodrigues, JLM Nusslein, K Bohannan, BJM AF Mueller, Rebecca C. Paula, Fabiana S. Mirza, Babur S. Rodrigues, Jorge L. M. Nuesslein, Klaus Bohannan, Brendan J. M. TI Links between plant and fungal communities across a deforestation chronosequence in the Amazon rainforest SO ISME JOURNAL LA English DT Article DE beta diversity; land-use change; tropical biodiversity ID LAND-USE; SOIL; DIVERSITY; BIODIVERSITY; BACTERIAL; DNA AB Understanding the interactions among microbial communities, plant communities and soil properties following deforestation could provide insights into the long-term effects of land-use change on ecosystem functions, and may help identify approaches that promote the recovery of degraded sites. We combined high-throughput sequencing of fungal rDNA and molecular barcoding of plant roots to estimate fungal and plant community composition in soil sampled across a chronosequence of deforestation. We found significant effects of land-use change on fungal community composition, which was more closely correlated to plant community composition than to changes in soil properties or geographic distance, providing evidence for strong links between above- and below-ground communities in tropical forests. C1 [Mueller, Rebecca C.; Bohannan, Brendan J. M.] Univ Oregon, Inst Ecol & Evolut, Eugene, OR 97403 USA. [Paula, Fabiana S.] Univ Sao Paulo, Inst Oceanog, Sao Paulo, Brazil. [Mirza, Babur S.; Rodrigues, Jorge L. M.] Univ Texas Arlington, Dept Biol, Arlington, TX 76019 USA. [Nuesslein, Klaus] Univ Massachusetts, Dept Microbiol, Amherst, MA 01003 USA. RP Mueller, RC (reprint author), Los Alamos Natl Lab, Biosci Div M888, POB 1663, Los Alamos, NM 87545 USA. EM beckymueller@gmail.com FU USDA Agriculture and Food Research Initiative Competitive Grant [2009-35319-05186]; APS Lewis and Clark Fund for Exploration and Research grant FX We thank the owners of the Fazenda Nova Vida for providing field site access, Vivian Pellizari for logistical support, Wagner Piccinini for field sampling, Jonas Frankel-Bricker and Roo Vandegrift for root amplification, and the helpful suggestions of two anonymous reviewers. Funding was provided by USDA Agriculture and Food Research Initiative Competitive Grant 2009-35319-05186 and by an APS Lewis and Clark Fund for Exploration and Research grant. NR 19 TC 17 Z9 19 U1 11 U2 93 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD JUL PY 2014 VL 8 IS 7 BP 1548 EP 1550 DI 10.1038/ismej.2013.253 PG 3 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AK1XZ UT WOS:000338213900019 PM 24451208 ER PT J AU Skomski, R Manchanda, P Takeuchi, I Cui, J AF Skomski, Ralph Manchanda, Priyanka Takeuchi, Ichiro Cui, Jun TI Geometry Dependence of Magnetization Reversal in Nanocomposite Alloys SO JOM LA English DT Article ID PERMANENT-MAGNETS; INTERACTION DOMAINS; NUCLEATION FIELDS; ENERGY PRODUCT; HIGH-REMANENCE; MODEL; MULTILAYERS; HYSTERESIS AB The geometrical optimization of aligned hard-soft permanent-magnet nanocomposites is investigated by model calculations. Considered criteria are the shapes of the soft and c-axis-aligned hard phases, the packing fraction of the soft phase, and magnetostatic interactions. Taking into account that the energy product is enhanced via the volume fraction of the soft phase, subject to maintaining coercivity, we find that the best structures are soft-magnetic cubes as well as long rods with a square cross section. Comparing embedded soft cubes with embedded soft spheres of the same size, our nucleation-field analysis shows that the volume fraction of the soft phase is enhanced by 91%, with a coercivity reduction of only 25%. Magnetostatic interactions often but not always deteriorate the permanent-magnet performance, as exemplified by the example of MnBi:FeCo bilayers and multilayers. C1 [Skomski, Ralph; Manchanda, Priyanka] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Skomski, Ralph; Manchanda, Priyanka] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Takeuchi, Ichiro] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Cui, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Skomski, R (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM rskomski@neb.rr.com FU PNNL ARPA-E; NSF MRSEC [DMR-0820521]; ARO [W911NF-10-2-0099] FX The research is supported primarily by PNNL ARPA-E (to J.C., I. T., P. M., and R. S.) and partially by NSF MRSEC DMR-0820521 and ARO W911NF-10-2-0099 (to R.S. and P.M.). NR 44 TC 2 Z9 2 U1 4 U2 41 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 EI 1543-1851 J9 JOM-US JI JOM PD JUL PY 2014 VL 66 IS 7 BP 1144 EP 1150 DI 10.1007/s11837-014-1005-0 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA AK6KI UT WOS:000338536100010 ER PT J AU Cardani, L Gironi, L Iachellini, NF Pattavina, L Beeman, JW Bellini, F Casali, N Cremonesi, O Dafinei, I Di Domizio, S Ferroni, F Galashov, E Gotti, C Nagorny, S Orio, F Pessina, G Piperno, G Pirro, S Previtali, E Rusconi, C Tomei, C Vignati, M AF Cardani, L. Gironi, L. Iachellini, N. Ferreiro Pattavina, L. Beeman, J. W. Bellini, F. Casali, N. Cremonesi, O. Dafinei, I. Di Domizio, S. Ferroni, F. Galashov, E. Gotti, C. Nagorny, S. Orio, F. Pessina, G. Piperno, G. Pirro, S. Previtali, E. Rusconi, C. Tomei, C. Vignati, M. TI First bolometric measurement of the two neutrino double beta decay of Mo-100 with a ZnMoO4 crystals array SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Article DE two neutrino double beta decay; cryogenic detectors; Monte Carlo simulation ID NUCLEAR-MATRIX ELEMENTS; SCINTILLATING BOLOMETER; CONTAMINATION; DETECTORS; PHYSICS; TABLES AB The large statistics collected during the operation of a ZnMoO4 array, for a total exposure of 1.3 kg day of Mo-100, allowed the first bolometric observation of the two neutrino double beta decay of Mo-100. The observed spectrum of each crystal was reconstructed taking into account the different background contributions due to environmental radioactivity and internal contamination. The analysis of coincidences between the crystals allowed the assignment of constraints to the intensity of the different background sources, resulting in a reconstruction of the measured spectrum down to an energy of similar to 300 keV. The half-life extracted from the data is T-1/2(2 nu) = [7.15 +/- 0.37 (stat) +/- 0.66 (syst)] x 10(18) y. C1 [Cardani, L.; Bellini, F.; Ferroni, F.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Cardani, L.; Bellini, F.; Dafinei, I.; Ferroni, F.; Orio, F.; Piperno, G.; Tomei, C.; Vignati, M.] INFN, Sez Roma, I-00185 Rome, Italy. [Gironi, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Gironi, L.; Iachellini, N. Ferreiro; Cremonesi, O.; Gotti, C.; Pessina, G.; Pirro, S.; Previtali, E.; Rusconi, C.] INFN, Sez Milano Bicocca, I-20126 Milan, Italy. [Pattavina, L.; Casali, N.; Nagorny, S.] INFN, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. [Beeman, J. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Di Domizio, S.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Di Domizio, S.] INFN, Sez Genova, I-16146 Genoa, Italy. [Galashov, E.] Novosibirsk State Univ, Dept Appl Phys, Novosibirsk 630090, Russia. RP Cardani, L (reprint author), Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. EM luca.gironi@mib.infn.it RI Bellini, Fabio/D-1055-2009; Di Domizio, Sergio/L-6378-2014; Pattavina, Luca/I-7498-2015; Vignati, Marco/H-1684-2013; Gironi, Luca/P-2860-2016; Casali, Nicola/C-9475-2017; OI Gotti, Claudio/0000-0003-2501-9608; Pessina, Gianluigi Ezio/0000-0003-3700-9757; Bellini, Fabio/0000-0002-2936-660X; Di Domizio, Sergio/0000-0003-2863-5895; Pattavina, Luca/0000-0003-4192-849X; Cardani, Laura/0000-0001-5410-118X; Vignati, Marco/0000-0002-8945-1128; Gironi, Luca/0000-0003-2019-0967; Casali, Nicola/0000-0003-3669-8247; Nahornyi, Serhii/0000-0002-8679-3747 FU European Research Council [247115]; ISOTTA project; ASPERA 2nd Common Call for RD Activities FX Part of the work was carried out thanks to LUCIFER Project, funded by the European Research Council (FP7/2007-2013) grant agreement no 247115. This work was also supported by the ISOTTA project, funded within the ASPERA 2nd Common Call for R&D Activities. Thanks are due to F Iachello and J Kotila for fruitful discussions and for providing us precise numerical calculation of the electron distributions for the 2 nu DBD of 100Mo. We wish to express our gratitude to the LNGS mechanical workshop and in particular to E Tatananni, A Rotilio, A Corsi, and B Romualdi for continuous and constructive help in the overall set-up construction. Finally, we are especially grateful to M Perego and M Guetti for their invaluable help. NR 24 TC 6 Z9 6 U1 2 U2 27 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD JUL PY 2014 VL 41 IS 7 AR 075204 DI 10.1088/0954-3899/41/7/075204 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK4WS UT WOS:000338425600025 ER PT J AU Casali, N Nagorny, SS Orio, F Pattavina, L Beeman, JW Bellini, F Cardani, L Dafinei, I Di Domizio, S Di Vacri, ML Gironi, L Kosmyna, MB Nazarenko, BP Nisi, S Pessina, G Piperno, G Pirro, S Rusconi, C Shekhovtsov, AN Tomei, C Vignati, M AF Casali, N. Nagorny, S. S. Orio, F. Pattavina, L. Beeman, J. W. Bellini, F. Cardani, L. Dafinei, I. Di Domizio, S. Di Vacri, M. L. Gironi, L. Kosmyna, M. B. Nazarenko, B. P. Nisi, S. Pessina, G. Piperno, G. Pirro, S. Rusconi, C. Shekhovtsov, A. N. Tomei, C. Vignati, M. TI Discovery of the Eu-151 alpha decay SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Article DE alpha decay; scintillation detectors; bolometers AB We report on the first compelling observation of a decay of Eu-151 to the ground state of Pm-147. The measurement was performed using a 6.15 g Li6Eu(BO3)(3) crystal operated as a scintillating bolometer. The Q-value and half-life measured are: Q = 1948.9 +/- 6.9(stat.) +/- 5.1(syst.) keV, and T-1/2 = (4.62 +/- 0.95(stat.) +/- 0.68(syst.)) x 10(18) y. The half-life prediction of nuclear theory using the Coulomb and proximity potentialmodel are in good agreement with this experimental result. C1 [Casali, N.; Nagorny, S. S.; Pattavina, L.; Di Vacri, M. L.; Nisi, S.] INFN, Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. [Casali, N.] Univ Aquila, Dipartimento Sci Fis & Chim, I-67100 Coppito, AQ, Italy. [Nagorny, S. S.] Natl Acad Sci Ukraine, Inst Nucl Res, UA-03680 Kiev, Ukraine. [Orio, F.; Bellini, F.; Cardani, L.; Dafinei, I.; Piperno, G.; Tomei, C.; Vignati, M.] INFN, Sez Roma, I-00185 Rome, Italy. [Beeman, J. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Di Domizio, S.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Di Domizio, S.] INFN, Sez Genova, I-16146 Genoa, Italy. [Gironi, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Gironi, L.; Pessina, G.; Pirro, S.; Rusconi, C.] INFN, Sez Milano Bicocca, I-20126 Milan, Italy. [Kosmyna, M. B.; Nazarenko, B. P.; Shekhovtsov, A. N.] Natl Acad Sci Ukraine, Inst Single Crystals, UA-61001 Kharkov, Ukraine. RP Casali, N (reprint author), INFN, Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. EM luca.pattavina@lngs.infn.it RI Bellini, Fabio/D-1055-2009; Di Domizio, Sergio/L-6378-2014; Pattavina, Luca/I-7498-2015; Vignati, Marco/H-1684-2013; Gironi, Luca/P-2860-2016; Casali, Nicola/C-9475-2017; OI Bellini, Fabio/0000-0002-2936-660X; Di Domizio, Sergio/0000-0003-2863-5895; Pattavina, Luca/0000-0003-4192-849X; Vignati, Marco/0000-0002-8945-1128; Gironi, Luca/0000-0003-2019-0967; Casali, Nicola/0000-0003-3669-8247; Nahornyi, Serhii/0000-0002-8679-3747 FU Italian Ministry of Research [PRIN 2010ZXAZK9 2010-2011]; ISOTTA project; ASPERA 2nd Common Call for RD Activities; European Research Council [247115] FX This project was supported by the Italian Ministry of Research under the PRIN 2010ZXAZK9 2010-2011 grant. This work was also supported by the ISOTTA project, funded within the ASPERA 2nd Common Call for R&D Activities. Part of the work was carried out thanks to LUCIFER Project, funded by the European Research Council (FP7/2007-2013) grant agreement no 247115. NR 25 TC 4 Z9 4 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD JUL PY 2014 VL 41 IS 7 AR 075101 DI 10.1088/0954-3899/41/7/075101 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK4WS UT WOS:000338425600013 ER PT J AU Dobaczewski, J Nazarewicz, W Reinhard, PG AF Dobaczewski, J. Nazarewicz, W. Reinhard, P-G TI Error estimates of theoretical models: a guide SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Article DE nuclear models; error estimates; error propagation; uncertainty quantification; systematic and statistical errors; correlation analysis; model-based extrapolations; regression analysis ID EQUATION-OF-STATE; MASSES AB This guide offers suggestions/insights on uncertainty quantification of nuclear structure models. We discuss a simple approach to statistical-error estimates, strategies to assess systematic errors, and show how to uncover inter-dependences by correlation analysis. The basic concepts are illustrated through simple examples. By providing theoretical error bars on predicted quantities and using statistical methods to study correlations between observables, theory can significantly enhance the feedback between experiment and nuclear modeling. C1 [Dobaczewski, J.; Nazarewicz, W.] Univ Warsaw, Fac Phys, Inst Theoret Phys, PL-00681 Warsaw, Poland. [Dobaczewski, J.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. [Nazarewicz, W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Nazarewicz, W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Reinhard, P-G] Univ Erlangen Nurnberg, Inst Theoret Phys 2, D-91058 Erlangen, Germany. RP Dobaczewski, J (reprint author), Univ Warsaw, Fac Phys, Inst Theoret Phys, Ul Hoza 69, PL-00681 Warsaw, Poland. EM Jacek.Dobaczewski@fuw.edu.pl; witek@utk.edu; Paul-Gerhard.Reinhard@physik.uni-erlangen.de FU US Department of Energy (University of Tennessee) [DE-FG02-96ER40963]; Stewardship Science Academic Alliances program [DE-FG52-09NA29461]; NUCLEI SciDAC Collaboration [DE-SC0008499]; Academy of Finland and University of Jyvaskyla within the FIDIPRO programme; Polish National Science Center [2012/07/B/ST2/03907]; Bundesministerium fur Bildung und Forschung (BMBF) [05P09RFFTB] FX This work was finalized during the Program INT-13-3 'Quantitative Large Amplitude Shape Dynamics: fission and heavy ion fusion' at the National Institute for Nuclear Theory in Seattle; it was supported by the US Department of Energy under Contract no. DE-FG02-96ER40963 (University of Tennessee), no. DE-FG52-09NA29461 (the Stewardship Science Academic Alliances program), no. DE-SC0008499 (NUCLEI SciDAC Collaboration); by the Academy of Finland and University of Jyvaskyla within the FIDIPRO programme; by the Polish National Science Center under Contract no. 2012/07/B/ST2/03907; and by the Bundesministerium fur Bildung und Forschung (BMBF) under contract number 05P09RFFTB. NR 49 TC 75 Z9 76 U1 0 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD JUL PY 2014 VL 41 IS 7 AR 074001 DI 10.1088/0954-3899/41/7/074001 PG 20 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK4WS UT WOS:000338425600001 ER PT J AU Kujala, N Marathe, S Shu, DM Shi, B Qian, J Maxey, E Finney, L Macrander, A Assoufid, L AF Kujala, Naresh Marathe, Shashidhara Shu, Deming Shi, Bing Qian, Jun Maxey, Evan Finney, Lydia Macrander, Albert Assoufid, Lahsen TI Kirkpatrick-Baez mirrors to focus hard X-rays in two dimensions as fabricated, tested and installed at the Advanced Photon Source SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE hard X-ray micro-focusing optics; fixed elliptical geometry K-B mirrors; optics and detector beamline ID SUBMICROMETER-RESOLUTION; REFRACTIVE LENS; OPTICS; MICROSCOPY AB The micro-focusing performance for hard X-rays of a fixed-geometry elliptical Kirkpatrick-Baez (K-B) mirrors assembly fabricated, tested and finally implemented at the micro-probe beamline 8-BM of the Advanced Photon Source is reported. Testing of the K-B mirror system was performed at the optics and detector test beamline 1-BM. K-B mirrors of length 80 mm and 60 mm were fabricated by profile coating with Pt metal to produce focal lengths of 250 mm and 155 mm for 3 mrad incident angle. For the critical angle of Pt, a broad bandwidth of energies up to 20 keV applies. The classical K-B sequential mirror geometry was used, and mirrors were mounted on micro-translation stages. The beam intensity profiles were measured by differentiating the curves of intensity data measured using a wire-scanning method. A beam size of 1.3 mu m (V) and 1.2 mu m (H) was measured with monochromatic X-rays of 18 keV at 1-BM. After installation at 8-BM the measured focus met the design requirements. In this paper the fabrication and metrology of the K-B mirrors are reported, as well as the focusing performances of the full mirrors-plus-mount set-up at both beamlines. C1 [Kujala, Naresh; Marathe, Shashidhara; Shu, Deming; Shi, Bing; Qian, Jun; Maxey, Evan; Finney, Lydia; Macrander, Albert; Assoufid, Lahsen] Argonne Natl Lab, Lemont, IL 60439 USA. RP Kujala, N (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. EM kujala@aps.anl.gov RI ID, MRCAT/G-7586-2011 FU US DOE [DE-AC02-06CH11357] FX The authors would like to thank Kurtz Goetze from the BCDA group for helping with the software motor controls and Chris Jacobsen for his support. Scientists at beamline 10-ID (MR-CAT) at the APS provided the tungsten wire sample. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 29 TC 2 Z9 2 U1 0 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 EI 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2014 VL 21 BP 662 EP 668 DI 10.1107/S1600577514006493 PN 4 PG 7 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA AK0SD UT WOS:000338124300003 PM 24971959 ER PT J AU Shi, XB Reininger, R del Rio, MS Assoufid, L AF Shi, Xianbo Reininger, Ruben del Rio, Manuel Sanchez Assoufid, Lahsen TI A hybrid method for X-ray optics simulation: combining geometric ray-tracing and wavefront propagation SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE hybrid method; beamline design; X-ray optics simulation; ray-tracing; wavefront propagation; partial coherence ID SYNCHROTRON-RADIATION; BESSY-II; GRATING MONOCHROMATOR; UNDULATOR BEAMLINE; ELLIPTIC MIRRORS; DESIGN; PERFORMANCE; SYSTEM; SHADOW; OPTIMIZATION AB A new method for beamline simulation combining ray-tracing and wavefront propagation is described. The 'Hybrid Method' computes diffraction effects when the beam is clipped by an aperture or mirror length and can also simulate the effect of figure errors in the optical elements when diffraction is present. The effect of different spatial frequencies of figure errors on the image is compared with SHADOW results pointing to the limitations of the latter. The code has been benchmarked against the multi-electron version of SRW in one dimension to show its validity in the case of fully, partially and non-coherent beams. The results demonstrate that the code is considerably faster than the multi-electron version of SRW and is therefore a useful tool for beamline design and optimization. C1 [Shi, Xianbo; Reininger, Ruben; Assoufid, Lahsen] Argonne Natl Lab, Argonne, IL 60439 USA. [del Rio, Manuel Sanchez] European Synchrotron Radiat Facil, F-38000 Grenoble, France. RP Shi, XB (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM xshi@aps.anl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors would like to thank Dr Oleg Chubar and Mr Niccolo Canestrari (Brookhaven National Laboratory) for the SRW support and helpful discussions about this work. NR 71 TC 11 Z9 11 U1 3 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 EI 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2014 VL 21 BP 669 EP 678 DI 10.1107/S160057751400650X PN 4 PG 10 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA AK0SD UT WOS:000338124300004 PM 24971960 ER PT J AU Gupta, S Celestre, R Petzold, CJ Chance, MR Ralston, C AF Gupta, Sayan Celestre, Richard Petzold, Christopher J. Chance, Mark R. Ralston, Corie TI Development of a microsecond X-ray protein footprinting facility at the Advanced Light Source SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE microsecond irradiation; radiolytic labeling; mass spectrometry; protein structure ID STRUCTURAL MASS-SPECTROMETRY; RADICAL PROBE; IN-VIVO; PHOTOCHEMICAL OXIDATION; ELECTROSPRAY-IONIZATION; HYDROGEN-PEROXIDE; DNA-BINDING; ACTIVATION; DYNAMICS; SURFACE AB X-ray footprinting (XF) is an important structural biology tool used to determine macromolecular conformations and dynamics of both nucleic acids and proteins in solution on a wide range of timescales. With the impending shut-down of the National Synchrotron Light Source, it is ever more important that this tool continues to be developed at other synchrotron facilities to accommodate XF users. Toward this end, a collaborative XF program has been initiated at the Advanced Light Source using the white-light bending-magnet beamlines 5.3.1 and 3.2.1. Accessibility of the microsecond time regime for protein footprinting is demonstrated at beamline 5.3.1 using the high flux density provided by a focusing mirror in combination with a micro-capillary flow cell. It is further reported that, by saturating samples with nitrous oxide, the radiolytic labeling efficiency is increased and the imprints of bound versus bulk water can be distinguished. These results both demonstrate the suitability of the Advanced Light Source as a second home for the XF experiment, and pave the way for obtaining high-quality structural data on complex protein samples and dynamics information on the microsecond timescale. C1 [Gupta, Sayan; Ralston, Corie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. [Celestre, Richard] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. [Petzold, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Chance, Mark R.] Case Western Reserve Univ, Sch Med, Ctr Prote & Bioinformat, Ctr Synchrotron Biosci, Cleveland, OH 44106 USA. RP Ralston, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley Ctr Struct Biol, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM cyralston@lbl.gov FU LBNL Laboratory Directed Research and Development (LDRD); Office of Science, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; NIBIB [P30-EB0966] FX The authors would like to thank Jun Hamamoto for assistance on beamline 3.2.1, Kurt Krueger for technical advice and fabrication of the microfluidic capillary cell, Simon Morton for advice and design of a focusing mirror for build-out of beamline 3.3.1, and Rhijuta D'Mello for assisting in beamline experiments at X28C at the NSLS. Funding for this research was provided by an LBNL Laboratory Directed Research and Development (LDRD) grant awarded to CR. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract No. DE-AC02-05CH11231. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-98CH10886. The Center for Synchrotron Biosciences at the National Synchrotron Light Sources is supported by NIBIB under P30-EB0966. NR 57 TC 6 Z9 6 U1 1 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 EI 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2014 VL 21 BP 690 EP 699 DI 10.1107/S1600577514007000 PN 4 PG 10 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA AK0SD UT WOS:000338124300006 PM 24971962 ER PT J AU Warwick, T Chuang, YD Voronov, DL Padmore, HA AF Warwick, Tony Chuang, Yi-De Voronov, Dmitriy L. Padmore, Howard A. TI A multiplexed high-resolution imaging spectrometer for resonant inelastic soft X-ray scattering spectroscopy SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE soft X-ray; scattering; spectrometer ID MONOCHROMATOR; MICROSCOPE AB The optical design of a two-dimensional imaging soft X-ray spectrometer is described. A monochromator will produce a dispersed spectrum in a narrow vertical illuminated stripe (similar to 2 mu m wide by similar to 2 mm tall) on a sample. The spectrometer will use inelastically scattered X-rays to image the extended field on the sample in the incident photon energy direction (vertical), resolving the incident photon energy. At the same time it will image and disperse the scattered photons in the orthogonal (horizontal) direction, resolving the scattered photon energy. The principal challenge is to design a system that images from the flat-field illumination of the sample to the flat field of the detector and to achieve sufficiently high spectral resolution. This spectrometer provides a completely parallel resonant inelastic X-ray scattering measurement at high spectral resolution (similar to 30000) over the energy bandwidth (similar to 5 eV) of a soft X-ray absorption resonance. C1 [Warwick, Tony; Chuang, Yi-De; Voronov, Dmitriy L.; Padmore, Howard A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Warwick, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM warwick@lbl.gov RI Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract No. DE-AC02-05CH11231. NR 20 TC 12 Z9 12 U1 0 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 EI 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2014 VL 21 BP 736 EP 743 DI 10.1107/S1600577514009692 PN 4 PG 8 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA AK0SD UT WOS:000338124300012 PM 24971968 ER PT J AU Bogdanov, B Zhao, XN Robinson, DB Ren, JH AF Bogdanov, Bogdan Zhao, Xiaoning Robinson, David B. Ren, Jianhua TI Electron Capture Dissociation Studies of the Fragmentation Patterns of Doubly Protonated and Mixed Protonated-Sodiated Peptoids SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE ECD; Radical assisted fragmentation; Odd-electron negative ion; Peptide-mimicking oligomer; Poly(N-substituted glycine) ID MASS-SPECTROMETRIC CHARACTERISTICS; PEPTIDE CATION-RADICALS; AROMATIC SIDE-CHAINS; GAS-PHASE; NONBIOLOGICAL POLYMER; CASCADE DISSOCIATIONS; SECONDARY STRUCTURE; PROTEIN-STRUCTURE; BOND-CLEAVAGE; AMINO-ACID AB The fragmentation patterns of a group of doubly protonated ([P + 2H](2+)) and mixed protonated-sodiated ([P + H + Na](2+)) peptide-mimicking oligomers, known as peptoids, have been studied using electron capturing dissociation (ECD) tandem mass spectrometry techniques. For all the peptoids studied, the primary backbone fragmentation occurred at the N-C-alpha bonds. The N-terminal fragment ions, the C-ions (protonated) and the C'-ions (sodiated) were observed universally for all the peptoids regardless of the types of charge carrier. The C-terminal ions varied depending on the type of charge carrier. The doubly protonated peptoids with at least one basic residue located at a position other than the N-terminus fragmented by producing the Z(aEuro cent)-series of ions. In addition, most doubly protonated peptoids also produced the Y-series of ions with notable abundances. The mixed protonated-sodiated peptoids fragmented by yielding the Z(aEuro cent)'-series of ions in addition to the C'-series. Chelation between the sodium cation and the amide groups of the peptoid chain might be an important factor that could stabilize both the N-terminal and the C-terminal fragment ions. Regardless of the types of the charge carrier, one notable fragmentation for all the peptoids was the elimination of a benzylic radical from the odd-electron positive ions of the protonated peptoids ([P + 2H](aEuro cent+)) and the sodiated peptoids ([P + H + Na](aEuro cent+)). The study showed potential utility of using the ECD technique for sequencing of peptoid libraries generated by combinatorial chemistry. C1 [Bogdanov, Bogdan; Zhao, Xiaoning; Ren, Jianhua] Univ Pacific, Dept Chem, Stockton, CA 95211 USA. [Robinson, David B.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Ren, JH (reprint author), Univ Pacific, Dept Chem, Stockton, CA 95211 USA. EM jren@pacific.edu RI Foundry, Molecular/G-9968-2014 FU National Science Foundation [CHE-0749737, CHE-1301505]; Laboratory-Directed Research and Development program at Sandia National Laboratories [DE-AC04-94AL85000]; Office of Science, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231] FX The authors thank Dr. Kiran Morishetti (University of the Pacific, currently at Abon Pharmaceuticals LLC) for helping to interpret some of the spectra data, and Dr. Ronald Zuckermann (The Molecular Foundry, Lawrence Berkeley National Laboratory) for providing peptoid-10. J.R. acknowledges the support from the National Science Foundation [CHE-0749737 (prior) and CHE-1301505 (current)]. D. R. acknowledges the support from the Laboratory-Directed Research and Development program at Sandia National Laboratories (DE-AC04-94AL85000). Peptoid synthesis at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, US Department of Energy (DE-AC02-05CH11231). All ECD experiments were conducted at the Center for Regulatory and Environmental Analytical Metabolomics (CREAM) of the University of Louisville. The authors thank Dr. Shenheng Guan for assisting with the ETD experiments at the mass spectrometry facility of the University of California at San Francisco. They are also thankful for performing some of the ETD experiments in Dr. Joseph Loo's laboratory at the University of California at Los Angeles. NR 72 TC 5 Z9 5 U1 0 U2 23 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 EI 1879-1123 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD JUL PY 2014 VL 25 IS 7 BP 1202 EP 1216 DI 10.1007/s13361-014-0869-0 PG 15 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA AK1RG UT WOS:000338192700012 PM 24845348 ER PT J AU Li, YZ Kessler, MR AF Li, Yuzhan Kessler, Michael R. TI Cure kinetics of liquid crystalline epoxy resins based on biphenyl mesogen SO JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY LA English DT Article DE Liquid crystalline epoxy resins (LCERs); Cure kinetics; Activation energy; Thermosets ID MAGNETIC-FIELD ORIENTATION; CURING KINETICS; RIGID-ROD; FRACTURE-TOUGHNESS; THERMOSETS; POLYDOMAIN; MECHANISM; POLYMERS; BEHAVIOR AB The cure kinetics of a biphenyl-based liquid crystalline (LC) epoxy resin (LCER) was studied using differential scanning calorimetry (DSC) and polarized optical microscopy. The effects of LC phase formation on the cure kinetics were investigated. Both a model-free isoconversional method and a model-fitting method were used to analyze the DSC data. Results from the isoconversional analysis were applied to develop tentative multi-step kinetic models describing the curing reaction. Kinetic analysis showed that compared to the resins cured in amorphous phase, LCERs exhibited higher values of reaction enthalpy and a complex dependence of activation energy on the degree of cure. The formation of the LC phase resulted in a decrease in activation energy, leading to higher degree of reaction. C1 [Li, Yuzhan; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA. [Li, Yuzhan; Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Kessler, MR (reprint author), Washington State Univ, Sch Mech & Mat Engn, POB 642920, Pullman, WA 99164 USA. EM MichaelR.Kessler@wsu.edu RI Kessler, Michael/C-3153-2008 OI Kessler, Michael/0000-0001-8436-3447 FU Air Force Office of Scientific Research (AFOSR) [FA9550-12-1-0108] FX The authors would like to thank Dr. Elena Moukhina for her technical support and helpful discussion. Support under Air Force Office of Scientific Research (AFOSR) Award No. FA9550-12-1-0108 is gratefully acknowledged. NR 29 TC 2 Z9 3 U1 1 U2 22 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1388-6150 EI 1572-8943 J9 J THERM ANAL CALORIM JI J. Therm. Anal. Calorim. PD JUL PY 2014 VL 117 IS 1 BP 481 EP 488 DI 10.1007/s10973-014-3647-0 PG 8 WC Thermodynamics; Chemistry, Analytical; Chemistry, Physical SC Thermodynamics; Chemistry GA AK0QS UT WOS:000338120100056 ER PT J AU Yeddu, HK Lookman, T Borgenstam, A Agren, J Saxena, A AF Yeddu, Hemantha Kumar Lookman, Turab Borgenstam, Annika Agren, John Saxena, Avadh TI Martensite formation in stainless steels under transient loading SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Martensite; Phase-field model; Microstructure; Transient loading; Steels ID 3-DIMENSIONAL PHASE-FIELD; MICROSTRUCTURE EVOLUTION; PLASTIC-ACCOMMODATION; LATH MARTENSITE; TRANSFORMATIONS; MODEL; CRYSTALLOGRAPHY; MORPHOLOGY; SIMULATION; AUSTENITE AB We present a 3D elastoplastic phase-field model to study the martensite formation in stainless steels under transient loading. Linear isotropic strain hardening is considered. Our results show that various combinations of martensite variants, which minimize the mechanical energy and maximize the net available driving force, are favored under different transient loading directions. The mechanical properties of steels under transient loading depend on the direction of loading. The areas where the load is applied, i.e. the grain boundaries, become favorable martensite nucleation sites. (C) 2014 Elsevier B.V. All rights reserved. C1 [Yeddu, Hemantha Kumar; Lookman, Turab; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Borgenstam, Annika; Agren, John] KTH Royal Inst Technol, Dept Mat Sci & Engn, S-10044 Stockholm, Sweden. RP Yeddu, HK (reprint author), Los Alamos Natl Lab, Div Theoret, MS-B262, Los Alamos, NM 87545 USA. EM hemu23@gmail.com FU US Department of Energy FX This work was supported by the US Department of Energy. Computer resources were provided by the National Supercomputer Center (NSC), Linkoping, Sweden. NR 25 TC 2 Z9 2 U1 0 U2 13 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JUL 1 PY 2014 VL 608 BP 101 EP 105 DI 10.1016/j.msea.2014.04.063 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AK4OU UT WOS:000338404800014 ER PT J AU Galan, J Verleysen, P Lebensohn, RA AF Galan, J. Verleysen, P. Lebensohn, R. A. TI An improved algorithm for the polycrystal viscoplastic self-consistent model and its integration with implicit finite element schemes SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE vpsc; polycrystal; fem; viscoplastic; elasto-viscoplastic; finite-element ID TEXTURE DEVELOPMENT; MECHANICAL ANISOTROPY; CRYSTAL PLASTICITY; FIELD FLUCTUATIONS; GRAIN-INTERACTION; ZIRCONIUM ALLOYS; DEFORMATION; PREDICTION; SIMULATION; BEHAVIOR AB A new algorithm for the solution of the deformation of a polycrystalline material using a self-consistent scheme, and its integration as part of the finite element software Abaqus/Standard are presented. The method is based on the original VPSC formulation by Lebensohn and Tome and its integration with Abaqus/Standard by Segurado et al. The new algorithm has been implemented as a set of Fortran 90 modules, to be used either from a standalone program or from Abaqus subroutines. The new implementation yields the same results as VPSC7, but with a significantly better performance, especially when used in multicore computers. C1 [Galan, J.; Verleysen, P.] Univ Ghent, Dept Mat Sci & Engn, Fac Engn & Architecture, B-9052 Ghent, Belgium. [Lebensohn, R. A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Mat Sci Radiat & Dynam Extremes MST 8, Los Alamos, NM 87845 USA. RP Galan, J (reprint author), Univ Ghent, Dept Mat Sci & Engn, Fac Engn & Architecture, Technol Pk 903, B-9052 Ghent, Belgium. EM Jesus.GalanLopez@UGent.be RI Lebensohn, Ricardo/A-2494-2008 OI Lebensohn, Ricardo/0000-0002-3152-9105 NR 39 TC 2 Z9 2 U1 1 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD JUL PY 2014 VL 22 IS 5 AR 055023 DI 10.1088/0965-0393/22/5/055023 PG 18 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AK5CL UT WOS:000338441700024 ER PT J AU Xiao, DJ Bloch, ED Mason, JA Queen, WL Hudson, MR Planas, N Borycz, J Dzubak, AL Verma, P Lee, K Bonino, F Crocella, V Yano, J Bordiga, S Truhlar, DG Gagliardi, L Brown, CM Long, JR AF Xiao, Dianne J. Bloch, Eric D. Mason, Jarad A. Queen, Wendy L. Hudson, Matthew R. Planas, Nora Borycz, Joshua Dzubak, Allison L. Verma, Pragya Lee, Kyuho Bonino, Francesca Crocella, Valentina Yano, Junko Bordiga, Silvia Truhlar, Donald G. Gagliardi, Laura Brown, Craig M. Long, Jeffrey R. TI Oxidation of ethane to ethanol by N2O in a metal-organic framework with coordinatively unsaturated iron(II) sites SO NATURE CHEMISTRY LA English DT Article ID 2ND-ORDER PERTURBATION-THEORY; SPIN OXOIRON(IV) COMPLEX; NITROUS-OXIDE; DIOXYGEN ACTIVATION; DINITROGEN OXIDE; ACTIVE-SITES; ENZYMES; OXO; REACTIVITY; BINDING AB Enzymatic haem and non-haem high-valent iron-oxo species are known to activate strong C-H bonds, yet duplicating this reactivity in a synthetic system remains a formidable challenge. Although instability of the terminal iron-oxo moiety is perhaps the foremost obstacle, steric and electronic factors also limit the activity of previously reported mononuclear iron(IV)-oxo compounds. In particular, although nature's non-haem iron(IV)-oxo compounds possess high-spin S = 2 ground states, this electronic configuration has proved difficult to achieve in a molecular species. These challenges may be mitigated within metal-organic frameworks that feature site-isolated iron centres in a constrained, weak-field ligand environment. Here, we show that the metal-organic framework Fe-2(dobdc) (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate) and its magnesium-diluted analogue, Fe0.1Mg1.9(dobdc), are able to activate the C-H bonds of ethane and convert it into ethanol and acetaldehyde using nitrous oxide as the terminal oxidant. Electronic structure calculations indicate that the active oxidant is likely to be a high-spin S = 2 iron(IV)-oxo species. C1 [Xiao, Dianne J.; Bloch, Eric D.; Mason, Jarad A.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Queen, Wendy L.; Lee, Kyuho] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Hudson, Matthew R.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Planas, Nora; Borycz, Joshua; Dzubak, Allison L.; Verma, Pragya; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Planas, Nora; Borycz, Joshua; Dzubak, Allison L.; Verma, Pragya; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Inst Supercomp, Minneapolis, MN 55455 USA. [Bonino, Francesca; Crocella, Valentina; Bordiga, Silvia] Univ Turin, Dept Chem, NIS Ctr, I-10135 Turin, Italy. [Bonino, Francesca; Crocella, Valentina; Bordiga, Silvia] Univ Turin, INSTM Reference Ctr, I-10135 Turin, Italy. [Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Xiao, DJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu RI Bordiga, Silvia/M-3875-2014; Brown, Craig/B-5430-2009; Truhlar, Donald/G-7076-2015; Foundry, Molecular/G-9968-2014; Crocella, Valentina/E-5203-2016; Bonino, Francesca/G-8234-2016 OI Bordiga, Silvia/0000-0003-2371-4156; Queen, Wendy/0000-0002-8375-2341; Brown, Craig/0000-0002-9637-9355; Truhlar, Donald/0000-0002-7742-7294; Crocella, Valentina/0000-0002-3606-8424; Bonino, Francesca/0000-0002-6822-6685 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-12ER16362]; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under US Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; US Department of Energy (DOE) Office of Science by Argonne National Laboratory; US DOE [DE-AC02-06CH11357]; Ateneo Project [2011 ORTO11RRT5] FX Synthesis, basic characterization experiments and all of the theoretical work were supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under award DE-FG02-12ER16362. Reactivity studies were supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under US Department of Energy Contract No. DE-AC02-05CH11231. Work at the Molecular Foundry, and XAS experiments performed at the Advanced Light Source (BL 10.3.2), Berkeley, were supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. X-ray diffraction experiments were performed at the Advanced Photon Source at Argonne National Laboratory (17-BM-B). Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. S. B., F. B. and V. C. acknowledge financial support from the Ateneo Project 2011 ORTO11RRT5. We also thank the National Science Foundation for providing graduate fellowship support (D. J. X. and J. A. M.). In addition, we are grateful for the support of E. D. B. through a Gerald K. Branch fellowship in chemistry, P. V. through a Phillips 66 Excellence Fellowship and M. R. H. through the National Institute of Standards and Technology/National Research Council Fellowship Program. We thank S. Chavan for help with the infrared spectroscopy experiments and fruitful discussion. NR 50 TC 83 Z9 84 U1 20 U2 168 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 EI 1755-4349 J9 NAT CHEM JI Nat. Chem. PD JUL PY 2014 VL 6 IS 7 BP 590 EP 595 DI 10.1038/NCHEM.1956 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AK5DM UT WOS:000338444600010 PM 24950328 ER PT J AU Shapiro, MG Ramirez, RM Sperling, LJ Sun, G Sun, J Pines, A Schaffer, DV Bajaj, VS AF Shapiro, Mikhail G. Ramirez, R. Matthew Sperling, Lindsay J. Sun, George Sun, Jinny Pines, Alexander Schaffer, David V. Bajaj, Vikram S. TI Genetically encoded reporters for hyperpolarized xenon magnetic resonance imaging SO NATURE CHEMISTRY LA English DT Article ID LASER-POLARIZED XE-129; GAS VESICLES; CONTRAST AGENTS; PICOMOLAR SENSITIVITY; FUNCTIONALIZED XENON; FLUORESCENT PROTEIN; MRI; NMR; EXCHANGE; BIOSENSOR AB Magnetic resonance imaging (MRI) enables high-resolution non-invasive observation of the anatomy and function of intact organisms. However, previous MRI reporters of key biological processes tied to gene expression have been limited by the inherently low molecular sensitivity of conventional H-1 MRI. This limitation could be overcome through the use of hyperpolarized nuclei, such as in the noble gas xenon, but previous reporters acting on such nuclei have been synthetic. Here, we introduce the first genetically encoded reporters for hyperpolarized Xe-129 MRI. These expressible reporters are based on gas vesicles (GVs), gas-binding protein nanostructures expressed by certain buoyant microorganisms. We show that GVs are capable of chemical exchange saturation transfer interactions with xenon, which enables chemically amplified GV detection at picomolar concentrations (a 100- to 10,000-fold improvement over comparable constructs for H-1 MRI). We demonstrate the use of GVs as heterologously expressed indicators of gene expression and chemically targeted exogenous labels in MRI experiments performed on living cells. C1 [Shapiro, Mikhail G.] Univ Calif Berkeley, Miller Res Inst, Berkeley, CA 94720 USA. [Shapiro, Mikhail G.; Sun, Jinny; Schaffer, David V.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Shapiro, Mikhail G.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Shapiro, Mikhail G.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Ramirez, R. Matthew; Sun, Jinny; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Ramirez, R. Matthew; Sperling, Lindsay J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Schaffer, David V.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Shapiro, MG (reprint author), Univ Calif Berkeley, Miller Res Inst, Berkeley, CA 94720 USA. EM mikhail@caltech.edu; vikbajaj@gmail.com FU Miller Research Fellowship; Burroughs Wellcome Career Award at the Scientific Interface (M.G.S.); California Institute For Regenerative Medicine [RT2-02022]; Department of Energy [DE-AC02-05CH11231] FX We thank P. Dao for assistance with NMR measurements, M. Cannon for providing the pNL29 plasmid and R. Zalpuri and K. McDonald for assistance with electron microscopy. This work was supported by the Miller Research Fellowship and Burroughs Wellcome Career Award at the Scientific Interface (M.G.S.), California Institute For Regenerative Medicine grant RT2-02022 (D.V.S.) and Department of Energy contract DE-AC02-05CH11231 (A.P., V.S.B). NR 50 TC 42 Z9 43 U1 11 U2 60 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 EI 1755-4349 J9 NAT CHEM JI Nat. Chem. PD JUL PY 2014 VL 6 IS 7 BP 630 EP 635 DI 10.1038/NCHEM.1934 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AK5DM UT WOS:000338444600016 PM 24950334 ER PT J AU Mortimer, SA Kidwell, MA Doudna, JA AF Mortimer, Stefanie A. Kidwell, Mary Anne Doudna, Jennifer A. TI Insights into RNA structure and function from genome-wide studies SO NATURE REVIEWS GENETICS LA English DT Review ID SELECTIVE 2'-HYDROXYL ACYLATION; LONG NONCODING RNAS; MESSENGER-RNA; SECONDARY STRUCTURE; IN-VIVO; GLOBAL ANALYSIS; SACCHAROMYCES-CEREVISIAE; NUCLEOTIDE RESOLUTION; TARGET RECOGNITION; PROTEIN EXPRESSION AB A comprehensive understanding of RNA structure will provide fundamental insights into the cellular function of both coding and non-coding RNAs. Although many RNA structures have been analysed by traditional biophysical and biochemical methods, the low-throughput nature of these approaches has prevented investigation of the vast majority of cellular transcripts. Triggered by advances in sequencing technology, genome-wide approaches for probing the transcriptome are beginning to reveal how RNA structure affects each step of protein expression and RNA stability. In this Review, we discuss the emerging relationships between RNA structure and the regulation of gene expression. C1 [Mortimer, Stefanie A.; Kidwell, Mary Anne; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Guardant Hlth Inc, 2686 Middlefield Rd, Redwood City, CA 94063 USA. EM doudna@berkeley.edu FU US National Institutes of Health FX The authors apologize to colleagues whose work was not cited owing to space limitation. They thank Y. Bai, R. Wilson, S. Floor, M. Hammond and members of J.A.D.'s laboratory for discussions; K Weeks for sharing HIV-1 SHAPE data; and J. Ji for reading the manuscript. This work was supported in part by a grant from the US National Institutes of Health (to J.A.D.). J.A.D. is a Howard Hughes Medical Institute Investigator. NR 103 TC 89 Z9 90 U1 6 U2 71 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1471-0056 EI 1471-0064 J9 NAT REV GENET JI Nat. Rev. Genet. PD JUL PY 2014 VL 15 IS 7 BP 469 EP 479 DI 10.1038/nrg3681 PG 11 WC Genetics & Heredity SC Genetics & Heredity GA AK4KT UT WOS:000338394300010 PM 24821474 ER PT J AU Balden, M Endstrasser, N Humrickhouse, PW Rohde, V Rasinski, M von Toussaint, U Elgeti, S Neu, R AF Balden, M. Endstrasser, N. Humrickhouse, P. W. Rohde, V. Rasinski, M. von Toussaint, U. Elgeti, S. Neu, R. CA ASDEX Upgrade Team TI Collection strategy, inner morphology, and size distribution of dust particles in ASDEX Upgrade SO NUCLEAR FUSION LA English DT Article DE dust; particles size distribution; tungsten; tokamak; SEM ID FUSION DEVICES; PLASMA PERFORMANCE; TUNGSTEN LAYERS; CARBON DUST; VACUUM ARCS; DIII-D; TOKAMAK; DEPOSITION; DISCHARGE; DIVERTOR AB The dust collection and analysis strategy in ASDEX Upgrade (AUG) is described. During five consecutive operation campaigns (2007-2011), Si collectors were installed, which were supported by filtered vacuum sampling and collection with adhesive tapes in 2009. The outer and inner morphology (e. g. shape) and elemental composition of the collected particles were analysed by scanning electron microscopy. The majority of the similar to 50 000 analysed particles on the Si collectors of campaign 2009 contain tungsten-the plasma-facing material in AUG-and show basically two different types of outer appearance: spheroids and irregularly shaped particles. By far most of the W-dominated spheroids consist of a solid W core, i.e. solidified W droplets. A part of these particles is coated with a low-Z material; a process that seems to happen presumably in the far scrape-off layer plasma. In addition, some conglomerates of B, C and W appear as spherical particles after their contact with plasma. By far most of the particles classified as B-, C- and W-dominated irregularly shaped particles consist of the same conglomerate with varying fraction of embedded W in the B-C matrix and some porosity, which can exceed 50%. The fragile structures of many conglomerates confirm the absence of intensive plasma contact. Both the ablation and mobilization of conglomerate material and the production of W droplets are proposed to be triggered by arcing. The size distribution of each dust particle class is best described by a log-normal distribution allowing an extrapolation of the dust volume and surface area. The maximum in this distribution is observed above the resolution limit of 0.28 mu m only for the W-dominated spheroids, at around 1 mu m. The amount of W-containing dust is extrapolated to be less than 300 mg on the horizontal areas of AUG. C1 [Balden, M.; Endstrasser, N.; Rohde, V.; Rasinski, M.; von Toussaint, U.; Elgeti, S.; Neu, R.; ASDEX Upgrade Team] Max Planck Inst Plasma Phys, EURATOM Assoc, D-85748 Garching, Germany. [Humrickhouse, P. W.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Rasinski, M.] Warsaw Univ Technol, Fac Mat Sci & Engn, PL-02507 Warsaw, Poland. RP Balden, M (reprint author), Max Planck Inst Plasma Phys, EURATOM Assoc, Boltzmannstr 2, D-85748 Garching, Germany. EM Martin.Balden@ipp.mpg.de RI Neu, Rudolf /B-4438-2010; OI Neu, Rudolf /0000-0002-6062-1955; Rasinski, Marcin/0000-0001-6277-4421 FU European Community FX This work, supported by the European Community under the contract of the EURATOM Association, was partly carried out within the framework of the EFDA Task Force on Plasma Wall Interactions. The views and opinions expressed herein do not necessarily reflect those of the European Commission. NR 77 TC 14 Z9 14 U1 1 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073010 DI 10.1088/0029-5515/54/7/073010 PG 16 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200016 ER PT J AU Futatani, S Huijsmans, G Loarte, A Baylor, LR Commaux, N Jernigan, TC Fenstermacher, ME Lasnier, C Osborne, TH Pegourie, B AF Futatani, S. Huijsmans, G. Loarte, A. Baylor, L. R. Commaux, N. Jernigan, T. C. Fenstermacher, M. E. Lasnier, C. Osborne, T. H. Pegourie, B. TI Non-linear MHD modelling of ELM triggering by pellet injection in DIII-D and implications for ITER SO NUCLEAR FUSION LA English DT Article DE ELM; ITER; ELM control; pellet pacing; ELM triggering; non-linear MHD AB Edge localized mode (ELM) triggering by pellet injection in the DIII-D tokamak has been simulated with the non-linear MHD code JOREK with a view to validating its physics models. JOREK has been subsequently applied to evaluate the requirements for ELM control by pellet injection in ITER. JOREK modelling results for DIII-D show that the key parameter for the triggering of ELMs by pellets is the value of the localized pressure perturbation caused by pellet injection which leads to a threshold minimum pellet size for a given injection velocity, injection geometry and H-mode plasma characteristics. The minimum pellet size for ELM triggering is found to depend on injection geometry with the largest value being required for injection at the outer midplane, intermediate for injection near the X-point and the smallest one for injection at the high-field side. The first results of studies for ELM triggering by pellet injection in ITER 15 MA Q = 10 plasmas with the foreseen injection geometry in ITER are presented. C1 [Futatani, S.; Huijsmans, G.; Loarte, A.] ITER Org, F-13115 St Paul Les Durance, France. [Baylor, L. R.; Commaux, N.; Jernigan, T. C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Fenstermacher, M. E.; Lasnier, C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Fenstermacher, M. E.; Lasnier, C.; Osborne, T. H.] Gen Atom Co, San Diego, CA 92186 USA. [Pegourie, B.] CEA IRFM, F-13108 St Paul Les Durance, France. RP Futatani, S (reprint author), ITER Org, F-13115 St Paul Les Durance, France. EM alberto.loarte@iter.org OI Futatani, Shimpei/0000-0001-5742-5454 FU US DOE [DE-AC05-00OR22725, DE-AC52-07NA27344, DE-FC02-04ER54698] FX This work was supported in part by the US DOE under DE-AC05-00OR22725, DE-AC52-07NA27344, and DE-FC02-04ER54698. Part of this work was carried out using the HELIOS supercomputer system at Computational Situational Centre of International Fusion Energy Research Centre (IFERC-CSC), Aomori, Japan, under the Broader Approach collaboration between Euratom and Japan, implemented by Fusion for Energy and JAEA. NR 19 TC 12 Z9 12 U1 2 U2 21 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073008 DI 10.1088/0029-5515/54/7/073008 PG 20 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200014 ER PT J AU Garofalo, AM Chan, VS Canik, JM Sawan, ME Choi, M Humphreys, DA Lao, LL Prater, R Stangeby, PC St John, HE Taylor, TS Turnbull, AD Wong, CPC AF Garofalo, A. M. Chan, V. S. Canik, J. M. Sawan, M. E. Choi, M. Humphreys, D. A. Lao, L. L. Prater, R. Stangeby, P. C. St John, H. E. Taylor, T. S. Turnbull, A. D. Wong, C. P. C. TI Progress in the physics basis of a Fusion Nuclear Science Facility based on the Advanced Tokamak concept SO NUCLEAR FUSION LA English DT Article DE fusion reactor design; steady-state scenario simulation; divertor analysis ID DIII-D; PLASMAS; PERFORMANCE; GEOMETRY; DIVERTOR AB Physics based integrated modelling of the baseline scenario for a Fusion Nuclear Science Facility based on the Advanced Tokamak concept (FNSF-AT) (Chan et al 2010 Fusion Sci. Technol. 57 66) has found steady-state equilibria with good stability and controllability properties at the fusion performance required to accomplish FNSF's nuclear science mission with margin. 2D divertor analysis for this baseline scenario predicts that peak heat flux <10 MW m(-2) can be obtained even with scrape-off layer power width similar to 1 mm. Using this baseline fusion performance, high fidelity and high-resolution 3D neutronics calculations show acceptable cumulative end-of-life organic insulator dose levels in all the device coils, and TBR > 1. Two current drive scenarios, two divertor configurations, and two blanket concepts have been analysed. FNSF-AT would complement ITER in addressing science and technology gaps to a commercially attractive DEMO, and could enable a DEMO construction decision triggered by the achievement of Q = 10 in ITER. C1 [Garofalo, A. M.; Chan, V. S.; Choi, M.; Humphreys, D. A.; Lao, L. L.; Prater, R.; St John, H. E.; Taylor, T. S.; Turnbull, A. D.; Wong, C. P. C.] Gen Atom Co, San Diego, CA 92186 USA. [Canik, J. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Sawan, M. E.] Univ Wisconsin, Fus Technol Inst, Madison, WI 53706 USA. [Stangeby, P. C.] Univ Toronto, Inst Aerosp Studies, Toronto, ON M3H 5T6, Canada. RP Garofalo, AM (reprint author), Gen Atom Co, POB 85608, San Diego, CA 92186 USA. EM garofalo@fusion.gat.com OI Canik, John/0000-0001-6934-6681 FU General Atomics IRD; US Department of Energy [DE-FC02-04ER54698, DE-FG02-95ER54309, DE AC05 00OR22725, DE-FG02-09ER54513] FX This work was supported in part by General Atomics IR&D funding, and the US Department of Energy under DE-FC02-04ER54698, DE-FG02-95ER54309, DE AC05 00OR22725 and DE-FG02-09ER54513. NR 37 TC 4 Z9 4 U1 2 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073015 DI 10.1088/0029-5515/54/7/073015 PG 13 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200021 ER PT J AU Gerasimov, SN Hender, TC Morris, J Riccardo, V Zakharov, LE AF Gerasimov, S. N. Hender, T. C. Morris, J. Riccardo, V. Zakharov, L. E. CA JET EFDA Contributors TI Plasma current asymmetries during disruptions in JET SO NUCLEAR FUSION LA English DT Article DE tokamak; disruption; VDE; kink instability; plasma current asymmetries ID ALCATOR C-MOD; MITIGATION; STABILITY AB A key feature of disruptions during vertical displacement events, discovered in JET in 1996, is the toroidal variation in the measured plasma current I-p, i.e. the plasma current asymmetries, lasting for almost the entire current quench. The unique magnetic diagnostics at JET (full set of poloidal coils and saddle loops recorded either from two toroidally opposite or from four toroidally orthogonal locations) allow for a comprehensive analysis of asymmetrical disruptions with a large scale database. This paper presents an analysis of 4854 disruptions over an 18 year period that includes both the JET carbon (C) wall and the ITER-like (IL) wall (a mixed beryllium/tungsten first wall). In spite of the I-p quench time significantly increasing for the IL-wall compared to C-wall disruptions, the observed toroidal asymmetry time integral (similar to sideways force impulse), did not increase for IL-wall disruptions. The I-p asymmetry has a dominantly n = 1 structure. Its motion in the toroidal direction has a sporadic behaviour, in general. The distributions of the number of rotation periods are found to be very similar for both C-and IL-wall disruptions, and multi-turn rotation was sometimes observed. The I-p asymmetry amplitude has no degradation with rotation frequency for either the C-or IL-wall disruption. Therefore dynamic amplification remains a potentially serious issue for ITER due to possible mechanical resonance of the machine components with the rotating asymmetry. C1 JET EFDA, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Gerasimov, S. N.; Hender, T. C.; Morris, J.; Riccardo, V.] Euratom CCFE Fus Assoc, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Zakharov, L. E.] Princeton Univ, PPPL, Princeton, NJ 08543 USA. RP Gerasimov, SN (reprint author), Euratom CCFE Fus Assoc, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. EM Sengei.Gerasimov@ccfe.ac.uk RI Gerasimov, Sergei/O-4881-2015; OI Gerasimov, Sergei/0000-0002-6249-2931; riccardo, valeria/0000-0003-2535-5257 FU European Communities; RCUK Energy Programme [EP/I501045]; US DoE [DE-AC02-09-CH11466] FX The authors would like to acknowledge M. F. Johnson for initial development of the JET disruption database and P. Noll for helpful discussions. This work, part-funded by the European Communities under the contract of Association between EURATOM/CCFE was carried out within the framework of the European Fusion Development Agreement. For further information on the contents of this paper please contact publications-officer@jet.efda.org. The views and opinions expressed herein do not necessarily reflect those of the European Commission. This work was also partially funded by the RCUK Energy Programme (grant number EP/I501045) and by the US DoE contract No DE-AC02-09-CH11466. NR 37 TC 17 Z9 17 U1 2 U2 33 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073009 DI 10.1088/0029-5515/54/7/073009 PG 14 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200015 ER PT J AU Kim, K Park, JK Boozer, AH Menard, JE Gerhardt, SP Logan, NC Wang, ZR Kramer, GJ Burrell, KH Garofalo, AM AF Kim, K. Park, J. -K. Boozer, A. H. Menard, J. E. Gerhardt, S. P. Logan, N. C. Wang, Z. R. Kramer, G. J. Burrell, K. H. Garofalo, A. M. TI Calculation of neoclassical toroidal viscosity with a particle simulation in the tokamak magnetic braking experiments SO NUCLEAR FUSION LA English DT Article DE tokamak; NTV; magnetic breaking; 3D field; drift-kinetic particle simulation ID BANANA-DRIFT TRANSPORT; MOMENTUM DISSIPATION; PLASMAS; RIPPLE AB Accurate calculation of perturbed distribution function delta f and perturbed magnetic field delta B is essential to achieve prediction of non-ambipolar transport and neoclassical toroidal viscosity (NTV) in perturbed tokamaks. This paper reports a study of the NTV with a delta f particle code (POCA) and improved understanding of magnetic braking in tokamak experiments. POCA calculates the NTV by computing delta f with guiding-centre orbit motion and using delta B from the ideal perturbed equilibrium code (IPEC). Theories of NTV for magnetic field resonance, collisionality dependency, and toroidal mode coupling are tested in the simple configurations using the particle simulations. The POCA simulations are also compared with experimental estimations for NTV, which are measured from angular momentum balance (DIII-D) and toroidal rotational damping rate (NSTX). The calculation shows reasonable agreement in total NTV torque for the DIII-D discharge with weak rotational resonances in the nu(-) root nu. regime. In NSTX discharges where the bounce-harmonic resonances dominantly appear, the POCA simulation gives total NTV torques comparable to the measurements, however large discrepancies are found in the detailed damping and NTV profiles. It is discussed that a self-consistent calculation of delta B using general perturbed equilibria is eventually necessary since a non-ideal plasma response can change the perturbed field and thereby the NTV torque. C1 [Kim, K.; Park, J. -K.; Menard, J. E.; Gerhardt, S. P.; Logan, N. C.; Wang, Z. R.; Kramer, G. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Boozer, A. H.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Burrell, K. H.; Garofalo, A. M.] Gen Atom Co, San Diego, CA 92186 USA. RP Kim, K (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM kkim@pppl.gov OI Menard, Jonathan/0000-0003-1292-3286 FU DOE [DE-AC02-09CH11466, DE-FC02-04ER54698] FX This work was supported by DOE Contract No DE-AC02-09CH11466 (PPPL) and No DE-FC02-04ER54698 (GA). NR 39 TC 7 Z9 7 U1 1 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073014 DI 10.1088/0029-5515/54/7/073014 PG 11 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200020 ER PT J AU Kolemen, E Welander, AS La Haye, RJ Eidietis, NW Humphreys, DA Lohr, J Noraky, V Penaflor, BG Prater, R Turco, F AF Kolemen, E. Welander, A. S. La Haye, R. J. Eidietis, N. W. Humphreys, D. A. Lohr, J. Noraky, V. Penaflor, B. G. Prater, R. Turco, F. TI State-of-the-art neoclassical tearing mode control in DIII-D using real-time steerable electron cyclotron current drive launchers SO NUCLEAR FUSION LA English DT Article DE spherical tokamaks; macroinstabilities; plasma diagnostic techniques; current drive; helicity injection ID D TOKAMAK; STABILIZATION; SYSTEM; JT-60U AB Real-time steerable electron cyclotron current drive (ECCD) has been demonstrated to reduce the power requirements and time needed to remove 3/2 and 2/1 neoclassical tearing modes (NTMs) in the DIII-D tokamak. In a world first demonstration of the techniques required in ITER, the island formation onset is detected automatically, gyrotrons are turned on and the real-time steerable ECCD launcher mirrors are moved promptly to drive current at the location of the islands. This shrinks and suppresses the modes well before saturation using real-time motional Stark effect constrained equilibria reconstruction with advanced feedback and search algorithms to target the deposition. In ITER, this method will reduce the ECCD energy requirement and so raise Q by keeping the EC system off when the NTM is not present. Further, in the experiments with accurate tracking of pre-emptive ECCD to resonant surfaces, both 3/2 and 2/1 modes are prevented from appearing with much lower ECCD peak power than required for removal of a saturated mode. C1 [Kolemen, E.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Welander, A. S.; La Haye, R. J.; Eidietis, N. W.; Humphreys, D. A.; Lohr, J.; Noraky, V.; Penaflor, B. G.; Prater, R.] Gen Atom Co, San Diego, CA 92186 USA. [Turco, F.] Columbia Univ, New York, NY 10027 USA. RP Kolemen, E (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU US Department of Energy [DE-AC02-09CH11466, DE-FC02-04ER54698, DE-FG0204ER54761] FX This work is supported by the US Department of Energy under DE-AC02-09CH11466, DE-FC02-04ER54698 and DE-FG0204ER54761. NR 16 TC 12 Z9 12 U1 2 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073020 DI 10.1088/0029-5515/54/7/073020 PG 7 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200026 ER PT J AU Paz-Soldan, C Buttery, RJ Garofalo, AM Hanson, JM La Haye, RJ Lanctot, MJ Park, JK Solomon, WM Strait, EJ AF Paz-Soldan, C. Buttery, R. J. Garofalo, A. M. Hanson, J. M. La Haye, R. J. Lanctot, M. J. Park, J. K. Solomon, W. M. Strait, E. J. TI The spectral basis of optimal error field correction on DIII-D SO NUCLEAR FUSION LA English DT Article DE error field correction; plasma response; resistive wall mode; kink mode; tokamak ID D TOKAMAK; MODES; PLASMAS AB Experimental optimum error field correction (EFC) currents found in a wide breadth of dedicated experiments on DIII-D are shown to be consistent with the currents required to null the poloidal harmonics of the vacuum field which drive the kink mode near the plasma edge. This allows the identification of empirical metrics which predict optimal EFC currents with accuracy comparable to that of first-principles modelling which includes the ideal plasma response. While further metric refinements are desirable, this work suggests optimal EFC currents can be effectively fed-forward based purely on knowledge of the vacuum error field and basic equilibrium properties which are routinely calculated in real-time. C1 [Paz-Soldan, C.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Buttery, R. J.; Garofalo, A. M.; La Haye, R. J.; Lanctot, M. J.; Strait, E. J.] Gen Atom Co, San Diego, CA 92186 USA. [Hanson, J. M.] Columbia Univ, New York, NY 10027 USA. [Park, J. K.; Solomon, W. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Paz-Soldan, C (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. EM paz-soldan@fusion.gat.com RI Lanctot, Matthew J/O-4979-2016; OI Lanctot, Matthew J/0000-0002-7396-3372; Solomon, Wayne/0000-0002-0902-9876 FU US Department of Energy [DE-AC05-06OR23100, DE-FC02-04ER54698, DE-FG02-04ER54761, DE-AC02-09CH11466] FX This work is supported by the US Department of Energy under DE-AC05-06OR23100, DE-FC02-04ER54698, DE-FG02-04ER54761, and DE-AC02-09CH11466. The authors would like to acknowledge all individuals involved with the execution of the dedicated experiments presented herein. Individuals such as D. Shiraki, Y. In, M. Okabayashi, J.T. Scoville, M.J. Schaffer, and H. Reimerdes, have contributed to the measurement of the experimental Iopt here presented. The authors also thank M.J. Schaffer, T. E. Evans, and D. M. Orlov for developing and maintaining the SURFMN code which was used extensively for this study. NR 38 TC 18 Z9 18 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073013 DI 10.1088/0029-5515/54/7/073013 PG 12 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200019 ER PT J AU Poli, FM Kessel, CE Bonoli, PT Batchelor, DB Harvey, RW Snyder, PB AF Poli, F. M. Kessel, C. E. Bonoli, P. T. Batchelor, D. B. Harvey, R. W. Snyder, P. B. TI External heating and current drive source requirements towards steady-state operation in ITER SO NUCLEAR FUSION LA English DT Article DE steady-state; heating; internal barriers; tokamak; reactor; current drive ID INTERNAL TRANSPORT BARRIERS; H-MODE PLASMAS; JET; TOKAMAKS; SIMULATION; ISSUES AB Steady state scenarios envisaged for ITER aim at optimizing the bootstrap current, while maintaining sufficient confinement and stability to provide the necessary fusion yield. Non-inductive scenarios will need to operate with internal transport barriers (ITBs) in order to reach adequate fusion gain at typical currents of 9 MA. However, the large pressure gradients associated with ITBs in regions of weak or negative magnetic shear can be conducive to ideal MHD instabilities, reducing the no-wall limit. The E x B flow shear from toroidal plasma rotation is expected to be low in ITER, with a major role in the ITB dynamics being played by magnetic geometry. Combinations of heating and current drive (H/CD) sources that sustain reversed magnetic shear profiles throughout the discharge are the focus of this work. Time-dependent transport simulations indicate that a combination of electron cyclotron (EC) and lower hybrid (LH) waves is a promising route towards steady state operation in ITER. The LH forms and sustains expanded barriers and the EC deposition at mid-radius freezes the bootstrap current profile stabilizing the barrier and leading to confinement levels 50% higher than typical H-mode energy confinement times. Using LH spectra with spectrum centred on parallel refractive index of 1.75-1.85, the performance of these plasma scenarios is close to the ITER target of 9 MA non-inductive current, global confinement gain H-98 = 1.6 and fusion gain Q = 5. C1 [Poli, F. M.; Kessel, C. E.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Bonoli, P. T.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Batchelor, D. B.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Harvey, R. W.] CompX, Del Mar, CA 92014 USA. [Snyder, P. B.] Gen Atom Co, San Diego, CA 92186 USA. RP Poli, FM (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RI poli, francesca/C-2226-2008 OI poli, francesca/0000-0003-3959-4371 FU TRANSP; IPS; US Department of Energy [DE-AC02-CH0911466, DE-AC05-00OR22725]; Scientific Discovery through Advanced Computing (SciDAC) program - US Department of Energy, Office of Science, Fusion Energy Sciences; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX We acknowledge R. Andre, M. Gorelenkova, X. Xuan and T. Ludescher-Furth for support with TRANSP, W. Elwasiv for support with the IPS, N. Bertelli for helpful discussion. This work was supported by the US Department of Energy under contract DE-AC02-CH0911466. ORNL is managed by UT-Battelle, LLC for the US Department of Energy under Contract DE-AC05-00OR22725. Partial support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) program, funded by US Department of Energy, Office of Science, Fusion Energy Sciences. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No DE-AC02-05CH11231. NR 47 TC 7 Z9 7 U1 1 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073007 DI 10.1088/0029-5515/54/7/073007 PG 12 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200013 ER PT J AU Rack, M Sieglin, B Eich, T Pearson, J Liang, Y Balboa, I Jachmich, S Wingen, A Pamela, SJP AF Rack, M. Sieglin, B. Eich, T. Pearson, J. Liang, Y. Balboa, I. Jachmich, S. Wingen, A. Pamela, S. J. P. CA JET EFDA Contributors TI Findings of pre-ELM structures through the observation of divertor heat load patterns at JET with applied n=2 perturbation fields SO NUCLEAR FUSION LA English DT Article DE edge-localized modes; resonant magnetic perturbations; divertor heat loads ID CONFINEMENT; DISCHARGES; TOKAMAK AB Resonant magnetic perturbation experiments at JET with the ITER-like wall have shown the formation of radially propagating pre-ELM structures in the heat flux profile on the outer divertor. These appear a few milliseconds before the major divertor heat load, caused by type-I edge-localized modes (ELMs). The formation of the pre-ELM structures is accompanied by an increase in the D-alpha emission. For some pronounced examples, the propagation appears to end at the positions where an increased heat load is seen during the ELM crash a few milliseconds later. These observations are presented and discussed along with a comparison of a thermoelectric edge currents model. C1 JET EFDA, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Rack, M.; Pearson, J.; Liang, Y.] Forschungszentrum Julich, Inst Energie & Klimaforsch Plasmaphys, EURATOM Assoc, D-52425 Julich, Germany. [Sieglin, B.; Eich, T.] EURATOM, Max Planck Inst Plasmaphys, D-85748 Garching, Germany. [Balboa, I.] EURATOM CCFE Fus Assoc, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Jachmich, S.] Ecole Royale Mil, Partner Trilateral Euregio Cluster, Assoc Euratom Belgian State, Plasma Phys Lab, B-1000 Brussels, Belgium. [Wingen, A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Pamela, S. J. P.] Aix Marseille Univ, CNRS, IIFS PIIM, F-13397 Marseille 20, France. RP Rack, M (reprint author), Forschungszentrum Julich, Inst Energie & Klimaforsch Plasmaphys, EURATOM Assoc, D-52425 Julich, Germany. EM m.rack@fz-juelich.de OI Wingen, Andreas/0000-0001-8855-1349 FU European Communities; Helmholtz Association in frame of the Helmholtz-University [VH-NG-410] FX Valuable discussions with Peter de Vries and Sebastijan Brezinsek are gratefully acknowledged. M R is thankful for the support of Evgenij Bleile and Gotz Lehmann. This work, supported by the European Communities under the contract of Association between EURATOM and FZJ, was carried out within the framework of the European Fusion Development Agreement. The views and opinions expressed herein do not necessarily reflect those of the European Commission. Additional support from the Helmholtz Association in frame of the Helmholtz-University Young Investigators Group VH-NG-410 is gratefully acknowledged. NR 33 TC 1 Z9 1 U1 2 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 072004 DI 10.1088/0029-5515/54/7/072004 PG 6 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200004 ER PT J AU Schmitz, L Zeng, L Rhodes, TL Hillesheim, JC Peebles, WA Groebner, RJ Burrell, KH McKee, GR Yan, Z Tynan, GR Diamond, PH Boedo, JA Doyle, EJ Grierson, BA Chrystal, C Austin, ME Solomon, WM Wang, G AF Schmitz, L. Zeng, L. Rhodes, T. L. Hillesheim, J. C. Peebles, W. A. Groebner, R. J. Burrell, K. H. McKee, G. R. Yan, Z. Tynan, G. R. Diamond, P. H. Boedo, J. A. Doyle, E. J. Grierson, B. A. Chrystal, C. Austin, M. E. Solomon, W. M. Wang, G. TI The role of zonal flows and predator-prey oscillations in triggering the formation of edge and core transport barriers SO NUCLEAR FUSION LA English DT Article DE tokamak; DIII-D; L-H transition; zonal flows; internal transport barriers; predator-prey oscillations ID DIII-D TOKAMAK; TURBULENCE; PLASMAS; SHEAR AB We present direct evidence of low frequency, radially sheared, turbulence-driven flows (zonal flows (ZFs)) triggering edge transport barrier formation preceding the L- to H-mode transition via periodic turbulence suppression in limit-cycle oscillations (LCOs), consistent with predator-prey dynamics. The final transition to edge-localized mode-free H-mode occurs after the equilibrium E x B flow shear increases due to ion pressure profile evolution. ZFs are also observed to initiate formation of an electron internal transport barrier (ITB) at the q = 2 rational surface via local suppression of electron-scale turbulence. Multi-channel Doppler backscattering (DBS) has revealed the radial structure of the ZF-induced shear layer and the E x B shearing rate, omega(ExB), in both barrier types. During edge barrier formation, the shearing rate lags the turbulence envelope during the LCO by 90 degrees, transitioning to anti-correlation (180 degrees) when the equilibrium shear dominates the turbulence-driven flow shear due to the increasing edge pressure gradient. The time-dependent flow shear and the turbulence envelope are anti-correlated (180 degrees out of phase) in the electron ITB. LCOs with time-reversed evolution dynamics (transitioning from an equilibrium-flow dominated to a ZF-dominated state) have also been observed during the H-L back-transition and are potentially of interest for controlled ramp-down of the plasma stored energy and pressure (normalized to the poloidal magnetic field) beta(theta) = 2 mu(0)n(T-e + T-i)/B-theta(2) in ITER. C1 [Schmitz, L.; Zeng, L.; Rhodes, T. L.; Peebles, W. A.; Doyle, E. J.; Wang, G.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Hillesheim, J. C.] EURATOM CCFE Fus Assoc, Abingdon OX14 3DB, Oxon, England. [Groebner, R. J.; Burrell, K. H.] Gen Atom Co, San Diego, CA 92186 USA. [McKee, G. R.; Yan, Z.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Tynan, G. R.; Diamond, P. H.; Boedo, J. A.] Univ Calif San Diego, Ctr Momentum Transport & Flow Org, La Jolla, CA 92093 USA. [Diamond, P. H.] NFRI, WCI Ctr Fus Theory, Taejon 305333, South Korea. [Grierson, B. A.; Solomon, W. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Chrystal, C.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Austin, M. E.] Univ Texas Austin, Inst Fus Studies, Austin, TX 78712 USA. RP Schmitz, L (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. EM lschmitz@ucla.edu OI Solomon, Wayne/0000-0002-0902-9876 FU US Department of Energy [DE-FG03-01ER54615, DE-FG02-08ER54984, DE-FC02-04ER54698, DE-FG02-89ER53296, DE-FG02-08ER54999, DE-FG02-07ER54917, DE-AC02-09CH11466, DE-FG03-97ER54415] FX This work was supported in part by the US Department of Energy under DE-FG03-01ER54615, DE-FG02-08ER54984, DE-FC02-04ER54698, DE-FG02-89ER53296, DE-FG02-08ER54999, DE-FG02-07ER54917, DE-AC02-09CH11466 and DE-FG03-97ER54415. NR 35 TC 14 Z9 14 U1 2 U2 33 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073012 DI 10.1088/0029-5515/54/7/073012 PG 11 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200018 ER PT J AU Stacey, WM Grierson, BA AF Stacey, Weston M. Grierson, Brian A. TI Interpretation of rotation and momentum transport in the DIII-D edge plasma and comparison with neoclassical theory SO NUCLEAR FUSION LA English DT Article DE rotation; intrinsic rotation; momentum transport ID TOKAMAK PLASMA; TOROIDAL ROTATION; ELECTRIC-FIELD AB A low-confinement mode discharge which optimizes the capability of the new main-ion charge-exchange-recombination spectroscopy system on DIII-D (Luxon 2002 Nucl. Fusion 42 614) to measure deuterium toroidal velocity is interpretted in comparison with the predictions of neoclassical theory, with an emphasis on the plasma edge region. The observed peaking in the deuterium toroidal velocity near the separatrix is shown to be consistent with intrinsic co-rotation due to ion orbit loss. In general, the standard neoclassical toroidal and poloidal momentum transport rates are found to be smaller than those inferred from experiment. C1 [Stacey, Weston M.] Georgia Inst Technol, Atlanta, GA 30332 USA. [Grierson, Brian A.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Stacey, WM (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA. FU DOE [DE-FG02-ER54538, DE-AC02-09CH11466]; Georgia Tech Research Corporation; Princeton Plasma Physics Laboratory; General Atomics [DE-AC03-99ER54463] FX The authors acknowledge their gratitude to other members of the DIII-D Team whose efforts have made these measurements possible, and in particular to Colin Chrystal for reducing the carbon spectroscopic data. The first author expresses his appreciation to General Atomics for their hospitality during part of this work. The work was supported by DOE grant DE-FG02-ER54538 with the Georgia Tech Research Corporation and by DOE contracts DE-AC02-09CH11466 with the Princeton Plasma Physics Laboratory and DE-AC03-99ER54463 with General Atomics. NR 37 TC 12 Z9 12 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2014 VL 54 IS 7 AR 073021 DI 10.1088/0029-5515/54/7/073021 PG 11 WC Physics, Fluids & Plasmas SC Physics GA AK3SE UT WOS:000338344200027 ER PT J AU Umeda, T Ueno, S Nakamura, TKM AF Umeda, Takayuki Ueno, Satoshi Nakamura, Takuma K. M. TI Ion kinetic effects on nonlinear processes of the Kelvin-Helmholtz instability SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE Kelvin-Helmholtz instability; Vlasov equation; hydrodynamic instability; plasma turbulence ID SOLAR-WIND; SIMULATION; BOUNDARY; MAGNETOPAUSE; RECONNECTION; TRANSPORT; VORTICES; EQUATION; SCHEME; FIELDS AB The nonlinear evolution of the Kelvin-Helmholtz (KH) instability at a transverse velocity shear layer in an inhomogeneous space plasma is investigated by means of a four-dimensional (two spatial and two velocity dimensions) electromagnetic Vlasov simulation. When the rotation direction of the primary KH vortex and the direction of ion gyro motion are the same (i.e., the inner product between the vorticity of the primary velocity shear and the magnetic field vector is negative) there exists a strong ion cyclotron damping. In this case, spatial inhomogeneity inside the primary KH vortex is smoothed and the secondary Rayleigh-Taylor/KH instabilities are suppressed. It is also found that another secondary instability on the electron inertial scale is simultaneously generated at secondary shear layers for both cases, but at different locations. The small-scale secondary instability takes place only when the inner product between the vorticity of the secondary shear layer and the magnetic field vector is positive, suggesting the damping of small-scale processes by ion gyro motion. These results indicate that secondary instabilities occurring in the nonlinear stage of the primary KHI show different evolutions depending on the sign of the inner product between the magnetic field and the vorticity of the velocity shear layer. C1 [Umeda, Takayuki; Ueno, Satoshi] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Nakamura, Takuma K. M.] Los Alamos Natl Lab, X Computat Phys Div, Los Alamos, NM 87545 USA. RP Umeda, T (reprint author), Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. EM umeda@stelab.nagoya-u.ac.jp FU MEXT/JSPS [23740367, 25610144]; JHPCN program at Joint Usage/Research Center for Interdisciplinary Large-Scale Information Infrastructures [jh130005-NA03]; HPCI Systems Research Project [hp120092] FX The authors thank Yosuke Matsumoto and Tatsuki Ogino for their discussions. This work was supported by MEXT/JSPS under Grant-in-Aid for Young Scientists (B) No 23740367 and Grant-in-Aid for Challenging Exploratory Research No 25610144. The computer simulations were performed on the DELL PowerEdge R815 supercomputer system at the Solar-Terrestrial Environment Laboratory (STEL), the Fujitsu FX1 and HX600 supercomputer systems at the Information Technology Center, Nagoya University, the Fujitsu CX400 supercomputer system at the Research Institute for Information Technology, Kyushu University, and the Fujitsu FX10 supercomputer system at the Information Technology Center, University of Tokyo, and the K computer at the RIKEN Advanced Institute for Computational Science. The computational resources are provided as a STEL computational joint research program, a Nagoya University HPC program, a JHPCN program at Joint Usage/Research Center for Interdisciplinary Large-Scale Information Infrastructures (No jh130005-NA03), and the HPCI Systems Research Project (No hp120092). NR 45 TC 5 Z9 5 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD JUL PY 2014 VL 56 IS 7 AR 075006 DI 10.1088/0741-3335/56/7/075006 PG 11 WC Physics, Fluids & Plasmas SC Physics GA AK6CL UT WOS:000338515300007 ER PT J AU Ellison, PA McLaughlin, JP Stavsetra, L Gregorich, KE Nitsche, H AF Ellison, Paul A. McLaughlin, Joseph P. Stavsetra, Liv Gregorich, Kenneth E. Nitsche, Heino TI Measurement of the Am-240 production cross section via proton irradiation of Pu-242 SO RADIOCHIMICA ACTA LA English DT Article DE Am-240; Production cross section; Proton irradiation ID EXCITATION-FUNCTIONS; ACTINIDE PRODUCTION; HEAVIEST ELEMENTS; NATURAL NICKEL; ENERGY-RANGE; FISSION; NP-237; PURPOSES; TARGETS; NUCLEI AB A new nuclear reaction for the production of Am-240 was experimentally investigated. Targets of 150-500 mu g/cm(2) Pu-242 on 2 mu mTi were produced through molecular deposition. Five irradiations, in which Pu-242, Ti-nat, and Ni-nat targets were jointly activated with protons from the Lawrence Berkeley National Laboratory 88-Inch Cyclotron produced Am-240, V-48, and Ni-57, respectively. The radioactive decay of these nuclides was monitored using high-purity Ge gamma ray detectors in the weeks following irradiation. A maximum Pu-242(p, 3n)Am-240 nuclear reaction cross section was measured to be 45 +/- 13 mb with 23 MeV protons. While this value is lower than theoretical predictions, it is high enough to be the most viable nuclear reaction for the large-scale production of Am-240. C1 [Ellison, Paul A.; McLaughlin, Joseph P.; Nitsche, Heino] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ellison, Paul A.; McLaughlin, Joseph P.; Gregorich, Kenneth E.; Nitsche, Heino] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Stavsetra, Liv] Inst Energy Technol, N-2007 Kjeller, Norway. RP Nitsche, H (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM HNitsche@berkeley.edu FU U.S. Department of Energy (DOE), National Nuclear Security Administration (NNSA) Steawardship Science Academic Alliance program [DE-FG52-06NA27480, DE-FG52-10NA29652]; DOE NNSA Stewardship Science Graduate Fellowship [DE-FC52-08NA28752] FX The authors would like to thank the LBNL staff, operators of the 88-Inch Cyclotron, Jan Dvorak, Zuzana Dvorakova, and Jacklyn Gates for their kind assistance during and following the 242Pu irradiations and Nicholas Esker for helpful editorial comments. Financial support was provided by U.S. Department of Energy (DOE), National Nuclear Security Administration (NNSA) Steawardship Science Academic Alliance program under Contracts No. DE-FG52-06NA27480 and DE-FG52-10NA29652. P.A.E. was supported by a DOE NNSA Stewardship Science Graduate Fellowship under Contract No. DE-FC52-08NA28752. NR 40 TC 1 Z9 1 U1 0 U2 6 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PD JUL PY 2014 VL 102 IS 7 BP 561 EP 568 DI 10.1515/ract-2014-2219 PG 8 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AK5UD UT WOS:000338491000001 ER PT J AU Engle, JW Weidner, JW Ballard, BD Fassbender, ME Hudston, LA Jackman, KR Dry, DE Wolfsberg, LE Bitteker, LJ Ullmann, JL Gulley, MS Pillai, C Goff, G Birnbaum, ER John, KD Mashnik, SG Nortier, FM AF Engle, Jonathan W. Weidner, John W. Ballard, Beau D. Fassbender, Michael E. Hudston, Lisa A. Jackman, Kevin R. Dry, Donald E. Wolfsberg, Laura E. Bitteker, Leo J. Ullmann, John L. Gulley, Mark S. Pillai, Chandra Goff, George Birnbaum, Eva R. John, Kevin D. Mashnik, Stepan G. Nortier, Francois M. TI Ac, La, and Ce radioimpurities in Ac-225 produced in 40-200 MeV proton irradiations of thorium SO RADIOCHIMICA ACTA LA English DT Article DE Ac-225; Ac-227; Ce-139; Ce-141; Ce-143; La-140; Ba-140; Alpha-emitting; Radionuclides; Radiotherapy; Proton irradiation; Thorium ID CROSS-SECTIONS; RADIOIMMUNOTHERAPY; ACTINIUM; ISOTOPES; THERAPY; SPECTRA AB Accelerator production of Ac-225 addresses the global supply deficiency currently inhibiting clinical trials fromestablishing Ac-225's therapeutic utility, provided that the accelerator product is of sufficient radionuclidic purity for patient use. Two proton activation experiments utilizing the stacked foil technique between 40 and 200MeV were employed to study the likely co-formation of radionuclides expected to be especially challenging to separate from Ac-225. Foils were assayed by nondestructive gamma-spectroscopy and by alpha-spectroscopy of chemically processed target material. Nuclear formation cross sections for the radionuclides Ac-226 and Ac-227 as well as lower lanthanide radioisotopes Ce-139, Ce-141, Ce-143, and La-140 whose elemental ionic radii closely match that of actinium were measured and are reported. The predictions of the latest MCNP6 event generators are compared with measured data, as they permit estimation of the formation rates of other radionuclides whose decay emissions are not clearly discerned in the complex spectra collected from Th-232(p,x) fission product mixtures. C1 [Engle, Jonathan W.; Ballard, Beau D.; Fassbender, Michael E.; Hudston, Lisa A.; Jackman, Kevin R.; Dry, Donald E.; Wolfsberg, Laura E.; Bitteker, Leo J.; Ullmann, John L.; Gulley, Mark S.; Pillai, Chandra; Goff, George; Birnbaum, Eva R.; John, Kevin D.; Mashnik, Stepan G.; Nortier, Francois M.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Weidner, John W.] Air Force Inst Technol, Wright Patterson AFB, OH USA. RP Engle, JW (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87544 USA. EM jwengle@lanl.gov RI Ballard, Beau/E-2925-2017; OI Ballard, Beau/0000-0003-1206-9358; John, Kevin/0000-0002-6181-9330 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA253996]; US DOE Office of Science via award from The Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics FX We are grateful for technical assistance from LANL C-NR, C-IIAC, AOT-OPS, and LANSCEWNR groups' staff. This study was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA253996 with partial funding by the US DOE Office of Science via an award from The Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics. NR 34 TC 9 Z9 9 U1 1 U2 17 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PD JUL PY 2014 VL 102 IS 7 BP 569 EP 581 DI 10.1515/ract-2013-2179 PG 13 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AK5UD UT WOS:000338491000002 ER PT J AU Zimmerman, T Zavarin, M Powell, BA AF Zimmerman, Trevor Zavarin, Mavrik Powell, Brian A. TI Influence of humic acid on plutonium sorption to gibbsite: Determination of Pu-humic acid complexation constants and ternary sorption studies SO RADIOCHIMICA ACTA LA English DT Article DE Plutonium; Humic acid; Sorption; Ternary complex; Gibbsite ID METAL-IONS; SUBSTANCES; REDUCTION; ADSORPTION; TETRAVALENT; KAOLINITE; GOETHITE; SYSTEMS; PU(V); PH AB In this work stability constants describing Pu(IV), Th(IV), and Np(V) binding to Leonardite humic acid (HA) were determined using a discrete pK(a). model. A hybrid ultra-filtration/equilibrium dialysis, ligand exchange technique was used to generate the partitioning data. Ethylenediaminetetraacetic acid (EDTA) was used as a reference ligand to allow the aqueous chemistry of the Pu(IV)-HA system to be examined over a range of pH values, while minimizing the possibility of precipitation of Pu(IV). The conditional stability constant for Pu(IV) complexation with HA determined as part of this work is log beta(112) = 6.76 +/- 0.14 based on the equation: Pu4+ + HL3 + 2H(2)O <-> Pu(OH)(2)L3(+) + 3H(+) where HA is represented by HL3 (a binding site on the HA with a pK(a) value of 7). This value is three orders of magnitude higher than the Th(IV)-HA constant and between six and eight orders of magnitude higher than the Np(V)-HA complex. The magnitude of the stability constants and the general trend of increasing complexation strength with increasing pH is consistent with previous observations. The Pu(IV)-HA stability constants were used to model sorption of Pu(IV) to gibbsite in the presence of HA. Assuming only aqueous Pu-HA complexes and AlOH-Pu surface complexes, the model was unable to predict the observed data which exhibited greater sorption at pH 4 relative to pH 6; a phenomenon which does not occur in the absence of HA. Therefore, this study demonstrates that ternary Pu-HA-gibbsite complexes may form under low pH conditions and exhibit greater sorption than that observed in the absence of HA. Although the presence of HA may increase the solubility/aqueous concentrations of Pu in the absence of a solid phase, formation of ternary complexes may indeed retard the subsurface migration of Pu. The corollary to this finding is that increased mobility may occur if the ternary surface complex forms on a mobile colloid rather than part of the subsurface matrix C1 [Zimmerman, Trevor; Powell, Brian A.] Clemson Univ, Anderson, SC 29625 USA. [Zavarin, Mavrik] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Glenn T Seaborg Inst, Livermore, CA 94551 USA. RP Powell, BA (reprint author), Clemson Univ, Anderson, SC 29625 USA. EM bpowell@clemson.edu RI Powell, Brian /C-7640-2011 OI Powell, Brian /0000-0003-0423-0180 FU Subsurface Biogeochemical Research Program of the U.S. Department of Energy's Office of Biological and Environmental Research FX The authors wish to thank Dr. Annie B. Kersting of Lawrence Livermore National Laboratory and Dr. Ruth Tinnacher of Lawrence Berkeley National Laboratory for helpful discussions regarding this work. This work was supported by the Subsurface Biogeochemical Research Program of the U. S. Department of Energy's Office of Biological and Environmental Research. NR 44 TC 7 Z9 7 U1 2 U2 43 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PD JUL PY 2014 VL 102 IS 7 BP 629 EP 643 DI 10.1515/ract-2014-2163 PG 15 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AK5UD UT WOS:000338491000008 ER PT J AU Chakrabarty, RK Beres, ND Moosmuller, H China, S Mazzoleni, C Dubey, MK Liu, L Mishchenko, MI AF Chakrabarty, Rajan K. Beres, Nicholas D. Moosmueller, Hans China, Swarup Mazzoleni, Claudio Dubey, Manvendra K. Liu, Li Mishchenko, Michael I. TI Soot superaggregates from flaming wildfires and their direct radiative forcing SO SCIENTIFIC REPORTS LA English DT Article ID INDIVIDUAL AEROSOL-PARTICLES; BIOMASS BURNING PARTICLES; SOUTHERN AFRICA; CARBONACEOUS PARTICLES; FRACTAL DIMENSION; LIGHT-SCATTERING; BROWN CARBON; MEXICO-CITY; T-MATRIX; ABSORPTION AB Wildfires contribute significantly to global soot emissions, yet their aerosol formation mechanisms and resulting particle properties are poorly understood and parameterized in climate models. The conventional view holds that soot is formed via the cluster-dilute aggregation mechanism in wildfires and emitted as aggregates with fractal dimension D-f approximate to 1.8 mobility diameter D-m <= 1 mu m, and aerodynamic diameter D-a <= 300 nm. Here we report the ubiquitous presence of soot superaggregates (SAs) in the outflow from a major wildfire in India. SAs are porous, low-density aggregates of cluster-dilute aggregates with characteristic D-f approximate to 2.6, D-m > 1 mu m, and D-a <= 300 nm that form via the cluster-dense aggregation mechanism. We present additional observations of soot SAs in wildfire smoke-laden air masses over Northern California, New Mexico, and Mexico City. We estimate that SAs contribute, per unit optical depth, up to 35% less atmospheric warming than freshly-emitted (Df approximate to 1.8) aggregates, and approximate to 90% more warming than the volume-equivalent spherical soot particles simulated in climate models. C1 [Chakrabarty, Rajan K.] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. [Chakrabarty, Rajan K.; Beres, Nicholas D.; Moosmueller, Hans] Nevada Syst Higher Educ, Desert Res Inst, Reno, NV USA. [China, Swarup; Mazzoleni, Claudio] Michigan Technol Univ, Atmospher Sci Program, Houghton, MI 49931 USA. [Dubey, Manvendra K.] Los Alamos Natl Lab, Earth Syst Observat, Los Alamos, NM USA. [Liu, Li; Mishchenko, Michael I.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. RP Chakrabarty, RK (reprint author), Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. EM rajan.chakrabarty@gmail.com RI Dubey, Manvendra/E-3949-2010; Mishchenko, Michael/D-4426-2012; OI Dubey, Manvendra/0000-0002-3492-790X; Moosmuller, Hans/0000-0002-1021-8877 FU NASA [NNX10AR89A, NNX11AB79G, NNX12AN97H]; U.S. Department of Energy Atmospheric System Research(PI-MKD) [DE-SC0010019, F265-LANL]; Desert Research Institute; U. S. National Science Foundation Division of Atmospheric and Geospace Sciences [ATM07-21142] FX This material is based upon work supported by NASA (NNX10AR89A, NNX11AB79G and NNX12AN97H), the U.S. Department of Energy Atmospheric System Research (DE-SC0010019 and F265-LANL(PI-MKD)), the U. S. National Science Foundation Division of Atmospheric and Geospace Sciences (ATM07-21142), and the Desert Research Institute. We thank V. Ramanathan for facilitating our participation in the field campaign at Maldives; K. Gorkowski for his help with sampling aerosols during CARES and the Las Conchas fire; O. Gustafsson for providing quartz fiber filter samples; B. Zielinska and her laboratory for performing mass spectrometry analyses of quartz fiber filters; M. Ahmadian for assisting with microscopy analysis; L. Wable for illustrations; R. Kreidberg for help with editing the manuscript; and C. M. Sorensen for insightful discussions. NR 56 TC 24 Z9 24 U1 3 U2 54 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 1 PY 2014 VL 4 AR 5508 DI 10.1038/srep05508 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK4UR UT WOS:000338420100005 PM 24981204 ER PT J AU MacCarthy, JK Rowe, CA AF MacCarthy, Jonathan K. Rowe, Charlotte A. TI Pisces: A Practical Seismological Database Library in Python SO SEISMOLOGICAL RESEARCH LETTERS LA English DT Editorial Material ID MANAGEMENT; OBSPY; TOOL C1 [MacCarthy, Jonathan K.; Rowe, Charlotte A.] Los Alamos Natl Lab, Geophys Grp EES 17, Los Alamos, NM 87545 USA. RP MacCarthy, JK (reprint author), Los Alamos Natl Lab, Geophys Grp EES 17, MS DF665, Los Alamos, NM 87545 USA. EM jkmacc@lanl.gov OI Rowe, Charlotte/0000-0001-5803-0147 NR 23 TC 0 Z9 0 U1 0 U2 3 PU SEISMOLOGICAL SOC AMER PI ALBANY PA 400 EVELYN AVE, SUITE 201, ALBANY, CA 94706-1375 USA SN 0895-0695 J9 SEISMOL RES LETT JI Seismol. Res. Lett. PD JUL-AUG PY 2014 VL 85 IS 4 BP 905 EP 911 DI 10.1785/0220140013 PG 7 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AK1NO UT WOS:000338182000017 ER PT J AU Ray, D Reichhardt, C Reichhardt, CJO AF Ray, D. Reichhardt, C. Reichhardt, C. J. Olson TI Vortex states in Archimedean tiling pinning arrays SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE periodic pinning; magnetization; vortex configurations ID SUPERCONDUCTING FILMS; CRITICAL CURRENTS; REGULAR ARRAY; MAGNETIC DOTS; FLUX; LATTICE; COMMENSURATE; DYNAMICS; DEFECTS AB We numerically study vortex ordering and pinning in Archimedean tiling substrates composed of square and triangular plaquettes. The two different plaquettes become occupied at different vortex densities, producing commensurate peaks in the magnetization at non-integer matching fields. We find that as the field increases, in some cases the fraction of occupied pins can decrease due to the competition between fillings of the different plaquette types. We also identify a number of different types of vortex orderings as a function of the field at integer and non-integer commensurate fillings. C1 [Ray, D.; Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ray, D.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. RP Ray, D (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of the US DoE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the US DoE at LANL under contract no. DE-AC52-06NA25396. NR 37 TC 4 Z9 4 U1 1 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD JUL PY 2014 VL 27 IS 7 AR 075006 DI 10.1088/0953-2048/27/7/075006 PG 9 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AK6KL UT WOS:000338536400009 ER PT J AU Susner, MA Sumption, MD Takase, A Collings, EW AF Susner, M. A. Sumption, M. D. Takase, A. Collings, E. W. TI Evidence for Zr site-substitution for Mg in PLD-deposited MgB2 thin films SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE magnesium diboride; pulsed laser deposition; thin films; superconducting critical fields ID CRITICAL-CURRENT DENSITY; UPPER CRITICAL-FIELD; IRREVERSIBILITY FIELD; SINGLE-CRYSTALS; SUPERCONDUCTIVITY; TRANSITION; NA AB In an investigation of possible atomic substitution for the Mg site in MgB2, superconducting thin films were deposited by pulsed laser deposition using MgB2 and ZrB2 targets. The resulting c-axis- oriented thin films contained various concentrations of Zr. The structural, chemical, and superconductive properties of these films were investigated. ZrB2 additions were found to increase the a lattice parameter; STEM-based chemical analysis showed Zr to be present within the grains. The superconducting critical temperature was suppressed for the heavily-doped samples. These observations are strong evidence for the substitution of Zr for Mg in the Mg sublattice of MgB2. C1 [Susner, M. A.; Sumption, M. D.; Collings, E. W.] Ohio State Univ, Dept Mat Sci & Engn, Ctr Superconducting & Magnet Mat, Columbus, OH 43210 USA. [Takase, A.] Rigaku Amer, The Woodlands, TX 77381 USA. RP Susner, MA (reprint author), ORNL, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Susner, Michael/G-3275-2015; Susner, Michael/B-1666-2013; Sumption, Mike/N-5913-2016 OI Susner, Michael/0000-0002-1211-8749; Susner, Michael/0000-0002-1211-8749; Sumption, Mike/0000-0002-4243-8380 FU United States Department of Energy, Office of High Energy Physics [DE-FG02-95ER40900]; National Science Foundation Cooperative Agreement [DMR-0654118]; State of Florida; US Department of Energy; Ohio State University NanoSystems Laboratory and Denis Pelekhov FX This work was supported by the United States Department of Energy, Office of High Energy Physics under grant DE-FG02-95ER40900. Additionally, a portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement no. DMR-0654118, the State of Florida, and the US Department of Energy. We also acknowledge the support of the Ohio State University NanoSystems Laboratory and Denis Pelekhov for use of their PPMS. Finally, the authors of this work would like to acknowledge Hendrik O Colijn and Daniel E Huber of the Ohio State CEOF/CEMAS facility for their assistance in electron microscopy characterization and training. NR 28 TC 1 Z9 1 U1 3 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD JUL PY 2014 VL 27 IS 7 AR 075009 DI 10.1088/0953-2048/27/7/075009 PG 7 WC Physics, Applied; Physics, Condensed Matter SC Physics GA AK6KL UT WOS:000338536400012 ER PT J AU Takahashi, M Herendeen, PS Xiao, XH Crane, PR AF Takahashi, Masamichi Herendeen, Patrick S. Xiao, Xianghui Crane, Peter R. TI Lauraceous Fossil Flowers from the Kamikitaba Assemblage (Coniacian, Late Cretaceous) of Northeastern Japan (Lauraceae) SO SYSTEMATIC BOTANY LA English DT Article DE Cretaceous; mesofossils; Microlaterus; SRXTM; Synchrotron-radiation X-Ray microtomography ID EASTERN NORTH-AMERICA; SP-NOV; POTOMAC GROUP; ANGIOSPERM RADIATION; FLORAL EVIDENCE; PHYLOGENY; GEN.; INFLORESCENCES; DIVERSITY; SEQUENCES AB A new genus and species of Lauraceae, Microlaurus perigynus gen. et sp. nov. is described based on fossil charcoalified flower buds recovered from the Kamikitaba assemblage (early Coniacian, Late Cretaceous; ca. 89 million years before present (myr BP)) in the Ashizawa Formation (Asamigawa Member) of the Futaba Group in northeastern Japan. Analysis of the internal structure of the fossil buds using synchrotron-radiation X-ray microtomography (SRXTM) at the 2-BM-B beamline of the Advanced Photon Source (APS), Argonne National Laboratory, shows that the flowers are small, pedicellate, bisexual, trimerous, and actinomorphic, with small outer tepals, larger inner tepals, three whorls of stamens, an innermost androecial whorl composed of staminodia, and a unicarpellate gynoecium containing a single ovule. Microlaurus perigynus is assigned to the Lauraceae based on the regular trimerous floral organization and other details of floral structure, but it is distinguished from most previously described lauraceous fossil flowers by the poorly differentiated filament and anther in the stamens of the third whorl and the marked size difference between the small outer tepals and the large inner tepals. Also unusual are the paired glandular appendages that appear to be associated with the first (outermost) whorl of stamens, rather than the stamens of the third whorl, although the precise position is not fully clear. The same feature occurs in Hernandiaceae, the sister group of Lauraceae, as well as in PowhaMnia connata, an earlier but fragmentary lauralean fossil flower from the Early to Middle Albian of Virginia. Microlaurus perigynus adds to the floral diversity of Lauraceae known from the Late Cretaceous, and its presence in the Kamikitaba assemblage from Japan underlines the broad geographic distribution and floristic significance of lauraceous plants during the Late Cretaceous. C1 [Takahashi, Masamichi] Niigata Univ, Fac Sci, Dept Environm Sci, Nishi Ku, Niigata 9502181, Japan. [Herendeen, Patrick S.] Chicago Bot Garden, Glencoe, IL 60022 USA. [Xiao, Xianghui] Adv Photon Source, Argonne, IL 60439 USA. [Crane, Peter R.] Yale Univ, Sch Forestry & Environm Studies, New Haven, CT 06511 USA. RP Takahashi, M (reprint author), Niigata Univ, Fac Sci, Dept Environm Sci, Nishi Ku, Niigata 9502181, Japan. EM masamichi@env.sc.niigata-u.ac.jp FU Japan Society for the Promotion of Science [18570083, 21570092, 24570092]; U.S. DOE [DE-AC02-06CH11357] FX We thank Drs. Hank van der Werff and Jens Rohwer for comments on the fossils and comparisons with extant Lauraceae, and two anonymous reviewers for helpful comments on the manuscript. The study was funded by Grants-in-Aid for Scientific Research (18570083, 21570092, and 24570092) from Japan Society for the Promotion of Science to M. Takahashi. Use of the Advanced Photon Source, an Office of Science User Facility, operated for the U. S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract no. DE-AC02-06CH11357. NR 57 TC 4 Z9 4 U1 4 U2 17 PU AMER SOC PLANT TAXONOMISTS PI LARAMIE PA UNIV WYOMING, DEPT BOTANY 3165, 1000 E UNIVERSITY AVE, LARAMIE, WY 82071 USA SN 0363-6445 EI 1548-2324 J9 SYST BOT JI Syst. Bot. PD JUL-SEP PY 2014 VL 39 IS 3 BP 715 EP 724 DI 10.1600/036364414X681464 PG 10 WC Plant Sciences; Evolutionary Biology SC Plant Sciences; Evolutionary Biology GA AK4OY UT WOS:000338405200004 ER PT J AU Provino, A Manfrinetti, P Gschneidner, KA Dhar, SK Schlagel, DL Lograsso, TA Miller, GJ Thimmaiah, S Wang, H Russell, AM Becker, A Mudryk, Y AF Provino, Alessia Manfrinetti, Pietro Gschneidner, Karl A., Jr. Dhar, Sudesh K. Schlagel, Deborah L. Lograsso, Thomas A. Miller, Gordon J. Thimmaiah, Srinivasa Wang, Hui Russell, Alan M. Becker, Andrew Mudryk, Yaroslav TI Self-assembled nano- to micron-size fibers from molten R11Ni4In9 intemietallics SO ACTA MATERIALIA LA English DT Article DE Rare-earth intermetallics; Nanocrystalline metals; Fibers; Anisotropic properties; Ferrimagnetism AB A study of the formation of Gd11M4In9 (M = Ni, Pd, Pt) and R11Ni4In9 (R = rare earth) compounds revealed a unique and peculiar property, which is to naturally crystallize in a bundle of self-assembled fibers when cooled from the melt. The fibers, which are nano- to millimeters in cross-section and approximate to 11-40 mm long, grow unidirectionally along a temperature gradient. These compounds adopt the orthorhombic Nd11Pd4In9 structure type (oC48-Cmmm). This structure is layered, with slabs of R atoms alternating with slabs of Ni/In atoms along a short c-axis (much shorter than either the a- or b-axis). The growth direction of the fibers is along the crystallographic c-axis, orthogonal to the a-b plane. Two strong and short In In bonds lie in the a-b plane, which are even shorter than in In metal. Integrated crystal orbital Hamilton population calculations show that the In In bonds create isolated "R8Ni4In9" rods growing along the c-axis, with the In In bonds being part of the rods. This appears to be an important factor explaining the microfibrous nature of these phases. Some physical properties have been measured on the Gd11Ni4In9 homolog. The compound orders ferrimagnetically at T-c approximate to 88 K, and at lower temperatures (46 and 10 K), two other magnetic anomalies were observed, probably due to spin reorientations. As expected from the bonding features, the mechanical, magnetic and electrical properties are strongly anisotropic. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Provino, Alessia; Manfrinetti, Pietro] Univ Genoa, Dept Chem, I-16146 Genoa, Italy. [Provino, Alessia; Manfrinetti, Pietro; Gschneidner, Karl A., Jr.; Schlagel, Deborah L.; Lograsso, Thomas A.; Miller, Gordon J.; Thimmaiah, Srinivasa; Wang, Hui; Mudryk, Yaroslav] Iowa State Univ, Ames Lab, US Dept Energy, Ames, IA 50011 USA. [Gschneidner, Karl A., Jr.; Russell, Alan M.; Becker, Andrew] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Miller, Gordon J.; Wang, Hui] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Gschneidner, KA (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM cagey@ameslab.gov FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; [NSF-DMR 10-05765] FX The research carried out at the Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. A.P. is grateful to Prof. L. Banfi (Director of the PhD School in Sciences and Technologies of Chemistry and Materials, University of Genova, Italy) for support of a one-year fellowship abroad. A.P. and P.M. thank Mr. Roger Rink for technical support provided during measurements, and Mrs. Carol Smith for preparing the manuscript. Theoretical calculations (G.J.M. and H.W.) were supported by NSF-DMR 10-05765. The authors wish to thank Prof. M.E. Glicksman, Florida Institute of Technology for his useful comments. NR 24 TC 4 Z9 4 U1 2 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUL PY 2014 VL 73 BP 27 EP 36 DI 10.1016/j.actamat.2014.03.061 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AJ7BV UT WOS:000337853100004 ER PT J AU Senninger, O Martinez, E Soisson, F Nastar, M Brechet, Y AF Senninger, Oriane Martinez, Enrique Soisson, Frederic Nastar, Maylise Brechet, Yves TI Atomistic simulations of the decomposition kinetics in Fe-Cr alloys: Influence of magnetism SO ACTA MATERIALIA LA English DT Article DE Fe-Cr alloys; Precipitation kinetics; Monte Carlo simulations; Magnetic transitions; Diffusion ID SMALL-ANGLE SCATTERING; SPINODAL DECOMPOSITION; ALPHA-IRON; DIFFUSION; CHROMIUM; MOSSBAUER; SYSTEM AB Magnetism plays a crucial role in the thermodynamic and kinetic properties of ferritic alloys. In fact, magnetism increases the solubility limit of Cr in Fe, inducing an asymmetrical phase diagram. Moreover, the phase transition from ferromagnetic to paramagnetic (F/P) iron alloys modifies to a large extent the system response to different environmental conditions by modification of the alloy diffusion properties. Indeed, experimental tracer diffusion coefficients deviate from an Arrhenius law during the F/P magnetic transition, leading to a large increase in the paramagnetic regime compared to the extrapolated value from the ferromagnetic domain. Furthermore, as the Curie temperature decreases with the Cr concentration, this evolution of the diffusion properties affects the decomposition kinetics in different ways depending on the alloy composition. An atomic diffusion model, with pair interactions that depend on the local composition and on temperature, has been developed to take into account this magnetic transition effect. The interaction model has been implemented in an atomistic kinetic Monte Carlo algorithm to study the diffusion coefficients and precipitation kinetics of the Fe Cr alloys. This model has been successfully compared to decomposition kinetic experiments for a wide range of concentrations and temperatures. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Senninger, Oriane; Soisson, Frederic; Nastar, Maylise] CEA, DEN, Serv Rech Met Phys, F-91191 Gif Sur Yvette, France. [Martinez, Enrique] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Brechet, Yves] CNRS UJF, INP Grenoble, SIMAP, St Martin Dheres, France. RP Soisson, F (reprint author), CEA, DEN, Serv Rech Met Phys, F-91191 Gif Sur Yvette, France. EM frederic.soisson@cea.fr OI Martinez Saez, Enrique/0000-0002-2690-2622 FU European fusion materials modeling program; European Atomic Energy Community 7th Framework Program [212175]; US Department of Energy through the LANL/LDRD Program FX We thank C.-C. Fu and E. Clouet for many fruitful discussions. This research has received partial funding from the European fusion materials modeling program and from the European Atomic Energy Community 7th Framework Program (FP7/2007-2011), under Grant Agreement No. 212175 (GetMat project). E.M. gratefully acknowledges the support of the US Department of Energy through the LANL/LDRD Program for this work. NR 46 TC 12 Z9 12 U1 2 U2 37 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUL PY 2014 VL 73 BP 97 EP 106 DI 10.1016/j.actamat.2014.03.019 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AJ7BV UT WOS:000337853100010 ER PT J AU Lee, SY Wang, H Gharghouri, MA Nayyeri, G Woo, W Shin, E Wu, PD Poole, WJ Wu, W An, K AF Lee, S. Y. Wang, H. Gharghouri, M. A. Nayyeri, G. Woo, W. Shin, E. Wu, P. D. Poole, W. J. Wu, W. An, K. TI Deformation behavior of solid-solution-strengthened Mg-9 wt.% Al alloy: In situ neutron diffraction and elastic-viscoplastic self-consistent modeling SO ACTA MATERIALIA LA English DT Article DE Magnesium; Deformation; In situ neutron diffraction; EVPSC model; Lattice strain ID WROUGHT MAGNESIUM ALLOY; TWINNING-DETWINNING BEHAVIOR; LATTICE STRAIN EVOLUTION; FINITE-ELEMENT-METHOD; MECHANICAL-BEHAVIOR; TEXTURE DEVELOPMENT; AZ31B SHEET; STRESS-RELAXATION; STAINLESS-STEEL; INTERNAL STRAIN AB In situ neutron diffraction and elastic-viscoplastic self-consistent (EVPSC) modeling have been employed to understand the deformation mechanisms of the loading-unloading process under uniaxial tension in a solid-solution-strengthened extruded Mg-9 wt.% Al alloy. The initial texture measured by neutron diffraction shows that the {00.2} basal planes in most grains are tilted around 20-30 from the extrusion axis, indicating that basal slip should be easily activated in a majority of grains under tension. Non-linear stress strain responses are observed during unloading and reloading after the material is fully plastically deformed under tension. In situ neutron diffraction measurements have also demonstrated the non-linear behavior of lattice strains during unloading and reloading, revealing that load redistribution continuously occurs between soft and hard grain orientations. The predicted macroscopic stress-strain curve and the lattice strain evolution by the EVPSC model are in good agreement with the experimental data. The EVPSC model provides the relative activities of the available slip and twinning modes, as well as the elastic and plastic strains of the various grain families. It is suggested that the non-linear phenomena in the macroscopic stress-strain responses and microscopic lattice strains during unloading and reloading are due to plastic deformation by the operation of basal (a) slip in the soft grain orientations (e.g. {10.1}, {11.2} and {10.2} grain families). (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Lee, S. Y.] Chungnam Natl Univ, Dept Mat Sci & Engn, Taejon 305764, South Korea. [Wang, H.; Wu, P. D.] McMaster Univ, Dept Mech Engn, Hamilton, ON L8S 4L7, Canada. [Gharghouri, M. A.] AECL Res, Chalk River Labs, Canadian Neutron Beam Ctr, Chalk River, ON K0J 1J0, Canada. [Nayyeri, G.; Poole, W. J.] Univ British Columbia, Dept Mat Engn, Vancouver, BC V6T 1Z4, Canada. [Woo, W.; Shin, E.] Korea Atom Energy Res Inst, Div Neutron Sci, Taejon 305353, South Korea. [Wu, W.; An, K.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Lee, SY (reprint author), Chungnam Natl Univ, Dept Mat Sci & Engn, Taejon 305764, South Korea. EM sylee2012@cnu.ac.kr RI An, Ke/G-5226-2011; Wang, Huamiao/F-7693-2010; Wu, Wei/G-3204-2014; Wu, Peidong/A-7009-2008; OI An, Ke/0000-0002-6093-429X; Wang, Huamiao/0000-0002-7167-2483; Wu, Wei/0000-0002-8596-9253; WOO, Wanchuck/0000-0003-0350-5357 FU National Research Foundation of Korea (NRF) - Korean government (MSIP) [2012M2B2A4029572, 2013R1A4A1069528]; NSERC Magnesium Strategic Research Network (MagNET); Chungnam National University; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the National Research Foundation of Korea (NRF) Grant funded by the Korean government (MSIP) (Nos. 2012M2B2A4029572 and 2013R1A4A1069528). This work was also supported by funding from the NSERC Magnesium Strategic Research Network (MagNET) and the Chungnam National University. This research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 69 TC 24 Z9 24 U1 4 U2 38 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUL PY 2014 VL 73 BP 139 EP 148 DI 10.1016/j.actamat.2014.03.038 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AJ7BV UT WOS:000337853100014 ER PT J AU Hunter, SD Bloser, PF Depaola, GO Dion, MP DeNolfo, GA Hanu, A Iparraguirre, M Legere, J Longo, F McConnell, ML Nowicki, SF Ryan, JM Son, S Stecker, FW AF Hunter, Stanley D. Bloser, Peter F. Depaola, Gerardo O. Dion, Michael P. DeNolfo, Georgia A. Hanu, Andrei Iparraguirre, Marcos Legere, Jason Longo, Francesco McConnell, Mark L. Nowicki, Suzanne F. Ryan, James M. Son, Seunghee Stecker, Floyd W. TI A pair production telescope for medium-energy gamma-ray polarimetry SO ASTROPARTICLE PHYSICS LA English DT Article DE Gamma rays; Pair production; Angular resolution; Polarimetry; Sensitivity; Time projection chamber ID DOUBLE RADIO-SOURCES; CARBON-DISULFIDE; LONGITUDINAL DIFFUSION; PROPORTIONAL-COUNTERS; MULTIPLE-SCATTERING; LINEAR-POLARIZATION; EGRET OBSERVATIONS; CRAB PULSAR; DETECTORS; EMISSION AB We describe the science motivation and development of a pair production telescope for medium-energy (similar to 5-200 MeV) gamma-ray polarimetry. Our instrument concept, the Advanced Energetic Pair Telescope (AdEPT), takes advantage of the Three-Dimensional Track Imager, a low-density gaseous time projection chamber, to achieve angular resolution within a factor of two of the pair production kinematics limit (similar to 0.6 degrees at 70 MeV), continuum sensitivity comparable with the Fermi-LAT front detector (<3 x 10(-6) MeV cm(-2) s(-1) 70 MeV), and minimum detectable polarization less than 10% for a 10 mCrab source in 10(6) s. Published by Elsevier B.V. C1 [Hunter, Stanley D.; DeNolfo, Georgia A.; Hanu, Andrei; Nowicki, Suzanne F.; Son, Seunghee; Stecker, Floyd W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Bloser, Peter F.; Legere, Jason; McConnell, Mark L.; Ryan, James M.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Depaola, Gerardo O.; Iparraguirre, Marcos] Univ Cordoba, Fac Matemat Astron & Fis, RA-5008 Cordoba, Argentina. [Dion, Michael P.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Longo, Francesco] Univ Trieste, Dipartimento Fis, Treste, Italy. [Nowicki, Suzanne F.; Son, Seunghee] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. RP Hunter, SD (reprint author), NASA, Goddard Space Flight Ctr, Code 661, Greenbelt, MD 20771 USA. EM stanley.d.hunter@nasa.gov OI Dion, Michael/0000-0002-3030-0050 NR 89 TC 12 Z9 12 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD JUL-AUG PY 2014 VL 59 BP 18 EP 28 DI 10.1016/j.astropartphys.2014.04.002 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AJ7MT UT WOS:000337881500004 ER PT J AU Ajello, M Albert, A Allafort, A Baldini, L Barbiellini, G Bastieri, D Bellazzini, R Bissaldi, E Bonamente, E Brandt, TJ Bregeon, J Brigida, M Bruel, P Buehler, R Buson, S Caliandro, GA Cameron, RA Caraveo, PA Cecchi, C Charles, E Chekhtman, A Chiang, J Chiaro, G Ciprini, S Claus, R Cohen-Tanugi, J Cominsky, LR Conrad, J Cutini, S D'Ammando, F de Palma, F Dermer, CD Desiante, R Digel, SW Silva, EDE Drell, PS Drlica-Wagner, A Favuzzi, C Focke, WB Franckowiak, A Fukazawa, Y Fusco, P Gargano, F Gasparrini, D Germani, S Giglietto, N Giommi, P Giordano, F Giroletti, M Glanzman, T Godfrey, G Grenier, IA Grove, JE Guiriec, S Hadasch, D Hayashida, M Hays, E Horan, D Hou, X Hughes, RE Inoue, Y Jackson, MS Jogler, T Johannesson, G Johnson, AS Johnson, WN Kamae, T Knodlseder, J Kocevski, D Kuss, M Lande, J Larsson, S Latronico, L Longo, F Loparco, F Lott, B Lovellette, MN Lubrano, P Mayer, M Mazziotta, MN McEnery, JE Michelson, PF Mizuno, T Moiseev, AA Monte, C Monzani, ME Morselli, A Moskalenko, IV Murgia, S Murphy, R Nakamori, T Nemmen, R Nuss, E Ohno, M Ohsugi, T Omodei, N Orienti, M Orlando, E Ormes, JF Paneque, D Panetta, JH Perkins, JS Pesce-Rollins, M Petrosian, V Piron, F Pivato, G Porter, TA Raino, S Rando, R Razzano, M Reimer, A Reimer, O Roth, M Schulz, A Sgro, C Siskind, EJ Spandre, G Spinelli, P Takahashi, H Thayer, JG Thayer, JB Thompson, DJ Tibaldo, L Tinivella, M Tosti, G Troja, E Usher, TL Vandenbroucke, J Vasileiou, V Vianello, G Vitale, V Werner, M Winer, BL Wood, DL Wood, KS Yang, Z AF Ajello, M. Albert, A. Allafort, A. Baldini, L. Barbiellini, G. Bastieri, D. Bellazzini, R. Bissaldi, E. Bonamente, E. Brandt, T. J. Bregeon, J. Brigida, M. Bruel, P. Buehler, R. Buson, S. Caliandro, G. A. Cameron, R. A. Caraveo, P. A. Cecchi, C. Charles, E. Chekhtman, A. Chiang, J. Chiaro, G. Ciprini, S. Claus, R. Cohen-Tanugi, J. Cominsky, L. R. Conrad, J. Cutini, S. D'Ammando, F. de Palma, F. Dermer, C. D. Desiante, R. Digel, S. W. do Couto e Silva, E. Drell, P. S. Drlica-Wagner, A. Favuzzi, C. Focke, W. B. Franckowiak, A. Fukazawa, Y. Fusco, P. Gargano, F. Gasparrini, D. Germani, S. Giglietto, N. Giommi, P. Giordano, F. Giroletti, M. Glanzman, T. Godfrey, G. Grenier, I. A. Grove, J. E. Guiriec, S. Hadasch, D. Hayashida, M. Hays, E. Horan, D. Hou, X. Hughes, R. E. Inoue, Y. Jackson, M. S. Jogler, T. Johannesson, G. Johnson, A. S. Johnson, W. N. Kamae, T. Knoedlseder, J. Kocevski, D. Kuss, M. Lande, J. Larsson, S. Latronico, L. Longo, F. Loparco, F. Lott, B. Lovellette, M. N. Lubrano, P. Mayer, M. Mazziotta, M. N. McEnery, J. E. Michelson, P. F. Mizuno, T. Moiseev, A. A. Monte, C. Monzani, M. E. Morselli, A. Moskalenko, I. V. Murgia, S. Murphy, R. Nakamori, T. Nemmen, R. Nuss, E. Ohno, M. Ohsugi, T. Omodei, N. Orienti, M. Orlando, E. Ormes, J. F. Paneque, D. Panetta, J. H. Perkins, J. S. Pesce-Rollins, M. Petrosian, V. Piron, F. Pivato, G. Porter, T. A. Raino, S. Rando, R. Razzano, M. Reimer, A. Reimer, O. Roth, M. Schulz, A. Sgro, C. Siskind, E. J. Spandre, G. Spinelli, P. Takahashi, H. Thayer, J. G. Thayer, J. B. Thompson, D. J. Tibaldo, L. Tinivella, M. Tosti, G. Troja, E. Usher, T. L. Vandenbroucke, J. Vasileiou, V. Vianello, G. Vitale, V. Werner, M. Winer, B. L. Wood, D. L. Wood, K. S. Yang, Z. TI IMPULSIVE AND LONG DURATION HIGH-ENERGY GAMMA-RAY EMISSION FROM THE VERY BRIGHT 2012 MARCH 7 SOLAR FLARES SO ASTROPHYSICAL JOURNAL LA English DT Article DE Sun: flares; Sun: X-rays, gamma rays ID LARGE-AREA TELESCOPE; STOCHASTIC ACCELERATION; X-RAY; VELA PULSAR; ELECTRON ACCELERATION; EGRET; CALIBRATION; PARTICLES; COMPTON; DIRECTIVITY AB The Fermi Large Area Telescope (LAT) detected gamma-rays up to 4 GeV from two bright X-class solar flares on 2012 March 7, showing both an impulsive and temporally extended emission phases. The gamma-rays appear to originate from the same active region as the X-rays associated with these flares. The >100 MeV gamma-ray flux decreases monotonically during the first hour (impulsive phase) followed by a slower decrease for the next 20 hr. A power law with a high-energy exponential cutoff can adequately describe the photon spectrum. Assuming that the gamma rays result from the decay of pions produced by accelerated protons and ions with a power-law spectrum, we find that the index of that spectrum is similar to 3, with minor variations during the impulsive phase. During the extended phase the photon spectrum softens monotonically, requiring the proton index varying from similar to 4 to >5. The >30 MeV proton flux observed by the GOES satellites also shows a flux decrease and spectral softening, but with a harder spectrum (index similar to 2-3). Based on these observations, we explore the relative merits of prompt or continuous acceleration scenarios, hadronic or leptonic emission processes, and acceleration at the solar corona or by the fast coronal mass ejections. We conclude that the most likely scenario is continuous acceleration of protons in the solar corona that penetrate the lower solar atmosphere and produce pions that decay into gamma rays. However, acceleration in the downstream of the shock cannot be definitely ruled out. C1 [Ajello, M.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Albert, A.; Allafort, A.; Caliandro, G. A.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Digel, S. W.; do Couto e Silva, E.; Drell, P. S.; Focke, W. B.; Franckowiak, A.; Glanzman, T.; Godfrey, G.; Inoue, Y.; Jogler, T.; Johnson, A. S.; Kamae, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Moskalenko, I. V.; Omodei, N.; Orlando, E.; Paneque, D.; Panetta, J. H.; Petrosian, V.; Porter, T. A.; Reimer, A.; Reimer, O.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Albert, A.; Allafort, A.; Caliandro, G. A.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Digel, S. W.; do Couto e Silva, E.; Drell, P. S.; Focke, W. B.; Franckowiak, A.; Glanzman, T.; Godfrey, G.; Inoue, Y.; Jogler, T.; Johnson, A. S.; Kamae, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Moskalenko, I. V.; Omodei, N.; Orlando, E.; Paneque, D.; Panetta, J. H.; Petrosian, V.; Porter, T. A.; Reimer, A.; Reimer, O.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Baldini, L.] Univ Pisa, I-56127 Pisa, Italy. [Baldini, L.; Bellazzini, R.; Bregeon, J.; Kuss, M.; Pesce-Rollins, M.; Razzano, M.; Sgro, C.; Spandre, G.; Tinivella, M.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Barbiellini, G.; Bissaldi, E.; Desiante, R.; Longo, F.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Barbiellini, G.; Longo, F.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Bastieri, D.; Buson, S.; Rando, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bastieri, D.; Buson, S.; Chiaro, G.; Pivato, G.; Rando, R.] Univ Padua, Dipartimento Fis & Astron G Galilei, I-35131 Padua, Italy. [Bissaldi, E.] Univ Trieste, I-34127 Trieste, Italy. [Bonamente, E.; Cecchi, C.; Germani, S.; Lubrano, P.; Tosti, G.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Bonamente, E.; Cecchi, C.; Germani, S.; Lubrano, P.; Tosti, G.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Brandt, T. J.; Guiriec, S.; Hays, E.; McEnery, J. E.; Moiseev, A. A.; Nemmen, R.; Perkins, J. S.; Thompson, D. J.; Troja, E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Monte, C.; Raino, S.; Spinelli, P.] Univ Bari, Dipartimento Fis M Merlin, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Monte, C.; Raino, S.; Spinelli, P.] Politecn Bari, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Gargano, F.; Giglietto, N.; Giordano, F.; Loparco, F.; Mazziotta, M. N.; Monte, C.; Raino, S.; Spinelli, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Bruel, P.; Horan, D.] Ecole Polytech, CNRS IN2P3, Lab Leprince Ringuet, Palaiseau, France. [Buehler, R.; Mayer, M.; Schulz, A.] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Caraveo, P. A.] INAF Ist Astrofis Spaziale & Fis Cosm, I-20133 Milan, Italy. [Chekhtman, A.] George Mason Univ, Coll Sci, Ctr Earth Observing & Space Res, Fairfax, VA 22030 USA. [Ciprini, S.; Cutini, S.; Gasparrini, D.; Giommi, P.] Agenzia Spaziale Italiana ASI Sci Data Ctr, I-00044 Frascati, Roma, Italy. [Ciprini, S.; Cutini, S.; Gasparrini, D.] Ist Nazl Astrofis Osservatorio Astron Roma, I-00040 Rome, Italy. [Cohen-Tanugi, J.; Nuss, E.; Piron, F.; Vasileiou, V.] Univ Montpellier 2, CNRS IN2P3, Lab Univers & Particules Montpellier, Montpellier, France. [Cominsky, L. R.] Sonoma State Univ, Dept Phys & Astron, Rohnert Pk, CA 94928 USA. [Conrad, J.; Larsson, S.; Yang, Z.] Stockholm Univ, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Conrad, J.; Jackson, M. S.; Larsson, S.; Yang, Z.] Oskar Klein Ctr Cosmoparticle Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Conrad, J.] Royal Swedish Acad Sci, SE-10405 Stockholm, Sweden. [D'Ammando, F.; Giroletti, M.; Orienti, M.] INAF Ist Radioastron, I-40129 Bologna, Italy. [Dermer, C. D.; Grove, J. E.; Johnson, W. N.; Lovellette, M. N.; Murphy, R.; Wood, K. S.] Naval Res Lab, Div Space Sci, Washington, DC 20375 USA. [Drlica-Wagner, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Fukazawa, Y.; Ohno, M.; Takahashi, H.] Hiroshima Univ, Dept Phys Sci, Hiroshima 7398526, Japan. [Grenier, I. A.] CEA IRFU CNRS Univ Paris Diderot, CEA Saclay, Serv Astrophys, Lab AIM, F-91191 Gif Sur Yvette, France. [Hadasch, D.; Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Hadasch, D.; Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Theoret Phys, A-6020 Innsbruck, Austria. [Hayashida, M.] Univ Tokyo, Inst Cosm Ray Res, Kashiwa, Chiba 2778582, Japan. [Hou, X.; Lott, B.] Univ Bordeaux 1, CNRS IN2P3, Ctr Etud Nucl Bordeaux Gradignan, F-33175 Gradignan, France. [Hughes, R. E.; Winer, B. L.] Ohio State Univ, Dept Phys, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Jackson, M. S.] Royal Inst Technol KTH, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Johannesson, G.] Univ Iceland, Inst Sci, IS-107 Reykjavik, Iceland. [Knoedlseder, J.] CNRS, IRAP, F-31028 Toulouse 4, France. [Knoedlseder, J.] Univ Toulouse, UPS OMP, IRAP, GAHEC, Toulouse, France. [Larsson, S.] Stockholm Univ, Dept Astron, SE-10691 Stockholm, Sweden. [Latronico, L.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [McEnery, J. E.; Moiseev, A. A.; Troja, E.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [McEnery, J. E.; Moiseev, A. A.; Troja, E.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Mizuno, T.; Ohsugi, T.] Hiroshima Univ, Hiroshima Astrophys Sci Ctr, Hiroshima 7398526, Japan. [Moiseev, A. A.] CRESST, Greenbelt, MD 20771 USA. [Morselli, A.; Vitale, V.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Murgia, S.] Univ Calif Irvine, Dept Phys & Astron, Ctr Cosmol, Irvine, CA 92697 USA. [Ormes, J. F.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Paneque, D.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Roth, M.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Siskind, E. J.] NYCB Real Time Comp Inc, Lattingtown, NY 11560 USA. [Vianello, G.] CIFS, I-10133 Turin, Italy. [Vitale, V.] Univ Roma Tor Vergata, Dipartimento Fis, I-00133 Rome, Italy. [Wood, D. L.] Praxis Inc, Alexandria, VA 22303 USA. RP Ajello, M (reprint author), Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA. EM nicola.omodei@stanford.edu; melissa.pesce.rollins@pi.infn.it; vahep@stanford.edu RI Bissaldi, Elisabetta/K-7911-2016; Reimer, Olaf/A-3117-2013; Morselli, Aldo/G-6769-2011; Nemmen, Rodrigo/O-6841-2014; Johannesson, Gudlaugur/O-8741-2015; Loparco, Francesco/O-8847-2015; Orlando, E/R-5594-2016; Mazziotta, Mario /O-8867-2015; Gargano, Fabio/O-8934-2015; giglietto, nicola/I-8951-2012; Moskalenko, Igor/A-1301-2007; Sgro, Carmelo/K-3395-2016 OI giommi, paolo/0000-0002-2265-5003; Caraveo, Patrizia/0000-0003-2478-8018; Sgro', Carmelo/0000-0001-5676-6214; SPINELLI, Paolo/0000-0001-6688-8864; Rando, Riccardo/0000-0001-6992-818X; Inoue, Yoshiyuki/0000-0002-7272-1136; Bastieri, Denis/0000-0002-6954-8862; Pesce-Rollins, Melissa/0000-0003-1790-8018; orienti, monica/0000-0003-4470-7094; Giroletti, Marcello/0000-0002-8657-8852; Gasparrini, Dario/0000-0002-5064-9495; Baldini, Luca/0000-0002-9785-7726; Larsson, Stefan/0000-0003-0716-107X; Bissaldi, Elisabetta/0000-0001-9935-8106; Reimer, Olaf/0000-0001-6953-1385; Morselli, Aldo/0000-0002-7704-9553; Johannesson, Gudlaugur/0000-0003-1458-7036; Loparco, Francesco/0000-0002-1173-5673; Giordano, Francesco/0000-0002-8651-2394; Mazziotta, Mario /0000-0001-9325-4672; Gargano, Fabio/0000-0002-5055-6395; giglietto, nicola/0000-0002-9021-2888; Moskalenko, Igor/0000-0001-6141-458X; NR 56 TC 25 Z9 25 U1 1 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2014 VL 789 IS 1 AR 20 DI 10.1088/0004-637X/789/1/20 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK0LD UT WOS:000338103400020 ER PT J AU Firestone, RB AF Firestone, R. B. TI OBSERVATION OF 23 SUPERNOVAE THAT EXPLODED <300 pc FROM EARTH DURING THE PAST 300 kyr SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic rays; Earth; ISM: supernova remnants; supernovae: general ID RADIOCARBON AGE CALIBRATION; NEARBY OB ASSOCIATIONS; VELA SUPERNOVA; COSMIC-RAYS; CLIMATE-CHANGE; CARBON-CYCLE; GAMMA-RAYS; HALF-LIFE; ICE CORE; REMNANTS AB Four supernovae (SNe), exploding <= 300 pc from Earth, were recorded 44, 37, 32, and 22 kyr ago in the radiocarbon (C-14) record during the past 50 kyr. Each SN left a nearly identical signature in the record, beginning with an initial sudden increase in atmospheric radiocarbon, when the SN exploded, followed by a hiatus of 1500 yr, and concluding with a sustained 2000 yr increase in global radiocarbon due to gamma-rays produced by diffusive shock in the SN remnant (SNR). For the past 18 kyr excess radiocarbon has decayed with the C-14 half-life. SN22kyrBP, is identified as the Vela SN that exploded 250 +/- 30 pc from Earth. These SN are confirmed in the Be-10, Al-26, Cl-36, and NO3- geologic records. The rate of near-Earth SNe is consistent with the observed rate of historical SNe giving a galactic rate of 14 +/- 3 kyr(-1) assuming the Chandra Galactic Catalog SNR distribution. The Earth has been used as a calorimeter to determine that approximate to 2 x 10(49) erg were released as gamma-rays at the time of each SN explosion and approximate to 10(50) erg in gamma-rays following each SN. The background rate of C-14 production by cosmic rays has been determined as 1.61 atoms cm(-2) s(-1). Approximately 1/3 of the cosmic ray energy produced by diffusive shock in the SNR was observed to be emitted as high-energy gamma-rays. Analysis of the Be-10/Be-9 ratio in marine sediment identified 19 additional near-Earth SNe that exploded 50-300 kyr ago. Comparison of the radiocarbon record with global temperature variations indicated that each SN explosion is correlated with a concurrent global warming of approximate to 3 degrees C-4 degrees C. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Firestone, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM rbfirestone@lbl.gov FU U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported, in part, by the U.S. Department of Energy Contract DE-AC02-05CH11231. The author is especially grateful for helpful discussions and suggestions by Allen West (Geoscience Consulting, Dewey, AZ), Jon Hagstrum (USGS, Menlo Park, CA), Spencer Klein (LBNL, Berkeley, CA), Christopher McKee (University of California, Berkeley, Department of Physics), and Mary Firestone (University of California, Berkeley, Department of Environmental Science Policy and Management. NR 65 TC 5 Z9 5 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2014 VL 789 IS 1 AR 29 DI 10.1088/0004-637X/789/1/29 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK0LD UT WOS:000338103400029 ER PT J AU Nynka, M Hailey, CJ Reynolds, SP An, HJ Baganoff, FK Boggs, SE Christensen, FE Craig, WW Gotthelf, EV Grefenstette, BW Harrison, FA Krivonos, R Madsen, KK Mori, K Perez, K Stern, D Wik, DR Zhang, WW Zoglauer, A AF Nynka, Melania Hailey, Charles J. Reynolds, Stephen P. An, Hongjun Baganoff, Frederick K. Boggs, Steven E. Christensen, Finn E. Craig, William W. Gotthelf, Eric V. Grefenstette, Brian W. Harrison, Fiona A. Krivonos, Roman Madsen, Kristin K. Mori, Kaya Perez, Kerstin Stern, Daniel Wik, Daniel R. Zhang, William W. Zoglauer, Andreas TI NuSTAR STUDY OF HARD X-RAY MORPHOLOGY AND SPECTROSCOPY OF PWN G21.5-0.9 SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: individual objects (G21.5-0.9); ISM: supernova remnants; radiation mechanisms: general; stars: neutron; X-rays: ISM ID SUPERNOVA REMNANT G21.5-0.9; PULSAR-WIND NEBULAE; XMM-NEWTON; CRAB-NEBULA; RELATIVISTIC ELECTRONS; INTERSTELLAR-MEDIUM; DUST SCATTERING; PSR J1833-1034; YOUNG PULSAR; HALO AB We present NuSTAR high-energy X-ray observations of the pulsar wind nebula (PWN)/supernova remnant G21.5-0.9. We detect integrated emission from the nebula up to similar to 40 keV, and resolve individual spatial features over a broad X-ray band for the first time. The morphology seen by NuSTAR agrees well with that seen by XMM-Newton and Chandra below 10 keV. At high energies, NuSTAR clearly detects non-thermal emission up to similar to 20 keV that extends along the eastern and northern rim of the supernova shell. The broadband images clearly demonstrate that X-ray emission from the North Spur and Eastern Limb results predominantly from non-thermal processes. We detect a break in the spatially integrated X-ray spectrum at similar to 9 keV that cannot be reproduced by current spectral energy distribution models, implying either a more complex electron injection spectrum or an additional process such as diffusion compared to what has been considered in previous work. We use spatially resolved maps to derive an energy-dependent cooling length scale, L(E) proportional to E-m with m = -0.21 +/- 0.01. We find this to be inconsistent with the model for the morphological evolution with energy described by Kennel & Coroniti. This value, along with the observed steepening in power-law index between radio and X-ray, can be quantitatively explained as an energy-loss spectral break in the simple scaling model of Reynolds, assuming particle advection dominates over diffusion. This interpretation requires a substantial departure from spherical magnetohydrodynamic, magnetic-flux-conserving outflow, most plausibly in the form of turbulent magnetic-field amplification. C1 [Nynka, Melania; Hailey, Charles J.; Gotthelf, Eric V.; Mori, Kaya; Perez, Kerstin] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Reynolds, Stephen P.] NC State Univ, Dept Phys, Raleigh, NC 27695 USA. [An, Hongjun] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Baganoff, Frederick K.] MIT, Ctr Space Res, Cambridge, MA 02139 USA. [Boggs, Steven E.; Craig, William W.; Krivonos, Roman; Zoglauer, Andreas] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wik, Daniel R.; Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Nynka, M (reprint author), Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; An, Hongjun/0000-0002-6389-9012; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C] FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTAR-DAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). NR 52 TC 10 Z9 10 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2014 VL 789 IS 1 AR 72 DI 10.1088/0004-637X/789/1/72 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK0LD UT WOS:000338103400072 ER PT J AU Vogel, JK Hascoet, R Kaspi, VM An, HJ Archibald, R Beloborodov, AM Boggs, SE Christensen, FE Craig, WW Gotthelf, EV Grefenstette, BW Hailey, CJ Harrison, FA Kennea, JA Madsen, KK Pivovaroff, MJ Stern, D Zhang, WW AF Vogel, Julia K. Hascoet, Romain Kaspi, Victoria M. An, Hongjun Archibald, Robert Beloborodov, Andrei M. Boggs, Steven E. Christensen, Finn E. Craig, William W. Gotthelf, Eric V. Grefenstette, Brian W. Hailey, Charles J. Harrison, Fiona A. Kennea, Jamie A. Madsen, Kristin K. Pivovaroff, Michael J. Stern, Daniel Zhang, William W. TI NuSTAR OBSERVATIONS OF THE MAGNETAR 1E 2259+586 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: individual (1E 2259+586); stars: magnetars; stars: neutron; X-rays: bursts ID X-RAY PULSAR; SOFT GAMMA REPEATERS; NEUTRON-STARS; 2002 OUTBURST; 4U 0142+61; EMISSION; SPECTRA; RXTE; ABSORPTION; G109.1-1.0 AB We report on new broad band spectral and temporal observations of the magnetar 1E 2259+586, which is located in the supernova remnant CTB 109. Our data were obtained simultaneously with the Nuclear Spectroscopic Telescope Array (NuSTAR) and Swift, and cover the energy range from 0.5-79 keV. We present pulse profiles in various energy bands and compare them to previous RXTE results. The NuSTAR data show pulsations above 20 keV for the first time and we report evidence that one of the pulses in the double-peaked pulse profile shifts position with energy. The pulsed fraction of the magnetar is shown to increase strongly with energy. Our spectral analysis reveals that the soft X-ray spectrum is well characterized by an absorbed double blackbody or blackbody plus power-law model in agreement with previous reports. Our new hard X-ray data, however, suggest that an additional component, such as a power law, is needed to describe the NuSTAR and Swift spectrum. We also fit the data with the recently developed coronal outflow model by Beloborodov for hard X-ray emission from magnetars. The outflow from a ring on the magnetar surface is statistically preferred over outflow from a polar cap. C1 [Vogel, Julia K.; Craig, William W.; Pivovaroff, Michael J.] Lawrence Livermore Natl Lab, Div Phys, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Hascoet, Romain; Beloborodov, Andrei M.; Gotthelf, Eric V.; Hailey, Charles J.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Hascoet, Romain; Beloborodov, Andrei M.; Gotthelf, Eric V.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Kaspi, Victoria M.; An, Hongjun; Archibald, Robert] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Kennea, Jamie A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Vogel, JK (reprint author), Lawrence Livermore Natl Lab, Div Phys, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RI Pivovaroff, Michael/M-7998-2014; Boggs, Steven/E-4170-2015; OI Pivovaroff, Michael/0000-0001-6780-6816; Boggs, Steven/0000-0001-9567-4224; An, Hongjun/0000-0002-6389-9012; Madsen, Kristin/0000-0003-1252-4891 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LDRD program [13-ERD-033]; NASA [NNG08FD60C]; National Aeronautics and Space Administration; NSERC; Centre de Recherche en Astrophysique du Quebec; Canadian Institute for Advanced Study; Canada Research Chairs Program; Lorne Trottier Chair in Astrophysics and Cosmology; NASA ATP [NNX 13AI34G] FX Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 with support from the LDRD program through grant 13-ERD-033. This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). V. M. K. receives support from an NSERC Discovery Grant and Accelerator Supplement, from the Centre de Recherche en Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Study, the Canada Research Chairs Program, and the Lorne Trottier Chair in Astrophysics and Cosmology. A. M. B. is supported by the NASA ATP grant NNX 13AI34G. This work made use of data supplied by the UK Swift Science Data Centre at the University of Leicester. We also thank Dr. A. M. Archibald for helpful discussions. NR 38 TC 9 Z9 9 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2014 VL 789 IS 1 AR 75 DI 10.1088/0004-637X/789/1/75 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK0LD UT WOS:000338103400075 ER PT J AU Zhang, HC Chen, XH Bottcher, M AF Zhang, Haocheng Chen, Xuhui Boettcher, Markus TI SYNCHROTRON POLARIZATION IN BLAZARS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: jets; gamma rays: galaxies; radiation mechanisms: non-thermal; relativistic processes ID TIME-DEPENDENT SIMULATIONS; GAMMA-RAY ACTIVITY; PKS 1510-089; MULTIWAVELENGTH OBSERVATIONS; INNER JET; VARIABILITY; EMISSION; MODELS; MARCH; FLARE AB We present a detailed analysis of time-and energy-dependent synchrotron polarization signatures in a shock-in-jet model for gamma-ray blazars. Our calculations employ a full three-dimensional radiation transfer code, assuming a helical magnetic field throughout the jet. The code considers synchrotron emission from an ordered magnetic field, and takes into account all light-travel-time and other relevant geometric effects, while the relevant synchrotron self-Compton and external Compton effects are handled with the two-dimensional Monte-Carlo/Fokker-Planck (MCFP) code. We consider several possible mechanisms through which a relativistic shock propagating through the jet may affect the jet plasma to produce a synchrotron and high-energy flare. Most plausibly, the shock is expected to lead to a compression of the magnetic field, increasing the toroidal field component and thereby changing the direction of the magnetic field in the region affected by the shock. We find that such a scenario leads to correlated synchrotron + synchrotron-self-Compton flaring, associated with substantial variability in the synchrotron polarization percentage and position angle. Most importantly, this scenario naturally explains large polarization angle rotations by greater than or similar to 180 degrees, as observed in connection with gamma-ray flares in several blazars, without the need for bent or helical jet trajectories or other nonaxisymmetric jet features. C1 [Zhang, Haocheng; Boettcher, Markus] Ohio Univ, Dept Phys & Astron, Inst Astrophys, Athens, OH 45701 USA. [Zhang, Haocheng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chen, Xuhui] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, Xuhui] DESY, D-15738 Zeuthen, Germany. [Boettcher, Markus] North West Univ, Ctr Space Res, ZA-2531 Potchefstroom, South Africa. RP Zhang, HC (reprint author), Ohio Univ, Dept Phys & Astron, Inst Astrophys, Athens, OH 45701 USA. OI Chen, Xuhui/0000-0002-9745-0248 FU NASA [NNX12AP20G]; LANL/LDRD program; DoE/Office of Fusion Energy Science through CMSO; Helmholtz Alliance for Astroparticle Physics HAP - Initiative and Networking Fund of the Helmholtz Association; South African Research Chairs Initiative of the Department of Science and Technology; National Research Foundation of South Africa FX We thank the anonymous referee for a careful review of the paper and helpful suggestions to improve the clarity of the manuscript, and Alan Marscher for valuable discussions and comments. This work was supported by NASA through Fermi Guest Investigator Grant no. NNX12AP20G. H.Z. is supported by the LANL/LDRD program and by DoE/Office of Fusion Energy Science through CMSO. X.C. acknowledges support by the Helmholtz Alliance for Astroparticle Physics HAP funded by the Initiative and Networking Fund of the Helmholtz Association. X.C. gratefully acknowledges the support during his visit to LANL when this work was started. M.B. acknowledges support by the South African Research Chairs Initiative of the Department of Science and Technology and the National Research Foundation of South Africa. Simulations were conducted on LANL's Institutional Computing machines. NR 26 TC 16 Z9 16 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2014 VL 789 IS 1 AR 66 DI 10.1088/0004-637X/789/1/66 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK0LD UT WOS:000338103400066 ER PT J AU Vinokur, JM Korman, TP Cao, Z Bowie, JU AF Vinokur, Jeffrey M. Korman, Tyler P. Cao, Zheng Bowie, James U. TI Evidence of a Novel Mevalonate Pathway in Archaea SO BIOCHEMISTRY LA English DT Article ID DIPHOSPHATE DECARBOXYLASE; PHYSIOLOGICAL-ASPECTS; CRYSTAL-STRUCTURES; BIOSYNTHESIS; ISOPRENOIDS; MECHANISM; EVOLUTION; BINDING; ORIGINS; SITE AB Isoprenoids make up a remarkably diverse class of more than 25000 biomolecules that include familiar compounds such as cholesterol, chlorophyll, vitamin A, ubiquinone, and natural rubber. The two essential building blocks of all isoprenoids, isopentenyl pyrophosphate (IPP) and dimethylallyl pyrophosphate (DMAPP), are ubiquitous in the three domains of life. In most eukaryotes and archaea, IPP and DMAPP are generated through the mevalonate pathway. We have identified two novel enzymes, mevalonate-3-kinase and mevalonate-3-phosphate-5-kinase from Thermoplasma acidophilum, which act sequentially in a putative alternate mevalonate pathway. We propose that a yet unidentified ATP-independent decarboxylase acts upon mevalonate 3,5-bisphosphate, yielding isopentenyl phosphate, which is subsequently phosphorylated by the known isopentenyl phosphate kinase from T. acidophilum to generate the universal isoprenoid precursor, IPP. C1 [Vinokur, Jeffrey M.; Korman, Tyler P.; Cao, Zheng; Bowie, James U.] Univ Calif Los Angeles, Dept Chem & Biochem, Inst Mol Biol, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. RP Bowie, JU (reprint author), Univ Calif Los Angeles, 659 Boyer Hall,611 Charles E Young Dr East, Los Angeles, CA 90095 USA. EM bowie@mbi.ucla.edu OI Cao, Zheng/0000-0002-9147-5540 FU U.S. Department of Energy [DE-FC02-02ER63421]; National Institutes of Health Chemistry Biology Interface Training Program (National Institute of General Medical Sciences) [5T32GM008496]; National Center for Research Resources [S10-RR025631]; National Science Foundation [CHE-1048804] FX The work was supported by U.S. Department of Energy Grant DE-FC02-02ER63421 to J.U.B., and J.M.V. received support from the National Institutes of Health Chemistry Biology Interface Training Program (National Institute of General Medical Sciences Grant 5T32GM008496). Use of the Waters LCT Premier XE time-of-flight instrument was supported by Grant S10-RR025631 from the National Center for Research Resources. NMR experiments were supported by the National Science Foundation via Equipment Grant CHE-1048804. NR 34 TC 8 Z9 10 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JUL 1 PY 2014 VL 53 IS 25 BP 4161 EP 4168 DI 10.1021/bi500566q PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AK0GA UT WOS:000338089700010 PM 24914732 ER PT J AU Lindedam, J Bruun, S Jorgensen, H Decker, SR Turner, GB DeMartini, JD Wyman, CE Felby, C AF Lindedam, Jane Bruun, Sander Jorgensen, Henning Decker, Stephen R. Turner, Geoffrey B. DeMartini, Jaclyn D. Wyman, Charles E. Felby, Claus TI Evaluation of high throughput screening methods in picking up differences between cultivars of lignocellulosic biomass for ethanol production SO BIOMASS & BIOENERGY LA English DT Article DE High throughput screening; Lignocellulosic ethanol; Wheat straw; Genetic selection; Microscale pretreatment ID WHEAT-STRAW; PRETREATMENT TECHNOLOGIES; ENZYMATIC-HYDROLYSIS; CELLULOSIC ETHANOL; CORN STOVER; IMPACT AB We present a unique evaluation of three advanced high throughput pretreatment and enzymatic hydrolysis systems (HTPH-systems) for screening of lignocellulosic biomass for enzymatic saccharification. Straw from 20 cultivars of winter wheat from two sites in Denmark was hydrothermally pretreated and enzymatically processed in each of the separately engineered HTPH-systems at 1) University of California, Riverside, 2) National Renewable Energy Laboratory (NREL), Colorado, and 3) University of Copenhagen (CPH). All three systems were able to detect significant differences between the cultivars in the release of fermentable sugars, with average cellulose conversions of 57%, 64%, and 71% from Riverside, NREL and CPH, respectively. The best correlation of glucose yields was found between the Riverside and NREL systems (R-2 = 0.2139), and the best correlation for xylose yields was found between Riverside and CPH (R-2 = 0.4269). All three systems identified Flair as the highest yielding cultivar and Dinosor, Glasgow, and Robigus as low yielding cultivars. Despite different conditions in the three HTPH-systems, the approach of microscale screening for phenotypically less recalcitrant feedstock seems sufficiently robust to be used as a generic analytical platform. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lindedam, Jane; Jorgensen, Henning; Felby, Claus] Univ Copenhagen, Dept Geosci & Nat Resource Management, DK-1958 Frederiksberg C, Denmark. [Lindedam, Jane; Bruun, Sander] Univ Copenhagen, Dept Plant & Environm Sci, DK-1871 Frederiksberg C, Denmark. [Decker, Stephen R.; Turner, Geoffrey B.] Natl Renewable Energy Lab, Prot Biochem Biosci Ctr, Golden, CO 80401 USA. [DeMartini, Jaclyn D.; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol, Riverside, CA 92507 USA. RP Lindedam, J (reprint author), Dept Plant & Environm Sci, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark. EM lindedam@life.ku.dk; sab@life.ku.dk; hnjoe@kt.dtu.dk; steve.decker@nrel.gov; geoffrey.turner@nrel.gov; jddemartini@gmail.com; cewyman@engr.ucr.edu; cf@life.ku.dk RI Bruun, Sander/G-3555-2014; Jorgensen, Henning/E-1728-2011; Lindedam, Jane/I-3523-2014; OI Bruun, Sander/0000-0002-2233-5122; Jorgensen, Henning/0000-0003-1220-6893; Lindedam, Jane/0000-0002-7063-7395; Felby, Claus/0000-0002-6537-0155 FU Danish Strategic Research Council [2117-05-0064]; BioEnergy Science Center, a U.S. Department of Energy Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science FX The collection of straw was funded through the OPUS project funded by the Danish Strategic Research Council (grant no. 2117-05-0064). Work at NREL and UCR was funded through the BioEnergy Science Center, a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 19 TC 3 Z9 3 U1 2 U2 38 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0961-9534 EI 1873-2909 J9 BIOMASS BIOENERG JI Biomass Bioenerg. PD JUL PY 2014 VL 66 BP 261 EP 267 DI 10.1016/j.biombioe.2014.03.006 PG 7 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AJ7LB UT WOS:000337877100028 ER PT J AU Iroba, KL Tabil, LG Sokhansanj, S Dumonceaux, T AF Iroba, Kingsley L. Tabil, Lope G. Sokhansanj, Shahab Dumonceaux, Tim TI Pretreatment and fractionation of barley straw using steam explosion at low severity factor SO BIOMASS & BIOENERGY LA English DT Article DE Biomass straw; Steam explosion; Severity factor; Chemical composition; Higher heating value; Carbon content ID LIGNOCELLULOSIC BIOMASS; HEATING VALUE; LIGNIN; FUELS; WOOD; TORREFACTION; COMPONENTS; CONVERSION; CELLULOSE; SOFTWOOD AB Agricultural residues represent an abundant, readily available, and inexpensive source of renewable lignocellulosic biomass. However, biomass has complex structural formation that binds cellulose and hemicellulose. This necessitates the initial breakdown of the lignocellulosic matrix. Steam explosion pretreatment was performed on barley straw grind to assist in the deconstruction and disaggregation of the matrix, so as to have access to the cellulose and hemicellulose. The following process and material variables were used: temperature (140-180 degrees C), corresponding saturated pressure (500-1100 kPa), retention time (5-10 min), and mass fraction of water 8-50%. The effect of the pretreatment was assessed through chemical composition analysis. The severity factor R-o, which combines the temperature and time of the hydrolytic process into a single reaction ordinate was determined. To further provide detailed chemical composition of the steam exploded and non-treated biomass, ultimate analysis was performed to quantify the elemental components. Data show that steam explosion resulted in the breakdown of biomass matrix with increase in acid soluble lignin. However, there was a considerable thermal degradation of cellulose and hemicellulose with increase in acid insoluble lignin content. The high degradation of the hemicellulose can be accounted for by its amorphous nature which is easily disrupted by external influences unlike the well-arranged crystalline cellulose. The carbon content of the solid steam exploded product increased at higher temperature and longer residence time, while the hydrogen and oxygen content decreased, and the higher heating value (HHV) increased. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Iroba, Kingsley L.; Tabil, Lope G.] Univ Saskatchewan, Dept Chem & Biol Engn, Saskatoon, SK S7N 5A9, Canada. [Sokhansanj, Shahab] Univ British Columbia, Dept Chem & Biol Engn, Vancouver, BC V6T 1Z3, Canada. [Sokhansanj, Shahab] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Dumonceaux, Tim] Agr & Agri Food Canada, Saskatoon Res Ctr, Saskatoon, SK S7N 0X2, Canada. RP Tabil, LG (reprint author), Univ Saskatchewan, Dept Chem & Biol Engn, 57 Campus Dr, Saskatoon, SK S7N 5A9, Canada. EM lope.tabil@usask.ca OI Dumonceaux, Tim/0000-0001-5165-0343 FU Natural Sciences and Engineering Research Council of Canada; Agriculture and Agri-Food Canada through the Agricultural Bioproduct Innovation Program FX The authors acknowledge the financial support of the Natural Sciences and Engineering Research Council of Canada and Agriculture and Agri-Food Canada through the Agricultural Bioproduct Innovation Program. Acknowledgment goes to Dr. Thomas Canam and Ms. Jennifer Town at Agriculture and AgriFood Canada for their technical assistance. The support from Zahra Tooyserkani and Bahman Ghiasi of the Department of Chemical and Biological Engineering, University of British Columbia and the technical support unit (Blondin Richard and Bill Crerar) of Chemical and Biological Engineering Department, University of Saskatchewan is highly appreciated. NR 46 TC 14 Z9 15 U1 4 U2 43 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0961-9534 EI 1873-2909 J9 BIOMASS BIOENERG JI Biomass Bioenerg. PD JUL PY 2014 VL 66 BP 286 EP 300 DI 10.1016/j.biombioe.2014.02.002 PG 15 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AJ7LB UT WOS:000337877100031 ER PT J AU Moon, M Kim, CW Farooq, W Suh, WI Shrivastav, A Park, MS Mishra, SK Yang, JW AF Moon, Myounghoon Kim, Chul Woong Farooq, Wasif Suh, William I. Shrivastav, Anupama Park, Min S. Mishra, Sanjiv K. Yang, Ji-Won TI Utilization of lipid extracted algal biomass and sugar factory wastewater for algal growth and lipid enhancement of Ettlia sp. SO BIORESOURCE TECHNOLOGY LA English DT Article DE Microalgae; Ettlia sp.; Lipid extracted algal biomass (LEA); Sugar factory; FAME yield ID BIODIESEL PRODUCTION; CHLORELLA-PROTOTHECOIDES; OIL PRODUCTION; CULTIVATION; MICROALGAE; HYDROLYSATE; VULGARIS; SORGHUM AB The present study assessed the use of hydrolysate of lipid extracted algal biomass (LEA) combined with the sugar factory wastewater (SFW) as a low cost nutrient and a carbon source, respectively for microalgal cultivation. Microalgal strain Ettlia sp. was both mixotrophically and heterotrophically cultivated using various amounts of hydrolysate and SFW. The culture which was grown in medium containing 50% LEA hydrolysate showed highest growth, achieving 5.26 +/- 0.14 g L-1 after 12 days of cultivation. The addition of SFW increased the lipid productivity substantially from 5.8 to 95.5 mg L-1 d(-1) when the culture medium was fortified with 20% SFW. Gas chromatography analysis indicated a noticeable increase of 20% in C16 and C18 fraction in FAME distribution under above condition. Therefore, it can be concluded that the combination of LEA hydrolysate and sugar factory waste water can be a powerful growth medium for economical algal cultivation. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Moon, Myounghoon; Kim, Chul Woong; Farooq, Wasif; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Dept Biomol & Chem Engn, Taejon 305701, South Korea. [Suh, William I.; Shrivastav, Anupama; Park, Min S.; Mishra, Sanjiv K.; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, Taejon 305701, South Korea. [Park, Min S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Mishra, SK (reprint author), Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, 291 Daehak Ro, Taejon 305701, South Korea. EM sanjivkm@kaist.ac.kr RI Yang, Ji-Won/C-1933-2011; Mishra, Sanjiv/I-4156-2014 OI Mishra, Sanjiv/0000-0002-0403-6575 FU Advanced Biomass R&D Center (ABC) of Korea - Ministry of Science, ICT and Future Planning [ABC-2010-0029728] FX This work was supported by the Advanced Biomass R&D Center (ABC) of Korea Grant funded by the Ministry of Science, ICT and Future Planning (ABC-2010-0029728). NR 32 TC 7 Z9 7 U1 0 U2 23 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD JUL PY 2014 VL 163 BP 180 EP 185 DI 10.1016/j.biortech.2014.04.033 PG 6 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AJ7KK UT WOS:000337875400025 PM 24811446 ER PT J AU Rouet-Leduc, B Barros, K Cieren, E Elango, V Junghans, C Lookman, T Mohd-Yusof, J Pavel, RS Rivera, AY Roehm, D McPherson, AL Germann, TC AF Rouet-Leduc, Bertrand Barros, Kipton Cieren, Emmanuel Elango, Venmugil Junghans, Christoph Lookman, Turab Mohd-Yusof, Jamaludin Pavel, Robert S. Rivera, Axel Y. Roehm, Dominic McPherson, Allen L. Germann, Timothy C. TI Spatial adaptive sampling in multiscale simulation SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Multiscale; Adaptive sampling ID HYPERBOLIC CONSERVATION-LAWS; GRAINED MOLECULAR-DYNAMICS; VIRIAL STRESS; CONTINUUM MODELS; MESH REFINEMENT; SOLIDS; DEFORMATION; MECHANICS; COMPUTATION; ALGORITHMS AB In a common approach to multiscale simulation, an incomplete set of macroscale equations must be supplemented with constitutive data provided by fine-scale simulation. Collecting statistics from these fine-scale simulations is typically the overwhelming computational cost. We reduce this cost by interpolating the results of fine-scale simulation over the spatial domain of the macro-solver. Unlike previous adaptive sampling strategies, we do not interpolate on the potentially very high dimensional space of inputs to the fine-scale simulation. Our approach is local in space and time, avoids the need for a central database, and is designed to parallelize well on large computer clusters. To demonstrate our method, we simulate one-dimensional elastodynamic shock propagation using the Heterogeneous Multiscale Method (HMM); we find that spatial adaptive sampling requires only approximate to 50 x N-0.14 fine-scale simulations to reconstruct the stress field at all N grid points. Related multiscale approaches, such as Equation Free methods, may also benefit from spatial adaptive sampling. (C) 2014 Elsevier B.V. All rights reserved. C1 [Rouet-Leduc, Bertrand; Barros, Kipton; Cieren, Emmanuel; Junghans, Christoph; Lookman, Turab; Roehm, Dominic; Germann, Timothy C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Elango, Venmugil; Mohd-Yusof, Jamaludin; Pavel, Robert S.; Rivera, Axel Y.; McPherson, Allen L.] Los Alamos Natl Lab, Comp & Computat Sci Div, Los Alamos, NM 87545 USA. [Rouet-Leduc, Bertrand] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Cieren, Emmanuel] CEA, DAM, DIF, F-91297 Arpajon, France. [Pavel, Robert S.] Univ Delaware, Dept Elect & Comp Engn, Newark, DE 19716 USA. [Rivera, Axel Y.] Univ Utah, Sch Comp, Salt Lake City, UT 84112 USA. [Roehm, Dominic] Univ Stuttgart, Inst Computat Phys, D-70569 Stuttgart, Germany. [Elango, Venmugil] Ohio State Univ, Dept Comp Sci & Engn, Columbus, OH 43210 USA. RP Barros, K (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kbarros@lanl.gov; tcg@lanl.gov RI Junghans, Christoph/G-4238-2010; OI Junghans, Christoph/0000-0003-0925-1458; Elango, Venmugil/0000-0002-7031-9020; Mohd Yusof, Jamaludin/0000-0002-9844-689X; Germann, Timothy/0000-0002-6813-238X; Barros, Kipton/0000-0002-1333-5972 FU Los Alamos Information Science & Technology Center (IS&T) Co-Design Summer School; US Department of Energy (DOE), Office of Advanced Scientific Computing Research (ASCR) through the Exascale Co-Design Center for Materials in Extreme Environments (ExMatEx, exmatex.org); Center for Nonlinear Studies (CNLS); Los Alamos National Laboratory Director's Fellowship; Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX This work was supported by the Los Alamos Information Science & Technology Center (IS&T) Co-Design Summer School, the US Department of Energy (DOE), Office of Advanced Scientific Computing Research (ASCR) through the Exascale Co-Design Center for Materials in Extreme Environments (ExMatEx, exmatex.org), and the Center for Nonlinear Studies (CNLS). C.J. acknowledges funding by a Los Alamos National Laboratory Director's Fellowship. Assigned: LA-UR 13-29626. Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. NR 53 TC 4 Z9 5 U1 4 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD JUL PY 2014 VL 185 IS 7 BP 1857 EP 1864 DI 10.1016/j.cpc.2014.03.011 PG 8 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AJ5ZF UT WOS:000337768700001 ER PT J AU Hu, LB Amine, K Zhang, ZC AF Hu, Libo Amine, Khalil Zhang, Zhengcheng TI Fluorinated electrolytes for 5-V Li-ion chemistry: Dramatic enhancement of LiNi0.5Mn1.5O4/graphite cell performance by a lithium reservoir SO ELECTROCHEMISTRY COMMUNICATIONS LA English DT Article DE Fluorinated solvents; High voltage electrolyte; Lithium reservoir; 5-V LiNi0.5Mn1.5O4 cathode; Lithium-ion batteries ID HIGH-VOLTAGE; BATTERIES; PRELITHIATION; STABILITY; CAPACITY; SURFACE; ANODE; SLMP AB A fluorinated electrolyte was galvanostatically charged and discharged for 100 cycles at an elevated temperature (55 degrees C) with a LiNi0.5Mn1.5O4 cathode coupled with a graphite anode in the presence of a lithium reservoir. The incorporation of the lithium reservoir was able to compensate for the loss of the active lithium from the LiNi0.5Mn1.5O4 cathode due to the electrolyte oxidative decomposition. Our experimental data demonstrate for the first time that lithium compensation is an efficient way to enhance the performance of high voltage LiNi0.5Mn1.5O4/graphite cell at a high temperature (55 degrees C). 2014 Elsevier B.V. All rights reserved. C1 [Hu, Libo; Amine, Khalil; Zhang, Zhengcheng] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Zhang, ZC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zzhang@anl.gov RI Hu, Libo/A-5911-2012 FU Advanced Battery Research (ABR) for Transportation, Vehicle Technologies Program; Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy; UChicago Argonne, LLC [DE-AC02-06CH11357] FX This research is supported by the Advanced Battery Research (ABR) for Transportation, Vehicle Technologies Program, and the Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC, under contract DE-AC02-06CH11357. NR 19 TC 18 Z9 18 U1 10 U2 102 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1388-2481 EI 1873-1902 J9 ELECTROCHEM COMMUN JI Electrochem. Commun. PD JUL PY 2014 VL 44 BP 34 EP 37 DI 10.1016/j.elecom.2014.04.006 PG 4 WC Electrochemistry SC Electrochemistry GA AJ8ZU UT WOS:000337997400010 ER PT J AU Guo, BK Yu, XQ Sun, XG Chi, MF Qiao, ZA Liu, J Hu, YS Yang, XQ Goodenough, JB Dai, S AF Guo, Bingkun Yu, Xiqian Sun, Xiao-Guang Chi, Miaofang Qiao, Zhen-An Liu, Jue Hu, Yong-Sheng Yang, Xiao-Qing Goodenough, John B. Dai, Sheng TI A long-life lithium-ion battery with a highly porous TiNb2O7 anode for large-scale electrical energy storage SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Article ID PERFORMANCE; ELECTROLYTE; FRAMEWORK; SILICON; LINI0.5MN1.5O4; COMPOSITES; LITHIATION; NANOWIRES; NANOTUBES; CHEMISTRY AB A high performance TiNb2O7 anode material with a nanoporous nature, which was prepared by a facile approach, exhibits an average storage voltage of 1.66 V, a reversible capacity of 281mA h g(-1), and an 84% capacity retention after 1000 cycles, and may be suitable for long-life stationary lithium-ion batteries. C1 [Guo, Bingkun; Sun, Xiao-Guang; Qiao, Zhen-An; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Yu, Xiqian; Liu, Jue; Yang, Xiao-Qing] Brookhaven Natl Lab, Upton, NY 11973 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Hu, Yong-Sheng] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Goodenough, John B.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Guo, BK (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM guobkun@hotmail.com; yshu@aphy.iphy.ac.cn; dais@ornl.gov RI Guo, Bingkun/J-5774-2014; Hu, Yong-Sheng/H-1177-2011; Chi, Miaofang/Q-2489-2015; Yu, Xiqian/B-5574-2014; LIU, JUE/I-8631-2016; Dai, Sheng/K-8411-2015 OI Qiao, Zhen-An/0000-0001-6064-9360; Goodenough, John Bannister/0000-0001-9350-3034; Hu, Yong-Sheng/0000-0002-8430-6474; Chi, Miaofang/0000-0003-0764-1567; Yu, Xiqian/0000-0001-8513-518X; LIU, JUE/0000-0002-4453-910X; Dai, Sheng/0000-0002-8046-3931 FU U.S. Department of Energy's office of Basic Energy Science, Division of Materials Sciences Engineering; U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, and the Office of Vehicle Technologies [DEAC02-98CH10886]; NSFC [51222210]; One Hundred Talent Project of the Chinese Academy of Sciences FX The research at Oak Ridge National Laboratory and the University of Texas at Austin was supported by the U.S. Department of Energy's office of Basic Energy Science, Division of Materials Sciences Engineering. The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, and the Office of Vehicle Technologies under Contract Number DEAC02-98CH10886. The authors thank the technical support from scientists at beamlines X14A, X18a, and X18B of the National Synchrotron Light Source (NSLS). Y.- S. H. thanks the funding support from NSFC (51222210) and the One Hundred Talent Project of the Chinese Academy of Sciences. NR 40 TC 62 Z9 63 U1 19 U2 186 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 EI 1754-5706 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD JUL PY 2014 VL 7 IS 7 BP 2220 EP 2226 DI 10.1039/c4ee00508b PG 7 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA AJ8SL UT WOS:000337977600010 ER PT J AU Quadros, WR AF Quadros, William Roshan TI Guest editorial: 20th international meshing roundtable special issue SO ENGINEERING WITH COMPUTERS LA English DT Editorial Material C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Quadros, WR (reprint author), Sandia Natl Labs, POB 5800,MS 0897, Albuquerque, NM 87185 USA. EM wrquadr@sandia.gov NR 0 TC 0 Z9 0 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0177-0667 EI 1435-5663 J9 ENG COMPUT-GERMANY JI Eng. Comput. PD JUL PY 2014 VL 30 IS 3 SI SI BP 287 EP 287 DI 10.1007/s00366-014-0365-y PG 1 WC Computer Science, Interdisciplinary Applications; Engineering, Mechanical SC Computer Science; Engineering GA AJ9JV UT WOS:000338026900001 ER PT J AU Owen, SJ Staten, ML Sorensen, MC AF Owen, Steven J. Staten, Matthew L. Sorensen, Marguerite C. TI Parallel hexahedral meshing from volume fractions SO ENGINEERING WITH COMPUTERS LA English DT Article DE Grid-based; Overlay grid; Hexahedral mesh generation; Parallel meshing ID GENERATION AB In this work, we introduce a new method for generating Lagrangian computational meshes from Eulerian-based data. We focus specifically on shock physics problems that are relevant to Eulerian-based codes that generate volume fraction data on a Cartesian grid. A step-by-step procedure for generating an all-hexahedral mesh is presented. We focus specifically on the challenges of developing a parallel implementation using the message passing interface to ensure a continuous, conformal and good quality hex mesh. C1 [Owen, Steven J.; Staten, Matthew L.; Sorensen, Marguerite C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Owen, SJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sjowen@sandia.gov; mlstate@sandia.gov; mcsoren@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 15 TC 1 Z9 1 U1 2 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0177-0667 EI 1435-5663 J9 ENG COMPUT-GERMANY JI Eng. Comput. PD JUL PY 2014 VL 30 IS 3 SI SI BP 301 EP 313 DI 10.1007/s00366-012-0292-8 PG 13 WC Computer Science, Interdisciplinary Applications; Engineering, Mechanical SC Computer Science; Engineering GA AJ9JV UT WOS:000338026900003 ER PT J AU Harris, JB Eldridge, ML Sayler, G Menn, FM Layton, AC Baudry, J AF Harris, Jason B. Eldridge, Melanie L. Sayler, Gary Menn, Fu-Min Layton, Alice C. Baudry, Jerome TI A COMPUTATIONAL APPROACH PREDICTING CYP450 METABOLISM AND ESTROGENIC ACTIVITY OF AN ENDOCRINE DISRUPTING COMPOUND (PCB-30) SO ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY LA English DT Article DE Endocrine disrupting compound; Cytochrome P450 2D6 (CYP2D6); Cytochrome P450 3A4 (CYP3A4); Polychlorinated biphenyl 30 (PCB-30); 2,4,6-trichlorobiphenyl (TCBP) ID POLYCYCLIC AROMATIC-HYDROCARBONS; RECOMBINANT YEAST ASSAY; POLYCHLORINATED-BIPHENYLS; CYTOCHROME-P450 2D6; IN-VITRO; MOLECULAR DOCKING; HYDROXYLATED METABOLITES; ANDROGENIC ACTIVITY; RECEPTOR BINDING; LIGAND-BINDING AB Endocrine disrupting chemicals influence growth and development through interactions with the hormone system, often through binding to hormone receptors such as the estrogen receptor. Computational methods can predict endocrine disrupting chemical activity of unmodified compounds, but approaches predicting activity following metabolism are lacking. The present study uses a well-known environmental contaminant, PCB-30 (2,4,6-trichlorobiphenyl), as a prototype endocrine disrupting chemical and integrates predictive (computational) and experimental methods to determine its metabolic transformation by cytochrome P450 3A4 (CYP3A4) and cytochrome P450 2D6 (CYP2D6) into estrogenic byproducts. Computational predictions suggest that hydroxylation of PCB-30 occurs at the 3- or 4-phenol positions and leads to metabolites that bind more strongly than the parent molecule to the human estrogen receptor alpha (hER-alpha). Gas chromatography-mass spectrometry experiments confirmed that the primary metabolite for CYP3A4 and CYP2D6 is 4-hydroxy-PCB-30, and the secondary metabolite is 3-hydroxy-PCB-30. Cell-based bioassays (bioluminescent yeast expressing hER-alpha) confirmed that hydroxylated metabolites are more estrogenic than PCB-30. These experimental results support the applied model's ability to predict the metabolic and estrogenic fate of PCB-30, which could be used to identify other endocrine disrupting chemicals involved in similar pathways. (C) 2014 SETAC C1 [Harris, Jason B.] Univ Tennessee, Genome Sci & Technol Grad Sch, Knoxville, TN USA. [Harris, Jason B.; Baudry, Jerome] Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA. [Eldridge, Melanie L.; Sayler, Gary; Menn, Fu-Min; Layton, Alice C.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. [Sayler, Gary; Menn, Fu-Min] Univ Tennessee, Oak Ridge Natl Lab, Joint Inst Biol Sci, Oak Ridge, TN USA. [Sayler, Gary] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Baudry, Jerome] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN USA. RP Baudry, J (reprint author), Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA. EM jbaudry@utk.edu FU University of Tennessee; Genome Science and Technology graduate school; IGERT: SCALE-IT fellowship (NSF) [0801540] FX J.B. Harris and M.L. Eldridge contributed equally to this work. A. C. Layton and J. Baudry contributed equally to supervision and expertise. This work was supported financially by a start-up grant from the University of Tennessee to J. Baudry. J. Harris acknowledges support by the Genome Science and Technology graduate school and the IGERT: SCALE-IT fellowship (NSF Award 0801540). NR 62 TC 5 Z9 5 U1 6 U2 29 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0730-7268 EI 1552-8618 J9 ENVIRON TOXICOL CHEM JI Environ. Toxicol. Chem. PD JUL PY 2014 VL 33 IS 7 BP 1615 EP 1623 DI 10.1002/etc.2595 PG 9 WC Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA AJ6FD UT WOS:000337784500024 PM 24687371 ER PT J AU Soteropoulos, DL Lance, SL Flynn, RW Scott, DE AF Soteropoulos, Diana L. Lance, Stacey L. Flynn, R. Wesley Scott, David E. TI EFFECTS OF COPPER EXPOSURE ON HATCHING SUCCESS AND EARLY LARVAL SURVIVAL IN MARBLED SALAMANDERS, AMBYSTOMA OPACUM SO ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY LA English DT Article DE Amphibian; Created wetland; Ecotoxicology; Metal toxicity; Treatment wetlands ID COAL-COMBUSTION WASTES; AMPHIBIAN EMBRYOS; CHRONIC TOXICITY; SOUTHERN TOADS; RANA-PIPIENS; FROG; TADPOLES; WETLANDS; RUNOFF; GROWTH AB The creation of wetlands, such as urban and industrial ponds, has increased in recent decades, and these wetlands often become enriched in pollutants over time. One metal contaminant trapped in created wetlands is copper (Cu2+). Copper concentrations in sediments and overlying water may affect amphibian species that breed in created wetlands. The authors analyzed the Cu concentration in dried sediments from a contaminated wetland and the levels of aqueous Cu released after flooding the sediments with different volumes of water, mimicking low, medium, and high pond-filling events. Eggs and larvae of Ambystoma opacum Gravenhorst, a salamander that lays eggs on the sediments in dry pond beds that hatch on pond-filling, were exposed to a range of Cu concentrations that bracketed potential aqueous Cu levels in created wetlands. Embryo survival varied among clutches, but increased Cu levels did not affect embryo survival. At Cu concentrations of 500 mu g/L or greater, however, embryos hatched earlier, and the aquatic larvae died shortly after hatching. Because Cu concentrations in sediments increase over time in created wetlands, even relatively tolerant species such as A. opacum may be affected by Cu levels in the posthatching environment. (C) 2014 SETAC C1 [Soteropoulos, Diana L.; Lance, Stacey L.; Flynn, R. Wesley; Scott, David E.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. RP Scott, DE (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM scott@srel.uga.edu RI Lance, Stacey/K-9203-2013 OI Lance, Stacey/0000-0003-2686-1733 FU US Department of Energy [DE-FC09-07SR22506]; Department of Energy National Nuclear Security Administration FX We thank J. Seaman for assistance with metals analysis. This research was partially supported by US Department of Energy under award number DE-FC09-07SR22506 to the University of Georgia Research Foundation. Project funding was provided by the Department of Energy National Nuclear Security Administration. Animals were collected under SCDNR permit #G-09-03 following IACUC procedures (AUP A2009 10-175-Y2-A0) from the University of Georgia. This manuscript was improved by comments from members of the Lance Lab-R. Beasley, C. Love, C. Rumrill, and M. Winzeler. NR 54 TC 1 Z9 1 U1 3 U2 29 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0730-7268 EI 1552-8618 J9 ENVIRON TOXICOL CHEM JI Environ. Toxicol. Chem. PD JUL PY 2014 VL 33 IS 7 BP 1631 EP 1637 DI 10.1002/etc.2601 PG 7 WC Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA AJ6FD UT WOS:000337784500026 PM 24729474 ER PT J AU Dong, B Li, XQ Xiao, LM Ruan, L AF Dong, Bin Li, Xiuqiao Xiao, Limin Ruan, Li TI Towards minimizing disk I/O contention: A partitioned file assignment approach SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF ESCIENCE LA English DT Article DE Parallel I/O system; Partitioned file; File assignment algorithm; I/O contention probability; Distributed resource management ID PARALLEL I/O; HIGH-PERFORMANCE; SYSTEMS; ISSUES; TIME; WORKLOADS; STORAGE; ARRAYS; RAID AB One problem with data-intensive computing facilitating is how to effectively manage massive amounts of data stored in a parallel I/O system. The file assignment method plays a significant role in data management. However, in the context of a parallel I/O system, most existing file assignment approaches share the following two limitations. First, most existing methods are designed for a non-partitioned file, while the file in a parallel I/O system is generally partitioned to provide aggregated bandwidth. Second, the file allocation metric, e.g. service time, of most existing methods is difficult to determine in practice, and also these metrics only reflect the static property of the file. In this paper, a new metric, namely file access density is proposed to capture the dynamic property of file access, i.e. disk contention property. Based on file access density definition, this paper introduces a new static file assignment algorithm named MinCPP and its dynamic version DMinCPP, both of which aim at minimizing the disk contention property. Furthermore MinCPP and DMinCPP take the file partition property into consideration by trying to allocate the partitions belonging to the same file onto different disks. By assuming file request arrival follows the Poisson process, we prove the effectiveness of the proposed schemes both analytically and experimentally. The MinCPP presented in this study can be applied to reorganize the files stored in a large-scale parallel I/O system and the DMinCPP can be integrated into file systems which dynamically allocate files in a batch. (C) 2013 Elsevier B.V. All rights reserved. C1 [Dong, Bin; Li, Xiuqiao; Xiao, Limin; Ruan, Li] Beihang Univ, Sch Comp Sci & Engn, Beijing 100191, Peoples R China. [Dong, Bin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Dong, B (reprint author), Beihang Univ, Sch Comp Sci & Engn, Beijing 100191, Peoples R China. EM Bdong@cse.buaa.edu.cn FU National Natural Science Foundation of China [61370059, 61232009]; Doctoral Fund of Ministry of Education of China [20101102110018] FX The work described in this paper is supported by the National Natural Science Foundation of China under Grant No. 61370059, supported by the National Natural Science Foundation of China under Grant No. 61232009, and supported by the Doctoral Fund of Ministry of Education of China under Grant No. 20101102110018. NR 53 TC 4 Z9 4 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 37 BP 178 EP 190 DI 10.1016/j.future.2013.12.022 PG 13 WC Computer Science, Theory & Methods SC Computer Science GA AJ8CV UT WOS:000337931200017 ER PT J AU Okoro, C Levine, LE Xu, RQ Hummler, K Obeng, YS AF Okoro, Chukwudi Levine, Lyle E. Xu, Ruqing Hummler, Klaus Obeng, Yaw S. TI Nondestructive Measurement of the Residual Stresses in Copper Through-Silicon Vias Using Synchrotron-Based Microbeam X-Ray Diffraction SO IEEE TRANSACTIONS ON ELECTRON DEVICES LA English DT Article DE Interconnect; keep-out-zone (KOZ); stress measurement; synchrotron; three-dimensional integrated circuits (3DIC); through-silicon via (TSV); X-ray diffraction ID FAILURE ANALYSIS; CU-TSV; DEFORMATION AB In this paper, we report a new method for achieving depth resolved determination of the full stress tensor in buried Cu through-silicon vias (TSVs), using a synchrotron-based X-ray microdiffraction technique. Two adjacent Cu TSVs were analyzed; one capped with SiO2 (0.17 mu m) and the other without. The uncapped Cu TSV was found to have higher stresses with an average hydrostatic stress value of 145 +/- 37 MPa, as compared with the capped Cu TSV, which had a value of 89 +/- 28 MPa. Finite element-based parametric analyses of the effect of cap thickness on TSV stress were also performed. The differences in the stresses in the adjacent Cu TSVs were attributed to their microstructural differences and not to the presence of a cap layer. Based on the experimentally determined stresses, the stresses in the surrounding Si for both Cu TSVs were calculated and the FinFET keep-out-zone (KOZ) from the Cu TSV was estimated. The FinFET KOZ is influenced by the microstructural variations in their neighboring Cu TSVs, thus, it should be accounted for in KOZ design rules. C1 [Okoro, Chukwudi; Obeng, Yaw S.] NIST, Semicond & Dimens Metrol Div, Gaithersburg, MD 20899 USA. [Levine, Lyle E.] NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. [Xu, Ruqing] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hummler, Klaus] SEMATECH, Albany, NY 12203 USA. RP Okoro, C (reprint author), NIST, Semicond & Dimens Metrol Div, Gaithersburg, MD 20899 USA. EM chukwudi.okoro@nist.gov; lyle.levine@nist.gov; ruqingxu@anl.gov; klaus.hummler@sematech.org; yaw.obeng@nist.gov RI Xu, Ruqing/K-3586-2012 OI Xu, Ruqing/0000-0003-1037-0059 FU U.S Department of Energy's (DOE) Office of Science [DE-AC02-06CH11357] FX The XOR/UNI facilities on Sector 34 at the Advanced Photon Source (APS) is supported by the U.S Department of Energy's (DOE) Office of Science, under Contract No. DE-AC02-06CH11357. The review of this paper was arranged by Editor R. Venkatasubramanian. NR 17 TC 11 Z9 11 U1 1 U2 22 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9383 EI 1557-9646 J9 IEEE T ELECTRON DEV JI IEEE Trans. Electron Devices PD JUL PY 2014 VL 61 IS 7 BP 2473 EP 2479 DI 10.1109/TED.2014.2321736 PG 7 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA AJ9JY UT WOS:000338027200036 ER PT J AU Santoso, S Lwin, M Ramos, J Singh, M Muljadi, E Jonkman, J AF Santoso, Surya Lwin, Min Ramos, Jaime Singh, Mohit Muljadi, Eduard Jonkman, Jason TI Designing and Integrating Wind Power Laboratory Experiments in Power and Energy Systems Courses SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Power engineering education; power system simulation; reactive power control; student experiments; wind power generation ID ELECTRONICS; CONVERSION AB The goal of this paper is to describe the approach in designing and constructing wind power laboratory experiments for undergraduate- and graduate-level courses in power and energy systems. These are separated into basic hands-on laboratory and advanced simulation-based experiments. The basic experiments are integrated into an undergraduate course that includes topics such as the steady-state operation of induction machines, fixed-speed, and variable-speed wind turbines. Advanced experiments are integrated into a stand-alone course dedicated to wind energy and power systems. Topics include the modeling of aerodynamic, mechanical, and electrical components for each type of wind turbine along with their steady-state and dynamic operations. The experiments were originally designed at the University of Texas at Austin. Their transferability to a different laboratory platform at the University of Texas Pan American is also discussed. C1 [Santoso, Surya; Lwin, Min] Univ Texas Austin, Dept Elect & Comp Engn, Austin, TX 78712 USA. [Ramos, Jaime] Univ Texas Pan Amer, Dept Elect Engn, Edinburg, TX 78539 USA. [Singh, Mohit; Muljadi, Eduard; Jonkman, Jason] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Santoso, S (reprint author), Univ Texas Austin, Dept Elect & Comp Engn, Austin, TX 78712 USA. EM ssantoso@mail.utexas.edu; m.lwin@utexas.edu; jramos8@utpa.edu; Mohit.Singh@nrel.gov; Eduard.Muljadi@nrel.gov; Jason.Jonkman@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; National Science Foundation [DUE-0736974, DUE-0737051] FX This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory and the National Science Foundationunder grants DUE-0736974 and DUE-0737051. Paper no. TPWRS-00712-2013. NR 16 TC 1 Z9 1 U1 1 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD JUL PY 2014 VL 29 IS 4 BP 1944 EP 1951 DI 10.1109/TPWRS.2014.2307324 PG 8 WC Engineering, Electrical & Electronic SC Engineering GA AK1QF UT WOS:000338189600051 ER PT J AU Soong, Y Hedges, SW Howard, BH Dilmore, RM Allen, DE AF Soong, Yee Hedges, Sheila W. Howard, Bret H. Dilmore, Robert M. Allen, Douglas E. TI Effect of contaminants from flue gas on CO2 sequestration in saline formation SO INTERNATIONAL JOURNAL OF ENERGY RESEARCH LA English DT Article DE CO2 sequestration; flue gas; saline aquifers ID CARBON SEQUESTRATION; SO2; INJECTION; WATER AB Deep saline aquifers are reported to have the largest estimated capacity for CO2 sequestration. Most geochemical studies on CO2 storage in saline formations are focused on the interactions of pure CO2 and do not consider the potential impacts of contaminants such as SO2 found in typical post-composition flue gas streams. This paper reports on results of a combined CO2-co-contaminant-brine-rock experimental and a simple modeling study of the potential impact of flue gas contaminants on saline formations. Chemical reactions of the sandstone from Mount Simon formation exposed to CO2 mixed with other gas species under sequestration conditions were studied (i.e. solid material-representative Mount Simon sandstone; liquid - synthetic Illinois Basin brine; T and P - 50 degrees C, 110 bar; gas composition - 1% SO2, 4% O-2, 95% CO2). The experimental study indicates that the co-injection of 1% SO2 would lead to substantially reduced brine pH due to the formation of sulfuric acid and the formation of bassanite (major) and anhydrites. Preliminary equilibrium computational modeling yielded similar results. Copyright (C) 2013 John Wiley & Sons, Ltd. C1 [Soong, Yee; Hedges, Sheila W.; Howard, Bret H.; Dilmore, Robert M.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Allen, Douglas E.] Salem State Univ, Salem, MA 01970 USA. RP Soong, Y (reprint author), US DOE, Natl Energy Technol Lab, POB 10940, Pittsburgh, PA 15236 USA. EM soong@netl.doe.gov FU Department of Energy, National Energy Technology Laboratory, an agency of the United States Government; URS Energy & Construction, Inc. FX This project was funded in part by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with URS Energy & Construction, Inc. Neither the United States Government nor any agency thereof, nor any of their employees, nor URS Energy & Construction, Inc., nor any of their employees, makes any warranty, expressed or implied; or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed; or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 20 TC 3 Z9 3 U1 2 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-907X EI 1099-114X J9 INT J ENERG RES JI Int. J. Energy Res. PD JUL PY 2014 VL 38 IS 9 BP 1224 EP 1232 DI 10.1002/er.3140 PG 9 WC Energy & Fuels; Nuclear Science & Technology SC Energy & Fuels; Nuclear Science & Technology GA AJ6KF UT WOS:000337801900012 ER PT J AU Hasanbeigi, A Jiang, ZY Price, L AF Hasanbeigi, Ali Jiang, Zeyi Price, Lynn TI Retrospective and prospective analysis of the trends of energy use in Chinese iron and steel industry SO JOURNAL OF CLEANER PRODUCTION LA English DT Article DE Energy intensity forecast; Decomposition analysis; Chinese steel industry; Structural change ID DECOMPOSITION ANALYSIS; CO2 EMISSIONS; EFFICIENCY; INTENSITY; SECTOR AB The iron and steel industry accounted for approximately 27% of China's primary energy use for the manufacturing industry in 2010. This study aims to analyze influential factors that affected the energy use of steel industry in the past in order to quantify the likely effect of those factors in the future. This study analyzes the energy use trends of China's key medium- and large-sized steel enterprises during 2000-2030. In addition, the study uses a refined Logarithmic Mean Divisia Index decomposition analysis to quantify the effects of various factors in shaping energy consumption trends in the past and in the future. The result of our forecast shows the final energy use of the key steel enterprises peaks in year 2020 under scenario 1 and 2 (low and medium scrap usage) and in 2015 under scenario 3 (high scrap usage). The three scenarios produced for the forward-looking decomposition analysis for 2010-2030 show that contrary to the experience during 2000-2010, the structural (activity share of each process route) effect and the pig iron ratio (the ratio of pig iron used as feedstock in each process route) effect plays an important role in reducing final energy use during 2010-2030. Published by Elsevier Ltd. C1 [Hasanbeigi, Ali; Jiang, Zeyi; Price, Lynn] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, China Energy Grp,Environm Energy Technol Div, Berkeley, CA 94720 USA. [Jiang, Zeyi] Univ Sci & Technol Beijing, Sch Mech Engn, Beijing, Peoples R China. RP Hasanbeigi, A (reprint author), 1 Cyclotron Rd MS 90R2002, Berkeley, CA 94720 USA. EM AHasanbeigi@lbl.gov FU China Sustainable Energy Program of the Energy Foundation through the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the China Sustainable Energy Program of the Energy Foundation through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We would like to thank David Fridley, Nina Khanna, and Ryan Triolo of the China Energy Group of Lawrence Berkeley National Laboratory for their contributions to this study. We are also thankful to Peng Wang and Fushan Tian of the School of Mechanical Engineering, University of Science and Technology Beijing, China for their research assistance in this study. We are grateful to Zhang Chunxia and Li Xiuping of the China Iron 82 Steel Research Institute for their valuable comments on an earlier version of the paper. NR 38 TC 8 Z9 8 U1 0 U2 26 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-6526 EI 1879-1786 J9 J CLEAN PROD JI J. Clean Prod. PD JUL 1 PY 2014 VL 74 BP 105 EP 118 DI 10.1016/j.jclepro.2014.03.065 PG 14 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental; Environmental Sciences SC Science & Technology - Other Topics; Engineering; Environmental Sciences & Ecology GA AJ6AV UT WOS:000337773000011 ER PT J AU English, JM Kay, JE Gettelman, A Liu, XH Wang, Y Zhang, YY Chepfer, H AF English, Jason M. Kay, Jennifer E. Gettelman, Andrew Liu, Xiaohong Wang, Yong Zhang, Yuying Chepfer, Helene TI Contributions of Clouds, Surface Albedos, and Mixed-Phase Ice Nucleation Schemes to Arctic Radiation Biases in CAM5 SO JOURNAL OF CLIMATE LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; GLOBAL CLIMATE MODEL; ENERGY SYSTEM CERES; STRATIFORM CLOUDS; PARAMETERIZATION; MICROPHYSICS; SIMULATIONS; INSTRUMENT; REPRESENTATION; DISTRIBUTIONS AB The Arctic radiation balance is strongly affected by clouds and surface albedo. Prior work has identified Arctic cloud liquid water path (LWP) and surface radiative flux biases in the Community Atmosphere Model, version 5 (CAMS), and reductions to these biases with improved mixed-phase ice nucleation schemes. Here, CAMS net top-of-atmosphere (TOA) Arctic radiative flux biases are quantified along with the contributions of clouds, surface albedos, and new mixed-phase ice nucleation schemes to these biases. CAMS net TOA all-sky shortwave (SW) and outgoing longwave radiation (OLR) fluxes are generally within 10W m(-2) of Clouds and the Earth's Radiant Energy System Energy Balanced and Filled (CERES-EBAF) observations. However, CAMS has compensating SW errors: Surface albedos over snow are too high while cloud amount and LWP are too low. Use of a new CAMS Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) lidar simulator that corrects an error in the treatment of snow crystal size confirms insufficient cloud amount in CAMS year-round. CAMS OLR is too low because of low surface temperature in winter, excessive atmospheric water vapor in summer, and excessive cloud heights year-round. Simulations with two new mixed-phase ice nucleation schemes-one based on an empirical fit to ice nuclei observations and one based on classical nucleation theory with prognostic ice nuclei improve surface climate in winter by increasing cloud amount and LWP. However, net TOA and surface radiation biases remain because of increases in midlevel clouds and a persistent deficit in cloud LWP. These findings highlight challenges with evaluating and modeling Arctic cloud, radiation, and climate processes. C1 [English, Jason M.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80303 USA. [Kay, Jennifer E.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80303 USA. [Gettelman, Andrew] Natl Ctr Atmospher Res, Earth Syst Lab, Boulder, CO 80307 USA. [Liu, Xiaohong; Wang, Yong] Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA. [Wang, Yong] Chinese Acad Sci, Inst Atmospher Phys, Beijing, Peoples R China. [Zhang, Yuying] Lawrence Livermore Natl Lab, Livermore, CA USA. [Chepfer, Helene] Univ Paris 06, LMD IPSL, Paris, France. RP English, JM (reprint author), Univ Colorado, Lab Atmospher & Space Phys, 3665 Discovery Dr,600 UCB, Boulder, CO 80303 USA. EM jayenglish@gmail.com RI Liu, Xiaohong/E-9304-2011; Zhang, Yuying/H-5011-2012; English, Jason/E-9365-2015; Kay, Jennifer/C-6042-2012 OI Liu, Xiaohong/0000-0002-3994-5955; English, Jason/0000-0001-9700-6860; FU NASA [NNX09AJ05G]; DOE Office of Science Atmospheric System Research (ASR) Program and Earth System Modeling Program; Earth System Modeling program of the U.S. Department of Energy; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX Support for J. M. English was provided by NASA Award NNX09AJ05G. Support for X. Liu was provided by the DOE Office of Science Atmospheric System Research (ASR) Program and Earth System Modeling Program. Support for Y. Zhang was provided by the Earth System Modeling program of the U.S. Department of Energy. Thanks to NOAA and Rutgers for snow-cover data and to Mark Flanner for providing them in a convenient format. Thanks to Gijs de Boer for providing SHEBA data in a convenient format, to David Bailey for insightful conversations regarding the sea ice model, to Dave Lawrence for insightful conversations regarding the land model, and to Neil Barton for providing new cloud plots using the new lidar code. Thanks to NASA and CNES for CALIOP and CERES data. The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. Work at LLNL was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 68 TC 13 Z9 13 U1 5 U2 44 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD JUL 1 PY 2014 VL 27 IS 13 BP 5174 EP 5197 DI 10.1175/JCLI-D-13-00608.1 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ8WG UT WOS:000337988200025 ER PT J AU Angleby, H Oskarsson, M Pang, JF Zhang, YP Leitner, T Braham, C Arvestad, L Lundeberg, J Webb, KM Savolainen, P AF Angleby, Helen Oskarsson, Mattias Pang, Junfeng Zhang, Ya-ping Leitner, Thomas Braham, Caitlyn Arvestad, Lars Lundeberg, Joakim Webb, Kristen M. Savolainen, Peter TI Forensic Informativity of similar to 3000bp of Coding Sequence of Domestic Dog mtDNA SO JOURNAL OF FORENSIC SCIENCES LA English DT Article DE forensic science; domestic dog; mitochondrial DNA; coding region; control region; exclusion capacity ID CANINE MICROSATELLITE POLYMORPHISMS; MITOCHONDRIAL GENOME; CONTROL REGION; WOLF HYBRIDIZATION; DNA; POPULATION; IDENTIFICATION; ORIGIN; HAIRS; AMPLIFICATION AB The discriminatory power of the noncoding control region (CR) of domestic dog mitochondrial DNA alone is relatively low. The extent to which the discriminatory power could be increased by analyzing additional highly variable coding regions of the mitochondrial genome (mtGenome) was therefore investigated. Genetic variability across the mtGenome was evaluated by phylogenetic analysis, and the three most variable similar to 1kb coding regions identified. We then sampled 100 Swedish dogs to represent breeds in accordance with their frequency in the Swedish population. A previously published dataset of 59 dog mtGenomes collected in the United States was also analyzed. Inclusion of the three coding regions increased the exclusion capacity considerably for the Swedish sample, from 0.920 for the CR alone to 0.964 for all four regions. The number of mtDNA types among all 159 dogs increased from 41 to 72, the four most frequent CR haplotypes being resolved into 22 different haplotypes. C1 [Angleby, Helen; Oskarsson, Mattias; Lundeberg, Joakim; Savolainen, Peter] KTH Royal Inst Technol, Sch Biotechnol, Div Gene Technol, Sci Life Lab, SE-17165 Solna, Sweden. [Pang, Junfeng; Zhang, Ya-ping] Chinese Acad Sci, Kunming Inst Zool, State Key Lab Genet Resources & Evolut, Kunming 650223, Yunnan, Peoples R China. [Leitner, Thomas] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Braham, Caitlyn; Webb, Kristen M.] Allegheny Coll, Dept Biol, Meadville, PA 16335 USA. [Arvestad, Lars] Stockholm Univ, Dept Numer Anal & Comp Sci, Swedish E Sci Res Ctr, SE-17121 Stockholm, Sweden. [Arvestad, Lars] KTH Royal Inst Technol, Sch Comp Sci & Commun, Dept Computat Biol, Sci Life Lab, SE-17165 Solna, Sweden. RP Webb, KM (reprint author), Allegheny Coll, Dept Biol, 520 North Main St,Box 10, Meadville, PA 16335 USA. EM kwebb@allegheny.edu RI Pang, Junfeng/I-9148-2014; OI Arvestad, Lars/0000-0001-5341-1733 FU Knut and Alice Wallenberg Foundation FX Co-author Peter Savolainen is a Royal Swedish Academy of Sciences Research Fellow supported by a grant from the Knut and Alice Wallenberg Foundation. NR 38 TC 1 Z9 1 U1 0 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-1198 EI 1556-4029 J9 J FORENSIC SCI JI J. Forensic Sci. PD JUL PY 2014 VL 59 IS 4 BP 898 EP 908 DI 10.1111/1556-4029.12504 PG 11 WC Medicine, Legal SC Legal Medicine GA AJ9NL UT WOS:000338038300003 PM 24814664 ER PT J AU Ekstrand, L Zhang, S Grieve, T Chumbley, LS Kreiser, MJ AF Ekstrand, Laura Zhang, Song Grieve, Taylor Chumbley, L. Scott Kreiser, M. James TI Virtual Tool Mark Generation for Efficient Striation Analysis SO JOURNAL OF FORENSIC SCIENCES LA English DT Article DE forensic science; tool mark comparison; computer simulation; screwdriver; statistics; striae AB This study introduces a tool mark analysis approach based upon 3D scans of screwdriver tip and marked plate surfaces at the micrometer scale from an optical microscope. An open-source 3D graphics software package is utilized to simulate the marking process as the projection of the tip's geometry in the direction of tool travel. The edge of this projection becomes a virtual tool mark that is compared to cross-sections of the marked plate geometry using the statistical likelihood algorithm introduced by Chumbley etal. In a study with both sides of six screwdriver tips and 34 corresponding marks, the method distinguished known matches from known nonmatches with zero false-positive matches and two false-negative matches. For matches, it could predict the correct marking angle within +/- 5-10 degrees. Individual comparisons could be made in seconds on a desktop computer, suggesting that the method could save time for examiners. C1 [Ekstrand, Laura; Zhang, Song; Grieve, Taylor; Chumbley, L. Scott] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Zhang, S (reprint author), Iowa State Univ, Dept Mech Engn, 2096 Black Engn, Ames, IA 50011 USA. EM song@iastate.edu RI Zhang, Song/C-5294-2012 OI Zhang, Song/0000-0001-8452-4837 FU National Institute of Justice [2009-DN-R-119]; U.S. Department of Energy [DE-AC02-07CH11358] FX Supported by Award No. 2009-DN-R-119 from the National Institute of Justice and performed at the Ames Laboratory, which is operated by Iowa State University under contract number DE-AC02-07CH11358 with the U.S. Department of Energy. NR 10 TC 4 Z9 4 U1 0 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-1198 EI 1556-4029 J9 J FORENSIC SCI JI J. Forensic Sci. PD JUL PY 2014 VL 59 IS 4 BP 950 EP 959 DI 10.1111/1556-4029.12435 PG 10 WC Medicine, Legal SC Legal Medicine GA AJ9NL UT WOS:000338038300009 PM 24502818 ER PT J AU McClintock, DA Vevera, BJ Riemer, BW Gallmeier, FX Hyres, JW Ferguson, PD AF McClintock, David A. Vevera, Bradley J. Riemer, Bernard W. Gallmeier, Franz X. Hyres, James W. Ferguson, Phillip D. TI Post-irradiation tensile properties of the first and second operational target modules at the Spallation Neutron Source SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID SOURCE MERCURY TARGET; AUSTENITIC STAINLESS-STEELS; RESEARCH-AND-DEVELOPMENT; MECHANICAL-PROPERTIES; CONTAINER MATERIALS; PROTON; IRRADIATION; SNS; DEFORMATION; WAVES AB During neutron production the target module at the Spallation Neutron Source (SNS) is damaged by cavitation-induced erosion and the mechanical properties of the AISI 316L vessel material are altered by high-energy proton and neutron. radiation. Recently the first and second operational target modules at the SNS reached the end of their useful lifetime, and disk shaped specimens were sampled from the beam entrance region of both targets. Tensile specimens ranging in dose from 3 to 7 displacements per atom (dpa) were fabricated from the disk specimens using wire electrical discharge machining and tested at room temperature. This paper presents the tensile properties of the irradiated 316L vessel material removed from the first and second operational SNS target modules. Results show an increase in tensile strength and decrease in elongation values similar to previous spallation irradiated 316L results. Abnormally large elongation, 57% total elongation, was observed in a specimen irradiated to 5.4 dpa and considerable scatter was observed in the uniform and total elongation data. One possible explanation for the abnormally large elongations and scatter observed in tensile test results is the so-called deformation wave phase transformation-induced plasticity effect. Microscopy characterization revealed the presence of large nonmetallic inclusions rich in Al, S, Ca, O, and Mg on the fracture surface, which may have also contributed to the scatter in the tensile elongation results. While all specimens exhibited radiation-induced hardening and a decrease in ductility, the predominate topographical morphology on all specimen fracture surfaces examined was ductile microvoid coalescence and all specimens experienced appreciable necking prior to fracture. These findings indicate that 316L retains sufficient ductility (10-20% total elongation) and fractures in a ductile manor after irradiation to approximately 6-7 dpa in the mixed proton/neutron radiation environment at the SNS. (C) 2014 Elsevier B.V. All rights reserved. C1 [McClintock, David A.; Riemer, Bernard W.; Gallmeier, Franz X.; Ferguson, Phillip D.] Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. [Vevera, Bradley J.; Hyres, James W.] Babcock & Wilcox Tech Serv Grp Inc, Lynchburg, VA USA. RP McClintock, DA (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, POB 2008,Bldg 8600,MS 6476, Oak Ridge, TN 37831 USA. EM mcclintockda@oml.gov OI Ferguson, Phillip/0000-0002-7661-4223; McClintock, David/0000-0002-9292-8951; Riemer, Bernard/0000-0002-6922-3056 FU Office of Science, U.S. Department of Energy; UT-Battelle, LLC for the U.S. Department of Energy [DE-AC05-00OR22725] FX The authors would like to thank Justin Carmichael for assistance with figures presented in this paper. The SNS is sponsored by the Office of Science, U.S. Department of Energy, and managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 26 TC 2 Z9 2 U1 0 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 130 EP 140 DI 10.1016/j.jnucmat.2014.02.037 PG 11 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600021 ER PT J AU Vevera, BJ McClintock, DA Hyres, JW Riemer, BW AF Vevera, Bradley J. McClintock, David A. Hyres, James W. Riemer, Bernard W. TI Characterization of irradiated AISI 316L stainless steel disks removed from the Spallation Neutron Source SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID TARGET; SNS AB Disk-shaped samples were removed from the first and second operational target modules at the Spallation Neutron Source for post-irradiation examination to assess the extent of radiation-induced changes in mechanical properties and the amount of cavitation-induced erosion to the AISI 316L stainless steel target vessel. Characterization techniques performed include: high-resolution photography of the disk specimens, ultrasonic cleaning to remove mercury residue and surface oxides, surface profile mapping of cavitation pits using high frequency ultrasonic testing, high-resolution surface replication, and scanning electron microscopy accompanied by energy dispersive spectroscopy. The target disk samples were machined using wire electrical discharge machining to produce microstructural and mechanical test specimens for tensile testing, Rockwell Superficial hardness testing, and Vickers microhardness testing. The effectiveness of the cleaning procedure was evident in the pre- and post-cleaning photography, and provided accurate photographs of areas on each disk that facilitated the creation of detailed machining maps. Due to the limited amount of material available and the unique geometry of the disks, test specimen design and development of fixturing for machining operations were critical aspects of this work; multiple designs were considered and refined during mock-up testing on unirradiated disks. The techniques used to successfully machine and test the various specimens will be presented along with a summary of important findings from the laboratory characterizations. (C) 2014 Elsevier B.V. All rights reserved. C1 [Vevera, Bradley J.; Hyres, James W.] Babcock & Wilcox Tech Serv Grp Inc, Lynchburg, VA USA. [McClintock, David A.; Riemer, Bernard W.] Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. RP McClintock, DA (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, POB 2008,Bldg 8600,MS 6466, Oak Ridge, TN 37831 USA. EM mcclintockda@ornl.gov OI McClintock, David/0000-0002-9292-8951; Riemer, Bernard/0000-0002-6922-3056 FU Office of Science, U.S. Department of Energy; UT-Battelle, LLC for the U.S. Department of Energy [DE-AC05-00OR22725] FX The SNS is sponsored by the Office of Science, U.S. Department of Energy, and managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 8 TC 2 Z9 2 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 147 EP 162 DI 10.1016/j.jnucmat.2014.02.035 PG 16 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600023 ER PT J AU McClintock, DA Janney, JG Parish, CM AF McClintock, David A. Janney, Jim G. Parish, Chad M. TI Characterization of an explosively bonded aluminum proton beam window for the Spallation Neutron Source SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID MECHANICAL-PROPERTIES; TENSILE PROPERTIES; STEEL; IRRADIATION; ALLOY; MICROSTRUCTURE; ENVIRONMENT; PLATES; FLOW AB effort is underway at the Spallation Neutron Source (SNS) to redesign the 1st Generation high-nickel alloy proton beam window (PEW) to a 2nd Generation design that utilizes aluminum for the window material. One of the key challenges to implementation of an aluminum PBW at the SNS was selection of an appropriate joining method to bond an aluminum window to the stainless steel shielding structure of the PBW assembly. An explosively formed bond was selected as the most promising joining method for the aluminum PBW design and a testing campaign was conducted to evaluate the strength and efficacy of explosively formed bonds that were produced using two different interlayer materials: niobium and titanium. The characterization methods reported here include tensile testing, thermal-shock leak testing, optical microscopy, and advanced scanning electron microscopy. All tensile specimens examined failed in an aluminum interlayer and measured tensile strengths were all slightly greater than the native properties of the aluminum interlayer, while elongation values were all slightly lower. A leak developed in the test vessel with an niobium interlayer after repeated thermal-shock cycles, which was attributed to an extensive crack network that formed in an interfacial layer of a niobium-rich constituent phase located on the bond interfaces of the niobium interlayer; the test vessel with a titanium interlayer did not develop a leak under the conditions tested. Due to the experience gained from these characterizations, an explosively formed bond with a titanium interlayer was selected for the aluminum PEW design at the SNS. (C) 2014 Elsevier B.V. All rights reserved. C1 [McClintock, David A.; Janney, Jim G.] Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. [Parish, Chad M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP McClintock, DA (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, POB 2008,Bldg 8600,MS 6466, Oak Ridge, TN 37831 USA. EM mcclintockda@ornl.gov RI Parish, Chad/J-8381-2013; OI McClintock, David/0000-0002-9292-8951 FU Office of Science, U.S. Department of Energy; UT-Battelle, LLC for the U.S. Department of Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program; Office of Basic Energy Sciences, U.S. Department of Energy FX The SNS is sponsored by the Office of Science, U.S. Department of Energy, and managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725.; Research sponsored by Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program, which is sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy. NR 28 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 163 EP 175 DI 10.1016/j.jnucmat.2014.02.016 PG 13 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600024 ER PT J AU McClintock, DA Hyres, JW Vevera, BJ AF McClintock, David A. Hyres, James W. Vevera, Bradley J. TI Hardness and stability of a carburized surface layer on AISI 316L stainless steel after irradiation in a spallation neutron environment SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID SNS TARGET TESTS; CAVITATION-EROSION; MERCURY TARGET; LANSCE-WNR; PRESSURE WAVES; DAMAGE; RESISTANCE; VESSELS; POWER AB The inner surfaces of mercury target vessels at the Spallation Neutron Source (SNS) experience material erosion caused by proton-beam induced cavitation of the liquid mercury. One approach developed and deployed to inhibit erosion of the target vessel material was surface hardening via a proprietary low-temperature carburization treatment, called Kolsterising, to the target surfaces most susceptible to cavitation-induced erosion. Previous testing has shown that the hardened surface produced by the Kolsterising treatment can delay the onset of erosion and inhibit erosion once initiated. But the stability of the carbon atmosphere in the treated surface layer after radiation to doses prototypic to the SNS target was unknown. Therefore, as part of the target Post Irradiation Examination program at the SNS, optical microscopy and microhardness testing were performed on material sampled from the first and second operational SNS target vessels. Optical micrographs contained no noticeable precipitation in the supersaturated carbon layer extending into the base material and several micrographs contained evidence of a proposed mechanism for mass wastage from the vessel surface. The hardened layer was characterized using Vickers microhardness testing and results show that the shape of hardness profile of the treated layer corresponded well with known pre-irradiation hardness values, though the microhardness results show some hardening occurred during irradiation. The results suggest that the hardened surface layer produced by the Kolsterising treatment is stable at the operational temperatures and dose levels experienced by the first and second operational SNS target modules. (C) 2014 Elsevier B.V. All rights reserved. C1 [McClintock, David A.] Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. [Hyres, James W.; Vevera, Bradley J.] Babcock & Wilcox Tech Serv Grp Inc, Lynchburg, VA USA. RP McClintock, DA (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, POB 2008,Bldg 8600,MS 6476, Oak Ridge, TN 37831 USA. EM mcclintockda@ornl.gov OI McClintock, David/0000-0002-9292-8951 FU Office of Science, U.S. Department of Energy; UT-Battelle, LLC for the U.S. Department of Energy [DE-AC05-00OR22725] FX The authors would like to thank Genevieve Martin for her assistance with figures presented in this paper. The SNS is sponsored by the Office of Science, U.S. Department of Energy, and managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 15 TC 1 Z9 1 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 176 EP 182 DI 10.1016/j.jnucmat.2014.01.005 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600025 ER PT J AU Riemer, BW McClintock, DA Kaminskas, S Abdou, AA AF Riemer, B. W. McClintock, D. A. Kaminskas, S. Abdou, A. A. TI Correlation between simulations and cavitation-induced erosion damage in Spallation Neutron Source target modules after operation SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID VESSELS AB An explicit finite element (FE) technique developed for estimating dynamic strain in the Spallation Neutron Source (SNS) mercury target module vessel is now providing insight into cavitation-induced erosion patterns observed on interior surfaces of SNS targets during post-irradiation examination. The technique uses an empirically developed material model for the mercury that describes its volumetric stiffness combined with a tensile pressure cut-off limit to approximate the threshold and effect of cavitation. The longest period each point in the mercury is at the tensile cut-off threshold is denoted as "saturation time". Patterns of saturation time can be obtained from the FE simulations and are being positively correlated with observed damage patterns as a qualitative measure of damage potential. Saturation time has been advocated by collaborators at the Japan Proton Accelerator Research Complex (J-PARC) as a factor in predicting bubble nuclei growth and collapse intensity. Larger ratios of maximum bubble-size-to-nucleus result in greater bubble collapse intensity; longer saturation times correlate to greater ratios. With the recent development of a user subroutine for the FE solver, saturation time is now provided over the entire mercury domain. Saturation time contour maps agree with patterns of damage seen on the SNS inner vessel beam window and elsewhere. The other simulation result which seems to correlate with observed damage patterns is the local mercury velocity. Related R&D has provided evidence that damage is mitigated by flow velocity. Surfaces which are near regions of low mercury velocity appear to be more vulnerable to damage than those where the mercury flow is strong and sustained. By combining the patterns of saturation time and velocity a viable explanation for observed damage patterns is presented. (C) 2013 Elsevier B.V. All rights reserved. C1 [Riemer, B. W.; McClintock, D. A.; Kaminskas, S.; Abdou, A. A.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Riemer, BW (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, POB 2008,Bldg 8600,MS 6476, Oak Ridge, TN 37831 USA. EM riemerbw@ornl.gov OI McClintock, David/0000-0002-9292-8951; Riemer, Bernard/0000-0002-6922-3056 NR 14 TC 2 Z9 2 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 183 EP 191 DI 10.1016/j.jnucmat.2013.10.057 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600026 ER PT J AU Riemer, BW Wendel, MW Felde, DK Sangrey, RL Abdou, A West, DL Shea, TJ Hasegawa, S Kogawa, H Naoe, T Farny, CH Kaminsky, AL AF Riemer, B. W. Wendel, M. W. Felde, D. K. Sangrey, R. L. Abdou, A. West, D. L. Shea, T. J. Hasegawa, S. Kogawa, H. Naoe, T. Farny, C. H. Kaminsky, A. L. TI Small gas bubble experiment for mitigation of cavitation damage and pressure waves in short-pulse mercury spallation targets SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID VESSELS AB Populations of small helium gas bubbles were introduced into a flowing mercury experiment test loop to evaluate mitigation of beam-pulse induced cavitation damage and pressure waves. The test loop was developed and thoroughly tested at the Spallation Neutron Source (SNS) prior to irradiations at the Los Alamos Neutron Science Center-Weapons Neutron Research (LANSCE-WNR) facility. Twelve candidate bubblers were evaluated over a range of mercury flow and gas injection rates by use of a novel optical measurement technique that accurately assessed the generated small bubble size distributions. Final selection for irradiation testing included two variations of a swirl bubbler provided by Japan Proton Accelerator Research Complex (j-PARC) collaborators and one orifice bubbler developed at SNS. Bubble populations of interest consisted of sizes up to 150 pm in radius with achieved gas volume fractions in the 10(-5)-10(-4) range. The nominal WNR beam pulse used for the experiment created energy deposition in the mercury comparable to SNS pulses operating at 2.5 MW. Nineteen test conditions were completed each with 100 pulses, including variations on mercury flow, gas injection and protons per pulse. The principal measure of cavitation damage mitigation was pitting damage assessment on test specimens that were manually replaced for each test condition. Damage assessment was done after radiation decay and decontamination by optical and laser profiling microscopy with damaged area fraction and maximum pit depth being the more valued results. Damage was reduced by flow alone; the best mitigation from bubble injection was to one-third that of stagnant mercury. Other data collected included surface motion tracking by three Laser Doppler Vibrometers (LDV), test loop wall dynamic strain, beam diagnostics for charge and beam profile assessment, embedded hydrophones and pressure sensors, and sound measurement by a suite of conventional and contact microphones. (C) 2013 Elsevier B.V. All rights reserved. C1 [Riemer, B. W.; Wendel, M. W.; Felde, D. K.; Sangrey, R. L.; Abdou, A.; West, D. L.; Shea, T. J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hasegawa, S.; Kogawa, H.; Naoe, T.] Japan Atom Energy Agcy, Tokai, Ibaraki 3191195, Japan. [Farny, C. H.] Boston Univ, Dept Mech Engn, Boston, MA 02215 USA. [Kaminsky, A. L.] Univ Tennessee, Knoxville, TN 37996 USA. RP Riemer, BW (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM riemerbw@ornl.gov RI West, David/A-3414-2009; OI West, David/0000-0002-1265-9350; Riemer, Bernard/0000-0002-6922-3056 FU US Department of Energy FX This work has benefited from the use of the Los Alamos Neutron Science Center at the Los Alamos National Laboratory. This facility is funded by the US Department of Energy. NR 15 TC 3 Z9 3 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 192 EP 203 DI 10.1016/j.Mucmat.2013.10.011 PG 12 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600027 ER PT J AU Marino, A Lim, J Keijers, S Van den Bosch, J Deconinck, J Rubio, F Woloshun, K Caro, M Maloy, SA AF Marino, A. Lim, J. Keijers, S. Van den Bosch, J. Deconinck, J. Rubio, F. Woloshun, K. Caro, M. Maloy, S. A. TI Temperature dependence of dissolution rate of a lead oxide mass exchanger in lead-bismuth eutectic SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 11th International Workshop on Spallation MaterialsTechnology (IWSMT-11) CY NOV 04-09, 2012 CL Ghent, BELGIUM ID TO-FLUID MASS; OXYGEN; SYSTEMS; COOLANT; LBE AB A Computational Fluid Dynamic (CFD) model of a lead oxide mass exchanger (MO MX) was developed. The mass exchanger consisted of a packed bed of PbO spheres. The geometry was created using Discrete Elements Method (DEM) software while the meshing, the solving and the post-processing were done by the commercial CFD package CFX. The dissolution process was modeled by implementing in the code oxygen mass transfer through the boundary layer. The dissolution rate was then predicted for different temperatures. Experiments were also performed at the LBE material test loop known as the DELTA loop. Oxygen concentration at the outlet of the PbO MX was measured for different conditions using a potentiometric oxygen sensor and the dissolution rate was determined for five different temperatures. The experimental data were compared with the numerical model. The temperature dependence of the dissolution rate was then determined in terms of Sherwood number by fitting the simulation results while keeping constant Reynolds number. The results showed that the Sherwood number for PbO MX in flowing LBE varies with Sc-0.323. (C) 2014 Elsevier B.V. All rights reserved. C1 [Marino, A.; Lim, J.; Keijers, S.; Van den Bosch, J.] SCK CEN, B-2400 Mol, Belgium. [Marino, A.; Deconinck, J.] Vrije Univ Brussel, B-1050 Elsene, Belgium. [Rubio, F.; Woloshun, K.; Caro, M.; Maloy, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Marino, A (reprint author), SCK CEN, Nucl Syst Res Conditioning & Chem Programme, Boeretang 200, B-2400 Mol, Belgium. EM amarino@sckcen.be RI Maloy, Stuart/A-8672-2009 OI Maloy, Stuart/0000-0001-8037-1319 FU US DOE-NE program on Advanced Small Modular Reactor Development FX The research at the DELTA loop was supported by the US DOE-NE program on Advanced Small Modular Reactor Development. The technical assistance of Frank Romero and Kenneth Hurtle is greatly appreciated. We also thank Simon Vanmaercke for his contribution on DEM. NR 17 TC 4 Z9 4 U1 1 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD JUL PY 2014 VL 450 IS 1-3 BP 270 EP 277 DI 10.1016/j.jnucmat.2013.12.023 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA AJ7FM UT WOS:000337862600036 ER PT J AU Sugita, T Bacon, J Ban, Y Borozdin, K Izumi, M Karino, Y Kume, N Miyadera, H Mizokami, S Morris, CL Nakayama, K Otsuka, Y Perry, JO Ramsey, J Sano, Y Yamada, D Yoshida, N Yoshioka, K AF Sugita, Tsukasa Bacon, Jeffery Ban, Yuichiro Borozdin, Konstantin Izumi, Mikio Karino, Yoshiji Kume, Naoto Miyadera, Haruo Mizokami, Shinya Morris, Christopher L. Nakayama, Kohichi Otsuka, Yasuyuki Perry, John O. Ramsey, John Sano, Yuji Yamada, Daichi Yoshida, Noriyuki Yoshioka, Kenichi TI Cosmic-ray muon radiography of UO2 fuel assembly SO JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY LA English DT Article DE fuel assembly; MonteCarlo; decommissioning; muon radiography; cosmic-ray muon; Geant4; NCA ID INNER-STRUCTURE AB A technical demonstration of cosmic-ray muon radiography of a UO2 fuel assembly was performed at Toshiba Nuclear Critical Assembly (NCA). The fuel assembly in the NCA was imaged through obstacles such as steel and concrete. The result suggested that the method can be applicable to assess the damage to the reactors at the Fukushima Daiichi nuclear power plant. Here, both scattering and displacement methods are presented, and the results are shown to agree with Monte Carlo simulations. In addition, detailed Monte Carlo simulations of the Fukushima Daiichi reactor were performed, which showed capability of muon radiography to locate the fuel in the damaged reactors. C1 [Sugita, Tsukasa; Yoshioka, Kenichi] Toshiba Co Ltd, Kawasaki, Kanagawa 2100862, Japan. [Ban, Yuichiro; Izumi, Mikio; Karino, Yoshiji; Kume, Naoto; Miyadera, Haruo; Nakayama, Kohichi; Sano, Yuji; Yoshida, Noriyuki] Toshiba Co Ltd, Isogo Ku, Yokohama, Kanagawa 2358523, Japan. [Bacon, Jeffery; Borozdin, Konstantin; Morris, Christopher L.; Perry, John O.; Ramsey, John] Los Alamos Natl Lab, Subat Phys Grp, Los Alamos, NM 87545 USA. [Mizokami, Shinya; Otsuka, Yasuyuki; Yamada, Daichi] Tokyo Elect Power Co Ltd, Chiyoda Ku, Tokyo 1008560, Japan. RP Miyadera, H (reprint author), Toshiba Co Ltd, Isogo Ku, 8 Shinsugita Cho, Yokohama, Kanagawa 2358523, Japan. EM haruo.miyadera@toshiba.co.jp OI Morris, Christopher/0000-0003-2141-0255; Perry, John/0000-0003-3639-5617 FU Tokyo Electric Power Company; Toshiba Corporation FX We thank staffs at Toshiba NCA for their support during the reactor imaging demonstration. This work has been supported by Tokyo Electric Power Company and by Toshiba Corporation. NR 15 TC 6 Z9 6 U1 0 U2 7 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0022-3131 EI 1881-1248 J9 J NUCL SCI TECHNOL JI J. Nucl. Sci. Technol. PD JUL-AUG PY 2014 VL 51 IS 7-8 SI SI BP 1024 EP 1031 DI 10.1080/00223131.2014.919884 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ8OQ UT WOS:000337966000017 ER PT J AU Edman, JP Romps, DM AF Edman, Jacob P. Romps, David M. TI An Improved Weak Pressure Gradient Scheme for Single-Column Modeling SO JOURNAL OF THE ATMOSPHERIC SCIENCES LA English DT Article ID CLOUD-RESOLVING MODEL; GRAVITY-WAVES; APPROXIMATION; CONVECTION; INSTABILITY; TROPOSPHERE AB A new formulation of the weak pressure gradient approximation (WPG) is introduced for parameterizing large-scale dynamics in limited-domain atmospheric models. This new WPG is developed in the context of the one-dimensional, linearized, damped, shallow-water equations and then extended to Boussinesq and compressible fluids. Unlike previous supradomain-scale parameterizations, this formulation of WPG correctly reproduces both steady-state solutions and first baroclinic gravity waves. In so doing, this scheme eliminates the undesirable gravity wave resonance in previous versions of WPG. In addition, this scheme can be extended to accurately model the emission of gravity waves with arbitrary vertical wavenumber. C1 [Edman, Jacob P.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Edman, JP (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, 449 McCone Hall, Berkeley, CA 94720 USA. EM jedman@berkeley.edu RI Romps, David/F-8285-2011; Edman, Jacob/J-5522-2014 OI Edman, Jacob/0000-0001-9130-7128 FU U.S. Department of Energy's Earth System Modeling, an Office of Science, Office of Biological and Environmental Research program [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy's Earth System Modeling, an Office of Science, Office of Biological and Environmental Research program under Contract DE-AC02-05CH11231. Thanks are due to Adam Sobel, David Raymond, and an anonymous reviewer for their helpful suggestions that improved this paper. NR 25 TC 7 Z9 7 U1 0 U2 5 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0022-4928 EI 1520-0469 J9 J ATMOS SCI JI J. Atmos. Sci. PD JUL PY 2014 VL 71 IS 7 BP 2415 EP 2429 DI 10.1175/JAS-D-13-0327.1 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ7ZF UT WOS:000337920200008 ER PT J AU Zhou, BW Simon, JS Chow, FK AF Zhou, Bowen Simon, Jason S. Chow, Fotini K. TI The Convective Boundary Layer in the Terra Incognita SO JOURNAL OF THE ATMOSPHERIC SCIENCES LA English DT Article ID LARGE-EDDY-SIMULATION; NONHYDROSTATIC ATMOSPHERIC SIMULATION; PREDICTION SYSTEM ARPS; VERTICAL DIFFUSION; MODEL; INSTABILITY; RESOLUTION; DYNAMICS; FLOW AB Numerical simulations of a convective boundary layer (CBL) are performed to investigate model behavior in the terra incognita, also known as the gray zone. The terra incognita of the CBL refers to a range of model grid spacing that is comparable to the size of the most energetic convective eddies, which are on the order of the boundary layer depth. Using the Rayleigh-Benard thermal instability as reference, a set of idealized simulations is used to show that gray zone modeling is not only a numerical challenge, but also poses dynamical difficulties. When the grid spacing falls within the CBL gray zone, grid-dependent convection can occur. The size of the initial instability structures is set by the grid spacing rather than the natural state of the flow. This changes higher-order flow statistics and poses fundamental difficulties for gray zone modeling applications. C1 [Zhou, Bowen] Nanjing Univ, MOE, Key Lab Mesoscale Severe Weather, Nanjing 210008, Jiangsu, Peoples R China. [Zhou, Bowen] Nanjing Univ, Sch Atmospher Sci, Nanjing 210008, Jiangsu, Peoples R China. [Zhou, Bowen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Simon, Jason S.; Chow, Fotini K.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. RP Chow, FK (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, 621 Davis Hall, Berkeley, CA 94720 USA. EM tinakc@berkeley.edu FU National Science Foundation [ATM-0645784, OCI-1053575] FX We gratefully acknowledge the comments and suggestions on the manuscript from Prof. Bob Street. We also thank Prof. David Romps for insightful discussions. We are grateful for the support from National Science Foundation Grant ATM-0645784 (Physical and Dynamic Meteorology Program). This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant OCI-1053575. NR 41 TC 16 Z9 16 U1 2 U2 14 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0022-4928 EI 1520-0469 J9 J ATMOS SCI JI J. Atmos. Sci. PD JUL PY 2014 VL 71 IS 7 BP 2545 EP 2563 DI 10.1175/JAS-D-13-0356.1 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ7ZF UT WOS:000337920200016 ER PT J AU Latch, EK Reding, DM Heffelfinger, JR Alcala-Galvan, CH Rhodes, OE AF Latch, Emily K. Reding, Dawn M. Heffelfinger, James R. Alcala-Galvan, Carlos H. Rhodes, Olin E. TI Range-wide analysis of genetic structure in a widespread, highly mobile species (Odocoileus hemionus) reveals the importance of historical biogeography SO MOLECULAR ECOLOGY LA English DT Review DE gene flow; isolation by distance; landscape genetics; Odocoileus hemionus; phylogeography; spatial genetic structure ID WHITE-TAILED DEER; MULTILOCUS GENOTYPE DATA; WESTERN NORTH-AMERICA; MULE DEER; POPULATION-STRUCTURE; MITOCHONDRIAL-DNA; INTROGRESSIVE HYBRIDIZATION; EVOLUTIONARY HISTORY; LANDSCAPE GENETICS; PLANT-POPULATIONS AB Highly mobile species that thrive in a wide range of habitats are expected to show little genetic differentiation across their range. A limited but growing number of studies have revealed that patterns of broad-scale genetic differentiation can and do emerge in vagile, continuously distributed species. However, these patterns are complex and often shaped by both historical and ecological factors. Comprehensive surveys of genetic variation at a broad scale and at high resolution are useful for detecting cryptic spatial genetic structure and for investigating the relative roles of historical and ecological processes in structuring widespread, highly mobile species. In this study, we analysed 10 microsatellite loci from over 1900 samples collected across the full range of mule deer (Odocoileus hemionus), one of the most widely distributed and abundant of all large mammal species in North America. Through both individual- and population-based analyses, we found evidence for three main genetic lineages, one corresponding to the mule deer' morphological type and two to the black-tailed deer' type. Historical biogeographic events likely are the primary drivers of genetic divergence in this species; boundaries of the three lineages correspond well with predictions based on Pleistocene glacial cycles, and substructure within each lineage demonstrates island vicariance. However, across large geographic areas, including the entire mule deer lineage, we found that genetic variation fit an isolation-by-distance pattern rather than discrete clusters. A lack of genetic structure across wide geographic areas of the continental west indicates that ecological processes have not resulted in restrictions to gene flow sufficient for spatial genetic structure to emerge. Our results have important implications for our understanding of evolutionary mechanisms of divergence, as well as for taxonomy, conservation and management. C1 [Latch, Emily K.] Univ Wisconsin, Behav & Mol Ecol Res Grp, Dept Biol Sci, Milwaukee, WI 53211 USA. [Reding, Dawn M.] Luther Coll, Dept Biol, Decorah, IA 52101 USA. [Reding, Dawn M.] Iowa State Univ, Dept Ecol Evolut & Organismal Biol, Ames, IA 50011 USA. [Heffelfinger, James R.] Arizona Game & Fish Dept, Tucson, AZ 85745 USA. [Alcala-Galvan, Carlos H.] DICTUS Univ Sonora, Hermosillo 83100, Sonora, Mexico. [Rhodes, Olin E.] Savannah River Ecol Lab, Aiken, SC 29802 USA. RP Latch, EK (reprint author), Univ Wisconsin, Behav & Mol Ecol Res Grp, Dept Biol Sci, 3209 N Maryland Ave, Milwaukee, WI 53211 USA. EM latch@uwm.edu FU Boone Crockett Club; Pope and Young Club; Campfire Conservation Fund of the Camp Fire Club; National Fish and Wildlife Foundation; University of Wisconsin-Milwaukee; Purdue University; University of Arizona; Arizona Game and Fish Department; California Deer Association; Dallas Safari Club; Safari Club International (National and Seattle Chapter) FX We appreciate the support provided by the Boone & Crockett Club, Pope and Young Club, Campfire Conservation Fund of the Camp Fire Club, National Fish and Wildlife Foundation, University of Wisconsin-Milwaukee, Purdue University, University of Arizona, Arizona Game and Fish Department, California Deer Association, Dallas Safari Club, Safari Club International (National and Seattle Chapter), Eldon 'Buck' Buckner, James deVos, Scott Fitkin, Richard Green, Jeff Gronauer, Winifred Kessler, Paul Krausman, Mike Schlegel and Don Whittaker. Samples from the entire range were collected by more than 150 volunteers, which, regrettably, are too numerous to mention individually. Francisco Abarca was instrumental in helping with international coordination. We appreciate helpful comments provided by Lisette Waits and anonymous reviewers on an earlier draft of the manuscript. NR 104 TC 10 Z9 10 U1 9 U2 87 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0962-1083 EI 1365-294X J9 MOL ECOL JI Mol. Ecol. PD JUL PY 2014 VL 23 IS 13 BP 3171 EP 3190 DI 10.1111/mec.12803 PG 20 WC Biochemistry & Molecular Biology; Ecology; Evolutionary Biology SC Biochemistry & Molecular Biology; Environmental Sciences & Ecology; Evolutionary Biology GA AJ9GE UT WOS:000338014900005 PM 24863151 ER PT J AU Bonito, G Reynolds, H Robeson, MS Nelson, J Hodkinson, BP Tuskan, G Schadt, CW Vilgalys, R AF Bonito, Gregory Reynolds, Hannah Robeson, Michael S. Nelson, Jessica Hodkinson, Brendan P. Tuskan, Gerald Schadt, Christopher W. Vilgalys, Rytas TI Plant host and soil origin influence fungal and bacterial assemblages in the roots of woody plants SO MOLECULAR ECOLOGY LA English DT Article DE 454 pyrosequencing; bacterial communities; fungal communities; Glomeromycota; phylotyping; Pinus; Populus; Quercus; root endophytes ID ARBUSCULAR MYCORRHIZAL FUNGI; ECTOMYCORRHIZAL FUNGI; MICROBIAL COMMUNITIES; ROCKY-MOUNTAINS; POPULUS; DIVERSITY; IDENTIFICATION; FOREST; ASPEN; RHIZOSPHERE AB Microbial communities in plant roots provide critical links between above- and belowground processes in terrestrial ecosystems. Variation in root communities has been attributed to plant host effects and microbial host preferences, as well as to factors pertaining to soil conditions, microbial biogeography and the presence of viable microbial propagules. To address hypotheses regarding the influence of plant host and soil biogeography on root fungal and bacterial communities, we designed a trap-plant bioassay experiment. Replicate Populus, Quercus and Pinus plants were grown in three soils originating from alternate field sites. Fungal and bacterial community profiles in the root of each replicate were assessed through multiplex 454 amplicon sequencing of four loci (i.e., 16S, SSU, ITS, LSU rDNA). Soil origin had a larger effect on fungal community composition than did host species, but the opposite was true for bacterial communities. Populus hosted the highest diversity of rhizospheric fungi and bacteria. Root communities on Quercus and Pinus were more similar to each other than to Populus. Overall, fungal root symbionts appear to be more constrained by dispersal and biogeography than by host availability. C1 [Bonito, Gregory] Royal Bot Gardens, Melbourne, Vic 3141, Australia. [Bonito, Gregory; Reynolds, Hannah; Nelson, Jessica; Hodkinson, Brendan P.; Vilgalys, Rytas] Duke Univ, Dept Biol, Durham, NC 27708 USA. [Robeson, Michael S.; Tuskan, Gerald; Schadt, Christopher W.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Bonito, G (reprint author), Royal Bot Gardens, Melbourne, Vic 3141, Australia. EM Gregory.Bonito@rbg.vic.gov.au RI Schadt, Christopher/B-7143-2008; Tuskan, Gerald/A-6225-2011; OI Schadt, Christopher/0000-0001-8759-2448; Tuskan, Gerald/0000-0003-0106-1289; Robeson, Michael/0000-0001-7119-6301; Vilgalys, Rytas/0000-0001-8299-3605 FU Genomic Science Program, U.S. Department of Energy, Office of Science - Biological and Environmental Research as part of the Plant Microbe Interfaces Scientific Focus Area; National Science Foundation [EF-0832858, DEB-1011504, DEB-1145511]; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the Genomic Science Program, U.S. Department of Energy, Office of Science - Biological and Environmental Research as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Support for B.P.H. was provided in part by the National Science Foundation under awards EF-0832858, DEB-1011504 and DEB-1145511. We thank Lee Gunter, Jud Isebrands, Zachary Moore, Paul Bloese and Bernard McMahon for supplying Populus cuttings, Joshua Steiger and Steve Mckeand from the NC State University's Forest Improvement Center for pine seed, Anthony Amend for helpful discussions regarding 454 primer design, and Victor Bonito for advice on ecological community statistics. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 76 TC 28 Z9 29 U1 7 U2 153 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0962-1083 EI 1365-294X J9 MOL ECOL JI Mol. Ecol. PD JUL PY 2014 VL 23 IS 13 BP 3356 EP 3370 DI 10.1111/mec.12821 PG 15 WC Biochemistry & Molecular Biology; Ecology; Evolutionary Biology SC Biochemistry & Molecular Biology; Environmental Sciences & Ecology; Evolutionary Biology GA AJ9GE UT WOS:000338014900017 PM 24894495 ER PT J AU Schmutz, J McClean, PE Mamidi, S Wu, GA Cannon, SB Grimwood, J Jenkins, J Shu, SQ Song, QJ Chavarro, C Torres-Torres, M Geffroy, V Moghaddam, SM Gao, DY Abernathy, B Barry, K Blair, M Brick, MA Chovatia, M Gepts, P Goodstein, DM Gonzales, M Hellsten, U Hyten, DL Jia, GF Kelly, JD Kudrna, D Lee, R Richard, MMS Miklas, PN Osorno, JM Rodrigues, J Thareau, V Urrea, CA Wang, M Yu, Y Zhang, M Wing, RA Cregan, PB Rokhsar, DS Jackson, SA AF Schmutz, Jeremy McClean, Phillip E. Mamidi, Sujan Wu, G. Albert Cannon, Steven B. Grimwood, Jane Jenkins, Jerry Shu, Shengqiang Song, Qijian Chavarro, Carolina Torres-Torres, Mirayda Geffroy, Valerie Moghaddam, Samira Mafi Gao, Dongying Abernathy, Brian Barry, Kerrie Blair, Matthew Brick, Mark A. Chovatia, Mansi Gepts, Paul Goodstein, David M. Gonzales, Michael Hellsten, Uffe Hyten, David L. Jia, Gaofeng Kelly, James D. Kudrna, Dave Lee, Rian Richard, Manon M. S. Miklas, Phillip N. Osorno, Juan M. Rodrigues, Josiane Thareau, Vincent Urrea, Carlos A. Wang, Mei Yu, Yeisoo Zhang, Ming Wing, Rod A. Cregan, Perry B. Rokhsar, Daniel S. Jackson, Scott A. TI A reference genome for common bean and genome-wide analysis of dual domestications SO NATURE GENETICS LA English DT Article ID DISEASE RESISTANCE GENES; PHASEOLUS-VULGARIS L.; ARABIDOPSIS-THALIANA; SEQUENCE DATA; DIVERSIFICATION; REVEALS; SELECTION; CLUSTER; ORIGIN; LOCI AB Common bean (Phaseolus vulgaris L.) is the most important grain legume for human consumption and has a role in sustainable agriculture owing to its ability to fix atmospheric nitrogen. We assembled 473 Mb of the 587-Mb genome and genetically anchored 98% of this sequence in 11 chromosome-scale pseudomolecules. We compared the genome for the common bean against the soybean genome to find changes in soybean resulting from polyploidy. Using resequencing of 60 wild individuals and 100 landraces from the genetically differentiated Mesoamerican and Andean gene pools, we confirmed 2 independent domestications from genetic pools that diverged before human colonization. Less than 10% of the 74 Mb of sequence putatively involved in domestication was shared by the two domestication events. We identified a set of genes linked with increased leaf and seed size and combined these results with quantitative trait locus data from Mesoamerican cultivars. Genes affected by domestication may be useful for genomics-enabled crop improvement. C1 [Schmutz, Jeremy; Wu, G. Albert; Shu, Shengqiang; Barry, Kerrie; Chovatia, Mansi; Goodstein, David M.; Hellsten, Uffe; Wang, Mei; Zhang, Ming; Rokhsar, Daniel S.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Schmutz, Jeremy; Grimwood, Jane; Jenkins, Jerry] HudsonAlpha Inst Biotechnol, Huntsville, AL USA. [McClean, Phillip E.; Mamidi, Sujan; Moghaddam, Samira Mafi; Lee, Rian; Osorno, Juan M.] N Dakota State Univ, Dept Plant Sci, Fargo, ND 58105 USA. [Cannon, Steven B.] USDA ARS, Corn Insects & Crop Genet Res Unit, Ames, IA USA. [Song, Qijian; Hyten, David L.; Jia, Gaofeng; Rodrigues, Josiane; Cregan, Perry B.] USDA ARS, Soybean Genom & Improvement Lab, Beltsville, MD USA. [Chavarro, Carolina; Torres-Torres, Mirayda; Gao, Dongying; Abernathy, Brian; Gonzales, Michael; Jackson, Scott A.] Univ Georgia, Ctr Appl Genet Technol, Athens, GA 30602 USA. [Geffroy, Valerie; Richard, Manon M. S.; Thareau, Vincent] Univ Paris 11, CNRS, Inst Biol Plantes, UMR 8618, F-91405 Orsay, France. [Geffroy, Valerie] Univ Paris 11, INRA, Unite Mixte Rech Genet Vegetale, Gif Sur Yvette, France. [Blair, Matthew] Tennessee State Univ, Dept Agr & Nat Sci, Nashville, TN 37203 USA. [Brick, Mark A.] Colorado State Univ, Dept Soil & Crop Sci, Ft Collins, CO 80523 USA. [Gepts, Paul] Univ Calif Davis, Dept Plant Sci, Davis, CA 95616 USA. [Kelly, James D.] Michigan State Univ, Dept Plant Soil & Microbial Sci, E Lansing, MI 48824 USA. [Kudrna, Dave; Yu, Yeisoo; Wing, Rod A.] Univ Arizona, Arizona Genom Inst, Tucson, AZ USA. [Miklas, Phillip N.] USDA ARS, Vegetable & Forage Crop Res Unit, Prosser, WA 99350 USA. [Urrea, Carlos A.] Univ Nebraska, Panhandle Res & Extens Ctr, Scottsbluff, NE USA. RP Jackson, SA (reprint author), Univ Georgia, Ctr Appl Genet Technol, Athens, GA 30602 USA. EM jschmutz@hudsonalpha.org; phillip.mcclean@ndsu.edu; sjackson@uga.edu OI Cannon, Steven/0000-0003-2777-8034; Hyten, David/0000-0001-6324-9389; mamidi, sujan/0000-0002-3837-6121; Wing, Rod/0000-0001-6633-6226 FU Office of Science of the US Department of Energy - US Department of Agriculture National Institute for Food and Agriculture [DE-AC02-05CH11231, 2006-35300-17266]; National Science Foundation [DBI 0822258]; US Department of Agriculture Cooperative State Research, Education and Extension Service [2009-01860, 2009-01929] FX The work conducted by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under contract DE-AC02-05CH11231. This research was funded by grants from the US Department of Agriculture National Institute for Food and Agriculture (2006-35300-17266) and the National Science Foundation (DBI 0822258) to S.A.J. and from the US Department of Agriculture Cooperative State Research, Education and Extension Service (2009-01860 and 2009-01929) to S.A.J. and P.E.M., respectively. NR 45 TC 210 Z9 213 U1 17 U2 125 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1061-4036 EI 1546-1718 J9 NAT GENET JI Nature Genet. PD JUL PY 2014 VL 46 IS 7 BP 707 EP 713 DI 10.1038/ng.3008 PG 7 WC Genetics & Heredity SC Genetics & Heredity GA AK0HP UT WOS:000338093800011 PM 24908249 ER PT J AU Ilas, G Gauld, IC Liljenfeldt, H AF Ilas, Germina Gauld, Ian C. Liljenfeldt, Henrik TI Validation of ORIGEN for LWR used fuel decay heat analysis with SCALE SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID ANALYSIS CAPABILITIES; SPENT FUEL; DEPLETION AB The energy release rate from the decay of radionuclides can be a critical design parameter for used nuclear fuel storage, transportation, and repository engineered systems. Validation of the SCALE nuclear analysis code system capabilities in predicting decay heat for commercial used fuel applications has been performed using decay heat measurements for fuel assemblies irradiated in pressurized and boiling water reactors. The experimental data used for validation include a large number of full-length-assembly decay heat measurements that were performed between 2003 and 2010 at the Swedish Central Interim Storage Facility for Spent Nuclear Fuel, Clab, operated by the Swedish Nuclear Fuel and Waste Management Company, SKB. The measured fuel assemblies cover the burnup range 14-51 GWd/MTU and cooling times between 12 and 27 years, which are times of interest to used fuel transportation and storage applications. The validation results indicate good agreement between calculated and measured decay heat values, generally within the reported measurement uncertainty. The effects of key modeling assumptions and data used in the calculations are presented and discussed. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ilas, Germina; Gauld, Ian C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Liljenfeldt, Henrik] Swedish Nucl Fuel & Waste Management Co AB SKB, S-10124 Stockholm, Sweden. RP Ilas, G (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM ilasg@ornl.gov; gauldi@ornl.gov; Henrik.Liljenfeldt@skb.se OI Gauld, Ian/0000-0002-3893-7515 FU UT-Battelle LLC [DE-AC05-000R22725]; US Department of Energy FX This manuscript has been authored by UT-Battelle LLC under contract DE-AC05-000R22725 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 18 TC 4 Z9 4 U1 0 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JUL 1 PY 2014 VL 273 BP 58 EP 67 DI 10.1016/j.nucengdes.2014.02.026 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ7DD UT WOS:000337856500006 ER PT J AU Craft, AE O'Brien, RC Howe, SD King, JC AF Craft, A. E. O'Brien, R. C. Howe, S. D. King, J. C. TI Submersion criticality safety of tungsten-rhenium urania cermet fuel for space propulsion and power applications SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID REACTORS; SYSTEM AB Nuclear thermal rockets are the preferred propulsion technology for a manned mission to Mars, and tungsten-uranium oxide cermet fuels could provide significant performance and cost advantages for nuclear thermal rockets. A nuclear reactor intended for use in space must remain subcritical before and during launch, and must remain subcritical in launch abort scenarios where the reactor falls back to Earth and becomes submerged in terrestrial materials (including seawater, wet sand, or dry sand). Submersion increases reflection of neutrons and also thermalizes the neutron spectrum, which typically increases the reactivity of the core. This effect is typically very significant for compact, fast-spectrum reactors. This paper provides a submersion criticality safety analysis for a representative tungsten/uranium oxide fueled reactor with a range of fuel compositions. Each submersion case considers both the rhenium content in the matrix alloy and the uranium oxide volume fraction in the cermet. The inclusion of rhenium significantly improves the submersion criticality safety of the reactor. While increased uranium oxide content increases the reactivity of the core, it does not significantly affect the submersion behavior of the reactor. There is no significant difference in submersion behavior between reactors with rhenium distributed within the cermet matrix and reactors with a rhenium clad in the coolant channels. The combination of the flooding of the coolant channels in submersion scenarios and the presence of a significant amount of spectral shift absorbers (i.e. high rhenium concentration) further decreases reactivity for short reactor cores compared to longer cores. (c) 2014 Elsevier B.V. All rights reserved. C1 [Craft, A. E.; O'Brien, R. C.; Howe, S. D.] INL, Ctr Space Nucl Res, Idaho Falls, ID USA. [King, J. C.] Colorado Sch Mines, Dept Met & Mat Engn, Nucl Sci & Engn Program, Golden, CO 80401 USA. RP Craft, AE (reprint author), 995 Univ Blvd, Idaho Falls, ID 83402 USA. EM aaron.craft@inl.gov; Robert.OBrien@inl.gov; Steven.Howe@inl.gov; kingjc@mines.edu RI O'Brien, Robert/C-3355-2017; Craft, Aaron/B-7579-2017 OI O'Brien, Robert/0000-0002-7479-6764; Craft, Aaron/0000-0002-7092-3826 NR 25 TC 0 Z9 0 U1 0 U2 16 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JUL 1 PY 2014 VL 273 BP 143 EP 149 DI 10.1016/j.nucengdes.2014.01.028 PG 7 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ7DD UT WOS:000337856500014 ER PT J AU Kryukov, A Nanstad, RK Brumovsky, M AF Kryukov, A. Nanstad, R. K. Brumovsky, M. TI Common comparison of the irradiation embrittlement of WWER/PWR reactor pressure vessel steels SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID ATOM-PROBE TOMOGRAPHY; SURVEILLANCE PROGRAM; EVOLUTION AB The paper presents the immediate comparison of Tk shifts due to neutron irradiation for WWER and PWR RPV materials and common experimental data analysis. The PWR and WWER RPV steels were irradiated at both the same temperature and neutron fluence range. For both PWR and WWER RPV material types, there is a similar degradation in mechanical properties. The comparison of "high sensitive" welds with "clean" welds reveals an expected influence of three main chemical elements (copper, nickel and phosphorus) on RPV steels irradiation embrittlement. The synergistic influence of these three elements is observed. Because the peak neutron fluence in WWER RPVs is significantly higher than for PWRs, the most part of WWER irradiation embrittlement data correspond to high fluence values. These additional data will greatly support the development of embrittlement correlations and embrittlement trend curves valid for long irradiation times. (C) 2014 Elsevier BM. All rights reserved. C1 [Kryukov, A.] Nucl Res Ee Consultancy Grp NRG, NL-1755 ZG Petten, Netherlands. [Nanstad, R. K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Brumovsky, M.] Nucl Res Inst, CZ-25068 Rez, Czech Republic. RP Kryukov, A (reprint author), Nucl Res Ee Consultancy Grp NRG, POB 25, NL-1755 ZG Petten, Netherlands. EM al.kryukov2013@yandex.ru NR 19 TC 2 Z9 2 U1 3 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JUL 1 PY 2014 VL 273 BP 175 EP 180 DI 10.1016/j.nucengdes.2014.03.018 PG 6 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AJ7DD UT WOS:000337856500018 ER PT J AU Seaver, SMD Gerdes, S Frelin, O Lerma-Ortiz, C Bradbury, LMT Zallot, R Hasnain, G Niehaus, TD El Yacoubi, B Pasternak, S Olson, R Pusch, G Overbeek, R Stevens, R de Crecy-Lagard, V Ware, D Hanson, AD Henry, CS AF Seaver, Samuel M. D. Gerdes, Svetlana Frelin, Oceane Lerma-Ortiz, Claudia Bradbury, Louis M. T. Zallot, Remi Hasnain, Ghulam Niehaus, Thomas D. El Yacoubi, Basma Pasternak, Shiran Olson, Robert Pusch, Gordon Overbeek, Ross Stevens, Rick de Crecy-Lagard, Valerie Ware, Doreen Hanson, Andrew D. Henry, Christopher S. TI High-throughput comparison, functional annotation, and metabolic modeling of plant genomes using the PlantSEED resource SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE systems biology; computational biochemistry; plant metabolism; plant genomics ID ESCHERICHIA-COLI; METACYC DATABASE; PATHWAY DATABASE; ARABIDOPSIS; NETWORK; RECONSTRUCTION; GENERATION; PROTEOMICS; BIOSYNTHESIS; OPTIMIZATION AB The increasing number of sequenced plant genomes is placing new demands on the methods applied to analyze, annotate, and model these genomes. Today's annotation pipelines result in inconsistent gene assignments that complicate comparative analyses and prevent efficient construction of metabolic models. To overcome these problems, we have developed the PlantSEED, an integrated, metabolism-centric database to support subsystems-based annotation and metabolic model reconstruction for plant genomes. PlantSEED combines SEED subsystems technology, first developed for microbial genomes, with refined protein families and biochemical data to assign fully consistent functional annotations to orthologous genes, particularly those encoding primary metabolic pathways. Seamless integration with its parent, the prokaryotic SEED database, makes PlantSEED a unique environment for cross-kingdom comparative analysis of plant and bacterial genomes. The consistent annotations imposed by PlantSEED permit rapid reconstruction and modeling of primary metabolism for all plant genomes in the database. This feature opens the unique possibility of model-based assessment of the completeness and accuracy of gene annotation and thus allows computational identification of genes and pathways that are restricted to certain genomes or need better curation. We demonstrate the PlantSEED system by producing consistent annotations for 10 reference genomes. We also produce a functioning metabolic model for each genome, gapfilling to identify missing annotations and proposing gene candidates for missing annotations. Models are built around an extended biomass composition representing the most comprehensive published to date. To our knowledge, our models are the first to be published for seven of the genomes analyzed. C1 [Seaver, Samuel M. D.; Gerdes, Svetlana; Olson, Robert; Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Pusch, Gordon; Stevens, Rick] Argonne Natl Lab, Argonne, IL 60439 USA. [Seaver, Samuel M. D.; Olson, Robert; Pusch, Gordon; Stevens, Rick; Henry, Christopher S.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Frelin, Oceane; Bradbury, Louis M. T.; Hasnain, Ghulam; Niehaus, Thomas D.] Univ Florida, Dept Hort Sci, Gainesville, FL 32611 USA. [Lerma-Ortiz, Claudia; Zallot, Remi; El Yacoubi, Basma; de Crecy-Lagard, Valerie] Univ Florida, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA. [Pasternak, Shiran; Ware, Doreen] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Ware, Doreen] Cornell Univ, USDA ARS, North Atlantic Area Plant Soil & Nutr Lab Res Uni, Ithaca, NY 14853 USA. RP Henry, CS (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM chenry@mcs.anl.gov RI ZALLOT, Remi/D-3933-2014 OI ZALLOT, Remi/0000-0002-7317-1578 FU National Science Foundation [IOS-1025398]; C V Griffin Sr Foundation; Office of Science, Office of Biological and Environmental Research, of the US Department of Energy (DOE) as part of the DOE Systems Biology Knowledgebase [DE-ACO2-06CH11357] FX We thank Kate Dreher for extensive discussions and support in the use of the AraCyc database and Joshua Stein for support in the use of the genomes and protein families. This work was supported by National Science Foundation Grant IOS-1025398, by an endowment from the C V Griffin Sr Foundation, and by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy (DOE) under Contract DE-ACO2-06CH11357, as part of the DOE Systems Biology Knowledgebase. NR 53 TC 21 Z9 21 U1 1 U2 23 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 1 PY 2014 VL 111 IS 26 BP 9645 EP 9650 DI 10.1073/pnas.1401329111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK0QG UT WOS:000338118900071 PM 24927599 ER PT J AU Guan, DB Lin, JT Davis, SJ Pan, D He, KB Wang, C Wuebbles, DJ Streets, DG Zhang, Q AF Guan, Dabo Lin, Jintai Davis, Steven J. Pan, Da He, Kebin Wang, Can Wuebbles, Donald J. Streets, David G. Zhang, Qiang TI Reply to Lopez et al.: Consumption-based accounting helps mitigate global air pollution SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Letter ID EMISSIONS C1 [Guan, Dabo; He, Kebin; Wang, Can; Zhang, Qiang] Tsinghua Univ, Minist Educ, Key Lab Earth Syst Modeling, Ctr Earth Syst Sci, Beijing 100084, Peoples R China. [Guan, Dabo] Univ Leeds, Sch Earth & Environm, Water Leeds, Leeds LS2 9JT, W Yorkshire, England. [Lin, Jintai] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China. [Davis, Steven J.] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Pan, Da] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [He, Kebin] Collaborat Innovat Ctr Reg Environm Qual, Beijing 100084, Peoples R China. [Wang, Can] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Wuebbles, Donald J.] Univ Illinois, Sch Earth Soc & Environm, Dept Atmospher Sci, Urbana, IL 61801 USA. [Streets, David G.] Argonne Natl Lab, Lemont, IL 60439 USA. RP Lin, JT (reprint author), Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China. EM linjt@pku.edu.cn RI Lin, Jintai/A-8872-2012; Zhang, Qiang/D-9034-2012; Chem, GEOS/C-5595-2014; OI Lin, Jintai/0000-0002-2362-2940; Davis, Steven/0000-0002-9338-0844; Guan, Dabo/0000-0003-3773-3403 NR 5 TC 7 Z9 7 U1 1 U2 18 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 1 PY 2014 VL 111 IS 26 BP E2631 EP E2631 DI 10.1073/pnas.1407383111 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK0QG UT WOS:000338118900002 PM 25115000 ER PT J AU Green, MA Emery, K Hishikawa, Y Warta, W Dunlop, ED AF Green, Martin A. Emery, Keith Hishikawa, Yoshihiro Warta, Wilhelm Dunlop, Ewan D. TI Solar cell efficiency tables (version 44) SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE solar cell efficiency; photovoltaic efficiency; energy conversion efficiency ID CONCENTRATOR; MULTICRYSTALLINE; STABILITY; MODULE AB Consolidated tables showing an extensive listing of the highest independently confirmed efficiencies for solar cells and modules are presented. Guidelines for inclusion of results into these tables are outlined and new entries since January 2014 are reviewed. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Green, Martin A.] Univ New S Wales, Australian Ctr Adv Photovolta, Sydney, NSW 2052, Australia. [Emery, Keith] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hishikawa, Yoshihiro] Natl Inst Adv Ind Sci & Technol, Res Ctr Photovolta Technol RCPVT, Tsukuba, Ibaraki 3058568, Japan. [Warta, Wilhelm] Fraunhofer Inst Solar Energy Syst, Dept Mat & Technol, D-79110 Freiburg, Germany. [Dunlop, Ewan D.] Commiss European Communities, Joint Res Ctr, Renewable Energy Unit, Inst Energy, IT-21027 Ispra, VA, Italy. RP Green, MA (reprint author), Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. EM m.green@unsw.edu.au FU Australian Government through the Australian Renewable Energy Agency (ARENA) FX The Australian Centre for Advanced Photovoltaics commenced operation in February 2013 with support from the Australian Government through the Australian Renewable Energy Agency (ARENA). Responsibility for the views, information or advice expressed herein is not accepted by the Australian Government. NR 47 TC 355 Z9 364 U1 7 U2 250 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD JUL PY 2014 VL 22 IS 7 BP 701 EP 710 DI 10.1002/pip.2525 PG 10 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AJ8KS UT WOS:000337953300001 ER PT J AU Hacke, P Smith, R Terwilliger, K Perrin, G Sekulic, B Kurtz, S AF Hacke, Peter Smith, Ryan Terwilliger, Kent Perrin, Greg Sekulic, Bill Kurtz, Sarah TI Development of an IEC test for crystalline silicon modules to qualify their resistance to system voltage stress SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE Energy conversion; Silicon ID POTENTIAL-INDUCED DEGRADATION; SOLAR-CELLS AB IEC 62804 Ed. 1, System voltage durability qualification test for crystalline silicon modules, is being developed. First, two module designs are compared in chamber and in the natural environment of Florida (USA). From these results, a stress level of 60 degrees C, 85% relative humidity, a bias of nameplate system voltage, 96h dwell, and a pass/fail limit of 5% relative power degradation at 25 degrees C and 1000W/m2 irradiance is initially proposed for the draft protocol. This paper next focuses on one of the main controversies within the development of this standardthe use of damp heat in an environmental chamber versus a conductive foil to complete the circuit to ground during the test. Conventional 60-cell multicrystalline silicon modules with (i) a standard aluminum frame, (ii) a modified frame, and (iii) a rear rail design were tested for potential-induced degradation (PID). These three module designs were stressed at the draft protocol conditions stated above and outdoors, applying negative system voltage bias during hours of daylight to simulate array voltage. The damp heat environmental chamber tests run according to the protocol distinguish the relative resistance of five module designs to PID in the field and correctly rank-order the durability in the field to the extent tested (up to 28months). Finally, the degradation rate is determined at 25 degrees C using a foil to ground the module face on a subset of modules susceptible to PID, and the results with respect to measured field performance of the modules are discussed. Copyright (c) 2013 John Wiley & Sons, Ltd. C1 [Hacke, Peter; Terwilliger, Kent; Perrin, Greg; Sekulic, Bill; Kurtz, Sarah] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Smith, Ryan] Pordis LLC, Austin, TX 78729 USA. RP Hacke, P (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM peter.hacke@nrel.gov FU US Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX The authors thank Bill Marion for helpful discussions; Steve Rummel and Allen Anderberg, Keith Emery, Showalter, Donard Metzger, and Stephen Barkaszi for module measurements; and Antonio Bonucci for providing module edge tape. This work was supported by the US Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 27 TC 12 Z9 12 U1 0 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD JUL PY 2014 VL 22 IS 7 BP 775 EP 783 DI 10.1002/pip.2434 PG 9 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AJ8KS UT WOS:000337953300008 ER PT J AU Feng, YZ Grogan, P Caporaso, JG Zhang, HY Lin, XG Knight, R Chu, HY AF Feng, Youzhi Grogan, Paul Caporaso, J. Gregory Zhang, Huayong Lin, Xiangui Knight, Rob Chu, Haiyan TI pH is a good predictor of the distribution of anoxygenic purple phototrophic bacteria in Arctic soils SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Anoxygenic purple phototrophic bacteria; Arctic soils; Pyrosequencing; Spatial distribution; Soil pH ID MOLECULAR EVIDENCE; DIVERSITY; COMMUNITIES; EVOLUTION; PHOTOSYNTHESIS; MICROBES; LIGHT; OCEAN; PROKARYOTES; ECOSYSTEMS AB Anoxygenic purple phototrophic bacteria (AnPPB) are ecologically important microorganisms that are sensitive to shifts in environmental variables. However, there is little information about the composition and distribution of AnPPB in the Arctic. Here we present the first study of the spatial distribution of soil AnPPB in Arctic soils using pyrosequencing and quantitative real-time PCR. We show that the AnPPB community in Arctic soils is as diverse and abundant as that in lower latitudes. The phylum Alphaproteobacteria accounted for 54.1% of the total sequences; about one third of total sequences were identified as novel phylotypes. Consistent with their anaerobic niche, AnPPB abundances were positively correlated with soil moisture content. Furthermore, the relative and absolute abundances of several dominant AnPPB taxa were significantly correlated with soil pH. AnPPB phylogenetic community structure was correlated with soil pH, as was alpha diversity, with a minimum around pH 6.0. Previous research has shown that pH is a good predictor of the structure of soil bacterial communities. Our results here suggest that pH could be a key factor driving phylogenetic diversity of not just overall bacterial communities but also of discrete functional guilds of bacteria in terrestrial ecosystems. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Feng, Youzhi; Zhang, Huayong; Lin, Xiangui; Chu, Haiyan] Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Jiangsu, Peoples R China. [Grogan, Paul] Queens Univ, Dept Biol, Kingston, ON K7L 3N6, Canada. [Caporaso, J. Gregory] No Arizona Univ, Dept Biol Sci, Flagstaff, AZ 86011 USA. [Caporaso, J. Gregory] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Knight, Rob] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Knight, Rob] Univ Colorado, Howard Hughes Med Inst, Boulder, CO 80309 USA. RP Chu, HY (reprint author), Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Jiangsu, Peoples R China. EM xglin@issas.ac.cn; hychu@issas.ac.cn RI Knight, Rob/D-1299-2010 FU National Natural Science Foundation of China [_501100001809, 41071167, 41371254, 41001142, 41271256]; Hundred Talents Program of the Chinese Academy of Sciences [_501100002367]; AWS in Education researcher's grant; Howard Hughes Medical Institute [_100000011] FX We sincerely thank our many colleagues who collected soil samples across the Arctic. We also thank Linda Cameron and several undergraduate students for help with soil processing and lab analyses. This work was supported by National Natural Science Foundation of China (_501100001809) to H. Chu (41071167, 41371254) and to Y. Feng (41001142, 41271256), the Hundred Talents Program of the Chinese Academy of Sciences (_501100002367) to H. Chu, and NSERC as part of the International Polar Year Project: Climate Change Impacts on Canadian Arctic Tundra (P. Grogan), Amazon Web Services (AWS in Education researcher's grant to JG. Caporaso and R. Knight) and the Howard Hughes Medical Institute (_100000011) (R. Knight). NR 53 TC 9 Z9 13 U1 4 U2 57 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD JUL PY 2014 VL 74 BP 193 EP 200 DI 10.1016/j.soilbio.2014.03.014 PG 8 WC Soil Science SC Agriculture GA AJ7BZ UT WOS:000337853500022 ER PT J AU Singh, D Timofeeva, EV Moravek, MR Cingarapu, S Yu, WH Fischer, T Mathur, S AF Singh, Dileep Timofeeva, Elena V. Moravek, Michael R. Cingarapu, Sreeram Yu, Wenhua Fischer, Thomas Mathur, Sanjay TI Use of metallic nanoparticles to improve the thermophysical properties of organic heat transfer fluids used in concentrated solar power SO SOLAR ENERGY LA English DT Article DE Copper nanoparticles; Nanofluids; Thermophysical properties; Heat transfer ID ENHANCED THERMAL-CONDUCTIVITY; ETHYLENE-GLYCOL; COPPER NANOPARTICLES; BROWNIAN-MOTION; NANOFLUIDS AB One of the approaches to enhance the efficiency, and consequently, reduce costs to produce electricity from concentrated solar power (CSP) is by the development of advanced high temperature heat transfer fluids (HTFs). Incorporation of metallic nanoparticles into conventional heat transfer fluids could significantly improve the thermal transport properties of the HTFs. This study reports on the synthesis and investigation of copper nanoparticles synthesized in-house and dispersed in two synthetic HTFs Therminol 59 (TH59) and Therminol 66 (TH66). Liquid phase reduction of a copper salt was used to produce copper nanoparticles. Suspensions with various copper nanoparticle loadings (0.5-2 vol.%) were prepared. Characterizations such as the thermal conductivity, dynamic viscosity, mass specific heat capacity, and fluid stability were performed on the suspensions. Thermal conductivity enhancements over the base fluids were as high as approximately 20% at a 2 vol.% particle loading. These enhancements in the thermal conductivity are higher than the predictions based on the Effective Medium Theory (EMT). Dynamic viscosity measurements showed that if good dispersion of nanoparticles is achieved, the composite fluids behave in a Newtonian manner and the dynamic viscosity increases over the base fluid are minor at temperatures 125 C and above. Stability of the suspensions with time was also investigated. Based on the measured properties of the suspensions, a figure of merit for heat transfer was calculated to evaluate the viability of the suspensions. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Singh, Dileep; Moravek, Michael R.; Cingarapu, Sreeram] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Timofeeva, Elena V.; Yu, Wenhua] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Fischer, Thomas; Mathur, Sanjay] Univ Cologne, Inst Inorgan Chem, D-50923 Cologne, Germany. RP Singh, D (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM dsingh@anl.gov RI Timofeeva, Elena/E-6391-2010; OI Timofeeva, Elena V./0000-0001-7839-2727 FU US Department of Energy's EERE Solar Energy Technology Program ARRA funding FX This work was supported by US Department of Energy's EERE Solar Energy Technology Program ARRA funding. Discussions with DOE project managers, Mr. Joe Stekli and Dr. Levi Irwin are much appreciated. The EMS was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a US Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago-Argonne, LLC. Assistance from Dr. Y. Yusufoglu is appreciated. NR 32 TC 11 Z9 11 U1 3 U2 29 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-092X J9 SOL ENERGY JI Sol. Energy PD JUL PY 2014 VL 105 BP 468 EP 478 DI 10.1016/j.solener.2014.02.036 PG 11 WC Energy & Fuels SC Energy & Fuels GA AJ8VJ UT WOS:000337985700045 ER PT J AU Yue, DJ You, FQ Darling, SB AF Yue, Dajun You, Fengqi Darling, Seth B. TI Domestic and overseas manufacturing scenarios of silicon-based photovoltaics: Life cycle energy and environmental comparative analysis SO SOLAR ENERGY LA English DT Article DE Life cycle assessment; Silicon-based photovoltaics; Manufacturing; Renewable energy ID SOLAR-CELLS; EMISSIONS; IMPACTS AB While life cycle assessment (LCA) has been recognized as an invaluable tool to assess the energy and environmental profiles of a photovoltaic (PV) system, current LCA studies are limited to Europe and North America. However, today most PV modules are outsourced to and manufactured in non-OECD countries (e.g., China), which have a substantially different degree of industrialization and environmental restriction. To investigate this issue, we perform a comparative LCA between domestic and overseas manufacturing scenarios illustrated by three kinds of silicon-based PV technologies, namely mono-crystalline silicon, multi-crystalline silicon and ribbon silicon. We take into account geographic diversity by utilizing localized inventory data for processes and materials. The energy payback time, energy return on investment and greenhouse gas (GHG) emissions for both scenarios are calculated and analyzed. Compared to the domestic manufacturing scenario, the energy use efficiency is generally 30% lower and the carbon footprint is almost doubled in the overseas manufacturing scenario. Moreover, based on the LCA results, we propose a break-even carbon tariff model for the international trade of silicon-based PV modules, indicating an appropriate carbon tariff in the range of is an element of 105-is an element of 129/ton CO2. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Yue, Dajun; You, Fengqi] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP You, FQ (reprint author), Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM you@northwestern.edu RI You, Fengqi/F-6894-2011; You, Fengqi/B-5040-2011 OI You, Fengqi/0000-0001-9609-4299 FU Institute for Sustainability and Energy at Northwestern (ISEN); Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX The authors gratefully acknowledge the financial support from the Institute for Sustainability and Energy at Northwestern (ISEN). This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract no. DE-AC02-06CH11357. We are also grateful to IKE Environmental Technology Co. Ltd. for providing part of the life cycle inventory data from the Chinese Life Cycle Database (CLCD) for the life cycle energy and environmental analysis of the overseas manufacturing scenario. NR 42 TC 29 Z9 29 U1 5 U2 54 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-092X J9 SOL ENERGY JI Sol. Energy PD JUL PY 2014 VL 105 BP 669 EP 678 DI 10.1016/j.solener.2014.04.008 PG 10 WC Energy & Fuels SC Energy & Fuels GA AJ8VJ UT WOS:000337985700061 ER PT J AU Liu, RL Bohac, DL Gundel, LA Hewett, MJ Apte, MG Hammond, SK AF Liu, Ruiling Bohac, David L. Gundel, Lara A. Hewett, Martha J. Apte, Michael G. Hammond, S. Katharine TI Assessment of risk for asthma initiation and cancer and heart disease deaths among patrons and servers due to secondhand smoke exposure in restaurants and bars SO TOBACCO CONTROL LA English DT Article DE Secondhand smoke; Smoking Caused Disease; Public policy; Priority; special populations; Environment ID ENVIRONMENTAL TOBACCO-SMOKE; PASSIVE SMOKING; LUNG-CANCER; MORTALITY RISK; PUBLIC PLACES; UNITED-STATES; EXCESS; WORKERS; NONSMOKERS; POPULATION AB Background Despite efforts to reduce exposure to secondhand smoke (SHS), only 5% of the world's population enjoy smoke-free restaurants and bars. Methods Lifetime excess risk (LER) of cancer death, ischaemic heart disease (IHD) death and asthma initiation among non-smoking restaurant and bar servers and patrons in Minnesota and the US were estimated using weighted field measurements of SHS constituents in Minnesota, existing data on tobacco use and multiple dose-response models. Results A continuous approach estimated a LER of lung cancer death (LCD) of 18x10(-6)(95% CI 13 to 23x10(-6)) for patrons visiting only designated non-smoking sections, 80x10(-6)(95% CI 66 to 95x10(-6)) for patrons visiting only smoking venues/sections and 802x10(-6)(95% CI 658 to 936x10(-6)) for servers in smoking-permitted venues. An attributable-risk (exposed/non-exposed) approach estimated a similar LER of LCD, a LER of IHD death about 10(-2) for non-smokers with average SHS exposure from all sources and a LER of asthma initiation about 5% for servers with SHS exposure at work only. These risks correspond to 214 LCDs and 3001 IHD deaths among the general non-smoking population and 1420 new asthma cases among non-smoking servers in the US each year due to SHS exposure in restaurants and bars alone. Conclusions Health risks for patrons and servers from SHS exposure in restaurants and bars alone are well above the acceptable level. Restaurants and bars should be a priority for governments' effort to create smoke-free environments and should not be exempt from smoking bans. C1 [Liu, Ruiling; Hammond, S. Katharine] Univ Calif Berkeley, Sch Publ Hlth, Dept Environm Hlth Sci, Berkeley, CA 94720 USA. [Bohac, David L.; Hewett, Martha J.] Ctr Energy & Environm, Minneapolis, MN USA. [Gundel, Lara A.; Apte, Michael G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Indoor Environm, Berkeley, CA 94720 USA. RP Hammond, SK (reprint author), Univ Calif Berkeley, Sch Publ Hlth, Dept Environm Hlth Sci, 50 Univ Hall 7360, Berkeley, CA 94720 USA. EM hammondk@berkeley.edu FU ClearWay Minnesota [RC 2006-0050]; Flight Attendants Medical Research Institute FX This research project was funded in part by ClearWay Minnesota through Grant Number RC 2006-0050 and in part by Dr William Cahan Distinguished Professor Award to SKH from the Flight Attendants Medical Research Institute. NR 49 TC 3 Z9 3 U1 1 U2 5 PU BMJ PUBLISHING GROUP PI LONDON PA BRITISH MED ASSOC HOUSE, TAVISTOCK SQUARE, LONDON WC1H 9JR, ENGLAND SN 0964-4563 EI 1468-3318 J9 TOB CONTROL JI Tob. Control PD JUL PY 2014 VL 23 IS 4 BP 332 EP 338 DI 10.1136/tobaccocontrol-2012-050831 PG 7 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA AJ7ZE UT WOS:000337920100019 PM 23407112 ER PT J AU Liu, XY Afzal, W He, MG Prausnitz, JM AF Liu, Xiangyang Afzal, Waheed He, Maogang Prausnitz, John M. TI Solubilities of small hydrocarbons, viscosities of diluted tetraalkylphosphonium bis(2,4,4-trimethylpentyl) phosphinates SO AICHE JOURNAL LA English DT Article DE solubility; density; viscosity; phosphonium-based ionic liquids; diluent; mixtures of ionic liquids ID TEMPERATURE IONIC LIQUIDS; PHOSPHONIUM CATION; GASES; IMIDAZOLIUM; DENSITIES; WATER; BIS(TRIFLUOROMETHYLSULFONYL)IMIDE; HEXAFLUOROPHOSPHATE; DIFFUSIVITY AB Tetraalkylphosphonium bis(2,4,4-trimethylpentyl)phosphinates show large solubilities for methane, ethane, ethylene, and propane. In these ionic liquids, solubilities of ethane are larger than those of ethylene. Therefore, these ionic liquids may be useful solvents for separation of ethane and ethylene; because the vapor pressure of ethylene is higher than that of ethane, the relative volatility ethylene/ethane is enhanced. However, the viscosities of these ionic liquids are too high for an industrial process. Low-viscosity 1-butyl-3-H-imidazolium acetate([BHMIM][AC]) is a suitable diluent for reducing the large viscosities of trihexyl tetradecylphosphonium bis(2,4,4-trimethylpentyl) phosphinate ([P(14)666][TMPP]) and tetrabutylphosphonium bis(2,4,4-trimethylpentyl) phosphinate ([P4444][TMPP]). Addition of 20 wt % [BHMIM][AC] gives a dramatic drop in the viscosities of these ionic liquids. Mixtures of [P(14)666][TMPP] or [P4444][TMPP] with 20 or 50 wt % [BHMIM][AC] show high solubilities for the four solutes when compared with those in other ionic liquids. In these mixtures, the solubility for ethane is higher than that for ethylene. (c) 2014 American Institute of Chemical Engineers C1 [Liu, Xiangyang; Afzal, Waheed; Prausnitz, John M.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Liu, Xiangyang; He, Maogang] Xi An Jiao Tong Univ, MOE Key Lab Thermofluid Sci & Engn, Xian 710049, Shaanxi, Peoples R China. [Afzal, Waheed; Prausnitz, John M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Afzal, Waheed] Univ Punjab, Inst Chem Engn & Technol, Lahore 54590, Pakistan. RP Prausnitz, JM (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM prausnit@cchem.berkeley.edu OI Afzal, Waheed/0000-0002-2927-0114 FU Environmental Energy Technologies Division of the Lawrence Berkeley National Laboratory FX The authors are grateful to the Environmental Energy Technologies Division of the Lawrence Berkeley National Laboratory for financial support, and to Profs. Alexis Bell and Scott Lynn and coworkers for general assistance. They are grateful to Prof. Michael Manga (Dept. of Earth and Planetary Sciences, University of California, Berkeley) for providing his density meter. NR 27 TC 8 Z9 9 U1 11 U2 40 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 EI 1547-5905 J9 AICHE J JI AICHE J. PD JUL PY 2014 VL 60 IS 7 BP 2607 EP 2612 DI 10.1002/aic.14453 PG 6 WC Engineering, Chemical SC Engineering GA AJ5BL UT WOS:000337695500020 ER PT J AU Kang, MK Lee, J Um, Y Lee, TS Bott, M Park, SJ Woo, HM AF Kang, Min-Kyoung Lee, Jungseok Um, Youngsoon Lee, Taek Soon Bott, Michael Park, Si Jae Woo, Han Min TI Synthetic biology platform of CoryneBrick vectors for gene expression in Corynebacterium glutamicum and its application to xylose utilization SO APPLIED MICROBIOLOGY AND BIOTECHNOLOGY LA English DT Article DE Corynebacterium glutamicum; Synthetic biology; Metabolic engineering; BglBrick ID ESCHERICHIA-COLI; ORGANIC-ACIDS; AMINO-ACIDS; PRECURSOR; PATHWAY; DNA; AMORPHA-4,11-DIENE; OVERPRODUCTION; OPTIMIZATION; PROMOTERS AB Currently, the majority of tools in synthetic biology have been designed and constructed for model organisms such as Escherichia coli and Saccharomyces cerevisiae. In order to broaden the spectrum of organisms accessible to such tools, we established a synthetic biological platform, called CoryneBrick, for gene expression in Corynebacterium glutamicum as a set of E. coli-C. glutamicum shuttle vectors whose elements are interchangeable with BglBrick standard parts. C. glutamicum is an established industrial microorganism for the production of amino acids, proteins, and commercially promising chemicals. Using the CoryneBrick vectors, we showed various time-dependent expression profiles of a red fluorescent protein. This CoryneBrick platform was also applicable for two-plasmid expression systems with a conventional C. glutamicum expression vector. In order to demonstrate the practical application of the CoryneBrick vectors, we successfully reconstructed the xylose utilization pathway in the xylose-negative C. glutamicum wild type by fast BglBrick cloning methods using multiple genes encoding for xylose isomerase and xylulose kinase, resulting in a growth rate of 0.11 +/- 0.004 h(-1) and a xylose uptake rate of 3.35 mmol/gDW/h when 1 % xylose was used as sole carbon source. Thus, CoryneBrick vectors were shown to be useful engineering tools in order to exploit Corynebacterium as a synthetic platform for the production of chemicals by controllable expression of the genes of interest. C1 [Kang, Min-Kyoung; Lee, Jungseok; Um, Youngsoon; Woo, Han Min] Korea Inst Sci & Technol, Clean Energy Res Ctr, Seoul 136791, South Korea. [Lee, Jungseok] Korea Univ, Dept Chem & Biol Engn, Seoul 136701, South Korea. [Woo, Han Min] Korea Univ, Green Sch, Seoul 136701, South Korea. [Um, Youngsoon; Woo, Han Min] Univ Sci & Technol, Dept Clean Energy & Chem Engn, Taejon 305350, South Korea. [Lee, Taek Soon] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Lee, Taek Soon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Bott, Michael] Forschungszentrum Julich, Inst Bio & Geosci, IBG Biotechnol 1, D-52425 Julich, Germany. [Park, Si Jae] Myongji Univ, Dept Environm Engn & Energy, Yongin 449728, Gyeonggido, South Korea. RP Woo, HM (reprint author), Korea Inst Sci & Technol, Clean Energy Res Ctr, Hwarangno 14 Gil 5, Seoul 136791, South Korea. EM hmwoo@kist.re.kr RI Woo, Han Min/J-1847-2015; Bott, Michael/E-8004-2011 OI Woo, Han Min/0000-0002-8797-0477; Bott, Michael/0000-0002-4701-8254 FU National Research Foundation of Korea - Korean Government (Ministry of Science, ICT & Future Planning); Creative Allied Program (CAP) of the Korea Research Council of Fundamental Science and Technology (KRCF)/Korea Institute of Science and Technology (KIST) [2E24832] FX The authors thank Prof. Anthony J. Sinskey for the kind gift of pZ8-1 and M. S. Jae Hee Jung for technical assistant. This work was supported by the National Research Foundation of Korea Grant funded by the Korean Government (Ministry of Science, ICT & Future Planning) (2014, University-Institute cooperation program) and Creative Allied Program (CAP) of the Korea Research Council of Fundamental Science and Technology (KRCF)/Korea Institute of Science and Technology (KIST) (project no. 2E24832). NR 46 TC 14 Z9 14 U1 3 U2 31 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0175-7598 EI 1432-0614 J9 APPL MICROBIOL BIOT JI Appl. Microbiol. Biotechnol. PD JUL PY 2014 VL 98 IS 13 BP 5991 EP 6002 DI 10.1007/s00253-014-5714-7 PG 12 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AJ5SL UT WOS:000337747900018 PM 24706215 ER PT J AU Wecker, MSA Ghirardi, ML AF Wecker, Matt S. A. Ghirardi, Maria L. TI High-throughput biosensor discriminates between different algal H-2-photoproducing strains SO BIOTECHNOLOGY AND BIOENGINEERING LA English DT Article DE Rhodobacter capsulatus; H-2 sensor; high-throughput screening; photobiohydrogen; Chlamydomonas reinhardtii; H-2 production ID HARVESTING CHLOROPHYLL ANTENNA; CYCLIC ELECTRON FLOW; CHLAMYDOMONAS-REINHARDTII; HYDROGEN-PRODUCTION; ESCHERICHIA-COLI; H-2 PRODUCTION; GENE; PHOTOPRODUCTION; EXPRESSION; PROTEIN AB A number of species of microalgae and cyanobacteria photosynthetically produce H2 gas by coupling water oxidation with the reduction of protons to molecular hydrogen, generating renewable energy from sunlight and water. Photosynthetic H2 production, however, is transitory, and there is considerable interest in increasing and extending it for commercial applications. Here we report a Petri-plate version of our previous, microplate-based assay that detects photosynthetic H2 production by algae. The assay consists of an agar overlay of H2-sensing Rhodobacter capsulatus bacteria carrying a green fluorescent protein that responds to H2 produced by single algal colonies in the bottom agar layer. The assay distinguishes between algal strains that photoproduce H2 at different levels under high light intensities, and it does so in a simple, inexpensive, and high-throughput manner. The assay will be useful for screening both natural populations and mutant libraries for strains having increased H2 production, and useful for identifying various genetic factors that physiologically or genetically alter algal hydrogen production. Biotechnol. Bioeng. 2014;111: 1332-1340. (c) 2014 Wiley Periodicals, Inc. C1 [Wecker, Matt S. A.] GeneBiologics LLC, Boulder, CO USA. [Ghirardi, Maria L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Ghirardi, ML (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM maria.ghirardi@nrel.gov FU Department of Energy, Office of Biological and Environmental Research; National Renewable Energy Laboratory [DE-AC36-08GC28308z] FX Contract grant sponsor: Funded by the Department of Energy, Office of Biological and Environmental Research; Grant numbers: with the National Renewable Energy Laboratory: DE-AC36-08GC28308z NR 37 TC 9 Z9 9 U1 0 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0006-3592 EI 1097-0290 J9 BIOTECHNOL BIOENG JI Biotechnol. Bioeng. PD JUL PY 2014 VL 111 IS 7 BP 1332 EP 1340 DI 10.1002/bit.25206 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AJ3PU UT WOS:000337580000007 PM 24578287 ER PT J AU Kumar, R Wyman, CE AF Kumar, Rajeev Wyman, Charles E. TI Strong cellulase inhibition by Mannan polysaccharides in cellulose conversion to sugars SO BIOTECHNOLOGY AND BIOENGINEERING LA English DT Article DE cellulase; inhibition; heteromannans; glucomannan; galactomannan; oligomers; xylan ID SOLIDS ENZYMATIC-HYDROLYSIS; LIGNOCELLULOSIC BIOMASS; LEADING TECHNOLOGIES; TRICHODERMA-REESEI; CLOSTRIDIUM-CELLULOVORANS; HYDROTHERMAL PRETREATMENT; PRODUCT INHIBITION; WHEAT-STRAW; XYLANASE; ETHANOL AB Cellulase enzymes contribute a major fraction of the total cost for biological conversion of lignocellulosic biomass to fuels and chemicals. Although a several fold reduction in cellulase production costs and enhancement of cellulase activity and stability have been reported in recent years, sugar yields are still lower at low enzyme doses than desired commercially. We recently reported that hemicellulose xylan and its oligomers strongly inhibit cellulase and that supplementation of cellulase with xylanase and -xylosidase would significantly reduce such inhibition. In this study, mannan polysaccharides and their enzymatically prepared hydrolyzates were discovered to be strongly inhibitory to fungal cellulase in cellulose conversion (>50% drop in % relative conversion), even at a small concentration of 0.1g/L, and inhibition was much greater than experienced by other known inhibitors such as cellobiose, xylooligomers, and furfural. Furthermore, cellulase inhibition dramatically increased with heteromannan loading and mannan substitution with galactose side units. In general, enzymatically prepared hydrolyzates were less inhibitory than their respective mannan polysaccharides except highly substituted ones. Supplementation of cellulase with commercial accessory enzymes such as xylanase, pectinase, and -glucosidase was effective in greatly relieving inhibition but only for less substituted heteromannans. However, cellulase supplementation with purified heteromannan specific enzymes relieved inhibition by these more substituted heteromannans as well, suggesting that commercial preparations need to have higher amounts of such activities to realize high sugar yields at the low enzyme protein loadings needed for low cost fuels production. Biotechnol. Bioeng. 2014;111: 1341-1353. (c) 2014 Wiley Periodicals, Inc. C1 [Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Ctr Environm Res & Technol CE CERT, Bourns Coll Engn, Riverside, CA 92507 USA. [Kumar, Rajeev; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. [Wyman, Charles E.] Univ Calif Riverside, Dept Chem & Environm Engn, Bourns Coll Engn, Riverside, CA 92507 USA. RP Kumar, R (reprint author), Univ Calif Riverside, Ctr Environm Res & Technol CE CERT, Bourns Coll Engn, 1084 Columbia Ave, Riverside, CA 92507 USA. EM rkumar@cert.ucr.edu OI Kumar, Rajeev/0000-0001-7523-0108 FU Office of Biological and Environmental Research in the DOE Office of Science through the BioEnergy Science Center (BESC) FX Contract grant sponsor: Office of Biological and Environmental Research in the DOE Office of Science through the BioEnergy Science Center (BESC) NR 72 TC 13 Z9 13 U1 2 U2 55 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0006-3592 EI 1097-0290 J9 BIOTECHNOL BIOENG JI Biotechnol. Bioeng. PD JUL PY 2014 VL 111 IS 7 BP 1341 EP 1353 DI 10.1002/bit.25218 PG 13 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AJ3PU UT WOS:000337580000008 PM 24522973 ER PT J AU Liu, CZ Greene, DL Bunch, DS AF Liu, Changzheng Greene, David L. Bunch, David S. TI Vehicle Manufacturer Technology Adoption and Pricing Strategies under Fuel Economy/Emissions Standards and Feebates SO ENERGY JOURNAL LA English DT Article DE CAFE; Emissions standards; Manufacturer pricing; Technology adoption ID ENERGY EFFICIENCY; ECONOMY; TAXES AB New post-2010 Corporate Average Fuel Economy (CAFE) standards and carbon dioxide (CO2) emissions standards have significantly increased the stringency of requirements for new light-duty vehicle fuel efficiency. This study investigates the role of technology adoption and pricing strategies in meeting the new standards, and the impact of possible feebate policies. The analysis simulates manufacturer decision making over the period (2011-2020) using a dynamic optimization model of the new vehicle market that maximizes social surplus while meeting the standards. Consumer surplus is determined from consumer demand, which is represented by a nested multinomial logit model, and the model is conservative in its assumptions on available technology. Results indicate that technology adoption will likely play a much larger role than pricing strategies in meeting the new standards (consistent with the intent of the policy). Feebates, when implemented along with the standards, can bring additional fuel economy improvement and emissions reduction, but the impact of feebates diminishes with the increasing stringency of the standards. Results also show that the impact of the policy on consumers could be relatively limited. In the long run the policy requires increasing up-front technology costs to consumers that outweigh the perceived benefit of fuel savings, and there is some loss in total new vehicle sales. However, the net effect is limited, and the full value of fuel savings to society is substantial. Results also show a small decrease in average vehicle footprint size, indicating that efficiency improvements are primarily distributed across all vehicle sizes, consistent with the intent of the policy. C1 [Liu, Changzheng; Greene, David L.] Oak Ridge Natl Lab, Knoxville, TN 37932 USA. [Bunch, David S.] Univ Calif Davis, Grad Sch Management, Davis, CA 95616 USA. RP Liu, CZ (reprint author), Oak Ridge Natl Lab, 2360 Cherahala Blvd, Knoxville, TN 37932 USA. EM linc2@ornl.gov RI Liu, Changzheng/J-4268-2014 OI Liu, Changzheng/0000-0003-0052-4552 FU California Air Resources Board; U.S. Department of Energy FX The study reported in this paper was sponsored in part by the California Air Resources Board and the U.S. Department of Energy. Opinions and views expressed are those of the authors and do not necessarily reflect those of either agency. NR 20 TC 2 Z9 2 U1 1 U2 15 PU INT ASSOC ENERGY ECONOMICS PI CLEVELAND PA 28790 CHAGRIN BLVD, STE 210, CLEVELAND, OH 44122 USA SN 0195-6574 EI 1944-9089 J9 ENERG J JI Energy J. PD JUL PY 2014 VL 35 IS 3 BP 71 EP 90 DI 10.5547/01956574.35.3.4 PG 20 WC Economics; Energy & Fuels; Environmental Studies SC Business & Economics; Energy & Fuels; Environmental Sciences & Ecology GA AJ4PC UT WOS:000337657300004 ER PT J AU Ma, TH Li, CJ Lu, ZM Wang, BX AF Ma, Tuhua Li, Changjiang Lu, Zhiming Wang, Baoxin TI An effective antecedent precipitation model derived from the power-law relationship between landslide occurrence and rainfall level SO GEOMORPHOLOGY LA English DT Article DE Landslides; Effective antecedent precipitation; Lower bound rainfall threshold determination; Power-law distributions; Fractals ID THRESHOLDS; SHALLOW AB Antecedent rainfall is an important predisposing factor in triggering landslides because it reduces soil suction and increases the pore-water pressure in soils. The existing approaches to quantify the antecedent rainfall were derived from empirical methods used to develop rainfall-runoff models in which the daily decays of rainfall within a given period preceding a given day are considered as independent processes. In this study, a methodology accounting for the effective antecedent rainfall that influences landslide occurrence is developed from a power-law relationship between the frequency of landslide occurrence and the landslide-triggering rainfall level. In this model, the decay rate of the daily rainfall is related to a scaling exponent defined by the power-law relationship, the decay process of daily rainfall within a given period preceding a given day is not independent but is interrelated, and the impact of rainfall in the preceding k days on soil moisture is associated with the precipitation from the preceding (k - 1) days. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ma, Tuhua; Li, Changjiang] Zhejiang Informat Ctr Land & Resources, Hangzhou 310007, Zhejiang, Peoples R China. [Lu, Zhiming] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87545 USA. [Wang, Baoxin] Zhejiang Bur Geol & Mineral Resource Explorat & D, Hydrogeol Sect, Ningbo 315000, Peoples R China. RP Li, CJ (reprint author), Zhejiang Informat Ctr Land & Resources, Hangzhou 310007, Zhejiang, Peoples R China. EM zjigmr@mail.hz.zj.cn; zhiming@lanl.gov OI Lu, Zhiming/0000-0001-5800-3368 FU Special Fund for Land and Resources Research in the Public Interest of P.R. China [201211055] FX This study was partially funded by the Special Fund for Land and Resources Research in the Public Interest of P.R. China (No. 201211055). We would like to thank the Editor Dr. Richard A. Marston and the three anonymous reviewers for their valuable comments and suggestions, which have improved the paper. NR 27 TC 8 Z9 11 U1 0 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-555X EI 1872-695X J9 GEOMORPHOLOGY JI Geomorphology PD JUL 1 PY 2014 VL 216 BP 187 EP 192 DI 10.1016/j.geomorph.2014.03.033 PG 6 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA AJ6CG UT WOS:000337776700015 ER PT J AU Bassu, S Brisson, N Durand, JL Boote, K Lizaso, J Jones, JW Rosenzweig, C Ruane, AC Adam, M Baron, C Basso, B Biernath, C Boogaard, H Conijn, S Corbeels, M Deryng, D De Sanctis, G Gayler, S Grassini, P Hatfield, J Hoek, S Izaurralde, C Jongschaap, R Kemanian, AR Kersebaum, KC Kim, SH Kumar, NS Makowski, D Muller, C Nendel, C Priesack, E Pravia, MV Sau, F Shcherbak, I Tao, F Teixeira, E Timlin, D Waha, K AF Bassu, Simona Brisson, Nadine Durand, Jean-Louis Boote, Kenneth Lizaso, Jon Jones, James W. Rosenzweig, Cynthia Ruane, Alex C. Adam, Myriam Baron, Christian Basso, Bruno Biernath, Christian Boogaard, Hendrik Conijn, Sjaak Corbeels, Marc Deryng, Delphine De Sanctis, Giacomo Gayler, Sebastian Grassini, Patricio Hatfield, Jerry Hoek, Steven Izaurralde, Cesar Jongschaap, Raymond Kemanian, Armen R. Kersebaum, K. Christian Kim, Soo-Hyung Kumar, Naresh S. Makowski, David Mueller, Christoph Nendel, Claas Priesack, Eckart Pravia, Maria Virginia Sau, Federico Shcherbak, Iurii Tao, Fulu Teixeira, Edmar Timlin, Dennis Waha, Katharina TI How do various maize crop models vary in their responses to climate change factors? SO GLOBAL CHANGE BIOLOGY LA English DT Article DE [CO2]; AgMIP; climate; maize; model intercomparison; simulation; temperature; uncertainty ID WATER-USE EFFICIENCY; AIR CO2 ENRICHMENT; SIMULATION-MODEL; ELEVATED CO2; SYSTEMS SIMULATION; NITROGEN DYNAMICS; CARBON-DIOXIDE; YIELD; WHEAT; AGRICULTURE AB Potential consequences of climate change on crop production can be studied using mechanistic crop simulation models. While a broad variety of maize simulation models exist, it is not known whether different models diverge on grain yield responses to changes in climatic factors, or whether they agree in their general trends related to phenology, growth, and yield. With the goal of analyzing the sensitivity of simulated yields to changes in temperature and atmospheric carbon dioxide concentrations [CO2], we present the largest maize crop model intercomparison to date, including 23 different models. These models were evaluated for four locations representing a wide range of maize production conditions in the world: Lusignan (France), Ames (USA), Rio Verde (Brazil) and Morogoro (Tanzania). While individual models differed considerably in absolute yield simulation at the four sites, an ensemble of a minimum number of models was able to simulate absolute yields accurately at the four sites even with low data for calibration, thus suggesting that using an ensemble of models has merit. Temperature increase had strong negative influence on modeled yield response of roughly -0.5 Mg ha(-1) per degrees C. Doubling [CO2] from 360 to 720 mu mol mol(-1) increased grain yield by 7.5% on average across models and the sites. That would therefore make temperature the main factor altering maize yields at the end of this century. Furthermore, there was a large uncertainty in the yield response to [CO2] among models. Model responses to temperature and [CO2] did not differ whether models were simulated with low calibration information or, simulated with high level of calibration information. C1 [Bassu, Simona; Brisson, Nadine; Makowski, David] INRA AgroParisTech, Unite Agron, F-78850 Thiverval Grignon, France. [Durand, Jean-Louis] INRA, Unite Rech Pluridisciplinaire Prairie & Plantes F, F-86600 Lusignan, France. [Boote, Kenneth] Univ Florida, Dept Agron, Gainesville, FL 32611 USA. [Lizaso, Jon; Sau, Federico] Univ Politecn Madrid, Dept Prod Vegetal, E-28040 Madrid, Spain. [Jones, James W.] Univ Florida, Dept Agr & Biol Engn, Gainesville, FL 32611 USA. [Rosenzweig, Cynthia; Ruane, Alex C.] NASA, Goddard Inst Space Studies, Climate Impacts Grp, New York, NY 10025 USA. [Adam, Myriam] CIRAD, UMR AGAP PAM, Montpellier, France. [Baron, Christian] CIRAD, UMR TETIS, F-34093 Montpellier, France. [Basso, Bruno; Shcherbak, Iurii] Michigan State Univ, Dept Geol Sci, E Lansing, MI 48824 USA. [Basso, Bruno; Shcherbak, Iurii] Univ Basilicata, Dept Crop Syst Forestry & Environm Sci, I-85100 Potenza, Italy. [Biernath, Christian; Priesack, Eckart] Helmholtz Zentrum Munchen, Inst Bodenokol, D-85764 Neuherberg, Germany. [Boogaard, Hendrik; Hoek, Steven] Alterra, Ctr Geoinformat, NL-6700 AA Wageningen, Netherlands. [Conijn, Sjaak; Jongschaap, Raymond] Univ Wageningen & Res Ctr, WUR Plant Res Int, NL-6700 AA Wageningen, Netherlands. [Corbeels, Marc] CIRAD Annual Cropping Syst, BR-73310970 Planaltina, DF, Brazil. [Deryng, Delphine] Univ E Anglia, Tyndall Ctr Climate Change Res, Norwich NR4 7TJ, Norfolk, England. [Deryng, Delphine] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England. [De Sanctis, Giacomo] INRA, Unite AGROCLIM, F-84914 Avignon 9, France. [Gayler, Sebastian] Univ Tubingen, Water & Earth Syst Sci WESS Competence Cluster, D-72074 Tubingen, Germany. [Grassini, Patricio] Univ Nebraska, Dept Agron & Hort, Lincoln, NE 68503 USA. [Hatfield, Jerry] USDA ARS, Natl Soil Tilth Lab Agr & Environm, Ames, IA 50011 USA. [Izaurralde, Cesar] Pacific NW Natl Lab, College Pk, MD 20740 USA. [Izaurralde, Cesar] Univ Maryland, College Pk, MD 20740 USA. [Kemanian, Armen R.; Pravia, Maria Virginia] Penn State Univ, Dept Plant Sci, University Pk, PA 16802 USA. [Kersebaum, K. Christian; Nendel, Claas] Leibniz Ctr Agr Landscape Res, ZALF, Inst Landscape Syst Anal, D-15374 Muencheberg, Germany. [Kim, Soo-Hyung] Univ Washington, Sch Environm & Forest Sci, Seattle, WA 98195 USA. [Kumar, Naresh S.; Waha, Katharina] Indian Agr Res Inst, Ctr Environm Sci & Climate Resilient Agr, New Delhi 110012, India. [Mueller, Christoph] Potsdam Inst Climate Impact Res, D-14412 Potsdam, Germany. [Tao, Fulu] Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China. [Teixeira, Edmar] New Zealand Inst Plant & Food Res Ltd, Sustainable Prod, Canterbury, New Zealand. [Timlin, Dennis] USDA ARS, Crop Syst & Global Change Lab, Beltsville, MD 20705 USA. RP Durand, JL (reprint author), INRA, Unite Rech Pluridisciplinaire Prairie & Plantes F, BP 80006, F-86600 Lusignan, France. EM jean-louis.durand@lusignan.inra.fr RI Kim, Soo-Hyung/A-3012-2009; Priesack, Eckart/M-7341-2014; Deryng, Delphine/F-7417-2010; Nendel, Claas/C-8844-2013; Basso, Bruno/A-3128-2012; Teixeira, Edmar/K-1238-2016; Mueller, Christoph/E-4812-2016; De Sanctis, Giacomo/F-3498-2017; OI Priesack, Eckart/0000-0002-5088-9528; Kim, Soo-Hyung/0000-0003-3879-4080; Deryng, Delphine/0000-0001-6214-7241; Nendel, Claas/0000-0001-7608-9097; Basso, Bruno/0000-0003-2090-4616; Teixeira, Edmar/0000-0002-4835-0590; Mueller, Christoph/0000-0002-9491-3550; De Sanctis, Giacomo/0000-0002-3527-8091; Shcherbak@qut.edu.au, Iurii/0000-0003-4153-3770; Boote, Kenneth/0000-0002-1358-5496; Kersebaum, Kurt Christian/0000-0002-3679-8427 NR 72 TC 96 Z9 97 U1 17 U2 175 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1354-1013 EI 1365-2486 J9 GLOBAL CHANGE BIOL JI Glob. Change Biol. PD JUL PY 2014 VL 20 IS 7 BP 2301 EP 2320 DI 10.1111/gcb.12520 PG 20 WC Biodiversity Conservation; Ecology; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA AJ4WU UT WOS:000337680700025 PM 24395589 ER PT J AU White, JA AF White, Joshua A. TI Anisotropic damage of rock joints during cyclic loading: constitutive framework and numerical integration SO INTERNATIONAL JOURNAL FOR NUMERICAL AND ANALYTICAL METHODS IN GEOMECHANICS LA English DT Article DE joints; fractures; anisotropy; damage; implicit integration ID ASPERITY DEGRADATION; SHEAR; MODEL; PLASTICITY; FRICTION; BEHAVIOR AB This work describes a constitutive framework for modeling the behavior of rough joints under cyclic loading. Particular attention is paid to the intrinsic links between dilatancy, surface degradation, and mobilized shear strength. The framework also accounts for the important effect of shear-induced anisotropy. The resulting approach is fully three-dimensional and is not restricted to plane-displacement kinematics. Both the governing formulation and an algorithm for implicit numerical integration are presented. While the proposed methods are general, we also postulate a specific model that is compared with experimental data. It employs relatively few free parameters but shows good agreement with laboratory tests. Copyright (c) 2013 John Wiley & Sons, Ltd. C1 Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. RP White, JA (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. EM jawhite@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. The author is grateful to Ronaldo Borja, Eric Herbold, and two anonymous reviewers for helpful comments. NR 28 TC 1 Z9 1 U1 1 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-9061 EI 1096-9853 J9 INT J NUMER ANAL MET JI Int. J. Numer. Anal. Methods Geomech. PD JUL PY 2014 VL 38 IS 10 BP 1036 EP 1057 DI 10.1002/nag.2247 PG 22 WC Engineering, Geological; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA AJ3WR UT WOS:000337599100003 ER PT J AU Koissin, V Demcenko, A Korneev, VA AF Koissin, V. Demcenko, A. Korneev, V. A. TI Isothermal epoxy-cure monitoring using nonlinear ultrasonics SO INTERNATIONAL JOURNAL OF ADHESION AND ADHESIVES LA English DT Article DE Epoxy; Cure kinetics; Nonlinear ultrasonics; Calorimetry; Rheometry; Glass transition; Vitrification ID DIFFERENTIAL SCANNING CALORIMETRY; VELOCITY-MEASUREMENTS; REAL-TIME; RESIN; WAVES; SHEAR; COMPRESSION; ADHESIVES; POLYMERIZATION; VITRIFICATION AB Isothermal curing of LY 1564SP resin in an aluminium-adhesive-aluminium laminate is investigated, using a nonlinear ultrasonic immersion technique, to prove its applicability for this type of dynamic material transformation. For verification and comparison, epoxy-cure kinetics and theological behavior are measured using differential scanning calorimetery (DSC) and dynamic mechanical analysis (DMA). Results reveal that the nonlinear ultrasonics, based on noncollinear wave mixing, can successfully be applied to in situ epoxy-cure monitoring-for example, to adhesive bonds-with reliable detection of gelation and vitrification time instants. (C) 2014 Published by Elsevier Ltd. C1 [Koissin, V.; Demcenko, A.] Univ Twente, Fac Engn Technol, NL-7500 AE Enschede, Netherlands. [Korneev, V. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Demcenko, A (reprint author), Univ Twente, Fac Engn Technol, NL-7500 AE Enschede, Netherlands. EM andriejus.demcenko@gmail.com OI Koissin, Vitaly/0000-0001-9639-6537 FU Office of Energy Research, Office of Basic Energy Sciences, Engineering and Geosciences Division, of the U.S. Department of Energy [DE-ACO2-05CH11231] FX Dr. Ir. Roy Visser and Mr. Bert Vos (University of Twente) are gratefully acknowledged for their help with DMA and DSC tests. This work was partially supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Engineering and Geosciences Division, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. NR 38 TC 4 Z9 6 U1 3 U2 14 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0143-7496 EI 1879-0127 J9 INT J ADHES ADHES JI Int. J. Adhes. Adhes. PD JUL PY 2014 VL 52 BP 11 EP 18 DI 10.1016/j.ijadhadh.2014.01.003 PG 8 WC Engineering, Chemical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA AJ4NJ UT WOS:000337652800002 ER PT J AU McCauley, SJ Davis, CJ Werner, EE Robeson, MS AF McCauley, Shannon J. Davis, Christopher J. Werner, Earl E. Robeson, Michael S., II TI Dispersal, niche breadth and population extinction: colonization ratios predict range size in North American dragonflies SO JOURNAL OF ANIMAL ECOLOGY LA English DT Article DE dispersal limitation; extinction-colonization; freshwater connectivity; geographic distribution; niche breadth; Odonata; range limits; range size ID GEOGRAPHIC RANGE; REGIONAL PROCESSES; CLIMATE-CHANGE; BODY-SIZE; TRAITS; OCCUPANCY; ABUNDANCE; SHIFTS; LIMITS; WATER AB Species' range sizes are shaped by fundamental differences in species' ecological and evolutionary characteristics, and understanding the mechanisms determining range size can shed light on the factors responsible for generating and structuring biological diversity. Moreover, because geographic range size is associated with a species' risk of extinction and their ability to respond to global changes in climate and land use, understanding these mechanisms has important conservation implications. Despite the hypotheses that dispersal behaviour is a strong determinant of species range areas, few data are available to directly compare the relationship between dispersal behaviour and range size. Here, we overcome this limitation by combining data from a multispecies dispersal experiment with additional species-level trait data that are commonly hypothesized to affect range size (e.g. niche breadth, local abundance and body size.). This enables us to examine the relationship between these species-level traits and range size across North America for fifteen dragonfly species. Ten models based on a priori predictions about the relationship between species traits and range size were evaluated and two models were identified as good predictors of species range size. These models indicated that only two species' level traits, dispersal behaviour and niche breadth were strongly related to range size. The evidence from these two models indicated that dragonfly species that disperse more often and further had larger North American ranges. Extinction and colonization dynamics are expected to be a key linkage between dispersal behaviour and range size in dragonflies. To evaluate how extinction and colonization dynamics among dragonflies were related to range size we used an independent data set of extinction and colonization rates for eleven dragonfly species and assessed the relationship between these populations rates and North American range areas for these species. We found a negative relationship between North American range size and species' extinction-to-colonization ratios. Our results indicate that metapopulation dynamics act to shape the extent of species' continental distributions. These population dynamics are likely to interact with dispersal behaviour, particularly at species range margins, to determine range limits and ultimately species range sizes. C1 [McCauley, Shannon J.] Univ Toronto, Dept Biol, Mississauga, ON L5L 1C6, Canada. [McCauley, Shannon J.] Univ Toronto, Dept Ecol & Evolutionary Biol, Toronto, ON M5S 3B2, Canada. [Davis, Christopher J.; Werner, Earl E.] Univ Michigan, Dept Ecol & Evolutionary Biol, Ann Arbor, MI 48109 USA. [Robeson, Michael S., II] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA. RP McCauley, SJ (reprint author), Univ Toronto, Dept Biol, 3359 Mississauga Rd North, Mississauga, ON L5L 1C6, Canada. EM shannon.mccauley@utoronto.ca OI Robeson, Michael/0000-0001-7119-6301; McCauley, Shannon/0000-0001-9649-6693 FU Natural Science and Engineering Research Council; NSF LTREB [DEB-9727014, DEB-0454519] FX We thank M. Benard, M-J. Fortin, L. Rowe, and two anonymous reviewers for comments and discussion on the manuscript. S.J.M. was supported by Natural Science and Engineering Research Council grants to L. Rowe and M-J. Fortin while conducting this research and initial preparation of this manuscript. We are grateful to M. Benard, J. Hovermann, R. Relyea, D. Skelly, K. Yurewicz and the numerous research assistants and volunteers who have conducting surveys of habitats on the E.S. George Reserve. We also thank J. Abbott for compiling the distributional data for North American odonates and making species distribution maps accessible through OdonataCentral. The Museum of Zoology provided access to and logistical support at E. S. George Reserve where data on dispersal behaviour and species niche breadth were collected. This work was supported by NSF LTREB Grants DEB-9727014 and DEB-0454519. NR 42 TC 6 Z9 7 U1 7 U2 70 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8790 EI 1365-2656 J9 J ANIM ECOL JI J. Anim. Ecol. PD JUL PY 2014 VL 83 IS 4 BP 858 EP 865 DI 10.1111/1365-2656.12181 PG 8 WC Ecology; Zoology SC Environmental Sciences & Ecology; Zoology GA AJ4CO UT WOS:000337618100012 PM 24237364 ER PT J AU Craig, EA Wang, NC Zhao, QJ AF Craig, Evisabel A. Wang, Nina Ching Zhao, Q. Jay TI Using quantitative structure-activity relationship modeling to quantitatively predict the developmental toxicity of halogenated azole compounds SO JOURNAL OF APPLIED TOXICOLOGY LA English DT Article DE QSAR; developmental toxicity; halogenated compounds; azoles ID VALIDATION; ACCEPTANCE; RISK AB Developmental toxicity is a relevant endpoint for the comprehensive assessment of human health risk from chemical exposure. However, animal developmental toxicity data remain unavailable for many environmental contaminants due to the complexity and cost of these types of analyses. Here we describe an approach that uses quantitative structure-activity relationship modeling as an alternative methodology to fill data gaps in the developmental toxicity profile of certain halogenated compounds. Chemical information was obtained and curated using the OECD Quantitative Structure-Activity Relationship Toolbox, version 3.0. Data from 35 curated compounds were analyzed via linear regression to build the predictive model, which has an R2 of 0.79 and a Q2 of 0.77. The applicability domain (AD) was defined by chemical category and structural similarity. Seven halogenated chemicals that fit the AD but are not part of the training set were employed for external validation purposes. Our model predicted lowest observed adverse effect level values with a maximal threefold deviation from the observed experimental values for all chemicals that fit the AD. The good predictability of our model suggests that this method may be applicable to the analysis of qualifying compounds whenever developmental toxicity information is lacking or incomplete for risk assessment considerations. Copyright (c) 2013 John Wiley & Sons, Ltd. C1 [Craig, Evisabel A.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Craig, Evisabel A.; Wang, Nina Ching; Zhao, Q. Jay] US EPA, Natl Ctr Environm Assessment, Off Res Dev, Cincinnati, OH 45268 USA. RP Zhao, QJ (reprint author), US EPA, Natl Ctr Environm Assessment, Off Res Dev, Cincinnati, OH 45268 USA. EM zhao.jay@epa.gov FU U.S. Department of Energy; EPA FX The authors wish to thank Drs. Scott Wesselkamper and Dan Petersen for their critical review of this manuscript. The views expressed in this report are those of the authors and do not necessarily represent the views or policies of the U.S. Environmental Protection Agency. Mention of trade names or commercial products does not constitute endorsement. This study was supported in part by the research participation program administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and EPA. NR 21 TC 0 Z9 0 U1 0 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0260-437X EI 1099-1263 J9 J APPL TOXICOL JI J. Appl. Toxicol. PD JUL PY 2014 VL 34 IS 7 BP 787 EP 794 DI 10.1002/jat.2940 PG 8 WC Toxicology SC Toxicology GA AJ3PJ UT WOS:000337578900006 PM 24122872 ER PT J AU Miller, A Wang, YF AF Miller, Andrew Wang, Yifeng TI Al-O-F materials as novel adsorbents for gaseous radioiodine capture SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Re-processing; Waste treatment; Iodine; Nanoporosity; Nanoporous materials ID SOL-GEL SYNTHESIS; METAL FLUORIDES; IODINE AB Re-processing used nuclear fuel requires a method to effectively capture and dispose of gaseous radioiodine. Previous work has shown that nanoporous Al-O materials are effective at capturing gaseous iodine; molecular dynamics simulations have shown that the addition of fluoride to the Al-O surface should increase the amount of iodine capture. Twelve different materials with different ratios of F:Al were created. These materials were chemically characterized and functionally characterized with respect to gaseous iodine uptake. The addition of fluoride does in fact lead to a substantial (10-100x) increase in iodine uptake per unit surface area. However, the amount of uptake does not appear to be directly related to the total fluoride content of the solid phase material. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Miller, Andrew; Wang, Yifeng] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Miller, A (reprint author), Sandia Natl Labs, 1515 Eubank Dr SE, Albuquerque, NM 87123 USA. EM andmill@sandia.gov FU Sandia Corporation; Lockheed Martin Company; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration, under contract DE-AC04-94AL85000. The synthesis and analytical work was greatly aided by Jessica Kruichak and Melissa Mills. NR 13 TC 3 Z9 3 U1 2 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD JUL PY 2014 VL 133 SI SI BP 35 EP 39 DI 10.1016/j.jenvrad.2013.02.018 PG 5 WC Environmental Sciences SC Environmental Sciences & Ecology GA AJ3GU UT WOS:000337555300007 PM 23582500 ER PT J AU Kochersberger, K Kroeger, K Krawiec, B Brewer, E Weber, T AF Kochersberger, Kevin Kroeger, Kenneth Krawiec, Bryan Brewer, Eric Weber, Thomas TI Post-disaster Remote Sensing and Sampling via an Autonomous Helicopter SO JOURNAL OF FIELD ROBOTICS LA English DT Article ID SEARCH AB An unmanned remote sensing and sampling system has been developed to aid first responders in urban disaster assessment and recovery. The system design is based on a 90 kg autonomous helicopter platform with interchangeable payloads ranging from radiation detection to tethered robot deployment. A typical response would begin with three-dimensional terrain mapping using the stereovision system and a survey of radiation levels with an onboard spectrometer. From this initial survey, amore targeted flight is planned at a lower altitude with the option to localize radioactive sources in the event that radiation is present. Finally, a robot can be tether-deployed into the area of interest to collect samples. It is teleoperated from the ground control station, and after collection is finished the robot is retracted back to the helicopter for retrieval. The terrain mapping, radiation detection, radiation localization, and robot deployment and retrieval have all been flight-tested. Results of these tests indicate that the systems functioned successfully in the context of a prototype demonstrator. (C) 2014 Wiley Periodicals, Inc. C1 [Kochersberger, Kevin] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. [Kroeger, Kenneth] Virginia Tech, Blacksburg, VA 24061 USA. [Krawiec, Bryan; Brewer, Eric] Rockwell Collin, Warrenton, VA 20187 USA. [Weber, Thomas] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Kochersberger, K (reprint author), Virginia Tech, Dept Mech Engn, 114 Randolph Hall, Blacksburg, VA 24061 USA. EM kbk@vt.edu; k609041@vt.edu; bmkrawie@rockwellcollins.com; etbrewer@rockwellcollins.com; tmweber@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 22 TC 2 Z9 2 U1 1 U2 16 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1556-4959 EI 1556-4967 J9 J FIELD ROBOT JI J. Field Robot. PD JUL-AUG PY 2014 VL 31 IS 4 SI SI BP 510 EP 521 DI 10.1002/rob.21502 PG 12 WC Robotics SC Robotics GA AJ4WI UT WOS:000337679200003 ER PT J AU Xia, GG Chen, BW Zhang, R Zhang, ZC AF Xia, Guan-Guang Chen, Baowei Zhang, Rui Zhang, Z. Conrad TI Catalytic hydrolytic cleavage and oxy-cleavage of lignin linkages SO JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL LA English DT Article DE Lignin depolymerisation; Organic base; Catalyst; Hydrolytic cleavage; Oxy-cleavage ID ORGANIC MEDIA; DEGRADATION; DEPOLYMERIZATION; SPECTROMETRY; CHEMICALS; BIOMASS; WATER; WOOD AB In this work, new strategies involving organic bases were evaluated to depolymerize lignin to reduced molecular fragments in aqueous medium. NaOH as an inorganic base was also investigated as a reference. Full nature lignin samples were used for the study. As research tools to unravel the complexity of the macro lignin structure and bulky molecular size under this study, size exclusion chromatography and high resolution mass spectrometric analysis, typically used for protein characterizations, were used to follow the progress of lignin depolymerisation by measuring the molecular weight distribution of the products and determining the key molecular mass fingerprints, respectively. The results show that sodium phenoxide and guanidine carbonate are effective catalysts for lignin depolymerization. It is observed that the organic bases enhance the oxy-cleavage effect of H2O2, which is strongest with guanidine carbonate. (C) 2013 Elsevier B.V. All rights reserved. C1 [Xia, Guan-Guang; Chen, Baowei; Zhang, Rui; Zhang, Z. Conrad] Pacific NW Natl Lab, Richland, WA 99352 USA. [Zhang, Z. Conrad] Dalian Inst Chem Physcis, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian, Peoples R China. RP Zhang, ZC (reprint author), Dalian Natl Lab Clean Energy, 457 Zhongshan Rd, Dalian 116023, Peoples R China. EM zczhang@yahoo.com FU Laboratory Directed Research and Development Program at the PNNL; Battelle for the U.S. DOE [AC06-76RL01830] FX This work was supported by the Laboratory Directed Research and Development Program at the PNNL, a multiprogram national laboratory operated by Battelle for the U.S. DOE under contract no. DE-AC06-76RL01830. Part of the research described in this paper was performed at the Environmental Molecular Science Laboratory, a national scientific user facility located at PNNL. NR 18 TC 5 Z9 5 U1 3 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1381-1169 EI 1873-314X J9 J MOL CATAL A-CHEM JI J. Mol. Catal. A-Chem. PD JUL PY 2014 VL 388 SI SI BP 35 EP 40 DI 10.1016/j.molcata.2013.08.016 PG 6 WC Chemistry, Physical SC Chemistry GA AJ3FL UT WOS:000337551800003 ER PT J AU Shatsky, M Arbelaez, P Han, BG Typke, D Brenner, SE Malik, J Glaeser, RM AF Shatsky, Maxim Arbelaez, Pablo Han, Bong-Gyoon Typke, Dieter Brenner, Steven E. Malik, Jitendra Glaeser, Robert M. TI Automated particle correspondence and accurate tilt-axis detection in tilted-image pairs SO JOURNAL OF STRUCTURAL BIOLOGY LA English DT Article DE Particle correspondence; Tilted pairs; Tilt-axis detection ID RANDOM CONICAL TILT; ELECTRON-MICROSCOPY; BIOLOGICAL MACROMOLECULES; RECONSTRUCTION METHOD; 3-D RECONSTRUCTION; SPECIMEN; CRYOMICROSCOPY; ORIENTATION; HANDEDNESS; RESOLUTION AB Tilted electron microscope images are routinely collected for an ab initio structure reconstruction as a part of the Random Conical Tilt (RCT) or Orthogonal Tilt Reconstruction (OTR) methods, as well as for various applications using the "free-hand" procedure. These procedures all require identification of particle pairs in two corresponding images as well as accurate estimation of the tilt-axis used to rotate the electron microscope (EM) grid. Here we present a computational approach, PCT (particle correspondence from tilted pairs), based on tilt-invariant context and projection matching that addresses both problems. The method benefits from treating the two problems as a single optimization task. It automatically finds corresponding particle pairs and accurately computes tilt-axis direction even in the cases when EM grid is not perfectly planar. (C) 2014 The Authors. Published by Elsevier Inc. C1 [Shatsky, Maxim; Brenner, Steven E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Arbelaez, Pablo; Malik, Jitendra] Univ Calif Berkeley, Elect Engn & Comp Sci Div, Berkeley, CA 94720 USA. [Han, Bong-Gyoon; Typke, Dieter; Glaeser, Robert M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Brenner, Steven E.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Shatsky, M (reprint author), Univ Calif Berkeley, 461 Koshland Hall, Berkeley, CA 94720 USA. EM max.shatsky@gmail.com RI Brenner, Steven/A-8729-2008; OI Brenner, Steven/0000-0001-7559-6185; Arbelaez, Pablo/0000-0001-5244-2407 FU Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-ACO2-05CH11231] FX We thank Florian Hauer and Holger Strak for providing program Maverick Tilt. This work conducted by ENIGMA - Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory, was supported by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under Contract No. DE-ACO2-05CH11231. NR 29 TC 3 Z9 3 U1 2 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1047-8477 EI 1095-8657 J9 J STRUCT BIOL JI J. Struct. Biol. PD JUL PY 2014 VL 187 IS 1 BP 66 EP 75 DI 10.1016/j.jsb.2014.03.017 PG 10 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA AJ6DD UT WOS:000337779000008 PM 24694675 ER PT J AU Labbe, J Uehling, J Payen, T Plett, J AF Labbe, Jessy Uehling, Jessie Payen, Thibaut Plett, Jonathan TI Fungal biology: compiling genomes and exploiting them SO NEW PHYTOLOGIST LA English DT Editorial Material DE effectors; fungal evolution; fungal genetics and genomics; mycorrhizal fungi; pathogenic and mutualistic interactions; saprotrophs; symbiosis C1 [Labbe, Jessy] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Uehling, Jessie] Duke Univ, Dept Biol, Durham, NC 27708 USA. [Payen, Thibaut] Lorraine Univ, Lab Excellence ARBRE, INRA, UMR 1136, F-54280 Nancy, Champenoux, France. [Plett, Jonathan] Univ Western Sydney, Hawkesbury Inst Environm, Richmond, NSW, Australia. RP Labbe, J (reprint author), Oak Ridge Natl Lab, Biosci Div, POB 2008, Oak Ridge, TN 37831 USA. EM labbejj@ornl.gov RI Labbe, Jessy/G-9532-2011; OI Labbe, Jessy/0000-0003-0368-2054; Plett, Jonathan/0000-0003-0514-8146 FU Genomic Science Program (project 'Plant-Microbe Interactions'), US Department of Energy, Office of Science, Biological and Environmental Research [DE-AC05-00OR22725] FX Many thanks to Krista Plett and Francis Martin for helpful comments on the manuscript. Thanks also to all who attended and gave freely of their data, thoughts and opinions. The authors acknowledge the Genomic Science Program (project 'Plant-Microbe Interactions'), US Department of Energy, Office of Science, Biological and Environmental Research, for supporting the authors' participation to this meeting, under the contract DE-AC05-00OR22725. NR 7 TC 1 Z9 1 U1 0 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD JUL PY 2014 VL 203 IS 2 BP 359 EP 361 DI 10.1111/nph.12891 PG 3 WC Plant Sciences SC Plant Sciences GA AJ4IW UT WOS:000337639800004 PM 24942153 ER PT J AU McKown, AD Klapste, J Guy, RD Geraldes, A Porth, I Hannemann, J Friedmann, M Muchero, W Tuskan, GA Ehlting, J Cronk, QCB El-Kassaby, YA Mansfield, SD Douglas, CJ AF McKown, Athena D. Klapste, Jaroslav Guy, Robert D. Geraldes, Armando Porth, Ilga Hannemann, Jan Friedmann, Michael Muchero, Wellington Tuskan, Gerald A. Ehlting, Juergen Cronk, Quentin C. B. El-Kassaby, Yousry A. Mansfield, Shawn D. Douglas, Carl J. TI Genome-wide association implicates numerous genes underlying ecological trait variation in natural populations of Populus trichocarpa SO NEW PHYTOLOGIST LA English DT Article DE biomass; ecophysiology; genome-wide association study (GWAS); phenology; pleiotropy; poplar; single nucleotide polymorphisms (SNP) array; Unified Mixed Model ID CARBON-ISOTOPE DISCRIMINATION; MULTILOCUS GENOTYPE DATA; SPRUCE PICEA-SITCHENSIS; PINE PINUS-TAEDA; LOCAL ADAPTATION; BLACK COTTONWOOD; BALSAMIFERA L.; COMPLEX TRAITS; PHENOTYPIC ASSOCIATIONS; ARABIDOPSIS-THALIANA AB In order to uncover the genetic basis of phenotypic trait variation, we used 448 unrelated wild accessions of black cottonwood (Populus trichocarpa) from much of its range in western North America. Extensive data from large-scale trait phenotyping (with spatial and temporal replications within a common garden) and genotyping (with a 34K Populus single nucleotide polymorphism (SNP) array) of all accessions were used for gene discovery in a genome-wide association study (GWAS). We performed GWAS with 40 biomass, ecophysiology and phenology traits and 29355 filtered SNPs representing 3518 genes. The association analyses were carried out using a Unified Mixed Model accounting for population structure effects among accessions. We uncovered 410 significant SNPs using a Bonferroni-corrected threshold (P<1.7x10-6). Markers were found across 19 chromosomes, explained 1-13% of trait variation, and implicated 275 unique genes in trait associations. Phenology had the largest number of associated genes (240 genes), followed by biomass (53 genes) and ecophysiology traits (25 genes). The GWAS results propose numerous loci for further investigation. Many traits had significant associations with multiple genes, underscoring their genetic complexity. Genes were also identified with multiple trait associations within and/or across trait categories. In some cases, traits were genetically correlated while in others they were not. C1 [McKown, Athena D.; Klapste, Jaroslav; Guy, Robert D.; Porth, Ilga; El-Kassaby, Yousry A.] Univ British Columbia, Forest Sci Ctr, Fac Forestry, Dept Forest & Conservat Sci, Vancouver, BC V6T 1Z4, Canada. [Klapste, Jaroslav] Czech Univ Life Sci, Fac Forestry & Wood Sci, Dept Dendrol & Forest Tree Breeding, Prague 16521, Czech Republic. [Geraldes, Armando; Friedmann, Michael; Cronk, Quentin C. B.; Douglas, Carl J.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [Porth, Ilga; Mansfield, Shawn D.] Univ British Columbia, Forest Sci Ctr, Fac Forestry, Dept Wood Sci, Vancouver, BC V6T 1Z4, Canada. [Hannemann, Jan; Ehlting, Juergen] Univ Victoria, Dept Biol, Victoria, BC V8W 3N5, Canada. [Hannemann, Jan; Ehlting, Juergen] Univ Victoria, Ctr Forest Biol, Victoria, BC V8W 3N5, Canada. [Muchero, Wellington; Tuskan, Gerald A.] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA. RP McKown, AD (reprint author), Univ British Columbia, Forest Sci Ctr, Fac Forestry, Dept Forest & Conservat Sci, 2424 Main Mall, Vancouver, BC V6T 1Z4, Canada. EM admckown@gmail.com RI Klapste, Jaroslav/B-6668-2016; Porth, Ilga/N-4862-2015; El-Kassaby, Yousry/K-9856-2016; Tuskan, Gerald/A-6225-2011; OI Klapste, Jaroslav/0000-0001-5504-3735; Porth, Ilga/0000-0002-9344-6348; El-Kassaby, Yousry/0000-0002-4887-8977; Tuskan, Gerald/0000-0003-0106-1289; McKown, Athena/0000-0002-7402-9952; Cronk, Quentin/0000-0002-4027-7368 FU Genome British Columbia Applied Genomics Innovation Program [103BIO]; Genome Canada Large-Scale Applied Research Project [168BIO]; US Department of Energy Bioenergy Research Facility [DE-AC05-00OR22725] FX We thank L. E. Gunter, M. S. Azam, E. Drewes, N. Farzaneh, L. Liao, E. Moreno, L. Muenter and L. Quamme for data monitoring, collection and image presentation. We also thank anonymous reviewers for their suggestions and revisions in improving the manuscript. This work was supported by the Genome British Columbia Applied Genomics Innovation Program (Project 103BIO) and Genome Canada Large-Scale Applied Research Project (Project 168BIO) funds to R. D. G., J.E., Q. C. B. C., Y.A.E-K., S. D. M. and C.J.D. and by funds within the BioEnergy Science Center, a US Department of Energy Bioenergy Research Facility under contract DE-AC05-00OR22725. NR 89 TC 40 Z9 40 U1 11 U2 93 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD JUL PY 2014 VL 203 IS 2 BP 535 EP 553 DI 10.1111/nph.12815 PG 19 WC Plant Sciences SC Plant Sciences GA AJ4IW UT WOS:000337639800019 PM 24750093 ER PT J AU Kim, TN AF Kim, Tania N. TI Plant damage and herbivore performance change with latitude for two old-field plant species, but rarely as predicted SO OIKOS LA English DT Article ID SOLANUM-CAROLINENSE; SOLIDAGO-ALTISSIMA; INSECT HERBIVORES; PROTEASE INHIBITORS; FLORAL HERBIVORY; SALT MARSHES; RESISTANCE; TOLERANCE; TRAITS; COMPETITION AB A long standing hypothesis in biogeography is that latitudinal gradients in plant defenses (LGPD) should arise because selection for plant defenses is greater in the tropics compared to temperate areas. Previous studies have focused on plant traits thought to confer resistance, yet many traits may not actually confer resistance (putative resistance) or interact to influence herbivore performance. In this study, I used a multi-trophic approach to examine relationships between latitude, herbivore pressure, and plant resistance (measured as the growth rates of herbivores) of two old-field plant species (Solanum carolinense and Solidago altissima) using a field survey across a 12 degree gradient in the eastern US combined with laboratory bioassays measuring the performance of generalist and specialist herbivores. I used structural equation modeling to examine the direct and indirect pathways by which latitude influences herbivore pressure and plant resistance. A latitudinal gradient in plant damage was observed in the expected direction for S. caroliense (damage decreased with latitude), but the opposite relationship was observed for S. altissima. Damage to both plant species was mediated by herbivore abundances, which was in turn influenced by predator abundances. Resistance to herbivores also varied with latitude but the form of the relationship was dependent on herbivore and plant species. There were direct, non-linear relationships between latitude and resistance (for Spodoptera exigua and Schistocerca americana feeding on S. altissima; S. exigua and Manduca sexta feeding on S. carolinense). Herbivore growth rates were also mediated by the density of S. carolinense for Leptinotarsa juncta and S. americana feeding on S. carolinense. There was no relationship between plant resistance and herbivore pressure and no indication of feedbacks. Results from this study indicate that latitudinal variation in plant resistance is complex, possibly constrained by resource availability and tradeoffs in plant defenses. C1 [Kim, Tania N.] Florida State Univ, Dept Biol Sci, Tallahassee, FL 32306 USA. RP Kim, TN (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. EM tkim@glbrc.wisc.edu FU Florida State Univ., Florida, USA FX I gratefully acknowledge M. Cipollini (Berry College, Georgia, USA), G. Crutsinger and L. Souza (Univ. of Tennessee, Tennessee, USA), M. Wise and D. Carr (Blandy Experimental Farm, Virginia, USA), and S. Campbell (Cornell Univ., New York, USA) for logistical support during latitudinal field surveys. I thank J. Capinera (Univ. of Florida, Florida, USA) for providing grasshoppers for bioassays. I thank J. Stanford for lab and greenhouse assistance. This manuscript was greatly improved by comments from N. Underwood, B. Spiesman, J. Grinath and A. Hakes. The Robert K. Godfrey Endowment Award for the Study of Botany (Florida State Univ., Florida, USA) helped fund this research. NR 54 TC 7 Z9 7 U1 13 U2 50 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0030-1299 EI 1600-0706 J9 OIKOS JI Oikos PD JUL PY 2014 VL 123 IS 7 BP 886 EP 896 DI 10.1111/j.1600-0706.2013.00946.x PG 11 WC Ecology SC Environmental Sciences & Ecology GA AJ5RP UT WOS:000337744900014 ER PT J AU Su, CC Radhakrishnan, A Kumar, N Long, F Bolla, JR Lei, HT Delmar, JA Do, SV Chou, TH Rajashankar, KR Zhang, QJ Yu, EW AF Su, Chih-Chia Radhakrishnan, Abhijith Kumar, Nitin Long, Feng Bolla, Jani Reddy Lei, Hsiang-Ting Delmar, Jared A. Do, Sylvia V. Chou, Tsung-Han Rajashankar, Kanagalaghatta R. Zhang, Qijing Yu, Edward W. TI Crystal structure of the Campylobacter jejuni CmeC outer membrane channel SO PROTEIN SCIENCE LA English DT Article DE efflux channel; multidrug resistance; resistance-nodulation-cell division; Campylobacter jejuni; membrane protein ID MULTIDRUG EFFLUX PUMP; PSEUDOMONAS-AERUGINOSA; FLUOROQUINOLONE RESISTANCE; MACROLIDE RESISTANCE; ACRB; PROTEIN; CMEABC; TRANSPORTER; SOFTWARE; SYSTEM AB As one of the world's most prevalent enteric pathogens, Campylobacter jejuni is a major causative agent of human enterocolitis and is responsible for more than 400 million cases of diarrhea each year. The impact of this pathogen on children is of particular significance. Campylobacter has developed resistance to many antimicrobial agents via multidrug efflux machinery. The CmeABC tripartite multidrug efflux pump, belonging to the resistance-nodulation-cell division (RND) superfamily, plays a major role in drug resistant phenotypes of C. jejuni. This efflux complex spans the entire cell envelop of C. jejuni and mediates resistance to various antibiotics and toxic compounds. We here report the crystal structure of C. jejuni CmeC, the outer membrane component of the CmeABC tripartite multidrug efflux system. The structure reveals a possible mechanism for substrate export. C1 [Su, Chih-Chia; Long, Feng; Delmar, Jared A.; Chou, Tsung-Han; Yu, Edward W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Radhakrishnan, Abhijith; Kumar, Nitin; Bolla, Jani Reddy; Lei, Hsiang-Ting; Yu, Edward W.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Do, Sylvia V.; Yu, Edward W.] Iowa State Univ, Bioinformat & Computat Biol Interdept Grad Progra, Ames, IA 50011 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, NE CAT, Argonne, IL 60439 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, Dept Chem & Chem Biol, Argonne, IL 60439 USA. [Zhang, Qijing] Iowa State Univ, Coll Vet Med, Dept Vet Microbiol, Ames, IA 50011 USA. RP Yu, EW (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM ewyu@iastate.edu RI Long, Feng/F-5475-2011 OI Long, Feng/0000-0001-6313-8558 FU NIH [R01DK063008, R01GM086431] FX Grant sponsor: NIH; Grant numbers: R01DK063008 (Q.Z.) and R01GM086431 (E.W.Y.). NR 38 TC 9 Z9 10 U1 2 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0961-8368 EI 1469-896X J9 PROTEIN SCI JI Protein Sci. PD JUL PY 2014 VL 23 IS 7 BP 954 EP 961 DI 10.1002/pro.2478 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AJ4TS UT WOS:000337669800011 PM 24753291 ER PT J AU Lohman, JR Ma, M Cuff, ME Bigelow, L Bearden, J Babnigg, G Joachimiak, A Phillips, GN Shen, B AF Lohman, Jeremy R. Ma, Ming Cuff, Marianne E. Bigelow, Lance Bearden, Jessica Babnigg, Gyorgy Joachimiak, Andrzej Phillips, George N., Jr. Shen, Ben TI The crystal structure of BlmI as a model for nonribosomal peptide synthetase peptidyl carrier proteins SO PROTEINS-STRUCTURE FUNCTION AND BIOINFORMATICS LA English DT Article DE protein-protein interaction; natural product; biosynthesis; phylogenetics; structural genomics; reductive methylation ID BIOSYNTHETIC GENE-CLUSTER; HIGH-THROUGHPUT; COMBINATORIAL MUTAGENESIS; SURFACTIN SYNTHETASE; SEQUENCE ALIGNMENTS; MAXIMUM-LIKELIHOOD; ADENYLATION; DOMAINS; CLONING; PURIFICATION AB Carrier proteins (CPs) play a critical role in the biosynthesis of various natural products, especially in nonribosomal peptide synthetase (NRPS) and polyketide synthase (PKS) enzymology, where the CPs are referred to as peptidyl-carrier proteins (PCPs) or acyl-carrier proteins (ACPs), respectively. CPs can either be a domain in large multifunctional polypeptides or standalone proteins, termed Type I and Type II, respectively. There have been many biochemical studies of the Type I PKS and NRPS CPs, and of Type II ACPs. However, recently a number of Type II PCPs have been found and biochemically characterized. In order to understand the possible interaction surfaces for combinatorial biosynthetic efforts we crystallized the first characterized and representative Type II PCP member, BlmI, from the bleomycin biosynthetic pathway from Streptomyces verticillus ATCC 15003. The structure is similar to CPs in general but most closely resembles PCPs. Comparisons with previously determined PCP structures in complex with catalytic domains reveals a common interaction surface. This surface is highly variable in charge and shape, which likely confers specificity for interactions. Previous nuclear magnetic resonance (NMR) analysis of a prototypical Type I PCP excised from the multimodular context revealed three conformational states. Comparison of the states with the structure of BlmI and other PCPs reveals that only one of the NMR states is found in other studies, suggesting the other two states may not be relevant. The state represented by the BlmI crystal structure can therefore serve as a model for both Type I and Type II PCPs. Proteins 2014; 82:1210-1218. (c) 2013 Wiley Periodicals, Inc. C1 [Lohman, Jeremy R.; Ma, Ming; Shen, Ben] Scripps Res Inst, Dept Chem, Jupiter, FL 33458 USA. [Cuff, Marianne E.; Bigelow, Lance; Bearden, Jessica; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Cuff, Marianne E.; Bigelow, Lance; Bearden, Jessica; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, Argonne, IL 60439 USA. [Phillips, George N., Jr.] Rice Univ, Dept Biochem & Cell Biol, Houston, TX 77251 USA. [Shen, Ben] Scripps Res Inst, Dept Mol Therapeut, Jupiter, FL 33458 USA. [Shen, Ben] Scripps Res Inst, Nat Prod Lib Initiat, Jupiter, FL 33458 USA. RP Shen, B (reprint author), Scripps Res Inst, 130 Scripps Way,3A1, Jupiter, FL 33458 USA. EM shenb@scripps.edu RI Lohman, Jeremy/M-1111-2015 OI Lohman, Jeremy/0000-0001-8199-2344 FU National Institute of General Medical Sciences Protein Structure Initiative [GM094596, GM094585]; National Institutes of Health [AI40475]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX Grant sponsor: National Institute of General Medical Sciences Protein Structure Initiative (to GNP and BS); Grant number: GM094596; Grant sponsor: National Institute of General Medical Sciences Protein Structure Initiative (to MC, LB, JB, GB, and AJ); Grant number: GM094585; Grant sponsor: National Institutes of Health (to BS); Grant number: AI40475; Grant sponsor: U.S. Department of Energy, Office of Biological and Environmental Research (to MC and AJ); Grant number: DE-AC02-06CH11357. NR 45 TC 16 Z9 16 U1 3 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-3585 EI 1097-0134 J9 PROTEINS JI Proteins PD JUL PY 2014 VL 82 IS 7 BP 1210 EP 1218 DI 10.1002/prot.24485 PG 9 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AJ2GV UT WOS:000337474700009 PM 25050442 ER PT J AU Takasuka, TE Bianchetti, CM Tobimatsu, Y Bergeman, LF Ralph, J Fox, BG AF Takasuka, Taichi E. Bianchetti, Christopher M. Tobimatsu, Yuki Bergeman, Lai F. Ralph, John Fox, Brian G. TI Structure-guided analysis of catalytic specificity of the abundantly secreted chitosanase SACTE_ 5457 from Streptomyces sp SirexAA-E SO PROTEINS-STRUCTURE FUNCTION AND BIOINFORMATICS LA English DT Article DE Streptomyces; chitosanase; chitosan; biomass degradation; X-ray structure; GH46 ID BACILLUS-CIRCULANS MH-K1; RECALCITRANT POLYSACCHARIDES; CRYSTAL-STRUCTURE; COELICOLOR A3(2); SP N174; PURIFICATION; SEQUENCE; CLONING; CHITIN; GENE AB SACTE_5457 is secreted by Streptomyces sp. SirexAA-E, a highly cellulolytic actinobacterium isolated from a symbiotic community composed of insects, fungi, and bacteria. Here we report the 1.84 angstrom resolution crystal structure and functional characterization of SACTE_5457. This enzyme is a member of the glycosyl hydrolase family 46 and is composed of two -helical domains that are connected by an -helical linker. The catalytic residues (Glu74 and Asp92) are separated by 10.3 angstrom, matching the distance predicted for an inverting hydrolysis reaction. Normal mode analysis suggests that the connecting -helix is flexible and allows the domain motion needed to place active site residues into an appropriate configuration for catalysis. SACTE_5457 does not react with chitin, but hydrolyzes chitosan substrates with an approximate to 4-fold improvement in k(cat)/K-M as the percentage of acetylation and the molecular weights decrease. Analysis of the time dependence of product formation shows that oligosaccharides with degree of polymerization <4 are not hydrolyzed. By combining the results of substrate docking to the X-ray structure and end-product analysis, we deduce that SACTE_5457 preferentially binds substrates spanning the -2 to +2 sugar binding subsites, and that steric hindrance prevents binding of N-acetyl-d-glucosamine in the +2 subsite and may weakly interfere with binding of N-acetyl-d-glucosamine in the +1 subsites. A proposal for how these constraints account for the observed product distributions is provided. Proteins 2014; 82:1245-1257. (c) 2013 Wiley Periodicals, Inc. C1 [Takasuka, Taichi E.; Bianchetti, Christopher M.; Tobimatsu, Yuki; Bergeman, Lai F.; Ralph, John; Fox, Brian G.] Univ Wisconsin, Dept Biochem, Madison, WI 53705 USA. [Takasuka, Taichi E.; Bianchetti, Christopher M.; Tobimatsu, Yuki; Bergeman, Lai F.; Ralph, John; Fox, Brian G.] Univ Wisconsin, Coll Engn, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. RP Fox, BG (reprint author), Univ Wisconsin, Dept Biochem, 420 Henry Mall, Madison, WI 53705 USA. EM bgfox@biochem.wisc.edu FU DOE Great Lakes Bioenergy Research Center (DOE Office of Science) [BER DE-FC02-07ER64494]; US Department of Energy, Basic Energy Sciences, Office of Science [W 31 109 ENG-38]; College of Agricultural and Life Sciences, Department of Biochemistry, the Graduate School of the University of Wisconsin; Michigan Economic Development Corporation; Michigan Technology Tri-Corridor [085P1000817] FX Grant sponsor: DOE Great Lakes Bioenergy Research Center (DOE Office of Science); Grant number: BER DE-FC02-07ER64494; Grant sponsor: US Department of Energy, Basic Energy Sciences, Office of Science; Grant number: W 31 109 ENG-38; Grant sponsor: College of Agricultural and Life Sciences, Department of Biochemistry, the Graduate School of the University of Wisconsin, the Michigan Economic Development Corporation, and the Michigan Technology Tri-Corridor; Grant number: 085P1000817. NR 63 TC 2 Z9 2 U1 1 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-3585 EI 1097-0134 J9 PROTEINS JI Proteins PD JUL PY 2014 VL 82 IS 7 BP 1245 EP 1257 DI 10.1002/prot.24491 PG 13 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AJ2GV UT WOS:000337474700012 PM 24338856 ER PT J AU Jungels, AM Brown, MA Stombler, M Yasumoto, S AF Jungels, Amanda M. Brown, Marni A. Stombler, Mindy Yasumoto, Saori TI Teaching Associates: Bridging Informal and Formal Mechanisms of Support for Graduate Student Instructors SO TEACHING SOCIOLOGY LA English DT Article DE formal networks; informal networks; bridging networks; teaching associate; graduate student instructors; director of instruction; graduate teacher training ID NETWORKS AB Faculty members and graduate student instructors (GSIs) spend a significant portion of their time in the classroom. Much of the literature calls for formal training for graduate students in pedagogy and teaching techniques (DeCesare 2003), and increasing attention has been paid to the benefits of informal supports for GSIs, such as peer networks. But scholars have paid far less attention to examining how formal and informal mechanisms of support might be bridged, thus strengthening support for GSIs. In this article, we explore and demonstrate the importance of bridging available support systems for GSIs, specifically through a position occupied by an advanced GSI, called the Teaching Associate. Using focus groups, semistructured interviews, and surveys, we argue that the Teaching Associate offers formal and informal forms of support for graduate student instructors and their departments and we advocate their use in teacher training. C1 [Jungels, Amanda M.] Oak Ridge Inst Sci & Educ, Baltimore, MD USA. [Brown, Marni A.] Georgia Gwinnett Coll, Lawrenceville, NJ USA. [Stombler, Mindy] Georgia State Univ, Dept Sociol, Atlanta, GA 30303 USA. [Yasumoto, Saori] Osaka Univ, Dept Human Sci, Program G30, Osaka, Japan. RP Stombler, M (reprint author), 38 Peachtree Ctr Ave,Langdale Hall Room 1041, Atlanta, GA 30303 USA. EM stombler@gsu.edu NR 17 TC 0 Z9 0 U1 2 U2 5 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 0092-055X EI 1939-862X J9 TEACH SOCIOL JI Teach. Sociol. PD JUL PY 2014 VL 42 IS 3 BP 220 EP 230 DI 10.1177/0092055X14527423 PG 11 WC Education & Educational Research; Sociology SC Education & Educational Research; Sociology GA AJ4CZ UT WOS:000337619400005 ER PT J AU Bhagatwala, A Chen, JH Lu, TF AF Bhagatwala, Ankit Chen, Jacqueline H. Lu, Tianfeng TI Direct numerical simulations of HCCl/SACI with ethanol SO COMBUSTION AND FLAME LA English DT Article DE HCCI; SACI; Thermal stratification; Mixture stratification; Premixed flame; Autoignition ID IGNITION FRONT PROPAGATION; EXPLOSIVE MODE ANALYSIS; TEMPERATURE INHOMOGENEITIES; CONSTANT VOLUME; DIAGNOSTICS; FLAMES; JET AB Two and three dimensional direct numerical simulations (DNS) of an autoignitive premixture of air and ethanol in Homogeneous Charge Compression Ignition (HCCI) mode have been conducted. A special feature of these simulations is the use of compression heating through mass source/sink terms to emulate the compression and expansion due to piston motion. Furthermore, combustion phasing is adjusted such that peak heat release occurs after Top Dead Center (TDC) during the expansion stroke, as in a real engine. Zero dimensional simulations were first conducted to identify important parameters for the higher dimensional simulations. They showed that for ethanol, temperature and dilution are the parameters the problem is most sensitive to. One set of two dimensional simulations were conducted with a uniform mixture composition and different levels of temperature stratification, both with and without compression heating. Another set of simulations varied the mixture stratification with constant temperature stratification. Both sets showed considerable differences in ignition delay, heat release and peak temperature and peak pressure. Compression heating was also found to have a significant effect on the heat release profile. A three dimensional simulation was conducted for Spark-Assisted HCCI (SACI). It was initiated with a small spark kernel, which evolved into a premixed flame. The entire mixture eventually underwent autoignition. Distance function based analysis showed a strongly attenuating flame. Analysis of scalar mixing frequencies shows that differential diffusion and reaction induced mixing play an important role in predicting the mixing of reactive scalars. This has significant implications for mixing models for reactive flows. Chemical explosive mode analysis (CEMA) was applied to the 3D simulation and showed promise in identifying the transition from flame propagation to autoignition. (C) 2014 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Bhagatwala, Ankit; Chen, Jacqueline H.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. [Lu, Tianfeng] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. RP Bhagatwala, A (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. EM abhagat@sandia.gov RI Lu, Tianfeng/D-7455-2014 OI Lu, Tianfeng/0000-0001-7536-1976 FU Combustion Energy Frontier Research Center (CEFRC), an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) [DE-SC0001198]; United States Department of Energy [DE-AC04-94AL85000]; Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-SC0008622]; Department of Energy's Advanced Leadership Computing Challenge (ALCC) at the National Energy Research Scientific Computing Center (NERSC) FX This research is supported by the Combustion Energy Frontier Research Center (CEFRC), an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) under Award No. DE-SC0001198. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000. The work at University of Connecticut was supported by the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy under Grant DE-SC0008622. Computer allocations were awarded by the Department of Energy's Advanced Leadership Computing Challenge (ALCC) at the National Energy Research Scientific Computing Center (NERSC). NR 35 TC 16 Z9 16 U1 5 U2 28 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 EI 1556-2921 J9 COMBUST FLAME JI Combust. Flame PD JUL PY 2014 VL 161 IS 7 BP 1826 EP 1841 DI 10.1016/j.combustflame.2013.12.027 PG 16 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA AI8TU UT WOS:000337200700013 ER PT J AU Anderson, EK Aslam, TD Jackson, SI AF Anderson, Eric K. Aslam, Tariq D. Jackson, Scott I. TI Transverse initiation of an insensitive explosive in a layered slab geometry: Front shapes and post-shock flow measurements SO COMBUSTION AND FLAME LA English DT Article DE Detonation; Shock; Explosive AB Experiments are presented that explore the shock initiating layer dynamics in an insensitive high explosive. Tests were conducted with a PBX 9502 slab bonded on one side to a PBX 9501 slab. For each test, a detonation in the PBX 9501 was generated to drive an oblique shock intended to initiate the PBX 9502. Shocks of sufficient strength generated an initiating layer, or region of delayed reaction (relative to typical PBX 9502 detonation reaction timescales) in the PBX 9502 immediately adjacent to the PBX 9501. These reactions result in a transition to detonation away from the 9501/9502 interface in a process analogous to the shock-to-detonation transition in shocked one-dimensional (1D) explosive configurations. The thickness of the PBX 9501 layer was varied from 0.5-2.5 mm to control the strength and duration of the transmitted shock into the 8 mm thick PBX 9502. Phase velocities at the explosive outer surfaces, wave front breakout shapes, and post shock particle velocity histories associated with the detonating and initiating zones in the two explosives are reported and discussed. The initiating layer thickness decreased with increasing PBX 9501 thickness for tests with PBX 9501 thicknesses larger than 1.0 mm. A 1.0 mm thick PBX 9501 slab was not able to initiate detonation in the 8.0 mm thick PBX 9502 slab. Further decreasing the PBX 9501 thickness to 0.5 mm resulted in detonation throughout both slabs, with no initiating layer due to the intersection of each explosive's thickness effect curve at this condition. Initiating layers exhibited particle velocity profiles characteristic of non-detonating shocks. Measured phase velocities are in good agreement with Detonation Shock Dynamics (DSD) predictions for PBX 9501. (C) 2014 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Anderson, Eric K.; Aslam, Tariq D.; Jackson, Scott I.] LANL, Shock & Detonat Phys Grp, Los Alamos, NM 87545 USA. RP Anderson, EK (reprint author), LANL, Shock & Detonat Phys Grp, WX-9, Los Alamos, NM 87545 USA. EM eanderson@lanl.gov OI Jackson, Scott/0000-0002-6814-3468; Aslam, Tariq/0000-0002-4263-0401; Anderson, Eric/0000-0002-5309-5686 FU US Department of Energy Campaign 2: "Dynamic Material Properties." FX This effort was funded by the US Department of Energy Campaign 2: "Dynamic Material Properties." Experiments were assembled and fielded with assistance provided by Sam Vincent and Tim Tucker. NR 19 TC 1 Z9 1 U1 0 U2 15 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 EI 1556-2921 J9 COMBUST FLAME JI Combust. Flame PD JUL PY 2014 VL 161 IS 7 BP 1944 EP 1954 DI 10.1016/j.combustflame.2013.12.023 PG 11 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA AI8TU UT WOS:000337200700022 ER PT J AU Dale, VH AF Dale, Virginia H. TI Environmental Management: Past and Future Communications SO ENVIRONMENTAL MANAGEMENT LA English DT Editorial Material C1 Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Dale, VH (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM dalevh@ornl.gov NR 3 TC 0 Z9 0 U1 1 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0364-152X EI 1432-1009 J9 ENVIRON MANAGE JI Environ. Manage. PD JUL PY 2014 VL 54 IS 1 BP 1 EP 2 DI 10.1007/s00267-014-0298-7 PG 2 WC Environmental Sciences SC Environmental Sciences & Ecology GA AI9UP UT WOS:000337285900001 ER PT J AU Grahame, TJ AF Grahame, Thomas J. TI PM2.5 Species Importance of Accurate Measurement SO EPIDEMIOLOGY LA English DT Letter ID AIR-POLLUTION; HEART-RATE; ERROR C1 US DOE, Washington, DC 20585 USA. RP Grahame, TJ (reprint author), US DOE, Washington, DC 20585 USA. EM Thomas.grahame@hq.doe.gov NR 4 TC 1 Z9 1 U1 0 U2 9 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA SN 1044-3983 EI 1531-5487 J9 EPIDEMIOLOGY JI Epidemiology PD JUL PY 2014 VL 25 IS 4 BP 615 EP 615 DI 10.1097/EDE.0000000000000112 PG 1 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA AJ0CM UT WOS:000337316700021 PM 24887164 ER PT J AU Landau, SM Thomas, BA Thurfjell, L Schmidt, M Margolin, R Mintun, M Pontecorvo, M Baker, SL Jagust, WJ AF Landau, S. M. Thomas, B. A. Thurfjell, L. Schmidt, M. Margolin, R. Mintun, M. Pontecorvo, M. Baker, S. L. Jagust, W. J. CA Alzheimer's Dis Neuroimaging Initi TI Amyloid PET imaging in Alzheimer's disease: a comparison of three radiotracers SO EUROPEAN JOURNAL OF NUCLEAR MEDICINE AND MOLECULAR IMAGING LA English DT Article DE Amyloid; Alzheimer's disease; PET imaging; Neurology ID PITTSBURGH COMPOUND-B; MILD COGNITIVE IMPAIRMENT; F 18; BETA; FLORBETAPIR; F-18-FLUTEMETAMOL; DEPOSITION; RADIOLIGAND; VALIDATION; DEMENTIA AB Purpose The increasing use of amyloid PET in Alzheimer's disease research and clinical trials has motivated efforts to standardize methodology. We compared retention of the C-11 radiotracer Pittsburgh Compound B (PiB) and that of two F-18 amyloid radiotracers (florbetapir and flutemetamol) using two study populations. We also examined the feasibility of converting between tracer-specific measures, using PiB as the common link between the two F-18 tracers. Methods One group of 40 subjects underwent PiB and flutemetamol imaging sessions and a separate group of 32 subjects underwent PiB and florbetapir imaging sessions. We compared cortical and white matter retention for each F-18 tracer relative to that of PiB, as well as retention in several reference regions and image analysis methods. Correlations between tracer pairs were used to convert tracer-specific threshold values for amyloid positivity between tracers. Results Cortical retention for each pair of tracers was strongly correlated regardless of reference region (PiB-flutemetamol, rho = 0.84-0.99; PiB-florbetapir, rho = 0.83-0.97) and analysis method (rho = 0.90-0.99). Compared to PiB, flutemetamol had higher white matter retention, while florbetapir had lower cortical retention. Two previously established independent thresholds for amyloid positivity were highly consistent when values were converted between tracer pairs. Conclusion Despite differing white and grey matter retention characteristics, cortical retention for each F-18 tracer was highly correlated with that of PiB, enabling conversion of thresholds across tracer measurement scales with a high level of internal consistency. Standardization of analysis methods and measurement scales may facilitate the comparison of amyloid PET data obtained using different tracers. C1 [Landau, S. M.; Jagust, W. J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Landau, S. M.; Baker, S. L.; Jagust, W. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Thomas, B. A.] UCL, Inst Nucl Med, London, England. [Thurfjell, L.] GE Healthcare, Uppsala, Sweden. [Schmidt, M.] Janssen Pharmaceut NV, Beerse, Belgium. [Margolin, R.] Janssen Alzheimer Immunotherapy, San Francisco, CA USA. [Mintun, M.; Pontecorvo, M.] Avid Radiopharmaceut Inc, Philadelphia, PA USA. RP Landau, SM (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 118 Barker Hall MC 3190, Berkeley, CA 94720 USA. EM slandau@berkeley.edu; Benjamin_Thomas@circ.a-star.edu.sg; lennart.thurfjell@ge.com; mschmid4@its.jnj.com; rmargoli@its.jnj.com; mintun@avidrp.com; pontecorvo@avidrp.com; slbaker@lbl.gov; jagust@berkeley.edu RI Schmidt, Mark/I-5052-2016; OI Schmidt, Mark/0000-0003-3417-8977; Thomas, Benjamin/0000-0002-9784-1177 FU GlaxoSmithKline (GSK); UCL/UCLH from the UK Department of Health Biomedical Research Centre; ADNI (National Institutes of Health) [U01 AG024904]; National Institute on Aging; National Institute of Biomedical Imaging and Bioengineering; Canadian Institutes of Health Research; NIH [P30 AG010129, K01 AG030514] FX B. T. acknowledges the support of GlaxoSmithKline (GSK) and also that UCL/UCLH receives a portion of its research funding from the UK Department of Health Biomedical Research Centre's funding scheme.; Data collection and sharing for this project was funded by the ADNI (National Institutes of Health grant U01 AG024904). ADNI is funded by the National Institute on Aging, and the National Institute of Biomedical Imaging and Bioengineering, and through generous contributions from the following: Abbott; Alzheimer's Association; Alzheimer's Drug Discovery Foundation; Amorfix Life Sciences Ltd.; AstraZeneca; Bayer HealthCare; BioClinica, Inc.; Biogen Idec Inc.; Bristol-Myers Squibb Company; Eisai Inc.; Elan Pharmaceuticals Inc.; Eli Lilly and Company; F. Hoffmann-La Roche Ltd and its affiliated company Genentech, Inc.; GE Healthcare; Innogenetics, N.V.; IXICO Ltd.; Janssen Alzheimer Immunotherapy Research & Development, LLC.; Johnson & Johnson Pharmaceutical Research & Development LLC.; Medpace, Inc.; Merck & Co., Inc.; Meso Scale Diagnostics, LLC.; Novartis Pharmaceuticals Corporation; Pfizer Inc.; Servier; Synarc Inc.; and Takeda Pharmaceutical Company. The Canadian Institutes of Health Research provides funds to support ADNI clinical sites in Canada. Private sector contributions are facilitated by the Foundation for the National Institutes of Health (www.fnih.org). The grantee organization is the Northern California Institute for Research and Education, and the study is coordinated by the Alzheimer's Disease Cooperative Study at the University of California, San Diego. ADNI data are disseminated by the Laboratory for Neuro Imaging at the University of California, Los Angeles. This research was also supported by NIH grants P30 AG010129 and K01 AG030514. NR 21 TC 47 Z9 47 U1 1 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1619-7070 EI 1619-7089 J9 EUR J NUCL MED MOL I JI Eur. J. Nucl. Med. Mol. Imaging PD JUL PY 2014 VL 41 IS 7 BP 1398 EP 1407 DI 10.1007/s00259-014-2753-3 PG 10 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA AI9UR UT WOS:000337286200016 PM 24647577 ER PT J AU Schaefer, JD Werner, BT Daniel, IM AF Schaefer, J. D. Werner, B. T. Daniel, I. M. TI Strain-Rate-Dependent Failure of a Toughened Matrix Composite SO EXPERIMENTAL MECHANICS LA English DT Article DE Composites; Toughened matrix; Strain rate dependence; Failure prediction; Dynamic testing ID SHEET WRINKLE DEFECTS; WIND TURBINE-BLADES; EPOXY COMPOSITES; PREDICTIVE CAPABILITIES; PROGRESSIVE FAILURE; NONLINEAR RESPONSE; FIBER COMPOSITES; FATIGUE FAILURE; PART-B; BEHAVIOR AB The strain-rate-dependent behavior of a toughened matrix composite (IM7/8552) was characterized under quasi-static and dynamic loading conditions. Unidirectional and off-axis composite specimens were tested at strain rates ranging from 10(-4) to 10(3) s(-1) using a servo-hydraulic testing machine and split Hopkinson pressure bar apparatus. The nonlinear response and failure were analyzed and evaluated based on classical failure criteria and the Northwestern (NU) failure theory. The predictive NU theory was shown to be in excellent agreement with experimental results and to accurately predict the strain-rate-dependent failure of the composite system based on measured average lamina properties. C1 [Schaefer, J. D.; Daniel, I. M.] Northwestern Univ, Ctr Intelligent Proc Composites, Evanston, IL 60208 USA. [Werner, B. T.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Daniel, IM (reprint author), Northwestern Univ, Ctr Intelligent Proc Composites, Evanston, IL 60208 USA. EM imdaniel@northwestern.edu RI Daniel, Isaac/B-6932-2009 FU Office of Naval Research (ONR) FX The work described in this paper was sponsored by the Office of Naval Research (ONR). The authors are grateful to Dr. Y.D.S. Rajapakse of ONR for his encouragement and cooperation. NR 43 TC 6 Z9 6 U1 0 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0014-4851 EI 1741-2765 J9 EXP MECH JI Exp. Mech. PD JUL PY 2014 VL 54 IS 6 BP 1111 EP 1120 DI 10.1007/s11340-014-9876-0 PG 10 WC Materials Science, Multidisciplinary; Mechanics; Materials Science, Characterization & Testing SC Materials Science; Mechanics GA AI8JJ UT WOS:000337159200015 ER PT J AU Wang, LF AF Wang, Li-Fang TI Meshfree-enriched electromagnetic finite element formulation using nodal integration SO INTERNATIONAL JOURNAL OF NUMERICAL MODELLING-ELECTRONIC NETWORKS DEVICES AND FIELDS LA English DT Article DE finite element; meshfree; electromagnetics; nodal integration ID MESHLESS METHOD; PARTICLE METHODS; SHAPE FUNCTION; COMPUTATIONS; FIELDS AB This paper presents a meshfree-enriched finite element formulation using nodal integration for electrostatic analysis. The meshfree-enriched finite element method, originally proposed to solve the incompressible constraint in mechanical problem, is revisited in this paper and applied to the analysis of electrostatic problems to improve the solution accuracy of conventional finite element method. A novel nodal integration scheme based on the meshfree-enriched finite element mesh is developed for the integration of discrete equation and is shown to pass the linear exactness in the Galerkin approximation. To demonstrate the accuracy of the proposed formulation, two numerical examples are studied and comparisons are made to several other finite element formulations. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Wang, LF (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM wang22@llnl.gov NR 23 TC 1 Z9 1 U1 0 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0894-3370 EI 1099-1204 J9 INT J NUMER MODEL EL JI Int. J. Numer. Model.-Electron. Netw. Device Fields PD JUL-AUG PY 2014 VL 27 IS 4 BP 669 EP 681 DI 10.1002/jnm.1940 PG 13 WC Engineering, Electrical & Electronic; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA AJ4EG UT WOS:000337623900004 ER PT J AU Barlat, F Vincze, G Gracio, JJ Lee, MG Rauch, EF Tome, CN AF Barlat, F. Vincze, G. Gracio, J. J. Lee, M. -G. Rauch, E. F. Tome, C. N. TI Enhancements of homogenous anisotropic hardening model and application to mild and dual-phase steels SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Yield condition; Constitutive behavior; Metallic material; Mechanical testing; Cross-loading ID LOW-CARBON STEEL; CHANGING STRAIN PATHS; ELASTIC-PLASTIC BEHAVIOR; SPRING-BACK PREDICTION; ALUMINUM-ALLOY SHEETS; STRESS YIELD FUNCTION; METAL PLASTICITY; PLANE-STRESS; CYCLIC PLASTICITY; PART-I AB The formulation of the so-called homogeneous anisotropic hardening (HAH) model, which was originally proposed in Barlat et al. (2011), is refined. With the new features, this distortional plasticity-based constitutive model predicts the mechanical response of metals subjected to non-proportional loading with improved accuracy, in particular for cross-loading. In that case, applications to two different steels are provided for illustration purposes. For mild steel, the stress overshoot of the monotonic flow curve observed during a double load change is well reproduced by the model. In addition, for a dual-phase steel deformed in a two-step tension test with axes at 450 from each other, the new features allow the reloading yield stress to be lower than the unloading flow stress, in good agreement with experimental observations. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Barlat, F.; Lee, M. -G.] Pohang Univ Sci & Technol POSTECH, GIFT, Pohang 790784, Gyeongbuk, South Korea. [Barlat, F.; Vincze, G.; Gracio, J. J.] Univ Aveiro, Ctr Mech Technol & Automat, Dept Mech Engn, P-3810 Aveiro, Portugal. [Rauch, E. F.] INPG UJF, CNRS, Grp GPM2, UMR 5266, F-38402 St Martin Dheres, France. [Tome, C. N.] Los Alamos Natl Lab, MST Div, Los Alamos, NM 87545 USA. RP Lee, MG (reprint author), Pohang Univ Sci & Technol POSTECH, GIFT, San 31 Hyoja Dong, Pohang 790784, Gyeongbuk, South Korea. EM f.barlat@postech.ac.kr; mglee@postech.ac.kr RI RAUCH, Edgar/C-9852-2011; Tome, Carlos/D-5058-2013; Group, GAME/B-3464-2014; Vincze, Gabriela/D-2383-2013; OI Vincze, Gabriela/0000-0002-0338-3911; Barlat, Frederic/0000-0002-4463-3454 FU POSCO; National Research Foundation of Korea (NRF) - Korean government (MSIP) [2012R1A5A1048294]; Foundation of Science and Technology of Portugal [PTDC/EME-PME/116683/2010] FX The supports of POSCO, the National Research Foundation of Korea (NRF), through the Grant No. 2012R1A5A1048294 funded by the Korean government (MSIP), and the Foundation of Science and Technology of Portugal through the Grant PTDC/EME-PME/116683/2010, are gratefully acknowledged. The comments and suggestions of Mr. Jinwoo Lee (GIFT) about this work are greatly appreciated. NR 84 TC 21 Z9 22 U1 1 U2 31 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD JUL PY 2014 VL 58 SI SI BP 201 EP 218 DI 10.1016/j.ijplas.2013.11.002 PG 18 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA AI9OM UT WOS:000337261900010 ER PT J AU Luszczek, P Kurzak, J Dongarra, J AF Luszczek, Piotr Kurzak, Jakub Dongarra, Jack TI Looking back at dense linear algebra software SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING LA English DT Article DE Decompositional approach; Parallel algorithms; Dense linear algebra ID MODEL IMPLEMENTATION; PROGRAM PARAGAUSS; EXTENDED SET; SUBPROGRAMS; COMPUTATION; ALGORITHMS; PLASMAS; FORTRAN AB Over the years, computational physics and chemistry served as an ongoing source of problems that demanded the ever increasing performance from hardware as well as the software that ran on top of it. Most of these problems could be translated into solutions for systems of linear equations: the very topic of numerical linear algebra. Seemingly then, a set of efficient linear solvers could be solving important scientific problems for years to come. We argue that dramatic changes in hardware designs precipitated by the shifting nature of the marketplace of computer hardware had a continuous effect on the software for numerical linear algebra. The extraction of high percentages of peak performance continues to require adaptation of software. If the past history of this adaptive nature of linear algebra software is any guide then the future theme will feature changes as well - changes aimed at harnessing the incredible advances of the evolving hardware infrastructure. Published by Elsevier Inc. C1 [Luszczek, Piotr] Univ Tennessee, Knoxville, TN USA. [Kurzak, Jakub] Univ Tennessee, Dept Elect Engn & Comp Sci, Innovat Comp Lab, Knoxville, TN USA. [Dongarra, Jack] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Dongarra, Jack] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Dongarra, Jack] Univ Manchester, Sch Comp Sci, Manchester M13 9PL, Lancs, England. [Dongarra, Jack] Univ Manchester, Sch Math, Manchester M13 9PL, Lancs, England. RP Dongarra, J (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. EM luszczek@eecs.utk.edu; kurzak@eecs.utk.edu; dongarra@cs.utk.edu NR 36 TC 1 Z9 1 U1 1 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0743-7315 EI 1096-0848 J9 J PARALLEL DISTR COM JI J. Parallel Distrib. Comput. PD JUL PY 2014 VL 74 IS 7 BP 2548 EP 2560 DI 10.1016/j.jpdc.2013.10.005 PG 13 WC Computer Science, Theory & Methods SC Computer Science GA AI9OD UT WOS:000337261000003 ER PT J AU Smith, KA Stewart, B Yager, KG Strzalka, J Verduzco, R AF Smith, Kendall A. Stewart, Bridget Yager, Kevin G. Strzalka, Joseph Verduzco, Rafael TI Control of all-conjugated block copolymer crystallization via thermal and solvent annealing SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE block copolymers; conducting polymers; crystallization; films; organic photovoltaics; poly(3-alkylthiophene); poly(9; 9-dioctylfluorene); poly(3-dodecylthiophene); rod-rod polymers ID MICROPHASE SEPARATION; CLICK CHEMISTRY; POLY(3-ALKYLTHIOPHENES); POLY(3-HEXYLTHIOPHENE); CRYSTALLINITY; EMISSION AB Control of the crystallization of conjugated polymers is of critical importance to the performance of organic electronics, such as organic photovoltaic devices, due to the effect on charge separation and transport, particularly for all-polymer devices. The block copolymer poly(3-dodecylthiophene)-block-poly(9,9-dioctylfluorene) (P3DDT-b-PF), which has matched crystallization temperatures for each block, is used to study the effects of processing history on resulting crystallization. For longer annealing times and rapid quenching to room temperature, P3DDT crystals are preferred whereas for shorter annealing times and slower quenching, PF crystals are preferred. Both crystal forms are evidenced for long annealing time and slow quenching. Additionally, for room temperature annealing in the presence of a chloroform vapor, PF crystals are found in the PF phase with the predominant crystal peak oriented perpendicular to the thermally annealed case. These results will provide guidance for optimizing annealing strategies for future donor/acceptor block copolymer photovoltaic devices. (c) 2014 Wiley Periodicals, Inc. J. Polym. Sci., Part B: Polym. Phys. 2014, 52, 900-906 C1 [Smith, Kendall A.; Stewart, Bridget; Verduzco, Rafael] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. [Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Strzalka, Joseph] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Verduzco, R (reprint author), Rice Univ, Dept Chem & Biomol Engn, 6100 Main MS 362 St, Houston, TX 77005 USA. EM rafaelv@rice.edu RI Yager, Kevin/F-9804-2011 OI Yager, Kevin/0000-0001-7745-2513 FU National Science Foundation [CBET-1264703]; Shell Center for Sustainability; Louis and Peaches Owen; Department of Homeland Security, Science, and Technology Division [2009-ST-062-000031]; US DOE [DE-AC02-06CH11357]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the National Science Foundation under Grant No. CBET-1264703, the Shell Center for Sustainability, and Louis and Peaches Owen. B. Stewart acknowledges the Department of Homeland Security, Science, and Technology Division, Award #2009-ST-062-000031. K. A. Smith acknowledges Aditya Mohite, Gautam Gupta, Hsing-LinWang, and Hsinhan Tsai of Los Alamos National Laboratory for useful discussion during the preparation of this manuscript. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. Use of the National Synchrotron Light Source and Center for Functional Nanomaterials, Brookhaven National Laboratory, were supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 24 TC 6 Z9 6 U1 6 U2 51 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD JUL 1 PY 2014 VL 52 IS 13 BP 900 EP 906 DI 10.1002/polb.23506 PG 7 WC Polymer Science SC Polymer Science GA AJ3OR UT WOS:000337576900007 ER PT J AU Luo, HB Beckles, GLA Zhang, XZ Sotnikov, S Thompson, T Bardenheier, B AF Luo, Huabin Beckles, Gloria L. A. Zhang, Xinzhi Sotnikov, Sergey Thompson, Ted Bardenheier, Barbara TI The Relationship Between County-Level Contextual Characteristics and Use of Diabetes Care Services SO JOURNAL OF PUBLIC HEALTH MANAGEMENT AND PRACTICE LA English DT Article DE Andersen's model; multilevel models; preventive diabetes care; social determinants ID SELF-MANAGEMENT EDUCATION; SAFETY-NET; GLYCEMIC CONTROL; UNITED-STATES; ACCESS; HEALTH; METAANALYSIS; COMPLICATIONS; COMMUNITIES; DISPARITIES AB Objectives: To examine the relationship between county-level measures of social determinants and use of preventive care among US adults with diagnosed diabetes. To inform future diabetes prevention strategies. Methods: Data are from the Behavioral Risk Factor Surveillance System (BRFSS) 2004 and 2005 surveys, the National Diabetes Surveillance System, and the Area Resource File. Use of diabetes care services was defined by self-reported receipt of 7 preventive care services. Our study sample included 46 806 respondents with self-reported diagnosed diabetes. Multilevel models were run to assess the association between county-level characteristics and receipt of each of the 7 preventive diabetes care service after controlling for characteristics of individuals. Results were considered significant if P < .05. Results: Controlling for individual-level characteristics, our analyses showed that 7 of the 8 county-level factors examined were significantly associated with use of 1 or more preventive diabetes care services. For example, people with diabetes living in a county with a high uninsurance rate were less likely to have an influenza vaccination, visit a doctor for diabetes care, have an A1c test, or a foot examination; people with diabetes living in a county with a high physician density were more likely to have an A1c test, foot examination, or an eye examination; and people with diabetes living in a county with more people with less than high-school education were less likely to have influenza vaccination, pneumococcal vaccination, or self-care education (all P < .05). Conclusions: Many of the county-level factors examined in this study were found to be significantly associated with use of preventive diabetes care services. County policy makers may need to consider local circumstances to address the disparities in use of these services. C1 [Luo, Huabin] Ctr Dis Control & Prevent, ORISE, OSTLTS, Atlanta, GA 30333 USA. [Sotnikov, Sergey] CDC, OSTLTS, Atlanta, GA 30333 USA. [Beckles, Gloria L. A.; Zhang, Xinzhi; Thompson, Ted; Bardenheier, Barbara] CDC, Div Diabet Translat, Natl Ctr Chron Dis Prevent & Hlth Promot, Atlanta, GA 30333 USA. RP Luo, HB (reprint author), Ctr Dis Control & Prevent, Off State Tribal Local & Territorial Support, 1600 Clifton Rd M-S E-70, Atlanta, GA 30333 USA. EM vbz7@CDC.gov FU Intramural CDC HHS [CC999999] NR 44 TC 1 Z9 1 U1 2 U2 10 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 1078-4659 EI 1550-5022 J9 J PUBLIC HEALTH MAN JI J. Public Health Manag. Pract. PD JUL-AUG PY 2014 VL 20 IS 4 BP 401 EP 410 DI 10.1097/PHH.0b013e31829bfa60 PG 10 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA AI8DV UT WOS:000337137700012 PM 23963254 ER PT J AU Roan, NR Liu, HC Usmani, SM Neidleman, J Muller, JA Avila-Herrera, A Gawanbacht, A Zirafi, O Chu, S Dong, M Kumar, ST Smith, JF Pollard, KS Fandrich, M Kirchhoff, F Munch, J Witkowska, HE Greene, WC AF Roan, Nadia R. Liu, Haichuan Usmani, Shariq M. Neidleman, Jason Mueller, Janis A. Avila-Herrera, Aram Gawanbacht, Ali Zirafi, Onofrio Chu, Simon Dong, Ming Kumar, Senthil T. Smith, James F. Pollard, Katherine S. Faendrich, Marcus Kirchhoff, Frank Muench, Jan Witkowska, H. Ewa Greene, Warner C. TI Liquefaction of Semen Generates and Later Degrades a Conserved Semenogelin Peptide That Enhances HIV Infection SO JOURNAL OF VIROLOGY LA English DT Article ID PROSTATE-SPECIFIC ANTIGEN; SPERM MOTILITY INHIBITOR; MEDIATED ENHANCEMENT; AMYLOID FIBRILS; PROTEIN; CELLS; COAGULUM; ASSAY AB Semen enhances HIV infection in vitro, but how long it retains this activity has not been carefully examined. Immediately postejaculation, semen exists as a semisolid coagulum, which then converts to a more liquid form in a process termed liquefaction. We demonstrate that early during liquefaction, semen exhibits maximal HIV-enhancing activity that gradually declines upon further incubation. The decline in HIV-enhancing activity parallels the degradation of peptide fragments derived from the semenogelins (SEMs), the major components of the coagulum that are cleaved in a site-specific and progressive manner upon initiation of liquefaction. Because amyloid fibrils generated from SEM fragments were recently demonstrated to enhance HIV infection, we set out to determine whether any of the liquefaction-generated SEM fragments associate with the presence of HIVenhancing activity. We identify SEM1 from amino acids 86 to 107 [ SEM1(86-107)] to be a short, cationic, amyloidogenic SEM peptide that is generated early in the process of liquefaction but that, conversely, is lost during prolonged liquefaction due to the activity of serine proteases. Synthetic SEM1(86-107) amyloids directly bind HIV-1 virions and are sufficient to enhance HIV infection of permissive cells. Furthermore, endogenous seminal levels of SEM1(86-107) correlate with donor-dependent variations in viral enhancement activity, and antibodies generated against SEM1(86-107) recognize endogenous amyloids in human semen. The amyloidogenic potential of SEM1(86-107) and its virus-enhancing properties are conserved among great apes, suggesting an evolutionarily conserved function. These studies identify SEM1(86-107) to be a key, HIV-enhancing amyloid species in human semen and underscore the dynamic nature of semen's HIV-enhancing activity. C1 [Roan, Nadia R.; Neidleman, Jason; Chu, Simon; Greene, Warner C.] Univ Calif San Francisco, Gladstone Inst Virol & Immunol, San Francisco, CA 94143 USA. [Roan, Nadia R.; Smith, James F.] Univ Calif San Francisco, Dept Urol, San Francisco, CA USA. [Liu, Haichuan; Witkowska, H. Ewa] Univ Calif San Francisco, Dept Obstet Gynecol & Reprod Sci, San Francisco, CA USA. [Liu, Haichuan; Witkowska, H. Ewa] Univ Calif San Francisco, Sandler Moore Mass Spectrometry Core Facil, San Francisco, CA 94143 USA. [Avila-Herrera, Aram; Pollard, Katherine S.] Univ Calif San Francisco, Gladstone Inst Cardiovasc Dis, San Francisco, CA USA. [Pollard, Katherine S.] Univ Calif San Francisco, Dept Epidemiol & Biostat, Inst Human Genet, San Francisco, CA 94143 USA. [Greene, Warner C.] Univ Calif San Francisco, Dept Med, San Francisco, CA USA. [Greene, Warner C.] Univ Calif San Francisco, Dept Microbiol & Immunol, San Francisco, CA 94143 USA. [Usmani, Shariq M.; Mueller, Janis A.; Gawanbacht, Ali; Zirafi, Onofrio; Kirchhoff, Frank; Muench, Jan] Univ Ulm, Inst Mol Virol, Med Ctr, D-89069 Ulm, Germany. [Dong, Ming] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kumar, Senthil T.; Faendrich, Marcus] Univ Ulm, Inst Pharmaceut Biotechnol, D-89069 Ulm, Germany. RP Roan, NR (reprint author), Univ Calif San Francisco, Gladstone Inst Virol & Immunol, San Francisco, CA 94143 USA. EM roann@urology.ucsf.edu OI Usmani, Shariq/0000-0002-6462-1098 FU Hellman Family Awards [1PO1 AI083050 PPG]; U.S. Department of Defense [W81XWH-11-1-0562, R01HD074511]; DFG; Ministry of Science; VW Stiftung; San Simeon Fund; Sandler Family Foundation; Gordon and Betty Moore Foundation; NIH/NCI Cancer Center [P30 CA082103]; CFAR [P30 AI027763, P30-AI027763]; [5K12 DK083021-04 KURe]; [K99/R00 1K99AI104262]; [DFG FA 456/10-1]; [DFG US116/1] FX This work was supported, in whole or in part, by grant 5K12 DK083021-04 KURe, grant K99/R00 1K99AI104262, and Hellman Family Awards grants (to N.R.R.), grant 1PO1 AI083050 PPG and U.S. Department of Defense grant W81XWH-11-1-0562 (to W.C.G.), grant R01HD074511 (to N.R.R. and W.C.G.), the DFG and the Ministry of Science (to J.M.), the VW Stiftung (to J.M. and F.K.), DFG FA 456/10-1 (to M.F.), DFG US116/1-funding (to S. M.U., a fellow of the DFG Junior Research Academy OFFSPRing), and institutional funds from the Gladstone Institutes and a gift from the San Simeon Fund (to K.S.P.). The UCSF Sandler-Moore Mass Spectrometry Core Facility acknowledges support from the Sandler Family Foundation, the Gordon and Betty Moore Foundation, and NIH/NCI Cancer Center support grant P30 CA082103. We also acknowledge CFAR for funding for the Flow Core (P30 AI027763) and for H.L. (P30-AI027763). NR 32 TC 12 Z9 12 U1 1 U2 4 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0022-538X EI 1098-5514 J9 J VIROL JI J. Virol. PD JUL PY 2014 VL 88 IS 13 BP 7221 EP 7234 DI 10.1128/JVI.00269-14 PG 14 WC Virology SC Virology GA AI9GN UT WOS:000337240700010 PM 24741080 ER PT J AU Bailey, DH Borwein, JM Crandall, RE AF Bailey, David H. Borwein, Jonathan M. Crandall, Richard E. TI COMPUTATION AND THEORY OF EXTENDED MORDELL-TORNHEIM-WITTEN SUMS SO MATHEMATICS OF COMPUTATION LA English DT Article ID RIEMANN ZETA-FUNCTION; VALUES; DERIVATIVES; INTEGRALS AB We consider some fundamental generalized Mordell-TornheimWitten (MTW) zeta-function values along with their derivatives, and explore connections with multiple-zeta values (MZVs). To achieve this, we make use of symbolic integration, high precision numerical integration, and some interesting combinatorics and special-function theory. Our original motivation was to represent unresolved constructs such as Eulerian log-gamma integrals. We are able to resolve all such integrals in terms of an MTW basis. We also present, for a substantial subset of MTW values, explicit closed-form expressions. In the process, we significantly extend methods for high-precision numerical computation of polylogarithms and their derivatives with respect to order. C1 [Bailey, David H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Borwein, Jonathan M.] Univ Newcastle, CARMA, Callaghan, NSW 2308, Australia. [Borwein, Jonathan M.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Crandall, Richard E.] Reed Coll, Ctr Adv Computat, Portland, OR 97202 USA. RP Bailey, DH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM DHBailey@lbl.gov; jonathan.borwein@newcastle.edu.au; crandall@reed.edu FU U.S. Department of Energy [DE-AC02-05CH11231] FX LBNL authored documents are sponsored by the U.S. Department of Energy under Contract DE-AC02-05CH11231. Accordingly, the U.S. Government retains a nonexclusive, royalty- free license to publish or reproduce these documents, or allow others to do so, for U.S. Government purposes. The documents may be freely distributed and used for noncommercial, scientific and educational purposes. NR 35 TC 5 Z9 5 U1 1 U2 1 PU AMER MATHEMATICAL SOC PI PROVIDENCE PA 201 CHARLES ST, PROVIDENCE, RI 02940-2213 USA SN 0025-5718 EI 1088-6842 J9 MATH COMPUT JI Math. Comput. PD JUL PY 2014 VL 83 IS 288 BP 1795 EP 1821 AR PII S 0025-5718(2014)02768-3 PG 27 WC Mathematics, Applied SC Mathematics GA AI9DT UT WOS:000337230000010 ER PT J AU Tafrova, JI Tafrov, ST AF Tafrova, Juliana I. Tafrov, Stefan T. TI Human histone acetyltransferase 1 (Hat1) acetylates lysine 5 of histone H2A in vivo SO MOLECULAR AND CELLULAR BIOCHEMISTRY LA English DT Article DE Hat1; Histone Acetylation; H2A; H4; Insoluble nuclear proteins; Gamma radiation ID STRAND BREAK REPAIR; DNA-DAMAGE; CHROMATIN; TIP60; REPLICATION; COMPLEX; YEAST; INVOLVEMENT; CHAPERONES; EXPRESSION AB The primary structure of Histone Acetyltransferase 1 (Hat1) has been conserved throughout evolution; however, despite its ubiquity, its cellular function is not well characterized. To study its in vivo acetylation pattern and function, we utilized shRNAmir against Hat1 expressed in the well-substantiated HeLa (human cervical cancer) cell line. To reduce the interference by enzymes with similar HAT specificity, we used HeLa cells expressing histone acetyltransferase Tip60 with mutated acetyl-CoA binding site that abrogates its enzyme activity (mutant HeLa-tip60). Two shRNAmir were identified that reduced the expression of the cytoplasmic and nuclear forms of Hat1. Cytosolic protein preparations from these two clones showed decreased levels of acetylation of lysine 5 (K5) and K12 on histone H4, with the concomitant loss of the acetylation of histone H2A at K5. This pattern of decreased acetylation of H2AK5 was well defined in preparations of histone protein and insoluble nuclear-protein (INP) fractions as well. Abrogating the Hat1 expression caused a 74 % decrease in colony-forming efficiency of mutant HeLa-tip60 cells, reduced the size of the colonies by 50 %, and decreased the amounts of proteins with molecular weights below 35 kDa in the INP fractions. C1 [Tafrova, Juliana I.] SUNY Stony Brook, Dept Oral Biol & Pathol, Stony Brook, NY 11794 USA. [Tafrova, Juliana I.] Genet Ctr, Smithtown, NY 11787 USA. [Tafrov, Stefan T.] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Tafrov, Stefan T.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Tafrov, ST (reprint author), Brookhaven Natl Lab, Dept Biol, 50 Bell Ave,Bldg 463, Upton, NY 11973 USA. EM tafrov@bnl.gov FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. Department of Energy; National Aeronautics and Space Administration under Department of Energy [DE-AC02-98CH10886, NNJ08HB63I]; Brookhaven National Laboratory FX We would like to thank Dr. Avril Woodhead for her critical help with the manuscript preparation and Dr. Rolf Sternglanz for the invaluable support, discussions, and comments throughout the years. We would like to thank Dr. David Schlyer, Dr. John Shanklin, and the entire Biosciences Department for the support; and Dr. Tsuyoshi Ikura for providing the HeLa-TIP60 and HeLa-tip60 cell lines. This article has been authored by Brookhaven Science Associates, LLC under contract number DE-AC02-98CH10886 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. This work was supported by a grant from the National Aeronautics and Space Administration NNJ08HB63I under Department of Energy Prime Contract DE-AC02-98CH10886 with the Brookhaven National Laboratory (to STT). NR 42 TC 2 Z9 2 U1 0 U2 14 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0300-8177 EI 1573-4919 J9 MOL CELL BIOCHEM JI Mol. Cell. Biochem. PD JUL PY 2014 VL 392 IS 1-2 BP 259 EP 272 DI 10.1007/s11010-014-2036-0 PG 14 WC Cell Biology SC Cell Biology GA AI9EW UT WOS:000337233900024 PM 24682716 ER PT J AU Karpinets, TV Park, BH Syed, MH Klotz, MG Uberbacher, EC AF Karpinets, Tatiana V. Park, Byung H. Syed, Mustafa H. Klotz, Martin G. Uberbacher, Edward C. TI Metabolic Environments and Genomic Features Associated with Pathogenic and Mutualistic Interactions Between Bacteria and Plants SO MOLECULAR PLANT-MICROBE INTERACTIONS LA English DT Article ID SOYBEAN ROOT-NODULES; EXPRESSION PROFILES; NITROGEN-FIXATION; PROTEIN FAMILIES; DATABASE; NETWORK; SYSTEM; RECONSTRUCTION; SPECIFICITY; SALMONELLA AB Genomic characteristics discriminating parasitic and mutualistic relationship of bacterial symbionts with plants are poorly understood. This study comparatively analyzed the genomes of 54 mutualists and pathogens to discover genomic markers associated with the different phenotypes. Using metabolic network models, we predict external environments associated with free-living and symbiotic lifestyles and quantify dependences of symbionts on the host in terms of the consumed metabolites. We show that specific differences between the phenotypes are pronounced at the levels of metabolic enzymes, especially carbohydrate active, and protein functions. Overall, biosynthetic functions are enriched and more diverse in plant mutualists whereas processes and functions involved in degradation and host invasion are enriched and more diverse in pathogens. A distinctive characteristic of plant pathogens is a putative novel secretion system with a circadian rhythm regulator. A specific marker of plant mutualists is the co-residence of genes encoding nitrogenase and ribulose bisphosphate carboxylase/oxygenase (RuBisCO). We predict that RuBisCO is likely used in a putative metabolic pathway to supplement carbon obtained heterotrophically with low-cost assimilation of carbon from CO2. We validate results of the comparative analysis by predicting correct phenotype, pathogenic or mutualistic, for 20 symbionts in an independent set of 30 pathogens, mutualists, and commensals. C1 [Karpinets, Tatiana V.; Syed, Mustafa H.; Uberbacher, Edward C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Park, Byung H.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Klotz, Martin G.] Univ N Carolina, Dept Biol Sci, Charlotte, NC 28223 USA. RP Karpinets, TV (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM karpinetstv@ornl.gov RI Klotz, Martin/D-2091-2009 OI Klotz, Martin/0000-0002-1783-375X FU Plant Microbe Interface Project of the Genomic Science Program, U.S. Department of Energy (DOE), Office of Science, Biological, and Environmental Research; U.S. DOE [DE-AC05-00OR22725]; Office of Biological and Environmental Research in the DOE Office of Science; University of North Carolina at Charlotte FX This research was sponsored by the Plant Microbe Interface Project of the Genomic Science Program, U.S. Department of Energy (DOE), Office of Science, Biological, and Environmental Research. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. DOE under contract DE-AC05-00OR22725. The work of M. H. Syed to adapt certain tools was supported by The BioEnergy Science Center (BESC). BESC is a U.S. DOE Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. M. G. Klotz was supported by incentive funds from the University of North Carolina at Charlotte. We thank anonymous reviewers of the manuscript for thoughtful suggestions and comments on the study. NR 67 TC 2 Z9 2 U1 2 U2 20 PU AMER PHYTOPATHOLOGICAL SOC PI ST PAUL PA 3340 PILOT KNOB ROAD, ST PAUL, MN 55121 USA SN 0894-0282 EI 1943-7706 J9 MOL PLANT MICROBE IN JI Mol. Plant-Microbe Interact. PD JUL PY 2014 VL 27 IS 7 BP 664 EP 677 DI 10.1094/MPMI-12-13-0368-R PG 14 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Plant Sciences SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Plant Sciences GA AI9FW UT WOS:000337238200006 PM 24580106 ER PT J AU Desai, S Naik, D Cumming, JR AF Desai, Shalaka Naik, Dhiraj Cumming, Jonathan R. TI The influence of phosphorus availability and Laccaria bicolor symbiosis on phosphate acquisition, antioxidant enzyme activity, and rhizospheric carbon flux in Populus tremuloides SO MYCORRHIZA LA English DT Article DE Ectomycorrhizal fungi; Environmental stress; Exudation; Organic acids; Poplar; Trembling aspen ID ORGANIC-ACID EXUDATION; ARBUSCULAR MYCORRHIZAL FUNGI; PINUS-SYLVESTRIS SEEDLINGS; LATERAL ROOT DEVELOPMENT; ECTOMYCORRHIZAL FUNGI; PHOSPHOENOLPYRUVATE CARBOXYLASE; ALUMINUM TOLERANCE; FOREST SOILS; WHITE LUPIN; DEFICIENCY AB Many forest tree species are dependent on their symbiotic interaction with ectomycorrhizal (ECM) fungi for phosphorus (P) uptake from forest soils where P availability is often limited. The ECM fungal association benefits the host plant under P limitation through enhanced soil exploration and increased P acquisition by mycorrhizas. To study the P starvation response (PSR) and its modification by ECM fungi in Populus tremuloides, a comparison was made between nonmycorrhizal (NM) and mycorrhizal with Laccaria bicolor (Myc) seedlings grown under different concentrations of phosphate (Pi) in sand culture. Although differences in growth between NM and Myc plants were small, Myc plants were more effective at acquiring P from low Pi treatments, with significantly lower k (m) values for root and leaf P accumulation. Pi limitation significantly increased the activity of catalase, ascorbate peroxidase, and guaiacol-dependent peroxidase in leaves and roots to greater extents in NM than Myc P. tremuloides. Phosphoenolpyruvate carboxylase activity also increased in NM plants under P limitation, but was unchanged in Myc plants. Formate, citrate, malonate, lactate, malate, and oxalate and total organic carbon exudation by roots was stimulated by P limitation to a greater extent in NM than Myc plants. Colonization by L. bicolor reduced the solution Pi concentration thresholds where PSR physiological changes occurred, indicating that enhanced Pi acquisition by P. tremuloides colonized by L. bicolor altered host P homeostasis and plant stress responses to P limitation. Understanding these plant-symbiont interactions facilitates the selection of more P-efficient forest trees and strategies for tree plantation production on marginal soils. C1 [Desai, Shalaka; Naik, Dhiraj; Cumming, Jonathan R.] W Virginia Univ, Dept Biol, Morgantown, WV 26506 USA. [Desai, Shalaka] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Naik, Dhiraj] Indian Inst Adv Res, Dept Environm Sci, Koba Inst Area, Gandhinagar 382007, Gujarat, India. RP Cumming, JR (reprint author), W Virginia Univ, Dept Biol, POB 6057, Morgantown, WV 26506 USA. EM jcumming@wvu.edu OI Naik, Dhiraj/0000-0002-1226-2337 FU United States Department of Energy [FG02-06ER64148]; West Virginia University Eberly College of Arts and Sciences FX We thank Joshua Smith and Nathaniel Chapman for their excellent technical support. The West Virginia University Eberly College of Arts and Sciences and the United States Department of Energy (FG02-06ER64148) provided financial support for this work. NR 88 TC 8 Z9 8 U1 7 U2 50 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0940-6360 EI 1432-1890 J9 MYCORRHIZA JI Mycorrhiza PD JUL PY 2014 VL 24 IS 5 BP 369 EP 382 DI 10.1007/s00572-013-0548-1 PG 14 WC Mycology SC Mycology GA AI9FC UT WOS:000337235000005 PM 24338046 ER PT J AU Li, L Huang, C Huang, HY Wang, YJ Yan, RS Zhang, GF Zhou, M Lou, SR Tao, SK Wang, HL Qiao, LP Chen, CH Streets, DG Fu, JS AF Li, L. Huang, C. Huang, H. Y. Wang, Y. J. Yan, R. S. Zhang, G. F. Zhou, M. Lou, S. R. Tao, S. K. Wang, H. L. Qiao, L. P. Chen, C. H. Streets, D. G. Fu, J. S. TI An integrated process rate analysis of a regional fine particulate matter episode over Yangtze River Delta in 2010 SO ATMOSPHERIC ENVIRONMENT LA English DT Article DE Integrated process rate; PM2.5; CMAQ; Yangtze River Delta ID QUALITY MODELING SYSTEM; AIR-QUALITY; PART II; PERFORMANCE EVALUATION; SECONDARY FORMATION; MASS-SPECTROMETRY; CHINA; AEROSOL; CMAQ; POLLUTION AB A high PM2.5 pollution episode was detected in Shanghai in November 2010. The integrated process rate method, an advanced diagnostic tool, was applied to account for the contribution of different atmospheric processes during the high pollution episode in the Yangtze River Delta region (YRD). The PM2.5 process analysis indicates that the emission of fine particles is the dominant source of high surface PM2.5 concentrations in the major cities of the YRD like Shanghai, Nanjing, and Hangzhou, following horizontal transportation and aerosols. The PM2.5 concentration could be reduced due to vertical advection and diffusion from lower levels to the upper air. The aerosols process such as homogeneous nucleation and condensation producing PM2.5 occurs throughout the PBL layer in urban areas, causing vertical transport from upper levels down to the surface layer. The aerosols process is much more significant in a downwind rural and coastal site like Zhoushan than in the urban areas. The PM2.5 change initiated by both horizontal transport and vertical transport is much stronger at 40-2000 m height than in the surface layer, while the PM2.5 change caused by horizontal diffusion is very small. Dry deposition can significantly reduce concentration of the particulates in the surface level of the atmosphere, and wet deposition can remove the particles in the planetary boundary layer (PBL). The cloud processes can either increase PM2.5 due to the aqueous-phase oxidation of SO2 and NO2 or remove PM2.5 due to cloud scavenging. Solar radiation and humidity are more important to secondary pollution, and they are the significant external factors affecting the chemical reactions among sulfur dioxide, nitrogen oxides, ammonia, volatile compounds and fine particles. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Li, L.; Huang, C.; Huang, H. Y.; Yan, R. S.; Zhang, G. F.; Zhou, M.; Lou, S. R.; Tao, S. K.; Wang, H. L.; Qiao, L. P.; Chen, C. H.] Sate Environm Protect Key Lab Cause & Prevent Urb, Shanghai 200233, Peoples R China. [Li, L.; Huang, C.; Huang, H. Y.; Yan, R. S.; Zhang, G. F.; Zhou, M.; Lou, S. R.; Tao, S. K.; Wang, H. L.; Qiao, L. P.; Chen, C. H.] Shanghai Acad Environm Sci, Shanghai 200233, Peoples R China. [Wang, Y. J.] Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China. [Streets, D. G.] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [Fu, J. S.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. RP Li, L (reprint author), Sate Environm Protect Key Lab Cause & Prevent Urb, Shanghai 200233, Peoples R China. EM lili@saes.sh.cn RI Huang, Cheng/I-7099-2015 FU National Natural Science Foundation of China (NSFC) [41205122, 41105102]; Science and Technology Commission of Shanghai Municipality Fund Project [11231200500]; National Non-profit Scientific Research Program for Environmental Protection [201409008] FX This study was supported by the National Natural Science Foundation of China (NSFC) via grant No. 41205122 and No. 41105102, the Science and Technology Commission of Shanghai Municipality Fund Project via grant No. 11231200500, and the National Non-profit Scientific Research Program for Environmental Protection via grant No. 201409008. NR 50 TC 3 Z9 5 U1 1 U2 74 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1352-2310 EI 1873-2844 J9 ATMOS ENVIRON JI Atmos. Environ. PD JUL PY 2014 VL 91 BP 60 EP 70 DI 10.1016/j.atmosenv.2014.03.053 PG 11 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA AI6AP UT WOS:000336952500007 ER PT J AU Yoon, H Leibeling, S Zhang, CY Muller, RH Werth, CJ Zilles, JL AF Yoon, Hongkyu Leibeling, Sabine Zhang, Changyong Mueller, Roland H. Werth, Charles J. Zilles, Julie L. TI Adaptation of Delftia acidovorans for degradation of 2,4-dichlorophenoxyacetate in a microfluidic porous medium SO BIODEGRADATION LA English DT Article DE 2,4-D; Adaptation; Chlorinated phenoxyalkanoates; Delftia acidovorans; Porous media; Micromodel ID TRANSVERSE MIXING ZONE; ALPHA-KETOGLUTARATE; ADAPTIVE RADIATION; MICROBIAL-GROWTH; BACTERIAL-GROWTH; VISUALIZATION; POPULATIONS; CHEMOTAXIS; HERBICIDES; MIGRATION AB Delftia acidovorans MC1071 can productively degrade R-2-(2,4-dichlorophenoxy)propionate (R-2,4-DP) but not 2,4-dichlorophenoxyacetate (2,4-D) herbicides. This work demonstrates adaptation of MC1071 to degrade 2,4-D in a model two-dimensional porous medium (referred to here as a micromodel). Adaptation for 2,4-D degradation in the 2 cm-long micromodel occurred within 35 days of exposure to 2,4-D, as documented by substrate removal. The amount of 2,4-D degradation in the adapted cultures in two replicate micromodels (similar to 10 and 20 % over 142 days) was higher than a theoretical maximum (4 %) predicted using published numerical simulation methods, assuming instantaneous biodegradation and a transverse dispersion coefficient obtained for the same pore structure without biomass present. This suggests that the presence of biomass enhances substrate mixing. Additional evidence for adaptation was provided by operation without R-2,4-DP, where degradation of 2,4-D slowly decreased over 20 days, but was restored almost immediately when R-2,4-DP was again provided. Compared to suspended growth systems, the micromodel system retained the ability to degrade 2,4-D longer in the absence of R-2,4-DP, suggesting slower responses and greater resilience to fluctuations in substrates might be expected in the soil environment than in a chemostat. C1 [Yoon, Hongkyu; Werth, Charles J.; Zilles, Julie L.] Univ Illinois, Dept Civil & Environm Engn, Newmark Civil Engn Lab 3230C MC 250, Urbana, IL 61801 USA. [Leibeling, Sabine; Mueller, Roland H.] UFZ Helmholtz Ctr Environm Res, Dept Environm Microbiol, D-04318 Leipzig, Germany. [Zhang, Changyong] Fundamental & Computat Sci Directorate, Div Chem & Mat Sci, Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zilles, JL (reprint author), Univ Illinois, Dept Civil & Environm Engn, Newmark Civil Engn Lab 3230C MC 250, 205 N Mathews Ave, Urbana, IL 61801 USA. EM jzilles@illinois.edu RI Zhang, Changyong/A-8012-2013; OI Zilles, Julie/0000-0001-8684-4519 FU United States Department of Agriculture National Institute of Food and Agriculture [2007-35107-17817]; German Academic Exchange Service (DAAD) fellowship; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy Office of Biological and Environmental Research, Subsurface Biogeochemistry Research Program Scientific Focus Area at the Pacific Northwest National Laboratory FX This work was supported by the National Research Initiative Grant 2007-35107-17817 from the United States Department of Agriculture National Institute of Food and Agriculture and a German Academic Exchange Service (DAAD) fellowship to SL. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. CYZ also acknowledges financial support from the U.S. Department of Energy Office of Biological and Environmental Research, Subsurface Biogeochemistry Research Program Scientific Focus Area at the Pacific Northwest National Laboratory. NR 32 TC 3 Z9 3 U1 2 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0923-9820 EI 1572-9729 J9 BIODEGRADATION JI Biodegradation PD JUL PY 2014 VL 25 IS 4 BP 595 EP 604 DI 10.1007/s10532-014-9684-3 PG 10 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA AI7JI UT WOS:000337064200010 PM 24519176 ER PT J AU Goldberg, N Kim, Y Leyffer, S Veselka, TD AF Goldberg, Noam Kim, Youngdae Leyffer, Sven Veselka, Thomas D. TI Adaptively refined dynamic program for linear spline regression SO COMPUTATIONAL OPTIMIZATION AND APPLICATIONS LA English DT Article DE Piecewise regression; Least squares; Change point detection; Dynamic programming; Mixed-integer programming AB The linear spline regression problem is to determine a piecewise linear function for estimating a set of given points while minimizing a given measure of misfit or error. This is a classical problem in computational statistics and operations research; dynamic programming was proposed as a solution technique more than 40 years ago by Bellman and Roth (J Am Stat Assoc 64:1079-1084, 1969). The algorithm requires a discretization of the solution space to define a grid of candidate breakpoints. This paper proposes an adaptive refinement scheme for the grid of candidate breakpoints in order to allow the dynamic programming method to scale for larger instances of the problem. We evaluate the quality of solutions found on small instances compared with optimal solutions determined by a novel integer programming formulation of the problem. We also consider a generalization of the linear spline regression problem to fit multiple curves that share breakpoint horizontal coordinates, and we extend our method to solve the generalized problem. Computational experiments verify that our nonuniform grid construction schemes are useful for computing high-quality solutions for both the single-curve and two-curve linear spline regression problem. C1 [Goldberg, Noam] Bar Ilan Univ, Dept Management, IL-52900 Ramat Gan, Israel. [Kim, Youngdae] Univ Wisconsin, Dept Comp Sci, Madison, WI 53706 USA. [Leyffer, Sven] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Veselka, Thomas D.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Goldberg, N (reprint author), Bar Ilan Univ, Dept Management, IL-52900 Ramat Gan, Israel. EM noam.goldberg@biu.ac.il; youngdae@cs.wisc.edu; leyffer@mcs.anl.gov; tdveselka@anl.gov FU Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 11 TC 0 Z9 0 U1 1 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0926-6003 EI 1573-2894 J9 COMPUT OPTIM APPL JI Comput. Optim. Appl. PD JUL PY 2014 VL 58 IS 3 BP 523 EP 541 DI 10.1007/s10589-014-9647-y PG 19 WC Operations Research & Management Science; Mathematics, Applied SC Operations Research & Management Science; Mathematics GA AI7PB UT WOS:000337084900001 ER PT J AU Li, Q Wu, G Johnston, CM Zelenay, P AF Li, Qing Wu, Gang Johnston, Christina M. Zelenay, Piotr TI Direct Dimethyl Ether Fuel Cell with Much Improved Performance SO ELECTROCATALYSIS LA English DT Article DE Dimethyl ether; DME; Electrooxidation; PtRu catalysts; Direct dimethyl ether fuel cell ID METHANOL ELECTROOXIDATION; ACID-SOLUTIONS; ANODE; CATALYSTS; ELECTRODE; DME; OXIDATION; CROSSOVER; MECHANISM AB Due to several apparent advantages over methanol, dimethyl ether (DME) has been viewed as a promising alternative fuel for direct fuel cell technology. Similar to methanol, DME oxidation requires a surface oxidant, such as OH, for the removal of adsorbed CO. Consequently, the reaction occurs at much faster rates on binary PtRu catalysts than Pt alone. In this work, PtRu catalysts with a wide variety of Pt-to-Ru ratios were systematically studied in the direct DME fuel cell (DDMEFC) operating at 80 degrees C. A Pt50Ru50 catalyst was found to perform the best at high and middle voltages, while a Pt80Ru20 catalyst performed best at low voltages. DDMEFC operation conditions, such as DME flow rate, anode back pressure, DME-to-water molar ratio, and membrane thickness, were also studied in order to maximize the cell performance. A maximum power density of 0.12 W cm(-2) obtained in this work exceeds the highest reported DME performance. In comparison with the direct methanol fuel cell (DMFC), the optimized DDMEFC performs better at cell voltages higher than 0.55 and 0.49 V with feed concentrations of methanol of 0.5 and 1.0 M, respectively. C1 [Li, Qing; Wu, Gang; Johnston, Christina M.; Zelenay, Piotr] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Zelenay, P (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. EM zelenay@lanl.gov RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU DOE-EERE Fuel Cell Technologies Program [FC091] FX Financial support from the DOE-EERE Fuel Cell Technologies Program (project ID: FC091) is gratefully acknowledged. NR 22 TC 3 Z9 3 U1 4 U2 51 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1868-2529 EI 1868-5994 J9 ELECTROCATALYSIS-US JI Electrocatalysis PD JUL PY 2014 VL 5 IS 3 BP 310 EP 317 DI 10.1007/s12678-014-0196-z PG 8 WC Chemistry, Physical; Electrochemistry SC Chemistry; Electrochemistry GA AI7DF UT WOS:000337041700013 ER PT J AU VandeVoort, AR Tappero, R Arai, Y AF VandeVoort, Allison Rick Tappero, Ryan Arai, Yuji TI Residence time effects on phase transformation of nanosilver in reduced soils SO ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH LA English DT Article DE Silver nanoparticles; Silver; Fate; Soils; X-ray microprobe; XANES ID SILVER NANOPARTICLES; SPECIATION; EXPOSURE; DISSOLUTION; ENVIRONMENT; INTERFACE; CHEMISTRY; KINETICS; RELEASE; SULFIDE AB Residence time effects on phase transformation of silver nanoparticles (AgNPs) (15-50 nm, with and without polyvinylpyrrolidone (PVP) coating) were investigated in reducing soils using experimental geochemistry and synchrotron-based x-ray techniques. After 30 days of anaerobic incubation, a substantial fraction of PVP-coated AgNPs (15 nm) were transformed into Ag2S and or humic acid (HA) complexed Ag(I), whereas only the HA fraction was dominant in uncoated AgNPs (50 nm). Several investigations recently reported that sulfidation of AgNPs to Ag2S was the predominant mechanism controlling the fate of AgNP in soil-water environments. However, this investigation showed each AgNP underwent particle-specific chemical transformations to different end compounds after 30 days. Considering the small contribution of Ag(I) dissolution from all AgNPs (less than 5%), we concluded that changes in solid-state chemical speciation of sorbed AgNPs was promoted by particle-specific interactions of NPs in soil chemical constituents, suggesting a critical role of soil absorbents in predicting the fate of AgNPs in terrestrial environments. C1 [VandeVoort, Allison Rick] Georgia Coll & State Univ, Dept Biol & Environm Sci, Milledgeville, GA 31061 USA. [Tappero, Ryan] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Arai, Yuji] Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA. RP Arai, Y (reprint author), Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA. EM yarai@illinois.edu FU AFRI Competitive Grants Program, Nanotechnology for Agriculture and Food systems [2011-03580]; US DOE-Geosciences [DE-FG02-92ER14244]; BNL-Department of Environmental Sciences; US DOE, Office of Science, Office of BES [DE-AC02-98CH10886] FX This research was supported by the 2011 AFRI Competitive Grants Program, Nanotechnology for Agriculture and Food systems (#2011-03580). Portions of this work were performed at BLX27A, NSLS, Brookhaven National Laboratory. X27A is supported in part by the US DOE-Geosciences (DE-FG02-92ER14244 to The University of Chicago - CARS) and BNL-Department of Environmental Sciences. Use of the NSLS was supported by the US DOE, Office of Science, Office of BES, under Contract No. DE-AC02-98CH10886. NR 35 TC 4 Z9 4 U1 5 U2 45 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 0944-1344 EI 1614-7499 J9 ENVIRON SCI POLLUT R JI Environ. Sci. Pollut. Res. PD JUL PY 2014 VL 21 IS 13 BP 7828 EP 7837 DI 10.1007/s11356-014-2743-9 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA AI7PO UT WOS:000337086600005 ER PT J AU McFarland, JA Greenough, JA Ranjan, D AF McFarland, Jacob A. Greenough, Jeffrey A. Ranjan, Devesh TI Simulations and Analysis of the Reshocked Inclined Interface Richtmyer-Meshkov Instability for Linear and Nonlinear Interface Perturbations SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article ID SHOCK-WAVES; HYDRODYNAMIC ISSUES; AIR/SF6 INTERFACE; GAS INTERFACE; TUBE; REFINEMENT; DEPOSITION; GROWTH; FLOW AB A computational study of the Richtmyer-Meshkov instability (RMI) is presented for an inclined interface perturbation in support of experiments being performed at the Texas A&M shock tube facility. The study is comprised of 2D, viscous, diffusive, compressible simulations performed using the arbitrary Lagrange Eulerian code, ARES, developed at Lawrence Livermore National Laboratory. These simulations were performed to late times after reshock with two initial interface perturbations, in the linear and nonlinear regimes each, prescribed by the interface inclination angle. The interaction of the interface with the reshock wave produced a complex 2D set of compressible wave interactions including expansion waves, which also interacted with the interface. Distinct differences in the interface growth rates prior to reshock were found in previous work. The current work provides in-depth analysis of the vorticity and enstrophy fields to elucidate the physics of reshock for the inclined interface RMI. After reshock, the two cases exhibit some similarities in integral measurements despite their disparate initial conditions but also show different vorticity decay trends, power law decay for the nonlinear and linear decay for the linear perturbation case. C1 [McFarland, Jacob A.; Ranjan, Devesh] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Greenough, Jeffrey A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Ranjan, D (reprint author), Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. EM jacmcfar@tamu.edu; greenough1@llnl.gov; dranjan@tamu.edu OI Ranjan, Devesh/0000-0002-1231-9313 FU U.S. Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; CAREER NSF [1254760] FX The authors would like to thank the HEDP summer student program at LLNL. The authors would like to thank the scientists and staff of LLNL that helped make this work possible. This work was performed under the auspices of the U.S. Department of Energy, Lawrence Livermore National Laboratory, under Contract No. DE-AC52-07NA27344. D. R. would like to acknowledge the support of CAREER NSF Award 1254760. NR 55 TC 4 Z9 4 U1 0 U2 8 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD JUL PY 2014 VL 136 IS 7 AR 071203 DI 10.1115/1.4026858 PG 11 WC Engineering, Mechanical SC Engineering GA AI7EL UT WOS:000337045900008 ER PT J AU Xie, ZL Graule, M Orlovskaya, N Payzant, EA Cullen, DA Blair, RG AF Xie, Zhilin Graule, Moritz Orlovskaya, Nina Payzant, E. Andrew Cullen, David A. Blair, Richard G. TI Novel high pressure hexagonal OsB2 by mechanochemistry SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE Osmium; Boron; Mechanochemistry; Ceramic ID OSMIUM DIBORIDE; SUPERHARD MATERIAL; CRYSTAL STRUCTURE; RHENIUM DIBORIDE; HARD MATERIAL; BORIDES; PHASE; RUB2; TRANSITION; IRIDIUM AB Hexagonal OsB2, a theoretically predicted high-pressure phase, has been synthesized for the first time by a mechanochemical method, i.e., high energy ball milling. X-ray diffraction indicated that formation of hexagonal OsB2 begins after 2.5 h of milling, and the reaction reaches equilibrium after 18 h of milling. Rietveld refinement of the powder data indicated that hexagonal OsB2 crystallizes in the P63/mmc space group (No. 194) with lattice parameters of a=2.916 angstrom and c=7.376 angstrom. Transmission electron microscopy confirmed the appearance of the hexagonal OsB2 phase after high energy ball milling, in situ X-ray diffraction experiments showed that the phase is stable from 225 degrees C to 1050 degrees C. The hexagonal OsB2 powder was annealed at 1050 degrees C for 6 days in vacua to improve crystallinity and remove strain induced during the mechanochemical synthesis. The structure partially converted to the orthorhombic phase (20 wt%) after fast current assisted sintering of hexagonal OsB2 at 1500 degrees C for 5 min. Mechanochemical approaches to the synthesis of hard boride materials allow new phases to be produced that cannot be prepared using conventional methods. (C) 2014 Elsevier Inc. All rights reserved. C1 [Xie, Zhilin; Graule, Moritz; Orlovskaya, Nina] Univ Cent Florida, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA. [Payzant, E. Andrew] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Cullen, David A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Blair, Richard G.] Univ Cent Florida, Dept Chem, Orlando, FL 32816 USA. RP Orlovskaya, N (reprint author), Univ Cent Florida, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA. EM Nina.Orlovskaya@ucf.edu RI Payzant, Edward/B-5449-2009; Cullen, David/A-2918-2015 OI Payzant, Edward/0000-0002-3447-2060; Cullen, David/0000-0002-2593-7866 FU Center for Nanophase Material Sciences, Oak Ridge National Laboratory; Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program - Office of Basic Energy Sciences, U.S. Department of Energy; U.S. DOE [DE-AC02-06CH11357] FX This work was supported by NSF projects- DMR-0748364. High and low temperature X-ray diffraction studies were supported by Center for Nanophase Material Sciences, Oak Ridge National Laboratory; STEM studies were supported by Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program, which is sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy. We gratefully acknowledge the use of WebEMAPS for generating simulated diffraction patterns, available online at http://emaps.mrl.uiuc.edu/. We acknowledge Prof. Miladin Radovic and Mr. Huili Gao, Texas A&M University, College Station, Texas for the help with SPS, and Dr. Yan Chen, Spallation Neutron Source, Oak Ridge National Laboratory, Oak Ridge, Tennessee for the help with Rietveld refinement Use of the Advanced Photon Source was supported by the Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract no. DE-AC02-06CH11357. NR 30 TC 8 Z9 8 U1 2 U2 33 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD JUL PY 2014 VL 215 BP 16 EP 21 DI 10.1016/j.jssc.2014.03.020 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA AI5FR UT WOS:000336891300003 ER PT J AU Dera, P Manghnani, MH Hushur, A Hu, Y Tkachev, S AF Dera, Przemyslaw Manghnani, Murli H. Hushur, Anwar Hu, Yi Tkachev, Sergey TI New insights into the enigma of boron carbide inverse molecular behavior SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE High pressure; Superhard materials; Boron carbide; Icosahedral boron compounds; Elastic properties; Phase transitions ID ALPHA-RHOMBOHEDRAL BORON; DEFORMATION DENSITIES; FORCE-CONSTANTS; B13C2; PRESSURE; CHAINS; B4C AB Equation of state and compression mechanism of nearly stoichiometric boron carbide B4C were investigated using diamond anvil cell single crystal synchrotron X-ray diffraction technique up to a maximum quasi-hydrostatic pressure of 74.0(1) GPa in neon pressure transmitting medium at ambient temperature. No signatures of structural phase transitions were observed on compression. Crystal structure refinements indicate that the icosahedral units are less compressible (13% volume reduction at 60 GPa) than the unit cell volume (18% volume reduction at 60 GPa), contrary to expectations based on the inverse molecular behavior hypothesis, but consistent with spectroscopic evidence and first principles calculations. The high-pressure crystallographic refinements reveal that the nature of the chemical bonds (two, versus three centered character) has marginal effect on the bond compressibility and the compression of the crystal is mainly governed by the force transfer between the rigid icosahedral structural units. (C) 2014 Elsevier Inc. All rights reserved. C1 [Dera, Przemyslaw; Manghnani, Murli H.; Hushur, Anwar; Hu, Yi] Univ Hawaii, Sch Ocean & Earth Sci & Technol, Hawaii Inst Geophys & Planetol, Honolulu, HI 96822 USA. [Tkachev, Sergey] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, Argonne, IL 60439 USA. RP Dera, P (reprint author), Univ Hawaii, Sch Ocean & Earth Sci & Technol, Hawaii Inst Geophys & Planetol, 1680 East West Rd,POST Bldg, Honolulu, HI 96822 USA. EM pdera@hawaii.edu FU Carnegie - Department of Energy Alliance Center (CDAC); National Science Foundation - Earth Sciences [EAR-1128799]; U.S. Department of Energy - Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We would like or express our thanks to all three anonymous reviewers for their valuable and constructive comments and suggestions. PD and YH were supported by a grant from Carnegie - Department of Energy Alliance Center (CDAC). This work was performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation - Earth Sciences (EAR-1128799) and U.S. Department of Energy - Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract no. DE-AC02-06CH11357. NR 40 TC 9 Z9 9 U1 5 U2 36 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD JUL PY 2014 VL 215 BP 85 EP 93 DI 10.1016/j.jssc.2014.03.018 PG 9 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA AI5FR UT WOS:000336891300013 ER PT J AU Zhang, HK Yao, ZW Kirk, MA Daymond, MR AF Zhang, He K. Yao, Zhongwen Kirk, Marquis A. Daymond, Mark R. TI Stability of Ni-3(Al, Ti) Gamma Prime Precipitates in a Nickel-Based Superalloy Inconel X-750 Under Heavy Ion Irradiation SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID NEUTRON DAMAGE; ALLOYS; AL; DISSOLUTION; MECHANISMS; EVOLUTION; KINETICS; HELIUM; ORDER; IRON AB Phase stability of Ni-3(Al, Ti) precipitates in Inconel X-750 under cascade damage was studied using heavy ion irradiation with transmission electron microscope (TEM) in situ observations. From 333 K to 673 K (60 A degrees C to 400 A degrees C), ordered Ni-3(Al, Ti) precipitates became completely disordered at low irradiation dose of 0.06 displacement per atom (dpa). At higher dose, a trend of precipitate dissolution occurring under disordered state was observed, which is due to the ballistic mixing effect by irradiation. However, at temperatures greater than 773 K (500 A degrees C), the precipitates stayed ordered up to 5.4 dpa, supporting the view that irradiation-induced disordering/dissolution and thermal recovery reach a balance between 673 K and 773 K (400 A degrees C and 500 A degrees C). Effects of Ti/Al ratio and irradiation dose rate are also discussed. (C) The Minerals, Metals & Materials Society and ASM International 2014 C1 [Zhang, He K.; Yao, Zhongwen; Daymond, Mark R.] Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. [Kirk, Marquis A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Yao, ZW (reprint author), Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. EM yaoz@me.queensu.ca OI Daymond, Mark/0000-0001-6242-7489 FU Canada UNENE-CRD Project; National Science and Engineering Research Council (NSERC); Industry Research Chair of Nuclear Program; US Department of Energy Office of Science FX The current study is funded by the Canada UNENE-CRD Project, National Science and Engineering Research Council (NSERC) and Industry Research Chair of Nuclear Program. Electron microscopy was accomplished at the Electron Microscopy Centre for Materials Research at Argonne National Laboratory, supported by the US Department of Energy Office of Science. The authors thank Mr. Pete Boldo and Mr. Ed Ryan of Argonne National Lab for their help with the microscopy and ion beam facility. The authors also thank Prof Rick Holt of Queen's University and Dr. Malcolm Griffiths of AECL Chalk River Laboratories for their insightful discussions. NR 29 TC 5 Z9 5 U1 2 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD JUL PY 2014 VL 45A IS 8 BP 3422 EP 3428 DI 10.1007/s11661-014-2309-y PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI7MX UT WOS:000337076900025 ER PT J AU Heo, TW Shih, DS Chen, LQ AF Heo, Tae Wook Shih, Donald S. Chen, Long-Qing TI Kinetic Pathways of Phase Transformations in Two-Phase Ti Alloys SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID TITANIUM-ALLOYS; BETA-PHASE; V ALLOYS; MARTENSITIC TRANSFORMATIONS; SPINODAL DECOMPOSITION; NB ALLOYS; MICROSTRUCTURE; TI-6AL-4V; OMEGA; MO AB Possible phase transformation kinetic pathways from the high temperature beta phase to the low temperature (alpha + beta) two-phase Ti alloys were analyzed using the graphical thermodynamic method and the assumption that diffusionless and displacive transformations take place much faster than phase separation which requires long-range diffusion. It is shown that depending on the composition of a beta-stabilizing element, many transformation mechanisms are possible, involving competing continuous and discontinuous displacive/diffusional transformations. We discuss the proposed phase transformation sequences employing existing experimental microstructures. C1 [Heo, Tae Wook; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Shih, Donald S.] Boeing Res & Technol, St Louis, MO 63166 USA. RP Heo, TW (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. EM heo1@llnl.gov FU Center for Computational Materials Design (CCMD); National Science Foundation (NSF) Industry/University Cooperative Research Center at Penn State [IIP-1034965]; Georgia Tech [IIP-1034968] FX This work is funded by the Center for Computational Materials Design (CCMD), a joint National Science Foundation (NSF) Industry/University Cooperative Research Center at Penn State (IIP-1034965) and Georgia Tech (IIP-1034968). NR 31 TC 3 Z9 3 U1 0 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD JUL PY 2014 VL 45A IS 8 BP 3438 EP 3445 DI 10.1007/s11661-014-2269-2 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI7MX UT WOS:000337076900027 ER PT J AU Cordero, ZC Huskins, EL Park, M Livers, S Frary, M Schuster, BE Schuh, CA AF Cordero, Zachary C. Huskins, Emily L. Park, Mansoo Livers, Steven Frary, Megan Schuster, Brian E. Schuh, Christopher A. TI Powder-Route Synthesis and Mechanical Testing of Ultrafine Grain Tungsten Alloys SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID PLASMA PRESSURE COMPACTION; NI-W ALLOYS; REFRACTORY-METALS; HIGH-STRAIN; NANOCRYSTALLINE; SIZE; BEHAVIOR; HARDNESS; COMPRESSION; DRAWN AB We report a W-rich alloy (W-7Cr-9Fe, at. pct) produced by high-energy ball milling, with alloying additions that both lower the densification temperature and retard grain growth. The alloy's consolidation behavior and the resultant compacts' microstructure and mechanical properties are explored. Under one condition, a 98 pct dense compact with a mean grain size of 130 nm was achieved, and exhibited a hardness of 13.5 GPa, a dynamic uniaxial yield strength of 4.14 GPa in Kolsky bar experiments, and signs of structural shear localization during deformation. C1 [Cordero, Zachary C.; Park, Mansoo; Schuh, Christopher A.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Huskins, Emily L.] Army Res Lab, Oak Ridge Inst Sci & Educ, Postdoctoral Fellowship Program, Aberdeen Proving Ground, MD 21005 USA. [Livers, Steven; Frary, Megan] Boise State Univ, Dept Mat Sci & Engn, Boise, ID 83725 USA. [Schuster, Brian E.] Army Res Laboratory, Expt & Computat Penetrat Mech Team, Weap & Mat Res Directorate, Adelphi, MD USA. RP Cordero, ZC (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. EM schuh@mit.edu FU US Defense Threat Reduction Agency [HDTRA1-11-1-0062]; Department of Defense through the NDSEG fellowship program; US Army Research Laboratory through the Oak Ridge Institute for Space and Education (ORISE) Program [1120-1120-99]; [11-24] FX This study was supported by the US Defense Threat Reduction Agency under Grant No. HDTRA1-11-1-0062. ZCC acknowledges support from the Department of Defense through the NDSEG fellowship program. ELH acknowledges support from the US Army Research Laboratory through the Oak Ridge Institute for Space and Education (ORISE) Program # 1120-1120-99. BES would like to acknowledge support work from the Cooperative Research and Development Agreement #11-24. We would like to thank Ms. Alexandria Will-Cole for her indentation work on the intermetallic phase, Dr. Kisub Cho for performing the THERMOCALC calculations, and Dr. Daniel T. Casem for his assistance with the Kolsky bar tests. NR 58 TC 3 Z9 3 U1 5 U2 34 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD JUL PY 2014 VL 45A IS 8 BP 3609 EP 3618 DI 10.1007/s11661-014-2286-1 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI7MX UT WOS:000337076900043 ER PT J AU Morris, CL Bacon, J Borozdin, K Fabritius, J Miyadera, H Perry, J Sugita, T AF Morris, Christopher L. Bacon, Jeffrey Borozdin, Konstantin Fabritius, Joseph Miyadera, Haruo Perry, John Sugita, Tsukasa TI Horizontal cosmic ray muon radiography for imaging nuclear threats SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Muon tomography; Coulomb scattering cosmic ray tracking detectors; Imaging with near horizontal muons; Imaging with near vertical muons ID TOMOGRAPHY; RECONSTRUCTION; SCATTERING; SYSTEM AB Muon tomography is a technique that uses information contained in the Coulomb scattering of cosmic ray muons to generate three dimension images of volumes between tracking detectors. Advantages of this technique are the muons ability to penetrate significant overburden and the absence of any additional dose beyond the natural cosmic ray flux. Disadvantages include the long exposure times and limited resolution because of the low flux. Here we compare the times needed to image objects using both vertically and horizontally mounted tracking detectors and we develop a predictive model for other geometries. (C) 2014 The Authors. Published by Elsevier B.V. C1 [Morris, Christopher L.; Bacon, Jeffrey; Borozdin, Konstantin; Fabritius, Joseph; Miyadera, Haruo; Perry, John] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Sugita, Tsukasa] Toshiba Co Ltd, Power Syst Co, Kawasaki Ku, Kawasaki, Kanagawa, Japan. RP Morris, CL (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM cmorris@lanl.gov OI Morris, Christopher/0000-0003-2141-0255; Perry, John/0000-0003-3639-5617 FU Toshiba Corporation Power Systems Company; Tokyo Electric Power Company; United States Department of Energy FX This work was supported in part by Toshiba Corporation Power Systems Company, Tokyo Electric Power Company and by the United States Department of Energy. NR 29 TC 6 Z9 7 U1 2 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD JUL 1 PY 2014 VL 330 BP 42 EP 46 DI 10.1016/j.nimb.2014.03.017 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AI6WD UT WOS:000337016800007 ER PT J AU He, LF Pakarinen, J Kirk, MA Gan, J Nelson, AT Bai, XM El-Azab, A Allen, TR AF He, L. F. Pakarinen, J. Kirk, M. A. Gan, J. Nelson, A. T. Bai, X. -M. El-Azab, A. Allen, T. R. TI Microstructure evolution in Xe-irradiated UO2 at room temperature SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Nuclear fuel; TEM; Irradiation; Dislocation; Inert gas bubble ID HIGH-RESOLUTION TEM; IN-SITU TEM; URANIUM-DIOXIDE; RADIATION-DAMAGE; BUBBLES; PRECIPITATION; KRYPTON; XENON; FUELS AB In situ Transmission Electron Microscopy was conducted for single crystal UO2 to understand the microstructure evolution during 300 key Xe irradiation at room temperature. The dislocation microstructure evolution was shown to occur as nucleation and growth of dislocation loops at low irradiation doses, followed by transformation to extended dislocation segments and tangles at higher doses. Xe bubbles with dimensions of 1-2 nm were observed after room-temperature irradiation. Electron Energy Loss Spectroscopy indicated that UO2 remained stoichiometric under room temperature Xe irradiation. Published by Elsevier B.V. C1 [He, L. F.; Pakarinen, J.; Allen, T. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Kirk, M. A.] Argonne Natl Lab, Argonne, IL 60439 USA. [Gan, J.; Bai, X. -M.; Allen, T. R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Nelson, A. T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [El-Azab, A.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. [El-Azab, A.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. RP He, LF (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. EM lhe33@wisc.edu RI Bai, Xianming/E-2376-2017; OI Bai, Xianming/0000-0002-4609-6576; Allen, Todd/0000-0002-2372-7259; He, Lingfeng/0000-0003-2763-1462 FU Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office [DE-AC07-051D14517]; Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This work was supported as part of the Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. A portion of this research was supported by the U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-051D14517. The in situ electron microscopy observation was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. We thank Peter M. Baldo of Argonne National Lab for his help in performing the irradiations. NR 23 TC 5 Z9 5 U1 0 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD JUL 1 PY 2014 VL 330 BP 55 EP 60 DI 10.1016/j.nimb.2014.03.018 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AI6WD UT WOS:000337016800009 ER PT J AU Yoon, SJ Sabharwall, P AF Yoon, Su-Jong Sabharwall, Piyush TI Parametric study on maximum transportable distance and cost for thermal energy transportation using various coolants SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE Advanced nuclear reactor; Thermal energy transportation; Maximum transportable distance; Cost estimation; Molten-salts; Helium AB The operation temperature of advanced nuclear reactors is generally higher than commercial light water reactors, and thermal energy from advanced nuclear reactor can be used for various purposes, such as district heating, desalination, hydrogen production and other process heat applications. The process heat industry/facilities will be located outside the nuclear island due to safety measures. This thermal energy from the reactor must be transported a fair distance. In this study, the analytical analysis was conducted to identify the maximum distance that thermal energy could be transported using various coolants such as molten-salts, helium, and water by varying the pipe diameter and mass flow rate. The cost required to transport each coolant was also analyzed. The coolants analyzed are molten salts (such as: KClMgCl2, LiF-NaF-KF (FLiNaK) and KF-ZrF4), helium, and water. Fluoride salts are superior because of better heat transport characteristics, but chloride salts are most economical for higher temperature transportation purposes. For lower temperature, the water is a possible alternative when compared with helium because low-pressure helium requires extremely high pumping power, which makes the process very inefficient and economically not viable for both low and high-temperature application. Published by Elsevier Ltd. C1 [Yoon, Su-Jong; Sabharwall, Piyush] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Yoon, SJ (reprint author), Idaho Natl Lab, 2525 Fremont Ave, Idaho Falls, ID 83415 USA. EM sujong.yoon@inl.gov FU agency of the U.S. Government FX This information was prepared as an account of work sponsored by an agency of the U.S. Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. References herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the U.S. Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the U.S. Government or any agency thereof. NR 12 TC 0 Z9 0 U1 0 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD JUL PY 2014 VL 74 BP 110 EP 119 DI 10.1016/j.pnucene.2014.02.016 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AI6VU UT WOS:000337015900010 ER PT J AU Hernandez-Garcia, MR Masri, SF Ghanem, R Figueiredo, E Farrar, CR AF Hernandez-Garcia, Miguel R. Masri, Sami F. Ghanem, Roger Figueiredo, Eloi Farrar, Charles R. TI An Evaluation of a Methodology for Detection, Localization, and Quantification of Changes in Nonlinear Systems Based on Experimental Measurements SO INGEGNERIA SISMICA LA English DT Article DE Structural Health Monitoring; reduced-order models; structural changes; restoring forces ID CHAIN-LIKE SYSTEMS; NONPARAMETRIC IDENTIFICATION; BUILDINGS; DYNAMICS AB Experimental data from a test-bed structure tested is used to evaluate and validate a methodology for detecting, localizing, and quantifying structural changes in nonlinear structures using chain-like reduced-order models estimated from measurements. This study showed that variations in the mathematical representation (i.e., two-dimensional polynomial expansion) of the restoring forces in the estimated chain-like reduced-order models could be employed to confidently detect the presence of physical structural changes introduced into the test-bed structure, accurately locate the structural section where the changes occurred, and provide an estimate of the severity or magnitude of the structural changes. C1 [Hernandez-Garcia, Miguel R.] Alta Vista Solut, Richmond, CA 94806 USA. [Hernandez-Garcia, Miguel R.; Masri, Sami F.; Ghanem, Roger] Univ So Calif, Viterbi Sch Engn, Los Angeles, CA 90089 USA. [Figueiredo, Eloi] Univ Lusfona, Fac Engn, Dept Civil Engn, Lisbon, Portugal. [Farrar, Charles R.] Los Alamos Natl Lab, Engn Inst, Los Alamos, NM 87545 USA. RP Hernandez-Garcia, MR (reprint author), Alta Vista Solut, 3260 Blume Dr,Suite 500, Richmond, CA 94806 USA. RI Ghanem, Roger/B-8570-2008 OI Ghanem, Roger/0000-0002-1890-920X FU National Science Foundation FX This study was supported in part by a grant from the National Science Foundation. NR 24 TC 0 Z9 0 U1 0 U2 0 PU PATRON EDITORE S R L PI BOLOGNA PA VIA BADINI 12, QUARTO INFERIORE, BOLOGNA, 00000, ITALY SN 0393-1420 J9 ING SISMICA-ITAL JI Ing. Sismica PD JUL-DEC PY 2014 VL 31 IS 3-4 BP 72 EP 86 PG 15 WC Engineering, Civil; Engineering, Geological SC Engineering GA CP6AO UT WOS:000359966900007 ER PT J AU Zhang, JS Cui, LS Yu, C Shao, Y Wang, ZQ Ru, YD Zhang, G Jiang, DQ Huan, Y Ren, Y AF Zhang, J. S. Cui, L. S. Yu, C. Shao, Y. Wang, Z. Q. Ru, Y. D. Zhang, G. Jiang, D. Q. Huan, Y. Ren, Y. TI Novel Ti3Sn based high damping material with high strength SO MATERIALS RESEARCH INNOVATIONS LA English DT Article DE Damping; Ti3Sn; Synchrotron ID METAL-MATRIX COMPOSITES; ALLOY; BEHAVIOR; CAPACITY AB In this paper, ductile beta-Ti was selected to toughen brittle high damping intermetallic compound Ti3Sn. An in situ Ti3Sn/beta-Ti composite with a composition of Ti77Mo3Sn20 was prepared by arc melting. The composite simultaneously exhibited high yield strength (500 MPa), large plasticity (35%) and high damping capacity (tan delta>0.06). In situ synchrotron high energy X-ray diffraction compression testing revealed that the beta-Ti mainly accounts for the plasticity, while Ti3Sn provided the strength of the composite. C1 [Zhang, J. S.; Cui, L. S.; Yu, C.; Shao, Y.; Wang, Z. Q.; Ru, Y. D.; Zhang, G.; Jiang, D. Q.] China Univ Petr, Dept Mat Sci & Engn, Beijing 102200, Peoples R China. [Huan, Y.] Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech LNM, Beijing 100190, Peoples R China. [Ren, Y.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Cui, LS (reprint author), China Univ Petr, Dept Mat Sci & Engn, Beijing 102200, Peoples R China. EM lishancui63@126.com RI Jiang, Daqiang /G-5511-2014; OI Yu, Cun/0000-0003-0084-6746 FU National Natural Science Foundation of China (NSFC) [51071175]; Key (key grant) Project of Chinese Ministry of Education [313055]; US Department of Energy, Office of Science and Office of Basic Energy Science [DE-AC02-06CH11357] FX This work was financially supported by the National Natural Science Foundation of China (NSFC) (Grant No. 51071175) and the Key (key grant) Project of Chinese Ministry of Education (Grant No. 313055). The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science and Office of Basic Energy Science under contract no. DE-AC02-06CH11357. NR 12 TC 0 Z9 0 U1 1 U2 1 PU MANEY PUBLISHING PI LEEDS PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND SN 1432-8917 EI 1433-075X J9 MATER RES INNOV JI Mater. Res. Innov. PD JUL PY 2014 VL 18 SU 4 BP 584 EP 587 DI 10.1179/1432891714Z.000000000750 PG 4 WC Materials Science, Multidisciplinary SC Materials Science GA AW3HZ UT WOS:000346178400118 ER PT J AU Khanna, N Fridley, D Hong, LX AF Khanna, Nina Fridley, David Hong, Lixuan TI China's pilot low-carbon city initiative: A comparative assessment of national goals and local plans SO SUSTAINABLE CITIES AND SOCIETY LA English DT Article DE China; Low carbon city; Energy consumption AB In the past decade, China's unprecedented urbanization has paralleled a 250% growth in primary energy demand and urban areas have emerged as the crux of energy and CO2 emissions reduction in China. In recognition of cities' importance in mitigating future energy and CO2 emissions growth, the Chinese government launched a demonstration program of 5 low-carbon pilot provinces and 8 pilot cities in 2010 to promote low-carbon urban development. As one of the first national programs to promote low-carbon urban development, the recent plans and policies adopted by these 8 pilot low-carbon cities can shed light on if and how low-carbon cities can shape China's future energy and emission trajectories. This paper reviews the historical development and context for low-carbon urban development in China and then presents an ex-ante comparative assessment of the low-carbon development plans and supporting measures formulated for each of China's 8 pilot low-carbon cities. We find that while the 8 pilot cities have made progress in establishing low-carbon plans, key barriers such as a lack of explicit definition for low-carbon city, complexity and confusion resulting from several parallel programs, and insufficient supporting policies and market-based instruments may hinder urban development that is truly low carbon. Published by Elsevier B.V. C1 [Khanna, Nina; Fridley, David; Hong, Lixuan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. RP Khanna, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, MS 90R2002, Berkeley, CA 94720 USA. EM xzheng@lbl.gov FU U.S, Department of Energy [DE-AC02-05CH11231] FX This work was supported through the U.S, Department of Energy under Contract No, DE-AC02-05CH11231, We are grateful to He Gang of LBNL for reviewing an earlier draft of this paper, and to the two anonymous reviewers for their valuable feedback and suggestions. NR 35 TC 12 Z9 12 U1 5 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2210-6715 J9 SUSTAIN CITIES SOC JI Sust. Cities Soc. PD JUL PY 2014 VL 12 BP 110 EP 121 DI 10.1016/j.scs.2014.03.005 PG 12 WC Construction & Building Technology; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Construction & Building Technology; Science & Technology - Other Topics; Energy & Fuels GA V41OE UT WOS:000209554700013 ER PT J AU Callejo, A Narayanan, SHK de Jalon, JG Norris, B AF Callejo, Alfonso Narayanan, Sri Hari Krishna Garcia de Jalon, Javier Norris, Boyana TI Performance of automatic differentiation tools in the dynamic simulation of multibody systems SO ADVANCES IN ENGINEERING SOFTWARE LA English DT Article DE Multibody dynamics; Semi-recursive penalty formulation; Automatic differentiation; Operator overloading; Source-to-source transformation; ADOL-C; ADIC2 ID ALGORITHMS AB Within the multibody systems literature, few attempts have been made to use automatic differentiation for solving forward multibody dynamics and evaluating its computational efficiency. The most relevant implementations are found in the sensitivity analysis field, but they rarely address automatic differentiation issues in depth. This paper presents a thorough analysis of automatic differentiation tools in the time integration of multibody systems. To that end, a penalty formulation is implemented. First, open-chain generalized positions and velocities are computed recursively, while using Cartesian coordinates to define local geometry. Second, the equations of motion are implicitly integrated by using the trapezoidal rule and a Newton-Raphson iteration. Third, velocity and acceleration projections are carried out to enforce kinematic constraints. For the computation of Newton-Raphson's tangent matrix, instead of using numerical or analytical differentiation, automatic differentiation is implemented here. Specifically, the source-to-source transformation tool ADIC2 and the operator overloading tool ADOL-C are employed, in both dense and sparse modes. The theoretical approach is backed with the numerical analysis of a 1-DOF spatial four-bar mechanism, three different configurations of a 15-DOF multiple four-bar linkage, and a 16-DOF coach maneuver. Numerical and automatic differentiation are compared in terms of their computational efficiency and accuracy. Overall, we provide a global perspective of the efficiency of automatic differentiation in the field of multibody system dynamics. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Callejo, Alfonso; Garcia de Jalon, Javier] Univ Politecn Madrid, Inst Univ Invest Automovil, Madrid, Spain. [Narayanan, Sri Hari Krishna; Norris, Boyana] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA. RP Callejo, A (reprint author), Univ Politecn Madrid, Inst Univ Invest Automovil, Madrid, Spain. EM a.callejo@upm.es OI Norris, Boyana/0000-0001-5811-9731 FU U.S. Dept. of Energy Office of Science Applied Mathematics Program [DE-ACO2-06CH11357]; Spanish Ministry of Science and Innovation [TRA2009-14513CO2-01]; Government of Navarra FX This work was supported by the U.S. Dept. of Energy Office of Science Applied Mathematics Program (DE-ACO2-06CH11357), the Spanish Ministry of Science and Innovation (TRA2009-14513CO2-01) and the Government of Navarra. NR 26 TC 3 Z9 3 U1 1 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0965-9978 EI 1873-5339 J9 ADV ENG SOFTW JI Adv. Eng. Softw. PD JUL PY 2014 VL 73 BP 35 EP 44 DI 10.1016/j.advengsoft.2014.03.002 PG 10 WC Computer Science, Interdisciplinary Applications; Computer Science, Software Engineering; Engineering, Multidisciplinary SC Computer Science; Engineering GA AI4GF UT WOS:000336823000004 ER PT J AU Dorcioman, G Socol, G Craciun, D Argibay, N Lambers, E Hanna, M Taylor, CR Craciun, V AF Dorcioman, G. Socol, G. Craciun, D. Argibay, N. Lambers, E. Hanna, M. Taylor, C. R. Craciun, V. TI Wear tests of ZrC and ZrN thin films grown by pulsed laser deposition SO APPLIED SURFACE SCIENCE LA English DT Article; Proceedings Paper CT European-Materials-Research-Society Fall Meeting / Symposium B on Stress, Dtructure and Dtoichiometry Rffects on the Properties of Nanomaterials II CY SEP 16-20, 2013 CL Warsaw, POLAND SP European Mat Res Soc DE ZrC; ZrN; Hard coatings; Pulsed laser deposition ID COATINGS; CORROSION; INDENTATION; EVAPORATION; BEHAVIOR AB Very thin ZrC and ZrN films (<500 nm) were grown on (1 0 0) Si substrates at 500 degrees C by the pulsed laser deposition (PLD) technique using a KrF excimer laser. X-ray reflectivity investigations showed that films exhibited mass densities similar to bulk values. X-ray diffraction investigations found that films were nanocristalline, exhibited a (1 1 1) texture and high micro-strain values. Auger electron spectroscopy investigations indicated that films contained in bulk a relatively low oxygen concentration, usually below 2.0%. Atomic force microscopy found that ZrN films deposited under 2 X 10(-2) Pa of N-2 exhibited a very smooth surface, with an rms value of only 3 angstrom, while wear tests found a low wear rate of only 4.5 X 10(-6) mm(3)/N m. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dorcioman, G.; Socol, G.; Craciun, D.; Craciun, V.] Natl Inst Lasers Plasma & Radiat Phys, Laser Dept, Bucharest, Romania. [Argibay, N.] Sandia Natl Labs, Ctr Mat Sci & Engn, Albuquerque, NM 87123 USA. [Lambers, E.] Univ Florida, Coll Engn, Major Analyt Instrumentat Ctr, Gainesville, FL 32611 USA. [Hanna, M.; Taylor, C. R.] Univ Florida, Gainesville, FL 32611 USA. RP Craciun, D (reprint author), Natl Inst Lasers Plasma & Radiat Phys, 409 Atomistilor, RO-077125 Magurele, Romania. EM doina.craciun@inflpr.ro RI Socol, Gabriel/A-5405-2011 OI Socol, Gabriel/0000-0002-1992-7346 FU Romanian Ministry of Education; CNCS-UEFISCDI [PN-II-ID 337/2011, PN-II-RU-2012-3-0346]; project Nucleu 2013; Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to thank the Major Analytical Instrumentation Center-University of Florida for help with samples characterization. This work was supported by grants of the Romanian Ministry of Education, CNCS-UEFISCDI, project number PN-II-ID 337/2011 and PN-II-RU-2012-3-0346, and project Nucleu 2013. This work was partially funded by the Sandia National Laboratories, a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 21 TC 11 Z9 12 U1 7 U2 36 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD JUL 1 PY 2014 VL 306 BP 33 EP 36 DI 10.1016/j.apsusc.2013.12.048 PG 4 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AI1DX UT WOS:000336591500007 ER PT J AU Hale, LM Zimmerman, JA Weinberger, CR AF Hale, Lucas M. Zimmerman, Jonathan A. Weinberger, Christopher R. TI Simulations of bcc tantalum screw dislocations: Why classical inter-atomic potentials predict {112} slip SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Molecular dynamic simulation; Dislocation structures; Tantalum; Plasticity of metals ID MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; TRANSITION-METALS; CORE STRUCTURE; PLASTIC-DEFORMATION; ANISOTROPIC ELASTICITY; SINGLE-CRYSTALS; SADDLE-POINTS; ALPHA-FE; GLIDE AB A thorough molecular dynamics study is performed to investigate the predicted {112} yield behavior associated with the slip of a single screw dislocation using classical atomistic potentials of body-centered cubic metals. Previous works have drawn an association between the structure of the stable screw dislocation core and the resulting slip nature showing that a polarized core can lead to {112} slip, while a non-polarized core is expected to slip on {110} planes. Here, results from five different potentials for tantalum are presented as they all show slip to be primarily active along {112} planes even though the stable core structure is non-polar. This {112} slip occurs through dislocation glide on two different {110} planes due to the presence of a metastable split core structure, and regardless of the relative magnitudes of resolved shear stresses for the two {110} planes. Further investigations shows that the split core structure, an artifact of the atomic potentials used, also influences slip behavior associated with dynamic motion of kinked dislocations in ambient temperature simulations. (C) 2014 Elsevier B. V. All rights reserved. C1 [Hale, Lucas M.; Zimmerman, Jonathan A.] Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94551 USA. [Weinberger, Christopher R.] Sandia Natl Labs, Mat Sci & Engn Ctr, Albuquerque, NM 87125 USA. [Weinberger, Christopher R.] Drexel Univ, Philadelphia, PA 19104 USA. RP Hale, LM (reprint author), Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94551 USA. EM lmhale99@gmail.com FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 47 TC 5 Z9 5 U1 2 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD JUL PY 2014 VL 90 BP 106 EP 115 DI 10.1016/j.commatsci.2014.03.064 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA AI1ZX UT WOS:000336656200014 ER PT J AU Zhao, Y Ke, J Ni, CC McNeil, M Khanna, NZ Zhou, N Fridley, D Li, QQ AF Zhao, Yue Ke, Jing Ni, Chun Chun McNeil, Michael Khanna, Nina Zheng Zhou, Nan Fridley, David Li, Qiqiang TI A comparative study of energy consumption and efficiency of Japanese and Chinese manufacturing industry SO ENERGY POLICY LA English DT Article DE Industry; Energy efficiency; Energy policies ID INDEX DECOMPOSITION APPROACH; PERSPECTIVE AB The industrial sector consumes about 50% of the world's delivered energy and thus has a large impact on the world's energy production and consumption. Japan is one of the leading countries in industrial efficiency while China is the world's largest industrial energy consumer. This study analyzes the energy consumption and efficiency of the Japanese and Chinese manufacturing industry Analysis shows that the energy intensity of both Japanese and Chinese manufacturing industry has decreased significantly. Decomposition analysis shows that the efficiency effect played an important role in reducing energy intensity; improvement of the energy efficiency of both Japanese and Chinese manufacturing industry showed a trend of exponential decay. Structural effect significantly reduced the energy intensity of the Japanese manufacturing industry while having a relatively small influence on the energy intensity of the Chinese manufacturing industry. Our analysis also shows a strong association of industrial energy efficiency improvement with energy policies, highlighting that energy efficiency policies can play an important role in the reduction of industrial energy intensity. The results of this study also underscore the important, yet very challenging, task of achieving structural change to further improve efficiency. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Zhao, Yue] China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China. [Ke, Jing; Ni, Chun Chun; McNeil, Michael; Khanna, Nina Zheng; Zhou, Nan; Fridley, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Li, Qiqiang] Shandong Univ, Sch Control Sci & Engn, Jinan 250061, Shandong, Peoples R China. RP Ke, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, Environm Energy Technol Div, MS 90R2002,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM Jke@lbl.gov RI Ke, Jing/H-4816-2016 OI Ke, Jing/0000-0002-5972-8042 FU Energy Foundation through the Department of Energy [DE-AC02-05CH11231]; Natural Science Foundation of Shandong Province of China [ZR2010FZ001] FX This work was supported by the Energy Foundation through the Department of Energy under Contract no. DE-AC02-05CH11231, the Key Project of Natural Science Foundation of Shandong Province of China under Grant no. ZR2010FZ001. The authors thank the anonymous reviewers for their valuable comments and suggestions. NR 49 TC 10 Z9 10 U1 3 U2 38 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 EI 1873-6777 J9 ENERG POLICY JI Energy Policy PD JUL PY 2014 VL 70 BP 45 EP 56 DI 10.1016/j.enpol.2014.02.034 PG 12 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA AI2OS UT WOS:000336698500004 ER PT J AU Dagle, RA Lizarazo-Adarme, JA Dagle, VL Gray, MJ White, JF King, DL Palo, DR AF Dagle, Robert A. Lizarazo-Adarme, Jair A. Dagle, Vanessa Lebarbier Gray, Michel J. White, James F. King, David L. Palo, Daniel R. TI Syngas conversion to gasoline-range hydrocarbons over Pd/ZnO/Al2O3 and ZSM-5 composite catalyst system SO FUEL PROCESSING TECHNOLOGY LA English DT Article DE Syngas; Methanol; Methanol-to-hydrocarbons; Methanol-to-gasoline (MTG); Gas-to-liquid; PdZn catalyst ID BIOMASS-DERIVED SYNGAS; ZEOLITE AB A composite Pd/ZnO/Al2O3-HZSM-5 (Si/Al = 40) catalytic system was evaluated for the synthesis of gasoline-range hydrocarbons directly from synthesis gas. A bifunctional catalyst comprising PdZn metal and zeolitic acid sites provides the required catalytically active sites necessary for the methanol synthesis, methanol dehydration, and dimethyl ether-to-gasoline reactions. Using a molar syngas H-2/CO feed ratio of 2, the effects of temperature (310-375 degrees C), pressure (300-1000 psig), and gas hourly space velocity (740-2970h(-1)) were investigated. The liquid hydrocarbon product provided by the Pd/ZnO/Al2O3 + ZSM-5 composite catalyst is aromatic-rich, and contains a significant amount of methylated benzenes. Catalytic stability was favorable due to the presence of hydrogen in the syngas, thus mitigating coke formation within the zeolite. When ZSM-5 is replaced by zeolite-Y (Si/Al = 15), the aromatic content of the hydrocarbon liquid markedly decreased while branched and cyclic hydrocarbons increased. The Pd/Zn/Al2O3 catalyst was found to be highly stable and resistant to sintering under the conditions of the testing, in contrast to the industry standard Cu/ZnO/Al2O3 methanol catalyst. Yield to C-5(+) liquid hydrocarbon product was limited by alternative syngas conversion pathways (water gas shift, methanation) and by hydrogenation of light olefins that would otherwise convert to a liquid hydrocarbon product. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dagle, Robert A.; Dagle, Vanessa Lebarbier; Gray, Michel J.; White, James F.; King, David L.; Palo, Daniel R.] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. [Lizarazo-Adarme, Jair A.; Palo, Daniel R.] Pacific NW Natl Lab, Microprod Breakthrough Inst Corvallis, Corvallis, OR 97330 USA. [White, James F.] 3 Rivers Catalysis LLC, Richland, WA USA. RP Dagle, RA (reprint author), Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. EM robert.dagle@pnnl.gov FU Energy Conversion Initiative at Pacific Northwest National Laboratory; National Advanced Biofuels Consortium - Department of Energy's Office of Biomass Program; U.S. Department of Energy [DEAC05-76RL01830] FX The authors would like to kindly thank the following either current or former colleagues: Yong Wang, Jianli (John) Hu, Ya-Huei (Cathy) Chin, Chunshe (James) Cao, Alex Platon, Jamie Holladay, and Guan-Guang (Gordon) Xia. Their previous efforts on development of the high temperature PdZn-based methanol catalyst were foundational. The authors also acknowledge that initial work on this concept was funded through the Energy Conversion Initiative at Pacific Northwest National Laboratory. The bulk of this work was supported by the National Advanced Biofuels Consortium which is funded by the Department of Energy's Office of Biomass Program with recovery act funds. PNNL work was conducted under U.S. Department of Energy contract DE-AC05-76RL01830. The facilities of the Microproducts Breakthrough Institute in Corvallis, OR were utilized for the mixed catalyst bed experiments. Finally, the authors would like to acknowledge that a portion of this work was done in the Environmental Molecular Sciences Laboratory (EMSL), a DOE sponsored user facility located in Richland, WA at the Pacific Northwest National Laboratory. NR 21 TC 13 Z9 15 U1 17 U2 105 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-3820 EI 1873-7188 J9 FUEL PROCESS TECHNOL JI Fuel Process. Technol. PD JUL PY 2014 VL 123 BP 65 EP 74 DI 10.1016/j.fuproc.2014.01.041 PG 10 WC Chemistry, Applied; Energy & Fuels; Engineering, Chemical SC Chemistry; Energy & Fuels; Engineering GA AH9NM UT WOS:000336469100009 ER PT J AU Katz, DS Zhang, Z AF Katz, Daniel S. Zhang, Zhao TI Special issue on eScience infrastructure and applications SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF ESCIENCE LA English DT Editorial Material DE eScience; eResearch; eInfrastructure; Cyberinfrastructure; CDS&E ID MAPREDUCE; WORKFLOW; ACCESS AB This special issue contains extensions of work presented at the 2012 IEEE International Conference on eScience, held in Chicago, IL in October 2012. For eScience to be successful, simultaneous advances in infrastructure and applications are required, which in turn requires research teams with widely varying expertise, from computer science to Earth sciences and biological sciences, as well as fora for different teams to interact and share knowledge and lessons learned, such as the eScience series of conferences. The papers in this special issue represent advances in both infrastructure and applications and how they can influence each other. (C) 2014 Published by Elsevier B.V. C1 [Katz, Daniel S.] Univ Chicago, Chicago, IL 60637 USA. [Zhang, Zhao] Univ Chicago, Dept Comp Sci, Chicago, IL 60637 USA. [Katz, Daniel S.] Argonne Natl Lab, Chicago, IL USA. RP Katz, DS (reprint author), Univ Chicago, Chicago, IL 60637 USA. EM d.katz@ieee.org; zhaozhang@uchicago.edu NR 18 TC 2 Z9 2 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 36 BP 335 EP 337 DI 10.1016/j.future.2014.03.007 PG 3 WC Computer Science, Theory & Methods SC Computer Science GA AI3OB UT WOS:000336770700029 ER PT J AU Fadika, Z Dede, E Govindaraju, M Ramakrishnan, L AF Fadika, Zacharia Dede, Elif Govindaraju, Madhusudhan Ramakrishnan, Lavanya TI MARIANE: Using MApReduce in HPC environments SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF ESCIENCE LA English DT Article DE Hadoop; MapReduce; Data intensive; Scientific computing AB MapReduce is increasingly becoming a popular programming model. However, the widely used implementation, Apache Hadoop, uses the Hadoop Distributed File System (HDFS), which is currently not directly applicable to a majority of existing HPC environments such as Teragrid and NERSC that support other distributed file systems. On such resourceful High Performance Computing (HPC) infrastructures, the MapReduce model can rarely make use of full resources, as special circumstances must be created for its adoption, or simply limited resources must be isolated to the same end. This paper not only presents a MapReduce implementation directly suitable for such environments, but also exposes the design choices for better performance gains in those settings. By leveraging inherent distributed file systems' functions, and abstracting them away from its MapReduce framework, MARIANE (MApReduce Implementation Adapted for HPC Environments) not only allows for the use of the model in an expanding number of HPC environments, but also shows better performance in such settings. This paper identifies the components and trade-offs necessary for this model, and quantifies the performance gains exhibited by our approach in HPC environments over Apache Hadoop in a data intensive setting at the National Energy Research Scientific Computing Center (NERSC). (C) 2014 Elsevier B.V. All rights reserved. C1 [Fadika, Zacharia; Dede, Elif; Govindaraju, Madhusudhan] SUNY Binghamton, Dept Comp Sci, Grid & Cloud Comp Res Lab, Vestal, NY 13902 USA. [Ramakrishnan, Lavanya] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Govindaraju, M (reprint author), SUNY Binghamton, Dept Comp Sci, Grid & Cloud Comp Res Lab, Vestal, NY 13902 USA. EM zfadika@cs.binghamton.edu; edede1@cs.binghamton.edu; mgovinda@cs.binghamton.edu; lramakrishnan@lbl.gov NR 22 TC 3 Z9 3 U1 0 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 36 BP 379 EP 388 DI 10.1016/j.future.2013.12.007 PG 10 WC Computer Science, Theory & Methods SC Computer Science GA AI3OB UT WOS:000336770700033 ER PT J AU Dede, E Fadika, Z Govindaraju, M Ramakrishnan, L AF Dede, Elif Fadika, Zacharia Govindaraju, Madhusudhan Ramakrishnan, Lavanya TI Benchmarking MapReduce implementations under different application scenarios SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF GRID COMPUTING AND ESCIENCE LA English DT Article DE Distributed Computing; MapReduce; Hadoop; Benchmarking AB The MapReduce paradigm provides a scalable model for large scale data intensive computing and associated fault-tolerance. Data volumes generated and processed by scientific applications are growing rapidly. Several MapReduce implementations, with various degrees of conformance to the key tenets of the model, are available today. Each of these implementations is optimized for specific features. To make the right decisions, HPC application and middleware developers must thus understand the complex dependences between MapReduce features and their application. We present a set of benchmarks for quantifying, comparing, and contrasting the performance of MapReduce implementations under a wide range of representative use cases. To demonstrate the utility of the benchmarks and to provide a snapshot of the current implementation landscape, we report the performance of three different MapReduce implementations, and draw conclusions about their current performance characteristics. The three implementations we chose for evaluation are the widely used Hadoop implementation, Twister, which has been widely discussed in the literature in the context of scientific applications, and LEMO-MR which is our own implementation. We present the performance of these three implementations and draw conclusions about their performance characteristics. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dede, Elif; Fadika, Zacharia; Govindaraju, Madhusudhan] SUNY Binghamton, Dept Comp Sci, Grid & Cloud Comp Res Lab, Vestal, NY 13902 USA. [Ramakrishnan, Lavanya] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Govindaraju, M (reprint author), SUNY Binghamton, Dept Comp Sci, Grid & Cloud Comp Res Lab, Vestal, NY 13902 USA. EM edede1@cs.binghamton.edu; zfadika@cs.binghamton.edu; mgovinda@cs.binghamton.edu; lramakrishnan@lbl.gov FU NSF [0958501]; Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported in part by NSF grant 0958501 and also in part by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 25 TC 4 Z9 4 U1 0 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 36 BP 389 EP 399 DI 10.1016/j.future.2014.01.001 PG 11 WC Computer Science, Theory & Methods SC Computer Science GA AI3OB UT WOS:000336770700034 ER PT J AU Cinquini, L Crichton, D Mattmann, C Harney, J Shipman, G Wang, FY Ananthakrishnan, R Miller, N Denvil, S Morgan, M Pobre, Z Bell, GM Doutriaux, C Drach, R Williams, D Kershaw, P Pascoe, S Gonzalez, E Fiore, S Schweitzer, R AF Cinquini, Luca Crichton, Daniel Mattmann, Chris Harney, John Shipman, Galen Wang, Feiyi Ananthakrishnan, Rachana Miller, Neill Denvil, Sebastian Morgan, Mark Pobre, Zed Bell, Gavin M. Doutriaux, Charles Drach, Robert Williams, Dean Kershaw, Philip Pascoe, Stephen Gonzalez, Estanislao Fiore, Sandro Schweitzer, Roland TI The Earth System Grid Federation: An open infrastructure for access to distributed geospatial data SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF GRID COMPUTING AND ESCIENCE LA English DT Article DE Climate science; Federation; Search; Discovery; Peer-to-peer; CMIP5 AB The Earth System Grid Federation (ESGF) is a multi-agency, international collaboration that aims at developing the software infrastructure needed to facilitate and empower the study of climate change on a global scale. The ESGF's architecture employs a system of geographically distributed peer nodes, which are independently administered yet united by the adoption of common federation protocols and application programming interfaces (APIs). The cornerstones of its interoperability are the peer-to-peer messaging that is continuously exchanged among all nodes in the federation; a shared architecture and API for search and discovery; and a security infrastructure based on industry standards (OpenID, SSL, GSI and SAML). The ESGF software stack integrates custom components (for data publishing, searching, user interface, security and messaging), developed collaboratively by the team, with popular application engines (Tomcat, Solr) available from the open source community. The full ESGF infrastructure has now been adopted by multiple Earth science projects and allows access to petabytes of geophysical data, including the entire Fifth Coupled Model Intercomparison Project (CMIP5) output used by the Intergovernmental Panel on Climate Change (IPCC) Fifth Assessment Report (AR5) and a suite of satellite observations (obs4MIPs) and reanalysis data sets (ANA4MIPs). This paper presents ESGF as a successful example of integration of disparate open source technologies into a cohesive, wide functional system, and describes our experience in building and operating a distributed and federated infrastructure to serve the needs of the global climate science community. (C) 2013 Elsevier B.V. All rights reserved. C1 [Cinquini, Luca; Crichton, Daniel; Mattmann, Chris] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Cinquini, Luca; Crichton, Daniel; Mattmann, Chris] CALTECH, Pasadena, CA 91106 USA. [Harney, John; Wang, Feiyi] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Shipman, Galen] Oak Ridge Natl Lab, Comp & Computat Sci Directorate, Oak Ridge, TN USA. [Ananthakrishnan, Rachana] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Miller, Neill] Univ Chicago, Chicago, IL 60637 USA. [Ananthakrishnan, Rachana; Miller, Neill] Argonne Natl Lab, Argonne, IL 60439 USA. [Denvil, Sebastian] Inst Pierre Simon Laplace, Climate Modeling Grp, Paris, France. [Morgan, Mark] Inst Pierre Simon Laplace, Earth Syst Modeling Platform, Paris, France. [Pobre, Zed] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Bell, Gavin M.; Doutriaux, Charles; Drach, Robert; Williams, Dean] Lawrence Livermore Natl Lab, Livermore, CA USA. [Kershaw, Philip] STEC Rutherford Appleton Lab, RAL Space, Ctr Environm Data Archival, Didcot, Oxon, England. [Pascoe, Stephen] STEC Rutherford Appleton Lab, Didcot, Oxon, England. [Kershaw, Philip; Pascoe, Stephen] NCAS BADC, Didcot, Oxon, England. [Gonzalez, Estanislao] German Climate Comp Ctr DKRZ, Hamburg, Germany. [Fiore, Sandro] Euromediterranean Ctr Climate Change CMCC, Lecce, Italy. [Schweitzer, Roland] NOAA, Pacific Marine Environm Lab, Seattle, WA 98115 USA. RP Cinquini, L (reprint author), CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. EM luca.cinquini@jpl.nasa.gov; daniel.j.crichton@jpl.nasa.gov; chris.a.mattmann@jpl.nasa.gov; harneyjf@ornl.gov; gshipman@ornl.gov; fwang2@ornl.gov; ranantha@mcs.anl.gov; neillm@mcs.anl.gov; sebastien.denvil@ipsl.jussieu.fr; momipsl@ipsl.jussieu.fr; zed.pobre@nasa.gov; gavin@llnl.gov; doutriaux1@llnl.gov; drach1@llnl.gov; williams13@llnl.gov; philip.kershaw@stfc.ac.uk; stephen.pascoe@stfc.ac.uk; estanislao.gonzalez@met.fu-berlin.de; sandro.fiore@unisalento.it; Roland.Schweitzer@noaa.gov OI Kershaw, Philip/0000-0002-7646-291X FU U.S. Department of Energy; National Atmospheric and Space Administration (NASA); European Infrastructure for the European Network for Earth System Modeling (IS-ENES) FX The development and operation of ESGF is supported by the efforts of principal investigators, software engineers, data managers and system administrators from many agencies and institutions worldwide. Primary contributors include ANL, ANU, BADC, CMCC, DKRZ, ESRL, GFDL, GSFC, JPL, IPSL, NCAR, ORNL, LBNL, LLNL (leading institution), PMEL, PNNL and SNL. Major funding provided by the U.S. Department of Energy, the National Atmospheric and Space Administration (NASA), and the European Infrastructure for the European Network for Earth System Modeling (IS-ENES). NR 18 TC 16 Z9 16 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 36 BP 400 EP 417 DI 10.1016/j.future.2013.07.002 PG 18 WC Computer Science, Theory & Methods SC Computer Science GA AI3OB UT WOS:000336770700035 ER PT J AU Hendrix, V Ramakrishnan, L Ryu, Y van Ingen, C Jackson, KR Agarwal, D AF Hendrix, Valerie Ramakrishnan, Lavanya Ryu, Youngryel van Ingen, Catharine Jackson, Keith R. Agarwal, Deborah TI CAMP: Community Access MODIS Pipeline SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF GRID COMPUTING AND ESCIENCE LA English DT Article DE MODIS; Data-intensive; High Performance computing ID LIFE SCIENCES AB The Moderate Resolution Imaging Spectroradiometer (MODIS) instrument's land and atmosphere data are important to many scientific analyses that study processes at both local and global scales. The Terra and Aqua MODIS satellites acquire data of the entire Earth's surface every one or two days in 36 spectral bands. MODIS data provide information to complement many of the ground-based observations but are extremely critical when studying global phenomena such as gross photosynthesis and evapotranspiration. However, data procurement and processing can be challenging and cumbersome due to difficulties in volume, size of data and scale of analyses. For example, the very first step in MODIS data processing is to ensure that all products are in the same resolution and coordinate system. The reprojection step involves a complex inverse gridding algorithm and involves downloading tens of thousands of files for a single year that is often infeasible to perform on a scientist's desktop. Thus, use of large-scale resource environments such as high performance computing (HPC) environments are becoming crucial for processing of MODIS data. However, HPC environments have traditionally been used for tightly coupled applications and present several challenges for managing data-intensive pipelines. We have developed a data-processing pipeline that downloads the MODIS swath products and reprojects the data to a sinusoidal system on an HPC system. The 10 year archive of the reprojected data generated using the pipeline is made available through a web portal. In this paper, we detail a system architecture (CAMP) to manage the lifecycle of MODIS data that includes procurement, storage, processing and dissemination. Our system architecture was developed in the context of the MODIS reprojection pipeline but is extensible to other analyses of MODIS data. Additionally, our work provides a framework and valuable experiences for future developments and deployments of data-intensive pipelines from other scientific domains on HPC systems. (C) 2014 Published by Elsevier B.V. C1 [Hendrix, Valerie; Ramakrishnan, Lavanya; Jackson, Keith R.; Agarwal, Deborah] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ryu, Youngryel] Seoul Natl Univ, Dept Landscape Architecture & Rural Syst Engn, Seoul 151, South Korea. [van Ingen, Catharine] Microsoft Res, Redmond, WA USA. RP Hendrix, V (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM vchendrix@lbl.gov; lramakrishnan@lbl.gov; yryu@snu.ac.kr; vaningen@microsoft.com; KRJackson@lbl.gov; daagarwal@lbl.gov RI Ryu, Youngryel/C-3072-2008 OI Ryu, Youngryel/0000-0001-6238-2479 FU Office of Science, Office of Advanced Scientific Computing, of the US Department of Energy [DEAC02-05CH11231]; Microsoft Research; Office of Science of the US Department of Energy [DEAC02-05CH11231] FX This work is supported in part by the Director, Office of Science, Office of Advanced Scientific Computing, of the US Department of Energy under Contract No. DEAC02-05CH11231 and Microsoft Research. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DEAC02-05CH11231. The authors would also like to thank Jie Li, and Christine Morin. NR 27 TC 3 Z9 3 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD JUL PY 2014 VL 36 BP 418 EP 429 DI 10.1016/j.future.2013.09.023 PG 12 WC Computer Science, Theory & Methods SC Computer Science GA AI3OB UT WOS:000336770700036 ER PT J AU Pandey, SN Chaudhuri, A Kelkar, S Sandeep, VR Rajaram, H AF Pandey, S. N. Chaudhuri, A. Kelkar, S. Sandeep, V. R. Rajaram, H. TI Investigation of permeability alteration of fractured limestone reservoir due to geothermal heat extraction using three-dimensional thermo-hydro-chemical (THC) model SO GEOTHERMICS LA English DT Article DE Geothermal reservoir; Renewable energy; Thermo-hydro-chemical model; Aperture alteration; Calcite; Dissolution/precipitation; Reactive transport ID GEOLOGICALLY RELEVANT SITUATIONS; COLD-WATER INJECTION; SOULTZ-SOUS-FORETS; CALCITE DISSOLUTION; CO2-WATER SYSTEMS; KARST AREAS; FLUID-FLOW; PRECIPITATION; KINETICS; ROCK AB Heat extraction by cold water circulation disturbs the thermo-chemical equilibrium of a geothermal reservoir, activating the dissolution/precipitation of minerals in the fractures. Calcite being a more reactive mineral than other rock minerals composing the earth curst, we investigate the permeability alteration during geothermal heat production from carbonate reservoirs. In this study the simulations are performed using the code FEHM with coupled thermo-hydro-chemical (THC) capabilities for a three dimensional domain. The computational domain consists of a single fracture connecting the injection and production wells. For reactive alteration of aperture, the model considers that the kinetics of dissolution/precipitation is coupled to the equilibrium interactions among the aqueous species/ions. The reaction rate predominantly depends on the temperature dependent solubility and advective-dispersive solute transport in the fracture. Due to the nonuniform flow fields resulting from injection and production, the coupled thermo-hydro-chemical processes initiate significant variation of the aperture alteration rate over the fracture. We have considered different operating conditions such as different mass injection rate, injection temperature and concentration of minerals. Our simulations show that dissolution and precipitation can occur simultaneously at different locations in fracture. Furthermore the reaction rate varies with time and the reaction rate can also switch between dissolution and precipitation. To illustrate this interesting behavior, the variations of shape and size of zero reaction rate contours with time are shown. An interesting outcome is a non-monotonic evolution of the overall transmissivity between the wells. The alteration of overall transmissivity largely depends on the concentration of mineral in the injected water. with respect to the solubility at the initial fracture temperature. For both dissolution and precipitation controlled cases, the rapid changes in transmissivity provide challenges for maintaining circulation of water at constant mass flow rate. (c) 2013 Elsevier Ltd. All rights reserved. C1 [Pandey, S. N.; Chaudhuri, A.; Sandeep, V. R.] Indian Inst Technol, Dept Appl Mech, Madras 600036, Tamil Nadu, India. [Kelkar, S.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Rajaram, H.] Univ Colorado, Dept Civil Environm & Architectural Engn, Boulder, CO 80309 USA. RP Chaudhuri, A (reprint author), Indian Inst Technol, Dept Appl Mech, Madras 600036, Tamil Nadu, India. EM abhijit.chaudhuri@iitm.ac.in NR 53 TC 13 Z9 13 U1 1 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 46 EP 62 DI 10.1016/j.geothermics.2013.11.004 PG 17 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700005 ER PT J AU Spycher, N Peiffer, L Sonnenthal, EL Saldi, G Reed, MH Kennedy, BM AF Spycher, N. Peiffer, L. Sonnenthal, E. L. Saldi, G. Reed, M. H. Kennedy, B. M. TI Integrated multicomponent solute geothermometry SO GEOTHERMICS LA English DT Article DE Geothermometer; Optimization; Exploration; Numerical modeling; Mixing; Geothermal ID MOLAL THERMODYNAMIC PROPERTIES; MINERAL EQUILIBRIA; WATERS; CHEMISTRY; ICELAND; TEMPERATURES; SIMULATION; PROGRAM; SPRINGS; GASES AB The previously developed and well-demonstrated mineral saturation geothermometry method is revisited with the objective to ease its application, and to improve the prediction of geothermal reservoir temperatures using full and integrated chemical analyses of geothermal fluids. Reservoir temperatures are estimated by assessing numerically the clustering of mineral saturation indices computed as a function of temperature. The reconstruction of the deep geothermal fluid compositions, and geothermometry computations, are implemented into one stand-alone program, allowing unknown or poorly constrained input parameters to be estimated by numerical optimization using existing parameter estimation software. The geothermometry system is tested with geothermal waters from previous studies, and with fluids at various degrees of fluid rock chemical equilibrium obtained from laboratory experiments and reactive transport simulations. Such an integrated geothermometry approach presents advantages over classical geothermometers for fluids that have not fully equilibrated with reservoir minerals and/or that have been subject to processes such as dilution and gas loss. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Spycher, N.; Peiffer, L.; Sonnenthal, E. L.; Saldi, G.; Kennedy, B. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Reed, M. H.] Univ Oregon, Dept Geol Sci, Eugene, OR 97403 USA. RP Spycher, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM nspycher@lbl.gov RI Sonnenthal, Eric/A-4336-2009; Spycher, Nicolas/E-6899-2010; OI Peiffer, Loic/0000-0002-2036-8449 FU U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office [DE-EE0002765] FX This work was supported by the U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office, Award No. DE-EE0002765. We thank Patrick Dobson and Jennifer Lewicki for their valuable inputs after testing GeoT, Kevin Knauss for his leadership with the experimental component of this study, Joe Iovenitti (Alta Rock) for providing data on the Newberry project, and Christoph Wanner for compiling and testing GeoT on various platforms. We are also grateful to Stuart F. Simmons and William C. Evans for their constructive reviews which helped improve the original manuscript. NR 40 TC 12 Z9 12 U1 5 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 113 EP 123 DI 10.1016/j.geothermics.2013.10.012 PG 11 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700010 ER PT J AU Wanner, C Peiffe, L Sonnenthal, E Spycher, N Iovenitti, J Kennedy, BM AF Wanner, Christoph Peiffe, Loic Sonnenthal, Eric Spycher, Nicolas Iovenitti, Joe Kennedy, Burton Mack TI Reactive transport modeling of the Dixie Valley geothermal area: Insights on flow and geothermometry SO GEOTHERMICS LA English DT Article DE Reactive transport modeling; Solute geothermometry; Dixie Valley; Fracture flow; Geothermal springs ID HYDROTHERMAL SYSTEM; YUCCA MOUNTAIN; FLUID-FLOW; SIMULATION; WATERS; EQUILIBRIA; FRACTURE; NEVADA; FORM AB A 2D reactive transport model of the Dixie Valley geothermal area in Nevada, USA was developed to assess fluid flow pathways and fluid rock interaction processes. The model includes two major normal faults and the incorporation of a dual continuum domain to simulate the presence of a small-scale thermal spring being fed by a highly permeable but narrow fracture zone. Simulations were performed incorporating fluid flow, heat conduction and advection, and kinetic mineral-water reactions. Various solute geothermometry methods were applied to simulated spring compositions, to compare estimated reservoir temperatures with "true" modeled reservoir temperatures, for a fluid ascending the simulated fracture and cooling on its way to the surface. Under the modeled conditions (cooling but no mixing or boiling), the classical Na-K(-Ca) geothermometers performed best because these are least affected by mineral precipitation upon cooling. Geothermometry based on computed mineral saturation indices and the quartz geothermometer were more sensitive to re-equilibration upon cooling, but showed good results for fluid velocities above ca. 0.1 m/d and a reactive fracture surface area 1-2 orders of magnitude lower than the corresponding geometric surface area. This suggests that such upflow rates and relatively low reactive fracture surface areas are likely present in many geothermal fields. The simulations also suggest that the presence of small-scale fracture systems having an elevated permeability of 10-12 to 10(-10) m(2) can significantly alter the shallow fluid flow regime of geothermal systems. For the Dixie Valley case, the model implies that such elevated permeabilities lead to a shallow (less than 1 km) convection cell where superficial water infiltrates along the range front normal fault and connects the small-scale geothermal spring through basin filling sediments. Furthermore, we conclude that a fracture permeability on the order of 10(-12) m(2) may lead to near surface temperature >100 degrees C whereas a permeability of 10-10 m2 is not realistic because this permeability led to extreme upflow velocities and to a short-circuit of the regional fault zone. (c) 2013 Elsevier Ltd. All rights reserved. C1 [Wanner, Christoph; Peiffe, Loic; Sonnenthal, Eric; Spycher, Nicolas; Kennedy, Burton Mack] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Iovenitti, Joe] AltaRockEnergy Inc, Sausalito, CA USA. RP Wanner, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM cwanner@lbl.gov RI Sonnenthal, Eric/A-4336-2009; Spycher, Nicolas/E-6899-2010; OI Wanner, Christoph/0000-0003-3488-8602; Peiffer, Loic/0000-0002-2036-8449 FU U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office [DE-EE0002765, DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office, Award Nos. DE-EE0002765 and DE-AC02-05CH11231. We thank one anonymous reviewer for a thorough review and constructive comments. NR 42 TC 6 Z9 6 U1 1 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 130 EP 141 DI 10.1016/j.geothermics.2013.12.003 PG 12 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700012 ER PT J AU Peiffer, L Wanner, C Spycher, N Sonnenthal, EL Kennedy, BM Iovenitti, J AF Peiffer, L. Wanner, C. Spycher, N. Sonnenthal, E. L. Kennedy, B. M. Iovenitti, J. TI Optimized multicomponent vs. classical geothermometry: Insights from modeling studies at the Dixie Valley geothermal area SO GEOTHERMICS LA English DT Article DE Geothermometer; Optimization; Exploration; Numerical modeling; Mixing; Geothermal ID NEVADA; WATERS; EQUILIBRIA; SIMULATION; BASIN AB A new geothermometry approach is explored, incorporating multicomponent geothermometry coupled with numerical optimization to provide more confident estimates of geothermal reservoir temperatures when results of classical geothermometers are inconsistent. This approach is applied to geothermal well and spring waters from the Dixie Valley geothermal area (Nevada), to evaluate the influence of salt brines mixing and dilution of geothermal fluids on calculated temperatures. The main advantage of the optimized multicomponent method over classical geothermometers is its ability to quantify the extent of dilution and gas loss experienced by a geothermal fluid, and to optimize other poorly constrained or unknown parameters (such as Al and Mg concentrations), allowing the reconstruction of the deep reservoir fluid composition and therefore gaining confidence in reservoir temperatures estimations. Because the chemical evolution of deep geothermal fluids is a combination of multiple time-dependent processes that take place when these fluids ascend to the surface, reactive transport modeling is used to assess constraints on the application of solute geothermometers. Simulation results reveal that Al and Mg concentrations of ascending fluids are sensitive to mineral precipitation-dissolution affecting reservoir temperatures inferred with multicomponent geothermometry. In contrast, simulations show that the concentrations of major elements such as Na, K, and SiO2 are less sensitive to re-equilibration. Geothermometers based on these elements give reasonable reservoir temperatures in many cases, except when dilution or mixing with saline waters has taken place. Optimized multicomponent geothermometry yields more representative temperatures for such cases. Taking into account differences in estimated temperatures, and chemical compositions of the Dixie Valley thermal waters, a conceptual model of two main geothermal reservoirs is proposed. The first reservoir is located along the Stillwater range normal fault system and has an estimated temperature of 240-260 degrees C. It covers the area corresponding to the geothermal field but could extend towards the south-west where deep temperatures of 200-225 degrees C are estimated. The second reservoir has an estimated temperature of 175-190 degrees C and extends from well 62-21 to northeastern Hyder, Lower Ranch, Fault Line, and Jersey springs. (c) 2014 Elsevier Ltd. All rights reserved. C1 [Peiffer, L.; Wanner, C.; Spycher, N.; Sonnenthal, E. L.; Kennedy, B. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Iovenitti, J.] AltaRockEnergy Inc, Sausalito, CA 94965 USA. RP Peiffer, L (reprint author), Univ Nacl Autonoma Mexico, Inst Energias Renovables, Temixco 62580, Morelos, Mexico. EM loic.peiffer@gmail.com; nspycher@lbl.gov RI Sonnenthal, Eric/A-4336-2009; Spycher, Nicolas/E-6899-2010; OI Wanner, Christoph/0000-0003-3488-8602; Peiffer, Loic/0000-0002-2036-8449 FU U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office [DE-EE0002765] FX This work was supported by the U.S. Department of Energy, Geothermal Technologies Program, Energy Efficiency and Renewable Energy Office, Award no. DE-EE0002765. We thank Susan Lutz for providing XRD analyses, and Dick Benoit and Lisa Shevenell for personal communications regarding Dixie Valley. We are also grateful to Patrick Dobson for a constructive review of the original manuscript. Reviews by S. Simmons and an anonymous reviewer are also greatly appreciated. NR 42 TC 6 Z9 7 U1 1 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 154 EP 169 DI 10.1016/j.geothermics.2013.12.002 PG 16 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700014 ER PT J AU Jeanne, P Rutqvist, J Vasco, D Garcia, J Dobson, PF Walters, M Hartline, C Borgia, A AF Jeanne, Pierre Rutqvist, Jonny Vasco, Donald Garcia, Julio Dobson, Patrick F. Walters, Mark Hartline, Craig Borgia, Andrea TI A 3D hydrogeological and geomechanical model of an Enhanced Geothermal System at The Geysers, California SO GEOTHERMICS LA English DT Article DE Enhanced Geothermal Systems; The Geysers; Induced seismicity; TerraSAR-X satellites; Shear zones; Thermo-hydromechanical simulation ID FIELD; DEFORMATION; ROCK AB In this study, integrated coupled process modeling and field observations are used to build a threedimensional hydrogeological and geomechanical model of an Enhanced Geothermal System (EGS) in the northwestern part of The Geysers geothermal field, California. We constructed a model and characterized hydraulic and mechanical properties of relevant geological layers and a system of multiple intersecting shear zones. This characterization was conducted through detailed coupled process modeling of a oneyear injection stimulation with simultaneous field monitoring of reservoir pressure, microseismicity, and surface deformations. The analysis of surface deformations was found to be particularly challenging as the subtle surface deformations caused by the injection taking place below 3 km depth are intermingled with deformations caused by both tectonic effects and seasonal surface effects associated with rainfall. However, through a detailed analysis of the field data we identified deformations associated with injection. Hydraulic and mechanical properties of relevant rock layers and shear zones were determined using a 3D hydrogeological and geomechanical model. Hydraulic properties were determined using inverse analysis by fitting the pressure evolution in monitoring wells surrounding the injection well. Mechanical properties were estimated by comparison of the predicted microseismicity potential with the observed microseismicity and by fitting the predicted vertical displacement with the surface deformations measured by satellite. The results show the critical importance of considering the regional fault system, especially reservoir-level faults and shear zones that modify injection water flow and steam pressure diffusion. In the vicinity of the EGS Demonstration Project, fluid flow pathways and pressure diffusion fronts appears to be at a maximum along N130 oriented shear zones and at a minimum along N50 oriented shear zones. Evidence for this comes from microseismic event hypocenters which extend several kilometers horizontally from the injection well and deep into a recent granitic intrusion that underlies the high temperature reservoir. Published by Elsevier Ltd. C1 [Jeanne, Pierre; Rutqvist, Jonny; Vasco, Donald; Dobson, Patrick F.; Borgia, Andrea] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Garcia, Julio; Walters, Mark; Hartline, Craig] Calpine Corp, Middletown, CA 95461 USA. RP Jeanne, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM pjeanne@lbl.gov RI Dobson, Patrick/D-8771-2015; Rutqvist, Jonny/F-4957-2015; Jeanne, Pierre/I-2996-2015; Vasco, Donald/I-3167-2016; Vasco, Donald/G-3696-2015 OI Dobson, Patrick/0000-0001-5031-8592; Rutqvist, Jonny/0000-0002-7949-9785; Jeanne, Pierre/0000-0003-1487-8378; Vasco, Donald/0000-0003-1210-8628; Vasco, Donald/0000-0003-1210-8628 FU Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department under the U.S. Department of Energy [DE-AC02-05CH11231]; Calpine Corporation FX This work was conducted with funding provided by the Assistant Secretary for Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department under the U.S. Department of Energy Contract No. DE-AC02-05CH11231, and by Calpine Corporation. We are grateful to Katie Boyle and Lawrence Hutchings from the Lawrence Berkeley National Laboratory (LBNL) for making their seismic data available to us. NR 24 TC 13 Z9 14 U1 0 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 240 EP 252 DI 10.1016/j.geothermics.2014.01.013 PG 13 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700020 ER PT J AU Jeanne, P Rutqvist, J Hartline, C Garcia, J Dobson, PF Walters, M AF Jeanne, Pierre Rutqvist, Jonny Hartline, Craig Garcia, Julio Dobson, Patrick F. Walters, Mark TI Reservoir structure and properties from geomechanical modeling and microseismicity analyses associated with an enhanced geothermal system at The Geysers, California SO GEOTHERMICS LA English DT Article DE Enhanced geothermal system; Micro-earthquake analysis; Fault zone network; Inverse fluid flow modeling; Thermo-hydromechanical simulation; Micro-earthquake predicted ID FLUID-FLOW; FIELD; ROCK; AREA; SEISMICITY AB This work contributes to modeling studies associated with an enhanced geothermal system demonstration project in the northwestern region of The Geysers, California. We first attempt to determine the structural configuration and reservoir properties of the steam-bearing reservoir, based on microseismicity recorded during a one-year water injection operation. This is particularly challenging because errors in hypocenter determination (due primarily to errors in the velocity model and first-arrival picks) tend to "defocus" any microseismic events related to a distributed network of fractures, resulting in a "cloud" of microseismic events. This work includes a dynamic analysis of the observed alignments in daily microseismicity hypocenters during water injection, along with the constraints provided by geological data (surface mapping and drill cuttings) to determine the location and orientation of shear zones. We then evaluate the viability of the resulting network of proposed shear zones, using a 2D fluid flow and geomechanical model simulation of the injection and comparing it to the evolution of observed (1) pressure in nearby monitoring wells and (2) microseismicity hypocenters. The shear-zone hydraulic properties were estimated using inverse analysis of the pressure evolution in the surrounding wells, while mechanical properties were estimated by comparing the calculated stress changes and associated microseismic potential with the observed microseismicity. The results indicate that a model including the network of proposed shear zones does calculate reservoir hydraulic and mechanical responses similar to those observed during water injection. Finally, the results confirm previous studies at The Geysers indicating that the injection-induced microseismicity is caused by thermal contraction near the injection wells where strong cooling prevails, whereas away from the injection wells, small increases in steam pressure are the primary trigger of microseismicity. Published by Elsevier Ltd. C1 [Jeanne, Pierre; Rutqvist, Jonny; Dobson, Patrick F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Hartline, Craig; Garcia, Julio; Walters, Mark] Calpine Corp, Middletown, CA 95461 USA. RP Jeanne, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM pjeanne@lbl.gov RI Dobson, Patrick/D-8771-2015; Rutqvist, Jonny/F-4957-2015; Jeanne, Pierre/I-2996-2015; OI Dobson, Patrick/0000-0001-5031-8592; Rutqvist, Jonny/0000-0002-7949-9785; Jeanne, Pierre/0000-0003-1487-8378; Walters, Mark/0000-0001-8458-4813 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department under the U.S. Department of Energy [DE-AC02-05CH11231]; Calpine Corporation FX This work was conducted with funding by the Assistant Secretary for Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department under the U.S. Department of Energy Contract No. DE-AC02-05CH11231, and by Calpine Corporation. We are grateful to Katie Boyle and Lawrence Hutchings from Lawrence Berkeley National Laboratory (LBNL) for making seismic data available to us, and for the constructive comments and recommendations of the reviewers. NR 33 TC 11 Z9 11 U1 0 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD JUL PY 2014 VL 51 BP 460 EP 469 DI 10.1016/j.geothermics.2014.02.003 PG 10 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA AI3RD UT WOS:000336778700039 ER PT J AU Solbrig, CW Pope, CL Andrus, JP AF Solbrig, Charles W. Pope, Chad L. Andrus, Jason P. TI Stress and diffusion in stored Pu ZPPR fuel from alpha generation SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Article DE Metal fuel failure in long term storage; Metal fuel swelling stress; Gas diffusion in metal; High Pu content nuclear fuel ID HELIUM AB ZPPR (Zero Power Physics Reactor) is a research reactor that has been used to investigate breeder reactor fuel designs. The reactor has been dismantled but its fuel is still stored there. Of concern are its plutonium containing metal fuel elements which are enclosed in stainless steel cladding with gas space filled with helium-argon gas and welded air tight. The fuel elements which are 5.08 cm by 0.508 cm up to 20.32 cm long (2 in x 0.2 in x 8 in) were manufactured in 1968. A few of these fuel elements have failed releasing contamination raising concern about the general state of the large number of other fuel elements. Inspection of the large number of fuel elements could lead to contamination release so analytical studies have been conducted to estimate the probability of failed fuel elements. This paper investigates the possible fuel failures due to generation of helium in the metal fuel from the decay of Pu and its possible damage to the fuel cladding from metal fuel expansion or from diffusion of helium into the fuel gas space. This paper (1) calculates the initial gas loading in a fuel element and its internal free volume after it has been brought into the atmosphere at ZPPR, (2) shows that the amount of helium generated by decay of Pu over 46 years since manufacture is significantly greater than this initial loading, (3) determines the amount of fuel swelling if the helium stays fixed in the fuel plate and estimates the amount of helium which diffuses out of the fuel plate into the fuel plenum assuming the helium does not remain fixed in the fuel plate but can diffuse to the plenum and possibly through the cladding. Since the literature is not clear as to which possibility occurs, as with Schroedinger's cat, both possibilities are analyzed. The paper concludes that (1) if the gas generated is fixed in the fuel, then the fuel swelling it can cause would not cause any fuel failure and (2) if the helium does diffuse out of the fuel (in accordance diffusivities estimated from the literature), then it is unlikely that fuel element bulging will occur. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Solbrig, Charles W.; Pope, Chad L.; Andrus, Jason P.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Solbrig, CW (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM charles.solbrig@inl.gov FU U.S. Department of Energy, Office of Nuclear Energy, under DOE Idaho Operations Office [DE-AC07-05ID14517] FX This work is supported by the U.S. Department of Energy, Office of Nuclear Energy, under DOE Idaho Operations Office Contract DE-AC07-05ID14517. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 13 TC 0 Z9 0 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD JUL PY 2014 VL 74 BP 251 EP 262 DI 10.1016/j.ijheatmasstransfer.2014.03.006 PG 12 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA AI2NV UT WOS:000336696100024 ER PT J AU Aguirre, BA Zubia, D Ordonez, R Anwar, F Prieto, H Sanchez, CA Salazar, MT Pimentel, AA Michael, JR Zhou, XW Mcclure, JC Nielson, GN Cruz-Campa, JL AF Aguirre, Brandon A. Zubia, David Ordonez, Rafael Anwar, Farhana Prieto, Heber Sanchez, Carlos A. Salazar, Maria T. Pimentel, Alejandro. A. Michael, Joseph R. Zhou, Xiaowang Mcclure, John C. Nielson, Gregory N. Cruz-Campa, Jose L. TI Selective Growth of CdTe on Nano-patterned CdS via Close-Space Sublimation SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE CdTe; solar cells; close space sublimation; nanoheteroepitaxy; selective growth ID VAPOR-PHASE EPITAXY; SOLAR-CELLS AB Selective-area deposition of CdTe on CdS via close-space sublimation is used to study the effect of window size (2 mu m and 300 nm) on grain growth. The basic fabrication procedures for each of the layers (CdS, SiO2, and CdTe) and for achieving selective-area growth are presented. Selective-area growth of both micro- and nano-scale CdTe islands on CdS substrates using close-spaced sublimation is demonstrated. Scanning electron microscopy and electron backscatter diffraction microstructure analysis show that the micro-scale CdTe islands remain polycrystalline. However, when the island size is reduced to 300 nm, single crystal CdTe can be achieved within the windows. The CdTe grains were most often in the (101) orientation for both the micro- and nano-sized CdTe islands. C1 [Aguirre, Brandon A.; Zubia, David; Ordonez, Rafael; Anwar, Farhana; Prieto, Heber; Sanchez, Carlos A.; Mcclure, John C.] Univ Texas El Paso, El Paso, TX 79968 USA. [Salazar, Maria T.] Sandia Natl Labs, MESAFAB Operat, Albuquerque, NM 87185 USA. [Pimentel, Alejandro. A.; Michael, Joseph R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Zhou, Xiaowang] Sandia Natl Labs, Livermore, CA USA. [Aguirre, Brandon A.; Nielson, Gregory N.; Cruz-Campa, Jose L.] Sandia Natl Labs, MEMS Technol, Albuquerque, NM 87185 USA. RP Aguirre, BA (reprint author), Univ Texas El Paso, El Paso, TX 79968 USA. EM baaguirre@miners.utep.edu FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Science Foundation [ECS-0335765]; National Institute of Nano Engineering (NINE); Solar Economy Integrative Graduate Education Research Traineeship (SEIGERT), NSF [DGE-0903670]; Solar Economy Integrative Graduate Education Research Traineeship (SEIGERT), DOE [DE-EE0005958] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U. S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was performed in part at the Microelectronics Research Center at UT Austin, a member of the National Nanotechnology Infrastructure Network, which is supported by the National Science Foundation under award no. ECS-0335765. This work is sponsored by the National Institute of Nano Engineering (NINE) and the Solar Economy Integrative Graduate Education Research Traineeship (SEIGERT), NSF award DGE-0903670, and DOE award DE-EE0005958. NR 21 TC 7 Z9 7 U1 1 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD JUL PY 2014 VL 43 IS 7 BP 2651 EP 2657 DI 10.1007/s11664-014-3104-7 PG 7 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA AI3WT UT WOS:000336796700024 ER PT J AU Reina, C Conti, S AF Reina, C. Conti, S. TI Kinematic description of crystal plasticity in the finite kinematic framework: A micromechanical understanding of F=(FFP)-F-e SO JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS LA English DT Article DE Crystal plasticity; Finite kinematics; Dislocation density tensor ID SINGLE-CRYSTALS; STRUCTURED DEFORMATIONS; CONTINUUM THEORY; DISLOCATIONS; ENERGY; ELASTOPLASTICITY; INCOMPATIBILITY; DECOMPOSITION; ENERGETICS; MECHANICS AB The plastic component of the deformation gradient plays a central role in finite kinematic models of plasticity. However, its characterization has been the source of extended debates in the literature and many important issues still remain unresolved. Some examples are the micromechanical understanding of F = (FFp)-F-e with multiple active slip systems, the uniqueness of the decomposition, or the characterization of the plastic deformation without reference to the so-called intermediate configuration. In this paper, we shed some light to these issues via a two-dimensional kinematic analysis of the plastic deformation induced by discrete slip surfaces and the corresponding dislocation structures. In particular, we supply definitions for the elastic and plastic components of the deformation gradient as a function of the active slip systems without any a priori assumption on the decomposition of the total deformation gradient. These definitions are explicitly and uniquely given from the microstructure and do not make use of any unrealizable intermediate configuration. The analysis starts from a semi-continuous mathematical description of the deformation at the microscale, where the displacements are considered continuous everywhere in the domain except at the discrete slip surfaces, over which there is a displacement jump. At this scale, where the microstructure is resolved, the deformation is uniquely characterized from purely kinematic considerations and the elastic and plastic components of the deformation gradient can be defined based on physical arguments. These quantities are then passed to the continuous limit via homogenization, i.e. by increasing the number of slip surfaces to infinity and reducing the lattice parameter to zero. This continuum limit is computed for several illustrative examples, where the well-known multiplicative decomposition of the total deformation gradient is recovered. Additionally, by similar arguments, an expression of the dislocation density tensor is obtained as the limit of discrete dislocation densities which are well characterized within the semi-continuous model. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Reina, C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Reina, C.; Conti, S.] Univ Bonn, Inst Angew Math, D-53115 Bonn, Germany. [Reina, C.] Univ Penn, Philadelphia, PA 19104 USA. RP Reina, C (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM creina@seas.upenn.edu RI Conti, Sergio/B-3214-2009 OI Conti, Sergio/0000-0001-7987-9174 FU Hausdorff Center for Mathematics; Deutsche Forschungsgemeinschaft [Forschergruppe 797, CO 304/4-2]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors acknowledge support from the Hausdorff Center for Mathematics and the Deutsche Forschungsgemeinschaft through Forschergruppe 797, project CO 304/4-2. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 41 TC 16 Z9 16 U1 2 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-5096 EI 1873-4782 J9 J MECH PHYS SOLIDS JI J. Mech. Phys. Solids PD JUL PY 2014 VL 67 BP 40 EP 61 DI 10.1016/j.jmps.2014.01.014 PG 22 WC Materials Science, Multidisciplinary; Mechanics; Physics, Condensed Matter SC Materials Science; Mechanics; Physics GA AI2PE UT WOS:000336699700005 ER PT J AU Hopkins, JB Vericella, JJ Harvey, CD AF Hopkins, Jonathan B. Vericella, John J. Harvey, Christopher D. TI Modeling and generating parallel flexure elements SO PRECISION ENGINEERING-JOURNAL OF THE INTERNATIONAL SOCIETIES FOR PRECISION ENGINEERING AND NANOTECHNOLOGY LA English DT Article DE Flexure elements; Compliant members; Flexible joints; Elements of constraint; Flexure systems; Screw theory; Freedom and Constraint Topologies; FACT ID DEGREE-OF-FREEDOM; THERMAL-EXPANSION; SYSTEM CONCEPTS AB This work introduces the principles necessary to model and generate parallel flexure elements (i.e., compliant members or flexible joints) that may be used to synthesize next-generation precision flexure systems. These principles are extensions of the Freedom and Constraint Topologies (FACT) synthesis approach, which utilizes geometric shapes to help designers synthesize flexure systems that achieve desired degrees of freedom (DOFs). Prior to this paper, FACT was limited to the design of flexure systems that consisted primarily of simple wire or blade flexure elements only. In this paper, the principles are introduced that enable designers to use the same shapes of FACT to synthesize parallel flexure elements of any geometry, including new and often irregularly-shaped elements (e.g., hyperboloids or hyperbolic paraboloids). The ability to recognize such elements within the shapes of FACT, therefore, enables designers to consider a larger body of solution options that satisfy a broader range of kinematic, elastomechanical, and dynamic design requirements. Example flexure systems that consist of flexure elements, generated using this theory, are provided as case studies. (c) 2014 Elsevier Inc. All rights reserved. C1 [Hopkins, Jonathan B.; Vericella, John J.; Harvey, Christopher D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Hopkins, JB (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM jonathanbhopkins@gmail.com FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-614192]; DARPA's Materials; Controlled Microstructural Architecture program in the Defense Sciences Office, Program Manager Judah Goldwasser FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-614192. Support from DARPA's Materials with Controlled Microstructural Architecture program in the Defense Sciences Office, Program Manager Judah Goldwasser, is gratefully acknowledged. NR 32 TC 3 Z9 3 U1 0 U2 10 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0141-6359 EI 1873-2372 J9 PRECIS ENG JI Precis. Eng.-J. Int. Soc. Precis. Eng. Nanotechnol. PD JUL PY 2014 VL 38 IS 3 BP 525 EP 537 DI 10.1016/j.precisioneng.2014.02.001 PG 13 WC Engineering, Multidisciplinary; Engineering, Manufacturing; Nanoscience & Nanotechnology; Instruments & Instrumentation SC Engineering; Science & Technology - Other Topics; Instruments & Instrumentation GA AI3OC UT WOS:000336770800009 ER PT J AU Barnette, AL Ohlhausen, JA Dugger, MT Kim, SH AF Barnette, Anna L. Ohlhausen, J. Anthony Dugger, Michael T. Kim, Seong H. TI Humidity Effects on In Situ Vapor Phase Lubrication with n-Pentanol SO TRIBOLOGY LETTERS LA English DT Article DE Nanotribology; Boundary lubrication chemistry; FTIR; Vapor phase lubrication ID SILICON-OXIDE; ADSORPTION-ISOTHERM; MICROELECTROMECHANICAL SYSTEMS; AMBIENT CONDITIONS; CAPILLARY FORCE; SURFACE; WATER; ADHESION; LIQUID; FRICTION AB The effect of water vapor on n-pentanol vapor phase lubrication (VPL) was studied with a microelectromechanical system (MEMS) side-wall tribometer, a pin-on-disc tribometer, and attenuated total reflection infrared (ATR-IR) spectroscopy. The n-pentanol vapor pressure was fixed at 50 % relative to its saturation vapor pressure (P (sat) = similar to 2.2 Torr at room temperature), which is sufficient to maintain a monolayer of n-pentanol on a SiO2 surface in a dry Ar environment. As the relative humidity (RH) was increased from zero to 30 %, ATR-IR measurements showed that the water adsorption on the surface increases and the adsorbed pentanol thickness decreases by 60 %. These changes in the adsorption isotherm were manifested as higher, and more scattered friction coefficients observed during the MEMS tribometer operation. The maximum RH tolerance appeared to be 25-30 % RH above which the MEMS tribometer failed to operate reliably. In contrast, the n-pentanol VPL efficiency was not affected significantly during the macro-scale pin-on-disc tribometer tests. These results imply that the friction behavior of the asperity contacts in MEMS is more susceptible to co-adsorption of water than the friction behavior of macro-scale contacts. C1 [Barnette, Anna L.; Kim, Seong H.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Barnette, Anna L.; Kim, Seong H.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Ohlhausen, J. Anthony; Dugger, Michael T.] Sandia Natl Labs, Mat Sci & Engn Ctr, Albuquerque, NM 87185 USA. RP Kim, SH (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM mtdugge@sandia.gov; shk10@psu.edu FU National Science Foundation [CMMI-1000021]; Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was financially supported by the National Science Foundation (Grant No. CMMI-1000021) and Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 30 TC 5 Z9 5 U1 4 U2 12 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1023-8883 EI 1573-2711 J9 TRIBOL LETT JI Tribol. Lett. PD JUL PY 2014 VL 55 IS 1 BP 177 EP 186 DI 10.1007/s11249-014-0345-9 PG 10 WC Engineering, Chemical; Engineering, Mechanical SC Engineering GA AI3AB UT WOS:000336729400018 ER PT J AU Bonvini, M Sohn, MD Granderson, J Wetter, M Piette, MA AF Bonvini, Marco Sohn, Michael D. Granderson, Jessica Wetter, Michael Piette, Mary Ann TI Robust on-line fault detection diagnosis for HVAC components based on nonlinear state estimation techniques SO APPLIED ENERGY LA English DT Article DE Fault detection and diagnosis; Bayesian Updating; Chiller plant faults; Unscented Kalman filtering ID QUANTITATIVE MODEL; BUILDING SYSTEMS; PART II; STRATEGY; PROGNOSTICS AB This work presents a robust and computationally efficient algorithm for both whole-building and component-level energy fault detection and diagnosis (FDD). The algorithm is able to provide reliable estimation of multiple and simultaneous fault conditions, even in the presence of noisy and sometimes erroneous sensor data, and to provide uncertainty estimation. The algorithm can be used to provide such outputs as the probability of a fault, the likely cause(s), and the expected consequences of the fault(s) on energy use. The approach is based on an advanced Bayesian nonlinear state estimation technique called Unscented Kalman Filtering, but with our addition of a back-smoothing method that provides fast and robust FDD for common building use cases. The approach is presented and demonstrated for detecting energy and hydraulic faults in a chiller plant. The model of the chiller plant is a subsystem of an actual chiller plant, calibrated to real data. The algorithm can detect common faults, such as (1) energy faults (e.g., the chiller is not working properly, or far from its nominal condition), (2) functional faults caused by issues in the compressor and (3) occlusions in the valves that may reduce the water flow rate through the condenser and evaporator water loop. It is also shown that estimates of uncertainty are consistent with the error in the synthetic data, and can be updated as new data stream in from sensors. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Bonvini, Marco; Granderson, Jessica; Wetter, Michael; Piette, Mary Ann] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Bldg Technol & Urban Syst Dept, Berkeley, CA 94720 USA. [Sohn, Michael D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. RP Sohn, MD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Bldg Technol & Urban Syst Dept, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mdsohn@lbl.gov FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; US Department of Defense under the ESTCP program FX This research was supported in part by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technologies of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. The research was also supported by the US Department of Defense under the ESTCP program. NR 25 TC 19 Z9 19 U1 2 U2 35 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD JUL 1 PY 2014 VL 124 BP 156 EP 166 DI 10.1016/j.apenergy.2014.03.009 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AH7TT UT WOS:000336338800014 ER PT J AU Zimmermann, EA Gludovatz, B Schaible, E Busse, B Ritchie, RO AF Zimmermann, Elizabeth A. Gludovatz, Bernd Schaible, Eric Busse, Bjoern Ritchie, Robert O. TI Fracture resistance of human cortical bone across multiple length-scales at physiological strain rates SO BIOMATERIALS LA English DT Article DE Bone; Strain rate; Fracture toughness; Plasticity; X-ray diffraction ID FATIGUE-CRACK-PROPAGATION; MECHANICAL-PROPERTIES; COMPACT-BONE; CEMENT LINE; BOVINE BONE; TOUGHNESS; COLLAGEN; DEFORMATION; NANOSCALE; DENSITY AB While most fracture-mechanics investigations on bone have been performed at low strain rates, physiological fractures invariably occur at higher loading rates. Here, at strain rates from 10(-5) to 10(-1) s(-1), we investigate deformation and fracture in bone at small length-scales using in situ small-angle x-ray scattering (SAXS) to study deformation in the mineralized collagen fibrils and at the microstructural level via fracture-mechanics experiments to study toughening mechanisms generating toughness through crack-tip shielding. Our results show diminished bone toughness at increasing strain rates as cracks penetrate through the osteons at higher strain rates instead of deflecting at the cement lines, which is a prime toughening mechanism in bone at low strain rates. The absence of crack deflection mechanisms at higher strain rates is consistent with lower intrinsic bone matrix toughness. In the SAXS experiments, higher fibrillar strains at higher strain rates suggest less inelastic deformation and thus support a lower intrinsic toughness. The increased incidence of fracture induced by high strain rates can be associated with a loss in toughness in the matrix caused by a strain rate induced stiffening of the fibril ductility, Le., a "locking-up" of the viscous sliding and sacrificial bonding mechanisms, which are the origin of inelastic deformation (and toughness) in bone at small length-scales. Published by Elsevier Ltd. C1 [Zimmermann, Elizabeth A.; Gludovatz, Bernd; Busse, Bjoern; Ritchie, Robert O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Schaible, Eric] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Expt Syst Grp, Berkeley, CA 94720 USA. [Busse, Bjoern] Univ Med Ctr, Dept Osteol & Biomech, Hamburg, Germany. [Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Ritchie, RO (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM RORitchie@lbl.gov RI Ritchie, Robert/A-8066-2008; Zimmermann, Elizabeth/A-4010-2015; Busse, Bjorn/O-8462-2016; OI Ritchie, Robert/0000-0002-0501-6998; Gludovatz, Bernd/0000-0002-2420-3879; Busse, Bjorn/0000-0002-3099-8073; Zimmermann, Elizabeth/0000-0001-9927-3372 FU National Institute of Health (NIH/NIDCR) [5R01 DE015633]; Emmy Noether program of the German Research Foundation (DFG) [BU 2562/2-1]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Institute of Health (NIH/NIDCR) under grant no. 5R01 DE015633 to the Lawrence Berkeley National Laboratory (LBNL). BB was supported by the Emmy Noether program of the German Research Foundation (DFG) under grant number BU 2562/2-1. We acknowledge the use of the x-ray synchrotron beamline 7.3.3 (SAXS/WAXD) at the Advanced Light Source (ALS) at LBNL, which is funded by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. The authors wish to thank Dr. Tony Tomsia at LBNL for his support. NR 61 TC 22 Z9 22 U1 6 U2 55 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0142-9612 EI 1878-5905 J9 BIOMATERIALS JI Biomaterials PD JUL PY 2014 VL 35 IS 21 BP 5472 EP 5481 DI 10.1016/j.biomaterials.2014.03.066 PG 10 WC Engineering, Biomedical; Materials Science, Biomaterials SC Engineering; Materials Science GA AH7WL UT WOS:000336346000006 PM 24731707 ER PT J AU Basu, A Sanford, RA Johnson, TM Lundstrom, CC Loffler, FE AF Basu, Anirban Sanford, Robert A. Johnson, Thomas M. Lundstrom, Craig C. Loeffler, Frank E. TI Uranium isotopic fractionation factors during U(VI) reduction by bacterial isolates SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SULFATE-REDUCING BACTERIA; MASS-DEPENDENT FRACTIONATION; ANAEROMYXOBACTER-DEHALOGENANS; MICROBIAL REDUCTION; CHROMIUM ISOTOPES; ELECTRON-TRANSFER; U-238/U-235; GROUNDWATER; RATIOS; CR(VI) AB We experimentally determined the magnitude of uranium isotopic fractionation induced by U(VI) reduction by metal reducing bacterial isolates. Our results indicate that microbial U(VI) reduction induces isotopic fractionation; heavier isotopes (i.e., U-238) partition into the solid U(IV) products. The magnitudes of isotopic fractionation (expressed as epsilon = 1000 parts per thousand * (alpha-1)) for U-238/U-235 were 0.68 parts per thousand +/- 0.05 parts per thousand and 0.99 parts per thousand +/- 0.12 parts per thousand for Geobacter sulfurreducens strain PCA and strain IFRC-N, respectively. The epsilon values for Anaeromyxobacter dehalogenans strain FRC-W, strain FRC-R5, a novel Shewanella isolate, and Desulfitobacterium sp. strain Viet1 were 0.72 parts per thousand +/- 0.15 parts per thousand, 0.99 parts per thousand +/- 0.12 parts per thousand, 0.96 parts per thousand +/- 0.16 parts per thousand and 0.86 parts per thousand +/- 0.06 parts per thousand, respectively. Our results show that the maximum epsilon values of similar to 1.0 parts per thousand were obtained with low biomass (similar to 10(7) cells/mL) and low electron donor concentrations (similar to 500 mu M). These results provide an initial assessment of U-238/U-235 shifts induced by microbially-mediated U(VI) reduction, which is needed as U-238/U-235 data are increasingly applied as redox indicators in various geochemical settings. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Basu, Anirban] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Sanford, Robert A.; Johnson, Thomas M.; Lundstrom, Craig C.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA. [Loeffler, Frank E.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Loeffler, Frank E.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Loeffler, Frank E.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Basu, A (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, 483 McCone Hall, Berkeley, CA 94720 USA. EM anirbanbasu@berkeley.edu RI Basu, Anirban/P-5048-2016 OI Basu, Anirban/0000-0002-4905-9156 FU US Department of Energy, Office of Science - Subsurface Biogeochemical Research Program [DE-SC0001281] FX This material is based upon work supported by US Department of Energy, Office of Science within the Subsurface Biogeochemical Research Program under grant DE-SC0001281. We thank three anonymous reviewers for their comments, which greatly improved the quality of this work. NR 62 TC 28 Z9 29 U1 7 U2 47 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUL 1 PY 2014 VL 136 BP 100 EP 113 DI 10.1016/j.gca.2014.02.041 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AH9SG UT WOS:000336481800007 ER PT J AU Lee, JH Zachara, JM Fredrickson, JK Heald, SM McKinley, JP Plymale, AE Resch, CT Moore, DA AF Lee, Ji-Hoon Zachara, John M. Fredrickson, James K. Heald, Steve M. McKinley, James P. Plymale, Andrew E. Resch, Charles T. Moore, Dean A. TI Fe(II)- and sulfide-facilitated reduction of Tc-99(VII) O-4(-) in microbially reduced hyporheic zone sediments SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID X-RAY-ABSORPTION; HANFORD SITE; VADOSE ZONE; PERTECHNETATE IMMOBILIZATION; TECHNETIUM SPECIATION; SUBSURFACE SEDIMENTS; HYDROGEN-SULFIDE; URANIUM; RIVER; IRON AB Redox-reactive, biogeochemical phases generated by reductive microbial activity in hyporheic zone sediments from a dynamic groundwater-river interaction zone were evaluated for their ability to reduce soluble pertechnetate [Tc-99(VII) O-4(-)] to less soluble Tc(IV). The sediments were bioreduced by indigenous microorganisms that were stimulated by organic substrate addition in synthetic groundwater with or without sulfate. In most treatments, 20 mu mol L-1 initial aqueous Tc(VII) was reduced to near or below detection (3.82 X 10(-9) mol L-1) over periods of days to months in suspensions of variable solids concentrations. Native sediments containing significant lithogenic Fe(II) in various phases were, in contrast, unreactive with Tc(VII). The reduction rates in the bioreduced sediments increased with increases in sediment mass, in proportion to weak acid-extractable Fe(II) and sediment-associated sulfide (AVS). The rate of Tc(VII) reduction was first order with respect to both aqueous Tc(VII) concentration and sediment mass, but correlations between specific reductant concentrations and reaction rate were not found. X-ray microprobe measurements revealed a strong correlation between Tc hot spots and Fe-containing mineral particles in the sediment. However, only a portion of Fe-containing particles were Tc-hosts. The Tc-hot spots displayed a chemical signature (by EDXRF) similar to pyroxene. The application of autoradiography and electron microprobe allowed further isolation of Tc-containing particles that were invariably found to be ca 100 mu m aggregates of primary mineral material embedded within a fine-grained phyllosilicate matrix. EXAFS spectroscopy revealed that the Tc(IV) within these were a combination of a Tc(IV) O-2-like phase and Tc(IV)-Fe surface clusters, with a significant fraction of a TcSx-like phase in sediments incubated with SO42-. AVS was implicated as a more selective reductant at low solids concentration even though its concentration was below that required for stoichiometric reduction of Tc(VII). These results demonstrate that composite mineral aggregates may be redox reaction centers in coarse-textured hyporheic zone sediments regardless of the dominant anoxic biogeochemical processes. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lee, Ji-Hoon; Zachara, John M.; Fredrickson, James K.; McKinley, James P.; Plymale, Andrew E.; Resch, Charles T.; Moore, Dean A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Heald, Steve M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Zachara, JM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.zachara@pnnl.gov FU Subsurface Biogeochemical Research Program (SBR); Office of Biological and Environmental Research (OBER); US DOE; PNNL Scientific Focus Area (SFA); Department of Energy's Office of Biological and Environmental Research; Office of Basic Energy Sciences, US DOE [DE-AC02-06CH11357] FX This research was supported by the Subsurface Biogeochemical Research Program (SBR), Office of Biological and Environmental Research (OBER), US DOE; and is a contribution of the PNNL Scientific Focus Area (SFA). Subsurface sediment samples were provided courtesy of the Integrated Field Research Challenge (IFRC) site at the Hanford 300 Area. Selected analyses were performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. PNNL is operated for the DOE by Battelle. XAS analyses were performed at the Advanced Photon Source supported by Office of Basic Energy Sciences, US DOE under Contract DE-AC02-06CH11357. The reviewers acknowledge, with apprecia-tion, three insightful reviews that improved the quality of this contribution. NR 49 TC 11 Z9 11 U1 14 U2 76 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUL 1 PY 2014 VL 136 BP 247 EP 264 DI 10.1016/j.gca.2013.08.017 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AH9SG UT WOS:000336481800015 ER PT J AU Bellomo, N Brezzi, F Manzini, G AF Bellomo, N. Brezzi, F. Manzini, G. TI Recent techniques for PDE discretizations on polyhedral meshes SO MATHEMATICAL MODELS & METHODS IN APPLIED SCIENCES LA English DT Article DE Polygonal meshes; polyhedral meshes; Mimetic Finite Differences; Virtual Element Methods; Finite Volumes; discontinuous Galerkin methods ID MIMETIC FINITE-DIFFERENCES; ELEMENT-METHOD; DIFFERENCE METHOD AB This brief paper is an introduction to the papers published in a special issue devoted to survey on recent techniques for discretizing Partial Differential Equations on general polygonal and polyhedral meshes. The number of different techniques to deal with discretizations on polygonal and polyhedral meshes is quite huge, and their history is quite long. Here we concentrate on the most recent techniques, including Mimetic Finite Differences, Virtual Element Methods, and the recent developments, in this direction, of Finite Volumes and Discontinuous Galerkin Methods. C1 [Bellomo, N.] Politecn Torino, Dept Math Sci, I-10129 Turin, Italy. [Brezzi, F.] IUSS, I-27100 Pavia, Italy. [Brezzi, F.] IMATI CNR, I-27100 Pavia, Italy. [Manzini, G.] Los Alamos Natl Lab, Appl Math & Plasma Phys Grp, Div Theoret, Los Alamos, NM 87545 USA. RP Brezzi, F (reprint author), IUSS, Via Ferrata 5, I-27100 Pavia, Italy. EM nicola.bellomo@polito.it; brezzi@imati.cnr.it; gmanzini@lanl.gov RI Brezzi, Franco/D-4362-2009; Bellomo, Nicola/B-3431-2010; OI Brezzi, Franco/0000-0003-4715-5475; Bellomo, Nicola/0000-0002-5989-1608; Manzini, Gianmarco/0000-0003-3626-3112 NR 21 TC 0 Z9 0 U1 0 U2 11 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0218-2025 EI 1793-6314 J9 MATH MOD METH APPL S JI Math. Models Meth. Appl. Sci. PD JUL PY 2014 VL 24 IS 8 SI SI BP 1453 EP 1455 DI 10.1142/S0218202514030018 PG 3 WC Mathematics, Applied SC Mathematics GA AH1ZS UT WOS:000335921100001 ER PT J AU Gyrya, V Lipnikov, K Manzini, G Svyatskiy, D AF Gyrya, Vitaliy Lipnikov, Konstantin Manzini, Gianmarco Svyatskiy, Daniil TI M-Adaptation in the mimetic finite difference method SO MATHEMATICAL MODELS & METHODS IN APPLIED SCIENCES LA English DT Article DE Mimetic discretization; unstructured polyhedral meshes; discrete maximum principles; numerical optimization ID DISCRETE MAXIMUM PRINCIPLE; ANISOTROPIC DIFFUSION-PROBLEMS; MULTIPOINT FLUX APPROXIMATION; TENSOR ARTIFICIAL VISCOSITY; ELLIPTIC PROBLEMS; POLYGONAL MESHES; POLYHEDRAL MESHES; VOLUME METHOD; TOPOLOGY OPTIMIZATION; UNSTRUCTURED GRIDS AB The mimetic finite difference method produces a family of schemes with equivalent properties such as the stencil size, stability region, and convergence order. Each member of this family is defined by a set of parameters which can be chosen locally for every mesh element. The number of parameters depends on the geometry of a particular mesh element. M-Adaptation is a new adaptation methodology that identifies a member of this family with additional (superior) properties compared to the other schemes in the family. We analyze the enforcement of the discrete maximum principles for the diffusion equation in the primal and dual forms, the reduction of numerical dispersion and anisotropy for the acoustic wave equation, and the optimization of the performance of multi-grid solvers. C1 [Gyrya, Vitaliy; Lipnikov, Konstantin; Manzini, Gianmarco; Svyatskiy, Daniil] Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. [Manzini, Gianmarco] CNR, Ist Matemat Appl & Tecnol Informat, I-27100 Pavia, Italy. RP Manzini, G (reprint author), Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. EM gyrya@lanl.gov; lipnikov@lanl.gov; gmanzini@lanl.gov; dasvyat@lanl.gov OI Manzini, Gianmarco/0000-0003-3626-3112; Gyrya, Vitaliy/0000-0002-5083-8878 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research FX This work was carried out under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The authors acknowledge support of the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research. The model in Sec. 6 was provided by the DOE Office of Environmental Management Advanced Simulation Capability for Environmental Management (ASCEM) Program. 128 NR 129 TC 7 Z9 7 U1 0 U2 7 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0218-2025 EI 1793-6314 J9 MATH MOD METH APPL S JI Math. Models Meth. Appl. Sci. PD JUL PY 2014 VL 24 IS 8 SI SI BP 1621 EP 1663 DI 10.1142/S0218202514400053 PG 43 WC Mathematics, Applied SC Mathematics GA AH1ZS UT WOS:000335921100006 ER PT J AU Manzini, G Russo, A Sukumar, N AF Manzini, Gianmarco Russo, Alessandro Sukumar, N. TI New perspectives on polygonal and polyhedral finite element methods SO MATHEMATICAL MODELS & METHODS IN APPLIED SCIENCES LA English DT Article DE Wachspress basis functions; barycentric finite elements; virtual element method; numerical integration; consistency ID TENSOR ARTIFICIAL VISCOSITY; ARBITRARY PLANAR POLYGONS; MOVING LEAST-SQUARES; DIFFERENCE METHOD; ELLIPTIC PROBLEMS; DIFFUSION-PROBLEMS; MIMETIC DISCRETIZATION; TOPOLOGY OPTIMIZATION; CONVEX POLYGONS; SOLID MECHANICS AB Generalized barycentric coordinates such as Wachspress and mean value coordinates have been used in polygonal and polyhedral finite element methods. Recently, mimetic finite difference schemes were cast within a variational framework, and a consistent and stable finite element method on arbitrary polygonal meshes was devised. The method was coined as the virtual element method (VEM), since it did not require the explicit construction of basis functions. This advance provides a more in-depth understanding of mimetic schemes, and also endows polygonal-based Galerkin methods with greater flexibility than three-node and four-node finite element methods. In the VEM, a projection operator is used to realize the decomposition of the stiffness matrix into two terms: a consistent matrix that is known, and a stability matrix that must be positive semi-definite and which is only required to scale like the consistent matrix. In this paper, we first present an overview of previous developments on conforming polygonal and polyhedral finite elements, and then appeal to the exact decomposition in the VEM to obtain a robust and efficient generalized barycentric coordinate-based Galerkin method on polygonal and polyhedral elements. The consistent matrix of the VEM is adopted, and numerical quadrature with generalized barycentric coordinates is used to compute the stability matrix. This facilitates post-processing of field variables and visualization in the VEM, and on the other hand, provides a means to exactly satisfy the patch test with efficient numerical integration in polygonal and polyhedral finite elements. We present numerical examples that demonstrate the sound accuracy and performance of the proposed method. For Poisson problems in R-2 and R-3, we establish that linearly complete generalized barycentric interpolants deliver optimal rates of convergence in the L-2-norm and the H-1-seminorm. C1 [Manzini, Gianmarco] Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. [Manzini, Gianmarco; Russo, Alessandro] CNR, Ist Matemat Appl & Tecnol Informat E Magenes, I-27100 Pavia, Italy. [Russo, Alessandro] Univ Milano Bicocca, Dipartimento Matemat & Applicaz, I-20153 Milan, Italy. [Sukumar, N.] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA. RP Manzini, G (reprint author), Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. EM gmanzini@lanl.gov; alessandro.russo@unimib.it; nsukumar@ucdavis.edu RI Sukumar, N/B-1660-2008; Russo, Alessandro/F-6081-2012; OI Russo, Alessandro/0000-0002-6878-402X; Manzini, Gianmarco/0000-0003-3626-3112 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics; National Science Foundation [CMMI-1334783] FX The work of G. M. was partially supported by the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics. N.S. gratefully acknowledges the research support of the National Science Foundation through Contract Grant CMMI-1334783 to the University of California at Davis. N.S. also thanks Michael Floater, Andrew Gillette and Kai Hormann for many helpful discussions. NR 136 TC 30 Z9 30 U1 6 U2 21 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0218-2025 EI 1793-6314 J9 MATH MOD METH APPL S JI Math. Models Meth. Appl. Sci. PD JUL PY 2014 VL 24 IS 8 SI SI BP 1665 EP 1699 DI 10.1142/S0218202514400065 PG 35 WC Mathematics, Applied SC Mathematics GA AH1ZS UT WOS:000335921100007 ER PT J AU Shim, YS Zhang, L Kim, DH Kim, YH Choi, YR Nahm, SH Kang, CY Lee, W Jang, HW AF Shim, Young-Seok Zhang, Lihua Kim, Do Hong Kim, Yeon Hoo Choi, You Rim Nahm, Seung Hoon Kang, Chong-Yun Lee, Wooyoung Jang, Ho Won TI Highly sensitive and selective H-2 and NO2 gas sensors based on surface-decorated WO3 nanoigloos SO SENSORS AND ACTUATORS B-CHEMICAL LA English DT Article DE WO3; Nanoigloos; Surface decoration; Metal nanoparticles; Sensitization ID ELECTRONIC NOSE; SENSING PROPERTIES; THIN-FILMS; CATALYSIS; SILVER; NANOSTRUCTURES; TEMPERATURE AB WO3 nanoigloos decorated with Ag-, Pd-. and Au nanoparticles are fabricated by soft-template method and self-agglomeration of metal films. The responses of WO3 nanoigloos decorated with metal nanoparticies to various gases such as NO2, CH3COCH3, C2H5OH, and H-2 are much higher than those of bare WO3 nanoigloos. According to the surface decoration, WO3 nanigloos show significantly different behaviors in the response enhancement, revealing that Pd-decorated WO3 nanoigloos exhibit the highest response to H-2 together with fast response time to H-2,H- C2H5OH, and CH3COCH3 (below 10s),Au-decorated WO3 nanoigloos exhibit the highest response to NO2. The catalytic effect of Ag is relatively weaker than Pd and Au nanoparticles, however, it exhibit the fastest response time to NO2. These are attributed to not only the varied catalytic activities of the metal nanoparticles, but also the different work function energies of them. Our results show that highly sensitive and selective WO3 nanoigloos decorated with metal nanoparticles can be an effective platform to fabricate an electronic nose for the further application of semiconducting metal oxide gas sensors. (C) 2014 Elsevier B.V. All rights reserved. C1 [Lee, Wooyoung] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. [Shim, Young-Seok; Lee, Wooyoung] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. [Shim, Young-Seok; Kim, Do Hong; Kim, Yeon Hoo; Choi, You Rim; Jang, Ho Won] Seoul Natl Univ, Res Inst Adv Mat, Dept Mat Sci & Engn, Seoul 151744, South Korea. [Kang, Chong-Yun] Korea Inst Sci & Technol, Ctr Elect Mat, Seoul 136791, South Korea. [Zhang, Lihua] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Nahm, Seung Hoon] Korea Res Inst Stand & Sci, Ctr Energy Mat Metrol, Taejon 305340, South Korea. Korea Univ, KU KIST Grad Sch Converging Sci & Technol, Seoul 136701, South Korea. RP Lee, W (reprint author), Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. EM wooyouong@yonsei.ac.kr; hwjang@snu.ac.kr RI Jang, Ho Won/D-9866-2011; OI Jang, Ho Won/0000-0002-6952-7359; Kang, Chong-Yun/0000-0002-4516-8160 FU Minstry of science, ICT AMP;Future Planning as the Globlal Frontier Project; Outstanding Young Researcher Program,; National Research Foundation of Korea; Korea Institure of science and Techmology; National Research Foundation of Korea (NRF) [2009-0093823]; U.S. Department of Energy, Office of Basic Energy Sciences, [DE-AC02-98CH10886] FX This work was financially supported by the Center for Integrated Smart Sensors funded by the Ministry of science, ICT & Future Planning as the Global Frontier Project, the Outstanding Young Researcher Program, and the National Research Foundation of Korea and a research program of the Korea Institute of science and Technology. WL is grateful for the support of priority Research Centers Program (2009-0093823) though the National Research Foundation of Korea (NRF). TEM Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory. which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences,under Contract No.DE-AC02-98CH10886. NR 38 TC 20 Z9 21 U1 6 U2 78 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-4005 J9 SENSOR ACTUAT B-CHEM JI Sens. Actuator B-Chem. PD JUL PY 2014 VL 198 BP 294 EP 301 DI 10.1016/j.snb.2014.03.073 PG 8 WC Chemistry, Analytical; Electrochemistry; Instruments & Instrumentation SC Chemistry; Electrochemistry; Instruments & Instrumentation GA AG7EE UT WOS:000335580100043 ER PT J AU Chen, CF Marksteiner, QR Reiten, MR Wynn, TA Guidry, DR AF Chen, Ching-Fong Marksteiner, Quinn R. Reiten, Matthew R. Wynn, Thomas A. Guidry, Dennis R. TI Lamination of magnesium oxide spacers to barium strontium zirconium titanate ceramics SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID SOLITON GENERATION; FREQUENCY AB We propose an innovative idea to bond the dielectric barium strontium zirconium titanate (BSTZO) plates with magnesium oxide (MgO) as the spacers to achieve a hermetic module without any air gaps between the dielectric and the spacer. The gold metallization can be applied across the whole assembly to create an integrated electrode. The gold metallization also eliminates pressure contact by external copper plates assemblies, which are required to achieve good contacts between the copper plates and the metallized surfaces of the BSTZO. The MgO spacers are processed using a dry-pressing and pressureless-sintering method. The thermal expansion coefficient (CTE) of BSTZO and MgO spacer was measured. In addition to matching the CTE between BSTZO dielectric and the MgO spacer, it is also critical to develop a good bonding material with CTE matching to BSTZO and MgO spacer. The effect of CTE for various bonding compositions on the dielectric properties was thoroughly studied and reported. The mechanism explaining the high and low dielectric constants for the laminates is proposed and discussed based on the CTE results and their effect on microstructural development. C1 [Chen, Ching-Fong; Wynn, Thomas A.; Guidry, Dennis R.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Marksteiner, Quinn R.; Reiten, Matthew R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chen, CF (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM cchen@lanl.gov FU US Department of Energy through the LANL LDRD program; DOE [DE-AC52-06NA25396] FX The authors would like to thank Elias N. Pulliam for measuring the dielectrical properties of some laminates. We gratefully acknowledge the support of the US Department of Energy through the LANL LDRD program for this work. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 14 TC 1 Z9 1 U1 0 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD JUL PY 2014 VL 49 IS 14 BP 5218 EP 5226 DI 10.1007/s10853-014-8238-8 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA AG5IC UT WOS:000335451700055 ER PT J AU Hecht, AA Blakeley, RE Martin, WJ Leonard, E AF Hecht, A. A. Blakeley, R. E. Martin, W. J. Leonard, E. TI Comparison of Geant4 and MCNP6 for use in delayed fission radiation simulation SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Fission distribution; Delayed radiation; Monte Carlo; Geant4; MCNP; CINDER ID GAMMA SIGNATURE CALCULATION; NEUTRON-INDUCED FISSION; MONTE-CARLO AB Neutron induced fission fragment distributions and delayed fission radiation are extremely important with reactor applications in fission cross sections and heating. Data on the fragment distributions are sparse so simulations use models or interpolations between known neutron energies. Different simulations perform different treatments of the distributions, and have different capabilities and flexibility in use. MCNP is a typical workhorse for fission simulations and coupled with burn-up codes such as CINDER can provide delayed radiation from fission. Geant4 is an extremely flexible physics based Monte Carlo simulation framework, but is not typically used for fission research. In this work the applicability of Geant4 for delayed fission radiation simulations is examined, with comparison to MCNP6 coupled with the CINDER2008 burn-up code. The Fisher and Engle fission experiment with the Godiva II subcritical assembly as a fission neutron source is used as a test case. Both simulations are adapted from that experiment and simulation results are compared with that experiment. Following Fisher and Engle, photons/fission/sec, MeV/fission/sec, and MeV/photon are examined. For the first two quantities results from both simulation codes are similar and are lower than experimental values, with Geant4 giving a higher value for earlier time bins and MCNP6/CINDER giving a higher value for the later time bins. For the last quantity both simulations are usually within uncertainty of the experimental values, with MCNP6/CINDER values consistently higher than both experimental and Geant4 values. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Hecht, A. A.; Blakeley, R. E.; Martin, W. J.; Leonard, E.] Univ New Mexico, Albuquerque, NM 87131 USA. [Martin, W. J.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Hecht, AA (reprint author), Univ New Mexico, Albuquerque, NM 87131 USA. EM hecht@unm.edu FU DTRA [DTRA01-03-D-0009-0025] FX This work was partially supported through DTRA contract DTRA01-03-D-0009-0025, Modeling and Simulation to Support Systems Development and Assessment for Standoff Detection of Nuclear Materials and through a UNM Junior Faculty Collaborative Research Grant. The authors acknowledge useful discussions on programming with John Perry of both UNM and LANL. NR 22 TC 1 Z9 1 U1 3 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD JUL PY 2014 VL 69 BP 134 EP 138 DI 10.1016/j.anucene.2014.02.004 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AG0LR UT WOS:000335107500017 ER PT J AU Hunt, RD Hickman, RR Ladd-Lively, JL Anderson, KK Collins, RT Collins, JL AF Hunt, R. D. Hickman, R. R. Ladd-Lively, J. L. Anderson, K. K. Collins, R. T. Collins, J. L. TI Production of small uranium dioxide microspheres for cermet nuclear fuel using the internal gelation process SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Internal gelation; Uranium oxide microspheres; Cermet fuel AB The U.S. National Aeronautics and Space Administration (NASA) is developing a uranium dioxide (UO2)/(tungsten cermet fuel for potential use as the nuclear cryogenic propulsion stage (NCPS). The first generation NCPS is expected to be made from dense UO2 microspheres with diameters between 75 and 150 mu m. Previously, the internal gelation process and a hood-scale apparatus with a vibrating nozzle were used to form gel spheres, which became UO2 kernels with diameters between 350 and 850 mu m. For the NASA spheres, the vibrating nozzle was replaced with a custom designed, two-fluid nozzle to produce gel spheres in the desired smaller size range. This paper describes the operational methodology used to make 3 kg of uranium oxide (UOx) microspheres. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Hunt, R. D.; Ladd-Lively, J. L.; Anderson, K. K.; Collins, R. T.; Collins, J. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hickman, R. R.] NASA, Marshall Space Flight Ctr, Huntsville, AL 35802 USA. RP Hunt, RD (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM huntrd@ornl.gov RI Ladd-Lively, Jennifer/I-6305-2016 OI Ladd-Lively, Jennifer/0000-0001-9353-675X NR 18 TC 3 Z9 3 U1 2 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD JUL PY 2014 VL 69 BP 139 EP 143 DI 10.1016/j.anucene.2014.02.003 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AG0LR UT WOS:000335107500018 ER PT J AU Ashley, SF Lindley, BA Parks, GT Nuttall, WJ Gregg, R Hesketh, KW Kannan, U Krishnani, PD Singh, B Thakur, A Cowper, M Talamo, A AF Ashley, S. F. Lindley, B. A. Parks, G. T. Nuttall, W. J. Gregg, R. Hesketh, K. W. Kannan, U. Krishnani, P. D. Singh, B. Thakur, A. Cowper, M. Talamo, A. TI Fuel cycle modelling of open cycle thorium-fuelled nuclear energy systems SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Thorium; Nuclear energy; Fuel cycle modelling; Open nuclear fuel cycle; Proliferation resistance ID REACTOR; DESIGN AB In this study, we have sought to determine the advantages, disadvantages, and viability of open cycle thorium-uranium-fuelled (Th-U-fuelled) nuclear energy systems. This has been done by assessing three such systems, each of which requires uranium enriched to similar to 20% U-235, in comparison to a reference uranium-fuelled (U-fuelled) system over various performance indicators, spanning material flows, waste composition, economics, and proliferation resistance. The values of these indicators were determined using the UK National Nuclear Laboratory's fuel cycle modelling code ORION. This code required the results of lattice-physics calculations to model the neutronics of each nuclear energy system, and these were obtained using various nuclear reactor physics codes and burn-up routines. In summary, all three Th-U-fuelled nuclear energy systems required more separative work capacity than the equivalent benchmark U-fuelled system, with larger levelised fuel cycle costs and larger levelised cost of electricity. Although a reduction of similar to 6% in the required uranium ore per kWh was seen for one of the Th-U-fuelled systems compared to the reference U-fuelled system, the other two Th-U-fuelled systems required more uranium ore per kWh than the reference. Negligible advantages and disadvantages were observed for the amount and the properties of the spent nuclear fuel (SNF) generated by the systems considered. Two of the Th-U-fuelled systems showed some benefit in terms of proliferation resistance of the SNF generated. Overall, it appears that there is little merit in incorporating thorium into nuclear energy systems operating with open nuclear fuel cycles. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [Ashley, S. F.; Lindley, B. A.; Parks, G. T.] Univ Cambridge, Dept Engn, Cambridge CB2 1PZ, England. [Nuttall, W. J.] Open Univ, Dept Engn & Innovat, Milton Keynes MK7 6AA, Bucks, England. [Gregg, R.; Hesketh, K. W.] UK Natl Nucl Lab, Preston PR4 0XJ, Lancs, England. [Kannan, U.; Krishnani, P. D.; Singh, B.; Thakur, A.] Bhabha Atom Res Ctr, Reactor Phys Design Div, Bombay 400085, Maharashtra, India. [Cowper, M.] Univ Liverpool, Oliver Lodge Lab, Dept Phys, NTEC, Liverpool L69 7ZE, Merseyside, England. [Talamo, A.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Ashley, SF (reprint author), Open Univ, Dept Engn & Innovat, Milton Keynes MK7 6AA, Bucks, England. EM sfa24@cam.ac.uk OI Ashley, Stephen/0000-0001-5139-2209; talamo, alberto/0000-0001-5685-0483 FU UK Engineering and Physical Sciences Research Council [EP/I018425/1] FX This work is supported by the UK Engineering and Physical Sciences Research Council under Grant No. EP/I018425/1. Two of the authors (SFA and WJN) would like to acknowledge the generous welcome provided by Bhabha Atomic Research Centre during a visit to their facilities. NR 62 TC 8 Z9 8 U1 2 U2 36 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD JUL PY 2014 VL 69 BP 314 EP 330 DI 10.1016/j.anucene.2014.01.042 PG 17 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AG0LR UT WOS:000335107500036 ER PT J AU Al-Azizi, AA Eryilmaz, O Erdemir, A Kim, SH AF Al-Azizi, Ala' A. Eryilmaz, Osman Erdemir, Ali Kim, Seong H. TI Nano-texture for a wear-resistant and near-frictionless diamond-like carbon SO CARBON LA English DT Article ID DLC FILMS; SUPERLOW-FRICTION; INTERNAL-STRESS; THIN-FILMS; SURFACE-ROUGHNESS; AMORPHOUS-CARBON; ELASTIC-MODULUS; COATINGS; LUBRICATION; HARDNESS AB The effect of nano-scale surface texture on wear resistance of diamond-like carbon 0)14 films was studied using a reciprocating ball-on-fiat tribometer in dry, humid, and liquid water environments. The nano-scale surface texture was produced by depositing similar to 1 gm thick DLC films onto silicon substrates pre-textured with pyramidal wells and polystyrene spheres. The surface roughness of the textured DLC films was about 50 nm in both cases. The friction and wear behavior of the flat and nano-textured DLC films were tested with AISI 440C-grade stainless steel balls at a contact load creating about 360 nm deep Hertzian deformation which is significantly larger than the surface roughness. At this condition, nano-texturing did not affect the friction coefficient, but it significantly reduced the wear of DLC films in dry and humid nitrogen compared to flat DLC. In dry nitrogen, the nanotextured DLC films showed the ultra-low friction without substantial wear of DLC and deposition of thick transfer films onto the counter-surface. The wear reduction appeared to be related to the stress relief in the nano-textured DLC film. In liquid water, surface features on the nano-textured DLC films were diminished due to tribochemical oxidation and material removal at the sliding interface. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Al-Azizi, Ala' A.; Kim, Seong H.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Eryilmaz, Osman; Erdemir, Ali] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Eryilmaz, Osman; Erdemir, Ali] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Kim, SH (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM shkim@engr.psu.edu FU National Science Foundation [CMMI-1131128]; U.S. Department of Energy, Basic 'Energy Sciences, Office of Energy Efficiency and Renewable Energy [DE-ACO2-06CH11357] FX This work was supported by the National Science Foundation (Grant No. CMMI-1131128). The authors acknowledged Dr. Shikuan Yang for his help with electron microscope imaging. O.E. and A.E. were supported by the U.S. Department of Energy, Basic 'Energy Sciences, Office of Energy Efficiency and Renewable Energy, under contract #DE-ACO2-06CH11357. NR 67 TC 9 Z9 9 U1 9 U2 102 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD JUL PY 2014 VL 73 BP 403 EP 412 DI 10.1016/j.carbon.2014.03.003 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AG0HK UT WOS:000335096300044 ER PT J AU Shin, SJ Tran, IC Willey, TM van Buuren, T Ilausky, J Biener, MM Worsley, MA Hamza, AV Kucheyev, SO AF Shin, S. J. Tran, I. C. Willey, T. M. van Buuren, T. Ilausky, J. Biener, M. M. Worsley, M. A. Hamza, A. V. Kucheyev, S. O. TI Robust nanoporous alumina monoliths by atomic layer deposition on low-density carbon-nanotube scaffolds SO CARBON LA English DT Article ID SENSING INDENTATION; AEROGELS; SOLIDS AB Synthesis of nanoporous alumina monoliths with controlled morphology and density is a challenge. Here, we demonstrate mechanically robust alumina monoliths synthesized by conformal overcoating of graphitic nanoligaments of low-density carbon-nanotube-based aerogels (CNT-CAs) by using atomic layer deposition. Young's modulus of resultant monoliths increases superlinearly with the monolith density with an exponent of -2.4, defined by the morphology and connectivity of the CNT-CA scaffold. As a result, for a given monolith density, alumina-carbon composites have moduli comparable to those of CNT-CAs and significantly superior to those of pure alumina aerogels reported previously. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Shin, S. J.; Tran, I. C.; Willey, T. M.; van Buuren, T.; Biener, M. M.; Worsley, M. A.; Hamza, A. V.; Kucheyev, S. O.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Ilausky, J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Shin, SJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM shin5@llnl.gov RI Worsley, Marcus/G-2382-2014; USAXS, APS/D-4198-2013; Tran, Ich/C-9869-2014; Foundry, Molecular/G-9968-2014; Ilavsky, Jan/D-4521-2013; Willey, Trevor/A-8778-2011 OI Worsley, Marcus/0000-0002-8012-7727; Ilavsky, Jan/0000-0003-1982-8900; Willey, Trevor/0000-0002-9667-8830 FU LLNL [DE-AC52-07NA27344]; US DOE [DE-ACO2-05CH11231, DE-ACO2-06CH11357]; National Science Foundation/DOE [NSF/CHE-0822838] FX This work was performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344. Transmission electron microscopy experiments were conducted at the National Center for Electron Microscopy, LBNL, which is supported by the US DOE under Contract DE-ACO2-05CH11231. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-ACO2-06CH11357. ChemMatCARS Sector 15 is principally supported by the National Science Foundation/ DOE under Grant No. NSF/CHE-0822838. NR 24 TC 5 Z9 5 U1 3 U2 36 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD JUL PY 2014 VL 73 BP 443 EP 447 DI 10.1016/j.carbon.2014.03.006 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AG0HK UT WOS:000335096300048 ER PT J AU Abdalla, M Hastings, A Helmy, M Prescher, A Osborne, B Lanigan, G Forristal, D Killi, D Maratha, P Williams, M Rueangritsarakul, K Smith, P Nolan, P Jones, MB AF Abdalla, M. Hastings, A. Helmy, M. Prescher, A. Osborne, B. Lanigan, G. Forristal, D. Killi, D. Maratha, P. Williams, M. Rueangritsarakul, K. Smith, P. Nolan, P. Jones, M. B. TI Assessing the combined use of reduced tillage and cover crops for mitigating greenhouse gas emissions from arable ecosystem SO GEODERMA LA English DT Article DE Reduced tillage; Conventional tillage; Cover crop; DNDC model; Greenhouse gas emissions; Future climate ID NITROUS-OXIDE EMISSIONS; SOIL CO2 EFFLUX; FLUXES FOLLOWING TILLAGE; FILLED PORE-SPACE; LOAMY SAND SOIL; CARBON-DIOXIDE; LONG-TERM; CONSERVATION TILLAGE; CROPPING SYSTEM; ORGANIC-MATTER AB Field management activities have significant impacts on greenhouse gas (GHG) emissions from cropland soils. In this study, the effectiveness of combining reduced tillage with a mustard cover crop (RT-CC) to mitigate present and future GHG emissions from a fertilized spring barley field in the southeast of Ireland was assessed. The field site which had a free-draining sandy loam soil with low soil moisture holding capacity, had been managed for three years prior to measurements under two different tillage systems; conventional (CT) and RT-CC. Field measurements of soil CO2, N2O and CH4 emissions, crop biomass, water filled pore space (WFPS), soil temperature and soil nitrate were made to capture both steady state conditions as well as the management events. Field data were used to validate the DNDC (DeNitrification-DeComposition) model and future GHG emissions under two sets of climate projections were predicted. Although fertilizer use was the same for both treatments the RT-CC treatment had significantly (p < 0.05) higher N2O emissions for both present and future climate. However, the inclusion of a cover crop with the RT treatment increased predicted soil organic carbon (SOC), which more than compensated for the higher N2O flux resulting in a lower total GHG balance (TGGB) compared with the CT treatment. Results show that the effectiveness of RT-CC in mitigating GHG emissions will depend crucially on the magnitude of compensatory increases in carbon dioxide uptake by the cover crop that will contribute to a reduction in the total GHG balance. (C) 2014 Elsevier B.V. All rights reserved. C1 [Abdalla, M.; Hastings, A.; Smith, P.] Univ Aberdeen, Sch Biol Sci, Inst Biol & Environm Sci, Aberdeen AB24 3UU, Scotland. [Abdalla, M.; Williams, M.; Rueangritsarakul, K.; Jones, M. B.] Univ Dublin Trinity Coll, Sch Nat Sci, Dept Bot, Dublin 2, Ireland. [Helmy, M.; Osborne, B.; Killi, D.; Maratha, P.] Univ Coll Dublin, Sch Biol & Environm Sci, Dublin 4, Ireland. [Prescher, A.] Inst Landscape Syst Anal, Leibniz Ctr Agr Landscape Res ZALF, D-15374 Muncheberg, Germany. [Lanigan, G.] TEAGASC, Johnstown Castle Res Ctr, Wexford, Ireland. [Forristal, D.] TEAGASC, Oak Pk Crops Res Ctr, Oak Pk, Co Carlow, Ireland. [Nolan, P.] Univ Coll Dublin, Meteorol & Climate Ctr, Dublin 4, Ireland. RP Abdalla, M (reprint author), Univ Aberdeen, Sch Biol Sci, Inst Biol & Environm Sci, 23 St Machar Dr, Aberdeen AB24 3UU, Scotland. EM mabdalla@abdn.ac.uk RI Lanigan, Gary/C-6864-2012; Smith, Pete/G-1041-2010 OI Lanigan, Gary/0000-0003-0813-3097; Smith, Pete/0000-0002-3784-1124 FU Irish Department of Agriculture Research Stimulus Fund [07 528] FX This work was funded by the Irish Department of Agriculture Research Stimulus Fund (project no: 07 528) and contributed to the EU FP7 project GHG-Europe. We are grateful to the staff of Teagasc Research Centre, Carlow for facilitating our field work. Pete Smith is a Royal Society-Wolfson Research Merit Award holder. NR 138 TC 6 Z9 6 U1 15 U2 122 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0016-7061 EI 1872-6259 J9 GEODERMA JI Geoderma PD JUL PY 2014 VL 223 BP 9 EP 20 DI 10.1016/j.geoderma.2014.01.030 PG 12 WC Soil Science SC Agriculture GA AG3CA UT WOS:000335292200002 ER PT J AU Chae, KY Ahn, S Bardayan, DW Chipps, KA Manning, B Pain, SD Peters, WA Schmitt, KT Smith, MS Strauss, SY AF Chae, K. Y. Ahn, S. Bardayan, D. W. Chipps, K. A. Manning, B. Pain, S. D. Peters, W. A. Schmitt, K. T. Smith, M. S. Strauss, S. Y. TI Construction of a fast ionization chamber for high-rate particle identification SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Gas-filled ionization chamber; Fast response; High-current heavy ion beams; Particle identification AB A new gas filled ionization chamber for high count rate particle identification has been constructed and commissioned at the Holifielcl Radioactive lon Beam Facility (RIME) at Oak Ridge National Laboratory (ORNL). To enhance the response Lime of the ionization chamber, a design utilizing a tilted entrance window and tilted electrodes was adopted, which is modified from art original design by Kimura et al. [1]. A maximum counting rate of 700,000 particles per second has been achieved. The detector has been used for several radioactive beam measurements performed at the HRIBF. (C) 2014 Elsevier BY. All rights reserved. C1 [Chae, K. Y.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Chae, K. Y.; Bardayan, D. W.; Chipps, K. A.; Pain, S. D.; Smith, M. S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Ahn, S.; Chipps, K. A.; Schmitt, K. T.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Bardayan, D. W.; Strauss, S. Y.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Chipps, K. A.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Manning, B.; Strauss, S. Y.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Peters, W. A.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. RP Chae, KY (reprint author), Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. EM kchae@skku.edu RI Pain, Steven/E-1188-2011; Peters, William/B-3214-2012; OI Pain, Steven/0000-0003-3081-688X; Peters, William/0000-0002-3022-4924; Chipps, Kelly/0000-0003-3050-1298 FU National Research Foundation of Korea (NRF) - Korea government (MEST) [NRF-2012R1A1A1041763]; US Department of Energy Office of Nuclear Physics [DE-AC05-00OR22725 (ORNL), DE-FG02-96ER40983, DE-SC0001174, DE-FG03-93ER40789]; National Nuclear Security Administration [DE-FG52-08NA28552] FX The authors wish to thank the staff members of the HRIBF for making this work possible. This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MEST) (No. NRF-2012R1A1A1041763), the US Department of Energy Office of Nuclear Physics under Contract nos. DE-AC05-00OR22725 (ORNL), DE-FG02-96ER40983 and DE-SC0001174 (University of Tennessee), DE-FG03-93ER40789 (Colorado School of Mines), and the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement no. DE-FG52-08NA28552. NR 15 TC 5 Z9 5 U1 1 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 1 PY 2014 VL 751 BP 6 EP 10 DI 10.1016/j.nima.2014.03.016 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AG0WD UT WOS:000335135500002 ER PT J AU Wang, CL Riedel, RA AF Wang, C. L. Riedel, R. A. TI Uniformity measurements and new positioning algorithms for wavelength-shifting fiber neutron detectors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Wavelength-shifting fiber neutron detector; Neutron diffraction; Quantum noise; Non-uniformity; Positioning algorithm; Gamma-ray sensitivity ID SCINTILLATION CAMERAS; LIGHT AB Wavelength-shifting (WLS) fiber scintillator detectors were successfully installed at two neutron powder diffractometers at the Spallation Neutron Source (SNS). However, they have the following second-order disadvantages: (i) they cannot have both high efficiency and images free of ghosting (position misassignment) concurrently; (ii) the apparent detection efficiency and spatial resolution are not uniform. These issues are related to the diffusion of scintillation photons and the fluctuation in the number of photons (quantum noise) collected by photo-multiplier tubes (PMTs). To mitigate these two issues, we developed two statistics-based positioning algorithms. i.e., a centroid algorithm (CEA) and a correlation algorithm (CA). Compared with the generally used maximum-photon algorithm (MPA), the CEA eliminates the ghosting with only about a 10% loss in detection efficiency, and provides better uniformity in detection efficiency and intrinsic background and lower gamma-ray sensitivity. The CA can effectively eliminate ghosting too, but the loss of efficiency at the group boundaries of PMTs is large. The results indicate that both algorithms can reduce the influence of quantum noise on the neutron positioning. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, C. L.; Riedel, R. A.] Oak Ridge Natl Lab, Neutron Sci Directorate, Instrument & Source Div, Oak Ridge, TN 37831 USA. RP Wang, CL (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Instrument & Source Div, Oak Ridge, TN 37831 USA. EM wangc@ornl.gov OI Wang, Cai-Lin/0000-0001-9745-2334 NR 19 TC 1 Z9 1 U1 1 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 1 PY 2014 VL 751 BP 55 EP 61 DI 10.1016/j.nima.2014.03.024 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AG0WD UT WOS:000335135500010 ER PT J AU Pawelczak, IA Glenn, AM Martinez, HP Carman, ML Zaitseva, NP Payne, A AF Pawelczak, I. A. Glenn, A. M. Martinez, H. P. Carman, M. L. Zaitseva, N. P. Payne, S. A. TI Boron-loaded plastic scintillator with neutron-gamma pulse shape discrimination capability SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE (10)Boron-loaded PSD plastic scintillator; Pulse shape discrimination; Thermal-neutron detection; Fast-neutron detection ID LIQUID SCINTILLATOR; DETECTORS AB Development of the plastic scintillator with neutron sensitivity from thermal to multi-MeV and pulse shape discrimination(PSD) has been demonstrated. Incorporation of B-10-containing compounds into the plastic scintillator with PSD capability leads to detector improvement in regard to neutron detection efficiency while preserving the discrimination between neutrons and gamma-rays. Effects of boron loading on scintillation and pulse shape discrimination properties are discussed. A PSD figure-of-merit value of 1.4 +/- 0.03 has been achieved for events in a thermal neutron energy domain, 50-100keV(ee), for PSD plastic loaded with 5 wt.% of m-carborane. (C) 2014 Elsevier B.V. All rights reserved. C1 [Pawelczak, I. A.; Glenn, A. M.; Martinez, H. P.; Carman, M. L.; Zaitseva, N. P.; Payne, S. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Pawelczak, IA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM pawelczak1@llnl.gov FU U.S.Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S.Department of Energy Office of Nonproliferation Research and Development [NA-22]; Defense and Thread Reduction Agency FX This work was performed under the auspices of the U.S.Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Financial support provided by the U.S.Department of Energy Office of Nonproliferation Research and Development (NA-22) and Defense and Thread Reduction Agency. The authors wish to thank Dr. Benjamin Rupert for preparation of liquid scintillator and Dr. Ronald Wurtz for valuable discussions. NR 20 TC 11 Z9 12 U1 0 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 1 PY 2014 VL 751 BP 62 EP 69 DI 10.1016/j.nima.2014.03.027 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AG0WD UT WOS:000335135500011 ER PT J AU Burr, T Hamada, MS Ticknor, L Weaver, B AF Burr, Tom Hamada, Michael S. Ticknor, Larry Weaver, Brian TI Model selection and change detection for a time-varying mean in process monitoring SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Approximate Bayesian computation; Model selection; Process monitoring residuals ID APPROXIMATE BAYESIAN COMPUTATION AB Process monitoring (PM) for nuclear safeguards sometimes requires estimation of thresholds corresponding to small false alarm rates. Thresholde stimation is an old topic; however, because possible new roles for PM are being evaluated in nuclear safeguards, it is timely to consider modern model selection options in the context of alarm threshold estimation. One of the possible new PM roles involves PM residuals, where a residual is defined as residual=data - prediction. This paper briefly reviews alarm threshold estimation, introduces model selection options, and considers several assumptions regarding the data-generating mechanism for PM residuals. Four PM examples from nuclear safeguards are included. One example involves frequent by-batch material balance closures where a dissolution vessel has time-varying efficiency, leading to time-varying material holdup. Another example involves periodic partial cleanout of in-process inventory, leading to challenging structure in the time series of PM residuals. Our main focus is model selection to select a defensible model for normal behavior with a time-varying mean in a PM residual stream. We use approximate Bayesian computation to perform the model selection and parameter estimation for normal behavior. We then describe a simple lag-one-differencing option similar to that used to monitor non-stationary times series to monitor for off-normal behavior. (C) 2014 Elsevier B.V. All rights reserved. C1 [Burr, Tom; Hamada, Michael S.; Ticknor, Larry; Weaver, Brian] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Burr, T (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM tburr@lanl.gov OI Ticknor, Lawrence/0000-0002-7967-7908 NR 31 TC 1 Z9 1 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 1 PY 2014 VL 751 BP 79 EP 87 DI 10.1016/j.nima.2014.03.023 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AG0WD UT WOS:000335135500013 ER PT J AU Wu, LZ Serpersu, EH AF Wu, Lingzhi Serpersu, Engin H. TI Erratum: "Deciphering interactions of the aminoglycoside phosphotransferase( 3')-IIIa with its ligands," Biopolymers 91( 9), 801- 809, ( 2009) SO BIOPOLYMERS LA English DT Correction C1 [Wu, Lingzhi; Serpersu, Engin H.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Wu, Lingzhi] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Wu, Lingzhi] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Serpersu, Engin H.] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA. [Serpersu, Engin H.] Oak Ridge Natl Lab, Knoxville, TN 37996 USA. RP Wu, LZ (reprint author), Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. NR 1 TC 0 Z9 0 U1 2 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0006-3525 EI 1097-0282 J9 BIOPOLYMERS JI Biopolymers PD JUL PY 2014 VL 101 IS 7 BP 819 EP 819 DI 10.1002/bip.22480 PG 1 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AF4KN UT WOS:000334681000011 ER PT J AU Tan, ECD Marker, TL Roberts, MJ AF Tan, Eric C. D. Marker, Terry L. Roberts, Michael J. TI Direct Production of Gasoline and Diesel Fuels from Biomass via Integrated Hydropyrolysis and Hydroconversion Process-A Techno- economic Analysis SO ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY LA English DT Article DE biomass to fuels; hydropyrolysis; gasoline; diesel; techno-economic analysis; process modeling ID LIGNOCELLULOSIC BIOMASS; FAST PYROLYSIS; TECHNOECONOMICS; GASIFICATION AB A techno-economic analysis (TEA) is performed to investigate the production of gasoline and diesel range hydrocarbon fuels by conversion of woody biomass via Gas Technology Institute (GTI)'s integrated hydropyrolysis plus hydroconversion (IH2) process. The processing capacity is 2000 dry metric tonnes (2205 dry US tons) of woody biomass per day. Major process areas include catalytic hydropyrolysis, catalytic hydroconversion, on-site hydrogen production, feedstock handling and storage, hydrocarbon absorber, sour water stripper, hydrogen sulfide scrubber, distillation tower, and all other operations support utilities. The TEA incorporates applicable commercial technologies, process modeling using Aspen HYSYS software, equipment cost estimation, and discounted cash flow analysis. The resulting minimum fuel selling price is $1.64 per gallon (or $1.68 per gallon of gasoline equivalent) in 2007 US dollars. The process yields 79 gallons of liquid fuels per dry US ton of woody biomass feedstock, for an annual fuel production rate of 61 million gallons at 96% on-stream time. The estimated total capital investment for an nth-plant is $264 million. A sensitivity analysis captures uncertainties in costs and plant performance. Results from this TEA can serve as the baseline for future comparison and as a basis for comparing this process to other biomass-to-liquid fuel pathways. (c) 2013 American Institute of Chemical Engineers Environ Prog, 33: 609-617, 2014 C1 [Tan, Eric C. D.] Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Marker, Terry L.; Roberts, Michael J.] Inst Gas Technol, Des Plaines, IL 60018 USA. RP Tan, ECD (reprint author), Natl Bioenergy Ctr, Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM eric.tan@nrel.gov FU US Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; DOE Cooperative Agreement [DE-EE-0002873] FX This work was supported by the US Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The work is based on joint work between NREL and GTI under NREL agreement number CRD-10-388. GTI would like to acknowledge funding of the research through DOE Cooperative Agreement DE-EE-0002873. The authors thank Sara Havig (NREL) for communications support. NR 23 TC 10 Z9 10 U1 6 U2 39 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1944-7442 EI 1944-7450 J9 ENVIRON PROG SUSTAIN JI Environ. Prog. Sustain. Energy PD JUL PY 2014 VL 33 IS 2 BP 609 EP 617 DI 10.1002/ep.11791 PG 9 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental; Engineering, Chemical; Engineering, Industrial; Environmental Sciences SC Science & Technology - Other Topics; Engineering; Environmental Sciences & Ecology GA AE9BL UT WOS:000334298800035 ER PT J AU Daldorff, LKS Toth, G Gombosi, TI Lapenta, G Amaya, J Markidis, S Brackbill, JU AF Daldorff, Lars K. S. Toth, Gabor Gombosi, Tamas I. Lapenta, Giovanni Amaya, Jorge Markidis, Stefano Brackbill, Jeremiah U. TI Two-way coupling of a global Hall magnetohydrodynamics model with a local implicit particle-in-cell model SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Plasma physics; MHD; PIC; Model coupling ID HYBRID DRIFT INSTABILITY; BLOCK-ADAPTIVE GRIDS; PLASMA SIMULATION; COLLISIONLESS DISSIPATION; MAGNETIC RECONNECTION; KINETIC SIMULATIONS; RADIATIVE SHOCKS; SPACE WEATHER; SCHEME; FIELD AB Computational models based on a fluid description of the plasma, such as magnetohydrodynamic (MHD) and extended magnetohydrodynamic (XMHD) codes are highly efficient, but they miss the kinetic effects due to the assumptions of small gyro radius, charge neutrality, and Maxwellian thermal velocity distribution. Kinetic codes can properly take into account the kinetic effects, but they are orders of magnitude more expensive than the fluid codes due to the increased degrees of freedom. If the fluid description is acceptable in a large fraction of the computational domain, it makes sense to confine the kinetic model to the regions where kinetic effects are important. This coupled approach can be much more efficient than a pure kinetic model. The speed up is approximately the volume ratio of the full domain relative to the kinetic regions assuming that the kinetic code uses a uniform grid. This idea has been advocated by [1] but their coupling was limited to one dimension and they employed drastically different grid resolutions in the fluid and kinetic models. We describe a fully two-dimensional two-way coupling of a Hall MHD model BATS-R-US with an implicit Particle-in-Cell (PIC) model iPIC3D. The coupling can be performed with identical grid resolutions and time steps. We call this coupled computational plasma model MHD-EPIC (MHD with Embedded PIC regions). Our verification tests show that MHD-EPIC works accurately and robustly. We show a two-dimensional magnetosphere simulation as an illustration of the potential future applications of MHD-EPIC. (C) 2014 Elsevier Inc. All rights reserved. C1 [Daldorff, Lars K. S.; Toth, Gabor; Gombosi, Tamas I.] Univ Michigan, Ctr Space Environm Modeling, Ann Arbor, MI 48109 USA. [Lapenta, Giovanni; Amaya, Jorge] Katholieke Univ Leuven, Louvain, Belgium. [Markidis, Stefano] KTH, Stockholm, Sweden. [Brackbill, Jeremiah U.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Toth, G (reprint author), Univ Michigan, Ctr Space Environm Modeling, Ann Arbor, MI 48109 USA. RI Daldorff, Lars/M-4117-2013; Toth, Gabor/B-7977-2013; Gombosi, Tamas/G-4238-2011; OI Daldorff, Lars/0000-0002-1198-5138; Toth, Gabor/0000-0002-5654-9823; Gombosi, Tamas/0000-0001-9360-4951; Lapenta, Giovanni/0000-0002-3123-4024 FU National Science Foundation [AGS-1322543]; European Commission [263340]; Interuniversity Attraction Poles Programme; Belgian Science Policy Office [IAP P7/08 CHARM] FX The work performed at the University of Michigan was supported by the National Science Foundation grant AGS-1322543. The research in support of iPic3D has been funded by the European Commission's Seventh Framework Programme (FP7/2007-2013) under the grant agreement SWIFF (project No. 263340, www.swiff.eu) and by the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (IAP P7/08 CHARM). NR 49 TC 22 Z9 23 U1 1 U2 14 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUL 1 PY 2014 VL 268 BP 236 EP 254 DI 10.1016/j.jcp.2014.03.009 PG 19 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AF3BP UT WOS:000334586800011 ER PT J AU Banks, JW Henshaw, WD Schwendeman, DW AF Banks, J. W. Henshaw, W. D. Schwendeman, D. W. TI An analysis of a new stable partitioned algorithm for FSI problems. Part II: Incompressible flow and structural shells SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Fluid-structure interaction; Added mass instability; Incompressible fluid flow; Structures; Shells; Beams ID FLUID-STRUCTURE PROBLEMS; OVERLAPPING GRIDS; EQUATIONS AB Stable partitioned algorithms for fluid-structure interaction (FSI) problems are developed and analyzed in this two-part paper. Part I describes an algorithm for incompressible flow coupled with compressible elastic solids, while Part II discusses an algorithm for incompressible flow coupled with structural shells. The numerical approach described here for structural shells uses Robin (mixed) interface conditions for the pressure and velocity in the fluid which are derived directly from the governing equations. The resulting added-mass partitioned (AMP) algorithm is stable even for very light structures, requires no subiterations per time step, and is second-order accurate. The stability and accuracy of the AMP algorithm is evaluated for linearized FSI model problems. A normal mode analysis is performed to show that the new AMP algorithm is stable, even for the case of very light structures when added-mass effects are large. Exact traveling wave solutions are derived for the FSI model problems, and these solutions are used to verify the stability and accuracy of the corresponding numerical results obtained from the AMP algorithm for the cases of light, medium and heavy structures. A summary comparison of the AMP algorithm developed here and the one in Part I is provided. (C) 2014 Elsevier Inc. All rights reserved. C1 [Banks, J. W.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. [Henshaw, W. D.; Schwendeman, D. W.] Rensselaer Polytech Inst, Dept Math Sci, Troy, NY 12180 USA. RP Henshaw, WD (reprint author), Rensselaer Polytech Inst, Dept Math Sci, 110 8th St, Troy, NY 12180 USA. EM banks20@llnl.gov; henshw@rpi.edu; schwed@rpi.edu RI Banks, Jeffrey/A-9718-2012 FU U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE contracts from the ASCR Applied Math Program; Lawrence Livermore National Laboratory [B548468]; National Science Foundation [DMS-1016188] FX This work was performed under the auspices of the U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and by DOE contracts from the ASCR Applied Math Program.; This research was supported by Lawrence Livermore National Laboratory under Subcontract B548468, and by the National Science Foundation under Grant DMS-1016188. NR 16 TC 9 Z9 9 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUL 1 PY 2014 VL 268 BP 399 EP 416 DI 10.1016/j.jcp.2014.03.004 PG 18 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AF3BP UT WOS:000334586800019 ER PT J AU Li, X Singh, RP Dudeck, KW Berchtold, KA Benicewicz, BC AF Li, Xin Singh, Rajinder P. Dudeck, Kevin W. Berchtold, Kathryn A. Benicewicz, Brian C. TI Influence of polybenzimidazole main chain structure on H-2/CO2 separation at elevated temperatures SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE Polybenzimidazole; Gas separation; Synthesis gas; Hydrogen separation membrane; Pre-combustion carbon capture ID MEMBRANE FUEL-CELLS; CARBON-DIOXIDE CAPTURE; IGCC POWER-PLANT; POLYMER ELECTROLYTE; HYDROGEN-PRODUCTION; POLYIMIDE MEMBRANES; GAS SEPARATIONS; CO2 CAPTURE; PBI; DMAC/LICL AB Four polybenzimidazole (PBI) derivatives were prepared to study the effects of main chain chemistry and structure on H-2/CO2 perm selectivity of cast films. These structural variations were designed to exhibit high localized mobility at elevated temperatures, contain rigid and bent configurations that frustrated close chain packing, or possess bulky side groups. The modified PBIs exhibited high molecular weights, slightly lower thermal stabilities, and higher organo-solubilities compared with commercial m-PBI. Dilute polymer solutions (< 3.0 wt%) were used to fabricate high quality thin films under carefully optimized film processing conditions. Gas permeation properties of these PBl films were evaluated aL elevated temperatures (up to 250 degrees C) and pressures (up to 50 psia). It was found that the main chain structural variations effectively disrupted the PBl chain packing resulting in much improved film H-2 permeability (up to 997.2 barrer) compared with m-PBI (76.81 barrer) at 250 degrees C and 50 psia. However, lower H-2/CO2 selectivities (5-7(modified PBIs) versus 23 (m-PBI) were also measured and reflected the general trade-off betvveen gas permeability and selectivity. When tested at 250 degrees C, PM -based materials exhibited gas separation performance higher than the Robeson upper bound prediction and are promising materials for high temperature H-2 separation horn syngas. (c) 2014 Elsevier B.V. All rights reserved. C1 [Li, Xin; Benicewicz, Brian C.] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Singh, Rajinder P.; Dudeck, Kevin W.; Berchtold, Kathryn A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Carbon Capture & Separat Energy Applicat CaSEA La, Los Alamos, NM 87545 USA. RP Benicewicz, BC (reprint author), Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. EM benice@sc.edu OI Benicewicz, Brian/0000-0003-4130-1232; Singh, Rajinder/0000-0003-4634-4290 FU U.S. DOE Energy Efficiency and Renewable Energy; Advanced Manufacturing Office; Industrial Technologies Program; Los Alamos National Laborator; Los Alamos National Security; DOE/NNSA [DE-AC52-06NA25396] FX This project supports the U.S. DOE Energy Efficiency and Renewable Energy-Advanced Manufacturing Office - Industrial Technologies Program. The authors gratefully acknowledge the U.S. DOE/EIRE for financial support of the project under Contract CPS #18990, Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for DOE/NNSA under Contract DE-AC52-06NA25396. The authors also acknowledge PBI Performance Products Inc. for their programmatic contributions. NR 41 TC 9 Z9 9 U1 8 U2 76 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 EI 1873-3123 J9 J MEMBRANE SCI JI J. Membr. Sci. PD JUL 1 PY 2014 VL 461 BP 59 EP 68 DI 10.1016/j.memsci.2014.03.008 PG 10 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA AF1YH UT WOS:000334509300007 ER PT J AU Layton, W Tran, H Trenchea, C AF Layton, W. Tran, H. Trenchea, C. TI Numerical analysis of two partitioned methods for uncoupling evolutionary MHD flows SO NUMERICAL METHODS FOR PARTIAL DIFFERENTIAL EQUATIONS LA English DT Article DE magnetohydrodynamics; finite element methods; partitioned methods ID FINITE-ELEMENT APPROXIMATION; INCOMPRESSIBLE MAGNETOHYDRODYNAMICS; STATIONARY; EQUATIONS; STABILITY; BLANKETS; BOUNDARY AB Magnetohydrodynamics (MHD) studies the dynamics of electrically conducting fluids, involving Navier-Stokes (NSE) equations in fluid dynamics and Maxwell equations in eletromagnetism. The physical processes of fluid flows and electricity and magnetism are quite different and numerical simulations of each subprocess can require different meshes, time steps, and methods. In most terrestrial applications, MHD flows occur at low-magnetic Reynold numbers. We introduce two partitioned methods to solve evolutionary MHD equations in such cases. The methods we study allow us at each time step to call NSE and Maxwell codes separately, each possibly optimized for the subproblem's respective physics. Complete error analysis and computational tests supporting the theory are given.Copyright (c) 2014 Wiley Periodicals, Inc. Numer Methods Partial Differential Eq 30: 1083-1102, 2014 C1 [Layton, W.; Trenchea, C.] Univ Pittsburgh, Dept Math, Pittsburgh, PA 15260 USA. [Tran, H.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Tran, H (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, 1 Bethel Valley Rd,POB 2008, Oak Ridge, TN 37831 USA. EM tranha@ornl.gov FU NSF grant [DMS1216465]; Air Force grant [9550-12-1-0191] FX Contract grant sponsor: NSF grant (W.L. and H.T.); contract grant number: DMS1216465; Contract grant sponsor: Air Force grant (W.L., H.T., and C.T.); contract grant number: 9550-12-1-0191 NR 22 TC 4 Z9 4 U1 1 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0749-159X EI 1098-2426 J9 NUMER METH PART D E JI Numer. Meth. Part Differ. Equ. PD JUL PY 2014 VL 30 IS 4 BP 1083 EP 1102 DI 10.1002/num.21857 PG 20 WC Mathematics, Applied SC Mathematics GA AF9CS UT WOS:000335013400001 ER PT J AU Shi, XB Cui, LS Jiang, DQ Yu, C Guo, FM Yu, MY Ren, Y Liu, YN AF Shi, Xiaobin Cui, Lishan Jiang, Daqiang Yu, Cun Guo, Fangmin Yu, Mengying Ren, Yang Liu, Yinong TI Grain size effect on the R-phase transformation of nanocrystalline NiTi shape memory alloys SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID EQUIATOMIC TINI ALLOY; MARTENSITIC-TRANSFORMATION; AT.PERCENT-NI; DEFORMATION; BEHAVIOR; TEM AB Development of nanoscale actuators and sensors in recent years calls for functional materials with small dimensions and high strengths. High strength nanocrystalline NiTi alloys which experience the R-phase transformation with a small thermal hysteresis are ideal candidates for these applications. To facilitate the application of the R-phase transformation in nanocrystalline NiTi alloys, this study investigated the effect of grain size on the R-phase transformation of a nanocrystalline Ti-50.2at.%Ni alloy. The nanometric grain size was created by severe cold deformation and low temperature anneal. It was found that in the recrystallized state, achieving nanoscale grain sizes (< 100 nm) was effective in suppressing the B2 -> B19' martensitic transformation and revealing the B2a dagger"R transformation. The B2a dagger"R transformation temperature was found to increase with the decreasing grain size within the range of 22-155 nm. The suppression of the B19' martensite in nanograins is attributed to the limited space within the grains to allow the formation of self-accommodation structures to contain the large lattice distortion of the martensite. C1 [Shi, Xiaobin; Cui, Lishan; Jiang, Daqiang; Yu, Cun; Guo, Fangmin; Yu, Mengying] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Liu, Yinong] Univ Western Australia, Sch Mech & Chem Engn, Crawley, WA 6009, Australia. RP Shi, XB (reprint author), China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. EM shyllen@sina.com RI Liu, Yinong/G-6637-2011; Jiang, Daqiang /G-5511-2014 OI Liu, Yinong/0000-0002-8784-8543; FU Natural Science Foundation of China (NSFC) [51231008]; Australian Research Council [DP140103805]; National 973 Programs of China [2012CB619400]; US Department of Energy, Office of Science [DE-AC02-06CH11357]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Natural Science Foundation of China (NSFC) (key program project 51231008), Australian Research Council (Grant No. DP140103805), and National 973 Programs of China (2012CB619400). The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, and Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 20 TC 6 Z9 6 U1 0 U2 55 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD JUL PY 2014 VL 49 IS 13 BP 4643 EP 4647 DI 10.1007/s10853-014-8167-6 PG 5 WC Materials Science, Multidisciplinary SC Materials Science GA AF1RW UT WOS:000334492000028 ER PT J AU Neubauer, J Wood, E AF Neubauer, Jeremy Wood, Eric TI The impact of range anxiety and home, workplace, and public charging infrastructure on simulated battery electric vehicle lifetime utility SO JOURNAL OF POWER SOURCES LA English DT Article DE Battery Lifetime Analysis and Simulation; Tool for Vehicles; Range anxiety; Electric vehicle; Workplace charging; Public charging; Fast charging AB Battery electric vehicles (BEVs) offer the potential to reduce both oil imports and greenhouse gas emissions, but have a limited utility due to factors including driver range anxiety and access to charging infrastructure. In this paper we apply NREL's Battery Lifetime Analysis and Simulation Tool for Vehicles (BLAST-V) to examine the sensitivity of BEV utility to range anxiety and different charging infrastructure scenarios, including variable time schedules, power levels, and locations (home, work, and public installations). We find that the effects of range anxiety can be significant, but are reduced with access to additional charging infrastructure. We also find that (1) increasing home charging power above that provided by a common 15 A, 120 V circuit offers little added utility, (2) workplace charging offers significant utility benefits to select high mileage commuters, and (3) broadly available public charging can bring many lower mileage drivers to near-100% utility while strongly increasing the achieved miles of high mileage drivers. (C) 2014 Elsevier B.V. All rights reserved. C1 [Neubauer, Jeremy; Wood, Eric] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Neubauer, J (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Jeremy.neubauer@nrel.gov FU Dave Howell and Brian Cunningham of the Energy Storage, Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy; U.S. Department of Energy's Vehicle Technologies Program FX This study was supported by Dave Howell and Brian Cunningham of the Energy Storage, Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy. The use of the battery degradation and FASTSim tools, both developed at the National Renewable Energy Laboratory under funding from the U.S. Department of Energy's Vehicle Technologies Program, was critical to the completion of this study. Special thanks to Kandler Smith for developing and supporting the integration of the battery degradation model, and Ahmad Pesaran, the National Renewable Energy Laboratory's Energy Storage team leader, for his continual guidance. NR 7 TC 24 Z9 24 U1 2 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUL 1 PY 2014 VL 257 BP 12 EP 20 DI 10.1016/j.jpowsour.2014.01.075 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AE2CD UT WOS:000333780000002 ER PT J AU Cao, WJ Shih, J Zheng, JP Doung, T AF Cao, W. J. Shih, J. Zheng, J. P. Doung, T. TI Development and characterization of Li-ion capacitor pouch cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Li-ion capacitor; Pouch cells; Activated carbon; Hard carbon; SLMP; Pore size distribution ID HYBRID ELECTROCHEMICAL CAPACITOR; ENERGY DENSITY; NEGATIVE ELECTRODES; CYCLE PERFORMANCE; LAYER CAPACITOR; SOFT CARBON; IMPROVEMENT; CATHODE AB High energy density Li-ion capacitor (LIC) pouch cell prototypes were assembled with lab-scale equipment using activated carbon cathode and hard carbon/lithium stabilized metal power (SLMP) anode. The specific energy and energy density as high as 30 Wh kg(-1) and 39 Wh L-1 have been achieved, respectively. The pouch cells can deliver over 50% of the maximum stored energy at a discharge rate over 100 Crate. After 10,000 cycles, the LIC pouch cell still has 80% of the initial capacitance. The average leakage current is 0.3 mu A cm(-2) during the first 72 h. (C) 2014 Published by Elsevier B.V. C1 [Cao, W. J.; Shih, J.; Zheng, J. P.] Florida A&M Univ, Dept Elect & Comp Engn, Tallahassee, FL 32310 USA. [Cao, W. J.; Shih, J.; Zheng, J. P.] Florida State Univ, Tallahassee, FL 32310 USA. [Cao, W. J.; Shih, J.; Zheng, J. P.] Florida State Univ, Aeropropuls Mechatron & Energy AME Ctr, Tallahassee, FL 32310 USA. [Zheng, J. P.] Florida State Univ, CAPS, Tallahassee, FL 32310 USA. [Doung, T.] US DOE, Off Vehicle Technol, Annandale, VA 22003 USA. RP Zheng, JP (reprint author), Florida State Univ, CAPS, Tallahassee, FL 32310 USA. EM zheng@eng.fsu.edu FU DOE BAIT Program through PNNL [212964]; Florida State University Research Foundation GAPS Program FX This study is supported by DOE BAIT Program through PNNL with contract No. 212964 and Florida State University Research Foundation GAPS Program. NR 23 TC 20 Z9 20 U1 8 U2 86 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUL 1 PY 2014 VL 257 BP 388 EP 393 DI 10.1016/j.jpowsour.2014.01.087 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AE2CD UT WOS:000333780000050 ER PT J AU Chou, YS Stevenson, JW Choi, JP AF Chou, Yeong-Shyung Stevenson, Jeffry W. Choi, Jung-Pyung TI Long-term evaluation of solid oxide fuel cell candidate materials in a 3-cell generic stack test fixture, part III: Stability and microstructure of Ce-(Mn,Co)-spinel coating, AISI441 interconnect, alumina coating, cathode and anode SO JOURNAL OF POWER SOURCES LA English DT Article DE Sealing glass; AISI441; Aluminization; (Mn,Co)-spinel; SOFC ID FERRITIC STAINLESS-STEEL; (MN,CO)(3)O-4 SPINEL COATINGS; OXIDATION BEHAVIOR; CHEMICAL COMPATIBILITY; SEALING GLASSES; SOFC CATHODES; CR; TEMPERATURE; PERFORMANCE; ALLOYS AB A generic solid oxide fuel cell stack test fixture was developed to evaluate candidate materials and processing under realistic conditions. Part III of the work investigated the stability of Ce-(Mn,Co) spinel coating, AISI441 metallic interconnect, alumina coating, and cell's degradation. After 6000 h test, the spinel coating showed densification with some diffusion of Cr. At the metal interface, segregation of Si and Ti was observed, however, no continuous layer formed. The alumina coating for perimeter sealing areas appeared more dense and thick at the air side than the fuel side. Both the spinel and alumina coatings remained bonded. EDS analysis of Cr within the metal showed small decrease in concentration near the coating interface and would expect to cause no issue of Cr depletion. Inter-diffusion of Ni, Fe, and Cr between spot-welded Ni wire and AISI441 interconnect was observed and Cr-oxide scale formed along the circumference of the weld. The microstructure of the anode and cathode was discussed relating to degradation of the top and middle cells. Overall, the Ce-(Mn,Co) spinet coating, alumina coating, and AISI441 steel showed the desired long-term stability and the developed generic stack fixture proved to be a useful tool to validate candidate materials for SOFC. (C) 2013 Published by Elsevier B.V. C1 [Chou, Yeong-Shyung; Stevenson, Jeffry W.; Choi, Jung-Pyung] Pacific NW Natl Lab, Energy & Efficiency Div, Richland, WA 99354 USA. RP Chou, YS (reprint author), Pacific NW Natl Lab, Energy & Efficiency Div, K2-44,POB 999, Richland, WA 99354 USA. EM yeong-shyung.chou@pnnl.gov FU US Department of Energy's Solid-State Energy Conversion Alliance (SECA) Core Technology Program; [DE-AC06-76RL0 1830] FX The authors would like to thank S. Carlson for SEM sample preparation, and J. Coleman for SEM analysis. The work summarized in this paper was funded by the US Department of Energy's Solid-State Energy Conversion Alliance (SECA) Core Technology Program. The authors would like to thank Shailesh Vora, Briggs White, Patcharin Burke, and Joe Stoffa from National Energy Technology Laboratory for helpful discussions. Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the US Department of Energy under Contract no. DE-AC06-76RL0 1830. NR 40 TC 4 Z9 4 U1 5 U2 70 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUL 1 PY 2014 VL 257 BP 444 EP 453 DI 10.1016/j.jpowsour.2013.11.086 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AE2CD UT WOS:000333780000055 ER PT J AU Grasso, S Tatarko, P Rizzo, S Porwal, H Hu, CF Katoh, Y Salvo, M Reece, MJ Ferraris, M AF Grasso, Salvatore Tatarko, Peter Rizzo, Stefano Porwal, Harshit Hu, Chunfeng Katoh, Yutai Salvo, Milena Reece, Michael J. Ferraris, Monica TI Joining of beta-SiC by spark plasma sintering SO JOURNAL OF THE EUROPEAN CERAMIC SOCIETY LA English DT Article DE beta-SiC; Joining; Spark plasma sintering ID SILICON-CARBIDE; TEMPERATURE; STRENGTH; DEPOSITION; CERAMICS; ALUMINUM AB Spark plasma sintering (SPS) was employed to join monolithic beta-SiC with or without titanium as intermediate joining material. Both the localized and rapid heating contributed to the inherent energy saving of electric current assisted joining technique. The effects of uniaxial pressure and surface preparation were analyzed independently with respect to the flexural strength and the morphology of the joints. In particular samples polished down to 1 mu m and joined at 1900 degrees C for 5 min achieved the strength of the as received material. The failure occurred outside the joining interface, confirming the optimum quality of the joint. Pressure in combination with surface preparation was necessary to achieve perfect adhesion and pore free direct joining of SiC. The use of Ti foil as a joining material and pressure allowed joining of unpolished SiC. Crown Copyright (C) 2013 Published by Elsevier Ltd. All rights reserved. C1 [Grasso, Salvatore; Porwal, Harshit; Reece, Michael J.] Queen Mary Univ London, Sch Engn & Mat Sci, London E1 4NS, England. [Grasso, Salvatore; Porwal, Harshit; Reece, Michael J.] Queen Mary Univ London, Nanoforce Technol Ltd, London E1 4NS, England. [Tatarko, Peter] Acad Sci Czech Republic, Inst Phys Mat, Brno 61662, Czech Republic. [Rizzo, Stefano; Salvo, Milena; Ferraris, Monica] Politecn Torino, Inst Mat Phys & Engn, Dept Appl Sci & Technol, I-10129 Turin, Italy. [Hu, Chunfeng] Chinese Acad Sci, NIMTE, Ningbo 315201, Zhejiang, Peoples R China. [Katoh, Yutai] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Grasso, S (reprint author), Queen Mary Univ London, Nanoforce Technol Ltd, Joseph Priestley Bldg,Mile End Rd, London E1 4NS, England. EM s.grasso@nanoforce.co.uk RI Porwal, Harshit/K-6738-2014; Tatarko, Peter/F-1446-2016 OI Porwal, Harshit/0000-0002-4817-6545; FU European Union [264526] FX The research leading to these results was supported by the European Union's Seventh Framework Programme managed by REA-Research Executive Agency (http://www.ec.europa.eu/research/rea) (Marie Curie Action, GlaCERCo GA 264526). NR 25 TC 12 Z9 13 U1 0 U2 49 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0955-2219 EI 1873-619X J9 J EUR CERAM SOC JI J. Eur. Ceram. Soc. PD JUL PY 2014 VL 34 IS 7 BP 1681 EP 1686 DI 10.1016/j.jeurceramsoc.2013.12.023 PG 6 WC Materials Science, Ceramics SC Materials Science GA AD8CD UT WOS:000333493200004 ER PT J AU Remillieux, MC Anderson, BE Le Bas, PY Ulrich, TJ AF Remillieux, Marcel C. Anderson, Brian E. Le Bas, Pierre-Yves Ulrich, T. J. TI Improving the air coupling of bulk piezoelectric transducers with wedges of power-law profiles: A numerical study SO ULTRASONICS LA English DT Article DE Piezoelectric transducers; Air-coupled ultrasound; Acoustic-structure interaction; Finite-element analysis; Time-reversed acoustics ID CHANNEL TIME-REVERSAL; NONDESTRUCTIVE EVALUATION; ULTRASONIC TRANSDUCERS; CHAOTIC CAVITIES; FLEXURAL WAVES; ACOUSTICS; PLATES AB An air-coupled ultrasonic transducer is created by bonding a bulk piezoelectric element onto the surface of a thick plate with a wedge of power-law profile. The wedge is used to improve the ultrasonic radiation efficiency. The power-law profile provides a smooth, impedance-matching transition for the mechanical energy to be transferred from the thick plate to the air, through the large-amplitude flexural waves observed in the thinnest region of the wedge. The performance of the proposed transducer is examined numerically and compared to that of a design where the piezoelectric element is isolated and where it is affixed to a thin plate of uniform thickness. The numerical analysis is first focused on the free-field radiation of the transducers. Then, time-reversal experiments are simulated by placing the transducers inside a cavity of arbitrary shape with some perfectly reflecting boundaries. In addition to time-reversal mirrors, the proposed concept could be integrated in the design of phased arrays and parametric arrays. Published by Elsevier B.V. C1 [Remillieux, Marcel C.; Anderson, Brian E.; Le Bas, Pierre-Yves; Ulrich, T. J.] Los Alamos Natl Lab, Geophys Grp EES 17, Los Alamos, NM 87545 USA. RP Remillieux, MC (reprint author), Los Alamos Natl Lab, Geophys Grp EES 17, MS D446, Los Alamos, NM 87545 USA. EM mcr1@lanl.gov; bea@lanl.gov; pylb@lanl.gov; tju@lanl.gov NR 30 TC 4 Z9 4 U1 5 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0041-624X EI 1874-9968 J9 ULTRASONICS JI Ultrasonics PD JUL PY 2014 VL 54 IS 5 BP 1409 EP 1416 DI 10.1016/j.ultras.2014.02.017 PG 8 WC Acoustics; Radiology, Nuclear Medicine & Medical Imaging SC Acoustics; Radiology, Nuclear Medicine & Medical Imaging GA AE1XK UT WOS:000333766300035 PM 24636675 ER PT J AU Calderon-Moreno, JM Pol, VG Suh, SH Shin, HK Popa, M AF Calderon-Moreno, J. M. Pol, V. G. Suh, S. -H. Shin, H. -K. Popa, M. TI Formation Mechanism and Red Light Emission Photoluminescence of Single-Phase Crystalline Eu2O2CO3 Nanoplates Compared with Y2O3:Eu Phosphor SO JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY LA English DT Article DE Phosphor; Nanoplate; Photoluminescence; Crystalline ID LUMINESCENCE PROPERTIES; THERMAL-DECOMPOSITION; FACILE SYNTHESIS; NANOPARTICLES; EU2O3; OXYCARBONATE; SUPERSTRUCTURES; NANOCRYSTALS; FABRICATION; SYMMETRY AB The photoluminescence properties and formation mechanism of a novel stoichiometric phosphor are presented. Nanoplates of pure single-phase crystalline Eu2O2CO3 oxycarbonate (hexagonal type-II) were synthesized by dry autoclaving under autogenic pressure (under 3 MPa) using an efficient, high yield solid state green-chemistry route that can be extended to other rare-earth oxycarbonate and oxide systems, resulting in the full conversion of a simple commercial precursor in single-crystalline nanoplates with strong visible luminescence. Phosphors made of an oxide host and an active luminescent dopant ion are the commercial standard (i.e., Y2O3:Eu). It is generally considered that the activity of luminescent species, such as Eu3+, is quenched and disappears above a certain concentration of them in the lattice (concentration quenching). The truly stoichoimetric oxycarbonate phosphor without active dopant ions exhibits very strong red emission when excited by different excitations, in the UV and visible range, without any concentration quenching effect. The bright red light emission spectra of the of the photo-excited phosphor nanoplates under UV and visible light excitation is compared with that of a standard Y2O3:Eu commercial red phosphor powder, and the thermal conversion mechanism is proposed to obtain the single-phase stable stoichiometric oxycarbonate nanoplates. C1 [Calderon-Moreno, J. M.] Acad Romana, Inst Phys Chem IG Murgulescu, Dept Surface Chem & Catalysis, Bucharest, Romania. [Pol, V. G.] Argonne Natl Lab, Chem Sci & Engn Div, Electrochem Energy Storage Dept, Argonne, IL 60439 USA. [Suh, S. -H.] Keimyung Univ, Dept Chem Engn, Taegu 704701, South Korea. [Shin, H. -K.] Natl Ctr Namomat Technol, Pohang 790784, South Korea. [Popa, M.] Acad Romana, Inst Phys Chem IG Murgulescu, Dept Phys Chem Oxide Mat, Bucharest, Romania. RP Suh, SH (reprint author), Keimyung Univ, Dept Chem Engn, Taegu 704701, South Korea. RI Calderon Moreno, Jose/B-2867-2008 OI Calderon Moreno, Jose/0000-0001-8376-9082 NR 37 TC 1 Z9 1 U1 0 U2 30 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1533-4880 EI 1533-4899 J9 J NANOSCI NANOTECHNO JI J. Nanosci. Nanotechnol. PD JUL PY 2014 VL 14 IS 7 BP 5473 EP 5479 DI 10.1166/jnn.2014.8408 PG 7 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AD0LV UT WOS:000332926400111 PM 24758052 ER PT J AU Bolotnikov, AE Camarda, GS Cui, Y De Geronimo, G Fried, J Hossain, A Lee, K Mahler, G Maritato, M Marshall, M Petryk, M Roy, U Vernon, E Yang, G James, RB AF Bolotnikov, A. E. Camarda, G. S. Cui, Y. De Geronimo, G. Fried, J. Hossain, A. Lee, K. Mahler, G. Maritato, M. Marshall, M. Petryk, M. Roy, U. Vernon, E. Yang, G. James, R. B. TI Use of high-granularity position sensing to correct response non-uniformities of CdZnTe detectors SO APPLIED PHYSICS LETTERS LA English DT Article ID CZT DETECTORS; SENSITIVE DETECTORS; READOUT; PERFORMANCE AB CdZnTe (CZT) is a promising medium for room-temperature gamma-ray detectors. However, the low production yield of acceptable quality crystals hampers the use of CZT detectors for gamma-ray spectroscopy. Significant efforts have been directed towards improving quality of CZT crystals to make them generally available for radiation detectors. Another way to address this problem is to implement detector designs that would allow for more accurate and predictable correction of the charge loss associated with crystal defects. In this work, we demonstrate that high-granularity position-sensitive detectors can significantly improve the performance of CZT detectors fabricated from CZT crystals with wider acceptance boundaries, leading to an increase of their availability and expected decrease in cost. (C) 2014 AIP Publishing LLC. C1 [Bolotnikov, A. E.; Camarda, G. S.; Cui, Y.; De Geronimo, G.; Fried, J.; Hossain, A.; Mahler, G.; Maritato, M.; Marshall, M.; Roy, U.; Vernon, E.; Yang, G.; James, R. B.] Brookhaven Natl Lab, Dept Nonproliferat & Natl Secur, Upton, NY 11793 USA. [Lee, K.] Korea Univ, Seoul 136855, South Korea. [Petryk, M.] SUNY Binghamton, Binghamton, NY 13902 USA. RP Bolotnikov, AE (reprint author), Brookhaven Natl Lab, Dept Nonproliferat & Natl Secur, Upton, NY 11793 USA. EM bolotnik@bnl.gov FU U.S. Department of Energy, Office of Nonproliferation and Verification Research and Development [NA-22]; U.S. Defense Threat Reduction Agency (DTRA); BNL's Technology Maturation Award; Brookhaven Science Associates, LLC [DE-AC02-98CH1-886] FX This work was supported by U.S. Department of Energy, Office of Nonproliferation and Verification Research and Development, NA-22, U.S. Defense Threat Reduction Agency (DTRA) and BNL's Technology Maturation Award. The manuscript has been authored by Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH1-886 with the U.S. Department of Energy. The United States Government retains, and the publisher, by accepting the article for publication, acknowledges, a world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. NR 16 TC 8 Z9 8 U1 4 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 263503 DI 10.1063/1.4883402 PG 5 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100062 ER PT J AU Hu, ZQ Ma, BH Koritala, RE Balachandran, U AF Hu, Zhongqiang Ma, Beihai Koritala, R. E. Balachandran, Uthamalingam TI Temperature-dependent energy storage properties of antiferroelectric Pb0.96La0.04Zr0.98Ti0.02O3 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROELECTRIC CERAMICS; DIELECTRIC-PROPERTIES; CAPACITORS AB The energy storage properties of antiferroelectric (AFE) Pb0.96La0.04Zr0.98Ti0.02O3 (PLZT 4/98/2) thin films were investigated as a function of temperature and applied electric field. The results indicated that recoverable energy density (U-re) and charge-discharge efficiency (eta) of PLZT (4/98/2) depend weakly on temperature (from room temperature to 225 degrees C), while U-re increases linearly and eta decreases exponentially with increasing electric field at room temperature. These findings are explained qualitatively on the basis of the kinetics of the temperature-induced transition of AFE-to-paraelectric phase and the field-induced transition of AFE-to-ferroelectric phase, respectively. The high U-re (approximate to 61 J/cm(3)) and low leakage current density (approximate to 3.5 x 10(-8) and 3.5 x 10(-5) A/cm(2) at 25 and 225 degrees C, respectively) indicate that antiferroelectric PLZT (4/98/2) is a promising material for high-power energy storage. (C) 2014 AIP Publishing LLC. C1 [Hu, Zhongqiang; Ma, Beihai; Balachandran, Uthamalingam] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Koritala, R. E.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. RP Ma, BH (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM bma@anl.gov RI Ma, Beihai/I-1674-2013; Hu, Zhongqiang/I-2528-2012 OI Ma, Beihai/0000-0003-3557-2773; Hu, Zhongqiang/0000-0002-7534-0427 FU U.S. Department of Energy, Vehicle Technologies Program [DE-AC02-06CH11357]; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This work was funded by the U.S. Department of Energy, Vehicle Technologies Program, under Contract No. DE-AC02-06CH11357. This work benefited from use of the Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 24 TC 30 Z9 30 U1 9 U2 96 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 263902 DI 10.1063/1.4887066 PG 4 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100076 ER PT J AU Lee, B Nakhmanson, SM Heinonen, O AF Lee, Byounghak Nakhmanson, Serge M. Heinonen, Olle TI Strain induced vortex-to-uniform polarization transitions in soft-ferroelectric nanoparticles SO APPLIED PHYSICS LETTERS LA English DT Article ID REAL-SPACE OBSERVATION; PHASE-TRANSITIONS; SKYRMION LATTICE; THIN-FILMS; CRYSTAL; STATES AB Domain structures of ferroelectric polarization in patterned nanostructures depend sensitively on an interplay between their geometry and crystallographic anisotropy. In the recently predicted layered perovskite PbSr2Ti2O7 [S. M. Nakhmanson and I. Naumov, Phys. Rev. Lett. 104, 097601 (2010)], the in-plane anisotropy can be controlled by strain to be along in-plane [110]-directions or to vanish, in which case the polarization is free to rotate in the perovskite-layer. Using a microscopic Landau-Ginzburg-Devonshire free energy functional theory, we demonstrate that the domain structure in patterned disks of PbSr2Ti2O7 can be varied between uniform polarization and a vortex structure, analogous to vortices in soft magnetic disks. This opens up the possibility of designing nanostructured layered materials whose dielectric response can be manipulated with small elastic distortions. (C) 2014 AIP Publishing LLC. C1 [Lee, Byounghak] Texas State Univ, Dept Phys, San Marcos, TX 78666 USA. [Nakhmanson, Serge M.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Nakhmanson, Serge M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Heinonen, Olle] Argonne Natl Lab, Lemont, IL 60439 USA. [Heinonen, Olle] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Lee, B (reprint author), Texas State Univ, Dept Phys, San Marcos, TX 78666 USA. EM byounghak@txstate.edu OI Heinonen, Olle/0000-0002-3618-6092 FU UChicago Argonne, LLC. [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX S.M.N. is grateful to G. Brian Stephenson for many useful discussions. Argonne National Laboratory is operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. Part of the work by O.H. was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 44 TC 4 Z9 4 U1 9 U2 38 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 262906 DI 10.1063/1.4887068 PG 5 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100049 ER PT J AU Li, J Tan, A Moon, KW Doran, A Marcus, MA Young, AT Arenholz, E Ma, S Yang, RF Hwang, C Qiu, ZQ AF Li, J. Tan, A. Moon, K. W. Doran, A. Marcus, M. A. Young, A. T. Arenholz, E. Ma, S. Yang, R. F. Hwang, C. Qiu, Z. Q. TI Stabilizing a magnetic vortex/antivortex array in single crystalline Fe/Ag(001) microstructures SO APPLIED PHYSICS LETTERS LA English DT Article ID DOMAIN-WALL; DYNAMICS AB While a magnetic antivortex state can be created in ring structures, much effort has been devoted to stabilizing a magnetic antivortex as the ground state in a single island. Among many proposals, less attention has been paid to the role of magnetocrystalline anisotropy because most magnetic microstructures are made of polycrystalline materials. By patterning epitaxial Fe/Ag(001) films along different in-plane directions, we show that the Fe magnetocrystalline anisotropy plays a very important role in stabilizing different types of vortex/antivortex states. In particular, we find that an Fe island in the shape of an elongated hexagon favors vortex array formation when the long edge is parallel to the Fe easy magnetization axis, and favors the vortex-antivortex array formation when the long edge is parallel to the Fe hard magnetization axis. (C) 2014 AIP Publishing LLC. C1 [Li, J.; Tan, A.; Ma, S.; Yang, R. F.; Qiu, Z. Q.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Moon, K. W.; Hwang, C.] Korea Res Inst Stand & Sci, Taejon 305340, South Korea. [Doran, A.; Marcus, M. A.; Young, A. T.; Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Li, J (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Qiu, Zi Qiang/O-4421-2016 OI Qiu, Zi Qiang/0000-0003-0680-0714 FU National Science Foundation NRF through Global Research Laboratory project of Korea [DMR-1210167]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; China Scholarship Council FX Financial support through National Science Foundation DMR-1210167 NRF through Global Research Laboratory project of Korea is gratefully acknowledged. The operations of the Advanced Light Source at Lawrence Berkeley National Laboratory are supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under contract number DE-AC02-05CH11231. S.M. and R.F.Y. acknowledge the fellowship support from China Scholarship Council. NR 43 TC 2 Z9 2 U1 1 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 262409 DI 10.1063/1.4887345 PG 5 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100041 ER PT J AU Piot, P Brau, CA Choi, BK Blomberg, B Gabella, WE Ivanov, B Jarvis, J Mendenhall, MH Mihalcea, D Panuganti, H Prieto, P Reid, J AF Piot, P. Brau, C. A. Choi, B. K. Blomberg, B. Gabella, W. E. Ivanov, B. Jarvis, J. Mendenhall, M. H. Mihalcea, D. Panuganti, H. Prieto, P. Reid, J. TI Operation of an ungated diamond field-emission array cathode in a L-band radiofrequency electron source SO APPLIED PHYSICS LETTERS LA English DT Article ID CARBON NANOTUBES AB We report on the operation of a field-emitter-array cathode in a conventional L-band radio-frequency electron source. The cathode consisted of an array of similar to 10(6) diamond tips on pyramids. Maximum current on the order of 15 mA was reached and the cathode did not show appreciable signs of fatigue after weeks of operation. The measured Fowler-Nordheim characteristics, transverse beam density, and current stability are discussed. (C) 2014 AIP Publishing LLC. C1 [Piot, P.; Blomberg, B.; Mihalcea, D.; Panuganti, H.] No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. [Piot, P.; Blomberg, B.; Mihalcea, D.; Panuganti, H.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Piot, P.] Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, Batavia, IL 60510 USA. [Brau, C. A.; Gabella, W. E.; Ivanov, B.; Mendenhall, M. H.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Choi, B. K.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA. [Choi, B. K.] Vanderbilt Univ, Vanderbilt Inst Nanoscale Sci & Engn, Nashville, TN 37235 USA. [Jarvis, J.] Adv Energy Syst Inc, Medford, NY 11763 USA. [Prieto, P.; Reid, J.] Fermilab Natl Accelerator Lab, Accelerator Div, Batavia, IL 60510 USA. RP Piot, P (reprint author), No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. OI Choi, Bo K./0000-0002-4984-5958; Ivanov, Borislav/0000-0003-1837-6113 FU DARPA [AXIS N66001-11-1-4196]; Vanderbilt University; DOE [DE-AC02-07CH11359]; Fermi Research Alliance, LLC; Northern Illinois University [DE-FG02-08ER41532] FX We are indebted to M. Church, E. Harms, E. Lopez, J. Santucci, and V. Shiltsev for their support. This work was supported by the DARPA Axis contract AXIS N66001-11-1-4196 with Vanderbilt University, DOE Contract No. DE-AC02-07CH11359 with the Fermi Research Alliance, LLC and No. DE-FG02-08ER41532 with Northern Illinois University. NR 17 TC 9 Z9 10 U1 0 U2 13 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 263504 DI 10.1063/1.4884375 PG 4 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100063 ER PT J AU Zubelewicz, A AF Zubelewicz, Aleksander TI Conditions for the coexistence of liquid-like and solid-like behaviors in viscoelastic liquids (vol 104, 151905, 2014) SO APPLIED PHYSICS LETTERS LA English DT Correction C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zubelewicz, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. NR 1 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 30 PY 2014 VL 104 IS 26 AR 269903 DI 10.1063/1.4886976 PG 1 WC Physics, Applied SC Physics GA AL4PE UT WOS:000339114100082 ER PT J AU Stringfellow, WT Domen, JK Camarillo, MK Sandelin, WL Borglin, S AF Stringfellow, William T. Domen, Jeremy K. Camarillo, Mary Kay Sandelin, Whitney L. Borglin, Sharon TI Physical, chemical, and biological characteristics of compounds used in hydraulic fracturing SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Review DE Hydraulic fracturing; Unconventional oil and gas; Chemicals, biocides, crosslinkers ID MARCELLUS SHALE; ACTIVATED-SLUDGE; WATER MANAGEMENT; GAS PLAYS; GUAR GUM; BIODEGRADATION; DEGRADATION; 2,2-DIBROMO-3-NITRILOPROPIONAMIDE; POLYACRYLAMIDE; GLUTARALDEHYDE AB Hydraulic fracturing (HF), a method to enhance oil and gas production, has become increasingly common throughout the U.S. As such, it is important to characterize the chemicals found in HF fluids to evaluate potential environmental fate, including fate in treatment systems, and human health impacts. Eighty-one common HF chemical additives were identified and categorized according to their functions. Physical and chemical characteristics of these additives were determined using publicly available chemical information databases. Fifty-five of the compounds are organic and twenty-seven of these are considered readily or inherently biodegradable. Seventeen chemicals have high theoretical chemical oxygen demand and are used in concentrations that present potential treatment challenges. Most of the HF chemicals evaluated are non-toxic or of low toxicity and only three are classified as Category 2 oral toxins according to standards in the Globally Harmonized System of Classification and Labeling of Chemicals; however, toxicity information was not located for thirty of the HF chemicals evaluated. Volatilization is not expected to be a significant exposure pathway for most HF chemicals. Gaps in toxicity and other chemical properties suggest deficiencies in the current state of knowledge, highlighting the need for further assessment to understand potential issues associated with HF chemicals in the environment. (C) 2014 Elsevier B.V. All rights reserved. C1 [Stringfellow, William T.; Domen, Jeremy K.; Camarillo, Mary Kay; Sandelin, Whitney L.] Univ Pacific, Sch Engn & Comp Sci, Ecol Engn Res Program, Stockton, CA 95211 USA. [Stringfellow, William T.; Borglin, Sharon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Stringfellow, WT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wstringfellow@lbl.gov RI Stringfellow, William/O-4389-2015; Borglin, Sharon/I-1013-2016 OI Stringfellow, William/0000-0003-3189-5604; FU Lawrence Berkeley National Laboratory under its U.S. Department of Energy [DE-AC02-05CH11231]; University of the Pacific, School of Engineering and Computer Science FX The work was completed by the Ecological Engineering Research Program with funding from the University of the Pacific, School of Engineering and Computer Science. Part of this work was conducted at Lawrence Berkeley National Laboratory under its U.S. Department of Energy contract DE-AC02-05CH11231. NR 118 TC 44 Z9 45 U1 25 U2 189 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JUN 30 PY 2014 VL 275 BP 37 EP 54 DI 10.1016/j.jhazmat.2014.04.040 PG 18 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AL5AU UT WOS:000339146700006 PM 24853136 ER PT J AU Benedict, LX Driver, KP Hamel, S Militzer, B Qi, TT Correa, AA Saul, A Schwegler, E AF Benedict, Lorin X. Driver, Kevin P. Hamel, Sebastien Militzer, Burkhard Qi, Tingting Correa, Alfredo A. Saul, A. Schwegler, Eric TI Multiphase equation of state for carbon addressing high pressures and temperatures SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; LASER-SHOCK COMPRESSION; AUGMENTED-WAVE METHOD; MONTE-CARLO; BASIS-SET; HYDROGEN; PHASE; SIMULATION AB We present a 5-phase equation of state for elemental carbon which addresses a wide range of density and temperature conditions: 3g/cc < rho < 20g/cc, 0 K < T < infinity. The phases considered are diamond, BC8, simple cubic, simple hexagonal, and the liquid/plasma state. The solid phase free energies are constrained by density functional theory (DFT) calculations. Vibrational contributions to the free energy of each solid phase are treated within the quasiharmonic framework. The liquid free energy model is constrained by fitting to a combination of DFT molecular dynamics performed over the range 10 000 K < T < 100 000 K, and path integral quantum Monte Carlo calculations for T > 100 000 K (both for rho between 3 and 12 g/cc, with select higher-rho DFT calculations as well). The liquid free energy model includes an atom-in-jellium approach to account for the effects of ionization due to temperature and pressure in the plasma state, and an ion-thermal model which includes the approach to the ideal gas limit. The precise manner in which the ideal gas limit is reached is greatly constrained by both the highest-temperature DFT data and the path integral data, forcing us to discard an ion-thermal model we had used previously in favor of a new one. Predictions are made for the principal Hugoniot and the room-temperature isotherm, and comparisons are made to recent experimental results. C1 [Benedict, Lorin X.; Hamel, Sebastien; Qi, Tingting; Correa, Alfredo A.; Schwegler, Eric] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Driver, Kevin P.; Militzer, Burkhard] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Militzer, Burkhard] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Saul, A.] Aix Marseille Univ, CINaM CNRS UMR 7325, F-13288 Marseille 9, France. [Saul, A.] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA. [Saul, A.] MIT, CNRS, UMI 3466, Cambridge, MA 02139 USA. RP Benedict, LX (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Condensed Matter & Mat Div, Livermore, CA 94550 USA. RI Schwegler, Eric/A-2436-2016; Saul, Andres/C-1282-2012 OI Schwegler, Eric/0000-0003-3635-7418; Saul, Andres/0000-0003-0540-703X FU U.S. Department of Energy [DE-AC52-07NA27344] FX We thank C. J. Pickard, M. Martinez-Canales, P. Blaha, J. DuBois, M. A. Morales, S. B. Trickey, J. E. Pask, G. W. Collins, P. A. Sterne, H. D. Whitley, D. M. Sanchez, J. I. Castor, D. Ho, D. Braun, R. F. Smith, and B. Sadigh for helpful discussions. We also extend a special thanks to M. Millo for making available to us his reanalysis of the some of the experimental data shown in Fig. 16, to reflect the current understanding of the EOSs of the shock impedance standards. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 81 TC 25 Z9 25 U1 6 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 30 PY 2014 VL 89 IS 22 AR 224109 DI 10.1103/PhysRevB.89.224109 PG 19 WC Physics, Condensed Matter SC Physics GA AL3SJ UT WOS:000339049000004 ER PT J AU Frazer, L Chang, KB Poeppelmeier, KR Ketterson, JB AF Frazer, Laszlo Chang, Kelvin B. Poeppelmeier, Kenneth R. Ketterson, John B. TI Photoionization cross section of 1s orthoexcitons in cuprous oxide SO PHYSICAL REVIEW B LA English DT Article ID COHERENT MANIPULATION; LYMAN SPECTROSCOPY; CU2O; EXCITONS; GENERATION; ABSORPTION; ANTHRACENE; CRYSTALS AB We report measurements of the attenuation of a beam of orthoexciton polaritons by a photoionizing optical probe. Excitons were prepared in a narrow resonance by two photon absorption of a 1.016 eV, 54 ps pulsed light source in cuprous oxide (Cu2O) at 1.4 K. A collinear, 1.165 eV, 54 ps probe delayed by 119 ps was used to measure the photoionization cross section of the excitons. Two photon absorption is quadratic with respect to the intensity of the pump and leads to polariton formation. Ionization is linear with respect to the intensity of the probe. Subsequent carrier recombination is quadratic with respect to the intensity of the probe, and is distinguished because it shifts the exciton momentum away from the polariton anticrossing; the photoionizing probe leads to a rise in phonon-linked luminescence in addition to the attenuation of polaritons. The evolution of the exciton density was determined by variably delaying the probe pulse. Using the probe irradiance and the reduction in the transmitted polariton light, a cross section of (3.9 +/- 0.2) x 10(-22) m(2) was deduced for the probe frequency. C1 [Frazer, Laszlo; Ketterson, John B.] Northwestern Univ, Dept Phys, Evanston, IL 60208 USA. [Chang, Kelvin B.; Poeppelmeier, Kenneth R.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Poeppelmeier, Kenneth R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Ketterson, John B.] Northwestern Univ, Dept Elect Engn & Comp Sci, Evanston, IL 60208 USA. RP Frazer, L (reprint author), Northwestern Univ, Dept Phys, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM prb@laszlofrazer.com FU NSF IGERT [DGE-0801685]; Institute for Sustainability and Energy at Northwestern (ISEN); NSF [DMR-1307698, DMR-1121262]; Argonne National Laboratory under US Department of Energy [DE-AC02-06CH11357]; Center for Inverse Design; Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC36-08GO28308] FX We gratefully acknowledge NSF IGERT DGE-0801685. This work was funded by the Institute for Sustainability and Energy at Northwestern (ISEN). Crystal growth was supported by NSF DMR-1307698 and in part by Argonne National Laboratory under US Department of Energy Contract No. DE-AC02-06CH11357. This work made use of the X-ray and OMM Facilities supported by the MRSEC program of the NSF (DMR-1121262) at the MRC of Northwestern. K.C. was supported as part of the Center for Inverse Design, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Grant No. DE-AC36-08GO28308. NR 44 TC 4 Z9 4 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 30 PY 2014 VL 89 IS 24 AR 245203 DI 10.1103/PhysRevB.89.245203 PG 7 WC Physics, Condensed Matter SC Physics GA AL3ST UT WOS:000339050100007 ER PT J AU Hashimoto, M Ghiringhelli, G Lee, WS Dellea, G Amorese, A Mazzoli, C Kummer, K Brookes, NB Moritz, B Yoshida, Y Eisaki, H Hussain, Z Devereaux, TP Shen, ZX Braicovich, L AF Hashimoto, M. Ghiringhelli, G. Lee, W. -S. Dellea, G. Amorese, A. Mazzoli, C. Kummer, K. Brookes, N. B. Moritz, B. Yoshida, Y. Eisaki, H. Hussain, Z. Devereaux, T. P. Shen, Z. -X. Braicovich, L. TI Direct observation of bulk charge modulations in optimally doped Bi1.5Pb0.6Sr1.54CaCu2O8+delta SO PHYSICAL REVIEW B LA English DT Article ID T-C SUPERCONDUCTOR; HIGH-TEMPERATURE SUPERCONDUCTORS; COPPER-OXIDE SUPERCONDUCTORS; PHASE-TRANSITIONS; PSEUDOGAP STATE; FERMI-SURFACE; BI2SR2CACU2O8+DELTA; ORDER; EXCITATIONS; COMPETITION AB Bulk charge density modulations, recently observed in high critical-temperature (T-c) cuprate superconductors, coexist with the so-called pseudogap and compete with superconductivity. However, its direct observation has been limited to a narrow doping region in the underdoped regime. Using energy-resolved resonant x-ray scattering we have found evidence for such bulk charge modulations, or soft collective charge modes (soft CCMs), in optimally doped Bi1.5Pb0.6Sr1.54CaCu2O8+delta (Pb-Bi2212) around the summit of the superconducting dome with momentum transfer q vertical bar vertical bar similar to 0.28 reciprocal lattice units (r. l. u.) along the Cu-O bond direction. The signal is stronger at T similar or equal to T-c than at lower temperatures, thereby confirming a competition between soft CCMs and superconductivity. These results demonstrate that soft CCMs are not constrained to the underdoped regime, suggesting that soft CCMs appear across a large part of the phase diagram of cuprates and are intimately entangled with high-T-c superconductivity. C1 [Hashimoto, M.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Ghiringhelli, G.; Dellea, G.; Amorese, A.; Mazzoli, C.; Braicovich, L.] Politecn Milan, CNISM, CNR SPIN, I-20133 Milan, Italy. [Ghiringhelli, G.; Dellea, G.; Amorese, A.; Mazzoli, C.; Braicovich, L.] Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. [Lee, W. -S.; Moritz, B.; Devereaux, T. P.; Shen, Z. -X.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Kummer, K.; Brookes, N. B.] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Yoshida, Y.; Eisaki, H.] AIST, Nanoelect Res Inst, Ibaraki 3058568, Japan. [Hussain, Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Shen, Z. -X.] Stanford Univ, Dept Phys, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Shen, Z. -X.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. RP Hashimoto, M (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RI Ghiringhelli, Giacomo/D-1159-2014; Moritz, Brian/D-7505-2015 OI Ghiringhelli, Giacomo/0000-0003-0867-7748; Moritz, Brian/0000-0002-3747-8484 FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-76SF00515]; Italian Ministry of University and Research (MIUR) [PRIN20094W2LAY, PIK-POLARIXS] FX This work was performed at the ID08 beam line of the ESRF (Grenoble, France). This work is supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-76SF00515, and by the Italian Ministry of University and Research (MIUR) through Grants PRIN20094W2LAY and PIK-POLARIXS. NR 43 TC 25 Z9 25 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 30 PY 2014 VL 89 IS 22 AR 220511 DI 10.1103/PhysRevB.89.220511 PG 5 WC Physics, Condensed Matter SC Physics GA AL3SJ UT WOS:000339049000001 ER PT J AU Anselmino, M Boglione, M D'Alesio, U Melis, S Murgia, F Prokudin, A AF Anselmino, M. Boglione, M. D'Alesio, U. Melis, S. Murgia, F. Prokudin, A. TI Single spin asymmetries in lp up arrow -> hX processes and transverse momentum dependent factorization SO PHYSICAL REVIEW D LA English DT Article ID DEEP-INELASTIC SCATTERING; HARD-SCATTERING; PI-X; POLARIZED ANTIPROTONS; CROSS-SECTIONS; DRELL-YAN; AZIMUTHAL; PROTONS; PREDICTIONS; PI(0) AB Some estimates for the transverse single spin asymmetry, A(N), in the inclusive processes lp up arrow -> hX, given in a previous paper, are expanded and compared with new experimental data. The predictions are based on the Sivers distributions and the Collins fragmentation functions which fit the azimuthal asymmetries measured in semi-inclusive deep inelastic scattering (SIDIS) processes (lp up arrow -> l'hX). The factorization in terms of transverse momentum dependent distribution and fragmentation functions (TMD factorization)-i.e. the theoretical framework in which SIDIS azimuthal asymmetries are analyzed-is assumed to hold also for the inclusive process lp -> hX at large P-T. The values of A(N) thus obtained agree in sign and shape with the data. Some predictions are given for future experiments. C1 [Anselmino, M.; Boglione, M.; Melis, S.] Univ Turin, Dipartimento Fis Teor, I-10125 Turin, Italy. [Anselmino, M.; Boglione, M.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [D'Alesio, U.] Univ Cagliari, Dipartimento Fis, I-09042 Monserrato, CA, Italy. [D'Alesio, U.; Murgia, F.] Ist Nazl Fis Nucl, Sez Cagliari, I-09042 Monserrato, CA, Italy. [Prokudin, A.] Jefferson Lab, Newport News, VA 23606 USA. RP D'Alesio, U (reprint author), Univ Cagliari, Dipartimento Fis, I-09042 Monserrato, CA, Italy. EM umberto.dalesio@ca.infn.it OI Anselmino, Mauro/0000-0003-0900-8001 FU U.S. Department of Energy [DE-AC05-06OR23177]; European Community [283286]; Progetto di Ricerca Ateneo/CSP [TO-Call3-2012-0103] FX A. P. work is supported by the U.S. Department of Energy under Contract No. DE-AC05-06OR23177. M. A., M. B., U. D., S. M. and F. M. acknowledge support from the European Community under the FP7 program "Capacities-Research Infrastructures" (HadronPhysics3, Grant Agreement No. 283286). M. A., M. B. and S. M. acknowledge support from the "Progetto di Ricerca Ateneo/CSP" (codice TO-Call3-2012-0103). U. D. is grateful to the Department of Theoretical Physics II of the Universidad Complutense of Madrid for the kind hospitality extended to him during the completion of this work. NR 54 TC 11 Z9 11 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 30 PY 2014 VL 89 IS 11 AR 114026 DI 10.1103/PhysRevD.89.114026 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL3TI UT WOS:000339051700004 ER PT J AU Hu, SX Boehly, TR Collins, LA AF Hu, S. X. Boehly, T. R. Collins, L. A. TI Properties of warm dense polystyrene plasmas along the principal Hugoniot SO PHYSICAL REVIEW E LA English DT Article ID EQUATION-OF-STATE; INITIO MOLECULAR-DYNAMICS; HYDROGEN PLASMA; SIMULATION; CONDUCTION; PLANETS; METALS; MODELS AB Polystyrene (CH) is often chosen as the ablator material for inertial confinement fusion (ICF) targets. Its static, dynamical, and optical properties in warm, dense conditions (due to shock compression) are important for ICF designs. Using the first-principles quantum molecular dynamics (QMD) method, we have investigated the equation of state (EOS) and optical reflectivity of shock-compressed CH up to an unprecedentedly high pressure of 62 Mbar along the principal Hugoniot. The QMD results are compared with existing experimental measurements as well as the SESAME EOS model. Although the Hugoniot pressure and/or temperature from QMD calculations agrees with experiments and the SESAME EOS model at low pressures below 10 Mbar, we have identified for the first time a stiffer behavior of shocked CH at higher pressures (>10 Mbar). Such a stiffer behavior of warm, dense CH can affect the ablation pressure (shock strength), shock coalescence dynamics, and nonuniformity growth in ICF implosions. In addition, we corrected the mistake made in literature for calculating the reflectivity of shocked CH and obtained good agreements with experimental measurements, which should lend credence to future opacity calculations in a first-principles fashion. C1 [Hu, S. X.; Boehly, T. R.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Collins, L. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Hu, SX (reprint author), Univ Rochester, Laser Energet Lab, 250 East River Rd, Rochester, NY 14623 USA. EM shu@lle.rochester.edu RI Hu, Suxing/A-1265-2007 OI Hu, Suxing/0000-0003-2465-3818 FU Department of Energy National Nuclear Security Administration [DE-NA0001944]; University of Rochester; New York State Energy Research and Development Authority; Scientific Campaign 10 at the Los Alamos National Laboratory; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; DOE FX This material is based upon work supported by the Department of Energy National Nuclear Security Administration under Award No. DE-NA0001944, the University of Rochester, and the New York State Energy Research and Development Authority. The support of DOE does not constitute an endorsement by DOE of the views expressed in this article. This work was also supported by Scientific Campaign 10 at the Los Alamos National Laboratory, operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 67 TC 16 Z9 16 U1 1 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUN 30 PY 2014 VL 89 IS 6 AR 063104 DI 10.1103/PhysRevE.89.063104 PG 6 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AL3TZ UT WOS:000339053600027 PM 25019901 ER PT J AU Aasi, J Abbott, BP Abbott, R Abbott, T Abernathy, MR Acernese, F Ackley, K Adams, C Adams, T Addesso, P Adhikari, RX Affeldt, C Agathos, M Aggarwal, N Aguiar, OD Ajith, P Alemic, A Allen, B Allocca, A Amariutei, D Andersen, M Anderson, RA Anderson, SB Anderson, WG Arai, K Araya, MC Arceneaux, C Areeda, JS Ast, S Aston, SM Astone, P Aufmuth, P Augustus, H Aulbert, C Aylott, BE Babak, S Baker, PT Ballardin, G Ballmer, SW Barayoga, JC Barbet, M Barish, BC Barker, D Barone, F Barr, B Barsotti, L Barsuglia, M Barton, MA Bartos, I Bassiri, R Basti, A Batch, JC Bauchrowitz, J Bauer, TS Baune, C Bavigadda, V Behnke, B Bejger, M Beker, MG Belczynski, C Bell, AS Bell, C Bergmann, G Bersanetti, D Bertolini, A Betzwieser, J Bilenko, IA Billingsley, G Birch, J Biscans, S Bitossi, M Biwer, C Bizouard, MA Black, E Blackburn, JK Blackburn, L Blair, D Bloemen, S Bock, O Bodiya, TP Boer, M Bogaert, G Bogan, C Bond, C Bondu, F Bonelli, L Bonnand, R Bork, R Born, M Boschi, V Bose, S Bosi, L Bradaschia, C Brady, PR Braginsky, VB Branchesi, M Brau, JE Briant, T Bridges, DO Brillet, A Bulik, T Bulten, HJ Buonanno, A Burman, R Buskulic, D Buy, C Cadonati, L Cagnoli, G Bustillo, JC Calloni, E Camp, JB Campsie, P Cannon, KC Canuel, B Cao, J Capano, CD Carbognani, F Carbone, L Caride, S Castaldi, G Caudill, S Cavaglia, M Cavalier, F Cavalieri, R Celerier, C Cella, G Cepeda, C Cesarini, E Chakraborty, R Chalermsongsak, T Chamberlin, SJ Chao, S Charlton, P Chassande-Mottin, E Chen, X Chen, Y Chincarini, A Chiummo, A Cho, HS Cho, M Chow, JH Christensen, N Chu, Q Chua, SSY Chung, S Ciani, G Clara, F Clark, DE Clark, JA Clayton, JH Cleva, F Coccia, E Cohadon, PF Colla, A Collette, C Colombini, M Cominsky, L Constancio, M Conte, A Cook, D Corbitt, TR Cornish, N Corsi, A Costa, CA Coughlin, MW Coulon, JP 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Fiori, I Fisher, RP Flaminio, R Fournier, JD Franco, S Frasca, S Frasconi, F Frede, M Frei, Z Freise, A Frey, R Fricke, TT Fritschel, P Frolov, VV Fulda, P Fyffe, M Gair, JR Gammaitoni, L Gaonkar, S Garufi, F Gehrels, N Gemme, G Gendre, B Genin, E Gennai, A Ghosh, S Giaime, JA Giardina, KD Giazotto, A Gleason, J Goetz, E Goetz, R Gondan, L Gonzalez, G Gordon, N Gorodetsky, ML Gossan, S Gossler, S Gouaty, R Graf, C Graff, PB Granata, M Grant, A Gras, S Gray, C Greenhalgh, RJS Gretarsson, AM Groot, P Grote, H Grover, K Grunewald, S Guidi, GM Guido, CJ Gushwa, K Gustafson, EK Gustafson, R Ha, J Hall, ED Hamilton, W Hammer, D Hammond, G Hanke, M Hanks, J Hanna, C Hannam, MD Hanson, J Harms, J Harry, GM Harry, IW Harstad, ED Hart, M Hartman, MT Haster, CJ Haughian, K Heidmann, A Heintze, M Heitmann, H Hello, P Hemming, G Hendry, M Heng, IS Heptonstall, AW Heurs, M Hewitson, M Hild, S Hoak, D Hodge, KA Hofman, D Holt, K Hopkins, P Horrom, T Hoske, D Hosken, DJ Hough, J Howell, EJ Hu, Y 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Van Heijningen, J. Van Veggel, A. A. Vass, S. Vasuth, M. Vaulin, R. Vecchio, A. Vedovato, G. Veitch, J. Veitch, P. J. Venkateswara, K. Verkindt, D. Vetrano, F. Vicere, A. Vincent-Finley, R. Vinet, J. -Y. Vitale, S. Vo, T. Vocca, H. Vorvick, C. Vousden, W. D. Vyachanin, S. P. Wade, A. R. Wade, L. Wade, M. Walker, M. Wallace, L. Walsh, S. Wang, M. Wang, X. Ward, R. L. Was, M. Weaver, B. Wei, L. -W. Weinert, M. Weinstein, A. J. Weiss, R. Welborn, T. Wen, L. Wessels, P. West, M. Westphal, T. Wette, K. Whelan, J. T. White, D. J. Whiting, B. F. Wiesner, K. Wilkinson, C. Williams, K. Williams, L. Williams, R. Williams, T. D. Williamson, A. R. Willis, J. L. Willke, B. Wimmer, M. Winkler, W. Wipf, C. C. Wiseman, A. G. Wittel, H. Woan, G. Wolovick, N. Worden, J. Wu, Y. Yablon, J. Yakushin, I. Yam, W. Yamamoto, H. Yancey, C. C. Yang, H. Yoshida, S. Yvert, M. Zadrozny, A. Zanolin, M. Zendri, J. -P. Zhang, Fan Zhang, L. Zhao, C. Zhu, H. Zhu, X. J. Zucker, M. E. Zuraw, S. Zweizig, J. Aptekar, R. L. Atteia, J. L. Cline, T. Connaughton, V. Frederiks, D. D. Golenetskii, S. V. Hurley, K. Krimm, H. A. Marisaldi, M. Pal'shin, V. D. Palmer, D. Svinkin, D. S. Terada, Y. Von Kienlin, A. CA LIGO Sci Collaboration Virgo Collaboration IPN Collaboration TI Search for Gravitational Waves Associated with gamma-ray Bursts Detected by the Interplanetary Network SO PHYSICAL REVIEW LETTERS LA English DT Article ID 25 APRIL 1998; SCIENCE RUN; SHORT-DURATION; GIANT FLARE; MASS-DISTRIBUTION; UNUSUAL SUPERNOVA; LIGO OBSERVATIONS; GRB 051103; REPEATER; REDSHIFT AB We present the results of a search for gravitational waves associated with 223 gamma-ray bursts (GRBs) detected by the InterPlanetary Network (IPN) in 2005-2010 during LIGO's fifth and sixth science runs and Virgo's first, second, and third science runs. The IPN satellites provide accurate times of the bursts and sky localizations that vary significantly from degree scale to hundreds of square degrees. We search for both a well-modeled binary coalescence signal, the favored progenitor model for short GRBs, and for generic, unmodeled gravitational wave bursts. Both searches use the event time and sky localization to improve the gravitational wave search sensitivity as compared to corresponding all-time, all-sky searches. We find no evidence of a gravitational wave signal associated with any of the IPN GRBs in the sample, nor do we find evidence for a population of weak gravitational wave signals associated with the GRBs. For all IPN-detected GRBs, for which a sufficient duration of quality gravitational wave data are available, we place lower bounds on the distance to the source in accordance with an optimistic assumption of gravitational wave emission energy of 10(-2)M(circle dot)c(2) at 150 Hz, and find a median of 13 Mpc. For the 27 short-hard GRBs we place 90% confidence exclusion distances to two source models: a binary neutron star coalescence, with a median distance of 12 Mpc, or the coalescence of a neutron star and black hole, with a median distance of 22 Mpc. Finally, we combine this search with previously published results to provide a population statement for GRB searches in first-generation LIGO and Virgo gravitational wave detectors and a resulting examination of prospects for the advanced gravitational wave detectors. C1 [Aasi, J.; Abbott, B. P.; Abbott, R.; Abernathy, M. R.; Adhikari, R. X.; Anderson, R. A.; Anderson, S. B.; Arai, K.; Araya, M. C.; Barayoga, J. C.; Barish, B. C.; Billingsley, G.; Black, E.; Blackburn, J. K.; Bork, R.; Cepeda, C.; Chakraborty, R.; Chalermsongsak, T.; Coyne, D. C.; Dergachev, V.; Drever, R. W. P.; Driggers, J. C.; Ehrens, P.; Etzel, T.; Gushwa, K.; Gustafson, E. K.; Hall, E. D.; Hamilton, W.; Harms, J.; Heptonstall, A. W.; Hodge, K. 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prodi, giovanni/0000-0001-5256-915X; Lam, Ping Koy/0000-0002-4421-601X; Gemme, Gianluca/0000-0002-1127-7406; Losurdo, Giovanni/0000-0003-0452-746X; Steinlechner, Sebastian/0000-0003-4710-8548; Danilishin, Stefan/0000-0001-7758-7493; Gammaitoni, Luca/0000-0002-4972-7062; Iyer, Bala R./0000-0002-4141-5179; Lee, Chang-Hwan/0000-0003-3221-1171; Gorodetsky, Michael/0000-0002-5159-2742; McClelland, David/0000-0001-6210-5842; Vecchio, Alberto/0000-0002-6254-1617; Sigg, Daniel/0000-0003-4606-6526; Puppo, Paola/0000-0003-4677-5015; Tacca, Matteo/0000-0003-1353-0441; Garufi, Fabio/0000-0003-1391-6168; Deleglise, Samuel/0000-0002-8680-5170; Neri, Igor/0000-0002-9047-9822; Shaddock, Daniel/0000-0002-6885-3494; Vicere, Andrea/0000-0003-0624-6231; Rocchi, Alessio/0000-0002-1382-9016; Martelli, Filippo/0000-0003-3761-8616; Strain, Kenneth/0000-0002-2066-5355; Miao, Haixing/0000-0003-4101-9958; Howell, Eric/0000-0001-7891-2817; Gehring, Tobias/0000-0002-4311-2593; Heidmann, Antoine/0000-0002-0784-5175; Nelemans, Gijs/0000-0002-0752-2974; Ott, Christian/0000-0003-4993-2055; Marchesoni, Fabio/0000-0001-9240-6793; Zhu, Xingjiang/0000-0001-7049-6468; Frasconi, Franco/0000-0003-4204-6587; Groot, Paul/0000-0002-4488-726X; Lazzaro, Claudia/0000-0001-5993-3372; Ferrante, Isidoro/0000-0002-0083-7228; Bondu, Francois/0000-0001-6487-5197; Travasso, Flavio/0000-0002-4653-6156; Punturo, Michele/0000-0001-8722-4485; Cella, Giancarlo/0000-0002-0752-0338; Cesarini, Elisabetta/0000-0001-9127-3167; Chow, Jong/0000-0002-2414-5402; Frey, Raymond/0000-0003-0341-2636; Ciani, Giacomo/0000-0003-4258-9338; Di Virgilio, Angela Dora Vittoria/0000-0002-2237-7533; Vedovato, Gabriele/0000-0001-7226-1320; Ward, Robert/0000-0001-5503-5241; Ricci, Fulvio/0000-0001-5475-4447; Dolique, Vincent/0000-0001-5644-9905; Whelan, John/0000-0001-5710-6576; Boschi, Valerio/0000-0001-8665-2293; Matichard, Fabrice/0000-0001-8982-8418; Papa, M.Alessandra/0000-0002-1007-5298; Frederiks, Dmitry/0000-0002-1153-6340; Aulbert, Carsten/0000-0002-1481-8319; Pinto, Innocenzo M./0000-0002-2679-4457; Farr, Ben/0000-0002-2916-9200; Swinkels, Bas/0000-0002-3066-3601; Guidi, Gianluca/0000-0002-3061-9870; Drago, Marco/0000-0002-3738-2431; Collette, Christophe/0000-0002-4430-3703; Pierro, Vincenzo/0000-0002-6020-5521; Coccia, Eugenio/0000-0002-6669-5787; Vetrano, Flavio/0000-0002-7523-4296; Denker, Timo/0000-0003-1259-5315; calloni, enrico/0000-0003-4819-3297; Scott, Jamie/0000-0001-6701-6515; Sorazu, Borja/0000-0002-6178-3198; Allen, Bruce/0000-0003-4285-6256; Vitale, Salvatore/0000-0003-2700-0767; Murphy, David/0000-0002-8538-815X; Veitch, John/0000-0002-6508-0713 FU Australian Research Council; International Science Linkages program of the Commonwealth of Australia; Council of Scientific and Industrial Research of India; Istituto Nazionale di Fisica Nucleare of Italy; Spanish Ministerio de Economia y Competitividad; Conselleria d'Economia Hisenda i Innovacio of the Govern de les Illes Balears; Netherlands Organisation for Scientific Research; Polish Ministry of Science and Higher Education; FOCUS Programme of Foundation for Polish Science; Royal Society; Scottish Funding Council; Scottish Universities Physics Alliance; National Aeronautics and Space Administration; Carnegie Trust; Leverhulme Trust; David and Lucile Packard Foundation; Research Corporation; Alfred P. Sloan Foundation; NASA [NNX06AI36G, NNX08AB84G, NNX08AZ85G, NNX09AV61G, NNX10AR12G, NNG06GI89G, NNX07AJ65G, NNX08AN23G, NNX09AO97G, NNX10AI23G, NNG06GE69G, NNX07AQ22G, NNX08AC90G, NNX08AX95G, NNX09AR28G]; Russian Space Agency; RFBR [12-02-00032-a, 13-02-12017-ofi_m] FX The authors gratefully acknowledge the support of the United States National Science Foundation for the construction and operation of the LIGO Laboratory, the Science and Technology Facilities Council of the United Kingdom, the Max Planck Society, and the State of Niedersachsen, Germany, for support of the construction and operation of the GEO600 detector and the Italian Istituto Nazionale di Fisica Nucleare and the French Centre National de la Recherche Scientifique for the construction and operation of the Virgo detector. The authors also gratefully acknowledge the support of the research by these agencies and by the Australian Research Council, the International Science Linkages program of the Commonwealth of Australia, the Council of Scientific and Industrial Research of India, the Istituto Nazionale di Fisica Nucleare of Italy, the Spanish Ministerio de Economia y Competitividad, the Conselleria d'Economia Hisenda i Innovacio of the Govern de les Illes Balears, the Foundation for Fundamental Research on Matter supported by the Netherlands Organisation for Scientific Research, the Polish Ministry of Science and Higher Education, the FOCUS Programme of Foundation for Polish Science, the Royal Society, the Scottish Funding Council, the Scottish Universities Physics Alliance, The National Aeronautics and Space Administration, the Carnegie Trust, the Leverhulme Trust, the David and Lucile Packard Foundation, the Research Corporation, and the Alfred P. Sloan Foundation. K. H. acknowledges IPN support from the following sources: NASA NNX06AI36G, NNX08AB84G, NNX08AZ85G, NNX09AV61G, and NNX10AR12G ( Suzaku), NASA NNG06GI89G, NNX07AJ65G, NNX08AN23G, NNX09AO97G, NNX10AI23G ( Swift), NASA NNG06GE69G, NNX07AQ22G, NNX08AC90G, NNX08AX95G, NNX09AR28G ( INTEGRAL). The Konus-Wind experiment is partially supported by a Russian Space Agency contract and RFBR Grants No. 12-02-00032-a and No. 13-02-12017-ofi_m. This document has been assigned LIGO Laboratory document number LIGO-P1300226-v10. NR 55 TC 15 Z9 16 U1 3 U2 59 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 30 PY 2014 VL 113 IS 1 AR 011102 DI 10.1103/PhysRevLett.113.011102 PG 14 WC Physics, Multidisciplinary SC Physics GA AL4GW UT WOS:000339091900001 PM 25032916 ER PT J AU Campion, SL Brodie, TM Fischer, W Korber, BT Rossetti, A Goonetilleke, N McMichael, AJ Sallusto, F AF Campion, Suzanne L. Brodie, Tess M. Fischer, William Korber, Bette T. Rossetti, Astrea Goonetilleke, Nilu McMichael, Andrew J. Sallusto, Federica TI Proteome-wide analysis of HIV-specific naive and memory CD4(+) T cells in unexposed blood donors SO JOURNAL OF EXPERIMENTAL MEDICINE LA English DT Article ID VARICELLA-ZOSTER-VIRUS; RESPONSES; IMMUNODOMINANCE; REPERTOIRE; ACTIVATION; MAGNITUDE; INFECTION; FREQUENCY; EPITOPES; ANTIGENS AB The preexisting HIV-1-specific T cell repertoire must influence both the immunodominance of T cells after infection and immunogenicity of vaccines. We directly compared two methods for measuring the preexisting CD4(+) T cell repertoire in healthy HIV-1-negative volunteers, the HLA-peptide tetramer enrichment and T cell library technique, and show high concordance (r = 0.989). Using the library technique, we examined whether naive, central memory, and/or effector memory CD4(+) T cells specific for overlapping peptides spanning the entire HIV-1 proteome were detectable in 10 HLA diverse, HIV-1-unexposed, seronegative donors. HIV-1-specific cells were detected in all donors at a mean of 55 cells/million naive cells and 38.9 and 34.1 cells/million in central and effector memory subsets. Remarkably, peptide mapping showed most epitopes recognized by naive (88%) and memory (56%) CD4(+) T cells had been previously reported in natural HIV-1 infection. Furthermore, 83% of epitopes identified in preexisting memory subsets shared epitope length matches (8-12 amino acids) with human microbiome proteins, suggestive of a possible cross-reactive mechanism. These results underline the power of a proteome-wide analysis of peptide recognition by human T cells for the identification of dominant antigens and provide a baseline for optimizing HIV-1-specific helper cell responses by vaccination. C1 [Campion, Suzanne L.; McMichael, Andrew J.] Univ Oxford, Nuffield Dept Med Res Bldg, Oxford OX3 7FZ, England. [Brodie, Tess M.; Rossetti, Astrea; Sallusto, Federica] IRB, CH-6500 Bellinzona, Switzerland. [Fischer, William; Korber, Bette T.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM 87545 USA. [Goonetilleke, Nilu] Univ N Carolina, Dept Microbiol & Immunol, Chapel Hill, NC 27599 USA. [Goonetilleke, Nilu] Univ N Carolina, Dept Med, Chapel Hill, NC 27599 USA. RP Campion, SL (reprint author), Univ Oxford, Nuffield Dept Med Res Bldg, Old Rd Campus, Oxford OX3 7FZ, England. EM Suzanne.Campion@ndm.ox.ac.uk FU NIH Tetramer Core Facility [HHSN272201300006C]; National Institute of Allergy and Infectious Diseases of the National Institutes of Health; Center for HIV/AIDS Vaccine Immunology and Immunogen Discovery [UM1-AI100645-01]; Medical Research Council; ERC [ERC-2012-ADG-2012314]; SNSF [CRSII3_147662] FX The authors wish to thank Mrs. V. E. Whale and Miss Elena Brenna for technical assistance, Dr. D. Jarrossay for cell sorting, Professor G. S. Ogg for advice and guidance on the work with varicella zoster-specific epitopes, and MHC class II tetramers, and Dr. T. Rostron for HLA typing. In addition, we acknowledge the NIH Tetramer Core Facility (contract HHSN272201300006C) for provision of GE- and IE63-specific HLA Class II tetramers.; Research reported in this publication was supported by the National Institute of Allergy and Infectious Diseases of the National Institutes of Health, and by the Center for HIV/AIDS Vaccine Immunology and Immunogen Discovery, grant number UM1-AI100645-01, the Medical Research Council, the ERC, grant number ERC-2012-ADG-2012314, and the SNSF, grant number CRSII3_147662. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. NR 27 TC 21 Z9 21 U1 2 U2 6 PU ROCKEFELLER UNIV PRESS PI NEW YORK PA 950 THIRD AVE, 2ND FLR, NEW YORK, NY 10022 USA SN 0022-1007 EI 1540-9538 J9 J EXP MED JI J. Exp. Med. PD JUN 30 PY 2014 VL 211 IS 7 BP 1273 EP 1280 DI 10.1084/jem.20130555 PG 8 WC Immunology; Medicine, Research & Experimental SC Immunology; Research & Experimental Medicine GA AL2AD UT WOS:000338927200001 PM 24958850 ER PT J AU Giorgi, EE Balachandran, H Muldoon, M Letvin, NL Haynes, BF Korber, BT Santra, S AF Giorgi, Elena E. Balachandran, Harikrishnan Muldoon, Mark Letvin, Norman L. Haynes, Barton F. Korber, Bette T. Santra, Sampa TI Cross-reactive potential of human T-lymphocyte responses in HIV-1 infection SO VACCINE LA English DT Article DE HIV-1; T lymphocyte; Cross-clade response ID CELL RESPONSES; IMMUNE-RESPONSES; RHESUS-MONKEYS; RECOGNITION; SEQUENCES; SELECTION; EPIDEMIC AB An effective HIV-1 vaccine should elicit sufficient breadth of immune recognition to protect against the genetically diverse forms of the circulating virus. Evaluation of the breadth and magnitude of cellular immune responses to epitope variants is important for HIV-1 vaccine assessment. We compared HIV-1 Gag-specific T-lymphocyte responses in 20 HIV-1-infected individuals representing two different HIV-1 subtypes, B and C. By assessing T lymphocyte responses with peptides based on natural HIV-1 variants, we found evidence for limited cross-reactivity and significantly enhanced within-clade responses among clade B-infected subjects, and not among clade C-infected subjects. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Giorgi, Elena E.; Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM USA. [Balachandran, Harikrishnan; Letvin, Norman L.; Santra, Sampa] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Muldoon, Mark] Univ Manchester, Sch Math, Manchester M60 1QD, Lancs, England. [Haynes, Barton F.] Duke Univ, Human Vaccine Inst, Durham, NC USA. [Haynes, Barton F.] Duke Ctr HIV AIDS Vaccine Immunol, Durham, NC USA. [Korber, Bette T.] Santa Fe Inst, Santa Fe, NM 87501 USA. RP Santra, S (reprint author), Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM ssantra@bidmc.harvard.edu RI Muldoon, Mark/C-7505-2009; OI Korber, Bette/0000-0002-2026-5757; Muldoon, Mark/0000-0002-5004-7195 FU NIH, NIAID (the Center for HIV/AIDS Vaccine Immunology) [U19-AI067854-07] FX This work was supported by grant from the NIH, NIAID U19-AI067854-07 (the Center for HIV/AIDS Vaccine Immunology). We thank Jennifer Kirchherr of Duke Human Vaccine Institute for PBMC sample coordination and also the CHAVI-001 protocol participants. NR 16 TC 2 Z9 2 U1 0 U2 0 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0264-410X EI 1873-2518 J9 VACCINE JI Vaccine PD JUN 30 PY 2014 VL 32 IS 31 BP 3995 EP 4000 DI 10.1016/j.vaccine.2014.04.040 PG 6 WC Immunology; Medicine, Research & Experimental SC Immunology; Research & Experimental Medicine GA AK4LO UT WOS:000338396400018 PM 24837783 ER PT J AU Brejnholt, NF Soufli, R Descalle, MA Fernandez-Perea, M Christensen, FE Jakobsen, AC Honkimaki, V Pivovaroff, MJ AF Brejnholt, Nicolai F. Soufli, Regina Descalle, Marie-Anne Fernandez-Perea, Monica Christensen, Finn E. Jakobsen, Anders C. Honkimaeki, Veijo Pivovaroff, Michael J. TI Demonstration of multilayer reflective optics at photon energies above 0.6 MeV SO OPTICS EXPRESS LA English DT Article ID NUCLEAR-MEDICINE; MISSION AB Focusing optics operating in the soft gamma-ray photon energy range can advance a range of scientific and technological applications that benefit from the large improvements in sensitivity and resolution that true imaging provides. An enabling technology to this end is multilayer coatings. We show that very short period multilayer coatings deposited on super-polished substrates operate efficiently above 0.6 MeV. These experiments demonstrate that Bragg scattering theory established for multilayer applications as low as 1 eV continues to work well into the gamma-ray band. (C) 2014 Optical Society of America C1 [Brejnholt, Nicolai F.; Soufli, Regina; Descalle, Marie-Anne; Fernandez-Perea, Monica; Pivovaroff, Michael J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Christensen, Finn E.; Jakobsen, Anders C.] Tech Univ Denmark, DK-2800 Lyngby, Denmark. [Honkimaeki, Veijo] European Synchrotron Radiat Facil, F-38043 Grenoble, France. RP Brejnholt, NF (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM brejnholt1@llnl.gov RI Pivovaroff, Michael/M-7998-2014 OI Pivovaroff, Michael/0000-0001-6780-6816 FU U.S. Department of Energy Office/LLNL LDRD office [13-ERD-048, LLNL-JRNL-652505]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The project is funded by the U.S. Department of Energy Office/LLNL LDRD office, through grant 13-ERD-048 (LLNL-JRNL-652505). We acknowledge the European Synchrotron Radiation Facility for provision of synchrotron beamtime and are grateful to Eric Ziegler and Thomas Buslaps for their assistance. NR 25 TC 8 Z9 8 U1 0 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 30 PY 2014 VL 22 IS 13 BP 15364 EP 15369 DI 10.1364/OE.22.015364 PG 6 WC Optics SC Optics GA AJ9TN UT WOS:000338055900023 PM 24977796 ER PT J AU Efimov, A AF Efimov, Anatoly TI Spatial coherence at the output of multimode optical fibers SO OPTICS EXPRESS LA English DT Article ID BEAM AB The modulus of the complex degree of coherence is directly measured at the output of a step-index multimode optical fiber using lateral-sheering, delay-dithering Mach-Zehnder interferometer. Pumping the multimode fiber with monochromatic light always results in spatially-coherent output, whereas for the broadband pumping the modal dispersion of the fiber leads to a partially coherent output. While the coherence radius is a function of the numerical aperture only, the residual coherence outside the main peak is an interesting function of two dimensionless parameters: the number of non-degenerate modes and the ratio of the modal dispersion to the coherence time of the source. We develop a simple model describing this residual coherence and verify its predictions experimentally. (C) 2014 Optical Society of America C1 Los Alamos Natl Lab, Ctr Integrated Nanotechnol Mat Phys & Applicat, Los Alamos, NM 87545 USA. RP Efimov, A (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol Mat Phys & Applicat, MS K771, Los Alamos, NM 87545 USA. EM efimov@lanl.gov OI Efimov, Anatoly/0000-0002-5559-4147 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 27 TC 2 Z9 2 U1 0 U2 11 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 30 PY 2014 VL 22 IS 13 BP 15577 EP 15588 DI 10.1364/OE.22.015577 PG 12 WC Optics SC Optics GA AJ9TN UT WOS:000338055900043 PM 24977816 ER PT J AU Ghasemkhani, M Albrecht, AR Melgaard, SD Seletskiy, DV Cederberg, JG Sheik-Bahae, M AF Ghasemkhani, Mohammadreza Albrecht, Alexander R. Melgaard, Seth D. Seletskiy, Denis V. Cederberg, Jeffrey G. Sheik-Bahae, Mansoor TI Intra-cavity cryogenic optical refrigeration using high power vertical external-cavity surface-emitting lasers (VECSELs) SO OPTICS EXPRESS LA English DT Article ID TEMPERATURES; RADIATION; YBYLF AB A 7% Yb:YLF crystal is laser cooled to 131 +/- 1 K from room temperature by placing it inside the external cavity of a high power InGaAs/GaAs VECSEL operating at 1020 nm with 0.15 nm linewidth. This is the lowest temperature achieved in the intracavity geometry to date and presents major progress towards realizing an all-solid-state compact optical cryocooler. (C)2014 Optical Society of America C1 [Ghasemkhani, Mohammadreza; Albrecht, Alexander R.; Melgaard, Seth D.; Seletskiy, Denis V.; Sheik-Bahae, Mansoor] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Melgaard, Seth D.] Air Force Res Lab, Space Vehicles Directorate, Kirtland AFB, NM 87117 USA. [Cederberg, Jeffrey G.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Seletskiy, Denis V.] Univ Konstanz, Dept Phys, Constance, Germany. [Seletskiy, Denis V.] Univ Konstanz, Ctr Appl Photon, Constance, Germany. RP Ghasemkhani, M (reprint author), Univ New Mexico, Dept Phys & Astron, 1919 Lomas Blvd NE MSC 07-4220, Albuquerque, NM 87131 USA. EM mrghasem@unm.edu RI Seletskiy, Denis/C-1372-2011 OI Seletskiy, Denis/0000-0003-3480-4595 FU UNM-Science and Technology Corporation (STC) Gap Fund, AFRL [FA94531310223]; DARPA [10669320]; AFOSR STTR - Thermodynamic Films (TDF) LLC [FA9550-13-C-0006]; National Research Council Research Associateship Award at AFRL; National Science Foundation [1160764]; Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to thank Dr. Richard Epstein for useful discussions, and AC Materials Inc. for customized sample growth and preparation. We acknowledge support provided by UNM-Science and Technology Corporation (STC) Gap Fund, AFRL contract FA94531310223, DARPA grant 10669320, and AFOSR STTR grant FA9550-13-C-0006 in collaboration with Thermodynamic Films (TDF) LLC. SDM acknowledges the support of a National Research Council Research Associateship Award at AFRL. DVS acknowledges support by the National Science Foundation under Grant No. 1160764. Sandia's Laboratory Directed Research and Development Office provided growth of VECSEL devices. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 27 TC 6 Z9 6 U1 3 U2 17 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 30 PY 2014 VL 22 IS 13 BP 16232 EP 16240 DI 10.1364/OE.22.016232 PG 9 WC Optics SC Optics GA AJ9TN UT WOS:000338055900101 PM 24977874 ER PT J AU Dyer, GC Aizin, GR Allen, SJ Grine, AD Bethke, D Reno, JL Shaner, EA AF Dyer, Gregory C. Aizin, Gregory R. Allen, S. James Grine, Albert D. Bethke, Don Reno, John L. Shaner, Eric A. TI Interferometric measurement of far infrared plasmons via resonant homodyne mixing SO OPTICS EXPRESS LA English DT Article ID FIELD-EFFECT TRANSISTORS; TEMPERATURE TERAHERTZ DETECTORS; 2-DIMENSIONAL ELECTRON-GAS; RADIATION; LAYERS AB We present an electrically tunable terahertz two dimensional plasmonic interferometer with an integrated detection element that down converts the terahertz fields to a DC signal. The integrated detector utilizes a resonant plasmonic homodyne mixing mechanism that measures the component of the plasma waves in-phase with an excitation field functioning as the local oscillator. Plasmonic interferometers with two independently tuned paths are studied. These devices demonstrate a means for developing a spectrometer-on-a-chip where the tuning of electrical length plays a role analogous to that of physical path length in macroscopic spectroscopic tools such as Fourier transform interferometers. (C) 2014 Optical Society of America C1 [Dyer, Gregory C.; Grine, Albert D.; Bethke, Don; Reno, John L.; Shaner, Eric A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Aizin, Gregory R.] CUNY, Kingsborough Coll, Brooklyn, NY 11235 USA. [Allen, S. James] Univ Calif Santa Barbara, Inst Terahertz Sci & Technol, Santa Barbara, CA 93106 USA. RP Dyer, GC (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM gcdyer@sandia.gov FU DOE Office of Basic Energy Sciences; Lockheed Martin Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; [SAND2014-2988] FX The work at Sandia National Laboratories was supported by the DOE Office of Basic Energy Sciences. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. (SAND2014-2988) NR 46 TC 2 Z9 2 U1 3 U2 15 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 30 PY 2014 VL 22 IS 13 BP 16254 EP 16266 DI 10.1364/OE.22.016254 PG 13 WC Optics SC Optics GA AJ9TN UT WOS:000338055900103 PM 24977876 ER PT J AU Li, XF Lin, MW Puretzky, AA Idrobo, JC Ma, C Chi, MF Yoon, M Rouleau, CM Kravchenko, II Geohegan, DB Xiao, K AF Li, Xufan Lin, Ming-Wei Puretzky, Alexander A. Idrobo, Juan C. Ma, Cheng Chi, Miaofang Yoon, Mina Rouleau, Christopher M. Kravchenko, Ivan I. Geohegan, David B. Xiao, Kai TI Controlled Vapor Phase Growth of Single Crystalline, Two-Dimensional GaSe Crystals with High Photoresponse SO SCIENTIFIC REPORTS LA English DT Article ID ATOMIC LAYERS; MOLYBDENUM-DISULFIDE; GALLIUM SELENIDE; GRAIN-BOUNDARY; HIGH-QUALITY; NANOSHEETS; GRAPHENE; TRANSISTORS; DEPOSITION; PHOTODETECTORS AB Compared with their bulk counterparts, atomically thin two-dimensional (2D) crystals exhibit new physical properties, and have the potential to enable next-generation electronic and optoelectronic devices. However, controlled synthesis of large uniform monolayer and multi-layer 2D crystals is still challenging. Here, we report the controlled synthesis of 2D GaSe crystals on SiO2/Si substrates using a vapor phase deposition method. For the first time, uniform, large (up to,60 mm in lateral size), single-crystalline, triangular monolayer GaSe crystals were obtained and their structure and orientation were characterized from atomic scale to micrometer scale. The size, density, shape, thickness, and uniformity of the 2D GaSe crystals were shown to be controllable by growth duration, growth region, growth temperature, and argon carrier gas flow rate. The theoretical modeling of the electronic structure and Raman spectroscopy demonstrate a direct-to-indirect bandgap transition and progressive confinement-induced bandgap shifts for 2D GaSe crystals. The 2D GaSe crystals show p-type semiconductor characteristics and high photoresponsivity (similar to 1.7 A/W under white light illumination) comparable to exfoliated GaSe nanosheets. These 2D GaSe crystals are potentially useful for next-generation electronic and optoelectronic devices such as photodetectors and field-effect transistors. C1 [Li, Xufan; Lin, Ming-Wei; Puretzky, Alexander A.; Idrobo, Juan C.; Ma, Cheng; Chi, Miaofang; Yoon, Mina; Rouleau, Christopher M.; Kravchenko, Ivan I.; Geohegan, David B.; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Xiao, K (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM xiaok@ornl.gov RI Ma, Cheng/C-9120-2014; Idrobo, Juan/H-4896-2015; Kravchenko, Ivan/K-3022-2015; Chi, Miaofang/Q-2489-2015; Rouleau, Christopher/Q-2737-2015; Yoon, Mina/A-1965-2016; Li, Xufan/A-8292-2013; Puretzky, Alexander/B-5567-2016; Geohegan, David/D-3599-2013 OI Idrobo, Juan/0000-0001-7483-9034; Kravchenko, Ivan/0000-0003-4999-5822; Chi, Miaofang/0000-0003-0764-1567; Rouleau, Christopher/0000-0002-5488-3537; Yoon, Mina/0000-0002-1317-3301; Li, Xufan/0000-0001-9814-0383; Puretzky, Alexander/0000-0002-9996-4429; Geohegan, David/0000-0003-0273-3139 FU Laboratory Directed Research and Development (LDRD) program at Oak Ridge National Laboratory; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Materials Science and Energy Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Growth, synthesis, and theoretical studies sponsored by the Laboratory Directed Research and Development (LDRD) program at Oak Ridge National Laboratory. Materials and device characterization conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Synthesis science supported by the Materials Science and Energy Division, Office of Basic Energy Sciences, U.S. Department of Energy. Computing resources provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 50 TC 55 Z9 55 U1 22 U2 170 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 30 PY 2014 VL 4 AR 5497 DI 10.1038/srep05497 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK0LG UT WOS:000338103700013 PM 24975226 ER PT J AU Jia, HL Liu, FX An, ZN Li, WD Wang, GY Chu, JP Jang, JSC Gao, YF Liaw, PK AF Jia, Haoling Liu, Fengxiao An, Zhinan Li, Weidong Wang, Gongyao Chu, Jinn P. Jang, Jason S. C. Gao, Yanfei Liaw, Peter K. TI Thin-film metallic glasses for substrate fatigue-property improvements SO THIN SOLID FILMS LA English DT Article DE Thin-film metallic glass (TFMG); Coating; Fatigue-crack initiation; Fatigue lifetime; Finite-element model ID ANNEALING-INDUCED AMORPHIZATION; AUSTENITIC STAINLESS-STEEL; ATOMIC-FORCE MICROSCOPY; STRESS-STRAIN RESPONSE; BULK AMORPHOUS-ALLOYS; AIR-OXIDATION BEHAVIOR; CRACK INITIATION; DISLOCATION-STRUCTURES; MECHANICAL-PROPERTIES; CYCLIC DEFORMATION AB Amorphous metallic films, a thin form of metallic glasses, have been attracting more and more attentions in the last two decades, due to their unique properties, compared with the conventional crystalline films, such as high strength, high toughness, large elastic limits, and high-corrosion resistance. However, the deformation mechanisms of thin-film metallic glasses (TFMGs) are still far from in-depth understanding, although some of their properties and characteristics are not as good as metallic or ceramic films. This paper will focus on reviewing and discussing the fatigue behavior of structural-material substrates coated with TFMGs. The substrates include 316L stainless steel, Al-based, Ni-based, Zr-based, and Ti-based alloys. The results show that the four-point-bending fatigue life of the substrates is greatly improved by Zr- and Cu-based TFMGs, while Fe-based TFMG, TiN, and pure-Cu films are not so beneficial in extending the fatigue life of 316L stainless steel. In comparison, the tension-tension fatigue lifetime and endurance limit of 316L stainless steel cannot be improved by the Zr- and Cu-based TFMGs. However, the TFMGs annealed at a temperature within the supercooled liquid region (AT) can further improve the fatigue behavior, compared to as-deposited TFMGs. The fatigue mechanisms of crystalline and bulk metallic glass (BMG) materials, together with TFMGs, are reviewed in the present work. Crystals and BMGs present 3-stage and 4-stage fatigue-deformation mechanisms, respectively. The fatigue life of medium-strength structural materials tends to be significantly improved by TFMG5. A synergistic experimental/theoretical study has shown the micro-mechanisms of the fatigue behavior of TFMGs adhered to substrates, as well as film-adhesion and thickness effects on fatigue behavior of the substrate. Furthermore, shear-band initiation and propagation under bending deformation are investigated using the Rudnicki-Rice instability theory and the free-volume models employing finite-element simulations. Published by Elsevier B.V. C1 [Jia, Haoling; Liu, Fengxiao; An, Zhinan; Li, Weidong; Wang, Gongyao; Gao, Yanfei; Liaw, Peter K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Chu, Jinn P.] Natl Taiwan Univ Sci & Technol, Dept Mat Sci & Engn, Taipei 10607, Taiwan. [Jang, Jason S. C.] Natl Cent Univ, Inst Mat Sci & Engn, Dept Mech Engn, Chungli 32001, Taiwan. [Gao, Yanfei] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Liaw, PK (reprint author), Univ Tennessee, Dept Mat Sci & Engn, 406 Ferris Hall, Knoxville, TN 37996 USA. EM pliaw@utk.edu RI Gao, Yanfei/F-9034-2010; Jia, Haoling/P-4853-2014 OI Gao, Yanfei/0000-0003-2082-857X; Jia, Haoling/0000-0002-4287-2929 FU US National Science Foundation [DMR-0909037, CMMI-0900271, CMMI-1100080]; Department of Energy (DOE), Office of Nuclear Energy's Nuclear Energy University Program (NEUP) [00119262]; Office of Fossil Energy, National Energy Technology Laboratory [DE-FE-0008855, DE-FE-0011194]; Army Research Office [W91NF-13-1-0438] FX The authors thank for Dr. Joseph E. Greene for his enlightening comments on this paper. HJ, FL, ZA, WL, GW, YG, and PKL acknowledge the financial support from the US National Science Foundation (DMR-0909037, CMMI-0900271, and CMMI-1100080), the Department of Energy (DOE), Office of Nuclear Energy's Nuclear Energy University Program (NEUP) 00119262, the Office of Fossil Energy, National Energy Technology Laboratory (DE-FE-0008855 and DE-FE-0011194), and the Army Research Office (W91NF-13-1-0438) with C. Huber, C.V. Cooper, D. Finotello, A. Ardell, E. Taleff, V. Cedro, R.O. Jensen, L Tan, S. Lesica, S. Markovich, and S.N. Mathaudha as contract monitors. NR 105 TC 20 Z9 20 U1 7 U2 116 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD JUN 30 PY 2014 VL 561 BP 2 EP 27 DI 10.1016/j.tsf.2013.12.024 PG 26 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA AJ7DJ UT WOS:000337857100002 ER PT J AU Zhang, JC Saikin, AA Kistler, LM Smith, CW Spence, HE Mouikis, CG Torbert, RB Larsen, BA Reeves, GD Skoug, RM Funsten, HO Kurth, WS Kletzing, CA Allen, RC Jordanova, VK AF Zhang, J. -C. Saikin, A. A. Kistler, L. M. Smith, C. W. Spence, H. E. Mouikis, C. G. Torbert, R. B. Larsen, B. A. Reeves, G. D. Skoug, R. M. Funsten, H. O. Kurth, W. S. Kletzing, C. A. Allen, R. C. Jordanova, V. K. TI Excitation of EMIC waves detected by the Van Allen Probes on 28 April 2013 SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID ION-CYCLOTRON WAVES; INNER MAGNETOSPHERE; RING CURRENT; PARTICLE INTERACTIONS; CLUSTER OBSERVATIONS; MAGNETIC STORMS; OMEGA-HE; DISTRIBUTIONS; PLASMA; GENERATION AB We report the wave observations, associated plasma measurements, and linear theory testing of electromagnetic ion cyclotron (EMIC) wave events observed by the Van Allen Probes on 28 April 2013. The wave events are detected in their generation regions as three individual events in two consecutive orbits of Van Allen Probe-A, while the other spacecraft, B, does not detect any significant EMIC wave activity during this period. Three overlapping H+ populations are observed around the plasmapause when the waves are excited. The difference between the observational EMIC wave growth parameter (Sigma(h)) and the theoretical EMIC instability parameter (S-h) is significantly raised, on average, to 0.10 +/- 0.01, 0.15 +/- 0.02, and 0.07 +/- 0.02 during the three wave events, respectively. On Van Allen Probe-B, this difference never exceeds 0. Compared to linear theory (Sigma(h)>S-h), the waves are only excited for elevated thresholds. C1 [Zhang, J. -C.; Saikin, A. A.; Kistler, L. M.; Smith, C. W.; Spence, H. E.; Mouikis, C. G.; Torbert, R. B.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Larsen, B. A.; Reeves, G. D.; Skoug, R. M.; Funsten, H. O.; Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. [Kurth, W. S.; Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Allen, R. C.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX USA. [Allen, R. C.] SW Res Inst, Space Sci & Engn Div, San Antonio, TX USA. RP Zhang, JC (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. EM jichun.zhang@unh.edu RI Allen, Robert/F-5187-2011; Funsten, Herbert/A-5702-2015; Reeves, Geoffrey/E-8101-2011; OI Allen, Robert/0000-0003-2079-5683; Funsten, Herbert/0000-0002-6817-1039; Reeves, Geoffrey/0000-0002-7985-8098; Kletzing, Craig/0000-0002-4136-3348; Kurth, William/0000-0002-5471-6202 FU RBSP-ECT - JHU/APL under NASA [967399, NAS5-01072]; Iowa [1000556126]; NASA [NNX11AO82G, NNX13AE23G]; United States Department of Energy; JHU/APL under NASA [NAS5-01072, 921647] FX This work was supported by RBSP-ECT funding provided by JHU/APL contract 967399 under NASA's Prime contract NAS5-01072 and by Iowa subcontract 1000556126 to UNH in support of the Van Allen Probes and EMFISIS/MAG instruments. Work at UNH was also supported by NASA under grant numbers NNX11AO82G and NNX13AE23G. Work at LANL was performed under the auspices of the United States Department of Energy. Work at the University of Iowa was performed under support on JHU/APL contract 921647 under NASA's Prime contract NAS5-01072. The authors thank RBSP team members for RBSP data preparation and software development. J.-C. Zhang thanks Brian Fraser and S. Peter Gary for helpful discussions. NR 34 TC 20 Z9 20 U1 0 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 28 PY 2014 VL 41 IS 12 BP 4101 EP 4108 DI 10.1002/2014GL060621 PG 8 WC Geosciences, Multidisciplinary SC Geology GA AN0SM UT WOS:000340294300001 ER PT J AU Dai, S Seol, Y AF Dai, Sheng Seol, Yongkoo TI Water permeability in hydrate-bearing sediments: A pore-scale study SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID POROUS-MEDIA; METHANE-HYDRATE; GAS-HYDRATE; MARINE-SEDIMENTS; RELATIVE PERMEABILITY; DISSOCIATION; FLOW; SATURATION; PARAMETERS; STABILITY AB Permeability is a critical parameter governing methane flux and fluid flow in hydrate-bearing sediments; however, limited valid data are available due to experimental challenges. Here we investigate the relationship between apparent water permeability (k') and hydrate saturation (S-h), accounting for hydrate pore-scale growth habit and meso-scale heterogeneity. Results from capillary tube models rely on cross-sectional tube shapes and hydrate pore habits, thus are appropriate only for sediments with uniform hydrate distribution and known hydrate pore character. Given our pore network modeling results showing that accumulating hydrate in sediments decreases sediment porosity and increases hydraulic tortuosity, we propose a modified Kozeny-Carman model to characterize water permeability in hydrate-bearing sediments. This model agrees well with experimental results and can be easily implemented in reservoir simulators with no empirical variables other than S-h. Results are also relevant to flow through other natural sediments that undergo diagenesis, salt precipitation, or bio-clogging. C1 [Dai, Sheng; Seol, Yongkoo] US DOE, Natl Energy Technol Lab, Morgantown, WV 26505 USA. RP Dai, S (reprint author), US DOE, Natl Energy Technol Lab, Morgantown, WV 26505 USA. EM shengdai.geo@gmail.com RI Dai, Sheng/A-1691-2015; OI Dai, Sheng/0000-0003-0221-3993 FU Oak Ridge Institute for Science and Education (ORISE) fellowship - NETL, U.S. Department of Energy FX S. Dai is supported via the Oak Ridge Institute for Science and Education (ORISE) fellowship granted by NETL, U.S. Department of Energy. Authors would like to thank M. Bayani Cardenas, William F. Waite, and another anonymous reviewer for insightful comments, which have greatly improved the quality of this manuscript. The pore network modeling method is described in supporting information SI1, and data supporting Figure 4b are available in supporting information SI2. NR 40 TC 13 Z9 13 U1 10 U2 39 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 28 PY 2014 VL 41 IS 12 BP 4176 EP 4184 DI 10.1002/2014GL060535 PG 9 WC Geosciences, Multidisciplinary SC Geology GA AN0SM UT WOS:000340294300010 ER PT J AU Zamora, LM Oschlies, A AF Zamora, Lauren M. Oschlies, Andreas TI Surface nitrification: A major uncertainty in marine N2O emissions SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID AMMONIA-OXIDIZING ARCHAEA; OCEAN IRON FERTILIZATION; SYSTEM CLIMATE MODEL; NITROUS-OXIDE FLUXES; SEA-TO-AIR; ATLANTIC-OCEAN; EUPHOTIC ZONE; PACIFIC-OCEAN; OXYGEN; RATES AB The ocean is responsible for up to a third of total global nitrous oxide (N2O) emissions, but uncertainties in emission rates of this potent greenhouse gas are high (> 100%). Here we use a marine biogeochemical model to assess six major uncertainties in estimates of N2O production, thereby providing guidance in how future studies may most effectively reduce uncertainties in current and future marine N2O emissions. Potential surface N2O production from nitrification causes the largest uncertainty in N2O emissions (estimated up to similar to 1.6 Tg N yr(-1) or 48% of modeled values), followed by the unknown oxygen concentration at which N2O production switches to N2O consumption (0.8 Tg N yr(-1) or 24% of modeled values). Other uncertainties are minor, cumulatively changing regional emissions by <15%. If production of N2O by surface nitrification could be ruled out in future studies, uncertainties in marine N2O emissions would be halved. C1 [Zamora, Lauren M.; Oschlies, Andreas] GEOMAR Helmholtz Ctr Ocean Res Kiel, Kiel, Germany. RP Zamora, LM (reprint author), Oak Ridge Associated Univ, NASA Postdoctoral Program, Oak Ridge, TN 37830 USA. EM laurenge@gmail.com RI Zamora, Lauren/E-6972-2011; OI Zamora, Lauren/0000-0002-0878-4378; Oschlies, Andreas/0000-0002-8295-4013 FU BMBF project SOPRAN [FKZ030611A, FKZ 03F0662A]; DFG [SFB 754]; NASA FX Funding for this study was provided by the BMBF project SOPRAN via grants FKZ030611A and FKZ 03F0662A, the DFG via SFB 754, and an appointment to the NASA Postdoctoral Program at Goddard Space Flight Center, administered by Oak Ridge Associated Universities through a contract with NASA. We would like to thank the MEMENTO database contributors. J.-F. Lamarque provided the model inorganic N deposition fields used in this study. D. Arevalo-Martinez, H. W. Bange, H. Dietze, J. Getzlaff, D. Grundle, K. B. Huebert, D. Keller, A. Kock, I. Montes, L. Nickelsen, M. Schartau, and B. Thamdrup provided technical assistance and/or comments helpful to the manuscript. Model files can be obtained at sopran.pangaea.de/data (doi.pangaea.de/10.1594/PANGAEA.833374). The authors thank an anonymous reviewer for the constructive comments. NR 42 TC 7 Z9 7 U1 4 U2 33 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 28 PY 2014 VL 41 IS 12 BP 4247 EP 4253 DI 10.1002/2014GL060556 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AN0SM UT WOS:000340294300019 ER PT J AU O'Brien, RE Neu, A Epstein, SA MacMillan, AC Wang, BB Kelly, ST Nizkorodov, SA Laskin, A Moffet, RC Gilles, MK AF O'Brien, Rachel E. Neu, Alexander Epstein, Scott A. MacMillan, Amanda C. Wang, Bingbing Kelly, Stephen T. Nizkorodov, Sergey A. Laskin, Alexander Moffet, Ryan C. Gilles, Mary K. TI Physical properties of ambient and laboratory-generated secondary organic aerosol SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID MEXICO-CITY; PHASE STATE; PARTICLES; ATMOSPHERE; PHOTOOXIDATION; TRANSMISSION; EVAPORATION; REACTIVITY; COMPONENTS; ISOPRENE AB The size and thickness of organic aerosol particles collected by impaction in five field campaigns were compared to those of laboratory-generated secondary organic aerosols (SOA). Scanning transmission X-ray microscopy was used to measure the total carbon absorbance (TCA) by individual particles as a function of their projection areas on the substrate. Particles with higher viscosity/surface tension can be identified by a steeper slope on a plot of TCA versus size because they flatten less upon impaction. The slopes of the ambient data are statistically similar indicating a small range of average viscosities/surface tensions across five field campaigns. Steeper slopes were observed for the plots corresponding to ambient particles, while smaller slopes were indicative of the laboratory-generated SOA. This comparison indicates that ambient organic particles have higher viscosities/surface tensions than those typically generated in laboratory SOA studies. C1 [O'Brien, Rachel E.; Neu, Alexander; Kelly, Stephen T.; Gilles, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [O'Brien, Rachel E.; Moffet, Ryan C.] Univ Pacific, Dept Chem, Stockton, CA 95211 USA. [Epstein, Scott A.; MacMillan, Amanda C.; Nizkorodov, Sergey A.] Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA. [Wang, Bingbing; Laskin, Alexander] Pacific NW Natl Lab, William R Wiley Environm & Mol Sci Lab, Richland, WA 99352 USA. RP O'Brien, RE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM resellon@lbl.gov RI Wang, Bingbing/B-6211-2011; Laskin, Alexander/I-2574-2012; Nizkorodov, Sergey/I-4120-2014 OI Laskin, Alexander/0000-0002-7836-8417; Nizkorodov, Sergey/0000-0003-0891-0052 FU U.S. Department of Energy's Atmospheric System Research, an Office of Science, Office of Biological and Environmental Research program; Division of Chemical Sciences, Geosciences, and Biosciences) of the U. S. Department of Energy [DE-AC02-05CH11231]; Condensed Phase and Interfacial Molecular Sciences Program; OBER at Pacific Northwest National Laboratory; National Science Foundation [CHE-0909227]; [DE-AC06-76RL0] FX Data supporting Figures 2 and 3 are available in Table S5 in the supporting information. This work was supported in part by the U.S. Department of Energy's Atmospheric System Research, an Office of Science, Office of Biological and Environmental Research program. STXM/NEXAFS was done at beamlines 5.3.2.2 and 11.0.2 at The Advanced Light Source at Lawrence Berkeley National Laboratory (LBNL) which are supported by the Director, Office of Science, Office of Basic Energy Sciences, (beamline 11.0.2 is also supported by the Division of Chemical Sciences, Geosciences, and Biosciences) of the U. S. Department of Energy under contract DE-AC02-05CH11231. M. K. G. and S. T. K. also acknowledge support from the Condensed Phase and Interfacial Molecular Sciences Program under the same contract. We wish to acknowledge the continued support of A. L. D. Kilcoyne and T. Tyliszczak. SEM imaging of particles was performed at Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by OBER at Pacific Northwest National Laboratory. PNNL is operated by the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RL0. The UCI team acknowledges support from the National Science Foundation grant CHE-0909227. NR 32 TC 15 Z9 15 U1 2 U2 47 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 28 PY 2014 VL 41 IS 12 BP 4347 EP 4353 DI 10.1002/2014GL060219 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AN0SM UT WOS:000340294300032 ER PT J AU Tomasino, D Jenei, Z Evans, W Yoo, CS AF Tomasino, Dane Jenei, Zsolt Evans, William Yoo, Choong-Shik TI Melting and phase transitions of nitrogen under high pressures and temperatures SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DIAMOND-ANVIL CELL; RAMAN-SPECTROSCOPY; GPA; DIFFRACTION; CALIBRATION; CURVES; STOKES; GAUGE; N-2 AB Dense nitrogen exhibits fascinating molecular and extended polymorphs as well as an anomalous melt maximum at high temperatures. However, the exact solid-liquid phase boundary is still the subject of debate, as both creating and probing hot dense nitrogen, solid and fluid alike, poses unique experimental challenges. Raman studies of nitrogen were performed to investigate the melting curve and solid-solid phase transitions in the pressure-temperature range of 25 to 103 GPa and 300 to 2000 K. The solid-liquid phase boundary has been probed with time-resolved Raman spectroscopy on ramp heated nitrogen in diamond anvil cell (DAC), showing a melting maximum at 73 GPa and 1690 K. The solid-solid phase boundaries have been measured with spatially resolved micro-confocal Raman spectroscopy on resistively heated DAC, probing the delta-epsilon phase line to 47 GPa and 914 K. At higher pressures the theta-phase was produced upon a repeated thermal heating of the zeta-phase, yet no evidence was found for the t-phase. Hence, the present results signify the path dependence of dense nitrogen phases and provide new constraints for the phase diagram. (C) 2014 AIP Publishing LLC. C1 [Tomasino, Dane; Yoo, Choong-Shik] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Tomasino, Dane; Yoo, Choong-Shik] Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. [Jenei, Zsolt; Evans, William] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Tomasino, D (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. RI Jenei, Zsolt/B-3475-2011 FU NSF-DMR [1203834]; DTRA [HDTRA1-12-010020]; U.S. Department of Energy [DE-AC52-07NA27344] FX The present study at WSU has been supported by NSF-DMR (Grant No. 1203834) and DTRA (HDTRA1-12-010020). The work at LLNL was performed under the auspices of the U.S. Department of Energy under Contract No. DE-AC52-07NA27344. NR 43 TC 2 Z9 2 U1 2 U2 30 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 28 PY 2014 VL 140 IS 24 AR 244510 DI 10.1063/1.4885724 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AK7UW UT WOS:000338634200048 PM 24985657 ER PT J AU Wu, Q AF Wu, Qin TI Variational nature of the frozen density energy in density-based energy decomposition analysis and its application to torsional potentials SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID EXCHANGE-CORRELATION POTENTIALS; MOLECULAR-INTERACTIONS; BASIS-SETS; STAGGERED CONFORMATION; ELECTRON-DENSITIES; FUNCTIONAL THEORY; ETHANE; HYDROGEN; SCHEME; CHEMISTRY AB The density-based energy decomposition analysis (DEDA) is the first of its kind to calculate the frozen density energy variationally. Defined with the constrained search formulation of density functional theory, the frozen density energy is optimized in practice using the Wu-Yang (WY) method for constrained minimizations. This variational nature of the frozen density energy, a possible reason behind some novel findings of DEDA, will be fully investigated in this work. In particular, we systematically study the dual basis set dependence in WY: the potential basis set used to expand the Lagrangian multiplier function and the regular orbital basis set. We explain how the convergence progresses differently on these basis sets and how an apparent basis-set independence is achieved. We then explore a new development of DEDA in frozen energy calculations of the ethane molecule, focusing on the internal rotation around the carbon-carbon bond and the energy differences between staggered and eclipsed conformations. We argue that the frozen density energy change at fixed bond lengths and bond angles is purely steric effects. Our results show that the frozen density energy profile follows closely that of the total energy when the dihedral angle is the only varying geometry parameter. We can further analyze the contributions from electrostatics and Pauli repulsions. These results lead to a meaningful DEDA of the torsional potential in ethane. (C) 2014 AIP Publishing LLC. C1 Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Wu, Q (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM qinwu@bnl.gov RI Wu, Qin/C-9483-2009 OI Wu, Qin/0000-0001-6350-6672 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX Research carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 47 TC 8 Z9 8 U1 4 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 28 PY 2014 VL 140 IS 24 AR 244109 DI 10.1063/1.4884961 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AK7UW UT WOS:000338634200012 PM 24985620 ER PT J AU Okoro, C Levine, LE Xu, RQ Hummler, K Obeng, Y AF Okoro, Chukwudi Levine, Lyle E. Xu, Ruqing Hummler, Klaus Obeng, Yaw TI Synchrotron-based measurement of the impact of thermal cycling on the evolution of stresses in Cu through-silicon vias SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FAILURE ANALYSIS; THIN-FILMS; COPPER; FATIGUE; DEFORMATION; METALLIZATION; MECHANISM AB One of the main causes of failure during the lifetime of microelectronics devices is their exposure to fluctuating temperatures. In this work, synchrotron-based X-ray micro-diffraction is used to study the evolution of stresses in copper through-silicon via (TSV) interconnects, "as-received" and after 1000 thermal cycles. For both test conditions, significant fluctuations in the measured normal and shear stresses with depth are attributed to variations in the Cu grain orientation. Nevertheless, the mean hydrostatic stresses in the "as-received" Cu TSV were very low, at (16 +/- 44) MPa, most likely due to room temperature stress relaxation. In contrast, the mean hydrostatic stresses along the entire length of the Cu TSV that had undergone 1000 thermal cycles (123 +/- 37) MPa were found to be eight times greater, which was attributed to increased strain-hardening. The evolution in stresses with thermal cycling is a clear indication that the impact of Cu TSVs on front-end-of-line (FEOL) device performance will change through the lifetime of the 3D stacked dies, and ought to be accounted for during FEOL keep-out-zone design rules development. (C) 2014 AIP Publishing LLC. C1 [Okoro, Chukwudi; Obeng, Yaw] NIST, Semicond & Dimens Metrol Div, Gaithersburg, MD 20899 USA. [Levine, Lyle E.] NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. [Xu, Ruqing] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hummler, Klaus] SEMATECH, Albany, NY 12203 USA. RP Okoro, C (reprint author), NIST, Semicond & Dimens Metrol Div, Gaithersburg, MD 20899 USA. EM chukwudi.okoro@nist.gov RI Xu, Ruqing/K-3586-2012 OI Xu, Ruqing/0000-0003-1037-0059 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The XOR/UNI facilities on Sector 34 at the APS are supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 34 TC 10 Z9 10 U1 2 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 28 PY 2014 VL 115 IS 24 AR 243509 DI 10.1063/1.4885461 PG 7 WC Physics, Applied SC Physics GA AK7UQ UT WOS:000338633600014 ER PT J AU Xu, DB Sun, CJ Brewe, DL Han, SW Ho, P Chen, JS Heald, SM Zhang, XY Chow, GM AF Xu, D. B. Sun, C. J. Brewe, D. L. Han, S. -W. Ho, P. Chen, J. S. Heald, S. M. Zhang, X. Y. Chow, G. M. TI Spatiotemporally separating electron and phonon thermal transport in L1(0) FePt films for heat assisted magnetic recording SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID X-RAY-DIFFRACTION; METAL-NONMETAL INTERFACES; KAPITZA CONDUCTANCE; LATTICE-DYNAMICS AB We report the spatio-temporal separation of electron and phonon thermal transports in nanostructured magnetic L1(0) FePt films at the nanometer length scale and the time domain of tens of picosecond, when heated with a pulsed laser. We demonstrate that lattice dynamics measured using the picosecond time-resolved laser pump/X-ray probe method on the FePt (002) and Ag (002) Bragg reflections from different layers provided the information of nanoscale thermal transport between the layers. We also describe how the electron and phonon thermal transports in nanostructured magnetic thin films were separated. (C) 2014 AIP Publishing LLC. C1 [Xu, D. B.; Brewe, D. L.; Heald, S. M.; Zhang, X. Y.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Xu, D. B.; Sun, C. J.; Ho, P.; Chen, J. S.; Chow, G. M.] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore. [Han, S. -W.] Chonbuk Natl Univ, Dept Phys Educ, Jeonju 561756, South Korea. [Han, S. -W.] Chonbuk Natl Univ, Inst Fus Sci, Jeonju 561756, South Korea. RP Sun, CJ (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM dongbin.xu@seagate.com; cjsun@aps.anl.gov; msecgm@nus.edu.sg OI Ho, Pin/0000-0002-2399-0823 FU U.S. DOE [DE-AC02-06CH11357]; Ministry of Education, Singapore [MOE2012-T2-2-031]; National Research Foundation of Korea government (NRF) - Basic Science Research Program [2012R1A1A4A01007669]; PAL XFEL project; U.S. Department of Energy-Basic Energy Sciences; Canadian Light Source; University of Washington; Advanced Photon Source FX PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the U.S. Department of Energy-Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Work at National University of Singapore was supported by Ministry of Education, Singapore under Grant No. MOE2012-T2-2-031. Work at Chonbuk National University was supported by the National Research Foundation of Korea government (NRF) grant funded by the Basic Science Research Program (No. 2012R1A1A4A01007669) and PAL XFEL project. The authors also thank Dr. Donald A. Walko for proof-reading the manuscript. G.M.C. also thanks the PNC/XSD facilities for his sabbatical support. NR 31 TC 0 Z9 0 U1 1 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 28 PY 2014 VL 115 IS 24 AR 243907 DI 10.1063/1.4885428 PG 5 WC Physics, Applied SC Physics GA AK7UQ UT WOS:000338633600029 ER PT J AU Kogar, A Vig, S Gan, Y Abbamonte, P AF Kogar, Anshul Vig, Sean Gan, Yu Abbamonte, Peter TI Temperature-resolution anomalies in the reconstruction of time dynamics from energy-loss experiments SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE electron and nuclear dynamics; explicit approach; momentum-resolved scattering experiments ID X-RAY-SCATTERING; INELASTIC-SCATTERING; SLOW-ELECTRONS; SUPERCONDUCTORS; SURFACES AB Inelastic scattering techniques provide a powerful approach to studying electron and nuclear dynamics, via reconstruction of a propagator that quantifies the time evolution of a system. There is now growing interest in applying such methods to very low energy excitations, such as lattice vibrations, but in this limit the cross section is no longer proportional to a propagator. Significant deviations occur due to the finite temperature Bose statistics of the excitations. Here we consider this issue in the context of high-resolution electron energy-loss experiments on the copper-oxide superconductor Bi2Sr2CaCu2O8. We find that simple division of a Bose factor yields an accurate propagator on energy scales greater than the resolution width. However, at low energy scales, the effects of resolution and finite temperature conspire to create anomalies in the dynamics at long times. We compare two practical ways for dealing with such anomalies, and discuss the range of validity of the technique in light of this comparison. C1 [Kogar, Anshul; Vig, Sean; Gan, Yu; Abbamonte, Peter] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kogar, Anshul; Vig, Sean; Gan, Yu; Abbamonte, Peter] Univ Illinois, Federick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Kogar, Anshul; Vig, Sean; Gan, Yu; Abbamonte, Peter] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Kogar, A (reprint author), Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. EM abbamonte@mrl.illinois.edu FU Office of Basic Energy Sciences, US Department of Energy [DE-FG02-06ER46285] FX This work was supported by the Office of Basic Energy Sciences, US Department of Energy, grant no. DE-FG02-06ER46285. NR 19 TC 4 Z9 4 U1 4 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUN 28 PY 2014 VL 47 IS 12 SI SI AR 124034 DI 10.1088/0953-4075/47/12/124034 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AJ5KN UT WOS:000337721200035 ER PT J AU Poullain, SM Elkharrat, C Li, WB Veyrinas, K Houver, JC Cornaggia, C Rescigno, TN Lucchese, RR Dowek, D AF Marggi Poullain, S. Elkharrat, C. Li, W. B. Veyrinas, K. Houver, J. C. Cornaggia, C. Rescigno, T. N. Lucchese, R. R. Dowek, D. TI Recoil frame photoemission in multiphoton ionization of small polyatomic molecules: photodynamics of NO2 probed by 400 nm fs pulses SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE molecular frame photoemission; recoil frame photoemission; multiphoton ionization by femtosecond pulses; Rydberg states; vibronic coupling ID PHOTOELECTRON ANGULAR-DISTRIBUTION; DISSOCIATIVE PHOTOIONIZATION; VECTOR CORRELATIONS; CROSS-SECTIONS; WAVE-FUNCTIONS; RYDBERG STATE; BASIS-SETS; DYNAMICS; SPECTROSCOPY; ION AB We report a general method for the complete analysis of the recoil frame photoelectron angular distribution (RFPAD) in n-photon dissociative ionization of small polyatomic molecules, resulting from (n - 1) bound-to-bound transitions plus one-photon ionization of a neutral excited state of the target. This method relies on the decomposition of the RFPAD in terms of the R-K (chi, theta(e)) recoil frame azimuthal harmonics (RFAHs) which are the components of its Fourier expansion in phi(e), where chi and theta(e) are the polar angles referring to the polarization axis P and the photoelectron momentum k relative to the ion fragment recoil direction, respectively, and fe is the azimuth of k relative to P. The RFAH expansion method is illustrated by a detailed experimental and theoretical study of one-colour multiphoton dissociative and non-dissociative ionization of the NO2 molecule of C-2v symmetry induced by 400 nm fs laser pulses, which involve electronic and nuclear dynamics within the pulse duration of the order of 70 fs. The reaction mechanism proposed to account for five-photon dissociative ionization of NO2 involves the role of [R*(6a(1))(-1)] Rydberg states populated by three-photon absorption, subsequently ionized by a fourth photon into the NO2+ (X-1 Sigma(+)(g), upsilon(1),upsilon(2),upsilon(3)) manifold involving autoionization of [R*(4b(2))(-1)] Rydberg states, and linear versus bent geometry selective dissociation of NO2+ (X-1 Sigma(+)(g), upsilon(1),upsilon(2),upsilon(3)) by a fifth photon. The reported calculations provide a coherent picture of the experimental findings although all features are not yet well reproduced. C1 [Marggi Poullain, S.; Elkharrat, C.; Li, W. B.; Veyrinas, K.; Houver, J. C.; Dowek, D.] Univ Paris 11, Inst Sci Mol Orsay, F-91405 Orsay, France. [Marggi Poullain, S.; Elkharrat, C.; Li, W. B.; Veyrinas, K.; Houver, J. C.; Dowek, D.] CNRS, F-91405 Orsay, France. [Cornaggia, C.] CEA IRAMIS Saclay, Lab Interact Dynam & Lasers, F-91191 Gif Sur Yvette, France. [Rescigno, T. N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lucchese, R. R.] Texas A&M Univ, Dept Chem, College Stn, TX 77840 USA. RP Poullain, SM (reprint author), Univ Complutense Madrid, Fac Ciencias Quim, Dept Quim Fis, Unidad Asociada CSIC, E-28040 Madrid, Spain. EM smarggi@ucm.es; danielle.dowek@u-psud.fr RI Lucchese, Robert/O-4452-2014; OI Lucchese, Robert/0000-0002-7200-3775; Marggi Poullain, Sonia/0000-0001-6712-3628 FU PICS (Programme International de Cooperation Scientifique CNRS) [2008-046T]; Triangle de la Physique (High Rep Image) [2010-078T]; ANR (Agence Nationale de la Recherche, projet Image Femto) [ANR-07-BLAN-0162-01]; LASERLAB-EUROPE (EC's Seventh Framework Programme) [284464]; Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy and of the R AWelch Foundation ( Houston, TX) [A-1020]; US DOE [DE-AC02-05CH11231]; Texas AM University; Triangle de la Physique (MOF-MPI) [2013-0569T] FX The support of the PICS (Programme International de Cooperation Scientifique CNRS no 2008-046T) and the Triangle de la Physique (High Rep Image no 2010-078T, MOF-MPI no 2013-0569T) is gratefully acknowledged. The SOFOCKLE femtosecond laser is supported by ANR (Agence Nationale de la Recherche, projet Image Femto, no. ANR-07-BLAN-0162-01). The research leading to these results performed at PLFA laser platform has received funding from LASERLAB-EUROPE (grant agreement no. 284464, EC's Seventh Framework Programme).; We acknowledge the support of the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy and of the R AWelch Foundation ( Houston, TX) under grant A-1020. Work at LBNL was performed under the auspices of the US DOE under contract no. DE-AC02-05CH11231. This work was also supported by the Texas A&M University Supercomputing Facility. NR 59 TC 2 Z9 2 U1 2 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUN 28 PY 2014 VL 47 IS 12 SI SI AR 124024 DI 10.1088/0953-4075/47/12/124024 PG 18 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AJ5KN UT WOS:000337721200025 ER PT J AU Grobner, J Reda, I Wacker, S Nyeki, S Behrens, K Gorman, J AF Groebner, J. Reda, I. Wacker, S. Nyeki, S. Behrens, K. Gorman, J. TI A new absolute reference for atmospheric longwave irradiance measurements with traceability to SI units SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID RADIATION MEASUREMENTS; WAVE-RADIATION; PYRGEOMETER; CALIBRATION; UNCERTAINTY; RADIOMETRY; ACCURACY; CAVITY AB Two independently designed and calibrated absolute radiometers measuring downwelling longwave irradiance were compared during two field campaigns in February and October 2013 at Physikalisch Meteorologisches Observatorium Davos/World Radiation Center (PMOD/WRC). One absolute cavity pyrgeometer (ACP) developed by NREL and up to four Integrating Sphere Infrared Radiometers (IRIS) developed by PMOD/WRC took part in these intercomparisons. The internal consistency of the IRIS radiometers and the agreement with the ACP were within +/- 1 W m(-2), providing traceability of atmospheric longwave irradiance to the international system of units with unprecedented accuracy. Measurements performed during the two field campaigns and over the past 4 years have shown that the World Infrared Standard Group (WISG) of pyrgeometers is underestimating clear-sky atmospheric longwave irradiance by 2 to 6 W m(-2), depending on the amount of integrated water vapor (IWV). This behavior is an instrument-dependent feature and requires an individual sensitivity calibration of each pyrgeometer with respect to an absolute reference such as IRIS or ACP. For IWV larger than 10 mm, an average sensitivity correction of +6.5% should be applied to the WISG in order to be consistent with the longwave reference represented by the ACP and IRIS radiometers. A concerted effort at international level will need to be implemented in order to correct measurements of atmospheric downwelling longwave irradiance traceable to the WISG. C1 [Groebner, J.; Wacker, S.; Nyeki, S.] World Radiat Ctr, Phys Meteorol Observ Davos, Davos, Switzerland. [Reda, I.] Natl Renewable Energy Lab, Golden, CO USA. [Behrens, K.] Deutsch Wetterdienst, Meteorol Observ Lindenberg, Richard Assmann Observ, Lindenberg, Germany. [Gorman, J.] Bureau Meteorol, Melbourne, Vic, Australia. RP Grobner, J (reprint author), World Radiat Ctr, Phys Meteorol Observ Davos, Davos, Switzerland. EM julian.groebner@pmodwrc.ch NR 16 TC 7 Z9 7 U1 1 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 27 PY 2014 VL 119 IS 12 BP 7083 EP 7090 DI 10.1002/2014JD021630 PG 8 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0BP UT WOS:000340247000005 ER PT J AU Blom, P Waxler, R Frazier, WG Talmadge, C AF Blom, Philip Waxler, Roger Frazier, Wm Garth Talmadge, Carrick TI Observations of the refraction of microbaroms generated by large maritime storms by the wind field of the generating storm SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID ARRAY; WAVES AB Microbaroms are a continuous infrasonic signal in the 0.15 to 0.3 Hz band caused by the collision of oceanic surface waves of equal period. Such signals are often generated by large maritime storms. Current formulation of the generation mechanism predicts that the microbarom source location due to a large maritime storm in the open ocean is generally located several hundreds of kilometers from the eye of the storm. Assuming such a source location to be correct, propagation of the microbaroms along paths which pass near the storm center as well as those which propagate away from the storm structure have been examined using geometric acoustics. Microbarom propagation paths which pass near the storm center are refracted by the storm winds and are found to have back azimuths directed toward a virtual source around the storm center. Microbarom propagation paths which do not pass near the storm center are found to have back azimuths directed toward the actual source region. To validate these predictions, data from microbarom signals generated by hurricanes in the Atlantic Ocean have been collected along the east coast of the United States during the 2010 and 2011 Atlantic hurricane seasons. Data from several storm events are presented here for comparison with model predictions. In general, the observations are in agreement with the predictions of the propagation model. C1 [Blom, Philip] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Waxler, Roger; Frazier, Wm Garth; Talmadge, Carrick] Univ Mississippi, NCPA, University, MS 38677 USA. RP Blom, P (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM pblom@lanl.gov FU University of Mississippi under National Oceanic and Atmospheric Administration, U.S. Department of Commerce [NA08NWS4680044] FX This publication was prepared by the University of Mississippi under award NA08NWS4680044 from National Oceanic and Atmospheric Administration, U.S. Department of Commerce. The statements, findings, conclusions, and recommendations are those of the author(s) and do not necessarily reflect the views of the National Oceanic and Atmospheric Administration or the U.S. Department of Commerce. We thank the McCoy family of Laurinburg, North Carolina, for allowing us to deploy equipment on their land. In addition, we thank Ocala National Forest, FL, Francis Marion National Forest, SC, Croatan National Forest, NC, Bass River State Forest, NJ, and Pachaug State Forest, CT. The infrasonic data collected during these experiments have been archived by the Infrasound Research Group at the National Center for Physical Acoustics, University of Mississippi (ncpadata@olemiss.edu). NR 30 TC 0 Z9 0 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 27 PY 2014 VL 119 IS 12 BP 7179 EP 7192 DI 10.1002/2014JD021795 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0BP UT WOS:000340247000011 ER PT J AU Zelinka, MD Andrews, T Forster, PM Taylor, KE AF Zelinka, Mark D. Andrews, Timothy Forster, Piers M. Taylor, Karl E. TI Quantifying components of aerosol-cloud-radiation interactions in climate models SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID SIMULATIONS; ECMWF AB The interaction of anthropogenic aerosols with radiation and clouds is the largest source of uncertainty in the radiative forcing of the climate during the industrial period. Here we apply novel techniques to diagnose the contributors to the shortwave (SW) effective radiative forcing (ERF) from aerosol-radiation-interaction (ERFari) and from aerosol cloud interaction (ERFaci) in experiments performed in phase 5 of the Coupled Model Intercomparison Project. We find that the ensemble mean SW ERFari+aci of -1.40 +/- 0.56 W m(-2) comes roughly 25% from ERFari (-0.35 +/- 0.20 W m(-2)) and 75% from ERFaci (-1.04 +/- 0.67 W m(-2)). ERFari is made up of -0.62 +/- 0.30 W m(-2) due to aerosol scattering opposed by +0.26 +/- 0.12 W m(-2) due to aerosol absorption and is largest near emission sources. The ERFari from nonsulfate aerosols is +0.13 +/- 0.09 W m(-2), consisting of -0.15 +/- 0.11 W m(-2) of scattering and +0.29 +/- 0.15 W m(-2) of absorption. The change in clear-sky flux is a negatively biased measure of ERFari, as the presence of clouds reduces the magnitude and intermodel spread of ERFari by 40-50%. ERFaci, which is large both near and downwind of emission sources, is composed of -0.99 +/- 0.54 W m(-2) from enhanced cloud scattering, with much smaller contributions from increased cloud amount and absorption. In models that allow aerosols to affect ice clouds, large increases in the optical depth of high clouds cause substantial longwave and shortwave radiative anomalies. Intermodel spread in ERFaci is dominated by differences in how aerosols increase cloud scattering, but even if all models agreed on this effect, over a fifth of the spread in ERFaci would remain due solely to differences in total cloud amount. C1 [Zelinka, Mark D.; Taylor, Karl E.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. [Andrews, Timothy] Met Off Hadley Ctr, Exeter, Devon, England. [Forster, Piers M.] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England. RP Zelinka, MD (reprint author), Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. EM zelinka1@llnl.gov RI Taylor, Karl/F-7290-2011; Zelinka, Mark/C-4627-2011; Andrews, Timothy/C-5912-2014; Forster, Piers/F-9829-2010 OI Taylor, Karl/0000-0002-6491-2135; Zelinka, Mark/0000-0002-6570-5445; Andrews, Timothy/0000-0002-8248-8753; Forster, Piers/0000-0002-6078-0171 FU Office of Science at the DOE; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; Royal Society; EPSRC IAGP [EP/I014721/1] FX We thank Ulrike Burkhardt, Steve Ghan, Yi Ming, Rob Wood, and two anonymous reviewers for their useful comments on this work and Jin-Ho Yoon for providing CAM5 output. The work of M.D.Z. and K.E.T. is supported by the Regional and Global Climate Modeling Program of the Office of Science at the DOE and is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. T.A. is supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). P.M.F. is a Royal Society Wolfson Merit Award holder and supported by the EPSRC IAGP project EP/I014721/1. We acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups (listed in the section 2 of this paper) for producing and making available their model output. For CMIP the U.S. Department of Energy's Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. NR 21 TC 17 Z9 17 U1 1 U2 20 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 27 PY 2014 VL 119 IS 12 BP 7599 EP 7615 DI 10.1002/2014JD021710 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0BP UT WOS:000340247000034 ER PT J AU Liou, KN Takano, Y He, C Yang, P Leung, LR Gu, Y Lee, WL AF Liou, K. N. Takano, Y. He, C. Yang, P. Leung, L. R. Gu, Y. Lee, W. L. TI Stochastic parameterization for light absorption by internally mixed BC/dust in snow grains for application to climate models SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID HEXAGONAL ICE CRYSTALS; SIERRA-NEVADA SNOW; BLACK CARBON; OPTICAL-PROPERTIES; SPECTRAL ALBEDO; CIRRUS CLOUDS; RADIATIVE-TRANSFER; SINGLE-SCATTERING; GEOMETRIC-OPTICS; SURFACE AB A stochastic approach has been developed to model the positions of BC (black carbon)/dust internally mixed with two snow grain types: hexagonal plate/column (convex) and Koch snowflake (concave). Subsequently, light absorption and scattering analysis can be followed by means of an improved geometric-optics approach coupled with Monte Carlo photon tracing to determine BC/dust single-scattering properties. For a given shape (plate, Koch snowflake, spheroid, or sphere), the action of internal mixing absorbs substantially more light than external mixing. The snow grain shape effect on absorption is relatively small, but its effect on asymmetry factor is substantial. Due to a greater probability of intercepting photons, multiple inclusions of BC/dust exhibit a larger absorption than an equal-volume single inclusion. The spectral absorption (0.2-5 mu m) for snow grains internally mixed with BC/dust is confined to wavelengths shorter than about 1.4 mu m, beyond which ice absorption predominates. Based on the single-scattering properties determined from stochastic and light absorption parameterizations and using the adding/doubling method for spectral radiative transfer, we find that internal mixing reduces snow albedo substantially more than external mixing and that the snow grain shape plays a critical role in snow albedo calculations through its forward scattering strength. Also, multiple inclusion of BC/dust significantly reduces snow albedo as compared to an equal-volume single sphere. For application to land/snow models, we propose a two-layer spectral snow parameterization involving contaminated fresh snow on top of old snow for investigating and understanding the climatic impact of multiple BC/dust internal mixing associated with snow grain metamorphism, particularly over mountain/snow topography. C1 [Liou, K. N.; Takano, Y.; He, C.; Gu, Y.] Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. [Liou, K. N.; Takano, Y.; He, C.; Gu, Y.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Yang, P.] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX USA. [Leung, L. R.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Lee, W. L.] Acad Sinica, Res Ctr Environm Changes, Taipei 115, Taiwan. RP Takano, Y (reprint author), Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. EM ytakano@atmos.ucla.edu RI Yang, Ping/B-4590-2011; OI He, Cenlin/0000-0002-7367-2815 FU Department of Energy [DESC0006742]; National Science Foundation [AGS-0946315]; Texas A&M Research Foundation [S100097]; NASA [NNX11AK39G] FX This research was supported by the Department of Energy under grant DESC0006742, by the National Science Foundation under grant AGS-0946315, and by subcontract S100097 from the Texas A&M Research Foundation, which is sponsored by NASA under grant NNX11AK39G. Users can access the data from this paper via the authors without any restrictions. NR 54 TC 9 Z9 10 U1 1 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 27 PY 2014 VL 119 IS 12 BP 7616 EP 7632 DI 10.1002/2014JD021665 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AN0BP UT WOS:000340247000035 ER PT J AU Bezrukov, F Shaposhnikov, M AF Bezrukov, Fedor Shaposhnikov, Mikhail TI Higgs inflation at the critical point SO PHYSICS LETTERS B LA English DT Article ID STANDARD MODEL; 3 LOOPS; BOSON; MASS AB Higgs inflation can occur if the Standard Model (SM) is a self-consistent effective field theory up to inflationary scale. This leads to an upper bound on the top Yukawa coupling, y(t)(phys) < y(t)(crit) and thus on the mass of the top quark m(t). If m(t) is more than a few hundred of MeV below the critical value, the Higgs inflation predicts the universal values of inflationary indexes, r similar or equal to 0.003 and n(s) similar or equal to 0.97, independently on the SM parameters. We show that in the vicinity of the critical point y(t)(crit) the inflationary indexes acquire an essential dependence on m(t) and on the mass of the Higgs boson M-h. In particular, the amplitude of the gravitational waves can exceed considerably the universal value. (C) 2014 Elsevier B.V. C1 [Bezrukov, Fedor; Shaposhnikov, Mikhail] CERN, CH-1211 Geneva, Switzerland. [Bezrukov, Fedor] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Bezrukov, Fedor] Brookhaven Natl Lab, RIKEN BNL, Res Ctr, Upton, NY 11973 USA. [Shaposhnikov, Mikhail] Ecole Polytech Fed Lausanne, Inst Theor Phenomenes Phys, CH-1015 Lausanne, Switzerland. RP Bezrukov, F (reprint author), CERN, CH-1211 Geneva, Switzerland. EM Fedor.Bezrukov@uconn.edu; Mikhail.Shaposhnikov@epfl.ch RI EPFL, Physics/O-6514-2016; OI Bezrukov, Fedor/0000-0003-3601-1003 FU European Commission under the ERC Advanced Grant [BSMOXFORD 228169]; Swiss National Science Foundation [200020_149729/1] FX The authors would like to thank CERN Theory Division, where this paper was written, for hospitality. We thank Dmitry Gorbunov for helpful comments. The work of M.S. is supported in part by the European Commission under the ERC Advanced Grant BSMOXFORD 228169 and by the Swiss National Science Foundation 200020_149729/1. NR 47 TC 44 Z9 45 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUN 27 PY 2014 VL 734 BP 249 EP 254 DI 10.1016/j.physletb.2014.05.074 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL2GM UT WOS:000338943900049 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hoermann, N Hrubec, J Jeitler, M Kiesenhofer, W Kniinz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schoefbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B DeLentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J OcampoRios, AA Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C Du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Vizan Garcia, JM Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM De Jesus Damiao, D De Oliveira Martins, C De Souza, SF Malbouisson, H Malek, M Matos Figueiredo, D Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Tonelli Manganote, EJ Vilela Pereira, A Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, S Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, W Liu, S Mao, Y Qian, SJ Teng, H Wang, D Zhang, L Zou, W Avila, C Carrillo Montoya, CA Chaparro Sierra, LF Gomez, JP Gomez Moreno, B Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Korpela, A Tuuva, T Besancon, M Choudhury, S Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gel, D Goerlach, U Goetzmann, C Juillot, P LeBihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P ElMamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, 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CA CMS Collaboration TI Observation of a peaking structure in the J/psi phi mass spectrum from B-+/- -> J/psi phi K-+/- decays SO PHYSICS LETTERS B LA English DT Article AB A peaking structure in the J/psi phi mass spectrum near threshold is observed in B-+/- -> J/psi phi K-+/- decays, produced in pp collisions at root s = 7 TeV collected with the CMS detector at the LHC. The data sample, selected on the basis of the dimuon decay mode of the J/psi, corresponds to an integrated luminosity of 5.2 fb(-1). Fitting the structure to an S-wave relativistic Breit-Wigner lineshape above a three-body phase-space nonresonant component gives a signal statistical significance exceeding five standard deviations. The fitted mass and width values are m = 4148.0 +/- 2.4 (stat.) +/- 6.3 (syst.) MeV and Gamma = 28(-11)(+15) (stat.) +/- 19 (syst.) MeV, respectively. Evidence for an additional peaking structure at higher J/psi phi mass is also reported. (C) 2014 The Authors. Published by Elsevier B.V. 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[Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Oriemtale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Riccaa, G.; Gobbo, B.; La Licata, C.; Maronea, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Riccaa, G.; La Licata, C.; Maronea, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; La Cruz, I. Heredia-De; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzandos, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; FerreiraParracho, P. G.; Gallinaro, M.; RodriguesAntunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Attikis, A.; Abdulsalam, A.; Afanasiev, S.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De Lacruz, B.; Peris, A. Delgado; Vazquez, D. Dom-Nguez; Bedoya, C. Fernandez; Ramos, J. P. Fernandez; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Lopez, O. Gonzalez; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; De Martino, E. Navarro; Pelayo, J. Puerta; Olmeda, A. Quintario; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Cifuentes, J. A. Brochero; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; DuarteCampderros, J.; Fernandez, M.; Gomez, G.; Sanchez, J. Gonzalez; Graziano, A.; Jorda, C.; LopezVirto, A.; Marco, J.; Marco, R.; Rivero, C. Martinez; Matorras, F.; Sanchez, F. J. Munoz; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, IFCA, Santander, Spain. [Attikis, A.; Abdulsalam, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Da Browski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Loureno, C.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moneta, L.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Palencia Cortezon, E.; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; PimiA, M.; Piparo, D.; Plagge, M.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schafer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wohri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Konig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Attikis, A.; Abdulsalam, A.; Bachmair, F.; Bani, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Dunser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Nageli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Ivova Rikova, M.; Kilminster, B.; Millan Mejias, B.; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; KayisTopaksu, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Sunar Cerci, D.; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della egra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Vazquez Acosta, M.; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Abdulsalam, A.; Cline, D.; Cousins, R.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wurthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA USA. [Abdulsalam, A.; Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Abdulsalam, A.; Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; DiMarco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Luiggi Lopez, E.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Abdulsalam, A.; Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; NicolasKaufman, G.; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT USA. [Abdulsalam, A.; Adiguzel, A.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, M.; Martinez Outschoorn, V. I.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Muniz, G. Mitselmakher L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, Vic, Australia. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; GomezCeballos, G.; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stockli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Gonzalez Suarez, R.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. 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[Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Pioppi, M.] Univ Perugia, INFN Sez Perugia, I-06100 Perugia, Italy. [Pioppi, M.] Utah Valley Univ, Orem, UT 84058 USA. [Milenovic, P.] Inst Nucl Res, Moscow, Russia. [Milenovic, P.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. RP Chatrchyan, S (reprint author), CERN, CH-1211 Geneva 23, Switzerland. RI Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; Novaes, Sergio/D-3532-2012; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Gonzalez Caballero, Isidro/E-7350-2010; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Lokhtin, Igor/D-7004-2012; Gonzalez Suarez, Rebeca/L-6128-2014; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; de Jesus Damiao, Dilson/G-6218-2012; Haj Ahmad, Wael/E-6738-2016; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015 OI Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Novaes, Sergio/0000-0003-0471-8549; Scodellaro, Luca/0000-0002-4974-8330; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Gonzalez Suarez, Rebeca/0000-0002-6126-7230; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Ogul, Hasan/0000-0002-5121-2893; de Jesus Damiao, Dilson/0000-0002-3769-1680; Haj Ahmad, Wael/0000-0003-1491-0446; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France) [CNRS/IN2P3]; BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation For Polish Science - EU, Regional Development Fund; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation For Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 32 TC 44 Z9 45 U1 7 U2 83 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUN 27 PY 2014 VL 734 BP 261 EP 281 DI 10.1016/j.physletb.2014.05.055 PG 21 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL2GM UT WOS:000338943900051 ER PT J AU Klein-Boesing, C McLerran, L AF Klein-Boesing, Christian McLerran, Larry TI Geometrical scaling of direct-photon production in hadron collisions from RHIC to the LHC SO PHYSICS LETTERS B LA English DT Article ID GLUON DISTRIBUTION-FUNCTIONS; TRANSVERSE-MOMENTUM; LARGE NUCLEI; MULTIPLICITY; SATURATION; PROTONS; GLASS; QCD; PP AB Geometric scaling is a property of hadronic interactions predicted by theories of gluon saturation and expressing rates in terms of dimensionless ratios of transverse momentum to the saturation momentum. In this paper we consider production of photons in pp, dAu and AuAu collisions at root s(NN) = 200 GeV (RHIC) and in PbPb collisions at root s(NN) = 2760 GeV (LHC) and show that the yield of direct photons in the transverse momentum range 1 GeV < pT <= 4GeV/c satisfies geometric scaling. Excellent agreement with geometric scaling is obtained with the only free parameter of the saturation momentum determined previously via the dependence of the saturation momentum upon Bjorken x and centrality. (C) 2014 The Authors. Published by Elsevier B.V. C1 [Klein-Boesing, Christian] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Klein-Boesing, Christian] GSI Darmstadt, ExtreMe Matter Inst, Darmstadt, Germany. [McLerran, Larry] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [McLerran, Larry] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [McLerran, Larry] Cent China Normal Univ, Dept Phys, Wuhan, Peoples R China. RP Klein-Boesing, C (reprint author), Univ Munster, Inst Kernphys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. EM Christian.Klein-Boesing@wwu.de; mclerran@bnl.gov FU DOE [DE-AC02-98CH10886]; Alliance Program of the Helmholtz Association [HA216/EMMI] FX The research of L. McLerran is supported under DOE Contract No. DE-AC02-98CH10886. The research of C. Klein-Bosing is supported by the Alliance Program of the Helmholtz Association (HA216/EMMI). The authors thank Johanna Stachel and Klaus Reygers for the organization of the EMMI Rapid Reaction Task Force Direct-Photon Flow Puzzle and the invitation to GSI, where this work has been started. NR 26 TC 8 Z9 8 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUN 27 PY 2014 VL 734 BP 282 EP 285 DI 10.1016/j.physletb.2014.05.063 PG 4 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL2GM UT WOS:000338943900052 ER PT J AU Green, JR Engelhardt, M Krieg, S Negele, JW Pochinsky, AV Syritsyn, SN AF Green, J. R. Engelhardt, M. Krieg, S. Negele, J. W. Pochinsky, A. V. Syritsyn, S. N. TI Nucleon structure from Lattice QCD using a nearly physical pion mass SO PHYSICS LETTERS B LA English DT Article DE Lattice QCD; Nucleon structure; Form factors AB We report the first Lattice QCD calculation using the almost physical pion mass m(pi) = 149MeVthat agrees with experiment for four fundamental isovector observables characterizing the gross structure of the nucleon: the Dirac and Pauli radii, the magnetic moment, and the quark momentum fraction. The key to this success is the combination of using a nearly physical pion mass and excluding the contributions of excited states. An analogous calculation of the nucleon axial charge governing beta decay has inconsistencies indicating a source of bias at low pion masses not present for the other observables and yields a result that disagrees with experiment. (C) 2014 Elsevier B. V. C1 [Green, J. R.; Negele, J. W.; Pochinsky, A. V.] MIT, Cambridge, MA 02139 USA. [Green, J. R.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Engelhardt, M.] New Mexico State Univ, Dept Phys, Las Cruces, NM 88003 USA. [Krieg, S.] Berg Univ Wuppertal, D-42119 Wuppertal, Germany. [Krieg, S.] Forschungszentrum Julich, Julich Supercomp Ctr, IAS, D-52425 Julich, Germany. [Syritsyn, S. N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Syritsyn, S. N.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Syritsyn, SN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM ssyritsyn@quark.phy.bnl.gov OI Krieg, Stefan/0000-0002-8417-9823 FU Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357]; Forschungszentrum Julich; U.S. Department of Energy Office of Nuclear Physics [DE-FG02-94ER40818]; DOE [DE-FG02-96ER40965]; Office of Nuclear Physics in the U.S. Department of EnergyOffice of Science [DE-AC02-05CH11231]; RIKEN Foreign Postdoctoral Researcher Program; Deutsche Forschungsgemeinschaft [SFB-TRR 55] FX We thank Zoltan Fodor for useful discussions and the Budapest-Marseille- Wuppertal Collaborationfor making some of their configurations available to us. This research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under contract #DE-AC02-06CH11357, and resources at Forschungszentrum Julich. During this research J.R.G., S. K., J. W. N., A.V. P. and S. N. S. were supported in part by the U.S. Department of Energy Office of Nuclear Physics under grant #DE-FG02-94ER40818, M. E. was supported by DOE grant #DE-FG02-96ER40965, S. N. S. was supported by the Office of Nuclear Physics in the U.S. Department of EnergyOffice of Science under contract#DE-AC02-05CH11231 and by RIKEN Foreign Postdoctoral Researcher Program, and S. K. was supported in part by Deutsche Forschungsgemeinschaft through grant SFB-TRR 55. NR 43 TC 27 Z9 27 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUN 27 PY 2014 VL 734 BP 290 EP 295 DI 10.1016/j.physletb.2014.05.075 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL2GM UT WOS:000338943900054 ER PT J AU Abelev, B Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelliz, A Agrawal, N Ahammed, Z Ahmad, N Masoodi, AA Ahmed, I Ahn, SU Ahn, SA Aimo, I Aiola, S Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arborbr, N Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Awes, TC Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bairathi, V Bala, R Baldisseri, A Pedrosa, FBDS Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Berger, ME Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blau, D Blume, C Bock, F Boehmer, FV Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bornschein, J Bossu, F Botje, M Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Caliva, A Calvo Villar, E Camerini, P Roman, VC Carena, F Carena, W Carminati, F Diaz, AC Castellanos, JC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellatodo, DD Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contin, G Contreras, JG Cormier, TM Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dainese, A Dang, R Danu, A Das, D Das, I Das, K Das, S Dash, A Dash, S De, S Delagrange, H Deloff, A Denes, E D'Erasmo, G De Barros, GOV De Carol, A De Cataldo, G De Cuvelandan, J De Falco, A De Gruttolaac, D De Marco, N De Pasquale, S De Rooij, R Corchero, MAD Dietel, T Divia, R Di Bari, D Di Liberto, S Di Mauro, A Di Nezza, P Djuvsland, O Dobrin, A Dobrowolski, T Imenez, DD Donigus, B Dordic, O Dorheim, S Dubey, AK Dubla, A Ducroux, L Dupieux, P Majumdar, AKD Elia, D Engel, H Erazmus, B Erdal, HA Eschweiler, D Espagnon, B Estienne, M Esumi, S Evans, D Evdokimov, S Eyyubova, G Fabris, D Faivre, J Falchieri, D Fantoni, A Fasel, M Fehlker, D Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floratos, E Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Girard, MF Gaardhoje, JJ Gagliardi, M Gallio, M Gangadharan, DR Ganoti, P Garabatos, C Garcia-Solis, E Gargiulo, C Garishvili, I Gerhard, J Germain, M Gheata, A Gheata, M Ghidini, B Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Gladysz-Dziadus, E Glassel, P Gomez, R Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Graczykowski, LK Grajcarek, R Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Guilbaud, M Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Khan, KH Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hanratty, LD Hansen, A Harris, JW Hartmann, H Harton, A Hatzifotiadou, D Hayashi, S Hayrapetyan, A Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hicks, B Hippolyte, B Hladky, J Hristov, P Huang, M Humanic, TJ Hutter, D Hwang, DS Ianigro, JC Ilkaev, R Ilkiv, I Inaba, M Incani, E Innocenti, GM Ionita, C Ippolitov, M Irfan, M Ivanov, M Ivanov, V Ivanytskyi, O Jacholkowski, A Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalcher, S Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S KarasuUysal, A Karavichev, O Karavicheva, T Karpechev, E Kebschull, U Keidel, R Ketzer, B Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, B Kim, DW Kim, DJ Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, J Klein-Bosing, C Kluge, A Knichel, ML Knospe, AG Kobdaj, C Kohler, MK Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Konevskikh, A Kovalenko, V Kowalski, M Kox, S Meethaleveedu, GK Kral, J Kralik, I Kramer, F Kravcakova, A Krelina, M Kretz, M Krivda, M Krizek, F Krus, M Kryshen, E Krzewicki, M Kucera, V Kucheriaev, Y Kugathasan, T Kuhn, C Kuijer, PG Kulakov, I Kumar, J Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kushpil, S Kushpil, V Kweon, MJ Kwon, Y de Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A La Pointe, SL La Rocca, P Lea, R Lee, GR Legrand, I Lehnert, J Lemmon, RC Lenhardt, M Lenti, V Leogrande, E Leoncino, M Monzon, I Levai, P Li, S Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loggins, VR Loginov, V Lohner, D Loizides, C Lopez, X Torres, EL Lu, XG Luettig, P Lunardon, M Luo, J Luparello, G Luzzi, C Gago, AM Jacobs, PM Ma, R Maevskaya, A Mager, M Mahapatra, DP Maire, A Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A 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CA ALICE Collaboration TI Centrality, rapidity and transverse momentum dependence of J/Psi suppression in Pb-Pb collisions at root(NN)-N-S=2.76TeV SO PHYSICS LETTERS B LA English DT Article DE Relativistic heavy ion collisions; Quark gluon plasma; Quarkonium; J/Psi suppression; Experimental results ID QED RADIATIVE-CORRECTIONS; UNIVERSAL MONTE-CARLO; PP COLLISIONS; NUCLEAR COLLISIONS; ROOT-S=7 TEV; PHOTOS; MODEL AB The inclusive J/.nuclear modification factor (R-AA) in Pb-Pb collisions at root(NN)-N-S = 2.76TeVhas been measured by ALICE as a function of centrality in the e+ e-decay channel at mid-rapidity (| y| < 0.8) and as a function of centrality, transverse momentum and rapidity in the + -decay channel at forward-rapidity (2.5 < y < 4). The J/.yields measured in Pb-Pb are suppressed compared to those in ppcollisions scaled by the number of binary collisions. The RAAintegrated over a centrality range corresponding to 90% of the inelastic Pb-Pb cross section is 0.72 - 0.06(stat.) - 0.10(syst.) at mid-rapidity and 0.58 - 0.01(stat.) - 0.09(syst.) at forward-rapidity. At low transverse momentum, significantly larger values of RAAare measured at forward-rapidity compared to measurements at lower energy. These features suggest that a contribution to the J/.yield originates from charm quark (re) combination in the deconfined partonic medium. (C) 2014 The Authors. Published by Elsevier B. V. C1 [Grigoryan, A.; Gulkanyan, H.; Hayrapetyan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Limon, S. Vergara] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Grinyov, B.; Ivanytskyi, O.; Martynov, Y.; Trubnikov, V.; Zinovjev, G.; Zynovyev, M.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. 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A.; Vallero, S.; Vercellin, E.] Univ & Sez INFN, Dipartimento Fis, Turin, Italy. [Agostinelliz, A.; Akindinov, A.; Basile, M.; Bellini, F.; Cifarelli, L.; Colocci, M.; Falchieri, D.; Guerzoni, B.; Scioli, G.; Zichichi, A.] Univ & Sez INFN, Dipartimento Fis, Bologna, Italy. [Jacholkowski, A.; Petta, C.; Riggi, F.; Santagati, G.] Univ & Sez INFN, Dipartimento Fis, Catania, Italy. [Caffarri, D.; Festanti, A.; Francescon, A.; Lunardon, M.; Morando, M.; Moretto, S.; Scarlassara, F.; Segato, G.; Soramel, F.; Viesti, G.] Univ & Sez INFN, Dipartimento Fis, Padua, Italy. [De Carol, A.; De Gruttolaac, D.; De Pasquale, S.; Girard, M. Fusco; Pagano, P.; Virgili, T.] ER Caianiello Univ, Dipartimento Fis, Salerno, Italy. [De Carol, A.; De Gruttolaac, D.; De Pasquale, S.; Girard, M. Fusco; Pagano, P.; Virgili, T.] Grp Collegato INFN, Salerno, Italy. [Altini, V.; Ramello, L.; Sputowska, I.] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, P.; Ramello, L.; Sitta, M.; Sputowska, I.] Grp Collegato INFN, Alessandria, Italy. [Agostinelliz, A.; Altini, V.; Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fionda, F. M.; Fiore, E. M.; Ghidini, B.; Mastroserio, A.; Tangaro, M. A.; Terrevoli, C.] Dipartimento Interateneo Fisica M Merlin, Bari, Italy. [Agostinelliz, A.; Akindinov, A.; Altini, V.; Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fionda, F. M.; Fiore, E. M.; Ghidini, B.; Mastroserio, A.; Tangaro, M. A.; Terrevoli, C.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Christiansen, P.; Ljunggren, H. M.; Velasquez, A. Ortiz; Oskarsson, A.; Richert, T.; Sogaard, C.; Stenlund, E.] Lund Univ, Div Expt High Energy Phys, Lund, Sweden. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Rinella, G. Aglieri; Agostinelliz, A.; Akindinov, A.; Alici, A.; Alkin, A.; Andronic, A.; Augustinus, A.; Badala, A.; Baldisseri, A.; Pedrosa, F. Baltasar Dos Santos; Bercuci, A.; Betev, L.; Bhasin, A.; Bilandzic, A.; Bogdanov, A.; Borissov, A.; Buncic, P.; Caliva, A.; Roman, V. Canoa; Carena, F.; Carena, W.; Carminati, F.; Cavicchioli, C.; Cepila, J.; Chapeland, S.; Barroso, V. Chibante; Chochula, P.; Collu, A.; del Valle, Z. Conesa; Costa, F.; Dainese, A.; Danu, A.; Dash, A.; Deloff, A.; De Carol, A.; De Falco, A.; Divia, R.; Di Mauro, A.; Erazmus, B.; Floris, M.; Francescon, A.; Fuchs, U.; Gargiulo, C.; Gheata, A.; Gheata, M.; Giubellino, P.; Grigoras, A.; Grigoras, C.; Grosse-Oetringhaus, J. F.; Grosso, R.; Hayrapetyan, A.; Hristov, P.; Ionita, C.; Kalweit, A.; Kluge, A.; Kobdaj, C.; Kryshen, E.; Kugathasan, T.; Legrand, I.; Luzzi, C.; Mager, M.; Manzari, V.; Markert, C.; Martinengo, P.; Milano, L.; Morsch, A.; Muller, H.; Musa, L.; Niculescu, M.; Pinazza, O.; Poghosyan, M. G.; Reidt, F.; Revol, J. -P.; Riedler, P.; Riegler, W.; Rossegger, S.; Rossi, A.; Safarik, K.; Schukraft, J.; Schutz, Y.; Shahoyan, R.; Szczepankiewicz, A.; Martinez, A. Tarazona; Tauro, A.; Telesca, A.; Vyvre, P. Vande; Van Hoorne, J. W.; Volpe, G.; Vonhaller, B.; Vranic, D.; Zimmermann, M. B.] European Org Nucl Res CERN, Geneva, Switzerland. [Ketzer, B.] Tech Univ Munich, Excellence Cluster Univ, D-80290 Munich, Germany. [Alme, J.; Erdal, H. A.; Hetland, K. F.; Kileng, B.] Bergen Univ Coll, Fac Engn, Bergen, Norway. [Broz, M.; Meres, M.; Pikna, M.; Sitar, B.; Szarka, I.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Adam, J.; Bielcik, J.; Cepila, J.; Krelina, M.; Krus, M.; Pachr, M.; Petracek, V.; Petran, M.; Pospisil, V.; Schulc, M.; Smakal, R.; Spacek, M.; Wagner, V.; Zach, C.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, Prague, Czech Republic. [Bombara, M.; Kravcakova, A.; Vrlakova, J.] Safarik Univ, Fac Sci, Kosice, Slovakia. [Alt, T.; Bach, M.; Bornschein, J.; De Cuvelandan, J.; Eschweiler, D.; Gerhard, J.; Gorbunov, S.; Hartmann, H.; Hutter, D.; Kalcher, S.; Kirsch, S.; Kisel, I.; Kollegger, T.; Kretz, M.; Lindenstruth, V.; Painke, F.; Rettig, F.; Rohr, D.] Goethe Univ Frankfurt, Frankfurt Inst Adv Studies, D-60054 Frankfurt, Germany. [Agostinelliz, A.; Baek, Y. W.; Jung, H.; Kim, D. W.; Kim, J. S.; Kim, M.; Oh, S. K.] Gangneung Wonju Natl Univ, Kangnung, South Korea. [Bhattacharjee, B.] Gauhati Univ, Dept Phys, Gauhati, India. [Krizek, F.; Pohjoisaho, E. H. O.; Rasanen, S. S.] HIP, Helsinki, Finland. [Shigaki, K.; Sugitate, T.; Yano, S.] Hiroshima Univ, Hiroshima, Japan. [Agrawal, N.; Behera, N. K.; De, S.; Jena, S.; Meethaleveedu, G. Koyithatta; Kumar, J.; Nandi, B. K.; Nyatha, A.; Pant, D.; Pujahari, P.; Varma, R.] Indian Inst Technol Bombay IIT, Mumbai, Maharashtra, India. [Mazumder, R.; Mishra, A. N.; Roy, A.] Indian Inst Technol Indore IITI, Indore, India. [Kweon, M. J.] Inha Univ, Coll Nat Sci, Inchon, South Korea. [del Valle, Z. Conesa; Das, I.; Espagnon, B.; Hadjidakis, C.; Lakomov, I.; Suire, C.; Takaki, J. D. Tapia; Palomo, L. Valencia] Univ Paris 11, CNRS IN2P3, IPNO, Orsay, France. [Bottger, S.; Breitner, T.; Engel, H.; Kebschull, U.; Lara, C.; Ulrich, J.] Goethe Univ Frankfurt, Inst Informat, D-60054 Frankfurt, Germany. [Agostinelliz, A.; Akindinov, A.; Alici, A.; Alkin, A.; Andronic, A.; Appelshauser, H.; Arslandok, M.; Bailhache, R.; Baumann, C.; Beck, H.; Blume, C.; Book, J.; Broker, T. A.; Buesching, H.; Donigus, B.; Heckel, S. T.; Kamin, J.; Kramer, F.; Kulakov, I.; Lehnert, J.; Luettig, P.; Marquard, M.; Reichelt, P.; Renfordt, R.; Sahlmuller, B.; Schuchmann, S.; Peloni, A. Tarantola; Toia, A.; Ulery, J.; Zyzak, M.] Goethe Univ Frankfurt, Inst Kernphys, D-60054 Frankfurt, Germany. [Oeschler, H.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Anielski, J.; Bathen, B.; Dietel, T.; Feldkamp, L.; Haake, R.; Heide, M.; Klein-Bosing, C.; Passfeld, A.; Rascanu, B. T.; Wessels, J. P.; Westerhoff, U.; Wilde, M.; Zimmermann, M. B.] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Maire, A.; Molnar, L.; Roy, C.; Castro, X. Sanchez] Univ Strasbourg, CNRS IN2P3, IPHC, Strasbourg, France. [Bogolyubsky, M.; Evdokimov, S.; Kharlov, Y.; Patalakha, D. I.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.; Stolpovskiy, M.] Inst High Energy Phys, Protvino, Russia. [Agostinelliz, A.; Finogeev, D.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A.; Kurepin, A. B.; Maevskaya, A.; Pshenichnov, I.; Reshetin, A.] Acad Sci, Inst Nucl Res, Moscow, Russia. [Agostinelliz, A.; Akindinov, A.; Bertens, R. A.; Bianchin, C.; Bjelogrlic, S.; Caliva, A.; De Rooij, R.; Dobrin, A.; Dubla, A.; Grelli, A.; La Pointe, S. L.; Leogrande, E.; Lodato, D. F.; Luparello, G.; Mischke, A.; Nooren, G.; Peitzmann, T.; Reicher, M.; Rocco, E.; Snellings, R. J. M.; Thomas, D.; Van Leeuwen, M.; Veldhoen, M.; Yang, H.; Zhou, Y.] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Agostinelliz, A.; Akindinov, A.; Kiselev, S.; Mal'Kevich, D.; Mikhaylov, K.; Nedosekin, A.; Sultanov, R.; Voloshin, K.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Agostinelliz, A.; Ban, J.; Kalinak, P.; Kralik, I.; Krivda, M.; Musinsky, J.; Sandor, L.; Vala, M.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia. [Hladky, J.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Baral, R. C.; Cunqueiro, L.; Mahapatra, D. P.; Sahu, P. K.; Sharma, N.] Inst Phys, Bhubaneswar 751007, Orissa, India. [Danu, A.; Felea, D.; Gheata, M.; Haiduc, M.; Mitu, C. M.; Niculescu, M.; Sevcenco, A.; Stan, I.; Zgurabi, I. S.] ISS, Bucharest, Romania. [Agostinelliz, A.; Cuautle, E.; Bustamante, R. T. Jimenez; de Guevara, P. Ladron; Cervantes, I. Maldonado; Paic, G.; Castro, X. Sanchez] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Belmont-Moreno, E.; Menchaca-Rocha, A.; Sandoval, A.; Serradilla, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. [Bossu, F.; Buthelezi, Z.; Foertsch, S.; Murray, S.; Steyn, G.; Vilakazi, Z.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Rogochaya, E.; Shabratova, G.; Vala, M.; Vodopyanov, A.; Zaporozhets, S.] JINR, Dubna, Russia. [Oh, S. K.] Konkuk Univ, Seoul, South Korea. [Ahn, S. U.; Ahn, S. A.; Jang, H. J.; Kim, D. W.] Korea Inst Sci & Technol Informat, Taejon, South Korea. [KarasuUysal, A.; Okatan, A.] KTO Karatay Univ, Konya, Turkey. [Baek, Y. W.; Barret, V.; Bastid, N.; Crochet, P.; Dupieux, P.; Li, S.; Lopez, X.; Manso, F.; Marchisone, M.; Porteboeuf-Houssais, S.; Rosnet, P.; Palomo, L. Valencia; Vulpescu, B.; Zhang, X.] Univ Blaise Pascal, Clermont Univ, CNRS IN2P3, LPC, Cleveland, Qld, Australia. [Arborbr, N.; Balbastre, G. Conesa; Faivre, J.; Furget, C.; Guernane, R.; Kox, S.; Mares, J.; Real, J. S.; Silvestre, C.] Univ Grenoble 1, CNRS IN2P3, LPSC, Grenoble, France. [Arborbr, N.; Balbastre, G. Conesa; Faivre, J.; Furget, C.; Guernane, R.; Kox, S.; Mares, J.; Real, J. S.; Silvestre, C.] Univ Grenoble 1, CNRS IN2P3, LPSC, Grenoble, France. [Bianchi, N.; Diaz, A. Casanova; Cunqueiro, L.; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, A. R.; Ronchetti, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Ricci, R. A.; Vannucci, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Bock, F.; Cosentino, M. R.; Gangadharan, D. R.; Loizides, C.; Jacobs, P. M.; Ploskon, M.; Porter, J.; Symons, T. J. M.; Zhang, X.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Abelev, B.; Garishvili, I.; Soltz, R.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Bogdanov, A.; Grigoriev, V.; Kaplin, V.; Kondratyeva, N.; Ter Minasyan, A.] Moscow Engn Phys Inst, Moscow, Russia. [Deloff, A.; Dobrowolski, T.; Ilkiv, I.; Kurashvili, P.; Redlich, K.; Siemiarczuk, T.; Stefanek, G.; Wilk, G.] Natl Ctr Nucl Studies, Warsaw, Poland. [Andrei, C.; Berceanu, I.; Bercuci, A.; Herghelegiu, A.; Petris, M.; Petrovici, M.; Pop, A.; Schiaua, C.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Mohanty, B.; Singha, S.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bearden, I. G.; Bilandzic, A.; Boggild, H.; Chojnacki, M.; Christensen, C. H.; Gaardhoje, J. J.; Gulbrandsen, K.; Hansen, A.; Nielsen, B. S.; Zaccolo, V.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Agostinelliz, A.; Botje, M.; Christakoglou, P.; Kuijer, P. G.; Lara, C. E. Perez; Manso, A. Rodriguez] Natl Inst Subat Phys, Nikhef, Amsterdam, Netherlands. [Lemmon, R. C.; Romita, R.] Nucl Phys Grp, STFC Daresbury Lab, Daresbury, Cheshire, England. [Adamova, D.; Bielcikova, J.; Ferencei, J.; Krizek, F.; Kucera, V.; Kushpil, S.; Sumbera, M.; Vajzer, M.] Acad Sci Czech Republic, Nucl Phys Inst, Rez, Czech Republic. [Altini, V.; Awes, T. C.; Cormier, T. M.; Ganoti, P.; Silvermyr, D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Berdnikov, Y.; Ivanov, V.; Khanzadeev, A.; Kryshen, E.; Malaev, M.; Nikulin, V.; Riabov, V.; Ryabov, Y.; Zhalov, M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Cherney, M.; Nilsen, B. S.; Seger, J. E.] Creighton Univ, Dept Phys, Omaha, NE 68178 USA. [Aggarwal, M. M.; Bhati, A. K.; Rathee, D.] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Floratos, E.; Ganoti, P.; Spyropoulou-Stassinaki, M.; Vasileiou, M.] Univ Athens, Dept Phys, Athens, Greece. [Azmi, M. D.; Cleymans, J.; Murray, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Bala, R.; Bhasin, A.; Gupta, A.; Gupta, R.; Potukuchi, B.; Rohni, S.; Sambyal, S.; Sharma, S.; Singh, R.] Univ Jammu, Dept Phys, Jammu 180004, India. [Bairathi, V.; Raniwala, R.; Raniwala, S.] Univ Rajasthan, Dept Phys, Jaipur, Rajasthan, India. [Agostinelliz, A.; Anguelov, V.; Bock, F.; Busch, O.; Fasel, M.; Glassel, P.; Grajcarek, R.; Klein, J.; Kweon, M. J.; Lohner, D.; Lu, X. -G.; Maire, A.; Perez, J. Mercado; Oeschler, H.; Oyama, K.; Pachmayer, Y.; Reygers, K.; Schicker, R.; Stachel, J.; Stiller, J. H.; Vallero, S.; Volkl, M. A.; Wang, Y.; Wilkinson, J.; Windelband, B.; Winn, M.; Zimmermann, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Agnello, M.; Aimo, I.; Bedda, C.] Politecn Torino, Turin, Italy. [Browning, T. A.; Scharenberg, R. P.; Srivastava, B. K.] Purdue Univ, W Lafayette, IN 47907 USA. [Borissov, A.; Seo, J.; Song, J.; Yic, J.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Agostinelliz, A.; Akindinov, A.; Andronic, A.; Arsene, I. C.; Averbeck, R.; Braun-Munzinger, P.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Knichel, M. L.; Kohler, M. K.; Krzewicki, M.; Lenhardt, M.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Otwinowski, J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thader, J.; Vranic, D.; Wagner, J.] GSI Helmholtzzentrum Schwerionenforsch, Res Div, Darmstadt, Germany. [Andronic, A.; Arsene, I. C.; Averbeck, R.; Braun-Munzinger, P.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Knichel, M. L.; Kohler, M. K.; Krzewicki, M.; Lenhardt, M.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Otwinowski, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thader, J.; Vranic, D.; Wagner, J.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, T.; Planinic, M.; Poljak, N.] Rudjer Boskovic Inst, Zagreb, Croatia. [Agostinelliz, A.; Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Vyushin, A.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Chattopadhyay, S.; Das, D.; Das, K.; Majumdar, A. K. Dutta; Khan, P.; Paul, B.; Roy, P.; Sinha, T.] Saha Inst Nucl Phys, Kolkata, India. [Alexandre, D.; Barnby, L. S.; Evans, D.; Hanratty, L. D.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Scott, P. A.; Baillie, O. Villalobos] Univ Birmingham, Dept Phys & Astron, Birmingham, W Midlands, England. [Calvo Villar, E.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [De Cataldo, G.; Elia, D.; Lenti, V.; Nappicx, E.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Alici, A.; Antonioli, P.; Cindolo, F.; Hatzifotiadou, D.; Margotti, A.; Nania, R.; Noferini, F.; Pesci, A.; Pinazza, O.; Preghenella, R.; Scapparone, E.; Williams, M. C. S.; Zampolli, C.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Cicalo, C.; Masoni, A.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Badala, A.; Palmeri, A.; Pappalardo, G. S.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Antinori, F.; Dainese, A.; Fabris, D.; Toia, A.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Di Liberto, S.; Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Aimo, I.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Bruna, E.; Bufalino, S.; Cerello, P.; De Marco, N.; Feliciello, A.; La Pointe, S. L.; Manceau, L.; Oppedisano, C.; Prino, F.; Scomparin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Agostinelliz, A.; Aphecetche, L.; Batigne, G.; Bergognon, A. A. E.; Bregant, M.; Delagrange, H.; Erazmus, B.; Estienne, M.; Germain, M.; Lardeux, A.; Garcia, G. Martinez; Blanco, J. Martin; Mas, A.; Massacrier, L.; Morreale, A.; Pillot, P.; Ronflette, L.; Samsonov, V.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.] Univ Nantes, Ecole Mines Nantes, SUBATECH, Nantes, France. [Kobdaj, C.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Berger, M. E.; Boehmer, F. V.; Ketzer, B.] Tech Univ Munich, D-80290 Munich, Germany. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Gorlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Rybicki, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Monzon, I. Leon; Podesta-Lerma, P. L. M.; Rodriguez, F. J. Sanchez] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De Barros, G. O. V.; imenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Fernandes, C. Lagana; De Godoy, D. A. Moreira; Munhoz, M. G.; Da Silva, A. C. Oliveira; Filho, E. Pereira De Oliveira; Suaide, A. A. P.; de Toledo, A. Szanto] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellatodo, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas, Campinas, Brazil. [Bellwied, R.; Chinellatodo, D. D.; Jayarathna, P. H. S. Y.; Jena, S.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.; Weber, M.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Kral, J.; Morreale, A.; Rak, J.; Trzaska, W. H.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Figueredo, M. A. S.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Sano, M.; Watanabe, D.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Planinic, M.; Poljak, N.; Simatovic, G.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Guilbaud, M.; Ianigro, J. -C.; Tieulent, R.; Uras, A.; Zoccarato, Y.] Univ Lyon 1, CNRS IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Vorobyev, I.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Ahammed, Z.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Vestfold Univ Coll, Tonsberg, Norway. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pawlak, T.; Peryt, W.; Pluta, J.; Szymanski, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Borissov, A.; Cormier, T. M.; Dobrin, A.; Mlynarz, J.; Prasad, S. K.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Agocs, A. G.; Barnafoldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Olah, L.; Pochybova, S.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Aronsson, T.; Caines, H.; Connors, M. E.; Harris, J. W.; Hicks, B.; Ma, R.; Oh, S.; Reed, R. J.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, B.; Kim, M.; Kim, T.; Kwon, Y.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] ZTT, Fachhochschule Worms, Worms, Germany. RP Abelev, B (reprint author), Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. RI Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Castillo Castellanos, Javier/G-8915-2013; Inst. of Physics, Gleb Wataghin/A-9780-2017; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Guber, Fedor/I-4271-2013; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; feofilov, grigory/A-2549-2013; Barnafoldi, Gergely Gabor/L-3486-2013; Wagner, Vladimir/G-5650-2014; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Sevcenco, Adrian/C-1832-2012; Ahmed, Ijaz/E-9144-2015; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Barnby, Lee/G-2135-2010; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Yang, Hongyan/J-9826-2014; Felea, Daniel/C-1885-2012; Kucera, Vit/G-8459-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Vajzer, Michal/G-8469-2014; Cosentino, Mauro/L-2418-2014; Bregant, Marco/I-7663-2012; Takahashi, Jun/B-2946-2012; Kovalenko, Vladimir/C-5709-2013; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014 OI Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Castillo Castellanos, Javier/0000-0002-5187-2779; Pshenichnov, Igor/0000-0003-1752-4524; Guber, Fedor/0000-0001-8790-3218; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Peitzmann, Thomas/0000-0002-7116-899X; Sevcenco, Adrian/0000-0002-4151-1056; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barnby, Lee/0000-0001-7357-9904; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Felea, Daniel/0000-0002-3734-9439; Cosentino, Mauro/0000-0002-7880-8611; Takahashi, Jun/0000-0002-4091-1779; Kovalenko, Vladimir/0000-0001-6012-6615; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323 FU Grid centres; Worldwide LHC Computing Grid (WLCG) Collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cient fico e Tecnol gico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace FX The ALICE Collaborationgratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) Collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cient fico e Tecnol gico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi -Museo Storico della Fisica e Centro Studi e Ricerche " Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, M xico, ALFA-EC and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Science Centre, Poland; Ministry of National Education/ Institute for Atomic Physics and CNCS-UEFISCDI -Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Econom a y Competitividad (MINECO) of Spain, Xunta de Galicia (Conseller a de Educaci n), CEADEN, Cubaenerg a, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 51 TC 58 Z9 59 U1 4 U2 81 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUN 27 PY 2014 VL 734 BP 314 EP 327 DI 10.1016/j.physletb.2014.05.064 PG 14 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL2GM UT WOS:000338943900058 ER PT J AU Dougherty, MJ Tran, HM Stavila, V Knierim, B George, A Auer, M Adams, PD Hadi, MZ AF Dougherty, Michael J. Tran, Huu M. Stavila, Vitalie Knierim, Bernhard George, Anthe Auer, Manfred Adams, Paul D. Hadi, Masood Z. TI Cellulosic Biomass Pretreatment and Sugar Yields as a Function of Biomass Particle Size SO PLOS ONE LA English DT Article ID IONIC LIQUID PRETREATMENT; 1-ETHYL-3-METHYLIMIDAZOLIUM ACETATE; ENZYMATIC SACCHARIFICATION; LIGNIN CONTENT; CORN STOVER; HYDROLYSIS; DECONSTRUCTION; DIGESTIBILITY; CELLULASE; ACID AB Three lignocellulosic pretreatment techniques (ammonia fiber expansion, dilute acid and ionic liquid) are compared with respect to saccharification efficiency, particle size and biomass composition. In particular, the effects of switchgrass particle size (32-200) on each pretreatment regime are examined. Physical properties of untreated and pretreated samples are characterized using crystallinity, surface accessibility measurements and scanning electron microscopy (SEM) imaging. At every particle size tested, ionic liquid (IL) pretreatment results in greater cell wall disruption, reduced crystallinity, increased accessible surface area, and higher saccharification efficiencies compared with dilute acid and AFEX pretreatments. The advantages of using IL pretreatment are greatest at larger particle sizes (>75 mu m). C1 [Dougherty, Michael J.; Tran, Huu M.; Knierim, Bernhard; George, Anthe; Auer, Manfred; Adams, Paul D.; Hadi, Masood Z.] Joint BioEnergy Inst, Emeryville, CA USA. [Dougherty, Michael J.; Tran, Huu M.; Stavila, Vitalie; George, Anthe; Hadi, Masood Z.] Sandia Natl Labs, Livermore, CA USA. [Knierim, Bernhard; Auer, Manfred; Adams, Paul D.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA USA. [Adams, Paul D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Hadi, MZ (reprint author), NASA, Ames Res Ctr, Space BioSci Div, Synthet Biol Program, Moffett Field, CA 94035 USA. EM Masood.Hadi@NASA.gov RI Adams, Paul/A-1977-2013 OI Adams, Paul/0000-0001-9333-8219 FU U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U. S. Department of Energy. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 21 TC 5 Z9 5 U1 4 U2 33 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 27 PY 2014 VL 9 IS 6 AR e100836 DI 10.1371/journal.pone.0100836 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK6BK UT WOS:000338512200067 PM 24971883 ER PT J AU Probst, AJ Birarda, G Holman, HYN DeSantis, TZ Wanner, G Andersen, GL Perras, AK Meck, S Volkel, J Bechtel, HA Wirth, R Moissl-Eichinger, C AF Probst, Alexander J. Birarda, Giovanni Holman, Hoi-Ying N. DeSantis, Todd Z. Wanner, Gerhard Andersen, Gary L. Perras, Alexandra K. Meck, Sandra Voelkel, Joerg Bechtel, Hans A. Wirth, Reinhard Moissl-Eichinger, Christine TI Coupling Genetic and Chemical Microbiome Profiling Reveals Heterogeneity of Archaeome and Bacteriome in Subsurface Biofilms That Are Dominated by the Same Archaeal Species SO PLOS ONE LA English DT Article ID PEARLS-LIKE MORPHOLOGY; NATURAL COMMUNITIES; SULFIDIC SPRINGS; SM1 EURYARCHAEON; DIVERSITY; GROWTH; LIPIDS; EPSILONPROTEOBACTERIA; ENVIRONMENTS; POPULATIONS AB Earth harbors an enormous portion of subsurface microbial life, whose microbiome flux across geographical locations remains mainly unexplored due to difficult access to samples. Here, we investigated the microbiome relatedness of subsurface biofilms of two sulfidic springs in southeast Germany that have similar physical and chemical parameters and are fed by one deep groundwater current. Due to their unique hydrogeological setting these springs provide accessible windows to subsurface biofilms dominated by the same uncultivated archaeal species, called SM1 Euryarchaeon. Comparative analysis of infrared imaging spectra demonstrated great variations in archaeal membrane composition between biofilms of the two springs, suggesting different SM1 euryarchaeal strains of the same species at both aquifer outlets. This strain variation was supported by ultrastructural and metagenomic analyses of the archaeal biofilms, which included intergenic spacer region sequencing of the rRNA gene operon. At 16S rRNA gene level, PhyloChip G3 DNA microarray detected similar biofilm communities for archaea, but site-specific communities for bacteria. Both biofilms showed an enrichment of different deltaproteobacterial operational taxonomic units, whose families were, however, congruent as were their lipid spectra. Consequently, the function of the major proportion of the bacteriome appeared to be conserved across the geographic locations studied, which was confirmed by dsrB-directed quantitative PCR. Consequently, microbiome differences of these subsurface biofilms exist at subtle nuances for archaea (strain level variation) and at higher taxonomic levels for predominant bacteria without a substantial perturbation in bacteriome function. The results of this communication provide deep insight into the dynamics of subsurface microbial life and warrant its future investigation with regard to metabolic and genomic analyses. C1 [Probst, Alexander J.; Perras, Alexandra K.; Meck, Sandra; Wirth, Reinhard; Moissl-Eichinger, Christine] Univ Regensburg, Inst Microbiol, D-93053 Regensburg, Germany. [Probst, Alexander J.; Perras, Alexandra K.; Meck, Sandra; Wirth, Reinhard; Moissl-Eichinger, Christine] Univ Regensburg, Archaea Ctr, D-93053 Regensburg, Germany. [Birarda, Giovanni; Holman, Hoi-Ying N.; Andersen, Gary L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Environm Biotechnol, Berkeley, CA 94720 USA. [Probst, Alexander J.; DeSantis, Todd Z.] Second Genome Inc, Dept Bioinformat, San Francisco, CA USA. [Wanner, Gerhard] Ludwig Maximilians Univ Munchen, Dept Biol 1, Biozentrum, Planegg Martinsried, Germany. [Voelkel, Joerg] Tech Univ Munich, Dept Geomorphol & Soil Sci, Ctr Life & Food Sci Weihenstephan, Freising Weihenstephan, Germany. [Bechtel, Hans A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Moissl-Eichinger, C (reprint author), Univ Regensburg, Inst Microbiol, D-93053 Regensburg, Germany. EM christine.moissl-eichinger@ur.de RI Holman, Hoi-Ying/N-8451-2014; Moissl-Eichinger, Christine/A-6682-2015; Andersen, Gary/G-2792-2015; Probst, Alexander/K-2813-2016 OI Holman, Hoi-Ying/0000-0002-7534-2625; Moissl-Eichinger, Christine/0000-0001-6755-6263; Andersen, Gary/0000-0002-1618-9827; FU DFG [MO 1977 3-1]; German National Academic Foundation (Studienstiftung des Deutschen Volkes); Office of Biological and Environmental Research's Structural Biology Program, Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory; German Research Foundation (DFG) FX This research was funded by the DFG (grant MO 1977 3-1). AJP was supported by the German National Academic Foundation (Studienstiftung des Deutschen Volkes). The SR-FTIR spectromicroscopy work was conducted through the Berkeley Synchrotron Infrared Structural Biology (BSISB) Program at the Advanced Light Source, which is supported by the Director, Office of Biological and Environmental Research's Structural Biology Program, Office of Science of the U.S. Department of Energy through contract DE-AC02-05CH11231 with Lawrence Berkeley National Laboratory. This work was supported by the German Research Foundation (DFG) within the funding programme Open Access Publishing. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 57 TC 5 Z9 6 U1 0 U2 19 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 27 PY 2014 VL 9 IS 6 AR e99801 DI 10.1371/journal.pone.0099801 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK6BK UT WOS:000338512200014 PM 24971452 ER PT J AU Pang, LG Wang, Q Wang, XN AF Pang, Longgang Wang, Qun Wang, Xin-Nian TI Relics of minijets amid anisotropic flows in high-energy heavy-ion collisions SO PHYSICAL REVIEW C LA English DT Article ID NUCLEUS-NUCLEUS COLLISIONS; PB-PB COLLISIONS; CENTRALITY DEPENDENCE; ANGULAR-CORRELATIONS; ROOT-S(NN)=2.76 TEV; PARTICLE-PRODUCTION; JET CORRELATIONS; TRANSPORT MODEL; PPB COLLISIONS; LONG-RANGE AB Two-dimensional low-p(T) dihadron correlations in azimuthal angle phi and pseudorapidity eta in high-energy heavy-ion collisions are investigated within both the HIJING Monte Carlo model and an event-by-event (3 + 1)D ideal hydrodynamic model. Without final-state interaction and collective expansion, dihadron correlations from HIJING simulations have a typical structure from minijets that contains a near-side two-dimensional peak and an away-side ridge along the eta direction. In contrast, event-by-event (3 + 1)D ideal hydrodynamic simulations with fluctuating initial conditions from the HIJING + AMPT model produce a strong dihadron correlation that has an away-side as well as a near-side ridge. Relics of intrinsic dihadron correlation from minijets in the initial conditions still remain as superimposed on the two ridges. By varying initial conditions from HIJING + AMPT, we study effects of minijets, nonvanishing initial flow, and longitudinal fluctuation on the final-state dihadron correlations. With a large rapidity gap, one can exclude near-side correlations from minijet relics and dihadron correlations can be described by the superposition of harmonic flows up to the sixth order. When long-range correlations with a large rapidity gap are subtracted from short-range correlations with a small rapidity gap, the remaining near-side short-range dihadron correlation is shown to result mainly from relics of minijets. Low-transverse-momentum hadron yields per trigger (p(T)(trig) < 4 GeV/c, p(T)(asso) < 2 GeV/c) owing to this short-range correlation in central heavy-ion collisions are enhanced over that in peripheral heavy-ion collisions and p + p collisions, while widths in azimuthal angle remain the same, in qualitative agreement with experimental data. The enhancement owing to influence by the transverse expansion of the bulk medium is also shown to increase with centrality and colliding energy but to be insensitive to the kinetic freeze-out temperature. C1 [Pang, Longgang; Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Pang, Longgang; Wang, Xin-Nian] Cent China Normal Univ, Key Lab Quarks & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Pang, Longgang; Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Wang, Qun] Univ Sci & Technol China, Interdisciplinary Ctr Theoret Study, Hefei 230026, Peoples R China. [Wang, Qun] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China. RP Pang, LG (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. OI Wang, Xin-Nian/0000-0002-9734-9967 FU National Natural Science Foundation of China [11221504, 11125524]; Major State Basic Research Development Program in China [2014CB845404]; Chinese Ministry of Science and Technology [2014DFG02050]; JET Collaboration; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, U.S. Department of Energy [DE-AC02-05CH11231] FX We would like to thank Wei Li, Victor Roy, and Fuqiang Wang for helpful discussions. This work was supported by the National Natural Science Foundation of China under Grants No. 11221504 and No. 11125524, the Major State Basic Research Development Program in China (Grant No. 2014CB845404), Chinese Ministry of Science and Technology under Grant No. 2014DFG02050, and the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231 and within the framework of the JET Collaboration. NR 97 TC 8 Z9 8 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 27 PY 2014 VL 89 IS 6 AR 064910 DI 10.1103/PhysRevC.89.064910 PG 18 WC Physics, Nuclear SC Physics GA AK7UD UT WOS:000338632300004 ER PT J AU Suchyta, S Liddick, SN Chiara, CJ Walters, WB Carpenter, MP Crawford, HL Grinyer, GF Gurdal, G Klose, A McCutchan, EA Pereira, J Zhu, S AF Suchyta, S. Liddick, S. N. Chiara, C. J. Walters, W. B. Carpenter, M. P. Crawford, H. L. Grinyer, G. F. Guerdal, G. Klose, A. McCutchan, E. A. Pereira, J. Zhu, S. TI beta and isomeric decay of V-64 SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON-RICH NUCLEI; LEVEL STRUCTURE; SHELL CLOSURES; DEFORMATION; ISOTOPES; REGION; MASSES; SYSTEM; BEAMS AB Background: Collectivity has been inferred in Cr-64 based on measurements of the excitation energy of the first excited 2(+) state and B(E2;2(1)(+) -> 0(1)(+)) value. However, the energy of the 2(1)(+) state in Cr-64 is not precisely known. Purpose: The objective was to precisely determine the energy of the 2(1)(+) -> 0(1)(+) transition in Cr-64 following the beta decay of V-64. Method: V-64 ions were produced by projectile fragmentation at the National Superconducting Cyclotron Laboratory and stopped in a double-sided Si strip detector. V-64 isomeric and beta-delayed gamma rays were detected in an ancillary array of high-purity Ge detectors in order to determine the energies of excited states in V-64 and Cr-64. Results: The first excited 2(+) state in Cr-64 was populated following the beta decay of V-64, and an energy of 430(2) keV was determined. Additionally, an isomeric state in V-64 with an energy of 81.0(7) keV and a half-life less than 1 mu s was discovered. Conclusion: The excitation energy of the 2(1)(+) state in Cr-64 has been precisely determined and an isomeric state is identified in V-64 for the first time. C1 [Suchyta, S.; Liddick, S. N.; Klose, A.; Pereira, J.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Suchyta, S.; Liddick, S. N.; Klose, A.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Chiara, C. J.; Walters, W. B.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Chiara, C. J.; Carpenter, M. P.; McCutchan, E. A.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Crawford, H. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Grinyer, G. F.] CEA DSM CNRS IN2P3, GANIL, F-14076 Caen, France. [Guerdal, G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Suchyta, S (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. RI Carpenter, Michael/E-4287-2015 OI Carpenter, Michael/0000-0002-3237-5734 FU NSF (NSCL) [PHY-1102511]; DOE (NNSA) [DE-NA0000979]; ANL [DE-AC02-06CH11357]; UM [DE-FG02-94-ER40834] FX This work was funded in part by the NSF under Contract No. PHY-1102511 (NSCL) and the DOE under Contract No. DE-NA0000979 (NNSA), Contract No. DE-AC02-06CH11357 (ANL), and Grant No. DE-FG02-94-ER40834 (UM). NR 28 TC 0 Z9 0 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 27 PY 2014 VL 89 IS 6 AR 067303 DI 10.1103/PhysRevC.89.067303 PG 4 WC Physics, Nuclear SC Physics GA AK7UD UT WOS:000338632300005 ER PT J AU Guo, YN Ungur, L Granroth, GE Powell, AK Wu, CJ Nagler, SE Tang, JK Chibotaru, LF Cui, DM AF Guo, Yun-Nan Ungur, Liviu Granroth, Garrett E. Powell, Annie K. Wu, Chunji Nagler, Stephen E. Tang, Jinkui Chibotaru, Liviu F. Cui, Dongmei TI An NCN-pincer ligand dysprosium single-ion magnet showing magnetic relaxation via the second excited state SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULE MAGNET; LANTHANIDE COMPLEXES; ANISOTROPY; EXCHANGE; TRANSITION; AXIALITY; BARRIER AB Single-molecule magnets are compounds that exhibit magnetic bistability purely of molecular origin. The control of anisotropy and suppression of quantum tunneling to obtain a comprehensive picture of the relaxation pathway manifold, is of utmost importance with the ultimate goal of slowing the relaxation dynamics within single-molecule magnets to facilitate their potential applications. Combined ab initio calculations and detailed magnetization dynamics studies reveal the unprecedented relaxation mediated via the second excited state within a new DyNCN system comprising a valence-localized carbon coordinated to a single dysprosium(III) ion. The essentially C-2v symmetry of the Dy-III ion results in a new relaxation mechanism, hitherto unknown for mononuclear DyIII complexes, opening new perspectives for means of enhancing the anisotropy contribution to the spin-relaxation barrier. C1 [Guo, Yun-Nan; Tang, Jinkui] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China. [Wu, Chunji; Cui, Dongmei] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China. [Guo, Yun-Nan] Xi An Jiao Tong Univ, Sch Sci, Xian 710049, Peoples R China. [Ungur, Liviu; Chibotaru, Liviu F.] Katholieke Univ Leuven, Dept Chem, Theory Nanomat Grp, B-3001 Louvain, Belgium. [Granroth, Garrett E.; Nagler, Stephen E.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Powell, Annie K.] Karlsruhe Inst Technol, Inst Inorgan Chem, D-76131 Karlsruhe, Germany. [Powell, Annie K.] Karlsruhe Inst Technol, Inst Nanotechnol, D-76344 Karlsruhe, Germany. RP Tang, JK (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China. EM tang@ciac.ac.cn; Liviu.Chibotaru@chem.kuleuven.be; dmcui@ciac.ac.cn RI Tang, Jinkui/A-1830-2014; Guo, Yunnan/D-5976-2015; Nagler, Stephen/E-4908-2010; Granroth, Garrett/G-3576-2012; Powell, Annie/B-8665-2012; Ungur, Liviu/G-2057-2012 OI Tang, Jinkui/0000-0002-8600-7718; Nagler, Stephen/0000-0002-7234-2339; Granroth, Garrett/0000-0002-7583-8778; Powell, Annie/0000-0003-3944-7427; Ungur, Liviu/0000-0001-5015-4225 FU National Natural Science Foundation of China [21221061, 21301136, 21371166, 21331003]; US Department of Energy Basic Energy Sciences Scientific User Facilities Division FX This work was supported by the National Natural Science Foundation of China 21221061, 21301136, 21371166 and 21331003). Work at the ORNL Spallation Neutron Source is supported by the US Department of Energy Basic Energy Sciences Scientific User Facilities Division. L.U. is a postdoc of the FWO-Vlaanderen (Flemish Science Foundation). INPAC and Methusalem projects of the KU Leuven are also gratefully acknowledged. We also thank Dr. Yupeng Pan, Dr. Yang Wang and Dr. Wei Zhao for the help in preparation of sample and fruitful discussions. NR 43 TC 61 Z9 61 U1 16 U2 115 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 27 PY 2014 VL 4 AR 5471 DI 10.1038/srep05471 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK0KP UT WOS:000338101800006 PM 24969218 ER PT J AU Xiang, X Qiao, L Xiao, HY Gao, F Zu, XT Li, S Zhou, WL AF Xiang, X. Qiao, L. Xiao, H. Y. Gao, F. Zu, X. T. Li, S. Zhou, W. L. TI Effects of surface defects on two-dimensional electron gas at NdAlO3/SrTiO3 interface SO SCIENTIFIC REPORTS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; OXIDES AB Density functional theory calculations of NdAlO3/SrTiO3 heterostructure show that two-dimensional electron gas (2-DEG) is produced at the interface with a built-in potential of similar to 0.3 eV per unit cell. The effects of surface defects on the phase stability and electric field of 2-DEG have been investigated. It is found that oxygen vacancy is easily to form on the NdAlO3(001) surface, with a low threshold displacement energy and a low formation energy. This point defect results in surface reconstruction and the formation of a zigzag-Al-O-Al-chain, which quenches the built-in potential and enhances the carrier density significantly. These results will provide fundamental insights into understanding how surface defects influence the electronic behavior of 2-DEG and tuning their electronic properties through surface modification. C1 [Xiang, X.; Xiao, H. Y.; Zu, X. T.] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Qiao, L.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Gao, F.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Li, S.] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. [Zhou, W. L.] Univ New Orleans, Adv Mat Res Inst, New Orleans, LA 70148 USA. RP Xiang, X (reprint author), Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. EM xiaxiang@uestc.edu.cn; qiaol@ornl.gov; sean.li@unsw.edu.au RI Qiao, Liang/A-8165-2012 FU NSAF Joint Foundations of China [U1330103, U1230124]; Education Ministry of China [20110185110007]; University of Electronic Science and Technology of China [Y02002010401085] FX X. Xiang and X.T. Zu were supported by the NSAF Joint Foundations of China (Grant No. U1330103 and U1230124) and Ph.D. Funding Support Program of Education Ministry of China (20110185110007). H.Y. Xiao acknowledges the scientific research starting funding of University of Electronic Science and Technology of China (Grant No. Y02002010401085). NR 40 TC 6 Z9 6 U1 9 U2 63 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 27 PY 2014 VL 4 AR 5477 DI 10.1038/srep05477 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK0KR UT WOS:000338102000002 PM 24969627 ER PT J AU Lou, Y Schwender, J Shanklin, J AF Lou, Ying Schwender, Jorg Shanklin, John TI FAD2 and FAD3 Desaturases Form Heterodimers That Facilitate Metabolic Channeling in Vivo SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID CARRIER-PROTEIN DESATURASE; FATTY-ACID DESATURASES; ENDOPLASMIC-RETICULUM; TRANSGENIC PLANTS; CRYSTAL-STRUCTURE; ARABIDOPSIS; ENZYME; GENE; HYDROXYLASE; ACCUMULATION AB Plant desaturases comprise two independently evolved classes, a structurally well characterized soluble class responsible for the production of monoenes in the plastids of higher plants and the poorly structurally characterized integral membrane class that has members in the plastid and endoplasmic reticulum that are responsible for producing mono-and polyunsaturated fatty acids. Both require iron and oxygen for activity and are inhibited by azide and cyanide underscoring their common chemical imperatives. We previously showed that the Delta(9) acyl-CoA integral membrane desaturase Ole1p from Saccharomyces cerevisiae exhibits dimeric organization, like the soluble plastidial acyl-ACP desaturases. Here we use two independent bimolecular complementation assays, i.e. yeast two-hybrid analysis and Arabidopsis leaf protoplast split luciferase assay, to demonstrate that members of the plant integral membrane fatty acid desaturase (FAD) family, FAD2, FAD3, FAD6, FAD7, and FAD8, self-associate. Further, the endoplasmic reticulum-localized desaturase FAD2 can associate with FAD3, as can the plastid-localized FAD6 desaturase with either FAD7 or FAD8. These pairings appear to be specific because pairs such as FAD3 and FAD7 (or FAD8) and FAD2 and FAD6 do not interact despite their high amino acid similarity. These results are consistent also with their known endoplasmic reticulum and plastid subcellular localizations. Chemical cross-linking experiments confirm that FAD2 and FAD3 can form dimers like the yeast Ole1p and, when coexpressed, can form FAD2-FAD3 heterodimers. Metabolic flux analysis of yeast coexpressing FAD2 and FAD3 indicates that heterodimers can form a metabolic channel in which 18:1-PC is converted to 18:3-PC without releasing a free 18:2-PC intermediate. C1 [Lou, Ying; Schwender, Jorg; Shanklin, John] Brookhaven Natl Lab, Biosci Dept, Upton, NY 11973 USA. RP Shanklin, J (reprint author), Brookhaven Natl Lab, Dept Biol, Bldg 463,50 Bell Ave, Upton, NY 11973 USA. EM shanklin@bnl.gov RI Schwender, Jorg/P-2282-2014 OI Schwender, Jorg/0000-0003-1350-4171 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (DOE) [DOE KC0304000] FX work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (DOE) under Grant DOE KC0304000. NR 41 TC 11 Z9 12 U1 3 U2 26 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUN 27 PY 2014 VL 289 IS 26 BP 17996 EP 18007 DI 10.1074/jbc.M114.572883 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AJ9OM UT WOS:000338042000004 PM 24811169 ER PT J AU Parks, DH Shi, X Kevan, SD AF Parks, D. H. Shi, X. Kevan, S. D. TI Partially coherent x-ray diffractive imaging of complex objects SO PHYSICAL REVIEW A LA English DT Article ID PHASE; MICROSCOPY; RECONSTRUCTION; CONSTRAINT AB Lack of both spatial and temporal coherence at present x-ray light sources has hindered the application of coherent diffractive imaging techniques, as the computational algorithms which solve the phase problem to invert coherent speckle patterns have traditionally required fully coherent illumination. For this reason, new algorithms which incorporate knowledge of the illumination's coherence properties have been developed and shown to improve the reconstructed image of the scatterer in relatively simple test systems. In this paper we examine the performance of a reconstruction algorithm which incorporates knowledge of the spatial coherence of the illumination in the case of samples with complicated phase structure, and find that even perfect knowledge of the illumination's coherence does not improve the reconstructed image. We speculate that this failure to improve the reconstruction results from an underdetermination of the phase problem in the case of partially coherent illumination. C1 [Parks, D. H.; Shi, X.; Kevan, S. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Parks, DH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02 11ER46831]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The work of D.P., X.S., and S.K. was partially supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Grant No. DE-FG02 11ER46831. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank S. Roy and S. Mishra for help in editing the manuscript. NR 39 TC 2 Z9 2 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JUN 27 PY 2014 VL 89 IS 6 AR 063824 DI 10.1103/PhysRevA.89.063824 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AJ8HF UT WOS:000337943200009 ER PT J AU Hodovanets, H Liu, Y Jesche, A Ran, S Mun, ED Lograsso, TA Bud'ko, SL Canfield, PC AF Hodovanets, Halyna Liu, Yong Jesche, Anton Ran, Sheng Mun, Eun Deok Lograsso, Thomas A. Bud'ko, Sergey L. Canfield, Paul C. TI Fermi surface reconstruction in (Ba1-xKx)Fe2As2 (0.44 <= x <= 1) probed by thermoelectric power measurements SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC TOPOLOGICAL TRANSITIONS; SUPERCONDUCTIVITY; BAFE2AS2; STATE; METAL AB We report in-plane thermoelectric power measurements on single crystals of (Ba1-xKx)Fe2As2 (0.44 <= x <= 1). We observe a minimum in the S vertical bar(T=const) versus x at x similar to 0.55 that can be associated with the change in the topology of the Fermi surface, a Lifshitz transition, related to the electron pockets at the center of M point crossing the Fermi level. This feature is clearly observable below similar to 75 K. Thermoelectric power also shows a change in the x similar to 0.8-0.9 range, where the maximum in the thermoelectric power collapses into a plateau. This Lifshitz transition is most likely related to the reconstruction of the Fermi surface associated with the transformation of the hole pockets at the M point into four blades as observed by ARPES measurements. C1 [Hodovanets, Halyna; Jesche, Anton; Ran, Sheng; Mun, Eun Deok; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Liu, Yong; Jesche, Anton; Ran, Sheng; Mun, Eun Deok; Lograsso, Thomas A.; Bud'ko, Sergey L.; Canfield, Paul C.] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Lograsso, Thomas A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Hodovanets, H (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; US DOE [DE-AC02-07CH11358.]; AFOSR-MURI Grant [FA9550-09-1-0603] FX The authors would like to thank R. Prozorov and M. A. Tanatar for bringing our attention to the possibility of these measurements; B. Coles for pointing out the versatility of this measurement technique; H. Kim, V. Taufour, and M. Sailer for useful discussions. This work was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the US DOE by Iowa State University under contract No. DE-AC02-07CH11358. E. Mun was supported by the AFOSR-MURI Grant No. FA9550-09-1-0603. NR 43 TC 11 Z9 11 U1 2 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 27 PY 2014 VL 89 IS 22 AR 224517 DI 10.1103/PhysRevB.89.224517 PG 6 WC Physics, Condensed Matter SC Physics GA AJ8HM UT WOS:000337944000005 ER PT J AU Manley, ME Jeffries, JR Lee, H Butch, NP Zabalegui, A Abernathy, DL AF Manley, M. E. Jeffries, J. R. Lee, H. Butch, N. P. Zabalegui, A. Abernathy, D. L. TI Multiple high-temperature transitions driven by dynamical structures in NaI SO PHYSICAL REVIEW B LA English DT Article ID INTRINSIC LOCALIZED MODES; PATTERN-FORMATION; DISCRETE BREATHERS; CRYSTALS; INTERFERENCE; EQUILIBRIUM; LATTICES AB Multiple, consecutive high-temperature transitions in NaI involving dynamical order and/or localization in the energy-momentum spectrum but not in the average crystal structure are revealed by lattice dynamics, x-ray lattice spacing, and heat-capacity measurements. Distinctive energy-momentum patterns and lattice distortions indicate dynamical structures forming within randomly stacked planes, rather than the isolated point-defect-like intrinsic localized modes predicted. Transition entropies are accounted for by vibrational entropy changes, and the transition enthalpies are explained by the strain energy of forming stacking-fault-like planar distortions deduced from x-ray-diffraction peak shifts. The vibrational entropy of the dynamical structures stabilizes surrounding elastic distortions. C1 [Manley, M. E.; Abernathy, D. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jeffries, J. R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lee, H.; Zabalegui, A.] Santa Clara Univ, Santa Clara, CA 95053 USA. [Butch, N. P.] Univ Maryland, Dept Phys, Ctr Nanophys & Adv Mat, College Pk, MD 20742 USA. [Butch, N. P.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. RP Manley, ME (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM manleyme@ornl.gov RI Abernathy, Douglas/A-3038-2012; Manley, Michael/N-4334-2015; BL18, ARCS/A-3000-2012 OI Abernathy, Douglas/0000-0002-3533-003X; FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; LDRD at Lawrence Livermore National Laboratory (LLNL) [14-ERD-041]; Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration [DE-AC52- 07NA27344]; CIW; CDAC; UNLV; DOE- NNSA; DOE-BES; NSF; U.S. DOE [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences FX We would like to thank W. J. Evans, D. Ruddle, and K. Visbeck for assistance with the high-temperature furnace used in these experiments. We would also like to thank N. Agladze for assistance with and discussions on the dilatometry and differential scanning calorimetry measurements. Research sponsored, in part (M. E. M.), by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. Portions of this work (J. R. J. and N. P. B.) were supported by LDRD (Tracking Code No. 14-ERD-041) at Lawrence Livermore National Laboratory (LLNL). LLNL is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract No. DE-AC52- 07NA27344. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT is supported by CIW, CDAC, UNLV, and LLNL through funding from the DOE- NNSA, DOE-BES, and NSF. Beam time was graciously provided through CDAC. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The portion of this research performed at the Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences. NR 31 TC 5 Z9 6 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 27 PY 2014 VL 89 IS 22 AR 224106 DI 10.1103/PhysRevB.89.224106 PG 9 WC Physics, Condensed Matter SC Physics GA AJ8HM UT WOS:000337944000002 ER PT J AU Shivaram, BS Hinks, DG Maple, MB deAndrade, MA Kumar, P AF Shivaram, B. S. Hinks, D. G. Maple, M. B. deAndrade, M. A. Kumar, P. TI Universality in the magnetic response of metamagnetic metals SO PHYSICAL REVIEW B LA English DT Article ID HEAVY-FERMION COMPOUNDS; NONLINEAR SUSCEPTIBILITY; ELECTRON METAMAGNETISM; TRANSITIONS; PRESSURE; LIV2O4; OXIDE AB We report measurements of the nonlinear susceptibility chi(3)(T) in the metamagnetic heavy fermion (HF) compound UPt3. At high temperatures, chi(3)(T) < 0 and is small. It turns positive for T <= 35 K, forms a peak at T congruent to 10 K, and then decreases to zero with further decreasing temperature. The peak in chi(3) occurs at a temperature T-3, which is roughly half of T-1, the temperature of the maximum in the linear susceptibility. We present results on URu2Si2 and UPd2Al3 to show that this feature is common to other HF materials. A two-level model to describe the metamagnetic transition, with separation between the levels being the only energy scale, captures all experimentally observed features. C1 [Shivaram, B. S.] Univ Virginia, Dept Phys, Charlottesville, VA 22901 USA. [Hinks, D. G.] Argonne Natl Lab, Argonne, IL 60637 USA. [Maple, M. B.; deAndrade, M. A.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Kumar, P.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RP Shivaram, BS (reprint author), Univ Virginia, Dept Phys, Charlottesville, VA 22901 USA. EM bss2d@virginia.edu FU University of Virginia [NSF DMR 0073456]; U.S. Department of Energy [DE-FG02-04-ER46105] FX The authors wish to thank L. P. Gorkov and T. V. Ramakrishnan for many discussions and for generously sharing their vast insight into quantum magnetism. Thanks are also due to Piers Coleman, Daniel Cox, and Tony Leggett for useful advice and conversations. Work at the University of Virginia was made possible through Grant No. NSF DMR 0073456. Research at UCSD was supported by the U.S. Department of Energy under Grant No. DE-FG02-04-ER46105. NR 34 TC 2 Z9 2 U1 1 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 27 PY 2014 VL 89 IS 24 AR 241107 DI 10.1103/PhysRevB.89.241107 PG 5 WC Physics, Condensed Matter SC Physics GA AJ8HR UT WOS:000337944600002 ER PT J AU Ben-Naim, E Krapivsky, PL AF Ben-Naim, E. Krapivsky, P. L. TI Persistence of random walk records SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE random walk; record; first passage; persistence; nonequilibrium dynamics; data analysis ID 1ST-PASSAGE PROPERTIES; STATISTICS; MAXIMUM AB We study records generated by Brownian particles in one dimension. Specifically, we investigate an ordinary random walk and define the record as the maximal position of the walk. We compare the record of an individual random walk with the mean record, obtained as an average over infinitely many realizations. We term the walk 'superior' if the record is always above average, and conversely, the walk is said to be 'inferior' if the record is always below average. We find that the fraction of superior walks, S, decays algebraically with time, S similar to t(-beta), in the limit t -> 8, and that the persistence exponent is nontrivial, beta = 0.382 258.... The fraction of inferior walks, I, also decays as a power law, I similar to t(-alpha), but the persistence exponent is smaller, alpha = 0.241 608.... Both exponents are roots of transcendental equations involving the parabolic cylinder function. To obtain these theoretical results, we analyze the joint density of superior walks with a given record and position, while for inferior walks it suffices to study the density as a function of position. C1 [Ben-Naim, E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ben-Naim, E.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Krapivsky, P. L.] Boston Univ, Dept Phys, Boston, MA 02215 USA. RP Ben-Naim, E (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM ebn@lanl.gov RI Ben-Naim, Eli/C-7542-2009; Krapivsky, Pavel/A-4612-2014 OI Ben-Naim, Eli/0000-0002-2444-7304; FU DOE [DE-AC52-06NA25396] FX We thank Satya Majumdar for useful discussions and correspondence and acknowledge DOE grant DE-AC52-06NA25396 for support (EB). NR 50 TC 5 Z9 5 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD JUN 27 PY 2014 VL 47 IS 25 AR 255002 DI 10.1088/1751-8113/47/25/255002 PG 11 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA AJ5CD UT WOS:000337697600003 ER PT J AU Haab, A Mikulics, M Sutter, E Jin, JH Stoica, T Kardynal, B Rieger, T Grutzmacher, D Hardtdegen, H AF Haab, Anna Mikulics, Martin Sutter, Eli Jin, Jiehong Stoica, Toma Kardynal, Beata Rieger, Torsten Gruetzmacher, Detlev Hardtdegen, Hilde TI Evolution and characteristics of GaN nanowires produced via maskless reactive ion etching SO NANOTECHNOLOGY LA English DT Article DE gallium nitride; reactive ion etching; nanowires; metal-organic vapour phase epitaxy; photoluminescence; transmission electron microscopy ID SI-DOPED GAN; PHOTOLUMINESCENCE BAND; THREADING DISLOCATIONS; YELLOW LUMINESCENCE; ELECTRON-MICROSCOPY; FILMS; SAPPHIRE; DEFECTS; GROWTH; LAYERS AB The formation of nanowires (NWs) by reactive ion etching (RIE) of maskless GaN layers was investigated. The morphological, structural and optical characteristics of the NWs were studied and compared to those of the layer they evolve from. It is shown that the NWs are the result of a defect selective etching process. The evolution of density and length with etching time is discussed. Densely packed NWs with a length of more than 1 mu m and a diameter of similar to 60 nm were obtained by RIE of a similar to 2.5 mu m thick GaN layer. The NWs are predominantly free of threading dislocations and show an improvement of optical properties compared to their layer counterpart. The production of NWs via a top down process on non-masked group III-nitride layers is assessed to be very promising for photovoltaic applications. C1 [Haab, Anna; Mikulics, Martin; Jin, Jiehong; Stoica, Toma; Kardynal, Beata; Rieger, Torsten; Gruetzmacher, Detlev; Hardtdegen, Hilde] Forschungszentrum Julich GmbH, Peter Grunberg Inst PGI 9, D-52425 Julich, Germany. [Haab, Anna; Mikulics, Martin; Jin, Jiehong; Stoica, Toma; Kardynal, Beata; Rieger, Torsten; Gruetzmacher, Detlev; Hardtdegen, Hilde] Forschungszentrum Julich GmbH, Julich Aachen Res Alliance, Fundamentals Future Informat Technol JARA FIT, D-52425 Julich, Germany. [Sutter, Eli] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Hardtdegen, H (reprint author), Forschungszentrum Julich GmbH, Peter Grunberg Inst PGI 9, D-52425 Julich, Germany. EM h.hardtdegen@fz-juelich.de RI Mikulics, Martin/B-6193-2014; Hardtdegen, Hilde/B-5163-2014; OI Mikulics, Martin/0000-0001-7210-611X; Hardtdegen, Hilde/0000-0003-0445-6489; Rieger, Torsten/0000-0003-4873-4022 FU German Ministry of Education and Research (BMBF); US Department of Energy [DE-AC02-98CH10886] FX The authors gratefully acknowledge the financial support of the German Ministry of Education and Research (BMBF) within the projects 'EPHQUAM' and 'QPENS'. This work was performed in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory under the auspices of the US Department of Energy, under contract No. DE-AC02-98CH10886. E S would like to thank K Kisslinger for technical support. NR 41 TC 2 Z9 2 U1 5 U2 34 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUN 27 PY 2014 VL 25 IS 25 AR 255301 DI 10.1088/0957-4484/25/25/255301 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AJ2PT UT WOS:000337501200006 PM 24896155 ER PT J AU Schreppler, S Spethmann, N Brahms, N Botter, T Barrios, M Stamper-Kurn, DM AF Schreppler, Sydney Spethmann, Nicolas Brahms, Nathan Botter, Thierry Barrios, Maryrose Stamper-Kurn, Dan M. TI Optically measuring force near the standard quantum limit SO SCIENCE LA English DT Article ID RADIATION-PRESSURE; CAVITY OPTOMECHANICS; NOISE AB The Heisenberg uncertainty principle sets a lower bound on the noise in a force measurement based on continuously detecting a mechanical oscillator's position. This bound, the standard quantum limit, can be reached when the oscillator subjected to the force is unperturbed by its environment and when measurement imprecision from photon shot noise is balanced against disturbance from measurement back-action. We applied an external force to the center-of-mass motion of an ultracold atom cloud in a high-finesse optical cavity and measured the resulting motion optically. When the driving force is resonant with the cloud's oscillation frequency, we achieve a sensitivity that is a factor of 4 above the standard quantum limit and consistent with theoretical predictions given the atoms' residual thermal disturbance and the photodetection quantum efficiency. C1 [Schreppler, Sydney; Spethmann, Nicolas; Brahms, Nathan; Botter, Thierry; Barrios, Maryrose; Stamper-Kurn, Dan M.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Stamper-Kurn, Dan M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Schreppler, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sschreppler@berkeley.edu RI Stamper-Kurn, Dan/B-5442-2015 OI Stamper-Kurn, Dan/0000-0002-4845-5835 FU Air Force Office of Scientific Research; NSF; U.S. Department of Defense through the National Defense Science and Engineering Graduate Fellowship program FX This work was supported by the Air Force Office of Scientific Research and NSF. S. S. was supported by the U.S. Department of Defense through the National Defense Science and Engineering Graduate Fellowship program. NR 32 TC 25 Z9 25 U1 1 U2 31 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 27 PY 2014 VL 344 IS 6191 BP 1486 EP 1489 DI 10.1126/science.1249850 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7PZ UT WOS:000337889900042 PM 24970079 ER PT J AU Liu, H Strobridge, FC Borkiewicz, OJ Wiaderek, KM Chapman, KW Chupas, PJ Grey, CP AF Liu, Hao Strobridge, Fiona C. Borkiewicz, Olaf J. Wiaderek, Kamila M. Chapman, Karena W. Chupas, Peter J. Grey, Clare P. TI Capturing metastable structures during high-rate cycling of LiFePO4 nanoparticle electrodes SO SCIENCE LA English DT Article ID LITHIUM RECHARGEABLE BATTERIES; DOMINO-CASCADE MODEL; X-RAY-ABSORPTION; CATHODE MATERIALS; PHASE-TRANSITION; SOLID-SOLUTION; 2-PHASE REACTION; ION BATTERIES; DIFFRACTION; FEPO4 AB The absence of a phase transformation involving substantial structural rearrangements and large volume changes is generally considered to be a key characteristic underpinning the high-rate capability of any battery electrode material. In apparent contradiction, nanoparticulate LiFePO4, a commercially important cathode material, displays exceptionally high rates, whereas its lithium-composition phase diagram indicates that it should react via a kinetically limited, two-phase nucleation and growth process. Knowledge concerning the equilibrium phases is therefore insufficient, and direct investigation of the dynamic process is required. Using time-resolved in situ x-ray powder diffraction, we reveal the existence of a continuous metastable solid solution phase during rapid lithium extraction and insertion. This nonequilibrium facile phase transformation route provides a mechanism for realizing high-rate capability of electrode materials that operate via two-phase reactions. C1 [Liu, Hao; Strobridge, Fiona C.; Grey, Clare P.] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. [Borkiewicz, Olaf J.; Wiaderek, Kamila M.; Chapman, Karena W.; Chupas, Peter J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Grey, Clare P.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Grey, CP (reprint author), Univ Cambridge, Dept Chem, Lensfield Rd, Cambridge CB2 1EW, England. EM cpg27@cam.ac.uk RI Liu, Hao/B-2416-2016 OI Liu, Hao/0000-0003-0345-6647 FU Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-SC0001294]; DOE [DE-AC02-06CH11357]; European Union [FP7-265368]; Cambridge Overseas Trust; Engineering Physical Science Research Council FX This work was supported as part of the Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under award no. DE-SC0001294. Work performed at Argonne National Laboratory and use of the Advanced Photon Source, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, were supported by DOE under contract no. DE-AC02-06CH11357. H. L. acknowledges the funding from European Union FP7-265368 via the Eurolion Project and the Cambridge Overseas Trust. F. C. S. acknowledges the funding from the Engineering Physical Science Research Council via a Doctoral Training Partnership Award. We thank B. Orvananos, H. C. Yu, K. Thornton, R. Malik, A. Abdellahi, G. Ceder, and M. S. Whittingham for helpful discussions and comments. H. L., F. C. S., O.J.B. and K. M. W. carried out the experiments; H. L., K. W. C., P.J.C. and C. P. G. performed the analysis; and C. P. G. and H. L. wrote the manuscript with help from all coauthors. NR 46 TC 125 Z9 125 U1 60 U2 393 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 27 PY 2014 VL 344 IS 6191 AR 1252817 DI 10.1126/science.1252817 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7PZ UT WOS:000337889900040 PM 24970091 ER PT J AU Moon, EJ Keavney, DJ May, SJ AF Moon, Eun Ju Keavney, David J. May, Steven J. TI Strain Effects in Narrow-Bandwidth Manganites: The Case of Epitaxial Eu0.7Sr0.3MnO3 Thin Films SO PHYSICAL REVIEW APPLIED LA English DT Article ID DOUBLE EXCHANGE; MAGNETORESISTIVE MANGANITES; OXIDE HETEROSTRUCTURES; PEROVSKITE MANGANITES; MAGNETIC-PROPERTIES; PHASE-TRANSITIONS; STATE; RESISTIVITY; CRYSTALS; DIAGRAM AB We have investigated the strain-dependent magnetic properties of epitaxial narrow-bandwidth manganite, Eu0.7Sr0.3MnO3 (ESMO), thin films on various substrates traversing from compressive (-2.4%) to tensile (+1.5%) strain. The stoichiometry and crystalline quality of the films were confirmed with diffraction and spectroscopic-based characterization. Using field-and temperature-dependent magnetometry, we find that the epitaxial strain acts to suppress the ferromagnetic state, although films under compressive strain retain a greater propensity for ferromagnetic behavior. However, temperature-dependent resistivity reveals that ESMO thin films exhibit a ferromagnetic insulating state in contrast to wide-bandwidth La0.7Sr0.3MnO3 films under a comparable strain. The combination of a highly strain-dependent ferromagnetic state and robust insulating behavior may offer novel applications in spin filtering, sensing, or electronics. C1 [Moon, Eun Ju; May, Steven J.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Keavney, David J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Moon, EJ (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. EM em582@drexel.edu; smay@coe.drexel.edu RI Moon, Eun Ju/C-7856-2014; May, Steven/D-8563-2011 OI May, Steven/0000-0002-8097-1549 FU U.S. Army Research Office [W911NF-12-1-0132, W911NF-11-1-0283]; U.S. DOE [DE-AC02-06CH11357] FX We thank Leszek Wielunski and Boris Yakshinskiy for RBS measurements at the Laboratory for Surface Modification at Rutgers University and Yujun Xie for ESMO resistivity measurements. This work is supported by the U.S. Army Research Office under Grant No. W911NF-12-1-0132. Acquisition of the PPMS is supported by the U.S. Army Research Office under Grant No. W911NF-11-1-0283. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 52 TC 4 Z9 4 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JUN 26 PY 2014 VL 1 IS 5 AR 054006 DI 10.1103/PhysRevApplied.1.054006 PG 6 WC Physics, Applied SC Physics GA AS5RX UT WOS:000344328400003 ER PT J AU Pendleton, AL NicolasFeau, KS Feau, N Martin, FM Grigoriev, IV Hamelin, R Nelson, CD Burleigh, JG Davis, JM AF Pendleton, Amanda L. Smith, Katherine E. Feau, Nicolas Martin, Francis M. Grigoriev, Igor V. Hamelin, Richard Nelson, C. Dana Burleigh, J. Gordon Davis, John M. TI Duplications and losses in gene families of rust pathogens highlight putative effectors SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE effectors; rust pathogens; secretome; genome evolution; comparative genomics ID F-SP FUSIFORME; SIGNAL PEPTIDES; GENOME SEQUENCE; CFEM DOMAIN; PLANT; FUNGI; PROTEINS; CRONARTIUM; PREDICTION; VIRULENCE AB Rust fungi are a group of fungal pathogens that cause some of the world's most destructive diseases of trees and crops. A shared characteristic among rust fungi is obligate biotrophy, the inability to complete a lifecycle without a host. This dependence on a host species likely affects patterns of gene expansion, contraction, and innovation within rust pathogen genomes. The establishment of disease by biotrophic pathogens is reliant upon effector proteins that are encoded in the fungal genome and secreted from the pathogen into the host's cell apoplast or within the cells. This study uses a comparative genomic approach to elucidate putative effectors and determine their evolutionary histories. We used OrthoMCL to identify nearly 20,000 gene families in proteomes of 16 diverse fungal species, which include 15 basidiomycetes and one ascomycete. We inferred patterns of duplication and loss for each gene family and identified families with distinctive patterns of expansion/contraction associated with the evolution of rust fungal genomes. To recognize potential contributors for the unique features of rust pathogens, we identified families harboring secreted proteins that: (i) arose or expanded in rust pathogens relative to other fungi, or (ii) contracted or were lost in rust fungal genomes. While the origin of rust fungi appears to be associated with considerable gene loss, there are many gene duplications associated with each sampled rust fungal genome. We also highlight two putative effector gene families that have expanded in Cqf that we hypothesize have roles in pathogenicity. C1 [Pendleton, Amanda L.; Burleigh, J. Gordon; Davis, John M.] Univ Florida, Plant Mol & Cell Biol Program, Gainesville, FL USA. [Smith, Katherine E.; Nelson, C. Dana] Southern Inst Forest Genet, USDA Forest Serv, Southern Research Stat, Saucier, MS USA. [Feau, Nicolas; Hamelin, Richard] Univ British Columbia, Dept Forest Sci, Vancouver, BC V6T 1W5, Canada. [Martin, Francis M.] Univ Lorraine, UMR Inst Natl Rech Agronom, INRA Nancy, Lab Excellence ARBRE, Champenoux, France. [Grigoriev, Igor V.] Joint Genome Inst, US Dept Energy, Walnut Creek, CA USA. [Burleigh, J. Gordon] Univ Florida, Dept Biol, Gainesville, FL USA. [Burleigh, J. Gordon; Davis, John M.] Univ Florida, Genet Inst, Gainesville, FL USA. [Davis, John M.] Univ Florida, Sch Forest Resources & Conservat, Gainesville, FL 32611 USA. RP Davis, JM (reprint author), Univ Florida, Sch Forest Resources & Conservat, 365 Newins Ziegler Hall, Gainesville, FL 32611 USA. EM jmdavis@ufl.edu FU USDA Forest Service, Southern Research Station [11-CA-11330126-120]; French National Research Agency through the Laboratory of Excellence ARBRE [ANR-11-LABX-0002-01]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge funding from the USDA Forest Service, Southern Research Station (Agreement 11-CA-11330126-120) (to John M. Davis). This work was partly supported by the French National Research Agency through the Laboratory of Excellence ARBRE (ANR-11-LABX-0002-01) (to Francis M. Martin). The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank the following fungal genome project PIs for pre-publication access to genome sequence information: Drs. Sharon Doty (Rhodotorula graminis) and Ken Wolfe (Sporobolomyces roseus). The Cqf genome assembly and annotations can be interactively accessed through the JGI fungal genome portal MycoCosm at jgi.doe.gov/Cronartium (unpublished). We acknowledge Alicia Clym and Andrea Aerts at JGI for their roles in assembling and annotating the Cqf reference genome, respectively. Dr. Annegret Kohler at INRA, as well as Dr. Alan Kuo at JGI, are acknowledged for their leading roles in the acquisition of mycorrhizal genome sequence data. NR 63 TC 11 Z9 11 U1 3 U2 24 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JUN 26 PY 2014 VL 5 AR 299 DI 10.3389/fpls.2014.00299 PG 13 WC Plant Sciences SC Plant Sciences GA AM0AF UT WOS:000339504300001 PM 25018762 ER PT J AU Engelbrektson, A Hubbard, CG Tom, LM Boussina, A Jin, YT Wong, H Piceno, YM Carlson, HK Conrad, ME Anderson, G Coates, JD AF Engelbrektson, Anna Hubbard, Christopher G. Tom, Lauren M. Boussina, Aaron Jin, Yong T. Wong, Hayden Piceno, Yvette M. Carlson, Hans k. Conrad, Mark E. Anderson, Gary Coates, John D. TI Inhibition of microbial sulfate reduction in a flow-through column system by (per)chlorate treatment SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE perchlorate reduction; petroleum microbiology; souring; sulfate reduction; sulfur ID SULFIDE-OXIDIZING BACTERIA; POLYCYCLIC AROMATIC-HYDROCARBONS; REDUCING CONDITIONS; SP-NOV.; ANAEROBIC DEGRADATION; NITRATE REDUCTION; DESULFOVIBRIO-DESULFURICANS; HYDROGEN-SULFIDE; OIL-FIELD; HYDROTHERMAL SEDIMENTS AB Microbial sulfate reduction is a primary cause of oil reservoir souring. Here we show that amendment with chlorate or perchlorate [collectively (per)chlorate] potentially resolves this issue. Triplicate packed columns inoculated with marine sediment were flushed with coastal water amended with yeast extract and one of nitrate, chlorate, or perchlorate. Results showed that although sulfide production was dramatically reduced by all treatments, effluent sulfide was observed in the nitrate (10 mM) treatment after an initial inhibition period. In contrast, no effluent sulfide was observed with (per)chlorate (10 mM). Microbial community analyses indicated temporal community shifts and phylogenetic clustering by treatment. Nitrate addition stimulated Xanthomonadaceae and Rhizobiaceae growth, supporting their role in nitrate metabolism. (Per)chlorate showed distinct effects on microbial community structure compared with nitrate and resulted in a general suppression of the community relative to the untreated control combined with a significant decrease in sulfate reducing species abundance indicating specific toxicity. Furthermore, chlorate stimulated Pseudomonadaceae and Pseudoalteromonadaceae, members of which are known chlorate respirers, suggesting that chlorate may also control sulfidogenesis by biocompetitive exclusion of sulfate-reduction. Perchlorate addition stimulated Desulfobulbaceae and Desulfomonadaceae, which contain sulfide oxidizing and elemental sulfur-reducing species respectively, suggesting that effluent sulfide concentrations may be controlled through sulfur redox cycling in addition to toxicity and biocompetitive exclusion. Sulfur isotope analyses further support sulfur cycling in the columns, even when sulfide is not detected. This study indicates that (per)chlorate show great promise as inhibitors of sulfidogenesis in natural communities and provides insight into which organisms and respiratory processes are involved. C1 [Engelbrektson, Anna; Boussina, Aaron; Jin, Yong T.; Wong, Hayden; Carlson, Hans k.; Coates, John D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Hubbard, Christopher G.; Tom, Lauren M.; Piceno, Yvette M.; Conrad, Mark E.; Anderson, Gary; Coates, John D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Coates, JD (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, 271 Koshland Hall, Berkeley, CA 94720 USA. EM jdcoates@berkeley.edu RI Hubbard, Christopher/J-6150-2014; Tom, Lauren/E-9739-2015; Conrad, Mark/G-2767-2010; Piceno, Yvette/I-6738-2016 OI Hubbard, Christopher/0000-0002-8217-8122; Piceno, Yvette/0000-0002-7915-4699 FU Energy Biosciences Institute (EBI) FX The authors would like to acknowledge the Energy Biosciences Institute (EBI) for funding this work. Additionally we would like to acknowledge Jay Patel and Yasmin Peled for experimental help, and Wenbo Yang for sulfur isotope analysis. NR 78 TC 12 Z9 12 U1 3 U2 44 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUN 26 PY 2014 VL 5 AR 315 DI 10.3389/fmicb.2014.00315 PG 11 WC Microbiology SC Microbiology GA AK9IR UT WOS:000338741300001 PM 25071731 ER PT J AU Carena, M Da Rold, L Ponton, E AF Carena, Marcela Da Rold, Leandro Ponton, Eduardo TI Minimal composite Higgs models at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Spontaneous Symmetry Breaking; Beyond Standard Model; Global Symmetries ID CUSTODIAL SU(2); STANDARD MODEL; BOSON; SYMMETRY; BREAKING; PARTICLE; ANATOMY; MASS AB We consider composite Higgs models where the Higgs is a pseudo-Nambu Goldstone boson arising from the spontaneous breaking of an approximate global symmetry by some underlying strong dynamics. We focus on the SO(5) -> SO(4) symmetry breaking pattern, assuming the "partial compositeness" paradigm. We study the consequences on Higgs physics of the fermionic representations produced by the strong dynamics, that mix with the Standard Model (SM) degrees of freedom. We consider models based on the lowest-dimensional representations of SO(5) that allow for the custodial protection of the Z(b) over bar b coupling, i.e. the 5, 10 and 14. We find a generic suppression of the gluon fusion process, while the Higgs branching fractions can be enhanced or suppressed compared to the SM. Interestingly, a precise measurement of the Higgs boson couplings can distinguish between different realizations in the fermionic sector, thus providing crucial information about the nature of the UV dynamics. C1 [Carena, Marcela] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Carena, Marcela] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carena, Marcela] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Da Rold, Leandro] Ctr Atom Bariloche, CONICET, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Da Rold, Leandro] Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Ponton, Eduardo] Univ Estadual Paulista, UNESP, ICTP South Amer Inst Fundamental Res, BR-01140070 Sao Paulo, Brazil. [Ponton, Eduardo] Univ Estadual Paulista, UNESP, Inst Fis Teor, BR-01140070 Sao Paulo, Brazil. RP Carena, M (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM carena@fnal.gov; daroldl@cab.cnea.gov.ar; eponton@ift.unesp.br FU Fermi Research Alliance, LLC - United States Department of Energy [DE-AC02-07CH11359]; FONCYT-Argentina [PICT-20101737]; CONICET-Argentina [PIP 114220100100319]; Sao Paulo Research Foundation (FAPESP) [2011/11973] FX We thank Carlos Wagner for enlightening discussions in the beginning of this work and Alex Pomarol for useful suggestions. We also thank Abdelhak Djouadi, Joseph Lykken, Giuliano Panico, Gilad Perez and Francesco Riva for discussions. E.P. and L.D. wish to thank the Fermilab Theory Group for hospitality during various stages of this work. M. C. would like to thank the Aspen Center for Physics, where part of this work was completed. M.C. would like to thank ICTP-SAIFR and Centro Atomico Bariloche for hospitality. M.C. and E.P. would like to thank the MITP at the Johannes Gutenberg-University Mainz, where part of this work was completed. Fermilab is operated by Fermi Research Alliance, LLC under contract no. DE-AC02-07CH11359 with the United States Department of Energy. L.D. is partly supported by FONCYT-Argentina under the contract PICT-2010-1737 and CONICET-Argentina under the contract PIP 114220100100319. This work was supported by the Sao Paulo Research Foundation (FAPESP) under grant # 2011/11973. NR 60 TC 16 Z9 16 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 26 PY 2014 IS 6 AR 159 DI 10.1007/JHEP06(2014)159 PG 58 WC Physics, Particles & Fields SC Physics GA AK8GK UT WOS:000338665300001 ER PT J AU Pelissier, FA Garbe, JC Ananthanarayanan, B Miyano, M Lin, CH Jokela, T Kumar, S Stampfer, MR Lorens, JB LaBarge, MA AF Pelissier, Fanny A. Garbe, James C. Ananthanarayanan, Badriprasad Miyano, Masaru Lin, ChunHan Jokela, Tiina Kumar, Sanjay Stampfer, Martha R. Lorens, James B. LaBarge, Mark A. TI Age-Related Dysfunction in Mechanotransduction Impairs Differentiation of Human Mammary Epithelial Progenitors SO CELL REPORTS LA English DT Article ID HEMATOPOIETIC STEM-CELLS; BREAST-CANCER; HIPPO PATHWAY; FOCAL ADHESIONS; YAP ONCOPROTEIN; IN-SITU; PHENOTYPE; GLAND; SPECIFICATION; POPULATION AB Dysfunctional progenitor and luminal cells with acquired basal cell properties accumulate during human mammary epithelial aging for reasons not understood. Multipotent progenitors from women aged <30 years were exposed to a physiologically relevant range of matrix elastic modulus (stiffness). Increased stiffness causes a differentiation bias towards myoepithelial cells while reducing production of luminal cells and progenitor maintenance. Lineage representation in progenitors from women >55 years is unaffected by physiological stiffness changes. Efficient activation of Hippo pathway transducers YAP and TAZ is required for the modulus-dependent myoepithelial/basal bias in younger progenitors. In older progenitors, YAP and TAZ are activated only when stressed with extraphysiologically stiff matrices, which bias differentiation towards luminal-like phenotypes. In vivo YAP is primarily active in myoepithelia of younger breasts, but localization and activity increases in luminal cells with age. Thus, aging phenotypes of mammary epithelia may arise partly because alterations in Hippo pathway activation impair microenvironment-directed differentiation and lineage specificity. C1 [Pelissier, Fanny A.; Garbe, James C.; Miyano, Masaru; Lin, ChunHan; Jokela, Tiina; Stampfer, Martha R.; LaBarge, Mark A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Pelissier, Fanny A.; Jokela, Tiina; Lorens, James B.] Univ Bergen, Dept Biomed, Ctr Canc Biomarkers, N-5009 Bergen, Norway. [Lin, ChunHan] Univ Calif Berkeley, Dept Comparat Biochem, Berkeley, CA 94720 USA. [Ananthanarayanan, Badriprasad; Kumar, Sanjay] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP LaBarge, MA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM malabarge@lbl.gov RI MIYANO, MASARU/I-1353-2015; Jokela, Tiina/O-9206-2015; Lorens, James/B-9737-2017 OI Jokela, Tiina/0000-0002-7521-3866; Lorens, James/0000-0002-6782-3349 FU NIH [NIA R00AG033176, R01AG040081, NCI U54CA143836]; US Department of Energy [DE-AC02-05CH11231]; California Institute for Regenerative Medicine [TG2-01164] FX We thank Prof. Matthias Lutolf, Gurkaran S. Buxi, and Thibault Vatter for expert advice. M.A.L. is supported by the NIH (NIA R00AG033176 and R01AG040081; NCI U54CA143836) and the US Department of Energy (DE-AC02-05CH11231). B.A. is supported by a postdoctoral fellowship from the California Institute for Regenerative Medicine (TG2-01164). NR 53 TC 11 Z9 11 U1 0 U2 9 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 2211-1247 J9 CELL REP JI Cell Reports PD JUN 26 PY 2014 VL 7 IS 6 BP 1926 EP 1939 DI 10.1016/j.celrep.2014.05.021 PG 14 WC Cell Biology SC Cell Biology GA AK3LL UT WOS:000338325400019 PM 24910432 ER PT J AU Liu, C Assary, RS Curtiss, LA AF Liu, Cong Assary, Rajeev S. Curtiss, Larry A. TI Investigation of Thermochemistry Associated with the Carbon-Carbon Coupling Reactions of Furan and Furfural Using ab Initio Methods SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; DIELS-ALDER REACTIONS; SET MODEL CHEMISTRY; QUANTUM-CHEMICAL METHODS; BOND FORMATION; TRANSPORTATION FUELS; OXYGENATED HYDROCARBONS; CATALYTIC CONVERSION; ALDOL REACTION; BIOMASS AB Upgrading furan and small oxygenates obtained from the decomposition of cellulosic materials via formation of carbon-carbon bonds is critical to effective conversion of biomass to liquid transportation fuels. Simulation-driven molecular level understanding of carbon-carbon bond formation is required to design efficient catalysts and processes. Accurate quantum chemical methods are utilized here to predict the reaction energetics for conversion of furan (C4H4O) to C-5-C-8 ethers and the transformation of furfural (C5H6O2) to C-13-C-26 alkanes. Furan can be coupled with various C-1 to C-4 low molecular weight carbohydrates obtained from the pyrolysis via Diels-Alder type reactions in the gas phase to produce C-5-C-8 cyclic ethers. The computed reaction barriers for these reactions (similar to 25 kcal/mol) are lower than the cellulose activation or decomposition reactions (similar to 50 kcal/mol). Cycloaddition of C-5-C-8 cyclo ethers with furans can also occur in the gas phase, and the computed activation energy is similar to that of the first Diets Alder reaction. Furfural, obtained from biomass, can be coupled with aldehydes or ketones with alpha-hydrogen atoms to form longer chain aldol products, and these aldol products can undergo vapor phase hydrocycloaddition (activation barrier of similar to 20 kcal/mol) to form the precursors of C-26 cyclic hydrocarbons. These thermochemical studies provide the basis for further vapor phase catalytic studies required for upgrading of furans/furfurals to longer chain hydrocarbons. C1 [Liu, Cong; Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Curtiss, LA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM curtiss@anl.gov RI Surendran Assary, Rajeev/E-6833-2012; OI Surendran Assary, Rajeev/0000-0002-9571-3307; Liu, Cong/0000-0002-2145-5034 FU Bioenergy Technologies Office (BETO) program of Energy Efficiency & Renewable Energy (EERE); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; ANL FX This research was supported by the Bioenergy Technologies Office (BETO) program of Energy Efficiency & Renewable Energy (EERE). We gratefully acknowledge the computing resources provided on "Fusion", a 320-node computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. We also thank the support of the Director's Postdoctoral Fellowship from ANL. NR 81 TC 4 Z9 4 U1 4 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUN 26 PY 2014 VL 118 IS 25 BP 4392 EP 4404 DI 10.1021/jp503702t PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AK1OO UT WOS:000338184600004 PM 24902118 ER PT J AU Del Razo, MJ Pan, WX Qian, H Lin, G AF Del Razo, Mauricio J. Pan, Wenxiao Qian, Hong Lin, Guang TI Fluorescence Correlation Spectroscopy and Nonlinear Stochastic Reaction-Diffusion SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FLUCTUATION SPECTROSCOPY; SIMULATION; KINETICS; STATE; BINDING AB The currently existing theory of fluorescence correlation spectroscopy (FCS) is based on the linear fluctuation theory originally developed by Einstein, Onsager, Lax, and others as a phenomenological approach to equilibrium fluctuations in bulk solutions. For mesoscopic reaction-diffusion systems with nonlinear chemical reactions among a small number of molecules, a situation often encountered in single-cell biochemistry, it is expected that FCS time correlation functions of a reaction-diffusion system can deviate from the classic results of Elson and Magde [Biopolymers 1974, 13, 1-27]. We first discuss this nonlinear effect for reaction systems without diffusion. For nonlinear stochastic reaction-diffusion systems, there are no closed solutions; therefore, stochastic Monte Carlo simulations are carried out. We show that the deviation is small for a simple bimolecular reaction; the most significant deviations occur when the number of molecules is small and of the same order. Our results show that current linear FCS theory could be adequate for measurements on biological systems that contain many other sources of uncertainties. At the same time, it provides a framework for future measurements of nonlinear, fluctuating chemical reactions with high-precision FCS. Extending Delbruck-Gillespie's theory for stochastic nonlinear reactions with rapid stirring to reaction-diffusion systems provides a mesoscopic model for chemical and biochemical reactions at nanometric and mesoscopic levels, such as a single biological cell. C1 [Del Razo, Mauricio J.; Qian, Hong] Univ Washington, Seattle, WA 98195 USA. [Pan, Wenxiao; Lin, Guang] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Del Razo, MJ (reprint author), Univ Washington, Seattle, WA 98195 USA. EM maojrs@uw.edu FU National Science and Technology Council of Mexico (CONACyT); Pacific Northwest National Laboratory (PNNL) [PR203607]; Applied Mathematics Program within the U.S. Department of Energy Office of Advanced Scientific Computing Research as part of the Collaboratory on Mathematics for Mesoscopic Modeling of Materials (CM4) [DE-SC0009247]; DOE [DE-AC05-76RL01830] FX We thank helpful discussions with Drs. Noam Agmon, Steve Andrews, Attila Szabo, and Nancy Thompson. The authors would also like to thank two anonymous reviewers who greatly improved the quality of this paper. M.J.d.R. acknowledges partial support from National Science and Technology Council of Mexico (CONACyT). H.Q acknowledges partial support from Pacific Northwest National Laboratory (PNNL) Subcontract PR203607. W.P. and G.L. acknowledge the funding support by the Applied Mathematics Program within the U.S. Department of Energy Office of Advanced Scientific Computing Research as part of the Collaboratory on Mathematics for Mesoscopic Modeling of Materials (CM4), under award number DE-SC0009247. PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RL01830. NR 38 TC 2 Z9 2 U1 1 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 26 PY 2014 VL 118 IS 25 BP 7037 EP 7046 DI 10.1021/jp5030125 PG 10 WC Chemistry, Physical SC Chemistry GA AK1OM UT WOS:000338184400005 PM 24877790 ER PT J AU Coltrin, ME Armstrong, AM Brener, I Chow, WW Crawford, MH Fischer, AJ Kelley, DF Koleske, DD Lauhon, LJ Martin, JE Nyman, M Schubert, EF Shea-Rohwer, LE Subramania, G Tsao, JY Wang, GT Wierer, JJ Wright, JB AF Coltrin, Michael E. Armstrong, Andrew M. Brener, Igal Chow, Weng W. Crawford, Mary H. Fischer, Arthur J. Kelley, David F. Koleske, Daniel D. Lauhon, Lincoln J. Martin, James E. Nyman, May Schubert, E. Fred Shea-Rohwer, Lauren E. Subramania, Ganapathi Tsao, Jeffrey Y. Wang, George T. Wierer, Jonathan J., Jr. Wright, Jeremy B. TI Energy Frontier Research Center for Solid-State Lighting Science: Exploring New Materials Architectures and Light Emission Phenomena SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; EMITTING DIODE-ARRAYS; GAN NANOWIRES; PHOTONIC CRYSTALS; QUANTUM-WELLS; MULTIPHONON EMISSION; DEEP LEVELS; LASERS; GROWTH; GAAS AB The Energy Frontier Research Center (EFRC) for Solid-State Lighting Science (SSLS) is one of 46 EFRCs initiated in 2009 to conduct basic and use-inspired research relevant to energy technologies. The overarching theme of the SSLS EFRC is the exploration of energy conversion in tailored photonic structures. In this article we review highlights from the research of the SSLS EFRC. Major research themes include: studies of the materials properties and emission characteristics of Ill-nitride semiconductor nanowires; development of new phosphors and II-VI quantum dots for use as wavelength downconverters; fundamental understanding of competing radiative and nonradiative processes in current-generation, planar light-emitting diode architectures; understanding of the electrical, optical, and structural properties of defects in InGaN materials and heterostructures; exploring ways to enhance spontaneous emission through modification of the environment in which the emission takes place; and investigating routes such as stimulated emission that might outcompete nonradiative processes. C1 [Coltrin, Michael E.; Armstrong, Andrew M.; Brener, Igal; Chow, Weng W.; Crawford, Mary H.; Fischer, Arthur J.; Koleske, Daniel D.; Martin, James E.; Shea-Rohwer, Lauren E.; Subramania, Ganapathi; Tsao, Jeffrey Y.; Wang, George T.; Wierer, Jonathan J., Jr.; Wright, Jeremy B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kelley, David F.] Univ Calif Merced, Merced, CA 95343 USA. [Lauhon, Lincoln J.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Nyman, May] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Schubert, E. Fred] Rensselaer Polytech Inst, Dept Elect Comp & Syst Engn, Troy, NY 12180 USA. RP Coltrin, ME (reprint author), Sandia Natl Labs, POB 5800,MS 1086, Albuquerque, NM 87185 USA. EM mecoltr@sandia.gov RI Lauhon, Lincoln/B-7526-2009; Lauhon, Lincoln/H-2976-2015; Wierer, Jonathan/G-1594-2013 OI Lauhon, Lincoln/0000-0001-6046-3304; Wierer, Jonathan/0000-0001-6971-4835 FU Sandia's Solid-State Lighting Science Energy Frontier Research Center - Department of Energy Office of Basic Energy Science; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by Sandia's Solid-State Lighting Science Energy Frontier Research Center, sponsored by the Department of Energy Office of Basic Energy Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 99 TC 4 Z9 4 U1 4 U2 63 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 26 PY 2014 VL 118 IS 25 BP 13330 EP 13345 DI 10.1021/jp501136j PG 16 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AK1OL UT WOS:000338184300002 ER PT J AU Kamath, G Cutler, RW Deshmukh, SA Shakourian-Fard, M Parrish, R Huether, J Butt, DP Xiong, H Sankaranarayanan, SKRS AF Kamath, Ganesh Cutler, Richard W. Deshmukh, Sanket A. Shakourian-Fard, Mehdi Parrish, Riley Huether, Joshua Butt, Darryl P. Xiong, H. Sankaranarayanan, Subramanian K. R. S. TI In Silico Based Rank-Order Determination and Experiments on Nonaqueous Electrolytes for Sodium Ion Battery Applications SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LITHIUM BATTERIES; AMORPHOUS TIO2; RECHARGEABLE BATTERIES; CATHODE MATERIALS; CHALLENGES; LI; NANOSTRUCTURES; ELECTRODES; DYNAMICS; FORCE AB Electrolytes are an important component of electrochemical energy storage systems and their optimization is critical for emerging beyond lithium ion technologies. Here, an integrated computational-experimental approach is used to rank-order and aid the selection of suitable electrolytes for a Na-ion battery. We present an in silico strategy based on both thermodynamic and kinetic descriptors derived from molecular dynamics simulations to rationally arrive at optimal electrolytes for Na-ion batteries. We benchmarked various electrolytes (pure and binary mixtures of cyclic and acyclic carbonates with NaClO4 salt) to identify appropriate formulations with the overarching goal of simultaneously enhancing cell performance while meeting safety norms. Fundamental insights from computationally derived thermodynamic and kinetic data considerations coupled with atomistic-level description of the solvation dynamics is used to rank order the various electrolytes. Thermodynamic considerations based on free energy evaluation indicate EC:PC as a top electrolyte formulation under equilibrium conditions. However, kinetic descriptors which are important factors dictating the rate capability and power performance suggest EC:DMC and EC:EMC to be among the best formulations. Experimental verification of these optimized formulations was carried out by examining the electrochemical performance of various electrolytes in Na/TiO2 nanotubes half cells with NaClO4 salt. Our rate capability studies confirm that EC:DMC and EC:EMC to be the best formulations. These optimized formulations have low-rate specific capacities similar to 120-140 mAh/g whereas the lower ranked electrolytes (EC: DEC) have capacities similar to 95 mAh/g. The various electrolytes are also evaluated from a safety perspective. Such results suggest encouraging prospects for this approach in the a priori prediction of optimal sodium ion systems with possible screening implications for novel battery formulations. C1 [Kamath, Ganesh; Shakourian-Fard, Mehdi] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Cutler, Richard W.; Parrish, Riley; Huether, Joshua; Butt, Darryl P.; Xiong, H.] Boise State Univ, Dept Mat Sci & Engn, Boise, ID 83725 USA. [Butt, Darryl P.; Xiong, H.] Ctr Adv Energy Studies, Idaho Falls, ID 83415 USA. [Deshmukh, Sanket A.; Sankaranarayanan, Subramanian K. R. S.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Xiong, H (reprint author), Boise State Univ, Dept Mat Sci & Engn, 1910 Univ Dr, Boise, ID 83725 USA. EM clairexiong@boisestate.edu; skrssank@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH1135]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH1135. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 9 Z9 9 U1 4 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 26 PY 2014 VL 118 IS 25 BP 13406 EP 13416 DI 10.1021/jp502319p PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AK1OL UT WOS:000338184300010 ER PT J AU Yang, YX Zhou, J Nakayama, M Nie, LZ Liu, P White, MG AF Yang, Yixiong Zhou, Jia Nakayama, Miki Nie, Lizhou Liu, Ping White, Michael G. TI Surface Dipoles and Electron Transfer at the Metal Oxide-Metal Interface: A 2PPE Study of Size-Selected Metal Oxide Clusters Supported on Cu(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GAS SHIFT REACTION; INITIO MOLECULAR-DYNAMICS; SELF-ASSEMBLED MONOLAYERS; TOTAL-ENERGY CALCULATIONS; PROBE FORCE MICROSCOPY; WAVE BASIS-SET; WORK FUNCTION; CHEMICAL-PROPERTIES; TIO2(110) SURFACE; AU NANOPARTICLES AB Two-photon photoemission spectroscopy (2PPE) was employed to investigate the electronic interactions at the interface of size-selected metal oxide clusters (Mo3O9, W3O9, Ti3O6, Mo3O6, W3O6, and Ti6O10) and a Cu(111) surface. The cluster Cu interactions were probed by work function shifts measured by 2PPE as a function of local cluster coverage. For all the clusters studied, the work functions shifted to higher energies after cluster deposition, indicating negative interfacial dipole moments pointing toward the surface. The magnitudes of the derived interfacial dipoles are found to be in the order Mo3O9 approximate to W3O9 > W3O6 approximate to Mo3O6 > Ti5O10 > Ti3O6. DFT calculations of the electrostatic potentials at the interface and Bader charge analyses were used to assess the relative contributions of electron transfer and the structure-dependent cluster dipole moment to the observed work function shifts (Delta Phi). For the fully oxidized Mo3O9 and W3O9 clusters (+6 cation oxidation states), DFT calculations indicate that electron transfer from the Cu(111) support to the cluster is the dominant contribution. The smaller interfacial dipole moments for the Mo3O6 and W3O6 clusters are qualitatively consistent with the decreased ability of the reduced cations (+4 oxidation state) to accommodate charge from the Cu surface. The DFT calculations also predict small changes in Delta Phi for the titania clusters on Cu(111) but in the opposite direction of that observed experimentally. In the case of the Ti5O10/Cu(111) surface, this result is due to the net balance of cluster dipole and electron transfer contributions that have opposite signs. Overall, the results presented in this study show that a combination of coverage-dependent work function measurements and DFT calculations can be a powerful tool to investigate the electronic interactions, especially electron transfer, at the metal oxide metal interface. C1 [Yang, Yixiong; Nie, Lizhou; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Zhou, Jia; Nakayama, Miki; Liu, Ping; White, Michael G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP White, MG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM mgwhite@bnl.gov FU Chemistry Department at Brookhaven National Laboratory [DE-AC02-98CH10086] FX This work was carried out in the Chemistry Department at Brookhaven National Laboratory under Contract No. DE-AC02-98CH10086 with the U.S. Department of Energy (Division of Chemical Sciences). The DFT calculations were performed using computational resources at the Center for Functional Nanomaterials, Brookhaven National Laboratory. NR 59 TC 6 Z9 6 U1 9 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 26 PY 2014 VL 118 IS 25 BP 13697 EP 13706 DI 10.1021/jp503646u PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AK1OL UT WOS:000338184300043 ER PT J AU Geier, B Gspan, C Winkler, R Schmied, R Fowlkes, JD Fitzek, H Rauch, S Rattenberger, J Rack, PD Plank, H AF Geier, Barbara Gspan, Christian Winkler, Robert Schmied, Roland Fowlkes, Jason D. Fitzek, Harald Rauch, Sebastian Rattenberger, Johannes Rack, Philip D. Plank, Harald TI Rapid and Highly Compact Purification for Focused Electron Beam Induced Deposits: A Low Temperature Approach Using Electron Stimulated H2O Reactions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID REPAIR; NANOSTRUCTURES; PLATINUM; MASKS AB Focused electron beam induced deposition (FEBID) is an important synthesis method as it is an extremely flexible tool for fabricating functional (3D) structures with nanometer spatial resolution. However, FEBID has historically suffered from carbon impurities up to 90 at %, which significantly limits the intended functionalities. In this study we demonstrate that (MeCpPtMe3)-Me-IV deposits can be fully purified by an electron-beam assisted approach using H2O vapor at room temperature, which eliminates sample and/or gas heating and complicated gas delivery systems, respectively. We demonstrate that local pressures of 10 Pa results in an electron-limited regime, thus enabling high purification rates of better than 5 min.nA(-1) mu m(-2) (30 C.cm(-2)) for initially 150 nm thick deposits. Furthermore, TEM measurements suggest the purification process for the highly compact deposits occurs via a bottom-up process. C1 [Geier, Barbara; Gspan, Christian; Winkler, Robert; Schmied, Roland; Fitzek, Harald; Rattenberger, Johannes; Plank, Harald] Graz Ctr Electron Microscopy, A-8010 Graz, Austria. [Fowlkes, Jason D.; Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Rauch, Sebastian; Plank, Harald] Graz Univ Technol, Inst Electron Microscopy & Nanoanal, A-8010 Graz, Austria. RP Plank, H (reprint author), Graz Ctr Electron Microscopy, Steyrergasse 17, A-8010 Graz, Austria. EM harald.plank@felmi-zfe.at OI Rack, Philip/0000-0002-9964-3254 FU COST action CELINA [CM1301]; EUROSTARS project TRIPLE-S [E! 8213]; ESTEEM2 (EU FP7 program, FP7) [312483]; Intel Corporation via Semiconductor Research Corporation [SRC-2012-In-2310]; Center for Materials Processing; Center for Nanophase Materials Sciences - Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors gratefully acknowledge Prof. Ferdinand Hofer, Prof. Werner Grogger, Ing. Hartmuth Schrottner, and Dr. Joo-Hyon Noh for support. We also acknowledge financial support by the 1) COST action CELINA (Nr. CM1301), 2) EUROSTARS project TRIPLE-S (Nr. E! 8213), and 3) ESTEEM2 (EU FP7 program, FP7/2007-2013, Nr. 312483). P.D.R. acknowledges support from Intel Corporation (and Ted Liang as program mentor) via the direct funding program at the Semiconductor Research Corporation (SRC-2012-In-2310) and matching funds from the Center for Materials Processing. J.D.F. acknowledges support from the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 41 TC 26 Z9 26 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 26 PY 2014 VL 118 IS 25 BP 14009 EP 14016 DI 10.1021/jp503442b PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AK1OL UT WOS:000338184300081 ER PT J AU Dambournet, D Duttine, M Chapman, KW Wattiaux, A Borkiewicz, O Chupas, PJ Demourgues, A Groult, H AF Dambournet, Damien Duttine, Mathieu Chapman, Karena W. Wattiaux, Alain Borkiewicz, Olaf Chupas, Peter J. Demourgues, Alain Groult, Henri TI Resolving and Quantifying Nanoscaled Phases in Amorphous FeF3 by Pair Distribution Function and Mossbauer Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLID-STATE NMR; LITHIUM BATTERIES; CRYSTAL-STRUCTURE; FLUORIDE; DIFFRACTION; REFINEMENT; PDF AB Probing the atomic structure of materials displaying a lack of long-range order has been a continuous challenge for the material science's community. X-ray amorphous Fe(F)3 has been shown to be a promising electrode material in Li and Na ion batteries. Providing structural information on this class of compounds is therefore of interest as it can help rationalize the material's properties and further enabled its optimization. Herein, we used the pair distribution function and Mossbauer spectroscopy to provide unique insights into the atomic structure of amorphous FeF3. The results showed that amorphous FeF3 contained two phases built from corner-sharing of FeF6 octahedra. According to X-ray diffraction data, the PDF was successfully modeled based on two structural models related to the distorted ReO3 and the hexagonal-tungsten-bronze networks of FeF3. The lack of long-range order shown by conventional XRD data and PDF analysis was shown to arise mostly from disorder. This study provides detailed atomic structure with corresponding spectroscopic signature of amorphous phases. Quantitative analysis of both techniques indicated similar trends. This showed that our approach can be employed to determine the structure of other complex materials. C1 [Dambournet, Damien; Duttine, Mathieu; Groult, Henri] Univ Paris 06, Sorbonne Univ, UMR 8234, PHENIX, F-75005 Paris, France. [Dambournet, Damien; Duttine, Mathieu; Groult, Henri] CNRS, UMR 8234, PHENIX, F-75005 Paris, France. [Duttine, Mathieu; Wattiaux, Alain; Demourgues, Alain] Univ Bordeaux, CNRS, ICMCB, UPR 9048, F-33600 Pessac, France. [Chapman, Karena W.; Borkiewicz, Olaf; Chupas, Peter J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Dambournet, D (reprint author), Univ Paris 06, Sorbonne Univ, UMR 8234, PHENIX, F-75005 Paris, France. EM damien.dambournet@upmc.fr FU People Programme (Marie Curie Actions) of the European Union [[321879] (FLUOSYNES)]; U.S. DOE [DE-AC02-06CH11357] FX The research leading to these results has received funding from the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme (FP7/2007-2013) under REA Grant Agreement No. [321879] (FLUOSYNES). Work done at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, were supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 35 TC 2 Z9 2 U1 5 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 26 PY 2014 VL 118 IS 25 BP 14039 EP 14043 DI 10.1021/jp504083g PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AK1OL UT WOS:000338184300085 ER PT J AU Dun, ZL Garlea, VO Yu, C Ren, Y Choi, ES Zhang, HM Dong, S Zhou, HD AF Dun, Z. L. Garlea, V. O. Yu, C. Ren, Y. Choi, E. S. Zhang, H. M. Dong, S. Zhou, H. D. TI LaSrVO4: A candidate for the spin-orbital liquid state SO PHYSICAL REVIEW B LA English DT Article ID LAYERED PEROVSKITE; MAGNETIC-BEHAVIOR; SINGLE-CRYSTAL; ORDER; FRUSTRATION; TRANSITION; OXIDES; FLUCTUATIONS; INSULATOR; SR2IRO4 AB A layered perovskite LaSrVO4 was studied by neutron diffraction, pair distribution function measurement using synchrotron x-ray, susceptibility, and specific heat measurements, and first-principles calculation. The results show (i) a weak structural distortion around 100 K with the existence of orbital fluctuations both above and below it; (ii) the absence of the long range magnetic ordering down to 0.35 K but the appearance of a short range magnetic ordering around 11 K with a T-2 behavior of the specific heat below it. Meanwhile, the calculation based on the density functional theory predicts a magnetic ordered ground state. All facts indicate a melting of the magnetic ordering due to the orbital fluctuations in LaSrVO4, which makes it a rare candidate for the spin-orbital liquid state related to t(2g) orbitals. C1 [Dun, Z. L.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Garlea, V. O.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Yu, C.; Ren, Y.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Choi, E. S.; Zhou, H. D.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA. [Zhang, H. M.; Dong, S.] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. RP Dun, ZL (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Dong (董), Shuai (帅)/A-5513-2008; Garlea, Vasile/A-4994-2016; Dun, Zhiling/F-5617-2016; Zhou, Haidong/O-4373-2016; OI Dong (董), Shuai (帅)/0000-0002-6910-6319; Garlea, Vasile/0000-0002-5322-7271; Dun, Zhiling/0000-0001-6653-3051; Yu, Cun/0000-0003-0084-6746 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US DOE [DE-AC02-06CH11357]; State of Florida; 973 projects of China [2011CB922101]; NSFC [51322206]; [NSF-DMR-1157490]; [NSF-DMR-1350002] FX Research at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. The NHMFL is supported by NSF-DMR-1157490 and the State of Florida. H.M.Z and S.D. were supported by the 973 projects of China (2011CB922101) and NSFC (51322206). Z.L.D. and H.D.Z. thank the support of NSF-DMR-1350002. NR 47 TC 7 Z9 7 U1 0 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 26 PY 2014 VL 89 IS 23 AR 235131 DI 10.1103/PhysRevB.89.235131 PG 7 WC Physics, Condensed Matter SC Physics GA AK2XF UT WOS:000338282800002 ER PT J AU Feldman, JL Singh, DJ Bernstein, N AF Feldman, J. L. Singh, D. J. Bernstein, N. TI Lattice-dynamical model for the filled skutterudite LaFe4Sb12: Harmonic and anharmonic couplings SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; THERMAL-CONDUCTIVITY; THERMOELECTRIC-MATERIALS; CRYSTALS AB The filled skutterudite LaFe4Sb12 shows greatly reduced thermal conductivity compared to that of the related unfilled compound CoSb3, although the microscopic reasons for this are unclear. We calculate harmonic and anharmonic force constants for the interaction of the La filler atom with the framework atoms. We find that force constants show a general trend of decaying rapidly with distance and are very small for the interaction of the La with its next-nearest-neighbor Sb and nearest-neighbor La. However, a few rather long-range interactions, such as with the next-nearest-neighbor La and with the third neighbor Sb, are surprisingly strong, although still small. We test the central-force approximation and find significant deviations from it. Using our force constants we calculate a bare La mode Gruneisen parameter and find a value of 3-4, substantially higher than values associated with cage atom anharmonicity, i.e., a value of about 1 for CoSb3 but much smaller than a previous estimate [Bernstein et al., Phys. Rev. B 81, 134301 (2010)]. This latter difference is primarily due to the previously used overestimate of the La-Fe cubic force constants. We also find a substantial negative contribution to this bare La Gruneisen parameter from the aforementioned third-neighbor La-Sb interaction. Our results underscore the need for rather long-range interactions in describing the role of anharmonicity on the dynamics in this material. C1 [Feldman, J. L.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Feldman, J. L.; Bernstein, N.] Naval Res Lab, Ctr Computat Mat Sci, Washington, DC 20375 USA. [Singh, D. J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Feldman, JL (reprint author), Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. FU Office of Naval Research through the Naval Research Laboratory's basic research program; DOE, BES through the Materials Sciences and Engineering Division FX Work at NRL was supported by the Office of Naval Research through the Naval Research Laboratory's basic research program. Work at ORNL was supported by the DOE, BES through the Materials Sciences and Engineering Division. Helpful suggestions by Dr. Russell Hemley and Dr. Andrew Shabaev are greatly appreciated. NR 39 TC 6 Z9 6 U1 7 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 26 PY 2014 VL 89 IS 22 AR 224304 DI 10.1103/PhysRevB.89.224304 PG 16 WC Physics, Condensed Matter SC Physics GA AK2XC UT WOS:000338282500003 ER PT J AU Mukherjee, S Nag, A Kocevski, V Santra, PK Balasubramanian, M Chattopadhyay, S Shibata, T Schaefers, F Rusz, J Gerard, C Eriksson, O Segre, CU Sarma, DD AF Mukherjee, Soham Nag, Angshuman Kocevski, Vancho Santra, Pralay K. Balasubramanian, Mahalingam Chattopadhyay, Soma Shibata, Tomohiro Schaefers, Franz Rusz, Jan Gerard, Celine Eriksson, Olle Segre, C. U. Sarma, D. D. TI Microscopic description of the evolution of the local structure and an evaluation of the chemical pressure concept in a solid solution SO PHYSICAL REVIEW B LA English DT Article ID ABSORPTION FINE-STRUCTURE; BUCKLED CRYSTALLINE-STRUCTURE; DISORDERED MIXED SALTS; VEGARDS LAW DEVIATION; X-RAY; TERNARY ALLOYS; BAND-GAP; SEMICONDUCTOR ALLOYS; ATOMIC CORRELATIONS; LATTICE-PARAMETER AB Extended x-ray absorption fine-structure studies have been performed at the Zn K and Cd K edges for a series of solid solutions of wurtzite Zn1-xCdxS samples with x = 0.0, 0.1, 0.25, 0.5, 0.75, and 1.0, where the lattice parameter as a function of x evolves according to the well-known Vegard's law. In conjunction with extensive, large-scale first-principles electronic structure calculations with full geometry optimizations, these results establish that the percentage variation in the nearest-neighbor bond distances are lower by nearly an order of magnitude compared to what would be expected on the basis of lattice parameter variation, seriously undermining the chemical pressure concept. With experimental results that allow us to probe up to the third coordination shell distances, we provide a direct description of how the local structure, apparently inconsistent with the global structure, evolves very rapidly with interatomic distances to become consistent with it. We show that the basic features of this structural evolution with the composition can be visualized with nearly invariant Zn-S-4 and Cd-S-4 tetrahedral units retaining their structural integrity, while the tilts between these tetrahedral building blocks change with composition to conform to the changing lattice parameters according to the Vegard's law within a relatively short length scale. These results underline the limits of applicability of the chemical pressure concept that has been a favored tool of experimentalists to control physical properties of a large variety of condensed matter systems. C1 [Mukherjee, Soham; Nag, Angshuman; Santra, Pralay K.; Sarma, D. D.] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India. [Kocevski, Vancho; Rusz, Jan; Gerard, Celine; Eriksson, Olle; Sarma, D. D.] Uppsala Univ, Dept Phys & Astron, Div Mat Theory, SE-75120 Uppsala, Sweden. [Balasubramanian, Mahalingam] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Chattopadhyay, Soma; Shibata, Tomohiro] Argonne Natl Lab, MRCAT, Argonne, IL 60439 USA. [Chattopadhyay, Soma; Shibata, Tomohiro; Segre, C. U.] IIT, CSRRI, Chicago, IL 60616 USA. [Chattopadhyay, Soma; Shibata, Tomohiro; Segre, C. U.] IIT, Dept Phys, Chicago, IL 60616 USA. [Schaefers, Franz] HZB BESSY II, Inst Nanometre Opt & Technol, D-12489 Berlin, Germany. [Sarma, D. D.] CSIR, Network Inst Solar Energy, New Delhi 110001, India. [Sarma, D. D.] Jawaharlal Nehru Ctr Adv Sci Res, Bangalore, Karnataka, India. RP Mukherjee, S (reprint author), Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India. EM sarma@sscu.iisc.ernet.in RI Segre, Carlo/B-1548-2009; Rusz, Jan/A-3324-2008; Eriksson, Olle/E-3265-2014; OI Segre, Carlo/0000-0001-7664-1574; Rusz, Jan/0000-0002-0074-1349; Eriksson, Olle/0000-0001-5111-1374; Kocevski, Vancho/0000-0002-2127-5834; Santra, Pralay/0000-0002-1951-5835 FU Department of Science and Technology (DST); Council of Scientific and Industrial Research (CSIR); National Science Foundation (NSF) [DMR-086935]; Deutsche Forschungsgemeinschaft (DFG); US Department of Energy (DOE)-Basic Energy Sciences; Natural Sciences and Engineering Research Council of Canada (NSERC); University of Washington; Canadian Light Source; DOE [DE-AC02-06CH11357]; Swedish Research Council (VR); KAW foundation; STANDUPP; eSSENCE; ERC [247062]; Advanced Photon Source FX We thank Department of Science and Technology (DST), Council of Scientific and Industrial Research (CSIR), National Science Foundation (NSF), and Deutsche Forschungsgemeinschaft (DFG) for funding this investigation. X-ray Science Division partnered with the Pacific Northwest Consortium (PNC/XSD) facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy (DOE)-Basic Energy Sciences, a Major Resources Support grant from The Natural Sciences and Engineering Research Council of Canada (NSERC), the University of Washington, the Canadian Light Source and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, was supported by the DOE under Contract No. DE-AC02-06CH11357. Support from the Swedish Research Council (VR), the KAW foundation, STANDUPP, eSSENCE and the ERC (ASD-Project No. 247062) is also acknowledged. Support for CUS was provided in part by the National Science Foundation under Grant No. DMR-086935. NR 76 TC 7 Z9 7 U1 5 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 26 PY 2014 VL 89 IS 22 AR 224105 DI 10.1103/PhysRevB.89.224105 PG 11 WC Physics, Condensed Matter SC Physics GA AK2XC UT WOS:000338282500002 ER PT J AU Schoop, L Hirschberger, M Tao, J Felser, C Ong, NP Cava, RJ AF Schoop, Leslie Hirschberger, Max Tao, Jing Felser, Claudia Ong, N. P. Cava, R. J. TI Paramagnetic to ferromagnetic phase transition in lightly Fe-doped Cr2B SO PHYSICAL REVIEW B LA English DT Article ID HEAVY-FERMION COMPOUNDS; QUANTUM CRITICALITY; METALS; RESISTIVITY; PRESSURE; ALLOYS AB Cr2B displays temperature-independent paramagnetism. We induce ferromagnetism by replacing less than 3% of the Cr atoms by Fe. By the lowest Fe doping level made, Curie-Weiss behavior is observed; Theta(CW) changes from -20 K for 0.5% Fe-doped Cr2B to positive values of about 50 K by 5% Fe doping. The ferromagnetic T-C is 8 K for 2.5% Fe doping and increases linearly to 46 K by 5% doping; we infer that a quantum phase transition occurs near the 2.0% Fe level. Magnetic fluctuations at the intermediate doping levels are reflected in the linear resistance and an anomalous heat capacity at low temperatures. Imaging and chemical analysis down to the atomic scale show that the Fe dopant is randomly distributed. C1 [Schoop, Leslie; Cava, R. J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Schoop, Leslie; Felser, Claudia] Max Planck Inst Chem Phys Fester Stoffe, D-01187 Dresden, Germany. [Hirschberger, Max; Ong, N. P.] Princeton Univ, Dept Phys, Joseph Henry Lab, Princeton, NJ 08544 USA. [Tao, Jing] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Schoop, L (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. EM lschoop@princeton.edu RI Schoop, Leslie/A-4627-2013; Felser, Claudia/A-5779-2009 OI Schoop, Leslie/0000-0003-3459-4241; Felser, Claudia/0000-0002-8200-2063 FU US Department of Energy (DOE) Office of Basic Energy Sciences [DOE FG02-08ER45706]; NSFMRSEC program [DMR-0819860]; DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-98CH10886] FX The materials preparation, structural characterization, and magnetic and specific heat measurements were supported by the US Department of Energy (DOE) Office of Basic Energy Sciences, Grant No. DOE FG02-08ER45706. The transport studies were supported by the NSFMRSEC program, Grant No. DMR-0819860. The electron microscopy study was supported by the DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-98CH10886. The authors acknowledge helpful discussions with David Huse, F. Malte Grosche, Kai Sun, and Neel Haldolaarachchige. NR 23 TC 5 Z9 5 U1 0 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 26 PY 2014 VL 89 IS 22 AR 224417 DI 10.1103/PhysRevB.89.224417 PG 7 WC Physics, Condensed Matter SC Physics GA AK2XC UT WOS:000338282500004 ER PT J AU Taylor, CD Francis, MF Schwartz, DS AF Taylor, Christopher D. Francis, Michael F. Schwartz, Daniel S. TI Thermodynamics, structure, and charge state of hydrogen-vacancy complexes in delta-plutonium SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; METAL-HYDRIDES; SUPERABUNDANT VACANCIES; AB-INITIO; H ALLOYS; KINETICS; EMBRITTLEMENT; DENSITY; PRESSURES; HELIUM AB Hydrogen-vacancy complexes can form in a material due to the exothermic binding of hydrogen atoms to vacancy sites. We explore the structure and electronic properties of hydrogen-vacancy complexes in delta-Pu using a density functional theory supercell approach, with up to eight hydrogen atoms stored in the vacancy site. We find that the hydrogen atoms bind to the inner edge of the vacancy site, preferring pseudo-octahedral configurations that optimize the Pu-H bond length. Hydrogen binding to the vacancy site remains exothermic, with binding energies around -0.4 eV/H atom. A statistical mechanics analysis is derived and applied to reveal the range of hydrogen chemical potentials that would lead to hydrogen-vacancy complex formation. We find that these chemical potentials are higher than those required to form the hydride phase, indicating that hydriding should occur before any appreciable concentration of vacancy-hydrogen complexes is realized. Some remarks are made comparing this theoretical finding to the experimental work on this topic, with suggestions given for future work that may help reconcile some apparent contradictions. C1 [Taylor, Christopher D.] DNV GL, Dublin, OH 43017 USA. [Taylor, Christopher D.] Ohio State Univ, Fontana Corros Ctr, Columbus, OH 43210 USA. [Francis, Michael F.] Ecole Polytech Fed Lausanne, Lausanne, Switzerland. [Francis, Michael F.] Brown Univ, Providence, RI 02912 USA. [Schwartz, Daniel S.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Taylor, CD (reprint author), DNV GL, Dublin, OH 43017 USA. OI Taylor, Christopher/0000-0002-0252-0988 FU LANL LDRD program; Seaborg Summer Student Fellowship program (Michael Francis); Los Alamos National Security LLC for the National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX The authors gratefully acknowledge conversations with W. A. Curtin (Brown University), Steve Valone (LANL), and Scott Richmond (LANL) regarding the findings and derivations included in this work. Funding to support this work was provided through the LANL LDRD program and the Seaborg Summer Student Fellowship program (Michael Francis). High performance institutional computing resources at LANL were used to complete this research. The Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the US Department of Energy under Contract DE-AC52-06NA25396. NR 45 TC 4 Z9 4 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 26 PY 2014 VL 89 IS 21 AR 214114 DI 10.1103/PhysRevB.89.214114 PG 10 WC Physics, Condensed Matter SC Physics GA AK2XA UT WOS:000338282300001 ER PT J AU Eibach, M Beyer, T Blaum, K Block, M Dullmann, CE Eberhardt, K Grund, J Nagy, S Nitsche, H Nortershauser, W Renisch, D Rykaczewski, KP Schneider, F Smorra, C Vieten, J Wang, M Wendt, K AF Eibach, M. Beyer, T. Blaum, K. Block, M. Duellmann, Ch. E. Eberhardt, K. Grund, J. Nagy, Sz. Nitsche, H. Noertershaeuser, W. Renisch, D. Rykaczewski, K. P. Schneider, F. Smorra, C. Vieten, J. Wang, M. Wendt, K. TI Direct high-precision mass measurements on Am-241,Am-243, Pu-244, and Cf-249 SO PHYSICAL REVIEW C LA English DT Article ID SUPERHEAVY NUCLEI; HEAVIEST ELEMENTS; CARBON CLUSTERS; PENNING TRAP; BETA-DECAY; SPECTROMETRY; SPECTROSCOPY; ISOLTRAP; IONS AB The absolute masses of four long-lived transuranium nuclides, Am-241,Am-243, Pu-244, and Cf-249, in the vicinity of the deformed N = 152 neutron shell closure have been measured directly with the Penning-trap mass spectrometer TRIGA-TRAP. Our measurements confirm the AME2012 mass values of 241,243Am and 244Pu within one standard deviation, which were indirectly determined, by decay spectroscopy studies. In the case of the Cf-249 mass, a discrepancy of more than three standard deviations has been observed, affecting absolute masses even in the superheavy element region. The implementation of the mass values into the AME2012 network yields a reduced mass uncertainty for 84 nuclides, particularly for Pu-244 and its strongly correlated a decay chains. C1 [Eibach, M.; Beyer, T.; Blaum, K.; Nagy, Sz.; Smorra, C.; Wang, M.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Eibach, M.; Duellmann, Ch. E.; Eberhardt, K.; Grund, J.; Noertershaeuser, W.; Renisch, D.; Schneider, F.] Johannes Gutenberg Univ Mainz, Inst Kernchem, D-55128 Mainz, Germany. [Block, M.; Duellmann, Ch. E.; Noertershaeuser, W.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Duellmann, Ch. E.; Grund, J.] Johannes Gutenberg Univ Mainz, PRISMA Cluster Excellence, D-55128 Mainz, Germany. [Duellmann, Ch. E.; Eberhardt, K.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Nitsche, H.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Noertershaeuser, W.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. [Rykaczewski, K. P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Schneider, F.; Wendt, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55128 Mainz, Germany. [Vieten, J.] Tech Univ Munich, D-80333 Munich, Germany. [Wang, M.] Univ Paris 11, Ctr Spectrometrie Nucl & Spectrometrie Masse, F-91405 Orsay, France. [Wang, M.] Inst Modern Phys, Lanzhou 730000, Peoples R China. RP Eibach, M (reprint author), Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. EM martin.eibach@uni-mainz.de RI Nortershauser, Wilfried/A-6671-2013; Block, Michael/I-2782-2015; Smorra, Christian/C-5606-2017 OI Nortershauser, Wilfried/0000-0001-7432-3687; Block, Michael/0000-0001-9282-8347; FU BMBF [05P09 UMFN5, 05P12UMFN8, 05P12UMFN3]; Alliance Program of the Helmholtz Association [HA216/EMMI]; Max Planck Society; PRISMA Cluster of Excellence; Helmholtz Institut Mainz FX We thank the Institut fur Kernchemie in Mainz and the U.S. DOE Office of Science for providing us with pure isotopic samples through ORNL as well as J. Runke and C. Mokry for their support during chemical preparation, and G. Audi for his support implementing the data into the AME. The 249Cf was made available by H.N. It was produced through the former Transplutonium Element Production Program at Oak Ridge National Laboratory (ORNL) under the auspices of the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U. S. Department of Energy. M.E. acknowledges support by the BMBF under contract no. 05P09 UMFN5 and Sz.N. acknowledges support by the Alliance Program of the Helmholtz Association (HA216/EMMI). This work has been supported by the Max Planck Society, the BMBF under contract nos. 05P12UMFN8 and 05P12UMFN3, the PRISMA Cluster of Excellence, and the Helmholtz Institut Mainz. NR 46 TC 9 Z9 9 U1 0 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 26 PY 2014 VL 89 IS 6 AR 064318 DI 10.1103/PhysRevC.89.064318 PG 8 WC Physics, Nuclear SC Physics GA AK2XK UT WOS:000338283300003 ER PT J AU Schmidt, A Link, A Welch, D Ellsworth, J Falabella, S Tang, V AF Schmidt, A. Link, A. Welch, D. Ellsworth, J. Falabella, S. Tang, V. TI Comparisons of dense-plasma-focus kinetic simulations with experimental measurements SO PHYSICAL REVIEW E LA English DT Article ID DISCHARGES; PINCH AB Dense-plasma-focus (DPF) Z-pinch devices are sources of copious high-energy electrons and ions, x rays, and neutrons. The mechanisms through which these physically simple devices generate such high-energy beams in a relatively short distance are not fully understood and past optimization efforts of these devices have been largely empirical. Previously we reported on fully kinetic simulations of a DPF and compared them with hybrid and fluid simulations of the same device. Here we present detailed comparisons between fully kinetic simulations and experimental data on a 1.2 kJ DPF with two electrode geometries, including neutron yield and ion beam energy distributions. A more intensive third calculation is presented which examines the effects of a fully detailed pulsed power driver model. We also compare simulated electromagnetic fluctuations with direct measurement of radiofrequency electromagnetic fluctuations in a DPF plasma. These comparisons indicate that the fully kinetic model captures the essential physics of these plasmas with high fidelity, and provide further evidence that anomalous resistivity in the plasma arises due to a kinetic instability near the lower hybrid frequency. C1 [Schmidt, A.; Link, A.; Ellsworth, J.; Falabella, S.; Tang, V.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Welch, D.] Voss Sci LLC, Albuquerque, NM 87108 USA. RP Schmidt, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU US Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [11-ERD-063] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract No. DE-AC52-07NA27344 and was supported by the Laboratory Directed Research and Development Program (11-ERD-063) at LLNL. Computing support for this work came from the LLNL Institutional Computing Grand Challenge program. NR 20 TC 6 Z9 6 U1 3 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUN 26 PY 2014 VL 89 IS 6 AR 061101 DI 10.1103/PhysRevE.89.061101 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AK2XS UT WOS:000338284200002 PM 25019717 ER PT J AU Bernardi, M Vigil-Fowler, D Lischner, J Neaton, JB Louie, SG AF Bernardi, Marco Vigil-Fowler, Derek Lischner, Johannes Neaton, Jeffrey B. Louie, Steven G. TI Ab Initio Study of Hot Carriers in the First Picosecond after Sunlight Absorption in Silicon SO PHYSICAL REVIEW LETTERS LA English DT Article ID LOCALIZED WANNIER FUNCTIONS; SOLAR-ENERGY CONVERSION; QUASI-PARTICLE; ELECTRON-GAS; SEMICONDUCTORS; EFFICIENCY; CELLS; TRANSPORT AB Hot carrier thermalization is a major source of efficiency loss in solar cells. Because of the subpicosecond time scale and complex physics involved, a microscopic characterization of hot carriers is challenging even for the simplest materials. We develop and apply an ab initio approach based on density functional theory and many-body perturbation theory to investigate hot carriers in semiconductors. Our calculations include electron-electron and electron-phonon interactions, and require no experimental input other than the structure of the material. We apply our approach to study the relaxation time and mean free path of hot carriers in Si, and map the band and k dependence of these quantities. We demonstrate that a hot carrier distribution characteristic of Si under solar illumination thermalizes within 350 fs, in excellent agreement with pump-probe experiments. Our work sheds light on the subpicosecond time scale after sunlight absorption in Si, and constitutes a first step towards ab initio quantification of hot carrier dynamics in materials. C1 [Bernardi, Marco; Vigil-Fowler, Derek; Lischner, Johannes; Neaton, Jeffrey B.; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bernardi, Marco; Vigil-Fowler, Derek; Lischner, Johannes; Neaton, Jeffrey B.; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Inst Energy Nanosci, Berkeley, CA 94720 USA. RP Neaton, JB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM jbneaton@lbl.gov; sglouie@berkeley.edu RI Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014 OI Neaton, Jeffrey/0000-0001-7585-6135; FU SciDAC Program on Excited State Phenomena in Energy Materials - U. S. Department of Energy, Office of Basic Energy Sciences and of Advanced Scientific Computing Research at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; National Science Foundation [DMR 10-1006184]; Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy [DE-AC02-05CH11231]; Simons Foundation Fellowship in Theoretical Physics; Office of Science of the U.S. Department of Energy FX M. B. thanks Sinisa Coh for discussion. This research was supported by the SciDAC Program on Excited State Phenomena in Energy Materials funded by the U. S. Department of Energy, Office of Basic Energy Sciences and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory, which provided for algorithm and code developments and simulations; and by the National Science Foundation under Grant No. DMR 10-1006184 which provided for basic theory and formalism. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy. NR 36 TC 44 Z9 44 U1 1 U2 43 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 26 PY 2014 VL 112 IS 25 AR 257402 DI 10.1103/PhysRevLett.112.257402 PG 5 WC Physics, Multidisciplinary SC Physics GA AK2XY UT WOS:000338284900014 PM 25014830 ER PT J AU Edwards, DE Zubarev, DY Packard, A Lester, WA Frenklach, M AF Edwards, David E. Zubarev, Dmitry Yu. Packard, Andrew Lester, William A., Jr. Frenklach, Michael TI Interval Prediction of Molecular Properties in Parametrized Quantum Chemistry SO PHYSICAL REVIEW LETTERS LA English DT Article ID MONTE-CARLO; WAVE-FUNCTIONS; MODEL; OPTIMIZATION; PERFORMANCE; ACCURACY; AM1 AB The accurate evaluation of molecular properties lies at the core of predictive physical models. Most reliable quantum-chemical calculations are limited to smaller molecular systems while purely empirical approaches are limited in accuracy and reliability. A promising approach is to employ a quantum-mechanical formalism with simplifications and to compensate for the latter with parametrization. We propose a strategy of directly predicting the uncertainty interval for a property of interest, based on training-data uncertainties, which sidesteps the need for an optimum set of parameters. C1 [Edwards, David E.; Packard, Andrew; Frenklach, Michael] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Edwards, David E.; Frenklach, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Zubarev, Dmitry Yu.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Lester, William A., Jr.] Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. [Lester, William A., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Edwards, DE (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM frenklach@berkeley.edu FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the U.S. Department of Energy [AC03-76F00098]; Air Force Office of Scientific Research [FA9550-12-1-0165]; National Energy Research Scientific Computing Center; Office of Science of the U. S. Department of Energy [DE AC02 05CH11231] FX D. E. E., W. A. L., and M. F. were supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the U.S. Department of Energy, under Contract No. DE AC03-76F00098. M. F. was supported by the Air Force Office of Scientific Research, Grant No. FA9550-12-1-0165. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE AC02 05CH11231. NR 42 TC 3 Z9 3 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 26 PY 2014 VL 112 IS 25 AR 253003 DI 10.1103/PhysRevLett.112.253003 PG 5 WC Physics, Multidisciplinary SC Physics GA AK2XY UT WOS:000338284900003 PM 25014809 ER PT J AU Glaser, A Barak, B Goldston, RJ AF Glaser, Alexander Barak, Boaz Goldston, Robert J. TI A zero-knowledge protocol for nuclear warhead verification SO NATURE LA English DT Article ID DOSIMETRY AB The verification of nuclear warheads for arms control involves a paradox: international inspectors will have to gain high confidence in the authenticity of submitted items while learning nothing about them. Proposed inspection systems featuring 'information barriers', designed to hide measurements stored in electronic systems, are at risk of tampering and snooping. Here we show the viability of a fundamentally new approach to nuclear warhead verification that incorporates a zero-knowledge protocol, which is designed in such a way that sensitive information is never measured and so does not need to be hidden. We interrogate submitted items with energetic neutrons, making, in effect, differential measurements of both neutron transmission and emission. Calculations for scenarios in which material is diverted from a test object show that a high degree of discrimination can be achieved while revealing zero information. Our ideas for a physical zero-knowledge system could have applications beyond the context of nuclear disarmament. The proposed technique suggests a way to perform comparisons or computations on personal or confidential data without measuring the data in the first place. C1 [Glaser, Alexander] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Barak, Boaz] Microsoft Res, Cambridge, MA 02142 USA. [Goldston, Robert J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. RP Glaser, A (reprint author), Princeton Univ, Dept Mech & Aerosp Engn, Olden St, Princeton, NJ 08544 USA. EM aglaser@princeton.edu FU Global Zero; US Department of State; Princeton Plasma Physics Laboratory (DOE) [DE-AC02-09CH11466] FX This project was supported by Global Zero and the US Department of State, the Princeton Plasma Physics Laboratory (DOE contract DE-AC02-09CH11466) and in-kind contributions from Microsoft Research New England. We thank D. Dobkin, F. d'Errico, J. Fuller, D. MacArthur, J. Mihalczo, S. Philippe and M. Walker for discussions and feedback. We thank S. Philippe (Princeton University) for graphics in Fig. 2. All simulations were run on Princeton University's High Performance Cluster. NR 18 TC 10 Z9 10 U1 1 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUN 26 PY 2014 VL 510 IS 7506 BP 497 EP 502 DI 10.1038/nature13457 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ6LK UT WOS:000337806300038 PM 24965650 ER PT J AU Cheng, C Guo, H Amini, A Liu, K Fu, D Zou, J Song, HS AF Cheng, Chun Guo, Hua Amini, Abbas Liu, Kai Fu, Deyi Zou, Jian Song, Haisheng TI Self-Assembly and Horizontal Orientation Growth of VO2 Nanowires SO SCIENTIFIC REPORTS LA English DT Article ID METAL-INSULATOR-TRANSITION; VANADIUM DIOXIDE; PHASE-TRANSITION; CRYSTAL; NANOPLATELETS; NANOBEAM; STRAIN AB Single-crystalline vanadium dioxide (VO2) nanostructures have attracted an intense research interest recently because of their unique single-domain metal-insulator phase transition property. Synthesis of these nanostructures in the past was limited in density, alignment, or single-crystallinity. The assembly of VO2 nanowires (NWs) is desirable for a "bottom-up" approach to the engineering of intricate structures using nanoscale building blocks. Here, we report the successful synthesis of horizontally aligned VO2 NWs with a dense growth mode in the [1-100] quartz direction of a polished x-cut quartz surface using a simple vapor transport method. Our strategy of controlled growth of VO2 NWs promisingly paves the way for designing novel metal-insulator transition devices based on VO2 NWs. C1 [Cheng, Chun] South Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China. [Guo, Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Amini, Abbas] Univ Western Sydney, Sch Comp Engn & Math, Kingswood, NSW 2751, Australia. [Liu, Kai; Fu, Deyi; Zou, Jian] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. Huazhong Univ Sci & Technol, WNLO, Wuhan 430074, Peoples R China. [Song, Haisheng] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Peoples R China. RP Cheng, C (reprint author), South Univ Sci & Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China. EM cheng.c@sustc.edu.cn RI cheng, chun/B-5043-2011; Liu, Kai/A-4754-2012; Fu, Deyi/C-6624-2011 OI cheng, chun/0000-0001-7319-4393; Liu, Kai/0000-0002-0638-5189; Fu, Deyi/0000-0003-1365-8963 FU South University of Science and Technology of China FX Financial support from starting grants from South University of Science and Technology of China is gratefully acknowledged. The authors would like to thank Professor Junqiao Wu of the Department of Materials Science and Engineering, University of California, Berkeley, CA, USA and his laboratory for their kind support and for providing resources. NR 26 TC 10 Z9 10 U1 9 U2 84 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 26 PY 2014 VL 4 AR 5456 DI 10.1038/srep05456 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7QT UT WOS:000337892000005 PM 24965899 ER PT J AU Fensin, SJ Cerreta, EK Gray, GT Valone, SM AF Fensin, S. J. Cerreta, E. K. Gray, G. T., III Valone, S. M. TI Why are some Interfaces in Materials Stronger than others? SO SCIENTIFIC REPORTS LA English DT Article ID GRAIN-BOUNDARIES; DYNAMIC FAILURE; METALS; COPPER; DAMAGE; DEFORMATION; SOLIDS AB Grain boundaries (GBs) are often the preferred sites for void nucleation in ductile metals. However, it has been observed that all boundaries do not contribute equally to this process. We present a mechanistic rationale for the role of GBs in damage nucleation in copper, along with a quantitative map for predicting preferred void nucleation at GBs based on molecular dynamics simulations in copper. Simulations show a direct correlation between the void nucleation stress and the ability of a grain boundary to plastically deform by emitting dislocations, during shock compression. Plastic response of a GB, affects the development of stress concentrations believed to be responsible for void nucleation by acting as a dissipation mechanism for the applied stress. C1 [Fensin, S. J.; Cerreta, E. K.; Gray, G. T., III; Valone, S. M.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87544 USA. RP Fensin, SJ (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87544 USA. EM saryuj@lanl.gov FU U.S Department of Energy [DE-AC52-06NA25396]; office of Basic Energy Sciences; Energy Frontier Research Centre of Materials at irradiation and mechanical extremes (CMIME) FX Los Alamos National Laboratory is operated by LANS, LLC, for the NNSA and the U.S Department of Energy under contract DE-AC52-06NA25396. This work has been supported by the office of Basic Energy Sciences and the Energy Frontier Research Centre of Materials at irradiation and mechanical extremes (CMIME). NR 39 TC 8 Z9 8 U1 4 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 26 PY 2014 VL 4 AR 5461 DI 10.1038/srep05461 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7QT UT WOS:000337892000010 PM 24964801 ER PT J AU Chen, XW Shekiro, J Pschorn, T Sabourin, M Tao, L Elander, R Park, S Jennings, E Nelson, R Trass, O Flanegan, K Wang, W Himmel, ME Johnson, D Tucker, MP AF Chen, Xiaowen Shekiro, Joseph Pschorn, Thomas Sabourin, Marc Tao, Ling Elander, Rick Park, Sunkyu Jennings, Ed Nelson, Robert Trass, Olev Flanegan, Keith Wang, Wei Himmel, Michael E. Johnson, David Tucker, Melvin P. TI A highly efficient dilute alkali deacetylation and mechanical (disc) refining process for the conversion of renewable biomass to lower cost sugars SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Biofuels; Pretreatment; Enzymatic hydrolysis; Deacetylation; Mechanical refining; Disc refining; No acid pretreatment; PFI milling; Clean sugar production ID PRETREATED CORN STOVER; EXPANSION AFEX PRETREATMENT; ENZYMATIC-HYDROLYSIS; ACID PRETREATMENT; EXTRUSION PRETREATMENT; ETHANOL-PRODUCTION; PHOSPHORIC-ACID; AMMONIA; PERFORMANCE; EXTRACTION AB Background: The deconstruction of renewable biomass feedstocks into soluble sugars at low cost is a critical component of the biochemical conversion of biomass to fuels and chemicals. Providing low cost high concentration sugar syrups with low levels of chemicals and toxic inhibitors, at high process yields is essential for biochemical platform processes using pretreatment and enzymatic hydrolysis. In this work, we utilize a process consisting of deacetylation, followed by mechanical refining in a disc refiner (DDR) for the conversion of renewable biomass to low cost sugars at high yields and at high concentrations without a conventional chemical pretreatment step. The new process features a low temperature dilute alkaline deacetylation step followed by disc refining under modest levels of energy consumption. Results: The proposed process was demonstrated using a commercial scale Andritz double disc refiner. Disc refined and deacetylated corn stover result in monomeric glucose yields of 78 to 84% and monomeric xylose yields of 71 to 77% after enzymatic hydrolysis at process-relevant solids and enzyme loadings. The glucose and xylose yields of the disc refined substrates in enzymatic hydrolysis are enhanced by 13% and 19%, respectively. Fermentation of the DDR substrates at 20% total solids with Z.mobilis utilized almost all sugars in 20hrs indicating the sugar hydrolyzate produced from the DDR process is highly fermentable due to low levels of chemical contaminants. The ethanol titer and ethanol process yield are approximately 70 g/L and 90% respectively. Conclusions: The proposed new process has been demonstrated using pilot scale deacetylation and disc refiners. The deacetylated and disc refined corn stover was rapidly deconstructed to monomeric sugars at 20% wt solids with enzymatic hydrolysis. High process sugar conversions were achieved, with high concentrations of monomeric sugars that exceeded 150 g/L. The sugar syrups produced were found to have low concentrations of known major fermentation inhibitors: acetic acid, furfural and HMF. The low levels of these fermentation inhibitors lead to high fermentation yields. The results suggest that this process is a very promising development for the nascent cellulosic biofuels industry. C1 [Chen, Xiaowen; Shekiro, Joseph; Tao, Ling; Elander, Rick; Jennings, Ed; Nelson, Robert; Tucker, Melvin P.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80127 USA. [Pschorn, Thomas; Sabourin, Marc] Andritz Inc, Springfield, OH 45504 USA. [Park, Sunkyu] N Carolina State Univ, Dept Forest Biomat, Raleigh, NC 27695 USA. [Trass, Olev] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON M5S 3E5, Canada. [Flanegan, Keith] IdeaCHEM Inc, Rapid City, SD 57701 USA. [Wang, Wei; Himmel, Michael E.; Johnson, David] Natl Renewable Energy Lab, Natl Biosci Ctr, Golden, CO 80127 USA. RP Chen, XW (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 1617 Cole Blvd, Golden, CO 80127 USA. EM Xiaowen.Chen@nrel.gov; Joseph.Shekiro@nrel.gov; Melvin.Tucker@nrel.gov FU BETO (Bioenergy Technologies Office) program in DOE (Department of Energy) EERE (Office of Energy Efficiency and Renewable Energy) FX We would like to acknowledge the funding support from the BETO (Bioenergy Technologies Office) program in DOE (Department of Energy) EERE (Office of Energy Efficiency and Renewable Energy). We also want to thank the biomass analytical team for their technical assistance and analysis. NR 43 TC 13 Z9 13 U1 3 U2 48 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUN 25 PY 2014 VL 7 AR 98 DI 10.1186/1754-6834-7-98 PG 11 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AM0YB UT WOS:000339572500001 ER PT J AU Lind, KR Sizmur, T Benomar, S Miller, A Cademartiri, L AF Lind, Kara R. Sizmur, Tom Benomar, Saida Miller, Anthony Cademartiri, Ludovico TI LEGO (R) Bricks as Building Blocks for Centimeter-Scale Biological Environments: The Case of Plants SO PLOS ONE LA English DT Article ID ROOT-SYSTEM ARCHITECTURE; 3D CELL-CULTURE; ARABIDOPSIS-THALIANA; MICROFLUIDIC CHIP; TISSUE; SOIL; GROWTH AB LEGO bricks are commercially available interlocking pieces of plastic that are conventionally used as toys. We describe their use to build engineered environments for cm-scale biological systems, in particular plant roots. Specifically, we take advantage of the unique modularity of these building blocks to create inexpensive, transparent, reconfigurable, and highly scalable environments for plant growth in which structural obstacles and chemical gradients can be precisely engineered to mimic soil. C1 [Lind, Kara R.; Sizmur, Tom; Benomar, Saida; Miller, Anthony; Cademartiri, Ludovico] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Sizmur, Tom; Benomar, Saida; Cademartiri, Ludovico] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA USA. [Miller, Anthony] Iowa State Univ, Dept Agron, Ames, IA USA. [Cademartiri, Ludovico] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA USA. RP Cademartiri, L (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM lcademar@iastate.edu RI Cademartiri, Ludovico/A-4142-2008 OI Cademartiri, Ludovico/0000-0001-8805-9434 FU Iowa State University FX The work was funded by Iowa State University through a startup grant to LC. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 37 TC 4 Z9 4 U1 5 U2 30 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 25 PY 2014 VL 9 IS 6 AR e100867 DI 10.1371/journal.pone.0100867 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK8WO UT WOS:000338709500092 PM 24963716 ER PT J AU Rosenstierne, MW McLoughlin, KS Olesen, ML Papa, A Gardner, SN Engler, O Plumet, S Mirazimi, A Weidmann, M Niedrig, M Fomsgaard, A Erlandsson, L AF Rosenstierne, Maiken W. McLoughlin, Kevin S. Olesen, Majken Lindholm Papa, Anna Gardner, Shea N. Engler, Olivier Plumet, Sebastien Mirazimi, Ali Weidmann, Manfred Niedrig, Matthias Fomsgaard, Anders Erlandsson, Lena TI The Microbial Detection Array for Detection of Emerging Viruses in Clinical Samples - A Useful Panmicrobial Diagnostic Tool SO PLOS ONE LA English DT Article ID CONGO HEMORRHAGIC-FEVER; REAL-TIME PCR; RESPIRATORY-TRACT INFECTIONS; REVERSE TRANSCRIPTION-PCR; WEST-NILE-VIRUS; RT-PCR; LABORATORY DETECTION; RNA; IDENTIFICATION; MICROARRAY AB Emerging viruses are usually endemic to tropical and sub-tropical regions of the world, but increased global travel, climate change and changes in lifestyle are believed to contribute to the spread of these viruses into new regions. Many of these viruses cause similar disease symptoms as other emerging viruses or common infections, making these unexpected pathogens difficult to diagnose. Broad-spectrum pathogen detection microarrays containing probes for all sequenced viruses and bacteria can provide rapid identification of viruses, guiding decisions about treatment and appropriate case management. We report a modified Whole Transcriptome Amplification (WTA) method that increases unbiased amplification, particular of RNA viruses. Using this modified WTA method, we tested the specificity and sensitivity of the Lawrence Livermore Microbial Detection Array (LLMDA) against a wide range of emerging viruses present in both non-clinical and clinical samples using two different microarray data analysis methods. C1 [Rosenstierne, Maiken W.; Olesen, Majken Lindholm; Fomsgaard, Anders; Erlandsson, Lena] Statens Serum Inst, Dept Microbiol Diagnost & Virol, DK-2300 Copenhagen, Denmark. [McLoughlin, Kevin S.; Gardner, Shea N.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Papa, Anna] Aristotle Univ Thessaloniki, Dept Microbiol, GR-54006 Thessaloniki, Greece. [Engler, Olivier] Fed Off Civil Protect, Spiez Lab, Spiez, Switzerland. [Plumet, Sebastien] French Army Forces Biomed Inst IRBA, Dept Virol, Marseille, France. [Mirazimi, Ali] Swedish Inst Communicable Dis Control, Solna, Sweden. [Mirazimi, Ali] Natl Vet Inst SVA, Uppsala, Sweden. [Mirazimi, Ali] Linkoping Univ, Dept Clin & Expt Med, Linkoping, Sweden. [Weidmann, Manfred] Univ Stirling, Inst Aquaculture, Stirling FK9 4LA, Scotland. [Niedrig, Matthias] Robert Koch Inst, Ctr Biosafety, Berlin, Germany. [Fomsgaard, Anders] Univ Southern Denmark, Inst Clin Res, Odense, Denmark. RP Rosenstierne, MW (reprint author), Statens Serum Inst, Dept Microbiol Diagnost & Virol, DK-2300 Copenhagen, Denmark. EM MWR@ssi.dk RI Weidmann, Manfred/G-1817-2015 OI Weidmann, Manfred/0000-0002-7063-7491 FU European Commission under the Health Cooperation Work Program of the 7th Framework Program for contributing with CCHFV-positive clinical samples [260427]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Solvej Jensen, Birgit Knudsen, Bente Ostergaard and Britt Christensen for expert technical help. We thank the CCH Fever Network supported by the European Commission under the Health Cooperation Work Program of the 7th Framework Program (no. 260427) for contributing with CCHFV-positive clinical samples. This work was performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 46 TC 4 Z9 4 U1 1 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 25 PY 2014 VL 9 IS 6 AR e100813 DI 10.1371/journal.pone.0100813 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK8WO UT WOS:000338709500083 PM 24963710 ER PT J AU Schaudinn, C Stoodley, P Hall-Stoodley, L Gorur, A Remis, J Wu, S Auer, M Hertwig, S Guerrero-Given, D Hu, FZ Ehrlich, GD Costerton, JW Robinson, DH Webster, P AF Schaudinn, Christoph Stoodley, Paul Hall-Stoodley, Luanne Gorur, Amita Remis, Jonathan Wu, Siva Auer, Manfred Hertwig, Stefan Guerrero-Given, Debbie Hu, Fen Ze Ehrlich, Garth D. Costerton, John William Robinson, Douglas H. Webster, Paul TI Death and Transfiguration in Static Staphylococcus epidermidis Cultures SO PLOS ONE LA English DT Article ID POLYSACCHARIDE INTERCELLULAR ADHESIN; TARGETED OLIGONUCLEOTIDE PROBES; IN-SITU HYBRIDIZATION; BIOFILM FORMATION; BINDING; ACCUMULATION; POPULATIONS; MICROSCOPY; ORGANISMS; BACTERIA AB The overwhelming majority of bacteria live in slime embedded microbial communities termed biofilms, which are typically adherent to a surface. However, when several Staphylococcus epidermidis strains were cultivated in static liquid cultures, macroscopic aggregates were seen floating within the broth and also sedimented at the test tube bottom. Light-and electron microscopy revealed that early-stage aggregates consisted of bacteria and extracellular matrix, organized in sheet-like structures. Perpendicular under the sheets hung a network of periodically arranged, bacteria-associated strands. During the extended cultivation, the strands of a subpopulation of aggregates developed into cross-connected wall-like structures, in which aligned bacteria formed the walls. The resulting architecture had a compartmentalized appearance. In late-stage cultures, the wall-associated bacteria disintegrated so that, henceforth, the walls were made of the coalescing remnants of lysed bacteria, while the compartment-like organization remained intact. At the same time, the majority of strand-containing aggregates with associated culturable bacteria continued to exist. These observations indicate that some strains of Staphylococcus epidermidis are able to build highly sophisticated structures, in which a subpopulation undergoes cell lysis, presumably to provide continued access to nutrients in a nutrient-limited environment, whilst maintaining structural integrity. C1 [Schaudinn, Christoph] Robert Koch Inst, Ctr Biol Threats & Special Pathogens, Berlin, Germany. [Stoodley, Paul; Hall-Stoodley, Luanne] Dept Microbial Infect & Immun, Columbus, OH USA. [Stoodley, Paul; Hall-Stoodley, Luanne] Dept Orthoped, Columbus, OH USA. [Gorur, Amita; Remis, Jonathan; Wu, Siva; Auer, Manfred] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Hertwig, Stefan] Fed Inst Risk Assessment, Dept Biol Safety, Berlin, Germany. [Guerrero-Given, Debbie] Max Planck Florida Inst, Jupiter, FL USA. [Hu, Fen Ze; Ehrlich, Garth D.; Costerton, John William] Drexel Univ, Coll Med, Ctr Genom Sci, Philadelphia, PA 19104 USA. [Hu, Fen Ze; Ehrlich, Garth D.; Costerton, John William] Drexel Univ, Coll Med, Ctr Adv Microbial Proc, Inst Mol Med & Infect Dis,Dept Microbiol & Immuno, Philadelphia, PA 19104 USA. [Robinson, Douglas H.] DeNovo Biol LLC, Arlington, VA USA. [Webster, Paul] Univ So Calif, Ctr Electron Microscopy & Microanal, Los Angeles, CA USA. [Webster, Paul] Oak Crest Inst Sci, Pasadena, CA USA. RP Schaudinn, C (reprint author), Robert Koch Inst, Ctr Biol Threats & Special Pathogens, Berlin, Germany. EM schaudinnc@rki.de RI Stoodley, Paul/E-5079-2013 OI Stoodley, Paul/0000-0001-6069-273X FU Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; NIDCD [5 P-30 DC006276-03]; National Science Foundation (NSF) [0722354] FX J. P. Remis and M. Auer acknowledge support by the Office of Biological and Environmental Research of the US Department of Energy under contract number DE-AC02-05CH11231. Furthermore, the authors would like to express gratitude to the House Research Institute (Los Angeles) for funding this project in part, and for the generosity of the Ahmanson Foundation in supporting the Ahmanson Imaging Core. Grants from the NIDCD (5 P-30 DC006276-03) and the National Science Foundation (NSF #0722354) also supported the Ahmanson Imaging Core where a substantial part of this work was performed. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 35 TC 4 Z9 4 U1 2 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 25 PY 2014 VL 9 IS 6 AR e100002 DI 10.1371/journal.pone.0100002 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK8WO UT WOS:000338709500026 PM 24964210 ER PT J AU Anand, N Fitzpatrick, AL Haxton, WC AF Anand, Nikhil Fitzpatrick, A. Liam Haxton, W. C. TI Weakly interacting massive particle-nucleus elastic scattering response SO PHYSICAL REVIEW C LA English DT Article ID DARK-MATTER CANDIDATES AB Background: A model-independent formulation of weakly interacting massive particle (WIMP)-nucleon scattering was recently developed in Galilean-invariant effective field theory. Purpose: Here we complete the embedding of this effective interaction in the nucleus, constructing the most general elastic nuclear cross section as a factorized product of WIMP and nuclear response functions. This form explicitly defines what can and cannot be learned about the low-energy constants of the effective theory-and consequently about candidate ultraviolet theories of dark matter-from elastic scattering experiments. Results: We identify those interactions that cannot be reliably treated in a spin-independent/spin-dependent (SI/SD) formulation: For derivative-or velocity-dependent couplings, the SI/SD formulation generally mischaracterizes the relevant nuclear operator and its multipolarity (e.g., scalar or vector) and greatly underestimates experimental sensitivities. This can lead to apparent conflicts between experiments when, in fact, none may exist. The new nuclear responses appearing in the factorized cross section are related to familiar electroweak nuclear operators such as angular momentum (l) over right arrow (i) and the spin-orbit coupling (sigma) over right arrow (i) . (l) over right arrow l(i). Conclusions: To unambiguously interpret experiments and to extract all of the available information on the particle physics of dark matter, experimentalists will need to (1) do a sufficient number of experiments with nuclear targets having the requisite sensitivities to the various operators and (2) analyze the results in a formalism that does not arbitrarily limit the candidate operators. In an appendix we describe a code that is available to help interested readers implement such an analysis. C1 [Anand, Nikhil; Haxton, W. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Fitzpatrick, A. Liam] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94305 USA. [Haxton, W. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Anand, N (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. NR 14 TC 46 Z9 46 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 25 PY 2014 VL 89 IS 6 AR 065501 DI 10.1103/PhysRevC.89.065501 PG 26 WC Physics, Nuclear SC Physics GA AK8DG UT WOS:000338656800003 ER PT J AU Fan, Y Iwashita, T Egami, T AF Fan, Yue Iwashita, Takuya Egami, Takeshi TI Evolution of elastic heterogeneity during aging in metallic glasses SO PHYSICAL REVIEW E LA English DT Article ID STRUCTURAL RELAXATION; AMORPHOUS SOLIDS; TRANSITION; LIQUID AB The properties of glasses vary widely depending on the way they are prepared, even though their structures appear similar. We show that the local potential energy landscape (PEL) sensitively reflects the stability differences through simulation of local structural excitation in a model metallic glass. It is observed that the spectrum of local structural excitation develops a pseudogap at low energies as the glass becomes more stable. We also demonstrate that the spatial variation of the atomic level shear modulus, rather than the distribution of the magnitude of the single atom shear modulus, is more closely related to the nature of the PEL and the stabilities of glasses. In particular, local aggregation of atoms with low shear modulus greatly contributes to instability of the system. C1 [Fan, Yue; Egami, Takeshi] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Iwashita, Takuya; Egami, Takeshi] Univ Tennessee, Joint Inst Neutron Sci, Dept Phys & Astron, Knoxville, TN 37996 USA. [Egami, Takeshi] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Fan, Y (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM fany@ornl.gov RI FAN, YUE/H-1737-2011; Iwashita, Takuya/D-2724-2009 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division FX We thank G. M. Stocks and Y. Q. Cheng for thoughtful discussions. Y. F. was supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. T. I. and T. E. were supported by the Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division. NR 35 TC 14 Z9 14 U1 3 U2 48 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUN 25 PY 2014 VL 89 IS 6 AR 062313 DI 10.1103/PhysRevE.89.062313 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AK8GV UT WOS:000338666500008 PM 25019782 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Akimoto, R Al-Bataineh, H Al-Ta'ani, H Alexander, J Andrews, KR Angerami, A Aoki, K Apadula, N Appelt, E Aramaki, Y Armendariz, R Aschenauer, EC Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Bannier, B Barish, KN Bassalleck, B Basye, AT Bathe, S Baublis, V Baumann, C Bazilevsky, A Belikov, S Belmont, R Ben-Benjamin, J Bennett, R Bhom, JH Blau, DS Bok, JS Boyle, K Brooks, ML Broxmeyer, D Buesching, H Bumazhnov, V Bunce, G Butsyk, S Campbell, S Caringi, A Castera, P Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choudhury, RK Christiansen, P Chujo, T Chung, P Chvala, O Cianciolo, V Citron, Z Cole, BA del Valle, ZC Connors, M Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Das, K Datta, A David, G Dayananda, MK Denisov, A Deshpande, A Desmond, EJ Dharmawardane, KV Dietzsch, O Dion, A Donadelli, M Drapier, O Drees, A Drees, KA Durham, JM Durum, A Dutta, D D'Orazio, L Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Fadem, B Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Gal, C Garishvili, I Glenn, A Gong, H Gong, X Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Grim, G Perdekamp, MG Gunji, T Guo, L Gustafsson, HA Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Han, R Hanks, J Harper, C Hashimoto, K Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Hollis, RS Holzmann, W Homma, K Hong, B Horaguchi, T Hori, Y Hornback, D Huang, S Ichihara, T Ichimiya, R Iinuma, H Ikeda, Y Imai, K Inaba, M Iordanova, A Isenhower, D Ishihara, M Issah, M Ivanischev, D Iwanaga, Y Jacak, BV Jia, J Jiang, X Jin, J John, D Johnson, BM Jones, T Joo, KS Jouan, D Jumper, DS Kajihara, F Kamin, J Kaneti, S Kang, BH Kang, JH Kang, JS Kapustinsky, J Karatsu, K Kasai, M Kawall, D Kawashima, M Kazantsev, AV Kempel, T Khanzadeev, A Kijima, KM Kikuchi, J Kim, A Kim, BI Kim, DJ Kim, EJ Kim, YJ Kim, YK Kinney, E Kiss, A Kistenev, E Kleinjan, D Kline, P Kochenda, L Komkov, B Konno, M Koster, J Kotov, D Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, J Lee, KB Lee, KS Lee, SH Lee, SR Leitch, MJ Leite, MAL Li, X Lichtenwalner, P Liebing, P Lim, SH Levy, LAL Liska, T Liu, H Liu, MX Love, B Lynch, D Maguire, CF Makdisi, YI Malik, MD Manion, A Manko, VI Mannel, E Mao, Y Masui, H Matathias, F McCumber, M McGaughey, PL McGlinchey, D McKinney, C Means, N Mendoza, M Meredith, B Miake, Y Mibe, T Mignerey, AC Miki, K Milov, A Mitchell, JT Miyachi, Y Mohanty, AK Moon, HJ Morino, Y Morreale, A Morrison, DP Motschwiller, S Moukhanova, TV Murakami, T Murata, J Nagamiya, S Nagle, JL Naglis, M Nagy, MI Nakagawa, I Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nam, S Newby, J Nguyen, M Nihashi, M Nouicer, R Nyanin, AS Oakley, C O'Brien, E Oda, SX Ogilvie, CA Oka, M Okada, K Onuki, Y Oskarsson, A Ouchida, M Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, BH Park, IH Park, SK Park, WJ Pate, SF Patel, L Pei, H Peng, JC Pereira, H Peressounko, DY Petti, R Pinkenburg, C Pisani, RP Proissl, M Purschke, ML Qu, H Rak, J Ravinovich, I Read, KF Rembeczki, S Reygers, K Riabov, V Riabov, Y Richardson, E Roach, D Roche, G Rolnick, SD Rosati, M Rosen, CA Rosendahl, SSE Ruzicka, P Sahlmueller, B Saito, N Sakaguchi, T Sakashita, K Samsonov, V Sano, S Sarsour, M Sato, T Savastio, M Sawada, S Sedgwick, K Seele, J Seidl, R Seto, R Sharma, D Shein, I Shibata, TA Shigaki, K Shim, HH Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Silvestre, C Sim, KS Singh, BK Singh, CP Singh, V Slunecka, M Sodre, T Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Stankus, PW Stenlund, E Stoll, SP Sugitate, T Sukhanov, A Sun, J Sziklai, J Takagui, EM Takahara, A Taketani, A Tanabe, R Tanaka, Y Taneja, S Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Tennant, E Themann, H Thomas, D Thomas, TL Togawa, M Toia, A Tomasek, L Tomasek, M Torii, H Towell, RS Tserruya, I Tsuchimoto, Y Utsunomiya, K Vale, C Valle, H van Hecke, HW Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Virius, M Vossen, A Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Watanabe, YS Wei, F Wei, R Wessels, J White, SN Winter, D Woody, CL Wright, RM Wysocki, M Yamaguchi, YL Yamaura, K Yang, R Yanovich, A Ying, J Yokkaichi, S Yoo, JS You, Z Young, GR Younus, I Yushmanov, IE Zajc, WA Zelenski, A Zhou, S AF Adare, A. Aidala, C. Ajitanand, N. N. Akiba, Y. Akimoto, R. Al-Bataineh, H. Al-Ta'ani, H. Alexander, J. Andrews, K. R. Angerami, A. Aoki, K. Apadula, N. Appelt, E. Aramaki, Y. Armendariz, R. Aschenauer, E. C. Atomssa, E. T. Averbeck, R. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Baksay, G. Baksay, L. Bannier, B. Barish, K. N. Bassalleck, B. Basye, A. T. Bathe, S. Baublis, V. Baumann, C. Bazilevsky, A. Belikov, S. Belmont, R. Ben-Benjamin, J. Bennett, R. Bhom, J. H. Blau, D. S. Bok, J. S. Boyle, K. Brooks, M. L. Broxmeyer, D. Buesching, H. Bumazhnov, V. Bunce, G. Butsyk, S. Campbell, S. Caringi, A. Castera, P. Chen, C. -H. Chi, C. Y. Chiu, M. Choi, I. J. Choi, J. B. Choudhury, R. K. Christiansen, P. Chujo, T. Chung, P. Chvala, O. Cianciolo, V. Citron, Z. Cole, B. A. del Valle, Z. Conesa Connors, M. Csanad, M. Csorgo, T. Dahms, T. Dairaku, S. Danchev, I. Das, K. Datta, A. David, G. Dayananda, M. K. Denisov, A. Deshpande, A. Desmond, E. J. Dharmawardane, K. V. Dietzsch, O. Dion, A. Donadelli, M. Drapier, O. Drees, A. Drees, K. A. Durham, J. M. Durum, A. Dutta, D. D'Orazio, L. Edwards, S. Efremenko, Y. V. Ellinghaus, F. Engelmore, T. Enokizono, A. En'yo, H. Esumi, S. Fadem, B. Fields, D. E. Finger, M. Finger, M., Jr. Fleuret, F. Fokin, S. L. Fraenkel, Z. Frantz, J. E. Franz, A. Frawley, A. D. Fujiwara, K. Fukao, Y. Fusayasu, T. Gal, C. Garishvili, I. Glenn, A. Gong, H. Gong, X. Gonin, M. Goto, Y. de Cassagnac, R. Granier Grau, N. Greene, S. V. Grim, G. Perdekamp, M. Grosse Gunji, T. Guo, L. Gustafsson, H. -A. Haggerty, J. S. Hahn, K. I. Hamagaki, H. Hamblen, J. Han, R. Hanks, J. Harper, C. Hashimoto, K. Haslum, E. Hayano, R. He, X. Heffner, M. Hemmick, T. K. Hester, T. Hill, J. C. Hohlmann, M. Hollis, R. S. Holzmann, W. Homma, K. Hong, B. Horaguchi, T. Hori, Y. Hornback, D. Huang, S. Ichihara, T. Ichimiya, R. Iinuma, H. Ikeda, Y. Imai, K. Inaba, M. Iordanova, A. Isenhower, D. Ishihara, M. Issah, M. Ivanischev, D. Iwanaga, Y. Jacak, B. V. Jia, J. Jiang, X. Jin, J. John, D. Johnson, B. M. Jones, T. Joo, K. S. Jouan, D. Jumper, D. S. Kajihara, F. Kamin, J. Kaneti, S. Kang, B. H. Kang, J. H. Kang, J. S. Kapustinsky, J. Karatsu, K. Kasai, M. Kawall, D. Kawashima, M. Kazantsev, A. V. Kempel, T. Khanzadeev, A. Kijima, K. M. Kikuchi, J. Kim, A. Kim, B. I. Kim, D. J. Kim, E. -J. Kim, Y. -J. Kim, Y. K. Kinney, E. Kiss, A. Kistenev, E. Kleinjan, D. Kline, P. Kochenda, L. Komkov, B. Konno, M. Koster, J. Kotov, D. Kral, A. Kravitz, A. Kunde, G. J. Kurita, K. Kurosawa, M. Kwon, Y. Kyle, G. S. Lacey, R. Lai, Y. S. Lajoie, J. G. Lebedev, A. Lee, D. M. Lee, J. Lee, K. B. Lee, K. S. Lee, S. H. Lee, S. R. Leitch, M. J. Leite, M. A. L. Li, X. Lichtenwalner, P. Liebing, P. Lim, S. H. Levy, L. A. Linden Liska, T. Liu, H. Liu, M. X. Love, B. Lynch, D. Maguire, C. F. Makdisi, Y. I. Malik, M. D. Manion, A. Manko, V. I. Mannel, E. Mao, Y. Masui, H. Matathias, F. McCumber, M. McGaughey, P. L. McGlinchey, D. McKinney, C. Means, N. Mendoza, M. Meredith, B. Miake, Y. Mibe, T. Mignerey, A. C. Miki, K. Milov, A. Mitchell, J. T. Miyachi, Y. Mohanty, A. K. Moon, H. J. Morino, Y. Morreale, A. Morrison, D. P. Motschwiller, S. Moukhanova, T. V. Murakami, T. Murata, J. Nagamiya, S. Nagle, J. L. Naglis, M. Nagy, M. I. Nakagawa, I. Nakamiya, Y. Nakamura, K. R. Nakamura, T. Nakano, K. Nam, S. Newby, J. Nguyen, M. Nihashi, M. Nouicer, R. Nyanin, A. S. Oakley, C. O'Brien, E. Oda, S. X. Ogilvie, C. A. Oka, M. Okada, K. Onuki, Y. Oskarsson, A. Ouchida, M. Ozawa, K. Pak, R. Pantuev, V. Papavassiliou, V. Park, B. H. Park, I. H. Park, S. K. Park, W. J. Pate, S. F. Patel, L. Pei, H. Peng, J. -C. Pereira, H. Peressounko, D. Yu. Petti, R. Pinkenburg, C. Pisani, R. P. Proissl, M. Purschke, M. L. Qu, H. Rak, J. Ravinovich, I. Read, K. F. Rembeczki, S. Reygers, K. Riabov, V. Riabov, Y. Richardson, E. Roach, D. Roche, G. Rolnick, S. D. Rosati, M. Rosen, C. A. Rosendahl, S. S. E. Ruzicka, P. Sahlmueller, B. Saito, N. Sakaguchi, T. Sakashita, K. Samsonov, V. Sano, S. Sarsour, M. Sato, T. Savastio, M. Sawada, S. Sedgwick, K. Seele, J. Seidl, R. Seto, R. Sharma, D. Shein, I. Shibata, T. -A. Shigaki, K. Shim, H. H. Shimomura, M. Shoji, K. Shukla, P. Sickles, A. Silva, C. L. Silvermyr, D. Silvestre, C. Sim, K. S. Singh, B. K. Singh, C. P. Singh, V. Slunecka, M. Sodre, T. Soltz, R. A. Sondheim, W. E. Sorensen, S. P. Sourikova, I. V. Stankus, P. W. Stenlund, E. Stoll, S. P. Sugitate, T. Sukhanov, A. Sun, J. Sziklai, J. Takagui, E. M. Takahara, A. Taketani, A. Tanabe, R. Tanaka, Y. Taneja, S. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Tennant, E. Themann, H. Thomas, D. Thomas, T. L. Togawa, M. Toia, A. Tomasek, L. Tomasek, M. Torii, H. Towell, R. S. Tserruya, I. Tsuchimoto, Y. Utsunomiya, K. Vale, C. Valle, H. van Hecke, H. W. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Virius, M. Vossen, A. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Watanabe, Y. S. Wei, F. Wei, R. Wessels, J. White, S. N. Winter, D. Woody, C. L. Wright, R. M. Wysocki, M. Yamaguchi, Y. L. Yamaura, K. Yang, R. Yanovich, A. Ying, J. Yokkaichi, S. Yoo, J. S. You, Z. Young, G. R. Younus, I. Yushmanov, I. E. Zajc, W. A. Zelenski, A. Zhou, S. CA PHENIX Collaboration TI Cold-Nuclear-Matter Effects on Heavy-Quark Production at Forward and Backward Rapidity in d + Au Collisions at root s(NN) = GeV SO PHYSICAL REVIEW LETTERS LA English DT Article AB The PHENIX experiment has measured open heavy-flavor production via semileptonic decay over the transverse momentum range 1 < p(T) < 6 GeV/c at forward and backward rapidity (1.4 < vertical bar y vertical bar < 2.0) in d + Au and p + p collisions at root s(NN) = 200 GeV. In central d + Au collisions, relative to the yield in p + p collisions scaled by the number of binary nucleon-nucleon collisions, a suppression is observed at forward rapidity (in the d-going direction) and an enhancement at backward rapidity (in the Au-going direction). Predictions using nuclear-modified-parton-distribution functions, even with additional nuclear-p(T) broadening, cannot simultaneously reproduce the data at both rapidity ranges, which implies that these models are incomplete and suggests the possible importance of final-state interactions in the asymmetric d + Au collision system. These results can be used to probe cold-nuclear-matter effects, which may significantly affect heavy-quark production, in addition to helping constrain the magnitude of charmonia-breakup effects in nuclear matter. C1 [Andrews, K. R.; Basye, A. T.; Isenhower, D.; Jones, T.; Jumper, D. S.; Thomas, D.; Towell, R. S.; Wright, R. M.] Abilene Christian Univ, Abilene, TX 79699 USA. [Grau, N.] Augustana Coll, Dept Phys, Sioux Falls, SD 57197 USA. [Singh, B. K.; Singh, C. P.; Singh, V.; Tarafdar, S.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Choudhury, R. K.; Dutta, D.; Mohanty, A. K.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Bathe, S.] CUNY Bernard M Baruch Coll, New York, NY 10010 USA. [Bai, M.; Drees, K. A.; Makdisi, Y. I.; Zelenski, A.] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Aschenauer, E. C.; Azmoun, B.; Bazilevsky, A.; Belikov, S.; Buesching, H.; Bunce, G.; Chiu, M.; David, G.; Desmond, E. J.; Franz, A.; Haggerty, J. S.; Jia, J.; Johnson, B. M.; Kistenev, E.; Lynch, D.; Milov, A.; Mitchell, J. T.; Morrison, D. P.; Nouicer, R.; O'Brien, E.; Pak, R.; Pinkenburg, C.; Pisani, R. P.; Purschke, M. L.; Sakaguchi, T.; Sickles, A.; Sourikova, I. V.; Stoll, S. P.; Sukhanov, A.; Tannenbaum, M. J.; Vale, C.; White, S. N.; Woody, C. L.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Armendariz, R.; Barish, K. N.; Bathe, S.; Chvala, O.; Hester, T.; Hollis, R. S.; Iordanova, A.; Kleinjan, D.; Mendoza, M.; Morreale, A.; Rolnick, S. D.; Sedgwick, K.; Seto, R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Finger, M.; Finger, M., Jr.; Slunecka, M.] Charles Univ Prague, CR-11636 Prague 1, Czech Republic. [Choi, J. B.; Kim, E. -J.; Lee, S. R.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Li, X.; Zhou, S.] China Inst Atom Energy, Sci & Technol Nucl Data Lab, Beijing 102413, Peoples R China. [Akimoto, R.; Aramaki, Y.; Gunji, T.; Hamagaki, H.; Hayano, R.; Hori, Y.; Kajihara, F.; Morino, Y.; Oda, S. X.; Ozawa, K.; Sano, S.; Takahara, A.; Utsunomiya, K.; Watanabe, Y. S.; Yamaguchi, Y. L.] Univ Tokyo, Grad Sch Sci, Ctr Nucl Study, Bunkyo Ku, Tokyo 1130033, Japan. [Adare, A.; Ellinghaus, F.; Kinney, E.; Levy, L. A. Linden; McCumber, M.; McGlinchey, D.; Nagle, J. L.; Rosen, C. A.; Seele, J.; Wysocki, M.] Univ Colorado, Boulder, CO 80309 USA. [Angerami, A.; Chi, C. Y.; Cole, B. A.; Engelmore, T.; Grau, N.; Hanks, J.; Holzmann, W.; Jin, J.; Kravitz, A.; Lai, Y. S.; Mannel, E.; Matathias, F.; Vazquez-Zambrano, E.; Veicht, A.; Winter, D.; Zajc, W. A.] Columbia Univ, New York, NY 10027 USA. [Angerami, A.; Chi, C. Y.; Cole, B. A.; Engelmore, T.; Grau, N.; Hanks, J.; Holzmann, W.; Jin, J.; Kravitz, A.; Lai, Y. S.; Mannel, E.; Matathias, F.; Vazquez-Zambrano, E.; Veicht, A.; Winter, D.; Zajc, W. A.] Nevis Labs, Irvington, NY 10533 USA. [Kral, A.; Liska, T.; Virius, M.] Czech Tech Univ, Prague 16636 6, Czech Republic. [Pereira, H.; Silvestre, C.] CEA Saclay, F-91191 Gif Sur Yvette, France. [Csanad, M.; Kiss, A.] Eotvos Lorand Univ, ELTE, H-1117 Budapest, Hungary. [Hahn, K. I.; Kim, A.; Lee, J.; Nam, S.; Park, I. H.; Yoo, J. S.] Ewha Womans Univ, Seoul 120750, South Korea. [Baksay, G.; Baksay, L.; Hohlmann, M.; Rembeczki, S.] Florida Inst Technol, Melbourne, FL 32901 USA. [Das, K.; Edwards, S.; Frawley, A. D.; McGlinchey, D.] Florida State Univ, Tallahassee, FL 32306 USA. [Dayananda, M. K.; He, X.; Oakley, C.; Patel, L.; Qu, H.; Sarsour, M.; Ying, J.] Georgia State Univ, Atlanta, GA 30303 USA. [Kang, B. H.; Kang, J. S.; Kim, Y. K.; Park, B. H.] Hanyang Univ, Seoul 133792, South Korea. [Homma, K.; Horaguchi, T.; Iwanaga, Y.; Kijima, K. M.; Nakamiya, Y.; Nihashi, M.; Ouchida, M.; Shigaki, K.; Sugitate, T.; Torii, H.; Tsuchimoto, Y.; Watanabe, D.; Yamaura, K.] Hiroshima Univ, Higashihiroshima 7398526, Japan. [Babintsev, V.; Bumazhnov, V.; Denisov, A.; Durum, A.; Shein, I.; Yanovich, A.] Inst High Energy Phys, State Res Ctr Russian Federat, IHEP Protvino, Protvino 142281, Russia. [Choi, I. J.; Perdekamp, M. Grosse; Kim, Y. -J.; Koster, J.; McKinney, C.; Meredith, B.; Peng, J. -C.; Seidl, R.; Veicht, A.; Vossen, A.; Yang, R.] Univ Illinois, Urbana, IL 61801 USA. [Pantuev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Ruzicka, P.; Tomasek, L.; Tomasek, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague 18221 8, Czech Republic. [Dion, A.; Hill, J. C.; Kempel, T.; Lajoie, J. G.; Lebedev, A.; Ogilvie, C. A.; Pei, H.; Rosati, M.; Silva, C. L.; Wei, F.] Iowa State Univ, Ames, IA 50011 USA. [Imai, K.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Kim, D. J.; Rak, J.] Helsinki Inst Phys, FI-40014 Jyvaskyla, Finland. [Kim, D. J.; Rak, J.] Univ Jyvaskyla, FI-40014 Jyvaskyla, Finland. [Iinuma, H.; Mibe, T.; Nagamiya, S.; Saito, N.; Sawada, S.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Hong, B.; Kim, B. I.; Lee, K. B.; Lee, K. S.; Park, S. K.; Park, W. J.; Shim, H. H.; Sim, K. S.] Korea Univ, Seoul 136701, South Korea. [Blau, D. S.; Fokin, S. L.; Kazantsev, A. V.; Manko, V. I.; Moukhanova, T. V.; Nyanin, A. S.; Peressounko, D. Yu.; Yushmanov, I. E.] Kurchatov Inst, Russian Res Ctr, Moscow 123098, Russia. [Aoki, K.; Dairaku, S.; Imai, K.; Karatsu, K.; Murakami, T.; Nakamura, K. R.; Shoji, K.; Tanida, K.] Kyoto Univ, Kyoto 6068502, Japan. [Atomssa, E. T.; del Valle, Z. Conesa; Drapier, O.; Fleuret, F.; Gonin, M.; de Cassagnac, R. Granier] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Younus, I.] Lahore Univ Management Sci, Dept Phys, Lahore 54792, Pakistan. [Glenn, A.; Heffner, M.; Newby, J.; Soltz, R. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Aidala, C.; Brooks, M. L.; Butsyk, S.; Durham, J. M.; Grim, G.; Guo, L.; Jiang, X.; Kapustinsky, J.; Kunde, G. J.; Lee, D. M.; Leitch, M. J.; Liu, H.; Liu, M. X.; McGaughey, P. L.; Sondheim, W. E.; van Hecke, H. W.; You, Z.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Roche, G.] Univ Clermont Ferrand, CNRS, IN2P3, LPC, F-63177 Aubiere, France. [Christiansen, P.; Gustafsson, H. -A.; Haslum, E.; Oskarsson, A.; Rosendahl, S. S. E.; Stenlund, E.] Lund Univ, Dept Phys, SE-22100 Lund, Sweden. [D'Orazio, L.; Mignerey, A. C.; Richardson, E.] Univ Maryland, College Pk, MD 20742 USA. [Aidala, C.; Datta, A.; Kawall, D.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Aidala, C.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Baumann, C.; Reygers, K.; Sahlmueller, B.; Wessels, J.] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Ben-Benjamin, J.; Broxmeyer, D.; Caringi, A.; Fadem, B.; Harper, C.; Lichtenwalner, P.; Motschwiller, S.; Sodre, T.] Muhlenberg Coll, Allentown, PA 18104 USA. [Joo, K. S.; Moon, H. J.] Myongji Univ, Yongin 449728, Kyonggido, South Korea. [Fusayasu, T.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki 8510193, Japan. [Bassalleck, B.; Fields, D. E.; Malik, M. D.; Thomas, T. L.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Al-Bataineh, H.; Al-Ta'ani, H.; Dharmawardane, K. V.; Kyle, G. S.; Papavassiliou, V.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Frantz, J. E.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Enokizono, A.; Hornback, D.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Young, G. R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris 11, CNRS, IN2P3, IPN Orsay, F-91406 Orsay, France. [Han, R.; Mao, Y.; You, Z.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanischev, D.; Khanzadeev, A.; Kochenda, L.; Komkov, B.; Kotov, D.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Akiba, Y.; Aoki, K.; Aramaki, Y.; Dairaku, S.; En'yo, H.; Fujiwara, K.; Fukao, Y.; Goto, Y.; Hashimoto, K.; Ichihara, T.; Ichimiya, R.; Imai, K.; Ishihara, M.; Karatsu, K.; Kasai, M.; Kawashima, M.; Kurita, K.; Kurosawa, M.; Mao, Y.; Miki, K.; Miyachi, Y.; Murata, J.; Nakagawa, I.; Nakamura, K. R.; Nakamura, T.; Nakano, K.; Onuki, Y.; Ouchida, M.; Sakashita, K.; Shibata, T. -A.; Shoji, K.; Taketani, A.; Tanida, K.; Watanabe, Y.; Yamaguchi, Y. L.; Yokkaichi, S.] RIKEN, Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. [Akiba, Y.; Bathe, S.; Boyle, K.; Bunce, G.; Deshpande, A.; En'yo, H.; Goto, Y.; Ichihara, T.; Kawall, D.; Liebing, P.; Nakagawa, I.; Okada, K.; Seidl, R.; Taketani, A.; Tanida, K.; Togawa, M.; Watanabe, Y.; Yokkaichi, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Hashimoto, K.; Kasai, M.; Kawashima, M.; Kurita, K.; Murata, J.] Rikkyo Univ, Dept Phys, Toshima Ku, Tokyo 1718501, Japan. [Dietzsch, O.; Donadelli, M.; Leite, M. A. L.; Takagui, E. M.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Tanida, K.] Seoul Natl Univ, Seoul, South Korea. [Ajitanand, N. N.; Alexander, J.; Chung, P.; Gong, X.; Jia, J.; Lacey, R.; Taranenko, A.; Wei, R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Averbeck, R.; Bannier, B.; Bennett, R.; Boyle, K.; Campbell, S.; Castera, P.; Chen, C. -H.; Citron, Z.; Connors, M.; Dahms, T.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Frantz, J. E.; Gal, C.; Gong, H.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Kaneti, S.; Kline, P.; Lee, S. H.; Manion, A.; McCumber, M.; Means, N.; Nguyen, M.; Pantuev, V.; Petti, R.; Proissl, M.; Sahlmueller, B.; Savastio, M.; Sun, J.; Taneja, S.; Themann, H.; Toia, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, I.; Hamblen, J.; Hornback, D.; John, D.; Read, K. F.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Miyachi, Y.; Sakashita, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Horaguchi, T.; Ikeda, Y.; Inaba, M.; Konno, M.; Masui, H.; Miake, Y.; Miki, K.; Oka, M.; Sato, T.; Shimomura, M.; Tanabe, R.; Watanabe, K.] Univ Tsukuba, Inst Phys, Tsukuba, Ibaraki 305, Japan. [Appelt, E.; Belmont, R.; Danchev, I.; Greene, S. V.; Huang, S.; Issah, M.; Love, B.; Maguire, C. F.; Roach, D.; Valle, H.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Kikuchi, J.; Sano, S.] Waseda Univ, Adv Res Inst Sci & Engn, Shinjuku Ku, Tokyo 1620044, Japan. [Fraenkel, Z.; Milov, A.; Naglis, M.; Ravinovich, I.; Sharma, D.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csorgo, T.; Nagy, M. I.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci, Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Wigner RCP,RMKI, H-1525 Budapest, Hungary. [Bhom, J. H.; Bok, J. S.; Choi, I. J.; Kang, J. H.; Kwon, Y.; Lim, S. H.] Yonsei Univ, IPAP, Seoul 120749, South Korea. RP Adare, A (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Blau, Dmitry/H-4523-2012; Dahms, Torsten/A-8453-2015; Taketani, Atsushi/E-1803-2017; En'yo, Hideto/B-2440-2015; Hayano, Ryugo/F-7889-2012; HAMAGAKI, HIDEKI/G-4899-2014; Durum, Artur/C-3027-2014; Sorensen, Soren /K-1195-2016; Yokkaichi, Satoshi/C-6215-2017 OI Dahms, Torsten/0000-0003-4274-5476; Taketani, Atsushi/0000-0002-4776-2315; Hayano, Ryugo/0000-0002-1214-7806; Sorensen, Soren /0000-0002-5595-5643; FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Abilene Christian University Research Council; Research Foundation of SUNY; College of Arts and Sciences, Vanderbilt University (U.S.A); Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (P. R. China); Ministry of Education; Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung; Deutscher Akademischer Austausch Dienst; Alexander von Humboldt Stiftung (Germany); Hungarian National Science Fund; Science and Technology (India); Israel Science Foundation (Israel); National Research Foundation and WCU program of the Ministry Education Science and Technology (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science; Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Hungarian Fulbright Foundation for Educational Exchange; US-Israel Binational Science Foundation; OTKA (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Russian Academy of Sciences FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A), Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil), Natural Science Foundation of China (P. R. China), Ministry of Education, Youth and Sports (Czech Republic), Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France), Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany), Hungarian National Science Fund, OTKA (Hungary), Department of Atomic Energy and Department of Science and Technology (India), Israel Science Foundation (Israel), National Research Foundation and WCU program of the Ministry Education Science and Technology (Korea), Physics Department, Lahore University of Management Sciences (Pakistan), Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia), VR and Wallenberg Foundation (Sweden), the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, the US-Hungarian Fulbright Foundation for Educational Exchange, and the US-Israel Binational Science Foundation. NR 39 TC 23 Z9 23 U1 6 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 25 PY 2014 VL 112 IS 25 AR 252301 DI 10.1103/PhysRevLett.112.252301 PG 8 WC Physics, Multidisciplinary SC Physics GA AK7YQ UT WOS:000338644200007 ER PT J AU Noji, S Zegers, RGT Austin, SM Baugher, T Bazin, D Brown, BA Campbell, CM Cole, AL Doster, HJ Gade, A Guess, CJ Gupta, S Hitt, GW Langer, C Lipschutz, S Lunderberg, E Meharchand, R Meisel, Z Perdikakis, G Pereira, J Recchia, F Schatz, H Scott, M Stroberg, SR Sullivan, C Valdez, L Walz, C Weisshaar, D Williams, SJ Wimmer, K AF Noji, S. Zegers, R. G. T. Austin, Sam M. Baugher, T. Bazin, D. Brown, B. A. Campbell, C. M. Cole, A. L. Doster, H. J. Gade, A. Guess, C. J. Gupta, S. Hitt, G. W. Langer, C. Lipschutz, S. Lunderberg, E. Meharchand, R. Meisel, Z. Perdikakis, G. Pereira, J. Recchia, F. Schatz, H. Scott, M. Stroberg, S. R. Sullivan, C. Valdez, L. Walz, C. Weisshaar, D. Williams, S. J. Wimmer, K. TI beta(+) Gamow-Teller Transition Strengths from Ti-46 and Stellar Electron-Capture Rates SO PHYSICAL REVIEW LETTERS LA English DT Article ID WEAK-INTERACTION RATES; INTERMEDIATE-MASS NUCLEI; SHELL-MODEL DESCRIPTION; PF-SHELL; SPECTROMETER; ENERGIES; BEAM AB The Gamow-Teller strength in the beta(+) direction to Sc-46 was extracted via the Ti-46(t, He-3 + gamma) reaction at 115 MeV/u. The gamma-ray coincidences served to precisely measure the very weak Gamow-Teller transition to a final state at 991 keV. Although this transition is weak, it is crucial for accurately estimating electron-capture rates in astrophysical scenarios with relatively low stellar densities and temperatures, such as presupernova stellar evolution. Shell-model calculations with different effective interactions in the pf shell-model space do not reproduce the experimental Gamow-Teller strengths, which is likely due to sd-shell admixtures. Calculations in the quasiparticle random phase approximation that are often used in astrophysical simulations also fail to reproduce the experimental Gamow-Teller strength distribution, leading to strongly overestimated electron-capture rates. Because reliable theoretical predictions of Gamow-Teller strengths are important for providing astrophysical electron-capture reaction rates for a broad set of nuclei in the lower pf shell, we conclude that further theoretical improvements are required to match astrophysical needs. C1 [Noji, S.; Zegers, R. G. T.; Austin, Sam M.; Baugher, T.; Bazin, D.; Brown, B. A.; Doster, H. J.; Gade, A.; Langer, C.; Lipschutz, S.; Lunderberg, E.; Meisel, Z.; Perdikakis, G.; Pereira, J.; Recchia, F.; Schatz, H.; Scott, M.; Stroberg, S. R.; Sullivan, C.; Valdez, L.; Walz, C.; Weisshaar, D.; Williams, S. J.; Wimmer, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Noji, S.; Zegers, R. G. T.; Austin, Sam M.; Langer, C.; Meisel, Z.; Schatz, H.; Sullivan, C.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Zegers, R. G. T.; Austin, Sam M.; Baugher, T.; Brown, B. A.; Doster, H. J.; Lipschutz, S.; Lunderberg, E.; Meisel, Z.; Schatz, H.; Scott, M.; Stroberg, S. R.; Sullivan, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Campbell, C. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Cole, A. L.] Kalamazoo Coll, Dept Phys, Kalamazoo, MI 49006 USA. [Guess, C. J.] Univ Massachusetts Lowell, Dept Phys & Appl Phys, Lowell, MA 01854 USA. [Guess, C. J.] Rowan Univ, Dept Phys & Astron, Glassboro, NJ 08028 USA. [Gupta, S.] Indian Inst Technol Ropar, Rupnagar 140001, Punjab, India. [Hitt, G. W.] Khalifa Univ Sci Technol & Res, Dept Appl Math & Sci, Abu Dhabi, U Arab Emirates. [Meharchand, R.] Los Alamos Natl Lab, Neutron & Nucl Sci Grp, Los Alamos, NM 87545 USA. [Perdikakis, G.; Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. RP Noji, S (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. EM noji@nscl.msu.edu RI Gade, Alexandra/A-6850-2008; Zegers, Remco/A-6847-2008; Scott, Michael/A-1974-2015; Hitt, George/F-7481-2011; Perdikakis, Georgios/K-4525-2014; Langer, Christoph/L-3422-2016 OI Gade, Alexandra/0000-0001-8825-0976; Scott, Michael/0000-0002-3697-7089; Hitt, George/0000-0003-3161-3283; Perdikakis, Georgios/0000-0002-8539-8737; FU US NSF [PHY-08-22648, PHY-10-68217]; US DOE Office of Science; NSF [PHY-11-02511]; DOE [DE-AC02-05CH11231] FX We thank all the staff at NSCL for their support. This work was supported by the US NSF grant PHY-08-22648 (Joint Institute for Nuclear Astrophysics) and PHY-10-68217. GRETINA was funded by the US DOE Office of Science. Operation of the array at NSCL is supported by NSF under Cooperative Agreement PHY-11-02511 (NSCL) and DOE under grant DE-AC02-05CH11231 (LBNL). NR 48 TC 6 Z9 6 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 25 PY 2014 VL 112 IS 25 AR 252501 DI 10.1103/PhysRevLett.112.252501 PG 6 WC Physics, Multidisciplinary SC Physics GA AK7YQ UT WOS:000338644200008 PM 25014806 ER PT J AU Li, MD Dai, ZY Cui, WP Wang, Z Katmis, F Wang, JY Le, PS Wu, LJ Zhu, YM AF Li, Mingda Dai, Zuyang Cui, Wenping Wang, Zhe Katmis, Ferhat Wang, Jiayue Le, Peisi Wu, Lijun Zhu, Yimei TI Tunable THz surface plasmon polariton based on a topological insulator/layered superconductor hybrid structure SO PHYSICAL REVIEW B LA English DT Article ID GRAPHENE PLASMONICS; METAMATERIALS; DEVICES AB We theoretically investigate the surface plasmon polariton (SPP) at the interface between a three-dimensional strong topological insulator (TI) and a layered superconductor/magnetic insulator structure, within the random phase approximation. The tunability of the SPP through electronic doping can be enhanced when the magnetic permeability of the layered structure becomes higher. When the interface is gapped by superconductivity or perpendicular magnetism, the SPP dispersion is further distorted, accompanied by a shift of group velocity and penetration depth. Such a shift of the SPP reaches a maximum when the magnitude of the Fermi level approaches the gap value, and may lead to observable effects. The tunable SPP at the interface between layered-superconductor and magnetic materials in proximity to the TI surface may provide new insight in the detection of Majorana fermions. C1 [Li, Mingda; Wang, Zhe; Le, Peisi] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Dai, Zuyang] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Cui, Wenping] Univ Cologne, Inst Theoret Phys, D-50937 Cologne, Germany. [Katmis, Ferhat] MIT, Dept Phys, Cambridge, MA 02139 USA. [Wang, Jiayue] Tsinghua Univ, Dept Engn Phys, Beijing 10084, Peoples R China. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Dept Condensed Matter Phys, Upton, NY 11973 USA. RP Li, MD (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM mingda@mit.edu OI Wang, Zhe/0000-0003-4103-0751 NR 45 TC 2 Z9 2 U1 12 U2 69 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 25 PY 2014 VL 89 IS 23 AR 235432 DI 10.1103/PhysRevB.89.235432 PG 6 WC Physics, Condensed Matter SC Physics GA AK8BV UT WOS:000338653100002 ER PT J AU Ning, FL Fu, M Torchetti, DA Imai, T Sefat, AS Cheng, P Shen, B Wen, HH AF Ning, F. L. Fu, M. Torchetti, D. A. Imai, T. Sefat, A. S. Cheng, P. Shen, B. Wen, H. -H. TI Critical behavior of the spin density wave transition in underdoped Ba(Fe1-xCox)(2)As-2 (x <= 0.05): As-75 NMR investigation SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY; RELAXATION AB We investigate the nature of the SDW (spin density wave) transition in the underdoped regime of an iron-based high-T-c superconductor Ba(Fe1-xCox)(2)As-2 by As-75 NMR, with primary focus on a composition with x = 0.02 (T-SDW = 99 K). We demonstrate that critical slowing down toward the three-dimensional SDW transition sets in at the tetragonal to orthorhombic structural phase transition T-s = 105 K, suggesting strong interplay between structural distortion and spin correlations. In the critical regime between T-s and T-SDW, the dynamical structure factor of electron spins S(q,omega(n)) measured with the longitudinal NMR relaxation rate 1/T-1 exhibits a divergent behavior obeying a power law 1/T-1 proportional to Sigma S-q(q,omega(n)) similar to (T/T-SDW - 1)(-delta) with the critical exponent delta similar to 0.33. C1 [Ning, F. L.] Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. [Fu, M.; Torchetti, D. A.; Imai, T.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Imai, T.; Wen, H. -H.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Sefat, A. S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Cheng, P.; Shen, B.; Wen, H. -H.] Chinese Acad Sci, Inst Phys, Natl Lab Superconduct, Beijing 100190, Peoples R China. [Cheng, P.; Shen, B.; Wen, H. -H.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Wen, H. -H.] Nanjing Univ, Dept Phys, Ctr Superconducting Phys & Mat, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. RP Ning, FL (reprint author), Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. EM ningfl@zju.edu.cn RI Shen, Bing/G-6514-2016; Sefat, Athena/R-5457-2016 OI Sefat, Athena/0000-0002-5596-3504 FU National Basic Research Program of China [2014CB921203, 2011CBA00103]; NSF of China [11274268]; NSERC; CIFAR; Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; NSFC; Ministry of Science and Technology of China; Chinese Academy of Sciences FX The work at Zhejiang was supported by National Basic Research Program of China (Grants No. 2014CB921203 and No. 2011CBA00103), NSF of China (Grant No. 11274268). The work at McMaster was supported by NSERC and CIFAR. The work at Oak Ridge National Laboratory was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The work at Beijing and Nanjing was supported by NSFC, the Ministry of Science and Technology of China, and the Chinese Academy of Sciences. NR 45 TC 6 Z9 6 U1 1 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 25 PY 2014 VL 89 IS 21 AR 214511 DI 10.1103/PhysRevB.89.214511 PG 8 WC Physics, Condensed Matter SC Physics GA AK8BE UT WOS:000338651300002 ER PT J AU Taufour, V Foroozani, N Tanatar, MA Lim, J Kaluarachchi, U Kim, SK Liu, Y Lograsso, TA Kogan, VG Prozorov, R Bud'ko, SL Schilling, JS Canfield, PC AF Taufour, Valentin Foroozani, Neda Tanatar, Makariy A. Lim, Jinhyuk Kaluarachchi, Udhara Kim, Stella K. Liu, Yong Lograsso, Thomas A. Kogan, Vladimir G. Prozorov, Ruslan Bud'ko, Sergey L. Schilling, James S. Canfield, Paul C. TI Upper critical field of KFe2As2 under pressure: A test for the change in the superconducting gap structure SO PHYSICAL REVIEW B LA English DT Article ID HYDROSTATIC LIMITS; TEMPERATURE; DEPENDENCE; LIQUIDS; KBAR; LINE; GPA AB We report measurements of electrical resistivity under pressure to 5.8 GPa, magnetization to 6.7 GPa, and ac susceptibility to 7.1 GPa in KFe2As2. The previously reported change of slope in the pressure dependence of the superconducting transition temperature Tc (p) at a pressure p*1.8 GPa is confirmed, and Tc (p) is found to be nearly constant above p* up to 7.1 GPa. The T - p phase diagram is very sensitive to the pressure conditions as a consequence of the anisotropic uniaxial pressure dependence of Tc. Across p*, a change in the behavior of the upper critical field is revealed through a scaling analysis of the slope of Hc2 with the effective mass as determined from the A coefficient of the T 2 term of the temperature-dependent resistivity. We show that this scaling provides a quantitative test for the changes of the superconducting gap structure and suggests the development of a kz modulation of the superconducting gap above p* as a most likely explanation. C1 [Taufour, Valentin; Tanatar, Makariy A.; Kaluarachchi, Udhara; Kim, Stella K.; Prozorov, Ruslan; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Taufour, Valentin; Tanatar, Makariy A.; Kim, Stella K.; Liu, Yong; Lograsso, Thomas A.; Kogan, Vladimir G.; Prozorov, Ruslan; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Ames Lab, US Dept Energy, Ames, IA 50011 USA. [Foroozani, Neda; Lim, Jinhyuk; Schilling, James S.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. RP Taufour, V (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM taufour@ameslab.gov FU AFOSR-MURI [FA9550-09-1-0603]; Ames Laboratory, US DOE [DE-AC02-07CH11358]; National Science Foundation (NSF) [DMR1104742]; Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE [DE-FC52-08NA28554] FX We would like to thank A. Jesche, L. Howald, D. Finnemore, T. Kong, and F. F. Tafti for useful discussions. This work was carried out at the Iowa State University and supported by AFOSR-MURI Grant No. FA9550-09-1-0603. Part of this work was performed at the Ames Laboratory, US DOE, under Contract No. DE-AC02-07CH11358. The ac susceptibility measurements in a diamond anvil cell were carried out at Washington University in St. Louis and supported by the National Science Foundation (NSF) through Grant No. DMR1104742 and by the Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant No. DE-FC52-08NA28554. NR 67 TC 14 Z9 14 U1 5 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 25 PY 2014 VL 89 IS 22 AR 220509 DI 10.1103/PhysRevB.89.220509 PG 5 WC Physics, Condensed Matter SC Physics GA AK8BL UT WOS:000338652100002 ER PT J AU Zhang, Q Ramazanoglu, M Chi, SX Liu, Y Lograsso, TA Vaknin, D AF Zhang, Qiang Ramazanoglu, Mehmet Chi, Songxue Liu, Yong Lograsso, Thomas A. Vaknin, David TI Magnetic excitations and anomalous spin-wave broadening in multiferroic FeV2O4 SO PHYSICAL REVIEW B LA English DT Article ID OXIDES AB We report on the different roles of two orbital-active Fe2+ at theAsite and V3+ at the B site in themagnetic excitations and on the anomalous spin-wave broadening in FeV2O4. FeV2O4 exhibits three structural transitions and successive paramagnetic (PM)-collinear ferrimagnetic (CFI)-noncollinear ferrimagnetic (NCFI)/ferroelectric transitions. The high-temperature tetragonal/PM-orthorhombic/CFI transition is accompanied by the appearance of a large energy gap in the magnetic excitations due to strong spin-orbit-coupling-induced anisotropy at the Fe2+ site. While there is no measurable increase in the energy gap from the orbital ordering of V3+ at the orthorhombic/CFI-tetragonal/NCFI transition, anomalous spin-wave broadening is observed in the orthorhombic/CFI state due to V3+ spin fluctuations at the B site. The spin-wave broadening is also observed at the zone boundary without softening in the NCFI/ferroelectric phase, which is discussed in terms of magnon-phonon coupling. Our study also indicates that the Fe2+ spins without the frustration at the A site may not play an important role in inducing ferroelectricity in the tetragonal/NCFI phase of FeV2O4. C1 [Zhang, Qiang; Ramazanoglu, Mehmet; Liu, Yong; Lograsso, Thomas A.; Vaknin, David] Ames Lab, Ames, IA 50011 USA. [Zhang, Qiang; Ramazanoglu, Mehmet; Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chi, Songxue] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Lograsso, Thomas A.] Iowa State Univ, Div Engn & Mat Sci, Ames, IA 50011 USA. RP Zhang, Q (reprint author), Ames Lab, Ames, IA 50011 USA. EM qzhangemail@gmail.com; vaknin@ameslab.gov RI Chi, Songxue/A-6713-2013; Vaknin, David/B-3302-2009; OI Chi, Songxue/0000-0002-3851-9153; Vaknin, David/0000-0002-0899-9248; Zhang, Qiang/0000-0003-0389-7039 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research at Ames Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. Use of the high flux isotope reactor at the Oak Ridge National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 31 TC 5 Z9 5 U1 2 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 25 PY 2014 VL 89 IS 22 AR 224416 DI 10.1103/PhysRevB.89.224416 PG 5 WC Physics, Condensed Matter SC Physics GA AK8BL UT WOS:000338652100004 ER PT J AU Berlin, A Hooper, D McDermott, SD AF Berlin, Asher Hooper, Dan McDermott, Samuel D. TI Simplified dark matter models for the Galactic Center gamma-ray excess SO PHYSICAL REVIEW D LA English DT Article ID PROTON-PROTON COLLISIONS; EFFECTIVE-FIELD THEORY; EXCLUSION LIMITS; NAIAD EXPERIMENT; SEARCH; TEV; DAMA/LIBRA; ABUNDANCES; ENERGIES; BOSONS AB Motivated by the gamma-ray excess observed from the region surrounding the Galactic Center, we explore particle dark matter models that could potentially account for the spectrum and normalization of this signal. Taking a model-independent approach, we consider an exhaustive list of tree-level diagrams for dark matter annihilation, and determine which could account for the observed gamma-ray emission while simultaneously predicting a thermal relic abundance equal to the measured cosmological dark matter density. We identify a wide variety of models that can meet these criteria without conflicting with existing constraints from direct detection experiments or the Large Hadron Collider (LHC). The prospects for detection in near future dark matter experiments and/or the upcoming 14 TeV LHC appear quite promising. C1 [Berlin, Asher] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Hooper, Dan; McDermott, Samuel D.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [McDermott, Samuel D.] Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. RP Berlin, A (reprint author), Univ Chicago, Dept Phys, Chicago, IL 60637 USA. NR 96 TC 91 Z9 91 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 25 PY 2014 VL 89 IS 11 AR 115022 DI 10.1103/PhysRevD.89.115022 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK8FQ UT WOS:000338663100004 ER PT J AU Lees, JP Poireau, V Tisserand, V Tico, JG Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lynch, G Koch, H Schroeder, T Asgeirsson, DJ Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Bondioli, M Kirkby, D Lankford, AJ Mandelkern, M Atmacan, H Gary, JW Liu, F Long, O Vitug, GM Campagnari, C Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Kroseberg, J Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Rakitin, AY Andreassen, R Huard, Z Meadows, BT Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schubert, KR Schwierz, R Bernard, D Verderi, M Clark, PJ Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Munerato, M Negrini, M Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Lee, CL Morii, M Edwards, AJ Adametz, A Uwer, U Lacker, HM Lueck, T Dauncey, PD Behera, PK Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Guo, ZJ Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Schune, MH Stocchi, A Wormser, G Lange, DJ Wright, DM Chavez, CA Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Sigamani, M Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Barlow, RJ Jackson, G Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Dallapiccola, C Cowan, R Dujmic, D Sciolla, G Cheaib, R Lindemann, D Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Stracka, S Cremaldi, L Godang, R Kroeger, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P de Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Wang, WF Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Gagliardi, N Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Hamon, O Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Telnov, AV Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Mazzoni, MA Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Schroder, H Vo, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Ysche, C Aston, D Bard, DJ Bartoldus, R Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Sevilla, MF Fulsom, BG Gabareen, AM Graham, MT Grenier, P Hast, C Innes, WR Kelsey, MH Kim, P Kocian, ML Leith, DWGS Lewis, P Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Young, CC Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Lund, P Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Puccio, EMT Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Tico, J. Garra Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lynch, G. Koch, H. Schroeder, T. Asgeirsson, D. J. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Bondioli, M. Kirkby, D. Lankford, A. J. Mandelkern, M. Atmacan, H. Gary, J. W. Liu, F. Long, O. Vitug, G. M. Campagnari, C. Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Kroseberg, J. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Rakitin, A. Y. Andreassen, R. Huard, Z. Meadows, B. T. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Clark, P. J. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Munerato, M. Negrini, M. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Lee, C. L. Morii, M. Edwards, A. J. Adametz, A. Uwer, U. Lacker, H. M. Lueck, T. Dauncey, P. D. Behera, P. K. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Guo, Z. J. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Schune, M. H. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Chavez, C. A. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Sigamani, M. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Barlow, R. J. Jackson, G. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Dallapiccola, C. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Lindemann, D. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Stracka, S. Cremaldi, L. Godang, R. Kroeger, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. de Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Wang, W. F. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Gagliardi, N. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Hamon, O. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Telnov, A. V. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Mazzoni, M. A. Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Schroeder, H. Vo, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Ysche, Ch. Aston, D. Bard, D. J. Bartoldus, R. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Sevilla, M. Franco Fulsom, B. G. Gabareen, A. M. Graham, M. T. Grenier, P. Hast, C. Innes, W. R. Kelsey, M. H. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Young, C. C. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Lund, P. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Puccio, E. M. T. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Study of the reaction e(+)e(-) -> psi(2S)pi(+)pi(-) via initial-state radiation at BABAR SO PHYSICAL REVIEW D LA English DT Article ID DETECTOR AB We study the process e(+)e(-) -> psi(2S)pi(+)pi(-) with initial-state-radiation events produced at the PEP-II asymmetric-energy collider. The data were recorded with the BABAR detector at center-of-mass energies at and near the (nS) (n = 2, 3, 4) resonances and correspond to an integrated luminosity of 520 fb(-1). We investigate the psi(2S)pi(+)pi(-) mass distribution from 3.95 to 5.95 GeV/c(2), and measure the center-of-mass energy dependence of the associated e(+)e(-) -> psi(2S)pi(+)pi(-) cross section. The mass distribution exhibits evidence of two resonant structures. A fit to the psi(2S)pi(+)pi(-) mass distribution corresponding to the decay mode psi(2S) -> J/psi pi(+)pi(-) yields a mass value of 4340 +/- 16 (stat) +/- 9 (syst) MeV/c(2) and a width of 94 +/- 32 (stat) +/- 13 (syst) MeV for the first resonance, and for the second a mass value of 4669 +/- 21 (stat) +/- 3 (syst) MeV/c(2) and a width of 104 +/- 48 (stat) +/- 10 (syst) MeV. In addition, we show the pi(+)pi(-) mass distributions for these resonant regions. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, Lab Annecy le Vieux Phys Particules LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. [Tico, J. Garra; Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys 1, D-44780 Bochum, Germany. [Asgeirsson, D. J.; Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.; Yushkov, A. N.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Bondioli, M.; Kirkby, D.; Lankford, A. J.; Mandelkern, M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Atmacan, H.; Gary, J. W.; Liu, F.; Long, O.; Vitug, G. M.] Univ Calif Riverside, Riverside, CA 92521 USA. [Campagnari, C.; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Kroseberg, J.; Lockman, W. S.; Martinez, A. J.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Inst Particle Phys, Santa Cruz, CA 95064 USA. [Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Ongmongkolkul, P.; Porter, F. C.; Rakitin, A. Y.] CALTECH, Pasadena, CA 91125 USA. [Andreassen, R.; Huard, Z.; Meadows, B. T.; Sokoloff, M. D.; Sun, L.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Bloom, P. C.; Ford, W. T.; Gaz, A.; Nauenberg, U.; Smith, J. G.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Ayad, R.; Toki, W. H.] Colorado State Univ, Ft Collins, CO 80523 USA. [Spaan, B.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dortmund, Germany. [Bernard, D.; Verderi, M.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Clark, P. J.; Playfer, S.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Bettoni, D.; Bozzi, C.; Calabrese, R.; Cibinetto, G.; Fioravanti, E.; Garzia, I.; Luppi, E.; Munerato, M.; Negrini, M.; Piemontese, L.; Santoro, V.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Calabrese, R.; Cibinetto, G.; Fioravanti, E.; Garzia, I.; Luppi, E.; Munerato, M.; Negrini, M.] Univ Ferrara, Dipartimento Fis, I-44100 Ferrara, Italy. [Baldini-Ferroli, R.; Calcaterra, A.; de Sangro, R.; Finocchiaro, G.; Patteri, P.; Peruzzi, I. M.; Piccolo, M.; Rama, M.; Zallo, A.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Contri, R.; Guido, E.; Lo Vetere, M.; Monge, M. R.; Passaggio, S.; Patrignani, C.; Robutti, E.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Contri, R.; Guido, E.; Lo Vetere, M.; Monge, M. R.; Patrignani, C.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Bhuyan, B.; Prasad, V.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Lee, C. L.; Morii, M.] Harvard Univ, Cambridge, MA 02138 USA. [Edwards, A. J.] Harvey Mudd Coll, Claremont, CA 91711 USA. [Adametz, A.; Uwer, U.] Heidelberg Univ, Inst Phys, D-69120 Heidelberg, Germany. [Lacker, H. M.; Lueck, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Dauncey, P. D.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Behera, P. K.; Mallik, U.] Univ Iowa, Iowa City, IA 52242 USA. [Chen, C.; Cochran, J.; Meyer, W. T.; Prell, S.; Rubin, A. E.] Iowa State Univ, Ames, IA 50011 USA. [Gritsan, A. V.; Guo, Z. J.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Arnaud, N.; Davier, M.; Derkach, D.; Grosdidier, G.; Le Diberder, F.; Lutz, A. M.; Malaescu, B.; Roudeau, P.; Schune, M. H.; Stocchi, A.; Wormser, G.] CNRS, IN2P3, Lab Accelerateur Lineaire, F-91898 Orsay, France. [Arnaud, N.; Davier, M.; Derkach, D.; Grosdidier, G.; Le Diberder, F.; Lutz, A. M.; Malaescu, B.; Roudeau, P.; Schune, M. H.; Stocchi, A.; Wormser, G.] Univ Paris 11, Ctr Sci Orsay, F-91898 Orsay, France. [Lange, D. J.; Wright, D. 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[Cheaib, R.; Lindemann, D.; Patel, P. M.; Robertson, S. H.] McGill Univ, Montreal, PQ H3A 2T8, Canada. [Biassoni, P.; Neri, N.; Palombo, F.; Stracka, S.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Biassoni, P.; Palombo, F.; Stracka, S.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Cremaldi, L.; Godang, R.; Kroeger, R.; Sonnek, P.; Summers, D. J.] Univ Mississippi, University, MS 38677 USA. [Nguyen, X.; Simard, M.; Taras, P.] Univ Montreal, Montreal, PQ H3C 3J7, Canada. [de Nardo, G.; Monorchio, D.; Onorato, G.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [de Nardo, G.; Monorchio, D.; Onorato, G.; Sciacca, C.] Univ Naples Federico II, Dipartimento Sci Fisiche, I-80126 Naples, Italy. [Martinelli, M.; Raven, G.] Natl Inst Nucl Phys & High Energy Phys, NIKHEF, NL-1009 DB Amsterdam, Netherlands. [Jessop, C. P.; LoSecco, J. M.; Wang, W. F.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Brau, J.; Frey, R.; Sinev, N. B.; Strom, D.; Torrence, E.] Univ Oregon, Eugene, OR 97403 USA. [Feltresi, E.; Gagliardi, N.; Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Feltresi, E.; Gagliardi, N.; Margoni, M.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Hamon, O.; Leruste, Ph.; Marchiori, G.; Ocariz, J.; Sitt, S.] Univ Paris 07, Univ Paris 06, CNRS, IN2P3,Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Manoni, E.; Pacetti, S.; Rossi, A.; Bianchi, F.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.; Telnov, A. V.] Princeton Univ, Princeton, NJ 08544 USA. [Anulli, F.; Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Mazzoni, M. A.; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Schroeder, H.; Vo, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Ysche, Ch.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Bartoldus, R.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Sevilla, M. Franco; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Grenier, P.; Hast, C.; Innes, W. R.; Kelsey, M. H.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Young, C. C.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Lund, P.; Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.; Puccio, E. M. T.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Peruzzi, I. M.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, Lab Annecy le Vieux Phys Particules LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. RI Calcaterra, Alessandro/P-5260-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Stracka, Simone/M-3931-2015; Di Lodovico, Francesca/L-9109-2016; Frey, Raymond/E-2830-2016; Patrignani, Claudia/C-5223-2009; Lo Vetere, Maurizio/J-5049-2012; Oyanguren, Arantza/K-6454-2014; Lusiani, Alberto/N-2976-2015; Monge, Maria Roberta/G-9127-2012; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Negrini, Matteo/C-8906-2014 OI Calcaterra, Alessandro/0000-0003-2670-4826; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Stracka, Simone/0000-0003-0013-4714; Di Lodovico, Francesca/0000-0003-3952-2175; Frey, Raymond/0000-0003-0341-2636; Patrignani, Claudia/0000-0002-5882-1747; Lo Vetere, Maurizio/0000-0002-6520-4480; Oyanguren, Arantza/0000-0002-8240-7300; Lusiani, Alberto/0000-0002-6876-3288; Monge, Maria Roberta/0000-0003-1633-3195; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Negrini, Matteo/0000-0003-0101-6963 FU SLAC; DOE; NSF (USA); NSERC (Canada); CEA; CNRS-IN2P3 (France); BMBF; DFG (Germany); INFN (Italy); FOM (The Netherlands); NFR (Norway); MES (Russia); MICIIN (Spain); STFC (United Kingdom); Marie Curie EIF (European Union); A.P. Sloan Foundation (U.S.A) FX We are grateful for the excellent luminosity and machine conditions provided by our PEP-II2 colleagues, and for the substantial dedicated effort from the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and kind hospitality. This work is supported by DOE and NSF (USA), NSERC (Canada), CEA and CNRS-IN2P3 (France), BMBF and DFG (Germany), INFN (Italy), FOM (The Netherlands), NFR (Norway), MES (Russia), MICIIN (Spain), and STFC (United Kingdom). Individuals have received support from the Marie Curie EIF (European Union) and the A.P. Sloan Foundation (U.S.A). NR 14 TC 22 Z9 22 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 25 PY 2014 VL 89 IS 11 AR 111103 DI 10.1103/PhysRevD.89.111103 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK8FQ UT WOS:000338663100001 ER PT J AU Li, DN Liao, JF Huang, M AF Li, Danning Liao, Jinfeng Huang, Mei TI Enhancement of jet quenching around phase transition: Result from the dynamical holographic model SO PHYSICAL REVIEW D LA English DT Article ID QUARK-GLUON PLASMA; PARTON ENERGY-LOSS; PB-PB COLLISIONS; ELLIPTIC FLOW; TRANSVERSE-MOMENTUM; ROOT-S(NN)=2.76 TEV; GAUGE-THEORY; QCD; SUPPRESSION; LHC AB The phase transition and jet quenching parameter (q) over cap are investigated in the framework of the dynamical holographic QCD model. We find that both the trace anomaly and the ratio of the jet quenching parameter over cubic temperature (q) over cap /T-3 show a peak around the critical temperature T-c, and the ratio of the jet quenching parameter over entropy density (q) over cap / s sharply rises at T-c. This indicates that the jet quenching parameter can characterize the phase transition. The effect of the jet quenching parameter enhancement around the phase transition on the nuclear modification factor R-AA and elliptic flow upsilon(2) are also analyzed, and we find that the temperature-dependent jet quenching parameter from the dynamical holographic QCD model can considerably improve the description of jet quenching azimuthal anisotropy as compared with the conformal case. C1 [Li, Danning; Huang, Mei] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Liao, Jinfeng] Indiana Univ, Ctr Explorat Energy & Matter, Dept Phys, Bloomington, IN 47408 USA. [Liao, Jinfeng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Huang, Mei] Chinese Acad Sci, Theoret Phys Ctr Sci Facil, Beijing 100049, Peoples R China. RP Li, DN (reprint author), Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. FU NSFC [11275213, CRC 110]; DFG; CAS [KJCX2-EW-N01]; K. C. Wong Education Foundation; Youth Innovation Promotion Association of CAS; National Science Foundation [PHY1352368]; RIKEN BNL Research Center FX This work is supported by the NSFC under Grant No. 11275213, DFG and NSFC (CRC 110), CAS key Project No. KJCX2-EW-N01, K. C. Wong Education Foundation, and the Youth Innovation Promotion Association of CAS. The research of J. L. is supported by the National Science Foundation under Grant No. PHY1352368. J. L. is grateful to the RIKEN BNL Research Center for partial support. NR 83 TC 16 Z9 16 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 25 PY 2014 VL 89 IS 12 AR 126006 DI 10.1103/PhysRevD.89.126006 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK8FY UT WOS:000338664000017 ER PT J AU Liu, HJ Dai, S Jiang, DE AF Liu, Hongjun Dai, Sheng Jiang, De-en TI Molecular Dynamics Simulation of Anion Effect on Solubility, Diffusivity, and Permeability of Carbon Dioxide in Ionic Liquids SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MONTE-CARLO SIMULATIONS; 1-N-BUTYL-3-METHYLIMIDAZOLIUM HEXAFLUOROPHOSPHATE; TETRACYANOBORATE ANION; CO2/N-2 SEPARATION; GAS SOLUBILITY; FORCE-FIELDS; CO2 CAPTURE; MEMBRANES; WATER; MIXTURES AB The solubility, diffusivity, and permeability of CO2 in three ionic liquids with a common cation were investigated by molecular dynamics simulations in order to understand the role of the anion in dictating permeability. The three ionic liquids are 1-ethyl-3-methyl imidazolium tetracyanoborate ([emim][B(CN)(4)]), 1-ethyl-3-methyl imidazolium bis-(trifluoromethylsulfonyl)imide ([emim][Tf2N]), and 1-ethyl-3-methyl imidazolium tetrafluoroborate ([emim][BF4]). The simulated solubility agrees satisfactorily with experiment with a trend of [emim][B(CN)(4)] > [emim][Tf2N] > [emim][BF4]. The higher solubility of CO2 in [emim][B(CN)(4)] appears to be due to weaker cation anion interaction, higher fraction of larger cavity, larger free volume, and more favorable interaction with CO2. CO2 diffusivity in ILs follows the same trend as solubility. On the basis of the solvation-diffusion mechanism, gas permeability was estimated and compared with experiment. The present work confirms the superiority of tetracyanoborate-based ILs for membrane-based gas separations. C1 [Liu, Hongjun; Dai, Sheng; Jiang, De-en] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37966 USA. RP Jiang, DE (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM jiangd@ornl.gov RI Jiang, De-en/D-9529-2011; Liu, Hongjun /A-2100-2012; Dai, Sheng/K-8411-2015 OI Jiang, De-en/0000-0001-5167-0731; Liu, Hongjun /0000-0003-3326-2640; Dai, Sheng/0000-0002-8046-3931 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 56 TC 6 Z9 6 U1 13 U2 102 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUN 25 PY 2014 VL 53 IS 25 BP 10485 EP 10490 DI 10.1021/ie501501k PG 6 WC Engineering, Chemical SC Engineering GA AK1OG UT WOS:000338183800026 ER PT J AU Fracaroli, AM Furukawa, H Suzuki, M Dodd, M Okajima, S Gandara, F Reimer, JA Yaghi, OM AF Fracaroli, Alejandro M. Furukawa, Hiroyasu Suzuki, Mitsuharu Dodd, Matthew Okajima, Satoshi Gandara, Felipe Reimer, Jeffrey A. Yaghi, Omar M. TI Metal-Organic Frameworks with Precisely Designed Interior for Carbon Dioxide Capture in the Presence of Water SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID POSTCOMBUSTION CO2 CAPTURE; VACUUM SWING ADSORPTION; FLUE-GAS; FUNCTIONALIZATION; SEPARATION; BINDING; ADSORBENTS; MECHANISM; SORBENTS; AIR AB The selective capture of carbon dioxide in the presence of water is an outstanding challenge. Here, we show that the interior of IRMOF-74-III can be covalently functionalized with primary amine (IRMOF-74-III-CH2NH2) and used for the selective capture of CO2 in 6596 relative humidity. This study encompasses the synthesis, structural characterization, gas adsorption, and CO2 capture properties of variously functionalized IRMOF-74-III compounds (IRMOF-74-III-CH3, -NH2, -CH(2)NHBoc, -CH(2)NMeBoc, -CH2NH2, and -CH2NHMe). Cross-polarization magic angle spinning C-13 NMR spectra showed that CO2 binds chemically to IRMOF-74-III-CH2NH2 and -CH2NHMe to make carbamic species. Carbon dioxide isotherms and breakthrough experiments show that IRMOF-74-III-CH2NH2 is especially efficient at taking up CO2 (3.2 mmol of CO2 per gram at 800 Torr) and, more significantly, removing CO2 from wet nitrogen gas streams with breakthrough time of 610 +/- 10 s g(-1) and full preservation of the IRMOF structure. C1 [Fracaroli, Alejandro M.; Furukawa, Hiroyasu; Suzuki, Mitsuharu; Okajima, Satoshi; Gandara, Felipe; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. [Fracaroli, Alejandro M.; Furukawa, Hiroyasu; Suzuki, Mitsuharu; Okajima, Satoshi; Gandara, Felipe; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. [Dodd, Matthew; Reimer, Jeffrey A.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Dodd, Matthew; Reimer, Jeffrey A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI Gandara, Felipe/B-9198-2013; EFRC, CGS/I-6680-2012; Stangl, Kristin/D-1502-2015; Furukawa, Hiroyasu/C-5910-2008; Fracaroli, Alejandro/B-5748-2012; OI Gandara, Felipe/0000-0002-1671-6260; Furukawa, Hiroyasu/0000-0002-6082-1738; Yaghi, Omar/0000-0002-5611-3325 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center [DE-SC0001015] FX This work was partially supported for synthesis and characterization by BASF SE (Ludwigshafen, Germany), gas adsorption by U.S. Department of Defense, Defense Threat Reduction Agency (HDTRA 1-12-1-0053), and carbon dioxide adsorption studies by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center (DE-SC0001015). NR 36 TC 125 Z9 125 U1 32 U2 274 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 25 PY 2014 VL 136 IS 25 BP 8863 EP 8866 DI 10.1021/ja503296c PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AK1OK UT WOS:000338184200007 PM 24911868 ER PT J AU Xie, J Yao, XH Madden, IP Jiang, DE Chou, LY Tsung, CK Wang, DW AF Xie, Jin Yao, Xiahui Madden, Ian P. Jiang, De-En Chou, Lien-Yang Tsung, Chia-Kuang Wang, Dunwei TI Selective Deposition of Ru Nanoparticles on TiSi2 Nanonet and Its Utilization for Li2O2 Formation and Decomposition SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ATOMIC LAYER DEPOSITION; NONAQUEOUS LI-O-2 BATTERIES; LITHIUM-OXYGEN BATTERIES; AIR BATTERIES; CATHODE; REDUCTION; PERFORMANCE; CHALLENGES; OXIDATION; DISCHARGE AB The Li-O-2 battery promises high capacity to meet the need for electrochemical energy storage applications. Successful development of the technology hinges on the availability of stable cathodes. The reactivity exhibited by a carbon support compromises the cyclability of Li-O-2 operation. A noncarbon cathode support has therefore become a necessity. Using a TiSi2 nanonet as a high surface area, conductive support, we obtained a new noncarbon cathode material that corrects the deficiency. To enable oxygen reduction and evolution, Ru nanoparticles were deposited by atomic layer deposition onto TiSi2 nanonets. A surprising site-selective growth whereupon Ru nanoparticles only deposit onto the b planes of TiSi2 was observed. DFT calculations show that the selectivity is a result of different interface energetics. The resulting heteronanostructure proves to be a highly effective cathode material. It enables Li-O-2 test cells that can be recharged more than 100 cycles with average round-trip efficiencies >70%. C1 [Xie, Jin; Yao, Xiahui; Madden, Ian P.; Chou, Lien-Yang; Tsung, Chia-Kuang; Wang, Dunwei] Boston Coll, Merkert Chem Ctr, Dept Chem, Chestnut Hill, MA 02467 USA. [Jiang, De-En] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wang, DW (reprint author), Boston Coll, Merkert Chem Ctr, Dept Chem, 2609 Beacon St, Chestnut Hill, MA 02467 USA. EM dunwei.wang@bc.edu RI Jiang, De-en/D-9529-2011; Xie, Jin/C-9509-2012; Xie, Jin/C-9581-2017 OI Jiang, De-en/0000-0001-5167-0731; FU Boston College FX The work is supported by Boston College. D.W. is an Alfred P. Sloan Fellow. We thank G. McMahon, J. Morabito, H. Wu, and G. Chen for their technical assistance. We also thank Y. Shao-Horn and her group for insightful discussions. XPS was performed at the Center for Nanoscale Systems (CNS). NR 31 TC 37 Z9 37 U1 7 U2 140 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 25 PY 2014 VL 136 IS 25 BP 8903 EP 8906 DI 10.1021/ja504431k PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AK1OK UT WOS:000338184200017 PM 24918260 ER PT J AU Ha, Y Tenderholt, AL Holm, RH Hedman, B Hodgson, KO Solomon, EI AF Ha, Yang Tenderholt, Adam L. Holm, Richard H. Hedman, Britt Hodgson, Keith O. Solomon, Edward I. TI Sulfur K-Edge X-ray Absorption Spectroscopy and Density Functional Theory Calculations on Monooxo Mo-IV and Bisoxo Mo-VI Bis-dithiolenes: Insights into the Mechanism of Oxo Transfer in Sulfite Oxidase and Its Relation to the Mechanism of DMSO Reductase SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OXYGEN-ATOM-TRANSFER; DIMETHYL-SULFOXIDE REDUCTASE; ACTIVE-SITE; BIS(DITHIOLENE) COMPLEXES; ELECTRONIC-STRUCTURE; TRANSFER REACTIVITY; CORRELATION-ENERGY; TUNGSTEN ENZYMES; MOLYBDENUM; MODELS AB Sulfur K-edge X-ray absorption spectroscopy (XAS) and density functional theory (DFT) calculations have been used to determine the electronic structures of two complexes [(MoO)-O-IV(bdt)(2)](2-) and [(MoO2)-O-VI(bdt)(2)](2-) (bdt = benzene-1,2-dithiolate(2-)) that relate to the reduced and oxidized forms of sulfite oxidase (SO). These are compared with those of previously studied dimethyl sulfoxide reductase (DMSOr) models. DFT calculations supported by the data are extended to evaluate the reaction coordinate for oxo transfer to a phosphite ester substrate. Three possible transition states are found with the one at lowest energy, stabilized by a P-S interaction, in good agreement with experimental kinetics data. Comparison of both oxo transfer reactions shows that in DMSOr, where the oxo is transferred from the substrate to the metal ion, the oxo transfer induces electron transfer, while in SO, where the oxo transfer is from the metal site to the substrate, the electron transfer initiates oxo transfer. This difference in reactivity is related to the difference in frontier molecular orbitals (FMO) of the metal-oxo and substrate-oxo bonds. Finally, these experimentally related calculations are extended to oxo transfer by sulfite oxidase. The presence of only one dithiolene at the enzyme active site selectively activates the equatorial oxo for transfer, and allows facile structural reorganization during turnover. C1 [Ha, Yang; Tenderholt, Adam L.; Hodgson, Keith O.; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Hedman, Britt; Hodgson, Keith O.; Solomon, Edward I.] Stanford Univ, SLAC, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Holm, Richard H.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. RP Holm, RH (reprint author), Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. EM holm@chemistry.harvard.edu; hedman@ssrl.slac.stanford.edu; hodgson@ssrl.slac.stanford.edu; solomone@stanford.edu FU NSF [CHE 0948211, CHE 0846397]; NIH [P41GM103393]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393] FX This study was supported by NSF grant (CHE 0948211, E.I.S. at Stanford University and CHE 0846397, R.H.H. at Harvard University) and NIH Grant (P41GM103393, K.O.H.). Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393). NR 59 TC 8 Z9 8 U1 8 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 25 PY 2014 VL 136 IS 25 BP 9094 EP 9105 DI 10.1021/ja503316p PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AK1OK UT WOS:000338184200041 PM 24884723 ER PT J AU Pham, TA Xu, JD Raymond, KN AF Pham, Tiffany A. Xu, Jide Raymond, Kenneth N. TI A Macrocyclic Chelator with Unprecedented Th4+ Affinity SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BASIS-SETS; COORDINATION CHEMISTRY; EQUILIBRIUM-CONSTANTS; ALPHA-PARTICLE; STABILITY; COMPLEXES; THERAPY; DENSITY; AGENTS; PSEUDOPOTENTIALS AB A novel macrocyclic octadentate ligand incorporating terephthalamide binding units has been synthesized and evaluated for the chelation of Th4+. The thorium complex was structurally characterized by X-ray diffraction and in solution with kinetic studies and spectrophotometric titrations. Dye displacement kinetic studies show that the ligand is a, much more rapid chelator of Th4+ than prevailing ligands (1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid and diethylenetriaminepentaacetic acid). Furthermore, the resulting complex was found to have a remarkably high thermodynamic stability, with a formation constant of 10(54). These data support potential radiotherapeutic applications. C1 [Pham, Tiffany A.; Xu, Jide; Raymond, Kenneth N.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Pham, Tiffany A.; Xu, Jide; Raymond, Kenneth N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Raymond, KN (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM raymond@socrates.berkeley.edu FU Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; NSF [CHE-0840505] FX This research is supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. The authors would like to thank Dr. Manuel Sturzbecher-Hoehne and Dr. Peter Gans for their help with titrations, Dr. Antonio DiPasquale for his help with the XRD data, and Dr. Casey J. Brown for helpful discussions. The computational work was made possible by NSF grant CHE-0840505, which funds the UC Berkeley Molecular Graphics Facility. NR 57 TC 6 Z9 6 U1 3 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 25 PY 2014 VL 136 IS 25 BP 9106 EP 9115 DI 10.1021/ja503456r PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AK1OK UT WOS:000338184200042 PM 24870296 ER PT J AU Hernandez, SC Schwartz, DS Taylor, CD Ray, AK AF Hernandez, Sarah C. Schwartz, Daniel S. Taylor, Christopher D. Ray, Asok K. TI Ab initio study of gallium stabilized delta-plutonium alloys and hydrogen-vacancy complexes (vol 26, 235502, 2014) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Correction C1 [Hernandez, Sarah C.; Ray, Asok K.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Schwartz, Daniel S.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Taylor, Christopher D.] DNV GL, Dublin, OH 43017 USA. [Taylor, Christopher D.] Ohio State Univ, Fontana Corros Ctr, Columbus, OH 43210 USA. RP Hernandez, SC (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. NR 1 TC 0 Z9 0 U1 3 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUN 25 PY 2014 VL 26 IS 25 AR 259601 DI 10.1088/0953-8984/26/25/259601 PG 1 WC Physics, Condensed Matter SC Physics GA AJ0MV UT WOS:000337348900025 ER PT J AU Zocco, DA Hamlin, JJ White, BD Kim, BJ Jeffries, JR Weir, ST Vohra, YK Allen, JW Maple, MB AF Zocco, D. A. Hamlin, J. J. White, B. D. Kim, B. J. Jeffries, J. R. Weir, S. T. Vohra, Y. K. Allen, J. W. Maple, M. B. TI Persistent non-metallic behavior in Sr2IrO4 and Sr3Ir2O7 at high pressures SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE iridates; metal-insulator transition; high pressure ID TEMPERATURE; TELLURIUM AB Iridium-based 5d transition-metal oxides are attractive candidates for the study of correlated electronic states due to the interplay of enhanced crystal-field, Coulomb and spin-orbit interaction energies. At ambient pressure, these conditions promote a novel J(eff) = 1/2 Mottinsulating state, characterized by a gap of the order of similar to 0.1 eV. We present high-pressure electrical resistivity measurements of single crystals of Sr2IrO4 and Sr3Ir2O7. While no indications of a pressure-induced metallic state up to 55 GPa were found in Sr2IrO4, a strong decrease of the gap energy and of the resistance of Sr3Ir2O7 between ambient pressure and 104 GPa confirm that this compound is in the proximity of a metal-insulator transition. C1 [Zocco, D. A.; Hamlin, J. J.; White, B. D.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Kim, B. J.] Max Planck Inst Solid State Res, Dept Solid State Spect, D-70569 Stuttgart, Germany. [Kim, B. J.; Allen, J. W.] Univ Michigan, Randall Lab, Dept Phys, Ann Arbor, MI 48109 USA. [Jeffries, J. R.; Weir, S. T.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Vohra, Y. K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RP Zocco, DA (reprint author), Karlsruhe Inst Technol, Inst Festkorperphys, D-76021 Karlsruhe, Germany. EM diego.zocco@kit.edu RI Zocco, Diego/O-3440-2014 FU National Nuclear Security Administration (NNSA) under the Stewardship Science Academic Alliance program through the US Department of Energy ( DOE) [DE-52-09NA29459.]; DOE Grant [DE-FG02-04-ER46105]; DOE-NNSA [DE-NA0002014, DE-AC52-07NA27344]; U S National Science Foundation [DMR-07-04480] FX High-pressure research at UC San Diego was supported by the National Nuclear Security Administration (NNSA) under the Stewardship Science Academic Alliance program through the US Department of Energy ( DOE) grant number DE-52-09NA29459. Physical properties characterization at ambient pressure was supported by DOE Grant DE-FG02-04-ER46105. LLNL is operated by Lawrence Livermore National Security, LLC, for the DOE-NNSA, under contract no. DE-AC52-07NA27344. YKV acknowledges support from the DOE-NNSA grant no. DE-NA0002014. This work was supported at UM by the U S National Science Foundation under grant no. DMR-07-04480. B J K acknowledges the Institute for Complex Adaptive Matter for a travel grant that enabled a visit to UC San Diago and thereby led to the conception of this work. NR 25 TC 12 Z9 12 U1 5 U2 61 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUN 25 PY 2014 VL 26 IS 25 AR 255603 DI 10.1088/0953-8984/26/25/255603 PG 5 WC Physics, Condensed Matter SC Physics GA AJ0MV UT WOS:000337348900016 PM 24888379 ER PT J AU Boucher, JI Jacobowitz, JR Beckett, BC Classen, S Theobald, DL AF Boucher, Jeffrey I. Jacobowitz, Joseph R. Beckett, Brian C. Classen, Scott Theobald, Douglas L. TI An atomic-resolution view of neofunctionalization in the evolution of apicomplexan lactate dehydrogenases SO ELIFE LA English DT Article ID CYTOPLASMIC MALATE-DEHYDROGENASE; PLASMODIUM-FALCIPARUM; TOXOPLASMA-GONDII; CRYSTAL-STRUCTURE; ESCHERICHIA-COLI; STRUCTURAL BASIS; ACTIVE-SITE; SUBSTRATE-SPECIFICITY; STRUCTURE VALIDATION; KINETIC-PROPERTIES AB Malate and lactate dehydrogenases (MDH and LDH) are homologous, core metabolic enzymes that share a fold and catalytic mechanism yet possess strict specificity for their substrates. In the Apicomplexa, convergent evolution of an unusual LDH from MDH resulted in a difference in substrate preference exceeding 12 orders of magnitude. The molecular and evolutionary mechanisms responsible for this extraordinary functional shift are currently unknown. Using ancestral sequence reconstruction, we find that the evolution of pyruvate specificity in apicomplexan LDHs arose through a classic neofunctionalization mechanism characterized by long-range epistasis, a promiscuous intermediate, and relatively few gain-of-function mutations of large effect. Residues far from the active site determine specificity, as shown by the crystal structures of three ancestral proteins that bracket the key gene duplication event. This work provides an unprecedented atomic-resolution view of evolutionary trajectories resulting in the de novo creation of a nascent enzymatic function. C1 [Boucher, Jeffrey I.; Jacobowitz, Joseph R.; Beckett, Brian C.; Theobald, Douglas L.] Brandeis Univ, Dept Biochem, Waltham, MA 02454 USA. [Classen, Scott] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Boucher, JI (reprint author), Brandeis Univ, Dept Biochem, Waltham, MA 02454 USA. RI Theobald, Douglas/F-3514-2013 OI Theobald, Douglas/0000-0002-2695-8343 NR 83 TC 11 Z9 11 U1 1 U2 2 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD JUN 25 PY 2014 VL 3 AR e02304 DI 10.7554/eLife.02304 PG 51 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AK9FQ UT WOS:000338733400001 ER PT J AU Magee, JW Zhou, WP White, MG AF Magee, Joseph W. Zhou, Wei-Ping White, Michael G. TI Promotion of Pt surfaces for ethanol electro-oxidation by the addition of small SnO2 nanoparticles: Activity and mechanism SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Ethanol oxidation; SnO2 nanoparticles; Pt surface; In situ IRRAS; Bi-functional catalyst ID ACETIC-ACID; FUEL-CELL; TIN OXIDE; ELECTROCATALYSTS; OXIDATION; CATALYSTS; PLATINUM; METHANOL; CO2; INTERFACE AB The catalytic effect of a SnO2 co-catalyst for ethanol electrooxidation on polycrystalline Pt is studied by electrochemical methods, in situ infrared reflection-absorption spectroscopy, and high resolution transmission electron microscopy. The electrochemical results show that deposition of small SnO2 NPs onto the pc-Pt electrode surface significantly enhances the catalytic performance of Pt. Infrared spectroscopy measurements show the effect that small SnO2 particles have on the removal of CO from the Pt surface and suggest that the electrocatalytic C-C bond splitting activity of Pt, the key step in full conversion of ethanol to CO2, is not affected by the addition of the -OH species provided by the SnO2 particles. Also, it is shown that controlled deposition of SnO2 is needed in order to,control the rate of partial oxidation to acetic acid compared to full oxidation to CO2. The combined results provide new insight into the role of SnO2 co-catalysts in promoting the electro-oxidation of ethanol to CO2 on Pt surfaces. (C) 2014 Elsevier B.V. All rights reserved. C1 [Magee, Joseph W.; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11974 USA. [Zhou, Wei-Ping; White, Michael G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP White, MG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11974 USA. EM jmagee@bnl.gov; wpzhou@bnl.gov; mgwhite@bnl.gov RI zhou, weiping/C-6832-2012 OI zhou, weiping/0000-0002-8058-7280 FU U.S Department of Energy, Office of Basic Energy Sciences, Divisions of Chemical Sciences [DE-AC02-98CH10886] FX This work carried out at Brookhaven National Laboratory was supported by U.S Department of Energy, Office of Basic Energy Sciences, Divisions of Chemical Sciences, under Contract No. DE-AC02-98CH10886. TEM images were obtained by Dong Su at the Center for Functional Nanomaterials at Brookhaven National Laboratory. NR 27 TC 9 Z9 10 U1 3 U2 88 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD JUN 25 PY 2014 VL 152 BP 397 EP 402 DI 10.1016/j.apcatb.2014.01.057 PG 6 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA AF1NY UT WOS:000334481800045 ER PT J AU Abergel, DSL Edge, JM Balatsky, AV AF Abergel, D. S. L. Edge, Jonathan M. Balatsky, Alexander V. TI The role of spin-orbit coupling in topologically protected interface states in Dirac materials SO NEW JOURNAL OF PHYSICS LA English DT Article DE Dirac materials; interface states; persistent currents; topological protection ID GRAPHENE; SPINTRONICS; INSULATORS; SURFACE; CONE AB We highlight the fact that two-dimensional (2D) materials with Dirac-like low energy band structures and spin-orbit coupling (SOC) will produce linearly dispersing topologically protected Jackiw-Rebbi modes at interfaces where the Dirac mass changes sign. These modes may support persistent spin or valley currents parallel to the interface, and the exact arrangement of such topologically protected currents depends crucially on the details of the SOC in the material. As examples, we discuss buckled 2D hexagonal lattices such as silicene or germanene, and transition metal dichalcogenides such as MoS2. C1 [Abergel, D. S. L.; Balatsky, Alexander V.] KTH Royal Inst Technol, NORDITA, SE-10691 Stockholm, Sweden. [Abergel, D. S. L.; Balatsky, Alexander V.] Stockholm Univ, SE-10691 Stockholm, Sweden. [Edge, Jonathan M.; Balatsky, Alexander V.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Abergel, DSL (reprint author), KTH Royal Inst Technol, NORDITA, Roslagstullsbacken 23, SE-10691 Stockholm, Sweden. EM david.abergel@nordita.org RI Abergel, David/D-4838-2015 OI Abergel, David/0000-0002-6166-181X FU ERC [DM-321031]; Nordita FX This work was supported by ERC DM-321031 and by Nordita. NR 28 TC 6 Z9 6 U1 6 U2 46 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 24 PY 2014 VL 16 AR 065012 DI 10.1088/1367-2630/16/6/065012 PG 8 WC Physics, Multidisciplinary SC Physics GA AL4EH UT WOS:000339085200001 ER PT J AU Brif, C Grace, MD Sarovar, M Young, KC AF Brif, Constantin Grace, Matthew D. Sarovar, Mohan Young, Kevin C. TI Exploring adiabatic quantum trajectories via optimal control SO NEW JOURNAL OF PHYSICS LA English DT Article DE adiabatic quantum computation; quantum optical control theory; adiabatic approximation; multiobjective optimization ID MULTIOBJECTIVE OPTIMIZATION; ALGORITHMS; DECOHERENCE; MECHANICS; GATES AB Adiabatic quantum computation employs a slow change of a time-dependent control function (or functions) to interpolate between an initial and final Hamiltonian, which helps to keep the system in the instantaneous ground state. When the evolution time is finite, the degree of adiabaticity (quantified in this work as the average ground-state population during evolution) depends on the particulars of a dynamic trajectory associated with a given set of control functions. We use quantum optimal control theory with a composite objective functional to numerically search for controls that achieve the target final state with a high fidelity while simultaneously maximizing the degree of adiabaticity. Exploring the properties of optimal adiabatic trajectories in model systems elucidates the dynamic mechanisms that suppress unwanted excitations from the ground state. Specifically, we discover that the use of multiple control functions makes it possible to access a rich set of dynamic trajectories, some of which attain a significantly improved performance (in terms of both fidelity and adiabaticity) through the increase of the energy gap during most of the evolution time. C1 [Brif, Constantin; Grace, Matthew D.; Sarovar, Mohan; Young, Kevin C.] Sandia Natl Labs, Dept Scalable & Secure Syst Res, Livermore, CA 94550 USA. RP Brif, C (reprint author), Sandia Natl Labs, Dept Scalable & Secure Syst Res, Livermore, CA 94550 USA. EM cnbrif@sandia.gov; mgrace@sandia.gov; mnsarov@sandia.gov; kyoung@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; United States Department of Energy' s National Nuclear Security Administration [DE-AC04-94AL85000] FX We acknowledge useful discussions with Sandia' s AQUARIUS Architecture team. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy' s National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 72 TC 5 Z9 5 U1 2 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 24 PY 2014 VL 16 AR 065013 DI 10.1088/1367-2630/16/6/065013 PG 20 WC Physics, Multidisciplinary SC Physics GA AL4EH UT WOS:000339085200002 ER PT J AU Chern, GW Reichhardt, C Reichhardt, CJO AF Chern, Gia-Wei Reichhardt, C. Reichhardt, C. J. Olson TI Avalanches and disorder-induced criticality in artificial spin ices SO NEW JOURNAL OF PHYSICS LA English DT Article DE avalanches; nonequilibrium phase transitions; artificial ice ID FRUSTRATION; DYNAMICS; NOISE AB We show that both square and kagome artificial spin ice systems exhibit disorder- induced nonequilibrium phase transitions, with power law avalanche distributions at the critical disorder level. The different nature of geometrical frustration in the two lattices produces distinct types of critical avalanche behavior. For the square ice, the avalanches involve the propagation of locally stable domain walls separating the two polarized ground states, and the scaling collapse agrees with an interface depinning mechanism. In contrast, avalanches in the fully frustrated kagome ice exhibit pronounced branching behaviors that resemble those found in directed percolation. The kagome ice also shows an interesting crossover in the power-law scaling of the avalanches at low disorder. Our results show that artificial spin ices are ideal systems in which to study nonequilibrium critical point phenomena. C1 [Chern, Gia-Wei; Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Ctr Nonlinear Studies & Theoret Div, Los Alamos, NM 87545 USA. RP Chern, GW (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies & Theoret Div, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov OI Reichhardt, Cynthia/0000-0002-3487-5089 NR 29 TC 4 Z9 4 U1 3 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 24 PY 2014 VL 16 AR 063051 DI 10.1088/1367-2630/16/6/063051 PG 9 WC Physics, Multidisciplinary SC Physics GA AL4CV UT WOS:000339081400003 ER PT J AU Li, XG Teng, A Ozer, MM Shen, J Weitering, HH Zhang, ZY AF Li, Xiaoguang Teng, Ao Oezer, Mustafa M. Shen, Jian Weitering, Hanno H. Zhang, Zhenyu TI Plasmonic excitations in ultrathin metal films on dielectric substrates SO NEW JOURNAL OF PHYSICS LA English DT Article DE ultrathin metal film; surface plasmon; multipole surface plasmon; plasmon hybridization; local optics model ID MULTIPOLE SURFACE-PLASMON; THIN-FILMS; OPTICAL-PROPERTIES; ALUMINUM SURFACE; DISPERSION; MODES; NANOPARTICLES; HYBRIDIZATION; PHOTOEMISSION; RESONANCE AB The optical properties of metals are mainly determined by their plasmonic excitations, with various intriguing phenomena associated with systems in reduced dimensions. In this paper, we present a systematic study of the plasmonic excitations in ultrathin metal films on dielectric substrates using two different theoretical approaches, and with Mg thin films on Si as prototype systems. The bulk of the results are obtained using the first approach within first-principles time-dependent local density approximation. We show that the presence of the substrate substantially modifies the plasmon hybridization of the metal films; in turn, the plasmon excitation in the films strongly enhances the absorption of the substrate. The detailed absorption spectra contain several intriguing features. Above the Mg surface plasmon mode, we observe a broad resonance due to the hybridization between the antisymmetric surface plasmon and multipole surface plasmon. Furthermore, below the Mg surface plasmon mode, there also exists a broad absorption feature, caused by individual electron-hole pair excitations. In the second approach, we use a semi-classical local optics model to reveal an intrinsic connection between the broad absorption feature and the multipole surface plasmon modes, which result from the single-particle and collective excitations of the same surface electrons, respectively. Our theoretical predictions on the plasmon dispersions and absorption spectra are also shown to be qualitatively consistent with the latest experimental observations using electron energy loss spectroscopy for Mg thin films grown on Si substrates. C1 [Li, Xiaoguang] Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China. [Li, Xiaoguang; Zhang, Zhenyu] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale HFNL, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China. [Li, Xiaoguang; Shen, Jian] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Li, Xiaoguang; Shen, Jian] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Teng, Ao; Oezer, Mustafa M.; Shen, Jian; Weitering, Hanno H.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Oezer, Mustafa M.; Weitering, Hanno H.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Li, XG (reprint author), Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China. EM lixg@siat.ac.cn FU NNSF of China [91121002, 11274071, 91021019, 11034006]; National Basic Research Program of China [2011CB921801]; USDOE [DE-FG03-02ER45958]; USNSF [0906025]; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, USDOE FX This work was supported in part by the NNSF of China (grant nos. 91121002, 11274071, 91021019 and 11034006), the National Basic Research Program of China (grant no. 2011CB921801), USDOE (grant no. DE-FG03-02ER45958), and USNSF (grant no. 0906025). HHW was supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, USDOE. NR 59 TC 0 Z9 0 U1 4 U2 48 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 24 PY 2014 VL 16 AR 065014 DI 10.1088/1367-2630/16/6/065014 PG 23 WC Physics, Multidisciplinary SC Physics GA AL4EH UT WOS:000339085200003 ER PT J AU Obermeyer, AC Capehart, SL Jarman, JB Francis, MB AF Obermeyer, Allie C. Capehart, Stacy L. Jarman, John B. Francis, Matthew B. TI Multivalent Viral Capsids with Internal Cargo for Fibrin Imaging SO PLOS ONE LA English DT Article ID VIRUS-LIKE PARTICLES; COMBINATORIAL LIBRARIES; CONTRAST AGENT; PEPTIDE; NANOPARTICLES; PROTEIN; POLYMERIZATION; BINDING; SURFACE; BACTERIOPHAGE-MS2 AB Thrombosis is the cause of many cardiovascular syndromes and is a significant contributor to life-threatening diseases, such as myocardial infarction and stroke. Thrombus targeted imaging agents have the capability to provide molecular information about pathological clots, potentially improving detection, risk stratification, and therapy of thrombosis-related diseases. Nanocarriers are a promising platform for the development of molecular imaging agents as they can be modified to have external targeting ligands and internal functional cargo. In this work, we report the synthesis and use of chemically functionalized bacteriophage MS2 capsids as biomolecule-based nanoparticles for fibrin imaging. The capsids were modified using an oxidative coupling reaction, conjugating similar to 90 copies of a fibrin targeting peptide to the exterior of each protein shell. The ability of the multivalent, targeted capsids to bind fibrin was first demonstrated by determining the impact on thrombin-mediated clot formation. The modified capsids out-performed the free peptides and were shown to inhibit clot formation at effective concentrations over ten-fold lower than the monomeric peptide alone. The installation of near-infrared fluorophores on the interior surface of the capsids enabled optical detection of binding to fibrin clots. The targeted capsids bound to fibrin, exhibiting higher signal-to-background than control, non-targeted MS2-based nanoagents. The in vitro assessment of the capsids suggests that fibrin-targeted MS2 capsids could be used as delivery agents to thrombi for diagnostic or therapeutic applications. C1 [Obermeyer, Allie C.; Capehart, Stacy L.; Jarman, John B.; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Francis, Matthew B.] Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA USA. RP Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mbfrancis@berkeley.edu FU DOD Breast Cancer Research Program [BC061995]; NSF; UC Berkeley Chemical Biology Graduate Program [1 T32 GMO66698] FX These studies were generously supported by the DOD Breast Cancer Research Program (BC061995). ACO and SLC were supported by graduate research fellowships from the NSF. The UC Berkeley Chemical Biology Graduate Program (Training Grant 1 T32 GMO66698) is acknowledged for their support of ACO. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 65 TC 15 Z9 15 U1 0 U2 17 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 24 PY 2014 VL 9 IS 6 AR e100678 DI 10.1371/journal.pone.0100678 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK7UT UT WOS:000338633900068 PM 24960118 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Sciolla, G Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Dittrich, S Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Anulli, F Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Lewis, P Lindemann, D Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wulsin, HW Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Anulli, F. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Lewis, P. Lindemann, D. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Antideuteron production in Upsilon(nS) decays and in e(+)e(-) -> q(q) over bar at root s approximate to 10.58 GeV SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; ENERGY; ANNIHILATION; MODEL AB We present measurements of the inclusive production of antideuterons in e(+)e(-) annihilation into hadrons at approximate to 10.58 GeV center-of-mass energy and in Upsilon(1S, 2S, 3S) decays. The results are obtained using data collected by the BABAR detector at the PEP-II electron-positron collider. Assuming a fireball spectral shape for the emitted antideuteron momentum, we find B(Upsilon(1S) -> (d) over barX) = (2.81 +/- 0.49(stat)-(+0.20)(0.24)(syst)) x 10(-5), B(Upsilon(2S) -> (d) over barX) = (2.64 +/- 0.11(stat)(-0.21)(+0.26)(syst)) x 10(-5), B(Upsilon(3S) -> (d) over barX) = (2.33 +/- 0.15(stat)(-0.28)(+0.31)(syst)) x 10(-5), and sigma(e(+)e(-) -> (d) over barX) = (9.63 +/- 0.41(stat)(-1.01)(+1.17)(syst) fb. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartmento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. 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[De Nardo, G.; Onorato, G.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [De Nardo, G.; Onorato, G.; Sciacca, C.] Univ Naples Federico II, Dipartimento Sci Fis, I-80126 Naples, Italy. [Martinelli, M.; Raven, G.] Natl Inst Nucl & High Energy Phys, NIKHEF, NL-1009 DB Amsterdam, Netherlands. [Jessop, C. P.; LoSecco, J. M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Feltresi, E.; Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Feltresi, E.; Margoni, M.; Simi, G.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph.; Marchiori, G.; Ocariz, J.; Sitt, S.] Univ Paris 07, Univ Paris 06, CNRS, Lab Phys Nucl & Hautes Energies,IN2P3, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Malaescu, B.; Biasini, M.; Pacetti, S.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.; Anulli, F.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Patrignani, Claudia/C-5223-2009; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Calcaterra, Alessandro/P-5260-2015; Oyanguren, Arantza/K-6454-2014; Monge, Maria Roberta/G-9127-2012; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Patrignani, Claudia/0000-0002-5882-1747; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Calcaterra, Alessandro/0000-0003-2670-4826; Oyanguren, Arantza/0000-0002-8240-7300; Monge, Maria Roberta/0000-0003-1633-3195; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 FU DOE (USA); NSF (USA); NSERC (Canada); CEA (France); BMBF (Germany); INFN (Italy); FOM (The Netherlands); NFR (Norway); MES (Russia); MICIIN (Spain); STFC (United Kingdom); Marie Curie EIF (European Union); A. P. Sloan Foundation (USA); Binational Science Foundation (USA-Israel); CNRS (France) [IN2P3]; DFG (Germany) FX We are grateful for the excellent luminosity and machine conditions provided by our PEP-II colleagues and for the substantial dedicated effort from the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and kind hospitality. This work is supported by DOE and NSF (USA), NSERC (Canada), CEA and CNRS-IN2P3 (France), BMBF and DFG (Germany), INFN (Italy), FOM (The Netherlands), NFR (Norway), MES (Russia), MICIIN (Spain), STFC (United Kingdom). Individuals have received support from the Marie Curie EIF (European Union), the A. P. Sloan Foundation (USA) and the Binational Science Foundation (USA-Israel). NR 20 TC 5 Z9 5 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 24 PY 2014 VL 89 IS 11 AR 111102 DI 10.1103/PhysRevD.89.111102 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK7XW UT WOS:000338642100001 ER PT J AU Li, F Yager, KG Dawson, NM Jiang, YB Malloy, KJ Qin, Y AF Li, Fei Yager, Kevin G. Dawson, Noel M. Jiang, Ying-Bing Malloy, Kevin J. Qin, Yang TI Stable and Controllable Polymer/Fullerene Composite Nanofibers through Cooperative Noncovalent Interactions for Organic Photovoltaics SO CHEMISTRY OF MATERIALS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; FIELD-EFFECT TRANSISTORS; ACID METHYL-ESTER; POLY(3-HEXYLTHIOPHENE) NANOFIBERS; POLY(3-BUTYLTHIOPHENE) NANOWIRES; DIBLOCK COPOLYMERS; BLOCK-COPOLYMER; POLYMER; MORPHOLOGY; PERFORMANCE AB A novel methodology of precisely constructing stable and controllable conjugated polymer (CP)/fullerene nanostructures is presented. By building in noncovalent interactions between CP nanofibers (NFs) and fullerene derivatives, supramolecular polymer/fullerene composite NFs are obtained in solution for the first time. Specifically, a conjugated block copolymer having poly(3-hexylthiophene) (P3HT) backbone selectively functionalized with polar isoorotic acid (IOA) moieties, P1, is used as the building block. Self-assembly of P1 in mixed solvents leads to well-defined NFs decorated with IOA groups on the periphery, onto which phenyl-C61-butyric acid methyl ester (PCBM) molecules are subsequently attached noncovalently. Formation of such complex structures are studied in detail and confirmed by UV-vis absorption spectroscopy, transmission electron microscopy (TEM), atomic force microscopy (AFM), and X-ray scattering measurements. Application of these composite NFs in organic photovoltaic (OPV) devices not only leads to superior performance but also much improved thermal stability and better defined and controllable morphology, when compared with conventional bulk heterojunction (BHJ) devices. C1 [Li, Fei; Qin, Yang] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. [Jiang, Ying-Bing] Univ New Mexico, TEM Lab, Albuquerque, NM 87131 USA. [Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Dawson, Noel M.; Malloy, Kevin J.] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87106 USA. RP Qin, Y (reprint author), Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. EM yangqin@unm.edu RI Yager, Kevin/F-9804-2011; Li, Fei/D-4426-2015; Malloy, Kevin/E-5994-2010 OI Yager, Kevin/0000-0001-7745-2513; Li, Fei/0000-0002-4177-2539; FU University of New Mexico; NSF [IIA-1301346]; Center for Functional Nanomaterials - U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors would like to acknowledge University of New Mexico for financial support for this research. Y.Q acknowledges NSF Grant No. IIA-1301346 for financial support. KY. is supported by the Center for Functional Nanomaterials, which is funded by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886. NR 69 TC 24 Z9 24 U1 4 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 24 PY 2014 VL 26 IS 12 BP 3747 EP 3756 DI 10.1021/cm501251n PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AK0FY UT WOS:000338089500025 ER PT J AU Thompson, CM Tan, XY Kovnir, K Garlea, VO Gippius, AA Yaroslavtsev, AA Menushenkov, AP Chernikov, RV Buttgen, N Kratschmer, W Zubavichus, YV Shatruk, M AF Thompson, Corey M. Tan, Xiaoyan Kovnir, Kirill Garlea, V. Ovidiu Gippius, Andrei A. Yaroslavtsev, Alexander A. Menushenkov, Alexey P. Chernikov, Roman V. Buettgen, Norbert Kraetschmer, Wolfgang Zubavichus, Yan V. Shatruk, Michael TI Synthesis, Structures, and Magnetic Properties of Rare-Earth Cobalt Arsenides, RCo2As2 (R = La, Ce, Pr, Nd) SO CHEMISTRY OF MATERIALS LA English DT Article ID PHOSPHIDES CACO2P2; POLE INVERSION; CRYSTAL; FERROMAGNETISM; DIFFRACTION; ORDER AB Four rare-earth cobalt arsenides, RCo2As2 (R = La, Ce, Pr, Nd), were obtained by reactions of constituent elements in molten Bi. The use of Bi flux also allowed the growth of representative single crystals. All compounds are isostructural and belong to the ThCr2Si2 type (space group I4/mmm). The formation of Co vacancies is observed in all structures, while the structures of La- and Ce-containing compounds also show incorporation of minor Bi defects next to the R crystallographic site. Correspondingly, the general formula of these materials can be written as R1-xBixCo2-delta As2, with x/delta = 0.03/0.1, 0.05/0.15, 0/0.2, and 0/0.3 for R = La, Ce, Pr, and Nd, respectively. All compounds exhibit high-temperature ferromagnetic ordering of Co magnetic moments in the range 60-200 K. Electronic band structure calculations revealed a high peak in the density of states at the Fermi level, thus supporting the itinerant nature of magnetism in the Co sublattice. The magnetic ordering in the lanthanide sublattice takes place at lower temperatures, with the R moments aligning antiparallel to the Co moments to give a ferrimagnetic ground state. The measurements on oriented single crystals demonstrated significant magnetic anisotropy in the ferrimagnetic state, with the preferred moment alignment along the c axis of the tetragonal lattice. Neutron powder diffraction failed to reveal the structure of magnetically ordered states but confirmed the presence of Co vacancies. X-ray absorption near-edge structure spectroscopy on Ce1.95Bi0.05Co1.85As2 showed the average oxidation state of Ce to be +3.06. Solid state NMR spectroscopy revealed a substantially reduced hyperfine field on the Co atoms in the vicinity of Bi defects. C1 [Thompson, Corey M.; Tan, Xiaoyan; Kovnir, Kirill; Shatruk, Michael] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Garlea, V. Ovidiu] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Gippius, Andrei A.] Moscow MV Lomonosov State Univ, Dept Phys, Moscow 119991, Russia. [Yaroslavtsev, Alexander A.; Menushenkov, Alexey P.] Natl Res Nucl Univ, Moscow Engn Phys Inst, Moscow 115409, Russia. [Yaroslavtsev, Alexander A.] European XFEL GmbH, D-22761 Hamburg, Germany. [Yaroslavtsev, Alexander A.] Univ Hamburg, Inst Theoret Phys, D-20355 Hamburg, Germany. [Chernikov, Roman V.] DESY Photon Sci, D-22603 Hamburg, Germany. [Buettgen, Norbert; Kraetschmer, Wolfgang] Univ Augsburg, D-86159 Augsburg, Germany. [Zubavichus, Yan V.] Kurchatov Inst, Natl Res Ctr, Moscow 123182, Russia. RP Shatruk, M (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. EM shatruk@chem.fsu.edu RI Gippius, Andrey/D-1139-2010; Yaroslavtsev, Alexander/A-5437-2013; Garlea, Vasile/A-4994-2016 OI Garlea, Vasile/0000-0002-5322-7271 FU National Science Foundation [DMR-0955353]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Russian Scientific Foundation; Deutsche Forschungsgemeinschaft (DFG) via Augsburg [TRR 80]; Deutsche Forschungsgemeinschaft (DFG) via Munich [TRR 80]; Deutsche Forschungsgemeinschaft (DFG) via Stuttgart [TRR 80] FX This research is supported by the National Science Foundation CAREER Award to M.S. (DMR-0955353). The work at the Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). The authors also acknowledge Helmholtz-Zentrum Berlin for providing the beamtime at experimental station of BESSY-II storage ring. A.Y. and A.M. thank the Russian Scientific Foundation for support. A.A.G., N.B., and W.K. were supported by the Deutsche Forschungsgemeinschaft (DFG) via TRR 80 (Augsburg, Munich, Stuttgart). NR 53 TC 10 Z9 10 U1 8 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 24 PY 2014 VL 26 IS 12 BP 3825 EP 3837 DI 10.1021/cm501522v PG 13 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AK0FY UT WOS:000338089500033 ER PT J AU Harrison, KL Bridges, CA Segre, CU Varnado, CD Applestone, D Bielawski, CW Paranthaman, MP Manthiram, A AF Harrison, Katharine L. Bridges, Craig A. Segre, Carlo U. Varnado, C. Daniel, Jr. Applestone, Danielle Bielawski, Christopher W. Paranthaman, Mariappan Parans Manthiram, Arumugam TI Chemical and Electrochemical Lithiation of LiVOPO4 Cathodes for Lithium-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID VANADYL PHOSPHATE; CRYSTAL-STRUCTURE; 4 V; HYDROTHERMAL SYNTHESIS; RECHARGEABLE BATTERY; PHASE-TRANSITION; INSERTION; FLUOROPHOSPHATE; BETA-LIVOPO4; EPSILON-VOPO4 AB The theoretical capacity of LiVOPO4 could be increased from 159 to 318 mAh/g with the insertion of a second Li+ ion into the lattice to form Li2VOPO4, significantly enhancing the energy density of lithium-ion batteries. The phase changes accompanying the second Li+ insertion into alpha-LiVOPO4 and beta-LiVOPO4 are presented here at various degrees of lithiation, employing both electrochemical and chemical lithiation. Inductively coupled plasma, X-ray absorption spectroscopy, and Fourier transform infrared spectroscopy measurements indicate that a composition of Li2VOPO4 can be realized with an oxidation state of V3+ by the chemical lithiation process. The accompanying structural changes are evidenced by X-ray and neutron powder diffraction. Spectroscopic and diffraction data collected with the chemically lithiated samples as well as diffraction data on the electrochemically lithiated samples reveal that a significant amount of lithium can be inserted into alpha-LiVOPO4 before a phase change occurs. In contrast, lithiation of beta-LiVOPO4 is more consistent with the formation of a two-phase mixture throughout most of the lithiation range. The phases observed with the ambient-temperature lithiation processes presented here are significantly different from those reported in the literature. C1 [Harrison, Katharine L.; Manthiram, Arumugam] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA. [Bridges, Craig A.; Paranthaman, Mariappan Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Segre, Carlo U.] IIT, Dept Phys, Chicago, IL 60616 USA. [Segre, Carlo U.] IIT, CSRRI, Chicago, IL 60616 USA. [Varnado, C. Daniel, Jr.; Bielawski, Christopher W.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Applestone, Danielle] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI Segre, Carlo/B-1548-2009; BM, MRCAT/G-7576-2011; Paranthaman, Mariappan/N-3866-2015 OI Segre, Carlo/0000-0001-7664-1574; Paranthaman, Mariappan/0000-0003-3009-8531 FU Office of Vehicle Technologies of the U.S. Department of Energy under the Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231, 7000389]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Department of Energy; MRCAT; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The synthesis, basic phase analysis, and electrochemical characterization work at the University of Texas at Austin was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 7000389, under the Batteries for Advanced Transportation Technologies (BATT) Program. The structural analysis work at Oak Ridge National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Research at the SNS and CNMS-ShaRE facility was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Use of the Advanced Photon Source at Argonne National Laboratory (CUS) was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors thank Dr. Ashfia Huq for assistance with collection of NPD data at SNS and Dr. Ray Unocic for assistance with structural investigations by electron microscopy. NR 59 TC 16 Z9 16 U1 3 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 24 PY 2014 VL 26 IS 12 BP 3849 EP 3861 DI 10.1021/cm501588j PG 13 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AK0FY UT WOS:000338089500035 ER PT J AU Kim, MD Dergunov, SA Richter, AG Durbin, J Shmakov, SN Jia, Y Kenbeilova, S Orazbekuly, Y Kengpeiil, A Lindner, E Pingali, SV Urban, VS Weigand, S Pinkhassik, E AF Kim, Mariya D. Dergunov, Sergey A. Richter, Andrew G. Durbin, Jeffrey Shmakov, Sergey N. Jia, Ying Kenbeilova, Saltanat Orazbekuly, Yerbolat Kengpeiil, Aigerim Lindner, Ernoe Pingali, Sai Venkatesh Urban, Volker S. Weigand, Steven Pinkhassik, Eugene TI Facile Directed Assembly of Hollow Polymer Nanocapsules within Spontaneously Formed Catanionic Surfactant Vesicles SO LANGMUIR LA English DT Article ID ANGLE NEUTRON-SCATTERING; THIN ORGANIC MATERIALS; AQUEOUS MIXTURES; PHASE-BEHAVIOR; CETYLTRIMETHYLAMMONIUM BROMIDE; RADICAL POLYMERIZATION; EQUILIBRIUM VESICLES; LIGHT-SCATTERING; BUILDING-BLOCKS; SPHERES AB Surfactant vesicles containing monomers in the interior of the bilayer were used to template hollow polymer nanocapsules. This study investigated the formation of surfactant/monomer assemblies by two loading methods, concurrent loading and diffusion loading. The assembly process and the resulting aggregates were investigated with dynamic light scattering, small angle neutron scattering, and small-angle X-ray scattering. Acrylic monomers formed vesicles with a mixture of cationic and anionic surfactants in a broad range of surfactant ratios. Regions with predominant formation of vesicles were broader for compositions containing acrylic monomers compared with blank surfactants. This observation supports the stabilization of the vesicular structure by acrylic monomers. Diffusion loading produced monomer-loaded vesicles unless vesicles were composed from surfactants at the ratios close to the boundary of a vesicular phase region on a phase diagram. Both concurrent-loaded and diffusion-loaded surfactant/monomer vesicles produced hollow polymer nanocapsules upon the polymerization of monomers in the bilayer followed by removal of surfactant scaffolds. C1 [Kim, Mariya D.; Dergunov, Sergey A.; Durbin, Jeffrey; Shmakov, Sergey N.; Jia, Ying; Pinkhassik, Eugene] St Louis Univ, Dept Chem, St Louis, MO 63103 USA. [Richter, Andrew G.] Valparaiso Univ, Dept Phys & Astron, Valparaiso, IN 46383 USA. [Kenbeilova, Saltanat; Orazbekuly, Yerbolat; Kengpeiil, Aigerim] Kazakh Natl Tech Univ, Dept Chem Technol Proc Petr Gas & Polymers, Alma Ata 050013, Kazakhstan. [Lindner, Ernoe] Univ Memphis, Dept Biomed Engn, Memphis, TN 38152 USA. [Pingali, Sai Venkatesh; Urban, Volker S.] Oak Ridge Natl Lab, Ctr Struct Mol Biol, Oak Ridge, TN 37831 USA. [Weigand, Steven] Argonne Natl Lab, Adv Photon Source, DND CAT, Argonne, IL 60439 USA. RP Pinkhassik, E (reprint author), St Louis Univ, Dept Chem, 3501 Laclede Ave, St Louis, MO 63103 USA. EM epinkhas@slu.edu RI Shmakov, Sergey/H-1106-2012; Urban, Volker/N-5361-2015; Dergunov, Sergey/O-6287-2014; OI Shmakov, Sergey/0000-0002-8713-4516; Urban, Volker/0000-0002-7962-3408; Dergunov, Sergey/0000-0001-6668-6445; Pingali, Sai Venkatesh/0000-0001-7961-4176 FU Fed Ex Institute of Technology; National Science Foundation [CHE-1316680, CHE-1012951, CHE-0933363]; Saint Louis University; Committee of Science of the Ministry of Education and Science of Republic of Kazakhstan [0547/GF2]; E.I. DuPont de Nemours Co.; Dow Chemical Company; Northwestern University; U.S. DOE [DE-AC02-06CH11357]; Office of Biological and Environmental Research; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by Fed Ex Institute of Technology, National Science Foundation (CHE-1316680, CHE-1012951, and CHE-0933363), and Saint Louis University Presidential Research Fund award. Work was partially supported by grant from the Committee of Science of the Ministry of Education and Science of Republic of Kazakhstan (No. 0547/GF2). Portions of this work were performed at the DuPont-Northwestern-Dow Collaborative Access Team (DND-CAT) located at Sector 5 of the Advanced Photon Source (APS). DND-CAT is supported by E.I. DuPont de Nemours & Co., the Dow Chemical Company and Northwestern University. Use of the APS, an Office of Science User Facility operated by the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Portions of this work were performed at Oak Ridge National Laboratory's Center for Structural Molecular Biology and High Flux Isotope Reactor, sponsored by the Office of Biological and Environmental Research and the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. V.U. acknowledges support by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. We acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the neutron research facilities used in portions of this work. NR 48 TC 12 Z9 12 U1 2 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUN 24 PY 2014 VL 30 IS 24 BP 7061 EP 7069 DI 10.1021/la404026w PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AK0FZ UT WOS:000338089600004 PM 24341533 ER PT J AU Schade, L Franzka, S Mathieu, M Biener, MM Biener, J Hartmann, N AF Schade, Lina Franzka, Steffen Mathieu, Mareike Biener, Monika M. Biener, Juergen Hartmann, Nils TI Photothermal Laser Microsintering of Nanoporous Gold SO LANGMUIR LA English DT Article ID SELF-ASSEMBLED MONOLAYERS; NANOMATERIALS; TEMPERATURE; FABRICATION; CATALYSTS; SURFACES; AU AB Photothermal processing of nanoporous gold using a microfocused continuous-wave laser at a wavelength of 532 nm and a 1/e(2) spot diameter of 2.9 mu m has been studied. In addition, complementary experiments have been carried out via conventional annealing. Scanning electron microscopy has been used for characterization. Local laser irradiation at distinct laser powers and pulse lengths results in coarsening of the porous gold structures. During laser processing the pore size of the native nanoporous gold increases to maximum values in the range of 0.25-3 mu m. The affected areas exhibit lateral dimensions in the range of 2-10 mu m. Overall two regions are distinguished. An inner region, where large pores and ligaments are formed and an outer region, where the pore size and ligament size gradually change and approach the feature sizes of the native material. A qualitative thermokinetic model allows one to reproduce the experimentally observed dependence of the laser-induced morphologies on the laser parameters. On the basis of this model the underlying processes are attributed to sintering and melting of the gold structures. The presented results demonstrate the prospects of photothermal laser processing in engineering porous gold with spatially varying porosities on micrometer to nanometer length scales. C1 [Schade, Lina; Franzka, Steffen; Mathieu, Mareike; Hartmann, Nils] Univ Duisburg Essen, Fak Chem, D-45141 Essen, Germany. [Schade, Lina; Franzka, Steffen; Mathieu, Mareike; Hartmann, Nils] Univ Duisburg Essen, Ctr Nanointegrat Duisburg Essen CENIDE, D-47057 Duisburg, Germany. [Mathieu, Mareike; Biener, Monika M.; Biener, Juergen] Lawrence Livermore Natl Lab, Nanoscale Synth & Characterizat Lab, Livermore, CA 94550 USA. RP Hartmann, N (reprint author), Univ Duisburg Essen, Fak Chem, Univ Str 5, D-45141 Essen, Germany. EM Nils.Hartmann@uni-due.de FU European Union; Ministry of Innovation, Science and Research of the State of North Rhine-Westphalia in Germany (NanoEnergieTechnikZentrum, NETZ); Ministry of Innovation, Science and Research of the State of North Rhine-Westphalia in Germany (Objective 2 Programme: European Regional Development Fund, ERDF); U.S. DOE by LLNL [DE-AC52-07NA27344]; Interdisciplinary Center for Analytics on the Nanoscale (ICAN) of the Universitat Duisburg-Essen FX Financial support by the European Union, and the Ministry of Innovation, Science and Research of the State of North Rhine-Westphalia in Germany (NanoEnergieTechnikZentrum, NETZ, Objective 2 Programme: European Regional Development Fund, ERDF) is gratefully acknowledged. Work at LLNL was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. We gratefully acknowledge Prof. Andrea Hodge, University of Southern California, who provided polished samples for mechanical testing. We also gratefully acknowledge support by the Interdisciplinary Center for Analytics on the Nanoscale (ICAN) of the Universitat Duisburg-Essen. NR 34 TC 13 Z9 13 U1 3 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUN 24 PY 2014 VL 30 IS 24 BP 7190 EP 7197 DI 10.1021/la5011192 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AK0FZ UT WOS:000338089600020 PM 24869898 ER PT J AU Choi, E Park, S Ahn, H Lee, M Bang, J Lee, B Ryu, DY AF Choi, Eunyoung Park, Sungmin Ahn, Hyungju Lee, Moongyu Bang, Joona Lee, Byeongdu Ryu, Du Yeol TI Substrate-Independent Lamellar Orientation in High-Molecular-Weight Polystyrene-b-poly(methyl methacrylate) Films: Neutral Solvent Vapor and Thermal Annealing Effect SO MACROMOLECULES LA English DT Article ID COPOLYMER THIN-FILMS; CONTROLLED INTERFACIAL INTERACTIONS; ABA BLOCK-COPOLYMERS; PS-B-PMMA; DIBLOCK COPOLYMER; MICRODOMAIN ORIENTATION; ORDERED STRUCTURE; SELECTIVE SOLVENTS; PHOTONIC CRYSTALS; PHASE-BEHAVIOR AB Lamellar microdomain orientation in polystyrene-b-poly(methyl methacrylate) (PS-b-PMMA) films was controlled by a solvent vapor annealing process, where the high-molecular-weight block copolymer (BCP) was used to self-assemble in a large period of 105 nm. A neutral solvent annealing with tetrahydrofuran vapor screened the difference in the surface energy between the two blocks and the interfacial interactions of the substrate with each block, leading to the substrate-independent perpendicular orientation of lamellar microdomains. Together with thermal annealing of the solvent-annealed BCP film, we demonstrate that highly ordered line arrays of perpendicularly oriented lamellae were well guided in topographic line and disk photoresist patterns composed of the PS-attractive cross-linked copolymer, where the interlamellar d-spacing compliant to the patterns was dependent on the confinement types. C1 [Choi, Eunyoung; Park, Sungmin; Ahn, Hyungju; Ryu, Du Yeol] Yonsei Univ, Dept Chem & Biomol Engn, Seoul 120749, South Korea. [Lee, Moongyu] Samsung Display Co, LCD R&D Ctr, LCD Business, Yongin 446711, South Korea. [Bang, Joona] Korea Univ, Dept Chem & Biol Engn, Seoul 136701, South Korea. [Lee, Byeongdu] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. RP Ryu, DY (reprint author), Yonsei Univ, Dept Chem & Biomol Engn, 50 Yonsei Ro, Seoul 120749, South Korea. EM dyryu@yonsei.ac.kr RI Bang, Joona/F-6589-2013; Ryu, Du Yeol/G-8278-2012; OI Lee, Byeongdu/0000-0003-2514-8805 FU Nuclear RD Programs; APCPI ERC [2007-0056091]; Converging Research Center - Ministry of Science, ICT & Future Planning (MSIP), Korea [2010K001430]; Samsung Display Co., Korea FX This work was supported by the Nuclear R&D Programs, APCPI ERC (2007-0056091), and Converging Research Center (2010K001430) funded by the Ministry of Science, ICT & Future Planning (MSIP), Korea. We also acknowledge the partial support from Samsung Display Co., Korea. NR 57 TC 12 Z9 12 U1 5 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUN 24 PY 2014 VL 47 IS 12 BP 3969 EP 3977 DI 10.1021/ma500716f PG 9 WC Polymer Science SC Polymer Science GA AK0FX UT WOS:000338089400024 ER PT J AU Phatak, C Petford-Long, AK Beleggia, M De Graef, M AF Phatak, C. Petford-Long, A. K. Beleggia, M. De Graef, M. TI Theoretical study of ferroelectric nanoparticles using phase reconstructed electron microscopy SO PHYSICAL REVIEW B LA English DT Article ID FIELD-EFFECT TRANSISTORS; DOMAIN-WALLS; ATOMIC-SCALE; TRANSITIONS; FILMS AB Ferroelectric nanostructures are important for a variety of applications in electronic and electro-optical devices, including nonvolatile memories and thin-film capacitors. These applications involve stability and switching of polarization using external stimuli, such as electric fields. We present a theoretical model describing how the shape of a nanoparticle affects its polarization in the absence of screening charges, and quantify the electron-optical phase shift for detecting ferroelectric signals with phase-sensitive techniques in a transmission electron microscope. We provide an example phase shift computation for a uniformly polarized prolate ellipsoid with varying aspect ratio in the absence of screening charges. C1 [Phatak, C.; Petford-Long, A. K.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. [Beleggia, M.] Tech Univ Denmark, Ctr Electron Nanoscopy, DK-2800 Lyngby, Denmark. [De Graef, M.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Phatak, C (reprint author), Argonne Natl Lab, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM cd@anl.gov RI DeGraef, Marc/G-5827-2010; Petford-Long, Amanda/P-6026-2014; OI DeGraef, Marc/0000-0002-4721-6226; Petford-Long, Amanda/0000-0002-3154-8090; Beleggia, Marco/0000-0002-2888-1888 FU U.S. Department of Energy (DOE), Office of Science, Materials Sciences and Engineering Division; DOE's Office of Basic Energy Sciences [DE-FG02-01ER45893] FX Work by C. P. and A.P.-L. was supported by the U.S. Department of Energy (DOE), Office of Science, Materials Sciences and Engineering Division. M. D. G acknowledges DOE's Office of Basic Energy Sciences for partial financial support (Grant No. DE-FG02-01ER45893). NR 23 TC 3 Z9 3 U1 1 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 24 PY 2014 VL 89 IS 21 AR 214112 DI 10.1103/PhysRevB.89.214112 PG 5 WC Physics, Condensed Matter SC Physics GA AK7WU UT WOS:000338639200001 ER PT J AU Quan, ZW Wu, D Zhu, JL Evers, WH Boncella, JM Siebbeles, LDA Wang, ZW Navrotsky, A Xu, HW AF Quan, Zewei Wu, Di Zhu, Jinlong Evers, Wiel H. Boncella, James M. Siebbeles, Laurens D. A. Wang, Zhongwu Navrotsky, Alexandra Xu, Hongwu TI Energy landscape of self-assembled superlattices of PbSe nanocrystals SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE PbSe nanocrystal superlattices; thermodynamics; ligand interaction ID QUANTUM DOTS; NANOPARTICLES AB Self-assembly of nanocrystals (NCs) into superlattices is an intriguing multiscale phenomenon that may lead to materials with novel collective properties, in addition to the unique properties of individual NCs compared with their bulk counterparts. By using different dispersion solvents, we synthesized three types of PbSe NC superlattices-body-centered cubic (bcc), body-centered tetragonal (bct), and face-centered cubic (fcc)-as confirmed by synchrotron small-angle X-ray scattering. Solution calorimetric measurements in hexane show that the enthalpy of formation of the superlattice from dispersed NCs is on the order of -2 kJ/mol. The calorimetric measurements reveal that the bcc superlattice is the energetically most stable polymorph, with the bct being 0.32 and the fcc 0.55 kJ/mol higher in enthalpy. This stability sequence is consistent with the decreased packing efficiency of PbSe NCs from bcc (17.2%) to bct (16.0%) and to fcc (15.2%). The small enthalpy differences among the three polymorphs confirm a closely spaced energy landscape and explain the ease of formation of different NC superlattices at slightly different synthesis conditions. C1 [Quan, Zewei; Xu, Hongwu] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Quan, Zewei; Boncella, James M.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Wu, Di; Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Wu, Di; Navrotsky, Alexandra] Univ Calif Davis, Nanomat Environm Agr & Technol Org Res Unit, Davis, CA 95616 USA. [Zhu, Jinlong] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. [Evers, Wiel H.; Siebbeles, Laurens D. A.] Delft Univ Technol, Dept Chem Engn, Optoelect Mat Sect, NL-2628 BL Delft, Netherlands. [Evers, Wiel H.] Delft Univ Technol, Kavli Inst Nanosci, NL-2628 CJ Delft, Netherlands. [Wang, Zhongwu] Cornell Univ, Wilson Lab, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. RP Navrotsky, A (reprint author), Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. EM anavrotsky@ucdavis.edu; hxu@lanl.gov RI Quan, Zewei/G-4759-2011; Wu, Di/A-3039-2014; Siebbeles, Laurens/I-2401-2012; OI Wu, Di/0000-0001-6879-321X; Siebbeles, Laurens/0000-0002-4812-7495; Xu, Hongwu/0000-0002-0793-6923; Boncella, James/0000-0001-8393-392X FU Los Alamos National Security LLC under Department of Energy (DOE) [DE-AC52-06NA25396]; DOE Office of Basic Energy Sciences [DEFG02-05ER15667]; National Science Foundation Award [DMR-0936384]; Dutch Foundation for Fundamental Research FX We thank Weizhong Han and Wei Gao for assistance with the TEM and ATR measurements and Welley Siu Loc for help with the figure drawing. Z.Q. acknowledges a J.Robert Oppenheimer fellowship supported by the laboratory-directed research and development program of Los Alamos National Laboratory, which is operated by Los Alamos National Security LLC under Department of Energy (DOE) Contract DE-AC52-06NA25396. Calorimetry at University of California, Davis was supported by the DOE Office of Basic Energy Sciences, Grant DEFG02-05ER15667. Cornell High Energy Synchrotron Source is supported by National Science Foundation Award DMR-0936384. W.H.E. and L.D.A.S. acknowledge the Dutch Foundation for Fundamental Research on Matter for supporting the program "Control over Functional Nanoparticle Solids." NR 29 TC 7 Z9 7 U1 11 U2 68 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 24 PY 2014 VL 111 IS 25 BP 9054 EP 9057 DI 10.1073/pnas.1408835111 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5WJ UT WOS:000337760600026 PM 24927573 ER PT J AU Maseyk, K Berry, JA Billesbach, D Campbell, JE Torn, MS Zahniser, M Seibt, U AF Maseyk, Kadmiel Berry, Joseph A. Billesbach, Dave Campbell, John Elliott Torn, Margaret S. Zahniser, Mark Seibt, Ulli TI Sources and sinks of carbonyl sulfide in an agricultural field in the Southern Great Plains SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbonic anhydrase; LRU; ERU; flux partitioning; soil metabolism ID STOMATAL CONDUCTANCE; DIMETHYL SULFIDE; THIOBACILLUS-THIOPARUS; SOIL-MICROORGANISMS; SULFUR-COMPOUNDS; GROWING-SEASON; GLOBAL BUDGET; GAS-EXCHANGE; FOREST SOILS; COS AB Net photosynthesis is the largest single flux in the global carbon cycle, but controls over its variability are poorly understood because there is no direct way of measuring it at the ecosystem scale. We report observations of ecosystem carbonyl sulfide (COS) and CO2 fluxes that resolve key gaps in an emerging framework for using concurrent COS and CO2 measurements to quantify terrestrial gross primary productivity. At a wheat field in Oklahoma we found that in the peak growing season the flux-weighted leaf relative uptake of COS and CO2 during photosynthesis was 1.3, at the lower end of values from laboratory studies, and varied systematically with light. Due to nocturnal stomatal conductance, COS uptake by vegetation continued at night, contributing a large fraction (29%) of daily net ecosystem COS fluxes. In comparison, the contribution of soil fluxes was small (1-6%) during the peak growing season. Upland soils are usually considered sinks of COS. In contrast, the well-aerated soil at the site switched from COS uptake to emissions at a soil temperature of around 15 degrees C. We observed COS production from the roots of wheat and other species and COS uptake by root-free soil up to a soil temperature of around 25 degrees C. Our dataset demonstrates that vegetation uptake is the dominant ecosystem COS flux in the peak growing season, providing support of COS as an independent tracer of terrestrial photosynthesis. However, the observation that ecosystems may become a COS source at high temperature needs to be considered in global modeling studies. C1 [Maseyk, Kadmiel; Seibt, Ulli] Univ Paris 06, Inst Ecol & Environm Sci, F-78850 Thiverval Grignon, France. [Berry, Joseph A.] Carnegie Inst, Dept Global Ecol, Stanford, CA 94305 USA. [Billesbach, Dave] Univ Nebraska, Biol Syst Engn Dept, Lincoln, NE 68583 USA. [Campbell, John Elliott] Univ Calif, Sierra Nevada Res Inst, Merced, CA 95343 USA. [Torn, Margaret S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zahniser, Mark] Aerodyne Res Inc, Ctr Atmospher & Environm Chem, Billerica, MA 01821 USA. [Seibt, Ulli] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. RP Maseyk, K (reprint author), Univ Paris 06, Inst Ecol & Environm Sci, Grignon Campus, F-78850 Thiverval Grignon, France. EM kadmiel.maseyk@upmc.fr; useibt@ucla.edu RI Torn, Margaret/D-2305-2015 FU DOE, Biological and Environmental Research Division [DE-SC0007094, DE-AC02-05CH11231]; European Research Council Starting Grant [202835]; National Science Foundation Major Research Instrumentation program; Air Liquide Foundation; DOE, Small Business Innovation Research Grant [DE-SC0001801] FX We thank the staff of the Department of Energy (DOE) Atmospheric Radiation Measurement Central Facility, particularly Pat Dowell, for hosting and assisting us in completing this project. We also thank two anonymous reviewers for their helpful comments and suggestions. This work was supported by the DOE, Biological and Environmental Research Division Award DE-SC0007094 and under Contract DE-AC02-05CH11231, European Research Council Starting Grant 202835 (to U.S.), and grants by the National Science Foundation Major Research Instrumentation program and the Air Liquide Foundation (to J.A.B.). Instrument development was supported by funding from the DOE, Small Business Innovation Research Grant DE-SC0001801. NR 46 TC 21 Z9 21 U1 3 U2 41 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 24 PY 2014 VL 111 IS 25 BP 9064 EP 9069 DI 10.1073/pnas.1319132111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5WJ UT WOS:000337760600028 PM 24927594 ER PT J AU Bhattacharya, S Lou, XH Hwang, P Rajashankar, KR Wang, XP Gustafsson, JA Fletterick, RJ Jacobson, RH Webb, P AF Bhattacharya, Suparna Lou, Xiaohua Hwang, Peter Rajashankar, Kanagalaghatta R. Wang, Xiaoping Gustafsson, Jan-Ake Fletterick, Robert J. Jacobson, Raymond H. Webb, Paul TI Structural and functional insight into TAF1-TAF7, a subcomplex of transcription factor II D SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE initiation complex; protein structure; protein-protein interaction; X-ray crystallography ID ACETYLTRANSFERASE ACTIVITY; COMPLEX; BINDING; SUBUNIT; TFIIF; STATE; DNA; RAP30/RAP74; CONTAINS; DOMAINS AB Transcription factor II D (TFIID) is a multiprotein complex that nucleates formation of the basal transcription machinery. TATA binding protein-associated factors 1 and 7 (TAF1 and TAF7), two subunits of TFIID, are integral to the regulation of eukaryotic transcription initiation and play key roles in preinitiation complex (PIC) assembly. Current models suggest that TAF7 acts as a dissociable inhibitor of TAF1 histone acetyltransferase activity and that this event ensures appropriate assembly of the RNA polymerase IImediated PIC before transcriptional initiation. Here, we report the 3D structure of a complex of yeast TAF1 with TAF7 at 2.9 angstrom resolution. The structure displays novel architecture and is characterized by a large predominantly hydrophobic heterodimer interface and extensive cofolding of TAF subunits. There are no obvious similarities between TAF1 and known histone acetyltransferases. Instead, the surface of the TAF1-TAF7 complex contains two prominent conserved surface pockets, one of which binds selectively to an inhibitory trimethylated histone H3 mark on Lys27 in a manner that is also regulated by phosphorylation at the neighboring H3 serine. Our findings could point toward novel roles for the TAF1-TAF7 complex in regulation of PIC assembly via reading epigenetic histone marks. C1 [Bhattacharya, Suparna; Lou, Xiaohua; Webb, Paul] Houston Methodist Res Inst, Genom Med Program, Houston, TX 77030 USA. [Lou, Xiaohua; Gustafsson, Jan-Ake] Univ Houston, Ctr Nucl Receptors & Cell Signaling, Houston, TX 77204 USA. [Hwang, Peter; Fletterick, Robert J.] Univ Calif San Francisco, Med Ctr, San Francisco, CA 94158 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, Northwestern Collaborat Access Team, Argonne, IL 60439 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Argonne Natl Lab, Dept Chem & Chem Biol, Argonne, IL 60439 USA. [Wang, Xiaoping; Jacobson, Raymond H.] Univ Texas MD Anderson Canc Ctr, Dept Mol Biol & Biochem, Houston, TX 77030 USA. RP Webb, P (reprint author), Houston Methodist Res Inst, Genom Med Program, Houston, TX 77030 USA. EM pwebb@tmhs.org FU National Institutes of Health [DK41482, UO1 GM094614]; Cancer Prevention Research Institute of Texas [RP011444-P3]; Robert A. Welch Foundation [E-0004]; National Institute of General Medical Sciences Grant from the National Institutes of Health [P41 GM103403] FX We thank Senapathy Rajagopalan and Stephen Ayers for comments. This study was supported by National Institutes of Health Grants DK41482 (to P. W.) UO1 GM094614 (to R.J.F.; with a subcomponent to P. W.), and Cancer Prevention Research Institute of Texas Grant RP011444-P3 (to P.W.). J.-angstrom.G. is grateful for a grant from the Robert A. Welch Foundation (E-0004). This work is based on research conducted at the Advanced Photon Source on the Northeastern Collaborative Access Team beamlines, which are supported by National Institute of General Medical Sciences Grant P41 GM103403 from the National Institutes of Health. NR 37 TC 8 Z9 8 U1 0 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 24 PY 2014 VL 111 IS 25 BP 9103 EP 9108 DI 10.1073/pnas.1408293111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5WJ UT WOS:000337760600035 PM 24927529 ER PT J AU Shcherbak, I Millar, N Robertson, GP AF Shcherbak, Iurii Millar, Neville Robertson, G. Philip TI Global metaanalysis of the nonlinear response of soil nitrous oxide (N2O) emissions to fertilizer nitrogen SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE fertilizer response; greenhouse gas emissions; agriculture; bioenergy; greenhouse gas mitigation ID CROPPING SYSTEMS; AGRICULTURE; FIELDS; CROPS AB Nitrous oxide (N2O) is a potent greenhouse gas (GHG) that also depletes stratospheric ozone. Nitrogen (N) fertilizer rate is the best single predictor of N2O emissions from agricultural soils, which are responsible for similar to 50% of the total global anthropogenic flux, but it is a relatively imprecise estimator. Accumulating evidence suggests that the emission response to increasing N input is exponential rather than linear, as assumed by Intergovernmental Panel on Climate Change methodologies. We performed a metaanalysis to test the generalizability of this pattern. From 78 published studies (233 site-years) with at least three N-input levels, we calculated N2O emission factors (EFs) for each nonzero input level as a percentage of N input converted to N2O emissions. We found that the N2O response to N inputs grew significantly faster than linear for synthetic fertilizers and for most crop types. N-fixing crops had a higher rate of change in EF (Delta EF) than others. A higher.EF was also evident in soils with carbon > 1.5% and soils with pH < 7, and where fertilizer was applied only once annually. Our results suggest a general trend of exponentially increasing N2O emissions as N inputs increase to exceed crop needs. Use of this knowledge in GHG inventories should improve assessments of fertilizer-derived N2O emissions, help address disparities in the global N2O budget, and refine the accuracy of N2O mitigation protocols. In low-input systems typical of sub-Saharan Africa, for example, modest N additions will have little impact on estimated N2O emissions, whereas equivalent additions (or reductions) in excessively fertilized systems will have a disproportionately major impact. C1 [Shcherbak, Iurii; Millar, Neville; Robertson, G. Philip] Michigan State Univ, WK Kellogg Biol Stn, Hickory Corners, MI 49060 USA. [Shcherbak, Iurii; Millar, Neville; Robertson, G. Philip] Michigan State Univ, Dept Plant Soil & Microbial Sci, E Lansing, MI 48824 USA. [Shcherbak, Iurii; Millar, Neville; Robertson, G. Philip] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. RP Shcherbak, I (reprint author), Michigan State Univ, WK Kellogg Biol Stn, Hickory Corners, MI 49060 USA. EM iurii.shcherbak@gmail.com OI Shcherbak@qut.edu.au, Iurii/0000-0003-4153-3770; Robertson, G/0000-0001-9771-9895 FU US National Science Foundation Long-Term Ecological Research [DEB 1027253]; Doctoral Dissertation Improvement [DEB 1110683]; US Department of Energy Office of Science [DE-FCO2-07ER64494]; Office of Energy Efficiency and Renewable Energy [DE-ACO5-76RL01830]; Electric Power Research Institute; Michigan State University AgBioResearch FX We thank many colleagues for helpful discussions during the development of this analysis, particularly A. N. Kravchenko, S. K. Hamilton, B. Basso, S. J. Del Grosso, M. D. Eve, I. Gelfand, S. M. Ogle, J. Six, C. van Kessel, and R. T. Venterea. We thank L. Ruan for help with Chinese translations of primary papers and J. Schuette for editorial assistance. Funding was provided by the US National Science Foundation Long-Term Ecological Research (Grant DEB 1027253) and Doctoral Dissertation Improvement (Grant DEB 1110683) programs, the US Department of Energy Office of Science (Grant DE-FCO2-07ER64494) and Office of Energy Efficiency and Renewable Energy (Grant DE-ACO5-76RL01830), the Electric Power Research Institute, and Michigan State University AgBioResearch. NR 38 TC 101 Z9 108 U1 30 U2 205 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 24 PY 2014 VL 111 IS 25 BP 9199 EP 9204 DI 10.1073/pnas.1322434111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5WJ UT WOS:000337760600051 PM 24927583 ER PT J AU Haft, RJF Keating, DH Schwaegler, T Schwalbach, MS Vinokur, J Tremaine, M Peters, JM Kotlajich, MV Pohlmann, EL Ong, IM Grass, JA Kiley, PJ Landick, R AF Haft, Rembrandt J. F. Keating, David H. Schwaegler, Tyler Schwalbach, Michael S. Vinokur, Jeffrey Tremaine, Mary Peters, Jason M. Kotlajich, Matthew V. Pohlmann, Edward L. Ong, Irene M. Grass, Jeffrey A. Kiley, Patricia J. Landick, Robert TI Correcting direct effects of ethanol on translation and transcription machinery confers ethanol tolerance in bacteria SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID COMPLETE GENOME SEQUENCE; COLI RNA-POLYMERASE; ESCHERICHIA-COLI; PHOSPHOLIPID-SYNTHESIS; IN-VIVO; GUANOSINE TETRAPHOSPHATE; METHIONINE BIOSYNTHESIS; STREPTOMYCIN DEPENDENCE; NEAMINE RESISTANCE; HEAT-SHOCK AB The molecular mechanisms of ethanol toxicity and tolerance in bacteria, although important for biotechnology and bioenergy applications, remain incompletely understood. Genetic studies have identified potential cellular targets for ethanol and have revealed multiple mechanisms of tolerance, but it remains difficult to separate the direct and indirect effects of ethanol. We used adaptive evolution to generate spontaneous ethanol-tolerant strains of Escherichia coli, and then characterized mechanisms of toxicity and resistance using genome-scale DNAseq, RNAseq, and ribosome profiling coupled with specific assays of ribosome and RNA polymerase function. Evolved alleles of metJ, rho, and rpsQ recapitulated most of the observed ethanol tolerance, implicating translation and transcription as key processes affected by ethanol. Ethanol induced miscoding errors during protein synthesis, from which the evolved rpsQ allele protected cells by increasing ribosome accuracy. Ribosome profiling and RNAseq analyses established that ethanol negatively affects transcriptional and translational processivity. Ethanol-stressed cells exhibited ribosomal stalling at internal AUG codons, which may be ameliorated by the adaptive inactivation of the MetJ repressor of methionine biosynthesis genes. Ethanol also caused aberrant intragenic transcription termination for mRNAs with low ribosome density, which was reduced in a strain with the adaptive rho mutation. Furthermore, ethanol inhibited transcript elongation by RNA polymerase in vitro. We propose that ethanol-induced inhibition and uncoupling of mRNA and protein synthesis through direct effects on ribosomes and RNA polymerase conformations are major contributors to ethanol toxicity in E. coli, and that adaptive mutations in metJ, rho, and rpsQ help protect these central dogma processes in the presence of ethanol. C1 [Haft, Rembrandt J. F.; Keating, David H.; Schwaegler, Tyler; Schwalbach, Michael S.; Vinokur, Jeffrey; Tremaine, Mary; Pohlmann, Edward L.; Ong, Irene M.; Grass, Jeffrey A.; Kiley, Patricia J.; Landick, Robert] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Peters, Jason M.; Kotlajich, Matthew V.; Landick, Robert] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Peters, Jason M.] Univ Wisconsin, Dept Genet, Madison, WI 53706 USA. [Kiley, Patricia J.] Univ Wisconsin, Dept Biomol Chem, Madison, WI 53706 USA. [Landick, Robert] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. RP Landick, R (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. EM landick@biochem.wisc.edu FU Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494] FX We thank our Great Lakes Bioenergy Research Center collaborators and R. L. laboratory colleagues for critical reading of the manuscript. We are grateful to Gene-Wei Li and David Burkhardt for advice and assistance with ribosome profiling experiments, P. Chu for technical assistance, and Gerwald Jogl for helpful discussions of ribosome decoding. This work was funded by the Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science Grant DE-FC02-07ER64494). NR 83 TC 24 Z9 24 U1 1 U2 39 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 24 PY 2014 VL 111 IS 25 BP E2576 EP E2585 DI 10.1073/pnas.1401853111 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5WJ UT WOS:000337760600011 PM 24927582 ER PT J AU Chen, AP Weigand, M Bi, ZX Zhang, WR Lu, XJ Dowden, P MacManus-Driscoll, JL Wang, HY Jia, QX AF Chen, Aiping Weigand, Marcus Bi, Zhenxing Zhang, Wenrui Lu, Xuejie Dowden, Paul MacManus-Driscoll, Judith L. Wang, Haiyan Jia, Quanxi TI Evolution of microstructure, strain and physical properties in oxide nanocomposite films SO SCIENTIFIC REPORTS LA English DT Article ID SELF-ASSEMBLED NANOSTRUCTURES; LOW-FIELD MAGNETORESISTANCE; THIN-FILMS; COLOSSAL MAGNETORESISTANCE; PHASE; POLARIZATION; CONDUCTIVITY; INTEGRATION; TRANSITION; ANISOTROPY AB We, using LSMO:ZnO nanocomposite films as a model system, have studied the effect of film thickness on the physical properties of nanocomposites. It shows that strain, microstructure, as well as magnetoresistance strongly rely on film thickness. The magnetotransport properties have been fitted by a modified parallel connection channel model, which is in agreement with the microstructure evolution as a function of film thickness in nanocomposite films on sapphire substrates. The strain analysis indicates that the variation of physical properties in nanocomposite films on LAO is dominated by strain effect. These results confirm the critical role of film thickness on microstructures, strain states, and functionalities. It further shows that one can use film thickness as a key parameter to design nanocomposites with optimum functionalities. C1 [Chen, Aiping; Weigand, Marcus; Bi, Zhenxing; Lu, Xuejie; Dowden, Paul; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. [Zhang, Wenrui; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [MacManus-Driscoll, Judith L.] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB2 3QZ, England. RP Chen, AP (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. EM apchen@lanl.gov; qxjia@lanl.gov RI Wang, Haiyan/P-3550-2014; Chen, Aiping/F-3212-2011; Lu, Xujie/L-9672-2014; Zhang, Wenrui/D-1892-2015 OI Wang, Haiyan/0000-0002-7397-1209; Chen, Aiping/0000-0003-2639-2797; Lu, Xujie/0000-0001-8402-7160; Zhang, Wenrui/0000-0002-0223-1924 FU U.S. DOE through the NNSA's Laboratory Directed Research and Development Program; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396]; ERC; Novox [ERC-2009-adG 247276]; EPSRC (U.K.) [EP/H047867/1]; U.S. National Science Foundation [DMR-1401266, 1007969, 0846504] FX This work was supported by the U.S. DOE through the NNSA's Laboratory Directed Research and Development Program and performed, in part, at the Center for Integrated Nanotechnologies (CINT), a U.S. DOE, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract DE-AC52-06NA25396. J.L.M.-D thanks the ERC for the Advanced Investigator Grant, Novox, ERC-2009-adG 247276 and the EPSRC (U.K.) for grant EP/H047867/1. The effort at Texas A&M University is supported by the U.S. National Science Foundation (DMR-1401266, 1007969 and 0846504). NR 51 TC 13 Z9 13 U1 4 U2 87 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 24 PY 2014 VL 4 AR 5426 DI 10.1038/srep05426 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7PY UT WOS:000337889800005 PM 24958206 ER PT J AU Bang, J Kim, YS Park, CH Gao, F Zhang, SB AF Bang, Junhyeok Kim, Youg-Sung Park, C. H. Gao, F. Zhang, S. B. TI Understanding the presence of vacancy clusters in ZnO from a kinetic perspective SO APPLIED PHYSICS LETTERS LA English DT Article ID ZINC-OXIDE; DOPANT DIFFUSION; POINT-DEFECTS; HYDROGEN; PHOTOLUMINESCENCE; INTERSTITIALS; SILICON AB Vacancy clusters have been observed in ZnO by positron-annihilation spectroscopy (PAS), but detailed mechanisms are unclear. This is because the clustering happens in non-equilibrium conditions, for which theoretical method has not been well established. Combining first-principles calculation and kinetic Monte Carlo simulation, we determine the roles of non-equilibrium kinetics on the vacancies clustering. We find that clustering starts with the formation of Zn and O vacancy pairs (V-Zn - Vo), which further grow by attracting additional mono-vacancies. At this stage, vacancy diffusivity becomes crucial: due to the larger diffusivity of V-Zn compared to V-O, more V-Zn-abundant clusters are formed than V-O-abundant clusters. The large dissociation energy barriers, e. g., over 2.5 eV for (V-Zn - Vo), suggest that, once formed, it is difficult for the clusters to dissociate. By promoting mono-vacancy diffusion, thermal annealing will increase the size of the clusters. As the PAS is insensitive to V-O donor defects, our results suggest an interpretation of the experimental data that could not have been made without the in-depth calculations. (C) 2014 AIP Publishing LLC. C1 [Bang, Junhyeok; Zhang, S. B.] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Kim, Youg-Sung] Korea Res Inst Stand & Sci, Taejon 305340, South Korea. [Kim, Youg-Sung] Univ Sci & Technol, Dept Nano Sci, Taejon 305350, South Korea. [Park, C. H.] Pusan Natl Univ, Res Ctr Dielectr & Adv Matter Phys, Pusan 609735, South Korea. [Gao, F.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Kim, YS (reprint author), Korea Res Inst Stand & Sci, Taejon 305340, South Korea. EM kimyongsung@gmail.com; zhangs9@rpi.edu RI Zhang, Shengbai/D-4885-2013 OI Zhang, Shengbai/0000-0003-0833-5860 FU DOE [DE-SC0002623]; Nano R&D Program through the National Research Foundation (NRF) of Korea [NRF-2009-0082489]; BRL program through National Research Fund of Korea - MEST [2012-0000345] FX J.B. and S.B.Z. were supported by DOE under Grant No. DE-SC0002623. Y.-S.K. acknowledges the support by Nano R&D Program through the National Research Foundation (NRF) of Korea (Grant No. NRF-2009-0082489). C. H. P. acknowledges the support from the BRL program through National Research Fund of Korea funded by MEST (Grant No. 2012-0000345). We also acknowledge the computational support by the Computational Center for Nanotechnology Innovations (CCNI) at Rensselaer Polytechnic Institute (RPI). NR 32 TC 11 Z9 11 U1 5 U2 47 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 252101 DI 10.1063/1.4884653 PG 5 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900041 ER PT J AU Jones, AM Kelly, JF Tedeschi, J McCloy, JS AF Jones, A. Mark Kelly, James F. Tedeschi, Jonathan McCloy, John S. TI Design considerations for high-Q bandpass microwave oscillator sensors based upon resonant amplification SO APPLIED PHYSICS LETTERS LA English DT Article ID FREQUENCY; MODULATOR AB A series of microwave resonant oscillator sensors were designed and characterized using bandpass planar and volumetric electrical resonators having loaded quality factor (Q) values in the range of 2 to 20. The use of these resonators in positive feedback circuits yielded sensor Q-factors of up to 2 x 10(7), demonstrating Q-factor amplifications on the order of 10(6). It is shown that the Q-factor amplification can be increased in a positive feedback system through the selection of feedback loop group delay, allowing use of resonators with lower static, loaded Q-factor values. A low-frequency electromagnetic interference sensing application is demonstrated for two resonant oscillator configurations, showing considerable frequency sensitivity to 45 kHz emitters. (C) 2014 AIP Publishing LLC. C1 [Jones, A. Mark; Kelly, James F.; Tedeschi, Jonathan] Pacific NW Natl Lab, Appl Phys Grp, Richland, WA 99352 USA. [McCloy, John S.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP McCloy, JS (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. EM john.mccloy@wsu.edu FU Laboratory Directed Research and Development funds at Pacific Northwest National Laboratory; U.S. Department of Energy [DE-AC05-76RL01830] FX This work was supported by Laboratory Directed Research and Development funds at Pacific Northwest National Laboratory, operated by Battelle Memorial Institute for the U.S. Department of Energy under Contract No. DE-AC05-76RL01830. NR 27 TC 9 Z9 9 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 253507 DI 10.1063/1.4885077 PG 5 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900094 ER PT J AU Loya, PE Xia, YZ Peng, C Bei, H Zhang, P Zhang, J George, EP Gao, YF Lou, J AF Loya, P. E. Xia, Y. Z. Peng, C. Bei, H. Zhang, P. Zhang, J. George, E. P. Gao, Y. F. Lou, J. TI Yield strength dependence on strain rate of molybdenum-alloy nanofibers SO APPLIED PHYSICS LETTERS LA English DT Article ID MECHANICAL-PROPERTIES; PLASTICITY; TENSILE; SCALE AB The yield strength dependence on strain rate was studied for molybdenum-alloy nanofibers with varying initial dislocation density at three different pre-strain levels. In-situ tensile experiments at three displacement rates were carried out in a scanning electron microscope. Yield strength and its scatter decreased as a function of the pre-strain level for different displacement rates. A statistical model was used to analyze the results, and a negative strain rate dependence was inferred from the yield experiments. This finding suggests the need for theoretical investigations since classical models such as dynamic strain aging may have limitations at such nanoscales. (C) 2014 AIP Publishing LLC. C1 [Loya, P. E.; Peng, C.; Zhang, P.; Zhang, J.; Lou, J.] Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA. [Xia, Y. Z.; George, E. P.; Gao, Y. F.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Bei, H.; George, E. P.; Gao, Y. F.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Loya, PE (reprint author), Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA. RI George, Easo/L-5434-2014; Gao, Yanfei/F-9034-2010; Peng, Cheng/C-3212-2014; OI Gao, Yanfei/0000-0003-2082-857X; Peng, Cheng/0000-0001-6090-2944; Bei, Hongbin/0000-0003-0283-7990 FU NSF [DMR-1128818, CMMI-0928297]; Welch Foundation [C-1716]; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences, and Engineering Division FX The authors acknowledge the support from NSF Grant Nos. DMR-1128818 and CMMI-0928297, and the Welch Foundation Grant No. C-1716 (P. E. L., C. P., P.Z., J.Z., and J.L.), and the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences, and Engineering Division (Y.Z.X., H. B., E. P. G., and Y.F.G.). NR 22 TC 3 Z9 3 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 251909 DI 10.1063/1.4885377 PG 5 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900034 ER PT J AU Rebola, A Klie, RF Zapol, P Ogut, S AF Rebola, Alejandro Klie, Robert F. Zapol, Peter Oeguet, Serdar TI Phonon and thermal transport properties of the misfit-layered oxide thermoelectric Ca3Co4O9 from first principles SO APPLIED PHYSICS LETTERS LA English DT Article ID STABILITY AB The full phonon spectra of two rational approximants to the incommensurate thermoelectric oxide material Ca3Co4O9 (CCO) are calculated from first principles within density functional theory (DFT) and its DFT + U extension. The computed phonon dispersion curves are then used to evaluate the constant volume heat capacity, as well as the full and partial (subsystem-projected) lattice thermal conductivity of CCO. The results are discussed in terms of the effects of the Hubbard U on the computed properties, the size of the rational approximants used to model CCO, the relative contributions of the two subsystems that comprise the misfit-layered material, and the anisotropic nature of the computed thermal conductivity. We obtain good agreement with available experimental data. (C) 2014 AIP Publishing LLC. C1 [Rebola, Alejandro; Klie, Robert F.; Oeguet, Serdar] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Rebola, Alejandro; Zapol, Peter] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Rebola, A (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA. RI Zapol, Peter/G-1810-2012 OI Zapol, Peter/0000-0003-0570-9169 FU National Science Foundation [DMR-0846784]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division; Office of Science of the U.S. Department of Energy FX We acknowledge support for this work by the National Science Foundation under Grant No. DMR-0846784 (R. F. K). S.O. acknowledges support by the National Science Foundation under the Independent Research/Development program, while working at the Foundation. Work at ANL was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. We also acknowledge computational support from the Argonne National Laboratory Computing Resource Center, Center for Nanoscale Materials, and the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy. NR 12 TC 8 Z9 8 U1 2 U2 55 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 251910 DI 10.1063/1.4885389 PG 5 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900035 ER PT J AU Richardson, M Sankaranarayanan, SKRS Bhethanabotla, VR AF Richardson, M. Sankaranarayanan, S. K. R. S. Bhethanabotla, V. R. TI Shear-horizontal surface acoustic wave phononic device with high density filling material for ultra-low power sensing applications SO APPLIED PHYSICS LETTERS LA English DT Article ID SENSOR AB Finite element simulations of a phononic shear-horizontal surface acoustic wave (SAW) sensor based on ST 90 degrees-X Quartz reveal a dramatic reduction in power consumption. The phononic sensor is realized by artificially structuring the delay path to form an acoustic meta-material comprised of a periodic microcavity array incorporating high-density materials such as tantalum or tungsten. Constructive interference of the scattered and secondary reflected waves at every microcavity interface leads to acoustic energy confinement in the high-density regions translating into reduced power loss. Tantalum filled cavities show the best performance while tungsten inclusions create a phononic bandgap. Based on our simulation results, SAW devices with tantalum filled microcavities were fabricated and shown to significantly decrease insertion loss. Our findings offer encouraging prospects for designing low power, highly sensitive portable biosensors. (C) 2014 AIP Publishing LLC. C1 [Richardson, M.; Bhethanabotla, V. R.] Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. [Sankaranarayanan, S. K. R. S.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Bhethanabotla, VR (reprint author), Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. EM bhethana@usf.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors wish to thank Research Computing, within USF Information Technology, University of South Florida for access to high performance computing resources. The Center for Nanoscale Materials is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 19 TC 1 Z9 1 U1 3 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 253501 DI 10.1063/1.4884655 PG 5 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900088 ER PT J AU Wang, FF Fan, LL Ren, Y Chen, J Xing, XR AF Wang, Fangfang Fan, Longlong Ren, Yang Chen, Jun Xing, Xianran TI Bi-O covalency in PbTiO3-BiInO3 with enhanced ferroelectric properties: Synchrotron radiation diffraction and first-principles study SO APPLIED PHYSICS LETTERS LA English DT Article ID POWDER DIFFRACTION; SOLID-SOLUTION; PHASE-BOUNDARY; 1ST PRINCIPLES; CERAMICS; PIEZOELECTRICS; TETRAGONALITY AB High-T-C ferroelectric (1 - x) PbTiO3-xBiInO(3) shows a sustainable spontaneous polarization in tetragonal phase by amount of BiInO3 augmented. It is rare and interesting that weak ferroelectric In3+ substitution does not reduce ferroelectricity as most of BiMeO3 materials. To understand this abnormality behavior, the structure and the cation displacements are studied by means of synchrotron radiation diffraction. The cation displacements of A-site atoms and B-site atoms exhibit a coupling property. Their sustainedly increasing trend is quantitatively associated with spontaneous polarization. Moreover, the structure, the valence electron density distributions, electron localization function, and Bader analysis have been researched on the chemical bond in (1 - x) PbTiO3-xBiInO(3) through first-principles calculations here. Although In atoms substitution reduces the covalency degree, this loss is offset by enhanced covalency between Bi-O bonds. The crucial role of Bi atom substitution not only contributes to enhance the covalency but also promotes the polarization. (C) 2014 AIP Publishing LLC. C1 [Wang, Fangfang; Fan, Longlong; Chen, Jun; Xing, Xianran] Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. [Ren, Yang] Argonne Natl Lab, XRay Sci Div, Argonne, IL 60439 USA. RP Chen, J (reprint author), Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. EM junchen@ustb.edu.cn; xing@ustb.edu.cn RI Chen, Jun/M-1669-2015 FU National Natural Science Foundation of China [21231001, 21031005, 21322102]; Program for Changjiang Scholars and Innovative Research Team in University [IRT1207]; U.S. DOE [DE-AC02-06CH11357] FX This work was financially supported by the National Natural Science Foundation of China (Nos. 21231001, 21031005, and 21322102) and the Program for Changjiang Scholars and Innovative Research Team in University (IRT1207). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The calculations were performed on the Quantum Materials Simulator of USTB. NR 33 TC 2 Z9 2 U1 5 U2 40 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 252901 DI 10.1063/1.4881614 PG 4 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900068 ER PT J AU Zhang, XF Guo, JJ Qin, GW AF Zhang, X. F. Guo, J. J. Qin, G. W. TI Assembled micro-nano particles with multiple interface polarizations for electromagnetic absorption at gigahertz SO APPLIED PHYSICS LETTERS LA English DT Article ID WAVE ABSORBER; NANOCOMPOSITES; ENHANCEMENT; FERRITE; NANOPARTICLES; PERMITTIVITY; PERMEABILITY; COMPOSITE; RESONANCE AB The usually utilized electromagnetic absorbers are fabricated by randomly dispersed fillers in polymer matrix, which limit the construction of multiple interfaces, thus influencing the optimization of absorption efficiency. In this Letter, the core/shell heterogeneous nanocapsules are chemically modified and subsequently conjugated on the micrometre-scale polymer units, forming a micro/nano-hybrided absorbent. Such a system creates multiple interfaces at sub-nanoscale, thus producing enhanced dielectric loss phenomena and resulting in an absorption efficiency of more than 90% over 2-18 GHz. The present study provides an effective concept to optimize the electromagnetic coupling and has important implications in the development of electromagnetic absorption materials. (C) 2014 AIP Publishing LLC. C1 [Zhang, X. F.; Qin, G. W.] Northeastern Univ, Key Lab Anisotropy & Texture Mat, Shenyang 110819, Peoples R China. [Guo, J. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Zhang, XF (reprint author), Northeastern Univ, Key Lab Anisotropy & Texture Mat, Shenyang 110819, Peoples R China. EM zhangxf@atm.neu.edu.cn; qingw@smm.neu.edu.cn RI Qin, Gaowu/C-8742-2015; guo, junjie/I-3189-2012; Zhang, Xuefeng/G-1960-2016 OI Qin, Gaowu/0000-0002-0852-6715; guo, junjie/0000-0002-3414-3734; FU Northeastern University of China; Program for Changjiang Scholars and Innovative Research Team in University [IRT0713] FX The authors gratefully acknowledge the start-up funding supported from the Northeastern University of China and the Program for Changjiang Scholars and Innovative Research Team in University (No. IRT0713). NR 26 TC 17 Z9 17 U1 10 U2 45 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 23 PY 2014 VL 104 IS 25 AR 252404 DI 10.1063/1.4885094 PG 4 WC Physics, Applied SC Physics GA AK6CQ UT WOS:000338515900056 ER PT J AU Alam, A Johnson, DD AF Alam, Aftab Johnson, D. D. TI Mixed valency and site-preference chemistry for cerium and its compounds: A predictive density-functional theory study SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; CE; TRANSITION; SYSTEMS AB Cerium and its technologically relevant compounds are examples of anomalous mixed valency, originating from two competing oxidation states-itinerant Ce4+ and localized Ce3+. Under applied stress, anomalous transitions are observed but not well understood. Here we treat mixed valency as an "alloy" problem involving two valences with competing and numerous site-occupancy configurations. We use density-functional theory with Hubbard U (i.e., DFT+U) to evaluate the effective valence and predict properties, including controlling the valence by pseudoternary alloying. For Ce and its compounds, such as (Ce, La)(2)(Fe,Co)(14)B permanent magnets, we find a stable mixed-valent alpha state near the spectroscopic value of nu(s) = 3.53. Ce valency in compounds depends on its steric volume and local chemistry. For La doping, Ce valency shifts towards gamma-like Ce3+, as expected from steric volume; for Co doping, valency depends on local Ce-site chemistry and steric volume. Our approach captures the key origins of anomalous valency and site-preference chemistry in complex compounds. C1 [Alam, Aftab] Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. [Johnson, D. D.] US DOE, Ames Lab, Ames, IA 50011 USA. [Johnson, D. D.] Iowa State Univ, Ames, IA 50011 USA. RP Alam, A (reprint author), Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. EM aftab@phy.iitb.ac.in; ddj@ameslab.gov OI Johnson, Duane/0000-0003-0794-7283 FU US Department of Energy (DOE) ARPA-E REACT [0472-1526]; Office of Basic Energy Sciences in our Division of Materials Science and Engineering; US DOE by Iowa State University [DE-AC02-07CH11358] FX Work at Ames Laboratory was supported by the US Department of Energy (DOE) ARPA-E REACT Program (Contract No. 0472-1526), using capabilities maintained and supported by the Office of Basic Energy Sciences in our Division of Materials Science and Engineering. The Ames Laboratory is operated for the US DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 20 TC 10 Z9 10 U1 7 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 23 PY 2014 VL 89 IS 23 AR 235126 DI 10.1103/PhysRevB.89.235126 PG 4 WC Physics, Condensed Matter SC Physics GA AK6CU UT WOS:000338516300004 ER PT J AU Hall, LJ Nomura, Y Shirai, S AF Hall, Lawrence J. Nomura, Yasunori Shirai, Satoshi TI Grand unification, axion, and inflation in Intermediate Scale Supersymmetry SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID DARK-MATTER; ISOCURVATURE PERTURBATIONS; COSMOLOGICAL CONSTANT; ANOMALY MEDIATION; PARTICLE PHYSICS; DOMAIN-WALLS; SUPERGRAVITY; BREAKING; MODELS; LHC AB A class of supersymmetric grand unified theories is introduced that has a single scale below the cutoff, that of the supersymmetry breaking masses (m) over tiled. For a wide range of the dimensionless parameters, agreement with the observed mass of the Higgs boson determines (m) over tiled similar to 10(9) 10(13) GeV, yielding Intermediate Scale Supersymmetry. We show that within this framework it is possible for seesaw neutrino masses, axions, and inflation to be described by the scale (m) over tiled, offering the possibility of a unified origin of disparate phenomena. Neutrino masses allowing for thermal leptogenesis can be obtained, and the axion decay constant lies naturally in the range f(a) similar to 10(9)-10(11) GeV, consistent with a recent observational suggestion of high scale inflation. A minimal SU(5) model is presented that illustrates these features. In this model, the only states at the grand unified scale are those of the heavy gauge supermultiplet. The grand unified partners of the Higgs doublets have a mass of order (m) tiled, leading to the dominant proton decay mode p -> (nu) over tiled K+, which may be probed in upcoming experiments. Dark matter may be winos, with mass environmentally selected to the TeV scale, and/or axions. Gauge coupling unification is found to be successful, especially if the wino is at the TeV scale. C1 [Hall, Lawrence J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Hall, LJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM ljhall@lbl.gov; ynomura@berkeley.edu; shirai@berkeley.edu OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-0855653, PHY-1214644] FX This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy under Contract DE-AC02-05CH11231 and in part by the National Science Foundation under grants PHY-0855653 and PHY-1214644. NR 78 TC 13 Z9 13 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 23 PY 2014 IS 6 AR 137 DI 10.1007/JHEP06(2014)137 PG 27 WC Physics, Particles & Fields SC Physics GA AK6HX UT WOS:000338529800001 ER PT J AU Ke, X Peng, J Tian, W Hong, T Zhu, M Mao, ZQ AF Ke, X. Peng, J. Tian, W. Hong, Tao Zhu, M. Mao, Z. Q. TI Commensurate-incommensurate magnetic phase transition in the Fe-doped bilayer ruthenate Ca3Ru2O7 SO PHYSICAL REVIEW B LA English DT Article ID METAL; INSULATOR; CRYSTAL; CA2RUO4; LATTICE; COPPER AB Neutron diffraction studies have revealed an uncommon commensurate-incommensurate magnetic phase transition with decreasing temperature in the (similar to 5%) Fe-doped bilayer ruthenate Ca-3(Ru,Fe)(2)O-7. An incommensurate phase formed of a cycloidal spiral spin structure coexists with a commensurate one below the phase transition at 42 K and persists down to the lowest temperature, accompanied by higher-order magnetic satellite peaks which indicate the formation of a magnetic soliton lattice. We ascribe these findings to the competing magnetic interactions in this system. This study demonstrates an effective approach to tune novel magnetic and electronic properties of ruthenates via 3d magnetic transition-metal substitution. C1 [Ke, X.; Zhu, M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Peng, J.; Mao, Z. Q.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. [Peng, J.] Nanjing Univ, Solid State Microstruct Lab, Nanjing 210093, Jiangsu, Peoples R China. [Peng, J.] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Tian, W.; Hong, Tao] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Ke, X (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM ke@pa.msu.edu RI Hong, Tao/F-8166-2010; Tian, Wei/C-8604-2013 OI Hong, Tao/0000-0002-0161-8588; Tian, Wei/0000-0001-7735-3187 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; NSF [DMR-1205469]; National Science Foundation of China (NNSFC) [11304149]; start-up funds at Michigan State University FX X.K. acknowledges the support from the start-up funds at Michigan State University. Research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Work at Tulane is supported by the NSF under Grant No. DMR-1205469. J.P. also acknowledges the support from the National Science Foundation of China (NNSFC) under Grant No. 11304149. NR 28 TC 3 Z9 3 U1 5 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 23 PY 2014 VL 89 IS 22 AR 220407 DI 10.1103/PhysRevB.89.220407 PG 5 WC Physics, Condensed Matter SC Physics GA AK6CS UT WOS:000338516100002 ER PT J AU Lei, SM Eliseev, EA Morozovska, AN Haislmaier, RC Lummen, TTA Cao, W Kalinin, SV Gopalan, V AF Lei, Shiming Eliseev, Eugene A. Morozovska, Anna N. Haislmaier, Ryan C. Lummen, Tom T. A. Cao, W. Kalinin, Sergei V. Gopalan, Venkatraman TI Comment on 'Origin of piezoelectric response under a biased scanning probe microscopy tip across a 180 degrees ferroelectric domain wall' Reply SO PHYSICAL REVIEW B LA English DT Editorial Material ID PIEZORESPONSE FORCE MICROSCOPY; RECONSTRUCTION; POLARIZATION AB In response to the preceding Comment of Jungk et al. [Phys. Rev. B 89, 226101 (2014)] regarding the validity of our finite element method (FEM) modeling in quantitatively predicting the piezoelectric response behavior in piezoresponse force microscopy (PFM), particularly the lateral response, we present here our latest experiment results that show quantitative agreement between FEM predictions and experiments. An approach to decouple the vertical PFM signal into cantilever vertical deflection and buckling contribution is proposed. Combined with simultaneously obtained lateral PFM, we show the possibility of performing quantitative three-dimensional PFM measurements (two lateral and one vertical response) from one single PFM image. A method to perform background subtraction for lateral signals is now presented that eliminates the spurious background issues seen in the past experimental works cited previously by Lei et al. [Phys. Rev. B 86, 134115 (2012)], as well as in the new results presented in the Comment of Jungk et al. The quantitative agreement between experiments and FEM then becomes clear with such a subtraction scheme. C1 [Lei, Shiming; Cao, W.] Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Harbin 150080, Peoples R China. [Lei, Shiming; Cao, W.] Harbin Inst Technol, Dept Phys, Harbin 150080, Peoples R China. [Lei, Shiming; Haislmaier, Ryan C.; Lummen, Tom T. A.; Cao, W.; Gopalan, Venkatraman] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Lei, Shiming; Haislmaier, Ryan C.; Lummen, Tom T. A.; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Eliseev, Eugene A.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Cao, W.] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Lei, SM (reprint author), Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Harbin 150080, Peoples R China. EM dzk@psu.edu; vxg8@psu.edu RI Cao, Wenwu/F-6091-2012; Kalinin, Sergei/I-9096-2012 OI Cao, Wenwu/0000-0002-2447-1486; Kalinin, Sergei/0000-0001-5354-6152 NR 30 TC 3 Z9 3 U1 3 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 23 PY 2014 VL 89 IS 22 AR 226102 DI 10.1103/PhysRevB.89.226102 PG 6 WC Physics, Condensed Matter SC Physics GA AK6CS UT WOS:000338516100011 ER PT J AU Adriani, O Berti, E Bonechi, L Bongi, M Castellini, G D'Alessandro, R Del Prete, M Haguenauer, M Itow, Y Kasahara, K Kawade, K Makino, Y Masuda, K Matsubayashi, E Menjo, H Mitsuka, G Muraki, Y Papini, P Perrot, AL Pfeiffer, D Ricciarini, S Sako, T Sakurai, N Suzuki, T Tamura, T Tiberio, A Torii, S Tricomi, A Turner, WC AF Adriani, O. Berti, E. Bonechi, L. Bongi, M. Castellini, G. D'Alessandro, R. Del Prete, M. Haguenauer, M. Itow, Y. Kasahara, K. Kawade, K. Makino, Y. Masuda, K. Matsubayashi, E. Menjo, H. Mitsuka, G. Muraki, Y. Papini, P. Perrot, A. -L. Pfeiffer, D. Ricciarini, S. Sako, T. Sakurai, N. Suzuki, T. Tamura, T. Tiberio, A. Torii, S. Tricomi, A. Turner, W. C. CA LHCf Collaboration TI Transverse-momentum distribution and nuclear modification factor for neutral pions in the forward-rapidity region in proton-lead collisions at root(NN)-N-S=5.02 TeV SO PHYSICAL REVIEW C LA English DT Article ID HIGH-ENERGY SCATTERING; HADRONS; HERA; LHC AB The transverse momentum (p(T)) distribution for inclusive neutral pions in the very forward rapidity region has been measured, with the Large Hadron Collider forward detector (LHCf), in proton-lead collisions at nucleon-nucleon center-of-mass energies of v sNN = 5.02 TeV at the LHC. The pT spectra obtained in the rapidity range -11.0 < ylab < -8.9 and 0 < pT < 0.6 GeV (in the detector reference frame) show a strong suppression of the production of neutral pions after taking into account ultraperipheral collisions. This leads to a nuclear modification factor value, relative to the interpolated pT spectra in proton-proton collisions at v s = 5.02 TeV, of about 0.1-0.4. This value is compared with the predictions of several hadronic interaction Monte Carlo simulations. C1 [Adriani, O.; Berti, E.; Bonechi, L.; Bongi, M.; Castellini, G.; D'Alessandro, R.; Del Prete, M.; Papini, P.; Ricciarini, S.; Tiberio, A.] Ist Nazl Fis Nucl, Sect Florence, I-50125 Florence, Italy. [Adriani, O.; Berti, E.; Bongi, M.; D'Alessandro, R.; Del Prete, M.; Mitsuka, G.; Tiberio, A.] Univ Florence, Florence, Italy. [Castellini, G.; Ricciarini, S.] CNR, IFAC, Florence, Italy. [Haguenauer, M.] Ecole Polytech, Palaiseau, France. [Itow, Y.; Kawade, K.; Makino, Y.; Masuda, K.; Matsubayashi, E.; Mitsuka, G.; Muraki, Y.; Sako, T.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Itow, Y.; Sako, T.; Sakurai, N.] Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univers, Nagoya, Aichi 4648601, Japan. [Kasahara, K.; Suzuki, T.; Torii, S.] Waseda Univ, RISE, Shinjuku Ku, Tokyo, Japan. [Menjo, H.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Perrot, A. -L.; Pfeiffer, D.] CERN, Geneva, Switzerland. [Tamura, T.] Kanagawa Univ, Yokohama, Kanagawa, Japan. [Tricomi, A.] Ist Nazl Fis Nucl, Sect Catania, I-95129 Catania, Italy. [Tricomi, A.] Univ Catania, Catania, Italy. [Turner, W. C.] LBNL, Berkeley, CA USA. RP Adriani, O (reprint author), Ist Nazl Fis Nucl, Sect Florence, I-50125 Florence, Italy. RI Sakurai, Nobuyuki/M-5009-2014; D'Alessandro, Raffaello/F-5897-2015; Bongi, Massimo/L-9417-2015; OI Tricomi, Alessia Rita/0000-0002-5071-5501; Papini, Paolo/0000-0003-4718-2895; Sakurai, Nobuyuki/0000-0002-1002-217X; D'Alessandro, Raffaello/0000-0001-7997-0306; Bongi, Massimo/0000-0002-6050-1937; Ricciarini, Sergio Bruno/0000-0001-6176-3368; Castellini, Guido/0000-0002-0177-0643 FU MEXT of Japan; JSPS Postdoctoral Fellowship for Research Abroad; MEXT; Istituto Nazionale di Fisica Nucleare (INFN) in Italy FX We thank the CERN staff and the ATLAS Collaboration for their essential contributions to the successful operation of LHCf. This work is partly supported by a Grant-in-Aid for Scientific research by MEXT of Japan, a Grant-in-Aid for a JSPS Postdoctoral Fellowship for Research Abroad, and a Grant-in-Aid for Nagoya University GCOE "QFPU" from MEXT. This work is also supported by Istituto Nazionale di Fisica Nucleare (INFN) in Italy. A part of this work was performed using the computer resources provided by the Institute for the Cosmic-Ray Research (University of Tokyo), CERN, and CNAF (INFN). NR 40 TC 12 Z9 12 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 23 PY 2014 VL 89 IS 6 DI 10.1103/PhysRevC.89.065209 PG 12 WC Physics, Nuclear SC Physics GA AK6DB UT WOS:000338517100004 ER PT J AU Kashiwa, K Tanizaki, Y AF Kashiwa, Kouji Tanizaki, Yuya TI Phase structure of SU(3) gauge-Higgs unification models at finite temperature SO PHYSICAL REVIEW D LA English DT Article ID SYMMETRY-BREAKING; EXTRA DIMENSIONS; STANDARD MODEL; WEINBERG ANGLE AB Five-dimensional SU(3) gauge-Higgs unification models are studied at finite temperature in the warped extra dimension S-1/Z(2). In order to investigate the phase structure, we develop a technique to compute the one-loop effective potential with the nontrivial Polyakov loop phase and with the nontrivial Wilson line phase along the extra dimension. Effective potentials as functions of two gauge-field condensations are shown for several simple matter contents, including fundamental, sextet, and adjoint representational Dirac fermions. Possible extensions and applications of our formalism are also briefly discussed. C1 [Kashiwa, Kouji] Brookhaven Natl Lab, RIKEN BNL, Upton, NY 11973 USA. [Kashiwa, Kouji] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Tanizaki, Yuya] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Tanizaki, Yuya] RIKEN, Nishina Ctr, Theoret Res Div, Wako, Saitama 3510198, Japan. RP Kashiwa, K (reprint author), Brookhaven Natl Lab, RIKEN BNL, Upton, NY 11973 USA. EM kouji.kashiwa@yukawa.kyoto-u.ac.jp; yuya.tanizaki@riken.jp RI Tanizaki, Yuya/M-4301-2013 OI Tanizaki, Yuya/0000-0003-1283-1808 FU RIKEN; JSPS Research Fellowships for Young Scientists; JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation; Program for Leading Graduate Schools, MEXT, Japan FX The authors thank Kazunori Takenaga for useful discussion. K. K. is supported by the RIKEN special postdoctoral researchers program and by JSPS Research Fellowships for Young Scientists. Y.T. is supported by JSPS Research Fellowships for Young Scientists. This work was partially supported by the JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation and by the Program for Leading Graduate Schools, MEXT, Japan. NR 27 TC 0 Z9 0 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 23 PY 2014 VL 89 IS 11 AR 116013 DI 10.1103/PhysRevD.89.116013 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK6DE UT WOS:000338517500002 ER PT J AU Rodriguez-Velamazan, JA Fabelo, O Beavers, CM Natividad, E Evangelisti, M Roubeau, O AF Alberto Rodriguez-Velamazan, J. Fabelo, Oscar Beavers, Christine M. Natividad, Eva Evangelisti, Marco Roubeau, Olivier TI A Multifunctional Magnetic Material under Pressure SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE magnetic properties; neutron diffraction; pressure effects; spin crossover; X-ray diffraction ID SPIN-CROSSOVER COMPLEX; COORDINATION POLYMERS; POWDER DIFFRACTION; ROOM-TEMPERATURE; TRANSITION; COEXISTENCE; FRAMEWORK; COMPOUND; CRYSTAL; DESIGN AB Fe-II(Metz)(6)]((FeBr4)-Br-III)(2) (Metz= 1-methyltetrazole) is one of the rare systems combining spin-crossover and long-range magnetic ordering. A joint neutron and X-ray diffraction and magnetometry study allows determining its collinear antiferromagnetic structure, and shows an increase of the Neel temperature from 2.4 K at ambient pressure, to 3.9 K at 0.95 GPa. Applied pressure also enables a full high-spin to low-spin switch at ambient temperature. C1 [Alberto Rodriguez-Velamazan, J.; Fabelo, Oscar; Natividad, Eva; Evangelisti, Marco; Roubeau, Olivier] CSIC, Inst Ciencia Mat Aragon ICMA, E-50009 Zaragoza, Spain. [Alberto Rodriguez-Velamazan, J.; Fabelo, Oscar; Natividad, Eva; Evangelisti, Marco; Roubeau, Olivier] Univ Zaragoza, E-50009 Zaragoza, Spain. [Alberto Rodriguez-Velamazan, J.; Fabelo, Oscar] Inst Max Von Laue Paul Langevin, F-38042 Grenoble, France. [Beavers, Christine M.] Berkeley Lab, Berkeley, CA 94720 USA. RP Rodriguez-Velamazan, JA (reprint author), CSIC, Inst Ciencia Mat Aragon ICMA, Plaza San Francisco, E-50009 Zaragoza, Spain. EM jarv@unizar.es; roubeau@unizar.es RI Beavers, Christine/C-3539-2009; Evangelisti, Marco/B-5878-2011; RODRIGUEZ-VELAMAZAN, Jose Alberto/E-7679-2012; Roubeau, Olivier/A-6839-2010; Natividad, Eva/C-7910-2015 OI Beavers, Christine/0000-0001-8653-5513; Evangelisti, Marco/0000-0002-8028-9064; RODRIGUEZ-VELAMAZAN, Jose Alberto/0000-0002-8505-5232; Roubeau, Olivier/0000-0003-2095-5843; Natividad, Eva/0000-0003-2553-0633 FU Spanish MINECO; FEDER [MAT2011-24284, MAT2011-27233-C02-02, MAT2012-38318-C03-01]; Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy [DE-AC02-05CH11231]; COMPRES, the Consortium for Materials Properties Research in Earth Sciences, under NSF [EAR 11-57758] FX This work was supported by the Spanish MINECO and FEDER, projects MAT2011-24284, MAT2011-27233-C02-02 and MAT2012-38318-C03-01. We are grateful to the Spanish CRG D1B and Institut Laue-Langevin for neutron beam time allocation. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy under contract no. DE-AC02-05CH11231. High pressure facilities at the Advanced Light Source are partially supported by COMPRES, the Consortium for Materials Properties Research in Earth Sciences, under NSF Cooperative Agreement EAR 11-57758. NR 67 TC 4 Z9 4 U1 4 U2 44 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUN 23 PY 2014 VL 20 IS 26 BP 7956 EP 7961 DI 10.1002/chem.201402046 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5RD UT WOS:000337742600016 PM 24807735 ER PT J AU Clausen, HF Jorgensen, MRV Cenedese, S Schmokel, MS Christensen, M Chen, YS Koutsantonis, G Overgaard, J Spackman, MA Iversen, BB AF Clausen, Henrik F. Jorgensen, Mads R. V. Cenedese, Simone Schmokel, Mette S. Christensen, Mogens Chen, Yu-Sheng Koutsantonis, George Overgaard, Jacob Spackman, Mark A. Iversen, Bo B. TI Host Perturbation in a beta-Hydroquinone Clathrate Studied by Combined X-ray/Neutron Charge-Density Analysis: Implications for Molecular Inclusion in Supramolecular Entities SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE clathrates; host-guest systems; neutron diffraction; supramolecular chemistry; X-ray diffraction ID EXPERIMENTAL ELECTRON-DENSITY; THEORETICAL DATA-BANK; CRYSTAL-STRUCTURE; FORCE-FIELD; NEUTRON-DIFFRACTION; ASPHERICAL ATOMS; AMINO-ACID; RAY; QUINOL; PARAMETERS AB X-ray/neutron (X/N) diffraction data measured at very low temperature (15 K) in conjunction with ab initio theoretical calculations were used to model the crystal charge density (CD) of the host-guest complex of hydroquinone (HQ) and acetonitrile. Due to pseudosymmetry, information about the ordering of the acetonitrile molecules within the HQ cavities is present only in almost extinct, very weak diffraction data, which cannot be measured with sufficient accuracy even by using the brightest X-ray and neutron sources available, and the CD model of the guest molecule was ultimately based on theoretical calculations. On the other hand, the CD of the HQ host structure is well determined by the experimental data. The neutron diffraction data provide hydrogen anisotropic thermal parameters and positions, which are important to obtain a reliable CD for this light-atom-only crystal. Atomic displacement parameters obtained independently from the X-ray and neutron diffraction data show excellent agreement with a vertical bar Delta U vertical bar value of 0.00058 angstrom(2) indicating outstanding data quality. The CD and especially the derived electrostatic properties clearly reveal increased polarization of the HQ molecules in the host-guest complex compared with the HQ molecules in the empty HQ apohost crystal structure. It was found that the origin of the increased polarization is inclusion of the acetonitrile molecule, whereas the change in geometry of the HQ host structure following inclusion of the guest has very little effect on the electrostatic potential. The fact that guest inclusion has a profound effect on the electrostatic potential suggests that nonpolarizable force fields may be unsuitable for molecular dynamics simulations of host-guest interaction (e. g., in protein-drug complexes), at least for polar molecules. C1 [Clausen, Henrik F.; Jorgensen, Mads R. V.; Schmokel, Mette S.; Christensen, Mogens; Overgaard, Jacob; Iversen, Bo B.] Aarhus Univ, Ctr Mat Crystallog, Dept Chem, DK-8000 Aarhus C, Denmark. [Clausen, Henrik F.; Jorgensen, Mads R. V.; Schmokel, Mette S.; Christensen, Mogens; Overgaard, Jacob; Iversen, Bo B.] Aarhus Univ, iNANO, DK-8000 Aarhus C, Denmark. [Cenedese, Simone] Univ Milan, CNR, ISTM, I-20122 Milan, Italy. [Cenedese, Simone] Univ Milan, Dipartimento Chim Fis & Elettrochim, I-20122 Milan, Italy. [Chen, Yu-Sheng] Univ Chicago, Adv Photon Source, ChemMatCARS, Chicago, IL 60637 USA. [Koutsantonis, George; Spackman, Mark A.] Univ Western Australia, Sch Chem & Biochem, Nedlands, WA 6009, Australia. RP Overgaard, J (reprint author), Aarhus Univ, Ctr Mat Crystallog, Dept Chem, DK-8000 Aarhus C, Denmark. EM jacobo@chem.au.dk; mark.spackman@uwa.edu.au; bo@chem.au.dk RI Spackman, Mark/D-1197-2010; Koutsantonis, George/G-1710-2011; Jorgensen, Mads Ry Vogel/C-6109-2017 OI Spackman, Mark/0000-0003-1521-2041; Koutsantonis, George/0000-0001-8755-3596; Jorgensen, Mads Ry Vogel/0000-0001-5507-9615 FU Danish National Research Foundation (Center for Materials Crystallography) [DNRF-93]; Danish Research Council for Nature and Universe (Danscatt); Australian Research Council [DP0879405, DP130103304]; National Science Foundation Department of Energy [NSF/CHE-0822838]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Danish National Research Foundation (Center for Materials Crystallography, DNRF-93), the Danish Research Council for Nature and Universe (Danscatt) and the Australian Research Council (DP0879405 and DP130103304). ChemMatCARS Sector 15 is principally supported by the National Science Foundation Department of Energy under grant number NSF/CHE-0822838. Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We would like to acknowledge the instrument time obtained at D19 at the ILL. NR 70 TC 3 Z9 3 U1 1 U2 18 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUN 23 PY 2014 VL 20 IS 26 BP 8089 EP 8098 DI 10.1002/chem.201400129 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5RD UT WOS:000337742600029 PM 24828367 ER PT J AU Harley, SJ Glascoe, EA Lewicki, JP Maxwell, RS AF Harley, Stephen J. Glascoe, Elizabeth A. Lewicki, James P. Maxwell, Robert S. TI Advances in Modeling Sorption and Diffusion of Moisture in Porous Reactive Materials SO CHEMPHYSCHEM LA English DT Article DE computational chemistry; diffusion; silicon; sorption; water chemistry ID WATER-VAPOR SORPTION; SULFONATED POLYIMIDE MEMBRANES; GROUNDWATER; COMPOSITES; ELASTOMER; FILLERS AB Water-vapor-uptake experiments were performed on a silicafilled poly(dimethylsiloxane) (PDMS) network and modeled by using two different approaches. The data was modeled by using established methods and the model parameters were used to predict moisture uptake in a sample. The predictions are reasonably good, but not outstanding; many of the shortcomings of the modeling are discussed. A high-fidelity modeling approach is derived and used to improve the modeling of moisture uptake and diffusion. Our modeling approach captures the physics and kinetics of diffusion and adsorption/desorption, simultaneously. It predicts uptake better than the established method; more importantly, it is also able to predict outgassing. The material used for these studies is a filled-PDMS network; physical interpretations concerning the sorption and diffusion of moisture in this network are discussed. C1 [Harley, Stephen J.; Glascoe, Elizabeth A.; Lewicki, James P.; Maxwell, Robert S.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Harley, SJ (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, 7000 East Ave, Livermore, CA 94550 USA. EM harley2@llnl.gov FU Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344, LLNL-JRNL-641873] FX The authors would like to thank Dr. Tom Wilson for helpful discussions involving polymer synthesis. The authors would also like to thank Dr. Yunwei Sun for his assistance in developing a reactive transport code. This work was performed by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344, LLNL-JRNL-641873. NR 23 TC 2 Z9 2 U1 3 U2 22 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1439-4235 EI 1439-7641 J9 CHEMPHYSCHEM JI ChemPhysChem PD JUN 23 PY 2014 VL 15 IS 9 BP 1809 EP 1820 DI 10.1002/cphc.201301097 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ9FI UT WOS:000338012700011 PM 24819028 ER PT J AU Bettencourt, LMA Samaniego, H Youn, H AF Bettencourt, Luis M. A. Samaniego, Horacio Youn, Hyejin TI Professional diversity and the productivity of cities SO SCIENTIFIC REPORTS LA English DT Article ID CITY SIZE; GROWTH; COMPLEXITY; LABOR AB Attempts to understand the relationship between diversity, productivity and scale have remained limited due to the scheme-dependent nature of the taxonomies describing complex systems. We analyze the diversity of US metropolitan areas in terms of profession diversity and employment to show how this frequency distribution takes a universal scale-invariant form, common to all cities, in the limit of infinite resolution of occupational taxonomies. We show that this limit is obtained under general conditions that follow from the analysis of the variation of the occupational frequency across taxonomies at different resolutions in a way analogous to finite-size scaling in statistical physical systems. We propose a theoretical framework that derives the form and parameters of the limiting distribution of professions based on the appearance, in urban social networks, of new occupations as the result of specialization and coordination of labor. By deriving classification scheme-independent measures of functional diversity and modeling cities as social networks embedded in infrastructural space, these results show how standard economic arguments of division and coordination of labor can be articulated in detail in cities and provide a microscopic basis for explaining increasing returns to population scale observed at the level of entire metropolitan areas. C1 [Bettencourt, Luis M. A.; Youn, Hyejin] Santa Fe Inst, Santa Fe, NM 87501 USA. [Samaniego, Horacio] Los Alamos Natl Lab, Ctr Non Linear Studies, Theoret Div MS B284, Los Alamos, NM 87545 USA. [Samaniego, Horacio] Univ Austral Chile, Inst Conservac Biodiversidad & Terr, Valdivia, Chile. [Youn, Hyejin] Oxford Martin Sch, Inst New Econ Thinking, Oxford OX2 6ED, England. [Youn, Hyejin] Univ Oxford, Math Inst, Oxford OX2 6GG, England. RP Samaniego, H (reprint author), Santa Fe Inst, 1399 Hyde Pk Rd, Santa Fe, NM 87501 USA. EM horacio@ecoinformatica.cl OI Youn, Hyejin/0000-0002-6190-4412 FU Rockefeller Foundation [2011 SRC 108]; James S. McDonnell Foundation [220020195]; John Templeton Foundation [15705]; Army Research Office Minerva Program [W911NF1210097]; Bill and Melinda Gates Foundation [OPP1076282]; U.S. Department of Energy through the LANL/LDRD Program [DE-AC52-06NA25396]; FONDEF [D10I1038] FX We thank Doug Erwin, Ricardo Hausmann, Cesar Hidalgo, Jose Lobo and Geoffrey West for discussions. This research was partially supported by the Rockefeller Foundation (grant no. 2011 SRC 108), the James S. McDonnell Foundation (grant no. 220020195), the John Templeton Foundation (grant no. 15705), the Army Research Office Minerva Program (grant no. W911NF1210097), the Bill and Melinda Gates Foundation (grant OPP1076282), the U.S. Department of Energy through the LANL/LDRD Program (contract no. DE-AC52-06NA25396), and a FONDEF grant (D10I1038). NR 45 TC 6 Z9 6 U1 2 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 23 PY 2014 VL 4 AR 5393 DI 10.1038/srep05393 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7PM UT WOS:000337888600007 PM 24953448 ER PT J AU Wang, YY Sun, X Wang, YD Hu, XH Zbib, HM AF Wang, Y. Y. Sun, X. Wang, Y. D. Hu, X. H. Zbib, H. M. TI A mechanism-based model for deformation twinning in polycrystalline FCC steel SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Deformation twinning; Pseudo-slip; Crystal plasticity model; Finite element model; Shear bands; Strain localization ID CRYSTALLOGRAPHIC TEXTURE EVOLUTION; INDUCED PLASTICITY STEELS; FINITE-ELEMENT MODEL; CRYSTAL PLASTICITY; SINGLE-CRYSTALS; SHEAR BANDS; TWIP-STEEL; ORIENTATION DEPENDENCE; HARDENING MECHANISMS; FAILURE MODES AB Deformation twinning, a common and important plastic deformation mechanism, is the key contributor to the excellent combination of strength and ductility in twinning-induced plasticity (TWIP) steel. In the open literature, a significant amount of research has been reported on the microstructural characteristics of deformation twinning and its influence on the overall deformation behavior of TWIP steel. In this study, we examine the feasibility of a mechanism-based crystal plasticity model in simulating the microstructural level deformation characteristics of TWIP steel. To this end, a model considering both double-slip and double-twin is developed to investigate the stress-strain behavior and local microstructural features related to the formation and growth of micro-twins in low stacking fault energy (SFE) TWIP steel. The twin systems are described as pseudo-slips that can be activated when their resolved shear stress reaches the corresponding critical value. A hardening law that accounts for the interaction among the slip and twin systems is also developed. Numerical simulations for different mesh sizes and single crystal patch tests under different loading modes are carried out to verify the modeling procedure. Our simulation results reveal that, despite its simple nature, the double-slip/double-twin model can capture the key deformation features of TWIP steel, including twin volume fraction evolution, continuous strain hardening, and the final fracture in the form of strain localization. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, Y. Y.; Wang, Y. D.] Northeastern Univ, Key Lab Anisotropy & Texture Mat, Shenyang 110819, Peoples R China. [Wang, Y. Y.; Sun, X.; Hu, X. H.] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. [Wang, Y. D.] Univ Sci & Technol, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Zbib, H. M.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Sun, X (reprint author), Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. EM xin.sun@pnnl.gov RI wang, yandong/G-9404-2013; Hu, Xiaohua/J-6519-2012 OI Hu, Xiaohua/0000-0002-7735-5091 FU U.S. Department of Energy (DOE) [DE-ACO5-76RL01830]; DOE's Vehicle Technologies Office under the Automotive Lightweighting Materials Program; National Science Foundation of China [51231002]; Fundamental Research Funds for the Central Universities [06111020]; China Scholarship Council; National Priorities Research Program from the Qatar National Research Fund [NPRP 05-1294-2-559] FX Pacific Northwest National Laboratory is operated by the Battelle for the U.S. Department of Energy (DOE) under Contract no. DE-ACO5-76RL01830. This work was funded by DOE's Vehicle Technologies Office under the Automotive Lightweighting Materials Program managed by Mr. William Joost, the National Science Foundation of China (Grant no. 51231002) and the Fundamental Research Funds for the Central Universities (Grant no. 06111020). Y.Y. Wang would like to acknowledge scholarship support from the China Scholarship Council. H.M. Zbib acknowledges that his contribution to this publication was made possible by a National Priorities Research Program grant (No. NPRP 05-1294-2-559) from the Qatar National Research Fund (a member of the Qatar Foundation). The statements made herein are the sole responsibility of the authors. NR 62 TC 3 Z9 3 U1 3 U2 32 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JUN 23 PY 2014 VL 607 BP 206 EP 218 DI 10.1016/j.msea.2014.04.010 PG 13 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AJ4KB UT WOS:000337644000026 ER PT J AU Detert, DM Tom, KB Battaglia, C Denlinger, JD Lim, SHN Javey, A Anders, A Dubon, OD Yu, KM Walukiewicz, W AF Detert, Douglas M. Tom, Kyle B. Battaglia, Corsin Denlinger, Jonathan D. Lim, Sunnie H. N. Javey, Ali Anders, Andre Dubon, Oscar D. Yu, Kin M. Walukiewicz, Wladek TI Fermi level stabilization and band edge energies in CdxZn1-xO alloys SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ELECTRONIC-STRUCTURE; SEMICONDUCTORS; FILMS; CDO AB We have measured the band edge energies of CdxZn1-xO thin films as a function of composition by three independent techniques: we determine the Fermi level stabilization energy by pinning the Fermi level with ion irradiation, measure the binding energy of valence band states and core levels by X-ray photoelectron spectroscopy, and probe shifts in the conduction band and valence band density of states using soft X-ray absorption and emission spectroscopy, respectively. The three techniques find consensus in explaining the origin of compositional trends in the optical-bandgap narrowing upon Cd incorporation in wurtzite ZnO and widening upon Zn incorporation in rocksalt CdO. The conduction band minimum is found to be stationary for both wurtzite and rocksalt alloys, and a significant upward rise of the valence band maximum accounts for the majority of these observed bandgap changes. Given these band alignments, alloy disorder scattering is found to play a negligible role in decreasing the electron mobility for all alloys. These band alignment details, combined with the unique optical and electrical properties of the two phase regimes, make CdZnO alloys attractive candidates for photoelectrochemical water splitting applications. (C) 2014 AIP Publishing LLC. C1 [Detert, Douglas M.; Tom, Kyle B.; Battaglia, Corsin; Javey, Ali; Dubon, Oscar D.; Yu, Kin M.; Walukiewicz, Wladek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Detert, Douglas M.; Tom, Kyle B.; Dubon, Oscar D.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Battaglia, Corsin; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Denlinger, Jonathan D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lim, Sunnie H. N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Anders, Andre] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. RP Detert, DM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RI Javey, Ali/B-4818-2013; Battaglia, Corsin/B-2917-2010; Anders, Andre/B-8580-2009; OI Anders, Andre/0000-0002-5313-6505; Yu, Kin Man/0000-0003-1350-9642 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work, carried out at LBNL in the Materials Sciences Division and at the Advanced Light Source, was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors would like to thank Jeffrey Beeman for his help with irradiation experiments and Alexander Luce for his help with XAS/SXE experiments. NR 27 TC 8 Z9 8 U1 4 U2 51 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 21 PY 2014 VL 115 IS 23 AR 233708 DI 10.1063/1.4884683 PG 6 WC Physics, Applied SC Physics GA AK0MB UT WOS:000338106000033 ER PT J AU Golge, S Vlahovic, B Wojtsekhowski, B AF Golge, S. Vlahovic, B. Wojtsekhowski, B. TI High-intensity positron microprobe at the Thomas Jefferson National Accelerator Facility SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID AUGER-ELECTRON-SPECTROSCOPY; SOLID NEON MODERATOR; BRIGHTNESS ENHANCEMENT; BEAM; ANNIHILATION; CONDENSATION; PHYSICS; TARGET; LAB; CU AB We present a conceptual design for a novel continuous wave electron-linac based high-intensity high-brightness slow-positron production source with a projected intensity on the order of 10(10) e(+)/s. Reaching this intensity in our design relies on the transport of positrons (T+ below 600 keV) from the electron-positron pair production converter target to a low-radiation and low-temperature area for moderation in a high-efficiency cryogenic rare gas moderator, solid Ne. This design progressed through Monte Carlo optimizations of: electron/positron beam energies and converter target thickness, transport of the e(+) beam from the converter to the moderator, extraction of the e(+) beam from the magnetic channel, a synchronized raster system, and moderator efficiency calculations. For the extraction of e(+) from the magnetic channel, a magnetic field terminator plug prototype has been built and experimental results on the effectiveness of the prototype are presented. The dissipation of the heat away from the converter target and radiation protection measures are also discussed. (C) 2014 AIP Publishing LLC. C1 [Golge, S.; Vlahovic, B.] N Carolina Cent Univ, Durham, NC 27707 USA. [Wojtsekhowski, B.] Jefferson Lab, Newport News, VA 23606 USA. RP Golge, S (reprint author), N Carolina Cent Univ, Durham, NC 27707 USA. EM serkan.golge@nasa.gov FU NASA [NNX09AV07A]; NSF under CREST [HRD-0833184]; U.S. DOE [DE-AC05-06OR23177] FX We would like to thank staff members of the Center for Advanced Studies of Accelerators and Radiation Control Group at JLab, Dr. M. Tiefenback, Dr. B. Barbiellini, and Professor A. Mills for their helpful discussions and support. This work was supported by NASA under the award NNX09AV07A and by NSF under the CREST award HRD-0833184. Authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. The U. S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce this manuscript for U. S. Government purposes. NR 54 TC 1 Z9 1 U1 1 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 21 PY 2014 VL 115 IS 23 AR 234907 DI 10.1063/1.4884781 PG 10 WC Physics, Applied SC Physics GA AK0MB UT WOS:000338106000084 ER PT J AU Lohn, AJ Mickel, PR Marinella, MJ AF Lohn, Andrew J. Mickel, Patrick R. Marinella, Matthew J. TI Analytical estimations for thermal crosstalk, retention, and scaling limits in filamentary resistive memory SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TEMPERATURE; DEVICE; RRAM AB We discuss the thermal effects on scaling, retention, and error rate in filamentary resistive memories from a theoretical perspective using an analytical approach. Starting from the heat equation, we derive the temperature profile surrounding a resistive memory device and calculate its effect on neighboring devices. We outline the engineering tradeoffs that are expected with continued scaling, such as retention and power use per device. Based on our calculations, we expect scaling to continue well below 10 nm, but that the effect of heating from neighboring devices needs to be considered for some applications even at current manufacturing capabilities. We discuss possible designs to alleviate some of these effects while further increasing device density. (C) 2014 AIP Publishing LLC. C1 [Lohn, Andrew J.; Mickel, Patrick R.; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Lohn, AJ (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM drewlohn@gmail.com FU Sandia's Laboratory Directed Research and Development program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Thomas Beechem for helpful discussion of thermal interfaces. This work was funded by Sandia's Laboratory Directed Research and Development program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 26 TC 8 Z9 8 U1 2 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 21 PY 2014 VL 115 IS 23 AR 234507 DI 10.1063/1.4885045 PG 7 WC Physics, Applied SC Physics GA AK0MB UT WOS:000338106000075 ER PT J AU Tschopp, MA Gao, F Solanki, KN AF Tschopp, M. A. Gao, F. Solanki, K. N. TI Binding of HenV clusters to alpha-Fe grain boundaries SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HELIUM-VACANCY CLUSTERS; MOLECULAR-DYNAMICS; BCC IRON; DISPLACEMENT CASCADES; STRUCTURAL-MATERIALS; DEFECT PRODUCTION; TENSILE-STRENGTH; ENERGY; FUSION; IRRADIATION AB The objective of this research is to explore the formation/binding energetics and length scales associated with the interaction between HenV clusters and grain boundaries in bcc alpha-Fe. In this work, we calculated formation/binding energies for 1-8 He atoms in a monovacancy at all potential grain boundary (GB) sites within 15 angstrom of the ten grain boundaries selected (122106 simulations total). The present results provide detailed information about the interaction energies and length scales of 1-8 He atoms with grain boundaries for the structures examined. A number of interesting new findings emerge from the present study. First, the Sigma 3(112) "twin" GB has significantly lower binding energies for all HenV clusters than all other boundaries in this study. For all grain boundary sites, the effect of the local environment surrounding each site on the HenV formation and binding energies decreases with an increasing number of He atoms in the HenV cluster. Based on the calculated dataset, we formulated a model to capture the evolution of the formation and binding energy of HenV clusters as a function of distance from the GB center, utilizing only constants related to the maximum binding energy and the length scale. (C) 2014 AIP Publishing LLC. C1 [Tschopp, M. A.] US Army Res Lab, Aberdeen Proving Ground, MD 21005 USA. [Gao, F.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Solanki, K. N.] Arizona State Univ, Tempe, AZ 85287 USA. RP Tschopp, MA (reprint author), US Army Res Lab, Aberdeen Proving Ground, MD 21005 USA. EM mark.a.tschopp.civ@mail.mil RI Solanki, Kiran/E-8337-2010; OI Tschopp, Mark/0000-0001-8471-5035 FU U.S. Army Research Laboratory (ARL); U.S. Department of Energy, Office of Fusion Energy Science [DE-AC06-76RLO 1830]; Alternate Sponsored Fellowship (ASF) at PNNL FX This work was supported in part by the U.S. Army Research Laboratory (ARL). F. G. is grateful for the support by the U.S. Department of Energy, Office of Fusion Energy Science, under Contract DE-AC06-76RLO 1830. The authors would like to acknowledge the support and discussions with Dr. Xin Sun at Pacific Northwest National Laboratory. Last, the authors would like to acknowledge Ms. Joanna Sun, a high school student support by the Alternate Sponsored Fellowship (ASF) at PNNL, for her contributions to this work. NR 83 TC 5 Z9 5 U1 4 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 21 PY 2014 VL 115 IS 23 AR 233501 DI 10.1063/1.4883357 PG 15 WC Physics, Applied SC Physics GA AK0MB UT WOS:000338106000009 ER PT J AU Alexandrov, V Rosso, KM AF Alexandrov, Vitaly Rosso, Kevin M. TI Electron transport in pure and substituted iron oxyhydroxides by small-polaron migration SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; GOETHITE ALPHA-FEOOH; AB-INITIO; HEMATITE ALPHA-FE2O3; CRYSTAL-STRUCTURE; ATOM EXCHANGE; CHARGE-TRANSPORT; AQUEOUS FE(II); METAL-OXIDES; GAMMA-FEOOH AB Iron oxyhydroxides (FeOOH) are common crystalline forms of iron that play a critical role in technology and the natural environment via a variety of important reduction-oxidation reactions, including electrical semiconduction as an aspect. However, a basic understanding of the electron transport properties of these systems is still lacking. We examine the electron mobility in goethite (alpha-FeOOH), akaganeite (beta-FeOOH), and lepidocrocite (gamma-FeOOH) polymorphs by means of density functional theory based (DFT+U) calculations. We show that room temperature charge transport should be dominated by the small-polaron hopping type, and that the attendant mobility should be highest for pure goethite and akaganeite. Hopping pathways through the various lattices are discussed in terms of individual electron exchange steps and rates for each. Given the usual occurrence of compositional impurities in natural iron oxyhydroxides, we also investigate the effect of common stoichiometric defects on the electron hopping activation energies such as Al and Cr substitutional cations in goethite, and Cl anions in the channels of akaganeite. (C) 2014 AIP Publishing LLC. C1 [Alexandrov, Vitaly; Rosso, Kevin M.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. RP Alexandrov, V (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. EM vitali.alexandrov@pnnl.gov FU U.S. Department of Energy (DOE) Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Geosciences program at Pacific Northwest National Laboratory (PNNL); DOE Office of Biological and Environmental Research FX This research was supported by the U.S. Department of Energy (DOE) Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Geosciences program at Pacific Northwest National Laboratory (PNNL). The calculations were performed using PNNL Institutional Computing at Pacific Northwest National Laboratory and the Molecular Science Computing Facility in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a U.S. national user facility sponsored by the DOE Office of Biological and Environmental Research. The authors also wish to acknowledge Sebastien Kerisit for fruitful discussions. NR 66 TC 7 Z9 7 U1 10 U2 88 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234701 DI 10.1063/1.4882065 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200041 PM 24952554 ER PT J AU Lam, RK Shih, O Smith, JW Sheardy, AT Rizzuto, AM Prendergast, D Saykally, RJ AF Lam, Royce K. Shih, Orion Smith, Jacob W. Sheardy, Alex T. Rizzuto, Anthony M. Prendergast, David Saykally, Richard J. TI Electrokinetic detection for X-ray spectra of weakly interacting liquids: n-decane and n-nonane SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID AA FORCE-FIELD; HYDROGEN-BOND NETWORK; ELECTRONIC-STRUCTURE; AQUEOUS-SOLUTIONS; WATER MICROJETS; ABSORPTION SPECTROSCOPY; MOLECULAR SIMULATION; PHASE; HYDROCARBONS; GENERATION AB The introduction of liquid microjets into soft X-ray absorption spectroscopy enabled the windowless study of liquids by this powerful atom-selective high vacuum methodology. However, weakly interacting liquids produce large vapor backgrounds that strongly perturb the liquid signal. Consequently, solvents (e. g., hydrocarbons, ethers, ketones, etc.) and solutions of central importance in chemistry and biology have been inaccessible by this technology. Here we describe a new detection method, upstream detection, which greatly reduces the vapor phase contribution to the X-ray absorption signal while retaining important advantages of liquid microjet sample introduction (e. g., minimal radiation damage). The effectiveness of the upstream detection method is demonstrated in this first study of room temperature liquid hydrocarbons: n-nonane and n-decane. Good agreement with first principles' calculations indicates that the eXcited electron and Core Hole theory adequately describes the subtle interactions in these liquids that perturb the electronic structure of the unoccupied states probed in core-level experiments. (C) 2014 AIP Publishing LLC. C1 [Lam, Royce K.; Shih, Orion; Smith, Jacob W.; Sheardy, Alex T.; Rizzuto, Anthony M.; Saykally, Richard J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lam, Royce K.; Smith, Jacob W.; Sheardy, Alex T.; Rizzuto, Anthony M.; Saykally, Richard J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Saykally, RJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM saykally@berkeley.edu RI Foundry, Molecular/G-9968-2014; OI Lam, Royce/0000-0003-2878-038X FU Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) through LBNL Chemical Sciences Division [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, through LBNL Chemical Sciences Division. Computational resources were provided by the National Energy Research Scientific Computing Center (NERSC), a DOE Advanced Scientific Computing Research User Facility. The authors would also like to thank Wanli Yang and Jon Spear for beamline support at the Advanced Light Source. The data presented are available upon request to saykally@berkeley.edu. NR 55 TC 2 Z9 2 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234202 DI 10.1063/1.4882901 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200021 PM 24952534 ER PT J AU Li, LS Giokas, PG Kanai, Y Moran, AM AF Li, Lesheng Giokas, Paul G. Kanai, Yosuke Moran, Andrew M. TI Modeling time-coincident ultrafast electron transfer and solvation processes at molecule-semiconductor interfaces SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CHARGE-TRANSFER PROCESSES; SENSITIZED SOLAR-CELLS; TRANSFER DYNAMICS; LIOUVILLE-SPACE; DYE; OXIDE; TIO2; FILMS; PSEUDOPOTENTIALS; SPECTROSCOPY AB Kinetic models based on Fermi's Golden Rule are commonly employed to understand photoinduced electron transfer dynamics at molecule-semiconductor interfaces. Implicit in such second-order perturbative descriptions is the assumption that nuclear relaxation of the photoexcited electron donor is fast compared to electron injection into the semiconductor. This approximation breaks down in systems where electron transfer transitions occur on 100-fs time scale. Here, we present a fourth-order perturbative model that captures the interplay between time-coincident electron transfer and nuclear relaxation processes initiated by light absorption. The model consists of a fairly small number of parameters, which can be derived from standard spectroscopic measurements (e.g., linear absorbance, fluorescence) and/or first-principles electronic structure calculations. Insights provided by the model are illustrated for a two-level donor molecule coupled to both (i) a single acceptor level and (ii) a density of states (DOS) calculated for TiO2 using a first-principles electronic structure theory. These numerical calculations show that second-order kinetic theories fail to capture basic physical effects when the DOS exhibits narrow maxima near the energy of the molecular excited state. Overall, we conclude that the present fourth-order rate formula constitutes a rigorous and intuitive framework for understanding photoinduced electron transfer dynamics that occur on the 100-fs time scale. (C) 2014 AIP Publishing LLC. C1 [Li, Lesheng; Giokas, Paul G.; Kanai, Yosuke; Moran, Andrew M.] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. [Kanai, Yosuke] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. RP Kanai, Y (reprint author), Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA. EM ykanai@unc.edu; ammoran@email.unc.edu RI Yambo, MBPT Code/O-4564-2015; Kanai, Yosuke/B-5554-2016; OI Li, Lesheng/0000-0002-1601-8868 FU UNC Energy Frontier Research Center (EFRC) "Center for Solar Fuels," an EFRC by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001011] FX This work was wholly funded by the UNC Energy Frontier Research Center (EFRC) "Center for Solar Fuels," an EFRC funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001011, which supported L.L. and P.G. NR 55 TC 3 Z9 3 U1 2 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234109 DI 10.1063/1.4882664 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200012 PM 24952525 ER PT J AU Moore, SG Crozier, PS AF Moore, Stan G. Crozier, Paul S. TI Extension and evaluation of the multilevel summation method for fast long-range electrostatics calculations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID PARTICLE MESH EWALD; MOLECULAR-DYNAMICS SIMULATIONS; COULOMBIC SYSTEMS; SUMS; CHARGE; ALGORITHMS; EQUATIONS; WATER AB Several extensions and improvements have been made to the multilevel summation method (MSM) of computing long-range electrostatic interactions. These include pressure calculation, an improved error estimator, faster direct part calculation, extension to non-orthogonal (triclinic) systems, and parallelization using the domain decomposition method. MSM also allows fully non-periodic long-range electrostatics calculations which are not possible using traditional Ewald-based methods. In spite of these significant improvements to the MSM algorithm, the particle-particle particle-mesh (PPPM) method was still found to be faster for the periodic systems we tested on a single processor. However, the fast Fourier transforms (FFTs) that PPPM relies on represent a major scaling bottleneck for the method when running on many cores (because the many-to-many communication pattern of the FFT becomes expensive) and MSM scales better than PPPM when using a large core count for two test problems on Sandia's Redsky machine. This FFT bottleneck can be reduced by running PPPM on only a subset of the total processors. MSM is most competitive for relatively low accuracy calculations. On Sandia's Chama machine, however, PPPM is found to scale better than MSM for all core counts that we tested. These results suggest that PPPM is usually more efficient than MSM for typical problems running on current high performance computers. However, further improvements to MSM algorithm could increase its competitiveness for calculation of long-range electrostatic interactions. (C) 2014 AIP Publishing LLC. C1 [Moore, Stan G.; Crozier, Paul S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Moore, SG (reprint author), Sandia Natl Labs, POB 5800,MS 1322, Albuquerque, NM 87185 USA. EM stamoor@sandia.gov; pscrozi@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Stephen Bond and Steve Plimpton from Sandia National Laboratories. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 43 TC 2 Z9 2 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234112 DI 10.1063/1.4883695 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200015 PM 24952528 ER PT J AU Robichaud, DJ Scheer, AM Mukarakate, C Ormond, TK Buckingham, GT Ellison, GB Nimlos, MR AF Robichaud, David J. Scheer, Adam M. Mukarakate, Calvin Ormond, Thomas K. Buckingham, Grant T. Ellison, G. Barney Nimlos, Mark R. TI Unimolecular thermal decomposition of dimethoxybenzenes SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INFRARED-ABSORPTION SPECTRA; MASS-SPECTROMETRY; PHOTOIONIZATION MASS; SUBSTITUTED ANISOLES; CHEMICAL-REACTIONS; ORGANIC RADICALS; PHENYL ETHER; SHOCK-WAVES; PYROLYSIS; MECHANISMS AB The unimolecular thermal decomposition mechanisms of o-, m-, and p-dimethoxybenzene (CH3O-C6H4-OCH3) have been studied using a high temperature, microtubular (mu tubular) SiC reactor with a residence time of 100 mu s. Product detection was carried out using single photon ionization (SPI, 10.487 eV) and resonance enhanced multiphoton ionization (REMPI) time-of-flight mass spectrometry and matrix infrared absorption spectroscopy from 400 K to 1600 K. The initial pyrolytic step for each isomer is methoxy bond homolysis to eliminate methyl radical. Subsequent thermolysis is unique for each isomer. In the case of o-CH3O-C6H4-OCH3, intramolecular H-transfer dominates leading to the formation of o-hydroxybenzaldehyde (o-HO-C6H4-CHO) and phenol (C6H5OH). Para-CH3O-C6H4-OCH3 immediately breaks the second methoxy bond to form p-benzoquinone, which decomposes further to cyclopentadienone (C5H4=O). Finally, the m-CH3O-C6H4-OCH3 isomer will predominantly follow a ring-reduction/CO-elimination mechanism to form C5H4=O. Electronic structure calculations and transition state theory are used to confirm mechanisms and comment on kinetics. Implications for lignin pyrolysis are discussed. (C) 2014 AIP Publishing LLC. C1 [Robichaud, David J.; Scheer, Adam M.; Mukarakate, Calvin; Ormond, Thomas K.; Buckingham, Grant T.; Nimlos, Mark R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Scheer, Adam M.; Ormond, Thomas K.; Buckingham, Grant T.; Ellison, G. Barney] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Robichaud, DJ (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM david.robichaud@nrel.gov FU U.S. Department of Energy's Bioenergy Technology Office [DE-AC36-99GO10337]; National Renewable Energy Laboratory; DOE's National Renewal Energy Laboratory [1544759]; National Science Foundation [CHE-0848606, CHE-111-2466] FX This work was funded by the U.S. Department of Energy's Bioenergy Technology Office, under Contract No. DE-AC36-99GO10337 with the National Renewable Energy Laboratory. Experiments at the University of Colorado were supported by the DOE's National Renewal Energy Laboratory (Contract No. 1544759) and by grants from the National Science Foundation (CHE-0848606 and CHE-111-2466). NR 55 TC 7 Z9 7 U1 3 U2 54 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234302 DI 10.1063/1.4879615 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200023 PM 24952536 ER PT J AU Ryazanov, M Harrison, AW Wang, G Crider, PE Neumark, DM AF Ryazanov, Mikhail Harrison, Aaron W. Wang, Gregory Crider, Paul E. Neumark, Daniel M. TI Investigation of 3-fragment photodissociation of O-3 at 193.4 and 157.6 nm by coincident measurements SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MICROCHANNEL PLATE DETECTOR; FLIGHT MASS-SPECTROMETER; SCHUMANN-RUNGE BANDS; FAST BEAM; OZONE; LASER; DYNAMICS; ENERGY; STATE; PHOTOELECTRON AB Photodissociation of the ozone molecule at 193.4 nm (6.41 eV) and 157.6 nm (7.87 eV) is studied by fast-beam translational spectroscopy. Coincident detection of the dissociation products allows direct observation of the 3-fragment channel and determination of its kinematic parameters. The results indicate that at each wavelength, 3-fragment dissociation proceeds through synchronous concerted bond breaking, but the energy partitioning among the fragments is different. The branching fraction of the 3-fragment channel increases from 5.2(6)% at 193.4 nm to 26(4)% at 157.6 nm, in agreement with previous studies. It is shown that vibrational excitation of the symmetric stretch mode in O-3 molecules created by photodetachment of O-3(-) anion enhances the absorption efficiency, especially at 193.4 nm, but does not have a strong effect on the 3-fragment dissociation. (C) 2014 AIP Publishing LLC. C1 [Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU Office of Basic Energy Science, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Basic Energy Science, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 56 TC 2 Z9 2 U1 2 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 21 PY 2014 VL 140 IS 23 AR 234304 DI 10.1063/1.4882644 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ7OO UT WOS:000337886200025 PM 24952538 ER PT J AU Liu, J Cai, B Carr, R Dwyer, DA Gu, WQ Li, GS Qian, X McKeown, RD Tsang, RHM Wang, W Wu, FF Zhang, C AF Liu, J. Cai, B. Carr, R. Dwyer, D. A. Gu, W. Q. Li, G. S. Qian, X. McKeown, R. D. Tsang, R. H. M. Wang, W. Wu, F. F. Zhang, C. TI Automated calibration system for a high-precision measurement of neutrino mixing angle theta(13) with the Daya Bay antineutrino detectors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Reactor neutri; theta(13); Daya Bay; Automated calibration system ID OSCILLATIONS AB We describe the automated calibration system for the antineutrino detectors in the Daya Bay Neutrino Experiment. This system consists of 24 identical units instrumented on 8 identical 20 ton liquid scintillator detectors. Each unit is a fully automated robotic system capable of deploying an LED and various radioactive sources into the detector along given vertical axes. Selected results from performance studies of the calibration system are reported. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liu, J.; Cai, B.; Carr, R.; Dwyer, D. A.; Qian, X.; McKeown, R. D.; Tsang, R. H. M.; Wu, F. F.; Zhang, C.] CALTECH, Kellogg Radiat Lab, Pasadena, CA 91125 USA. [Liu, J.; Gu, W. Q.; Li, G. S.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [McKeown, R. D.; Wang, W.] Coll William & Mary, Dept Phys, Williamsburg, VA 23185 USA. [Dwyer, D. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Qian, X.; Zhang, C.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Liu, J (reprint author), Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. EM jianglai.liu@sjtu.edu.cn RI Liu, Jianglai/P-2587-2015; OI Liu, Jianglai/0000-0002-4563-3157; Qian, Xin/0000-0002-7903-7935; Zhang, Chao/0000-0003-2298-6272 FU US DoE, Office of Science, High Energy Physics; US National Science Foundation; Natural Science Foundation of China [11005073, 11175116]; Shuguang Foundation of Shanghai [Z1127941]; Shanghai Laboratory for Particle Physics and Cosmology at the Shanghai Jiao Tong University FX This work was done with support from the US DoE, Office of Science, High Energy Physics, the US National Science Foundation, the Natural Science Foundation of China Grants 11005073 and 11175116, the Shuguang Foundation of Shanghai Grant Z1127941, and Shanghai Laboratory for Particle Physics and Cosmology at the Shanghai Jiao Tong University. NR 22 TC 9 Z9 9 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUN 21 PY 2014 VL 750 BP 19 EP 37 DI 10.1016/j.nima.2014.02.049 PG 19 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AF9BC UT WOS:000335009000003 ER PT J AU Liu, C Luo, Y Minty, M AF Liu, C. Luo, Y. Minty, M. TI Simultaneous global coupling and vertical dispersion correction in RHIC SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Global coupling; Dispersion; Skew quadrupole; Simultaneous correction; Spin polarization; SVD AB Residual vertical dispersion in the order of +/ - 0.2 m( peak to peak) has been measured at store energies for both polarized proton and heavy ion beams in RHIC. The hypothesis is that this may have impact on the polarization transmission efficiency during the energy ramp, the polarization lifetime at store and, for heavy ions, the dynamic aperture. An algorithm to correct global coupling and vertical dispersion simultaneously using existing skew quadrupoles was developed. Measured coupling and vertical dispersion functions acquired before and after correction are presented. & (C) 2014 Elsevier B.V.All rights reserved. C1 [Liu, C.; Luo, Y.; Minty, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Liu, C (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM cliu1@bnl.gov NR 23 TC 1 Z9 1 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUN 21 PY 2014 VL 750 BP 56 EP 60 DI 10.1016/j.nima.2014.02.015 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AF9BC UT WOS:000335009000006 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besanon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buesche, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrina, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Gruenendahl, S Gruenewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Ak, AJ Kajfasz, E Karmanov, D Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Raja, R Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soeldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S VanKooten, R Vanleeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besanon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Borysova, M. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buesche, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrina, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Ak, A. Juste Kajfasz, E. Karmanov, D. Katsanos, I. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Raja, R. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. VanKooten, R. Vanleeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA DO Collaboration TI Electron and photon identification in the Do experiment SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Fermilab; DZero; DO; Tevatron Run II; Electron and photon identification; Electron and photon reconstruction ID CALORIMETER; DETECTOR AB The electron and photon reconstruction and identification algorithms used by the DO Collaboration at the Fermilab Tevatron collider are described. The determination of the electron energy scale and resolution is presented. Studies of the performance of the electron and photon reconstruction and identification are summarized. The results are based on measurements of Z boson decay events of Z ee and Z gamma ll(i=e mu) collected in pp(over bar) collisions at a center- of- mass energy of 1.96 TeV using an integrated luminosity of up to10 fb(-1.) (C) 2014 Elsevier B.V. All rights reserved. C1 [Hensel, C.; Maciel, A. K. 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F.; Harder, K.; Hegab, H.; Hesketh, G.; McGivern, C. L.; Peters, Y.; Petridis, K.; Price, D.; Schwanenberger, C.; Soeldner-Rembold, S.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Johns, K.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Fortner, M.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Feng, L.; Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; VanKooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumel, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Chandra, A.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; de Sa, R. Lopes; Schwienhorst, R.; Shaw, S.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhat, P. C.; Bhatia, S.; Bhatnagar, V.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Garbincius, P. H.; Katsanos, I.; Malik, S.; Rubinov, P.; Skubic, P.; Snow, G. R.; Wobisch, M.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Blazey, G.; Blessing, S.; Bloom, K.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Abbott, B.; Boehnlein, A.; Boline, D.; Boos, E. E.; Borissov, G.; Borysova, M.; Lobodenko, A.; Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Head, T.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Suter, L.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Brandt, A.; Brandt, O.; Brock, R.; Bross, A.; Brown, D.; Khanov, A.; Partridge, R.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Haley, J.; Hebbeker, T.; Heintz, U.; Hobbs, J. D.; Jabeen, S.; Narain, M.; Parihar, V.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Bu, X. B.; Buehler, M.; Buesche, V.; Bunichev, V.; Burdin, S.; Buszello, C. P.; Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Bandurin, D. V.; Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Bu, XB (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM xbbu@fnal.gov RI Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Simak, Vladislav/H-2996-2014; Kozelov, Alexander/J-3812-2014; Dudko, Lev/D-7127-2012; Lei, Xiaowen/O-4348-2014; Gutierrez, Phillip/C-1161-2011; Sharyy, Viatcheslav/F-9057-2014; Merkin, Mikhail/D-6809-2012; Li, Liang/O-1107-2015 OI Chapon, Emilien/0000-0001-6968-9828; Melnychuk, Oleksandr/0000-0002-2089-8685; Ding, Pengfei/0000-0002-4050-1753; Bassler, Ursula/0000-0002-9041-3057; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; Bertram, Iain/0000-0003-4073-4941; Dudko, Lev/0000-0002-4462-3192; Williams, Mark/0000-0001-5448-4213; Grohsjean, Alexander/0000-0003-0748-8494; Lei, Xiaowen/0000-0002-2564-8351; Sharyy, Viatcheslav/0000-0002-7161-2616; Li, Liang/0000-0001-6411-6107 FU DOE; NSF; CEA; CNRS/IN2P3; NRC KI; RFBR; CNPq; FAPERJ; FAPESP; FUNDUNESP; DAE; DST; Colciencias; CONACyT; NRF; FOM; STFC; Royal Society; MSMT; GACR; BMBF; DFG; SFI; The Swedish Research Council; CAS; CNSF FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the DOE and NSF(USA); CEA and CNRS/IN2P3 (France); MON, NRC KI and RFBR(Russia); CNPq, FAPERJ, FAPESP and FUNDUNESP(Brazil); DAE and DST(India); Colciencias (Colombia); CONACyT(Mexico); NRF(Korea); FOM (The Netherlands); STFC and the Royal Society(United Kingdom); MSMT and GACR(Czech Republic); BMBF and DFG(Germany); SFI (Ireland); The Swedish Research Council(Sweden); and CAS and CNSF (China). NR 25 TC 18 Z9 18 U1 2 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUN 21 PY 2014 VL 750 BP 78 EP 95 DI 10.1016/j.nima.2014.03.013 PG 18 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AF9BC UT WOS:000335009000009 ER PT J AU Amanullah, R Goobar, A Johansson, J Banerjee, DPK Venkataraman, V Joshi, V Ashok, NM Cao, Y Kasliwal, MM Kulkarni, SR Nugent, PE Petrushevska, T Stanishev, V AF Amanullah, R. Goobar, A. Johansson, J. Banerjee, D. P. K. Venkataraman, V. Joshi, V. Ashok, N. M. Cao, Y. Kasliwal, M. M. Kulkarni, S. R. Nugent, P. E. Petrushevska, T. Stanishev, V. TI THE PECULIAR EXTINCTION LAW OF SN 2014J MEASURED WITH THE HUBBLE SPACE TELESCOPE SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE dust, extinction; galaxies: individual (Messier 82); supernovae: individual (SN 2014J) ID IA SUPERNOVAE; CIRCUMSTELLAR DUST; INFRARED-EMISSION; K-CORRECTIONS; TIME-SERIES; LIGHT-CURVE; GALAXY M82; 2011FE; SPECTROSCOPY; PROGENITOR AB The wavelength dependence of the extinction of Type Ia SN 2014J in the nearby galaxy M82 has been measured using UV to near-IR photometry obtained with the Hubble Space Telescope, the Nordic Optical Telescope, and the Mount Abu Infrared Telescope. This is the first time that the reddening of an SN Ia is characterized over the full wavelength range of 0.2-2 mu m. A total-to-selective extinction, R-V >= 3.1, is ruled out with high significance. The best fit at maximum using a Galactic type extinction law yields R-V = 1.4 +/- 0.1. The observed reddening of SN 2014J is also compatible with a power-law extinction, A(lambda)/A(V) = (lambda/lambda(V))(p) as expected from multiple scattering of light, with p = -2.1 +/- 0.1. After correcting for differences in reddening, SN 2014J appears to be very similar to SN 2011 fe over the 14 broadband filter light curves used in our study. C1 [Amanullah, R.; Goobar, A.; Johansson, J.; Petrushevska, T.] Stockholm Univ, Oskar Klein Ctr, Dept Phys, SE-10691 Stockholm, Sweden. [Banerjee, D. P. K.; Venkataraman, V.; Joshi, V.; Ashok, N. M.] Phys Res Lab, Ahmadabad 380009, Gujarat, India. [Cao, Y.; Kulkarni, S. R.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Kasliwal, M. M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Nugent, P. E.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Nugent, P. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Computat Res Div, Berkeley, CA 94720 USA. [Stanishev, V.] CENTRA, Inst Super Tecn, Ctr Multidisciplinar Astrofis, P-1049001 Lisbon, Portugal. RP Amanullah, R (reprint author), Stockholm Univ, Oskar Klein Ctr, Dept Phys, SE-10691 Stockholm, Sweden. EM rahman@fysik.su.se RI Stanishev, Vallery/M-8930-2013 OI Stanishev, Vallery/0000-0002-7626-1181 FU Swedish Research Council; Swedish Space Board; Hubble Fellowship; Carnegie-Princeton Fellowship; Fundacao para a Ciencia e a Tecnologia (Ciencia); [PTDC/CTE-AST/ 112582/2009] FX We thank Denise Taylor, Claus Leitherer, and John Mackenty at the Space Telescope Science Institute for advising and assisting us in carrying out this program. R.A. and A.G. acknowledge support from the Swedish Research Council and the Swedish Space Board. M.M.K. acknowledges support from the Hubble Fellowship and Carnegie-Princeton Fellowship.; Observations were made with the Hubble Space Telescope; the Nordic Optical Telescope, operated by the Nordic Optical Telescope Scientific Association at the Observatorio del Roque de los Muchachos, La Palma, Spain; and the Mount Abu 1.2 m Infrared Telescope, India. STSDAS is a product of the Space Telescope Science Institute, which is operated by AURA for NASA. V.S. acknowledges support from Fundacao para a Ciencia e a Tecnologia (Ciencia 2008) and grant PTDC/CTE-AST/ 112582/2009. NR 35 TC 40 Z9 41 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUN 20 PY 2014 VL 788 IS 2 AR L21 DI 10.1088/2041-8205/788/2/L21 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK5YX UT WOS:000338504500002 ER PT J AU Fu, W Li, H Lubow, S Li, ST AF Fu, Wen Li, Hui Lubow, Stephen Li, Shengtai TI LONG-TERM EVOLUTION OF PLANET-INDUCED VORTICES IN PROTOPLANETARY DISKS SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE accretion, accretion disks; hydrodynamics; instabilities; protoplanetary disks ID ROSSBY-WAVE INSTABILITY; THIN ACCRETION DISKS; INDUCED GAP EDGES; TRANSITIONAL DISKS; PRETRANSITIONAL DISKS; SCALE ASYMMETRIES; TIDAL INTERACTION; DUST FILTRATION; LAMINAR DISKS; GIANT-PLANET AB Recent observations of large-scale asymmetric features in protoplanetary disks suggest that large-scale vortices exist in such disks. Massive planets are known to be able to produce deep gaps in protoplanetary disks. The gap edges could become hydrodynamically unstable to the Rossby wave/vortex instability and form large-scale vortices. In this study we examine the long-term evolution of these vortices by carrying out high-resolution two-dimensional hydrodynamic simulations that last more than 104 orbits (measured at the planet's orbit). We find that the disk viscosity has a strong influence on both the emergence and lifetime of vortices. In the outer disk region where asymmetric features are observed, our simulation results suggest that the disk viscous alpha needs to be low, similar to 10(-5)-10(-4), to sustain vortices to thousands and up to 10(4) orbits in certain cases. The chance of finding a vortex feature in a disk then decreases with smaller planet orbital radius. For alpha similar to 10(-3) or larger, even planets with masses of 5 M-J will have difficulty either producing or sustaining vortices. We have also studied the effects of different disk temperatures and planet masses. We discuss the implications of our findings on current and future protoplanetary disk observations. C1 [Fu, Wen] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Fu, Wen; Li, Hui; Li, Shengtai] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lubow, Stephen] Space Telescope Sci Inst, Baltimore, MD 21218 USA. RP Fu, W (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM wf5@rice.edu OI Li, Shengtai/0000-0002-4142-3080 FU LDRD program; IGPP program; DOE/Office of Fusion Energy Science through CMSO at LANL; NASA [NNX11AK61G] FX Simulations in this work were performed using the Institutional Computing Facilities at LANL. W.F., H.L., and S.L. gratefully acknowledge the support by the LDRD and IGPP programs and DOE/Office of Fusion Energy Science through CMSO at LANL. W.F. and S.L. acknowledge support from NASA grant NNX11AK61G. We thank Til Birnstiel and Zhaohuan Zhu for valuable comments. NR 47 TC 16 Z9 16 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUN 20 PY 2014 VL 788 IS 2 AR L41 DI 10.1088/2041-8205/788/2/L41 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AK5YX UT WOS:000338504500022 ER PT J AU Daniilidis, N Gerber, S Bolloten, G Ramm, M Ransford, A Ulin-Avila, E Talukdar, I Haffner, H AF Daniilidis, N. Gerber, S. Bolloten, G. Ramm, M. Ransford, A. Ulin-Avila, E. Talukdar, I. Haeffner, H. TI Surface noise analysis using a single-ion sensor SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM ERROR-CORRECTION; TRANSISTOR AB We use a single-ion electric-field noise sensor in combination with in situ surface treatment and analysis tools, to investigate the relationship between electric-field noise from metal surfaces in vacuum and the composition of the surface. These experiments are performed in a setup that integrates ion trapping capabilities with surface analysis tools. We find that treatment of an aluminum-copper surface with energetic argon ions significantly reduces the level of room-temperature electric-field noise, but the surface does not need to be atomically clean to show noise levels comparable to those of the best cryogenic traps. The noise levels after treatment are low enough to allow fault-tolerant trapped-ion quantum information processing on a microfabricated surface trap at room temperature. C1 [Daniilidis, N.; Gerber, S.; Bolloten, G.; Ramm, M.; Ransford, A.; Ulin-Avila, E.; Talukdar, I.; Haeffner, H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haeffner, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Daniilidis, N (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM hhaeffner@berkeley.edu RI ulin-avila, erick/M-3278-2014; Haeffner, Hartmut/D-8046-2012 OI Haeffner, Hartmut/0000-0002-5113-9622 FU Office of the Director of National Intelligence (ODNI); Intelligence Advanced Research Projects Activity (IARPA), through the Army Research Office [W911NF-10-1-0284] FX We would like to acknowledge M. Crommie for useful feedback and the loan of a LEED/AES spectrometer; D. Hite, D. Leibfried, G. Somorjai, E. Yablanovitch, and J. Bokor for useful discussions; and P. Schindler for a critical reading of the manuscript. This research was funded by the Office of the Director of National Intelligence (ODNI), Intelligence Advanced Research Projects Activity (IARPA), through the Army Research Office Grant No. W911NF-10-1-0284. All statements of fact, opinion, or conclusions contained herein are those of the authors and should not be construed as representing the official views or policies of IARPA, the ODNI, or the US Government. NR 43 TC 18 Z9 18 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2014 VL 89 IS 24 AR 245435 DI 10.1103/PhysRevB.89.245435 PG 7 WC Physics, Condensed Matter SC Physics GA AK5UZ UT WOS:000338493200005 ER PT J AU Agnese, R Anderson, AJ Asai, M Balakishiyeva, D Thakur, RB Bauer, DA Beaty, J Billard, J Borgland, A Bowles, MA Brandt, D Brink, PL Bunker, R Cabrera, B Caldwell, DO Cerdeno, DG Chagani, H Chen, Y Cherry, M Cooley, J Cornell, B Crewdson, CH Cushman, P Daal, M DeVaney, D Di Stefano, PCF Silva, EDE Doughty, T Esteban, L Fallows, S Figueroa-Feliciano, E Godfrey, GL Golwala, SR Hall, J Hansen, S Harris, HR Hertel, SA Hines, BA Hofer, T Holmgren, D Hsu, L Huber, ME Jastram, A Kamaev, O Kara, B Kelsey, MH Kenany, S Kennedy, A Kiveni, M Koch, K Leder, A Loer, B Asamar, EL Mahapatra, R Mandic, V Martinez, C McCarthy, KA Mirabolfathi, N Moffatt, RA Nelson, RH Novak, L Page, K Partridge, R Pepin, M Phipps, A Platt, M Prasad, K Pyle, M Qiu, H Rau, W Redl, P Reisetter, A Resch, RW Ricci, Y Ruschman, M Saab, T Sadoulet, B Sander, J Schmitt, RL Schneck, K Schnee, RW Scorza, S Seitz, DN Serfass, B Shank, B Speller, D Tomada, A Upadhyayula, S Villano, AN Welliver, B Wright, DH Yellin, S Yen, JJ Young, BA Zhang, J AF Agnese, R. Anderson, A. J. Asai, M. Balakishiyeva, D. Thakur, R. Basu Bauer, D. A. Beaty, J. Billard, J. Borgland, A. Bowles, M. A. Brandt, D. Brink, P. L. Bunker, R. Cabrera, B. Caldwell, D. O. Cerdeno, D. G. Chagani, H. Chen, Y. Cherry, M. Cooley, J. Cornell, B. Crewdson, C. H. Cushman, P. Daal, M. DeVaney, D. Di Stefano, P. C. F. Silva, E. Do Couto E. Doughty, T. Esteban, L. Fallows, S. Figueroa-Feliciano, E. Godfrey, G. L. Golwala, S. R. Hall, J. Hansen, S. Harris, H. R. Hertel, S. A. Hines, B. A. Hofer, T. Holmgren, D. Hsu, L. Huber, M. E. Jastram, A. Kamaev, O. Kara, B. Kelsey, M. H. Kenany, S. Kennedy, A. Kiveni, M. Koch, K. Leder, A. Loer, B. Asamar, E. Lopez Mahapatra, R. Mandic, V. Martinez, C. McCarthy, K. A. Mirabolfathi, N. Moffatt, R. A. Nelson, R. H. Novak, L. Page, K. Partridge, R. Pepin, M. Phipps, A. Platt, M. Prasad, K. Pyle, M. Qiu, H. Rau, W. Redl, P. Reisetter, A. Resch, R. W. Ricci, Y. Ruschman, M. Saab, T. Sadoulet, B. Sander, J. Schmitt, R. L. Schneck, K. Schnee, R. W. Scorza, S. Seitz, D. N. Serfass, B. Shank, B. Speller, D. Tomada, A. Upadhyayula, S. Villano, A. N. Welliver, B. Wright, D. H. Yellin, S. Yen, J. J. Young, B. A. Zhang, J. CA SuperCDMS Collaboration TI Search for Low-Mass Weakly Interacting Massive Particles with SuperCDMS SO PHYSICAL REVIEW LETTERS LA English DT Article ID DARK-MATTER CANDIDATES AB We report a first search for weakly interacting massive particles (WIMPs) using the background rejection capabilities of SuperCDMS. An exposure of 577 kg days was analyzed for WIMPs with mass < 30 GeV/c(2), with the signal region blinded. Eleven events were observed after unblinding. We set an upper limit on the spin-independent WIMP-nucleon cross section of 1.2 x 10(-42) cm(2) at 8 GeV/c(2). This result is in tension with WIMP interpretations of recent experiments and probes new parameter space for WIMP-nucleon scattering for WIMP masses < 6 GeV/c(2). C1 [Cornell, B.; Golwala, S. R.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Thakur, R. Basu; Bauer, D. A.; Hansen, S.; Holmgren, D.; Hsu, L.; Loer, B.; Ruschman, M.; Schmitt, R. L.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Sadoulet, B.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Anderson, A. J.; Billard, J.; Figueroa-Feliciano, E.; Hertel, S. A.; Leder, A.; McCarthy, K. A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Hall, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Crewdson, C. H.; Di Stefano, P. C. F.; Kamaev, O.; Martinez, C.; Page, K.; Rau, W.; Ricci, Y.] Queens Univ, Dept Phys, Kingston, ON K7 3N6, Canada. [Young, B. A.] Santa Clara Univ, Dept Phys, Santa Clara, CA 95053 USA. [Asai, M.; Borgland, A.; Brandt, D.; Brink, P. L.; Cherry, M.; Godfrey, G. L.; Kelsey, M. H.; Partridge, R.; Schneck, K.; Tomada, A.; Wright, D. H.] Kavli Inst Particle Astrophys & Cosmol, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Cooley, J.; Kara, B.; Qiu, H.; Scorza, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Cabrera, B.; Moffatt, R. A.; Novak, L.; Redl, P.; Yellin, S.; Yen, J. J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Bunker, R.; Chen, Y.; Kiveni, M.; Schnee, R. W.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Jastram, A.; Mahapatra, R.; Platt, M.; Prasad, K.; Upadhyayula, S.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cerdeno, D. G.; Esteban, L.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Cerdeno, D. G.; Esteban, L.] Univ Autonoma Madrid, Inst Fis Teor UAM CSIC, E-28049 Madrid, Spain. [Daal, M.; Doughty, T.; Kenany, S.; Mirabolfathi, N.; Pyle, M.; Sadoulet, B.; Serfass, B.; Speller, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Caldwell, D. O.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Hines, B. A.] Univ Colorado, Dept Phys, Denver, CO 80217 USA. [Reisetter, A.] Univ Evansville, Dept Phys, Evansville, IN 47722 USA. [Agnese, R.; Balakishiyeva, D.; Saab, T.; Welliver, B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Thakur, R. Basu] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Beaty, J.; Chagani, H.; Cushman, P.; DeVaney, D.; Fallows, S.; Hofer, T.; Kennedy, A.; Koch, K.; Mandic, V.; Pepin, M.; Villano, A. N.; Zhang, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Sander, J.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. RP Anderson, AJ (reprint author), MIT, Dept Phys, Cambridge, MA 02139 USA. EM adama@mit.edu RI Pyle, Matt/E-7348-2015; Hall, Jeter/E-9294-2015; OI Pyle, Matt/0000-0002-3490-6754; Holmgren, Donald/0000-0001-6701-7737; Cerdeno, David G./0000-0002-7649-1956 FU National Science Foundation; United States Department of Energy; NSERC Canada; MultiDark (Spanish MINECO); Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy [DE-AC02-76SF00515] FX The SuperCDMS Collaboration gratefully acknowledges the contributions of numerous engineers and technicians. In addition, we gratefully acknowledge assistance from the staff of the Soudan Underground Laboratory and the Minnesota Department of Natural Resources. The iZIP detectors were fabricated in the Stanford Nanofabrication Facility, which is a member of the National supported in part by the National Science Foundation, by the United States Department of Energy, by NSERC Canada, and by MultiDark (Spanish MINECO). Fermilab is operated by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359. SLAC is operated under Contract No. DE-AC02-76SF00515 with the United States Department of Energy. NR 38 TC 213 Z9 213 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 20 PY 2014 VL 112 IS 24 AR 241302 DI 10.1103/PhysRevLett.112.241302 PG 6 WC Physics, Multidisciplinary SC Physics GA AK5YD UT WOS:000338502300003 ER PT J AU Martinez, RJ Wu, CH Beazley, MJ Andersen, GL Conrad, ME Hazen, TC Taillefert, M Sobecky, PA AF Martinez, Robert J. Wu, Cindy H. Beazley, Melanie J. Andersen, Gary L. Conrad, Mark E. Hazen, Terry C. Taillefert, Martial Sobecky, Patricia A. TI Microbial Community Responses to Organophosphate Substrate Additions in Contaminated Subsurface Sediments SO PLOS ONE LA English DT Article ID PLANT-GROWTH PROMOTION; 16S RIBOSOMAL-RNA; IN-SITU BIOREDUCTION; PHOSPHATASE-ACTIVITY; URANIUM BIOMINERALIZATION; PHYLOGENETIC ANALYSIS; METHANOGENIC ARCHAEA; ANAEROBIC CONDITIONS; BACTERIAL DIVERSITY; REDUCING CONDITIONS AB Background: Radionuclide-and heavy metal-contaminated subsurface sediments remain a legacy of Cold War nuclear weapons research and recent nuclear power plant failures. Within such contaminated sediments, remediation activities are necessary to mitigate groundwater contamination. A promising approach makes use of extant microbial communities capable of hydrolyzing organophosphate substrates to promote mineralization of soluble contaminants within deep subsurface environments. Methodology/Principal Findings: Uranium-contaminated sediments from the U. S. Department of Energy Oak Ridge Field Research Center (ORFRC) Area 2 site were used in slurry experiments to identify microbial communities involved in hydrolysis of 10 mM organophosphate amendments [i.e., glycerol-2-phosphate (G2P) or glycerol-3-phosphate (G3P)] in synthetic groundwater at pH 5.5 and pH 6.8. Following 36 day (G2P) and 20 day (G3P) amended treatments, maximum phosphate (PO43-) concentrations of 4.8 mM and 8.9 mM were measured, respectively. Use of the PhyloChip 16S rRNA microarray identified 2,120 archaeal and bacterial taxa representing 46 phyla, 66 classes, 110 orders, and 186 families among all treatments. Measures of archaeal and bacterial richness were lowest under G2P (pH 5.5) treatments and greatest with G3P (pH 6.8) treatments. Members of the phyla Crenarchaeota, Euryarchaeota, Bacteroidetes, and Proteobacteria demonstrated the greatest enrichment in response to organophosphate amendments and the OTUs that increased in relative abundance by 2-fold or greater accounted for 9%-50% and 3%-17% of total detected Archaea and Bacteria, respectively. Conclusions/Significance: This work provided a characterization of the distinct ORFRC subsurface microbial communities that contributed to increased concentrations of extracellular phosphate via hydrolysis of organophosphate substrate amendments. Within subsurface environments that are not ideal for reductive precipitation of uranium, strategies that harness microbial phosphate metabolism to promote uranium phosphate precipitation could offer an alternative approach for in situ sequestration. C1 [Martinez, Robert J.; Beazley, Melanie J.; Sobecky, Patricia A.] Univ Alabama, Dept Biol Sci, Tuscaloosa, AL 35487 USA. [Wu, Cindy H.; Andersen, Gary L.; Conrad, Mark E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Taillefert, Martial] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. RP Martinez, RJ (reprint author), Univ Alabama, Dept Biol Sci, Tuscaloosa, AL 35487 USA. EM rmartinez@ua.edu RI Andersen, Gary/G-2792-2015; Conrad, Mark/G-2767-2010; Hazen, Terry/C-1076-2012; OI Andersen, Gary/0000-0002-1618-9827; Hazen, Terry/0000-0002-2536-9993; Beazley, Melanie/0000-0001-9973-7798 FU Office of Science (BER), U.S. Department of Energy [DE-FG02-04ER63906, SC0002530]; [DE-AC02-05CH11231] FX This research was supported by the Office of Science (BER), U.S. Department of Energy Grant No. DE-FG02-04ER63906 (University of Alabama), Subcontract No. SC0002530 (Georgia Institute of Technology), and partially by No. DE-AC02-05CH11231 (Lawrence Berkeley National Laboratory). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 82 TC 6 Z9 6 U1 6 U2 47 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 20 PY 2014 VL 9 IS 6 AR e100383 DI 10.1371/journal.pone.0100383 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK2UZ UT WOS:000338276300070 PM 24950228 ER PT J AU Zhu, JX Wen, XD Haraldsen, JT He, M Panagopoulos, C Chia, EEM AF Zhu, Jian-Xin Wen, Xiao-Dong Haraldsen, J. T. He, Mi Panagopoulos, C. Chia, Elbert E. M. TI Induced Ferromagnetism at BiFeO3/YBa2Cu3O7 Interfaces SO SCIENTIFIC REPORTS LA English DT Article ID SUPERCONDUCTING OXIDES; MAGNETISM AB Transition metal oxides (TMOs) exhibit many emergent phenomena ranging from high-temperature superconductivity and giant magnetoresistance to magnetism and ferroelectricity. In addition, when TMOs are interfaced with each other, new functionalities can arise, which are absent in individual components. Here, we report results from first-principles calculations on the magnetism at the BiFeO3/YBa2Cu3O7 interfaces. By comparing the total energy for various magnetic spin configurations inside BiFeO3, we are able to show that a metallic ferromagnetism is induced near the interface. We further develop an interface exchange-coupling model and place the extracted exchange coupling interaction strengths, from the first-principles calculations, into a resultant generic phase diagram. Our conclusion of interfacial ferromagnetism is confirmed by the presence of a hysteresis loop in field-dependent magnetization data. The emergence of interfacial ferromagnetism should have implications to electronic and transport properties. C1 [Zhu, Jian-Xin; Wen, Xiao-Dong; Haraldsen, J. T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin; Haraldsen, J. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Haraldsen, J. T.] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22807 USA. [He, Mi; Panagopoulos, C.; Chia, Elbert E. M.] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. RP Zhu, JX (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jxzhu@lanl.gov RI Chia, Elbert/B-6996-2011; Haraldsen, Jason/B-9809-2012 OI Chia, Elbert/0000-0003-2066-0834; Haraldsen, Jason/0000-0002-8641-5412 FU U.S. DOE at LANL [DEAC52-06NA25396]; LANL LDRD-DR Program, Singapore [NRF-CRP-2008-04]; MOE AcRF [RG 13/12] FX One of the authors (J.-X.Z.) thanks W. Luo for helpful discussions, and is also grateful to J. Qi, R. Prasankumar, and Q. Jia for collaboration on related topics. This work was supported by U.S. DOE at LANL under Contract No. DEAC52-06NA25396 and LANL LDRD-DR Program (J.-X.Z., X. D. W., & J. T. H.), Singapore NRF-CRP-2008-04 (M. H., C. P., & E. E. M. C.) and MOE AcRF Tier 1 RG 13/12 (E. E. M. C.). This work was also, in part, supported by the Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences user facility. NR 29 TC 6 Z9 6 U1 3 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 20 PY 2014 VL 4 AR 5368 DI 10.1038/srep05368 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ7PD UT WOS:000337887700006 PM 24947500 ER PT J AU Archambault, S Arlen, T Aune, T Beilicke, M Benbow, W Bird, R Bottcher, M Bouvier, A Buckley, JH Bugaev, V Ciupik, L Collins-Hughes, E Connolly, MP Cui, W Dickherber, R Dumm, J Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortson, L Furniss, A Galante, N Gall, D Garson, AI Gillanders, GH Griffin, S Grube, J Gusbar, C Gyuk, G Hanna, D Holder, J Hughes, G Kaaret, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Lamerato, A Lang, MJ Li, K Madhavan, AS Maier, G Majumdar, P McArthur, S McCann, A Millis, J Moriarty, P Mukherjee, R Nieto, D De Bhroithe, AO Ong, RA Orr, M Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Reynolds, PT Richards, GT Roache, E Roustazadeh, P Saxon, DB Sembroski, GH Senturk, GD Skole, C Staszak, D Telezhinsky, I Tesic, G Theiling, M Varlotta, A Vassiliev, VV Vincent, S Wakely, SP Weinstein, A Welsing, R Williams, DA Zitzer, B AF Archambault, S. Arlen, T. Aune, T. Beilicke, M. Benbow, W. Bird, R. Boettcher, M. Bouvier, A. Buckley, J. H. Bugaev, V. Ciupik, L. Collins-Hughes, E. Connolly, M. P. Cui, W. Dickherber, R. Dumm, J. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortson, L. Furniss, A. Galante, N. Gall, D. Garson, A. III. Gillanders, G. H. Griffin, S. Grube, J. Gusbar, C. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Lamerato, A. Lang, M. J. Li, K. Madhavan, A. S. Maier, G. Majumdar, P. McArthur, S. McCann, A. Millis, J. Moriarty, P. Mukherjee, R. Nieto, D. De Bhroithe, A. O'Faolain Ong, R. A. Orr, M. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Reynolds, P. T. Richards, G. T. Roache, E. Roustazadeh, P. Saxon, D. B. Sembroski, G. H. Senturk, G. D. Skole, C. Staszak, D. Telezhinsky, I. Tesic, G. Theiling, M. Varlotta, A. Vassiliev, V. V. Vincent, S. Wakely, S. P. Weinstein, A. Welsing, R. Williams, D. A. Zitzer, B. TI TEST OF MODELS OF THE COSMIC INFRARED BACKGROUND WITH MULTIWAVELENGTH OBSERVATIONS OF THE BLAZAR 1ES 1218+30.4 IN 2009 SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: general; BL Lacertae objects: individual (1ES1218+30.4); cosmic background radiation; diffuse radiation; galaxies: jets; gamma rays: galaxies ID GAMMA-RAY OBSERVATIONS; EXTRAGALACTIC MAGNETIC-FIELDS; ACTIVE GALACTIC NUCLEI; LARGE-AREA TELESCOPE; X-RAY; TEV BLAZARS; PARTICLE-ACCELERATION; VERITAS OBSERVATIONS; TIMING EXPLORER; STRONG FLARES AB We present the results of a multi-wavelength campaign targeting the blazar 1ES 1218+30.4 with observations with the 1.3 m McGraw-Hill optical telescope, the Rossi X-ray Timing Explorer (RXTE), the Fermi Gamma-Ray Space Telescope, and the Very Energetic Radiation Imaging Telescope Array System (VERITAS). The RXTE and VERITAS observations were spread over a 13 day period and revealed clear evidence for flux variability, and a strong X-ray and gamma-ray flare on 2009 February 26 (MJD 54888). The campaign delivered a well-sampled broadband energy spectrum with simultaneous RXTE and VERITAS very high energy (VHE, > 100 GeV) observations, as well as contemporaneous optical and Fermi observations. The 1ES 1218+30.4 broadband energy spectrum-the first with simultaneous X-ray and VHE gamma-ray energy spectra-is of particular interest as the source is located at a high cosmological redshift for a VHE source (z = 0.182), leading to strong absorption of VHE gamma rays by photons from the optical/infrared extragalactic background light (EBL) via gamma VHE +gamma EBL -> e(+) e(-)pair-creation processes. We model the data with a one-zone synchrotron self-Compton (SSC) emission model and with the extragalactic absorption predicted by several recent EBL models. We find that the observations are consistent with the SSC scenario and all the EBL models considered in this work. We discuss observational and theoretical avenues to improve on the EBL constraints. C1 [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Staszak, D.; Tesic, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Arlen, T.; Aune, T.; Ong, R. A.; Vassiliev, V. V.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Beilicke, M.; Buckley, J. H.; Bugaev, V.; Dickherber, R.; Garson, A. III.; Krawczynski, H.; Li, K.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Collins-Hughes, E.; Khassen, Y.; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Boettcher, M.; Gusbar, C.; Gyuk, G.; Lamerato, A.; Roustazadeh, P.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Ciupik, L.; Grube, J.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Cui, W.; Finley, J. P.; Sembroski, G. H.; Theiling, M.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Errando, M.; Mukherjee, R.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Federici, S.; Hughes, G.; Maier, G.; Pohl, M.; Prokoph, H.; Skole, C.; Telezhinsky, I.; Vincent, S.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam Golm, Germany. [Gall, D.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Holder, J.; Saxon, D. B.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Holder, J.; Saxon, D. B.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Madhavan, A. S.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Majumdar, P.] Saha Inst Nucl Phys, Kolkata 700064, India. [McArthur, S.; Park, N.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Millis, J.] Anderson Univ, Dept Phys, Anderson, IN 46012 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Nieto, D.; Senturk, G. D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Perkins, J. S.] NASA, GSFC, CRESST, Greenbelt, MD 20771 USA. [Perkins, J. S.] NASA, GSFC, Astroparticle Phys Lab, Greenbelt, MD 20771 USA. [Perkins, J. S.] Univ Maryland, Baltimore, MD 21250 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Archambault, S (reprint author), McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. RI Khassen, Yerbol/I-3806-2015; Nieto, Daniel/J-7250-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Nieto, Daniel/0000-0003-3343-0755; Cui, Wei/0000-0002-6324-5772; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation, and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748), and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. NR 72 TC 1 Z9 1 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 158 DI 10.1088/0004-637X/788/2/158 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200061 ER PT J AU Beresnyak, A Li, H AF Beresnyak, Andrey Li, Hui TI BASIC BELL-MHD TURBULENCE SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic rays; instabilities; ISM: supernova remnants; magnetohydrodynamics (MHD); shock waves ID MAGNETIC-FIELD AMPLIFICATION; DIFFUSIVE SHOCK ACCELERATION; PARTICLE-ACCELERATION; COSMIC-RAYS; ASTROPHYSICAL SHOCKS; DRIVEN TURBULENCE; INSTABILITY; WAVE AB Nonresonant current instability was identified by Bell as an important mechanism for magnetic field amplification in supernova remnants. In this paper we focus on studying the nonlinear stage of this instability using the incompressible MHD formulation. We demonstrate that the evolution of magnetic turbulence driven by the Bell instability resembles turbulence driven on large scales. More importantly, we demonstrate that the energy- containing scale for magnetic fields is proportional to the square root of the magnetic energy density. Given the observational constraints of the possible field amplification, this new relation allows us to directly estimate the maximum energy of particles scattered by such fields, and this estimate is normally below the average particle energy. This implies that, without taking into account the feedback to cosmic rays (CRs), the typical scales of Bell fields, in either the linear or nonlinear regime, will be too small to affect high- energy particle acceleration. We mention several scenarios of back reaction to CRs that could be important. C1 [Beresnyak, Andrey; Li, Hui] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Beresnyak, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Beresnyak, Andrey/0000-0002-2124-7024 FU LANL/LDRD; DoE/Office of Fusion Energy Sciences through CMSO FX A. B. is grateful to Mischa Malkov, Axel Brandenburg, Tony Bell, Vladimir Zirakashvili, Pat Diamond, and Alex Schekochihin for useful discussions. The work is supported by the LANL/LDRD program and the DoE/Office of Fusion Energy Sciences through CMSO. Computing resources at LANL are provided through the Institutional Computing Program. NR 26 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 107 DI 10.1088/0004-637X/788/2/107 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200010 ER PT J AU Gotthelf, EV Tomsick, JA Halpern, JP Gelfand, JD Harrison, FA Boggs, SE Christensen, FE Craig, WW Hailey, JC Kaspi, VM Stern, DK Zhang, WW AF Gotthelf, E. V. Tomsick, J. A. Halpern, J. P. Gelfand, J. D. Harrison, F. A. Boggs, S. E. Christensen, F. E. Craig, W. W. Hailey, J. C. Kaspi, V. M. Stern, D. K. Zhang, W. W. TI NuSTAR DISCOVERY OF A YOUNG, ENERGETIC PULSAR ASSOCIATED WITH THE LUMINOUS GAMMA-RAY SOURCE HESS J1640-465 SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: individual objects (G338.3-0.0, HESS J1640-465, 1FHL J1640.5-4634, AX J1640.7-4632, XMMU J164045.4-463131); ISM: supernova remnants; pulsars: individual (PSR J1640-4631); stars: neutron ID X-RAY; SUPERNOVA REMNANT; NEUTRON-STAR; WIND NEBULAE; CATALOG; CLUSTER; POPULATION; PROGENITOR; MAGNETAR; WESTERLUND-1 AB We report the discovery of a 206 ms pulsar associated with the TeV gamma-ray source HESS J1640-465 using the Nuclear Spectroscopic Telescope Array (NuSTAR) X-ray observatory. PSR J1640-4631 lies within the shelltype supernova remnant (SNR) G338.3-0.0, and coincides with an X-ray point source and putative pulsar wind nebula (PWN) previously identified in XMM-Newton and Chandra images. It is spinning down rapidly with period derivative P = 9.758(44) x 10(-13), yielding a spin-down luminosity E = 4.4 x 10(36) erg s(-1), characteristic age tau(c) = P/2P. = 3350 yr, and surface dipole magnetic field strength B-s = 1.4x10(13) G. For the measured distance of 12 kpc to G338.3-0.0, the 0.2-10 TeV luminosity of HESS J1640-465 is 6% of the pulsar's present E . The Fermi source 1FHL J1640.5-4634 is marginally coincident with PSR J1640-4631, but we find no gamma - ray pulsations in a search using five years of Fermi Large Area Telescope (LAT) data. The pulsar energetics support an evolutionary PWN model for the broadband spectrum of HESS J1640-465, provided that the pulsar's braking index is n approximate to 2, and that its initial spin period was P-0 similar to 15 ms. C1 [Gotthelf, E. V.; Halpern, J. P.; Hailey, J. C.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Tomsick, J. A.; Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Gelfand, J. D.] NYU Abu Dhabi, Abu Dhabi, U Arab Emirates. [Gelfand, J. D.] NYU, Ctr Cosmol & Particle Phys, New York, NY USA. [Harrison, F. A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Christensen, F. E.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kaspi, V. M.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Stern, D. K.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Gotthelf, EV (reprint author), Columbia Univ, Columbia Astrophys Lab, 550 West 120th St, New York, NY 10027 USA. EM eric@astro.columbia.edu RI Boggs, Steven/E-4170-2015; Gelfand, Joseph/F-1110-2015 OI Boggs, Steven/0000-0001-9567-4224; Gelfand, Joseph/0000-0003-4679-1058 FU National Aeronautics and Space Administration; NASA through Chandra Award [SAO GO2-13097X, GO1-12068A]; NASA [NAS8-03060]; Fermi Guest Investigator [NNX12AO89G]; Australian Research Council; Science Foundation for Physics within The University of Sydney FX This work made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. This work has also made use of archival data from the Chandra X-ray Observatory. Partial support for E.V.G. and J.A.T were provided by NASA through Chandra Award Numbers SAO GO2-13097X and GO1-12068A, respectively, issued by the Chandra X-ray Observatory Center, which is operated by the Smithsonian Astrophysical Observatory for and on behalf of NASA under contract NAS8-03060. E.V.G acknowledges support by Fermi Guest Investigator Grant NNX12AO89G. Radio contours were obtained from Molonglo Observatory Synthesis Telescope (MOST) data provided by the University of Sydney with support from the Australian Research Council and the Science Foundation for Physics within The University of Sydney. NR 42 TC 13 Z9 13 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 155 DI 10.1088/0004-637X/788/2/155 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200058 ER PT J AU Liu, N Gallino, R Bisterzo, S Davis, AM Savina, MR Pellin, MJ AF Liu, Nan Gallino, Roberto Bisterzo, Sara Davis, Andrew M. Savina, Michael R. Pellin, Michael J. TI THE C-13-POCKET STRUCTURE IN AGB MODELS: CONSTRAINTS FROM ZIRCONIUM ISOTOPE ABUNDANCES IN SINGLE MAINSTREAM SiC GRAINS SO ASTROPHYSICAL JOURNAL LA English DT Article DE circumstellar matter; meteorites, meteors, meteoroids; nuclear reactions, nucleosynthesis, abundances; stars: abundances; stars: AGB and post-AGB ID GIANT BRANCH STARS; S-PROCESS NUCLEOSYNTHESIS; SILICON-CARBIDE GRAINS; CAPTURE CROSS-SECTIONS; LOW-METALLICITY STARS; NEUTRON-CAPTURE; STELLAR MODELS; REACTION-RATES; EVOLUTION; METEORITES AB We present postprocess asymptotic giant branch (AGB) nucleosynthesis models with different C-13- pocket internal structures to better explain zirconium isotope measurements in mainstream presolar SiC grains by Nicolussi et al. and Barzyk et al. We show that higher-than-solar Zr-92/Zr-94 ratios can be predicted by adopting a C-13- pocket with a flat C-13 profile, instead of the previous decreasing-with-depth C-13 profile. The improved agreement between grain data for zirconium isotopes and AGB models provides additional support for a recent proposal of a flat C-13 profile based on barium isotopes in mainstream SiC grains by Liu et al. C1 [Liu, Nan; Davis, Andrew M.; Pellin, Michael J.] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. [Liu, Nan; Davis, Andrew M.; Savina, Michael R.; Pellin, Michael J.] Chicago Ctr Cosmochem, Chicago, IL 60637 USA. [Liu, Nan; Savina, Michael R.; Pellin, Michael J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Gallino, Roberto; Bisterzo, Sara] Univ Torino, Dipartimento Fis, I-10125 Turin, Italy. [Bisterzo, Sara] INAF Osservatorio Astrofis Torino, I-10025 Pino Torinese, Italy. [Davis, Andrew M.; Pellin, Michael J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Liu, N (reprint author), Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. EM lnsmile@uchicago.edu RI Pellin, Michael/B-5897-2008; OI Pellin, Michael/0000-0002-8149-9768; Liu, Nan/0000-0002-4456-4065 FU NASA Earth and Space Sciences Fellowship Program [NNX11AN63H]; NASA Cosmo-chemistry program [NNX09AG39G]; Joint Institute for Nuclear Astrophysics (JINA, University of Notre Dame, USA); Karlsruhe Institute of Technology (KIT, Karlsruhe, Germany) FX We thank the anonymous referee for a careful and constructive reading of the manuscript. Part of the Torino model numerical calculations has been sustained by the B2FH Association (http://www.b2fh.org/). N.L. acknowledges the NASA Earth and Space Sciences Fellowship Program (NNX11AN63H) for support. This work was also supported by the NASA Cosmo-chemistry program through grant NNX09AG39G (to AMD). S. B. acknowledges financial support from the Joint Institute for Nuclear Astrophysics (JINA, University of Notre Dame, USA) and from Karlsruhe Institute of Technology (KIT, Karlsruhe, Germany). NR 39 TC 11 Z9 12 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 163 DI 10.1088/0004-637X/788/2/163 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200066 ER PT J AU Malone, CM Zingale, M Nonaka, A Almgren, AS Bell, JB AF Malone, C. M. Zingale, M. Nonaka, A. Almgren, A. S. Bell, J. B. TI MULTIDIMENSIONAL MODELING OF TYPE I X-RAY BURSTS. II. TWO-DIMENSIONAL CONVECTION IN A MIXED H/He ACCRETOR SO ASTROPHYSICAL JOURNAL LA English DT Article DE convection; hydrodynamics; methods: numerical; stars: neutron; X-rays: bursts ID EQUATION-OF-STATE; NEUTRON-STARS; SUPERNOVAE; HYDRODYNAMICS; PROPAGATION; CONSISTENCY; ENERGY; ASHES AB Type I X-ray bursts are thermonuclear explosions of accreted material on the surface of neutron stars in low-mass X-ray binaries. Prior to the ignition of a subsonic burning front, runaway burning at the base of the accreted layer drives convection that mixes fuel and heavy-element ashes. In this paper, the second in a series, we explore the behavior of this low Mach number convection in mixed hydrogen/helium layers on the surface of a neutron star using two-dimensional simulations with the Maestro code. Maestro takes advantage of the highly subsonic flow field by filtering dynamically unimportant sound waves while retaining local compressibility effects, such as those due to stratification and energy release from nuclear reactions. In these preliminary calculations, we find that the rp-process approximate network creates a convective region that is split into two layers. While this splitting appears artificial due to the approximations of the network regarding nuclear flow out of the breakout reaction Ne-18(alpha, p)(21) Na, these calculations hint at further simplifications and improvements of the burning treatment for use in subsequent calculations in three dimensions for a future paper. C1 [Malone, C. M.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Malone, C. M.; Zingale, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Nonaka, A.; Almgren, A. S.; Bell, J. B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. RP Malone, CM (reprint author), Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. EM malone@ucolick.org OI Zingale, Michael/0000-0001-8401-030X FU DOE/Office of Nuclear Physics [DE-FG02-06ER41448, DE-FG02-87ER40317]; UCSC, by the National Science Foundation [AST 0909129]; NASA Theory Program [NNX09AK36G]; DOE HEP Program [DEFC02- 06ER41438, DE-SC00010676]; Applied Mathematics Program of the DOE Office of Advance Scientific Computing Research under U.S. Department of Energy [DE-AC02-05CH11231]; National Energy Research Scientific Computing Center; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank the referee for useful comments that helped clarify some points of the paper. We especially thank Stan Woosley for providing us with data from simple Kepler burns, allowing us to compare our implementation of the approximate network to a full production network. We also thank Alex Heger for sharing some Kepler X-ray burst models, on which we based the parameterized models used here. As always, we thank Frank Timmes for making his equation of state publicly available. The work at Stony Brook was supported by DOE/Office of Nuclear Physics grants no. DE-FG02-06ER41448 and DE-FG02-87ER40317 to Stony Brook. This work was also supported, at UCSC, by the National Science Foundation (AST 0909129), the NASA Theory Program (NNX09AK36G), and especially by the DOE HEP Program through grants No. DEFC02- 06ER41438 and DE-SC00010676. The work at LBNL was supported by the Applied Mathematics Program of the DOE Office of Advance Scientific Computing Research under U.S. Department of Energy contract no. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 45 TC 3 Z9 3 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 115 DI 10.1088/0004-637X/788/2/115 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200018 ER PT J AU Materese, CK Cruikshank, DP Sandford, SA Imanaka, H Nuevo, M White, DW AF Materese, Christopher K. Cruikshank, Dale P. Sandford, Scott A. Imanaka, Hiroshi Nuevo, Michel White, Douglas W. TI ICE CHEMISTRY ON OUTER SOLAR SYSTEM BODIES: CARBOXYLIC ACIDS, NITRILES, AND UREA DETECTED IN REFRACTORY RESIDUES PRODUCED FROM THE UV PHOTOLYSIS OF N2: CH4: CO-CONTAINING ICES SO ASTROPHYSICAL JOURNAL LA English DT Article DE astrochemistry; Kuiper belt: general; molecular data; molecular processes; planets and satellites: surfaces; solid state: refractory ID CHARGED-PARTICLE IRRADIATION; TRANS-NEPTUNIAN OBJECTS; ADVANCED LIGHT-SOURCE; ULTRAVIOLET PHOTOIRRADIATION; OPTICAL-CONSTANTS; BUTYLDIMETHYLSILYL DERIVATIVES; INFRARED-SPECTROSCOPY; PREBIOTIC MOLECULES; SOLID NITROGEN; ANALOGS AB Radiation processing of the surface ices of outer solar system bodies may result in the production of new chemical species even at low temperatures. Many of the smaller, more volatile molecules that are likely produced by the photolysis of these ices have been well characterized by laboratory experiments. However, the more complex refractory material formed in these experiments remains largely uncharacterized. In this work, we present a series of laboratory experiments in which low-temperature (15-20 K) N2: CH4: CO ices in relative proportions 100: 1: 1 are subjected to UV irradiation, and the resulting materials are studied with a variety of analytical techniques including infrared spectroscopy, X-ray absorption near-edge structure spectroscopy, gas chromatography coupled with mass spectrometry, and high-resolution mass spectroscopy. Despite the simplicity of the reactants, these experiments result in the production of a highly complex mixture of molecules from relatively low-mass volatiles (tens of daltons) to high-mass refractory materials (hundreds of daltons). These products include various carboxylic acids, nitriles, and urea, which are also expected to be present on the surface of outer solar system bodies, including Pluto and other transneptunian objects. If these compounds occur in sufficient concentrations in the ices of outer solar system bodies, their characteristic bands may be detectable in the near-infrared spectra of these objects. C1 [Materese, Christopher K.; Cruikshank, Dale P.; Sandford, Scott A.; Imanaka, Hiroshi; Nuevo, Michel] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Materese, Christopher K.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Imanaka, Hiroshi] SETI Inst, Mountain View, CA 94043 USA. [Imanaka, Hiroshi] Univ Arizona, Lunar & Planetary Lab, Tucson, AZ 85721 USA. [Nuevo, Michel] Bay Area Environm Res Inst, Petaluma, CA 94952 USA. [White, Douglas W.] Jacksonville State Univ, Jacksonville, AL 36265 USA. RP Materese, CK (reprint author), NASA, Ames Res Ctr, MS 245-6, Moffett Field, CA 94035 USA. OI Materese, Christopher/0000-0003-2146-4288 NR 58 TC 15 Z9 15 U1 0 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 DI 10.1088/0004-637X/788/2/111 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200014 ER PT J AU Ofek, EO Arcavi, I Tal, D Sullivan, M Gal-Yam, A Kulkarni, SR Nugent, PE Ben-Ami, S Bersier, D Cao, Y Cenko, SB De Cia, A Filippenko, AV Fransson, C Kasliwal, MM Laher, R Surace, J Quimby, R Yaron, O AF Ofek, Eran O. Arcavi, Iair Tal, David Sullivan, Mark Gal-Yam, Avishay Kulkarni, Shrinivas R. Nugent, Peter E. Ben-Ami, Sagi Bersier, David Cao, Yi Cenko, S. Bradley De Cia, Annalisa Filippenko, Alexei V. Fransson, Claes Kasliwal, Mansi M. Laher, Russ Surace, Jason Quimby, Robert Yaron, Ofer TI INTERACTION-POWERED SUPERNOVAE: RISE-TIME VERSUS PEAK-LUMINOSITY CORRELATION AND THE SHOCK-BREAKOUT VELOCITY SO ASTROPHYSICAL JOURNAL LA English DT Article DE stars: massive; stars: mass-loss; supernovae: general ID DENSE MASS-LOSS; X-RAY-EMISSION; LIGHT CURVES; SN 2009IP; CIRCUMSTELLAR MEDIUM; LOW-RESOLUTION; CORE-COLLAPSE; STAR; WIND; OUTBURST AB Interaction of supernova (SN) ejecta with the optically thick circumstellar medium (CSM) of a progenitor star can result in a bright, long-lived shock-breakout event. Candidates for such SNe include Type IIn and superluminous SNe. If some of these SNe are powered by interaction, then there should be a specific relation between their peak luminosity, bolometric light-curve rise time, and shock-breakout velocity. Given that the shock velocity during shock breakout is not measured, we expect a correlation, with a significant spread, between the rise time and the peak luminosity of these SNe. Here, we present a sample of 15 SNe IIn for which we have good constraints on their rise time and peak luminosity from observations obtained using the Palomar Transient Factory. We report on a possible correlation between the R-band rise time and peak luminosity of these SNe, with a false-alarm probability of 3%. Assuming that these SNe are powered by interaction, combining these observables and theory allows us to deduce lower limits on the shock-breakout velocity. The lower limits on the shock velocity we find are consistent with what is expected for SNe (i.e., similar to 10(4) km s(-1)). This supports the suggestion that the early-time light curves of SNe IIn are caused by shock breakout in a dense CSM. We note that such a correlation can arise from other physical mechanisms. Performing such a test on other classes of SNe ( e. g., superluminous SNe) can be used to rule out the interaction model for a class of events. C1 [Ofek, Eran O.; Arcavi, Iair; Tal, David; Gal-Yam, Avishay; Ben-Ami, Sagi; De Cia, Annalisa; Yaron, Ofer] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Kulkarni, Shrinivas R.; Cao, Yi] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Nugent, Peter E.; Filippenko, Alexei V.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Bersier, David] Liverpool John Moores Univ, Astrophys Res Inst, Liverpool L3 5RF, Merseyside, England. [Cenko, S. Bradley] NASA Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Fransson, Claes] Stockholm Univ, AlbaNova Univ Ctr, Oskar Klein Ctr, Dept Astron, SE-10691 Stockholm, Sweden. [Kasliwal, Mansi M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Laher, Russ; Surace, Jason] CALTECH, Spitzer Sci Ctr, Pasadena, CA 91125 USA. [Quimby, Robert] Univ Tokyo, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. RP Ofek, EO (reprint author), Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. OI Sullivan, Mark/0000-0001-9053-4820; Gal-Yam, Avishay/0000-0002-3653-5598 FU Willner Family Leadership Institute Ilan Gluzman (Secaucus NJ); Israeli Ministry of Science; I-CORE Program of the Planning and Budgeting Committee; ISF; BSF; GIF; Minerva; EU/FP7 via ERC grant [307260]; Israel Science Foundation; Israel Science Foundation, Minerva, Weizmann-UK; Hubble Fellowship; Carnegie-Princeton Fellowship; Christopher R.Redlich Fund; Richard and Rhoda Goldman Fund; TABASGO Foundation; NSF [AST-1211916] FX We thank Dan Perley for obtaining some spectra. E.O.O. thanks Ehud Nakar and Orly Gnat for discussions. This paper is based on observations obtained with the Samuel Oschin Telescope as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, Las Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford, and the Weizmann Institute of Science. Some of the data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the Observatory was made possible by the generous financial support of the W. M. Keck Foundation. We are grateful for excellent staff assistance at Palomar, Lick, and Keck Observatories. E.O.O. is incumbent of the Arye Dissentshik career development chair and is grateful to support by grants from the Willner Family Leadership Institute Ilan Gluzman (Secaucus NJ), Israeli Ministry of Science, Israel Science Foundation, Minerva, Weizmann-UK and the I-CORE Program of the Planning and Budgeting Committee and The Israel Science Foundation. A. G-Y. acknowledge grants from the ISF, BSF, GIF, Minerva, the EU/FP7 via ERC grant (307260), and the I-CORE program of the Planning and Budgeting Committee and The Israel Science Foundation. M.M.K. acknowledges generous support from the Hubble Fellowship and Carnegie-Princeton Fellowship. A.V.F.'s SN group at UC Berkeley has received generous financial assistance from Gary and Cynthia Bengier, the Christopher R.Redlich Fund, the Richard and Rhoda Goldman Fund, the TABASGO Foundation, and NSF grant AST-1211916. NR 61 TC 16 Z9 16 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 154 DI 10.1088/0004-637X/788/2/154 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200057 ER PT J AU Wu, WLK Errard, J Dvorkin, C Kuo, CL Lee, AT McDonald, P Slosar, A Zahn, O AF Wu, W. L. K. Errard, J. Dvorkin, C. Kuo, C. L. Lee, A. T. McDonald, P. Slosar, A. Zahn, O. TI A GUIDE TO DESIGNING FUTURE GROUND-BASED COSMIC MICROWAVE BACKGROUND EXPERIMENTS SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic background radiation; cosmological parameters; dark energy; dark matter; inflation; large-scale structure of universe ID POLE TELESCOPE DATA; DARK-MATTER; POLARIZATION; SUPERNOVAE; EMISSION; CMB; SUBMILLIMETER; ANISOTROPIES; PARTICLES; COSMOLOGY AB In this follow-up work to the high energy physics Community Summer Study 2013 (aka Snowmass), we explore the scientific capabilities of a future Stage IV cosmic microwave background polarization experiment under various assumptions on detector count, resolution, and sky coverage. We use the Fisher matrix technique to calculate the expected uncertainties of cosmological parameters in upsilon Lambda CDM that are especially relevant to the physics of fundamental interactions, including neutrino masses, effective number of relativistic species, dark energy equation of state, dark matter annihilation, and inflationary parameters. To further chart the landscape of future cosmology probes, we include forecasted results from the baryon acoustic oscillation signal as measured by Dark Energy Spectroscopic Instrument to constrain parameters that would benefit from low redshift information. We find the following best 1 sigma constraints: sigma(M upsilon) = 15 meV, sigma(N-eff) = 0.0156, dark energy figure of merit = 303, sigma(p(ann)) = 0.00588 x 3 x 10(-26) cm(3) s(-1) GeV-1, sigma(Omega K) = 0.00074,s(alpha(s)) = 0.00110, s(as) = 0.00145, and sigma(r) = 0.00009. We also detail the dependencies of the parameter constraints on detector count, resolution, and sky coverage. C1 [Wu, W. L. K.; Kuo, C. L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Wu, W. L. K.; Kuo, C. L.] SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Errard, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Center, Berkeley, CA 94720 USA. [Errard, J.; Lee, A. T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Dvorkin, C.] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. [Lee, A. T.; McDonald, P.; Zahn, O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Slosar, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Zahn, O.] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. RP Wu, WLK (reprint author), Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. OI Wu, Kimmy/0000-0001-5411-6920; McDonald, Patrick/0000-0001-8346-8394 FU National Science Foundation [AST-0807444, ANT-0638937, ANT-0130612]; NSF grant [PHY-088855425]; Raymond and Beverly Sackler Funds; NSF Faculty Early Career Development (CAREER) Award [1056465]; U.S. Department of Energy Office of Science; Alfred P. Sloan Research Fellowship FX We acknowledge the use of the PSM, developed by the Component Separation Working Group (WG2) of the Planck Collaboration. We also used CAMB and an implementation of iterative delensing developed by Wei-Hsieng Teng. C.D. was supported by the National Science Foundation grant number AST-0807444, NSF grant number PHY-088855425, and the Raymond and Beverly Sackler Funds. C.L.K. acknowledges the support of an Alfred P. Sloan Research Fellowship and an NSF Faculty Early Career Development (CAREER) Award (award number: 1056465). A.T.L. acknowledges support from the U.S. Department of Energy Office of Science. O.Z. acknowledges support by National Science Foundation through grants ANT-0638937 and ANT-0130612. NR 88 TC 46 Z9 46 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2014 VL 788 IS 2 AR 138 DI 10.1088/0004-637X/788/2/138 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AJ2DT UT WOS:000337466200041 ER PT J AU Aytug, T Bogorin, DF Paranthaman, PM Mathis, JE Simpson, JT Christen, DK AF Aytug, Tolga Bogorin, Daniela F. Paranthaman, Parans M. Mathis, John E. Simpson, John T. Christen, David K. TI Superhydrophobic ceramic coatings enabled by phase-separated nanostructured composite TiO2-Cu2O thin films SO NANOTECHNOLOGY LA English DT Article DE nanostructure; superhydrophobic; phase-separation; thin-film ID ELECTROCHEMICAL DEPOSITION; SURFACES; WETTABILITY; WATER; FABRICATION; TIO2; ADHESION; ZNO AB By exploiting phase-separation in oxide materials, we present a simple and potentially low-cost approach to create exceptional superhydrophobicity in thin-film based coatings. By selecting the TiO2-Cu2O system and depositing through magnetron sputtering onto single crystal and metal templates, we demonstrate growth of nanostructured, chemically phase-segregated composite films. These coatings, after appropriate chemical surface modification, demonstrate a robust, non-wetting Cassie-Baxter state and yield an exceptional superhydrophobic performance, with water droplet contact angles reaching to similar to 172 degrees and sliding angles <1 degrees. As an added benefit, despite the photo-active nature of TiO2, the chemically coated composite film surfaces display UV stability and retain superhydrophobic attributes even after exposure to UV (275 nm) radiation for an extended period of time. The present approach could benefit a variety of outdoor applications of superhydrophobic coatings, especially for those where exposure to extreme atmospheric conditions is required. C1 [Aytug, Tolga; Paranthaman, Parans M.; Simpson, John T.; Christen, David K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bogorin, Daniela F.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Mathis, John E.] Embry Riddle Aeronaut Univ, Daytona Beach, FL 32114 USA. RP Aytug, T (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM aytugt@ornl.gov FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; UT-Battelle; LLC for the US Department of Energy FX This work was supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC for the US Department of Energy. Microstructural property research was conducted at the Center for Nanophase Materials Sciences (CNMS), which are sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of BES, US DOE. NR 39 TC 1 Z9 1 U1 7 U2 75 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUN 20 PY 2014 VL 25 IS 24 AR 245601 DI 10.1088/0957-4484/25/24/245601 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AI8NE UT WOS:000337173600008 PM 24857856 ER PT J AU Zheng, XY Lee, H Weisgraber, TH Shusteff, M DeOtte, J Duoss, EB Kuntz, JD Biener, MM Ge, Q Jackson, JA Kucheyev, SO Fang, NX Spadaccini, CM AF Zheng, Xiaoyu Lee, Howon Weisgraber, Todd H. Shusteff, Maxim DeOtte, Joshua Duoss, Eric B. Kuntz, Joshua D. Biener, Monika M. Ge, Qi Jackson, Julie A. Kucheyev, Sergei O. Fang, Nicholas X. Spadaccini, Christopher M. TI Ultralight, Ultrastiff Mechanical Metamaterials SO SCIENCE LA English DT Article ID METALLIC MICROLATTICES; COMPRESSIVE BEHAVIOR; DEFORMATION; FILTRATION; STIFFNESS; STRENGTH; SILICA; KELVIN; FOAMS AB The mechanical properties of ordinary materials degrade substantially with reduced density because their structural elements bend under applied load. We report a class of microarchitected materials that maintain a nearly constant stiffness per unit mass density, even at ultralow density. This performance derives from a network of nearly isotropic microscale unit cells with high structural connectivity and nanoscale features, whose structural members are designed to carry loads in tension or compression. Production of these microlattices, with polymers, metals, or ceramics as constituent materials, is made possible by projection microstereolithography (an additive micromanufacturing technique) combined with nanoscale coating and postprocessing. We found that these materials exhibit ultrastiff properties across more than three orders of magnitude in density, regardless of the constituent material. C1 [Zheng, Xiaoyu; Weisgraber, Todd H.; Shusteff, Maxim; DeOtte, Joshua; Duoss, Eric B.; Kuntz, Joshua D.; Biener, Monika M.; Jackson, Julie A.; Kucheyev, Sergei O.; Spadaccini, Christopher M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lee, Howon; Ge, Qi; Fang, Nicholas X.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. RP Zheng, XY (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM zheng3@llnl.gov; nicfang@mit.edu; spadaccini2@llnl.gov RI Fang, Nicholas/A-5856-2008; Lee, Howon/A-1486-2012; Ge, Qi/B-2485-2015; OI Fang, Nicholas/0000-0001-5713-629X; Lee, Howon/0000-0001-5778-2398; Ge, Qi/0000-0002-8666-8532; Zheng, Xiaoyu/0000-0001-8685-5728 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LDRD Strategic Initiative [11-SI-005]; DARPA MCMA (Materials with Controlled Microstructural Architecture) FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. Supported by LDRD Strategic Initiative 11-SI-005 and DARPA MCMA (Materials with Controlled Microstructural Architecture, Program Manager J. Goldwasser). The authors at Lawrence Livermore National Laboratory thank H. Rathbun for useful discussions on modeling the lattice structures, M. Worsley for taking SEM images, and C. Harvey for technical support. N.X.F. thanks S. Cai at University of California San Diego for insightful input regarding buckling modes in ceramic octet-truss lattices (LLNL-JRNL-640334). NR 44 TC 167 Z9 169 U1 84 U2 427 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 20 PY 2014 VL 344 IS 6190 BP 1373 EP 1377 DI 10.1126/science.1252291 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2YQ UT WOS:000337531700034 PM 24948733 ER PT J AU Zherebetskyy, D Scheele, M Zhang, YJ Bronstein, N Thompson, C Britt, D Salmeron, M Alivisatos, P Wang, LW AF Zherebetskyy, Danylo Scheele, Marcus Zhang, Yingjie Bronstein, Noah Thompson, Christopher Britt, David Salmeron, Miquel Alivisatos, Paul Wang, Lin-Wang TI Hydroxylation of the surface of PbS nanocrystals passivated with oleic acid SO SCIENCE LA English DT Article ID COLLOIDAL NANOCRYSTALS; SHAPE; WATER; DISSOCIATION; NANOPARTICLES; CHEMISTRY; EVOLUTION; FACETS; GROWTH; POLAR AB Controlling the structure of colloidal nanocrystals (NCs) is key to the generation of their complex functionality. This requires an understanding of the NC surface at the atomic level. The structure of colloidal PbS NCs passivated with oleic acid has been studied theoretically and experimentally. We show the existence of surface OH-groups, which play a key role in stabilizing the PbS(111) facets, consistent with x-ray photoelectron spectroscopy as well as other spectroscopic and chemical experiments. The role of water in the synthesis process is also revealed. Our model, along with existing observations of NC surface termination and passivation by ligands, helps to explain and predict the properties of NCs and their assemblies. C1 [Zherebetskyy, Danylo; Scheele, Marcus; Zhang, Yingjie; Thompson, Christopher; Salmeron, Miquel; Alivisatos, Paul; Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Scheele, Marcus; Bronstein, Noah; Thompson, Christopher; Alivisatos, Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Zhang, Yingjie] Univ Calif Berkeley, Appl Sci & Technol Grad Program, Berkeley, CA 94720 USA. [Britt, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Wang, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM lwwang@lbl.gov RI Britt, David/D-4675-2009; Zherebetskyy, Danylo/B-3404-2015; Foundry, Molecular/G-9968-2014; Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU Office of Science, the Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy (DOE) through the organic/inorganic nanocomposite program [DE-AC02-05CH11231]; Office of Science of the DOE [DE-AC05-00OR22725]; Alexander von Humboldt-Foundation FX We thank R. Cai and Z. Zhu for helpful discussions and J. Engel for help in the XPS experiments. This work was supported by the Director, Office of Science, the Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy (DOE) through the organic/inorganic nanocomposite program under contract DE-AC02-05CH11231. It used resources of the National Energy Research Scientific Computing Center, the Molecular Foundry, and the Advanced Light Source, which are supported by the Office of Science of the DOE. Computations also used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the DOE under contract no. DE-AC05-00OR22725, with computational time allocated by the Innovative and Novel Computational Impact on Theory and Experiment project. M. S. thanks the Alexander von Humboldt-Foundation for a Feodor Lynen-Fellowship. Materials and methods, supporting information, and the coordinates of NC models are included in the supplementary materials. NR 36 TC 85 Z9 85 U1 26 U2 193 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 20 PY 2014 VL 344 IS 6190 BP 1380 EP 1384 DI 10.1126/science.1252727 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2YQ UT WOS:000337531700036 PM 24876347 ER PT J AU Lee, K Zhong, XF Gu, SY Kruel, AM Dorner, MB Perry, K Rummel, A Dong, M Jin, RS AF Lee, Kwangkook Zhong, Xiaofen Gu, Shenyan Kruel, Anna Magdalena Dorner, Martin B. Perry, Kay Rummel, Andreas Dong, Min Jin, Rongsheng TI Molecular basis for disruption of E-cadherin adhesion by botulinum neurotoxin A complex SO SCIENCE LA English DT Article ID CLOSTRIDIUM-BOTULINUM; ADHERENS JUNCTIONS; CRYSTAL-STRUCTURE; ORAL TOXICITIES; BINDING; CELL; TOXINS; TRANSCYTOSIS; DOMAINS AB How botulinum neurotoxins (BoNTs) cross the host intestinal epithelial barrier in foodborne botulism is poorly understood. Here, we present the crystal structure of a clostridial hemagglutinin (HA) complex of serotype BoNT/A bound to the cell adhesion protein E-cadherin at 2.4 angstroms. The HA complex recognizes E-cadherin with high specificity involving extensive intermolecular interactions and also binds to carbohydrates on the cell surface. Binding of the HA complex sequesters E-cadherin in the monomeric state, compromising the E-cadherin-mediated intercellular barrier and facilitating paracellular absorption of BoNT/A. We reconstituted the complete 14-subunit BoNT/A complex using recombinantly produced components and demonstrated that abolishing either E-cadherin- or carbohydrate-binding of the HA complex drastically reduces oral toxicity of BoNT/A complex in vivo. Together, these studies establish the molecular mechanism of how HAs contribute to the oral toxicity of BoNT/A. C1 [Lee, Kwangkook; Gu, Shenyan; Jin, Rongsheng] Univ Calif Irvine, Dept Physiol & Biophys, Irvine, CA 92697 USA. [Zhong, Xiaofen; Dong, Min] Harvard Univ, Sch Med, Dept Microbiol & Immunol, Div Neurosci,New England Primate Res Ctr, Southborough, MA 01772 USA. [Kruel, Anna Magdalena; Rummel, Andreas] Hannover Med Sch, Inst Toxikol, D-30625 Hannover, Germany. [Dorner, Martin B.] Robert Koch Inst, Ctr Biol Threats & Special Pathogens Biol Toxins, D-13353 Berlin, Germany. [Perry, Kay] Cornell Univ, Northeastern Collaborat Access Team NE CAT, Argonne Natl Lab, Argonne, IL 60439 USA. [Perry, Kay] Cornell Univ, Dept Chem & Chem Biol, Argonne Natl Lab, Argonne, IL 60439 USA. RP Jin, RS (reprint author), Univ Calif Irvine, Dept Physiol & Biophys, Irvine, CA 92697 USA. EM r.jin@uci.edu RI Jin, Rongsheng/M-7797-2013 OI Jin, Rongsheng/0000-0003-0348-7363 FU National Institute of Allergy and Infectious Diseases (NIAID) [R01AI091823]; NIH [8P51OD011103-51, 1R56AI097834-01, 1R01NS080833-01]; Swiss Federal Office for Civil Protection BABS [353003325]; National Institute of General Medical Sciences [P41 GM103403]; U.S. DOE [DE-AC02-06CH11357] FX We thank A. Bobkov for technical assistance. This work was partly supported by National Institute of Allergy and Infectious Diseases (NIAID) grant R01AI091823 to R.J.; by the NIH grant 8P51OD011103-51 (to the New England Primate Research Center), 1R56AI097834-01, and 1R01NS080833-01 to M. D.; and by the Swiss Federal Office for Civil Protection BABS #353003325 to A. R. NE-CAT at the Advanced Photon Source (APS) is supported by a grant from the National Institute of General Medical Sciences (P41 GM103403). Use of the APS, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under contract DE-AC02-06CH11357. The atomic coordinates and structure factors of the mini-HA-EC1-EC2 complex have been deposited in the Protein Data Bank under the accession code 4QD2. BoNT availability is subject to the restrictions that apply to Centers for Disease Control and Prevention select agents and NIAID Category A pathogens. R.J. is named as an inventor on a U.S. patent application applied for by University of California, Irvine related to oral drug delivery systems. NR 28 TC 24 Z9 24 U1 0 U2 27 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 20 PY 2014 VL 344 IS 6190 BP 1405 EP 1410 DI 10.1126/science.1253823 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2YQ UT WOS:000337531700042 PM 24948737 ER PT J AU Engelhardt, L Demmel, F Luban, M Timco, GA Tuna, F Winpenny, REP AF Engelhardt, Larry Demmel, Franz Luban, Marshall Timco, Grigore A. Tuna, Floriana Winpenny, Richard E. P. TI Refined model of the {Fe-9} magnetic molecule from low-temperature inelastic neutron scattering studies SO PHYSICAL REVIEW B LA English DT Article AB We present a refined model of the {Fe-9} tridiminished icosahedron magnetic molecule system. This molecule was originally modeled as being composed of two ({Fe-3} and {Fe-6}) clusters, with the Fe3+ ions within each cluster being coupled via exchange interactions, but with no coupling between the clusters. The present inelastic neutron scattering (INS) measurements were used to probe the low-lying energy spectrum of {Fe-9}, and these results demonstrate that the previously published model of two uncoupled clusters is incomplete. To achieve agreement between the experiment and theory, we have augmented the model with relatively small exchange coupling between the clusters. A combination of Lanczos matrix diagonalization and quantum Monte Carlo simulations have been used to achieve good agreement between the experimental data and the improved model of the full {Fe-9} system despite the complexity of this model (with Hilbert space dimension >10(7)). C1 [Engelhardt, Larry] Francis Marion Univ, Dept Phys & Astron, Florence, SC 29501 USA. [Demmel, Franz] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Luban, Marshall] Iowa State Univ, Dept Phys & Astron, Ames Lab, Ames, IA 50011 USA. [Timco, Grigore A.; Tuna, Floriana; Winpenny, Richard E. P.] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England. RP Engelhardt, L (reprint author), Francis Marion Univ, Dept Phys & Astron, Florence, SC 29501 USA. EM lengelhardt@fmarion.edu FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-07CH11358] FX We thank D. Vaknin for useful discussions. L.E. acknowledges the NSF EPSCoR RII Track 1 cooperative agreement awarded to the University of South Carolina which provided the computational resources that were used. F.D. acknowledges the superb support of the ISIS cryogenics team. The work at Ames Laboratory was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC02-07CH11358. NR 15 TC 0 Z9 0 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 19 PY 2014 VL 89 IS 21 AR 214415 DI 10.1103/PhysRevB.89.214415 PG 8 WC Physics, Condensed Matter SC Physics GA AN5UU UT WOS:000340657700001 ER PT J AU Shin, H Schwarze, A Diehl, RD Pussi, K Colombier, A Gaudry, E Ledieu, J McGuirk, GM Loli, LNS Fournee, V Wang, LL Schull, G Berndt, R AF Shin, Heekeun Schwarze, A. Diehl, R. D. Pussi, K. Colombier, A. Gaudry, E. Ledieu, J. McGuirk, G. M. Loli, L. N. Serkovic Fournee, V. Wang, L. L. Schull, G. Berndt, R. TI Structure and dynamics of C-60 molecules on Au(111) SO PHYSICAL REVIEW B LA English DT Article ID AG(111) SURFACES; METAL-SURFACES; GROUND-STATE; SOLID C-60; RECONSTRUCTION; FULLERENES; CU(111); GROWTH; FILMS AB Earlier studies of C-60 adsorption on Au(111) reported many interesting and complex features. We have performed coordinated low-energy electron diffraction, scanning tunneling microscopy (STM), and density functional theory studies to elucidate some of the details of the monolayer commensurate (2 root 3 x 2 root 3) R30 degrees phase. We have identified the adsorption geometries of the two states that image as dim and bright in STM. These consist of a C-60 molecule with a hexagon side down in a vacancy (hex-vac) and a C-60 molecule with a carbon-carbon 6: 6 bond down on a top site (6:6-top), respectively. We have studied the detailed geometries of these states and find that there is little distortion of the C-60 molecules, but there is a rearrangement of the substrate near the C-60 molecules. The two types of molecules differ in height, by about 0.7 angstrom, which accounts for most of the difference in their contrast in the STM images. The monolayer displays dynamical behavior, in which the molecules flip from bright to dim, and vice versa. We interpret this flipping as the result of the diffusion of vacancies in the surface layers of the substrate. Our measurements of the dynamics of this flipping from one state to the other indicate that the activation energy is 0.66 +/- 0.03 eV for flips that involve nearest-neighbor C-60 molecules, and 0.93 +/- 0.03 for more distant flips. Based on calculated activation energies for vacancies diffusing in Au, we interpret these to be a result of surface vacancy diffusion and bulk vacancy diffusion. These results are compared to the similar system of Ag(111)-(2 root 3 x 2 root 3) R30 degrees- C-60. In both systems, the formation of the commensurate C-60 monolayer produces a large number of vacancies in the top substrate layer that are highly mobile, effectively melting the interfacial metal layer at temperatures well below their normal melting temperatures. C1 [Shin, Heekeun; Schwarze, A.; Diehl, R. D.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Pussi, K.] Lappeenranta Univ Technol, Dept Math & Phys, FIN-53851 Lappeenranta, Finland. [Colombier, A.; Gaudry, E.; Ledieu, J.; McGuirk, G. M.; Loli, L. N. Serkovic; Fournee, V.] Univ Lorraine, CNRS, Inst Jean Lamour, UMR 7198, F-54011 Nancy, France. [Wang, L. L.] US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Schull, G.] Univ Strasbourg, UMR 7504, Inst Phys & Chim Mat Strasbourg, F-67034 Strasbourg, France. [Berndt, R.] Univ Kiel, Inst Expt & Angew Phys, D-24098 Kiel, Germany. RP Shin, H (reprint author), Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA. RI Ledieu, Julian/F-1430-2010; Gaudry, Emilie/G-9682-2011; Serkovic Loli, Laura/C-9603-2015; Schull, Guillaume/B-6256-2016 FU DAAD; CNRS [PICS05892]; Academy of Finland [130818, 263634]; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; LDRD; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We thank D. L. Allara for the use of the Au(111) crystal in LEED experiments and Kristin Marino for assistance with preparing figures. A. S. gratefully acknowledges DAAD for the financial support for summer research at Penn State. We also thank the CNRS for the INCAS project (No. PICS05892) funding, Academy of Finland Projects No. 130818 and No. 263634, and CSC-IT Center for Science. The work at the Ames Laboratory was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Additional capabilities were made possible from LDRD funding for materials discovery and design. Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 40 TC 13 Z9 13 U1 8 U2 61 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 19 PY 2014 VL 89 IS 24 AR 245428 DI 10.1103/PhysRevB.89.245428 PG 11 WC Physics, Condensed Matter SC Physics GA AN5UX UT WOS:000340658000004 ER PT J AU Durand, M Kraynik, AM van Swol, F Kafer, J Quilliet, C Cox, S Talebi, SA Graner, F AF Durand, Marc Kraynik, Andrew M. van Swol, Frank Kaefer, Jos Quilliet, Catherine Cox, Simon Talebi, Shirin Ataei Graner, Francois TI Statistical mechanics of two-dimensional shuffled foams: Geometry-topology correlation in small or large disorder limits SO PHYSICAL REVIEW E LA English DT Article ID CELLULAR STRUCTURES; 2 DIMENSIONS; PATTERNS AB Bubble monolayers are model systems for experiments and simulations of two-dimensional packing problems of deformable objects. We explore the relation between the distributions of the number of bubble sides (topology) and the bubble areas (geometry) in the low liquid fraction limit. We use a statistical model [M. Durand, Europhys. Lett. 90, 60002 (2010)] which takes into account Plateau laws. We predict the correlation between geometrical disorder (bubble size dispersity) and topological disorder (width of bubble side number distribution) over an extended range of bubble size dispersities. Extensive data sets arising from shuffled foam experiments, SURFACE EVOLVER simulations, and cellular Potts model simulations all collapse surprisingly well and coincide with the model predictions, even at extremely high size dispersity. At moderate size dispersity, we recover our earlier approximate predictions [M. Durand, J. Kafer, C. Quilliet, S. Cox, S. A. Talebi, and F. Graner, Phys. Rev. Lett. 107, 168304 (2011)]. At extremely low dispersity, when approaching the perfectly regular honeycomb pattern, we study how both geometrical and topological disorders vanish. We identify a crystallization mechanism and explore it quantitatively in the case of bidisperse foams. Due to the deformability of the bubbles, foams can crystallize over a larger range of size dispersities than hard disks. The model predicts that the crystallization transition occurs when the ratio of largest to smallest bubble radii is 1.4. C1 [Durand, Marc; Graner, Francois] MSC, F-75205 Paris 13, France. [Kraynik, Andrew M.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [van Swol, Frank] Sandia Natl Labs, Albuquerque, NM 87185 USA. [van Swol, Frank] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM USA. [Kaefer, Jos] Lab Biometrie & Biol Evolut, F-69622 Villeurbanne, France. [Quilliet, Catherine; Talebi, Shirin Ataei] Lab Interdisciplinaire Phys, F-38402 St Martin Dheres, France. [Cox, Simon] Aberystwyth Univ, Dept Math, Aberystwyth SY23 3BZ, Dyfed, Wales. [Cox, Simon] Aberystwyth Univ, Dept Phys, Aberystwyth SY23 3BZ, Dyfed, Wales. RP Durand, M (reprint author), CNRS, UMR 7057, F-75700 Paris, France. EM marc.durand@univ-paris-diderot.fr RI Kafer, Jos/E-7714-2017; OI Kafer, Jos/0000-0002-0561-8008; Cox, Simon/0000-0001-6129-3394 FU FP7 IAPP project HYDROFRAC [PIAP-GA-2009-251475]; Royal Academy of Engineering; United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX J.K. thanks A. F. M. Maree for help with the Potts simulations. A. M. K. thanks P. Grassia, G. Schroeder-Turk, and K. Mecke for their hospitality. S. C. thanks the FP7 IAPP project HYDROFRAC (Grant No. PIAP-GA-2009-251475) for funding. S. C. and A. M. K. acknowledge financial support from the Royal Academy of Engineering Distinguished Visiting Fellowship Scheme, and hospitality from S. Neethling. F. v. S. is supported by the United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. M. D., C. Q., and F. G. have belonged to the CNRS consortium "Foams and Emulsions," F. G. and J.K. to the CNRS consortium "CellTis," and M. D. to the CNRS consortium "MePhy." NR 40 TC 4 Z9 4 U1 2 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUN 19 PY 2014 VL 89 IS 6 AR 062309 DI 10.1103/PhysRevE.89.062309 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AN5VI UT WOS:000340659200003 PM 25019778 ER PT J AU van Tilborg, J Daniels, J Gonsalves, AJ Schroeder, CB Esarey, E Leemans, WP AF van Tilborg, J. Daniels, J. Gonsalves, A. J. Schroeder, C. B. Esarey, E. Leemans, W. P. TI Measurement of the laser-pulse group velocity in plasma waveguides SO PHYSICAL REVIEW E LA English DT Article ID ACCELERATORS AB Electrically discharged plasma channels can guide laser pulses, extending the laser-plasma interaction length to many Rayleigh ranges. In applications such as the laser-plasma accelerator, the laser group velocity in the channel plays a critical role. The laser travel time (and thus the averaged group velocity) was measured through two-pulse frequency-domain interferometry and was found to depend on the on-axis plasma density and laser spot size. The data is in agreement with theory. C1 [van Tilborg, J.; Daniels, J.; Gonsalves, A. J.; Schroeder, C. B.; Esarey, E.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Daniels, J.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. RP van Tilborg, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RI Daniels, Joost/N-2378-2015; OI Daniels, Joost/0000-0002-9480-6077; Schroeder, Carl/0000-0002-9610-0166 FU Office of Science, Office of High Energy Physics of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge contributions from F. Mollica. This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 16 TC 8 Z9 8 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUN 19 PY 2014 VL 89 IS 6 AR 063103 DI 10.1103/PhysRevE.89.063103 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AN5VI UT WOS:000340659200007 PM 25019900 ER PT J AU Bulla, I Schultz, AK Chesneau, C Mark, T Serea, F AF Bulla, Ingo Schultz, Anne-Kathrin Chesneau, Christophe Mark, Tanya Serea, Florin TI A model-based information sharing protocol for profile Hidden Markov Models used for HIV-1 recombination detection SO BMC BIOINFORMATICS LA English DT Article ID IMMUNODEFICIENCY-VIRUS TYPE-1; NATURAL-POPULATIONS; GENETIC DIVERSITY; SUBTYPE-I; CLASSIFICATION; SEQUENCES; COMPLEX; IDENTIFICATION; EVOLUTIONARY; BREAKPOINTS AB Background: In many applications, a family of nucleotide or protein sequences classified into several subfamilies has to be modeled. Profile Hidden Markov Models (pHMMs) are widely used for this task, modeling each subfamily separately by one pHMM. However, a major drawback of this approach is the difficulty of dealing with subfamilies composed of very few sequences. One of the most crucial bioinformatical tasks affected by the problem of small-size subfamilies is the subtyping of human immunodeficiency virus type 1 (HIV-1) sequences, i.e., HIV-1 subtypes for which only a small number of sequences is known. Results: To deal with small samples for particular subfamilies of HIV-1, we introduce a novel model-based information sharing protocol. It estimates the emission probabilities of the pHMM modeling a particular subfamily not only based on the nucleotide frequencies of the respective subfamily but also incorporating the nucleotide frequencies of all available subfamilies. To this end, the underlying probabilistic model mimics the pattern of commonality and variation between the subtypes with regards to the biological characteristics of HI viruses. In order to implement the proposed protocol, we make use of an existing HMM architecture and its associated inference engine. Conclusions: We apply the modified algorithm to classify HIV-1 sequence data in the form of partial HIV-1 sequences and semi-artificial recombinants. Thereby, we demonstrate that the performance of pHMMs can be significantly improved by the proposed technique. Moreover, we show that our algorithm performs significantly better than Simplot and Bootscanning. C1 [Bulla, Ingo] Ernst Moritz Arndt Univ Greifswald, Inst Math & Informat, D-17487 Greifswald, Germany. [Bulla, Ingo] Los Alamos Natl Lab, Grp T 6, Los Alamos, NM USA. [Schultz, Anne-Kathrin] Univ Gottingen, Inst Microbiol & Genet, D-37077 Gottingen, Germany. [Chesneau, Christophe] Univ Caen, LMNO, CNRS, UMR 6139, F-14032 Caen, France. [Mark, Tanya] Univ Guelph, Guelph, ON N1G 2W1, Canada. [Serea, Florin] Tech Univ Gheorghe Asachi, Fac Elect Engn Power Engn & Appl Informat, Iasi 700050, Romania. RP Bulla, I (reprint author), Ernst Moritz Arndt Univ Greifswald, Inst Math & Informat, Walther Rathenau Str 47, D-17487 Greifswald, Germany. EM ingobulla@gmail.com OI Schultz, Anne-Kathrin/0000-0002-0963-4275 FU Deutsche Forschungsgemeinschaft [STA 1009/5-1, BU 2685/4-1]; National Institutes of Health [AI087520] FX This work was supported by the Deutsche Forschungsgemeinschaft (STA 1009/5-1 and BU 2685/4-1) and the National Institutes of Health (AI087520). We thank Thomas Leitner for his comments on the draft. NR 50 TC 2 Z9 2 U1 0 U2 9 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2105 J9 BMC BIOINFORMATICS JI BMC Bioinformatics PD JUN 19 PY 2014 VL 15 AR 205 DI 10.1186/1471-2105-15-205 PG 16 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Mathematical & Computational Biology SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Mathematical & Computational Biology GA AL8RG UT WOS:000339406000001 PM 24946781 ER PT J AU Parfrey, LW Walters, WA Lauber, CL Clemente, JC Berg-Lyons, D Teiling, C Kodira, C Mohiuddin, M Brunelle, J Driscoll, M Fierer, N Gilbert, JA Knight, R AF Parfrey, Laura Wegener Walters, William A. Lauber, Christian L. Clemente, Jose C. Berg-Lyons, Donna Teiling, Clotilde Kodira, Chinnappa Mohiuddin, Mohammed Brunelle, Julie Driscoll, Mark Fierer, Noah Gilbert, Jack A. Knight, Rob TI Communities of microbial eukaryotes in the mammalian gut within the context of environmental eukaryotic diversity SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE protist; microbial ecology; microbial diversity; salinity; host-associated eukaryotes; parasites; intestinal protozoa; human microbiome ID AIRBORNE BACTERIAL COMMUNITIES; PROTISTAN DIVERSITY; MAXIMUM-LIKELIHOOD; FUNGAL MICROBIOTA; HUMAN SKIN; BLASTOCYSTIS; SOIL; EVOLUTIONARY; SEQUENCES; CHILDREN AB Eukaryotic microbes (protists) residing in the vertebrate gut influence host health and disease, but their diversity and distribution in healthy hosts is poorly understood. Protists found in the gut are typically considered parasites, but many are commensal and some are beneficial. Further, the hygiene hypothesis predicts that association with our co-evolved microbial symbionts may be important to overall health. It is therefore imperative that we understand the normal diversity of our eukaryotic gut microbiota to test for such effects and avoid eliminating commensal organisms. We assembled a dataset of healthy individuals from two populations, one with traditional, agrarian lifestyles and a second with modern, westernized lifestyles, and characterized the human eukaryotic microbiota via high-throughput sequencing. To place the human gut microbiota within a broader context our dataset also includes gut samples from diverse mammals and samples from other aquatic and terrestrial environments. We curated the SILVA ribosomal database to reflect current knowledge of eukaryotic taxonomy and employ it as a phylogenetic framework to compare eukaryotic diversity across environment. We show that adults from the non-western population harbor a diverse community of protists, and diversity in the human gut is comparable to that in other mammals. However, the eukaryotic microbiota of the western population appears depauperate. The distribution of symbionts found in mammals reflects both host phylogeny and diet. Eukaryotic microbiota in the gut are less diverse and more patchily distributed than bacteria. More broadly, we show that eukaryotic communities in the gut are less diverse than in aquatic and terrestrial habitats, and few taxa are shared across habitat types, and diversity patterns of eukaryotes are correlated with those observed for bacteria. These results outline the distribution and diversity of microbial eukaryotic communities in the mammalian gut and across environments. C1 [Parfrey, Laura Wegener; Clemente, Jose C.; Berg-Lyons, Donna; Knight, Rob] Univ Colorado, Biofrontiers Inst, Boulder, CO 80309 USA. [Walters, William A.] Univ Colorado, Dept Mol Cellular & Dev Biol, Boulder, CO 80309 USA. [Lauber, Christian L.; Fierer, Noah] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Teiling, Clotilde; Kodira, Chinnappa; Mohiuddin, Mohammed; Brunelle, Julie; Driscoll, Mark] Roche Co, Branford, CT USA. [Fierer, Noah] Univ Colorado, Dept Ecol & Evolutionary Biol, Boulder, CO 80309 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. RP Parfrey, LW (reprint author), Univ British Columbia, Biofrontiers Inst, 3529-6270 Univ Blvd, Vancouver, BC V6T 1Z4, Canada. EM lwparfrey@botany.ubc.ca RI Knight, Rob/D-1299-2010 FU National Science Foundation; Crohn's and Colitis Foundation of America [WU-09-72]; National Institutes of Health [NHGRI HG004872-03]; Howard Hughes Medical Institute FX Many thanks to Jessica Metcalf for helpful discussions and comments throughout. Thanks to Se Jin Song and Jon Leff for comments and consultations on statistics and to Antonio Gonzalez for technical help. We wish to thank the National Ecological Observatory Network (a project sponsored by the National Science Foundation and managed under cooperative agreement by NEON, Inc.) for donation of the soil samples. Thanks to Jeffrey Gordon for providing access to fecal samples. Funding was provided the Crohn's and Colitis Foundation of America to Rob Knight (WU-09-72), National Institutes of Health to Rob Knight (NHGRI HG004872-03) and the Howard Hughes Medical Institute. NR 90 TC 21 Z9 22 U1 9 U2 97 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUN 19 PY 2014 VL 5 AR 298 DI 10.3389/fmicb.2014.00298 PG 13 WC Microbiology SC Microbiology GA AK9DV UT WOS:000338728700001 PM 24995004 ER PT J AU Guslienko, KY Kakazei, GN Kobljanskyj, YV Melkov, GA Novosad, V Slavin, AN AF Guslienko, K. Y. Kakazei, G. N. Kobljanskyj, Yu V. Melkov, G. A. Novosad, V. Slavin, A. N. TI Microwave absorption properties of permalloy nanodots in the vortex and quasi-uniform magnetization states SO NEW JOURNAL OF PHYSICS LA English DT Article DE ferromagnetic resonance; magnetic vortex; dynamical susceptibility; magnetic dot; microwaves ID FERROMAGNETIC-RESONANCE; FREQUENCY; DOTS AB When the in-plane bias magnetic field acting on a flat circular magnetic dot is smaller than the saturation field, there are two stable competing magnetization configurations of the dot: the vortex and the quasi-uniform (C-state). We measured microwave absorption properties in an array of non-interacting permalloy dots in the frequency range 1-8 GHz when the in-plane bias magnetic field was varied in the region of the dot magnetization state bi-stability. We found that the microwave absorption properties in the vortex and quasi-uniform stable states are substantially different, so that switching between these states in a fixed bias field can be used for the development of reconfigurable microwave magnetic materials. C1 [Guslienko, K. Y.] Univ Basque Country, UPV EHU, Dept Fis Mat, San Sebastian 20018, Spain. [Guslienko, K. Y.] Basque Fdn Sci, Ikerbasque, Bilbao 48011, Spain. [Kakazei, G. N.] Univ Porto, Dept Fis & Astron, IFIMUP, P-4169007 Oporto, Portugal. [Kakazei, G. N.] Univ Porto, Dept Fis & Astron, IN Inst Nanosci & Nanotechnol, P-4169007 Oporto, Portugal. [Kakazei, G. N.] Natl Acad Sci Ukraine, Inst Magnetism, UA-03142 Kiev, Ukraine. [Kobljanskyj, Yu V.; Melkov, G. A.] Taras Shevchenko Natl Univ Kyiv, Fac Radiophys, UA-01601 Kiev, Ukraine. [Novosad, V.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Slavin, A. N.] Oakland Univ, Dept Phys, Rochester, MI 48309 USA. RP Guslienko, KY (reprint author), Univ Basque Country, UPV EHU, Dept Fis Mat, San Sebastian 20018, Spain. EM kostyantyn.gusliyenko@ehu.es RI Kakazei, Gleb/A-5106-2008; Novosad, V /J-4843-2015 OI Kakazei, Gleb/0000-0001-7081-581X; FU State Fund for Fundamental Research of Ukraine [UU34/008]; National Science Foundation of USA [DMR-1015175]; DARPA; US Army TARDEC; US DOE Office of Science [DEAC02-06CH11357]; Spanish MINECO [PIB2010US-00153, FIS201020979-C02-01]; IKERBASQUE (the Basque Science Foundation); Foundation of Science & Technology of Portugal through the program 'Investigador FCT [IF/00981/2013] FX G M and Y K are grateful to the Rohde & Schwarz Oestereich GmbH Representative Office for the opportunity to use the R&S® ZVA8 Vector Network Analyzer. This work was supported in part by grant No. UU34/008 from the State Fund for Fundamental Research of Ukraine, by the National Science Foundation of USA (grant DMR-1015175), by DARPA, by the contract from the US Army TARDEC, by the US DOE Office of Science (contract DEAC02-06CH11357), and by the Spanish MINECO grants PIB2010US-00153 and FIS201020979- C02-01. K G acknowledges support by IKERBASQUE (the Basque Science Foundation). G N K is supported by Foundation of Science & Technology of Portugal through the program 'Investigador FCT (grant IF/00981/2013)'. NR 21 TC 5 Z9 5 U1 3 U2 43 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 19 PY 2014 VL 16 AR 063044 DI 10.1088/1367-2630/16/6/063044 PG 10 WC Physics, Multidisciplinary SC Physics GA AL4CQ UT WOS:000339080900004 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Xiao, H Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, AC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M 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Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI Search for pair production of excited top quarks in the lepton plus jets final state SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Top physics ID LHC; COLLIDERS; BOSON; MASS AB A search is performed for pair-produced spin-3/2 excited top quarks , each decaying to a top quark and a gluon. The search uses data collected with the CMS detector from pp collisions at a center-of-mass energy of = 8 TeV, selecting events that have a single isolated muon or electron, an imbalance in transverse momentum, and at least six jets, of which one must be compatible with originating from the fragmentation of a b quark. The data, corresponding to an integrated luminosity of 19.5 fb(-1), show no significant excess over standard model predictions, and provide a lower limit of 803 GeV at 95% confidence on the mass of the spin-3/2 t(*) quark in an extension of the Randall-Sundrum model, assuming a 100% branching fraction of its decay into a top quark and a gluon. This is the first search for a spin-3/2 excited top quark performed at the LHC. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. 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T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Da Cruz E Silva, C. Beirao; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIE, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; D'Agnolo, R. T.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woeohri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Nageli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Nageli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Abdelalim, A. A.; Elgammal, S.] Zewail City Sci & Technol, Zewail, Egypt. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. 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Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Calderon, Alicia/K-3658-2014; Moon, Chang-Seong/J-3619-2014; Gregores, Eduardo/F-8702-2012; Gribushin, Andrei/J-4225-2012; Montanari, Alessandro/J-2420-2012; Josa, Isabel/K-5184-2014; Novaes, Sergio/D-3532-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Lokhtin, Igor/D-7004-2012; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Lopez Virto, Amparo/K-9996-2014; Gonzalez Caballero, Isidro/E-7350-2010; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015 OI Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Ogul, Hasan/0000-0002-5121-2893; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Moon, Chang-Seong/0000-0001-8229-7829; Montanari, Alessandro/0000-0003-2748-6373; Novaes, Sergio/0000-0003-0471-8549; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Scodellaro, Luca/0000-0002-4974-8330; Lopez Virto, Amparo/0000-0002-8707-5392; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Sogut, Kenan/0000-0002-9682-2855; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Ulrich, Ralf/0000-0002-2535-402X; Lenzi, Piergiulio/0000-0002-6927-8807; Lucchini, Marco Toliman/0000-0002-7497-7450; Gutsche, Oliver/0000-0002-8015-9622; Raval, Amita/0000-0003-0164-4337; Torassa, Ezio/0000-0003-2321-0599; Verdier, Patrice/0000-0003-3090-2948; CHANG, PAO-TI/0000-0003-4064-388X; Goldstein, Joel/0000-0003-1591-6014; Heath, Helen/0000-0001-6576-9740; Grassi, Marco/0000-0003-2422-6736; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680 FU BMWF and FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland; MEC; MEC, and HIP (Finland); CEA; CNRS/IN2P3 (France); BMBF; DFG; HGF (Germany); NKTH (Hungary) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP- FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie- Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation ` a la Recherche dans l'Industrie et dans l'Agriculture (FRIA- Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT- Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU- ESF and the Greek NSRF. NR 45 TC 2 Z9 2 U1 7 U2 80 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 19 PY 2014 IS 6 AR 125 DI 10.1007/JHEP06(2014)125 PG 35 WC Physics, Particles & Fields SC Physics GA AK5EV UT WOS:000338448300001 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Akesson, TPA Akimoto, G Akimov, AV Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V 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CA ATLAS Collaboration TI Search for direct top-squark pair production in final states with two leptons in pp collisions at root s=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hardron-Hadron Scattering ID HADRON COLLIDERS; SUPERGAUGE TRANSFORMATIONS; PARTON DISTRIBUTIONS; MEASURING MASSES; SUPERSYMMETRY; PARTICLE; MODEL; QUARK; CURRENTS; PIONS AB A search is presented for direct top-squark pair production in final states with two leptons (electrons or muons) of opposite charge using 20.3 fb(-1) of pp collision data at root s = 8 TeV, collected by the ATLAS experiment at the Large Hadron Collider in 2012. No excess over the Standard Model expectation is found. The results are interpreted under the separate assumptions (i) that the top squark decays to a b-quark in addition to an on-shell chargino whose decay occurs via a real or virtual W boson, or (ii) that the top squark decays to a t-quark and the lightest neutralino. A top squark with a mass between 150 GeV and 445 GeV decaying to a b-quark and an on-shell chargino is excluded at 95% confidence level for a top squark mass equal to the chargino mass plus 10 GeV, in the case of a 1 GeV lightest neutralino. Top squarks with masses between 215 (90) GeV and 530 (170) GeV decaying to an on-shell (off-shell) t-quark and a neutralino are excluded at 95% confidence level for a 1 GeV neutralino. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. 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A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Yau Wong, K. H.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattani, G.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Burmeister, I.; Esch, H.; Goeringer, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Univ Dortmund, Inst Expt Phys 4, D-44227 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagaova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fakr Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Katre, A.; Lacour, D.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, J.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monnier, E.; Stark, J.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimares; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lange, C.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, Y.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, A.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kerevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kerevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S. G.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schramm, S.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. 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E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] NE Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Liang, Z.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. G.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Centro Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Inst Rech Lois Fondament Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Eifert, T.; Fulsom, B. G.; Gao, J.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Huang, Y.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg 2050, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjoelin, J.; Strandberg, S.; Tskhadadze, E. G.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, M.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridis, A.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Nanava, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, G.; Fassi, F.; Ferrer, A.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Hign-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Hign-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldatov, E. Yu.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Hign-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Hign-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Gimenez, V. Castillo; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrington, R. D.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Pan, Y. B.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, Y.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Montreal, PQ, Canada. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Peleganchuk, Sergey/J-6722-2014; Ferrando, James/A-9192-2012; Bosman, Martine/J-9917-2014; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Warburton, Andreas/N-8028-2013; Kuday, Sinan/C-8528-2014; Kuleshov, Sergey/D-9940-2013; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Gabrielli, Alessandro/H-4931-2012; Lokajicek, Milos/G-7800-2014; Castro, Nuno/D-5260-2011; Staroba, Pavel/G-8850-2014; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; de Groot, Nicolo/A-2675-2009; Nemecek, Stanislav/G-5931-2014; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009 OI Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Peleganchuk, Sergey/0000-0003-0907-7592; Ferrando, James/0000-0002-1007-7816; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Kuday, Sinan/0000-0002-0116-5494; Kuleshov, Sergey/0000-0002-3065-326X; Doria, Alessandra/0000-0002-5381-2649; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Coccaro, Andrea/0000-0003-2368-4559; Monzani, Simone/0000-0002-0479-2207; REALE, MARILEA/0000-0002-5478-6059; Longo, Luigi/0000-0002-2357-7043; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; INFN, Italy; MEXT, Japan; CNRST, Morocco; FOM, Netherlands; BRF, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; DOE, United States of America; NSF, United States of America; Benoziyo Center, Israel; JSPS, Japan; FCT, Portugal; ROSATOM, Russian Federation; MIZS, Slovenia; Wallenberg Foundation, Sweden; Leverhulme Trust, United Kingdom; NWO, Netherlands; RCN, Norway FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 95 TC 19 Z9 19 U1 9 U2 107 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 19 PY 2014 IS 6 AR 124 DI 10.1007/JHEP06(2014)124 PG 66 WC Physics, Particles & Fields SC Physics GA AK3TA UT WOS:000338346400001 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, A Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, V Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Xiao, H Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, M Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M 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Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI Measurement of the production cross sections for a Z boson and one or more b jets in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jet physics; Hadron-Hadron Scattering ID LHC AB The production of a Z boson, decaying into two leptons and produced in association with one or more b jets, is studied using proton-proton collisions delivered by the LHC at a centre-of-mass energy of 7 TeV. The data were recorded in 2011 with the CMS detector and correspond to an integrated luminosity of 5 fb(-1). The Z(ll) + b-jets cross sections (where ll = mu mu or ee) are measured separately for a Z boson produced with exactly one b jet and with at least two b jets. In addition, a cross section ratio is extracted for a Z boson produced with at least one b jet, relative to a Z boson produced with at least one jet. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Beiro Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. 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[Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; De Martino, E. Navarro; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Trocniz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Raspereza, A.; Guthoff, M.; Hartmann, F.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; D'Agnolo, R. T.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, F.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lu, Y. J.; Volpe, R.; Yu, S. S.; Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Aliev, T.] Natl Cent Univ, Chungli 32054, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.; Goldenzweig, P.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. 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Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Apresyan, A.; Bornheim, A.; Bunn, J.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Pauss, F.; Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, MN USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI USA. [Fabjan, C.; Fruehwirth, R.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Elgammal, S.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Biasotto, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Grippo, M. T.; Martini, L.] Univ Siena, I-53100 Siena, Italy. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.; Dubinin, M.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Scodellaro, Luca/K-9091-2014; Lopez Virto, Amparo/K-9996-2014; Gonzalez Caballero, Isidro/E-7350-2010; Calvo Alamillo, Enrique/L-1203-2014; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Lokhtin, Igor/D-7004-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; Novaes, Sergio/D-3532-2012; de la Cruz, Begona/K-7552-2014; Moon, Chang-Seong/J-3619-2014; Gregores, Eduardo/F-8702-2012; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; OI Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Russ, James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Ogul, Hasan/0000-0002-5121-2893; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Scodellaro, Luca/0000-0002-4974-8330; Lopez Virto, Amparo/0000-0002-8707-5392; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Novaes, Sergio/0000-0003-0471-8549; Moon, Chang-Seong/0000-0001-8229-7829; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538 FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Funda, cao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy, and the US National Science Foundation; Marie-Curie programme; European Research Council and EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU; Regional Development Fund; Thalis and Aristeia programmes; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Funda, cao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; ; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 48 TC 4 Z9 4 U1 6 U2 74 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 19 PY 2014 IS 6 AR 120 DI 10.1007/JHEP06(2014)120 PG 39 WC Physics, Particles & Fields SC Physics GA AK3SY UT WOS:000338346200001 ER PT J AU Dixon, LJ Drummond, JM Duhr, C Pennington, J AF Dixon, Lance J. Drummond, James M. Duhr, Claude Pennington, Jeffrey TI The four-loop remainder function and multi-Regge behavior at NNLLA in planar N=4 super-Yang-Mills theory SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Scattering Amplitudes; Wilson; 't Hooft and Polyakov loops; Extended Supersymmetry ID SUNRISE GRAPH; ZETA VALUES; POLYLOGARITHMS; AMPLITUDES; EQUATION; LOOPS AB We present the four-loop remainder function for six-gluon scattering with maximal helicity violation in planar N = 4 super-Yang-Mills theory, as an analytic function of three dual-conformal cross ratios. The function is constructed entirely from its analytic properties, without ever inspecting any multi-loop integrand. We employ the same approach used at three loops, writing an ansatz in terms of hexagon functions, and fixing coefficients in the ansatz using the multi-Regge limit and the operator product expansion in the near-collinear limit. We express the result in terms of multiple polylogarithms, and in terms of the coproduct for the associated Hopf algebra. From the remainder function, we extract the BFKL eigenvalue at next-to-next-to-leading logarithmic accuracy (NNLLA), and the impact factor at N(3)LLA. We plot the remainder function along various lines and on one surface, studying ratios of successive loop orders. As seen previously through three loops, these ratios are surprisingly constant over large regions in the space of cross ratios, and they are not far from the value expected at asymptotically large orders of perturbation theory. C1 [Dixon, Lance J.; Pennington, Jeffrey] Stanford Univ, Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Stanford, CA 94309 USA. [Drummond, James M.] CERN, CH-1211 Geneva 23, Switzerland. [Drummond, James M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Drummond, James M.] CNRS, LAPTH, F-74941 Annecy Le Vieux, France. [Drummond, James M.] Univ Savoie, F-74941 Annecy Le Vieux, France. [Duhr, Claude] Univ Durham, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. RP Dixon, LJ (reprint author), Stanford Univ, Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Stanford, CA 94309 USA. EM lance@slac.stanford.edu; drummond@cern.ch; claude.duhr@durham.ac.uk; jpennin@stanford.edu NR 93 TC 37 Z9 37 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 19 PY 2014 IS 6 AR 116 DI 10.1007/JHEP06(2014)116 PG 59 WC Physics, Particles & Fields SC Physics GA AK3BN UT WOS:000338297700001 ER PT J AU Bowman, GR Geissler, PL AF Bowman, Gregory R. Geissler, Phillip L. TI Extensive Conformational Heterogeneity within Protein Cores SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID X-RAY CRYSTALLOGRAPHY; COLI RIBONUCLEASE HI; ENERGY LANDSCAPE; NMR RELAXATION; MOLECULAR SIMULATION; BACKBONE DYNAMICS; HUMAN UBIQUITIN; SIDE-CHAINS; MODEL; N-15 AB Basic principles of statistical mechanics require that proteins sample an ensemble of conformations at any nonzero temperature. However, it is still common to treat the crystallographic structure of a protein as the structure of its native state, largely because high-resolution structural characterization of protein flexibility remains a profound challenge. To assess the typical degree of conformational heterogeneity within folded proteins, we construct Markov state models describing the thermodynamics and kinetics of proteins ranging from 72 to 263 residues in length. Each of these models is built from hundreds of microseconds of atomically detailed molecular dynamics simulations. Examination of the side-chain degrees of freedom reveals that almost every residue visits at least two rotameric states over this time frame, with rotamer transition rates spanning a wide range of time scales (from nanoseconds to tens of microseconds). We also report substantial backbone dynamics on time scales longer than are typically addressed by experimental measures of protein flexibility, such as NMR order parameters. Finally, we demonstrate that these extensive rearrangements are consistent with NMR and crystallographic data, which supports the validity of our models. Altogether, these results depict the interior of proteins not as well-ordered solids, as is often imagined, but instead as dense fluids, which undergo substantial structural fluctuations despite their high packing fraction. C1 [Bowman, Gregory R.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Bowman, Gregory R.; Geissler, Phillip L.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Geissler, Phillip L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Bowman, GR (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. FU Burroughs Wellcome Fund; Miller Institute; NSF [CHE-1048789] FX G.R.B. would like to thank Bill Swope for being a scientific role model in his pursuit of truth and rigor and the editors for the opportunity to contribute to this Festschrift in Bill's honor. We also thank Kelsey Schuster and Milo Lin for helpful discussions. G.R.B. holds a Career Award at the Scientific Interface from the Burroughs Wellcome Fund and was also supported by the Miller Institute. Computing resources were provided by NSF award CHE-1048789 and the users of the Folding@home distributed computing environment and NIH R01-GM062868, courtesy of Vijay Pande. NR 42 TC 11 Z9 11 U1 1 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 19 PY 2014 VL 118 IS 24 SI SI BP 6417 EP 6423 DI 10.1021/jp4105823 PG 7 WC Chemistry, Physical SC Chemistry GA AJ6FC UT WOS:000337784100007 PM 24564338 ER PT J AU Sivak, DA Chodera, JD Crooks, GE AF Sivak, David A. Chodera, John D. Crooks, Gavin E. TI Time Step Rescaling Recovers Continuous-Time Dynamical Properties for Discrete-Time Langevin Integration of Nonequilibrium Systems SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-DYNAMICS; TRANSITION; CONSTRAINTS; ALGORITHMS; SIMULATION; CONSTANTS; ACCURACY; WATER AB When simulating molecular systems using deterministic equations of motion (e.g., Newtonian dynamics), such equations are generally numerically integrated according to a well-developed set of algorithms that share commonly agreed-upon desirable properties. However, for stochastic equations of motion (e.g., Langevin dynamics), there is still broad disagreement over which integration algorithms are most appropriate. While multiple desiderata have been proposed throughout the literature, consensus on which criteria are important is absent, and no published integration scheme satisfies all desiderata simultaneously. Additional nontrivial complications stem from simulating systems driven out of equilibrium using existing stochastic integration schemes in conjunction with recently developed nonequilibrium fluctuation theorems. Here, we examine a family of discrete time integration schemes for Langevin dynamics, assessing how each member satisfies a variety of desiderata that have been enumerated in prior efforts to construct suitable Langevin integrators. We show that the incorporation of a novel time step rescaling in the deterministic updates of position and velocity can correct a number of dynamical defects in these integrators. Finally, we identify a particular splitting (related to the velocity Verlet discretization) that has essentially universally appropriate properties for the simulation of Langevin dynamics for molecular systems in equilibrium, nonequilibrium, and path sampling contexts. C1 [Sivak, David A.; Crooks, Gavin E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Chodera, John D.] Mem Sloan Kettering Canc Ctr, Computat Biol Program, New York, NY 10065 USA. RP Sivak, DA (reprint author), Univ Calif San Francisco, Ctr Syst & Synthet Biol, San Francisco, CA 94158 USA. EM david.sivak@ucsf.edu OI Chodera, John/0000-0003-0542-119X FU California Institute for Quantitative Biosciences (QB3) at the University of California, Berkeley; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; NIGMS Systems Biology Center [P50 GM081879] FX The authors dedicate this work to William C. Swope on the occasion of his 60th birthday and celebration of his seminal contributions to the field of molecular simulation. Additionally, J.D.C. would like to acknowledge the mentorship and insightful advice he has provided over many happy years of collaboration. The authors thank Manuel Athenes (Commissariat a l'Energie Atomique/Saclay), Gabriel Stoltz (CERMICS, Ecole des Ponts Paris Tech), Benoit Roux (University of Chicago), Jerome P. Nilmeier (Lawrence Livermore National Laboratory), Todd Gingrich (UC Berkeley), Jesus A. Izaguirre (University of Notre Dame), Huafeng Xu and Cristian Predescu (D. E. Shaw Research), Patrick Varily (University of Cambridge), and Michael Shirts (University of Virginia) for enlightening discussions and constructive feedback on the manuscript. J.D.C. acknowledges support from a Distinguished Postdoctoral Fellowship from the California Institute for Quantitative Biosciences (QB3) at the University of California, Berkeley. D.A.S. and G.E.C. were funded by the Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. D.A.S. was partially supported by NIGMS Systems Biology Center Grant P50 GM081879. NR 39 TC 8 Z9 8 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 19 PY 2014 VL 118 IS 24 SI SI BP 6466 EP 6474 DI 10.1021/jp411770f PG 9 WC Chemistry, Physical SC Chemistry GA AJ6FC UT WOS:000337784100013 PM 24555448 ER PT J AU Goldey, M Head-Gordon, M AF Goldey, Matthew Head-Gordon, Martin TI Separate Electronic Attenuation Allowing a Spin-Component-Scaled Second-Order Moller-Plesset Theory to Be Effective for Both Thermocheniistry and Noncovalent Interactions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MATRIX RENORMALIZATION-GROUP; DENSITY-FUNCTIONAL THEORY; SULFATE-WATER CLUSTERS; PERTURBATION-THEORY; INTERACTION ENERGIES; QUANTUM-CHEMISTRY; BASIS-SET; CONFIGURATION-INTERACTION; BENCHMARK DATABASE; BINDING-ENERGIES AB Spin-component-scaled (SCS) second-order Moller-Plesset perturbation theory (MP2) improves the treatment of thermochemistry and noncovalent interactions relative to MP2, although the optimal scaling coefficients are quite different for thermochemistry versus noncovalent interactions. This work reconciles these two different scaling regimes for SCS-MP2 by using two different length scales for electronic attenuation of the two spin components. The attenuation parameters and scaling coefficients are optimized in the aug-cc-pVTZ (aTZ) basis using the S66 database of intermolecular interactions and the W4-11 database of thermochemistry. Transferability tests are performed for atomization energies and barrier heights, as well as on further test sets for inter- and intramolecular interactions. SCS dual-attenuated MP2 in the aTZ basis, SCS-MP2(2terfc, aTZ), performs similarly to SCS-MP2/aTZ for thermochemistry while frequently outperforming MP2 at the complete basis set limit (CBS) for nonbonded interactions. C1 [Goldey, Matthew; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Goldey, Matthew; Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Head-Gordon, M (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu FU U.S. Department of Energy [DE-AC02-05CH11231]; NSF [CHE-1048789] FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We acknowledge computational resources obtained under NSF Award CHE-1048789. The authors wish to thank Narbe Mardirossian for helpful discussions regarding training and testing sets. NR 69 TC 7 Z9 7 U1 1 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 19 PY 2014 VL 118 IS 24 SI SI BP 6519 EP 6525 DI 10.1021/jp4126478 PG 7 WC Chemistry, Physical SC Chemistry GA AJ6FC UT WOS:000337784100019 PM 24564860 ER PT J AU Beers, KM Yakovlev, S Jackson, A Wang, X Hexemer, A Downing, KH Balsara, NP AF Beers, Keith M. Yakovlev, Sergey Jackson, Andrew Wang, Xin Hexemer, Alexander Downing, Kenneth H. Balsara, Nitash P. TI Absence of Schroeder's Paradox in a Nanostructured Block Copolymer Electrolyte Membrane SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID HUMID AIR; CONDUCTIVITY; NAFION; EQUILIBRIUM; TRANSITIONS; DISORDER; CELLS; MODEL AB This is a study of morphology, water uptake, and proton conductivity of a sulfonated polystyrene-block-polyethylene (PSS-PE) copolymer equilibrated in humid air with controlled relative humidity (RH), and in liquid water. Extrapolation of the domain size, water uptake, and conductivity obtained in humid air to RH = 100% allowed for an accurate comparison between the properties of PSS-PE hydrated in saturated vapor and in liquid water. We demonstrate that extrapolations of domain size and water uptake on samples equilibrated in humid air are consistent with measurements on samples equilibrated in liquid water. Small (5%) differences in proton conductivity were found in samples equilibrated in humid air and liquid water. We argue that differences in transport coefficients in disordered heterogeneous systems, particularly small differences, present no paradox whatsoever. Schroeder's Paradox, wherein properties of polymers measured in saturated water vapor are different from those obtained in liquid water, is thus not observed in the PSS-PE sample. C1 [Beers, Keith M.] Exponent, Natick, MA 01760 USA. [Beers, Keith M.; Yakovlev, Sergey; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Jackson, Andrew; Wang, Xin; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Downing, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Beers, Keith M.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Jackson, Andrew] European Spallat Source ESS AB, S-22100 Lund, Sweden. [Jackson, Andrew] Univ Delaware, Dept Chem Engn, Newark, DC 19716 USA. [Jackson, Andrew] NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu RI Jackson, Andrew/B-9793-2008 OI Jackson, Andrew/0000-0002-6296-0336 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy FX Primary funding for the work was provided by the Electron Microscopy of Soft Matter Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. SAXS experiments were performed at the Advanced Light Source (ALS). The ALS is a DOE national user facility and is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under the same contract. Certain commercial equipment, instruments, materials, suppliers, and software are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the National Institute of Standards and Technology nor does it imply that the materials or equipment identified are necessarily the best available for the purpose. NR 24 TC 3 Z9 3 U1 3 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 19 PY 2014 VL 118 IS 24 SI SI BP 6785 EP 6791 DI 10.1021/jp501374r PG 7 WC Chemistry, Physical SC Chemistry GA AJ6FC UT WOS:000337784100046 PM 24842682 ER PT J AU Sanchez-Diaz, LE Shew, CY Li, X Wu, B Smith, GS Chen, WR AF Sanchez-Diaz, Luis E. Shew, Chwen-Yang Li, Xin Wu, Bin Smith, Gregory S. Chen, Wei-Ren TI Phase Behavior Under a Noncentrosymmetric Interaction: Shifted-Charge Colloids Investigated by Monte Carlo Simulation SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID PROTEIN CRYSTAL-GROWTH; JANUS DENDRIMERS; COMPLEX ARCHITECTURES; PARTICLES AB Using Monte Carlo simulations, we investigate the structural characteristics of an interacting hard-sphere system with shifted charge to elucidate the effect of the noncentrosymmetric interaction on its phase behavior. Two different phase transitions are identified for this model system. With increasing volume fraction, an abrupt liquid-to-crystal transition first occurs at a significantly lower volume fraction than in centrosymmetrically charged systems. This is due to the stronger effective interparticle repulsion caused by the additional charge anisotropy. Moreover, within the crystal state at higher volume fraction, the system further undergoes a continuous disorder-to-order transition with respect to charge orientation. Detailed analyses in this work disclose the nature of these transitions, and orientation fluctuation can cause noncentrosymmetric unit cells. The dependence of crystal formation and orientational ordering on temperature was also examined. These findings indicate that the noncentrosymmetric interaction in this work results in additional freedoms to fine-tune the phase diagram and increase the functionalities of materials. Moreover, these model studies are essential to advance the future understanding regarding the fundamental physiochemical properties of novel Janus colloidal particles and protein crystallization conditions. C1 [Sanchez-Diaz, Luis E.; Li, Xin; Wu, Bin; Smith, Gregory S.; Chen, Wei-Ren] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Shew, Chwen-Yang] CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA. RP Shew, CY (reprint author), CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA. EM chwenyang.shew@csi.cuny.edu; chenw@ornl.gov RI Smith, Gregory/D-1659-2016 OI Smith, Gregory/0000-0001-5659-1805 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. This research at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 31 TC 0 Z9 0 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 19 PY 2014 VL 118 IS 24 SI SI BP 6963 EP 6971 DI 10.1021/jp504049r PG 9 WC Chemistry, Physical SC Chemistry GA AJ6FC UT WOS:000337784100064 PM 24849261 ER PT J AU Brenner, TM Flores, TA Ndione, PF Meinig, EP Chen, G Olson, DC Furtak, TE Collins, RT AF Brenner, Thomas M. Flores, Thomas A. Ndione, Paul F. Meinig, Erich P. Chen, Gang Olson, Dana C. Furtak, Thomas E. Collins, Reuben T. TI Etch-Resistant Zn1-xMgxO Alloys: An Alternative to ZnO for Carboxylic Acid Surface Modification SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SENSITIZED SOLAR-CELLS; PHOTOVOLTAIC CELLS; ENERGY-CONVERSION; AQUEOUS-SOLUTIONS; ZINC-OXIDE; THIN-FILMS; DYE; NI; NANOSTRUCTURES; SEMICONDUCTOR AB Zinc oxide (ZnO) is a high bandgap transparent metal oxide used extensively in organic electronic devices and dye-sensitized solar cells (DSSCs) as an electron accepting and transporting material. Carboxylic and other organic acid attachment schemes are often employed to sensitize or functionalize the surface of ZnO in these applications. Unfortunately, one weakness of ZnO is its high susceptibility to etching by even weak acids. This has a substantial negative impact on ZnO DSSCs which use carboxylic acid groups to attach dyes to ZnO and also influences attachment techniques for functionalizing ZnO in organic electronic devices. By substituting Mg for Zn atoms to form Zn1-xMgxO (ZnMgO) alloys, a material with similar electronic properties but higher etch resistance is achieved. Here, we show that the etch rate of Zn0.8Mg0.2O, when exposed to the prototypical modifier benzoic acid (BA), is an order of magnitude lower than that of ZnO. Infrared spectroscopic characterization of BA-modified ZnMgO indicates that BA binds surface in two different conformations, the relative proportion of which changes with Mg content. The IR spectra also provide evidence of the presence of physisorbed zinc benzoate complexes that are likely a product of etching, as their presence increases with exposure time. Possibilities for the mechanism of improved etch resistance are discussed via the literature on metal oxide dissolution. C1 [Brenner, Thomas M.; Meinig, Erich P.; Chen, Gang; Furtak, Thomas E.; Collins, Reuben T.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Flores, Thomas A.] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. [Ndione, Paul F.; Olson, Dana C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Collins, RT (reprint author), Colorado Sch Mines, Dept Phys, 1523 Illinois St, Golden, CO 80401 USA. EM tfurtak@mines.edu; rtcollin@mines.edu RI Ndione, Paul/O-6152-2015; Collins, Reuben/O-2545-2014 OI Ndione, Paul/0000-0003-4444-2938; Collins, Reuben/0000-0001-7910-3819 FU National Science Foundation [DMR-0907409]; National Science Foundation through Renewable Energy Materials Research Science and Engineering Center [DMR-0820518]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory through the DOE SETP program; Center for Interface Science: Solar Electric Materials (CISSEM), an Energy Frontier Research Center through the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001084] FX This material is based upon work supported by the National Science Foundation through Grant DMR-0907409 and through the Renewable Energy Materials Research Science and Engineering Center under Grant DMR-0820518. DCO's funding is provided by the U.S. Department of Energy under Contract DE-AC36-08-GO28308 with the National Renewable Energy Laboratory through the DOE SETP program. PFN's funding is provided by the Center for Interface Science: Solar Electric Materials (CISSEM), an Energy Frontier Research Center funded through the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001084. NR 53 TC 0 Z9 0 U1 5 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 19 PY 2014 VL 118 IS 24 BP 12599 EP 12607 DI 10.1021/jp500605t PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ6FA UT WOS:000337783900003 ER PT J AU Holden, D Jelfs, KE Trewin, A Willock, DJ Haranczyk, M Cooper, AI AF Holden, Daniel Jelfs, Kim E. Trewin, Abbie Willock, David J. Haranczyk, Maciej Cooper, Andrew I. TI Gas Diffusion in a Porous Organic Cage: Analysis of Dynamic Pore Connectivity Using Molecular Dynamics Simulations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DIANINS COMPOUND; SILICA ZEOLITES; GUEST TRANSPORT; CARBON-DIOXIDE; FORCE-FIELD; SHAPE; FRAMEWORKS; SIZE; CRYSTALLINE; METHANE AB Molecular dynamics simulations were used to investigate the diffusion of six small gas molecules in a crystalline porous organic cage, CC3. A flexible host model was used to simulate transient channel formation, the effects of which are reflected in the calculated diffusion coefficients for the six gases of 5.64 x 10(-8), 5.94 x 10(-9), 2.60 x 10(-9), 9.60 x 10(-9), 2.40 x 10(-9), and 1.83 x 10(-10) m(2) s(-1), respectively, for H-2, N-2, CO2, CH4, Kr, and Xe. By contrast, a larger gas molecule, SF6, was predicted to be unable to diffuse in the pores of this material. We introduce a new method a void space histogram to analyze dynamic pore topologies and to graphically illustrate the structural factors determining guest diffusion. C1 [Holden, Daniel; Jelfs, Kim E.; Trewin, Abbie; Cooper, Andrew I.] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England. [Holden, Daniel; Jelfs, Kim E.; Trewin, Abbie; Cooper, Andrew I.] Univ Liverpool, Ctr Mat Discovery, Liverpool L69 7ZD, Merseyside, England. [Jelfs, Kim E.] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England. [Trewin, Abbie] Univ Lancaster, Dept Chem, Lancaster LA1 4YB, England. [Willock, David J.] Cardiff Univ, Sch Chem, Cardiff Catalysis Inst, Cardiff CF10 3AT, S Glam, Wales. [Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Holden, D (reprint author), Univ Liverpool, Dept Chem, Crown St, Liverpool L69 7ZD, Merseyside, England. RI EFRC, CGS/I-6680-2012; Willock, David/A-2819-2011; Haranczyk, Maciej/A-6380-2014; Trewin, Abbie/B-2432-2010; Stangl, Kristin/D-1502-2015; Jelfs, Kim/E-1802-2011 OI Haranczyk, Maciej/0000-0001-7146-9568; Jelfs, Kim/0000-0001-7683-7630 FU EPSRC; ERC [EP/H000925/1]; ERC (ERG); Royal Society; Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015] FX We thank the EPSRC and the ERC for financial support (EP/H000925/1; ERG Advanced Investigator Grant, RobOT). A.I.C. is a Royal Society Wolfson Research Merit Award holder. K.E.J. and A.T. hold Royal Society University Research Fellowships. M.H. was supported by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001015. The portion of this work done at the Lawrence Berkeley National Laboratory was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 59 TC 12 Z9 12 U1 7 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 19 PY 2014 VL 118 IS 24 BP 12734 EP 12743 DI 10.1021/jp500293s PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ6FA UT WOS:000337783900019 ER PT J AU Liu, XG Cole, JM Chow, PCY Zhang, L Tan, YZ Zhao, T AF Liu, Xiaogang Cole, Jacqueline M. Chow, Philip C. Y. Zhang, Lei Tan, Yizhou Zhao, Teng TI Dye Aggregation and Complex Formation Effects in 7-(Diethylamino)-coumarin-3-carboxylic Acid SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLVATOCHROMIC COMPARISON METHOD; MOLECULAR-ORIGINS; HYDROGEN-BOND; OPTOELECTRONIC PROPERTIES; ELECTRONIC-TRANSITIONS; REVERSE MICELLES; INDUCED EMISSION; ORGANIC-DYES; LASER-DYES; PI-STAR AB 7-(Diethylamino)-coumarin-3-carboxylic acid (1) has been used as a laser dye, fluorescent label, and biomedical inhibitor in many different applications. Although this dye is typically used in the solution phase, it is prone to molecular aggregation, resulting in many inconsistent optoelectronic properties being reported in the literature. In this paper, the ultraviolet visible absorption and fluorescence spectra of 1 are investigated in three representative solvents: cyclohexane [nonpolar and non-hydrogen bonding (NHB)], ethanol (moderately polar and hydrogen bond accepting and donating), and dimethyl sulfoxide (DMSO) (strongly polar and hydrogen bond accepting). These experimental results, in conjunction with (time-dependent) density functional theory (DFT/TD-DFT)-based quantum calculations, have led to the identification of the J-aggregates of 1 and rationalized its different aggregation characteristic in cyclohexane in contrast to that of another similar compound, coumarin 343. We show here that these aggregates are largely responsible for the anomalous optoelectronic properties of this compound. In addition, DFT calculations and H-1 NMR spectroscopy measurements suggest that the intramolecular hydrogen bond in 1 could be "opened up" in hydrogen bond accepting solvents, affording significant molecular conformational changes and complex formation effects. The comprehensive understanding of the molecular aggregation and complex formation mechanisms of 1 acquired through this work forms a foundation for the knowledge-based molecular design of organic dyes with tailored aggregation tendencies or antiaggregation characteristics catering to different optoelectronic applications. C1 [Liu, Xiaogang; Cole, Jacqueline M.; Chow, Philip C. Y.; Zhang, Lei; Tan, Yizhou; Zhao, Teng] Univ Cambridge, Cavendish Lab, Dept Phys, Cambridge CB3 0HE, England. [Cole, Jacqueline M.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cole, JM (reprint author), Univ Cambridge, Cavendish Lab, Dept Phys, JJ Thomson Ave, Cambridge CB3 0HE, England. EM jmc61@cam.ac.uk RI Cole, Jacqueline/C-5991-2008; Liu, Xiaogang/H-2189-2011; OI Liu, Xiaogang/0000-0002-2553-2068; Zhang, Lei/0000-0001-6873-7314 FU EPSRC UK National Service for Computational Chemistry Software (NSCCS), based at Imperial College London; Singapore Economic Development Board; Fulbright Commission; DOE Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors thank Dr. Paul Waddell from the Department of Physics, University of Cambridge, U.K., for his helpful comments on this manuscript and the EPSRC UK National Service for Computational Chemistry Software (NSCCS), based at Imperial College London, for supporting this work. X.L. is indebted to the Singapore Economic Development Board for a Clean Energy Scholarship. J.M.C. thanks the Fulbright Commission for a UK-US Fulbright Scholar Award, hosted by Argonne National Laboratory where work done was supported by DOE Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 51 TC 5 Z9 5 U1 2 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 19 PY 2014 VL 118 IS 24 BP 13042 EP 13051 DI 10.1021/jp409435v PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ6FA UT WOS:000337783900052 ER PT J AU Faraone, A Fratini, E Garai, S Muller, A Tyagi, M Jenkins, T Mamontov, E Paul, RL Copley, JRD Baglioni, P AF Faraone, Antonio Fratini, Emiliano Garai, Somenath Mueller, Achim Tyagi, Madhusudan Jenkins, Timothy Mamontov, Eugene Paul, Rick L. Copley, John R. D. Baglioni, Piero TI Incoherent Quasielastic Neutron Scattering Study of the Relaxation Dynamics in Molybdenum-Oxide Keplerate-Type Nanocages SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID METHYL-GROUP DYNAMICS; HYDRATION WATER DYNAMICS; SINGLE-PARTICLE DYNAMICS; HYDROGEN-BONDED LIQUIDS; MOLECULAR-DYNAMICS; SUPERCOOLED WATER; MESOSCOPIC CONFINEMENT; ENCAPSULATED WATER; DIFFUSIVE MOTIONS; INTERNAL DYNAMICS AB The single-particle relaxation dynamics of hydrogen atoms in different oxomolybdate Keplerate-type nanocages characterized by a (metal)(30) icosahedron and a size of approximate to 2.5 nm were studied using incoherent quasielastic neutron scattering. Measurements were performed on a compound with a {Mo72Cr30} nanocage containing internal acetate ligands and a sodium cation coordinated to 12 water molecules. Because of the presence of the methyl groups of the acetate ligands, the related cavity is mostly hydrophobic and represents an interesting model system for investigating the properties of water molecules under confined conditions in contact with hydrophobic surfaces. The single-particle dynamics of both the methyl groups and the water molecules inside the cavity were studied and characterized to. be thermally activated processes. The volume explored by the hydrogen atoms during their motions was also determined. Elastic scan measurements of the {Mo72Cr30} cage, in comparison with the {Mo72V30} cage, which has the same skeletal structure as {Mo72Cr30} but a hydrophilic interior, have allowed an investigation into the vibrational dynamics of the cages themselves and the determination of the effect of the cage polarity. C1 [Faraone, Antonio; Tyagi, Madhusudan; Jenkins, Timothy; Copley, John R. D.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Faraone, Antonio; Tyagi, Madhusudan] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Fratini, Emiliano; Baglioni, Piero] Univ Florence, Dept Chem Ugo Schiff, I-50019 Florence, Italy. [Fratini, Emiliano; Baglioni, Piero] Univ Florence, CSGI, I-50019 Florence, Italy. [Garai, Somenath; Mueller, Achim] Univ Bielefeld, Fak Chem, D-33615 Bielefeld, Germany. [Paul, Rick L.] NIST, Mat Measurement Lab, Div Analyt Chem, Gaithersburg, MD 20899 USA. [Jenkins, Timothy] US Army Res Lab, Adelphi, MD 21005 USA. [Mamontov, Eugene] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Faraone, A (reprint author), NIST, Ctr Neutron Res, 100 Bur Dr, Gaithersburg, MD 20899 USA. EM antonio.faraone@nist.gov; piero.baglioni@unifi.it RI Tyagi, Madhu Sudan/M-4693-2014; Mamontov, Eugene/Q-1003-2015; Baglioni, Piero/B-1208-2011; OI Tyagi, Madhu Sudan/0000-0002-4364-7176; Mamontov, Eugene/0000-0002-5684-2675; Baglioni, Piero/0000-0003-1312-8700; Muller, Achim/0000-0003-0117-4021 FU ERC (Brussels); National Science Foundation [DMR-0944772]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Consorzio Interuniversitario per lo Sviluppo dei Sistemi a Grande Interfase, CSGI; Minister dell'Istruzione, Universita e della Ricerca Scientifica, MiUR FX We thank Dr. A.M. Todea for initial experiments. The authors are indebted to Dr. R. Bindel for performing some of the PGAA measurements. A.M. thanks the ERC (Brussels) for an Advanced Grant. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. The neutron scattering experiments at Oak Ridge National Laboratory's (ORNL) Spallation Neutron Source were supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). E.F. and P.B. acknowledge financial support from Consorzio Interuniversitario per lo Sviluppo dei Sistemi a Grande Interfase, CSGI, and Minister dell'Istruzione, Universita e della Ricerca Scientifica, MiUR. NR 70 TC 3 Z9 3 U1 2 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 19 PY 2014 VL 118 IS 24 BP 13300 EP 13312 DI 10.1021/jp504547z PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ6FA UT WOS:000337783900078 ER PT J AU Bergren, MR Kendrick, CE Neale, NR Redwing, JM Collins, RT Furtak, TE Beard, MC AF Bergren, Matthew R. Kendrick, Chito E. Neale, Nathan R. Redwing, Joan M. Collins, Reuben T. Furtak, Thomas E. Beard, Matthew C. TI Ultrafast Electrical Measurements of Isolated Silicon Nanowires and Nanocrystals SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID TIME-DOMAIN SPECTROSCOPY; CARRIER DYNAMICS; QUANTUM DOTS; SI NANOWIRES; SEMICONDUCTOR NANOCRYSTALS; EXCITON POLARIZABILITY; SURFACE RECOMBINATION; GOLD; CONFINEMENT; METAL AB We simultaneously determined the charge carrier mobility and picosecond to nanosecond carrier dynamics of isolated silicon nanowires (Si NWs) and nanocrystals (Si NCs) using time-resolved terahertz spectroscopy. We then compared these results to data measured on bulk c-Si as a function of excitation fluence. We find >1 ns carrier lifetimes in Si NA/Vs that are dominated by surface recombination with surface recombination velocities (SRV) between similar to 1100-1700 cm s(-1) depending on process conditions. The Si NCs have markedly different decay dynamics. Initially, free-carriers are produced, but relax within similar to 1.5 ps to form bound excitons. Subsequently, the excitons decay with lifetimes >7 ns, similar to free carriers produced in bulk Si. The isolated Si NWs exhibit bulk-like mobilities that decrease with increasing excitation density, while the hot-carrier mobilities in the Si NCs are lower than bulk mobilities and could only be measured within the initial 1.5 ps decay. We discuss the implications of our measurements on the utilization of Si NWs and NCs in macroscopic optoelectronic applications. C1 [Bergren, Matthew R.; Kendrick, Chito E.; Collins, Reuben T.; Furtak, Thomas E.; Beard, Matthew C.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Bergren, Matthew R.; Neale, Nathan R.; Beard, Matthew C.] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Kendrick, Chito E.; Redwing, Joan M.] Penn State Univ, Mat Sci & Engn Dept, State Coll, PA 16801 USA. RP Bergren, MR (reprint author), Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RI Beard, MATTHEW/E-4270-2015; Collins, Reuben/O-2545-2014 OI Beard, MATTHEW/0000-0002-2711-1355; Collins, Reuben/0000-0001-7910-3819 FU National Science Foundation through the Renewable Energy Materials Research Science and Engineering Center [DMR-0820518]; Center for Advanced Solar Photophysics (CASP) an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences; DOE [DE-AC36-08G028308]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy [DE-EE0005323] FX M.R.B., R.T.C., and T.E.F. were supported by the National Science Foundation through the Renewable Energy Materials Research Science and Engineering Center under Grant Number DMR-0820518. M.C.B. and N.R.N. acknowledge support from the Center for Advanced Solar Photophysics (CASP) an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences. The terahertz experimental apparatus is supported by the Solar Photochemistry program within the division of Chemical Sciences, Geosciences, and Biosciences, Office of Science, Office of Basic Energy Sciences within DOE. DOE funding was provided to the National Renewable Energy Laboratory (NREL) through contract DE-AC36-08G028308. Funding from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy under Grant Number DE-EE0005323 supported C.E.K. and J.M.R. for the Si NW sample synthesis at Penn State University. NR 45 TC 7 Z9 7 U1 2 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUN 19 PY 2014 VL 5 IS 12 BP 2050 EP 2057 DI 10.1021/jz500863a PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ7IJ UT WOS:000337870100001 PM 26270492 ER PT J AU Carrillo, C Johns, TR Xiong, HF DeLaRiva, A Challa, SR Goeke, RS Artyushkova, K Li, W Kim, CH Datye, AK AF Carrillo, Cristihan Johns, Tyne R. Xiong, Haifeng DeLaRiva, Andrew Challa, Sivakumar R. Goeke, Ronald S. Artyushkova, Kateryna Li, Wei Kim, Chang H. Datye, Abhaya K. TI Trapping of Mobile Pt Species by PdO Nanoparticles under Oxidizing Conditions SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID REACTIVE ATMOSPHERES; METAL-OXIDES; PLATINUM; STABILITY; SPECTROSCOPY; CATALYSTS AB Pt is an active catalyst for diesel exhaust catalysis but is known to sinter and form large particles under oxidizing conditions. Pd is added to improve the performance of the Pt catalysts. To investigate the role of Pd, we introduced metallic Pt nanoparticles via physical vapor deposition to a sample containing PdO nanoparticles. When the catalyst was aged in air, the Pt particles disappeared, and the Pt was captured by the PdO, forming bimetallic Pt Pd nanoparticles. The formation of metallic Pt Pd alloys under oxidizing conditions is indeed remarkable but is consistent with bulk thermodynamics. The results show that mobile Pt species are effectively trapped by PdO, representing a novel mechanism by which Ostwald ripening is slowed down. The results have implications for the development of sinter-resistant catalysts and help explain the improved performance and durability of Pt-Pd in automotive exhaust catalytic converters. C1 [Carrillo, Cristihan; Johns, Tyne R.; Xiong, Haifeng; DeLaRiva, Andrew; Challa, Sivakumar R.; Artyushkova, Kateryna; Datye, Abhaya K.] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Carrillo, Cristihan; Johns, Tyne R.; Xiong, Haifeng; DeLaRiva, Andrew; Challa, Sivakumar R.; Artyushkova, Kateryna; Datye, Abhaya K.] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Goeke, Ronald S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Li, Wei; Kim, Chang H.] Gen Motors Global Res & Dev, Chem Sci & Mat Syst Lab, Warren, MI 48090 USA. RP Datye, AK (reprint author), Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. EM datye@unm.edu RI Artyushkova, Kateryna/B-4709-2008; xiong, haifeng/F-6638-2016 OI Artyushkova, Kateryna/0000-0002-2611-0422; FU NSF GOALI Grant [CBET-1067803]; GM Global RD FX This work was supported by NSF GOALI Grant CBET-1067803 and by GM Global R&D. NR 13 TC 6 Z9 6 U1 3 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUN 19 PY 2014 VL 5 IS 12 BP 2089 EP 2093 DI 10.1021/jz5009483 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ7IJ UT WOS:000337870100007 PM 26270497 ER PT J AU Deng, SHM Kong, XY Zhang, GX Yang, Y Zheng, WJ Sun, ZR Zhang, DQ Wang, XB AF Deng, S. H. M. Kong, Xiang-Yu Zhang, GuanXin Yang, Yan Zheng, Wei-Jun Sun, Zhen-Rong Zhang, De-Qing Wang, Xue-Bin TI Vibrationally Resolved Photoelectron Spectroscopy of the Model GFP Chromophore Anion Revealing the Photoexcited S-1 State Being Both Vertically and Adiabatically Bound against the Photodetached D-0 Continuum SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID GREEN FLUORESCENT PROTEIN; DYNAMICS AB The first excited state of the model green fluorescence protein (GFP) chromophore anion (S-1) and its energy level against the electron-detached neutral radical D-0 state are crucial in determining the photophysics and the photoinduced dynamics of GFP. Extensive experimental and theoretical studies, particularly several very recent gas-phase investigations, concluded that S-1 is a bound state in the Franck-Condon vertical region with respect to D-0. However, what remains unknown and challenging is if S-1 is bound adiabatically, primarily due to lack of accurate experimental measurements as well as due to the close proximity in energy for these two states that even sophisticated high-level ab initio calculations cannot reliably predict. Here, we report a negative ion photoelectron spectroscopy study on the model GFP chromophore anion, the deprotonated p-hydroxybenzylidene-2,3-dimethylimidazolinone anion (HBDI-) taken under low-temperature conditions with improved energy resolution. Despite the considerable size and low symmetry of the molecule, resolved vibrational structures were obtained with the 0-0 transition being the most intense peak, The adiabatic (ADE) and vertical detachment (VDE) energies therefore are determined both to be 2.73 +/- 0.01 eV, indicating that the detached D-0 state is 0.16 eV higher in energy than the photon excited S-1 state. The accurate ADE and VDE values and the well-resolved photoelectron spectra reported here provide much needed robust benchmarks for future theoretical investigations. C1 [Deng, S. H. M.; Kong, Xiang-Yu; Yang, Yan; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Zhang, GuanXin; Zhang, De-Qing] Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China. [Kong, Xiang-Yu; Zheng, Wei-Jun] Chinese Acad Sci, Inst Chem, State Key Lab Mol React Dynam, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China. [Yang, Yan; Sun, Zhen-Rong] E China Normal Univ, State Key Lab Precis Spect, Shanghai 200062, Peoples R China. [Yang, Yan] Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K8-88, Richland, WA 99352 USA. EM xuebin.wang@pnnl.gov RI Kong, Xiang-Yu/A-1990-2011 OI Kong, Xiang-Yu/0000-0002-4475-2162 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; DOE's Office of Biological and Environmental Research; National Natural Science Foundation of China FX This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences (X.-B.W.) and was performed at the EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The synthesis of HBDI was supported by the National Natural Science Foundation of China (D.-Q. Z). NR 22 TC 12 Z9 12 U1 3 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUN 19 PY 2014 VL 5 IS 12 BP 2155 EP 2159 DI 10.1021/jz500869b PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ7IJ UT WOS:000337870100018 PM 26270508 ER PT J AU Myburg, AA Grattapaglia, D Tuskan, GA Hellsten, U Hayes, RD Grimwood, J Jenkins, J Lindquist, E Tice, H Bauer, D Goodstein, DM Dubchak, I Poliakov, A Mizrachi, E Kullan, ARK Hussey, SG Pinard, D Van der Merwe, K Singh, P Van Jaarsveld, I Silva, OB Togawa, RC Pappas, MR Faria, DA Sansaloni, CP Petroli, CD Yang, XH Ranjan, P Tschaplinski, TJ Ye, CY Li, T Sterck, L Vanneste, K Murat, F Soler, M Clemente, HS Saidi, N Cassan-Wang, H Dunand, C Hefer, CA Bornberg-Bauer, E Kersting, AR Vining, K Amarasinghe, V Ranik, M Naithani, S Elser, J Boyd, AE Liston, A Spatafora, JW Dharmwardhana, P Raja, R Sullivan, C Romanel, E Alves-Ferreira, M Lheim, CK Foley, W Carocha, V Paiva, J Kudrna, D Brommonschenkel, SH Pasquali, G Byrne, M Rigault, P Tibbits, J Spokevicius, A Jones, RC Steane, DA Vaillancourt, RE Potts, BM Joubert, F Barry, K Pappas, GJ Strauss, SH Jaiswal, P Grima-Pettenati, J Salse, J Van de Peer, Y Rokhsar, DS Schmutz, J AF Myburg, Alexander A. Grattapaglia, Dario Tuskan, Gerald A. Hellsten, Uffe Hayes, Richard D. Grimwood, Jane Jenkins, Jerry Lindquist, Erika Tice, Hope Bauer, Diane Goodstein, David M. Dubchak, Inna Poliakov, Alexandre Mizrachi, Eshchar Kullan, Anand R. K. Hussey, Steven G. Pinard, Desre Van der Merwe, Karen Singh, Pooja Van Jaarsveld, Ida Silva-Junior, Orzenil B. Togawa, Roberto C. Pappas, Marilia R. Faria, Danielle A. Sansaloni, Carolina P. Petroli, Cesar D. Yang, Xiaohan Ranjan, Priya Tschaplinski, Timothy J. Ye, Chu-Yu Li, Ting Sterck, Lieven Vanneste, Kevin Murat, Florent Soler, Maral Clemente, Helene San Saidi, Naijib Cassan-Wang, Hua Dunand, Christophe Hefer, Charles A. Bornberg-Bauer, Erich Kersting, Anna R. Vining, Kelly Amarasinghe, Vindhya Ranik, Martin Naithani, Sushma Elser, Justin Boyd, Alexander E. Liston, Aaron Spatafora, Joseph W. Dharmwardhana, Palitha Raja, Rajani Sullivan, Christopher Romanel, Elisson Alves-Ferreira, Marcio Lheim, Carsten Ku Foley, William Carocha, Victor Paiva, Jorge Kudrna, David Brommonschenkel, Sergio H. Pasquali, Giancarlo Byrne, Margaret Rigault, Philippe Tibbits, Josquin Spokevicius, Antanas Jones, Rebecca C. Steane, Dorothy A. Vaillancourt, Rene E. Potts, Brad M. Joubert, Fourie Barry, Kerrie Pappas, Georgios J., Jr. Strauss, Steven H. Jaiswal, Pankaj Grima-Pettenati, Jacqueline Salse, Jerome Van de Peer, Yves Rokhsar, Daniel S. Schmutz, Jeremy TI The genome of Eucalyptus grandis SO NATURE LA English DT Article ID WHOLE-GENOME; FOREST TREES; NUCLEAR-DNA; RNA-SEQ; EVOLUTION; PLANT; ALIGNMENT; DATABASE; TOOL; GENE AB Eucalypts are the world's most widely planted hardwood trees. Their outstanding diversity, adaptability and growth have made them a global renewable resource of fibre and energy. We sequenced and assembled >94% of the 640-megabase genome of Eucalyptus grandis. Of 36,376 predicted protein-coding genes, 34% occur in tandem duplications, the largest proportion thus far in plant genomes. Eucalyptus also shows the highest diversity of genes for specialized metabolites such as terpenes that act as chemical defence and provide unique pharmaceutical oils. Genome sequencing of the E. grandis sister species E. globulus and a set of inbred E. grandis tree genomes reveals dynamic genome evolution and hotspots of inbreeding depression. The E. grandis genome is the first reference for the eudicot order Myrtales and is placed here sister to the eurosids. This resource expands our understanding of the unique biology of large woody perennials and provides a powerful tool to accelerate comparative biology, breeding and biotechnology. C1 [Myburg, Alexander A.; Mizrachi, Eshchar; Kullan, Anand R. K.; Hussey, Steven G.; Pinard, Desre; Van der Merwe, Karen; Singh, Pooja] Univ Pretoria, Dept Genet, Forestry & Agr Biotechnol Inst FABI, ZA-0028 Pretoria, South Africa. [Myburg, Alexander A.; Mizrachi, Eshchar; Kullan, Anand R. K.; Hussey, Steven G.; Pinard, Desre; Van der Merwe, Karen; Singh, Pooja; Joubert, Fourie; Van de Peer, Yves] Univ Pretoria, Genom Res Inst GRI, ZA-0028 Pretoria, South Africa. [Grattapaglia, Dario; Pappas, Marilia R.; Faria, Danielle A.; Sansaloni, Carolina P.; Petroli, Cesar D.] EPQB Final W5 Norte, EMBRAPA Recursos Genet & Biotecnol, Lab Genet Vegetal, BR-70770917 Brasilia, DF, Brazil. [Grattapaglia, Dario] Univ Catolica Brasilia SGAN 916, Programa Ciencias Genom & Biotecnol, BR-70790160 Brasilia, DF, Brazil. [Tuskan, Gerald A.; Hellsten, Uffe; Hayes, Richard D.; Lindquist, Erika; Tice, Hope; Bauer, Diane; Goodstein, David M.; Dubchak, Inna; Poliakov, Alexandre; Barry, Kerrie; Rokhsar, Daniel S.; Schmutz, Jeremy] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Tuskan, Gerald A.; Yang, Xiaohan; Ranjan, Priya; Tschaplinski, Timothy J.; Ye, Chu-Yu; Li, Ting] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Grimwood, Jane; Jenkins, Jerry; Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL 35801 USA. [Van Jaarsveld, Ida; Hefer, Charles A.; Joubert, Fourie] Univ Pretoria, Dept Biochem, Bioinformat & Computat Biol Unit, ZA-0028 Pretoria, South Africa. [Silva-Junior, Orzenil B.; Togawa, Roberto C.] EPQB Final W5 Norte, EMBRAPA Recursos Genet & Biotecnol, Lab Bioinformat, BR-70770917 Brasilia, DF, Brazil. [Sterck, Lieven; Vanneste, Kevin; Van de Peer, Yves] Univ Ghent VIB, Dept Plant Biotechnol & Bioinformat, B-9000 Ghent, Belgium. [Murat, Florent; Salse, Jerome] INRA UBP UMR 1095, F-63100 Clermont Ferrand, France. [Soler, Maral; Clemente, Helene San; Saidi, Naijib; Cassan-Wang, Hua; Dunand, Christophe; Carocha, Victor; Grima-Pettenati, Jacqueline] Univ Toulouse 3, Lab Rech Sci Vegetales, UMR 5546, CNRS, F-31326 Castanet Tolosan, France. [Hefer, Charles A.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [Bornberg-Bauer, Erich; Kersting, Anna R.] Univ Munster, Inst Evolut & Biodivers, D-48149 Munster, Germany. [Kersting, Anna R.] Univ Dusseldorf, Inst Comp Sci, Dept Bioinformat, D-40225 Dusseldorf, Germany. [Vining, Kelly; Amarasinghe, Vindhya; Ranik, Martin; Strauss, Steven H.] Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. [Naithani, Sushma; Elser, Justin; Liston, Aaron; Spatafora, Joseph W.; Dharmwardhana, Palitha; Raja, Rajani; Jaiswal, Pankaj] Oregon State Univ, Dept Bot & Plant Pathol, Corvallis, OR 97331 USA. [Naithani, Sushma; Boyd, Alexander E.; Liston, Aaron; Spatafora, Joseph W.; Sullivan, Christopher; Jaiswal, Pankaj] Oregon State Univ, Ctr Genome Res & Biocomp, Corvallis, OR 97331 USA. [Romanel, Elisson] Univ Fed Rio de Janeiro, Dept Genet, Lab Biol Evolut Teor & Aplicada, BR-21949900 Rio de Janeiro, Brazil. [Romanel, Elisson] EEL USP, Dept Biotecnol, BR-12602810 Lorena, SP, Brazil. [Romanel, Elisson; Alves-Ferreira, Marcio] Univ Fed Rio de Janeiro, Dept Genet, LGMV, BR-21949900 Rio de Janeiro, Brazil. [Lheim, Carsten Ku; Foley, William] Australian Natl Univ, Res Sch Biol, Canberra, ACT 0200, Australia. [Carocha, Victor; Paiva, Jorge] IICT MNE, P-1349007 Lisbon, Portugal. [Carocha, Victor; Paiva, Jorge] IBET ITQB, P-2781901 Oeiras, Portugal. [Kudrna, David] Univ Arizona, Arizona Genom Inst, Tucson, AZ 85721 USA. [Brommonschenkel, Sergio H.] Univ Fed Vicosa, Dep Fitopatol, BR-36570000 Vicosa, MG, Brazil. [Pasquali, Giancarlo] Univ Fed Rio Grande do Sul, Ctr Biotecnol, BR-91501970 Porto Alegre, RS, Brazil. [Byrne, Margaret] Dept Parks & Wildlife, Sci & Conservat Div, Bentley, WA 6983, Australia. [Rigault, Philippe] GYDLE, Quebec City, PQ G1T 1Z2, Canada. [Tibbits, Josquin] Victorian Govt, Dept Environm & Primary Ind, Yallambie, Vic 3085, Australia. [Spokevicius, Antanas] Univ Melbourne, Melbourne Sch Land & Environm, Melbourne, Vic 3010, Australia. [Jones, Rebecca C.; Steane, Dorothy A.; Vaillancourt, Rene E.; Potts, Brad M.] Univ Tasmania, Sch Biol Sci, Hobart, Tas 7001, Australia. [Jones, Rebecca C.; Steane, Dorothy A.; Vaillancourt, Rene E.; Potts, Brad M.] Univ Tasmania, Natl Ctr Future Forest Ind, Hobart, Tas 7001, Australia. [Steane, Dorothy A.] Univ Sunshine Coast, Fac Sci Hlth Educ & Engn, Sippy Downs, Qld 4558, Australia. [Pappas, Georgios J., Jr.] Univ Brasilia, Dept Biol Celular, BR-70910900 Brasilia, DF, Brazil. RP Myburg, AA (reprint author), Univ Pretoria, Dept Genet, Forestry & Agr Biotechnol Inst FABI, Private Bag X20, ZA-0028 Pretoria, South Africa. EM zander.myburg@up.ac.za RI Myburg, Alexander/C-5426-2008; Yang, Xiaohan/A-6975-2011; Pasquali, Giancarlo/L-6421-2013; Vaillancourt, Rene/C-6123-2013; Romanel, Elisson/F-1933-2013; Oliveira, Nadir/H-3532-2015; Byrne, Margaret/H-8198-2015; Sterck, Lieven/A-9439-2016; Pappas Jr, Georgios/D-5933-2016; Jones, Rebecca/J-7901-2014; Soler, Marcal/G-3522-2016; Jaiswal, Pankaj/H-7599-2016; Tuskan, Gerald/A-6225-2011; da Silva Junior, Orzenil/B-3488-2013; Hefer, Charles/A-6093-2011; Bornberg-Bauer, Erich/A-1563-2013; Vaillancourt, Rene/J-7456-2014; Van de Peer, Yves/D-4388-2009; dunand, christophe/I-6424-2012; Kulheim, Carsten/F-4720-2010; Paiva, Jorge/C-2858-2008; Mizrachi, Eshchar/N-3179-2014; Potts, Brad/C-6489-2013; Alves-Ferreira, Marcio/C-5849-2009; Foley, William/C-8069-2009 OI Tschaplinski, Timothy/0000-0002-9540-6622; Hussey, Steven/0000-0002-1079-8373; Pinard, Desre/0000-0001-5600-0139; Hayes, Richard/0000-0002-5236-7918; Alves-Ferreira, Marcio/0000-0002-6107-3700; Myburg, Alexander/0000-0003-0644-5003; Yang, Xiaohan/0000-0001-5207-4210; Romanel, Elisson/0000-0002-4794-4215; Pasquali, Giancarlo/0000-0003-1256-544X; Vaillancourt, Rene/0000-0002-1159-9149; Byrne, Margaret/0000-0002-7197-5409; Sterck, Lieven/0000-0001-7116-4000; Pappas Jr, Georgios/0000-0002-1100-976X; Jones, Rebecca/0000-0002-6491-1423; Soler, Marcal/0000-0002-9138-9394; Jaiswal, Pankaj/0000-0002-1005-8383; Tuskan, Gerald/0000-0003-0106-1289; Hefer, Charles/0000-0001-7527-5461; Bornberg-Bauer, Erich/0000-0002-1826-3576; Vaillancourt, Rene/0000-0002-1159-9149; Van de Peer, Yves/0000-0003-4327-3730; dunand, christophe/0000-0003-1637-4042; Paiva, Jorge/0000-0003-3162-4396; Potts, Brad/0000-0001-6244-289X; Foley, William/0000-0001-8587-1814 FU Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research in the US Department of Energy Office of Science, US DOE Bioenergy Center [DE-AC05-00OR22725]; Brazilian Ministry of Science, Technology and Innovation (MCTI) through (CNPq); Brazilian Ministry of Science, Technology and Innovation (MCTI) through (FINEP); Brazilian Federal District Research Foundation (FAP-DF); Technology and Human Resources for Industry Programme (THRIP) [UID 80118]; South African Department of Science and Technology (DST); National Research Foundation (NRF) [UID 18312, 86936]; Laboratoire d'Excellence [LABEX TULIP ANR-10-LABX-41]; Agence Nationale pour la Recherche (Project Tree For Joules) [ANR-2010-KBBE-007-01]; Fundacao para a Ciencia e Tecnologia (FCT) [P-KBBE/AGR_GPL/0001/2010]; Centre National pour la Recherche Scientifique (CNRS); University Paul Sabatier Toulouse III (UPS); Ghent University; Hercules Foundation; Flemish Government-department EWI FX The work conducted by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. The research and writing of the manuscript was supported, in part, by the Office of Biological and Environmental Research in the US Department of Energy Office of Science under contract DE-AC05-00OR22725 as part of the US DOE Bioenergy Center. Funding for additional components of the study was provided by the Brazilian Ministry of Science, Technology and Innovation (MCTI) through its research funding agencies (CNPq and FINEP), the Brazilian Federal District Research Foundation (FAP-DF), the public-private Genolyptus network of Brazilian forestry companies, the Tree Biosafety and Genomics Research Cooperative (TBGRC, Oregon State University), South African forestry companies Sappi and Mondi, the Technology and Human Resources for Industry Programme (THRIP, UID 80118), the South African Department of Science and Technology (DST) and National Research Foundation (NRF, UID 18312 and 86936), the Laboratoire d'Excellence (LABEX TULIP ANR-10-LABX-41), the Agence Nationale pour la Recherche (Project Tree For Joules ANR-2010-KBBE-007-01; Fundacao para a Ciencia e Tecnologia (FCT, P-KBBE/AGR_GPL/0001/2010), the Centre National pour la Recherche Scientifique (CNRS), the University Paul Sabatier Toulouse III (UPS). Part of this work was carried out using the Stevin Supercomputer Infrastructure at Ghent University, funded by Ghent University, the Hercules Foundation, and the Flemish Government-department EWI. We also acknowledge S. Oda and E. Gonzalez of Suzano Paper and Pulp for providing genetic material of E. grandis genotypes BRASUZ1, G7J1, M35D2 and their progeny used for genome sequencing and resequencing, Forestal Mininco (Chile) for genetic material of X46, the E. globulus genotype used for genome resequencing, M. Hinchee and W. Rottmann of ArborGen for EST sequences used to support gene annotation, Sappi (South Africa) for genetic material of the population used for genetic linkage mapping, and Sappi and Mondi (South Africa) for E. grandis tissues used for RNA sequencing. We acknowledge M. O'Neill of the University of Pretoria for technical assistance with E. grandis RNA sequencing. NR 70 TC 174 Z9 180 U1 16 U2 200 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUN 19 PY 2014 VL 510 IS 7505 BP 356 EP + DI 10.1038/nature13308 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0NG UT WOS:000337350200027 PM 24919147 ER PT J AU Bailey, JA Bazavov, A Bernard, C Bouchard, M Detar, C Du, D El-Khadra, AX Foley, J Freeland, ED Gamiz, E Gottlieb, S Heller, UM Kronfeld, AS Laiho, J Levkova, L Mackenzie, PB Neil, ET Qiu, SW Simone, J Sugar, R Toussaint, D Van de Water, RS Zhou, R AF Bailey, Jon A. Bazavov, A. Bernard, C. Bouchard, M. Detar, C. Du, Daping El-Khadra, A. X. Foley, J. Freeland, E. D. Gamiz, E. Gottlieb, Steven Heller, U. M. Kronfeld, A. S. Laiho, J. Levkova, L. Mackenzie, P. B. Neil, E. T. Qiu, Si-Wei Simone, J. Sugar, R. Toussaint, D. Van de Water, R. S. Zhou, Ran CA Fermilab Lattice & MILC Collaborat TI Update of vertical bar V-cb vertical bar from the (B)over-bar -> D*l(nu)over-bar form factor at zero recoil with three-flavor lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID YANG-MILLS THEORY; QUARK EFFECTIVE THEORY; RADIATIVE-CORRECTIONS; GAUGE-THEORIES; QUANTUM CHROMODYNAMICS; SEMILEPTONIC-B; D-ASTERISK; FERMIONS; DECAYS; SIMULATIONS AB We compute the zero-recoil form factor for the semileptonic decay (B) over bar (0) -> D*(+)l(-)(nu) over bar (and modes related by isospin and charge conjugation) using lattice QCD with three flavors of sea quarks. We use an improved staggered action for the light valence and sea quarks (the MILC asqtad configurations), and the Fermilab action for the heavy quarks. Our calculations incorporate higher statistics, finer lattice spacings, and lighter quark masses than our 2008 work. As a byproduct of tuning the new data set, we obtain the D-s and B-s hyperfine splittings with few-MeV accuracy. For the zero-recoil form factor, we obtain F(1) = 0.906(4)(12), where the first error is statistical and the second is the sum in quadrature of all systematic errors. With the latest Heavy Flavor Averaging Group average of experimental results and a cautious treatment of QED effects, we find vertical bar V-cb vertical bar = (39.04 +/- 0.49(expt) +/- 0.53(QCD) +/- 0.19(QED)) x 10(-3). The QCD error is now commensurate with the experimental error. C1 [Bailey, Jon A.] Seoul Natl Univ, Dept Phys & Astron, Seoul, South Korea. [Bazavov, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Bernard, C.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Bouchard, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Detar, C.; Foley, J.; Levkova, L.; Qiu, Si-Wei] Univ Utah, Dept Phys & Astron, Salt Lake City, UT USA. [Du, Daping; El-Khadra, A. X.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Du, Daping; Laiho, J.] Syracuse Univ, Dept Phys, Syracuse, NY USA. [El-Khadra, A. X.; Kronfeld, A. S.; Mackenzie, P. B.; Neil, E. T.; Simone, J.; Van de Water, R. S.; Zhou, Ran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Freeland, E. D.] Benedictine Univ, Dept Phys, Lisle, IL USA. [Freeland, E. D.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL USA. [Gamiz, E.] Univ Granada, CAFPE, Granada, Spain. [Gamiz, E.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Gottlieb, Steven] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Heller, U. M.] Amer Phys Soc, Ridge, NY USA. [Laiho, J.] Univ Glasgow, Dept Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Neil, E. T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Neil, E. T.] Brookhaven Natl Lab, RIKEN, Res Ctr, Upton, NY 11973 USA. [Sugar, R.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Toussaint, D.] Univ Arizona, Dept Phys, Tucson, AZ USA. RP Bailey, JA (reprint author), Seoul Natl Univ, Dept Phys & Astron, Seoul, South Korea. EM ask@fnal.gov; jlaiho@fnal.gov RI Gamiz, Elvira/E-8009-2016; Bouchard, Christopher/N-3723-2016 OI Gamiz, Elvira/0000-0001-5125-2687; Bouchard, Christopher/0000-0003-1639-7164 FU Office of Science of the United States Department of Energy; National Science Foundation's Teragrid/XSEDE Program; U.S. Department of Energy [DE-FG02-91ER40628, DE-FC02-06ER41446, DE-SC0010120, DE-FG02-91ER40661, DE-FC02-06ER41443, DE-FG02-13ER42001, DE-FG02-13ER41976]; National Science Foundation [PHY-1067881, PHY-0757333, PHY-0703296, PHY-1212389, PHY-1316748]; URA Visiting Scholars' program; Science and Technology Facilities Council and the Scottish Universities Physics Alliance; MINECO (Spain) [FPA201016696, FPA2006-05294]; Ramon y Cajal program; Junta de Andalucia (Spain) [FQM-101, FQM-6552]; European Commission [PCIG10-GA-2011-303781]; Creative Research Initiatives program of the NRF - Korean government (MEST) [3348-20090015]; U.S. Department of Energy. [DE-AC02-98CH10886, DE-AC02-07CH11359] FX We thank Vincenzo Cirigliano, Christoph Schwanda, and Zbigniew Was for useful correspondance. A. X. K. thanks the Fermilab Theory Group for hospitality while this work was finalized. Computations for this work were carried out with resources provided by the USQCD Collaboration, the Argonne Leadership Computing Facility, the National Energy Research Scientific Computing Center, and the Los Alamos National Laboratory, which are funded by the Office of Science of the United States Department of Energy; and with resources provided by the National Institute for Computational Science, the Pittsburgh Supercomputer Center, the San Diego Supercomputer Center, and the Texas Advanced Computing Center, which are funded through the National Science Foundation's Teragrid/XSEDE Program. This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG02-91ER40628 (C. B.), No. DE-FC02-06ER41446 (C. D., J. F., L. L.), No. DE-SC0010120 (S. G.), No. DE-FG02-91ER40661 (S. G., R. Z.), No. DE-FC02-06ER41443 (R. Z.), No. DE-FG02-13ER42001 (D. D., A. X. K.), No. DE-FG02-13ER41976 (D. T.); by the National Science Foundation under Grants No. PHY-1067881, No. PHY-0757333, No. PHY-0703296 (C. D., J. F., L. L.), No. PHY-1212389 (R. Z.), No. PHY-1316748 (R. S.); by the URA Visiting Scholars' program (C. M. B., D. D., A. X. K.); by the Science and Technology Facilities Council and the Scottish Universities Physics Alliance (J. L.); by the MINECO (Spain) under Grants FPA201016696, FPA2006-05294, and Ramon y Cajal program (E. G.); by the Junta de Andalucia (Spain) under Grants FQM-101 and FQM-6552 (E. G.); by European Commission under Grant No. PCIG10-GA-2011-303781 (E. G.); and by the Creative Research Initiatives program (3348-20090015) of the NRF grant funded by the Korean government (MEST) (J. A. B.). This manuscript has been coauthored by an employee of Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 90 TC 24 Z9 24 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 19 PY 2014 VL 89 IS 11 AR 114504 DI 10.1103/PhysRevD.89.114504 PG 35 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CJ2ME UT WOS:000355318100001 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Akesson, TPA Akimoto, G Akimov, AV Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A 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CA ATLAS Collaboration TI Measurement of the low-mass Drell-Yan differential cross section at root s=7 TeV using the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; PAIR PRODUCTION; COLLISIONS; LHC; QCD AB The differential cross section for the process Z/gamma* -> ll (l = e, mu) as a function of dilepton invariant mass is measured in pp collisions at root s = 7 TeV at the LHC using the ATLAS detector. The measurement is performed in the e and mu channels for invariant masses between 26 GeV and 66 GeV using an integrated luminosity of 1.6 fb(-1) collected in 2011 and these measurements are combined. The analysis is extended to invariant masses as low as 12 GeV in the muon channel using 35 pb(-1) of data collected in 2010. The cross sections are determined within fiducial acceptance regions and corrections to extrapolate the measurements to the full kinematic range are provided. 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G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Banfi, D.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Liberti, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dresden, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Barber, T.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Saxon, J.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-69115 Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, C.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Grinstein, S.; Juste Rozas, A.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Martinez, M.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Liberti, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S. G.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Liberti, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S. G.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, S.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muio, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muio, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Myska, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Apolle, R.; Benslama, K.; Davies, E.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Messina, A.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondament Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Huang, Y.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H. L.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Esta, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Sandstroem, R.; Schreyer, M.; Siragusa, G.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Jenni, P.] CERN, Geneva, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow MV Lomonosov State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Tikhomirov, Vladimir/M-6194-2015; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Maneira, Jose/D-8486-2011; Turchikhin, Semen/O-1929-2013; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Andreazza, Attilio/E-5642-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Vranjes Milosavljevic, Marija/F-9847-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Perrino, Roberto/B-4633-2010; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Ferrer, Antonio/H-2942-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Grancagnolo, Sergio/J-3957-2015; Gabrielli, Alessandro/H-4931-2012; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Brooks, William/C-8636-2013; Bosman, Martine/J-9917-2014; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Ferrando, James/A-9192-2012; Lokajicek, Milos/G-7800-2014; Wemans, Andre/A-6738-2012; Castro, Nuno/D-5260-2011; Boyko, Igor/J-3659-2013; Nemecek, Stanislav/G-5931-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Villa, Mauro/C-9883-2009; Moraes, Arthur/F-6478-2010; Kuleshov, Sergey/D-9940-2013; Di Domenico, Antonio/G-6301-2011; Doyle, Anthony/C-5889-2009; de Groot, Nicolo/A-2675-2009; Lei, Xiaowen/O-4348-2014; Kuday, Sinan/C-8528-2014; OI Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Tikhomirov, Vladimir/0000-0002-9634-0581; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maneira, Jose/0000-0002-3222-2738; Turchikhin, Semen/0000-0001-6506-3123; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Andreazza, Attilio/0000-0001-5161-5759; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Perrino, Roberto/0000-0002-5764-7337; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Ferrer, Antonio/0000-0003-0532-711X; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Grancagnolo, Sergio/0000-0001-8490-8304; Gabrielli, Alessandro/0000-0001-5346-7841; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Brooks, William/0000-0001-6161-3570; Bosman, Martine/0000-0002-7290-643X; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Ferrando, James/0000-0002-1007-7816; Wemans, Andre/0000-0002-9669-9500; Castro, Nuno/0000-0001-8491-4376; Boyko, Igor/0000-0002-3355-4662; Ventura, Andrea/0000-0002-3368-3413; Villa, Mauro/0000-0002-9181-8048; Moraes, Arthur/0000-0002-5157-5686; Kuleshov, Sergey/0000-0002-3065-326X; Di Domenico, Antonio/0000-0001-8078-2759; Doyle, Anthony/0000-0001-6322-6195; Lei, Xiaowen/0000-0002-2564-8351; Kuday, Sinan/0000-0002-0116-5494; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; MOST; NSFC, China; COLCIENCIAS, Colombia; MSMT CR; MPO CR; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT; NSRF, Greece; ISF; MINERVA; GIF; I-CORE; Benoziyo Center, Israel; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, Netherlands; BRF; RCN, Norway; MNiSW; NCN, Poland; GRICES; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MIZ FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 67 TC 13 Z9 13 U1 12 U2 89 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 18 PY 2014 IS 6 AR 112 DI 10.1007/JHEP06(2014)112 PG 46 WC Physics, Particles & Fields SC Physics GA AK6HI UT WOS:000338528300001 ER PT J AU Alam-Faruque, Y Hill, DP Dimmer, EC Harris, MA Foulger, RE Tweedie, S Attrill, H Howe, DG Thomas, SR Davidson, D Woolf, AS Blake, JA Mungall, CJ O'Donovan, C Apweiler, R Huntley, RP AF Alam-Faruque, Yasmin Hill, David P. Dimmer, Emily C. Harris, Midori A. Foulger, Rebecca E. Tweedie, Susan Attrill, Helen Howe, Douglas G. Thomas, Stephen Randall Davidson, Duncan Woolf, Adrian S. Blake, Judith A. Mungall, Christopher J. O'Donovan, Claire Apweiler, Rolf Huntley, Rachael P. TI Representing Kidney Development Using the Gene Ontology SO PLOS ONE LA English DT Article ID DIABETIC-NEPHROPATHY; TRANSCRIPTION FACTOR; MASS-SPECTROMETRY; EXPRESSION; APOPTOSIS; DATABASE; DISEASE; CELLS; PAX2; DIFFERENTIATION AB Gene Ontology (GO) provides dynamic controlled vocabularies to aid in the description of the functional biological attributes and subcellular locations of gene products from all taxonomic groups (www.geneontology.org). Here we describe collaboration between the renal biomedical research community and the GO Consortium to improve the quality and quantity of GO terms describing renal development. In the associated annotation activity, the new and revised terms were associated with gene products involved in renal development and function. This project resulted in a total of 522 GO terms being added to the ontology and the creation of approximately 9,600 kidney-related GO term associations to 940 UniProt Knowledgebase (UniProtKB) entries, covering 66 taxonomic groups. We demonstrate the impact of these improvements on the interpretation of GO term analyses performed on genes differentially expressed in kidney glomeruli affected by diabetic nephropathy. In summary, we have produced a resource that can be utilized in the interpretation of data from small- and large-scale experiments investigating molecular mechanisms of kidney function and development and thereby help towards alleviating renal disease. C1 [Alam-Faruque, Yasmin; Dimmer, Emily C.; Foulger, Rebecca E.; O'Donovan, Claire; Apweiler, Rolf; Huntley, Rachael P.] European Bioinformat Inst EMBL EBI, European Mol Biol Lab, Cambridge, England. [Hill, David P.; Blake, Judith A.] Jackson Lab, Bar Harbor, ME 04609 USA. [Harris, Midori A.] Univ Cambridge, Cambridge Syst Biol Ctr, Cambridge, England. [Harris, Midori A.] Univ Cambridge, Dept Biochem, Cambridge CB2 1QW, England. [Tweedie, Susan; Attrill, Helen] Univ Cambridge, Dept Genet, FlyBase, Cambridge CB2 3EH, England. [Howe, Douglas G.] Univ Oregon, Zebrafish Model Organism Database ZFIN, Eugene, OR 97403 USA. [Thomas, Stephen Randall] Univ Paris 11, CNRS, IR4M UMR8081, F-91405 Orsay, France. [Davidson, Duncan] Western Gen Hosp, Inst Genet & Mol Med, MRC Human Genet Unit, Edinburgh EH4 2XU, Midlothian, Scotland. [Woolf, Adrian S.] Univ Manchester, Fac Med & Human Sci, Inst Human Dev, Manchester, Lancs, England. [Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. RP Alam-Faruque, Y (reprint author), European Bioinformat Inst EMBL EBI, European Mol Biol Lab, Cambridge, England. EM yasmin.alamfaruque@gmail.com RI Huntley, Rachael/R-1036-2016; OI Huntley, Rachael/0000-0001-6718-3559; Apweiler, Rolf/0000-0001-7078-200X; Foulger, Rebecca/0000-0001-8682-8754; Tweedie, Susan/0000-0003-1818-8243; Woolf, Adrian/0000-0001-5541-1358; O'Donovan, Claire/0000-0001-8051-7429 FU Kidney Research UK (KRUK) [RP26/2008]; National Institutes of Health (NIH) - National Human Genome Research Institute (NIHGR) [R01HG02273]; European Molecular Biology Laboratory (EMBL); British Heart Foundation (BHF) [RG/13/5/30112]; NIH-NHGRI grant [U41HG002273, U41HG00330, HG000739, U41HG002659]; Medical Research Council (MRC) [G1000968, MR/L2744/1]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; VPH NoE [EU FP7] [23920] FX YA-F was supported by Kidney Research UK (KRUK; http://www.kidneyresearchuk.org) grant [RP26/2008]. The UniProt-GO Annotation Project is supported by the National Institutes of Health (NIH; www.nih.gov/) - National Human Genome Research Institute (NIHGR; www.genome.gov) grant [R01HG02273], the European Molecular Biology Laboratory (EMBL; www.embl.de) core funding and the British Heart Foundation (BHF; www.bhf.org.uk) grant [RG/13/5/30112]. The GO Consortium is supported by NIH-NHGRI grant [U41HG002273]. The Mouse Genome Informatics group is supported by NIH-NHGRI grant [U41HG00330]. FlyBase is supported by NIH-NHGRI grant [HG000739]. ST is supported by Medical Research Council (MRC; http://www.mrc.ac.uk) grant [G1000968]. DGH is supported by the NIH-NHGRI grant [U41HG002659]. ASW is supported by MRC grant [MR/L2744/1]. CJM was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. SRT was supported by VPH NoE [EU FP7, Grant 23920]. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 55 TC 7 Z9 7 U1 2 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 18 PY 2014 VL 9 IS 6 AR e99864 DI 10.1371/journal.pone.0099864 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK6AC UT WOS:000338508200047 PM 24941002 ER PT J AU Weir, SM Talent, LG Anderson, TA Salice, CJ AF Weir, Scott M. Talent, Larry G. Anderson, Todd A. Salice, Christopher J. TI Unraveling the Relative Importance of Oral and Dermal Contaminant Exposure in Reptiles: Insights from Studies Using the Western Fence Lizard (Sceloporus occidentalis) SO PLOS ONE LA English DT Article ID SNAKES ELAPHE-GUTTATA; NONDIETARY ROUTES; PHTHALATE-ESTERS; ECOLOGICAL RISK; MINIATURE PIGS; SHED SKINS; PESTICIDE; EXCRETION; TOXICITY; BIRDS AB Despite widespread recognition of significant data deficiencies, reptiles remain a relatively understudied taxon in ecotoxicology. To conduct ecological risk assessments on reptiles frequently requires using surrogate taxa such as birds, but recent research suggests that reptiles have significantly different exposure profiles and toxicant sensitivity. We exposed western fence lizards, Sceloporus occidentalis, to the same quantities of three model chemicals via oral (gavage) and dermal (ventral skin application) exposure for either 24 or 48 hours. Three phthalate esters (di-methyl phthalate [DMP], di-iso-butyl phthalate [DIBP], and di-n-octyl phthalate [DNOP]) were chosen as model chemicals because they represent a gradient of lipophilicity but are otherwise structurally similar. Overall, the more lipophilic phthalates (DIBP and DNOP) were found to have higher concentrations in tissues than the less lipophilic DMP. Significant differences in tissue concentrations between DIBP and DNOP were tissue-dependent, suggesting that delivery to a site of action following exposure is not only a simple function of lipophilicity. In dermal treatments, DMP usually had fewer detections (except in ventral skin samples), suggesting that lipophilicity (log K-ow>2) is a requirement for uptake across the skin. In general, tissue residues were greater in oral treatments than dermal treatments (significant in adipose and liver tissue), but differences were driven strongly by differences in DMP which did not appear to be absorbed well across skin. When differences in tissue residue concentrations between oral and dermal exposure did occur, the difference was not drastic. Taken together these results suggest that dermal exposure should be considered in risk assessments for reptilian receptors. Dermal exposure may be an especially important route for reptiles as their ectothermic physiology translates to lower energetic demands and dietary exposure compared to birds and mammals. C1 [Weir, Scott M.; Anderson, Todd A.; Salice, Christopher J.] Texas Tech Univ, Inst Environm & Human Hlth, Dept Environm Toxicol, Lubbock, TX 79409 USA. [Talent, Larry G.] Oklahoma State Univ, Dept Nat Resource Ecol & Management, Stillwater, OK 74078 USA. RP Weir, SM (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM smweir@uga.edu FU Helen Jones Foundation; Office of the Provost of Texas Tech University; Permian Basin Petroleum Association FX SMW was provided funding by the Helen Jones Foundation and the Office of the Provost of Texas Tech University. SMW was partially funded by the Permian Basin Petroleum Association during the period this work took place. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 32 TC 8 Z9 10 U1 5 U2 32 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 18 PY 2014 VL 9 IS 6 AR e99666 DI 10.1371/journal.pone.0099666 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK6AC UT WOS:000338508200034 PM 24941063 ER PT J AU Bardeen, WA Moshe, M AF Bardeen, William A. Moshe, Moshe TI Spontaneous breaking of scale invariance in a D=3 U(N) model with Chern-Simons gauge fields SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE AdS-CFT Correspondence; 1/N Expansion; Nonperturbative Effects; Renormalization Group ID MASSLESS HIGHER SPINS AB We study spontaneous breaking of scale invariance in the large N limit of three dimensional U(N )(kappa) Chern-Simons theories coupled to a scalar field in the fundamental representation. When a lambda(6)(phi(dagger) . phi)(3) self interaction term is added to the action we find a massive phase at a certain critical value for a combination of the lambda(6) and 't Hooft's lambda = N/kappa couplings. This model attracted recent attention since at finite kappa it contains a singlet sector which is conjectured to be dual to Vasiliev's higher spin gravity on AdS(4). Our paper concentrates on the massive phase of the 3d boundary theory. We discuss the advantage of introducing masses in the boundary theory through spontaneous breaking of scale invariance. C1 [Bardeen, William A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Moshe, Moshe] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. RP Bardeen, WA (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM bardeen@fnal.gov; moshe@technion.ac.il FU United States Department of Energy [DE-AC02-07CH11359] FX MM thanks Fermilab and Saclay theory groups for their warm hospitality while different parts oft his work were done. This work was completed while WB and MM visited CERN and we thank the CERNTH group for their warm hospitality. We would like to thank Ofer Aharony, Eliezer Rabinovici and Jean Zinn-Justin for useful discussion sand correspondence on some of the issues discussed here. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 25 TC 7 Z9 7 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 18 PY 2014 IS 6 AR 113 DI 10.1007/JHEP06(2014)113 PG 18 WC Physics, Particles & Fields SC Physics GA AK3ME UT WOS:000338327600001 ER PT J AU Wirth, M Villeneuve, S La Joie, R Marks, SM Jagust, WJ AF Wirth, Miranka Villeneuve, Sylvia La Joie, Renaud Marks, Shawn M. Jagust, William J. TI Gene-Environment Interactions: Lifetime Cognitive Activity, APOE Genotype, and Beta-Amyloid Burden SO JOURNAL OF NEUROSCIENCE LA English DT Article DE aging; Alzheimer's disease; APOE; beta-amyloid; lifestyle activity; PIB-PET ID ALZHEIMERS-DISEASE; APOLIPOPROTEIN-E; OLDER-ADULTS; STIMULATING ACTIVITIES; PHYSICAL-ACTIVITY; BRAIN ACTIVITY; BIOMARKERS; RISK; DEPOSITION; STYLE AB Carriers of the apolipoprotein E (APOE) epsilon 4 allele, the major genetic risk for Alzheimer's disease (AD), harbor an increased load of beta-amyloid (A beta) plaque burden that is felt to be a major instigator of AD development. Data has suggested that lifestyle factors may reduce AD risk by directly mitigating A beta pathology, which could be particularly beneficial in APOE epsilon 4 carriers. We therefore examined the interaction between lifetime cognitive activity and the APOE epsilon 4 allele in relation to brain A beta burden. We obtained measures of lifetime cognitive activity in 118 cognitively normal human individuals (mean age: 76.13 +/- 5.56 years, 70 women) using a validated questionnaire that included measures over early, middle, and current age epochs. Hierarchical regression models (adjusted for age, gender, and years of education) were conducted to examine effects of APOE epsilon 4 carrier status, lifetime cognitive activity, and the interaction of the two factors with cortical A beta deposition, quantified using [C-11] Pittsburgh-compound-B (PIB)-PET. As expected, the epsilon 4 carriers exhibited higher PIB retention compared with noncarriers. Lifetime cognitive activity moderated the APOE genotype effect such that cortical PIB retention was diminished in epsilon 4 carriers that reported higher cognitive activity over the life course. The findings suggest that greater lifetime cognitive activity may forestall AD pathology, specifically in genetically susceptible individuals. The effect could imply that cognitive training promotes increased neural efficiency that might retard the lifelong neurally mediated deposition of A beta. C1 [Wirth, Miranka; Villeneuve, Sylvia; La Joie, Renaud; Marks, Shawn M.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94704 USA. [Jagust, William J.] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94704 USA. [Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Wirth, M (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 132 Barker Hall 3190, Berkeley, CA 94704 USA. EM miranka.wirth@gmail.com OI La Joie, Renaud/0000-0003-2581-8100 FU NIH [AG034570]; Swiss National Science Foundation [PA00P1-131515] FX This research work was supported by NIH Grant AG034570, and the Swiss National Science Foundation Grant PA00P1-131515. We thank Grace Tang (UC Berkeley, behavioral data analysis support), Cindee Madison (UC Berkeley, neuroimaging data analysis support), and Jacob Vogel (UC Berkeley, data collection and discussion). NR 44 TC 25 Z9 25 U1 1 U2 16 PU SOC NEUROSCIENCE PI WASHINGTON PA 11 DUPONT CIRCLE, NW, STE 500, WASHINGTON, DC 20036 USA SN 0270-6474 J9 J NEUROSCI JI J. Neurosci. PD JUN 18 PY 2014 VL 34 IS 25 BP 8612 EP 8617 DI 10.1523/JNEUROSCI.4612-13.2014 PG 6 WC Neurosciences SC Neurosciences & Neurology GA AK5FD UT WOS:000338449200022 PM 24948815 ER PT J AU Conradson, SD Bock, N Castro, JM Conradson, DR Cox, LE Dmowski, W Dooley, DE Egami, T Espinosa-Faller, FJ Freibert, FJ Garcia-Adeva, AJ Hess, NJ Holmstrom, EK Howell, RC Katz, B Lashley, JC Martinez, RJ Moore, DP Morales, LA Olivas, JD Pereyra, RA Ramos, M Rudin, SP Villella, PM AF Conradson, Steven D. Bock, Nicolas Castro, Julio M. Conradson, Dylan R. Cox, Lawrence E. Dmowski, Wojciech Dooley, David E. Egami, Takeshi Espinosa-Faller, Francisco J. Freibert, Franz J. Garcia-Adeva, Angel J. Hess, Nancy J. Holmstroem, Erik K. Howell, Rafael C. Katz, Barbara Lashley, Jason C. Martinez, Raymond J. Moore, David P. Morales, Luis A. Olivas, J. David Pereyra, Ramiro A. Ramos, Michael Rudin, Sven P. Villella, Phillip M. TI Nanoscale heterogeneity, premartensitic nucleation, and a new plutonium structure in metastable delta fcc Pu-Ga alloys SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-ABSORPTION; FINE-STRUCTURE SPECTROSCOPY; LOCAL ATOMIC-STRUCTURE; ELECTRONIC-STRUCTURE; MARTENSITIC TRANSFORMATIONS; VIBRATIONAL PROPERTIES; PHASE-TRANSFORMATIONS; STABILIZED PLUTONIUM; MAGNETIC PHASES; ELASTIC-MODULI AB The scientifically fascinating question of the spatial extent and bonding of the 5f orbitals of Pu and its six different phases extends to its delta-retained alloys and the mechanism by which Ga and a number of other unrelated elements stabilize its lowdensity face-centered-cubic (fcc) structure. This issue of phase stability is also important technologically because of its significance to Science-Based Stockpile Stewardship. Answering these questions requires information on the local order and structure around the Ga and its effects on the Pu. We have addressed this by characterizing the structures of a large number of Pu-Ga and two Pu-In and one Pu-Ce delta alloys, including a set of high purity delta Pu1-xGax materials with 1.7 <= x <= 6.4 at. % Ga that span the low [Ga] portion of the d region of the phase diagram across the similar to 3.3 at. % Ga metastability boundary, with extended x-ray absorption fine structure (EXAFS) spectroscopy that probes the element specific local structure, supplemented by x-ray pair distribution function analysis that gives the total local structure to longer distances, and x-ray diffraction that gives the long-range average structure of the periodic component of the materials. Detailed analyses indicate that the alloys at and below a nominal composition of similar to 3.3 at. % Ga are heterogeneous and in addition to the delta phase also contain up to similar to 20% of a novel, coexisting "sigma" structure for Pu that forms in nanometer scale domains that are locally depleted in Ga. The invariance of the Ga EXAFS with composition indicates that this sigma structure forms in Ga-depleted domains that result from the Ga atoms in the delta phase self-organizing into a quasi-intermetallic with a stoichiometry of Pu25-35Ga so that delta Pu-Ga is neither a random solid solution nor the more stable Pu3Ga + alpha. Above this similar to 3.3 at. % Ga nominal composition, the delta Pu-Ga alloy is homogeneous, and no s phase is present. These results that demonstrate that collective and cooperative behavior in the interactions between the alloy elements as well as local elastic forces are crucial in determining the properties of complex materials and contradict the conventional mechanism for martensitic transformations, in this case indicating that nucleation is not the rate limiting step. C1 [Conradson, Steven D.; Freibert, Franz J.; Howell, Rafael C.; Lashley, Jason C.; Martinez, Raymond J.; Moore, David P.; Morales, Luis A.; Olivas, J. David; Ramos, Michael; Villella, Phillip M.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Bock, Nicolas; Conradson, Dylan R.; Holmstroem, Erik K.; Rudin, Sven P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Castro, Julio M.] Los Alamos Natl Lab, Hlth Safety Radiat Protect Div, Los Alamos, NM 87545 USA. [Cox, Lawrence E.; Dooley, David E.; Katz, Barbara; Pereyra, Ramiro A.] Los Alamos Natl Lab, Div Nucl Mat Technol, Los Alamos, NM 87545 USA. [Dmowski, Wojciech; Egami, Takeshi] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Espinosa-Faller, Francisco J.] Univ Marista Merida, Dept Fis Ingenieros, Merida 97300, Yucatan, Mexico. [Garcia-Adeva, Angel J.] Univ Basque Country, Dept Fis Aplicada 1, ETS Ingn Bilbao, Bilbao 48013, Spain. [Hess, Nancy J.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Conradson, SD (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM conradson@lanl.gov RI Garcia Adeva, Angel/L-5157-2014; OI Garcia Adeva, Angel/0000-0003-2776-2390; Freibert, Franz/0000-0003-4434-3446; Moore, David/0000-0002-0645-587X FU Heavy Element Chemistry Program, Chemical Sciences, Biosciences, and Geosciences Division, Office of Basic Energy Sciences; US Department of Energy [DEAC52-06NA25396]; I + D + i programme [FIS2009-14293] FX Interpretation of the data was supported by the Heavy Element Chemistry Program, Chemical Sciences, Biosciences, and Geosciences Division, Office of Basic Energy Sciences; measurements and analysis by the Enhanced Surveillance Campaign, National Nuclear Security Administration. Los Alamos National Laboratory (LANL) is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract No. DEAC52-06NA25396. X-ray absorption fine structure and XRD were performed at Stanford Synchrotron Radiation Lightsource (SSRL; Stanford Linear Accelerator Center) and Advanced Photon Source (APS; Argonne National Laboratory), which are operated by the US Department of Energy, Office of Basic Energy Sciences. Materials Research Collaborative Access Team and Pacific Northwest Consortium-Collaborative Access Team operations are supported by the member institutions. Health Physics operations at SSRL and APS were supported by the Seaborg Institute for Transactinium Science at LANL. We thank Angus Lawson for the analysis of supporting diffraction data and Joe Wong for editing assistance. A.J.G.A. thanks the Spanish Ministerio de Ciencia e Innovacion for financial support under the I + D + i programme (Grant No. FIS2009-14293). NR 113 TC 3 Z9 3 U1 6 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 18 PY 2014 VL 89 IS 22 AR 224102 DI 10.1103/PhysRevB.89.224102 PG 22 WC Physics, Condensed Matter SC Physics GA AK6AV UT WOS:000338510600005 ER PT J AU Lin, SZ Barros, K Mun, E Kim, JW Frontzek, M Barilo, S Shiryaev, SV Zapf, VS Batista, CD AF Lin, Shi-Zeng Barros, Kipton Mun, Eundeok Kim, Jae-Wook Frontzek, Matthias Barilo, S. Shiryaev, S. V. Zapf, Vivien S. Batista, Cristian D. TI Magnetic-field-induced phases in anisotropic triangular antiferromagnets: Application to CuCrO2 SO PHYSICAL REVIEW B LA English DT Article ID HEISENBERG ANTIFERROMAGNETS; LATTICE AB We introduce a minimal spin model for describing the magnetic properties of CuCrO2. Our Monte Carlo simulations of this model reveal a rich magnetic-field-induced phase diagram, which explains the measured field dependence of the electric polarization. The sequence of phase transitions between different multiferroic states arises from a subtle interplay between spatial and spin anisotropy, magnetic frustration, and thermal fluctuations. Our calculations are compared to new measurements up to 92 T. C1 [Lin, Shi-Zeng; Mun, Eundeok; Kim, Jae-Wook; Zapf, Vivien S.] Los Alamos Natl Lab, MPA CMMS Grp, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Lin, Shi-Zeng; Barros, Kipton; Batista, Cristian D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Frontzek, Matthias] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. [Barilo, S.; Shiryaev, S. V.] Inst Solid State & Semicond Phys, Minsk 220072, Byelarus. RP Lin, SZ (reprint author), Los Alamos Natl Lab, MPA CMMS Grp, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016; Frontzek, Matthias/C-5146-2012; OI Lin, Shi-Zeng/0000-0002-4368-5244; Frontzek, Matthias/0000-0001-8704-8928; Barros, Kipton/0000-0002-1333-5972 FU Institutional Computing Program in LANL; NNSA of the US DOE at LANL [DEAC52-06NA25396]; US Department of Energy, Office of BES "Science at 100 Tesla" program; US National Science Foundation [DMR-1157490]; State of Florida; US Department of Energy; European Community [290605] FX The authors are grateful to Yoshitomo Kamiya and Gia-Wei Chern for helpful discussions. Computer resources were supported by the Institutional Computing Program in LANL. This work was carried out under the auspices of the NNSA of the US DOE at LANL under Award No. DEAC52-06NA25396, and was supported by the US Department of Energy, Office of BES "Science at 100 Tesla" program. The NHMFL Pulsed Field Facility is funded by the US National Science Foundation through Cooperative Grant No. DMR-1157490, the State of Florida, and the US Department of Energy. The research leading to these results has also received funding from the European Community's Seventh Framework Programme (FP7/2007-2013) under Grant Agreement No. 290605 (PSIFELLOW/COFUND). NR 29 TC 7 Z9 7 U1 3 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 18 PY 2014 VL 89 IS 22 AR 220405 DI 10.1103/PhysRevB.89.220405 PG 5 WC Physics, Condensed Matter SC Physics GA AK6AV UT WOS:000338510600001 ER PT J AU Lalkovski, S Ivanova, D Stefanova, EA Korichi, A Petkov, P Kownacki, J Kutsarova, T Minkova, A Bazzacco, D Bergstrom, M Gorgen, A Herskind, B Hubel, H Jansen, A Kisyov, S Khoo, TL Kondev, FG Lopez-Martens, A Podolyak, Z Schonwasser, G Yordanov, O AF Lalkovski, S. Ivanova, D. Stefanova, E. A. Korichi, A. Petkov, P. Kownacki, J. Kutsarova, T. Minkova, A. Bazzacco, D. Bergstroem, M. Goergen, A. Herskind, B. Huebel, H. Jansen, A. Kisyov, S. Khoo, T. L. Kondev, F. G. Lopez-Martens, A. Podolyak, Zs. Schoenwasser, G. Yordanov, O. TI Coexisting structures in Ru-105 SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; HIGH-SPIN; ODD-A; EXCITATIONS; STATES AB New positive-parity states, having a bandlike structure, were observed in Ru-105. The nucleus was produced in an induced fission reaction, and the prompt gamma-rays, emitted from the fragments, were detected by the EUROBALL III multidetector array. The partial scheme of excited Ru-105 levels is analyzed within the triaxial-rotor-plus-particle approach. C1 [Lalkovski, S.; Ivanova, D.; Minkova, A.; Kisyov, S.] Univ Sofia, Fac Phys, Sofia 1164, Bulgaria. [Stefanova, E. A.; Petkov, P.; Kutsarova, T.; Lopez-Martens, A.; Yordanov, O.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, BU-1784 Sofia, Bulgaria. [Korichi, A.] IN2P3 CNRS, CSNSM Orsay, F-91405 Orsay, France. [Kownacki, J.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Bazzacco, D.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bergstroem, M.; Herskind, B.] Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Goergen, A.; Huebel, H.; Jansen, A.; Schoenwasser, G.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Khoo, T. L.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Podolyak, Zs.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. RP Lalkovski, S (reprint author), Univ Sofia, Fac Phys, Sofia 1164, Bulgaria. EM stl@phys.uni-sofia.bg FU Bulgarian National Science fund [DMU02/1]; German BMBF [06 BN 109] FX This work is supported by the Bulgarian National Science fund under Contract No. DMU02/1 and the German BMBF under Contract No. 06 BN 109. NR 28 TC 1 Z9 1 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 18 PY 2014 VL 89 IS 6 AR 064312 DI 10.1103/PhysRevC.89.064312 PG 6 WC Physics, Nuclear SC Physics GA AK6BG UT WOS:000338511800002 ER PT J AU Viviani, M Baroni, A Girlanda, L Kievsky, A Marcucci, LE Schiavilla, R AF Viviani, M. Baroni, A. Girlanda, L. Kievsky, A. Marcucci, L. E. Schiavilla, R. TI Chiral effective field theory analysis of hadronic parity violation in few-nucleon systems SO PHYSICAL REVIEW C LA English DT Article ID PROTON-PROTON-SCATTERING; PHENOMENOLOGICAL LAGRANGIANS; CIRCULAR-POLARIZATION; NONCONSERVATION; FORCES; GAMMA; DYNAMICS; CAPTURE; NP AB Background: Weak interactions between quarks induce a parity-violating (PV) component in the nucleon-nucleon potential, whose effects are currently being studied in a number of experiments involving few-nucleon systems. In the present work, we reconsider the derivation of this PV component within a chiral effective field theory (chi EFT) framework. Purpose: The objectives of the present work are twofold. The first is to perform a detailed analysis of the PV nucleon-nucleon potential up to next-to-next-to-leading (N2LO) order in the chiral expansion, in particular, by determining the number of independent low-energy constants (LECs) at N2LO. The second objective is to investigate PV effects in a number of few-nucleon observables, including the (p) over right arrow -p longitudinal asymmetry, the neutron spin rotation in (n) over right arrow -p and (n) over right arrow -d scattering, and the longitudinal asymmetry in the He-3((n) over right arrow, p)H-3 charge-exchange reaction. Methods: The chi EFT PV potential includes one-pion-exchange, two-pion-exchange, and contact terms as well as 1/M (M being the nucleon mass) nonstatic corrections. Dimensional regularization is used to renormalize pion loops. The wave functions for the A = 2-4 nuclei are obtained by using strong two- and three-body potentials also derived, for consistency, from chi EFT. In the case of the A = 3-4 systems, the wave functions are computed by expanding on a hyperspherical harmonics functions basis. Results: We find that the PV potential at N2LO depends on six LECs: the pion-nucleon PV coupling constant h(pi)(1) and five parameters multiplying contact interactions. An estimate for the range of values of the various LECs is provided by using available experimental data, and these values are used to obtain predictions for the other PV observables. Conclusions: The chi EFT approach provides a very satisfactory framework to analyze PV effects in few-nucleon systems. C1 [Viviani, M.; Kievsky, A.; Marcucci, L. E.] Ist Nazl Fis Nucl, I-56127 Pisa, Italy. [Baroni, A.; Schiavilla, R.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Girlanda, L.] Univ Salento, Dept Math & Phys, I-73100 Lecce, Italy. [Girlanda, L.] Ist Nazl Fis Nucl, I-73100 Lecce, Italy. [Marcucci, L. E.] Univ Pisa, Dept Phys, I-56127 Pisa, Italy. [Schiavilla, R.] Jefferson Lab, Newport News, VA 23606 USA. RP Viviani, M (reprint author), Ist Nazl Fis Nucl, I-56127 Pisa, Italy. OI Girlanda, Luca/0000-0002-5560-005X FU US Department of Energy, Office of Nuclear Physics [DE-AC05-06OR23177]; National Energy Research Scientific Computing Center; Jefferson Science Associates Theory Fellowship FX The work of A.B. and R.S. was supported by the US Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC05-06OR23177. The calculations were made possible by grants of computing time from the National Energy Research Scientific Computing Center. A.B. was supported by a Jefferson Science Associates Theory Fellowship. NR 73 TC 14 Z9 14 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 18 PY 2014 VL 89 IS 6 AR 064004 DI 10.1103/PhysRevC.89.064004 PG 27 WC Physics, Nuclear SC Physics GA AK6BG UT WOS:000338511800001 ER PT J AU Aoki, Y Aoyama, T Kurachi, M Maskawa, T Miura, K Nagai, K Ohki, H Rinaldi, E Shibata, A Yamawaki, K Yamazaki, T AF Aoki, Yasumichi Aoyama, Tatsumi Kurachi, Masafumi Maskawa, Toshihide Miura, Kohtaroh Nagai, Kei-ichi Ohki, Hiroshi Rinaldi, Enrico Shibata, Akihiro Yamawaki, Koichi Yamazaki, Takeshi TI Light composite scalar in eight-flavor QCD on the lattice SO PHYSICAL REVIEW D LA English DT Article ID LHC; HYPERCOLOR; DILATON; BOSON; MODEL AB We present the first observation of a flavor-singlet scalar meson as light as the pion in N-f = 8 QCD on the lattice, using the highly improved staggered quark action. Such a light scalar meson can be regarded as a composite Higgs with mass 125 GeV. In accord with our previous lattice results showing that the theory exhibits walking behavior, the light scalar may be a technidilaton, a pseudo-Nambu-Goldstone boson of the approximate scale symmetry in walking technicolor. C1 [Aoki, Yasumichi; Aoyama, Tatsumi; Kurachi, Masafumi; Maskawa, Toshihide; Miura, Kohtaroh; Nagai, Kei-ichi; Ohki, Hiroshi; Yamawaki, Koichi; Yamazaki, Takeshi] Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univers, Nagoya, Aichi 4648602, Japan. [Rinaldi, Enrico] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Shibata, Akihiro] High Energy Accelerator Res Org KEK, Ctr Res Comp, Tsukuba, Ibaraki 3050801, Japan. RP Aoki, Y (reprint author), Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univers, Nagoya, Aichi 4648602, Japan. OI Rinaldi, Enrico/0000-0003-4134-809X FU JSPS [22224003, 23540300, 25800139, 25800138]; Japanese Ministry for Scientific Research on Innovative Areas [23105708]; U.S. Department of Energy [AC52-07NA27344 (LLNL)] FX Numerical simulation has been carried out on the supercomputer system phi at KMI in Nagoya University, the computer facilities of the Information Technology Center in Nagoya University, and the computer facilities of the Research Institute for Information Technology in Kyushu University. This work is supported by the JSPS Grants-in-Aid for Scientific Research (S) No. 22224003, (C) No. 23540300 (K. Y.), for Young Scientists (B) No. 25800139 (H. O.) and No. 25800138 (T. Y.), and also by Grants-in-Aid of the Japanese Ministry for Scientific Research on Innovative Areas No. 23105708 (T. Y.). E. R. acknowledges the support of the U.S. Department of Energy under Contract No. DE-AC52-07NA27344 (LLNL). We would like to thank Ed Bennett, Philippe de Forcrand, Anna Hasenfratz, Julius Kuti, Shinya Matsuzaki, and Volodya Miransky for fruitful discussions. NR 31 TC 31 Z9 31 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 18 PY 2014 VL 89 IS 11 AR 111502 DI 10.1103/PhysRevD.89.111502 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK6IJ UT WOS:000338531000001 ER PT J AU Martinez, E Uberuaga, BP Voter, AF AF Martinez, Enrique Uberuaga, Blas P. Voter, Arthur F. TI Sublattice parallel replica dynamics SO PHYSICAL REVIEW E LA English DT Article ID ALGORITHMS; SYSTEMS AB Exascale computing presents a challenge for the scientific community as new algorithms must be developed to take full advantage of the new computing paradigm. Atomistic simulation methods that offer full fidelity to the underlying potential, i.e., molecular dynamics (MD) and parallel replica dynamics, fail to use the whole machine speedup, leaving a region in time and sample size space that is unattainable with current algorithms. In this paper, we present an extension of the parallel replica dynamics algorithm [A. F. Voter, Phys. Rev. B 57, R13985 (1998)] by combining it with the synchronous sublattice approach of Shim and Amar [Y. Shim and J. G. Amar, Phys. Rev. B 71, 125432 (2005)], thereby exploiting event locality to improve the algorithm scalability. This algorithm is based on a domain decomposition in which events happen independently in different regions in the sample. We develop an analytical expression for the speedup given by this sublattice parallel replica dynamics algorithm and compare it with parallel MD and traditional parallel replica dynamics. We demonstrate how this algorithm, which introduces a slight additional approximation of event locality, enables the study of physical systems unreachable with traditional methodologies and promises to better utilize the resources of current high performance and future exascale computers. C1 [Martinez, Enrique; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Voter, Arthur F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Martinez, E (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST 8, Los Alamos, NM 87545 USA. EM enriquem@lanl.gov OI Martinez Saez, Enrique/0000-0002-2690-2622; Voter, Arthur/0000-0001-9788-7194 FU US Department of Energy through the LANL/LDRD Program FX D. Perez, L. Sandoval, and T. German are acknowledged for useful discussions and suggestions. The authors gratefully acknowledge the support of the US Department of Energy through the LANL/LDRD Program for this work. Parallel computations were performed on the Conejo machine at the High Performance Computing clusters at Los Alamos National Laboratory. NR 19 TC 2 Z9 2 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUN 18 PY 2014 VL 89 IS 6 AR 063308 DI 10.1103/PhysRevE.89.063308 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AK6JF UT WOS:000338533200009 PM 25019913 ER PT J AU Lashley, JC Munns, JHD Echizen, M Ali, MN Rowley, SE Scott, JF AF Lashley, J. C. Munns, J. H. D. Echizen, M. Ali, M. N. Rowley, S. E. Scott, J. F. TI Phase Transitions in the Brominated Ferroelectric Tris-Sarcosine Calcium Chloride SO ADVANCED MATERIALS LA English DT Article ID POLARIZATION REVERSAL PROCESS; THERMAL-EXPANSION; DIELECTRIC MEASUREMENTS; THERMODYNAMIC RELATIONS; TEMPERATURE-DEPENDENCE; RELAXOR FERROELECTRICS; CRITICAL EXPONENTS; LAMBDA-TRANSITION; CRITICAL-BEHAVIOR; SOLID-SOLUTIONS AB We demonstrate that the Curie temperature, T-c, of tris-sarcosine calcium chloride can be lowered from 130 K to near 0 K by chemical doping of the anion. In the low temperature limit, quantum fluctuations persist over a range of chemical doping concentrations. Below T-C the temperature dependence of the fractional length change, Delta L/L-o, scales as (Delta L/L-o )(-1) =a broken vertical bar at(lambda) (red line) where t is the reduced temperature, and lambda = -1.5. The behavior of linear coefficient of thermal expansion near T-C is shown in the inset. Three additional phase transitions near 43, 50, and 61 K are resolved. C1 [Lashley, J. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lashley, J. C.; Munns, J. H. D.; Echizen, M.; Rowley, S. E.; Scott, J. F.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Echizen, M.] Samco Int Co, Fushimi Ku, Kyoto 6128443, Japan. [Ali, M. N.; Rowley, S. E.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Ali, M. N.; Rowley, S. E.] Princeton Univ, PCCM, Princeton, NJ 08544 USA. [Rowley, S. E.] Ctr Brasileiro Pesquisas Fis, BR-22290180 Rio De Janeiro, Brazil. RP Lashley, JC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM j.lash@lanl.gov RI Ali, Mazhar/C-6473-2013 OI Ali, Mazhar/0000-0002-1129-6105 FU EPSRC; United States Department of Energy FX We thank S. S. Saxena, M. Ivanov, J. Banys, R. Cava, and M. A. Carpenter for helpful discussions. Work at Cambridge was supported by a grant from the EPSRC. Work at the Los Alamos National Laboratory was performed under the auspices of the United States Department of Energy. NR 58 TC 4 Z9 4 U1 5 U2 27 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUN 18 PY 2014 VL 26 IS 23 BP 3860 EP 3866 DI 10.1002/adma.201305065 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ4CS UT WOS:000337618600008 PM 24789107 ER PT J AU Wangweerawong, A Bergman, RG Ellman, JA AF Wangweerawong, Apiwat Bergman, Robert G. Ellman, Jonathan A. TI Asymmetric Synthesis of alpha-Branched Amines via Rh(III)-Catalyzed C-H Bond Functionalization SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IMINES; ACTIVATION; ARYLATION; ALKYNES; DIARYLMETHYLAMINES; SULFINIMINES; BENZAMIDES; COMPLEXES; MECHANISM; CATALYSIS AB The first asymmetric intermolecular addition of non-acidic C-H bonds to imines is reported. The use of the activating N-perfluorobutanesulfinyl imine substituent is essential for achieving sufficient reactivity and provides outstanding diastereoselectivity (>98:2 dr). Straightforward removal of the sulfinyl group with HCl yields the highly enantiomerically enriched amine hydrochlorides. C1 [Wangweerawong, Apiwat; Ellman, Jonathan A.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Bergman, Robert G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Bergman, Robert G.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Ellman, JA (reprint author), Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. EM jonathan.ellman@yale.edu RI Ellman, Jonathan/C-7732-2013 FU NSF; NIH [GM069559]; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX This work was supported by the NSF (J.A.E.) and by the NIH under Grant No. GM069559 (J.A.E.). R.G.B. was supported by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. We gratefully acknowledge Brandon Mercado (Yale University) for solving the crystal structure of 3a. NR 42 TC 36 Z9 36 U1 3 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8520 EP 8523 DI 10.1021/ja5033452 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200009 PM 24901217 ER PT J AU Rajeshwar, TR Smith, JC Krishnan, M AF Rajeshwar, Rajitha T. Smith, Jeremy C. Krishnan, Marimuthu TI Hidden Regularity and Universal Classification of Fast Side Chain Motions in Proteins SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; AXIS ORDER PARAMETERS; C-13 NMR RELAXATION; MAGNETIC-RESONANCE RELAXATION; MODEL-FREE APPROACH; MALATE-SYNTHASE-G; X-RAY STRUCTURES; CONFORMATIONAL ENTROPY; GLOBULAR-PROTEINS; METHYL ROTATION AB Proteins display characteristic dynamical signatures that appear to be universal across all proteins regardless of topology and size. Here, we systematically characterize the universal features of fast side chain motions in proteins by examining the conformational energy surfaces of individual residues obtained using enhanced sampling molecular dynamics simulation (618 free energy surfaces obtained from 0.94 mu s MD simulation). The side chain conformational free energy surfaces obtained using the adaptive biasing force (ABF) method for a set of eight proteins with different molecular weights and secondary structures are used to determine the methyl axial NMR order parameters (O-axis(2)), populations of side chain rotamer states (rho), conformational entropies (S-conf), probability fluxes, and activation energies for side chain inter-rotameric transitions. The free energy barriers separating side chain rotamer states range from 0.3 to 12 kcal/mol in all proteins and follow a trimodal distribution with an intense peak at similar to 5 kcal/mol and two shoulders at similar to 3 and similar to 7.5 kcal/mol, indicating that some barriers are more favored than others by proteins to maintain a balance between their conformational stability and flexibility. The origin and the influences of the trimodal barrier distribution on the distribution of O-axis(2), and the side chain conformational entropy are discussed. A hierarchical grading of rotamer states based on the conformational free energy barriers, entropy, and probability flux reveals three distinct classes of side chains in proteins. A unique nonlinear correlation is established between O-axis(2), and the side chain rotamer populations (rho). The apparent universality in O-axis(2) versus rho correlation, trimodal barrier distribution, and distinct characteristics of three classes of side chains observed among all proteins indicates a hidden regularity (or commonality) in the dynamical heterogeneity of fast side chain motions in proteins. C1 [Rajeshwar, Rajitha T.; Krishnan, Marimuthu] Int Inst Informat Technol, Ctr Computat Nat Sci & Bioinformat, Hyderabad 500032, Andhra Pradesh, India. [Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. [Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Mol & Cellular Biol, Knoxville, TN 37996 USA. RP Krishnan, M (reprint author), Int Inst Informat Technol, Ctr Computat Nat Sci & Bioinformat, Hyderabad 500032, Andhra Pradesh, India. EM m.krishnan@iiit.ac.in RI smith, jeremy/B-7287-2012 OI smith, jeremy/0000-0002-2978-3227 FU Department of Science and Technology (DST), New Delhi under SERC Fast Track scheme for Young Scientists [SR/FTP/PS-033/2010]; DST; National Science Foundation (MCB section) FX M.K. acknowledges financial support provided by Department of Science and Technology (DST), New Delhi under SERC Fast Track scheme for Young Scientists (No. SR/FTP/PS-033/2010). R.R.T. acknowledges DST for the Inspire fellowship. J.C.S. acknowledges funding from the National Science Foundation (MCB section). NR 119 TC 1 Z9 1 U1 1 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8590 EP 8605 DI 10.1021/ja5024783 PG 16 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200023 ER PT J AU Nocton, G Lukens, WW Booth, CH Rozenel, SS Medling, SA Maron, L Andersen, RA AF Nocton, Gregory Lukens, Wayne W. Booth, Corwin H. Rozenel, Sergio S. Medling, Scott A. Maron, Laurent Andersen, Richard A. TI Reversible Sigma C-C Bond Formation Between Phenanthroline Ligands Activated by (C5Me5)(2)Yb SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AB-INITIO PSEUDOPOTENTIALS; ELECTRONIC-STRUCTURE; DECAMETHYLYTTERBOCENE COMPLEXES; LANTHANIDE COMPLEXES; PHENALENYL RADICALS; GROUND-STATES; X-RAY; 1,10-PHENANTHROLINE; DIMERIZATIONS; SPECTROSCOPY AB The electronic structure and associated magnetic properties of the 1,10-phenanthroline adducts of Cp-2*Yb are dramatically different from those of the 2,2'-bipyridine adducts. The monomeric phenanthroline adducts are ground state triplets that are based upon trivalent Yb(III), f(13), and (phen(center dot-)) that are only weakly exchange coupled, which is in contrast to the bipyridine adducts whose ground states are multiconfigurational, open-shell singlets in which ytterbium is intermediate valent (J. Am. Chem. Soc 2009, 131, 6480; J. Am. Chem. Soc 2010, 132, 17537). The origin of these different physical properties is traced to the number and symmetry of the LUMO and LUMO+1 of the heterocyclic diimine ligands. The bipy(center dot-) has only one pi(1)* orbital of b(1) symmetry of accessible energy, but phen(center dot-) has two pi* orbitals of b(1) and a(2) symmetry that are energetically accessible. The carbon p(pi)-orbitals have different nodal properties and coefficients and their energies, and therefore their populations change depending on the position and number of methyl substitutions on the ring. A chemical ramification of the change in electronic structure is that Cp-2*Yb(phen) is a dimer when crystallized from toluene solution, but a monomer when sublimed at 180-190 degrees C. When 3,8-Me(2)phenanthroline is used, the adduct Cp-2*Yb(3,8-Me(2)phen) exists in the solution in a dimer-monomer equilibrium in which Delta G is near zero. The adducts with 3-Me, 4-Me, 5-Me, 3,8-Me-2, and 5,6-Me-2-phenanthroline are isolated and characterized by solid state X-ray crystallography, magnetic susceptibility and L-III-edge XANES spectroscopy as a function of temperature and variable-temperature H-1 NMR spectroscopy. C1 [Nocton, Gregory] Ecole Polytech, CNRS, Lab Chim Mol, F-91128 Palaiseau, France. [Nocton, Gregory; Rozenel, Sergio S.; Andersen, Richard A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lukens, Wayne W.; Booth, Corwin H.; Rozenel, Sergio S.; Medling, Scott A.; Andersen, Richard A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Maron, Laurent] Univ Toulouse, CNRS, INSA, UPS,LPCNO,UMR 5215, Toulouse, France. RP Nocton, G (reprint author), Ecole Polytech, CNRS, Lab Chim Mol, F-91128 Palaiseau, France. EM greg.nocton@polytechnique.edu; raandersen@lbl.gov RI Nocton, Greg/D-4435-2009 FU CNRS; Ecole polytechnique; Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division, Heavy Element Chemistry Program of the U.S. Department of Energy [DE-AC02-05CH11231]; Humboldt Foundation FX G.N. would like to thank CNRS and Ecole polytechnique for funding. Work at University of California, Berkeley and at Lawrence Berkeley National Laboratory was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division, Heavy Element Chemistry Program of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. X-ray absorption data were collected at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. We thank Antonio DiPasquale at CHEXRAY Berkeley for his help with crystal structures. L.M. is member of the Institut Universitaire de France. Cines and CALMIP are acknowledged for a generous grant of computing time. L.M. would also like to thank the Humboldt Foundation for a fellowship. The authors thank a referee for suggestions that resulted in an improved manuscript. NR 56 TC 18 Z9 18 U1 5 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8626 EP 8641 DI 10.1021/ja502271q PG 16 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200026 PM 24852897 ER PT J AU Li, BY Zhang, YM Krishna, R Yao, KX Han, Y Wu, ZL Ma, DX Shi, Z Pham, T Space, B Liu, J Thallapally, PK Liu, J Chrzanowski, M Ma, SQ AF Li, Baiyan Zhang, Yiming Krishna, Rajamani Yao, Kexin Han, Yu Wu, Zili Ma, Dingxuan Shi, Zhan Pham, Tony Space, Brian Liu, Jian Thallapally, Praveen K. Liu, Jun Chrzanowski, Matthew Ma, Shengqian TI Introduction of pi-Complexation into Porous Aromatic Framework for Highly Selective Adsorption of Ethylene over Ethane SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; CONJUGATED MICROPOROUS POLYMERS; CARBON-DIOXIDE CAPTURE; KINETIC SEPARATION; OLEFIN-PARAFFIN; OLEFIN/PARAFFIN SEPARATIONS; SMALL HYDROCARBONS; HYDROGEN STORAGE; ROOM-TEMPERATURE; CO2 ADSORPTION AB In this work, we demonstrate for the first time the introduction of pi-complexation into a porous aromatic framework (PAF), affording significant increase in ethylene uptake capacity, as illustrated in the context of Ag(I) ion functionalized PAF-1, PAF-1-SO3Ag. LAST calculations using single-component-isotherm data and an equimolar ethylene/ethane ratio at 296 K reveal that PAF-1-SO3Ag shows exceptionally high ethylene/ethane adsorption selectivity (S-ads: 27 to 125), far surpassing benchmark zeolite and any other MOF reported in literature. The formation of pi-complexation between ethylene molecules and Ag(I) ions in PAF-1-SO3Ag has been evidenced by the high isosteric heats of adsorption of C2H4 and also proved by in situ IR spectroscopy studies. Transient breakthrough experiments, supported by simulations, indicate the feasibility of PAF-1-SO3Ag for producing 99.95%+ pure C2H4 in a Pressure Swing Adsorption operation. Our work herein thus suggests a new perspective to functionalizing PAFs and other types of advanced porous materials for highly selective adsorption of ethylene over ethane. C1 [Li, Baiyan; Zhang, Yiming; Pham, Tony; Space, Brian; Chrzanowski, Matthew; Ma, Shengqian] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. [Krishna, Rajamani] Univ Amsterdam, Vant Hoff Inst Mol Sci, NL-1098 XH Amsterdam, Netherlands. [Yao, Kexin; Han, Yu] King Abdullah Univ Sci & Technol, Phys Sci & Engn Div, Adv Membranes & Porous Mat Ctr, Thuwal 239556900, Saudi Arabia. [Wu, Zili] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wu, Zili] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Ma, Dingxuan; Shi, Zhan] Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China. [Liu, Jian; Thallapally, Praveen K.; Liu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Ma, SQ (reprint author), Univ S Florida, Dept Chem, 4202 E Fowler Ave, Tampa, FL 33620 USA. EM sqma@usf.edu RI thallapally, praveen/I-5026-2014; Pham, Tony/A-3787-2014; Krishna, Rajamani/A-1098-2012; Ma, Shengqian/B-4022-2012; Han, Yu /N-2036-2015; Wu, Zili/F-5905-2012; Liu, Jian/C-4707-2011; Liu, Jian/D-3393-2009 OI thallapally, praveen/0000-0001-7814-4467; Krishna, Rajamani/0000-0002-4784-8530; Ma, Shengqian/0000-0002-1897-7069; Han, Yu /0000-0003-1462-1118; Wu, Zili/0000-0002-4468-3240; Liu, Jian/0000-0001-5329-7408; Liu, Jian/0000-0001-5329-7408 FU University of South Florida; National Science Foundation [DMR-1352065]; Scientific User Facility Division, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); DOE/BES/Division of Materials Sciences and Engineering [KC020105-FWP12152]; National Natural Science Foundation of China [21371069] FX The authors acknowledge the University of South Florida for financial support of this work, and an award from the National Science Foundation (DMR-1352065) is also acknowledged. Part of the work including the in situ IR studies was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facility Division, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). DOE/BES/Division of Materials Sciences and Engineering (Award No. KC020105-FWP12152) (P.K.T.) and the National Natural Science Foundation of China (No. 21371069) (Z.S.) are acknowledged. We thank Prof. Jeffrey R. Long and Eric Bloch for their kind help on the calculation of regeneration energies. NR 99 TC 67 Z9 67 U1 34 U2 347 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8654 EP 8660 DI 10.1021/ja502119z PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200028 PM 24901372 ER PT J AU Wiedner, ES Appel, AM AF Wiedner, Eric S. Appel, Aaron M. TI Thermochemical Insight into the Reduction of CO to CH3OH with [Re(CO)](+) and [Mn(CO)](+) Complexes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL FORMYL COMPLEXES; ALPHA-HYDROXYALKYL COMPLEX; DISSOCIATION FREE-ENERGIES; HYDRIDE DONOR ABILITIES; CARBON-MONOXIDE; ELECTRODE-POTENTIALS; 1ST CARBONYLATION; RHODIUM FORMYL; BOND-ENERGIES; THERMODYNAMICS AB To gain insight into thermodynamic barriers for reduction of CO into CH3OH, free energies for reduction of [CpRe(PPh3)(NO)(CO)](+) into CpRe(PPh3)(NO)(CH2OH) have been determined from experimental measurements. Using model complexes, the free energies for the transfer of H+, H-, and e(-) have been determined. A pK(a) of 10.6 was estimated for [CpRe(PPh3)(NO)(CHOH)](+) by measuring the pK(a) for the analogous [CpRe(PPh3)(NO)(CMeOH)](+). The hydride donor ability (Delta G(H-)degrees) of CpRe(PPh3)(NO)(CH2OH) was estimated to be 58.0 kcal mol(-1), based on calorimetry measurements of the hydride-transfer reaction between CpRe(PPh3)(NO)(CHO) and [CpRe(PPh3)(NO)(CHOMe)](+) to generate the methylated analogue, CpRe(PPh3)(NO)(CH2OMe). Cyclic voltammograms recorded on CpRe(PPh3)(NO)(CMeO), CpRe(PPh3)(NO)(CH2OMe), and [CpRe(PPh3)(NO)(CHOMe)](+) displayed either a quasireversible oxidation (neutral species) or reduction (cationic species). These potentials were used as estimates for the oxidation of CpRe(PPh3)(NO)(CHO) or CpRe(PPh3)(NO)(CH2OH) or the reduction of [CpRe(PPh3)(NO)(CHOH)](+). Combination of the thermodynamic data permits construction of three-dimensional free energy landscapes under varying conditions of pH and PH2. The free energy for H-2 addition (Delta GH(2)degrees) to [CpRe(PPh3)(NO)(CO)](+) (+15 kcal mol(-1)) was identified as the most significant thermodynamic impediment for the reduction of CO. DFT computations on a series of [(CpM)-M-X(L)(NO)(CO)](+) (M = Re, Mn) complexes indicate that Delta GH(2)degrees can be varied by 11 kcal mol(-1) through variation of both the ancillary ligands and the metal. C1 [Wiedner, Eric S.; Appel, Aaron M.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Wiedner, ES (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,K2-57, Richland, WA 99352 USA. EM eric.wiedner@pnnl.gov OI Wiedner, Eric/0000-0002-7202-9676; Appel, Aaron/0000-0002-5604-1253 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Computational resources were provided at the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 61 TC 8 Z9 8 U1 2 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8661 EP 8668 DI 10.1021/ja502316e PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200029 PM 24853114 ER PT J AU Zhang, XY Canton, SE Smolentsev, G Wallentin, CJ Liu, YZ Kong, QY Attenkofer, K Stickrath, AB Mara, MW Chen, LX Warnmark, K Sundstrom, V AF Zhang, Xiaoyi Canton, Sophie E. Smolentsev, Grigory Wallentin, Carl-Johan Liu, Yizhu Kong, Qingyu Attenkofer, Klaus Stickrath, Andrew B. Mara, Michael W. Chen, Lin X. Warnmark, Kenneth Sundstrom, Villy TI Highly Accurate Excited-State Structure of [Os(bpy)(2)dcbpy](2+) Determined by X-ray Transient Absorption Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID INTERLIGAND ELECTRON-TRANSFER; POLYPYRIDYL COMPLEXES; DYE; COORDINATION; RUTHENIUM; OXIDATION; DYNAMICS; BASE AB Determining the electronic and geometric structures of photoexcited transient species with high accuracy is crucial for understanding their fundamental photochemistry and controlling their photoreactivity. We have applied X-ray transient absorption spectroscopy to measure the XANES and EXAFS spectra of a dilute (submillimolar) solution of the osmium(II) polypyridyl complex [Os(bpy)(2)dcbpy](PF6)(2) (dcbpy = 4,4'-dicarboxy-2,2'-bipyridine) (OsL2L') in methanol at the Os L-III edge. We have obtained spectra of superb quality for both the ground state and the photoinduced (MLCT)-M-3 excited state that have allowed us not only to extract detailed information about the Os 5d orbitals but also to resolve very small differences of 0.010 +/- 0.008 angstrom in the average Os-N bond lengths of the ground and excited states. Theoretical calculations using a recently developed DFT-based approach support the measured electronic structures and further identify the nature of the molecular orbitals that contribute to the main absorption bands in the XANES spectra. C1 [Zhang, Xiaoyi; Kong, Qingyu; Attenkofer, Klaus] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Canton, Sophie E.] Lund Univ, Dept Synchrotron Radiat Instrumentat, S-22100 Lund, Sweden. [Smolentsev, Grigory] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Wallentin, Carl-Johan; Liu, Yizhu; Warnmark, Kenneth] Lund Univ, Dept Chem, Ctr Anal & Synth, S-22100 Lund, Sweden. [Mara, Michael W.; Chen, Lin X.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Stickrath, Andrew B.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Sundstrom, Villy] Lund Univ, Dept Chem Phys, S-22100 Lund, Sweden. RP Zhang, XY (reprint author), Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM xyzhang@aps.anl.gov RI Wallentin, Carl-Johan/D-2559-2015; Canton, Sophie/A-8432-2016 OI Wallentin, Carl-Johan/0000-0003-1983-9378; FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Swedish Research Council; European Research Council [ERC-AdvG-VISCHEM-226136]; Swiss National Science Foundation [200021-135226]; European Commission [290605] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. S.E.C. acknowledges support from the Swedish Research Council. V.S. was supported by the Swedish Research Council and the European Research Council via Contract ERC-AdvG-VISCHEM-226136. G.S. was supported by the Swiss National Science Foundation (Grant 200021-135226) and the European Commission's Seventh Framework Program (FP7/2007-2013) under Grant Agreement 290605 (COFUND: PSI-FELLOW). Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 28 TC 10 Z9 10 U1 6 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8804 EP 8809 DI 10.1021/ja5040733 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200047 PM 24875220 ER PT J AU Knott, BC Crowley, MF Himmel, ME Stahlberg, J Beckham, GT AF Knott, Brandon C. Crowley, Michael F. Himmel, Michael E. Stahlberg, Jerry Beckham, Gregg T. TI Carbohydrate-Protein Interactions That Drive Processive Polysaccharide Translocation in Enzymes Revealed from a Computational Study of Cellobiohydrolase Processivity SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRICHODERMA-REESEI CELLOBIOHYDROLASE; PHANEROCHAETE-CHRYSOSPORIUM CEL7D; FAMILY 7 CELLOBIOHYDROLASE; 2.2 ANGSTROM RESOLUTION; BINDING FREE-ENERGY; CRYSTAL-STRUCTURE; CELLULOSE HYDROLYSIS; MOLECULAR-DYNAMICS; STRUCTURAL BASIS; ENDOGLUCANASE I AB Translocation of carbohydrate polymers through protein tunnels and clefts is a ubiquitous biochemical phenomenon in proteins such as polysaccharide synthases, glycoside hydrolases, and carbohydrate-binding modules. Although static snapshots of carbohydrate polymer binding in proteins have long been studied via crystallography and spectroscopy, the molecular details of polysaccharide chain processivity have not been elucidated. Here, we employ simulation to examine how a cellulose chain translocates by a disaccharide unit during the processive cycle of a glycoside hydrolase family 7 cellobiohydrolase. Our results demonstrate that these biologically and industrially important enzymes employ a two-step mechanism for chain threading to form a Michaelis complex and that the free energy barrier to chain threading is significantly lower than the hydrolysis barrier. Taken with previous studies, our findings suggest that the rate-limiting step in enzymatic cellulose degradation is the glycosylation reaction, not chain processivity. Based on the simulations, we find that strong electrostatic interactions with polar residues that are conserved in GH7 cellobiohydrolases, but not in GH7 endoglucanases, at the leading glucosyl ring provide the thermodynamic driving force for polysaccharide chain translocation. Also, we consider the role of aromatic carbohydrate interactions, which are widespread in carbohydrate-active enzymes and have long been associated with processivity. Our analysis suggests that the primary role for these aromatic residues is to provide tunnel shape and guide the carbohydrate chain to the active site. More broadly, this work elucidates the role of common protein motifs found in carbohydrate-active enzymes that synthesize or depolymerize polysaccharides by chain translocation mechanisms coupled to catalysis. C1 [Knott, Brandon C.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Crowley, Michael F.; Himmel, Michael E.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Stahlberg, Jerry] Swedish Univ Agr Sci, Dept Mol Biol, SE-75007 Uppsala, Sweden. RP Stahlberg, J (reprint author), Swedish Univ Agr Sci, Dept Mol Biol, SE-75007 Uppsala, Sweden. EM Jerry.Stahlberg@slu.se; Gregg.Beckham@nrel.gov RI Stahlberg, Jerry/D-4163-2013 OI Stahlberg, Jerry/0000-0003-4059-8580 FU NREL Director's Fellowship Program; Department of Energy BioEnergy Technologies Office; NREL Laboratory Directed Research and Development funds FX B.C.K. and G.T.B. thank the NREL Director's Fellowship Program for funding. M.F.C. and G.T.B. acknowledge funding from the Department of Energy BioEnergy Technologies Office and NREL Laboratory Directed Research and Development funds. The authors thank Prof. Christina M. Payne for creating the GH7 sequence alignment presented in the Supporting Information and Dr. Seonah Kim for creating the free energy profile figure (Figure 6). NR 90 TC 34 Z9 35 U1 4 U2 91 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 18 PY 2014 VL 136 IS 24 BP 8810 EP 8819 DI 10.1021/ja504074g PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AJ5KD UT WOS:000337720200048 PM 24869982 ER PT J AU Qu, D Zheng, M Zhang, LG Zhao, HF Xie, ZG Jing, XB Haddad, RE Fan, HY Sun, ZC AF Qu, Dan Zheng, Min Zhang, Ligong Zhao, Haifeng Xie, Zhigang Jing, Xiabin Haddad, Raid E. Fan, Hongyou Sun, Zaicheng TI Formation mechanism and optimization of highly luminescent N-doped graphene quantum dots SO SCIENTIFIC REPORTS LA English DT Article ID VISIBLE-LIGHT PHOTOCATALYSTS; CARBON DOTS; PHOTOVOLTAIC DEVICES; EMERGENT NANOLIGHTS; NITROGEN; NANODOTS; SENSORS AB Photoluminescent graphene quantum dots (GQDs) have received enormous attention because of their unique chemical, electronic and optical properties. Here a series of GQDs were synthesized under hydrothermal processes in order to investigate the formation process and optical properties of N-doped GQDs. Citric acid (CA) was used as a carbon precursor and self-assembled into sheet structure in a basic condition and formed N-free GQD graphite framework through intermolecular dehydrolysis reaction. N-doped GQDs were prepared using a series of N-containing bases such as urea. Detailed structural and property studies demonstrated the formation mechanism of N-doped GQDs for tunable optical emissions. Hydrothermal conditions promote formation of amide between -NH2 and -COOH with the presence of amine in the reaction. The intramoleculur dehydrolysis between neighbour amide and COOH groups led to formation of pyrrolic N in the graphene framework. Further, the pyrrolic N transformed to graphite N under hydrothermal conditions. N-doping results in a great improvement of PL quantum yield (QY) of GQDs. By optimized reaction conditions, the highest PL QY (94%) of N-doped GQDs was obtained using CA as a carbon source and ethylene diamine as a N source. The obtained N-doped GQDs exhibit an excitation-independent blue emission with single exponential lifetime decay. C1 [Qu, Dan; Zheng, Min; Zhang, Ligong; Zhao, Haifeng; Sun, Zaicheng] Changchun Inst Opt Fine Mech & Phys, State Key Lab Luminescence & Applicat, Changchun 130033, Jilin, Peoples R China. [Xie, Zhigang; Jing, Xiabin] Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Jilin, Peoples R China. [Qu, Dan] Univ Chinese Acad Sci, Beijing 100000, Peoples R China. [Haddad, Raid E.; Fan, Hongyou] Univ New Mexico, Ctr Microengn & Mat, Dept Chem & Nucl Engn, Albuquerque, NM 87106 USA. [Fan, Hongyou] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. RP Fan, HY (reprint author), Univ New Mexico, Ctr Microengn & Mat, Dept Chem & Nucl Engn, Albuquerque, NM 87106 USA. EM hfan@sandia.gov; sunzc@ciomp.ac.cn RI Zheng, Min/B-6267-2013; Sun, Zaicheng/B-5397-2012 OI Sun, Zaicheng/0000-0001-5277-5308 FU Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry; National Natural Science Foundation of China [21201159, 61176016]; "Hundred Talent Program" of CAS; Innovation and Entrepreneurship Program of Jilin; Science and technology department of Jilin [20121801]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The project was supported by Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry. The financial support from the National Natural Science Foundation of China (No. 21201159, 61176016), Z. S. thanks the support of the "Hundred Talent Program" of CAS, and Innovation and Entrepreneurship Program of Jilin. Science and technology department of Jilin (No. 20121801) Z. X. thanks the support of CIAC start-up fund. Sandia is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 34 TC 0 Z9 0 U1 28 U2 371 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 18 PY 2014 VL 4 AR 5294 DI 10.1038/srep05294 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ2PA UT WOS:000337498900001 ER PT J AU Taylor, R Monson, T Gullapalli, R AF Taylor, Robert M. Monson, Todd C. Gullapalli, Rama R. TI Influence of carbon chain length on the synthesis and yield of fatty amine-coated iron-platinum nanoparticles SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Iron-Platinum nanoparticles; SIPPs; Magnetic nanoparticles; Nanoparticle synthesis; Nanoparticle characterization; Cancer biology ID OXIDE NANOPARTICLES; STEALTH IMMUNOMICELLES; IN-VIVO AB Iron oxide nanoparticles are among the most widely used and characterized magnetic nanoparticles. However, metal alloys such as superparamagnetic iron-platinum particles (SIPPs), which have better magnetic properties, are receiving increased attention. Scalable techniques to routinely synthesize SIPPs in bulk need further study. Here, we focus on the role played by the fatty amine ligand in the formation of the bimetallic FePt nanocrystal. More specifically, we compare the effect of varying lengths of fatty amine ligands on the shape, structure, uniformity, composition, and magnetic properties of the SIPPs. We synthesized SIPPs by employing a 'green' thermal decomposition reaction using fatty amine ligands containing 12 to 18 carbons in length. Greater fatty amine chain length increased the polydispersity, particle concentration, iron concentration, and the stability of the SIPPs. Additionally, longer reflux times increased the diameter of the particles, but decreased the iron concentration, suggesting that shorter reaction times are preferable. Fourier transform infrared spectroscopy of the SIPPs indicates that the ligands are successfully bound to the FePt cores through the amine group. Superconducting quantum interference device magnetometry measurements suggest that all of the SIPPs were superparamagnetic at room temperature and that SIPPs synthesized using tetradecylamine had the highest saturation magnetization. Our findings indicate that the octadecylamine ligand, which is currently used for the routine synthesis of SIPPs, may not be optimal. Overall, we found that using tetradecylamine and a 30-min reflux reaction resulted in optimal particles with the highest degree of monodispersity, iron content, stability, and saturation magnetization. C1 [Taylor, Robert M.; Gullapalli, Rama R.] Univ New Mexico, Dept Pathol, Albuquerque, NM 87131 USA. [Monson, Todd C.] Sandia Natl Labs, Nanoscale Sci Dept, Albuquerque, NM 87185 USA. [Gullapalli, Rama R.] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. RP Gullapalli, R (reprint author), Univ New Mexico, Dept Pathol, Room 308,MSC06-4840, Albuquerque, NM 87131 USA. EM rgullapalli@salud.unm.edu OI Monson, Todd/0000-0002-9782-7084 FU ASERT-IRACDA [K12GM088021]; National Institute of General Medical Sciences; UNM Department of Pathology FX This research was supported by an ASERT-IRACDA grant, K12GM088021, from the National Institute of General Medical Sciences (RMT) and UNM Department of Pathology start up funds (RRG). We would also like to thank Dr. Lorraine Deck (UNM Department of Chemistry) for the use of the FTIR. NR 17 TC 3 Z9 3 U1 2 U2 26 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD JUN 17 PY 2014 VL 9 AR 306 DI 10.1186/1556-276X-9-306 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AL4PP UT WOS:000339115200001 PM 25006334 ER PT J AU Bullard, Z Girao, EC Daniels, C Sumpter, BG Meunier, V AF Bullard, Zachary Girao, Eduardo Costa Daniels, Colin Sumpter, Bobby G. Meunier, Vincent TI Quantifying energetics of topological frustration in carbon nanostructures SO PHYSICAL REVIEW B LA English DT Article ID HYDROCARBONS; NANOTUBES; GRAPHENE AB We develop a graph theoretical formalism to account for the fact that sp(2) carbon can become spin ordered or generate free radicals for purely topological reasons. While this phenomenon has been previously considered a binary operator, we here show a quantification in discrete units of frustrations. The graph theory method is combined with open density functional theory calculations to establish the existence of an energy of frustration that is shown to greatly improve the description of carbon nanostructure energetics using classical force fields. The methodology is illustrated for a number of systems and, owing to the small computational overhead associated with its evaluation, is expected to be easily integrable into any modeling approach based on a structure's adjacency matrix. C1 [Bullard, Zachary; Meunier, Vincent] Rensselaer Polytech Inst, Dept Mat Sci, Troy, NY 12180 USA. [Girao, Eduardo Costa] Univ Fed Piaui, Dept Fis, BR-64049550 Teresina, Piaui, Brazil. [Daniels, Colin; Meunier, Vincent] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci & Comp Sci, Oak Ridge, TN 37830 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Div Math, Oak Ridge, TN 37830 USA. RP Bullard, Z (reprint author), Rensselaer Polytech Inst, Dept Mat Sci, Troy, NY 12180 USA. RI Meunier, Vincent/F-9391-2010; Girao, Eduardo/C-5620-2012; Sumpter, Bobby/C-9459-2013 OI Meunier, Vincent/0000-0002-7013-179X; Sumpter, Bobby/0000-0001-6341-0355 FU Office of Naval Research; APS through the Brazil-US Physics Student Visitation Program; CNPq [473714/2013-2]; CAPES [A085/2013]; CNMS - Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the Office of Naval Research. Z.B. and E.C.G. acknowledge support from APS through the Brazil-US Physics Student Visitation Program. E.C.G. acknowledges support from CNPq (process number 473714/2013-2). E.C.G. and V.M. acknowledge support from CAPES through the Science Without Borders program (Project No. A085/2013). Calculations were performed on resources from the Computational Center for Innovations at Rensselaer Polytechnic Institute and the Center for Nanophase Materials Sciences (CNMS). Bobby G. Sumpter was supported by the CNMS, sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 29 TC 3 Z9 3 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 17 PY 2014 VL 89 IS 24 AR 245425 DI 10.1103/PhysRevB.89.245425 PG 7 WC Physics, Condensed Matter SC Physics GA AL3SR UT WOS:000339049900005 ER PT J AU Pathak, AK Paudyal, D Jayasekara, WT Calder, S Kreyssig, A Goldman, AI Gschneidner, KA Pecharsky, VK AF Pathak, Arjun K. Paudyal, D. Jayasekara, W. T. Calder, S. Kreyssig, A. Goldman, A. I. Gschneidner, K. A., Jr. Pecharsky, V. K. TI Unexpected magnetism, Griffiths phase, and exchange bias in the mixed lanthanide Pr0.6Er0.4Al2 SO PHYSICAL REVIEW B LA English DT Article ID BEHAVIOR; SYSTEMS; FIELD AB We report an unusual coexistence of ferromagnetism and ferrimagnetism, and metamagnetism in Pr0.6Er0.4Al2. In addition, this compound retains a clear Griffiths phase behavior even at 1 kOe magnetic field and shows a large exchange bias after field cooling from the paramagnetic state. The crystal-field excitations and opposite exchange interactions between nearest-neighbor and next-nearest-neighbor rare earth sites explain these behaviors. C1 [Pathak, Arjun K.; Paudyal, D.; Jayasekara, W. T.; Kreyssig, A.; Goldman, A. I.; Gschneidner, K. A., Jr.; Pecharsky, V. K.] Iowa State Univ, Ames Lab, US Dept Energy, Ames, IA 50011 USA. [Jayasekara, W. T.; Kreyssig, A.; Goldman, A. I.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Calder, S.] Oak Ridge Natl Lab, Neutron Sci Directorate, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Gschneidner, K. A., Jr.; Pecharsky, V. K.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Pathak, AK (reprint author), Iowa State Univ, Ames Lab, US Dept Energy, Ames, IA 50011 USA. EM pathak138@ameslab.gov OI Calder, Stuart/0000-0001-8402-3741 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. Research at the Oak Ridge National Laboratory High Flux Isotope Reactor is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE. NR 40 TC 10 Z9 10 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 17 PY 2014 VL 89 IS 22 AR 224411 DI 10.1103/PhysRevB.89.224411 PG 9 WC Physics, Condensed Matter SC Physics GA AL3SE UT WOS:000339048500001 ER PT J AU Vanhoefer, P Dalseno, J Kiesling, C Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Bakich, AM Bala, A Bhardwaj, V Bhuyan, B Bonvicini, G Bozek, A Bracko, M Browder, TE Chang, MC Chang, P Chekelian, V Chen, A Chen, P Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dolezal, Z Drasal, Z Eidelman, S Farhat, H Fast, JE Ferber, T Gaur, V Gabyshev, N Ganguly, S Garmash, A Gillard, R Goh, YM Golob, B Hara, T Hayasaka, K Hayashii, H Higuchi, T Horii, Y Hoshi, Y Hou, WS Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Iwashita, T Jaegle, I Julius, T Kah, DH Kato, E Kawai, H Kawasaki, T Kim, DY Kim, HO Kim, JB Kim, JH Kim, MJ Kim, YJ Kinoshita, K Klucar, J Ko, BR Korpar, S Krizan, P Krokovny, P Kronenbitter, B Kuhr, T Kumita, T Kuzmin, A Kwon, YJ Lange, JS Lee, SH Li, J Gioi, LL Libby, J Liu, C Liu, Y Liventsev, D Lukin, P Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Moser, HG Mussa, R Nakano, E Nakao, M Natkaniec, Z Nedelkovska, E Nisar, NK Nishida, S Nitoh, O Ogawa, S Pakhlov, P Pakhlova, G Park, CW Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Ryu, S Sahoo, H Saito, T Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Schwartz, AJ Semmler, D Senyo, K Seon, O Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumiyoshi, T Tamponi, U Tatishvili, G Teramoto, Y Trabelsi, K Tsuboyama, T Uchida, M Uehara, S Unno, Y Uno, S Vahsen, SE Van Hulse, C Varner, G Varvell, KE Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, Y Williams, KM Won, E Yamashita, Y Yashchenko, S Yook, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Vanhoefer, P. Dalseno, J. Kiesling, C. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Bakich, A. M. Bala, A. Bhardwaj, V. Bhuyan, B. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Chang, M. -C. Chang, P. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dolezal, Z. Drasal, Z. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Gaur, V. Gabyshev, N. Ganguly, S. Garmash, A. Gillard, R. Goh, Y. M. Golob, B. Hara, T. Hayasaka, K. Hayashii, H. Higuchi, T. Horii, Y. Hoshi, Y. Hou, W. -S. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Iwashita, T. Jaegle, I. Julius, T. Kah, D. H. Kato, E. Kawai, H. Kawasaki, T. Kim, D. Y. Kim, H. O. Kim, J. B. Kim, J. H. Kim, M. J. Kim, Y. J. Kinoshita, K. Klucar, J. Ko, B. R. Korpar, S. Krizan, P. Krokovny, P. Kronenbitter, B. Kuhr, T. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, S. -H. Li, J. Gioi, L. Li Libby, J. Liu, C. Liu, Y. Liventsev, D. Lukin, P. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Moser, H. -G. Mussa, R. Nakano, E. Nakao, M. Natkaniec, Z. Nedelkovska, E. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Pakhlov, P. Pakhlova, G. Park, C. W. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Ryu, S. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Schwartz, A. J. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumiyoshi, T. Tamponi, U. Tatishvili, G. Teramoto, Y. Trabelsi, K. Tsuboyama, T. Uchida, M. Uehara, S. Unno, Y. Uno, S. Vahsen, S. E. Van Hulse, C. Varner, G. Varvell, K. E. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, Y. Williams, K. M. Won, E. Yamashita, Y. Yashchenko, S. Yook, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Study of B-0 -> rho(0)rho(0) decays, implications for the CKM angle phi(2) and search for other B-0 decay modes with a four-pion final state (vol 89, 072008, 2014) SO PHYSICAL REVIEW D LA English DT Correction C1 [Vanhoefer, P.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. Beihang Univ, Beijing 100191, Peoples R China. SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. Novosibirsk State Univ, Novosibirsk 630090, Russia. Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. Chiba Univ, Chiba 2638522, Japan. Univ Cincinnati, Cincinnati, OH 45221 USA. DESY, D-22607 Hamburg, Germany. Fu Jen Catholic Univ, Dept Phys, Taipei 24205, Taiwan. Univ Giessen, D-35392 Giessen, Germany. Hanyang Univ, Seoul 133791, South Korea. Univ Hawaii, Honolulu, HI 96822 USA. High Energy Accelerator Org, KEK, Tsukuba, Ibaraki 3050801, Japan. Ikerbasque, Bilbao 48011, Spain. Indian Inst Technol, Gauhati 781039, Assam, India. Indian Inst Technol, Madras 600036, Tamil Nadu, India. Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. Inst High Energy Phys, A-1050 Vienna, Austria. Inst High Energy Phys, Protvino 142281, Russia. Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. Inst Theoret & Expt Phys, Moscow 117218, Russia. J Stefan Inst, Ljubljana 1000, Slovenia. Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. Univ Tokyo, Kavli Inst Phys & Math Univ WPI, Kashiwa, Chiba 2778583, Japan. Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. Korea Univ, Seoul 136713, South Korea. Kyungpook Natl Univ, Taegu 702701, South Korea. Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. Luther Coll, Decorah, IA 52101 USA. Univ Maribor, SLO-2000 Maribor, Slovenia. Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. Moscow Engn Phys Inst, Moscow 115409, Russia. Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. Nara Womens Univ, Nara 6308506, Japan. Natl Cent Univ, Chungli 32054, Taiwan. Natl United Univ, Miaoli 36003, Taiwan. Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. Nippon Dent Univ, Niigata 9518580, Japan. Niigata Univ, Niigata 9502181, Japan. Osaka City Univ, Osaka 5588585, Japan. Pacific NW Natl Lab, Richland, WA 99352 USA. Panjab Univ, Chandigarh 160014, India. Univ Pittsburgh, Pittsburgh, PA 15260 USA. Univ Sci & Technol China, Hefei 230026, Peoples R China. Seoul Natl Univ, Seoul 151742, South Korea. Soongsil Univ, Seoul 156743, South Korea. Sungkyunkwan Univ, Suwon 440746, South Korea. Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. Toho Univ, Funabashi, Chiba 2748510, Japan. Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. Tohoku Univ, Sendai, Miyagi 9808578, Japan. Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. Tokyo Inst Technol, Tokyo 1528550, Japan. Tokyo Metropolitan Univ, Tokyo 1920397, Japan. Tokyo Univ Agr & Technol, Tokyo 1848588, Japan. Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. Wayne State Univ, Detroit, MI 48202 USA. Yamagata Univ, Yamagata 9908560, Japan. Yonsei Univ, Seoul 120749, South Korea. Univ Turin, I-10124 Turin, Italy. RP Vanhoefer, P (reprint author), Univ Basque Country, UPV EHU, Bilbao 48080, Spain. RI Aihara, Hiroaki/F-3854-2010; Pakhlov, Pavel/K-2158-2013; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Pakhlova, Galina/C-5378-2014; Solovieva, Elena/B-2449-2014 OI Aihara, Hiroaki/0000-0002-1907-5964; Pakhlov, Pavel/0000-0001-7426-4824; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Solovieva, Elena/0000-0002-5735-4059 NR 1 TC 1 Z9 1 U1 1 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 17 PY 2014 VL 89 IS 11 AR 119903 DI 10.1103/PhysRevD.89.119903 PG 2 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AL3TF UT WOS:000339051400002 ER PT J AU Schenke, B Tribedy, P Venugopalan, R AF Schenke, Bjoern Tribedy, Prithwish Venugopalan, Raju TI Initial-state geometry and fluctuations in Au plus Au, Cu plus Au, and U plus U collisions at energies available at the BNL Relativistic Heavy Ion Collider SO PHYSICAL REVIEW C LA English DT Article ID HIGH-DENSITY QCD; ROOT-S(NN)=200 GEV; ELLIPTIC FLOW; NUCLEAR; SATURATION AB We study within the IP-Glasma and two-component MC-Glauber models the effects of initial-state geometry and fluctuations on multiplicities and eccentricities for several collision species at the Relativistic Heavy Ion Collider (RHIC). These include copper-gold (Cu + Au), gold-gold (Au + Au), and uranium-uranium (U + U) collisions. The multiplicity densities per participant pair are very similar in all systems studied. Ellipticities vary strongly between collision systems, most significantly for central collisions, while fluctuation driven odd moments vary little between systems. Event-by-event distributions of eccentricities in mid-central collisions are wider in Cu + Au relative to Au + Au and U + U systems. An anticorrelation between multiplicity and eccentricity is observed in ultracentral U + U collisions which is weaker in the IP-Glasma model than the two-component MC-Glauber model. In ultracentral Au + Au collisions the two models predict opposite signs for the slope of this correlation. Measurements of elliptic flow as a function of multiplicity in such central events can therefore be used to discriminate between models with qualitatively different particle production mechanisms. C1 [Schenke, Bjoern; Venugopalan, Raju] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Tribedy, Prithwish] Ctr Variable Energy Cyclotron, Kolkata 700064, India. RP Schenke, B (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. FU Office of Science of the US Department of Energy [DE-AC02-05CH11231]; DRONA and PRAFULLA cluster of Computer Division; LHC grid computing center at the Variable Energy Cyclotron Centre - Department of Atomic Energy, Government of India; DOE [DE-AC02-98CH10886] FX We thank Adam Bzdak, Subhasis Chattopadhyay, Roy Lacey, Hiroshi Masui, Pratap Roy, Paul Sorensen, and Hui Wang for interesting discussions. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231, the DRONA and PRAFULLA cluster of Computer Division and the LHC grid computing center at the Variable Energy Cyclotron Centre, supported by the Department of Atomic Energy, Government of India. B.P.S. and R.V. are supported under DOE Contract No. DE-AC02-98CH10886. NR 51 TC 14 Z9 14 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 17 PY 2014 VL 89 IS 6 AR 064908 DI 10.1103/PhysRevC.89.064908 PG 10 WC Physics, Nuclear SC Physics GA AL3SZ UT WOS:000339050800003 ER PT J AU Dugan, VG Emrich, SJ Giraldo-Calderon, GI Harb, OS Newman, RM Pickett, BE Schriml, LM Stockwell, TB Stoeckert, CJ Sullivan, DE Singh, I Ward, DV Yao, A Zheng, J Barrett, T Birren, B Brinkac, L Bruno, VM Caler, E Chapman, S Collins, FH Cuomo, CA Di Francesco, V Durkin, S Eppinger, M Feldgarden, M Fraser, C Fricke, WF Giovanni, M Henn, MR Hine, E Hotopp, JD Karsch-Mizrachi, I Kissinger, JC Lee, EM Mathur, P Mongodin, EF Murphy, CI Myers, G Neafsey, DE Nelson, KE Nierman, WC Puzak, J Rasko, D Roos, DS Sadzewicz, L Silva, JC Sobral, B Squires, RB Stevens, RL Tallon, L Tettelin, H Wentworth, D White, O Will, R Wortman, J Zhang, Y Scheuermann, RH AF Dugan, Vivien G. Emrich, Scott J. Giraldo-Calderon, Gloria I. Harb, Omar S. Newman, Ruchi M. Pickett, Brett E. Schriml, Lynn M. Stockwell, Timothy B. Stoeckert, Christian J., Jr. Sullivan, Dan E. Singh, Indresh Ward, Doyle V. Yao, Alison Zheng, Jie Barrett, Tanya Birren, Bruce Brinkac, Lauren Bruno, Vincent M. Caler, Elizabet Chapman, Sinead Collins, Frank H. Cuomo, Christina A. Di Francesco, Valentina Durkin, Scott Eppinger, Mark Feldgarden, Michael Fraser, Claire Fricke, W. Florian Giovanni, Maria Henn, Matthew R. Hine, Erin Hotopp, Julie Dunning Karsch-Mizrachi, Ilene Kissinger, Jessica C. Lee, Eun Mi Mathur, Punam Mongodin, Emmanuel F. Murphy, Cheryl I. Myers, Garry Neafsey, Daniel E. Nelson, Karen E. Nierman, William C. Puzak, Julia Rasko, David Roos, David S. Sadzewicz, Lisa Silva, Joana C. Sobral, Bruno Squires, R. Burke Stevens, Rick L. Tallon, Luke Tettelin, Herve Wentworth, David White, Owen Will, Rebecca Wortman, Jennifer Zhang, Yun Scheuermann, Richard H. TI Standardized Metadata for Human Pathogen/Vector Genomic Sequences SO PLOS ONE LA English DT Article ID BIOINFORMATICS RESOURCE; METAGENOMIC PROJECTS; MINIMUM INFORMATION; DATABASE GOLD; ONTOLOGIES AB High throughput sequencing has accelerated the determination of genome sequences for thousands of human infectious disease pathogens and dozens of their vectors. The scale and scope of these data are enabling genotype-phenotype association studies to identify genetic determinants of pathogen virulence and drug/insecticide resistance, and phylogenetic studies to track the origin and spread of disease outbreaks. To maximize the utility of genomic sequences for these purposes, it is essential that metadata about the pathogen/vector isolate characteristics be collected and made available in organized, clear, and consistent formats. Here we report the development of the GSCID/BRC Project and Sample Application Standard, developed by representatives of the Genome Sequencing Centers for Infectious Diseases (GSCIDs), the Bioinformatics Resource Centers (BRCs) for Infectious Diseases, and the U. S. National Institute of Allergy and Infectious Diseases (NIAID), part of the National Institutes of Health (NIH), informed by interactions with numerous collaborating scientists. It includes mapping to terms from other data standards initiatives, including the Genomic Standards Consortium's minimal information (MIxS) and NCBI's BioSample/BioProjects checklists and the Ontology for Biomedical Investigations (OBI). The standard includes data fields about characteristics of the organism or environmental source of the specimen, spatial-temporal information about the specimen isolation event, phenotypic characteristics of the pathogen/vector isolated, and project leadership and support. By modeling metadata fields into an ontology-based semantic framework and reusing existing ontologies and minimum information checklists, the application standard can be extended to support additional project-specific data fields and integrated with other data represented with comparable standards. The use of this metadata standard by all ongoing and future GSCID sequencing projects will provide a consistent representation of these data in the BRC resources and other repositories that leverage these data, allowing investigators to identify relevant genomic sequences and perform comparative genomics analyses that are both statistically meaningful and biologically relevant. C1 [Dugan, Vivien G.; Pickett, Brett E.; Stockwell, Timothy B.; Singh, Indresh; Brinkac, Lauren; Caler, Elizabet; Durkin, Scott; Nelson, Karen E.; Nierman, William C.; Wentworth, David; Zhang, Yun; Scheuermann, Richard H.] J Craig Venter Inst, Rockville, MD 20850 USA. [Dugan, Vivien G.; Pickett, Brett E.; Stockwell, Timothy B.; Singh, Indresh; Brinkac, Lauren; Caler, Elizabet; Durkin, Scott; Nelson, Karen E.; Nierman, William C.; Wentworth, David; Zhang, Yun; Scheuermann, Richard H.] J Craig Venter Inst, La Jolla, CA USA. [Dugan, Vivien G.; Yao, Alison; Di Francesco, Valentina; Giovanni, Maria; Lee, Eun Mi; Mathur, Punam; Squires, R. Burke] NIAID, Rockville, MD USA. [Emrich, Scott J.; Giraldo-Calderon, Gloria I.; Collins, Frank H.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Harb, Omar S.; Stoeckert, Christian J., Jr.; Zheng, Jie; Roos, David S.] Univ Penn, Philadelphia, PA 19104 USA. [Newman, Ruchi M.; Ward, Doyle V.; Birren, Bruce; Chapman, Sinead; Cuomo, Christina A.; Feldgarden, Michael; Henn, Matthew R.; Murphy, Cheryl I.; Neafsey, Daniel E.; Wortman, Jennifer] Broad Inst, Cambridge, MA USA. [Schriml, Lynn M.; Bruno, Vincent M.; Eppinger, Mark; Fraser, Claire; Fricke, W. Florian; Hine, Erin; Hotopp, Julie Dunning; Mongodin, Emmanuel F.; Myers, Garry; Rasko, David; Sadzewicz, Lisa; Silva, Joana C.; Tallon, Luke; Tettelin, Herve; White, Owen] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Sullivan, Dan E.; Sobral, Bruno; Will, Rebecca] Virginia Bioinformat Inst, Cyberinfrastruct Div, Blacksburg, VA USA. [Barrett, Tanya; Karsch-Mizrachi, Ilene] Natl Lib Med, Natl Ctr Biotechnol Informat, Bethesda, MD 20894 USA. [Kissinger, Jessica C.] Univ Georgia, Athens, GA 30602 USA. [Puzak, Julia] Kelly Govt Solut, Rockville, MD USA. [Stevens, Rick L.] Argonne Natl Lab, Lemont, IL USA. [Scheuermann, Richard H.] Univ Calif San Diego, Dept Pathol, San Diego, CA 92103 USA. RP Scheuermann, RH (reprint author), J Craig Venter Inst, Rockville, MD 20850 USA. EM rscheuermann@jcvi.org RI Zheng, Jie/M-1191-2015; OI Zheng, Jie/0000-0002-2999-0103; Cuomo, Christina/0000-0002-5778-960X; Wortman, Jennifer/0000-0002-8713-1227; Harb, Omar/0000-0003-4446-6200; David, Rasko/0000-0002-7337-7154; Fraser, Claire/0000-0003-1462-2428; Schriml, Lynn/0000-0001-8910-9851; Wentworth, David/0000-0002-5190-980X; Kissinger, Jessica/0000-0002-6413-1101; Squires, R Burke/0000-0001-9666-6285 FU U.S. National Institute of Allergy and Infectious Diseases [HHSN272200900018C, HHSN272200900009C, HHSN272200900007C]; Institute for Genome Sciences Genome at the University of Maryland; J. Craig Venter Institute; Bioinformatics Resource Centers [HHSN272200900038C, HHSN266200400041C, HHSN272200900040C, HHSN272200900039C, HHSN272200900041C]; EuPathDB; IRD; PATRIC; VectorBase; ViPR; NIH, National Library of Medicine; [R01GM093132] FX This work was made possible by the generous financial and philosophical support from the U.S. National Institute of Allergy and Infectious Diseases to the Genome Sequencing Centers for Infectious Diseases located at the Broad Institute of MIT and Harvard, the Institute for Genome Sciences Genome at the University of Maryland, and the J. Craig Venter Institute (Contract Numbers HHSN272200900018C, HHSN272200900009C, and HHSN272200900007C, respectively), and the Bioinformatics Resource Centers, including EuPathDB, IRD, PATRIC, VectorBase, and ViPR (Contract Numbers HHSN272200900038C, HHSN266200400041C, HHSN272200900040C, HHSN272200900039C, and HHSN272200900041C, respectively). This work was also supported in part by R01GM093132 and the Intramural Research Program of the NIH, National Library of Medicine. Although the funders were involved in manuscript editing and coordination, they had no direct role in study design, data collection and analysis, or the decision to publish. NR 29 TC 10 Z9 10 U1 2 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 17 PY 2014 VL 9 IS 6 AR e99979 DI 10.1371/journal.pone.0099979 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AK5YM UT WOS:000338503400061 PM 24936976 ER PT J AU Lupoi, JS Singh, S Davis, M Lee, DJ Shepherd, M Simmons, BA Henry, RJ AF Lupoi, Jason S. Singh, Seema Davis, Mark Lee, David J. Shepherd, Merv Simmons, Blake A. Henry, Robert J. TI High-throughput prediction of eucalypt lignin syringyl/guaiacyl content using multivariate analysis: a comparison between mid-infrared, near-infrared, and Raman spectroscopies for model development SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Biomass; Raman spectroscopy; Near-infrared spectroscopy; Fourier-transform infrared spectroscopy; High-throughput; Multivariate analysis; Lignin S/G ID GLOBULUS WOOD; MONOMER COMPOSITION; BAND ASSIGNMENTS; SYRINGYL LIGNIN; RAPID ANALYSIS; PY-GC/MS; GUAIACYL; SPECTRA; COMPONENTS; PYROLYSIS AB Background: In order to rapidly and efficiently screen potential biofuel feedstock candidates for quintessential traits, robust high-throughput analytical techniques must be developed and honed. The traditional methods of measuring lignin syringyl/guaiacyl (S/G) ratio can be laborious, involve hazardous reagents, and/or be destructive. Vibrational spectroscopy can furnish high-throughput instrumentation without the limitations of the traditional techniques. Spectral data from mid-infrared, near-infrared, and Raman spectroscopies was combined with S/G ratios, obtained using pyrolysis molecular beam mass spectrometry, from 245 different eucalypt and Acacia trees across 17 species. Iterations of spectral processing allowed the assembly of robust predictive models using partial least squares (PLS). Results: The PLS models were rigorously evaluated using three different randomly generated calibration and validation sets for each spectral processing approach. Root mean standard errors of prediction for validation sets were lowest for models comprised of Raman (0.13 to 0.16) and mid-infrared (0.13 to 0.15) spectral data, while near-infrared spectroscopy led to more erroneous predictions (0.18 to 0.21). Correlation coefficients (r) for the validation sets followed a similar pattern: Raman (0.89 to 0.91), mid-infrared (0.87 to 0.91), and near-infrared (0.79 to 0.82). These statistics signify that Raman and mid-infrared spectroscopy led to the most accurate predictions of S/ G ratio in a diverse consortium of feedstocks. Conclusion: Eucalypts present an attractive option for biofuel and biochemical production. Given the assortment of over 900 different species of Eucalyptus and Corymbia, in addition to various species of Acacia, it is necessary to isolate those possessing ideal biofuel traits. This research has demonstrated the validity of vibrational spectroscopy to efficiently partition different potential biofuel feedstocks according to lignin S/ G ratio, significantly reducing experiment and analysis time and expense while providing non-destructive, accurate, global, predictive models encompassing a diverse array of feedstocks. C1 [Lupoi, Jason S.; Simmons, Blake A.; Henry, Robert J.] Univ Queensland, Queensland Alliance Agr & Food Innovat, St Lucia, Qld 4072, Australia. [Lupoi, Jason S.; Singh, Seema; Simmons, Blake A.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Singh, Seema; Simmons, Blake A.] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA 94551 USA. [Davis, Mark] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Davis, Mark] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Lee, David J.] Univ Sunshine Coast, Forest Ind Res Ctr, Maroochydore, Qld 4558, Australia. [Lee, David J.] Queensland Dept Agr Fisheries & Forestry, Maroochydore, Qld 4558, Australia. [Shepherd, Merv] So Cross Univ, Lismore, NSW 2480, Australia. RP Lupoi, JS (reprint author), Univ Queensland, Queensland Alliance Agr & Food Innovat, 306 Carmody Rd, St Lucia, Qld 4072, Australia. EM jslupoi@lbl.gov RI Henry, Robert/B-5824-2008; Shepherd, Mervyn/F-1068-2011; OI Henry, Robert/0000-0002-4060-0292; Shepherd, Mervyn/0000-0001-8708-4670; davis, mark/0000-0003-4541-9852 FU Queensland Alliance for Agriculture and Food Innovation; Joint BioEnergy Institute; Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-AC02-05CH11231] FX This manuscript was supported as part of a collaboration between the Queensland Alliance for Agriculture and Food Innovation and the Joint BioEnergy Institute. The work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under contract number DE-AC02-05CH11231. The authors would like to thank Robert Sykes and Erica Gjersing at the National Renewable Energy Lab for obtaining the pyMBMS data and providing assistance and guidance with respect to the high-throughput pyMBMS pipeline, John Bartle at the Western Australian Department of Environment and Conservation, and Adam Healey at the University of Queensland, for the collecting and processing of some the wood samples and for information regarding the environmental specifications of the growing sites. The material from the Queensland and New South Wales sites was accessed from Queensland Department of Agriculture, Fisheries and Forestry trials. NR 50 TC 6 Z9 6 U1 4 U2 58 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUN 17 PY 2014 VL 7 AR 93 DI 10.1186/1754-6834-7-93 PG 14 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AK4FW UT WOS:000338380400001 PM 24955114 ER PT J AU Jacobs, CB Ivanov, IN Nguyen, MD Zestos, AG Venton, BJ AF Jacobs, Christopher B. Ivanov, Ilia N. Nguyen, Michael D. Zestos, Alexander G. Venton, B. Jill TI High Temporal Resolution Measurements of Dopamine with Carbon Nanotube Yarn Microelectrodes SO ANALYTICAL CHEMISTRY LA English DT Article ID SCAN CYCLIC VOLTAMMETRY; ELECTRON-TRANSFER KINETICS; FIBER MICROELECTRODES; RAMAN-SPECTRA; IN-VIVO; PYROLYTIC-GRAPHITE; POROUS LAYERS; SURFACES; ELECTROCHEMISTRY; NEUROTRANSMITTERS AB Fast-scan cyclic voltammetry (FSCV) can detect small changes in dopamine concentration; however, measurements are typically limited to scan repetition frequencies of 10 Hz. Dopamine oxidation at carbon-fiber microelectrodes (CFMEs) is dependent on dopamine adsorption, and increasing the frequency of FSCV scan repetitions decreases the oxidation current, because the time for adsorption is decreased. Using a commercially available carbon nanotube yarn, we characterized carbon nanotube yarn microelectrodes (CNTYMEs) for high-speed measurements with FSCV. For dopamine, CNTYMEs have a significantly lower Delta E-p than CFMEs, a limit of detection of 10 +/- 0.8 nM, and a linear response to 25 mu M. Unlike CFMEs, the oxidation current of dopamine at CNTYMEs is independent of scan repetition frequency. At a scan rate of 2000 V/s, dopamine can be detected, without any loss in sensitivity, with scan frequencies up to 500 Hz, resulting in a temporal response that is four times faster than CFMEs. While the oxidation current is adsorption-controlled at both CFMEs and CNTYIVLEs, the adsorption and desorption kinetics differ. The desorption coefficient of dopamine-o-quinone (DOQ), the oxidation product of dopamine, is an order of magnitude larger than that of dopamine at CFMEs; thus, DOQ desorbs from the electrode and can diffuse away. At CNTYMEs, the rates of desorption for dopamine and dopamine-o-quinone are about equal, resulting in current that is independent of scan repetition frequency. Thus, there is no compromise with CNTYMEs: high sensitivity, high sampling frequency, and high temporal resolution can be achieved simultaneously. Therefore, CNTYMEs are attractive for high-speed applications. C1 [Jacobs, Christopher B.; Nguyen, Michael D.; Zestos, Alexander G.; Venton, B. Jill] Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. [Ivanov, Ilia N.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Venton, BJ (reprint author), Univ Virginia, Dept Chem, McCormick Rd,Box 400319, Charlottesville, VA 22904 USA. EM bjv2n@virginia.edu RI Venton, B. Jill/A-2902-2008; ivanov, ilia/D-3402-2015; OI Venton, B. Jill/0000-0002-5096-9309; ivanov, ilia/0000-0002-6726-2502; Jacobs, Christopher/0000-0001-7906-6368 FU Center for Nanophase Materials Sciences [CNMS2012-070, CNMS2014-083]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation (NSF) [CHE0645587522]; NIH [R21DA037584, R01MH085159] FX A portion of this research was conducted at the Center for Nanophase Materials Sciences, (through user grant Nos. CNMS2012-070 and CNMS2014-083), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research was funded by the National Science Foundation (NSF) (CHE0645587522) and NIH (Nos. R21DA037584 and R01MH085159). NR 62 TC 16 Z9 16 U1 2 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUN 17 PY 2014 VL 86 IS 12 BP 5721 EP 5727 DI 10.1021/ac404050t PG 7 WC Chemistry, Analytical SC Chemistry GA AJ4JX UT WOS:000337643500022 PM 24832571 ER PT J AU Myung, JH Gajjar, KA Chen, JH Molokie, RE Hong, S AF Myung, Ja Hye Gajjar, Khyati A. Chen, Jihua Molokie, Robert E. Hong, Seungpyo TI Differential Detection of Tumor Cells Using a Combination of Cell Rolling, Multivalent Binding, and Multiple Antibodies SO ANALYTICAL CHEMISTRY LA English DT Article ID METASTATIC BREAST-CANCER; RESISTANT PROSTATE-CANCER; CAPTURE; EXPRESSION; PROGRESSION; SURVIVAL; THERAPY; BLOOD; EPCAM; ASSAY AB Effective quantification and in situ identification of circulating tumor cells (CTCs) in blood are still elusive because of the extreme rarity and heterogeneity of the cells. In our previous studies, we developed a novel platform that captures tumor cells at significantly improved efficiency in vitro using a unique biomimetic combination of two physiological processes: E-selectin-induced cell rolling and poly(amidoamine) (PAMAM) dendrimer-mediated strong multivalent binding. Herein, we have engineered a novel multifunctional surface, on the basis of the biomimetic cell capture, through optimized incorporation of multiple antibodies directed to cancer cell-specific surface markers, such as epithelial cell adhesion molecule (EpCAM), human epidermal growth factor receptor-2 (HER-2), and prostate specific antigen (PSA). The surfaces were tested using a series of tumor cells, MDA-PCa-2b, MCF-7, and MDA-MB-361, both in mixture in vitro and after being spiked into human blood. Our multifunctional surface demonstrated highly efficient capture of tumor cells in human blood, achieving up to 82% capture efficiency (similar to 10-fold enhancement than a surface with the antibodies alone) and up to 90% purity. Furthermore, the multipatterned antibodies allowed differential capturing of the tumor cells. These results support that our multifunctional surface has great potential as an effective platform that accommodates virtually any antibodies, which will likely lead to clinically significant, differential detection of CTCs that are rare and highly heterogeneous. C1 [Myung, Ja Hye; Gajjar, Khyati A.; Molokie, Robert E.; Hong, Seungpyo] Univ Illinois, Dept Biopharmaceut Sci, Chicago, IL 60612 USA. [Molokie, Robert E.] Univ Illinois, Dept Med, Chicago, IL 60612 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Molokie, Robert E.] Jesse Brown VA Med Ctr, Chicago, IL 60612 USA. RP Hong, S (reprint author), Univ Illinois, Dept Biopharmaceut Sci, Chicago, IL 60612 USA. EM sphong@uic.edu RI Chen, Jihua/F-1417-2011 OI Chen, Jihua/0000-0001-6879-5936 FU National Science Foundation (NSF) [CBET-0931472]; University of Illinois Cancer Center; Office of Technology Managements of the University of Illinois at Chicago (UIC); NCRR NIH [C06RR15482]; UIC; Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy FX This work was supported by National Science Foundation (NSF) under Grant CBET-0931472, University of Illinois Cancer Center, and the Office of Technology Managements of the University of Illinois at Chicago (UIC). This investigation was conducted in a facility constructed with support from grant C06RR15482 from the NCRR NIH. The authors thank Dr. Shawn Oppegard for his help in fabricating the PDMS gaskets with the customized channels and helpful discussion throughout the work J.H.M. was partially supported by Dean's scholarship and Chancellor's Graduate Fellowship, both from UIC. Energy filtered transmission electron microscopy was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy. NR 39 TC 11 Z9 12 U1 7 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUN 17 PY 2014 VL 86 IS 12 BP 6088 EP 6094 DI 10.1021/ac501243a PG 7 WC Chemistry, Analytical SC Chemistry GA AJ4JX UT WOS:000337643500070 PM 24892731 ER PT J AU Perticaroli, S Nickels, JD Ehlers, G Sokolov, AP AF Perticaroli, Stefania Nickels, Jonathan D. Ehlers, Georg Sokolov, Alexei P. TI Rigidity, Secondary Structure, and the Universality of the Boson Peak in Proteins SO BIOPHYSICAL JOURNAL LA English DT Article ID INELASTIC NEUTRON-SCATTERING; RAMAN-SCATTERING; LIGHT-SCATTERING; DYNAMICS; GLASSES; MODES; VIBRATIONS; LIQUIDS; ORIGIN; ENZYME AB Complementary neutron- and light-scattering results on nine proteins and amino acids reveal the role of rigidity and secondary structure in determining the time- and lengthscales of low-frequency collective vibrational dynamics in proteins. These dynamics manifest in a spectral feature, known as the boson peak (BP), which is common to all disordered materials. We demonstrate that BP position scales systematically with structural motifs, reflecting local rigidity: disordered proteins appear softer than a-helical proteins; which are softer than beta-sheet proteins. Our analysis also reveals a universal spectral shape of the BP in proteins and amino acid mixtures; superimposable on the shape observed in typical glasses. Uniformity in the underlying physical mechanism, independent of the specific chemical composition, connects the BP vibrations to nanometer-scale heterogeneities, providing an experimental benchmark for coarse-grained simulations, structure/rigidity relationships, and engineering of proteins for novel applications. C1 [Perticaroli, Stefania; Nickels, Jonathan D.; Sokolov, Alexei P.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37830 USA. [Perticaroli, Stefania; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem & Mat Sci, Oak Ridge, TN USA. [Perticaroli, Stefania; Nickels, Jonathan D.; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ehlers, Georg] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN USA. RP Nickels, JD (reprint author), Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37830 USA. EM nickelsjd@ornl.gov RI Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; Nickels, Jonathan/I-1913-2012 OI Ehlers, Georg/0000-0003-3513-508X; Nickels, Jonathan/0000-0001-8351-7846 FU Department of Energy [DE-FG02-08ER46528]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; UT-Battelle, LLC; U.S. Department of Energy [DEAC05-00OR22725] FX The authors acknowledge Department of Energy support through the EPSCoR program (grant DE-FG02-08ER46528) and the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Oak Ridge National Laboratory facilities are sponsored by UT-Battelle, LLC, for the U.S. Department of Energy under contract No. DEAC05-00OR22725. NR 63 TC 15 Z9 15 U1 4 U2 26 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JUN 17 PY 2014 VL 106 IS 12 BP 2667 EP 2674 DI 10.1016/j.bpj.2014.05.009 PG 8 WC Biophysics SC Biophysics GA AJ4QY UT WOS:000337662100016 PM 24940784 ER PT J AU Dong, WM Wan, JM AF Dong, Wenming Wan, Jiamin TI Additive Surface Complexation Modeling of Uranium(VI) Adsorption onto Quartz-Sand Dominated Sediments SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SAVANNA RIVER SITE; HUMIC SUBSTANCES; FULVIC-ACID; CONTAMINANT MIGRATION; TAILINGS IMPOUNDMENT; NATURAL ATTENUATION; SORPTION COMPLEXES; GROUNDWATER PLUME; URANYL ADSORPTION; CLAY-MINERALS AB Many aquifers contaminated by U(VI)-containing acidic plumes are composed predominantly of quartz-sand sediments. The F-Area of the Savannah River Site (SRS) in South Carolina (USA) is an example. To predict U(VI) mobility and natural attenuation, we conducted U(VI) adsorption experiments using the F-Area plume sediments and reference quartz, goethite, and kaolinite. The sediments are composed of similar to 96% quartz-sand and 3-4% fine fractions of kaolinite and goethite. We developed a new humic acid adsorption method for determining the relative surface area abundances of goethite and kaolinite in the fine fractions. This method is expected to be applicable to many other binary mineral pairs, and allows successful application of the component additivity (CA) approach based surface complexation modeling (SCM) at the SRS F-Area and other similar aquifers. Our experimental results indicate that quartz has stronger U(VI) adsorption ability per unit surface area than goethite and kaolinite at pH <= 4.0. Our modeling results indicate that the binary (goethite/kaolinite) CA-SCM under-predicts U(VI) adsorption to the quartz-sand dominated sediments at pH <= 4.0. The new ternary (quartz/goethite/kaolinite) CA-SCM provides excellent predictions. The contributions of quartz-sand, kaolinite, and goethite to U(VI) adsorption and the potential influences of dissolved Al, Si, and Fe are also discussed. C1 [Dong, Wenming; Wan, Jiamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Dong, WM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM wenmingdong@lbl.gov RI Dong, Wenming/G-3221-2015; Wan, Jiamin/H-6656-2014 OI Dong, Wenming/0000-0003-2074-8887; FU Sustainable Systems (SS) Scientific Focus Area (SFA) program at LBNL by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program [DE-AC02-05CH11231] FX The work reported here is supported as part of the Sustainable Systems (SS) Scientific Focus Area (SFA) program at LBNL, supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program, through Contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. We thank Dr. Miles Denham (SRNL) for providing us the sediment samples from SRS, and the anonymous reviewers for their helpful comments. NR 67 TC 11 Z9 11 U1 4 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUN 17 PY 2014 VL 48 IS 12 BP 6569 EP 6577 DI 10.1021/es501782g PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AJ4KU UT WOS:000337646000007 PM 24865372 ER PT J AU Pallagi, A Bajnoczi, EG Canton, SE Bolin, T Peintler, G Kutus, B Kele, Z Palinko, I Sipos, P AF Pallagi, Attila Bajnoczi, Eva G. Canton, Sophie E. Bolin, Trudy Peintler, Gabor Kutus, Bence Kele, Zoltan Palinko, Istvan Sipos, Pal TI Multinuclear Complex Formation between Ca(II) and Gluconate Ions in Hyperalkaline Solutions SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ABSORPTION FINE-STRUCTURE; ISOSACCHARINIC ACID; ALKALINE CONDITIONS; AQUEOUS-SOLUTION; CARBOXYLIC-ACIDS; DEGRADATION; SOLUBILITY; CALCIUM; CELLULOSE; PRODUCTS AB Alkaline solutions containing polyhydroxy carboxylates and Ca(II) are typical in cementitious radioactive waste repositories. Gluconate (Gluc(-)) is a structural and functional representative of these sugar carboxylates. In the current study, the structure and equilibria of complexes forming in such strongly alkaline solutions containing Ca2+ and gluconate have been studied. It was found that Gluc(-) significantly increases the solubility of portlandite (Ca(OH)(2)(s)) under these conditions and Ca2+ complexes of unexpectedly high stability are formed. The mononuclear (CaGluc(+) and [CaGlucOH](0)) complexes were found to be minor species, and predominant multinuclear complexes were identified. The formation of the neutral [Ca(2)Gluc(OH)(3)](0) (log beta(213) = 8.03) and [Ca(3)Gluc(2)(OH)(4)](0) (log beta(324) = 12.39) has been proven via H-2/Pt-electrode potentiometric measurements and was confirmed via XAS, H-1 NMR, ESI-MS, conductometry, and freezing-point depression experiments. The binding sites of Gluc- were identified from multinuclear NMR measurements. Besides the carboxylate group, the O atoms on the second and third carbon atoms were proved to be the most probable sites for Ca2+ binding. The suggested structure of the trinuclear complex was deduced from ab initio calculations. These observations are of relevance in the thermodynamic modeling of radioactive waste repositories, where the predominance of the binuclear Ca2+ complex, which is a precursor of various high-stability ternary complexes with actinides, is demonstrated. C1 [Pallagi, Attila; Bajnoczi, Eva G.; Kutus, Bence; Sipos, Pal] Univ Szeged, Dept Inorgan & Analyt Chem, H-6720 Szeged, Hungary. [Pallagi, Attila; Bajnoczi, Eva G.; Peintler, Gabor; Kutus, Bence; Palinko, Istvan; Sipos, Pal] Univ Szeged, Mat & Solut Struct Res Grp, H-6720 Szeged, Hungary. [Canton, Sophie E.] Lund Univ, Dept Synchrotron Radiat Instrumentat, SE-22100 Lund, Sweden. [Bolin, Trudy] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Peintler, Gabor] Univ Szeged, Dept Phys Chem & Mat Sci, H-6720 Szeged, Hungary. [Kele, Zoltan] Univ Szeged, Dept Med Chem, H-6720 Szeged, Hungary. [Palinko, Istvan] Univ Szeged, Dept Organ Chem, H-6720 Szeged, Hungary. RP Sipos, P (reprint author), Univ Szeged, Dept Inorgan & Analyt Chem, Dom ter 7, H-6720 Szeged, Hungary. EM sipos@chem.u-szeged.hu RI Palinko, Istvan/A-3943-2008; Canton, Sophie/A-8432-2016 OI Palinko, Istvan/0000-0002-8508-309X; FU European Union; State of Hungary - European Social Fund [TAMOP-4.2.4.A/2-11/1-2012-0001]; National Research Fund of Hungary [OTKA 83889, TAMOP-4.2.2/C]; U.S. DOE [DE-AC02-06CH11357] FX We are grateful for the useful discussions received from Dr. Xavier Gaona and for technical assistance provided by Ilona Halasine-Varga. The research of A.P. and B.K. was supported by the European Union and the State of Hungary, cofinanced by the European Social Fund in the framework of TAMOP-4.2.4.A/2-11/1-2012-0001 "National Excellence Program". Research leading to this contribution was financed by the National Research Fund of Hungary through grant OTKA 83889 and TAMOP-4.2.2/C. The use of the Advanced Photon Source, an Office of Science User Facility operated for DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract DE-AC02-06CH11357. All these supports are highly appreciated. NR 54 TC 8 Z9 8 U1 3 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUN 17 PY 2014 VL 48 IS 12 BP 6604 EP 6611 DI 10.1021/es501067w PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AJ4KU UT WOS:000337646000011 PM 24865662 ER PT J AU Mason, HE Walsh, SDC DuFrane, WL Carroll, SA AF Mason, Harris E. Walsh, Stuart D. C. DuFrane, Wyatt L. Carroll, Susan A. TI Determination of Diffusion Profiles in Altered Wellbore Cement Using X-ray Computed Tomography Methods SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID GEOLOGIC SEQUESTRATION CONDITIONS; GEOTHERMAL GROUTS; CALCIUM HYDROXIDE; CO2-RICH BRINE; CARBON-DIOXIDE; CO2 ATTACK; SYSTEMS; MICROTOMOGRAPHY; DEGRADATION; INTEGRITY AB The development of accurate, predictive models for use in determining wellbore integrity requires detailed information about the chemical and mechanical changes occurring in hardened Portland cements. X-ray computed tomography (XRCT) provides a method that can nondestructively probe these changes in three dimensions. Here, we describe a method for extracting subvoxel mineralogical and chemical information from synchrotron XRCT images by combining advanced image segmentation with geochemical models of cement alteration. The method relies on determining "effective linear activity coefficients" (ELAC) for the white light source to generate calibration curves that relate the image grayscales to material composition. The resulting data set supports the modeling of cement alteration by CO2-rich brine with discrete increases in calcium concentration at reaction boundaries. The results of these XRCT analyses can be used to further improve coupled geochemical and mechanical models of cement alteration in the wellbore environment. C1 [Mason, Harris E.; Walsh, Stuart D. C.; DuFrane, Wyatt L.; Carroll, Susan A.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94559 USA. RP Mason, HE (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94559 USA. EM mason42@llnl.gov RI Mason, Harris/F-7194-2011; OI Mason, Harris/0000-0002-1840-0550; Walsh, Stuart/0000-0001-8155-4870 FU DOE National Energy Technology Laboratory [AA3030100]; Office of Basic Energy Sciences of the US Department of Energy [DE-AC0-2-05CH11231]; LLNL [DE-AC52-07NA27344] FX We are grateful for the support of this work under the DOE National Energy Technology Laboratory, Project AA3030100. The Advanced Light Source is supported by the Director, Office of Basic Energy Sciences of the US Department of Energy under Contract No. DE-AC0-2-05CH11231. We thank A. MacDowell and D. Parkinson for their assistance at the beamline. We would like to thank M. Smith for assistance with the initial setup of the core-flood experiment, Z. Dai for assistance with performing SEM/EDS analyses, S. Torres and D. Ruddle for preparation of sample cores, and L. Knauer and the California Well Sample Repository for the caprock samples. This work was performed by LLNL under Contract DE-AC52-07NA27344. NR 36 TC 6 Z9 6 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUN 17 PY 2014 VL 48 IS 12 BP 7094 EP 7100 DI 10.1021/es4055737 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AJ4KU UT WOS:000337646000069 PM 24869420 ER PT J AU White, JA Chiaramonte, L Ezzedine, S Foxall, W Hao, Y Ramirez, A McNab, W AF White, Joshua A. Chiaramonte, Laura Ezzedine, Souheil Foxall, William Hao, Yue Ramirez, Abelardo McNab, Walt TI Geomechanical behavior of the reservoir and caprock system at the In Salah CO2 storage project SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbon sequestration; geomechanics ID SAR INTERFEROMETRY; INJECTION WELL; SURFACE UPLIFT; ALGERIA; KRECHBA; FIELD; SIMULATION; SLEIPNER AB Almost 4 million metric tons of CO2 were injected at the In Salah CO2 storage site between 2004 and 2011. Storage integrity at the site is provided by a 950-m-thick caprock that sits above the injection interval. This caprock consists of a number of low-permeability units that work together to limit vertical fluid migration. These are grouped into main caprock units, providing the primary seal, and lower caprock units, providing an additional buffer and some secondary storage capacity. Monitoring observations at the site indirectly suggest that pressure, and probably CO2, have migrated upward into the lower portion of the caprock. Although there are no indications that the overall storage integrity has been compromised, these observations raise interesting questions about the geomechanical behavior of the system. Several hypotheses have been put forward to explain the measured pressure, seismic, and surface deformation behavior. These include fault leakage, flow through preexisting fractures, and the possibility that injection pressures induced hydraulic fractures. This work evaluates these hypotheses in light of the available data. We suggest that the simplest and most likely explanation for the observations is that a portion of the lower caprock was hydrofractured, although interaction with preexisting fractures may have played a significant role. There are no indications, however, that the overall storage complex has been compromised, and several independent data sets demonstrate that CO2 is contained in the confinement zone. C1 [White, Joshua A.; Chiaramonte, Laura; Foxall, William; Hao, Yue; Ramirez, Abelardo; McNab, Walt] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. [Ezzedine, Souheil] Lawrence Livermore Natl Lab, Computat Engn Div, Livermore, CA 94550 USA. RP White, JA (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. EM jawhite@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We are grateful for collaboration with the Joint Industry Project, other research partners, and members of the Science Advisory Board. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Data and cofunding were provided by the In Salah Joint Industry Project. NR 24 TC 21 Z9 22 U1 2 U2 26 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 17 PY 2014 VL 111 IS 24 BP 8747 EP 8752 DI 10.1073/pnas.1316465111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9XO UT WOS:000337300100023 PM 24912156 ER PT J AU Glotter, M Elliott, J McInerney, D Best, N Foster, I Moyer, EJ AF Glotter, Michael Elliott, Joshua McInerney, David Best, Neil Foster, Ian Moyer, Elisabeth J. TI Evaluating the utility of dynamical downscaling in agricultural impacts projections SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE agriculture; food security; NARCCAP; CORDEX ID CLIMATE-CHANGE SCENARIOS; GENERAL-CIRCULATION MODEL; SOUTHEASTERN UNITED-STATES; SPATIAL SCALE; CROPS; ADAPTATION; WHEAT; PRECIPITATION; TEMPERATURES; SIMULATIONS AB Interest in estimating the potential socioeconomic costs of climate change has led to the increasing use of dynamical downscalingnested modeling in which regional climate models (RCMs) are driven with general circulation model (GCM) output-to produce fine-spatial-scale climate projections for impacts assessments. We evaluate here whether this computationally intensive approach significantly alters projections of agricultural yield, one of the greatest concerns under climate change. Our results suggest that it does not. We simulate US maize yields under current and future CO2 concentrations with the widely used Decision Support System for Agrotechnology Transfer crop model, driven by a variety of climate inputs including two GCMs, each in turn downscaled by two RCMs. We find that no climate model output can reproduce yields driven by observed climate unless a bias correction is first applied. Once a bias correction is applied, GCM-and RCM-driven US maize yields are essentially indistinguishable in all scenarios (< 10% discrepancy, equivalent to error from observations). Although RCMs correct some GCM biases related to fine-scale geographic features, errors in yield are dominated by broad-scale (100s of kilometers) GCM systematic errors that RCMs cannot compensate for. These results support previous suggestions that the benefits for impacts assessments of dynamically downscaling raw GCM output may not be sufficient to justify its computational demands. Progress on fidelity of yield projections may benefit more from continuing efforts to understand and minimize systematic error in underlying climate projections. C1 [Glotter, Michael; McInerney, David; Moyer, Elisabeth J.] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. [Elliott, Joshua; Best, Neil; Foster, Ian] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Foster, Ian] Argonne Natl Lab, Lemont, IL 60439 USA. RP Elliott, J (reprint author), Univ Chicago, Computat Inst, Chicago, IL 60637 USA. EM jelliott@ci.uchicago.edu RI McInerney, David/I-4896-2015 OI McInerney, David/0000-0003-4876-8281 FU National Science Foundation (NSF) [SES-0951576]; NSF Graduate Fellowship [DGE-1144082]; NSF Science, Engineering and Education for Sustainability Fellowship [1215910]; NSF [OCI-0821678, OCI-1148443]; Department of Energy (DOE); DOE; NOAA; Environmental Protection Agency; NOAA Climate Prediction Center FX We thank L. Mearns for valuable comments and suggestions during this work and M. Stein and W. Leeds for consultation on the statistical analysis. This research was performed as part of the Center for Robust Decision-Making on Climate and Energy Policy (RDCEP) at the University of Chicago. RDCEP is funded by National Science Foundation (NSF) Grant SES-0951576 through the Decision Making Under Uncertainty program. M.G. acknowledges support of NSF Graduate Fellowship DGE-1144082 and J.E. was supported by NSF Science, Engineering and Education for Sustainability Fellowship 1215910. Data storage was provided by PADS (petascale active data store; NSF Grant OCI-0821678) at Argonne National Laboratory (ANL) and by the University of Chicago Computing Cooperative at the Computation Institute, a joint institute of ANL and the University of Chicago. Some computing was facilitated using the Swift parallel scripting language (supported in part by NSF Grant OCI-1148443). GCM output was made available through the World Climate Research Program CMIP3 archive, made possible by the modeling groups Program for Climate Model Diagnosis and Intercomparison and WCRP's Working Group on Coupled Modeling. This work uses output from the Community Climate System Model (CSSM), supported by the NSF and Department of Energy (DOE), and the Coupled Global Climate Model, from the Canadian Centre for Climate Modelling and Analysis. CCSM data in a geographic information systems (GIS) format was provided by the National Center for Atmospheric Research GIS Initiative. Dynamically downscaled output was provided by the North American Regional Climate Change Assessment Program, funded by the NSF, DOE, NOAA, and Environmental Protection Agency, and precipitation data was funded by the NOAA Climate Prediction Center. NR 54 TC 16 Z9 16 U1 5 U2 30 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 17 PY 2014 VL 111 IS 24 BP 8776 EP 8781 DI 10.1073/pnas.1314787111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9XO UT WOS:000337300100028 PM 24872455 ER PT J AU Kjaergaard, CH Qayyum, MF Wong, SD Xu, F Hemsworth, GR Walton, DJ Young, NA Davies, GJ Walton, PH Johansen, KS Hodgson, KO Hedman, B Solomon, EI AF Kjaergaard, Christian H. Qayyum, Munzarin F. Wong, Shaun D. Xu, Feng Hemsworth, Glyn R. Walton, Daniel J. Young, Nigel A. Davies, Gideon J. Walton, Paul H. Johansen, Katja Salomon Hodgson, Keith O. Hedman, Britt Solomon, Edward I. TI Spectroscopic and computational insight into the activation of O-2 by the mononuclear Cu center in polysaccharide monooxygenases SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE X-ray absorption spectroscopy; DFT; dioxygen activation; biofuels ID DOPAMINE BETA-MONOOXYGENASE; ALPHA-HYDROXYLATING MONOOXYGENASE; CRYSTAL-STRUCTURE; ACTIVE-SITE; END-ON; COPPER; OXYGEN; CELLULOSE; COMPLEX; DIOXYGEN AB Strategies for O-2 activation by copper enzymes were recently expanded to include mononuclear Cu sites, with the discovery of the copper-dependent polysaccharide monooxygenases, also classified as auxiliary-activity enzymes 9-11 (AA9-11). These enzymes are finding considerable use in industrial biofuel production. Crystal structures of polysaccharide monooxygenases have emerged, but experimental studies are yet to determine the solution structure of the Cu site and how this relates to reactivity. From X-ray absorption near edge structure and extended X-ray absorption fine structure spectroscopies, we observed a change from four-coordinate Cu(II) to three-coordinate Cu(I) of the active site in solution, where three protein-derived nitrogen ligands coordinate the Cu in both redox states, and a labile hydroxide ligand is lost upon reduction. The spectroscopic data allowed for density functional theory calculations of an enzyme active site model, where the optimized Cu(I) and (II) structures were consistent with the experimental data. The O-2 reactivity of the Cu(I) site was probed by EPR and stopped-flow absorption spectroscopies, and a rapid one-electron reduction of O-2 and regeneration of the resting Cu(II) enzyme were observed. This reactivity was evaluated computationally, and by calibration to Cu-superoxide model complexes, formation of an end-on Cu-AA9-superoxide species was found to be thermodynamically favored. We discuss how this thermodynamically difficult one-electron reduction of O-2 is enabled by the unique protein structure where two nitrogen ligands from His1 dictate formation of a T-shaped Cu(I) site, which provides an open coordination position for strong O-2 binding with very little reorganization energy. C1 [Kjaergaard, Christian H.; Qayyum, Munzarin F.; Wong, Shaun D.; Hodgson, Keith O.; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Xu, Feng] Novozymes Inc, Davis, CA 95618 USA. [Hemsworth, Glyn R.; Walton, Daniel J.; Davies, Gideon J.; Walton, Paul H.] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England. [Young, Nigel A.] Univ Hull, Dept Chem, Kingston Upon Hull HU6 7RX, Yorks, England. [Johansen, Katja Salomon] Novozymes AS, Bagsvaerd, Denmark. [Hodgson, Keith O.; Hedman, Britt; Solomon, Edward I.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lab, Stanford, CA 94309 USA. RP Solomon, EI (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA. EM edward.solomon@stanford.edu RI Johansen, Katja /J-7939-2016; OI Johansen, Katja /0000-0002-7587-5990; Walton, Paul Howard/0000-0002-1152-1480; Hemsworth, Glyn/0000-0002-8226-1380 FU National Institute of Diabetes and Digestive and Kidney Diseases of the National Institutes of Health [R01DK031450, NIH P41GM103393]; Biotechnology and Biological Sciences Research Council [BB/I014802/1, BB/L000423/1]; John Stauffer Stanford Graduate Fellowship; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Department of Energy Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393] FX Research reported in this publication was supported by the National Institute of Diabetes and Digestive and Kidney Diseases of the National Institutes of Health under Award R01DK031450 (to E.I.S.) and Grant NIH P41GM103393 (to K.O.H.) and by Biotechnology and Biological Sciences Research Council Grants BB/I014802/1 (to G.J.D.) and BB/L000423/1 (to P.H.W.). C.H.K. acknowledges a John Stauffer Stanford Graduate Fellowship. Use of the Stanford Synchrotron Radiation Lightsource (SSRL), Stanford Linear Accelerator Center National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the Department of Energy Office of Biological and Environmental Research, and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393). NR 39 TC 36 Z9 36 U1 12 U2 88 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 17 PY 2014 VL 111 IS 24 BP 8797 EP 8802 DI 10.1073/pnas.1408115111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9XO UT WOS:000337300100032 PM 24889637 ER PT J AU Chung, D Cha, M Guss, AM Westpheling, J AF Chung, Daehwan Cha, Minseok Guss, Adam M. Westpheling, Janet TI Direct conversion of plant biomass to ethanol by engineered Caldicellulosiruptor bescii SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE metabolic engineering; bioenergy and thermophiles ID CLOSTRIDIUM-THERMOCELLUM; THERMOPHILIC BACTERIUM; ADVANCED BIOFUELS; DSM 6725; SWITCHGRASS; DEGRADATION; EXPRESSION; TOLERANCE; CELLULOSE; ENZYMES AB Ethanol is the most widely used renewable transportation biofuel in the United States, with the production of 13.3 billion gallons in 2012 [John UM (2013) Contribution of the Ethanol Industry to the Economy of the United States]. Despite considerable effort to produce fuels from lignocellulosic biomass, chemical pretreatment and the addition of saccharolytic enzymes before microbial bioconversion remain economic barriers to industrial deployment [Lynd LR, et al. (2008) Nat Biotechnol 26(2): 169-172]. We began with the thermophilic, anaerobic, cellulolytic bacterium Caldicellulosiruptor bescii, which efficiently uses unpretreated biomass, and engineered it to produce ethanol. Here we report the direct conversion of switchgrass, a nonfood, renewable feedstock, to ethanol without conventional pretreatment of the biomass. This process was accomplished by deletion of lactate dehydrogenase and heterologous expression of a Clostridium thermocellum bifunctional acetaldehyde/alcohol dehydrogenase. Whereas wild-type C. bescii lacks the ability to make ethanol, 70% of the fermentation products in the engineered strain were ethanol [12.8 mM ethanol directly from 2% (wt/vol) switchgrass, a real-world substrate] with decreased production of acetate by 38% compared with wild-type. Direct conversion of biomass to ethanol represents a new paradigm for consolidated bioprocessing, offering the potential for carbon neutral, cost-effective, sustainable fuel production. C1 [Chung, Daehwan; Cha, Minseok; Westpheling, Janet] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Chung, Daehwan; Cha, Minseok; Guss, Adam M.; Westpheling, Janet] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Guss, Adam M.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Westpheling, J (reprint author), Univ Georgia, Dept Genet, Athens, GA 30602 USA. EM janwest@uga.edu RI Guss, Adam/A-6204-2011 OI Guss, Adam/0000-0001-5823-5329 FU Office of Biological and Environmental Research in the Department of Energy Office of Science FX We thank Jennifer Copeland for outstanding technical assistance; Brian Davison for providing the switchgrass used in this study; Sidney Kushner for expert advice in the execution of the experiments; and Joe Groom and Jenna Young for critical review of the manuscript. The BioEnergy Science Center is a US Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the Department of Energy Office of Science. NR 34 TC 41 Z9 41 U1 3 U2 75 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 17 PY 2014 VL 111 IS 24 BP 8931 EP 8936 DI 10.1073/pnas.1402210111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9XO UT WOS:000337300100055 PM 24889625 ER PT J AU Qu, D Zheng, M Zhang, LG Zhao, HF Xie, ZG Jing, XB Haddad, RE Fan, HY Sun, ZC AF Qu, Dan Zheng, Min Zhang, Ligong Zhao, Haifeng Xie, Zhigang Jing, Xiabin Haddad, Raid E. Fan, Hongyou Sun, Zaicheng TI Formation mechanism and optimization of highly luminescent N-doped graphene quantum dots SO SCIENTIFIC REPORTS LA English DT Article ID VISIBLE-LIGHT PHOTOCATALYSTS; CARBON DOTS; PHOTOVOLTAIC DEVICES; EMERGENT NANOLIGHTS; NITROGEN; NANODOTS; SENSORS AB Photoluminescent graphene quantum dots (GQDs) have received enormous attention because of their unique chemical, electronic and optical properties. Here a series of GQDs were synthesized under hydrothermal processes in order to investigate the formation process and optical properties of N-doped GQDs. Citric acid (CA) was used as a carbon precursor and self-assembled into sheet structure in a basic condition and formed N-free GQD graphite framework through intermolecular dehydrolysis reaction. N-doped GQDs were prepared using a series of N-containing bases such as urea. Detailed structural and property studies demonstrated the formation mechanism of N-doped GQDs for tunable optical emissions. Hydrothermal conditions promote formation of amide between -NH2 and -COOH with the presence of amine in the reaction. The intramoleculur dehydrolysis between neighbour amide and COOH groups led to formation of pyrrolic N in the graphene framework. Further, the pyrrolic N transformed to graphite N under hydrothermal conditions. N-doping results in a great improvement of PL quantum yield (QY) of GQDs. By optimized reaction conditions, the highest PL QY (94%) of N-doped GQDs was obtained using CA as a carbon source and ethylene diamine as a N source. The obtained N-doped GQDs exhibit an excitation-independent blue emission with single exponential lifetime decay. C1 [Qu, Dan; Zheng, Min; Zhang, Ligong; Zhao, Haifeng; Sun, Zaicheng] Changchun Inst Opt Fine Mech & Phys, State Key Lab Luminescence & Applicat, Changchun 130033, Jilin, Peoples R China. [Xie, Zhigang; Jing, Xiabin] Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Jilin, Peoples R China. [Qu, Dan] Univ Chinese Acad Sci, Beijing 100000, Peoples R China. [Haddad, Raid E.; Fan, Hongyou] Univ New Mexico, Ctr Microengn & Mat, Dept Chem & Nucl Engn, Albuquerque, NM 87106 USA. [Fan, Hongyou] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. RP Fan, HY (reprint author), Univ New Mexico, Ctr Microengn & Mat, Dept Chem & Nucl Engn, Albuquerque, NM 87106 USA. EM hfan@sandia.gov; sunzc@ciomp.ac.cn FU Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry; National Natural Science Foundation of China [21201159, 61176016]; "Hundred Talent Program'' of CAS, and Innovation and Entrepreneurship Program of Jilin; Science and technology department of Jilin [20121801]; CIAC start-up fund; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The project was supported by Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry. The financial support from the National Natural Science Foundation of China (No. 21201159, 61176016), Z.S. thanks the support of the ''Hundred Talent Program'' of CAS, and Innovation and Entrepreneurship Program of Jilin. Science and technology department of Jilin (No. 20121801) Z.X. thanks the support of CIAC start-up fund. Sandia is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 34 TC 0 Z9 0 U1 15 U2 151 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 17 PY 2014 VL 4 AR 5294 DI 10.1038/srep05294 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ0LF UT WOS:000337342700001 ER PT J AU Donahue, CM Black, IK Pecnik, SL Savage, TR Scott, BL Daly, SR AF Donahue, Courtney M. Black, Isabella K. Pecnik, Samantha L. Savage, Thomas R. Scott, Brian L. Daly, Scott R. TI Synthesis, characterization and structural comparisons of phosphonium and arsenic dithiocarbamates with alkyl and phenyl substituents SO POLYHEDRON LA English DT Article DE Dithiocarbamates; Arsenic; Phosphonium; Crystal structure; X-ray diffraction; Sulfur ligand ID HALIDE-COMPLEXES; ANTIMONY; LIGANDS; CRYSTAL; BISMUTH; RADII; VAN AB The synthesis and characterization of the new arsenic dithiocarbamate complex As[S2CNPh2](3) and three new phosphonium dithiocarbamates [PPh4][S2CNR2], where R-2 = Et-2, (CH2)(5) and Ph-2, are reported. As[S2CNPh2](3) was prepared by treating AsI3 with three equivalents of NaS2CNPh2 in a 2:1 mixture of H2O and EtOH. The precipitate that formed was recrystallized from hot toluene to yield yellow prisms of As[S2CNPh2](3) suitable for single-crystal X-ray diffraction (XRD). Attempts to prepare the known compound As[S2CN(CH2)(5)](3) using a similar route resulted in a mixture of As[S2CN(CH2)(5)](3) and the mixed iodide species As[S2CN(CH2)(5)](2)I. Single-crystals of both compounds were isolated from concentrated Et2O/CHCl3 solutions and their structures are described here for the first time. [PPh4][S2CNR2] salts were prepared for comparison to arsenic dithiocarbamates by metathesis reactions with PPh4Br and NaS2CNR2 in acetonitrile. All three salts could be obtained in high-purity from MeCN/Et2O solutions and crystal structures of [PPh4][S2CNEt2] and [PPh4][S2CN(CH2)(5)] reveal charge-separated phosphonium cations and dithiocarbamate anions. The five new crystal structures are used to compare dithiocarbamate bond distances and angles in the presence and absence of arsenic. Nuclear magnetic resonance (NMR) spectra, infrared (IR) spectra, microanalyses, and melting points of the compounds are reported. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Donahue, Courtney M.; Black, Isabella K.; Pecnik, Samantha L.; Savage, Thomas R.; Daly, Scott R.] George Washington Univ, Dept Chem, Washington, DC 20052 USA. [Scott, Brian L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Daly, SR (reprint author), George Washington Univ, Dept Chem, 725 21st St NW, Washington, DC 20052 USA. EM srdaly@gwu.edu RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU George Washington University; National Nuclear Security Administration of U.S. Department of Energy [DEAC52-06NA25396] FX Funding for this work was provided by the George Washington University. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy under Contract DEAC52-06NA25396. We would like to thank the Cahill Group at GW, especially Gian Surbella and Andrew Kerr, for their assistance collecting portions of the XRD data. NR 26 TC 2 Z9 2 U1 0 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD JUN 17 PY 2014 VL 75 BP 110 EP 117 DI 10.1016/j.poly.2014.03.003 PG 8 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA AI3QQ UT WOS:000336777400014 ER PT J AU Bourassa, MW Brown, HH Borchelt, DR Vogt, S Miller, LM AF Bourassa, Megan W. Brown, Hilda H. Borchelt, David R. Vogt, Stefan Miller, Lisa M. TI Metal-deficient aggregates and diminished copper found in cells expressing SOD1 mutations that cause ALS SO FRONTIERS IN AGING NEUROSCIENCE LA English DT Article DE amyotrophic lateral sclerosis; superoxide dismutase; X-ray fluorescence microscopy; synchrotron ID AMYOTROPHIC-LATERAL-SCLEROSIS; ZINC SUPEROXIDE-DISMUTASE; ALZHEIMERS-DISEASE; PARKINSONS-DISEASES; ALPHA-SYNUCLEIN; PATHOGENESIS; PROTEIN; VARIANTS; BETA; SUPEROXIDE-DISMUTASE-1 AB Disruptions in metal ion homeostasis have been described in association with amyotrophic lateral sclerosis (ALS) for a number of years but the precise mechanism of involvement is poorly understood. Metal ions are especially important to familial ALS cases caused by mutations in the metalloenzyme copper-zinc superoxide dismutase (SOD1). To investigate the role of metals in aggregation of mutant SOD1, we have examined the localization of metal ions in a cell culture model of overexpression. Chinese hamster ovary cells (CHO-K1) were transfected to overexpress SOD1 fused to yellow fluorescent protein (YEP) to readily identify the transfected cells and the intracellular aggregates that develop in the cells expressing mutant or wild-type (WT) SOD1. The concentration and distribution of iron, copper, and zinc were determined for four SOD1 mutants (A4V, G37R, H80R, and D125H) as well as a WT SOD1 using X-ray fluorescence microscopy (XFM). Results demonstrated that the SOD1 aggregates were metal-deficient within the cells, which is consistent with recent in vitro studies. In addition, all SOD1 mutants showed significantly decreased copper content compared to the WT SOD1 cells, regardless of the mutant's ability to bind copper. These results suggest that SOD1 overexpression creates an unmet demand on the cell for copper. This is particularly true for the SOD1 mutants where copper delivery may also be impaired. Hence, the SOD1 mutants are less stable than WT SOD1 and if copper is limited, aggregate formation of the metal-deficient, mutant SOD1 protein occurs. C1 [Bourassa, Megan W.; Miller, Lisa M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Brown, Hilda H.; Borchelt, David R.] Univ Florida, Dept Neurosci,McKnight Brain Inst, Ctr Translat Res Neurodegenerat Dis, Santa Fe Hlth Care Alzheimers Dis Res Ctr, Gainesville, FL 32610 USA. [Vogt, Stefan] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Miller, Lisa M.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Miller, LM (reprint author), Brookhaven Natl Lab, Photon Sci Directorate, NSLS 2,Bldg 743, Upton, NY 11973 USA. EM lmiller@bnl.gov RI Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013 OI Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513 FU National Institutes of Neurological Disease and Stroke [P01 NSO49134]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-AC02-06CH11357] FX This work was partially supported by a grant from the National Institutes of Neurological Disease and Stroke (P01 NSO49134- Program Project; David R. Borchelt). The NSLS is funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 42 TC 10 Z9 10 U1 6 U2 17 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1663-4365 J9 FRONT AGING NEUROSCI JI Front. Aging Neurosci. PD JUN 16 PY 2014 VL 6 AR 1 DI 10.3389/fnagi.2014.00110 PG 6 WC Geriatrics & Gerontology; Neurosciences SC Geriatrics & Gerontology; Neurosciences & Neurology GA AM0SY UT WOS:000339558300001 ER PT J AU Longo, AF Ingall, ED Diaz, JM Oakes, M King, LE Nenes, A Mihalopoulos, N Violaki, K Avila, A Benitez-Nelson, CR Brandes, J McNulty, I Vine, DJ AF Longo, Amelia F. Ingall, Ellery D. Diaz, Julia M. Oakes, Michelle King, Laura E. Nenes, Athanasios Mihalopoulos, Nikolaos Violaki, Kaliopi Avila, Anna Benitez-Nelson, Claudia R. Brandes, Jay McNulty, Ian Vine, David J. TI P-NEXFS analysis of aerosol phosphorus delivered to the Mediterranean Sea SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID ATMOSPHERIC DEPOSITION; XANES SPECTROSCOPY; IRON SOLUBILITY; NORTH-ATLANTIC; PRODUCTIVITY; SPECIATION; VARIABILITY; PARTICLES; PHOSPHATE; TRANSPORT AB Biological productivity in many ocean regions is controlled by the availability of the nutrient phosphorus. In the Mediterranean Sea, aerosol deposition is a key source of phosphorus and understanding its composition is critical for determining its potential bioavailability. Aerosol phosphorus was investigated in European and North African air masses using phosphorus near-edge X-ray fluorescence spectroscopy (P-NEXFS). These air masses are the main source of aerosol deposition to the Mediterranean Sea. We show that European aerosols are a significant source of soluble phosphorus to the Mediterranean Sea. European aerosols deliver on average 3.5 times more soluble phosphorus than North African aerosols and furthermore are dominated by organic phosphorus compounds. The ultimate source of organic phosphorus does not stem from common primary emission sources. Rather, phosphorus associated with bacteria best explains the presence of organic phosphorus in Mediterranean aerosols. C1 [Longo, Amelia F.; Ingall, Ellery D.; Diaz, Julia M.; Oakes, Michelle; King, Laura E.; Nenes, Athanasios] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Nenes, Athanasios] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Nenes, Athanasios; Mihalopoulos, Nikolaos] Fdn Res & Technol Hellas, Patras, Greece. [Mihalopoulos, Nikolaos; Violaki, Kaliopi] Univ Crete, Dept Chem, Iraklion, Greece. [Avila, Anna] Univ Autonoma Barcelona, CREAF, Bellaterra, Spain. [Benitez-Nelson, Claudia R.] Univ S Carolina, Coll Arts & Sci, Sch Earth Ocean & Environm, Dept Earth & Ocean Sci, Columbia, SC 29208 USA. [Benitez-Nelson, Claudia R.] Univ S Carolina, Marine Sci Program, Sch Earth Ocean & Environm, Coll Arts & Sci, Columbia, SC 29208 USA. [Brandes, Jay] Skidaway Inst Oceanog, Savannah, GA USA. [McNulty, Ian; Vine, David J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Ingall, ED (reprint author), Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. EM ingall@eas.gatech.edu RI Ingall, Ellery/A-5447-2008; Mihalopoulos, Nikolaos/H-5327-2016; OI Avila, Anna/0000-0002-4137-0839; Ingall, Ellery/0000-0003-1954-0317; Mihalopoulos, Nikolaos/0000-0002-1282-0896; Benitez-Nelson, Claudia/0000-0002-1004-5048 FU National Science Foundation [OCE 1060884, OCE 1357375]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; European Union (European Social Fund); Greek national funds through the Operational Program "Education and Lifelong Learning" of the National Strategic Reference Framework Research Funding Program, ARISTEIA FX This material is based upon work supported by the National Science Foundation under grants OCE 1060884 and OCE 1357375, and the data used to produce these results are available upon request to the corresponding author. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under contract DE-AC02-06CH11357. N.M. and K. V. acknowledge support from European Union (European Social Fund) and Greek national funds through the Operational Program "Education and Lifelong Learning" of the National Strategic Reference Framework Research Funding Program, ARISTEIA. We thank John Jansen at Southern Co. and Bill Preston at the EPA for providing source emission samples. Finally, we thank Terry Lathem for the volcanic ash sample. NR 38 TC 4 Z9 4 U1 2 U2 36 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 16 PY 2014 VL 41 IS 11 BP 4043 EP 4049 DI 10.1002/2014GL060555 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AL6YP UT WOS:000339280200048 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Homann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T DeWolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Grebenyuk, A Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Klein, B Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, TD Pol, ME Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E 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CA CMS Collaboration TI Measurement of the t-channel single-top-quark production cross section and of the |V (tb)| CKM matrix element in pp collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Top physics ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; LHC AB Measurements are presented of the t-channel single-top-quark production cross section in proton-proton collisions at root s = 8 TeV. The results are based on a data sample corresponding to an integrated luminosity of 19.7 fb(-1) recorded with the CMS detector at the LHC. The cross section is measured inclusively, as well as separately for top (t) and antitop (t) over bar, in final states with a muon or an electron. The measured inclusive t-channel cross section is sigma(t-ch.) = 83.6 +/- 2.3 (stat.) +/- 7.4 (syst.) pb. The single t and (t) cross sections are measured to be sigma(t-ch.)(t) = 53.8 +/- 1.5 (stat.) +/- 4.4 (syst.) pb and sigma(t-ch.)(t) over bar = 27.6 +/- 1.3 (stat.) +/- 3.7 (syst.) pb, respectively. The measured ratio of cross sections is Rt-ch. = sigma(t-ch.)(t)/sigma(t-ch.)(t) over bar = 1.95 +/- 0.10 (stat.) +/- 0.19 (syst.), in agreement with the standard model prediction. The modulus of the Cabibbo-Kobayashi-Maskawa matrix element V-tb is extracted and, in combination with a previous CMS result at root s = 7 TeV, a value vertical bar V-tb vertical bar = 0.998 +/- 0.038 (exp.) +/- 0.016 (theo.) is obtained. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephysik OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; DeWolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Ochesanu, S.; Roland, B.; Rougny, R.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Daci, N.; Heracleous, N.; Kalogeropoulos, A.; Keaveney, J.; Kim, T. J.; Lowette, S.; Maes, M.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Crucy, S.; Dildick, S.; Fagot, A.; Garcia, G.; Klein, B.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, P.; Komm, M.; Lemaitre, V.; Liao, J.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Garcia, J. M. Vizan] Catholic Univ Louvain, Louvain La Neuve, Belgium. 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[Ata, M.; Caudron, J.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.; Pardos, C. Diez] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. 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A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] ATOMKI, Inst Nucl Res, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Kalsi, A. K.; Kaur, M.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. 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[Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trent, Trento, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Ctr Invest Energet Medioambient & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Contardo, D.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Evangelou, I.; Foudas, C.; Bencze, G.; Giordano, F.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Meola, S.; Paolucci, P.; Palla, F.; Pelliccioni, M.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. 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Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Surat, N.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Ctr Nat Sci, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; St. John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Calderon De la Barca Sanchez, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Yu, I.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Vartak, A.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Eggert, N.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Harris, P.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Gray, J.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. 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G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. 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[Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Roland, C.] Scuola Normale & Sez INFN, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. 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Ferguson, Thomas/O-3444-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Sen, Sercan/C-6473-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Lopez Virto, Amparo/K-9996-2014; Gonzalez Caballero, Isidro/E-7350-2010; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014 OI Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Azzi, Patrizia/0000-0002-3129-828X; Novaes, Sergio/0000-0003-0471-8549; Moon, Chang-Seong/0000-0001-8229-7829; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; 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ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Russ, James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Ferguson, Thomas/0000-0001-5822-3731; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Sen, Sercan/0000-0001-7325-1087; Scodellaro, Luca/0000-0002-4974-8330; Lopez Virto, Amparo/0000-0002-8707-5392; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889 FU Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science; EU; EU-ESF; Greek NSRF; BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIEN-CIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Compagnia di San Paolo (Torino); Thalis programme; Aristeia programme FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIEN-CIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 55 TC 17 Z9 17 U1 8 U2 75 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 16 PY 2014 IS 6 AR 090 DI 10.1007/JHEP06(2014)090 PG 43 WC Physics, Particles & Fields SC Physics GA AK3MU UT WOS:000338329300001 ER PT J AU Marathe, S Shi, XB Wojcik, MJ Kujala, NG Divan, R Mancini, DC Macrander, AT Assoufid, L AF Marathe, Shashidhara Shi, Xianbo Wojcik, Michael J. Kujala, Naresh G. Divan, Ralu Mancini, Derrick C. Macrander, Albert T. Assoufid, Lahsen TI Probing transverse coherence of x-ray beam with 2-D phase grating interferometer SO OPTICS EXPRESS LA English DT Article ID SPATIAL COHERENCE; LIGHT; DIFFRACTION; RADIATION; CONTRAST AB Transverse coherence of the x-ray beam from a bending magnet source was studied along multiple directions using a 2-D pi/2 phase grating by measuring interferogram visibilities at different distances behind the grating. These measurements suggest that the preferred measuring orientation of a 2-D checkerboard grating is along the diagonal directions of the square blocks, where the interferograms have higher visibility and are not sensitive to the deviation of the duty cycle of the grating period. These observations are verified by thorough wavefront propagation simulations. The accuracy of the measured coherence values was also validated by the simulation and analytical results obtained from the source parameters. In addition, capability of the technique in probing spatially resolved local transverse coherence is demonstrated. (C) 2014 Optical Society of America C1 [Marathe, Shashidhara; Shi, Xianbo; Wojcik, Michael J.; Kujala, Naresh G.; Macrander, Albert T.; Assoufid, Lahsen] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. [Divan, Ralu] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. [Mancini, Derrick C.] PSE Argonne Natl Lab, Lemont, IL 60439 USA. RP Marathe, S (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Lemont, IL 60439 USA. EM marathe@aps.anl.gov FU U.S. DOE [DE-AC02-06CH11357] FX Use of the Advanced Photon Source and Center for Nanoscale Materials, Office of Science User Facilities operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. We acknowledge Dr. Han Wen, NHLBI/National Institutes of Health, Bethesda, MD 20892, USA, for many helpful suggestions during the data processing. NR 25 TC 9 Z9 9 U1 1 U2 15 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 16 PY 2014 VL 22 IS 12 BP 14041 EP 14053 DI 10.1364/OE.22.014041 PG 13 WC Optics SC Optics GA AJ9PH UT WOS:000338044300001 PM 24977503 ER PT J AU Guss, GM Sridharan, AK Elhadj, S Johnson, MA Matthews, MJ AF Guss, Gabriel M. Sridharan, Arun K. Elhadj, Selim Johnson, Michael A. Matthews, Manyalibo J. TI Nanoscale surface tracking of laser material processing using phase shifting diffraction interferometry SO OPTICS EXPRESS LA English DT Article ID FUSED-SILICA; RELAXATION; GLASS AB Phase shifting diffraction interferometry (PSDI) was adapted to provide real-time feedback control of a laser-based chemical vapor deposition (LCVD) process with nanometer scale sensitivity. PSDI measurements of laser heated BK7 and fused silica substrates were used to validate a finite element model that accounts for both refractive index changes and displacement contributions to the material response. Utilizing PSDI and accounting for the kinetics of the modeled thermomechanical response, increased control of the LCVD process was obtained. This approach to surface tracking is useful in applications where extreme environments on the working surface require back-side optical probing through the substrate. (C) 2014 Optical Society of America C1 [Guss, Gabriel M.; Elhadj, Selim; Johnson, Michael A.; Matthews, Manyalibo J.] Lawrence Livermore Natl Lab, Livermore, CA 95520 USA. [Sridharan, Arun K.] Gen Elect, John F Welch Technol Ctr, Bangalore 560048, Karnataka, India. RP Matthews, MJ (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 95520 USA. EM ibo@llnl.gov FU UCFR [12-LR-237713]; U.S. Department of Energy [DE-AC52-07NA27344] FX The authors express deep gratitude to R. Negres for her careful reading and input to this manuscript. Enlightening conversations with C. Grigoropoulos, J. Yoo and D. Lee of the UC Berkeley Thermal Lab regarding LCVD are gratefully acknowledged. The authors thank N. Nielsen, J. Hughes and F. Ravizza for technical assistance. S. Elhadj and M. Matthews acknowledge support from UCFR grant # 12-LR-237713. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 21 TC 2 Z9 2 U1 0 U2 13 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUN 16 PY 2014 VL 22 IS 12 BP 14493 EP 14504 DI 10.1364/OE.22.014493 PG 12 WC Optics SC Optics GA AJ9PH UT WOS:000338044300043 PM 24977545 ER PT J AU Bansal, N Koirala, N Brahlek, M Han, MG Zhu, YM Cao, Y Waugh, J Dessau, DS Oh, S AF Bansal, Namrata Koirala, Nikesh Brahlek, Matthew Han, Myung-Geun Zhu, Yimei Cao, Yue Waugh, Justin Dessau, Daniel S. Oh, Seongshik TI Robust topological surface states of Bi2Se3 thin films on amorphous SiO2/Si substrate and a large ambipolar gating effect SO APPLIED PHYSICS LETTERS LA English DT Article ID INSULATORS AB The recent emergence of topological insulators (TI) has spurred intensive efforts to grow TI thin films on various substrates. However, little is known about how robust the topological surface states (TSS) are against disorders and other detrimental effects originating from the substrates. Here, we report the observation of a well-defined TSS on Bi2Se3 films grown on amorphous SiO2 (a-SiO2) substrates and a large gating effect on these films using the underneath doped-Si substrate as the back gate. The films on a-SiO2 were composed of c-axis ordered but random in-plane domains. However, despite the in-plane randomness induced by the amorphous substrate, the transport properties of these films were superior to those of similar films grown on single-crystalline Si(111) substrates, which are structurally better matched but chemically reactive with the films. This work sheds light on the importance of chemical compatibility, compared to lattice matching, for the growth of TI thin films, and also demonstrates that the technologically important and gatable a-SiO2/Si substrate is a promising platform for TI films. (C) 2014 AIP Publishing LLC. C1 [Bansal, Namrata] Rutgers State Univ, Dept Elect & Comp Engn, Piscataway, NJ 08854 USA. [Koirala, Nikesh; Brahlek, Matthew; Oh, Seongshik] Rutgers State Univ, Dept Phys & Astron, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. [Koirala, Nikesh; Brahlek, Matthew; Oh, Seongshik] Rutgers State Univ, Inst Adv Mat Devices & Nanotechnol, Piscataway, NJ 08854 USA. [Han, Myung-Geun; Zhu, Yimei] Brookhaven Natl Lab, Upton, NY 11973 USA. [Cao, Yue; Waugh, Justin; Dessau, Daniel S.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. RP Oh, S (reprint author), Rutgers State Univ, Dept Phys & Astron, Rutgers Ctr Emergent Mat, POB 849, Piscataway, NJ 08854 USA. EM ohsean@physics.rutgers.edu OI Cao, Yue/0000-0002-3989-158X FU National Science Foundation [NSF DMR-0845464, NSF DMR-1007014]; Office of Naval Research [ONR N000141210456]; U.S. Department of Energy, Office of Basic Science, Division of Materials Science and Engineering [DE-AC02-98CH10886]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by National Science Foundation (NSF DMR-0845464) and Office of Naval Research (ONR N000141210456). The electron microscopy work was supported by the U.S. Department of Energy, Office of Basic Science, Division of Materials Science and Engineering, under the Contract No. DE-AC02-98CH10886. STEM sample preparation was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory. The ARPES work was supported by the National Science Foundation (NSF DMR-1007014), with the Advanced Light Source supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 23 TC 11 Z9 11 U1 0 U2 40 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 16 PY 2014 VL 104 IS 24 AR 241606 DI 10.1063/1.4884348 PG 5 WC Physics, Applied SC Physics GA AJ7XQ UT WOS:000337915000019 ER PT J AU Barabash, RI Barabash, OM Karapetrova, EA Manley, ME AF Barabash, R. I. Barabash, O. M. Karapetrova, E. A. Manley, M. E. TI Structural and dynamical fluctuations in off-stoichiometric NiMnGa shape-memory alloys SO APPLIED PHYSICS LETTERS LA English DT Article ID X-RAY-SCATTERING; PHASE-TRANSFORMATION; MOSSBAUER RADIATION; DIFFUSE-SCATTERING; NI2MNGA; TRANSITIONS; DEFECTS; CRYSTAL; DIFFRACTION; DETECTOR AB Measurements and modeling of the 3D diffuse scattering from off-stoichiometric NiMnGa shape memory alloys reveal evidence of structural and dynamical precursors to the phase transition. A model of the diffuse scattering in the high temperature cubic L2(1) phase indicates that at temperatures tens of degrees higher than transition temperature, T-c, the lattice exhibits tetragonally distorted local regions that are clear precursors to the phase transition. The model also accounts for lattice deformation caused by precursor nanoregions of the martensite phase and thermal scattering from phonons and agrees well with the observed diffuse scattering maps in reciprocal space. A distinctive feature of the diffuse scattering is that it is highly anisotropic: Around (H0H) reflections, the diffuse scattering is strongly compressed along the [H0H] and enhanced along the [-H0H] direction. Additionally, localized intensity maxima associated with phasons are observed at temperatures 30-50K above T-c. They clearly demonstrate that each phason corresponds to an individual point in reciprocal space, which is consistent with dynamical phase fluctuations of a well-formed charge density wave resulting from Peierls instability. (C) 2014 AIP Publishing LLC. C1 [Barabash, R. I.; Manley, M. E.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Barabash, O. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Karapetrova, E. A.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Barabash, RI (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RI Manley, Michael/N-4334-2015 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX Research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. The work benefited from the use of the Advanced Photon Source, supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Research by MEM sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. NR 34 TC 2 Z9 2 U1 2 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 16 PY 2014 VL 104 IS 24 AR 241905 DI 10.1063/1.4884062 PG 4 WC Physics, Applied SC Physics GA AJ7XQ UT WOS:000337915000024 ER PT J AU D'Aquila, K Phatak, C Holt, MV Stripe, BD Tong, S Park, WI Hong, S Petford-Long, AK AF D'Aquila, Kenneth Phatak, Charudatta Holt, Martin V. Stripe, Benjamin D. Tong, Sheng Park, Woon Ik Hong, Seungbum Petford-Long, Amanda K. TI Bipolar resistance switching in Pt/CuOx/Pt via local electrochemical reduction SO APPLIED PHYSICS LETTERS LA English DT Article ID MEMORIES; OXYGEN; CHALLENGES; ELECTRODES; SUBOXIDES; FILMS AB The local changes in copper oxidation state and the corresponding resistance changes in Pt/CuOx/Pt nanoscale heterostructures have been investigated using x-ray nanoprobe spectro-microscopy and current-voltage characterization. After gentle electroforming, during which the current-voltage behavior remains non-linear, the low resistance state was reached, and we observed regions of 160 nm width that show an increase in Cu K-alpha fluorescence intensity, indicative of partial reduction of the CuOx. Analysis of the current voltage curves showed that the dominant conduction mechanism is Schottky emission and that the resistance state is correlated with the Schottky barrier height. We propose that the reversible resistivity change in these Pt/CuOx/Pt heterostructures occurs through local electrochemical reduction leading to change of the Schottky barrier height at the interface between Pt and the reduced CuOx layers and to change of the CuOx resistivity within laterally confined portions of the CuOx layer. These experiments reveal important insights into the mechanism of resistance switching of Pt/CuOx/Pt performed in a current and voltage regime that does not create a metallic conduction path. (C) 2014 AIP Publishing LLC. C1 [D'Aquila, Kenneth; Phatak, Charudatta; Park, Woon Ik; Hong, Seungbum; Petford-Long, Amanda K.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [D'Aquila, Kenneth; Petford-Long, Amanda K.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Holt, Martin V.; Stripe, Benjamin D.; Tong, Sheng] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. RP Hong, S (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. EM hong@anl.gov RI Hong, Seungbum/B-7708-2009; Tong, Sheng/A-2129-2011; Petford-Long, Amanda/P-6026-2014; OI Hong, Seungbum/0000-0002-2667-1983; Tong, Sheng/0000-0003-0355-7368; Petford-Long, Amanda/0000-0002-3154-8090; Park, Woon Ik/0000-0002-2577-477X FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX The work was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. We acknowledge use of the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. We acknowledge C. Alvarez, Y. Liu, Y.-Y. Choi, S. Zhang, and A. Roelofs at Argonne National Laboratory for their support in x-ray nanoprobe experiment. NR 30 TC 7 Z9 7 U1 1 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 16 PY 2014 VL 104 IS 24 AR 242902 DI 10.1063/1.4883398 PG 5 WC Physics, Applied SC Physics GA AJ7XQ UT WOS:000337915000066 ER PT J AU Simakov, EI Arsenyev, SA Haynes, WB Shchegolkov, DY Suvorova, NA Tajima, T Boulware, CH Grimm, TL AF Simakov, Evgenya I. Arsenyev, Sergey A. Haynes, W. Brian Shchegolkov, Dmitry Yu Suvorova, Natalya A. Tajima, Tsuyoshi Boulware, Chase H. Grimm, Terry L. TI Raising gradient limitations in 2.1 GHz superconducting photonic band gap accelerator cavities SO APPLIED PHYSICS LETTERS LA English DT Article ID LINACS AB We report results from recent 2.1 GHz superconducting radio frequency (SRF) photonic band gap (PBG) resonator experiments at Los Alamos. Two 2.1 GHz PBG cells with elliptical rods were fabricated and tested at high power in a liquid helium bath at the temperatures of 4K and below 2K. The described SRF PBG cells were designed with a particular emphasis on changing the shape of the PBG rods to reduce peak surface magnetic fields and at the same time to preserve its effectiveness at damping higher-order-modes. The superconducting PBG cavities have great potential for damping long-range wakefields in SRF accelerator structures without affecting the fundamental accelerating mode. The cells performed in accordance with simulation's predictions and the maximum achieved accelerating gradient was 18.3 MV/m. This represents a 30% increase over gradients previously demonstrated in superconducting PBG cavities with round rods. (C) 2014 AIP Publishing LLC. C1 [Simakov, Evgenya I.; Arsenyev, Sergey A.; Haynes, W. Brian; Shchegolkov, Dmitry Yu; Suvorova, Natalya A.; Tajima, Tsuyoshi] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Boulware, Chase H.; Grimm, Terry L.] Niowave Inc, Lansing, MI 48906 USA. RP Simakov, EI (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM smirnova@lanl.gov OI Boulware, Chase/0000-0002-8648-336X; Shchegolkov, Dmitry/0000-0002-0721-3397; Simakov, Evgenya/0000-0002-7483-1152 FU U.S. Department of Energy (DOE) Office of Science Early Career Research Program; Department of Defense High Energy Laser Joint Technology Office through the Office of Naval Research FX Work was supported in part by the Department of Defense High Energy Laser Joint Technology Office through the Office of Naval Research and by the U.S. Department of Energy (DOE) Office of Science Early Career Research Program. The authors gratefully acknowledge discussions with Frank L. Krawczyk, Sergey S. Kurennoy, James F. O'Hara, and Eric F. Olivas, and technical help of David Lizon. NR 21 TC 3 Z9 3 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 16 PY 2014 VL 104 IS 24 AR 242603 DI 10.1063/1.4884428 PG 4 WC Physics, Applied SC Physics GA AJ7XQ UT WOS:000337915000063 ER PT J AU Zhernenkov, M Gill, S Stanic, V DiMasi, E Kisslinger, K Baldwin, JK Misra, A Demkowicz, MJ Ecker, L AF Zhernenkov, Mikhail Gill, Simerjeet Stanic, Vesna DiMasi, Elaine Kisslinger, Kim Baldwin, J. Kevin Misra, Amit Demkowicz, M. J. Ecker, Lynne TI Design of radiation resistant metallic multilayers for advanced nuclear systems SO APPLIED PHYSICS LETTERS LA English DT Article ID GRAIN-BOUNDARIES; BUBBLE FORMATION; HELIUM; IRRADIATION; COPPER; INTERFACES; HE AB Helium implantation from transmutation reactions is a major cause of embrittlement and dimensional instability of structural components in nuclear energy systems. Development of novel materials with improved radiation resistance, which is of the utmost importance for progress in nuclear energy, requires guidelines to arrive at favorable parameters more efficiently. Here, we present a methodology that can be used for the design of radiation tolerant materials. We used synchrotron X-ray reflectivity to nondestructively study radiation effects at buried interfaces and measure swelling induced by He implantation in Cu/Nb multilayers. The results, supported by transmission electron microscopy, show a direct correlation between reduced swelling in nanoscale multilayers and increased interface area per unit volume, consistent with helium storage in Cu/Nb interfaces in forms that minimize dimensional changes. In addition, for Cu/Nb layers, a linear relationship is demonstrated between the measured depth-dependent swelling and implanted He density from simulations, making the reflectivity technique a powerful tool for heuristic material design. (C) 2014 AIP Publishing LLC. C1 [Zhernenkov, Mikhail; Gill, Simerjeet; Stanic, Vesna; DiMasi, Elaine; Kisslinger, Kim; Ecker, Lynne] Brookhaven Natl Lab, Upton, NY 11973 USA. [Baldwin, J. Kevin; Misra, Amit] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Demkowicz, M. J.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Zhernenkov, M (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM zherne@bnl.gov; gills@bnl.gov RI Kisslinger, Kim/F-4485-2014; stanic, vesna/J-9013-2012; Misra, Amit/H-1087-2012; OI stanic, vesna/0000-0003-0318-9454; Zhernenkov, Mikhail/0000-0003-3604-0672 FU U.S. D.O.E. [DE-AC02-98CH10886]; DOE, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center program [2008LANL1026] FX The National Synchrotron Light Source and the Center for Functional Nanomaterials at Brookhaven National Laboratory are supported under U.S. D.O.E. Grant No. DE-AC02-98CH10886. LANL acknowledges support from DOE, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center program Award No. 2008LANL1026. We would like to thank Dr. Y. Q. Wang for He ion implantation at the Ion Beam Materials Laboratory at Los Alamos National Laboratory. NR 27 TC 10 Z9 10 U1 6 U2 71 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 16 PY 2014 VL 104 IS 24 AR 241906 DI 10.1063/1.4883481 PG 4 WC Physics, Applied SC Physics GA AJ7XQ UT WOS:000337915000025 ER PT J AU Lin, QS Miller, GJ Corbettt, JD AF Lin, Qisheng Miller, Gordon J. Corbettt, John D. TI Ordered BaAl4-Type Variants in the BaAuxSn4-x System: A Unified View on Their Phase Stabilities versus Valence Electron Counts SO INORGANIC CHEMISTRY LA English DT Article ID INTERMETALLICS; EXAMPLES; SOLIDS; AU AB Three ordered structures of the tetragonal BaAl4 type were identified in the Ba-Au-Sn system, from which a unified view of the interplay between the valence electron counts (VECs) and phase stabilities of these three types of derivatives can be developed. The BaNiSn3 (I4mm), ThCr2Si2 (I4/mmm), and CaBe2Ge2 (P4/nmm) type BaAuxSn4-x, phases occurred respectively at x = 0.78(1)-1, 1.38(1)-1.47(1), and 1.52(1)-2.17(1), consistent with theoretical atomic "coloring" analyses that reveal an optimal VEC of similar to 14 for the ThCr2Si2 type but larger and smaller values respectively for the BaNiSn3- and CaBe2Ge2-type structures. C1 [Lin, Qisheng] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Lin, QS (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM qslin@ameslab.gov FU Office of the Basic Energy Sciences, Materials Sciences Division, U.S. Department of Energy (DOE); DOE [DE-AC02-07CH11358] FX The research was supported by the Office of the Basic Energy Sciences, Materials Sciences Division, U.S. Department of Energy (DOE). Ames Laboratory is operated for DOE by Iowa State University under Contract DE-AC02-07CH11358. NR 22 TC 4 Z9 4 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 16 PY 2014 VL 53 IS 12 BP 5875 EP 5877 DI 10.1021/ic402991d PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AJ3HT UT WOS:000337557800001 PM 24870951 ER EF