FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Wang, LJ Deng, HX Furukawa, H Gandara, F Cordova, KE Peri, D Yaghi, OM AF Wang, Lisa J. Deng, Hexiang Furukawa, Hiroyasu Gandara, Felipe Cordova, Kyle E. Peri, Dani Yaghi, Omar M. TI Synthesis and Characterization of Metal-Organic Framework-74 Containing 2, 4, 6, 8, and 10 Different Metals SO INORGANIC CHEMISTRY LA English DT Article ID ADSORPTION BEHAVIOR; HYDROGEN ADSORPTION; FUNCTIONAL-GROUPS; SITES; BINDING; LIGAND; MOF-5 AB Metal-organic frameworks (MOFs) containing more than two kinds of metal ions mixed in one secondary building unit are rare because the synthesis often yields mixed MOF phases rather than a pure phase of a mixed-metal MOF (MM-MOF). In this study, we use a one-pot reaction to make microcrystalline MOF-74 [M,(DOT); DOT =: dioxidoterephthalate] with 2 (Mg and Co), 4 (Mg, Co, Ni, and Zn), 6 (Mg, Sr, Mn, Co, Ni, and Zn), 8 (Mg, Ca, Sr, Mn, Fe, Co, Ni, and Zn), and 10 (Mg, Ca, Sr, Ba, Mn, Fe, Co, Ni, Zn, and Cd) different kinds of divalent metals. The powder X-ray diffraction patterns of MM-MOF-74 were identical with those of single-metal MOF-74, and no amorphous phases were found by scanning electron microscopy. The successful preparation of guest-free MM-MOF-74 samples was confirmed by N2 adsorption measurements. Elemental analysis data also support the fact that all metal ions used in the MOF synthesis are incorporated within the same MOF-74 structure. Energy-dispersive X-ray spectroscopies indicate that metal ions are heterogeneously distributed within each of the crystalline particles. This approach is also employed to incorporate metal ions (i.e., Ca, Sr, Ba, and Cd) from which the parent MOF structure could not be made as a single-metal-containing MOF. C1 [Wang, Lisa J.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Deng, Hexiang; Furukawa, Hiroyasu; Gandara, Felipe; Cordova, Kyle E.; Peri, Dani; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Div Mat Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Deng, Hexiang; Furukawa, Hiroyasu; Gandara, Felipe; Cordova, Kyle E.; Peri, Dani; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Div Mat Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI Gandara, Felipe/B-9198-2013; Cordova, Kyle/I-2556-2014; EFRC, CGS/I-6680-2012; Stangl, Kristin/D-1502-2015; Furukawa, Hiroyasu/C-5910-2008; OI Gandara, Felipe/0000-0002-1671-6260; Cordova, Kyle/0000-0002-4988-0497; Furukawa, Hiroyasu/0000-0002-6082-1738; Yaghi, Omar/0000-0002-5611-3325 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Defense Threat Reduction Agency [HDTRA1-12-1-0053]; U.S. Army Research Office [BB11PHM120] FX This work was partially supported for synthesis by BASF SE (Ludwigshafen, Germany), for general characterization by U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (Grant DE-SC0001015), and for the adsorption measurements by Defense Threat Reduction Agency (Grant HDTRA1-12-1-0053) and U.S. Army Research Office (Grant BB11PHM120). Prof. Walter G. Klemperer (University of Illinois) is gratefully acknowledged for his input and advice on this project. We also thank Dr. Carolyn B. Knobler (UCLA) for valuable discussion and the UCLA Laboratory of Molecular & Nano Archaeology facility. NR 28 TC 60 Z9 60 U1 40 U2 365 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 16 PY 2014 VL 53 IS 12 BP 5881 EP 5883 DI 10.1021/ic500434a PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AJ3HT UT WOS:000337557800003 PM 24878113 ER PT J AU Jensen, MP Chiarizia, R Shkrob, IA Ulicki, JS Spindler, BD Murphy, DJ Hossain, M Roca-Sabio, A Platas-Iglesias, C de Blas, A Rodriguez-Blas, T AF Jensen, Mark P. Chiarizia, Renato Shkrob, Ilya A. Ulicki, Joseph S. Spindler, Brian D. Murphy, Daniel J. Hossain, Mahmun Roca-Sabio, Adrian Platas-Iglesias, Carlos de Blas, Andres Rodriguez-Blas, Teresa TI Aqueous Complexes for Efficient Size-based Separation of Americium from Curium SO INORGANIC CHEMISTRY LA English DT Article ID SEGMENTED CONTRACTION SCHEME; PSEUDOPOTENTIAL BASIS-SETS; RARE-EARTH-ELEMENTS; MACROCYCLE INTERACTION; CROWN-ETHERS; KINETIC-DATA; LANTHANIDE(III)/ACTINIDE(III) DIFFERENTIATION; ACTINIDE CONTRACTION; ELECTRON-DENSITY; ION-EXCHANGE AB Complexation of the adjacent actinide ions americium(III) and curium(III) by the ligand N,N'-bis[(6-carboxy-2-pyridyl)methyl]-1,10-diaza-18-crown-6 (H(2)bp18c6) in aqueous solution was studied to quantify and characterize its americium/curium selectivity. Liquid-liquid extraction and spectrophotometric titration indicated the presence of both fully deprotonated and monoprotonated complexes, An(bp18c6)(+) and An(Hbp18c6)(2+) (An = Am or Cm), at the acidities that would be encountered when treating nuclear wastes. The stability constants of the complexes in 1 M NaNO3 determined using competitive complexation were log beta(101) = 15.49 +/- 0.06 for Am and 14.88 +/- 0.03 for Cm, indicating a reversal of the usual order of complex stability, where ligands bind the smaller Cm-III ion more tightly than Am-III. The Am/Cm selectivity of bp18c6(2-) that is defined by the ratio of the Am and Cm stability constants (beta(101) Am/beta(101) Cm = 4.1) is the largest reported so far for binary An(III)-ligand complexes. Theoretical density functional theory calculations using the B3LYP functional suggest that the ligand's size-selectivity for larger 4f- and 5f-element cations arises from steric constraints in the crown ether ring. Enhanced 5f character in molecular orbitals involving actinide nitrogen interactions is predicted to favor actinide(III) complexation by bp18c6(2-) over the complexation of similarly sized lanthanide(III) cations. C1 [Jensen, Mark P.; Chiarizia, Renato; Shkrob, Ilya A.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Ulicki, Joseph S.; Spindler, Brian D.; Murphy, Daniel J.; Hossain, Mahmun] Univ Wisconsin, Dept Chem & Biochem, Milwaukee, WI 53201 USA. [Roca-Sabio, Adrian; Platas-Iglesias, Carlos; de Blas, Andres; Rodriguez-Blas, Teresa] Univ A Coruna, Dept Quim Fundamental, La Coruna 15008, Spain. RP Jensen, MP (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mjensen@anl.gov; mayter@udc.es RI de Blas Varela, Andres/F-9632-2010; Rodriguez-Blas, Teresa/M-6100-2014; Platas-Iglesias, Carlos/L-4592-2013; Jensen, Mark/G-9131-2012 OI de Blas Varela, Andres/0000-0001-8548-9658; Rodriguez-Blas, Teresa/0000-0001-5078-1093; Platas-Iglesias, Carlos/0000-0002-6989-9654; Jensen, Mark/0000-0003-4494-6693 FU Argonne [DE-AC02-06CH11357]; U.S. Department of Energy, Assistant Secretary of the Office of Nuclear Energy, Fuel Cycle Research and Development Program; Xunta de Galicia [CN 2012/011] FX Work at Argonne (contract number DE-AC02-06CH11357) and UWM was supported by the U.S. Department of Energy, Assistant Secretary of the Office of Nuclear Energy, Fuel Cycle Research and Development Program. A.R.-S., A.d.B., C.P.-I., and T.R.-B. thank Xunta de Galicia (CN 2012/011) for generous financial support and Centro de Supercomputacion de Galicia (CESGA) for providing the computer facilities. NR 81 TC 12 Z9 12 U1 6 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 16 PY 2014 VL 53 IS 12 BP 6003 EP 6012 DI 10.1021/ic500244p PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AJ3HT UT WOS:000337557800020 PM 24890863 ER PT J AU Zhou, SX Mishra, T Wang, M Shatruk, M Cao, HB Latturner, SE AF Zhou, Sixuan Mishra, Trinath Wang, Man Shatruk, Michael Cao, Huibo Latturner, Susan E. TI Synthesis, Crystal Structure, and Magnetic Properties of Novel Intermetallic Compounds R2Co2SiC (R = Pr, Nd) SO INORGANIC CHEMISTRY LA English DT Article ID TRANSITION-METAL DIMERS; ELECTRONIC-STRUCTURE; FLUX; DIFFRACTION; INSULATORS; PHASES; ENERGY; CARBON AB The intermetallic compounds R2Co2SiC (R = Pr, Nd) were prepared from the reaction of silicon and carbon in either Pr/Co or Nd/Co eutectic flux. These phases crystallize with a new stuffed variant of the W2CoB2 structure type in orthorhombic space group minim with unit cell parameters a = 3.978(4) angstrom, b = 6.094(5) angstrom, c = 8.903(8) angstrom (z = 2; R-1 = 0.0302) for Nd2Co2SiC. Silicon, cobalt, and carbon atoms form two-dimensional flat sheets, which are separated by puckered layers of rare-earth cations. Magnetic susceptibility measurements indicate that the rare earth cations in both analogues order ferromagnetically at low temperature (T-C approximate to 12 K for Nd2Co2SiC and T-C approximate to 20 K for Pr2Co2SiC). Single-crystal neutron diffraction data for Nd2Co2SiC indicate that Nd moments initially align ferromagnetically along the c axis around similar to 12 K, but below 11 K, they tilt slightly away from the c axis, in the ac plane. Electronic structure calculations confirm the lack of spin polarization for Co 3d moments. C1 [Zhou, Sixuan; Mishra, Trinath; Wang, Man; Shatruk, Michael; Latturner, Susan E.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Cao, Huibo] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Latturner, SE (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. EM latturner@chem.fsu.edu RI Cao, Huibo/A-6835-2016 OI Cao, Huibo/0000-0002-5970-4980 FU National Science Foundation (Division of Materials Research) [DMR-11-06150, DMR-09-55353]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This research was supported by funding from the National Science Foundation (Division of Materials Research) through Grant No. DMR-11-06150 to S.E.L. and partially through Grant No. DMR-09-55353 to M.S. This work made use of the SEM Facilities of the FSU Physics Department. The research at ORNL High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 36 TC 4 Z9 4 U1 1 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 16 PY 2014 VL 53 IS 12 BP 6141 EP 6148 DI 10.1021/ic5005984 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AJ3HT UT WOS:000337557800036 PM 24898034 ER PT J AU Kalaji, A Skanthakumar, S Kanatzidis, MG Mitchell, JF Soderholm, L AF Kalaji, Ali Skanthakumar, S. Kanatzidis, Mercouri G. Mitchell, John F. Soderholm, L. TI Changing Hafnium Speciation in Aqueous Sulfate Solutions: A High-Energy X-ray Scattering Study SO INORGANIC CHEMISTRY LA English DT Article ID BASIC ZIRCONIUM SULFATE; SOL-GEL TRANSITION; CRYSTAL-STRUCTURE; CHLORIDE COMPLEXES; SULFURIC-ACID; HEXANUCLEAR; CHEMISTRY; CLUSTERS; HYDROLYSIS; RAMAN AB The relationship of solution speciation and the structures of corresponding precipitates is examined for an aqueous Hf4+ . sulfate series. High-energy X-ray scattering (HEXS) and Raman spectroscopy data are used to probe atomic correlations in solutions. Hf4+ in acidic perchlorate solution shows no evidence of a mononuclear metal species but instead has a peak in the pair-distribution function (PDF), generated from the HEXS data, at 3.55 angstrom, indicating Hf4+- Hf4+ solution correlations. The peak intensity is consistent with clusters that are, on average, larger than the tetramic unit [M-4(OH)(8)(H2O)(16)](8+) usually attributed to Zr4+ and Hf4+ solution speciation under these conditions. Addition of sulfate results in a breakup of hydroxo-bridged oligomers into sulfate-capped dimers and, for higher concentrations, Hf-sulfate monomers. The bidentate coordination mode of sulfate dominates the dissolved precursors, although it is not found in the structure of the final crystallized product, which instead is comprised of bridging-bidentate sulfate ligation. Neither the PDF patterns nor the Raman spectra show any evidence of the larger oligomers, such as the octadecameric metal clusters, found in similar Zr4+ solutions. The oligomeric units found in solution provide insights into possible assembly routes for crystallization. In addition to expanding our understanding of synthesis science this study also reveals differences in the aqueous chemistries between Hf and Zr, two elements with ostensibly very similar chemical behavior. C1 [Kalaji, Ali; Skanthakumar, S.; Soderholm, L.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Kanatzidis, Mercouri G.; Mitchell, John F.] Argonne Natl Lab, Div Sci Mat, Argonne, IL 60439 USA. RP Soderholm, L (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. EM LS@anl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. DOE, OBES, Materials Sciences [DE-AC02-06CH11357] FX This work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract DE-AC02-06CH11357. The Advanced Photon Source, used to obtain the HEXS data described in this study, is supported by the U.S. DOE, OBES, Materials Sciences under the same contract number. NR 63 TC 10 Z9 10 U1 1 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 16 PY 2014 VL 53 IS 12 BP 6321 EP 6328 DI 10.1021/ic500938k PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA AJ3HT UT WOS:000337557800054 PM 24871556 ER PT J AU Gong, DY Wang, WS Qian, Y Bai, WB Guo, YX Mao, R AF Gong, Dao-Yi Wang, Wenshan Qian, Yun Bai, Wenbing Guo, Yuanxi Mao, Rui TI Observed holiday aerosol reduction and temperature cooling over East Asia SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE Chinese New Year; temperature cooling; PM10 ID ANTHROPOGENIC HEAT RELEASE; AIR-QUALITY; AMBIENT AIR; ATMOSPHERIC-POLLUTION; URBAN AGGLOMERATIONS; REGIONAL CLIMATE; DIWALI FESTIVAL; FIREWORK EVENTS; SULFUR-DIOXIDE; LUCKNOW CITY AB The air pollution in Chinese Spring Festival (CSF) period over eastern China was investigated using the long-term observations from 2001 to 2012 over 323 stations. The dominant feature of the pollutants around the CSF holidays is the significant reduction of concentration. During the 10day period around the CSF (but excluding the Lunar New Year's Day, LNYD), PM10 experiences a reduction of -9.24%. In association with the aerosol reduction, temperature significantly drops over eastern China. From the third day before the LNYD to the second day after, the daily mean temperature anomaly is -0.81 degrees C, and for no-rain days the anomaly is -0.85 degrees C. The simultaneous anomalies of the daily maximum and minimum temperatures are -0.79 degrees C and -0.82 degrees C, respectively. From the third day to seventh day after the LNYD, the significant negative temperature anomalies move out of China, extending to a broad area from the South China Sea to the western North Pacific. Between the 8th and the 12th days, the significant temperature anomalies can still be found over 140 degrees E-160 degrees E and 15 degrees N-25 degrees N. The reduced downward longwave flux might play an important role in holiday cooling. The possible atmospheric feedback is discernable. The thermal and circulation configuration accompanying the cooling favors baroclinic interaction between upper and lower troposphere for the midlatitude cyclone. The anomalous cyclone becomes mature during the third to the seventh day after the LNYD and disappears 12 days later. The anomalous northern winds in association with the cyclone decrease the temperature and also help disperse the holiday aerosols over eastern China. C1 [Gong, Dao-Yi; Guo, Yuanxi; Mao, Rui] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Wang, Wenshan] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA USA. [Qian, Yun] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bai, Wenbing] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. RP Gong, DY (reprint author), Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. EM gdy@bnu.edu.cn RI qian, yun/E-1845-2011; mao, rui/C-3499-2013 FU US Department of Energy's Office of Science as part of the Regional and Global Climate Modeling Program; DOE [DE-AC05-76RL01830]; [NSFC-41321001]; [NSFC-40975043]; [2012CB955302] FX This research was supported by projects NSFC-41321001 and NSFC-40975043. D.Y. Gong was supported by 2012CB955302. The contribution of Yun Qian in this study is supported by the US Department of Energy's Office of Science as part of the Regional and Global Climate Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. ERA-Interim reanalysis data used in this study were obtained from ECMWF at http://www.ecmwf.int/. NR 62 TC 5 Z9 5 U1 3 U2 31 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 16 PY 2014 VL 119 IS 11 BP 6306 EP 6324 DI 10.1002/2014JD021464 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ8RK UT WOS:000337974500003 ER PT J AU Huang, N Gu, LH Niu, Z AF Huang, Ni Gu, Lianhong Niu, Zheng TI Estimating soil respiration using spatial data products: A case study in a deciduous broadleaf forest in the Midwest USA SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE Soil respiration; Vegetation index; Land surface temperature; root-zone soil moisture; MODIS; Temperate deciduous forest ID LAND-SURFACE TEMPERATURE; GROSS PRIMARY PRODUCTION; MODIS LST DATA; ECOSYSTEM RESPIRATION; ENVIRONMENTAL CONTROLS; VEGETATION INDEXES; AIR TEMPERATURES; ALBEDO PRODUCTS; WATER-CONTENT; DAILY MAXIMUM AB This study aimed to investigate the potential of spatially distributed data products in estimating soil respiration (Rs), including land surface temperature (LST) and spectral vegetation index from the Moderate Resolution Imaging Spectroradiometer (MODIS) and root zone soil moisture derived from the assimilation of the NASA Advanced Microwave Scanning Radiometer-EOS and a land surface model, at a deciduous broadleaf forest site in the Midwest USA. Several statistical models were used to examine the dependencies of Rs on these spatial data products, and accuracy of these models was compared to the models based on in situ measurements. The models based on mean LST (i.e., averaging nighttime and daytime LST from MODIS) and root zone soil moisture explained 82% and 72% of seasonal variations in Rs for spring and winter dormant periods, respectively. In the growing season, the models depending on mean LST, root zone soil moisture, and photosynthesis-related enhanced vegetation index showed comparable accuracy with the models entirely based on in situ measured data, except for the midgrowing period. Drought stress led to a relatively low explanation capacity for the Rs model based on spatial data products during the midgrowing period. However, this model still explained 76% of temporal dynamics of Rs over the midgrowing period. Our results suggested that simple models based entirely on spatial data products have the potential to estimate Rs at the temperate deciduous forest site. The conclusions drawn from the present study provided valuable information for large-scale estimates of Rs in temperate deciduous forest ecosystems. C1 [Huang, Ni; Niu, Zheng] Chinese Acad Sci, Inst Remote Sensing & Digital Earth, State Key Lab Remote Sensing Sci, Beijing, Peoples R China. [Gu, Lianhong] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Huang, N (reprint author), Chinese Acad Sci, Inst Remote Sensing & Digital Earth, State Key Lab Remote Sensing Sci, Beijing, Peoples R China. EM huangni@radi.ac.cn RI Gu, Lianhong/H-8241-2014 OI Gu, Lianhong/0000-0001-5756-8738 FU National Natural Science Foundation of China [41301498]; Special Foundation for Young Scientists of the State Laboratory of Remote Sensing Science [13RC-07]; Major State Basic Research Development Program of China [2013CB733405] FX We sincerely thank the anonymous reviewers for their important and constructive revision advices on the manuscript. We like to offer thanks to the America Fluxnet (http://public.ornl.gov/ameriflux/) which provides the data for our analysis. We also thank B. Yang from Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee, USA, for useful suggestions about the use of soil CO2 flux data, and J.D. Bolten from Hydrological Sciences Branch, NASA Goddard Space Flight Center, Beltsville, MD, for helpful explanation about the root zone soil moisture product. This work was supported by the National Natural Science Foundation of China (41301498), the Special Foundation for Young Scientists of the State Laboratory of Remote Sensing Science (13RC-07), and the Major State Basic Research Development Program of China (2013CB733405). NR 86 TC 4 Z9 5 U1 3 U2 39 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 16 PY 2014 VL 119 IS 11 BP 6393 EP 6408 DI 10.1002/2013JD020515 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ8RK UT WOS:000337974500008 ER PT J AU Navarro, JCA Smolander, S Struthers, H Zorita, E Ekman, AML Kaplan, JO Guenther, A Arneth, A Riipinen, I AF Navarro, J. C. Acosta Smolander, S. Struthers, H. Zorita, E. Ekman, A. M. L. Kaplan, J. O. Guenther, A. Arneth, A. Riipinen, I. TI Global emissions of terpenoid VOCs from terrestrial vegetation in the last millennium SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE VOC emissions; land cover; isoprene; monoterpene; sesquiterpene ID ORGANIC-COMPOUND EMISSIONS; ISOPRENE EMISSION; EARTH SYSTEM; LAND-USE; MONOTERPENE EMISSIONS; CO2 CONCENTRATION; ATMOSPHERIC CO2; CARBON-CYCLE; CLIMATE; AEROSOL AB We investigated the millennial variability (1000 A.D.-2000 A.D.) of global biogenic volatile organic compound (BVOC) emissions by using two independent numerical models: The Model of Emissions of Gases and Aerosols from Nature (MEGAN), for isoprene, monoterpene, and sesquiterpene, and Lund-Potsdam-Jena-General Ecosystem Simulator (LPJ-GUESS), for isoprene and monoterpenes. We found the millennial trends of global isoprene emissions to be mostly affected by land cover and atmospheric carbon dioxide changes, whereas monoterpene and sesquiterpene emission trends were dominated by temperature change. Isoprene emissions declined substantially in regions with large and rapid land cover change. In addition, isoprene emission sensitivity to drought proved to have significant short-term global effects. By the end of the past millennium MEGAN isoprene emissions were 634 TgC yr-1 (13% and 19% less than during 1750-1850 and 1000-1200, respectively), and LPJ-GUESS emissions were 323 TgC yr-1(15% and 20% less than during 1750-1850 and 1000-1200, respectively). Monoterpene emissions were 89 TgC yr-1(10% and 6% higher than during 1750-1850 and 1000-1200, respectively) in MEGAN, and 24 TgC yr-1 (2% higher and 5% less than during 1750-1850 and 1000-1200, respectively) in LPJ-GUESS. MEGAN sesquiterpene emissions were 36 TgC yr-1(10% and 4% higher than during 1750-1850 and 1000-1200, respectively). Although both models capture similar emission trends, the magnitude of the emissions are different. This highlights the importance of building better constraints on VOC emissions from terrestrial vegetation. C1 [Navarro, J. C. Acosta; Riipinen, I.] Stockholm Univ, Dept Appl Environm Sci, S-10691 Stockholm, Sweden. [Navarro, J. C. Acosta; Ekman, A. M. L.; Riipinen, I.] Stockholm Univ, Bolin Ctr Climate Res, S-10691 Stockholm, Sweden. [Smolander, S.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Struthers, H.] Linkoping Univ, NSC, Linkoping, Sweden. [Zorita, E.] Inst Coastal Res, Geesthacht, Germany. [Ekman, A. M. L.] Stockholm Univ, Dept Meteorol, S-10691 Stockholm, Sweden. [Kaplan, J. O.] Ecole Polytech Fed Lausanne, Inst Environm Engn, Lausanne, Switzerland. [Guenther, A.] PNNL, Atmospher Sci & Global Change Div, Richland, WA USA. [Arneth, A.] Karlsruhe Inst Technol, Inst Meteorol & Climate Res, Garmisch Partenkirchen, Germany. RP Navarro, JCA (reprint author), Stockholm Univ, Dept Appl Environm Sci, S-10691 Stockholm, Sweden. EM Juan-Camilo.acosta@itm.su.se RI Riipinen, Ilona/I-9379-2012; Guenther, Alex/B-1617-2008; Acosta Navarro, Juan Camilo/J-8307-2015; Kaplan, Jed/P-1796-2015; OI Guenther, Alex/0000-0001-6283-8288; Acosta Navarro, Juan Camilo/0000-0001-5375-0639; Kaplan, Jed/0000-0001-9919-7613; Smolander, Sampo/0000-0003-4538-6384 FU European Research Council Starting grant ATMOGAIN [ERC-StG-278277]; Swedish Research Council [2011-5120]; Academy of Finland [132100] FX The European Research Council Starting grant ATMOGAIN (ERC-StG-278277), Swedish Research Council (grant 2011-5120), and the Academy of Finland (grant 132100) are gratefully acknowledged for financial support. We also acknowledge CSC IT Center for Science Ltd. for the allocation of computational resources. All the data used or produced in this study are available upon request by contacting the correspondence author. NR 62 TC 14 Z9 14 U1 8 U2 61 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUN 16 PY 2014 VL 119 IS 11 BP 6867 EP 6885 DI 10.1002/2013JD021238 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ8RK UT WOS:000337974500038 ER PT J AU Alioli, S Bauer, CW Berggren, C Tackmann, FJ Walsh, JR Zuberi, S AF Alioli, Simone Bauer, Christian W. Berggren, Calvin Tackmann, Frank J. Walsh, Jonathan R. Zuberi, Saba TI Matching fully differential NNLO calculations and parton showers SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Monte Carlo Simulations; NLO Computations ID TO-LEADING ORDER AB We present a general method to match fully differential next-to-next-to-leading-order (NNLO) calculations to parton shower programs. We discuss in detail the perturbative accuracy criteria a complete NNLO + PS matching has to satisfy. Our method is based on consistently improving a given NNLO calculation with the leading-logarithmic (LL) resummation in a chosen jet resolution variable. The resulting NNLO + LL calculation is cast in the form of an event generator for physical events that can be directly interfaced with a parton shower routine, and we give an explicit construction of the input "Monte Carlo cross sections" satisfying all required criteria. We also show how other proposed approaches naturally arise as special cases in our method. C1 [Alioli, Simone; Bauer, Christian W.; Berggren, Calvin; Walsh, Jonathan R.; Zuberi, Saba] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tackmann, Frank J.] Deutsches Elekt Synchrotron DESY, Theory Grp, D-22607 Hamburg, Germany. RP Alioli, S (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM salioli@lbl.gov; cwbauer@lbl.gov; cjberggren@lbl.gov; frank.tackmann@desy.de; jwalsh@lbl.gov; szuberi@lbl.gov RI Alioli, Simone/Q-4971-2016 OI Alioli, Simone/0000-0001-8234-2247 FU Department of Energy [DE-PS02-09ER09-26]; DFG [TA 867/1-1]; Office of Science, Office of High Energy Physics of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Department of Energy Early Career Award with Funding Opportunity No. DE-PS02-09ER09-26 (SA, CWB, CB, SZ), the DFG Emmy-Noether Grant No. TA 867/1-1 (FT), and the Director, Office of Science, Office of High Energy Physics of the U.S. Department of Energy under the Contract No. DE-AC02-05CH11231 (CWB, CB, JW). NR 55 TC 21 Z9 21 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 16 PY 2014 IS 6 AR 089 DI 10.1007/JHEP06(2014)089 PG 52 WC Physics, Particles & Fields SC Physics GA AK1WL UT WOS:000338209000001 ER PT J AU Winston, ME Hampton-Marcell, J Zarraonaindia, I Owens, SM Moreau, CS Gilbert, JA Hartsel, J Kennedy, SJ Gibbons, SM AF Winston, Max E. Hampton-Marcell, Jarrad Zarraonaindia, Iratxe Owens, Sarah M. Moreau, Corrie S. Gilbert, Jack A. Hartsel, Josh Kennedy, Suzanne J. Gibbons, S. M. TI Understanding Cultivar-Specificity and Soil Determinants of the Cannabis Microbiome SO PLOS ONE LA English DT Article ID SOLANUM-TUBEROSUM L.; BACTERIAL COMMUNITIES; RHIZOSPHERE BACTERIA; ENDOPHYTIC BACTERIA; PLANT; GROWTH; DIVERSITY; PHYTOREMEDIATION; COLONIZATION; TAXONOMY AB Understanding microbial partnerships with the medicinally and economically important crop Cannabis has the potential to affect agricultural practice by improving plant fitness and production yield. Furthermore, Cannabis presents an interesting model to explore plant-microbiome interactions as it produces numerous secondary metabolic compounds. Here we present the first description of the endorhiza-, rhizosphere-, and bulk soil-associated microbiome of five distinct Cannabis cultivars. Bacterial communities of the endorhiza showed significant cultivar-specificity. When controlling cultivar and soil type the microbial community structure was significantly different between plant cultivars, soil types, and between the endorhiza, rhizosphere and soil. The influence of soil type, plant cultivar and sample type differentiation on the microbial community structure provides support for a previously published two-tier selection model, whereby community composition across sample types is determined mainly by soil type, while community structure within endorhiza samples is determined mainly by host cultivar. C1 [Winston, Max E.; Moreau, Corrie S.] Field Museum, Dept Sci & Educ, Chicago, IL 60605 USA. [Winston, Max E.] Univ Chicago, Comm Evolutionary Biol, Chicago, IL 60637 USA. [Hampton-Marcell, Jarrad; Zarraonaindia, Iratxe; Owens, Sarah M.; Gilbert, Jack A.; Gibbons, S. M.] Inst Genom & Syst Biol, Argonne Natl Lab, Lemont, IL USA. [Hampton-Marcell, Jarrad; Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Zarraonaindia, Iratxe] Basque Country Govt, Bilbao, Spain. [Owens, Sarah M.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Hartsel, Josh] Cannavest, San Diego, CA USA. [Kennedy, Suzanne J.] MO BIO Labs, Carlsbad, CA USA. [Gibbons, S. M.] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. RP Winston, ME (reprint author), Field Museum, Dept Sci & Educ, Chicago, IL 60605 USA. EM mewinsto@gmail.com OI Moreau, Corrie/0000-0003-1139-5792; Gibbons, Sean/0000-0002-8724-7916 FU U.S. Dept. of Energy [DE-AC02-06CH11357]; U.S. Department of Education GAANN grant; U.S. Environmental Protection Agency STAR Graduate Fellowship; Amazon Web Services education grant FX This work was supported in part by the U.S. Dept. of Energy under Contract DE-AC02-06CH11357. MEW was supported by a U.S. Department of Education GAANN grant. Funding for SMG was provided U.S. Environmental Protection Agency STAR Graduate Fellowship. Computational resources were funded by a Amazon Web Services education grant. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 51 TC 6 Z9 7 U1 8 U2 42 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 16 PY 2014 VL 9 IS 6 AR e99641 DI 10.1371/journal.pone.0099641 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AJ5PV UT WOS:000337738600051 PM 24932479 ER PT J AU Alsmadi, AM Choi, Y Keavney, DJ Eid, KF Kirby, BJ Liu, X Leiner, J Tivakornsasithorn, K Dobrowolska, M Furdyna, JK AF Alsmadi, A. M. Choi, Y. Keavney, D. J. Eid, K. F. Kirby, B. J. Liu, X. Leiner, J. Tivakornsasithorn, K. Dobrowolska, M. Furdyna, J. K. TI Interfacial exchange coupling in Fe/(Ga,Mn)As bilayers SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC CIRCULAR-DICHROISM; NEUTRON REFLECTOMETRY; FE; SEMICONDUCTORS; FILMS; MN; HETEROSTRUCTURES; ABSORPTION; GA1-XMNXAS; SPECTRA AB We carried out a systematic study of magnetic order and magnetic interlayer coupling in Fe/(Ga,Mn) As bilayers using superconducting quantum interference device magnetometry, polarized neutron reflectometry, element-specific x-ray absorption spectroscopy, x-raymagnetic circular dichroism, and x-ray specular reflectivity. Our results clearly show that Fe/(Ga,Mn) As bilayers are strongly exchange coupled at the interface. However, contrary to recent reports in the literature, we observe a ferromagnetic rather than antiferromagnetic coupling between the magnetic moments of the Mn ions and the Fe layer. It is interesting in this context that the surface region of the (Ga,Mn) As layer that is in direct contact with the Fe film displays a nearly identical coercivity to that of Fe (indicating perfect ferromagnetic coupling of that region), while the bulk of the (Ga,Mn) As layer, which is more weakly ferromagnetically coupled with Fe, shows a significantly smaller coercive field. C1 [Alsmadi, A. M.] Kuwait Univ, Dept Phys, Safat 13060, Kuwait. [Alsmadi, A. M.] Hashemite Univ, Dept Phys, Zarqa 13115, Jordan. [Alsmadi, A. M.; Eid, K. F.] Miami Univ, Dept Phys, Oxford, OH 45056 USA. [Choi, Y.; Keavney, D. J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Kirby, B. J.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Liu, X.; Leiner, J.; Tivakornsasithorn, K.; Dobrowolska, M.; Furdyna, J. K.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Leiner, J.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN USA. [Tivakornsasithorn, K.] Mahidol Univ, Dept Phys, Fac Sci, Bangkok 10400, Thailand. RP Alsmadi, AM (reprint author), Kuwait Univ, Dept Phys, Safat 13060, Kuwait. EM abdel.alsmadi@ku.edu.kw FU National Science Foundation [DMR10-05851]; U.S. DOE [DE-AC02-06CH11357] FX The work at Notre Dame was supported by the National Science Foundation Grant No. DMR10-05851. The work at the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 30 TC 2 Z9 2 U1 2 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 16 PY 2014 VL 89 IS 22 AR 224409 DI 10.1103/PhysRevB.89.224409 PG 7 WC Physics, Condensed Matter SC Physics GA AJ5NF UT WOS:000337730000002 ER PT J AU Lazarevic, N Bozin, ES Scepanovic, M Opacic, M Lei, HC Petrovic, C Popovic, ZV AF Lazarevic, N. Bozin, E. S. Scepanovic, M. Opacic, M. Lei, Hechang Petrovic, C. Popovic, Z. V. TI Probing IrTe2 crystal symmetry by polarized Raman scattering SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METAL DITELLURIDES; BAND-STRUCTURE; BONDS AB Polarized Raman scattering measurements on IrTe2 single crystals carried out over the 15-640 K temperature range, and across the structural phase transition, reveal different insights regarding the crystal symmetry. In the high temperature regime three Raman active modes are observed at all of the studied temperatures above the structural phase transition, rather than two as predicted by the factor group analysis for the assumed P (3) over bar m1 symmetry. This indicates that the actual symmetry of the high temperature phase is lower than previously thought. The observation of an additional E-g mode at high temperature can be explained by doubling of the original trigonal unit cell along the c axis and within the P (3) over bar c1 symmetry. In the low temperature regime (below 245 K) the other Raman modes appear as a consequence of the symmetry lowering phase transition and the corresponding increase of the primitive cell. All of the modes observed below the phase transition temperature can be assigned within the monoclinic crystal symmetry. The temperature dependence of the Raman active phonons in both phases is mainly driven by anharmonicity effects. The results call for reconsideration of the crystallographic phases of IrTe2. C1 [Lazarevic, N.; Scepanovic, M.; Opacic, M.; Popovic, Z. V.] Univ Belgrade, Ctr Solid State Phys & New Mat, Inst Phys Belgrade, Belgrade 11080, Serbia. [Bozin, E. S.; Lei, Hechang; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Lazarevic, N (reprint author), Univ Belgrade, Ctr Solid State Phys & New Mat, Inst Phys Belgrade, Pregrevica 118, Belgrade 11080, Serbia. RI Petrovic, Cedomir/A-8789-2009; LEI, Hechang/H-3278-2016 OI Petrovic, Cedomir/0000-0001-6063-1881; FU Serbian Ministry of Education, Science and Technological Development [ON171032, III45018]; Serbian-Germany bilateral project "Interplay of Fe-vacancy ordering and spin fluctuations in iron-based high temperature superconductors."; US Department of Energy by Brookhaven Science Associates [DE-AC02-98CH10886] FX We gratefully acknowledge discussions with R. Hackl. This work was supported by the Serbian Ministry of Education, Science and Technological Development under Projects No. ON171032 and No. III45018, as well as the Serbian-Germany bilateral project "Interplay of Fe-vacancy ordering and spin fluctuations in iron-based high temperature superconductors."Part of this work was carried out at the Brookhaven National Laboratory which is, as well as the NSLS facility, operated for the Office of Basic Energy Sciences, US Department of Energy by Brookhaven Science Associates, under Contract No. DE-AC02-98CH10886. NR 25 TC 0 Z9 0 U1 10 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 16 PY 2014 VL 89 IS 22 AR 224301 DI 10.1103/PhysRevB.89.224301 PG 6 WC Physics, Condensed Matter SC Physics GA AJ5NF UT WOS:000337730000001 ER PT J AU An, HP Wang, LT Zhang, H AF An, Haipeng Wang, Lian-Tao Zhang, Hao TI Dark matter with t-channel mediator: A simple step beyond contact interaction SO PHYSICAL REVIEW D LA English DT Article ID GENERIC MODEL; RELIC DENSITY; CONSTRAINTS AB Effective contact operators provide the simplest parametrization of dark matter searches at colliders. However, light mediators can significantly change the sensitivity and search strategies. Considering simple models of mediators is an important next step for collider searches. In this paper, we consider the case of a t-channel mediator. Its presence opens up new contributions to the monojet + is not an element of(T) searches and can change the reach significantly. We also study the complementarity between searches for processes of monojet + is not an element of(T) and direct pair production of the mediators. Mediator pair production also gives an important contribution to a CMS-like monojet + is not an element of(T) search, where a second hard jet is allowed. There is a large region of parameter space in which the monojet + is not an element of(T) search provides the stronger limit. Assuming the relic abundance of the dark matter is thermally produced within the framework of this model, we find that in the Dirac fermion dark matter case, there is no region in the parameter space that satisfies the combined constraint of monojet + is not an element of(T) search and direct detection; whereas in the Majorana fermion dark matter case, the mass of dark matter must be larger than about 100 GeV. If the relic abundance requirement is not assumed, the discovery of the t-channel mediator predicts additional new physics. C1 [An, Haipeng] Perimeter Inst, Waterloo, ON N2L 2Y5, Canada. [Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Zhang, Hao] IIT, Chicago, IL 60616 USA. [Zhang, Hao] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Zhang, Hao] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP An, HP (reprint author), Perimeter Inst, Waterloo, ON N2L 2Y5, Canada. RI ZHANG, Hao/G-6430-2015 FU Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation; NSF [PHY-0756966]; DOE Early Career Award [de-sc0003930]; U.S. DOE [DE-AC02-06CH11357, DE- FG02-94ER40840, DE-FG02-91ER40618] FX We thank Maxim Pospelov and Itay Yavin for useful discussions. H. A.'s research at Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. L. T. W. is supported by the NSF under Grant No. PHY-0756966 and by the DOE Early Career Award under Grant No. de-sc0003930. H. Z. is supported by the U.S. DOE under the Grants No. DE-AC02-06CH11357, No. DE- FG02-94ER40840, and No. DE-FG02-91ER40618. NR 52 TC 50 Z9 50 U1 2 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 16 PY 2014 VL 89 IS 11 AR 115014 DI 10.1103/PhysRevD.89.115014 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AJ5NT UT WOS:000337731800005 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Sciolla, G Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Li Gioi, L Piredda, G Bunger, C Dittrich, S Grunberg, O Hartmann, T Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Anulli, F Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Lewis, P Lindemann, D Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wulsin, HW Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Li Gioi, L. Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hartmann, T. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Anulli, F. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Lewis, P. Lindemann, D. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Dalitz plot analysis of eta(c) -> K+K-eta and eta(c) -> K+K-pi(0) in two-photon interactions SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; K-ETA; DECAYS AB We study the processes gamma gamma -> K+K-eta and gamma gamma -> K+K-pi(0) using a data sample of 519 fb(-1) recorded with the BABAR detector operating at the SLAC PEP-II asymmetric-energy e(+)e(-) collider at center-of-mass energies at and near the Upsilon(nS) (n = 2, 3, 4) resonances. We observe eta(c) -> K+K-pi(0) and eta(c) -> K+K-eta decays, measure their relative branching fraction, and perform a Dalitz plot analysis for each decay. We observe the K*(0)(1430) -> K eta decay and measure its branching fraction relative to the K pi decay mode to be R(K*(0)(1430)) = B(K*(0)(1430)-> K eta)/B(K*(0)(1430)-> K pi) = 0.092 +/- 0.025(- 0.025)(+0.010). The eta(c) -> K+K-eta and K*(0)(1430) -> K eta results correspond to the first observations of these channels. The data also show evidence for eta(c)(2S) -> K+K-pi(0) and first evidence for eta(c)(2S) -> K+K-eta. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept Estruct & Constituents Mat, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. 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S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Li Gioi, L.; Piredda, G.; Anulli, F.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hartmann, T.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassarik, Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Calcaterra, Alessandro/P-5260-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Patrignani, Claudia/C-5223-2009; Oyanguren, Arantza/K-6454-2014; Monge, Maria Roberta/G-9127-2012; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Forti, Francesco/H-3035-2011 OI Calcaterra, Alessandro/0000-0003-2670-4826; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Patrignani, Claudia/0000-0002-5882-1747; Oyanguren, Arantza/0000-0002-8240-7300; Monge, Maria Roberta/0000-0003-1633-3195; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Forti, Francesco/0000-0001-6535-7965 FU U.S. Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique; Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA); Binational Science Foundation (USA-Israel); SLAC FX We are grateful for the extraordinary contributions of our PEP-II2 colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union), the A. P. Sloan Foundation (USA) and the Binational Science Foundation (USA-Israel). NR 38 TC 3 Z9 3 U1 0 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 16 PY 2014 VL 89 IS 11 AR 112004 DI 10.1103/PhysRevD.89.112004 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AJ5NT UT WOS:000337731800001 ER PT J AU Wang, X Mostovoy, M Han, MG Horibe, Y Aoki, T Zhu, Y Cheong, SW AF Wang, X. Mostovoy, M. Han, M. G. Horibe, Y. Aoki, T. Zhu, Y. Cheong, S. -W. TI Unfolding of Vortices into Topological Stripes in a Multiferroic Material SO PHYSICAL REVIEW LETTERS LA English DT Article ID DOMAIN-WALLS; SUPERCONDUCTORS; YMNO3 AB Multiferroic hexagonal RMnO3 (R = rare earths) crystals exhibit dense networks of vortex lines at which six domain walls merge. While the domain walls can be readily moved with an applied electric field, the vortex cores so far have been impossible to control. Our experiments demonstrate that shear strain induces a Magnus-type force pulling vortices and antivortices in opposite directions and unfolding them into a topological stripe domain state. We discuss the analogy between this effect and the current-driven dynamics of vortices in superconductors and superfluids. C1 [Wang, X.; Horibe, Y.; Cheong, S. -W.] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. [Wang, X.; Horibe, Y.; Cheong, S. -W.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Mostovoy, M.] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands. [Han, M. G.; Zhu, Y.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Aoki, T.] JEOL USA Inc, Peabody, MA 01960 USA. RP Cheong, SW (reprint author), Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. EM sangc@physics.rutgers.edu RI Aoki, Toshihiro/I-4852-2015 FU National Science Foundation [DMR-1104484]; U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Science and Engineering Grant [DE-AC02-98CH10886] FX We thank Seung Chul Chae and Lijun Wu for fruitful discussions, and Hyeon Na Woo (RISD) for providing a three-dimensional cartoon. The work at Rutgers was supported by the National Science Foundation Grant No. DMR-1104484, and the work at Brookhaven National Laboratory was supported by the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Science and Engineering Grant No. DE-AC02-98CH10886. NR 24 TC 8 Z9 8 U1 2 U2 77 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 16 PY 2014 VL 112 IS 24 AR 247601 DI 10.1103/PhysRevLett.112.247601 PG 5 WC Physics, Multidisciplinary SC Physics GA AJ5OP UT WOS:000337734700005 PM 24996108 ER PT J AU Han, NR de Geofroy, A Burghoff, DP Chan, CWI Lee, AWM Reno, JL Hu, Q AF Han, Ningren de Geofroy, Alexander Burghoff, David P. Chan, Chun Wang I. Lee, Alan Wei Min Reno, John L. Hu, Qing TI Broadband all-electronically tunable MEMS terahertz quantum cascade lasers SO OPTICS LETTERS LA English DT Article ID WIRE-LASER AB In this work, we demonstrate all-electronically tunable terahertz quantum cascade lasers (THz QCLs) with MEMS tuner structures. A two-stage MEMS tuner device is fabricated by a commercial open-foundry process performed by the company MEMSCAP. This provides an inexpensive, rapid, and reliable approach for MEMS tuner fabrication for THz QCLs with a high-precision alignment scheme. In order to electronically actuate the MEMS tuner device, an open-loop cryogenic piezo nanopositioning stage is integrated with the device chip. Our experimental result shows that at least 240 GHz of single-mode continuous electronic tuning can be achieved in cryogenic environments (similar to 4 K) without mode hopping. This provides an important step toward realizing turn-key bench-top tunable THz coherent sources for spectroscopic and coherent tomography applications. (C) 2014 Optical Society of America C1 [Han, Ningren; Burghoff, David P.; Chan, Chun Wang I.; Hu, Qing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [de Geofroy, Alexander; Lee, Alan Wei Min] LongWave Photon LLC, Mountain View, CA 94043 USA. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87123 USA. RP Han, NR (reprint author), MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. EM ningren@mit.edu FU NASA; NSF; Siebel Foundation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The work at MIT is supported by NASA, NSF and the Siebel Foundation. The work at Sandia is performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The author would like to acknowledge Qi Qin and Tsung-Yu Kao for their help in experimental design and device fabrication. NR 16 TC 7 Z9 7 U1 0 U2 18 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD JUN 15 PY 2014 VL 39 IS 12 BP 3480 EP 3483 DI 10.1364/OL.39.003480 PG 4 WC Optics SC Optics GA AL1FF UT WOS:000338870500031 PM 24978516 ER PT J AU Zhang, P Phipps, ME Goodwin, PM Werner, JH AF Zhang, P. Phipps, M. E. Goodwin, P. M. Werner, J. H. TI Confocal line scanning of a Bessel beam for fast 3D Imaging SO OPTICS LETTERS LA English DT Article ID LIGHT-SHEET MICROSCOPY; SINGLE-MOLECULE LOCALIZATION; FLUORESCENCE MICROSCOPY; PLANE ILLUMINATION; THICK MEDIA; EXCITATION; CELLS AB We have developed a light-sheet illumination microscope that can perform fast 3D imaging of transparent biological samples with inexpensive visible lasers and a single galvo mirror (GM). The light-sheet is created by raster scanning a Bessel beam with a GM, with this same GM also being used to rescan the fluorescence across a chip of a camera to construct an image in real time. A slit is used to reject out-of-focus fluorescence such that the image formed in real time has minimal contribution from the sidelobes of the Bessel beam. Compared with two-photon Bessel beam excitation or other confocal line-scanning approaches, our method is of lower cost, is simpler, and does not require calibration and synchronization of multiple GMs. We demonstrated the optical sectioning and out-of-focus background rejection capabilities of this microscope by imaging fluorescently labeled actin filaments in fixed 3T3 cells. (C) 2014 Optical Society of America C1 [Zhang, P.; Phipps, M. E.; Goodwin, P. M.; Werner, J. H.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Werner, JH (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM jwerner@lanl.gov FU Los Alamos National Laboratory Directed Research and Development (LDRD) program; Center for Integrated Nanotechnologies, U.S. Department of Energy, Office of Basic Energy Sciences at the Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was supported through the Los Alamos National Laboratory Directed Research and Development (LDRD) program and was performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at the Los Alamos National Laboratory (Contract DE-AC52-06NA25396). NR 23 TC 3 Z9 3 U1 1 U2 34 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD JUN 15 PY 2014 VL 39 IS 12 BP 3682 EP 3685 DI 10.1364/OL.39.003682 PG 4 WC Optics SC Optics GA AL1FF UT WOS:000338870500082 PM 24978567 ER PT J AU Nielsen, S Minchin, T Kimber, S van Zwieten, L Gilbert, J Munroe, P Joseph, S Thomas, T AF Nielsen, Shaun Minchin, Tom Kimber, Stephen van Zwieten, Lukas Gilbert, Jack Munroe, Paul Joseph, Stephen Thomas, Torsten TI Comparative analysis of the microbial communities in agricultural soil amended with enhanced biochars or traditional fertilisers SO AGRICULTURE ECOSYSTEMS & ENVIRONMENT LA English DT Article DE Biochar; Microbial communities; 16S rRNA gene; High-throughput sequencing; Network analysis ID NITRITE-OXIDIZING BACTERIA; PHYLUM ACIDOBACTERIA; ORGANIC-CARBON; DIVERSITY; WASTE; MICROORGANISMS; PRODUCTIVITY; VARIABILITY; COEXISTENCE; ANTHROSOLS AB Biochar can have a positive effect on agricultural soils and plant yields. The underlying mechanisms that deliver beneficial outcomes are still poorly understood. Soils contain complex communities of hundreds or thousands of distinct microorganisms, and it has been shown that biochar can have an impact on their composition and function. Here we analyse the microbial communities in a controlled field trial that compared the effect of enhanced biochars (EBs) against a farmer practice (FP) of traditional fertilisation (urea, superphosphate and potash) on sweet corn yield. During sequential crop cycles (barley and sweet corn) two types of EBs were applied at low and high levels (total of 1.1 and 5.44 t ha(-1), respectively). Samples were taken at the end of a second crop cycle and over 50,000 16S ribosomal RNA (16S rRNA) tag sequences were generated per sample to characterise microbial communities. Despite the lower amounts of nutrients provided by EBs, their amendment to soil produced similar crop yields to the FP. In addition, significant differences in microbial community composition were observed between the high EB and FP treatments. This was driven by differences in the relative abundances of only a few community members. Community level differences were also correlated with a higher soil pH associated with EB laden soil. Network analysis showed that the low EB application had more correlation patterns (co-occurrences and exclusions) between microbial taxa, and highlighted the importance of associations between members of the phyla Acidobacteria and Verrucomicrobia in the biochar environment. Overall, a large number of microorganisms appear to be influenced by EB amendment compared with fertiliser use leading to a complex re-wiring of community composition and associations. (C) 2014 Elsevier B.V. All rights reserved. C1 [Nielsen, Shaun; Minchin, Tom; Thomas, Torsten] Univ New S Wales, Ctr Marine Bioinnovat, Sch Biotechnol & Biomol Sci, Sydney, NSW 2052, Australia. [Munroe, Paul; Joseph, Stephen] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia. [Kimber, Stephen; van Zwieten, Lukas] New South Wales Dept Primary Ind, Wollongbar, NSW 2477, Australia. [Gilbert, Jack] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, Jack] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. RP Nielsen, S (reprint author), Univ New S Wales, Ctr Marine Bioinnovat, Sch Biotechnol & Biomol Sci, Sydney, NSW 2052, Australia. EM s.nielsen@unsw.edu.au RI Munroe, Paul/I-9313-2016; OI Munroe, Paul/0000-0002-5091-2513; Van Zwieten, Lukas/0000-0002-8832-360X FU Australian Research Council [LP120200418] FX We would like to thank the Earth Microbiome Project (www.earthmicrobiome.org) for DNA sample processing and sequencing. All amplicon and metadata has been made public through the data portal (www.microbio.me/emp). This work was supported through funding from the Australian Research Council LP120200418. NR 54 TC 25 Z9 28 U1 7 U2 134 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8809 EI 1873-2305 J9 AGR ECOSYST ENVIRON JI Agric. Ecosyst. Environ. PD JUN 15 PY 2014 VL 191 SI SI BP 73 EP 82 DI 10.1016/j.agee.2014.04.006 PG 10 WC Agriculture, Multidisciplinary; Ecology; Environmental Sciences SC Agriculture; Environmental Sciences & Ecology GA AK4KL UT WOS:000338393500008 ER PT J AU Curley, KC Greenspan, A Hicks, RA Hoffman, SW Miller, AC AF Curley, K. C. Greenspan, A. Hicks, R. A. Hoffman, S. W. Miller, A. C. TI FEDERAL COORDINATION FOR TRAUMATIC BRAIN INJURY RESEARCH: THE NATIONAL RESEARCH ACTION PLAN SO JOURNAL OF NEUROTRAUMA LA English DT Meeting Abstract CT 32nd Annual National Neurotrauma Symposium CY JUN 29-JUL 02, 2014 CL San Francisco, CA DE federal funding agencies; research coordination; strategic planning C1 [Curley, K. C.] US Army MRMC, Ft Detrick, MD USA. [Greenspan, A.] Ctr Dis Control & Prevent, Atlanta, GA USA. [Hicks, R. A.] NINDS, NIH, Rockville, MD USA. [Hoffman, S. W.] Dept Vet Affairs, Washington, DC USA. [Miller, A. C.] US DOE, Washington, DC 20585 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 0897-7151 EI 1557-9042 J9 J NEUROTRAUM JI J. Neurotrauma PD JUN 15 PY 2014 VL 31 IS 12 MA B1-22 BP A51 EP A52 PG 2 WC Critical Care Medicine; Clinical Neurology; Neurosciences SC General & Internal Medicine; Neurosciences & Neurology GA AK5DC UT WOS:000338443600138 ER PT J AU Kelley, AM Ranes, B Estrada, A Grandizio, CM AF Kelley, A. M. Ranes, B. Estrada, A. Grandizio, C. M. TI EVALUATION OF THE MILITARY FUNCTIONAL ASSESSMENT PROGRAM: ASSESSMENT OF THE CONSTRUCT VALIDITY USING ARCHIVED CLINICAL DATA SO JOURNAL OF NEUROTRAUMA LA English DT Meeting Abstract CT 32nd Annual National Neurotrauma Symposium CY JUN 29-JUL 02, 2014 CL San Francisco, CA DE fitness-for-duty; military; return-to-duty C1 [Kelley, A. M.; Estrada, A.; Grandizio, C. M.] US Army Aeromed Res Lab, Ft Rucker, AL USA. [Ranes, B.] Oak Ridge Inst Sci & Educ, Belcamp, MD USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 0897-7151 EI 1557-9042 J9 J NEUROTRAUM JI J. Neurotrauma PD JUN 15 PY 2014 VL 31 IS 12 MA B1-01 BP A44 EP A45 PG 2 WC Critical Care Medicine; Clinical Neurology; Neurosciences SC General & Internal Medicine; Neurosciences & Neurology GA AK5DC UT WOS:000338443600118 ER PT J AU Tagge, CA Fisher, AM Gaudreau, AB Wojnarowicz, MW Minaeva, O Moncaster, JA Casey, N Stein, TD Moss, WC Moir, RD Tanzi, RE Stanton, PK Mckee, AC Goldstein, LE AF Tagge, C. A. Fisher, A. M. Gaudreau, A. B. Wojnarowicz, M. W. Minaeva, O. Moncaster, J. A. Casey, N. Stein, T. D. Moss, W. C. Moir, R. D. Tanzi, R. E. Stanton, P. K. McKee, A. C. Goldstein, L. E. TI ELUCIDATING THE PATHOBIOLOGY OF IMPACT CONCUSSION IN A MOUSE MODEL OF MILD TRAUMATIC BRAIN INJURY SO JOURNAL OF NEUROTRAUMA LA English DT Meeting Abstract CT 32nd Annual National Neurotrauma Symposium CY JUN 29-JUL 02, 2014 CL San Francisco, CA DE traumatic brain injury C1 [Tagge, C. A.; Fisher, A. M.; Gaudreau, A. B.; Wojnarowicz, M. W.; Minaeva, O.; Moncaster, J. A.; Casey, N.; Stein, T. D.; McKee, A. C.; Goldstein, L. E.] Boston Univ, Coll Engn, Sch Med, Boston, MA 02215 USA. [Stein, T. D.; Goldstein, L. E.] Boston Univ, Alzheimers Dis Ctr, Boston, MA 02215 USA. [Stein, T. D.; McKee, A. C.] Boston VA Healthcare Syst, Boston, MA USA. [Moss, W. C.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Stanton, P. K.] New York Med Coll, Valhalla, NY 10595 USA. [Moir, R. D.; Tanzi, R. E.] Massachusetts Gen Hosp, Charlestown, MA USA. NR 0 TC 0 Z9 0 U1 2 U2 6 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 0897-7151 EI 1557-9042 J9 J NEUROTRAUM JI J. Neurotrauma PD JUN 15 PY 2014 VL 31 IS 12 MA D2-25 BP A122 EP A122 PG 1 WC Critical Care Medicine; Clinical Neurology; Neurosciences SC General & Internal Medicine; Neurosciences & Neurology GA AK5DC UT WOS:000338443600331 ER PT J AU Wojnarowicz, MW Fisher, AM Tagge, CA Gaudreau, AB Minaeva, O Moncaster, JA Casey, N Stein, TD Moss, WC Moir, RD Tanzi, RE Stanton, PK McKee, AC Goldstein, LE AF Wojnarowicz, M. W. Fisher, A. M. Tagge, C. A. Gaudreau, A. B. Minaeva, O. Moncaster, J. A. Casey, N. Stein, T. D. Moss, W. C. Moir, R. D. Tanzi, R. E. Stanton, P. K. McKee, A. C. Goldstein, L. E. TI ELUCIDATING THE KINEMATICS AND PATHOBIOLOGY OF BLAST-RELATED TRAUMATIC BRAIN INJURY AND SEQUELAE IN A MOUSE MODEL SO JOURNAL OF NEUROTRAUMA LA English DT Meeting Abstract CT 32nd Annual National Neurotrauma Symposium CY JUN 29-JUL 02, 2014 CL San Francisco, CA DE blast; CTE; murine model; neuropathology C1 [Wojnarowicz, M. W.; Fisher, A. M.; Tagge, C. A.; Gaudreau, A. B.; Minaeva, O.; Moncaster, J. A.; Casey, N.; Stein, T. D.; McKee, A. C.; Goldstein, L. E.] Boston Univ, Coll Engn, Sch Med, Boston, MA 02215 USA. [Stein, T. D.; McKee, A. C.; Goldstein, L. E.] Boston Univ, Alzheimers Dis Ctr, Boston, MA 02215 USA. [Stein, T. D.; McKee, A. C.] Boston VA Healthcare Syst, Boston, MA USA. [Moss, W. C.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Stanton, P. K.] New York Med Coll, Valhalla, NY 10595 USA. [Moir, R. D.; Tanzi, R. E.] Massachusetts Gen Hosp, Charlestown, MA USA. NR 0 TC 0 Z9 0 U1 1 U2 9 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 0897-7151 EI 1557-9042 J9 J NEUROTRAUM JI J. Neurotrauma PD JUN 15 PY 2014 VL 31 IS 12 MA D2-07 BP A115 EP A115 PG 1 WC Critical Care Medicine; Clinical Neurology; Neurosciences SC General & Internal Medicine; Neurosciences & Neurology GA AK5DC UT WOS:000338443600313 ER PT J AU Wang, YF AF Wang, Yifeng TI Nanogeochemistry: Nanostructures, emergent properties and their control on geochemical reactions and mass transfers SO CHEMICAL GEOLOGY LA English DT Review DE Nanogeochemistry; Nanoparticles; Nanopores; Nanofluids; Emergent properties; Size-dependent properties; Nanocomposite; Mineral-water interface; Surface chemistry; Phase stability; Reaction kinetics; Waste forms ID SHALE GAS-RESERVOIRS; NEVADA TEST-SITE; PARTICLE-SIZE; CARBON NANOTUBES; CONFINED FLUIDS; ORGANIC-MATTER; HEMATITE NANOPARTICLES; IN-SITU; METHANE ADSORPTION; TIO2 NANOPARTICLES AB Nanogeochemistry-a newly emerging research field-attempts to understand geochemical reactions and mass transfers at nanometer scales, especially with regards to the formation of nanostructures in geochemical systems, emergent properties of these structures, and their controls on geochemical processes. The research also includes use of nanotechnology to design new materials and engineering approaches for effective natural resource extraction and environmental management. At the core of this new research field is the concept that, as the size of a material is reduced to nanometers, novel physical or chemical properties of the material may emerge that can be drastically different from those of the corresponding bulk phase and the material properties then become size-dependent. Nanostructures, which frequently occur in geologic materials, may directly control mineral phase stability, mineral-water interface chemistry, geochemical reaction kinetics, geo-fluid migration and transport, and even global biogeochemical cycles as a whole. This paper aims to provide a comprehensive review of recent progress in nanogeochemical research. The review is focused on two general types of nanostructures-nano solid phases and nanopores (nanofluids)-with an emphasis on the occurrence of each nanostructure in natural environments, the associated emergent properties, and the potential geochemical implications. Stemming from an increasing interest in shale gas research, a special discussion is provided on gas/oil disposition and migration in unconventional low-permeability reservoirs, wherein shale is treated as a nanocomposite material. Nanogeochemistry is a relatively young research field, and much remains to be explored. There is an urgent need for systematically characterizing specific nanostructures over the whole nanometer-size range and developing a general theoretical framework for data analysis and synthesis. There is also a need for developing experimental and modeling techniques to extrapolate the knowledge obtained from simple model systems to complex natural systems. (C) 2014 Elsevier B.V. All rights reserved. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Wang, YF (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Lockheed Martin Corporation [DE-AC04-94AL85000]; DOE Sandia LDRD Program [173102] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work is supported by DOE Sandia LDRD Program (#173102). The author would like to thank Reviewer Papers Coordinator Tim Horscroft for the invitation for this review paper and also Dr. Young-Shin Jun at Washington University in St. Louis and an anonymous reviewer for their constructive comments. The author also thanks Dr. Andrew Miller of Emporia State University and Drs. Carlos Jove-Colon and Edward Matteo of Sandia National Laboratories for their help during the manuscript preparation. NR 206 TC 20 Z9 23 U1 12 U2 134 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD JUN 15 PY 2014 VL 378 BP 1 EP 23 DI 10.1016/j.chemgeo.2014.04.007 PG 23 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AJ8YQ UT WOS:000337994400001 ER PT J AU Cervini-Silva, J Antonio-Nieto-Camacho Gomez-Vidales, V Ramirez-Apan, MT Palacios, E Montoya, A Kaufhold, S Abidin, Z Theng, BKG AF Cervini-Silva, Javiera Antonio-Nieto-Camacho Gomez-Vidales, Virginia Teresa Ramirez-Apan, Maria Palacios, Eduardo Montoya, Ascencion Kaufhold, Stephan Abidin, Zeanal Theng, Benny K. G. TI Lipid peroxidation and cytotoxicity induced by respirable volcanic ash SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Naturally-occurring allophane; Mineral Fe3+; Redox; Oxidative stress ID OXIDATIVE STRESS; DESFERRIOXAMINE-B; HEALTH-HAZARDS; ALLOPHANE; DISSOLUTION; HALLOYSITE; IMOGOLITE; TOXICITY; IRON; SUSPENSIONS AB This paper reports that the main component of respirable volcanic ash, allophane, induces lipid peroxidation (LP), the oxidative degradation of lipids in cell membranes, and cytotoxicity in murin monocyle/macrophage cells. Naturally-occurring allophane collected from New Zealand, japan, and Ecuador was studied. The quantification of LP was conducted using the Thiobarbituric Acid Reactive Substances (TBARS) assay. The cytotoxic effect was determined by the 3-[4,5-dimethylthiazol-2-yl]-2,5-diphenyltetrazolium bromide calorimetric assay. Electron-Paramagnetic Resonance (EPR) determinations of naturally-occurring allophane confirmed the incorporation in the structure and clustering of structural Fe3+, and nucleation and growth of small-sized Fe (oxyhydr)oxide or gibb-site. LP induced by allophane varied with time, and solid concentration and composition, reaching 6.7 +/- 0.2 nmol TBARS mg prot(-1). LP was surface controlled but not restricted by structural or surfacebound Fe3+, because redox processes induced by soluble components other than perferryl iron. The reactivity of Fe3+ soluble species stemming from surface-bound Fe3+ or small-sized Fe3+ refractory minerals in allophane surpassed that of structural Fe3+ located in tetrahedral or octahedral sites of phyllosilicates or bulk iron oxides. Desferrioxamine B mesylate salt (DFOB) or ethylenediaminetetraacetic acid (EDTA) inhibited LP. EDTA acted as a more effective inhibitor, explained by multiple electron transfer pathways. Registered cell-viability values were as low as 68.5 +/- 6.7%. (C) 2014 Elsevier B.V. All rights reserved. C1 [Cervini-Silva, Javiera] Univ Autonoma Metropolitana, Unidad Cuajimalpa, Dept Proc & Tecnol, Mexico City 01120, DF, Mexico. [Cervini-Silva, Javiera] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Antonio-Nieto-Camacho; Teresa Ramirez-Apan, Maria] Univ Nacl Autonoma Mexico, Inst Quim, Lab Pruebas Biol, Mexico City 04510, DF, Mexico. [Gomez-Vidales, Virginia] Univ Nacl Autonoma Mexico, Inst Quim, Lab Resonancia Paramagnet Elect, Mexico City 04510, DF, Mexico. [Palacios, Eduardo; Montoya, Ascencion] Inst Mexicano Petr, Direcc Invest & Posgrado, Mexico City, DF, Mexico. [Kaufhold, Stephan] BGR Bundesansalt Geowissensch & Rohstoffe, D-30655 Hannover, Germany. [Abidin, Zeanal] Ehime Univ, Fac Agr, Appl Chem Environm Ind Lab, Matsuyama, Ehime 7908566, Japan. [Abidin, Zeanal] Bogor Agr Univ, Fac Sci & Math, Dept Chem, Jl Meranti, Bogor West Of J, Indonesia. [Theng, Benny K. G.] Landcare Res, Palmerston North 4442, New Zealand. RP Cervini-Silva, J (reprint author), Univ Autonoma Metropolitana, Unidad Cuajimalpa, Dept Proc & Tecnol, Artificios 40,6 Piso, Mexico City 01120, DF, Mexico. EM jcervini@correo.cua.uam.mx FU Universidad Autonoma Metropolitana Unidad Cuajimalpa FX The authors are thankful to Dr. S.-I. Wada (Kyushu University, Japan) and Professor N. Yoshinaga (Ehime University) for providing the KiP allophane (Table 1), respectively; Maria del Rocio Galindo Ortega and Natalia Alfonsina Mena (UAM-Cuajimalpa) for technical assistance. This project was supported in part by Universidad Autonoma Metropolitana Unidad Cuajimalpa. NR 59 TC 4 Z9 4 U1 1 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JUN 15 PY 2014 VL 274 BP 237 EP 246 DI 10.1016/j.jhazmat.2014.04.015 PG 10 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AJ8VI UT WOS:000337985600029 PM 24793297 ER PT J AU Quach, DL Mincher, BJ Wai, CM AF Quach, Donna L. Mincher, Bruce J. Wai, Chien M. TI Supercritical fluid extraction and separation of uranium from other actinides SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Nuclear fuel cycle; Actinide separations; Supercritical fluid extraction; High level waste ID CARBON-DIOXIDE EXTRACTION; TRI-N-BUTYLPHOSPHATE; NITRIC-ACID SOLUTION; HYDROXAMIC ACIDS; ORGANOPHOSPHORUS REAGENTS; BENZOHYDROXAMIC ACID; ORGANIC EXTRACTANTS; REDUCTION KINETICS; IRRADIATED FUELS; COMPLEXING POWER AB The feasibility of separating U from nitric acid solutions of mixed actinides using tri-n-butylphosphate (TBP)-modified supercritical fluid carbon dioxide (sc-CO2) was investigated. The actinides U, Np, Pu, and Am were extracted into sc-CO2 modified with TBP from a range of nitric acid concentrations, in the absence of, or in the presence of, a number of traditional reducing and/or complexing agents to demonstrate the separation of these metals from U under sc-CO2 conditions. The separation of U from Pu using sc-CO2 was successful at nitric acid concentrations of less than 3M in the presence of acetohydroxamic acid (AHA) or oxalic acid (OA) to mitigate Pu extraction, and the separation of U from Np was successful at nitric acid concentrations of less than 1 M in the presence of AHA, OA, or sodium nitrite to mitigate Np extraction. Americium was not well extracted under any condition studied. (C) 2014 Elsevier B.V. All rights reserved. C1 [Quach, Donna L.; Wai, Chien M.] Univ Idaho, Dept Chem, Moscow, ID 83844 USA. [Mincher, Bruce J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Mincher, BJ (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM bruce.mincher@inl.gov RI Mincher, Bruce/C-7758-2017 FU INL-LDRD Program [DE-AC07-05ID14517] FX This work was supported by INL-LDRD Program under Idaho Operations Contract DE-AC07-05ID14517. NR 46 TC 10 Z9 11 U1 1 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JUN 15 PY 2014 VL 274 BP 360 EP 366 DI 10.1016/j.jhazmat.2014.04.023 PG 7 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AJ8VI UT WOS:000337985600041 PM 24801893 ER PT J AU Villarini, G Lavers, DA Scoccimarro, E Zhao, M Wehner, MF Vecchi, GA Knutson, TR Reed, KA AF Villarini, Gabriele Lavers, David A. Scoccimarro, Enrico Zhao, Ming Wehner, Michael F. Vecchi, Gabriel A. Knutson, Thomas R. Reed, Kevin A. TI Sensitivity of Tropical Cyclone Rainfall to Idealized Global-Scale Forcings SO JOURNAL OF CLIMATE LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; GENERAL-CIRCULATION MODEL; SEA-SURFACE TEMPERATURE; CLIMATE SIMULATIONS; CUMULUS CONVECTION; CO2 INCREASE; RESOLUTION; PARAMETERIZATION; PRECIPITATION; IMPACT AB Heavy rainfall and flooding associated with tropical cyclones (TCs) are responsible for a large number of fatalities and economic damage worldwide. Despite their large socioeconomic impacts, research into heavy rainfall and flooding associated with TCs has received limited attention to date and still represents a major challenge. The capability to adapt to future changes in heavy rainfall and flooding associated with TCs is inextricably linked to and informed by understanding of the sensitivity of TC rainfall to likely future forcing mechanisms. Here a set of idealized high-resolution atmospheric model experiments produced as part of the U.S. Climate Variability and Predictability (CLIVAR) Hurricane Working Group activity is used to examine TC response to idealized global-scale perturbations: the doubling of CO2, uniform 2-K increases in global sea surface temperature (SST), and their combined impact. As a preliminary but key step, daily rainfall patterns of composite TCs within climate model outputs are first compared and contrasted to the observational records. To assess similarities and differences across different regions in response to the warming scenarios, analyses are performed at the global and hemispheric scales and in, six global TC ocean basins. The results indicate a reduction in TC daily precipitation rates in the doubling CO2 scenario (on the order of 5% globally) and an increase in TC rainfall rates associated with a uniform increase of 2K in SST (both alone and in combination with CO2 doubling; on the order of 10%-20% globally). C1 [Villarini, Gabriele; Lavers, David A.] Univ Iowa, IIHR Hydrosci & Engn, Iowa City, IA 52242 USA. [Scoccimarro, Enrico] Ist Nazl Geofis & Vulcanol, Bologna, Italy. [Scoccimarro, Enrico] Ctr Euromediterraneo Cambiamenti Climat, Lecce, Italy. [Zhao, Ming; Vecchi, Gabriel A.; Knutson, Thomas R.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Wehner, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Reed, Kevin A.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. RP Villarini, G (reprint author), Univ Iowa, IIHR Hydrosci & Engn, Iowa City, IA 52242 USA. EM gabriele-villarini@uiowa.edu RI Vecchi, Gabriel/A-2413-2008; Reed, Kevin/C-4466-2012; Zhao, Ming/C-6928-2014; Villarini, Gabriele/F-8069-2016 OI Vecchi, Gabriel/0000-0002-5085-224X; Reed, Kevin/0000-0003-3741-7080; Villarini, Gabriele/0000-0001-9566-2370 FU U.S. CLIVAR; Iowa Flood Center; IIHR-Hydroscience Engineering; National Science Foundation [AGS-1262099]; Italian Ministry of Education, University and Research; Italian Ministry of Environment, Land and Sea under the GEMINA project; Regional and Global Climate Modeling Program of the Office of Biological and Environmental Research in the Department of Energy Office of Science [DE-AC02-05CH11231] FX This work was carried out as part of a Hurricane and Climate Working Group activity supported by the U.S. CLIVAR. We acknowledge the support provided by Naomi Henderson, who downloaded and organized the data at the Lamont data library. Gabriele Villarini and David Lavers acknowledge financial support from the Iowa Flood Center, IIHR-Hydroscience & Engineering. This material is based in part upon work supported by the National Science Foundation under Grant AGS-1262099 (Gabriele Villarini and Gabriel A. Vecchi), and in part from the Italian Ministry of Education, University and Research and the Italian Ministry of Environment, Land and Sea under the GEMINA project (Enrico Scoccimarro). Michael Wehner was supported by the Regional and Global Climate Modeling Program of the Office of Biological and Environmental Research in the Department of Energy Office of Science under Contract DE-AC02-05CH11231. CAM5 calculations were performed at the National Energy Research Supercomputing Center (NERSC) at the Lawrence Berkeley National Laboratory. NR 53 TC 24 Z9 24 U1 3 U2 22 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD JUN 15 PY 2014 VL 27 IS 12 BP 4622 EP 4641 DI 10.1175/JCLI-D-13-00780.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AJ4PV UT WOS:000337659200018 ER PT J AU Boley, N Wan, KH Bickel, PJ Celniker, SE AF Boley, Nathan Wan, Kenneth H. Bickel, Peter J. Celniker, Susan E. TI Navigating and mining modENCODE data SO METHODS LA English DT Article DE modENCODE; Mining; Drosophila; Transcription; Chromatin ID CHIP-SEQ EXPERIMENTS; FULL-LENGTH CDNAS; RNA-SEQ; DROSOPHILA-MELANOGASTER; GENE-EXPRESSION; MESSENGER-RNAS; HUMAN GENOME; DNA; MICRORNAS; SEQUENCE AB modENCODE was a 5 year NHGRI funded project (2007-2012) to map the function of every base in the genomes of worms and flies characterizing positions of modified histones and other chromatin marks, origins of DNA replication, RNA transcripts and the transcription factor binding sites that control gene expression. Here we describe the Drosophila modENCODE datasets and how best to access and use them for genome wide and individual gene studies. (C) 2014 Elsevier Inc. All rights reserved. C1 [Boley, Nathan] Univ Calif Berkeley, Dept Biostat, Berkeley, CA 94720 USA. [Wan, Kenneth H.; Celniker, Susan E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Bickel, Peter J.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. RP Celniker, SE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. FU National Human Genome Research Institute modENCODE Project under Department of Energy [U01 HG004271, DE-AC02-05CH11231]; ENCODE DAC [5U01HG004695-04]; [1U01HG007031-01] FX We thank the members of the modENCODE transcription consortium and especially Ben Brown for helpful discussions. This work was funded by a contract from the National Human Genome Research Institute modENCODE Project, contract U01 HG004271, to S.E.C. (Principal Investigator) under Department of Energy contract no. DE-AC02-05CH11231. N.B. and P.B. (Principle Investigator) were support by 1U01HG007031-01 and the ENCODE DAC 5U01HG004695-04. NR 60 TC 7 Z9 7 U1 0 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1046-2023 EI 1095-9130 J9 METHODS JI Methods PD JUN 15 PY 2014 VL 68 IS 1 BP 38 EP 47 DI 10.1016/j.ymeth.2014.03.007 PG 10 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AJ3FG UT WOS:000337551300005 PM 24636835 ER PT J AU Groenewold, GS Delmore, JE Benson, MT Tsuda, T Hagiwara, R AF Groenewold, Gary S. Delmore, James E. Benson, Michael T. Tsuda, Tetsuya Hagiwara, Rika TI Generation of gas-phase zirconium fluoroanions by electrospray of an ionic liquid SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID ACCELERATOR MASS-SPECTROMETRY; EFFECTIVE CORE POTENTIALS; 1-ETHYL-3-METHYLIMIDAZOLIUM BIFLUORIDE; STRUCTURAL CHARACTERISTICS; PHYSICOCHEMICAL PROPERTIES; MOLECULAR CALCULATIONS; MOLTEN-SALTS; FLUORIDE; DENSITY; ANIONS AB RATIONALE New approaches for forming anions are sought that have strong abundance and no isobaric overlap, attributes that are compatible with the measurement of isotope ratios. Fluoroanions are particularly attractive because fluorine is monoisotopic, and thus will not have overlapping isobars with the isotope of interest. Since many elements do not have positive electron affinity values, they do not form stable negative atomic ions, and hence are not compatible with isotope ratio measurement using high sensitivity isotope ratio mass spectrometers such as accelerator mass spectrometers. METHODS Zirconium fluoroanions were prepared using the fluorinating ionic liquid (IL) 1-ethyl-3-methylimidazolium fluorohydrogenate, which was used to generate abundant [ZrF5]- ions using electrospray ionization. The IL was dissolved in acetonitrile, combined with a dilute solution of either Zr4+ or ZrO2+, and then electrosprayed. Mass analysis and collision-induced dissociation experiments were conducted using a time-of-flight mass spectrometer. Cluster structures were predicted using density functional theory calculations. RESULTS The fluorohydrogenate IL solutions generated abundant [ZrF5]- ions starting from solutions of both Zr4+ and ZrO2+. The mass spectra also contained IL-bearing cluster ions, whose compositions indicated the presence of [ZrF6]2- in solution, a conclusion supported by the structural calculations. Rinsing out the zirconium-IL solution with acetonitrile decreased the IL clusters, but enhanced [ZrF5]-, which was sorbed by the polymeric electrospray supply capillary, and then released upon rinsing. This reduced the ion background in the mass spectrum. CONCLUSIONS The fluorohydrogenate-IL solutions are a facile way to form zirconium fluoroanions in the gas phase using electrospray. The approach has potential as a source of fluoroanions for isotope ratio measurements, which would enable high-sensitivity measurement of minor zirconium isotopes without overlapping isobars caused by the charge carrier (i.e., the monoisotopic fluorine atoms). Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Groenewold, Gary S.; Delmore, James E.; Benson, Michael T.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Tsuda, Tetsuya] Osaka Univ, Grad Sch Engn, Dept Appl Chem, Osaka, Japan. [Hagiwara, Rika] Kyoto Univ, Grad Sch Energy Sci, Dept Fundamental Energy Sci, Kyoto, Japan. RP Groenewold, GS (reprint author), Idaho Natl Lab, 2351 North Blvd, Idaho Falls, ID 83415 USA. EM gary.groenewold@inl.gov RI Tsuda, Tetsuya/F-7234-2014; Benson, Michael/B-8855-2017 OI Tsuda, Tetsuya/0000-0001-9462-8066; Benson, Michael/0000-0003-4927-614X FU United States Department of Energy [DE-AC07-05ID14517] FX This research was funded by the United States Department of Energy, under contract DE-AC07-05ID14517. NR 27 TC 1 Z9 1 U1 1 U2 21 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD JUN 15 PY 2014 VL 28 IS 11 BP 1233 EP 1242 DI 10.1002/rcm.6890 PG 10 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA AJ2SE UT WOS:000337510800008 PM 24760564 ER PT J AU Lorenz, M Ovchinnikova, OS Van Berkel, GJ AF Lorenz, Matthias Ovchinnikova, Olga S. Van Berkel, Gary J. TI Fully automated laser ablation liquid capture surface analysis using nanoelectrospray ionization mass spectrometry SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID ELECTROSPRAY-IONIZATION; ATMOSPHERIC-PRESSURE; ALSTROEMERIA; GLYCOSIDES; FLOWERS; CHROMATOGRAPHY; EMITTER; LESA; MS AB RATIONALE Laser ablation provides for the possibility of sampling a large variety of surfaces with high spatial resolution. This type of sampling when employed in conjunction with liquid capture followed by nanoelectrospray ionization provides the opportunity for sensitive and prolonged interrogation of samples by mass spectrometry as well as the ability to analyze surfaces not amenable to direct liquid extraction. METHODS A fully automated, reflection geometry, laser ablation liquid capture spot sampling system was achieved by incorporating appropriate laser fiber optics and a focusing lens into a commercially available, liquid extraction surface analysis (LESA (R))-ready Advion TriVersa NanoMate system. RESULTS Under optimized conditions about 10% of laser-ablated material could be captured in a droplet positioned vertically over the ablation region using the NanoMate robot-controlled pipette. The sampling spot size area with this laser ablation liquid capture surface analysis (LA/LCSA) mode of operation (typically about 120 mu mx160 mu m) was approximately 50 times smaller than that achievable by direct liquid extraction using LESA (R) (ca 1 mm diameter liquid extraction spot). The setup was successfully applied for the analysis of ink on glass and paper as well as the endogenous components in Alstroemeria Yellow King flower petals. In a second mode of operation with a comparable sampling spot size, termed laser ablation/LESA (R), the laser system was used to drill through, penetrate, or otherwise expose material beneath a solvent resistant surface. Once drilled, LESA (R) was effective in sampling soluble material exposed at that location on the surface. CONCLUSIONS Incorporating the capability for different laser ablation liquid capture spot sampling modes of operation into a LESA (R)-ready Advion TriVersa NanoMate enhanced the spot sampling spatial resolution of this device and broadened the surface types amenable to analysis to include absorbent and solvent-resistant materials. Published in 2014. This article is a U.S. Government work and is in the public domain in the USA. C1 [Lorenz, Matthias; Ovchinnikova, Olga S.; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. RP Van Berkel, GJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. EM vanberkelgj@ornl.gov RI Lorenz, Matthias/F-8273-2016 OI Lorenz, Matthias/0000-0003-0867-8548 FU ORNL Technology Transfer and Economic Development Royalty Funds; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Government [DE-AC05-00OR22725] FX Early stage concept development for LA/LCSA and LA/LESA (R) was funded by ORNL Technology Transfer and Economic Development Royalty Funds. Fundamental studies and proof of concept experiments presented here were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. This manuscript has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. Accordingly, the U.S. Government retains a paid-up, nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this contribution, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U.S. Government purposes. NR 34 TC 6 Z9 6 U1 1 U2 22 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD JUN 15 PY 2014 VL 28 IS 11 BP 1312 EP 1320 DI 10.1002/rcm.6904 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA AJ2SE UT WOS:000337510800016 PM 24760572 ER PT J AU Jost, AB Mundil, R He, B Brown, ST Altiner, D Sun, YD DePaolo, DJ Payne, JL AF Jost, Adam B. Mundil, Roland He, Bin Brown, Shaun T. Altiner, Demir Sun, Yadong DePaolo, Donald J. Payne, Jonathan L. TI Constraining the cause of the end-Guadalupian extinction with coupled records of carbon and calcium isotopes SO EARTH AND PLANETARY SCIENCE LETTERS LA English DT Article DE Capitanian; Emeishan; Middle Permian diagenesis large igneous province ID PERMIAN MASS EXTINCTION; SEA-LEVEL CHANGE; SOUTH CHINA; TRIASSIC BOUNDARY; SW CHINA; FRACTIONATION FACTOR; CHEMICAL EVOLUTION; MIDDLE; SEAWATER; OXYGEN AB A negative delta C-13 excursion in carbonate sediments near the Guadalupian/Lopingian (Middle/Late Permian) boundary has been interpreted to have resulted from a large carbon cycle disturbance during the end-Guadalupian extinction event (ca. 260 Ma). However, the carbon isotope data alone are insufficient to uniquely determine the type and magnitude of perturbation to the global carbon cycle. Calcium isotopes can be used to further constrain the cause of a carbon isotope excursion because the carbon and calcium cycles are coupled via CaCO3 burial. In this study, we present coupled carbon and calcium isotope records from three Guadalupian-Lopingian (G/L) sections in China (Penglaitan and Chaotian) and Turkey (Koserelik Tepe). The delta C-13 and delta Ca-44/40 records differ among our studied sections and do not co-vary in the same manner. No section shows delta C-13 and delta Ca-44/40 changes consistent with massive, rapid volcanic CO2 emissions or methane clathrate destabilization. Additionally, many sections with large (>3 parts per thousand) changes in delta C-13 exhibit 8180 evidence for diagenetic alteration. Only one section exhibits a large excursion in the delta Ca-44/40 of limestone but the absence of a similar excursion in the delta Ca-44/40 of conodont apatite suggests that the limestone excursion reflects a mineralogical control rather than a perturbation to the global calcium cycle. Hence, we interpret the large isotopic changes observed in some sections to have resulted from local burial conditions or diagenetic effects, rather than from a large carbon and calcium cycle disturbance. Perturbations to the global carbon and calcium cycles across the G/L transition were much less intense than the disturbances that occurred across the subsequent Permian-Triassic boundary. This finding is consistent with the much smaller magnitude of the end-Guadalupian extinction relative to the end-Permian. (C) 2014 Elsevier B.V. All rights reserved. C1 [Jost, Adam B.; Payne, Jonathan L.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Mundil, Roland] Berkeley Geochronol Ctr, Berkeley, CA 94709 USA. [He, Bin] Chinese Acad Sci, State Key Lab Isotope Geochem, Guangzhou 510640, Guangdong, Peoples R China. [Brown, Shaun T.; DePaolo, Donald J.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Brown, Shaun T.; DePaolo, Donald J.] Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Geochem, Berkeley, CA 94270 USA. [Altiner, Demir] Middle E Tech Univ, Dept Geol Engn, TR-06531 Ankara, Turkey. [Sun, Yadong] China Univ Geosci, State Key Lab Geobiol & Environm Geol, Wuhan 430074, Hubei, Peoples R China. RP Jost, AB (reprint author), Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. EM abjost@stanford.edu RI Brown, Shaun/E-9398-2015; Sun, Yadong/N-6907-2013; OI Brown, Shaun/0000-0002-2159-6718; Payne, Jonathan/0000-0002-9601-3310 FU NSF [0923669, 0923620]; NASA [NNX09AN6767]; Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This study was supported by NSF grants 0923669 (R.M.) and 0923620 (J.L.P.), and by NASA grant NNX09AN6767 S.T. Brown and DJ. DePaolo were supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank D.A. Fike and 2 anonymous reviewers for their constructive comments; S. Denyszyn and Y. Zhong for assistance in the field; and P. Blisniuk, J.L. Hinojosa, A. Jin, G. Li, D. Mucciarone, P. Srinivasan, and T. Owens for assistance in the laboratory. NR 82 TC 13 Z9 15 U1 2 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-821X EI 1385-013X J9 EARTH PLANET SC LETT JI Earth Planet. Sci. Lett. PD JUN 15 PY 2014 VL 396 BP 201 EP 212 DI 10.1016/j.epsl.2014.04.014 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AI4FA UT WOS:000336819900020 ER PT J AU Beyerlein, IJ Mayeur, JR McCabe, RJ Zheng, SJ Carpenter, JS Mara, NA AF Beyerlein, I. J. Mayeur, J. R. McCabe, R. J. Zheng, S. J. Carpenter, J. S. Mara, N. A. TI Influence of slip and twinning on the crystallographic stability of bimetal interfaces in nanocomposites under deformation SO ACTA MATERIALIA LA English DT Article DE Twinning; Nanocomposites; Interfaces; Severe plastic deformation; Crystal plasticity ID SEVERE PLASTIC-DEFORMATION; POLYCRYSTALLINE FCC METALS; GRAIN-BOUNDARY STRUCTURE; ULTRA-HIGH STRENGTH; CU-NB MULTILAYERS; ROLLING TEXTURES; NANOSTRUCTURED METALS; NANOCRYSTALLINE MATERIALS; NANOLAYERED COMPOSITES; MECHANICAL-PROPERTIES AB In this work, we examine the microstructural development of a bimetal multilayered composite over a broad range of individual layer thicknesses h from microns to nanometers during deformation. We observe two microstructural transitions, one at the submicron scale and another at the nanoscale. Remarkably, each transition is associated with the development of a preferred interface character. We show that the characteristics of these prevailing interfaces are strongly influenced by whether the adjoining crystals are deforming by slip only or by slip and twinning. We present a generalized theory that suggests that, in spite of their different origins, the crystallographic stability of their interface character with respect to deformation depends on the same few basic variables. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Beyerlein, I. J.; Mayeur, J. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zheng, S. J.; Mara, N. A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [McCabe, R. J.; Carpenter, J. S.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Beyerlein, IJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM irene@lanl.gov RI Mara, Nathan/J-4509-2014; Beyerlein, Irene/A-4676-2011; OI McCabe, Rodney /0000-0002-6684-7410; Carpenter, John/0000-0001-8821-043X FU Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; Laboratory Directed Research and Development (LDRD) [20140348ER] FX The authors gratefully acknowledge support by the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. R.J.M. and J.S.C. acknowledge support by a Laboratory Directed Research and Development (LDRD) program 20140348ER. NR 85 TC 17 Z9 17 U1 5 U2 66 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2014 VL 72 BP 137 EP 147 DI 10.1016/j.actamat.2014.03.041 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI2OD UT WOS:000336696900012 ER PT J AU Ekiz, EH Lach, TG Averback, RS Mara, NA Beyerlein, IJ Pouryazdan, M Hahn, H Bellon, P AF Ekiz, E. H. Lach, T. G. Averback, R. S. Mara, N. A. Beyerlein, I. J. Pouryazdan, M. Hahn, H. Bellon, P. TI Microstructural evolution of nanolayered Cu-Nb composites subjected to high-pressure torsion SO ACTA MATERIALIA LA English DT Article DE Copper alloys; Niobium alloys; Nanocomposite; High-pressure torsion; Severe plastic deformation ID SEVERE PLASTIC-DEFORMATION; SUPERSATURATED SOLID-SOLUTIONS; ULTRA-HIGH STRENGTH; HPT-PROCESSED CU; NANOCRYSTALLINE MATERIALS; NANOLAMELLAR COMPOSITES; TEXTURE EVOLUTION; PURE COPPER; SHEAR; AG AB Bulk nanolayered Cu/Nb composites fabricated by accumulative roll bonding (ARB), leading to a nominal layer thickness of 18 nm, were subjected to large shear deformation by high-pressure torsion at room temperature. The evolution of the microstructure was characterized using X-ray diffraction, transmission electron microscopy and atom probe tomography. At shear strains of the crystallographic texture started to change from the one stabilized by ARB, with a Kurdjumov-Sachs orientation relationship and a dominant {1 1 2}(Cu)parallel to{1 1 2}(Nb) interface plane, toward textures unlike the shear texture of monolithic Cu and Nb. At larger strains, exceeding 10, the initial layered structure was progressively replaced by a three-dimensional Cu-Nb nanocomposite. This structure remained stable with respect to grain size, morphology and global texture from strains of similar to 290 to the largest ones used in this study, 5900. The three-dimensional self-organized nanocomposites comprised biconnected Cu-rich and Nb-rich regions, with a remarkably small coexistence length scale, similar to 10 nm. The results are discussed in the context of the effect of severe plastic deformation and strain path on microstructure and texture stability in highly immiscible alloy systems. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Ekiz, E. H.; Lach, T. G.; Averback, R. S.; Bellon, P.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Mara, N. A.; Beyerlein, I. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Pouryazdan, M.; Hahn, H.] KIT, Inst Nanotechnol, D-76021 Karlsruhe, Germany. [Pouryazdan, M.; Hahn, H.] Tech Univ Darmstadt, Joint Res Lab Nanomat, D-64287 Darmstadt, Germany. RP Bellon, P (reprint author), Univ Illinois, Dept Mat Sci & Engn, 1304 West Green St, Urbana, IL 61801 USA. EM bellon@uiuc.edu RI Mara, Nathan/J-4509-2014; Hahn, Horst/G-9018-2011; Beyerlein, Irene/A-4676-2011; OI Hahn, Horst/0000-0001-9901-3861; Lach, Timothy/0000-0002-4745-4179 FU Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; NSF-MRI [DMR-0420532]; ONR-DURIP [N00014-0400798, N00014-0610539, N00014-0910781]; National Science Foundation's MRSEC program [DMR-1121262] FX This work was supported as part of the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. APT was performed at the Northwestern University Center for Atom-Probe Tomography (NUCAPT) whose local-electrode atom-probe (LEAP) tomograph was purchased and upgraded with funding from NSF-MRI (DMR-0420532) and ONR-DURIP (N00014-0400798, N00014-0610539, N00014-0910781) Grants. Instrumentation at NUCAPT was supported by the Initiative for Sustainability and Energy at Northwestern (ISEN). NUCAPT is a Shared Facility at the Materials Research Center of Northwestern University, supported by the National Science Foundation's MRSEC program (DMR-1121262. Stimulating discussions with Drs. A. Misra and J. Carpenter (LANL), and Prof. A. Rollett (CMU), are gratefully acknowledged. NR 67 TC 20 Z9 20 U1 8 U2 75 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2014 VL 72 BP 178 EP 191 DI 10.1016/j.actamat.2014.03.040 PG 14 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AI2OD UT WOS:000336696900016 ER PT J AU Stubkier, S Pedersen, HC Jonkman, JM AF Stubkier, S. Pedersen, H. C. Jonkman, J. M. TI Analysis of load reduction possibilities using a hydraulic soft yaw system for a 5-MW turbine and its sensitivity to yaw-bearing friction SO ENGINEERING STRUCTURES LA English DT Article DE Yaw system; Friction; Load reduction; Soft yaw AB With the increasing size of wind turbines and with increasing lifetime demands, new methods for load reduction in the turbines need to be examined. One method is to make the yaw system of the turbine flexible, thereby dampening the loads to the system. This paper presents a hydraulic soft yaw concept and investigates the effect this has on critical loads in the turbine. To analyze the system, a novel friction model is developed and implemented for the yaw system using the NREL 5-MW turbine in the aerodynamic code FAST. Based on this model, the influence of friction is investigated and the results on load reduction for three different design load cases are presented and discussed. From the investigation, it is found that load reductions of up to 40% on fatigue loads and 37% on ultimate loads are possible when considering the yaw system. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Stubkier, S.] Hydratech Ind, Silkeborg, Denmark. [Pedersen, H. C.] Aalborg Univ, Dept Energy Technol, Aalborg, Denmark. [Jonkman, J. M.] NREL, Golden, CO USA. RP Stubkier, S (reprint author), Hydratech Ind, Silkeborg, Denmark. EM sst@hydratech-industries.com NR 11 TC 2 Z9 2 U1 2 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-0296 EI 1873-7323 J9 ENG STRUCT JI Eng. Struct. PD JUN 15 PY 2014 VL 69 BP 123 EP 134 DI 10.1016/j.engstruct.2014.01.022 PG 12 WC Engineering, Civil SC Engineering GA AI3RR UT WOS:000336780100012 ER PT J AU Windham-Myers, L Fleck, JA Ackerman, JT Marvin-DiPasquale, M Stricker, CA Heim, WA Bachand, PAM Eagles-Smith, CA Gill, G Stephenson, M Alpers, CN AF Windham-Myers, Lisamarie Fleck, Jacob A. Ackerman, Joshua T. Marvin-DiPasquale, Mark Stricker, Craig A. Heim, Wesley A. Bachand, Philip A. M. Eagles-Smith, Collin A. Gill, Gary Stephenson, Mark Alpers, Charles N. TI Mercury cycling in agricultural and managed wetlands: A synthesis of methylmercury production, hydrologic export, and bioaccumulation from an integrated field study SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Rice; Wetlands; Microbes; Hydrology; Bioaccumulation; Mercury ID DISSOLVED ORGANIC-MATTER; INORGANIC MERCURY; YOLO BYPASS; WATER-QUALITY; ROOT-ZONE; CALIFORNIA; SEDIMENT; USA; FISH; BIOGEOCHEMISTRY AB With seasonal wetting and drying, and high biological productivity, agricultural wetlands (rice paddies) may enhance the conversion of inorganic mercury (Hg(II)) to methylmercury (MeHg), the more toxic, organic form that biomagnifies through food webs. Yet, the net balance of MeHg sources and sinks in seasonal wetland environments is poorly understood because it requires an annual, integrated assessment across biota, sediment, and water components. We examined a suite of wetlands managed for rice crops or wildlife during 2007-2008 in California's Central Valley, in an area affected by Hg contamination from historic mining practices. Hydrologic management of agricultural wetlands for rice, wild rice, or fallowed - drying for field preparation and harvest, and flooding for crop growth and post-harvest rice straw decay - led to pronounced seasonality in sediment and aqueous MeHg concentrations that were up to 95-fold higher than those measured concurrently in adjacent, non-agricultural permanently-flooded and seasonally-flooded wetlands. Flooding promoted microbial MeHg production in surface sediment of all wetlands, but extended water residence time appeared to preferentially enhance MeHg degradation and storage. When incoming MeHg loads were elevated, individual fields often served as a MeHg sink, rather than a source. Slow, horizontal flow of shallow water in the agricultural wetlands led to increased importance of vertical hydrologic fluxes, including evapoconcentration of surface water MeHg and transpiration-driven advection into the root zone, promoting temporary soil storage of MeHg. Although this hydrology limited MeHg export from wetlands, it also increased MeHg exposure to resident fish via greater in situ aqueous MeHg concentrations. Our results suggest that the combined traits of agricultural wetlands - slow-moving shallow water, manipulated flooding and drying, abundant labile plant matter, and management for wildlife - may enhance microbial methylation of Hg(II) and MeHg exposure to local biota, as well as export to downstream habitats during uncontrolled winter-flow events. Published by Elsevier B.V. C1 [Windham-Myers, Lisamarie; Marvin-DiPasquale, Mark] US Geol Survey, Western Reg Branch Reg Res, Menlo Pk, CA 94025 USA. [Fleck, Jacob A.; Alpers, Charles N.] US Geol Survey, Calif Water Sci Ctr, Sacramento, CA 95819 USA. [Ackerman, Joshua T.] US Geol Survey, Western Ecol Res Ctr, Dixon Field Stn, Dixon, CA 95620 USA. [Stricker, Craig A.] US Geol Survey, Ft Collins Sci Ctr, Denver, CO 80225 USA. [Heim, Wesley A.; Stephenson, Mark] Moss Landing Marine Labs, Moss Landing, CA 95039 USA. [Bachand, Philip A. M.] Tetra Tech, Davis, CA 95616 USA. [Eagles-Smith, Collin A.] US Geol Survey, Forest & Rangeland Ecosyst Sci Ctr, Corvallis, OR 97331 USA. [Gill, Gary] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Windham-Myers, L (reprint author), US Geol Survey, 345 Middlefield Rd,MS 480, Menlo Pk, CA 94025 USA. EM lwindham@usgs.gov; jafleck@usgs.gov; jackerman@usgs.gov; mmarvin@usgs.gov; cstricker@usgs.gov; wheim@mlml.calstate.edu; philip.bachand@tetratech.com; ceagles-smith@usgs.gov; gary.gill@pnnl.gov; mstephenson@mlml.calstate.edu; cnalpers@usgs.gov OI Alpers, Charles/0000-0001-6945-7365 FU State Water Resources Control Board FX We gratefully acknowledge the State Water Resources Control Board for financial support, the USGS Toxics Program for ongoing support, the USGS Cooperative Water Program, and the land managers of the Yolo Bypass for broad access and field support. Detailed comments from Peter van Metre (USGS), Stephen McCord (MEI), 3 anonymous reviewers and the associate editor Mae S. Gustin greatly improved the clarity of the manuscript. Especially helpful were the logistical assistance of David Feliz, Mary Schiedt and Chris Rocco (California Department of Fish and Game) and Jack DeWit (DeWit Farms). We thank Ann Brice and Robin Kulakow (Yolo Basin Foundation) for supporting outreach and bi-directional information exchange between land managers and the scientific team. We thank many USGS staff members for exemplary field and laboratory support: Elizabeth (Beaulieu) Stumpner, Frank Anderson, Will Kerlin, Jennifer Agee, Le Kieu, Evangelos Kakouros, Pilar Heredia-Middleton, Sherrie Wren, Steven Quistad, Justin Kanerva, Cayce Gulbransen, and Kathy Akstin.The use of trade or product names is for identification purposes only and does not constitute endorsement by the U.S. Government. NR 48 TC 22 Z9 22 U1 8 U2 121 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD JUN 15 PY 2014 VL 484 BP 221 EP 231 DI 10.1016/j.scitotenv.2014.01.033 PG 11 WC Environmental Sciences SC Environmental Sciences & Ecology GA AH7VO UT WOS:000336343600026 PM 24530187 ER PT J AU Fleck, JA Gill, G Bergamaschi, BA Kraus, TEC Downing, BD Alpers, CN AF Fleck, Jacob A. Gill, Gary Bergamaschi, Brian A. Kraus, Tamara E. C. Downing, Bryan D. Alpers, Charles N. TI Concurrent photolytic degradation of aqueous methylmercury and dissolved organic matter SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Methyl mercury; DOM; Photodegradation; Photodemethylation; Optical properties; Fluorescence ID FRANCISCO BAY ESTUARY; FLUORESCENCE SPECTROSCOPY; OPTICAL-PROPERTIES; HUMIC SUBSTANCES; MANAGED WETLANDS; NATURAL-WATERS; METHYL MERCURY; ULTRAVIOLET ABSORBENCY; MOLECULAR-WEIGHT; AQUATIC SYSTEMS AB Monomethyl mercury (MeHg) is a potent neurotoxin that threatens ecosystem viability and human health. In aquatic systems, the photolytic degradation of MeHg (photodemethylation) is an important component of the MeHg cycle. Dissolved organic matter (DOM) is also affected by exposure to solar radiation (light exposure) leading to changes in DOM composition that can affect its role in overall mercury (Hg) cycling. This study investigated changes in MeHg concentration, DOM concentration, and the optical signature of DOM caused by light exposure in a controlled field-based experiment using water samples collected from wetlands and rice fields. Filtered water from all sites showed a marked loss in MeHg concentration after light exposure. The rate of photodemethylation was 7.5 x 10(-3) m(2) mol(-1) (s.d. 3.5 x 10(-3)) across all sites despite marked differences in DOM concentration and composition. Light exposure also caused changes in the optical signature of the DOM despite there being no change in DOM concentration, indicating specific structures within the DOM were affected by light exposure at different rates. MeHg concentrations were related to optical signatures of labile DOM whereas the percent loss of MeHg was related to optical signatures of less labile, humic DOM. Relationships between the loss of MeHg and specific areas of the DOM optical signature indicated that aromatic and quinoid structures within the DOM were the likely contributors to MeHg degradation, perhaps within the sphere of the Hg-DOM bond. Because MeHg photodegradation rates are relatively constant across freshwater habitats with natural Hg-DOM ratios, physical characteristics such as shading and hydrologic residence time largely determine the relative importance of photolytic processes on the MeHg budget in these mixed vegetated and open-water systems. Published by Elsevier B.V. C1 [Fleck, Jacob A.; Bergamaschi, Brian A.; Kraus, Tamara E. C.; Downing, Bryan D.; Alpers, Charles N.] US Geol Survey, Calif Water Sci Ctr, Sacramento, CA 95819 USA. [Gill, Gary] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Fleck, JA (reprint author), US Geol Survey, Calif Water Sci Ctr, 6000 J St,Placer Hall, Sacramento, CA 95819 USA. EM jafleck@usgs.gov; gary.gill@pnnl.gov; bbergama@usgs.gov; tkraus@usgs.gov; bdowning@usgs.gov; cnalpers@usgs.gov OI Alpers, Charles/0000-0001-6945-7365; Downing, Bryan/0000-0002-2007-5304; Bergamaschi, Brian/0000-0002-9610-5581; Kraus, Tamara/0000-0002-5187-8644 FU California State Water Resources Control Board [Proposition 40]; USGS Cooperative Water Program FX The authors would like to thank the staff at the USGS California Water Science Center in Sacramento, particularly Frank Anderson and Liz Beaulieu for field and data support and Will Kerlin for laboratory support. We extend sincere appreciation to the California Department of Fish and Game staff at the Yolo Bypass Wildlife Management Area particularly Dave Feliz, Mary Schiedt, Waylon, Spencer, and Chris Rocco. We would also like to thank Yolo Basin Foundation staff Robin Kulako and Ann Brice and De Wit Farms staff for their cooperation and guidance on local history and rice production as well as for providing valuable information on site management. Base funding provided by Proposition 40 via California State Water Resources Control Board, additional funds provided by the USGS Cooperative Water Program. The use of brand or firm names in this article is for identification purposes only and does not constitute endorsement by United States Geological Survey. We greatly appreciate reviews by Dr. Edward Nater, Dr. Mae Gustin and several journal reviewers whose comments helped to improve this manuscript. The U.S. Geological Survey has approved this manuscript for publication. NR 107 TC 14 Z9 14 U1 10 U2 77 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD JUN 15 PY 2014 VL 484 BP 263 EP 275 DI 10.1016/j.scitotenv.2013.03.107 PG 13 WC Environmental Sciences SC Environmental Sciences & Ecology GA AH7VO UT WOS:000336343600029 PM 23642571 ER PT J AU Alton, GD Bilheux, JC Zhang, Y Liu, Y AF Alton, G. D. Bilheux, J. -C. Zhang, Y. Liu, Y. TI Molecular-flow time properties of RIB type vapor-transport systems using a fast-valve SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Fast-valve; Molecular-flow; Vapor-transport system; Monte-Carlo simulation; Radioactive ion beam ID PRODUCTION TARGET APPLICATIONS; ISOTOPE-SEPARATION ONLINE; COMPOUND MATERIALS; ION; FACILITIES; MATRICES AB The advent of the fast-valve device, described previously, permits measurement of molecular-flow times of chemically active or inactive gaseous species through radioactive ion beam (RIB) target-ion-source systems, independent of size, geometry and materials of construction. Thus, decay losses of short-half-life RIBs can be determined for a given target/vapor-transport system in advance of on-line operation, thereby ascertaining the feasibility of the system design for successful processing of a given isotope. In this article, molecular-flow-time theory and experimentally measured molecular-flow time data are given for serial- and parallel-coupled Ta metal RIB vapor-transport systems similar to those used at ISOL based RIB facilities. In addition, the effect of source type on the molecular-flow time properties of a given system is addressed, and a chemical passivation method for negating surface adsorption enthalpies for chemically active gaseous species on Ta surfaces is demonstrated. Published by Elsevier B.V. C1 [Alton, G. D.; Bilheux, J. -C.; Zhang, Y.; Liu, Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Zhang, Y.] Michigan State Univ, E Lansing, MI 48824 USA. RP Alton, GD (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM altondgd@aim.com RI Bilheux, Jean/A-2823-2016 OI Bilheux, Jean/0000-0003-2172-6487 NR 27 TC 0 Z9 0 U1 2 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD JUN 15 PY 2014 VL 329 BP 30 EP 39 DI 10.1016/j.nimb.2014.02.129 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AH9QW UT WOS:000336477900006 ER PT J AU Adams, DP Murphy, RD Saiz, DJ Hirschfeld, DA Rodriguez, MA Kotula, PG Jared, BH AF Adams, D. P. Murphy, R. D. Saiz, D. J. Hirschfeld, D. A. Rodriguez, M. A. Kotula, P. G. Jared, B. H. TI Nanosecond pulsed laser irradiation of titanium: Oxide growth and effects on underlying metal SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Laser color marking; Titanium oxide; Coating; X-ray diffraction; Transmission electron microscopy ID INDUCED OXIDATION; ASSISTED OXIDATION; STAINLESS-STEEL; OXYGEN; FILMS; MONOXIDE AB Titanium oxide/oxynitride coatings were created on the polished surface of commercially pure, grade 2 titanium substrates by irradiating samples in air using a nanosecond-pulsed, infrared (1064 nm) fiber laser. Coatings consist of three distinct layers, including a thin TiO2 rutile cap, a TiO middle layer, and an inhomogeneous bottom layer that is composed of TiOxN1-x x and possibly oxygen-intercalated phases such as Ti6O. The combined thickness of TiO2 and TiO layers was varied from similar to 10 to 120 nm by increasing the accumulated laser fluence. Lasergrown coatings exhibit different colors, which vary with oxide thickness. The observed color is attributed to the interference of incident white light reflected from the upper and lower boundaries of the TiO2 capping layer. (c) 2014 Elsevier B.V. All rights reserved. C1 [Adams, D. P.; Murphy, R. D.; Saiz, D. J.; Hirschfeld, D. A.; Rodriguez, M. A.; Kotula, P. G.; Jared, B. H.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Adams, DP (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM dpadams@sandia.gov RI Kotula, Paul/A-7657-2011 OI Kotula, Paul/0000-0002-7521-2759 FU Defense Threat Reduction Agency, Basic Research Award [IACRO 12-20261] FX The authors appreciate the assistance of V. C. Hodges and E. D. Jones, Jr. This work was supported by the Defense Threat Reduction Agency, Basic Research Award no. IACRO 12-20261, to Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract no. DE-AC04-94AL85000. NR 41 TC 6 Z9 7 U1 0 U2 32 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD JUN 15 PY 2014 VL 248 BP 38 EP 45 DI 10.1016/j.surfcoat.2013.12.052 PG 8 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA AH3IT UT WOS:000336017600005 ER PT J AU Zhong, J He, LN Li, CB Cao, YJ Wang, JH Fang, BL Zeng, L Xiao, GX AF Zhong, Jin He, Lina Li, Canbing Cao, Yijia Wang, Jianhui Fang, Baling Zeng, Long Xiao, Guoxuan TI Coordinated control for large-scale EV charging facilities and energy storage devices participating in frequency regulation SO APPLIED ENERGY LA English DT Article DE Electric vehicles (EVs); Energy storage; Frequency regulation (FR); Vehicle-to-grid (V2G); Renewable energy ID ELECTRIC-DRIVE VEHICLES; WIND POWER; RENEWABLE ENERGY; DEMAND RESPONSE; INTEGRATION; SYSTEMS; BATTERIES; OPERATION; PRICE AB With the increasing penetration of renewable energy, automatic generation control (AGC) capacity requirements will increase dramatically, becoming a challenging task that must be addressed. The rapid growth of electric vehicles (EVs) provides new approaches for the stable operation of power systems. Vehicle-to-grid (V2G) technology has the potential to provide frequency regulation (FR) services. Fully taking into account the advantages of EVs and battery energy storage stations (BESSs), i.e. rapid response and large instantaneous power, this paper presents a coordinated control strategy for large-scale EVs, BESSs and traditional FR resources involved in AGC. Response priorities and control strategies for the FR resources vary with different operating states. To verify the effectiveness of the proposed control strategy, dynamic simulations for EV/BESS to participate in AGC of a two-area interconnected power system are performed in the Matlab/Simulink program. The simulation results show that the proposed method can not only fully utilize the advantages of EV/BESS, but also achieve the coordination among different FR resources, thus improving the frequency stability and facilitating the integration of renewable energy. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Zhong, Jin] Univ Hong Kong, Dept Elect & Elect Engn, Hong Kong, Hong Kong, Peoples R China. [He, Lina; Li, Canbing; Cao, Yijia; Wang, Jianhui; Fang, Baling; Zeng, Long; Xiao, Guoxuan] Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Li, CB (reprint author), Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. EM jzhong@eee.hku.hk; licanbing@gmail.com; yjcao@hnu.edu.cn OI Li, Canbing/0000-0001-9116-7487 FU HKU University Development Funding (Initiative on Clean Energy Environment); National Science and Technology Support Program of China [2010BAE00816]; Fund of Sci-tech Innovation and Entrepreneur for Hunan Young Talents FX This work was supported in part by HKU University Development Funding (Initiative on Clean Energy & Environment), the National Science and Technology Support Program of China (2010BAE00816), and the Fund of Sci-tech Innovation and Entrepreneur for Hunan Young Talents. NR 60 TC 31 Z9 34 U1 5 U2 59 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD JUN 15 PY 2014 VL 123 SI SI BP 253 EP 262 DI 10.1016/j.apenergy.2014.02.074 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AH3IR UT WOS:000336017400025 ER PT J AU Arent, D Pless, J Mai, T Wiser, R Hand, M Baldwin, S Heath, G Macknick, J Bazilian, M Schlosser, A Denholm, P AF Arent, Doug Pless, Jacquelyn Mai, Trieu Wiser, Ryan Hand, Maureen Baldwin, Sam Heath, Garvin Macknick, Jordan Bazilian, Morgan Schlosser, Adam Denholm, Paul TI Implications of high renewable electricity penetration in the US for water use, greenhouse gas emissions, land-use, and materials supply SO APPLIED ENERGY LA English DT Article DE Renewable energy; Supply chains; Greenhouse gas emissions; Water use; Land use; Critical materials ID ENERGY-SYSTEM; LIFE-CYCLE; GENERATION AB Recent work found that renewable energy could supply 80% of electricity demand in the contiguous United States in 2050 at the hourly level. This paper explores some of the implications of achieving such high levels of renewable electricity for supply chains and the environment in scenarios with renewable supply up to such levels. Expanding the renewable electricity supply at this scale by 2050 implies annual capacity additions of roughly 20 gigawatts per year (GW/year) over the next decade, rising to roughly 40 GW/year from 2040 to 2050. Given total 2012 renewable electricity capacity additions of slightly more than 16 GW, this suggests moderate growth of the related supply chains, averaging overall roughly 4% annual growth to 2040. Transitioning to high renewable electricity supply would lead to significant reductions in greenhouse gas emissions and water use, with only modest land-use implications. While renewable energy expansion implies moderate growth of the renewable electricity supply chains, no insurmountable long-term constraints to renewable electricity technology manufacturing capacity or materials supply are identified. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Arent, Doug; Pless, Jacquelyn; Mai, Trieu; Hand, Maureen; Heath, Garvin; Macknick, Jordan; Bazilian, Morgan; Denholm, Paul] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Wiser, Ryan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Baldwin, Sam] US DOE, Off Energy Efficiency & Renewable Energy, Washington, DC 20585 USA. [Schlosser, Adam] MIT, Joint Program Sci & Policy Global Change, Ctr Global Change Sci, Cambridge, MA 02139 USA. RP Pless, J (reprint author), Natl Renewable Energy Lab, RSF300,15013 Denver West Pkwy, Golden, CO 80401 USA. EM doug.arent@nrel.gov; jacquelyn.pless@nrel.gov; trieu.mai@nrel.gov; rhwiser@lbl.gov; maureen.hand@nrel.gov; sam.baldwin@ee.doe.gov; garvin.heath@nrel.gov; jordan.macknick@nrel.gov; morgan.bazilian@nrel.gov; casch@mit.edu; paul.denholm@nrel.gov FU U.S. Department of Energy [DE-AC36-09GO28308]; National Renewable Energy Laboratory; U.S. DOE Office of Energy Efficiency and Renewable Energy FX This work was supported by the U.S. Department of Energy under contract number DE-AC36-09GO28308 with the National Renewable Energy Laboratory. Funding provided by the U.S. DOE Office of Energy Efficiency and Renewable Energy. The opinions represented in this article are the authors' own and do not reflect the view of the U.S. Department of Energy or the U.S. Government. NR 47 TC 28 Z9 28 U1 3 U2 28 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD JUN 15 PY 2014 VL 123 SI SI BP 368 EP 377 DI 10.1016/j.apenergy.2013.12.022 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AH3IR UT WOS:000336017400037 ER PT J AU Katsiev, K Losovyj, Y Lozova, N Wang, L Mei, WN Zheng, JX Vescovo, E Liu, L Dowben, PA Goodman, DW AF Katsiev, K. Losovyj, Y. Lozova, N. Wang, Lu Mei, Wai-Ning Zheng, Jiaxin Vescovo, E. Liu, Li Dowben, P. A. Goodman, D. W. TI The band structure of carbonmonoxide on 2-D Au islands on graphene SO APPLIED SURFACE SCIENCE LA English DT Article; Proceedings Paper CT 6th International Workshops on Surface Physics (IWSP) CY SEP 01-06, 2013 CL Niemcza, POLAND DE CO on Au; CO band structure; Au adsorption; Graphene; CO catalysis; Density functional theory ID ELECTRONIC-STRUCTURE; GOLD NANOPARTICLES; CATALYTIC-ACTIVITY; CO OXIDATION; SURFACES; PHOTOEMISSION; SPECTROSCOPY; CLUSTERS; RU(0001); GROWTH AB The dispersion of the occupied molecular orbitals of carbon monoxide adsorbed on Au 2D islands, vapordeposited on graphene/Ru(0 0 0 1), is seen to be wave vector dependent, as revealed by angle-resolved photoemission. The band dispersion is similar to CO monolayers adsorbed on many single crystal metal surfaces. Thus not only are the adsorbed gold islands on graphene flat and crystalline, as evident in the dispersion of the Au d-states, but the CO molecular adlayer is both molecular and ordered as well. The experimental angle-resolved photoemission combined with model calculations of the occupied CO band structure, suggest that, in spite of being a very weakly bound adsorbate, the CO adlayer on Au 2D islands on graphene is strongly hybridized to the Au layer. (C) 2014 Elsevier B.V. All rights reserved. C1 [Katsiev, K.; Liu, Li; Goodman, D. W.] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA. [Losovyj, Y.; Lozova, N.] Louisiana State Univ, J Bennett Johnston Sr Ctr Adv Microstruct & Devic, Baton Rouge, LA 70806 USA. [Wang, Lu; Mei, Wai-Ning; Zheng, Jiaxin] Univ Nebraska, Dept Phys, Omaha, NE 68182 USA. [Zheng, Jiaxin] Peking Univ, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China. [Zheng, Jiaxin] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Vescovo, E.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Dowben, P. A.] Univ Nebraska, Dept Phys & Astron, Nebraska Ctr Nanostruct & Mat, Lincoln, NE 68588 USA. RP Losovyj, Y (reprint author), Indiana Univ, Dept Chem, A421C,800 E Kirkwood Ave, Bloomington, IN 47405 USA. EM ylozovyy@indiana.edu RI Liu, Li/E-8959-2013; OI Liu, Li/0000-0002-4852-1580; Dowben, Peter/0000-0002-2198-4710 NR 49 TC 1 Z9 1 U1 2 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD JUN 15 PY 2014 VL 304 BP 35 EP 39 DI 10.1016/j.apsusc.2014.01.089 PG 5 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AH1TM UT WOS:000335904000007 ER PT J AU Wang, N Rokkam, S Hochrainer, T Pernice, M El-Azab, A AF Wang, Nan Rokkam, Srujan Hochrainer, Thomas Pernice, Michael El-Azab, Anter TI Asymptotic and uncertainty analyses of a phase field model for void formation under irradiation SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Phase field modeling; Void formation; Irradiation effects; Uncertainty quantification; Asymptotic analysis ID MICROSTRUCTURE EVOLUTION; COPPER; ENERGY; TEMPERATURE; SIMULATIONS; EQUATIONS; METALS; SILVER; CHAOS; GOLD AB We perform asymptotic analysis and uncertainty quantification of a phase field model for void formation and evolution in materials subject to irradiation. The parameters of the phase field model are obtained in terms of the underlying material specific quantities by matching the sharp interface limit of the phase field model with the corresponding sharp interface theory for void growth. To evaluate the sensitivity of phase field simulations to uncertainties in input parameters we quantify the predictions using the stochastic collocation method. Uncertainties arising from material parameters are investigated based on available experimental and atomic scale data. The results of our analysis suggest that the uncertainty in the formation and migration energies of vacancies are found to have a strong influence on the void volume fraction (or porosity). In contrast, the uncertainty resulting from the void surface energy has minimal affect. The analysis also shows that the model is consistent in the sense that its predictions do not drastically change as a result of small variations of the model input parameters. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, Nan; El-Azab, Anter] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. [Rokkam, Srujan; Hochrainer, Thomas] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. [Pernice, Michael] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP El-Azab, A (reprint author), Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. EM aelazab@purdue.edu RI Rokkam, Srujan/E-7061-2010; OI Hochrainer, Thomas/0000-0003-0501-7306 FU Laboratory Directed Research and Development at Idaho National Laboratory; U.S. Department of Energy, Office of Sciences, Office of Basic Energy Sciences through at Purdue University [FWP 1356, 00122223] FX This work is supported in part by the Laboratory Directed Research and Development funding at Idaho National Laboratory. The phase field model was developed as part of the Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Sciences, Office of Basic Energy Sciences under award number FWP 1356, through subcontract number 00122223 at Purdue University. NR 35 TC 1 Z9 1 U1 1 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD JUN 15 PY 2014 VL 89 BP 165 EP 175 DI 10.1016/j.commatsci.2014.03.045 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA AH1SD UT WOS:000335900300023 ER PT J AU Lee, N Foustoukos, DI Sverjensky, DA Cody, GD Hazen, RM AF Lee, Namhey Foustoukos, Dionysis I. Sverjensky, Dimitri A. Cody, George D. Hazen, Robert M. TI The effects of temperature, pH and redox state on the stability of glutamic acid in hydrothermal fluids SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID MOLAL THERMODYNAMIC PROPERTIES; MOLECULAR-WEIGHT HYDROCARBONS; THERMAL REACTION KINETICS; MID-ATLANTIC RIDGE; AMINO-ACIDS; ASPARTIC-ACID; METASTABLE EQUILIBRIUM; AQUEOUS-SOLUTIONS; ORGANIC-COMPOUNDS; HEAT-CAPACITIES AB Natural hydrothermal vent environments cover a wide range of physicochemical conditions involving temperature, pH and redox state. The stability of simple biomolecules such as amino acids in such environments is of interest in various fields of study from the origin of life to the metabolism of microbes at the present day. Numerous previous experimental studies have suggested that amino acids are unstable under hydrothermal conditions and decompose rapidly. However, previous studies have not effectively controlled the redox state of the hydrothermal fluids. Here we studied the stability of glutamate with and without reducing hydrothermal conditions imposed by 13 mM aqueous H-2 at temperatures of 150, 200 and 250 degrees C and initial (25 degrees C) pH values of 6 and 10 in a flow-through hydrothermal reactor with reaction times from 3 to 36 min. We combined the experimental measurements with theoretical calculations to model the in situ aqueous speciation and pH values. As previously observed under hydrothermal conditions, the main reaction involves glutamate cyclizing to pyroglutamate through a simple dehydration reaction. However, the amounts of decomposition products of the glutamate detected, including succinate, formate, carbon dioxide and ammonia depend on the temperature, the pH and particularly the redox state of the fluid. In the absence of dissolved H-2, glutamate decomposes in the sequence glutamate, glutaconate, alpha-hydroxyglutarate, ketoglutarate, formate and succinate, and ultimately to CO2 and micromolar quantities of H-2(aq). Model speciation calculations indicate the CO2, formate and H-2(aq) are not in metastable thermodynamic equilibrium. However, with 13 mM H-2(aq) concentrations, the amounts of decomposition products are suppressed at all temperatures and pH values investigated. The small amounts of CO2 and formate present are calculated to be in metastable equilibrium with the H-2. It is further proposed that there is a metastable equilibrium between glutamate, glutaconate, alpha-hydroxyglutarate, ketoglutarate and H-2. The key redox-sensitive step is the reaction of alpha-hydroxyglutarate to alpha-ketoglutarate, which is effectively inhibited by the elevated H-2 concentrations, which in turn dramatically lowers the amounts of all decomposition products including ammonia. Theoretical calculations of the metastable thermodynamic equilibrium between glutamate and ketoglutarate are consistent with the experimentally determined effects of reducing conditions. These findings establish that redox state is as important a variable as temperature and pH in affecting the stability of amino acids under hydrothermal conditions. It is suggested that when natural hydrothermal fluids contain enough dissolved H-2, the stability of amino acids may be enhanced in fluids at least on short time scales. In turn, this result suggests that reducing hydrothermal environments may have been favorable for assembling the building blocks of biomolecules in the origin of life. Furthermore, in present day hydrothermal vents the microbial ecosystems may in part be supported by the availability of metastable amino acids through heterotrophic metabolism. Published by Elsevier Ltd. C1 [Lee, Namhey; Sverjensky, Dimitri A.] Johns Hopkins Univ, Dept Earth & Planetary Sci, Baltimore, MD 21218 USA. [Lee, Namhey; Foustoukos, Dionysis I.; Sverjensky, Dimitri A.; Cody, George D.; Hazen, Robert M.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. RP Lee, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. EM nlee@lbl.gov RI Sverjensky, Dimitri/A-4612-2017 FU NSF [OCE-0928443, OCE-1038114, EAR-1023865, EAR-1023889]; DOE [DE-FG02-96ER-14616]; NASA Astrobiology Institute; Carnegie Institution of Washington FX The authors greatly appreciate discussions with and assistance in the laboratory from M. L. Fogel, I. Perez-Rodriguez, C. F. Estrada, K. Klochko and S. Ohara. In addition, N. Lee acknowledges inspirational advice from Bjorn Mysen in initiating this study. N. Lee and D. A. Sverjensky greatly appreciate the support of R. J. Hemley during their stay as visiting researchers at the Geophysical Laboratory. This research was conducted with support from the NSF OCE-0928443 (D.F.), NSF OCE-1038114 (D.F.), NSF EAR-1023865 (D.A.S.), DOE DE-FG02-96ER-14616 (D.A.S.), NSF EAR-1023889 (R.M.H.), NASA Astrobiology Institute, and the Carnegie Institution of Washington. NR 62 TC 5 Z9 5 U1 0 U2 32 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUN 15 PY 2014 VL 135 BP 66 EP 86 DI 10.1016/j.gca.2014.02.043 PG 21 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AG8GN UT WOS:000335656900004 ER PT J AU Boyd, V Yoon, H Zhang, CY Oostrom, M Hess, N Fouke, B Valocchi, AJ Werth, CJ AF Boyd, Victoria Yoon, Hongkyu Zhang, Changyong Oostrom, Mart Hess, Nancy Fouke, Bruce Valocchi, Albert J. Werth, Charles J. TI Influence of Mg2+ on CaCO3 precipitation during subsurface reactive transport in a homogeneous silicon-etched pore network SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID CALCIUM-CARBONATE PRECIPITATION; TRANSVERSE MIXING ZONE; GROUNDWATER COMPOSITION; CRYSTAL-GROWTH; POROUS-MEDIUM; MODEL; SCALE; MAGNESIUM; ARAGONITE; CRYSTALLIZATION AB Calcium carbonate (CaCO3) geochemical reactions exert a fundamental control on the evolution of porosity and permeability in shallow-to-deep subsurface siliciclastic and limestone rock reservoirs. As a result, these carbonate water-rock interactions play a critically important role in research on groundwater remediation, geological carbon sequestration, and hydrocarbon exploration. A study was undertaken to determine the effects of Mg2+ concentration on CaCO3 crystal morphology, precipitation rate, and porosity occlusion under flow and mixing conditions similar to those in subsurface aquifers. This was accomplished by promoting CaCO3 precipitation through the mixing of two solutions flowing parallel to each other in a microfluidic pore structure, containing uniform concentrations of dissolved Ca2+ and carbonate (CO32 ), and systematic variations in the concentration of Mg2+. Raman spectroscopy indicates that all three polymorphs of CaCO3 (calcite, aragonite, and vaterite) were present under all experimental conditions. Coordinated brightfield imaging results show the morphology of calcite with increasing Mg2+ progressed from blocky and dogtooth approximately 10-80 mu m in size, to anhedral spheroidal approximately 5-30 mu m in size. The morphology of aragonite with increasing Mg2+ progressed from shrubs and fuzzy dumbells to spheroidal, and the size increased from approximately 5-60 mu m to 20-200 mu m. Recrystallization was observed in all experiments, but more so at low Mg2+, in which many small microcrystals dissolved and re-precipitated as one or a few larger calcite crystals. Analysis of brightfield images indicates calcite is the most abundant polymorph under all conditions. However, the area of pore space with aragonite increased from < 5% when no Mg2+ was present to > 20% at the highest Mg2+ concentration. The initial apparent precipitation rate of mineral polymorphs with no Mg2+ present was 2.5 times greater than when 40 mM Mg2+ was added, and large (20-00 mu m) aragonite crystals formed primarily near to and below the center mixing zone with increasing Mg2+ concentration. Pore-scale modeling results are consistent with experiments, and indicate that all three polymorphs are thermodynamically favorable, with calcite and aragonite being the most favorable and having similar saturation ratios (SR > 100). The influence of Mg2+ on mineral precipitation rates is consistent with previous studies showing that calcite precipitation rates decrease with increasing Mg2+ concentrations. The precipitation of aragonite below the center-mixing zone is not predicted by thermodynamic SRs, but is consistent with the literature and our modeling results showing aragonite precipitation is kinetically more favorable in regions with higher Mg2+/Ca2+ ratios. Hence, both thermodynamic and kinetic constraints affect precipitation rates, the distribution of mineral polymorphs, and the corresponding extent of porosity occlusion. A tracer study demonstrated that mineral precipitation along the center-mixing zone under all experimental conditions led to substantial pore blockage. Imaging results suggest that with increasing Mg2+ concentration, slower crystal growth rates will increase the time period before pore blockage occurs, and the transition to more spherical and larger aragonite crystals below the center mixing line will increase pore occlusion and decrease mixing. Hence, understanding how Mg2+ affects calcium carbonate precipitation is very important for predicting mixing and reactive transport in subsurface reservoirs. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Boyd, Victoria; Valocchi, Albert J.; Werth, Charles J.] Univ Illinois, Dept Civil & Environm Engn, Newmark Lab, Urbana, IL 61801 USA. [Yoon, Hongkyu] Sandia Natl Labs, Geomech Dept, Albuquerque, NM 87123 USA. [Zhang, Changyong] Exxon Mobil Upstream Res Co, Houston, TX USA. [Oostrom, Mart; Hess, Nancy] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Fouke, Bruce] Univ Illinois, Dept Geol, Inst Genom Biol, Urbana, IL 61801 USA. RP Werth, CJ (reprint author), 205 North Mathews Ave, Urbana, IL 61801 USA. EM vhboyd2@illinois.edu; hyoon@sandia.gov; changyong.zhang@exxonmobil.com; mart.oostrom@pnnl.gov; nancy.hess@pnnl.gov; fouke@illinois.edu; valocchi@illinois.edu; werth@illinois.edu RI Zhang, Changyong/A-8012-2013; OI Hess, Nancy/0000-0002-8930-9500 FU U.S. Department of Energy LDRD [82552-001-10]; Los Alamos National laboratory; Office of Science (BER); U.S. Department of Energy (DOE) [DEFG02- 06ER64207]; Pacific Northwest National Laboratory Directed Research and Development Program under PNNL's Carbon Sequestration Initiative,; National Aeronautics and Space Administration (NASA) through the NASA Astrobiology Institute [NNA13AA91A]; Energy Biosciences Institute (EBI); University of Illinois Urbana-Champaign (UIUC); United States Department of Energy (DOE); Center for Frontiers of Subsurface Energy Security; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This paper was primarily supported by the U.S. Department of Energy LDRD 82552-001-10 sponsored by the Los Alamos National laboratory, and partially supported by the Office of Science (BER), U.S. Department of Energy (DOE), Grant No. DEFG02- 06ER64207, by the Pacific Northwest National Laboratory Directed Research and Development Program under PNNL ' s Carbon Sequestration Initiative, by the National Aeronautics and Space Administration (NASA) through the NASA Astrobiology Institute under Cooperative Agreement No. NNA13AA91A, and by the Energy Biosciences Institute (EBI) at the University of Illinois Urbana-Champaign (UIUC). A portion of the experiments were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory, a United States Department of Energy (DOE) scientific user facility operated for the DOE by PNNL. H.Y. was supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001114. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy ' s National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 71 TC 7 Z9 7 U1 4 U2 73 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUN 15 PY 2014 VL 135 BP 321 EP 335 DI 10.1016/j.gca.2014.03.018 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AG8GN UT WOS:000335656900017 ER PT J AU Zhang, F McBrearty, I Ott, RT Park, E Mendelev, MI Kramer, MJ Wang, CZ Ho, KM AF Zhang, Feng McBrearty, Ian Ott, R. T. Park, E. Mendelev, Mikhail I. Kramer, M. J. Wang, Cai-Zhuang Ho, Kai-Ming TI Discovery of a meta-stable Al-Sm phase with unknown stoichiometry using a genetic algorithm SO SCRIPTA MATERIALIA LA English DT Article DE Bulk metallic glass; Melt spinning; X-ray diffraction; First-principles calculation; Genetic algorithm ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; ALLOYS; TRANSITION; ALUMINUM AB Unknown crystalline phases observed during the devitrification process of glassy metal alloys significantly limit our ability to understand and control phase selection in these systems driven far from equilibrium. Here, we report a new meta-stable Al5Sm phase identified by simultaneously searching Al-rich compositions of the Al-Sm system, using an efficient genetic algorithm. The excellent match between calculated and experimental X-ray diffraction patterns confirms that this new phase appeared in the crystallization of melt-spun Al90Sm10 alloys. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Zhang, Feng; McBrearty, Ian; Ott, R. T.; Park, E.; Mendelev, Mikhail I.; Kramer, M. J.; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Zhang, F (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM fzhang@ameslab.gov FU US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; National Energy Research Supercomputing Center (NERSC) in Berkeley; Argonne National Laboratory [DE-AC02-06CH11357] FX Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. The high-energy X-ray experiments were performed at the XOR beamline (sector 1) of the Advanced Photon Source, Argonne National Laboratory, under Grant No. DE-AC02-06CH11357. We would like to thank Jon Almer for his assistance in setting up these experiments. NR 18 TC 2 Z9 2 U1 5 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD JUN 15 PY 2014 VL 81 BP 32 EP 35 DI 10.1016/j.scriptamat.2014.02.019 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AG7TY UT WOS:000335622900009 ER PT J AU Kim, S Fornasiero, F Park, HG Bin In, J Meshot, E Giraldo, G Stadermann, M Fireman, M Shan, J Grigoropoulos, CP Bakajin, O AF Kim, Sangil Fornasiero, Francesco Park, Hyung Gyu Bin In, Jung Meshot, Eric Giraldo, Gabriel Stadermann, Michael Fireman, Micha Shan, Jerry Grigoropoulos, Costas P. Bakajin, Olgica TI Fabrication of flexible, aligned carbon nanotube/polymer composite membranes by in-situ polymerization SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE Carbon nanotubes; Nanocomposites; Membrane; Separations; Nanofluidics ID NANOCOMPOSITE MEMBRANES; MASS-TRANSPORT; GAS-TRANSPORT; NANOTUBES; DIFFUSION; DENSITY; FILMS; FLOW; SUPPORTS; SILICA AB Vertically aligned (VA) carbon nanotubes (CNTs) have shown orders of magnitude enhancement for gas and liquid flow compared to conventional mass transport theories. Flexible, large surface-area VACNT membranes may provide a cost-efficient solution to various separation processes such as water purification and gas separation. However, all the VACNT membranes produced so far suffer from rather small membrane area. long fabrication process, poor mechanical stability, local agglomeration of CNIs, and low CNT packing density. Here, we present flexible, VACNT/polymer composite membranes having relatively densely packed CNTs as the only mass transport paths. In order to prevent CNT condensation that could disturb CNT orientation during liquid phase processing, we developed a novel in-situ bulk polymerization method to prepare VACNT/polymer composite films. A VACNT array was infiltrated with styrene monomer with a certain amount of polystyrene-polybutadiene (PS-PB) copolymer that acts as a plasticizer. Indeed, micro-indentation measurements confirmed that the addition PS-b-PB copolymer into the matrix improved the elongation at break of the CNT/PS composite film. SEM images showed that well aligned CNTs were embedded in a high-density polymer matrix free of any macroscopic voids or structural defects. Measured fluid rates and selectivity for gas and liquid mixtures are consistent with CNT membranes produced with different methods. These CNTs/polymer composite membranes showed high gas and water permeability comparable to the other VACNT composite membranes, potentially enabling applications that may require membranes with high flux, flexibility and durability. (C) 2014 Elsevier B.V. All rights reserved. C1 [Kim, Sangil; Fornasiero, Francesco; Meshot, Eric; Stadermann, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Park, Hyung Gyu] ETH, Dept Mech & Proc Engn, CH-8092 Zurich, Switzerland. [Bin In, Jung; Grigoropoulos, Costas P.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Giraldo, Gabriel; Shan, Jerry] Rutgers State Univ, Dept Mech & Aerosp Engn, Piscataway, NJ 08854 USA. [Fireman, Micha; Bakajin, Olgica] Porifera Inc, Hayward, CA 94545 USA. RP Kim, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kim55@llnl.gov RI Fornasiero, Francesco/I-3802-2012; Park, Hyung Gyu/F-3056-2013 OI Park, Hyung Gyu/0000-0001-8121-2344 FU NSF NIRT [CBET-0709090]; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; Swiss National Science Foundation [200021-137964] FX This work was partially supported by NSF NIRT CBET-0709090. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. C. Grigoropoulos, O. Bakajin, and S. Kim acknowledge support by NSF NIRT CBET-0709090. H.G. Park acknowledges support by Swiss National Science Foundation (Contract no. 200021-137964). NR 38 TC 20 Z9 25 U1 17 U2 133 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 EI 1873-3123 J9 J MEMBRANE SCI JI J. Membr. Sci. PD JUN 15 PY 2014 VL 460 BP 91 EP 98 DI 10.1016/j.memsci.2014.02.016 PG 8 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA AE8YC UT WOS:000334287900010 ER PT J AU Tselev, A Ivanov, IN Lavrik, NV Belianinov, A Jesse, S Mathews, JP Mitchell, GD Kalinin, SV AF Tselev, Alexander Ivanov, Ilia N. Lavrik, Nickolay V. Belianinov, Alexei Jesse, Stephen Mathews, Jonathan P. Mitchell, Gareth D. Kalinin, Sergei V. TI Mapping internal structure of coal by confocal micro-Raman spectroscopy and scanning microwave microscopy SO FUEL LA English DT Article DE Macerals mapping; Sub-100-nm spatial resolution; Confocal micro-Raman spectroscopy; Bayesian analysis; Scanning near-field microwave microscopy ID ARGONNE PREMIUM COALS; VICTORIAN BROWN-COAL; DIELECTRIC-PROPERTIES; ELECTRON-MICROPROBE; PYROLYSIS; RANK; REACTIVITY; EVOLUTION; MACERALS; FUSINITE AB Structural complexity and variability of the chemical properties define technological applicability of coal and demand increasing accuracy and spatial resolution from the techniques used for coal characterization for development of new, clean, and efficient technologies of coal utilization. Here, we combined spatially-resolved reflectometry, fluorescence, and confocal micro-Raman spectroscopy with high-resolution scanning probe microwave imaging to achieve a nondestructive sub-100-nm spatial resolution mapping of coal structure. It was found that this approach allows for high spatial resolution identification of individual elements in coal architecture, thus potentially generating valuable input for knowledge-driven optimization and design of coal utilization processes. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Tselev, Alexander; Ivanov, Ilia N.; Lavrik, Nickolay V.; Belianinov, Alexei; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Mathews, Jonathan P.] Penn State Univ, Leone Family Dept Energy & Mineral Engn, EMS Energy Inst, University Pk, PA 16802 USA. [Mitchell, Gareth D.] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. RP Tselev, A (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM tseleva@ornl.gov RI ivanov, ilia/D-3402-2015; Tselev, Alexander/L-8579-2015; Lavrik, Nickolay/B-5268-2011; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; OI ivanov, ilia/0000-0002-6726-2502; Tselev, Alexander/0000-0002-0098-6696; Lavrik, Nickolay/0000-0002-9543-5634; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Belianinov, Alex/0000-0002-3975-4112 FU Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, US. Department of Energy; Leone Family Department of Energy and Mineral Engineering,; EMS Energy Institute; Pennsylvania State University, PA FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US. Department of Energy, as well as Leone Family Department of Energy and Mineral Engineering, and the EMS Energy Institute, The Pennsylvania State University, PA. NR 39 TC 13 Z9 14 U1 6 U2 57 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0016-2361 EI 1873-7153 J9 FUEL JI Fuel PD JUN 15 PY 2014 VL 126 BP 32 EP 37 DI 10.1016/j.fuel.2014.02.029 PG 6 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AE4UB UT WOS:000333978500005 ER PT J AU Hanson, JC Si, R Xu, W Senanayake, SD Mudiyanselage, K Stacchiola, D Rodriguez, JA Zhao, H Beyer, KA Jennings, G Chapman, KW Chupas, PJ Martinez-Arias, A AF Hanson, J. C. Si, R. Xu, W. Senanayake, S. D. Mudiyanselage, K. Stacchiola, D. Rodriguez, J. A. Zhao, H. Beyer, K. A. Jennings, G. Chapman, K. W. Chupas, P. J. Martinez-Arias, A. TI Pulsed-reactant in situ studies of ceria/CuO catalysts using simultaneous XRD, PDF and DRIFTS measurements SO CATALYSIS TODAY LA English DT Article DE In situ XRD; Combined DRIFTS/XRD; Catalyst; Cu/ceria; Pair distribution function ID CO; OPERANDO; CONFIGURATIONS; SPECTROSCOPY; DIFFRACTION; CU/CEO2 AB The transient reduction-oxidation (redox) response of a ceria/CuO catalyst has been studied with pulsed gas techniques. The experimental setup allowed for simultaneous measurement of X-ray diffraction (XRD) and diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) coupled to mass spectrometric (MS) analysis of reactants and products. The DRIFTS showed the bonding of CO to CuxO and formation of carbonates on ceria. The CO stretch signal was observed in the DRIFTS as the Cu2O phase appeared in the simultaneous XRD pattern. This signal was still observed when XRD indicated that the Cu2O phase had converted to Cu(0). This unexpected result could arise from an amorphous surface of Cu2O which could not be detected by XRD or because the surface sensitivity of the DRIFTS technique is much higher than the surface sensitivity of the XRD technique. Time-resolved pair distribution function (PDF) analysis was useful for tracking the appearance or disappearance of key structural features (Cu-O, Ce-O, Ce-Ce, and Cu-Cu) during the pulse experiments. The in situ PDF analysis provided new evidence that oxygen vacancies in the ceria could be detected with XRD data. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hanson, J. C.; Si, R.; Xu, W.; Senanayake, S. D.; Mudiyanselage, K.; Stacchiola, D.; Rodriguez, J. A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Zhao, H.; Beyer, K. A.; Jennings, G.; Chapman, K. W.; Chupas, P. J.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Martinez-Arias, A.] CSIC, Inst Catalisis & Petroleoquim, Madrid, Spain. RP Hanson, JC (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM hanson1@bnl.gov RI Stacchiola, Dario/B-1918-2009; Senanayake, Sanjaya/D-4769-2009; COST, CM1104/I-8057-2015; Mudiyanselage, Kumudu/B-2277-2013 OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232; Mudiyanselage, Kumudu/0000-0002-3539-632X FU US Department of Energy (Div. of Materials and Chemical Sciences); Ministerio de Economia y Competitividad [CTQ2012-32928, EU COST CMT104]; BNL under DOE [DE-AC02-98CH10886]; U.S. DOE [DE-AC02-06CH11357] FX The NSLS and APS synchrotrons at Brookhaven National Laboratory are supported by the US Department of Energy (Div. of Materials and Chemical Sciences). Thanks are due to Mr. A. Lopez Camara from the ICP-CSIC (Spain) for preparation of the sample. Financial support from Ministerio de Economia y Competitividad (project CTQ2012-32928 and EU COST CMT104) is acknowledged. The work at BNL was supported under DOE contract DE-AC02-98CH10886. Work done at Argonne and use of the Advanced Photon Source (APS), an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory, were supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 18 TC 15 Z9 15 U1 11 U2 108 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD JUN 15 PY 2014 VL 229 BP 64 EP 71 DI 10.1016/j.cattod.2013.10.087 PG 8 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA AD7NE UT WOS:000333450100008 ER PT J AU Godfrey, BB Vay, JL AF Godfrey, Brendan B. Vay, Jean-Luc TI Suppressing the numerical Cherenkov instability in FDTD PIC codes SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Particle-in-cell; Finite difference time domain; Relativistic beam; Numerical stability ID NONSTANDARD FINITE-DIFFERENCES; PARTICLE CODES; ALGORITHM; SIMULATIONS; PLASMA; ACCELERATOR; STABILITY; BEAMS C1 [Godfrey, Brendan B.] Univ Maryland, College Pk, MD 20742 USA. [Godfrey, Brendan B.; Vay, Jean-Luc] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Godfrey, BB (reprint author), Univ Maryland, College Pk, MD 20742 USA. EM brendan.godfrey@ieee.org OI Godfrey, Brendan/0000-0003-2311-7060 FU Office of Science, Office of High Energy Physics, U.S. Dept. of Energy [DE-AC02-05CH11231]; US-DOE SciDAC ComPASS collaboration; United States Government FX We wish to thank Irving Haber for suggesting this collaboration and for helpful recommendations. We also are indebted to David Grote for assistance in using the code WARP. This work was supported in part by the Director, Office of Science, Office of High Energy Physics, U.S. Dept. of Energy under Contract No. DE-AC02-05CH11231 and the US-DOE SciDAC ComPASS collaboration, and used resources of the National Energy Research Scientific Computing Center.; This document was prepared as an account of work sponsored in part by the United States Government. While this document is believed to contain correct information, neither the United States Government nor any agency thereof, nor The Regents of the University of California, nor any of their employees, nor the authors makes any warranty, express or implied, or assumes any legal responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by its trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof, or The Regents of the University of California. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof or The Regents of the University of California. NR 27 TC 16 Z9 16 U1 1 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2014 VL 267 BP 1 EP 6 DI 10.1016/j.jcp.2014.02.022 PG 6 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AE1VS UT WOS:000333759800001 ER PT J AU Yao, J AF Yao, Jin TI An easy method to accelerate an iterative algebraic equation solver SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Nonlinear; Root-finding; Iterative AB This article proposes to add a single function calls to an iterative algebraic equation solver with an order n convergence rate, and to raise (for n > 1) the order of convergence to 2n - 1. (C) 2014 Elsevier Inc. All rights reserved. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Yao, J (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 6 TC 0 Z9 0 U1 0 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2014 VL 267 BP 139 EP 145 DI 10.1016/j.jcp.2014.02.027 PG 7 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AE1VS UT WOS:000333759800008 ER PT J AU Guba, O Taylor, M St-Cyr, A AF Guba, Oksana Taylor, Mark St-Cyr, Amik TI Optimization-based limiters for the spectral element method SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Spectral element method; Finite element method; Limiters; Monotone; Local extrema diminishing; Mimetic; High order ID 2-DIMENSIONAL LINEAR TRANSPORT; SHALLOW-WATER MODEL; TEST-CASE SUITE; DYNAMICAL CORE; ATMOSPHERIC MODEL; FINITE-ELEMENTS; CUBED SPHERE; SCHEMES; SIMULATIONS; POSITIVITY AB We introduce a new family of optimization based limiters for the h-p spectral element method. The native spectral element advection operator is oscillatory, but due to its mimetic properties it is locally conservative and has a monotone property with respect to element averages. We exploit this property to construct locally conservative quasimonotone and sign-preserving limiters. The quasimonotone limiter prevents all overshoots and undershoots at the element level, but is not strictly non-oscillatory. It also maintains quasimonotonicity even with the addition of a dissipation term such as viscosity or hyperviscosity. The limiters are based on a least-squares formulation with equality and inequality constraints and are local to each element. We evaluate the new limiters using a deformational flow test case for advection on the surface of the sphere. We focus on mesh refinement for moderate (p = 3) and high order (p = 6) elements. As expected, the spectral element method obtains its formal order of accuracy for smooth problems without limiters. For advection of fields with cusps and discontinuities, the high order convergence is lost, but in all cases, p = 6 outperforms p = 3 for the same degrees of freedom. (C) 2014 Elsevier Inc. All rights reserved. C1 [Guba, Oksana] Univ New Mexico, Albuquerque, NM 87131 USA. [Taylor, Mark] Sandia Natl Labs, Albuquerque, NM 87185 USA. [St-Cyr, Amik] NCAR, Boulder, CO 80305 USA. RP Guba, O (reprint author), Univ New Mexico, MSC01 1115, Albuquerque, NM 87131 USA. EM oksana@unm.edu; mataylo@sandia.gov; Amik.St-Cyr@shell.com FU Department of Energy Biological and Environmental Research [06-013194, 09-014487]; National Science Foundation [OCI-0904599] FX We would like to thank anonymous reviewers for their very helpful comments that have significantly improved this manuscript. We are grateful for challenging us to extend the proof of bounds preservation to hold in the presence of dissipation and hyperviscosity. O.G. and M.T. were supported by the Department of Energy Biological and Environmental Research Grants 06-013194 and 09-014487. A.S. was supported by the National Science Foundation Grant OCI-0904599. NR 43 TC 9 Z9 9 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2014 VL 267 BP 176 EP 195 DI 10.1016/j.jcp.2014.02.029 PG 20 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AE1VS UT WOS:000333759800011 ER PT J AU Waltz, J Canfield, TR Morgan, NR Risinger, LD Wohlbier, JG AF Waltz, J. Canfield, T. R. Morgan, N. R. Risinger, L. D. Wohlbier, J. G. TI Manufactured solutions for the three-dimensional Euler equations with relevance to Inertial Confinement Fusion SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE ICF modeling; Hydrodynamics; Method of manufactured solutions ID UNSTRUCTURED GRIDS; VERIFICATION; HYDRODYNAMICS; CODES AB We present a set of manufactured solutions for the three-dimensional (3D) Euler equations. The purpose of these solutions is to allow for code verification against true 3D flows with physical relevance, as opposed to 3D simulations of lower-dimensional problems or manufactured solutions that lack physical relevance. Of particular interest are solutions with relevance to Inertial Confinement Fusion (ICF) capsules. While ICF capsules are designed for spherical symmetry, they are hypothesized to become highly 3D at late time due to phenomena such as Rayleigh-Taylor instability, drive asymmetry, and vortex decay. ICF capsules also involve highly nonlinear coupling between the fluid dynamics and other physics, such as radiation transport and thermonuclear fusion. The manufactured solutions we present are specifically designed to test the terms and couplings in the Euler equations that are relevant to these phenomena. Example numerical results generated with a 3D Finite Element hydrodynamics code are presented, including mesh convergence studies. (C) 2014 Elsevier Inc. All rights reserved. C1 [Waltz, J.; Morgan, N. R.] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. [Canfield, T. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Risinger, L. D.; Wohlbier, J. G.] Los Alamos Natl Lab, Computat & Comp Sci Div, Los Alamos, NM USA. RP Waltz, J (reprint author), Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. EM jwaltz@lanl.gov FU U.S. Department of Energy through the LANL LDRD Program [DE-AC52-06NA25396, LA-UR-13-20185] FX This work was supported by the U.S. Department of Energy through the LANL LDRD Program (grant No. DE-AC52-06NA25396). LANL Report no. LA-UR-13-20185. NR 28 TC 3 Z9 3 U1 0 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2014 VL 267 BP 196 EP 209 DI 10.1016/j.jcp.2014.02.040 PG 14 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AE1VS UT WOS:000333759800012 ER PT J AU Nagendra, K Tafti, DK Viswanath, K AF Nagendra, Krishnamurthy Tafti, Danesh K. Viswanath, Kamal TI A new approach for conjugate heat transfer problems using immersed boundary method for curvilinear grid based solvers SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Immersed boundary method; Curvilinear coordinates; Non-staggered grid; Conjugate heat transfer; Micro-channel flows ID FINITE-VOLUME METHOD; FLUID-STRUCTURE INTERACTION; INERTIAL FLOW REGIMES; INCOMPRESSIBLE FLOWS; COMPLEX GEOMETRIES; SIMULATING FLOWS; NUMERICAL-SOLUTIONS; CIRCULAR-CYLINDER; REYNOLDS-NUMBERS; CARTESIAN GRIDS AB Use of immersed boundary method (IBM) based techniques have helped considerably in easing the grid generation process in flows involving complex geometries and/or large boundary movements. Body fitting grid based techniques still, however, are advantageous in terms of accuracy and efficiency. In this work, we have developed an IBM scheme applicable to curvilinear coordinates, aiming at taking advantage of both the methodologies. The framework uses efficient algorithms for search, locate, and interpolate operations. A new method of implementing the conjugate heat transfer (CHT) boundary condition is proposed which is a direct extension of the method used for other boundary conditions and does not involve any complex interpolations like previous CHT implementations using IBM. The developed scheme is shown to be applicable to complex geometries on curvilinear grids, while also being very efficient, consuming less than 1% of the total simulation time per time-step. Very good scalability on massive computations is demonstrated using strong scaling study up to 1024 cores. Detailed code verification process is undertaken to show that the method is second-order accurate for both the velocity and temperature fields for all the boundary conditions considered. Further, validation studies involving uniform flow over stationary and oscillating cylinders are carried out to demonstrate the accuracy of the developed method. Lastly, simulations are performed to study flow and conjugate heat transfer through thick-walled micro-channels using body-fitted background grids and the results are shown to be in excellent agreement with previously published results. (C) 2014 Elsevier Inc. All rights reserved. C1 [Nagendra, Krishnamurthy; Tafti, Danesh K.] Natl Energy Technol Lab, Pittsburgh, PA USA. [Nagendra, Krishnamurthy; Tafti, Danesh K.; Viswanath, Kamal] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. RP Tafti, DK (reprint author), Virginia Tech, Dept Mech Engg, 114-I Randolph Hall, Blacksburg, VA 24061 USA. EM dtafti@exchange.vt.edu OI Krishnamurthy, Nagendra/0000-0002-8047-282X FU National Energy Technology Laboratory's Regional University Alliance (NETL-RUA) [4000.2.683.062.002/632] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES grant number 4000.2.683.062.002/632. NR 41 TC 13 Z9 13 U1 3 U2 21 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2014 VL 267 BP 225 EP 246 DI 10.1016/j.jcp.2014.02.045 PG 22 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AE1VS UT WOS:000333759800014 ER PT J AU Xu, G LaManna, JM Clement, JT Mench, MM AF Xu, G. LaManna, J. M. Clement, J. T. Mench, M. M. TI Direct measurement of through-plane thermal conductivity of partially saturated fuel cell diffusion media SO JOURNAL OF POWER SOURCES LA English DT Article DE Thermal conductivity; Diffusion media; Polymer electrolyte fuel cell (PEFC); Saturation; Microporous layer (MPL); Heat transfer ID HETEROGENEOUS MATERIALS; WATER TRANSPORT; LAYERS; MANAGEMENT; BEHAVIOR; MODEL; FLOW AB An experimental study to investigate the through-plane thermal conductivity of three different diffusion media (DM) used in polymer electrolyte fuel cells (PEFCs) as a function of compression (from 0.1 MPa to 2 MPa) and saturation (from 0 to 25%) was performed. Additionally, measurements to determine the stress-strain relationship for the materials were made using an optical microscope. Both compression and water content had a significant impact on the through-plane thermal conductivity, which should be accounted for in multiphase modeling efforts. An analytical expression for the theoretical maximum of the through-plane thermal conductivity, as a function of both compression and saturation, was developed to help understand the nature of liquid connectivity in saturated pores. Additionally, a relationship was developed to predict actual thermal conductivity of the tested materials as a function of both compression and saturation based on experimentally measured data. (C) 2014 Elsevier B.V. All rights reserved. C1 [Xu, G.; LaManna, J. M.; Clement, J. T.; Mench, M. M.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Electrochem Energy Storage & Convers Lab, Knoxville, TN 37996 USA. [Mench, M. M.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37931 USA. RP Mench, MM (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37931 USA. EM mmench@utk.edu FU Department of Energy [DE-EE0000470]; General Motors FX This material is based upon work supported by the Department of Energy under Award Number DE-EE0000470. The authors' would also like to acknowledge the support of Jon Owejan, Paul Nicotera, Wenbin Gu and General Motors. NR 37 TC 9 Z9 10 U1 2 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUN 15 PY 2014 VL 256 BP 212 EP 219 DI 10.1016/j.jpowsour.2014.01.015 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AE1IX UT WOS:000333724100030 ER PT J AU Allu, S Asokan, BV Shelton, WA Philip, B Pannala, S AF Allu, S. Asokan, B. Velamur Shelton, W. A. Philip, B. Pannala, S. TI A generalized multi-dimensional mathematical model for charging and discharging processes in a supercapacitor SO JOURNAL OF POWER SOURCES LA English DT Article DE Supercapacitors; Computer modeling; Electrochemical modeling; Multidimensional simulations; Energy storage ID DOUBLE-LAYER CAPACITORS; NANOPOROUS CARBON SUPERCAPACITORS; ELECTROCHEMICAL CAPACITORS; PORE STRUCTURE; ENERGY-STORAGE; FUEL-CELLS; PERFORMANCE; ELECTRODES; POWER; BATTERIES AB A generalized three dimensional computational model based on unified formulation of electrode electrolyte system of an electric double layer supercapacitor has been developed. This model accounts for charge transport across the electrode-electrolyte system. It is based on volume averaging, a widely used technique in multiphase flow modeling ([1,2]) and is analogous to porous media theory employed for electrochemical systems [3-5]. A single-domain approach is considered in the formulation where there is no need to model the interfacial boundary conditions explicitly as done in prior literature ([6]). Spatio-temporal variations, anisotropic physical properties, and upscaled parameters from lower length-scale simulations and experiments can be easily introduced in the formulation. Model complexities like irregular geometric configuration, porous electrodes, charge transport and related performance characteristics of the supercapacitor can be effectively captured in higher dimensions. This generalized model also provides insight into the applicability of 1D models ([6]) and where multidimensional effects need to be considered. A sensitivity analysis is presented to ascertain the dependence of the charge and discharge processes on key model parameters. Finally, application of the formulation to non-planar supercapacitors is presented. (C) 2014 Elsevier B.V. All rights reserved. C1 [Allu, S.; Philip, B.; Pannala, S.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Asokan, B. Velamur] Exrconmobil Upstream Res Co, Houston, TX 77098 USA. [Shelton, W. A.] Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Shelton, W. A.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. RP Allu, S (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM allus@ornl.gov; badri.velamur.asokan@exxonmobil.com; shelton@lsu.edu; philipb@ornl.gov; pannalas@ornl.gov OI Philip, Bobby/0000-0001-6716-3515; allu, srikanth/0000-0003-2841-4398 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Applied Mathematics Program of U. S. DOE's Advanced Scientific Computing Research (ASCR) office; ORNL/ORISE Post-doctoral Program; Nuclear Energy office of U. S. Department of Energy FX We would like to acknowledge the support and help from the AMP developers team in providing the back-plane and infrastructure for the multi-physics code framework. This research is supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U. S. Department of Energy (SA, WAS, and SP). Additional support for SP was provided by Applied Mathematics Program of U. S. DOE's Advanced Scientific Computing Research (ASCR) office. BVA was funded through the ORNL/ORISE Post-doctoral Program and BP was funded by Nuclear Energy office of U. S. Department of Energy. NR 42 TC 6 Z9 6 U1 4 U2 70 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUN 15 PY 2014 VL 256 BP 369 EP 382 DI 10.1016/j.jpowsour.2014.01.054 PG 14 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AE1IX UT WOS:000333724100051 ER PT J AU Geisler, MP Meinert, M Schmalhorst, J Reiss, G Arenholz, E AF Geisler, Manuel P. Meinert, Markus Schmalhorst, Jan Reiss, Guenter Arenholz, Elke TI Multiple phases in sputtered Cr2CoGa films SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Heusler compound; Half-metal; Thin film; Phase decomposition ID HEUSLER COMPOUNDS; STABILITY; CRYSTAL; GALLIUM; B2 AB By magnetron co-sputtering, thin films of a nominal Cr2CoGa compound were deposited on MgO and MgAl2O4. To achieve crystallization in the inverse Heusler structure, different heat treatments were tested. Instead of the inverse Heusler structure, we observed phase separation and precipitate formation in dependence on the heat treatment. The main precipitate is Cr3Ga in A15 structure. The remainder forms Co-rich CoGa in the B2 structure and possibly Cr-rich CoCr in the r-phase. (C) 2014 Elsevier B. V. All rights reserved. C1 [Geisler, Manuel P.; Meinert, Markus; Schmalhorst, Jan; Reiss, Guenter] Univ Bielefeld, Ctr Spinelect Mat & Devices, Dept Phys, D-33501 Bielefeld, Germany. [Arenholz, Elke] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Meinert, M (reprint author), Univ Bielefeld, Ctr Spinelect Mat & Devices, Dept Phys, D-33501 Bielefeld, Germany. EM meinert@physik.uni-bielefeld.de RI Meinert, Markus/E-8794-2011; Reiss, Gunter/A-3423-2010 OI Meinert, Markus/0000-0002-7813-600X; Reiss, Gunter/0000-0002-0918-5940 FU European Commission [604398]; Deutsche Forschungsgemeinschaft (DFG); Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the European Commission via the Collaborative Project HARFIR (Project No. 604398). Further financial support by the Deutsche Forschungsgemeinschaft (DFG) is gratefully acknowledged. We thank Dr. Karsten Rott for help with EDX mappings and SEM images. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 23 TC 5 Z9 5 U1 2 U2 36 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD JUN 15 PY 2014 VL 598 BP 213 EP 216 DI 10.1016/j.jallcom.2014.02.035 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AD2SA UT WOS:000333084200034 ER PT J AU Li, YH Guo, SK Ma, ZQ Qu, GH Shi, TT Gong, XG Xia, Q Wei, SH AF Li, Yong-Hua Guo, Shu-Kuan Ma, Zhong-Quan Qu, Guo-Hui Shi, Ting-Ting Gong, Xin-Gao Xia, Qin Wei, Su-Huai TI Magnetic property of transition metal-Si atomic line on silicon Sigma 3 grain boundary: A theoretical study SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID AUGMENTED-WAVE METHOD; SEMICONDUCTORS; ENERGY AB Using first-principles calculations within density functional theory, we investigate the electronic and magnetic properties of different 3d transition metal-Si atomic lines on silicon Sigma 3 (112) grain boundary, which can be formed through grain boundary segregation. We find that (i) Fe atoms occupy the substitutional sites at the grain boundary and form an Fe-Si atomic line, but the interaction between the Fe atoms is antiferromagnetic. (ii) The ferromagnetic stability increases with the atomic number of the transition metals and Co-Si atomic line is more stable in the ferromagnetic phase and shows a semimetallic behavior. We suggest that this special TM-Si atomic line formed by thermodynamically favorable transition metal segregation on Si grain boundary could be used in design of spin-dependent quantum devices. (C) 2014 AIP Publishing LLC. C1 [Li, Yong-Hua; Guo, Shu-Kuan; Ma, Zhong-Quan; Qu, Guo-Hui; Shi, Ting-Ting; Xia, Qin] Shanghai Univ, Dept Phys, SHU Solar Energy R&D Lab, Shanghai 200444, Peoples R China. [Gong, Xin-Gao] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Li, YH (reprint author), Shanghai Univ, Dept Phys, SHU Solar Energy R&D Lab, Shanghai 200444, Peoples R China. EM lyhua@shu.edu.cn RI gong, xingao/D-6532-2011 FU Natural Science Foundation of China [11004128, 61274067]; U.S. Department of Energy [DE-AC36-08GO28308] FX The work at Shanghai University was supported by the Natural Science Foundation of China (Grant Nos. 11004128 and 61274067). Computing resources was provided by the High Performance Computing Center of Shanghai University. The work at NREL was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. NR 25 TC 2 Z9 2 U1 0 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUN 14 PY 2014 VL 115 IS 22 AR 223906 DI 10.1063/1.4883316 PG 4 WC Physics, Applied SC Physics GA AJ7QR UT WOS:000337891800044 ER PT J AU Buonaugurio, A Graham, J Buytendyk, A Bowen, KH Ryder, MR Keolopile, ZG Haranczyk, M Gutowski, M AF Buonaugurio, Angela Graham, Jacob Buytendyk, Allyson Bowen, Kit H. Ryder, Matthew R. Keolopile, Zibo G. Haranczyk, Maciej Gutowski, Maciej TI Communication: Remarkable electrophilicity of the oxalic acid monomer: An anion photoelectron spectroscopy and theoretical study SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ELECTRON-AFFINITIES; MATRIX-ISOLATION; SPECTRA; CONFORMERS; ENERGIES; GUANINE AB Our experimental and computational results demonstrate an unusual electrophilicity of oxalic acid, the simplest dicarboxylic acid. The monomer is characterized by an adiabatic electron affinity and electron vertical detachment energy of 0.72 and 1.08 eV (+/- 0.05 eV), respectively. The electrophilicity results primarily from the bonding carbon-carbon interaction in the singly occupied molecular orbital of the anion, but it is further enhanced by intramolecular hydrogen bonds. The well-resolved structure in the photoelectron spectrum is reproduced theoretically, based on Franck-Condon factors for the vibronic anion -> neutral transitions. (C) 2014 AIP Publishing LLC. C1 [Buonaugurio, Angela; Graham, Jacob; Buytendyk, Allyson; Bowen, Kit H.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [Ryder, Matthew R.; Keolopile, Zibo G.; Gutowski, Maciej] Heriot Watt Univ, Sch Engn & Phys Sci, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland. [Keolopile, Zibo G.] Univ Botswana, Dept Phys, Gaborone, Botswana. [Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Bowen, KH (reprint author), Johns Hopkins Univ, Dept Chem, Charles & 34th St, Baltimore, MD 21218 USA. EM kbowen@jhu.edu; keolopilezg@mopipi.ub.bw; m.gutowski@hw.ac.uk RI Haranczyk, Maciej/A-6380-2014; OI Haranczyk, Maciej/0000-0001-7146-9568; Ryder, Matthew/0000-0002-1363-8148 FU (U.S.) National Science Foundation [CHE-1360692]; University of Botswana; U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This material is based, in part, upon experimental work supported by the (U.S.) National Science Foundation under Grant No. CHE-1360692 (K. H. B.). Z.G.K. was supported by the fellowship from the University of Botswana. This research was supported in part (to M. H.) by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 5 Z9 5 U1 0 U2 13 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 14 PY 2014 VL 140 IS 22 AR 221103 DI 10.1063/1.4882655 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ6LJ UT WOS:000337806100003 PM 24929367 ER PT J AU Koziol, L Morales, MM AF Koziol, Lucas Morales, Miguel M. TI A fixed-node Diffusion Monte Carlo study of the 1,2,3-tridehydrobenzene triradical SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID WAVE-FUNCTIONS; BONDING PATTERNS; BENZENE AB The electronic structure of 1,2,3-tridehydrobenzene was investigated using quantum Monte Carlo methods. The radical contains two low-lying electronic states that are nearly degenerate adiabatically (within 2 kcal/mol separation), according to previous coupled cluster calculations. We performed Diffusion Monte Carlo (DMC) calculations starting from Multi-Reference Configuration Interaction (MRCI) trial wavefunctions, with a complete active space (CAS) containing 9 electrons in 9 orbitals, CAS(9,9). Our converged DMC results are in close agreement with the best coupled-cluster results, and further strengthen the assignment of a (2)A(1) ground state. (C) 2014 AIP Publishing LLC. C1 [Koziol, Lucas; Morales, Miguel M.] Lawrence Livermore Natl Lab, Phys & Life Sci Div, Livermore, CA 94550 USA. RP Koziol, L (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Div, 7000 East Ave, Livermore, CA 94550 USA. EM moralessilva2@llnl.gov FU Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES), DOE; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357, DE-AC02-05CH11231] FX This work was supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES), DOE and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. This research also used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. This research also used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors would like to thank Jeff Hammond for performing part of the NWChem calculations. NR 20 TC 1 Z9 1 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 14 PY 2014 VL 140 IS 22 AR 224316 DI 10.1063/1.4880275 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ6LJ UT WOS:000337806100033 PM 24929397 ER PT J AU McGovern, M de Pablo, JJ AF McGovern, Michael de Pablo, Juan J. TI A boundary correction algorithm for metadynamics in multiple dimensions (vol 139, 084102, 2013) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Correction C1 [McGovern, Michael] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [de Pablo, Juan J.] Argonne Natl Lab, Lemont, IL 60439 USA. RP McGovern, M (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. EM depablo@uchicago.edu NR 1 TC 0 Z9 0 U1 2 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUN 14 PY 2014 VL 140 IS 22 AR 229901 DI 10.1063/1.4883057 PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ6LJ UT WOS:000337806100054 ER PT J AU Jung, AW AF Jung, Andreas W. TI Review of recent measurements in the top quark sector at the Tevatron SO MODERN PHYSICS LETTERS A LA English DT Review DE Top quark; properties; cross-section; Tevatron; D0; CDF ID STANDARD MODEL; P(P)OVER-BAR COLLISIONS; PARTON DISTRIBUTIONS; LHC; BOSON; DETECTOR; EVENTS AB Recent measurements in the top quark sector at the Fermilab Tevatron collider are discussed. Measurements at the Tevatron use up to 9.7 fb(-1) of data corresponding to the full data sets recorded by each of the experiments, CDF and DO. This review discusses the most recent measurements of inclusive and differential top quark cross-sections in strong and electroweak production of top quarks and related measurements, as well as measurements of angular distributions related to asymmetries in top quark production. Furthermore, the current status of precision measurements of the mass of the top quark is discussed. Where available, combinations of CDF and DO results are presented. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Jung, AW (reprint author), Fermilab Natl Accelerator Lab, DAB5-MS 357,POB 500, Batavia, IL 60510 USA. EM ajung@fnal.gov NR 57 TC 0 Z9 0 U1 0 U2 7 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-7323 EI 1793-6632 J9 MOD PHYS LETT A JI Mod. Phys. Lett. A PD JUN 14 PY 2014 VL 29 IS 18 AR 1430014 DI 10.1142/S0217732314300146 PG 22 WC Physics, Nuclear; Physics, Particles & Fields; Physics, Mathematical SC Physics GA AI6CV UT WOS:000336958300001 ER PT J AU Yen, HJ Tsai, HH Kuo, CY Nie, WY Mohite, AD Gupta, G Wang, J Wu, JH Liou, GS Wang, HL AF Yen, Hung-Ju Tsai, Hsinhan Kuo, Cheng-Yu Nie, Wanyi Mohite, Aditya D. Gupta, Gautam Wang, Jian Wu, Jia-Hao Liou, Guey-Sheng Wang, Hsing-Lin TI Flexible memory devices with tunable electrical bistability via controlled energetics in donor-donor and donor-acceptor conjugated polymers SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID SOLAR-CELLS; NONVOLATILE; PERFORMANCE AB Flexible nonvolatile memory devices were fabricated from benzodi-thiophene-based donor-donor and donor-acceptor conjugated polymers with thermally/non-thermally recoverable memory behaviors. C1 [Yen, Hung-Ju; Tsai, Hsinhan; Kuo, Cheng-Yu; Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Phys Chem & Appl Spect C PCS, Los Alamos, NM 87545 USA. [Nie, Wanyi; Mohite, Aditya D.; Gupta, Gautam] Los Alamos Natl Lab, Mat Phys & Applicat Div, Mat Synth & Integrated Devices MPA 11, Los Alamos, NM 87545 USA. [Wang, Jian] Los Alamos Natl Lab, Div Mat Sci & Technol, Mat Sci Radiat & Dynam MST 8, Los Alamos, NM 87545 USA. [Wu, Jia-Hao; Liou, Guey-Sheng] Natl Taiwan Univ, Inst Polymer Sci & Engn, Taipei 10617, Taiwan. RP Wang, HL (reprint author), Los Alamos Natl Lab, Div Chem, Phys Chem & Appl Spect C PCS, POB 1663, Los Alamos, NM 87545 USA. EM hwang@lanl.gov RI Wang, Jian/F-2669-2012; OI Wang, Jian/0000-0001-5130-300X; Liou, Guey-Sheng/0000-0003-3725-3768; Yen, Hung-Ju/0000-0002-6316-9124 NR 27 TC 15 Z9 15 U1 4 U2 42 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 EI 2050-7534 J9 J MATER CHEM C JI J. Mater. Chem. C PD JUN 14 PY 2014 VL 2 IS 22 BP 4374 EP 4378 DI 10.1039/c4tc00039k PG 5 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA AI4HO UT WOS:000336826500002 ER PT J AU Wang, HR Wang, XN Li, T Lee, B AF Wang, Haoran Wang, Xinnan Li, Tao Lee, Byeongdu TI Transient viscoelasticity study of tobacco mosaic virus/Ba2+ superlattice SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Tobacco mosaic virus; Viscoelasticity; Atomic force microscopy; Nanoindentation ID STEM-CELLS; CONTACT; PARTICLES; ADHESION; NANOINDENTATION; SPHERES; FILMS; NANOSTRUCTURES; MICRORHEOLOGY; SCAFFOLDS AB Recently, we reported a new method to synthesize the rod-like tobacco mosaic virus (TMV) superlattice. To explore its potentials in nanolattice templating and tissue scaffolding, this work focused the viscoelasticity of the superlattice with a novel transient method via atomic force microscopy (AFM). For measuring viscoelasticity, in contrast to previous methods that assessed the oscillating response, the method proposed in this work enabled us to determine the transient response (creep or relaxation) of micro/nanobiomaterials. The mathematical model and numerical process were elaborated to extract the viscoelastic properties from the indentation data. The adhesion between the AFM tip and the sample was included in the indentation model. Through the functional equation method, the elastic solution for the indentation model was extended to the viscoelastic solution so that the time dependent force vs. displacement relation could be attained. To simplify the solving of the differential equation, a standard solid model was modified to obtain the elastic and viscoelastic components of the sample. The viscoelastic responses with different mechanical stimuli and the dynamic properties were also investigated. C1 [Wang, Haoran; Wang, Xinnan] N Dakota State Univ, Dept Mech Engn, Fargo, ND 58108 USA. [Li, Tao; Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Wang, XN (reprint author), N Dakota State Univ, Dept Mech Engn, Fargo, ND 58108 USA. EM xinnan.wang@ndsu.edu RI li, tao/K-8911-2012; Wang, Haoran/G-1942-2011; OI li, tao/0000-0001-5454-1468; Wang, Haoran/0000-0002-0769-600X; Lee, Byeongdu/0000-0003-2514-8805 FU ND NASA EPSCoR [FAR0017788]; U.S. DOE [DE-AC02-06CH11357] FX Funding support is provided by ND NASA EPSCoR FAR0017788. Use of the Advanced Photon Source, Electron Microscopy Center, and Center of Nanoscale Materials, an Office of Science User Facilities operated for the U. S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 55 TC 0 Z9 0 U1 1 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD JUN 13 PY 2014 VL 9 AR 300 DI 10.1186/1556-276X-9-300 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CC9ZU UT WOS:000350730500001 PM 24994956 ER PT J AU Bhat, CM AF Bhat, C. M. TI Longitudinal phase-space coating of beam in a storage ring SO PHYSICS LETTERS A LA English DT Article DE Beam stacking; Beam emittance; Longitudinal beam dynamics; Synchrotrons; Barrier rf ID SYNCHROTRON AB In this Letter, I report on a novel scheme for beam stacking without any beam emittance dilution using a barrier rf system in synchrotrons. The general principle of the scheme called longitudinal phase-space coating, validation of the concept via multi-particle beam dynamics simulations applied to the Fermilab Recycler, and its experimental demonstration are presented. In addition, it has been shown and illustrated that the rf gymnastics involved in this scheme can be used in measuring the incoherent synchrotron tune spectrum of the beam in barrier buckets and in producing a clean hollow beam in longitudinal phase space. The method of beam stacking in synchrotrons presented here is the first of its kind. (C) 2014 Elsevier B.V. All rights reserved. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Bhat, CM (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM cbhat@fnal.gov FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; U.S. Department of Energy FX The author would like to thank D. Neuffer, D. Wildman, P. Bhat and Jim MacLachlan for many useful discussions. Special thanks are due to Shreyas Bhat and Nita Bhat for careful editing of the manuscript and the Fermilab Accelerator Division MCR crew for their help during the beam experiments. This work is supported by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 40 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9601 EI 1873-2429 J9 PHYS LETT A JI Phys. Lett. A PD JUN 13 PY 2014 VL 378 IS 30-31 BP 2171 EP 2175 DI 10.1016/j.physleta.2014.05.038 PG 5 WC Physics, Multidisciplinary SC Physics GA AM2RD UT WOS:000339697600037 ER PT J AU Harrison, N Sebastian, SE AF Harrison, N. Sebastian, S. E. TI On the relationship between charge ordering and the Fermi arcs observed in underdoped high T-c superconductors SO NEW JOURNAL OF PHYSICS LA English DT Article DE superconductivity; charge density waves; Fermi surface ID SURFACE; CA2-XNAXCUO2CL2; DEPENDENCE; POCKETS AB We address the origin of the recently discovered close correspondence between the charge ordering wave vectors and the momentum-space separation between the tips of the Fermi arcs seen in angle-resolved photoemission measurements in underdoped high-temperature superconducting cuprates. This observation has been interpreted as a signature of charge order forming as an instability of preexisting Fermi arcs of a different origin. We calculate the Fermi surface spectral weight for a charge density-wave model, considering a Fermi surface, charge ordering wave vectors and short correlation lengths similar to those found experimentally. We show that the observation of wave vectors spanning the tips of remnant Fermi surface sections is a natural consequence of a Fermi surface having been reconstructed by charge order. The presence of short-range charge order therefore cannot be ruled out as a potential origin of the observed Fermi arcs. C1 [Harrison, N.] Los Alamos Natl Labs, Los Alamos, NM 87545 USA. [Sebastian, S. E.] Univ Cambridge, Cavendish Lab, Cambridge CB3 OHE, England. RP Harrison, N (reprint author), Los Alamos Natl Labs, Mail Stop E536, Los Alamos, NM 87545 USA. EM nharrison@lanl.gov OI Harrison, Neil/0000-0001-5456-7756 FU US Department of Energy BES 'Science at 100 T' [LANLF100]; National Science Foundation; State of Florida; Royal Society; European Research Council under the European Union's Seventh Framework Programme [337425-SUPERCONDUCTINGMOTT] FX This work is supported by the US Department of Energy BES 'Science at 100 T' grant no. LANLF100, the National Science Foundation and the State of Florida. SES acknowledges support from the Royal Society and the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013) / ERC Grant Agreement no. 337425-SUPERCONDUCTINGMOTT. NR 35 TC 11 Z9 11 U1 1 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUN 13 PY 2014 VL 16 AR 063025 DI 10.1088/1367-2630/16/6/063025 PG 9 WC Physics, Multidisciplinary SC Physics GA AL4BU UT WOS:000339078700001 ER PT J AU Buchmueller, O Cavanaugh, R De Roeck, A Dolan, MJ Ellis, JR Flacher, H Heinemeyer, S Isidori, G Marrouche, J Santos, DM Olive, KA Rogerson, S Ronga, FJ de Vries, KJ Weiglein, G AF Buchmueller, O. Cavanaugh, R. De Roeck, A. Dolan, M. J. Ellis, J. R. Flaecher, H. Heinemeyer, S. Isidori, G. Marrouche, J. Santos, D. Martinez Olive, K. A. Rogerson, S. Ronga, F. J. de Vries, K. J. Weiglein, G. TI The CMSSM and NUHM1 after LHC Run 1 SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID MINIMAL FLAVOR VIOLATION; EVEN HIGGS BOSONS; RELIC DENSITY; DARK-MATTER; STANDARD MODEL; EXPERIMENTAL CONSTRAINTS; ATLAS DETECTOR; XENON100 DATA; MSSM; SUPERSYMMETRY AB We analyze the impact of data from the full Run 1 of the LHC at 7 and 8 TeV on the CMSSM with and and the NUHM1 with , incorporating the constraints imposed by other experiments such as precision electroweak measurements, flavour measurements, the cosmological density of cold dark matter and the direct search for the scattering of dark matter particles in the LUX experiment. We use the following results from the LHC experiments: ATLAS searches for events with accompanied by jets with the full 7 and 8 TeV data, the ATLAS and CMS measurements of the mass of the Higgs boson, the CMS searches for heavy neutral Higgs bosons and a combination of the LHCb and CMS measurements of and . Our results are based on samplings of the parameter spaces of the CMSSM for both and and of the NUHM1 for with 6.8, 6.2 and 1.6 points, respectively, obtained using the MultiNest tool. The impact of the Higgs-mass constraint is assessed using FeynHiggs 2.10.0, which provides an improved prediction for the masses of the MSSM Higgs bosons in the region of heavy squark masses. It yields in general larger values of than previous versions of FeynHiggs, reducing the pressure on the CMSSM and NUHM1. We find that the global functions for the supersymmetric models vary slowly over most of the parameter spaces allowed by the Higgs-mass and the searches, with best-fit values that are comparable to the for the best Standard Model fit. We provide 95 % CL lower limits on the masses of various sparticles and assess the prospects for observing them during Run 2 of the LHC. C1 [Buchmueller, O.; Marrouche, J.; Rogerson, S.; de Vries, K. J.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys Grp, London SW7 2AZ, England. [Cavanaugh, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Cavanaugh, R.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [De Roeck, A.; Ellis, J. R.; Isidori, G.] CERN, Dept Phys, CH-1211 Geneva 23, Switzerland. [De Roeck, A.] Univ Antwerp, B-2610 Antwerp, Belgium. [Dolan, M. J.] SLAC Natl Accelerator Lab, Theory Grp, Menlo Pk, CA 94025 USA. [Ellis, J. R.] Kings Coll London, Theoret Particle Phys & Cosmol Grp, Dept Phys, London WC2R 2LS, England. [Flaecher, H.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Heinemeyer, S.] Inst Fis Cantabria CSIC UC, Santander 39005, Spain. [Isidori, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Santos, D. Martinez] NIKHEF H, NL-1098 XG Amsterdam, Netherlands. [Santos, D. Martinez] Vrije Univ Amsterdam, NL-1098 XG Amsterdam, Netherlands. [Olive, K. A.] Univ Minnesota, William I Fine Theoret Phys Inst, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Ronga, F. J.] ETH, Inst Particle Phys, CH-8093 Zurich, Switzerland. [Weiglein, G.] DESY, D-22607 Hamburg, Germany. RP Buchmueller, O (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys Grp, Prince Consort Rd, London SW7 2AZ, England. EM maitiu.o.dolain@gmail.com OI Olive, Keith/0000-0001-7201-5998; DOLAN, MATTHEW/0000-0003-3420-8718 FU London Centre for Terauniverse Studies (LCTS); European Research Council [267352]; CICYT [FPA 2010-22163-C02-01]; Spanish MICINN's Consolider-Ingenio Program [MultiDark CSD2009-00064]; DOE at the University of Minnesota [DE-FG02-94ER-40823] FX The work of O.B., J.E., J.M., K.A.O. and K.J.de V. is supported in part by the London Centre for Terauniverse Studies (LCTS), using funding from the European Research Council via the Advanced Investigator Grant 267352. The work of S. H. is supported in part by CICYT (grant FPA 2010-22163-C02-01) and by the Spanish MICINN's Consolider-Ingenio 2010 Program under grant MultiDark CSD2009-00064. The work of K.A.O. is supported in part by DOE grant DE-FG02-94ER-40823 at the University of Minnesota. NR 122 TC 41 Z9 41 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUN 13 PY 2014 VL 74 IS 6 AR 2922 DI 10.1140/epjc/s10052-014-2922-3 PG 22 WC Physics, Particles & Fields SC Physics GA AJ4IV UT WOS:000337639700001 ER PT J AU Ruiz, A Alonso, D Plenio, MB del Campo, A AF Ruiz, A. Alonso, D. Plenio, M. B. del Campo, A. TI Tuning heat transport in trapped-ion chains across a structural phase transition SO PHYSICAL REVIEW B LA English DT Article ID QUADRUPOLE STORAGE-RING; COULOMB CRYSTALS; DEFECT FORMATION; CONDUCTION; SYSTEMS; STATE AB We analyze the heat transport in an ion chain that is confined in a strongly anisotropic Paul trap. To drive a heat current across the chain different pairs of counterpropagating laser beams are applied to the ions on the edges. The lasers behave as heat reservoirs operating at different temperatures, and a nonequilibrium heat flow can be sustained. The control of the spatial distribution of the ions in the chain by variation of the trapping frequencies makes ion chains an ideal testbed to study heat transport properties in finite open systems of low dimensionality with tunable nonlinearities. We explore heat transport across a structural phase transition between the linear and zigzag configurations, identifying the condition for optimal heat transport. C1 [Ruiz, A.; Alonso, D.] Univ La Laguna, Dept Fis, San Cristobal la Laguna 38203, Spain. [Ruiz, A.; Alonso, D.] Univ La Laguna, IUdEA Inst Univ Estudios Avanzados, San Cristobal la Laguna 38203, Spain. [Plenio, M. B.] Univ Ulm, Inst Theoret Phys, D-89069 Ulm, Germany. [del Campo, A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [del Campo, A.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Ruiz, A (reprint author), Univ La Laguna, Dept Fis, San Cristobal la Laguna 38203, Spain. RI Alonso, Daniel/E-1775-2011; del Campo, Adolfo/B-8439-2009; Plenio, Martin/I-7895-2013 OI Alonso, Daniel/0000-0002-9471-2783; del Campo, Adolfo/0000-0003-2219-2851; FU Spanish MICINN; European Union (FEDER) [FIS2010-19998]; EU Integrating project SIQS; EU STREP EQUAM; Alexander von Humboldt Professorship; U.S. Department of Energy through the LANL/LDRD Program; LANL J. Robert Oppenheimer Fellowship FX It is a pleasure to acknowledge discussions with H. Haffner, T. E. Mehlstaubler, J. P. Palao, J. M. Plata and D. Roy. We thank A. Munoz for access to his computer facilities. This project was funded by the Spanish MICINN, the European Union (FEDER) (FIS2010-19998), the EU Integrating project SIQS, the EU STREP EQUAM, the Alexander von Humboldt Professorship (M.B.P.) and the U.S. Department of Energy through the LANL/LDRD Program and a LANL J. Robert Oppenheimer Fellowship (AdC). NR 39 TC 8 Z9 8 U1 2 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 13 PY 2014 VL 89 IS 21 AR 214305 DI 10.1103/PhysRevB.89.214305 PG 8 WC Physics, Condensed Matter SC Physics GA AJ0KR UT WOS:000337340600002 ER PT J AU Hoffman, CR Kay, BP Schiffer, JP AF Hoffman, C. R. Kay, B. P. Schiffer, J. P. TI Neutron s states in loosely bound nuclei SO PHYSICAL REVIEW C LA English DT Article ID LIGHT-NUCLEI; ENERGY-LEVELS; SHELL-MODEL; A=13-15; BE-11; N-15 AB In reviewing the data that has accumulated about light nuclei, we find that the binding energy plays a critical role in describing the variation in energy of s states relative to other states. The behavior of states with zero angular momentum within a few MeV of threshold is qualitatively different from that of neutron states with any other l value or of any proton state. This observation is explored for simple Woods-Saxon potentials and is remarkably successful in describing a wealth of experimental data for nuclei with neutron numbers between 5 and 10. The lingering of neutron s states just below threshold is associated with the increases in radii of the neutron density distributions, the neutron halos, and leads to speculations about possible halos in heavier nuclei. C1 [Hoffman, C. R.; Kay, B. P.; Schiffer, J. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Hoffman, CR (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RI Hoffman, Calem/H-4325-2016; Kay, Benjamin/F-3291-2011 OI Hoffman, Calem/0000-0001-7141-9827; Kay, Benjamin/0000-0002-7438-0208 FU US Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX The authors thank S. C. Pieper and A. Volya for their help with the Woods-Saxon calculations, J. Millener, N. Orr, and A. Macchiavelli for calling our attention to relevant literature, and a number of other colleagues for helpful discussions. This work was supported by the US Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 45 TC 12 Z9 12 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 13 PY 2014 VL 89 IS 6 AR 061305 DI 10.1103/PhysRevC.89.061305 PG 5 WC Physics, Nuclear SC Physics GA AJ0LE UT WOS:000337342600001 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Bertsche, D Besana, MI Besjes, GJ Bessidskaia, O Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G 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CA ATLAS Collaboration TI Measurements of Four-Lepton Production at the Z Resonance in pp Collisions at root s=7 and 8 TeV with ATLAS SO PHYSICAL REVIEW LETTERS LA English DT Article ID LHC; BOSON AB Measurements of four-lepton (4l, l = e,mu) production cross sections at the Z resonance in pp collisions at the LHC with the ATLAS detector are presented. For dilepton and four-lepton invariant mass regions m (l+l)- > 5 GeV and 80 < m(4l) < 100 GeV, the measured cross sections are 76 +/- 18(stat) +/- 4(syst) +/- 1.4(lumi) fb and 107 +/- 9(stat) +/- 4(syst) +/- 3.0(lumi) fb at root s=7 and 8 TeV, respectively. By subtracting the nonresonant 4l production contributions and normalizing with Z -> mu(+)mu(-) events, the branching fraction for the Z boson decay to 4l is determined to be (3.20 +/- 0.25(stat) +/- 0.13(syst)) x10(-6), consistent with the standard model prediction. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Hernandez Jimenez, Y.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Hernandez Jimenez, Y.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Anastopoulos, C.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Di Mattia, A.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Anastopoulos, C.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Onyisi, P. U. E.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E-E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, G.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, Inst Tech Informat, ZITI, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, A.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, S.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Carter, A. A.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Ahmad, A.; Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Jenni, P.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Mal, P.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Mal, P.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Mal, P.; Malaescu, B.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Conventi, F.; Della Pietra, M.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Conventi, F.; Della Pietra, M.; Djama, F.; Feligioni, L.; Hoffman, J.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, Y.; Dai, T.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk 220602, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vickey, T.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, S.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, W. C.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lin, S. C.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Li, Y.; Lin, S. C.; Lounis, A.; Makovec, N.; Matricon, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Xu, L.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; do Vale, M. A. B.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas, LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Valle Wemans, A. Do] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. [Valle Wemans, A. Do] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Azuelos, G.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gingrich, D. M.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Oakham, F. G.; Phillips, P. W.; Sankey, D. P. C.; Savard, P.; Scott, W. G.; Tyndel, M.; Vetterli, M. C.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Aielli, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Cardarelli, R.; Ciapetti, G.; De Zorzi, G.; Di Ciaccio, A.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Grossi, G. C.; Kuna, M.; Lacava, F.; Liberti, B.; Luci, C.; Mazzaferro, L.; Monzani, S.; Myagkov, A. G.; Nikolaenko, V.; Paolozzi, L.; Salamon, A.; Santonico, R.; Camillocci, E. Solfaroli; Vanadia, M.; Zaitsev, A. M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J-B.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, Commissariat Energie Atom & Aux Energies Alternat, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S-C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammensee, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Ahmad, A.; Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Huang, Y.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, J.; Tylmad, M.] Univ Stockholm, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, M.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Liang, Z.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Blum, W.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, K.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Bawa, H. S.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gao, Y. S.; Koutsman, A.; Lowe, A. J.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Shimmin, C. O.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, IN2P3, Ctr Calcul, Villeurbanne, France. [Ahmadov, F.; Huseynov, N.] Kings Coll London, Dept Phys, London, England. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Chen, L.; Gao, J.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Univ Napoli Parthenope, Naples, Italy. [Gkialas, I.; Papageorgiou, K.] Inst Particle Phys, Ottawa, ON, Canada. [Greenwood, Z. D.; Sawyer, L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Kono, T.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Li, B.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Li, Y.] Manhattan Coll, New York, NY USA. [Liu, K.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Messina, A.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Nessi, M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pasztor, G.; Toth, J.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tamsett, M. C.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Wildt, M. A.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Peleganchuk, Sergey/J-6722-2014; Warburton, Andreas/N-8028-2013; Kuday, Sinan/C-8528-2014; Ferrando, James/A-9192-2012; Bosman, Martine/J-9917-2014; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Gabrielli, Alessandro/H-4931-2012; Lokajicek, Milos/G-7800-2014; Castro, Nuno/D-5260-2011; Staroba, Pavel/G-8850-2014; Lei, Xiaowen/O-4348-2014; Doyle, Anthony/C-5889-2009; Di Domenico, Antonio/G-6301-2011; de Groot, Nicolo/A-2675-2009; Wemans, Andre/A-6738-2012; Nemecek, Stanislav/G-5931-2014; Ventura, Andrea/A-9544-2015; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Gauzzi, Paolo/D-2615-2009; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Li, Liang/O-1107-2015; Fassi, Farida/F-3571-2016; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; OI Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Peleganchuk, Sergey/0000-0003-0907-7592; Warburton, Andreas/0000-0002-2298-7315; Kuday, Sinan/0000-0002-0116-5494; Ferrando, James/0000-0002-1007-7816; Bosman, Martine/0000-0002-7290-643X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Gabrielli, Alessandro/0000-0001-5346-7841; Castro, Nuno/0000-0001-8491-4376; Lei, Xiaowen/0000-0002-2564-8351; Doyle, Anthony/0000-0001-6322-6195; Di Domenico, Antonio/0000-0001-8078-2759; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Gauzzi, Paolo/0000-0003-4841-5822; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Li, Liang/0000-0001-6411-6107; Fassi, Farida/0000-0002-6423-7213; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Della Volpe, Domenico/0000-0001-8530-7447; Mendes Saraiva, Joao Gentil/0000-0002-7006-0864; Salamanna, Giuseppe/0000-0002-0861-0052; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Price, Darren/0000-0003-2750-9977; Belanger-Champagne, Camille/0000-0003-2368-2617 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, CEA- DSM/ IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Cantons of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, USA; NSF, USA FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA- DSM/ IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; NiMSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, USA. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFNCNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 28 TC 19 Z9 19 U1 8 U2 118 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 13 PY 2014 VL 112 IS 23 AR 231806 DI 10.1103/PhysRevLett.112.231806 PG 18 WC Physics, Multidisciplinary SC Physics GA AJ0MB UT WOS:000337345600003 PM 24972200 ER PT J AU Beiersdorfer, P Trabert, E Brown, GV Clementson, J Thorn, DB Chen, MH Cheng, KT Sapirstein, J AF Beiersdorfer, P. Traebert, E. Brown, G. V. Clementson, J. Thorn, D. B. Chen, M. H. Cheng, K. T. Sapirstein, J. TI Hyperfine Splitting of the 2s(1/2) and 2p(1/2) Levels in Li- and Be-like Ions of Pr-141(59) SO PHYSICAL REVIEW LETTERS LA English DT Article ID LITHIUM-LIKE IONS; X-RAY; RADIATIVE-CORRECTIONS; TRAP; MICROCALORIMETER; SPECTROSCOPY; SPECTROMETER; TRANSITION; ENERGY; RADII AB High-resolution spectroscopy of the 2s(1/2)-2p(1/2) transition in the extreme ultraviolet region is shown to resolve the level splitting induced by the nuclear magnetic field of both the 2s(1/2) and the 2p(1/2) levels in lithiumlike Pr-141(56+) and of the 2s(1/2)2p(1/2)(3)P(1) level in berylliumlike Pr-141(55+). The Pr-141 ions are an ideal test of this measurement approach because their energy levels are known well from first principles and are unaffected by small energy contributions from QED and nuclear magnetization effects. The accuracy attained in the measured 196.5 +/- 1.2 meV 2s(1/2) splitting is more than an order of magnitude better than that achieved before using crystal spectroscopy of the 2s(1/2)-2p(3/2) x-ray transition and at the level needed to implement a proposed scheme for disentangling the contributions from QED and nuclear magnetization effects in higher-Z ions, such as Bi-209. C1 [Beiersdorfer, P.; Traebert, E.; Brown, G. V.; Clementson, J.; Thorn, D. B.; Chen, M. H.; Cheng, K. T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Sapirstein, J.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Traebert, E.] Ruhr Univ Bochum, D-44780 Bochum, Germany. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM beiersdorfer1@llnl.gov FU German Research Association (DFG) [Tr171/18, Tr171/19]; LDRD [12-LW-026]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge the dedicated technical support by Ed Magee. E. T. acknowledges travel support by the German Research Association (DFG) (Tr171/18 and Tr171/19). This work was supported in part by LDRD project 12-LW-026 and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 30 TC 2 Z9 2 U1 3 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 13 PY 2014 VL 112 IS 23 AR 233003 DI 10.1103/PhysRevLett.112.233003 PG 5 WC Physics, Multidisciplinary SC Physics GA AJ0MB UT WOS:000337345600006 PM 24972204 ER PT J AU Xia, YD Luo, H Nourgaliev, R AF Xia, Yidong Luo, Hong Nourgaliev, Robert TI An implicit Hermite WENO reconstruction-based discontinuous Galerkin method on tetrahedral grids SO COMPUTERS & FLUIDS LA English DT Article DE Discontinuous Galerkin; Reconstruction method; WENO; Compressible flows; Implicit method; Tetrahedral grids ID NAVIER-STOKES EQUATIONS; FINITE-ELEMENT-METHOD; COMPRESSIBLE FLOWS; UNSTRUCTURED MESHES; CONSERVATION-LAWS; ELLIPTIC PROBLEMS; EULER EQUATIONS; SCHEMES; CONSTRUCTION; SOLVERS AB An Implicit Reconstructed Discontinuous Galerkin method, IRDG (P1P2), is presented for solving the compressible Euler equations on tetrahedral grids. In this method, a quadratic polynomial (P-2) solution is first reconstructed using a least-squares method from the underlying linear polynomial (P-1) DG solution. By taking advantage of the derivatives in the DG formulation, the stencils used in the reconstruction involve only von Neumann neighborhood (adjacent face-neighboring cells) and thus are compact and consistent with the underlying DG method. The final P-2 solution is then obtained using a WENO reconstruction, which is necessary to ensure stability of the RDG ((Pi P2)) method. A matrix-free GMRES (generalized minimum residual) algorithm is presented to solve the approximate system of linear equations arising from Newton linearization. The LU-SGS (lower-upper symmetric Gauss-Seidel) preconditioner is applied with both the simplified and approximate Jacobian matrices. The numerical experiments on a variety of flow problems demonstrate that the developed IRDG (P1P2) method is able to obtain a speedup of at least two orders of magnitude than its explicit counterpart, maintain the linear stability, and achieve the designed third order of accuracy: one order of accuracy higher than the underlying second-order DG (P-1) method without significant increase in computing costs and storage requirements. It is also found that a well approximated Jacobian matrix is essential for the IRDG method to achieve fast converging speed and maintain robustness on large-scale problems. (c) 2014 Elsevier Ltd. All rights reserved. C1 [Xia, Yidong; Luo, Hong] N Carolina State Univ, Raleigh, NC 27695 USA. [Nourgaliev, Robert] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Xia, YD (reprint author), N Carolina State Univ, Raleigh, NC 27695 USA. EM yxia2@ncsu.edu RI Luo, Hong/A-9133-2011 FU Battelle Energy Alliance, LLC [DE-AC07-05ID14517]; U.S. Department of Energy [INL/CON-09-16255]; United States Government; DOE under Nuclear Engineering University Program FX This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 (INL/CON-09-16255) with the U.S. Department of Energy. The United States Government retains and the published, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The authors would like to acknowledge the partial support for this work provided by DOE under Nuclear Engineering University Program. NR 48 TC 4 Z9 6 U1 0 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD JUN 13 PY 2014 VL 96 BP 406 EP 421 DI 10.1016/j.compfluid.2014.02.027 PG 16 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA AI3PZ UT WOS:000336775700031 ER PT J AU Xu, K Wu, ZH Renier, N Antipenko, A Tzvetkova-Robev, D Xu, Y Minchenko, M Nardi-Dei, V Rajashankar, KR Himanen, J Tessier-Lavigne, M Nikolov, DB AF Xu, Kai Wu, Zhuhao Renier, Nicolas Antipenko, Alexander Tzvetkova-Robev, Dorothea Xu, Yan Minchenko, Maria Nardi-Dei, Vincenzo Rajashankar, Kanagalaghatta R. Himanen, Juha Tessier-Lavigne, Marc Nikolov, Dimitar B. TI NEURAL MIGRATION Structures of netrin-1 bound to two receptors provide insight into its axon guidance mechanism SO SCIENCE LA English DT Article ID HEPARAN-SULFATE; DCC; BINDING; EXPRESSION; FAMILY; MOLECULE; MIDLINE; UNC5; SLIT AB Netrins are secreted proteins that regulate axon guidance and neuronal migration. Deleted in colorectal cancer (DCC) is a well-established netrin-1 receptor mediating attractive responses. We provide evidence that its close relative neogenin is also a functional netrin-1 receptor that acts with DCC to mediate guidance in vivo. We determined the structures of a functional netrin-1 region, alone and in complexes with neogenin or DCC. Netrin-1 has a rigid elongated structure containing two receptor-binding sites at opposite ends through which it brings together receptor molecules. The ligand/receptor complexes reveal two distinct architectures: a 2:2 heterotetramer and a continuous ligand/receptor assembly. The differences result from different lengths of the linker connecting receptor domains fibronectin type III domain 4 (FN4) and FN5, which differs among DCC and neogenin splice variants, providing a basis for diverse signaling outcomes. C1 [Xu, Kai; Antipenko, Alexander; Tzvetkova-Robev, Dorothea; Xu, Yan; Minchenko, Maria; Nardi-Dei, Vincenzo; Himanen, Juha; Nikolov, Dimitar B.] Mem Sloan Kettering Canc Ctr, Struct Biol Program, New York, NY 10065 USA. [Wu, Zhuhao; Renier, Nicolas; Tessier-Lavigne, Marc] Rockefeller Univ, Lab Brain Dev & Repair, New York, NY 10065 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Dept Chem & Chem Biol, Argonne, IL 60439 USA. [Rajashankar, Kanagalaghatta R.] Argonne Natl Lab, Adv Photon Source, Northeastern Collaborat Access Team, Argonne, IL 60439 USA. RP Tessier-Lavigne, M (reprint author), Rockefeller Univ, Lab Brain Dev & Repair, New York, NY 10065 USA. EM marctl@mail.rockefeller.edu; nikolovd@mskcc.org OI Wu, Zhuhao/0000-0002-2471-0555 FU National Institute of General Medical Sciences from NIH [P41 GM103403]; U.S. DOE [DE-AC02-06CH11357]; Bristol-Myers Squibb postdoctoral fellowship at the Rockefeller University; European Molecular Biology Organization long-term postdoctoral fellowship FX We thank M. Kolev for technical support, M. Himanen for illustrations, Y. Goldgur for help with data collection and processing, and O. Olsen for help and support. X-ray diffraction studies were conducted at the Advanced Photon Source on the Northeastern Collaborative Access Team beamlines, which are supported by a grant from the National Institute of General Medical Sciences (P41 GM103403) from NIH. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under contract no. DE-AC02-06CH11357. Z.W. was supported in part by a Bristol-Myers Squibb postdoctoral fellowship at the Rockefeller University; N.R. was supported by a European Molecular Biology Organization long-term postdoctoral fellowship. The netrin-1, netrin-1/neogenin, and netrin-1/DCC structures have been deposited in the Protein Data Bank under codes 4PLM, 4PLN, and 4PLO, respectively. NR 30 TC 41 Z9 41 U1 2 U2 23 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUN 13 PY 2014 VL 344 IS 6189 BP 1275 EP 1279 DI 10.1126/science.1255149 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI7ND UT WOS:000337077500039 PM 24876346 ER PT J AU Arnold, R Augier, C Baker, JD Barabash, AS Basharina-Freshville, A Blondel, S Blot, S Bongrand, M Brudanin, V Busto, J Caffrey, AJ Cerna, C Chapon, A Chauveau, E Duchesneau, D Durand, D Egorov, V Eurin, G Evans, JJ Flack, R Garrido, X Gomez, H Guillon, B Guzowski, P Hodak, R Hubert, P Hugon, C Jullian, S Klimenko, A Kochetov, O Konovalov, SI Kovalenko, V Lalanne, D Lang, K Lemiere, Y Liptak, Z Loaiza, P Lutter, G Mamedov, F Marquet, C Mauger, F Morgan, B Mott, J Nemchenok, I Nomachi, M Nova, F Nowacki, F Ohsumi, H Pahlka, RB Perrot, F Piquemal, F Povinec, P Ramachers, YA Remoto, A Reyss, JL Richards, B Riddle, CL Rukhadze, E Saakyan, R Sarazin, X Shitov, Y Simard, L Simkovic, F Smetana, A Smolek, K Smolnikov, A Soldner-Rembold, S Soule, B Stekl, I Suhonen, J Sutton, CS Szklarz, G Thomas, J Timkin, V Torre, S Tretyak, VI Tretyak, VI Umatov, VI Vanushin, I Vilela, C Vorobel, V Waters, D Zukauskas, A AF Arnold, R. Augier, C. Baker, J. D. Barabash, A. S. Basharina-Freshville, A. Blondel, S. Blot, S. Bongrand, M. Brudanin, V. Busto, J. Caffrey, A. J. Cerna, C. Chapon, A. Chauveau, E. Duchesneau, D. Durand, D. Egorov, V. Eurin, G. Evans, J. J. Flack, R. Garrido, X. Gomez, H. Guillon, B. Guzowski, P. Hodak, R. Hubert, P. Hugon, C. Jullian, S. Klimenko, A. Kochetov, O. Konovalov, S. I. Kovalenko, V. Lalanne, D. Lang, K. Lemiere, Y. Liptak, Z. Loaiza, P. Lutter, G. Mamedov, F. Marquet, C. Mauger, F. Morgan, B. Mott, J. Nemchenok, I. Nomachi, M. Nova, F. Nowacki, F. Ohsumi, H. Pahlka, R. B. Perrot, F. Piquemal, F. Povinec, P. Ramachers, Y. A. Remoto, A. Reyss, J. L. Richards, B. Riddle, C. L. Rukhadze, E. Saakyan, R. Sarazin, X. Shitov, Yu. Simard, L. Simkovic, F. Smetana, A. Smolek, K. Smolnikov, A. Soeldner-Rembold, S. Soule, B. Stekl, I. Suhonen, J. Sutton, C. S. Szklarz, G. Thomas, J. Timkin, V. Torre, S. Tretyak, Vl. I. Tretyak, V. I. Umatov, V. I. Vanushin, I. Vilela, C. Vorobel, V. Waters, D. Zukauskas, A. CA NEMO-3 Collaboration TI Search for neutrinoless double-beta decay of Mo-100 with the NEMO-3 detector SO PHYSICAL REVIEW D LA English DT Article ID GE-76 AB We report the results of a search for the neutrinoless double-beta decay (0 upsilon beta beta) of Mo-100, using the NEMO-3 detector to reconstruct the full topology of the final state events. With an exposure of 34.7 kg . y, no evidence for the 0 upsilon beta beta signal has been found, yielding a limit for the light Majorana neutrino mass mechanism of T-1/2(0 upsilon beta beta) > 1.1 x 10(24) years (90% C.L.) once both statistical and systematic uncertainties are taken into account. Depending on the nuclear matrix elements this corresponds to an upper limit on the Majorana effective neutrino mass of < m(upsilon)> < 0.3-0.9 eV (90% C.L.). Constraints on other lepton number violating mechanisms of 0 upsilon beta beta decays are also given. Searching for high-energy double electron events in all suitable sources of the detector, no event in the energy region [3.2-10] MeV is observed for an exposure of 47 kg . y. C1 [Arnold, R.; Nowacki, F.] CNRS, IN2P3, ULP, IPHC, F-67037 Strasbourg, France. [Augier, C.; Blondel, S.; Bongrand, M.; Eurin, G.; Garrido, X.; Gomez, H.; Jullian, S.; Lalanne, D.; Sarazin, X.; Simard, L.; Szklarz, G.] Univ Paris 11, CNRS, IN2P3, LAL, F-91405 Orsay, France. [Baker, J. D.; Caffrey, A. J.; Riddle, C. L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Barabash, A. S.; Konovalov, S. I.; Umatov, V. I.; Vanushin, I.] ITEP, Moscow 117218, Russia. [Basharina-Freshville, A.; Eurin, G.; Flack, R.; Mott, J.; Richards, B.; Saakyan, R.; Thomas, J.; Torre, S.; Vilela, C.; Waters, D.] UCL, London WC1E 6BT, England. [Blot, S.; Chauveau, E.; Evans, J. J.; Guzowski, P.; Soeldner-Rembold, S.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Brudanin, V.; Egorov, V.; Klimenko, A.; Kochetov, O.; Kovalenko, V.; Nemchenok, I.; Shitov, Yu.; Smolnikov, A.; Timkin, V.; Tretyak, V. I.] Joint Inst Nucl Res, Dubna 141980, Russia. [Busto, J.] Univ Marseille, CNRS, IN2P3, CPPM, F-13288 Marseille, France. [Cerna, C.; Hubert, P.; Hugon, C.; Lutter, G.; Marquet, C.; Perrot, F.; Piquemal, F.; Soule, B.] Univ Bordeaux, CNRS, IN2P3, CENBG, F-33175 Gradignan, France. [Chapon, A.; Durand, D.; Guillon, B.; Lemiere, Y.; Mauger, F.] Univ Caen, CNRS, IN2P3, ENSICAEN,LPC Caen, F-14050 Caen, France. [Duchesneau, D.; Remoto, A.] Univ Savoie, CNRS, IN2P3, LAPP, F-74941 Annecy Le Vieux, France. [Hodak, R.; Mamedov, F.; Rukhadze, E.; Smetana, A.; Smolek, K.; Stekl, I.] Czech Tech Univ, Inst Expt & Appl Phys, CZ-12800 Prague, Czech Republic. [Lang, K.; Liptak, Z.; Nova, F.; Pahlka, R. B.] Univ Texas Austin, Austin, TX 78712 USA. [Loaiza, P.; Piquemal, F.] Lab Souterrain Modane, F-73500 Modane, France. [Morgan, B.; Ramachers, Y. A.] Univ Warwick, Coventry CV4 7AL, W Midlands, England. [Nomachi, M.] Osaka Univ, Osaka 5600043, Japan. [Ohsumi, H.] Saga Univ, Saga 8408502, Japan. [Povinec, P.; Simkovic, F.] Comenius Univ, FMFI, SK-84248 Bratislava, Slovakia. [Reyss, J. L.] CNRS, LSCE, F-91190 Gif Sur Yvette, France. [Shitov, Yu.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Simard, L.] Inst Univ France, F-75005 Paris, France. [Suhonen, J.] Univ Jyvaskyla, FIN-40351 Jyvaskyla, Finland. [Sutton, C. S.] Mt Holyoke Coll, S Hadley, MA 01075 USA. [Tretyak, Vl. I.] Inst Nucl Res, MSP, UA-03680 Kiev, Ukraine. [Vorobel, V.; Zukauskas, A.] Charles Univ Prague, Fac Math & Phys, CZ-12116 Prague, Czech Republic. RP Arnold, R (reprint author), CNRS, IN2P3, ULP, IPHC, F-67037 Strasbourg, France. RI Nemchenok, Igor/F-9715-2014; Evans, Justin/P-4981-2014; Hodak, Rastislav/O-4243-2016; Barabash, Alexander/S-8851-2016; OI Evans, Justin/0000-0003-4697-3337; Hodak, Rastislav/0000-0001-7640-5643; Torre, Stefano/0000-0002-7565-0118 FU RFBR in Russia; STFC in the U.K.; NSF in the U.S.; [CNRS/IN2P3] FX We thank the staff of the Modane Underground Laboratory for its technical assistance in running the experiment. We acknowledge support by the grants agencies of the Czech Republic, CNRS/IN2P3 in France, RFBR in Russia, STFC in the U.K. and NSF in the U.S. NR 38 TC 34 Z9 34 U1 0 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 12 PY 2014 VL 89 IS 11 AR 111101 DI 10.1103/PhysRevD.89.111101 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK8EN UT WOS:000338660100001 ER PT J AU Davoudiasl, H Marciano, WJ Ramos, R Sher, M AF Davoudiasl, Hooman Marciano, William J. Ramos, Raymundo Sher, Marc TI Discovering charged Higgs bosons in the W plus dark vector boson decay mode SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; PP COLLISIONS; SEARCH; MASS; U(1)S; LHC AB In two-Higgs doublet extensions of the Standard Model, flavor-changing neutral current constraints can be addressed by introducing a U(1)' gauge symmetry, under which the Higgs doublets carry different charges. That scenario implies the presence of a H(+/-)W(-/+)Z' vertex at tree level. For the light "dark" Z model (Z' = Z(d)) with m(Zd) < 10 GeV, such a coupling leads to the dominant decay mode H-+/- -> W-+/- + Z(d) (for m(II +/-) less than or similar to 175 GeV), rather than the usual type I model decay H-+/- -> tau(+/-)upsilon, for a broad range of parameters. We find that current analyses do not place significant bounds on this scenario. Over much of the parameter space considered, the decay of a pair-produced t((t)over bar) into H+ b (H-(b)over bar) provides the dominant H-+/- production. Analysis of available LHC data can likely cover significant ranges of our parameters, if Z(d) -> mu(+) mu(-) has a branching ratio of similar to 20%. If the Z(d) decays mainly invisibly then probing the entire relevant parameter space would likely require additional data from future LHC runs. We briefly discuss the phenomenology for m(II +/-) greater than or similar to 175 GeV. C1 [Davoudiasl, Hooman; Marciano, William J.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Ramos, Raymundo; Sher, Marc] Coll William & Mary, High Energy Theory Grp, Williamsburg, VA 23187 USA. RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hooman@bnl.gov; marciano@bnl.gov; raramos@email.wm.edu; mtsher@wm.edu FU U.S. DOE [DE-AC02-98CH10886]; NSF [PHY1068008] FX We thank H.-S. Lee for discussions. The work of H. D. and W. J. M. is supported by the U.S. DOE under Grant Contract No. DE-AC02-98CH10886. The work of R. R. and M. S. is supported by the NSF under Grant No. PHY1068008. The opinions and conclusions expressed herein are those of the authors and do not represent the NSF. NR 38 TC 5 Z9 5 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 12 PY 2014 VL 89 IS 11 AR 115008 DI 10.1103/PhysRevD.89.115008 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK8EN UT WOS:000338660100003 ER PT J AU Keseler, IM Skrzypek, M Weerasinghe, D Chen, AY Fulcher, C Li, GW Lemmer, KC Mladinich, KM Chow, ED Sherlock, G Karp, PD AF Keseler, Ingrid M. Skrzypek, Marek Weerasinghe, Deepika Chen, Albert Y. Fulcher, Carol Li, Gene-Wei Lemmer, Kimberly C. Mladinich, Katherine M. Chow, Edmond D. Sherlock, Gavin Karp, Peter D. TI Curation accuracy of model organism databases SO DATABASE-THE JOURNAL OF BIOLOGICAL DATABASES AND CURATION LA English DT Article ID PROTEIN-INTERACTION DATASETS; ANNOTATION AB Manual extraction of information from the biomedical literature-or biocuration-is the central methodology used to construct many biological databases. For example, the UniProt protein database, the EcoCyc Escherichia coli database and the Candida Genome Database (CGD) are all based on biocuration. Biological databases are used extensively by life science researchers, as online encyclopedias, as aids in the interpretation of new experimental data and as golden standards for the development of new bioinformatics algorithms. Although manual curation has been assumed to be highly accurate, we are aware of only one previous study of biocuration accuracy. We assessed the accuracy of EcoCyc and CGD by manually selecting curated assertions within randomly chosen EcoCyc and CGD gene pages and by then validating that the data found in the referenced publications supported those assertions. A database assertion is considered to be in error if that assertion could not be found in the publication cited for that assertion. We identified 10 errors in the 633 facts that we validated across the two databases, for an overall error rate of 1.58%, and individual error rates of 1.82% for CGD and 1.40% for EcoCyc. These data suggest that manual curation of the experimental literature by Ph.D-level scientists is highly accurate. C1 [Keseler, Ingrid M.; Weerasinghe, Deepika; Fulcher, Carol; Chow, Edmond D.; Karp, Peter D.] SRI Int, Ctr Artificial Intelligence, Bioinformat Res Grp, Menlo Pk, CA 94025 USA. [Skrzypek, Marek; Sherlock, Gavin] Stanford Univ, Dept Genet, Stanford, CA 94305 USA. [Chen, Albert Y.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Li, Gene-Wei] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94158 USA. [Lemmer, Kimberly C.] Wisconsin Energy Inst, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. [Mladinich, Katherine M.] Univ Wisconsin, Dept Med Microbiol & Immunol, Madison, WI 53706 USA. RP Karp, PD (reprint author), SRI Int, Ctr Artificial Intelligence, Bioinformat Res Grp, Menlo Pk, CA 94025 USA. EM pkarp@ai.sri.com OI Karp, Peter/0000-0002-5876-6418; Sherlock, Gavin/0000-0002-1692-4983 FU National Institute of General Medical Sciences of the National Institutes of Health [U24GM077678, R01DE015873]; NIH [U24GM077678, R01DE015873] FX The National Institute of General Medical Sciences of the National Institutes of Health (U24GM077678 to P. K. and R01DE015873 to G. S.). Funding for open access charge: NIH grant U24GM077678 and R01DE015873. NR 20 TC 2 Z9 2 U1 0 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1758-0463 J9 DATABASE-OXFORD JI Database PD JUN 12 PY 2014 AR bau058 DI 10.1093/database/bau058 PG 6 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA AK6ZC UT WOS:000338574800001 ER PT J AU Wang, Z Liu, KH Le, PS Li, MD Chiang, WS Leao, JB Copley, JRD Tyagi, M Podlesnyak, A Kolesnikov, AI Mou, CY Chen, SH AF Wang, Zhe Liu, Kao-Hsiang Le, Peisi Li, Mingda Chiang, Wei-Shan Leao, Juscelino B. Copley, John R. D. Tyagi, Madhusudan Podlesnyak, Andrey Kolesnikov, Alexander I. Mou, Chung-Yuan Chen, Sow-Hsin TI Boson Peak in Deeply Cooled Confined Water: A Possible Way to Explore the Existence of the Liquid-to-Liquid Transition in Water SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-SCATTERING; SUPERCOOLED WATER; DYNAMIC CROSSOVER; CRITICAL-POINT; DENSITY; GLASS; LINE AB The boson peak in deeply cooled water confined in nanopores is studied with inelastic neutron scattering. We show that in the (P, T) plane, the locus of the emergence of the boson peak is nearly parallel to the Widom line below similar to 1600 bar. Above 1600 bar, the situation is different and from this difference the end pressure of the Widom line is estimated. The frequency and width of the boson peak correlate with the density of water, which suggests a method to distinguish the hypothetical "low-density liquid" and "high-density liquid" phases in deeply cooled water. C1 [Wang, Zhe; Liu, Kao-Hsiang; Le, Peisi; Li, Mingda; Chiang, Wei-Shan; Chen, Sow-Hsin] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Liu, Kao-Hsiang] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. [Leao, Juscelino B.; Copley, John R. D.; Tyagi, Madhusudan] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Tyagi, Madhusudan] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Podlesnyak, Andrey; Kolesnikov, Alexander I.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Mou, Chung-Yuan] Natl Taiwan Univ, Dept Chem, Taipei 106, Taiwan. RP Chen, SH (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM sowhsin@mit.edu RI Tyagi, Madhu Sudan/M-4693-2014; Instrument, CNCS/B-4599-2012; Podlesnyak, Andrey/A-5593-2013; OI Tyagi, Madhu Sudan/0000-0002-4364-7176; Podlesnyak, Andrey/0000-0001-9366-6319; Wang, Zhe/0000-0003-4103-0751; MOU, CHUNG-YUAN/0000-0001-7060-9899 FU DOE [DE-FG02-90ER45429]; National Science Council of Taiwan, "New Partnership Program for the Connection to the Top Labs in the World."; National Science Foundation [DMR-0944772]; Scientific User Facilities Division, Office of Basic Energy Sciences, and U.S. Department of Energy FX The research at MIT was supported by DOE Grant No. DE-FG02-90ER45429. K. H. L. is sponsored by the National Science Council of Taiwan, "New Partnership Program for the Connection to the Top Labs in the World." The work at NIST was supported in part by the National Science Foundation under Agreement No. DMR-0944772. The work at ORNL was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, and U.S. Department of Energy. We thank Professor Li Liu for providing the RCM parameters. NR 24 TC 15 Z9 15 U1 2 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 12 PY 2014 VL 112 IS 23 AR 237802 DI 10.1103/PhysRevLett.112.237802 PG 5 WC Physics, Multidisciplinary SC Physics GA AK7XX UT WOS:000338642200001 PM 24972226 ER PT J AU Nah, T Kessler, SH Daumit, KE Kroll, JH Leone, SR Wilson, KR AF Nah, Theodora Kessler, Sean H. Daumit, Kelly E. Kroll, Jesse H. Leone, Stephen R. Wilson, Kevin R. TI Influence of Molecular Structure and Chemical Functionality on the Heterogeneous OH-Initiated Oxidation of Unsaturated Organic Particles SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID PHASE TROPOSPHERIC CHEMISTRY; AEROSOL MASS-SPECTROMETER; OLEIC-ACID PARTICLES; GAS-PHASE; HYDROXYL RADICALS; HIGH-RESOLUTION; RATE CONSTANTS; AQUEOUS-SOLUTION; UPTAKE KINETICS; PRODUCTS AB The kinetics and products of the heterogeneous OH-initiated oxidation of squalene (C30H50, a branched alkene with 6 C=C double bonds) particles are measured. These results are compared to previous measurements of the OH-initiated oxidation of linoleic acid (C18H32O2, a linear carboxylic acid with 2 C=C double bonds) particles to understand how molecular structure and chemical functionality influence reaction rates and mechanisms. In a 10% mixture of O-2 in N-2 in the flow reactor, the effective uptake coefficients (gamma(eff)) for squalene and linoleic acid are larger than unity, providing clear evidence for particle-phase secondary chain chemistry. gamma(eff) for squalene is 2.34 +/- 0.07, which is smaller than gamma(eff) for linoleic acid (3.75 +/- 0.18) despite the larger number of C=C double bonds in squalene. gamma(eff) for squalene increases with [O-2] in the reactor, whereas gamma(eff) for linoleic acid decreases with increasing [O-2]. This suggests that the chain cycling mechanism in these two systems is different since O-2 promotes chain propagation in the OH + squalene reaction but promotes chain termination in the OH + linoleic acid reaction. Elemental analysis of squalene aerosol shows that an average of 1.06 +/- 0.12 O atoms are added per reactive loss of squalene prior to the onset of particle volatilization. O-2 promotes particle volatilization in the OH + squalene reaction, suggesting that fragmentation reactions are important when O-2 is present in the OH oxidation of branched unsaturated organic aerosol. In contrast, O-2 does not influence the rate of particle volatilization in the OH + linoleic acid reaction. This indicates that O-2 does not alter the relative importance of fragmentation reactions in the OH oxidation of linear unsaturated organic aerosol. C1 [Nah, Theodora; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Nah, Theodora; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Kessler, Sean H.; Kroll, Jesse H.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. [Daumit, Kelly E.; Kroll, Jesse H.] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Wilson, KR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM krwilson@lbl.gov FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy, Office of Science Early Career Research Program; National Science Foundation [CHE-1012809, AGS-1056225] FX T.N., S.R.L., and K.R.W. are supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. K.R.W. is additionally supported by the Department of Energy, Office of Science Early Career Research Program. J.H.K., S.H.K., and K.E.D. are supported by the National Science Foundation (Grants No. CHE-1012809 and AGS-1056225). NR 55 TC 10 Z9 10 U1 4 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUN 12 PY 2014 VL 118 IS 23 BP 4106 EP 4119 DI 10.1021/jp502666g PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AJ2ON UT WOS:000337497300012 PM 24840787 ER PT J AU Ryerson, JL Schrauben, JN Ferguson, AJ Sahoo, SC Naumov, P Havlas, Z Michl, J Nozik, AJ Johnson, JC AF Ryerson, Joseph L. Schrauben, Joel N. Ferguson, Andrew J. Sahoo, Subash Chandra Naumov, Pance Havlas, Zdenek Michl, Josef Nozik, Arthur J. Johnson, Justin C. TI Two Thin Film Polymorphs of the Singlet Fission Compound 1,3-Diphenylisobenzofuran SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EXCITON-FISSION; ELECTRONIC-STRUCTURE; OPTICAL-PROPERTIES; ALPHA-PERYLENE; SOLID-STATE; PHOTOPHYSICS; TETRACENE; DYNAMICS; CRYSTAL; FLUORESCENCE AB Polycrystalline thin films of 1,3-diphenylisobenzofuran (1) with a morphology referred to here as alpha exhibit highly efficient singlet fission, producing two triplet states for every absorbed photon at 77 K, and about 1.4 triplet states per absorbed photon at room temperature. However, the triplet yield depends strongly on the specific crystalline form of 1, and for the morphology referred to as beta the triplet yields are roughly an order of magnitude smaller. In this study, alpha, beta, and mixed alpha/beta films of 1 are prepared by thermal evaporation and solution drop-casting, and the structural and photophysical differences that may account for the very different triplet quantum yields are explored. The crystallites of 1 in thin films have been identified with two bulk crystal polymorphs grown from solution and structurally characterized. Analysis of absorption spectra of the films reveals a 600 cm(-1) blue shift in the onset and a unique spectral profile for the form alpha crystallites as compared to form beta. Intermolecular interactions between columns of slip-stacked molecules are different in the two polymorphs, and this likely gives rise to the much smaller triplet quantum yield for beta-1. C1 [Ryerson, Joseph L.; Schrauben, Joel N.; Ferguson, Andrew J.; Nozik, Arthur J.; Johnson, Justin C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ryerson, Joseph L.; Michl, Josef; Nozik, Arthur J.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Sahoo, Subash Chandra; Naumov, Pance] New York Univ Abu Dhabi, Abu Dhabi, U Arab Emirates. [Havlas, Zdenek; Michl, Josef] Acad Sci Czech Republic, Inst Organ Chem & Biochem, CR-16610 Prague 6, Czech Republic. RP Johnson, JC (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM justin.johnson@nrel.gov RI Michl, Josef/G-9376-2014; Naumov, Pance/B-7838-2013; Nozik, Arthur/A-1481-2012; Havlas, Zdenek/B-2164-2012; Nozik, Arthur/P-2641-2016; OI Naumov, Pance/0000-0003-2416-6569; Havlas, Zdenek/0000-0002-8369-7303; Ferguson, Andrew/0000-0003-2544-1753 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical and Biosciences [DE-AC36-08GO28308]; NREL [DE-SC0007004] FX This material is based upon work supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical and Biosciences, under Contract DE-AC36-08GO28308 with NREL and DE-SC0007004 at CU-Boulder. P.N. and S.C.S. thank NYU Abu Dhabi for financial support and Dr. N. K. Nath for advice. NR 54 TC 20 Z9 21 U1 4 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 12 PY 2014 VL 118 IS 23 BP 12121 EP 12132 DI 10.1021/jp502122d PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ2OO UT WOS:000337497400006 ER PT J AU Jin, L Fu, Q Dong, AY Ning, YX Wang, ZJ Bluhm, H Bao, XH AF Jin, Li Fu, Qiang Dong, Aiyi Ning, Yanxiao Wang, Zhoujun Bluhm, Hendrik Bao, Xinhe TI Surface Chemistry of CO on Ru(0001) under the Confinement of Graphene Cover SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EPITAXIAL GRAPHENE; METAL-SURFACES; OXIDATION; OXYGEN; INTERCALATION; ADSORPTION; CATALYST; GROWTH; DEACTIVATION; MECHANISMS AB In heterogeneous catalysis, graphitic carbon formed on metal often poisons metal-catalyzed reactions through physical blockage of surface active sites. In materials science, recent works show that graphene overlayers can passivate metal surfaces acting as gas-impermeable protection coatings. However, here we show using in situ surface electron microscopy and photoemission spectroscopy that CO can be readily trapped inside the two-dimensional space between the graphene overlayer and Ru(0001) surface under near-ambient conditions. The intercalated CO molecules effectively decouple the graphene overlayer from the Ru substrate. Meanwhile, the graphene cover exerts a strong confinement effect on the surface chemistry of CO on Ru(0001), showing that a high-coverage CO adlayer can be kept at the graphene/Ru interface at room temperature which desorbs intensively and completely around 390 K. This finding challenges the traditional concept of graphene films as passivation layers, indicating that the surface graphitic carbon can be used to modify the surface chemistry of metals. C1 [Jin, Li; Fu, Qiang; Dong, Aiyi; Ning, Yanxiao; Wang, Zhoujun; Bao, Xinhe] Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Fu, Q (reprint author), Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China. EM qfu@dicp.ac.cn RI li, haobo/P-5373-2014; Jin, Li/H-3383-2011; Fu, Qiang/E-7109-2015; OI li, haobo/0000-0002-9215-3754; Fu, Qiang/0000-0001-5316-6758; Wang, Zhoujun/0000-0002-9196-8062 FU National Natural Science Foundation of China [21222305, 21373208, 21033009]; Ministry of Science and Technology of China [2011CB932704, 2013CB834603]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This work was financially supported by the National Natural Science Foundation of China (21222305, 21373208, and 21033009) and Ministry of Science and Technology of China (2011CB932704 and 2013CB834603). The ALS and the MES beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. NR 53 TC 28 Z9 29 U1 14 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 12 PY 2014 VL 118 IS 23 BP 12391 EP 12398 DI 10.1021/jp5034855 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ2OO UT WOS:000337497400033 ER PT J AU Bu, W Kim, D Vaknin, D AF Bu, Wei Kim, Doseok Vaknin, David TI Density Profiles of Liquid/Vapor Interfaces Away from Their Critical Points SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY REFLECTIVITY; THERMAL CAPILLARY WAVES; VAPOR INTERFACE; FLUID INTERFACES; FREE ENERGY; SURFACE; FLUCTUATIONS; SCATTERING; THICKNESS AB We examine the applicability of various model profiles for the liquid/vapor interface by X-ray reflectivities on water and ethanol and their mixtures at room temperature. Analysis of the X-ray reflecivities using various density profiles shows an error-function like profile is the most adequate within experimental error. Our findings, together with recent observations from simulation studies on liquid surfaces, strongly suggest that the capillary-wave dynamics shapes the interfacial density profile in terms of the error function. C1 [Bu, Wei; Vaknin, David] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Bu, Wei; Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Kim, Doseok] Sogang Univ, Dept Phys, Seoul 121742, South Korea. RP Vaknin, D (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM vaknin@ameslab.gov RI Kim, Doseok/J-8776-2013; Vaknin, David/B-3302-2009; Bu, Wei/Q-1390-2016 OI Vaknin, David/0000-0002-0899-9248; Bu, Wei/0000-0002-9996-3733 FU Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Research Foundation (NRF) - Korea government (MEST) [2011-0017435] FX The work at the Ames Laboratory was supported by the Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-07CH11358. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. D.K. was supported by the National Research Foundation (NRF) grant funded by the Korea government (MEST) No. 2011-0017435. NR 30 TC 1 Z9 1 U1 2 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 12 PY 2014 VL 118 IS 23 BP 12405 EP 12409 DI 10.1021/jp504374z PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ2OO UT WOS:000337497400035 ER PT J AU Olsen, RE Alam, TM Bartholomew, CH Enfield, DB Schliesser, JM Woodfield, BF AF Olsen, Rebecca E. Alam, Todd M. Bartholomew, Calvin H. Enfield, David B. Schliesser, Jacob M. Woodfield, Brian F. TI Structure Analysis of Al-Modified TiO2 Nanocatalyst Supports (vol 118, pg 9176, 2014) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Correction C1 [Olsen, Rebecca E.; Enfield, David B.; Schliesser, Jacob M.; Woodfield, Brian F.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Alam, Todd M.] Sandia Natl Labs, Dept Elect Opt & Nanostruct Mat, Albuquerque, NM 87185 USA. [Bartholomew, Calvin H.] Brigham Young Univ, Dept Chem Engn, Provo, UT 84602 USA. RP Olsen, RE (reprint author), Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. NR 1 TC 0 Z9 0 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 12 PY 2014 VL 118 IS 23 BP 12575 EP 12575 DI 10.1021/jp504875z PG 1 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AJ2OO UT WOS:000337497400058 ER PT J AU Mac Dowell, N Llovell, F Sun, N Hallett, JP George, A Hunt, PA Welton, T Simmons, BA Vega, LF AF Mac Dowell, N. Llovell, F. Sun, N. Hallett, J. P. George, A. Hunt, P. A. Welton, T. Simmons, B. A. Vega, L. F. TI New Experimental Density Data and Soft-SAFT Models of Alkylimidazolium ([C(n)C(1)im](+)) Chloride (Cl-), Methylsulfate ([MeSO4](-)), and Dimethylphosphate ([Me2PO4](-)) Based Ionic Liquids SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ASSOCIATING FLUID THEORY; EQUATION-OF-STATE; DIRECTIONAL ATTRACTIVE FORCES; THERMODYNAMIC PERTURBATION-THEORY; PRESSURE PHASE-BEHAVIOR; LENNARD-JONES CHAINS; ETHANOL PLUS WATER; CARBON-DIOXIDE; BINARY-SYSTEMS; N-ALKANES AB Ionic liquids have been shown to have application in several areas of importance in the context of sustainable industrial activity. One application of particular interest is the ability of certain ionic liquids to dissolve biomass. This clearly marks them as useful materials with application within biorefineries. In this contribution, we present new coarse-grained soft-SAFT models and experimental density data of chloride (Cl-), methylsulfate ([MeSO4](-)), and dimethylphosphate ([Me2PO4](-)) based ionic liquids which are relevant for biomass deconstruction processes. Model parameters were obtained by fitting to pure component temperature density data, and the models were subsequently tested by assessing their ability to accurately calculate viscosity and interfacial surface tension. We also developed models of mixtures of the ionic liquids with water and short-chain linear alcohols. We decomposed the contributions to the excess Gibbs energy of mixing to chemical and structural contributions, and used this to provide some insight into the driving forces for solubility of molecular species in these ionic liquids. C1 [Mac Dowell, N.] Univ London Imperial Coll Sci Technol & Med, Ctr Environm Policy, London SW7 1NA, England. [Llovell, F.; Vega, L. F.] MATGAS Res Ctr, Barcelona 08193, Spain. [Sun, N.; George, A.; Simmons, B. A.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Emeryville, CA 94608 USA. [Sun, N.; George, A.; Simmons, B. A.] Sandia Natl Labs, Biomass Sci & Convers Technol Dept, Livermore, CA 94550 USA. [Hallett, J. P.] Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, London SW7 2AZ, England. [Hunt, P. A.; Welton, T.] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England. [Vega, L. F.] Carburos Met Air Prod Grp, Barcelona 08009, Spain. RP Mac Dowell, N (reprint author), Univ London Imperial Coll Sci Technol & Med, Ctr Environm Policy, London SW7 1NA, England. EM nmac-dow@imperial.ac.uk RI Llovell, Felix/F-3067-2012; Hallett, Jason/A-3281-2012; OI Simmons, Blake/0000-0002-1332-1810; Llovell, Felix/0000-0001-7109-6810; Hallett, Jason/0000-0003-3431-2371; Welton, Tom/0000-0002-1750-1683; Vega, Lourdes/0000-0002-7609-4184 FU European Union's Seventh Framework Programme (FP7) under CO2QUEST [309102]; Spanish government, Ministerio de Economia y Competitividad [CENIT SOST-CO2 CEN2008-01027]; Carburos Metalicos, Air Products Group; Generalitat of Catalonia, AGAUR [SGR2009-666]; Natural Environment Research Council (NERC) of the UK [NE/H01392X/1]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; ERC FX The research leading to these results has received funding from the European Union's Seventh Framework Programme (FP7/2007-2013) under CO2QUEST Grant Agreement number 309102. F.L. acknowledges a TALENT fellowship from the Catalan Government. This work has been financed by the Spanish government, Ministerio de Economia y Competitividad, under Project CENIT SOST-CO2 CEN2008-01027 (a CENIT project belonging to the Ingenio 2010 program, CDTI), by Carburos Metalicos, Air Products Group, with additional support from the Generalitat of Catalonia, AGAUR under Grant SGR2009-666 also being gratefully acknowledged, and the Natural Environment Research Council (NERC) of the UK (Grant Number: NE/H01392X/1), and was part of work of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through Contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. Finally, additional support from the ERC is gratefully acknowledged. NR 107 TC 10 Z9 10 U1 3 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 12 PY 2014 VL 118 IS 23 BP 6206 EP 6221 DI 10.1021/jp501619y PG 16 WC Chemistry, Physical SC Chemistry GA AJ0JI UT WOS:000337336400018 PM 24840068 ER PT J AU del Campo, A Boshier, MG Saxena, A AF del Campo, Adolfo Boshier, Malcolm G. Saxena, Avadh TI Bent waveguides for matter-waves: supersymmetric potentials and reflectionless geometries SO SCIENTIFIC REPORTS LA English DT Article ID EXACTLY SOLVABLE POTENTIALS; BOSE-EINSTEIN CONDENSATE; BOUND-STATES; QUANTUM-MECHANICS; COLD ATOMS; CARPETS AB Non-zero curvature in a waveguide leads to the appearance of an attractive quantum potential which crucially affects the dynamics in matter-wave circuits. Using methods of supersymmetric quantum mechanics, pairs of bent waveguides are found whose geometry-induced potentials share the same scattering properties. As a result, reflectionless waveguides, dual to the straight waveguide, are identified. Strictly isospectral waveguides are also found by modulating the depth of the trapping potential. Numerical simulations are used to demonstrate the efficiency of these approaches in tailoring and controlling curvature-induced quantum-mechanical effects. C1 [del Campo, Adolfo; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [del Campo, Adolfo; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Boshier, Malcolm G.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. RP del Campo, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM delcampo@lanl.gov RI del Campo, Adolfo/B-8439-2009; Boshier, Malcolm/A-2128-2017 OI del Campo, Adolfo/0000-0003-2219-2851; Boshier, Malcolm/0000-0003-0769-1927 FU U. S Department of Energy through the LANL/LDRD Program; LANL J. Robert Oppenheimer fellowship FX It is a pleasure to thank X.-W. Guan, E. Passemar, M. Pons, N. Sinitsyn and A. Szameit for stimulating discussions. This research is supported by the U. S Department of Energy through the LANL/LDRD Program and a LANL J. Robert Oppenheimer fellowship (AD). NR 55 TC 2 Z9 2 U1 0 U2 10 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 12 PY 2014 VL 4 AR 5274 DI 10.1038/srep05274 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9CR UT WOS:000337226100012 PM 24919423 ER PT J AU Hao, SJ Cui, LS Jiang, J Guo, FM Xiao, XH Jiang, DQ Yu, C Chen, ZH Zhou, H Wang, YD Liu, YZ Brown, DE Ren, Y AF Hao, Shijie Cui, Lishan Jiang, Jiang Guo, Fangmin Xiao, Xianghui Jiang, Daqiang Yu, Cun Chen, Zonghai Zhou, Hua Wang, Yandong Liu, YuZi Brown, Dennis E. Ren, Yang TI A novel multifunctional NiTi/Ag hierarchical composite SO SCIENTIFIC REPORTS LA English DT Article ID ELASTIC CONDUCTORS; ARTIFICIAL NACRE; BEHAVIOR; ALLOYS; NITINOL; LIGHT AB Creating multifunctional materials is an eternal goal of mankind. As the properties of monolithic materials are necessary limited, one route to extending them is to create a composite by combining contrasting materials. The potential of this approach is neatly illustrated by the formation of nature materials where contrasting components are combined in sophisticated hierarchical designs. In this study, inspired by the hierarchical structure of the tendon, we fabricated a novel composite by subtly combining two contrasting components: NiTi shape-memory alloy and Ag. The composite exhibits simultaneously exceptional mechanical properties of high strength, good superelasticity and high mechanical damping, and remarkable functional properties of high electric conductivity, high visibility under fluoroscopy and excellent thermal-driven ability. All of these result from the effective-synergy between the NiTi and Ag components, and place the composite in a unique position in the properties chart of all known structural-functional materials providing new opportunities for innovative electrical, mechanical and biomedical applications. Furthermore, this work may open new avenues for designing and fabricating advanced multifunctional materials by subtly combining contrasting multi-components. C1 [Hao, Shijie; Cui, Lishan; Jiang, Jiang; Guo, Fangmin; Jiang, Daqiang; Yu, Cun] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Hao, Shijie; Cui, Lishan; Jiang, Jiang; Guo, Fangmin; Jiang, Daqiang; Yu, Cun] China Univ Petr, Dept Mat Sci & Engn, Beijing 102249, Peoples R China. [Xiao, Xianghui; Zhou, Hua; Ren, Yang] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Chen, Zonghai] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Wang, Yandong] Univ Sci & Technol, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Liu, YuZi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Brown, Dennis E.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Cui, LS (reprint author), China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. EM lishancui63@126.com; ren@aps.anl.gov RI wang, yandong/G-9404-2013; Chen, Zonghai/F-1067-2015; Liu, Yuzi/C-6849-2011; Jiang, Daqiang /G-5511-2014 OI Chen, Zonghai/0000-0001-5371-9463; FU key National Natural Science Foundation of China (NSFC) [51231008]; National 973 program of China [2012CB619403]; Science Foundation of China University of Petroleum, Beijing [2462013YJRC005]; Key Project of Chinese Ministry of Education [313055]; US Department of Energy, Office of Science, and Office of Basic Energy Science [DE-AC02-06CH11357] FX The authors thank Prof. B. M. Huang (BEIJING SMART TECHNOLOGY CO., LTD.) for great help in preparing the material. This work was supported by the key National Natural Science Foundation of China (NSFC) (51231008), the National 973 program of China (2012CB619403), the Science Foundation of China University of Petroleum, Beijing (No. 2462013YJRC005), the Key Project of Chinese Ministry of Education (313055). The use of the Advanced Photon Source and the Center for Nanoscale Materials were supported by the US Department of Energy, Office of Science, and Office of Basic Energy Science under Contract No. DE-AC02-06CH11357. NR 33 TC 3 Z9 3 U1 3 U2 58 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 12 PY 2014 VL 4 AR 5267 DI 10.1038/srep05267 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI9CR UT WOS:000337226100005 PM 24919945 ER PT J AU Adelstein, N Neaton, JB Asta, M De Jonghe, LC AF Adelstein, Nicole Neaton, Jeffrey B. Asta, Mark De Jonghe, Lutgard C. TI Density functional theory based calculation of small-polaron mobility in hematite SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METAL OXIDES; AB-INITIO; ELECTRON-TRANSFER; DOPED HEMATITE; MOLECULAR-DYNAMICS; 1ST PRINCIPLES; ALPHA-FE2O3; TRANSPORT; OXIDATION; FE2O3 AB The mobility of electron small polarons in hematite, alpha-Fe2O3, is calculated by density functional theory within the generalized gradient approximation including Hubbard U corrections. Our work goes beyond previous computational investigations of this system by computing both the prefactor and activation energies for adiabatic polaron transport. The results obtained using a Hubbard U value of 4.3 eV yield a calculated value of the room-temperature basal plane mobility of 0.009 S*cm(2)/s, which compares to within an order of magnitude with experimental measurements. Further, the values of the electronic-coupling parameter in the Marcus theory for small-polaron transport are estimated from DFT + U calculations of the defect energy levels in the stable and saddle-point configurations. Our results predict an adiabatic polaron transfer, in good agreement with previous wave function based calculations. C1 [Adelstein, Nicole] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Asta, Mark; De Jonghe, Lutgard C.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Asta, Mark; De Jonghe, Lutgard C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Adelstein, N (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. EM adelstein1@llnl.gov RI Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014 OI Neaton, Jeffrey/0000-0001-7585-6135; FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy [DE-AC02-05CH11231]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC-52-07NA27344]; Molecularly Engineered Energy Materials (MEEM); Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001342]; US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]; Molecular Foundry through the US Department of Energy, Office of Basic EnergySciences FX This work was initially supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05CH11231. N.A.'s final efforts were performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC-52-07NA27344. Portions of the work of M. A. were supported by Molecularly Engineered Energy Materials (MEEM), an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001342. J.B.N. is supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. Portions of this work are also supported by the Molecular Foundry through the US Department of Energy, Office of Basic EnergySciences under the same contract number. The authors would like to thank Kevin Hong Ding and Babak Sadigh for their useful discussions on polaron adiabatic and nonadiabatic activation energy calculations and Joel B. Varley and Hannah L. Ray for their clarifying comments. NR 81 TC 8 Z9 8 U1 7 U2 59 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 11 PY 2014 VL 89 IS 24 AR 245115 DI 10.1103/PhysRevB.89.245115 PG 9 WC Physics, Condensed Matter SC Physics GA AK7XI UT WOS:000338640600004 ER PT J AU Anand, VK Dhaka, RS Lee, Y Harmon, BN Kaminski, A Johnston, DC AF Anand, V. K. Dhaka, R. S. Lee, Y. Harmon, B. N. Kaminski, Adam Johnston, D. C. TI Physical properties of metallic antiferromagnetic CaCo1.86As2 single crystals SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; MAGNETIC-PROPERTIES; PHOSPHIDES CACO2P2; TERNARY ARSENIDES; TRANSITION; LACO2P2; ORDER; HEAT AB X-ray powder diffraction (XRD), magnetic susceptibility., isothermal magnetization M, heat capacity Cp, and in-plane electrical resistivity. measurements as a function of temperature T and magnetic field H are presented for CaCo1.86As2 single crystals. The electronic structure is probed by angle-resolved photoemission spectroscopy (ARPES) measurements of CaCo1.86As2 and by full-potential linearized augmented-plane-wave calculations for the supercell CaCo1.86As2 (CaCo1.86As2). OurXRDcrystal structure refinement is consistent with the previous combined refinement of x-ray and neutron powder diffraction data showing a collapsed-tetragonal ThCr2Si2-type structure with 7(1)% vacancies on the Co sites corresponding to the composition CaCo1.86As2 [ D. G. Quirinale et al., Phys. Rev. B 88, 174420 (2013)]. The anisotropic.(T) data are consistent with the magnetic neutron diffraction data of Quirianale et al. that demonstrate the presence of A-type collinear antiferromagnetic order below the N ' eel temperature TN = 52(1) K with the easy axis being the tetragonal c axis. However, no clear evidence from the.(T) and Cp(T) data for a magnetic transition at TN is observed. A metallic ground state is demonstrated from the band calculations and the.(T), C-p(T), and ARPES data, and spin-polarized calculations indicate a competition between the A-type AFM and FM ground states. The C-p(T) data exhibit a large Sommerfield electronic coefficient reflecting a large density of states at the Fermi energy D(EF) that is enhanced compared with the band structure calculation where the bare D(EF) arises from Co 3d bands. At 1.8 K, theM(H) data for Hc exhibit a well-defined first-order spin-flop transition at an applied field of 3.5 T. The small ordered moment of 0.3 B/Co obtained from the M(H) data at low T, the large exchange enhancement of. and the lack of a self-consistent interpretation of the.(T) and M(H, T) data in terms of a local moment Heisenberg model together indicate that the magnetism of CaCo1.86As2 is itinerant. C1 Iowa State Univ, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Anand, VK (reprint author), Helmholtz Zentrum Berlin Mat & Energie, Hahn Meitner Pl 1, D-14109 Berlin, Germany. EM johnston@ameslab.gov RI Dhaka, Rajendra/C-2486-2013; Anand, Vivek Kumar/J-3381-2013 OI Anand, Vivek Kumar/0000-0003-2023-7040 FU U.S. Department of Energy by Iowa State University [DEAC02-07CH11358]; U. S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX We thank A. I. Goldman, A. Kreyssig, R. J. McQueeney, and A. Pandey for helpful discussions. This researchwas supported by the U. S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DEAC02-07CH11358. NR 62 TC 15 Z9 15 U1 2 U2 43 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 11 PY 2014 VL 89 IS 21 AR 214409 DI 10.1103/PhysRevB.89.214409 PG 17 WC Physics, Condensed Matter SC Physics GA AK7WT UT WOS:000338639100002 ER PT J AU Chapler, BC Post, KW Richardella, AR Lee, JS Tao, J Samarth, N Basov, DN AF Chapler, B. C. Post, K. W. Richardella, A. R. Lee, J. S. Tao, J. Samarth, N. Basov, D. N. TI Infrared electrodynamics and ferromagnetism in the topological semiconductors Bi2Te3 and Mn-doped Bi2Te3 SO PHYSICAL REVIEW B LA English DT Article ID OPTICAL-PROPERTIES; MAGNETIC-PROPERTIES; BISMUTH TELLURIDE; INSULATOR; CONDUCTIVITY; SPECTRA; SB2TE3 AB We report on infrared (IR) optical experiments on Bi2Te3 and Mn-doped Bi2Te3 epitaxial thin films. In the latter film, dilute Mn doping (4.5%) of the topologically nontrivial semiconductor host results in a time-reversal-symmetry-breaking ferromagnetic order below T-C = 15 K. Our spectroscopic study shows that both materials share the Bi2Te3 crystal structure, as well as classification as bulk degenerate semiconductors. Hence the Fermi energy is located in the Bi2Te3 conduction band in both materials, and furthermore, there is no need to invoke topological surface states to describe the conductivity spectra. We also demonstrate that the Drude oscillator strength gives a simple metric with which to distinguish the possibility of topological surface state origins of the low frequency conductance, and we conclude that in both the pristine and Mn-doped Bi2Te3 samples the electromagnetic response is indeed dominated by the bulk material properties, rather than those of the surface. An encouraging aspect for taking advantage of the interplay between nontrivial topology and magnetism, however, is that the temperature dependence of the Mn-doped Bi2Te3 film suggests bulk charge carriers do not play a significant role in mediating ferromagnetism. Thus, a truly insulating bulk may still be suitable for the formation of a ferromagnetic ground state in this dilute magnetic topological semiconductor. C1 [Chapler, B. C.; Post, K. W.; Basov, D. N.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Richardella, A. R.; Lee, J. S.; Samarth, N.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Tao, J.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Chapler, BC (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. RI Samarth, Nitin/C-4475-2014 OI Samarth, Nitin/0000-0003-2599-346X FU DARPA [N66001-11-1-4110]; ONR [N00014-12-1-0117]; ARO-MURI [W911NF-12-1-0461]; Pennsylvania State University Materials Research Institute Nanofabrication Lab [ECS-0335765]; US Department of Energy (DOE)/Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-98CH10886] FX Sample growth and characterization at Penn State was supported by DARPA (N66001-11-1-4110), ONR (N00014-12-1-0117), ARO-MURI (W911NF-12-1-0461), and the Pennsylvania State University Materials Research Institute Nanofabrication Lab (ECS-0335765). Research at Brookhaven National Laboratory was sponsored by the US Department of Energy (DOE)/Basic Energy Sciences, Materials Sciences and Engineering Division under Contract DE-AC02-98CH10886. Work at UCSD is supported by DARPA. NR 66 TC 11 Z9 11 U1 5 U2 69 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 11 PY 2014 VL 89 IS 23 AR 235308 DI 10.1103/PhysRevB.89.235308 PG 8 WC Physics, Condensed Matter SC Physics GA AK7XA UT WOS:000338639800002 ER PT J AU Lopez-Bezanilla, A von Lilienfeld, OA AF Lopez-Bezanilla, Alejandro von Lilienfeld, O. Anatole TI Modeling electronic quantum transport with machine learning SO PHYSICAL REVIEW B LA English DT Article AB We present a machine learning approach to solve electronic quantum transport equations of one-dimensional nanostructures. The transmission coefficients of disordered systems were computed to provide training and test data sets to the machine. The system's representation encodes energetic as well as geometrical information to characterize similarities between disordered configurations, while the Euclidean norm is used as a measure of similarity. Errors for out-of-sample predictions systematically decrease with training set size, enabling the accurate and fast prediction of new transmission coefficients. The remarkable performance of our model to capture the complexity of interference phenomena lends further support to its viability in dealing with transport problems of undulatory nature. C1 [Lopez-Bezanilla, Alejandro] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [von Lilienfeld, O. Anatole] Argonne Natl Lab, Argonne Leadership Comp Facil, Lemont, IL 60439 USA. [von Lilienfeld, O. Anatole] Univ Basel, Dept Chem, Inst Phys Chem, CH-4056 Basel, Switzerland. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM alejandrolb@gmail.com; anatole.vonlilienfeld@unibas.ch RI von Lilienfeld, O. Anatole/D-8529-2011; Lopez-Bezanilla, Alejandro/B-9125-2015 OI Lopez-Bezanilla, Alejandro/0000-0002-4142-2360 FU DOE BES [FWP#70081]; Office of Science of the U.S. DOE [DE-AC02-06CH11357]; Swiss National Science foundation [PPOOP2_138932] FX Both authors acknowledge DOE BES glue funding through Grant No. FWP#70081. This research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC02-06CH11357. O.A.vL. also acknowledges funding from the Swiss National Science foundation (No. PPOOP2_138932). NR 16 TC 13 Z9 13 U1 6 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 11 PY 2014 VL 89 IS 23 AR 235411 DI 10.1103/PhysRevB.89.235411 PG 5 WC Physics, Condensed Matter SC Physics GA AK7XA UT WOS:000338639800004 ER PT J AU Miao, H Wang, LM Richard, P Wu, SF Ma, J Qian, T Xing, LY Wang, XC Jin, CQ Chou, CP Wang, Z Ku, W Ding, H AF Miao, H. Wang, L. -M. Richard, P. Wu, S. -F. Ma, J. Qian, T. Xing, L. -Y. Wang, X. -C. Jin, C. -Q. Chou, C. -P. Wang, Z. Ku, W. Ding, H. TI Coexistence of orbital degeneracy lifting and superconductivity in iron-based superconductors SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION; ANISOTROPY; LIFEAS AB We report the angle-resolved photoemission spectroscopy observation of the lifting of symmetry-protected band degeneracy, and consequently the breakdown of local tetragonal symmetry in the superconducting state of Li( Fe1-x Co-x) As. Supported by theoretical simulations, we analyze the doping and temperature dependences of this band splitting and demonstrate an intimate connection between ferro-orbital correlations and superconductivity. C1 [Miao, H.; Richard, P.; Wu, S. -F.; Ma, J.; Qian, T.; Xing, L. -Y.; Wang, X. -C.; Jin, C. -Q.; Ding, H.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Miao, H.; Richard, P.; Wu, S. -F.; Ma, J.; Qian, T.; Xing, L. -Y.; Wang, X. -C.; Jin, C. -Q.; Ding, H.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Wang, L. -M.; Chou, C. -P.; Ku, W.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Richard, P.; Jin, C. -Q.; Ding, H.] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. [Chou, C. -P.] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Wang, Z.] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. RP Miao, H (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM p.richard@iphy.ac.cn; dingh@iphy.ac.cn RI Richard, Pierre/F-7652-2010 OI Richard, Pierre/0000-0003-0544-4551 FU CAS [2010Y1JB6]; MOST [2010CB923000, 2011CBA001000, 2013CB921703]; NSFC [11004232, 11274362]; U.S. Department of Energy, Office of Science [DE-AC02-98CH10886]; University of Wisconsin-Madison - University of Wisconsin-Milwaukee FX We thank A. Tsvelik, J.-P. Hu, F. Wang, P. D. Johnson, and H.-B. Yang for useful discussions. This work was supported by grants from CAS (No. 2010Y1JB6), MOST (No. 2010CB923000, No. 2011CBA001000, and No. 2013CB921703), and NSFC (No. 11004232 and No. 11274362). The theoretical study is supported by U.S. Department of Energy, Office of Science DE-AC02-98CH10886. This work is based in part on research conducted at the Synchrotron Radiation Center, which is primarily funded by the University of Wisconsin-Madison with the University of Wisconsin-Milwaukee. NR 31 TC 17 Z9 17 U1 2 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 11 PY 2014 VL 89 IS 22 AR 220503 DI 10.1103/PhysRevB.89.220503 PG 5 WC Physics, Condensed Matter SC Physics GA AK7WW UT WOS:000338639400002 ER PT J AU Song, YK Liang, ZT Wang, XN AF Song, Yu-kun Liang, Zuo-tang Wang, Xin-Nian TI Nuclear suppression of azimuthal asymmetries in semi-inclusive deep inelastic scattering off polarized targets SO PHYSICAL REVIEW D LA English DT Article AB We extend the study of nuclear dependence of the transverse momentum dependent parton distribution functions and azimuthal asymmetries to semi-inclusive deep inelastic scattering (SIDIS) off polarized nuclear targets. We show that azimuthal asymmetries are suppressed for SIDIS off a polarized nuclear target relative to that off a polarized nucleon due to multiple scattering inside the nucleus. Using the value of transport parameter inside large nuclei extracted from jet quenching analyses in SIDIS off nuclear targets, we also present a numerical estimate of the nuclear suppression of the azimuthal asymmetry that might be useful to guide the future experimental studies of SIDIS off polarized nuclear targets. C1 [Song, Yu-kun] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Liang, Zuo-tang] Shandong Univ, Key Lab Particle Phys & Particle Irradiat MOE, Jinan 250100, Peoples R China. [Liang, Zuo-tang] Shandong Univ, Sch Phys, Jinan 250100, Peoples R China. [Wang, Xin-Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Song, YK (reprint author), Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. OI Wang, Xin-Nian/0000-0002-9734-9967; Song, Yu-kun/0000-0003-1854-5167 FU National Natural Science Foundation of China [11035003, 11105137, 11221504]; Major State Basic Research Development Program in China [2014CB845404]; Ministry of Science and Technology of China [2014DFG02050]; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; CCNU-QLPL Innovation Fund [QLPL2011P01] FX We thank Harut Avakian for communications. This work was supported in part by the National Natural Science Foundation of China (Projects No. 11035003, No. 11105137, and No. 11221504), the Major State Basic Research Development Program in China (Contract No. 2014CB845404), the Ministry of Science and Technology of China under Grant No. 2014DFG02050, the Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by the CCNU-QLPL Innovation Fund (QLPL2011P01). NR 9 TC 7 Z9 7 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 11 PY 2014 VL 89 IS 11 AR 117501 DI 10.1103/PhysRevD.89.117501 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AK7XU UT WOS:000338641800006 ER PT J AU Strelnikov, NO Vasserman, IB AF Strelnikov, N. O. Vasserman, I. B. TI Earth's field effect on magnetic performance of horizontally and vertically polarizing undulators SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Effects of the interaction of the Earth's magnetic field with different types of insertion devices (IDs) were studied at the Advanced Photon Source (APS) at Argonne National Laboratory (Argonne) according to the improvement of high-precision field measurements and field correction techniques that should meet the tight requirements for next-generation x-ray sources. The magnetic measurements of two Advanced Photon Source hybrid-type IDs with periods of 33 and 27 mm have been performed. The impact of different design elements was considered. It was demonstrated that the specified limits for IDs can be exceeded if the effect of the Earth's field is not taken into account for various orientations of the IDs in the storage ring. Numerical simulations were done to better interpret experimental results for both devices and to estimate the effect for novel ID with the horizontal main field, which is now under development. C1 [Strelnikov, N. O.; Vasserman, I. B.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Strelnikov, N. O.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. RP Strelnikov, NO (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM niks.str@gmail.com; vasserman@aps.anl.gov FU U.S. Department of Energy, Basic Energy Sciences, Office of Science [DE-AC02-06CH11357] FX This work is supported by the U.S. Department of Energy, Basic Energy Sciences, Office of Science, under Contract No. DE-AC02-06CH11357. N. O. Strelnikov thanks E. Gluskin for fruitful discussions and advice during the paper's preparation. NR 11 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD JUN 11 PY 2014 VL 17 IS 6 AR 062401 DI 10.1103/PhysRevSTAB.17.062401 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AK8GU UT WOS:000338666400001 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Lowette, S Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Dias, FA Tomei, TRFP Lagana, C Novaes, SF Padula, SS Bernardes, CA Gregores, EM Mercadante, PG Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Mutel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M U Beaudette, F Benhabib, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Heracleous, N Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Flucke, G Geiser, A Glushkov, I Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Horton, D Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Kramer, M Krucker, D Kuznetsova, E Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Olzem, J Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Walsh, R Wissing, C Martin, MA Blobel, V Enderle, H Erfle, J Garutti, E Gebbert, U Gorner, M Gosselink, M Haller, J Heine, K Hoing, RS Kaussen, G Kirschenmann, H Klanner, R Kogler, R Lange, J Marchesini, I Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Thomsen, J Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Komaragiri, JR Kornmayer, A Pardo, PL Martschei, D Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Ott, J Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Topsis-Giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B 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CA CMS Collaboration TI Probing color coherence effects in pp collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID E+E-ANNIHILATION; P(P)OVER-BAR COLLISIONS; PARTON FRAGMENTATION; GLUON INTERFERENCE; 3-JET EVENTS; SIMULATION; RADIATION; SHOWERS; PHYSICS; MODELS AB A study of color coherence effects in pp collisions at a center-of-mass energy of 7 is presented. The data used in the analysis were collected in 2010 with the CMS detector at the LHC and correspond to an integrated luminosity of 36 pb. Events are selected that contain at least three jets and where the two jets with the largest transverse momentum exhibit a back-to-back topology. The measured angular correlation between the second- and third-leading jet is shown to be sensitive to color coherence effects, and is compared to the predictions of Monte Carlo models with various implementations of color coherence. None of the models describe the data satisfactorily. 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[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.; Kim, Y.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Vilela Pereira, A.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Mohanty, A. K.; Giordano, F.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Llatas, M. Chamizo; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Worm, S. D.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Lucas, C.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Cerci, D. Sunar; Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.; Di Matteo, L.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, Vic, Australia. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, Y.; Barfuss, A. F.; Chakaberia, I.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. 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RI Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Venturi, Andrea/J-1877-2012; Lokhtin, Igor/D-7004-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; Novaes, Sergio/D-3532-2012; Moon, Chang-Seong/J-3619-2014; Gregores, Eduardo/F-8702-2012; Gribushin, Andrei/J-4225-2012; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Menasce, Dario Livio/A-2168-2016; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Codispoti, Giuseppe/F-6574-2014; Yazgan, Efe/A-4915-2015; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Lopez Virto, Amparo/K-9996-2014; Gonzalez Caballero, Isidro/E-7350-2010; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009 OI Azzi, Patrizia/0000-0002-3129-828X; Novaes, Sergio/0000-0003-0471-8549; Moon, Chang-Seong/0000-0001-8229-7829; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Ogul, Hasan/0000-0002-5121-2893; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Fiorendi, Sara/0000-0003-3273-9419; Diemoz, Marcella/0000-0002-3810-8530; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Ligabue, Franco/0000-0002-1549-7107; Tricomi, Alessia Rita/0000-0002-5071-5501; Demaria, Natale/0000-0003-0743-9465; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Scodellaro, Luca/0000-0002-4974-8330; Lopez Virto, Amparo/0000-0002-8707-5392; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074 FU BMWF, Austria; FWF, Austria; FNRS, Belgium; FWO, Belgium; CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland; Academy of Finland, MEC; HIP (Finland); CEA; CNRS/IN2P3 (France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NIH (Hungary); DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU (Republic of Korea); LAS (Lithuania); CINVESTAV; CONACYT; SEP; UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE; NSC (Poland); FCT (Portugal); JINR (Dubna); MON; RosAtom; RAS; RFBR (Russia); MESTD (Serbia); SEIDI; CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter; IPST; STAR; NSTDA (Thailand); TUBITAK; TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE; NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLPFAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 44 TC 2 Z9 2 U1 7 U2 68 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUN 11 PY 2014 VL 74 IS 6 AR 2901 DI 10.1140/epjc/s10052-014-2901-8 PG 22 WC Physics, Particles & Fields SC Physics GA AI9FU UT WOS:000337238000001 ER PT J AU Blakely, RJ Sherrod, BL Weaver, CS Wells, RE Rohay, AC AF Blakely, Richard J. Sherrod, Brian L. Weaver, Craig S. Wells, Ray E. Rohay, Alan C. TI The Wallula fault and tectonic framework of south-central Washington, as interpreted from magnetic and gravity anomalies SO TECTONOPHYSICS LA English DT Article DE Yakima fold and thrust belt; Earthquakes; Magnetic anomalies; Gravity anomalies; Crustal structure ID OLYMPIC-WALLOWA LINEAMENT; UPPER-CRUSTAL STRUCTURE; LATE CENOZOIC STRUCTURE; COLUMBIA PLATEAU; UNITED-STATES; PUGET-SOUND; QUATERNARY FAULTS; STRUCTURE BENEATH; CASCADE RANGE; SEATTLE FAULT AB The Yakima fold and thrust belt (YFTB) in central Washington has accommodated regional, mostly north-directed, deformation of the Cascadia backarc since prior to emplacement of Miocene flood basalt of the Columbia River Basalt Group (CRBG). The YFTB consists of two structural domains. Northern folds of the YFTB strike eastward and terminate at the western margin of a 20-mGal negative gravity anomaly, the Pasco gravity low, straddling the North American continental margin. Southern folds of the YFTB strike southeastward, form part of the Olympic-Wallowa lineament (OWL), and pass south of the Pasco gravity low as the Wallula fault zone. An upper crustal model based on gravity and magnetic anomalies suggests that the Pasco gravity low is caused in part by an 8-km-deep Tertiary basin, the Pasco sub-basin, abutting the continental margin and concealed beneath CRBG. The Pasco sub-basin is crossed by north-northwest-striking magnetic anomalies caused by dikes of the 8.5 Ma Ice Harbor Member of the CRBG. At their northern end, dikes connect with the eastern terminus of the Saddle Mountains thrust of the YFTB. At their southern end, dikes are disrupted by the Wallula fault zone. The episode of NE-SW extension that promoted Ice Harbor dike injection apparently involved strike-slip displacement on the Saddle Mountains and Wallula faults. The amount of lateral shear on the OWL impacts the level of seismic hazard in the Cascadia region. Ice Harbor dikes, as mapped with aeromagnetic data, are dextrally offset by the Wallula fault zone a total of 6.9 km. Assuming that dike offsets are tectonic in origin, the Wallula fault zone has experienced an average dextral shear of 0.8 mm/y since dike emplacement 8.5 Ma, consistent with right-lateral stream offsets observed at other locations along the OWL Southeastward, the Wallula fault transfers strain to the north-striking Hite fault the possible location of the M 5.7 Milton-Freewater earthquake in 1936. Published by Elsevier B.V. C1 [Blakely, Richard J.; Wells, Ray E.] US Geol Survey, Menlo Pk, CA 94025 USA. [Sherrod, Brian L.; Weaver, Craig S.] Univ Washington, US Geol Survey, Dept Earth & Space Sci, Seattle, WA 98195 USA. [Rohay, Alan C.] Pacific NW Natl Lab, Environm Characterizat & Risk Assessment Grp, Richland, WA 99352 USA. RP Blakely, RJ (reprint author), US Geol Survey, 345 Middlefield Rd,MS 989, Menlo Pk, CA 94025 USA. EM blakely@usgs.gov NR 56 TC 6 Z9 6 U1 3 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0040-1951 EI 1879-3266 J9 TECTONOPHYSICS JI Tectonophysics PD JUN 11 PY 2014 VL 624 SI SI BP 32 EP 45 DI 10.1016/j.tecto.2013.11.006 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AJ8VA UT WOS:000337984800005 ER PT J AU Gordin, ML Dai, F Chen, SR Xu, T Song, JX Tang, DH Azimi, N Zhang, ZC Wang, DH AF Gordin, Mikhail L. Dai, Fang Chen, Shuru Xu, Terrence Song, Jiangxuan Tang, Duihai Azimi, Nasim Zhang, Zhengcheng Wang, Donghai TI Bis(2,2,2-trifluoroethyl) Ether As an Electrolyte Co-solvent for Mitigating Self-Discharge in Lithium-Sulfur Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE lithium-sulfur batteries; self-discharge; fluorinated ether; electrolyte; polysulfide shuttle; solid-electrolyte interphase ID FLUOROETHYLENE CARBONATE; LIQUID ELECTROLYTE; FUNDAMENTAL CHEMISTRY; PERFORMANCE; CATHODES; ANODES AB Lithium sulfur batteries suffer from severe self-discharge because of polysulfide dissolution and side reaction. In this work, a novel electrolyte containing bis(2,2,2-trifluoroethyl) ether (BTFE) was used to mitigate self-discharge of Li-S cells having both low- and high-sulfur-loading sulfur cathodes. This electrolyte meaningfully decreased self-discharge at elevated temperature, though differences in behavior of cells with high- and low-sulfur-loading were also noted. Further investigation showed that this effect likely stems from the formation of a more robust protective film on the anode surface. C1 [Gordin, Mikhail L.; Dai, Fang; Chen, Shuru; Xu, Terrence; Song, Jiangxuan; Tang, Duihai; Wang, Donghai] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Azimi, Nasim; Zhang, Zhengcheng] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Wang, DH (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM dwang@psu.edu RI Wang, Donghai/L-1150-2013; Xu, Terrence/M-8741-2014; Chen, Shuru/F-6964-2015; Song, Jiangxuan/G-8536-2015; Dai, Fang/O-2626-2013 OI Wang, Donghai/0000-0001-7261-8510; Xu, Terrence/0000-0002-9385-6881; Chen, Shuru/0000-0003-3805-8331; Dai, Fang/0000-0002-9229-5576 FU Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-EE0005475] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-EE0005475. NR 25 TC 45 Z9 46 U1 10 U2 105 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 11 PY 2014 VL 6 IS 11 BP 8006 EP 8010 DI 10.1021/am501665s PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AJ0JN UT WOS:000337336900006 PM 24833106 ER PT J AU Yoon, H Na, SH Choi, JY Kim, MW Kim, H An, HS Min, BK Ahn, S Yun, JH Gwak, J Yoon, K Kolekar, SS van Hest, MFAM Al-Deyab, SS Swihart, MT Yoon, SS AF Yoon, Hyun Na, Seung Heon Choi, Jae Young Kim, Min Woo Kim, Hayong An, Hee Sang Min, Byoung Koun Ahn, SeJin Yun, Jae Ho Gwak, Jihye Yoon, KyungHoon Kolekar, Sanjay S. van Hest, Maikel F. A. M. Al-Deyab, Salem S. Swihart, Mark T. Yoon, Sam S. TI Carbon- and Oxygen-Free Cu(InGa)(SSe)(2) Solar Cell with a 4.63% Conversion Efficiency by Electrostatic Spray Deposition SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE CIGSSe; thin film; solar cell; electrostatic spray; carbon free; oxygen free ID THIN-FILMS; NANOCRYSTAL INKS; CUINSE2; CU(IN,GA)SE-2; NANOPARTICLES; PERFORMANCE; PYROLYSIS; GROWTH; DEVICE AB We have demonstrated the first example of carbon- and oxygen-free Cu(In,Ga)(SSe)(2) (CIGSSe) absorber layers prepared by electrospraying a CuInGa (CIG) precursor followed by annealing, sulfurization, and selenization at elevated temperature. X-ray diffraction and scanning electron microscopy showed that the amorphous as-deposited (CIG) precursor film was converted into polycrystalline CIGSSe with a flat-grained morphology after post-treatment. The optimal post-treatment temperature was 300 degrees C for annealing and 500 degrees C for both sulfurization and selenization, with a ramp rate of 5 degrees C/min. The carbon impurities in the precursor film were removed by air annealing, and oxide that was formed during annealing was removed by sulfurization. The fabricated CIGSSe solar cell showed a conversion efficiency of 4.63% for a 0.44 cm(2) area, with V-oc = 0.4 V, J(sc) = 21 mA/cm(2), and FF = 0.53. C1 [Yoon, Hyun; Na, Seung Heon; Choi, Jae Young; Kim, Min Woo; Kim, Hayong; Yoon, Sam S.] Korea Univ, Sch Mech Engn, Seoul 136713, South Korea. [Kim, Min Woo; An, Hee Sang; Min, Byoung Koun] Korea Univ, Green Sch, Seoul 136713, South Korea. [An, Hee Sang; Min, Byoung Koun] Korea Inst Sci & Technol, Clean Energy Res Ctr, Seoul 136791, South Korea. [Ahn, SeJin; Yun, Jae Ho; Gwak, Jihye; Yoon, KyungHoon] Korea Inst Energy Res, Photovolta Res Ctr, Taejon 305343, South Korea. [Kolekar, Sanjay S.] Shivaji Univ, Dept Chem, Kolhapur 416004, Maharashtra, India. [van Hest, Maikel F. A. M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Al-Deyab, Salem S.] King Saud Univ, Dept Chem, Coll Sci, Petrochem Res Chair, Riyadh 11451, Saudi Arabia. [Swihart, Mark T.] SUNY Buffalo, Dept Chem & Biol Engn, Buffalo, NY 14260 USA. RP Yoon, SS (reprint author), Korea Univ, Sch Mech Engn, Seoul 136713, South Korea. EM skyoon@korea.ac.kr RI Swihart, Mark/A-3182-2008; OI Swihart, Mark/0000-0002-9652-687X; Kolekar, Sanjay/0000-0002-4367-6014 FU Human Resources Development Program of KETEP [20124030200120]; Industrial Strategic Technology Development Program of MICE [10045221]; Deanship of Scientific Research at King Saud University [RGP-089] FX This work was supported by the Human Resources Development Program (no. 20124030200120) of KETEP and also by the Industrial Strategic Technology Development Program (10045221) of MICE. The authors extend their appreciation to the Deanship of Scientific Research at King Saud University for funding the work through the research group project no. RGP-089. NR 36 TC 11 Z9 11 U1 1 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 11 PY 2014 VL 6 IS 11 BP 8369 EP 8377 DI 10.1021/am501286d PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AJ0JN UT WOS:000337336900050 PM 24765921 ER PT J AU Ha, TJ Kiriya, D Chen, K Javey, A AF Ha, Tae-Jun Kiriya, Daisuke Chen, Kevin Javey, Ali TI Highly Stable Hysteresis-Free Carbon Nanotube Thin-Film Transistors by Fluorocarbon Polymer Encapsulation SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE carbon nanotubes; electronics; stability; hydrophobic; passivation ID FIELD-EFFECT TRANSISTORS; ELECTRONIC-PROPERTIES; LOW-VOLTAGE; CIRCUITS; LIGHT; TRANSPARENT; NETWORKS; DEVICES; DIELECTRICS; TRANSPORT AB We report hysteresis-free carbon nanotube thin-film transistors (CNT-TFTs) employing a fluorocarbon polymer (Teflon-AF) as an encapsulation layer. Such fluorocarbon encapsulation improves device uniformity with excellent operation stability in air and even in water. The fluoropolymers possess high hydrophobicity for efficient removal of water molecules from the vicinity of nanotubes, which are known to induce charge trapping. In addition, the strong dipole associated with the carbon-fluorine bonds can provide effective screening of the charge carriers in nanotubes from various trap states in the substrate. We also report on the extended applications of encapsulation with Teflon-AF for the realization of dual-gate CNT-TFTs, where one gate is used to control the threshold voltage and the other to switch the device. The fluorocarbon encapsulation technique presents a promising approach for enhanced device reliability, which is critical for future system-level electronics based on CNTs. C1 [Ha, Tae-Jun; Kiriya, Daisuke; Chen, Kevin; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Ha, Tae-Jun; Kiriya, Daisuke; Chen, Kevin; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM ajavey@eecs.berkeley.edu RI Javey, Ali/B-4818-2013; Kashima, Taiga/I-1199-2016 FU NSF NASCENT Center FX This work was supported by the NSF NASCENT Center. NR 58 TC 28 Z9 28 U1 7 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 11 PY 2014 VL 6 IS 11 BP 8441 EP 8446 DI 10.1021/am5013326 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AJ0JN UT WOS:000337336900059 PM 24796606 ER PT J AU Hoffeditz, WL Katz, MJ Deria, P Martinson, ABF Pellin, MJ Farha, OK Hupp, JT AF Hoffeditz, William L. Katz, Michael J. Deria, Pravas Martinson, Alex B. F. Pellin, Michael J. Farha, Omar K. Hupp, Joseph T. TI High-Surface-Area Architectures for Improved Charge Transfer Kinetics at the Dark Electrode in Dye-Sensitized Solar Cells SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE dark electrode; inverse opal; dye cell; fill factor ID REDOX SHUTTLES; COUNTER ELECTRODES; TRANSFER MEDIATORS; EFFICIENCY; COMPLEXES; FILMS AB Dye-sensitized solar cell (DSC) redox shuttles other than triiodide/iodide have exhibited significantly higher charge transfer resistances at the dark electrode. This often results in poor fill factor, a severe detriment to device performance. Rather than moving to dark electrodes of untested materials that may have higher catalytic activity for specific shuttles, the surface area of platinum dark electrodes could be increased, improving the catalytic activity by simply presenting more catalyst to the shuttle solution. A new copper-based redox shuttle that experiences extremely high charge-transfer resistance at conventional Pt dark electrodes yields cells having fill-factors of less than 0.3. By replacing the standard Pt dark electrode with an inverse opal Pt electrode fabricated via atomic layer deposition, the dark electrode surface area is boosted by ca. 50-fold. The resulting increase in interfacial electron transfer rate (decrease in charge-transfer resistance) nearly doubles the fill factor and therefore the overall energy conversion efficiency, illustrating the utility of this high-area electrode for DSCs C1 [Hoffeditz, William L.; Katz, Michael J.; Deria, Pravas; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Hoffeditz, William L.; Martinson, Alex B. F.; Pellin, Michael J.; Hupp, Joseph T.] Argonne Natl Lab, Argonne Northwestern Solar Energy Res ANSER Ctr, Argonne, IL 60439 USA. [Martinson, Alex B. F.; Pellin, Michael J.; Hupp, Joseph T.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hupp, Joseph T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah, Saudi Arabia. RP Farha, OK (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM o-farha@northwestern.edu; j-hupp@northwestern.edu RI Pellin, Michael/B-5897-2008; Faculty of, Sciences, KAU/E-7305-2017; OI Pellin, Michael/0000-0002-8149-9768; Katz, Michael/0000-0002-7744-3956; Martinson, Alex/0000-0003-3916-1672 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059] FX This work was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001059. NR 30 TC 8 Z9 8 U1 2 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 11 PY 2014 VL 6 IS 11 BP 8646 EP 8650 DI 10.1021/am501455b PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AJ0JN UT WOS:000337336900083 PM 24828106 ER PT J AU Cheng, YW Lin, CK Chu, YC Abouimrane, A Chen, ZH Ren, Y Liu, CP Tzeng, YH Auciello, O AF Cheng, Yin-Wei Lin, Chi-Kai Chu, Yueh-Chieh Abouimrane, Ali Chen, Zonghai Ren, Yang Liu, Chuan-Pu Tzeng, Yonhua Auciello, Orlando TI Electrically Conductive Ultrananocrystalline Diamond-Coated Natural Graphite-Copper Anode for New Long Life Lithium-Ion Battery SO ADVANCED MATERIALS LA English DT Article ID CARBONACEOUS MATERIALS; PERFORMANCE; ELECTRODE; ALKALI; FILMS AB Science and technology are presented for novel nitrogen-incorporated ultrananocrystalline diamond (N-UNCD) encapsulated NG/copper anode and UNCD coatings that may enable next generation Li-ion batteries (LIBs) with potential 10x longer lifetime and superior performance than current LIBs. N-UNCD films (similar to 5-10 nm grain size) exhibit electrical conductivity and extreme resistance to chemical corrosion, providing superior performance with respect to current uncoated anodes. C1 [Cheng, Yin-Wei; Liu, Chuan-Pu] Natl Cheng Kung Univ, Dept Mat Sci & Engn, Tainan 70101, Taiwan. [Lin, Chi-Kai; Abouimrane, Ali; Chen, Zonghai] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Chu, Yueh-Chieh; Tzeng, Yonhua] Natl Cheng Kung Univ, Dept Elect Engn, Inst Microelect, Tainan 70101, Taiwan. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Auciello, Orlando] Univ Texas Dallas, Mat Sci & Eng Dept, Richardson, TX 75080 USA. [Auciello, Orlando] Univ Texas Dallas, Dept Bioengn, Richardson, TX 75080 USA. RP Tzeng, YH (reprint author), Natl Cheng Kung Univ, Dept Elect Engn, Inst Microelect, 1 Univ Rd, Tainan 70101, Taiwan. EM tzengyo@mail.ncku.edu.tw; orlando.auciello@utdallas.edu RI Chen, Zonghai/F-1067-2015 OI Chen, Zonghai/0000-0001-5371-9463 FU National Science Council of Taiwan [99-2911-I-006-504, 100-2120-M-006-001-, 100-2221-E-006-169-MY3]; US Department of Energy, Office of Science [DE-AC02-06CH11357]; National Science Foundation [1343461] FX This work was supported by the National Science Council of Taiwan via grants No.99-2911-I-006-504, 100-2120-M-006-001-, and 100-2221-E-006-169-MY3. N-UNCD films were grown at Argonne National Laboratory, supported by the US Department of Energy, Office of Science, under contract No. DE-AC02-06CH11357. The National Science Foundation supported part of recent work via grant No. 1343461 to University of Texas-Dallas. NR 36 TC 14 Z9 15 U1 10 U2 125 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUN 11 PY 2014 VL 26 IS 22 BP 3724 EP 3729 DI 10.1002/adma.201400280 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AJ4ZF UT WOS:000337688400020 PM 24665020 ER PT J AU Lu, J Li, L Park, JB Sun, YK Wu, F Amine, K AF Lu, Jun Li, Li Park, Jin-Bum Sun, Yang-Kook Wu, Feng Amine, Khalil TI Aprotic and Aqueous Li-O-2 Batteries SO CHEMICAL REVIEWS LA English DT Review ID LITHIUM-AIR BATTERIES; NONAQUEOUS LIQUID ELECTROLYTES; DOPED GRAPHENE NANOSHEETS; CONDUCTING GLASS-CERAMICS; ETHER-BASED ELECTROLYTES; LI-AIR; OXYGEN BATTERIES; SOLID-STATE; LI/AIR BATTERIES; HIGH-CAPACITY C1 [Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Li, Li; Wu, Feng] Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. [Park, Jin-Bum; Sun, Yang-Kook] Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea. [Amine, Khalil] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah 80203, Saudi Arabia. RP Sun, YK (reprint author), Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea. EM yksun@hanyang.ac.kr; wufeng863@bit.edu.cn; amine@anl.gov RI Faculty of, Sciences, KAU/E-7305-2017 FU U.S. Department of Energy (DOE) [DE-AC0206CH11357]; Vehicle Technologies Office, DOE Office of Energy Efficiency and Renewable Energy (EERE); DOE EERE Postdoctoral Research Award under the EERE Vehicles Technology Program; International S&T Cooperation Program of China [2010DFB63370]; Chinese National 973 Program [2009CB220100]; Human Resources Development program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea government Ministry of Trade, Industry and Energy [20124010203310]; National Research Foundation (NRF) of Korea by the Korean government (MEST) [2009-0092780] FX This work was supported by the U.S. Department of Energy (DOE) under Contract DE-AC0206CH11357, with the main support provided by the Vehicle Technologies Office, DOE Office of Energy Efficiency and Renewable Energy (EERE). J.L. was supported by a DOE EERE Postdoctoral Research Award under the EERE Vehicles Technology Program administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. This work was also partially supported by the International S&T Cooperation Program of China (Grant 2010DFB63370) and the Chinese National 973 Program (Grant 2009CB220100). This work was supported by the Human Resources Development program (No. 20124010203310) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Trade, Industry and Energy and by a National Research Foundation (NRF) of Korea grant funded by the Korean government (MEST) (2009-0092780). We are also thankful for useful discussions with Dr. David Howell and Mr. Tien Duong of the EERE Vehicle Technologies Office. NR 275 TC 229 Z9 231 U1 43 U2 441 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JUN 11 PY 2014 VL 114 IS 11 BP 5611 EP 5640 DI 10.1021/cr400573b PG 30 WC Chemistry, Multidisciplinary SC Chemistry GA AJ0JJ UT WOS:000337336500001 PM 24725101 ER PT J AU Ravcheev, DA Khoroshkin, MS Laikova, ON Tsoy, OV Sernova, NV Petrova, SA Rakhmaninova, AB Novichkov, PS Gelfand, MS Rodionov, DA AF Ravcheev, Dmitry A. Khoroshkin, Matvei S. Laikova, Olga N. Tsoy, Olga V. Sernova, Natalia V. Petrova, Svetlana A. Rakhmaninova, Aleksandra B. Novichkov, Pavel S. Gelfand, Mikhail S. Rodionov, Dmitry A. TI Comparative genomics and evolution of regulons of the Lacl-family transcription factors SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE bacteria; transcription factors; regulons; sugar metabolism; comparative genomics ID LACTOBACILLUS-PLANTARUM WCFS1; FACTOR-BINDING SITES; BACILLUS-SUBTILIS; REGULATORY NETWORKS; ESCHERICHIA-COLI; SPECIFICITY DETERMINANTS; FUNCTIONAL SPECIFICITY; STAPHYLOCOCCUS-AUREUS; GLUCONATE METABOLISM; PHYLOGENETIC TREES AB DNA-binding trascription factors (TFs) are essential components of transcriptional regulatory networks in bacteria. Lacl-family TFs (Lacl-TFs) are broadly distributed among certain lineages of bacteria. The majority of characterized Lacl-TFs sense sugar effectors and regulate carbohydrate utilization genes. The comparative genomics approaches enable in silico identification of TF-binding sites and reulon reconstruction. To study the function and evolution of Lacl-TFs, we performed genomics-based reconstruction and comparative analysis of their regulations. For over 1300 Lacl-TFs from over 270 bacterial genomies, we predicted their congnated DNA-binding mostifs and identified taged genes. Using the genome context and metabolic subsystem analyses of reconstructed teguions, we tentatively assigned funtional roles and predicted condidtate effectors fo 78 and 67% of the analyzed Lacl-TFs, respectively. Nearly 90% of the studid Lacl-TFs are local regulators of sugar utilization pathways, wherreas the remaining 125 global regulators control large and diverse sets of metabolic genes. The golobal Lacl-TFs include the previously known regulators CcpA in Firmicutes, FruR in Enterobacteria, and PurR in Gammaproteobacteria, as well as the three novel regulator-GluR, GapR, and PckR-that are predicted to control the central carbohydrate metabolism in three lieages of Alphaproteobacteria. Phylogenetic analysis of regulators combined with the reconstructed regulons provides a model of evolutionary diversitication of the Lacl protein family. The obtained genomic collection of in silico reconstructed Lacl-TF regulons n bacteria is available in the RegPrecise database (http://regprecise.lbl.gov.) It provides a framework for future structural and functional classification of the Lacl protein family and identification of molecular determinants of the DNA and ligand specificity. The inferred regulons can be also used for functional gene annotation and reconstruction of sugar catabolic networks in diverse bacterial lineages. C1 [Ravcheev, Dmitry A.; Khoroshkin, Matvei S.; Laikova, Olga N.; Tsoy, Olga V.; Sernova, Natalia V.; Petrova, Svetlana A.; Gelfand, Mikhail S.; Rodionov, Dmitry A.] Russian Acad Sci, Res Sci Ctr Bioinformat, AA Kharkevich Inst Informat Transmiss Problems, Moscow 127994, Russia. [Tsoy, Olga V.; Petrova, Svetlana A.; Rakhmaninova, Aleksandra B.] Moscow MV Lomonosov State Univ, Fac Bioengn & Bioinformat, Moscow, Russia. [Novichkov, Pavel S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Genom, Berkeley, CA 94720 USA. [Rodionov, Dmitry A.] Sanford Burnham Med Res Inst, Dept Bioinformat, La Jolla, CA 92093 USA. RP Gelfand, MS (reprint author), Russian Acad Sci, Res Sci Ctr Bioinformat, AA Kharkevich Inst Informat Transmiss Problems, 19-1 Bolshoi Karetny Pereulok, Moscow 127994, Russia. EM gelfand@iitp.ru; rodionov@sanfordburnham.org RI Ravcheev, Dmitry/B-5899-2013; Gelfand, Mikhail/F-3425-2012; Ravcheev, Dmitry/M-6877-2015 OI Ravcheev, Dmitry/0000-0002-8435-5516 FU Russian Foundation for Basic Research [14-04-00870, 14-04-91154]; Russian Academy of Sciences; Genomic Science Program (GSP); Office of Biological and Environmental Research (OBER); U.S. Department of Energy (DOE) FX This work was supported by the Russian Foundation for Basic Research (14-04-00870, 14-04-91154) and by the Russian Academy of Sciences via the programs "Molecular and Cellular Biology" and "Liveing Nature." This research was also partially supported by the Genomic Science Program (GSP), Office of Biological and Environmental Research (OBER), and U.S. Department of Energy (DOE) and is a contribution of the Pacific Northwest National Laboratory (PNNL) Foundational Scientific Focus Area. Prliminary reconstruction of regulons was done by students of the Spring 2013 Bioinformatics course at the Faculty of Bioengineering and Bioinformatics in the Lomonosov Moscow State University as a part of regular coursework. NR 92 TC 11 Z9 11 U1 2 U2 13 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUN 11 PY 2014 VL 5 AR 294 DI 10.3389/fmicb.2014.00294 PG 16 WC Microbiology SC Microbiology GA AJ2ZM UT WOS:000337534200001 PM 24966856 ER PT J AU Vjunov, A Fulton, JL Huthwelker, T Pin, S Mei, DH Schenter, GK Govind, N Camaioni, DM Hu, JZ Lercher, JA AF Vjunov, Aleksei Fulton, John L. Huthwelker, Thomas Pin, Sonia Mei, Donghai Schenter, Gregory K. Govind, Niranjan Camaioni, Donald M. Hu, Jian Zhi Lercher, Johannes A. TI Quantitatively Probing the Al Distribution in Zeolites SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HIGH-RESOLUTION AL-27; RAY-ABSORPTION SPECTROSCOPY; MQ MAS NMR; MOLECULAR-SIEVES; LOCAL-STRUCTURE; ACID CATALYSIS; RICH ZEOLITES; BASIS-SETS; T-SITES; BETA AB The degree of substitution of Si4+ by Al3+ in the oxygen-terminated tetrahedra (Al T-sites) of zeolites determines the concentration of ion-exchange and Bronsted acid sites. Because the location of the tetrahedra and the associated subtle variations in bond angles influence the acid strength, quantitative information about Al T-sites in the framework is critical to rationalize catalytic properties and to design new catalysts. A quantitative analysis is reported that uses a combination of extended X-ray absorption fine structure (EXAFS) analysis and Al-27 MAS NMR spectroscopy supported by DFT-based molecular dynamics simulations. To discriminate individual Al atoms, sets of ab initio EXAFS spectra for various T-sites are generated from DFT-based molecular dynamics simulations, allowing quantitative treatment of the EXAFS single- and multiple-photoelectron scattering processes out to 3-4 atom shells surrounding the Al absorption center. It is observed that identical zeolite types show dramatically different Al distributions. A preference of Al for T-sites that are part of one or more 4-member rings in the framework over those T-sites that are part of only 5- and 6-member rings in an HBEA150 zeolite has been determined using this analysis. C1 [Vjunov, Aleksei; Fulton, John L.; Mei, Donghai; Schenter, Gregory K.; Camaioni, Donald M.; Hu, Jian Zhi; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Govind, Niranjan] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Huthwelker, Thomas; Pin, Sonia] Paul Scherrer Inst, Lab Catalysis & Sustainable Chem LSK, Swiss Light Source, CH-5232 Villigen, Switzerland. [Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85748 Garching, Germany. [Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Inst, D-85748 Garching, Germany. RP Fulton, JL (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM john.fulton@pnnl.gov; johannes.lercher@pnnl.gov RI Schenter, Gregory/I-7655-2014; Mei, Donghai/A-2115-2012; Mei, Donghai/D-3251-2011; Hu, Jian Zhi/F-7126-2012 OI Schenter, Gregory/0000-0001-5444-5484; Mei, Donghai/0000-0002-0286-4182; FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; PNNL Chemical Imaging Initiative LDRD (Laboratory Directed Research and Development) Fund; DOE's Office of Biological and Environmental Research; DOE [DE-AC06-76RL0-1830] FX The Al EXAFS measurements were performed at the Swiss Light Source, Paul Scherrer Institute, Villigen, Switzerland. The authors thank M. Y. Hu and J. Feng (PNNL) for support during 27Al MAS NMR experiments. They also thank S. D. Burton (PNNL) for support during 29Si MAS NMR experiments. This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. N.G. acknowledges support from the PNNL Chemical Imaging Initiative LDRD (Laboratory Directed Research and Development) Fund. Sample preparation, NMR experiments, and a portion of the computations were performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research, located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for the DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RL0-1830. NR 73 TC 28 Z9 29 U1 18 U2 183 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 11 PY 2014 VL 136 IS 23 BP 8296 EP 8306 DI 10.1021/ja501361v PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA AJ0JM UT WOS:000337336800029 PM 24815517 ER PT J AU Srivastava, S Nykypanchuk, D Fukuto, M Halverson, JD Tkachenko, AV Yager, KG Gang, O AF Srivastava, Sunita Nykypanchuk, Dmytro Fukuto, Masafumi Halverson, Jonathan D. Tkachenko, Alexei V. Yager, Kevin G. Gang, Oleg TI Two-Dimensional DNA-Programmable Assembly of Nanoparticles at Liquid Interfaces SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AIR-WATER-INTERFACE; RAY REFLECTIVITY; MONOLAYERS; MEMBRANES; SURFACE; PHASE; CRYSTALLIZATION; TRANSITIONS; DYNAMICS; SYSTEMS AB DNA-driven assembly of nanoscale objects has emerged as a powerful platform for the creation of materials by design via self-assembly. Recent years have seen much progress in the experimental realization of this approach for three-dimensional systems. In contrast, two-dimensional (2D) programmable nanoparticle (NP) systems are not well explored, in part due to the difficulties in creating such systems. Here we demonstrate the use of charged liquid interfaces for the assembly and reorganization of 2D systems of DNA-coated NPs. The absorption of DNA-coated NPs to the surface is controlled by the interaction between a positively charged lipid layer and the negatively charged DNA shells of particles. At the same time, interparticle interactions are switchable, from electrostatic repulsion between DNA shells to attraction driven by DNA complementarity, by increasing ionic strength. Using in situ surface X-ray scattering methods and ex situ electron microscopy, we reveal the corresponding structural transformation of the NP monolayer, from a hexagonally ordered 2D lattice to string-like clusters and finally to a weakly ordered network of DNA cross-linked particles. Moreover, we demonstrate that the ability to regulate 2D morphology yields control of the interfacial rheological properties of the NP membrane: from viscous to elastic. Theoretical modeling suggests that the structural adaptivity of interparticle DNA linkages plays a crucial role in the observed 2D transformation of DNA-NP systems at liquid interfaces. C1 [Srivastava, Sunita; Nykypanchuk, Dmytro; Halverson, Jonathan D.; Tkachenko, Alexei V.; Yager, Kevin G.; Gang, Oleg] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Fukuto, Masafumi] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Gang, O (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM ogang@bnl.gov RI Yager, Kevin/F-9804-2011; Tkachenko, Alexei/I-9040-2012 OI Yager, Kevin/0000-0001-7745-2513; Tkachenko, Alexei/0000-0003-1291-243X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-98CH10886] FX We thank Prof. G. G. Fuller, Department of Chemistry, Stanford University, for help with interface rheological measurements. Research carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. M.F. acknowledges support by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-98CH10886. Use of the National Synchrotron Light Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 45 TC 26 Z9 26 U1 11 U2 99 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 11 PY 2014 VL 136 IS 23 BP 8323 EP 8332 DI 10.1021/ja501749b PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AJ0JM UT WOS:000337336800032 PM 24803304 ER PT J AU Li, JT Cushing, SK Zheng, P Senty, T Meng, FK Bristow, AD Manivannan, A Wu, NQ AF Li, Jiangtian Cushing, Scott K. Zheng, Peng Senty, Tess Meng, Fanke Bristow, Alan D. Manivannan, Ayyakkannu Wu, Nianqiang TI Solar Hydrogen Generation by a CdS-Au-TiO2 Sandwich Nanorod Array Enhanced with Au Nanoparticle as Electron Relay and Plasmonic Photosensitizer SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRANSIENT ABSORPTION-SPECTROSCOPY; NANOCRYSTALLINE TIO2 FILMS; SEMICONDUCTOR QUANTUM DOTS; P-N-JUNCTION; PHOTOCATALYTIC ACTIVITY; METAL NANOPARTICLES; Z-SCHEME; AUGER RECOMBINATION; GOLD NANOPARTICLES; CHARGE SEPARATION AB This paper presents a sandwich-structured CdSAu-TiO2 nanorod array as the photoanode in a photoelectrochemical cell (PEC) for hydrogen generation via splitting water. The gold nanoparticles sandwiched between the TiO2 nanorod and the CdS quantum dot (QD) layer play a dual role in enhancing the solar-to-chemical energy conversion efficiency. First, the Au nanoparticles serve as an electron relay, which facilitates the charge transfer between CdS and TiO2 when the CdS QDs are photoexcited by wavelengths shorter than 525 nm. Second, the Au nanoparticles act as a plasmonic photosensitizer, which enables the solar-to-hydrogen conversion at wavelengths longer than the band edge of CdS, extending the photoconversion wavelength from 525 to 725 nm. The dual role of Au leads to a photocurrent of 4.07 mA/cm(2) at 0 V (vs AglAgCl) under full solar spectrum irradiation and a maximum solar-to-chemical energy conversion efficiency of 2.8%. An inversion analysis is applied to the transient absorption spectroscopy data, tracking the transfer of electrons and holes in the heterostructure, relating the relaxation dynamics to the underlying coupled rate equation and revealing that trap-state Auger recombination is a dominant factor in interfacial charge transfer. It is found that addition of Au nanoparticles increases the charge-transfer lifetime, reduces the trap-state Auger rate, suppresses the long-time scale back transfer, and partially compensates the negative effects of the surface trap states. Finally, the plasmonic energy-transfer mechanism is identified as direct transfer of the plasmonic hot carriers, and the interfacial Schottky barrier height is shown to modulate the plasmonic hot electron transfer and back transfer. Transient absorption characterization of the charge transfer shows defect states cannot be ignored when designing QD-sensitized solar cells. This facile sandwich structure combines both the electrical and the optical functions of Au nanoparticles into a single structure, which has implications for the design of efficient solar-energy-harvesting devices. C1 [Li, Jiangtian; Cushing, Scott K.; Zheng, Peng; Meng, Fanke; Wu, Nianqiang] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Cushing, Scott K.; Senty, Tess; Bristow, Alan D.] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. [Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Wu, NQ (reprint author), W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. EM nick.wu@mail.wvu.edu RI Meng, Fanke /F-3978-2010; Wu, Nianqiang/B-9798-2015; Meng, Fanke/D-7395-2017; OI Wu, Nianqiang/0000-0002-8888-2444; Meng, Fanke/0000-0001-7961-4248; Zheng, Peng/0000-0001-5907-8505; Cushing, Scott/0000-0003-3538-2259 FU National Science Foundation [CBET-1233795]; NSF Graduate Research Fellowship [1102689]; NSF [EPS 1003907]; West Virginia University Research Corporation EPSCoR Grant FX This work was supported by the National Science Foundation (CBET-1233795) and NSF Graduate Research Fellowship (1102689). The resource and facilities used were partially supported by NSF (EPS 1003907), the West Virginia University Research Corporation EPSCoR Grant. The use of WVU Shared Facility was appreciated. NR 83 TC 146 Z9 147 U1 94 U2 689 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 11 PY 2014 VL 136 IS 23 BP 8438 EP 8449 DI 10.1021/ja503508g PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA AJ0JM UT WOS:000337336800045 PM 24836347 ER PT J AU Kong, M Albrecht, KO Shanks, BH Wheelock, TD AF Kong, Meng Albrecht, Karl O. Shanks, Brent H. Wheelock, Thomas D. TI Development of a Combined Catalyst and Sorbent for the Water Gas Shift Reaction SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID HYDROGEN-PRODUCTION; NI CATALYSTS; CO2 CAPTURE; CAO; METHANE AB A combined catalyst and sorbent was developed for reacting CO with steam to produce H-2 in a single reaction stage at 600 degrees C by employing the water gas shift (WGS) reaction. The combined material was in the form of spherical pellets where each pellet consisted of a CaO core for absorbing byproduct CO2 surrounded by a porous shell of Al2O3 which supported a Ni catalyst. The best results were achieved by incorporating 5 wt % limestone in the shell material to suppress coking. By employing the best core-in-shell pellets and supplying a 3:1 mol ratio of steam to CO at 600 degrees C, more than 97% of the CO was converted to H-2 by the WGS reaction and less than 1% was converted to CH4 by a side reaction. Also, none of the CO was converted to coke. C1 [Kong, Meng] Zhejiang Univ, Key Lab Appl Chem Zhejiang Prov, Inst Catalysis, Hangzhou 310028, Zhejiang, Peoples R China. [Albrecht, Karl O.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Shanks, Brent H.; Wheelock, Thomas D.] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. RP Wheelock, TD (reprint author), Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. EM wheel@iastate.edu NR 16 TC 1 Z9 1 U1 0 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUN 11 PY 2014 VL 53 IS 23 BP 9570 EP 9577 DI 10.1021/ie402607a PG 8 WC Engineering, Chemical SC Engineering GA AJ0JO UT WOS:000337337000006 ER PT J AU Srivastava, VK Quinlan, RA Agapov, AL Kisliuk, A Bhat, GS Mays, JW AF Srivastava, Vikram K. Quinlan, Ronald A. Agapov, Alexander L. Kisliuk, Alexander Bhat, Gajanan S. Mays, Jimmy W. TI High-Yield Synthesis of Mesoscopic Conductive and Dispersible Carbon Nanostructures via Ultrasonication of Commercial Precursors SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID LIQUID-PHASE EXFOLIATION; REDUCED GRAPHENE OXIDE; ORGANIC-SOLVENTS; GRAPHITE OXIDE; RAMAN-SPECTROSCOPY; AQUEOUS-SOLUTION; THIN-FILMS; REDUCTION; NANOSCROLLS; SOLUBILITY AB The need to produce large quantities of graphenic materials displaying excellent conductivity, thermal resistance, and tunable properties for industrial applications has spurred interest in new techniques for exfoliating graphite. In this paper, sonication-assisted exfoliation of graphitic precursors in the presence of chloroform is shown to produce chemically and structurally unique exfoliated graphitic materials in high yields. These exfoliated graphites, referred to as mesographite and mesographene, respectively, exhibit unique properties which depend on the number of layers and exfoliation conditions. Structural characterization of mesographene reveals the presence of nanoscale two-dimensional graphene layers, and three-dimensional carbon nanostructures sandwiched between layers, similar to those found in ball-milled and intercalated graphites. The conductivities of mesographite and mesographene are 2700 and 2000 S/m, respectively, indicating high conductivity despite flake damage. Optical absorption measurements of mesographite sonicated in various solvents showed significant changes in dispersion characteristics, and also indicated significant changes to mesoscopic colloidal behavior. A mechanism for functionalization and formation of capped carbon nanostructures is proposed by integrating the chemical and structural characterization in relation to the various carbon structures observed by electron microscopy. Composites based on common polymers were prepared by solution processing, and changes in thermal properties indicate improved dispersion of mesographite in polar polymers. C1 [Srivastava, Vikram K.; Agapov, Alexander L.; Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Bhat, Gajanan S.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Quinlan, Ronald A.] Naval Surface Warfare Ctr, Carderock Div, Bethesda, MD 20817 USA. [Kisliuk, Alexander; Mays, Jimmy W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Srivastava, VK (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM vsrivast@utk.edu; jimmy@utk.edu FU Office of Naval Research; Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences [DEAC05-00OR22725]; UT - Battelle, LLC, at Oak Ridge National Laboratory; Carderock Division of the Naval Surface Warfare Center's In-house Laboratory Independent Research Program [0601152N]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the Office of Naval Research. A.L.A., A.K., and J.W.M. acknowledge partial support from the Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DEAC05-00OR22725 with UT - Battelle, LLC, at Oak Ridge National Laboratory. R.A.Q, acknowledges financial support by the Carderock Division of the Naval Surface Warfare Center's In-house Laboratory Independent Research Program administrated under ONR's Program Element 0601152N. The XAS experiments were conducted at the National Synchrotron Light Source of Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. V.K.S. thanks Dr. John Dunlap for help in acquiring the TEM images. We thank Dr. Durairaj Baskaran for his contributions to the early stage of this project. NR 84 TC 0 Z9 0 U1 4 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUN 11 PY 2014 VL 53 IS 23 BP 9781 EP 9791 DI 10.1021/ie501659n PG 11 WC Engineering, Chemical SC Engineering GA AJ0JO UT WOS:000337337000029 ER PT J AU Mee, JK Raghunathan, R Wright, JB Lester, LF AF Mee, J. K. Raghunathan, R. Wright, J. B. Lester, L. F. TI Device geometry considerations for ridge waveguide quantum dot mode-locked lasers SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Review DE quantum dot; mode-locked laser; ridge waveguide; semicoductor laser; optical pulse generation ID LINEWIDTH ENHANCEMENT FACTOR; SEGMENTED CONTACT METHOD; SHORT-PULSE GENERATION; SEMICONDUCTOR-LASERS; OPTICAL PULSES; TIMING JITTER; DIODE-LASERS; HIGH-SPEED; GAIN; NOISE AB Quantum dot mode-locked lasers have emerged as a leading source for the efficient generation of high-quality optical pulses from a compact package, attracting considerable attention for support of multiple high-speed applications, owing to characteristics such as low noise operation and high pulse peak power, in addition to the ability to multiplex the output pulse train in temporal and frequency domains in order to obtain hundreds of GHz pulse repetition rates potentially operating at 1 Tbps. This topical review provides a detailed explanation into the primary advantages of quantum dots, identifying the key features that have made them superior to other material systems for passive mode-locking in semiconductor lasers. Following this account, the impact of the device's cavity geometry on the operational range of two-section, monolithic passively mode-locked lasers is investigated both experimentally and analytically. A model is described that predicts regimes of pulsed operation as a function of absorber length to gain length ratio. Experimental measurements of the pulse time-domain characteristics over a wide range of operating temperatures are found to be in excellent agreement with analytical predictions. The impact of ridge waveguide design on the operational range is also examined and the key dimensions that most strongly impact efficient operation are identified. C1 [Mee, J. K.] Air Force Res Lab, Space Elect Branch, Kirtland AFB, NM 87117 USA. [Raghunathan, R.; Lester, L. F.] Virginia Polytech Inst & State Univ, Bradley Dept Elect & Comp Engn, Blacksburg, VA 24061 USA. [Wright, J. B.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Mee, JK (reprint author), Air Force Res Lab, Space Elect Branch, Kirtland AFB, NM 87117 USA. FU Air Force Research Laboratory, AFOSR [FA9550-10-1-0276, FA9550-10-1-0463]; NSF [ECCS-0903448]; SRC [SRC-2009-HJ-2000]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported in part by the Air Force Research Laboratory, AFOSR under grants FA9550-10-1-0276 and FA9550-10-1-0463, the NSF under grant ECCS-0903448 and by the SRC under contract SRC-2009-HJ-2000. This work was also performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 77 TC 3 Z9 3 U1 1 U2 21 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD JUN 11 PY 2014 VL 47 IS 23 AR 233001 DI 10.1088/0022-3727/47/23/233001 PG 16 WC Physics, Applied SC Physics GA AI3TH UT WOS:000336785800001 ER PT J AU Hernandez, SC Schwartz, DS Taylor, CD Ray, AK AF Hernandez, Sarah C. Schwartz, Daniel S. Taylor, Christopher D. Ray, Asok K. TI Ab initio study of gallium stabilized delta-plutonium alloys and hydrogen-vacancy complexes SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE electronic structure; density functional theory; gallium-stabilized delta-plutonium; vacancy; hydrogen ID GENERALIZED GRADIENT APPROXIMATION; PU-GA ALLOYS; STRUCTURAL STABILITIES; PHASE-STABILITY; GROUND-STATE; PRESSURE; SPECTROSCOPY; COLLAPSE; PA; NP AB All-electron density functional theory was used to investigate delta-plutonium (delta-Pu) alloyed with gallium (Ga) impurities at 3.125, 6.25, 9.375 atomic (at)% Ga concentrations. The results indicated that the lowest energy structure is anti-ferromagnetic, independent of the Ga concentration. At higher Ga concentrations (>3.125 at%), the position of the Ga atoms are separated by four nearest neighbor Pu-Pu shells. The results also showed that the lattice constant contracts with increasing Ga concentration, which is in agreement with experimental data. Furthermore with increasing Ga concentration, the face-centered-cubic structure becomes more stably coupled with increasing short-range disorder. The formation energies show that the alloying process is exothermic, with an energy range of -0.028 to -0.099 eV/atom. The analyses of the partial density of states indicated that the Pu-Ga interactions are dominated by Pu 6d and Ga 4p hybridizations, as well as Ga 4s-4p hybridizations. Finally, the computed formation energies for vacancy and hydrogen-vacancy complexes within the 3.125 at% Ga cell were 1.12 eV (endothermic) and -3.88 eV (exothermic), respectively. In addition, the hydrogen atom prefers to interact much more strongly to the Pu atom than the Ga atom in the hydrogen-vacancy complex. C1 [Hernandez, Sarah C.; Ray, Asok K.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Schwartz, Daniel S.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Taylor, Christopher D.] DNV GL, Dublin, OH 43017 USA. [Taylor, Christopher D.] Ohio State Univ, Fontana Corros Ctr, Columbus, OH 43210 USA. RP Hernandez, SC (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. EM sarahchernandez@mavs.uta.edu FU US Department of Energy through the Los Alamos National Laboratory LDRD Program; Welch Foundation [Y-1525] FX This work was supported by the US Department of Energy through the Los Alamos National Laboratory LDRD Program and the Welch Foundation (grant no. Y-1525). Computational support from the Texas Advanced Computing Center (www.tacc.utexas.edu) and the University of Texas at Arlington supercomputing facilities are also gratefully acknowledged. SCH would also like to gratefully acknowledge discussions with Dr Raymond Atta-Fynn and Dr Muhammad Huda. This work is dedicated to the memory of Professor Asok K Ray. He will be remembered for his significant contribution to the field of theoretical actinide physics and chemistry. NR 52 TC 6 Z9 6 U1 1 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUN 11 PY 2014 VL 26 IS 23 AR 235502 DI 10.1088/0953-8984/26/23/235502 PG 14 WC Physics, Condensed Matter SC Physics GA AH8LR UT WOS:000336389800007 PM 24832613 ER PT J AU Zagatto, VAB Oliveira, JRB Allegro, PRP Chamon, LC Cybulska, EW Medina, NH Ribas, RV Seale, WA Silva, CP Gasques, LR Zahn, GS Genezini, FA Shorto, JMB Lubian, J Linares, R Toufen, DL Silveira, MAG Rossi, ES Nobre, GP AF Zagatto, V. A. B. Oliveira, J. R. B. Allegro, P. R. P. Chamon, L. C. Cybulska, E. W. Medina, N. H. Ribas, R. V. Seale, W. A. Silva, C. P. Gasques, L. R. Zahn, G. S. Genezini, F. A. Shorto, J. M. B. Lubian, J. Linares, R. Toufen, D. L. Silveira, M. A. G. Rossi, E. S., Jr. Nobre, G. P. TI gamma-Particle coincidence technique for the study of nuclear reactions SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE gamma-Ray spectrometer; gamma-Particle coincidence; Inelastic reactions AB The Saci-Perere gamma ray spectrometer (located at the Pelletron AcceleratorLaboratory - IFUSP) was employed to implement the gamma-particle coincidence technique for the study of nuclear reaction mechanisms. For this, the O-18+Pd-110 reaction has been studied in the beam energy range of 45-54 MeV. Several corrections to the data due to various effects (energy and angle integrations, beam spot size, gamma detector finite size and the vacuum dealignment) are small and well controlled. The aim of this work was to establish a proper method to analyze the data and identify the reaction mechanisms involved. To achieve this goal the inelastic scattering to the first excited state of Pd-110 has been extracted and compared to coupled channel calculations using the Sao Paulo Potential (PSP), being reasonably well described by it. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zagatto, V. A. B.; Oliveira, J. R. B.; Allegro, P. R. P.; Chamon, L. C.; Cybulska, E. W.; Medina, N. H.; Ribas, R. V.; Seale, W. A.; Silva, C. P.; Gasques, L. R.] Univ Sao Paulo, Inst Fis, BR-05508 Sao Paulo, Brazil. [Zahn, G. S.; Genezini, F. A.; Shorto, J. M. B.] Inst Pesquisas Energet & Nucl, Sao Paulo, Brazil. [Lubian, J.; Linares, R.] Univ Fed Fluminense, Inst Fis, BR-24220000 Niteroi, RJ, Brazil. [Toufen, D. L.] Inst Fed Educ Ciencia & Tecnol, Fortaleza, Ceara, Brazil. [Nobre, G. P.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Zagatto, VAB (reprint author), Univ Sao Paulo, Inst Fis, BR-05508 Sao Paulo, Brazil. EM vinicius.zagatto@gmail.com RI Chamon, Luiz/N-4591-2014; Shorto, Julian/I-3870-2013; Oliveira, Jose Roberto/J-3124-2012; Gasques, Leandro Romero/E-2530-2012; Toufen, Dennis/I-5131-2012; Medina, Nilberto/D-8992-2012 OI Oliveira, Jose Roberto/0000-0003-1362-7382; Medina, Nilberto/0000-0003-0650-6507 FU FAPESP; Cnpq; CAPES, Brazil FX This work was supported by FAPESP, Cnpq and CAPES, Brazil. NR 8 TC 1 Z9 1 U1 2 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUN 11 PY 2014 VL 749 BP 19 EP 26 DI 10.1016/j.nima.2014.02.014 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AE6CC UT WOS:000334075000004 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Liang, D Liang, S Meng, X Plestina, R Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Hempel, M Horton, D Jung, H Kasemann, M Katsas, P Kieseler, J Kleinwort, C Kramer, M Krucker, D Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schmidt, R Schoerner-Sadenius, T Schroder, M Stein, M Trevino, ADRV Walsh, R Wissing, C Martin, MA Blobel, V Draeger, AR Enderle, H Erfle, J Garutti, E Goebel, K Gorner, M Gosselink, M Haller, J Hoing, RS Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Kornmayer, A Kuznetsova, E Pardo, PL Martschei, D Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Psallidas, A Topsis-giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Jones, J Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A 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CA CMS Collaboration TI Search for new physics in the multijet and missing transverse momentum final state in proton-proton collisions at root s=8 Tev SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry; Hadron-Hadron Scattering ID GRAND UNIFICATION; SQUARK; LHC; SUPERSYMMETRY; BOSON; MASS AB A search for new physics is performed in multijet events with large missing transverse momentum produced in proton-proton collisions at root s = 8TeV using a data sample corresponding to an integrated luminosity of 19.5 fb(-1) collected with the CMS detector at the LHC. The data sample is divided into three jet multiplicity categories (3-5, 6-7, and >= 8 jets), and studied further in bins of two variables: the scalar sum of jet transverse momenta and the missing transverse momentum. The observed numbers of events in various categories are consistent with backgrounds expected from standard model processes. 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U.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Psallidas, A.; Topsis-giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Jones, J.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. 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S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. 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[Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. 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[Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. 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[Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Dubna Joint Nucl Res Inst, Dubna 141980, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. 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A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; Pelliccioni, M.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Theofilatos, K.; Treille, D.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Favaro, C.; Hinzmann, A.; Hreus, T.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Ctr Nat Sci, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Abdulsalam, A.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Schleper, P.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdulsalam, A.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swart, M.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Yoo, J.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, MN USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Sakharov, A.; Sarangi, T.; Savin, A.; Smith, W. 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My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Codispoti, Giuseppe/0000-0003-0217-7021; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Gonzalez Caballero, Isidro/0000-0002-8087-3199; Calvo Alamillo, Enrique/0000-0002-1100-2963; Dudko, Lev/0000-0002-4462-3192; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; FU CERN accelerator departments; LHC; LHC and thank the technical and administrative staffs at CERN; CMS institutes; computing centres and personnel of the Worldwide LHC Computing Grid; BMWF; FWF; FNRS; FWO; CNPq; CAPES; FAPERJ; FAPESP; MES; CERN; CAS; MoST; NSFC; COLCIENCIAS; MSES; CSF; RPF; MoER [SF0690030s09]; ERDF; Academy of Finland; MEC; HIP; CEA; CNRS [IN2P3]; BMBF; DFG; HGF; GSRT; OTKA; NIH; DAE; DST; IPM; SFI; INFN; NRF; WCU; LAS; MOE and UM; CINVESTAV; CONACYT; SEP; UASLP-FAI; MBIE; PAEC; MSHE; NSC; FCT; JINR; MON; RAS and RFBR; MESTD; SEIDI and CPAN; Swiss Funding Agencies; ThEPCenter; IPST; STAR; NSTDA; TUBITAK; TAEK; NASU; STFC; DOE and NSF; Marie-Curie programme; European Research Council; EPLANET; Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation ` a la Recherche dans l'Industrie et dans l'Agriculture; Agentschap voor Innovatie door Wetenschap en Technologie; Ministry of Education, Youth and Sports (MEYS); Council of Science and Industrial Research; Compagnia di San Paolo; HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis and Aristeia programmes; EU-ESF and the Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/ IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (U. S. A.).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation ` a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 62 TC 34 Z9 34 U1 6 U2 73 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 10 PY 2014 IS 6 AR 055 DI 10.1007/JHEP06(2014)055 PG 38 WC Physics, Particles & Fields SC Physics GA AJ9KK UT WOS:000338028800001 ER PT J AU Ren, J Fransson, J Zhu, JX AF Ren, Jie Fransson, Jonas Zhu, Jian-Xin TI Nanoscale Spin Seebeck Rectifier: Controlling Thermal Spin Transport across Insulating Magnetic Junctions with Localized Spin SO PHYSICAL REVIEW B LA English DT Article ID SINGLE-MOLECULE MAGNETS; SPINTRONICS; EFFICIENCY AB The spin Seebeck effect is studied across a charge insulating magnetic junction, in which thermal-spin conjugate transport is assisted by the exchange interactions between the localized spin in the center and electrons in metallic leads. We show that, in contrast with bulk spin Seebeck effect, the figure of merit of such nanoscale thermal-spin conversion can be infinite, leading to the ideal Carnot efficiency in the linear response regime. We also find that in the nonlinear spin Seebeck transport regime the device possesses the asymmetric and negative differential spin Seebeck effects. In the last, the situations with leaking electron tunneling are also discussed. This nanoscale thermal spin rectifier, by tuning the junction parameters, can act as a spin Seebeck diode, spin Seebeck transistor, and spin Seebeck switch, which could have substantial implications for flexible thermal and information control in molecular spin caloritronics. C1 [Ren, Jie; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Fransson, Jonas] Uppsala Univ, Dept Phys & Astron, SE-75121 Uppsala, Sweden. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Ren, J (reprint author), MIT, Dept Chem, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM jieustc@gmail.com RI Ren, Jie/G-5314-2010 OI Ren, Jie/0000-0003-2806-7226 FU National Nuclear Security Administration of the U.S. Department of Energy (DOE) at Los Alamos National Laboratory (LANL) [DE-AC52-06NA25396]; LANL Laboratory Directed Research Development Program; Swedish Research Council and Wenner-Gren Foundation; Center for Integrated Nanotechnologies; U.S. DOE Office of Basic Energy Sciences FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy (DOE) at Los Alamos National Laboratory (LANL) under Contract No. DE-AC52-06NA25396 and supported by the LANL Laboratory Directed Research Development Program (J.R.), and the Swedish Research Council and Wenner-Gren Foundation are also acknowledged (J.F.). The work was supported, in part, by the Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences user facility (J.-X. Z.). J.R. thanks J. Thingna for bringing [20] to our attention. NR 64 TC 13 Z9 13 U1 3 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUN 10 PY 2014 VL 89 IS 21 AR 214407 DI 10.1103/PhysRevB.89.214407 PG 8 WC Physics, Condensed Matter SC Physics GA AJ9GT UT WOS:000338016600001 ER PT J AU Ethier, JJ Doshi, N Malace, S Melnitchouk, W AF Ethier, J. J. Doshi, N. Malace, S. Melnitchouk, W. TI Quasielastic electron-deuteron scattering in the weak-binding approximation SO PHYSICAL REVIEW C LA English DT Article ID DEEP-INELASTIC-SCATTERING; NUCLEAR-STRUCTURE FUNCTIONS; HIGH MOMENTUM-TRANSFER; CROSS-SECTIONS AB We perform a global analysis of all available electron-deuteron (ed) quasielastic scattering data using Q(2)-dependent smearing functions that describe inclusive inelastic ed scattering within the weak-binding approximation. We study the dependence of the cross sections on the deuteron wave function and the off-shell extrapolation of the elastic electron-nucleon cross sections, which show particular sensitivity at x >> 1. The excellent overall agreement with data over a large range of Q(2) and x suggests a limited need for effects beyond the impulse approximation, with the exception of the very high-x and very low-Q(2) regions, where short-range meson exchange and final state interaction effects become more relevant. C1 [Ethier, J. J.; Doshi, N.; Malace, S.; Melnitchouk, W.] Jefferson Lab, Newport News, VA 23606 USA. [Ethier, J. J.] Coll William & Mary, Dept Phys, Williamsburg, VA 23185 USA. [Doshi, N.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. RP Ethier, JJ (reprint author), Jefferson Lab, 12000 Jefferson Ave, Newport News, VA 23606 USA. FU U.S. DOE [DE-AC05-06OR23177]; DOD's ASSURE program; NSF [1062320] FX We thank J. Arrington, D. Day, S. Kulagin, A. Lung, and J. W. Van Orden for helpful discussions and communications. This work was supported by the U.S. DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, operates Jefferson Lab. N.D. acknowledges support from DOD's ASSURE program and NSF Grant No. 1062320 for an REU internship at ODU/Jefferson Lab. NR 52 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 10 PY 2014 VL 89 IS 6 AR 065203 DI 10.1103/PhysRevC.89.065203 PG 12 WC Physics, Nuclear SC Physics GA AJ9HG UT WOS:000338018300008 ER PT J AU Gross, F AF Gross, Franz TI Covariant spectator theory of np scattering: Deuteron magnetic moment SO PHYSICAL REVIEW C LA English DT Article ID MESON-EXCHANGE CURRENTS; ELECTROMAGNETIC STRUCTURE; FORM-FACTORS; MODEL; EQUATIONS; ENERGY AB The deuteron magnetic moment is calculated using two model wave functions obtained from 2007 high-precision fits to np scattering data. Included in the calculation are a new class of isoscalar np interaction currents, which are automatically generated by the nuclear force model used in these fits. After normalizing the wave functions, nearly identical predictions are obtained: model WJC-1, with larger relativistic P-state components, gives 0.863(2), while model WJC-2 with very small P-state components gives 0.864(2). These are about 1% larger than the measured value of the moment, 0.857 n.m., giving a new CST prediction for the size of the rho pi gamma exchange, and other purely transverse interaction currents that are largely unconstrained by the nuclear dynamics. The physical significance of these results is discussed, and general formulas for the deuteron form factors, expressed in terms of deuteron wave functions and a new class of interaction current wave functions, are given. C1 [Gross, Franz] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Gross, Franz] Coll William & Mary, Williamsburg, VA 23185 USA. RP Gross, F (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM gross@jlab.org FU Jefferson Science Associates, LLC, under U.S. DOE [DE-AC0506OR23177] FX This work was partially supported by Jefferson Science Associates, LLC, under U.S. DOE Contract No. DE-AC0506OR23177. NR 23 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 10 PY 2014 VL 89 IS 6 AR 064002 DI 10.1103/PhysRevC.89.064002 PG 27 WC Physics, Nuclear SC Physics GA AJ9HG UT WOS:000338018300003 ER PT J AU Gross, F AF Gross, Franz TI Covariant spectator theory of np scattering: Isoscalar interaction currents SO PHYSICAL REVIEW C LA English DT Article ID ELECTRON-DEUTERON SCATTERING; ELECTROMAGNETIC FORM FACTOR; BOSON-EXCHANGE MODEL; 3-BODY BOUND-STATE; RELATIVISTIC CALCULATION; MOMENTUM-TRANSFER; VERTEX FUNCTION; EQUATIONS; SYSTEMS; ENERGY AB Using the covariant spectator theory (CST), one boson exchange models have been found that give precision fits to low-energy np scattering and the deuteron binding energy. The boson-nucleon vertices used in these models contain a momentum dependence that requires a new class of interaction currents for use with electromagnetic interactions. Current conservation requires that these new interaction currents satisfy a two-body Ward-Takahashi identity, and using principals of simplicity and picture independence, these currents can be uniquely determined. The results lead to general formulas for a two-body current that can be expressed in terms of relativistic np wave functions, Psi, and two convenient truncated wave functions, Psi((2)) and (Psi) over cap, which contain all of the information needed for the explicit evaluation of the contributions from the interaction current. These three wave functions can be calculated from the CST bound- or scattering-state equations (and their off-shell extrapolations). A companion paper uses this formalism to evaluate the deuteron magnetic moment. C1 [Gross, Franz] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Gross, Franz] Coll William & Mary, Williamsburg, VA 23185 USA. RP Gross, F (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM gross@jlab.org FU Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX It is a pleasure to acknowledge helpful conversations with J. W. Van Orden, who also contributed to the early stages of this work. This work was partially support by Jefferson Science Associates, LLC, under U.S. DOE Contract No. DE-AC05-06OR23177. NR 33 TC 2 Z9 2 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 10 PY 2014 VL 89 IS 6 AR 064001 DI 10.1103/PhysRevC.89.064001 PG 23 WC Physics, Nuclear SC Physics GA AJ9HG UT WOS:000338018300002 ER PT J AU Henderson, J Jenkins, DG Davies, PJ Alcorta, M Carpenter, MP Kay, BP Lister, CJ Zhu, S AF Henderson, J. Jenkins, D. G. Davies, P. J. Alcorta, M. Carpenter, M. P. Kay, B. P. Lister, C. J. Zhu, S. TI Upper limit on the two-photon emission branch for the 0(2)(+) -> 0(1)(+) transition in Mo-98 SO PHYSICAL REVIEW C LA English DT Article ID DOUBLE GAMMA-DECAY; ZR-90 AB Background: Two-photon emission, while well known in atomic physics, is a rare second-order process in nuclear physics with only three cases where a two-photon branch is measured. The limited knowledge stems from the experimental difficulty in resolving two-photon emission from dominant single-photon emission, restricting practical cases for study to 0(+) -> 0(+) (E0) transitions, since single-photon emission is forbidden. In practical terms, this limits the range of easily accessible cases to even-even nuclei with the unusual property of a first excited state with spin/parity of 0+. Purpose: Two-photon branches are measured for the closed-shell nuclei, O-16, Ca-40, and Zr-90. The intention of the present work was to obtain data for a case which was not a closed-shell nucleus. Of the possible nuclei relevant to such a study, Mo-98 was chosen as its first-excited state is 0(+) and lies below 1 MeV, meaning that internal pair transitions are not allowed. Method: The first excited state (J(pi) = 0(+)) in Mo-98 was excited in resonant inelastic proton scattering using a 6.7-MeV proton beam. The population of the state was selected using an annular double-sided silicon strip detector (DSSD). The decay of the state by conversion electrons was observed using the same DSSD, while Gammasphere was used to detect possible two-photon events. Results: An upper limit on the two-photon branch obtained was 1 x 10(-4) at the 95% confidence level (CL). Conclusions The upper limit obtained is smaller than any other previously obtained two-photon branch. Phase space considerations suggest that the actual value of the branching ratio in this case may be significantly smaller than the upper limit obtained. C1 [Henderson, J.; Jenkins, D. G.; Davies, P. J.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Jenkins, D. G.] Univ Strasbourg, Inst Adv Study, Strasbourg, France. [Alcorta, M.; Carpenter, M. P.; Kay, B. P.; Lister, C. J.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Henderson, J (reprint author), Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. RI Henderson, Jack/E-4326-2015; Carpenter, Michael/E-4287-2015; Alcorta, Martin/G-7107-2011 OI Henderson, Jack/0000-0002-6010-9644; Carpenter, Michael/0000-0002-3237-5734; Alcorta, Martin/0000-0002-6217-5004 FU UK Science and Technology Facilities Council; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX The authors would like to acknowledge the work of the ATLAS operators and of John Greene for preparing the target. This work was supported by the UK Science and Technology Facilities Council and the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 19 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 10 PY 2014 VL 89 IS 6 AR 064307 DI 10.1103/PhysRevC.89.064307 PG 5 WC Physics, Nuclear SC Physics GA AJ9HG UT WOS:000338018300006 ER PT J AU Kumbartzki, GJ Benczer-Koller, N Burcher, S Ratkiewicz, A Rice, SL Sharon, YY Zamick, L Speidel, KH Torres, DA Sieja, K McCleskey, M Cudd, A Henry, M Saastamoinen, A Slater, M Spiridon, A Torilov, SY Zherebchevsky, VI Gurdal, G Robinson, SJQ Pain, SD Burke, JT AF Kumbartzki, G. J. Benczer-Koller, N. Burcher, S. Ratkiewicz, A. Rice, S. L. Sharon, Y. Y. Zamick, L. Speidel, K. -H. Torres, D. A. Sieja, K. McCleskey, M. Cudd, A. Henry, M. Saastamoinen, A. Slater, M. Spiridon, A. Torilov, S. Yu. Zherebchevsky, V. I. Guerdal, G. Robinson, S. J. Q. Pain, S. D. Burke, J. T. TI Transition from collectivity to single-particle degrees of freedom from magnetic moment measurements on Sr-82(38)44 and Sr-90(38)52 SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; STATES; DEPENDENCE; CLOSURE AB Background: The Sr-88(38) and Zr-90(40) nuclei have been utilized as closed cores for large-scale shell-model calculations in the 28 <= Z <= 50 region around the N = 50 shell. Measurements of magnetic moments for nuclei in this region would provide microscopic information about the use of Sr-88 and Zr-90 as stable closed-core nuclei. While the g factors of the 2(1)(+) states in the stable Sr isotopes have been previously measured, experimental g factors for the radioactive Sr-82,Sr-90 have not been obtained to date. Purpose: The purpose was to measure the g factors of the 2(1)(+) and 4(1)(+) states in the unstable Sr-82 and Sr-90 nuclei in order to extend the systematics along the Sr isotopic chain. A comparison of the structure of the N = 52 isotopes Sr-90 and Zr-92 will shed light on the relative robustness of proton subshell closures at Z = 38 and Z = 40. Methods: The pickup reaction of alpha particles in inverse kinematics together with the transient field technique were applied to beams of Kr-78 and Kr-86 at the Cyclotron Institute of Texas A&M University. Results: The values g(Sr-82; 2(1)(+)) = +0.44(19), g(Sr-82; 4(1)(+)) = +0.53(39), g(Sr-90; 2(1)(+)) = -0.12(11), and g(Sr-90; 4(1)(+)) = -0.02(17) were measured for the first time. Simultaneously, the g factors of the low-lying states in the Coulomb-excited beam projectiles were remeasured. The g(4(1)(+)) = +1.03(14) in Kr-86 was also measured for the first time. Conclusions: For Sr-82 both g factors are in agreement with the collective value Z/A expected for nuclei in the middle of a major shell. The g factors in Sr-90 are negative but smaller than in the isotone Zr-92. The results also indicate that Sr-88 is a proton-soft core nucleus and perhaps even softer than Zr-90. C1 [Kumbartzki, G. J.; Benczer-Koller, N.; Burcher, S.; Ratkiewicz, A.; Rice, S. L.; Sharon, Y. Y.; Zamick, L.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. [Speidel, K. -H.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Torres, D. A.] Univ Nacl Colombia, Dept Fis, Bogota, Colombia. [Sieja, K.] Univ Strasbourg, IPHC, CNRS, UMR7178, F-67037 Strasbourg, France. [McCleskey, M.; Cudd, A.; Henry, M.; Saastamoinen, A.; Slater, M.; Spiridon, A.; Torilov, S. Yu.; Zherebchevsky, V. I.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Guerdal, G.; Robinson, S. J. Q.] Millsaps Coll, Dept Phys, Jackson, MS 39210 USA. [Pain, S. D.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Burke, J. T.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Kumbartzki, GJ (reprint author), Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. EM kum@physics.rutgers.edu RI Torilov, Sergey/I-6325-2013; Pain, Steven/E-1188-2011; Zherebchevsky, Vladimir/F-5515-2014 OI Torilov, Sergey/0000-0001-6566-7525; Pain, Steven/0000-0003-3081-688X; Zherebchevsky, Vladimir/0000-0002-6021-5113 FU Rutgers; COLCIENCIAS Travel [613-2013]; Universidad Nacional de Colombia and Rutgers; US National Science Foundation; Lawrence Livermore National Security, LLCL [DE-AC52-07NA27344]; Department of Energy's NNSA Office of Defense Nuclear Nonproliferation Research and Development; US Department of Energy Office [DE-FG02-93ER40773, DE-NA0001785] FX The experimental work was done at the Texas A&M Cyclotron Institute; the help of local students, postdoctoral fellows, and staff is greatly appreciated. K.-H. S. is grateful for travel support from Rutgers. D.A.T. is thankful for support from COLCIENCIAS Travel Grant No. 613-2013 and for financial support from Universidad Nacional de Colombia and Rutgers. This work was supported in part by the US National Science Foundation, by US Department of Energy Office Grants No. DE-FG02-93ER40773 and No. DE-NA0001785, by Lawrence Livermore National Security, LLCL, under Contract No. DE-AC52-07NA27344, and by the Department of Energy's NNSA Office of Defense Nuclear Nonproliferation Research and Development. NR 31 TC 8 Z9 8 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 10 PY 2014 VL 89 IS 6 AR 064305 DI 10.1103/PhysRevC.89.064305 PG 9 WC Physics, Nuclear SC Physics GA AJ9HG UT WOS:000338018300004 ER PT J AU Sakai, H Tokunaga, Y Kambe, S Urbano, RR Suzuki, MT Kuhns, PL Reyes, AP Tobash, PH Ronning, F Bauer, ED Thompson, JD AF Sakai, H. Tokunaga, Y. Kambe, S. Urbano, R. R. Suzuki, M. -T. Kuhns, P. L. Reyes, A. P. Tobash, P. H. Ronning, F. Bauer, E. D. Thompson, J. D. TI Emergent Antiferromagnetism out of the "Hidden-Order" State in URu2Si2: High Magnetic Field Nuclear Magnetic Resonance to 40 T SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERCONDUCTOR URU2SI2; CERH2SI2; PRESSURE; NMR AB Very high field Si-29-NMR measurements using a fully Si-29-enriched URu2Si2 single crystal were carried out in order to microscopically investigate the "hidden order" (HO) state and adjacent magnetic phases in the high field limit. At the lowest measured temperature of 0.4 K, a clear anomaly reflecting a Fermi surface instability near 22 T inside the HO state is detected by the Si-29 shift, K-29(c) Moreover, a strong enhancement of K-29(c) develops near a critical field H-c similar or equal to 35.6 T, and the Si-29-NMR signal disappears suddenly at H-c, indicating the total suppression of the HO state. Nevertheless, a weak and shifted Si-29-NMR signal reappears for fields higher than H-c at 4.2 K, providing evidence for a magnetic structure within the magnetic phase caused by the Ising-type anisotropy of the uranium ordered moments. C1 [Sakai, H.; Tokunaga, Y.; Kambe, S.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Urbano, R. R.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil. [Urbano, R. R.; Kuhns, P. L.; Reyes, A. P.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Suzuki, M. -T.] Japan Atom Energy Agcy, CCSE, Kashiwa, Chiba 2778587, Japan. [Tobash, P. H.; Ronning, F.; Bauer, E. D.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Sakai, H (reprint author), Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. EM sakai.hironori@jaea.go.jp RI Suzuki, Michi-To/G-6298-2013; Inst. of Physics, Gleb Wataghin/A-9780-2017; OI Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU NSF [DMR-0654118]; State of Florida; FAPESP [2012/05903-6] FX We thank H. Ikeda, K. Kuwahara, D. Aoki, and K. Sugiyama for valuable discussions. Work in Japan was supported by the Reimei Research Program of JAEA. Work at NHMFL was performed under the auspices of the NSF through the Cooperative Agreement No. DMR-0654118 and the State of Florida. R. R. U. also acknowledges FAPESP (No. 2012/05903-6). Work at LANL was performed under the auspices of the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 21 TC 1 Z9 1 U1 4 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 10 PY 2014 VL 112 IS 23 AR 236401 DI 10.1103/PhysRevLett.112.236401 PG 5 WC Physics, Multidisciplinary SC Physics GA AJ9HY UT WOS:000338020500006 ER PT J AU Chong, J Xun, SD Zhang, JP Song, XY Xie, HM Battaglia, V Wang, RS AF Chong, Jin Xun, Shidi Zhang, Jingping Song, Xiangyun Xie, Haiming Battaglia, Vincent Wang, Rongshun TI Li3PO4-Coated LiNi0.5Mn1.5O4: A Stable High-Voltage Cathode Material for Lithium-Ion Batteries SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE interfaces; Li3PO4; LiNi0.5Mn1.5O4; lithium-ion batteries; solid-state reactions ID LONG CYCLE LIFE; ELECTROCHEMICAL PROPERTIES; COATED LINI0.5MN1.5O4; SPINEL LINI0.5MN1.5O4; ELEVATED-TEMPERATURES; SECONDARY BATTERIES; RATE CAPABILITY; PERFORMANCE; METAL; INSERTION AB LiNi0.5Mn1.5O4 is regarded as a promising cathode material to increase the energy density of lithium-ion batteries due to the high discharge voltage (ca. 4.7 V). However, the interface between the LiNi0.5Mn1.5O4 cathode and the electrolyte is a great concern because of the decomposition of the electrolyte on the cathode surface at high operational potentials. To build a stable and functional protecting layer of Li3PO4 on LiNi0.5Mn1.5O4 to avoid direct contact between the active materials and the electrolyte is the emphasis of this study. Li3PO4-coated LiNi0.5Mn1.5O4 is prepared by a solid-state reaction and noncoated LiNi0.5Mn1.5O4 is prepared by the same method as a control. The materials are fully characterized by XRD, FT-IR, and high-resolution TEM. TEM shows that the Li3PO4 layer (<6 nm) is successfully coated on the LiNi0.5Mn1.5O4 primary particles. XRD and FT-IR reveal that the synthesized Li3PO4-coated LiNi0.5Mn1.5O4 has a cubic spinel structure with a space group of Fd<(3)over bar>m, whereas noncoated LiNi0.5Mn1.5O4 shows a cubic spinel structure with a space group of P4(3)32. The electrochemical performance of the prepared materials is characterized in half and full cells. Li3PO4-coated LiNi0.5Mn1.5O4 shows dramatically enhanced cycling performance compared with noncoated LiNi0.5Mn1.5O4. C1 [Chong, Jin; Zhang, Jingping; Xie, Haiming; Wang, Rongshun] NE Normal Univ, Inst Funct Mat Chem, Fac Chem Natl & Local United Engn Lab Power Batte, Changchun 130024, Jilin, Peoples R China. [Xun, Shidi; Song, Xiangyun; Battaglia, Vincent] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Xun, SD (reprint author), DuPont Cent Res & Dev, Wilmington, DE 19803 USA. EM shidixun@gmail.com; wangrs@nenu.edu.cn RI Zhang, Jingping/C-1312-2014 OI Zhang, Jingping/0000-0001-8004-3673 FU National High Technology Research and Development Program of China [SS2012AA110301, 2013AA110103]; Program for New Century Excellent Talents in University [NCET-12-0816]; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by National High Technology Research and Development Program of China (SS2012AA110301, 2013AA110103), Program for New Century Excellent Talents in University (NCET-12-0816), and the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The National Center for Electron Microscopy at LBNL is acknowledged for the TEM experiments. NR 48 TC 19 Z9 21 U1 15 U2 164 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUN 10 PY 2014 VL 20 IS 24 BP 7479 EP 7485 DI 10.1002/chem.201304744 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AJ4CI UT WOS:000337617500036 PM 24782138 ER PT J AU Bell, JR Luo, HM Dai, S AF Bell, Jason R. Luo, Huimin Dai, Sheng TI Superbase-derived protic ionic liquid extractants for metal ion separation SO SEPARATION AND PURIFICATION TECHNOLOGY LA English DT Article DE Solvent extraction; Ionic liquids; beta-Diketone; La3+/Ba2+ ID SOLVENT-EXTRACTION; CROWN-ETHERS; AQUEOUS-SOLUTIONS; BETA-DIKETONES; GREENNESS; MECHANISM; ACTINIDES; EXCHANGE; ANIONS; SR2+ AB Solvent extraction of La3+ and Ba2+ by an ionic liquid extractant in an imidazolium-based ionic liquid diluent was investigated. Seven protic ionic liquid extractants were examined and these PILs are based on five organic superbases and either 6,6,7,7,8,8,8-heptafluoro-2,2-dimethy1-3,5-octadione (Hfod) or 1,1,1,5,5,5-hexafluoroacetylacetone (Hhfac) beta-diketones as anion. For these PIL extractants, the extraction efficiencies and separation factors were found to be concentration dependent. The effects of aqueous phase acidity, extractant structure, and extractant concentration on separation properties of La3+ and Ba2+ are discussed in this paper. (C) 2014 Elsevier B.V. All rights reserved. C1 [Bell, Jason R.; Luo, Huimin] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Luo, HM (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. EM luoh@ornl.gov RI Dai, Sheng/K-8411-2015 OI Dai, Sheng/0000-0002-8046-3931 FU US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-ACO5-00960R22725]; Oak Ridge National Laboratory; U.S. DOE, the Office of Nuclear Physics; Oak Ridge Associated Universities (ORAU) FX This research was supported by the US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences under Contract DE-ACO5-00960R22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. HML was partially supported by the U.S. DOE, the Office of Nuclear Physics. JRB acknowledges Oak Ridge Associated Universities (ORAU) for postdoctoral fellowships. NR 35 TC 7 Z9 7 U1 7 U2 52 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-5866 EI 1873-3794 J9 SEP PURIF TECHNOL JI Sep. Purif. Technol. PD JUN 10 PY 2014 VL 130 BP 147 EP 150 DI 10.1016/j.seppur.2014.04.023 PG 4 WC Engineering, Chemical SC Engineering GA AJ3HB UT WOS:000337556000018 ER PT J AU Hardin, WG Mefford, JT Slanac, DA Patel, BB Wang, XQ Dai, S Zhao, X Ruoff, RS Johnston, KP Stevenson, KJ AF Hardin, William G. Mefford, J. Tyler Slanac, Daniel A. Patel, Bijal B. Wang, Xiqing Dai, Sheng Zhao, Xin Ruoff, Rodney S. Johnston, Keith P. Stevenson, Keith J. TI Tuning the Electrocatalytic Activity of Perovskites through Active Site Variation and Support Interactions SO CHEMISTRY OF MATERIALS LA English DT Article ID OXYGEN REDUCTION REACTION; METAL-AIR BATTERIES; EVOLUTION REACTION; OXIDE CATALYSTS; WATER OXIDATION; DISK ELECTRODE; CARBON; MECHANISM; DECOMPOSITION; PRINCIPLES AB We present a series of perovskite electrocatalysts that are highly active for both the oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) in an aqueous alkaline electrolyte. Lanthanum-based perovskites containing different transition metal active sites (LaBO3, B = Ni, Ni0.75Fe0.25, Co, Mn) are synthesized by a general colloidal method, yielding phase pure catalysts of homogeneous morphology and surface area (8-14 m(2)/g). Each perovskite's ability to catalyze the OER and ORR is examined using thin film rotating disk electrochemistry (RDE). LaCoO3 supported on nitrogen-doped carbon is shown to be similar to 3 times more active for the OER than high-surface-area IrO2. Furthermore, LaCoO3 is demonstrated to be highly bifunctional by having a lower total overpotential between the OER and ORR (Delta E = 1.00 V) than Pt (Delta E = 1.16) and Ru (Delta E = 1.01). The OER and ORR pathways are perturbed by the introduction of peroxide disproportionation functionality via support interactions and selective doping of the catalyst. LaNi0.75Fe0.25O3's ability to disproportionate peroxide is hypothesized to be responsible for the similar to 50% improvement over LaNiO3 in catalytic activity toward the ORR, despite similar electronic structure. These results allow us to examine the pathways for OER and ORR in context of support interactions, transition metal redox processes, and catalytic bifunctionality. C1 [Hardin, William G.; Ruoff, Rodney S.; Stevenson, Keith J.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Mefford, J. Tyler; Stevenson, Keith J.] Univ Texas Austin, Dept Chem, Univ Stn A5300 1, Austin, TX 78712 USA. [Slanac, Daniel A.; Patel, Bijal B.; Johnston, Keith P.] Univ Texas Austin, Dept Chem Engn, Univ Stn C0400 1, Austin, TX 78712 USA. [Ruoff, Rodney S.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA. [Wang, Xiqing; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Zhao, Xin] Donghua Univ, Coll Mat Sci & Engn, Shanghai 201620, Peoples R China. RP Johnston, KP (reprint author), Univ Texas Austin, Dept Chem Engn, Univ Stn C0400 1, Austin, TX 78712 USA. EM kpj@che.utexas.edu; stevenson@cm.utexas.edu RI Wang, Xiqing/E-3062-2010; Ruoff, Rodney/K-3879-2015; Dai, Sheng/K-8411-2015 OI Wang, Xiqing/0000-0002-1843-008X; Dai, Sheng/0000-0002-8046-3931 FU R. A. Welch Foundation [F-1529, F-1319]; NSF [CHE-0618242] FX Financial support for this work was provided by the R. A. Welch Foundation (Grants F-1529 and F-1319). The Kratos XPS was funded by the NSF under Grant CHE-0618242. We would like to thank Ameya Borwankar for his assistance taking electron micrographs. NR 45 TC 41 Z9 41 U1 23 U2 220 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3368 EP 3376 DI 10.1021/cm403785q PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400007 ER PT J AU Wang, CC Chen, SY Yang, JH Lang, L Xiang, HJ Gong, XG Walsh, A Wei, SH AF Wang, Congcong Chen, Shiyou Yang, Ji-Hui Lang, Li Xiang, Hong-Jun Gong, Xin-Gao Walsh, Aron Wei, Su-Huai TI Design of I-2-II-IV-VI4 Semiconductors through Element Substitution: The Thermodynamic Stability Limit and Chemical Trend SO CHEMISTRY OF MATERIALS LA English DT Article ID CRYSTAL-STRUCTURE; THIN-FILMS; SOLAR-CELL; NANOCRYSTALS; CU2ZNSNS4; FABRICATION; CU2HGSNS4; CU2ZNGES4; VELIKITE; SE AB Through element substitution in Cu2ZnSnS4, a class of kesterite-structured I-2-II-IV-VI4 semiconductors can be designed as novel functional materials. Using the first-principles calculations, we show that this element-substitution design is thermodynamically limited, that is, although I-2-II-IV-VI4 with I = Cu, Ag II = Zn, Cd, Hg, IV = Si, Ge, Sn, and VI = S, Se, Te are stable quaternary compounds, those with II = Mg, Ca, Sr, Ba, IV =Ti, Zr, Hf, and VI = 0 are unstable against the phase-separation into the competing binary and ternary compounds. Three main phase-separation pathways are revealed. In general, we show that if the secondary II-VI or I-2-IV-VI3 phases prefer to have nontetrahedral structures, then the I-2-II-IV-VI4 semiconductors tend to phase separate. This finding can be used as a guideline for future design of new quaternary semiconductors. C1 [Wang, Congcong; Chen, Shiyou; Yang, Ji-Hui; Lang, Li; Xiang, Hong-Jun; Gong, Xin-Gao] Fudan Univ, Key Lab Computat Phys Sci MOE, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Wang, Congcong; Chen, Shiyou; Yang, Ji-Hui; Lang, Li; Xiang, Hong-Jun; Gong, Xin-Gao] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Chen, Shiyou] E China Normal Univ, Key Lab Polar Mat & Devices MOE, Shanghai 200241, Peoples R China. [Walsh, Aron] Univ Bath, Ctr Sustainable Chem Technol, Bath BA2 7AY, Avon, England. [Walsh, Aron] Univ Bath, Dept Chem, Bath BA2 7AY, Avon, England. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Chen, SY (reprint author), Fudan Univ, Key Lab Computat Phys Sci MOE, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. EM chensy@fudan.edu.cn; xggong@fudan.edu.cn; suhuai.wei@nrel.gov RI Walsh, Aron/A-7843-2008; Xiang, Hongjun/I-4305-2016; gong, xingao/D-6532-2011 OI Walsh, Aron/0000-0001-5460-7033; Xiang, Hongjun/0000-0002-9396-3214; FU Special Funds for Major State Basic Research, National Natural Science Foundation of China (NSFC), International collaboration project; Program for Professor of Special Appointment (Eastern Scholar); NSFC [61106087, 10934002, 91233121]; U.S Department of Energy (DOE) [DE-AC36-08GO28308]; CAS/ESPRC [EP/101330X/1]; EPSRC [EP/K016288/1] FX The work at Fudan University was supported by the Special Funds for Major State Basic Research, National Natural Science Foundation of China (NSFC), International collaboration project, and Program for Professor of Special Appointment (Eastern Scholar). S.C. is supported by NSFC under Grant Nos. 61106087, 10934002, and 91233121. The work at NREL was funded by the U.S Department of Energy (DOE), under Contract No. DE-AC36-08GO28308. The work in Bath was supported by joint CAS/ESPRC Project No. EP/101330X/1 and EPSRC Project EP/K016288/1. NR 51 TC 29 Z9 29 U1 17 U2 107 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3411 EP 3417 DI 10.1021/cm500598x PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400012 ER PT J AU Jung, IH Lo, WY Jang, J Chen, W Zhao, DL Landry, ES Lu, LY Talapin, DV Yu, LP AF Jung, In Hwan Lo, Wai-Yip Jang, Jaeyoung Chen, Wei Zhao, Donglin Landry, Erik S. Lu, Luyao Talapin, Dmitri V. Yu, Luping TI Synthesis and Search for Design Principles of New Electron Accepting Polymers for All-Polymer Solar Cells SO CHEMISTRY OF MATERIALS LA English DT Article ID FIELD-EFFECT TRANSISTORS; CONJUGATED POLYMERS; N-TYPE; PHOTOVOLTAIC CELLS; FILL FACTOR; MOBILITY; DONOR; PERFORMANCE; EFFICIENCY; TRANSPORT AB New electron withdrawing monomers, thieno-[2',3':5',6']pyrido[3,4-g] thieno [3,2-c] isoquinoline-5,11(4H,10H)-dione (TPTI) and fluorenedicyclopentathiophene dimalononitrile (CN), have been developed and used to form 12 alternating polymers having different monomer combinations: (a) weak donating monomer-strong accepting monomer, (b) weak accepting monomer-strong accepting monomer, (c) weak accepting monomer-weak accepting monomer, and (d) strong donating monomer-strong accepting monomer. It was found that lowest unoccupied molecular orbital (LUMO) energy levels of polymers are significantly determined by stronger electron accepting monomers and highest occupied molecular orbital (HOMO) energy levels by the weak electron accepting monomers. In addition, fluorescent quantum yields of the TPTI-based polymers in chloroform solution are significantly decreased as the LUMO energy levels of the TPTI series of polymers become deeper. The quantum yield was found to be closely related with the photovoltaic properties, which reflects the effect of internal polarization on the photovoltaic properties. Only the electron accepting polymers showing SCLC mobility higher than 10(-4) cm(2)/(Vs) exhibited photovoltaic performance in blend films with a donor polymer, and the PTB7:PNPDI (1:1.8 w/w) device exhibited the highest power conversion efficiency of 1.03% (V-oc = 0.69 V, J(cc) = -4.13 mA/cm(2), FF = 0.36) under AM 1.5G condition, 100 W/cm(2). We provide a large set of systematic structure-property relationships, which gives new perspectives for the design of electron accepting materials. C1 [Jung, In Hwan; Lo, Wai-Yip; Jang, Jaeyoung; Zhao, Donglin; Lu, Luyao; Talapin, Dmitri V.; Yu, Luping] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Jung, In Hwan; Lo, Wai-Yip; Jang, Jaeyoung; Zhao, Donglin; Lu, Luyao; Talapin, Dmitri V.; Yu, Luping] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Chen, Wei; Landry, Erik S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Yu, LP (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM lupingyu@uchicago.edu RI Chen, Wei/G-6055-2011; Lu, Luyao/J-6553-2015 OI Chen, Wei/0000-0001-8906-4278; FU U.S. National Science Foundation [NSF DMR-1263006]; Air Force Office of Scientific Research; SF MRSEC program at the University of Chicago [DMR-0213745]; Department of Energy (DOE) via the ANSER Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059, KC020301, DE-AC02-06CH11357] FX This work is supported by a U.S. National Science Foundation Grant (NSF DMR-1263006), the Air Force Office of Scientific Research and NSF MRSEC program at the University of Chicago (Grant DMR-0213745), Department of Energy (DOE) via the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001059. W.C. gratefully acknowledges financial support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. KC020301. We also thank Dr. Joseph Strzalka and Dr. Zhang Jiang for the assistance with GISAXS measurements. Use of the Advanced Photon Source (APS) at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 58 TC 47 Z9 47 U1 11 U2 93 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3450 EP 3459 DI 10.1021/cm500832h PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400017 ER PT J AU Yang, WC Miskin, CK Hages, CJ Hanley, EC Handwerker, C Stach, EA Agrawal, R AF Yang, Wei-Chang Miskin, Caleb K. Hages, Charles J. Hanley, Evan C. Handwerker, Carol Stach, Eric A. Agrawal, Rakesh TI Kesterite Cu2ZnSn(S,Se)(4) Absorbers Converted from Metastable, Wurtzite-Derived Cu2ZnSnS4 Nanoparticles SO CHEMISTRY OF MATERIALS LA English DT Article ID CZTSSE SOLAR-CELLS; NANOCRYSTALS; PERFORMANCE; CHALCOGENIDES; FILMS AB Wurtzite-derived copper-zinc-tin sulfide nanoparticle films were observed to undergo a phase transformation to a kesterite phase when exposed to Se vapor at 500 degrees C. The resulting dense and selenized Cu2ZnSn4(S,Se)(4) (CZTSSe) films were found to have the same bilayer kesterite structure as absorber layers derived directly from kesterite Cu2ZnSnS4 (CZTS) nanoparticles (Guo, Q; Ford, G. M.; Yang, W.-C.; Walker, B. C.; Stach, E. A.; Hillhouse, H. W.; Agrawal, R J. Am. Chem. Soc. 2010, 132, 17384-17386). The top layer was fully sintered into micrometer size grains, while the bottom unsintered layer consisted of small, nanometer size kesterite grains. When compared to films formed from kesterite CZTS nanoparticles, solar cells fabricated from the wurtzite-derived CZTS nanoparticles were found to have lower power conversion efficiencies (PCE). Surprisingly, for those CZTSSe films that were formed from wurtzite-derived nanoparticles, it was found that extensive selenization leads to the disappearance of the bottom unsintered layer and the formation of a thin film composed of only micrometer-sized grains. These results have significant importance for the improvement of the performance of CZTSSe solar materials. Solar cells fabricated from kesterite nanoparticles have delivered a PCE of 9%-despite the presence of an unsintered layer. These results indicate that the use of wurtzite-derived CZTS nanoparticles has the potential to remove the unsintered layer in kesterite CZTSSe solar cells (Miskin, C. K.; Yang, W.-C.; Hages, C. J.; Carter, N. J.; Joglekar, C. S.; Stach, E. A.; Agrawal, R. Prog. Photovoltaics: Res. Appl. 2014, DOI: 10.1002/pip.2472). C1 [Yang, Wei-Chang; Miskin, Caleb K.; Hages, Charles J.; Hanley, Evan C.; Agrawal, Rakesh] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Yang, Wei-Chang; Handwerker, Carol; Stach, Eric A.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Stach, EA (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM estach@bnl.gov; agrawalr@purdue.edu RI Stach, Eric/D-8545-2011; Hages, Charles/J-6074-2015 OI Stach, Eric/0000-0002-3366-2153; Hages, Charles/0000-0003-4054-1218 FU NSF Solar economy IGERT program [0903670-DGE]; DOE Sun Shot program [DE-EE0005328]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors would like to thank Peter W. Stephens and David C. Palmer for discussing the simulation of crystallographic structures. Financial support from the NSF Solar economy IGERT program (0903670-DGE) and the DOE Sun Shot program (DE-EE0005328) is acknowledged. E.A.S. acknowledges funding to the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 26 TC 35 Z9 35 U1 5 U2 94 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3530 EP 3534 DI 10.1021/cm501111z PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400027 ER PT J AU Gobet, M Greenbaum, S Sahu, G Liang, CD AF Gobet, Mallory Greenbaum, Steve Sahu, Gayatri Liang, Chengdu TI Structural Evolution and Li Dynamics in Nanophase Li3PS4 by Solid-State and Pulsed-Field Gradient NMR SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-SULFUR BATTERIES; CONDUCTOR; GLASSES; SPECTRA; SULFIDE; P-31 AB The ceramic lithium ion conductor beta-Li3PS4 has a disordered and nanoporous structure that leads to an enhancement in ionic conductivity by some 3 orders of magnitude compared to the crystalline gamma phase. The beta phase is prepared by thermal treatment of an inorganic-organic complex based on Li3PS4 and THF. Multinuclear (H-1, Li-6,Li-7, P-31) solid-state NMR spectroscopy is used to characterize the structural phase evolution of the starting material at various steps in the thermal treatment. The beta phase formed after high temperature treatment is recognized as spectroscopically distinct from the bulk gamma-Li3PS4 compound. Also formed is an amorphous lithium thiophosphate phase that is metastable as verified by annealing over an extended period. Lithium ion self-diffusion coefficients are measurable by standard pulsed-field gradient NMR methods at 100 degrees C and with values consistent with the high ionic conductivity previously reported for this material. C1 [Gobet, Mallory; Greenbaum, Steve] CUNY Hunter Coll, Dept Phys & Astron, New York, NY 10065 USA. [Sahu, Gayatri; Liang, Chengdu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Greenbaum, S (reprint author), CUNY Hunter Coll, Dept Phys & Astron, New York, NY 10065 USA. EM steve.greenbaum@hunter.cuny.edu RI Gobet, Mallory/I-2498-2013 OI Gobet, Mallory/0000-0001-9735-0741 FU US. Department of Energy, Office of Science, Basic Energy Sciences; DOE BES Division of Materials Chemistry [DE-SC0005029]; Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. DOE FX The work at ORNL was supported by the US. Department of Energy, Office of Science, Basic Energy Sciences. The NMR measurements were supported by the DOE BES Division of Materials Chemistry under award DE-SC0005029. Synthesis and XRD characterization of materials were conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. DOE. NR 11 TC 9 Z9 9 U1 11 U2 115 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3558 EP 3564 DI 10.1021/cm5012058 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400031 ER PT J AU Long, BR Croy, JR Dogan, F Suchomel, MR Key, B Wen, JG Miller, DJ Thackeray, MM Balasubramanian, M AF Long, Brandon R. Croy, Jason R. Dogan, Fulya Suchomel, Matthew R. Key, Baris Wen, Jianguo Miller, Dean J. Thackeray, Michael M. Balasubramanian, Mahalingam TI Effect of Cooling Rates on Phase Separation in 0.5Li(2)MnO(3)center dot 0.5LiCoO(2) Electrode Materials for Li-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID X-RAY-ABSORPTION; NICKEL MANGANESE OXIDES; LOCAL-STRUCTURE; LITHIUM BATTERIES; CATHODE MATERIALS; SOLID-SOLUTION; ELECTROCHEMICAL PROPERTIES; PSEUDOTERNARY SYSTEM; ATOMIC-STRUCTURE; 1ST PRINCIPLES AB The results of a detailed structural investigation on the influence of cooling rates in the synthesis of lithium- and manganese-rich 0.5Li(2)MnO(3)center dot 0.5LiCoO(2) composite electrode materials, which are of interest for Li-ion battery applications, are presented. It is shown that a low-temperature, intermediate firing step, often employed in cathode synthesis, yields a minor secondary component representing a polydisperse distribution of lattice parameters, not found in the absence of low-temperature treatments. However, regardless of the heating and cooling conditions employed, all samples present two distinctly different local environments as evidenced by X-ray absorption fine structure spectroscopy (XAFS) and nuclear magnetic resonance (NMR) analysis. Transmission electron microscopy (TEM) data show discrete domain structures that are consistent with the XAFS and NMR findings. Furthermore, high resolution synchrotron X-ray diffraction (HR-XRD), as well as the XAFS and NMR data show no discernible differences between sample sets heated in similar fashion and subsequently cooled at different rates. The results contradict recent reports, using X-ray diffraction, that rapidly quenched samples of the same composition are true solid solutions. This apparent discrepancy is assigned, in part, to the inherent nature of conventional diffraction, which firmly elucidates the average long-range structure but does not capture the local domain microstructure of these nanocomposite materials. The combined use of HR-XRD, XAFS, NMR, and TEM data indicate that charge ordering, which is initiated at relatively low temperatures, is the dominant force that produces a nanoscale, inhomogeneous composite structure, irrespective of the cooling rate. C1 [Long, Brandon R.; Croy, Jason R.; Dogan, Fulya; Key, Baris; Thackeray, Michael M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Suchomel, Matthew R.; Balasubramanian, Mahalingam] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Wen, Jianguo; Miller, Dean J.] Argonne Natl Lab, Electron Microscopy Ctr, Argonne, IL 60439 USA. RP Croy, JR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM croy@anl.gov; mali@aps.anl.gov RI Suchomel, Matthew/C-5491-2015; OI SUCHOMEL, Matthew/0000-0002-9500-5079 FU Vehicle Technologies Program, Hybrid and Electric Systems at the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; U.S. DOE, Basic Energy Sciences; National Sciences and Engineering Research Council of Canada; Office of Science [DE-AC02-06CH11357]; Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX Support from the Vehicle Technologies Program, Hybrid and Electric Systems, in particular, David Howell, Tien Duong, and Peter Faguy, at the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy is gratefully acknowledged. Sector 20 facilities at the Advanced Photon Source of Argonne National Laboratory, and research at these facilities, are supported by the U.S. DOE, Basic Energy Sciences, and National Sciences and Engineering Research Council of Canada and its founding institutions. Electron microscopy was carried out in the Electron Microscopy Center at Argonne, which is supported by the Office of Science under contract No. DE-AC02-06CH11357. We thank Dr. Eungje Lee for his assistance in preparing structural models. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. NR 53 TC 20 Z9 20 U1 8 U2 89 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUN 10 PY 2014 VL 26 IS 11 BP 3565 EP 3572 DI 10.1021/cm501229t PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA AI8TH UT WOS:000337199400032 ER PT J AU Lindenmaier, R Dubey, MK Henderson, BG Butterfield, ZT Herman, JR Rahn, T Lee, SH AF Lindenmaier, Rodica Dubey, Manvendra K. Henderson, Bradley G. Butterfield, Zachary T. Herman, Jay R. Rahn, Thom Lee, Sang-Hyun TI Multiscale observations of CO2, (CO2)-C-13, and pollutants at Four Corners for emission verification and attribution SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE air pollution; greenhouse gases; climate change ID DIOXIDE; REGION; URBAN; GAS AB There is a pressing need to verify air pollutant and greenhouse gas emissions from anthropogenic fossil energy sources to enforce current and future regulations. We demonstrate the feasibility of using simultaneous remote sensing observations of column abundances of CO2, CO, and NO2 to inform and verify emission inventories. We report, to our knowledge, the first ever simultaneous column enhancements in CO2 (3-10 ppm) and NO2 (1-3 Dobson Units), and evidence of delta(CO2)-C-13 depletion in an urban region with two large coal-fired power plants with distinct scrubbing technologies that have resulted in Delta NOx/Delta CO2 emission ratios that differ by a factor of two. Ground-based total atmospheric column trace gas abundances change synchronously and correlate well with simultaneous in situ point measurements during plume interceptions. Emission ratios of Delta NOx/Delta CO2 and Delta SO2/Delta CO2 derived from in situ atmospheric observations agree with those reported by in-stack monitors. Forward simulations using in-stack emissions agree with remote column CO2 and NO2 plume observations after fine scale adjustments. Both observed and simulated column Delta NO2/Delta CO2 ratios indicate that a large fraction (70-75%) of the region is polluted. We demonstrate that the column emission ratios of Delta NO2/Delta CO2 can resolve changes from day-to-day variation in sources with distinct emission factors (clean and dirty power plants, urban, and fires). We apportion these sources by using NO2, SO2, and CO as signatures. Our high-frequency remote sensing observations of CO2 and coemitted pollutants offer promise for the verification of power plant emission factors and abatement technologies from ground and space. C1 [Lindenmaier, Rodica; Dubey, Manvendra K.; Henderson, Bradley G.; Butterfield, Zachary T.; Rahn, Thom; Lee, Sang-Hyun] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Herman, Jay R.] Univ Maryland, Goddard Space Flight Ctr, Joint Ctr Earth Syst Technol, Greenbelt, MD 20771 USA. RP Lindenmaier, R (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM rodica@lanl.gov; dubey@lanl.gov RI Dubey, Manvendra/E-3949-2010; Lee, Sang-Hyun/B-5974-2013; Rahn, Thom/C-5211-2012 OI Dubey, Manvendra/0000-0002-3492-790X; FU LANL Laboratory Directed Research and Development project "Multi-Scale Science Framework for Climate Treaty Verification: Attributing & Tracking GHG Fluxes Using Co-Emitted Signatures" FX We thank TCCON (D. Wunch and P. Wennberg) for providing resources to achieve high-accuracy retrievals. We thank A. Cede and N. Abuhassan for their continuous effort to optimize and maintain the Pandora instrument. We acknowledge the New Mexico Environment Department (T. Hertel, M. Jones, and R. Szkoda), EPA (M. Sather), and Bureau of Land and Management (M. Uhl) for providing us access to the site and in situ air quality data. S.-H. L. thanks the Korean Meteorological Administration for support with supercomputing resources. We thank R. Middleton and J. Muss [Los Alamos National Laboratory (LANL)] for editorial assistance. The reported research was supported by the LANL Laboratory Directed Research and Development project "Multi-Scale Science Framework for Climate Treaty Verification: Attributing & Tracking GHG Fluxes Using Co-Emitted Signatures" (principal investigator M.K.D.). NR 16 TC 12 Z9 12 U1 1 U2 18 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 10 PY 2014 VL 111 IS 23 BP 8386 EP 8391 DI 10.1073/pnas.1321883111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI6IJ UT WOS:000336976000037 PM 24843169 ER PT J AU Odokonyero, D Sakai, A Patskovsky, Y Malashkevich, VN Fedorov, AA Bonanno, JB Fedorov, EV Toro, R Agarwal, R Wang, CX Ozerova, NDS Yew, WS Sauder, JM Swaminathan, S Burley, SK Almo, SC Glasner, ME AF Odokonyero, Denis Sakai, Ayano Patskovsky, Yury Malashkevich, Vladimir N. Fedorov, Alexander A. Bonanno, Jeffrey B. Fedorov, Elena V. Toro, Rafael Agarwal, Rakhi Wang, Chenxi Ozerova, Nicole D. S. Yew, Wen Shan Sauder, J. Michael Swaminathan, Subramanyam Burley, Stephen K. Almo, Steven C. Glasner, Margaret E. TI Loss of quaternary structure is associated with rapid sequence divergence in the OSBS family SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE enolase superfamily; protein structure; protein structure-function relationships ID O-SUCCINYLBENZOATE SYNTHASE; ACYLAMINO ACID RACEMASE; HIGHLY EXPRESSED PROTEINS; ENOLASE SUPERFAMILY; ENZYMATIC-ACTIVITIES; MANDELATE RACEMASE; ESCHERICHIA-COLI; ACTIVE-SITE; UNIVERSAL DISTRIBUTION; DOMAIN SUPERFAMILIES AB The rate of protein evolution is determined by a combination of selective pressure on protein function and biophysical constraints on protein folding and structure. Determining the relative contributions of these properties is an unsolved problem in molecular evolution with broad implications for protein engineering and function prediction. As a case study, we examined the structural divergence of the rapidly evolving o-succinylbenzoate synthase (OSBS) family, which catalyzes a step in menaquinone synthesis in diverse microorganisms and plants. On average, the OSBS family is much more divergent than other protein families from the same set of species, with the most divergent family members sharing <15% sequence identity. Comparing 11 representative structures revealed that loss of quaternary structure and large deletions or insertions are associated with the family's rapid evolution. Neither of these properties has been investigated in previous studies to identify factors that affect the rate of protein evolution. Intriguingly, one subfamily retained a multimeric quaternary structure and has small insertions and deletions compared with related enzymes that catalyze diverse reactions. Many proteins in this subfamily catalyze both OSBS and N-succinylamino acid racemization (NSAR). Retention of ancestral structural characteristics in the NSAR/OSBS subfamily suggests that the rate of protein evolution is not proportional to the capacity to evolve new protein functions. Instead, structural features that are conserved among proteins with diverse functions might contribute to the evolution of new functions. C1 [Odokonyero, Denis; Wang, Chenxi; Ozerova, Nicole D. S.; Glasner, Margaret E.] Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. [Sakai, Ayano] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. [Patskovsky, Yury; Malashkevich, Vladimir N.; Fedorov, Alexander A.; Bonanno, Jeffrey B.; Fedorov, Elena V.; Toro, Rafael; Almo, Steven C.] Albert Einstein Coll Med, Dept Biochem, Bronx, NY 10461 USA. [Almo, Steven C.] Albert Einstein Coll Med, Dept Physiol & Biophys, Bronx, NY 10461 USA. [Agarwal, Rakhi; Swaminathan, Subramanyam] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Yew, Wen Shan] Natl Univ Singapore, Dept Biochem, Singapore 117597, Singapore. [Sauder, J. Michael] Lilly Biotechnol Ctr, San Diego, CA 92121 USA. [Burley, Stephen K.] Rutgers State Univ, BioMaPS Inst Quantitat Biol, Piscataway, NJ 08854 USA. [Burley, Stephen K.] Rutgers State Univ, Res Collaboratory Struct Bioinformat Prot Data Ba, Piscataway, NJ 08854 USA. [Burley, Stephen K.] Rutgers State Univ, Ctr Integrat Prote Res, Piscataway, NJ 08854 USA. [Burley, Stephen K.] Rutgers State Univ, Rutgers Canc Inst New Jersey, Piscataway, NJ 08854 USA. [Burley, Stephen K.] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. RP Glasner, ME (reprint author), Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. EM margy.glasner@tamu.edu OI Glasner, Margaret/0000-0003-1818-1965 FU Robert A. Welch Foundation [A-1758]; Norman Hackerman Advanced Research Program [000517-0016-2011]; National Institutes of Health (NIH) [U54 GM074945]; NIH [U54 GM094662]; US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; National Institute of Biomedical Imaging and Bioengineering [P30-EB-009998]; NIH National Center for Research Resources; DOE Office of Biological and Environmental Research; Rockefeller University; Albert Einstein College of Medicine; Sloan Kettering Institute; New York Structural Biology Center; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We acknowledge the efforts of all New York SGX Research Center for Structural Genomics (NYSGXRC) and New York Structural Genomics Research Consortium (NYSGRC) personnel who contributed to the structure determination and manuscript preparation. We thank Dr. Larry Dangott of the Protein Chemistry Laboratory at Texas A&M University for assistance with size exclusion chromatography. We thank Jacob Jipp and Christine Jones for assistance with subcloning and Dr. Andrew McMillan for insightful comments on the manuscript. This work was supported by Grant A-1758 from the Robert A. Welch Foundation and Grant 000517-0016-2011 from the Norman Hackerman Advanced Research Program (to M. E. G.). The NYSGXRC was supported by National Institutes of Health (NIH) Grant U54 GM074945 (to S. K. B.). The NYSGRC was supported by NIH Grant U54 GM094662 (to S. C. A.). Diffraction data were collected at the National Synchrotron Light Source, Brookhaven National Laboratory [supported by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886]: beamlines X29A and X12C (supported by Grant P30-EB-009998 from the National Institute of Biomedical Imaging and Bioengineering to The Center for Synchrotron Biosciences, and the NIH National Center for Research Resources and the DOE Office of Biological and Environmental Research to the National Synchrotron Light Source Research Resource for Macromolecular Crystallography); beamline X9A (supported by Rockefeller University, Albert Einstein College of Medicine, and Sloan Kettering Institute); and beamline X4A (supported by the New York Structural Biology Center). Diffraction data were also collected at the Advanced Photon Source, Argonne National Laboratory (supported by the DOE, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357): LRL-CAT31-ID-D beamline (data collection at sector 31 of the Advanced Photon Source was provided by Eli Lilly, which operates the facility). NR 60 TC 1 Z9 1 U1 1 U2 8 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 10 PY 2014 VL 111 IS 23 BP 8535 EP 8540 DI 10.1073/pnas.1318703111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI6IJ UT WOS:000336976000062 PM 24872444 ER PT J AU Zhao, CQ Hwang, SH Buchholz, BA Carpenter, TS Lightstone, F Yang, J Hammock, BD Casida, JE AF Zhao, Chunqing Hwang, Sung Hee Buchholz, Bruce A. Carpenter, Timothy S. Lightstone, Felice Yang, Jun Hammock, Bruce D. Casida, John E. TI GABA(A) receptor target of tetramethylenedisulfotetramine SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE neurotoxicity; convulsant; molecular modeling ID GATED CHLORIDE CHANNEL; STRUCTURE-TOXICITY RELATIONSHIPS; ACCELERATOR MASS-SPECTROMETRY; SUBUNIT COMPOSITION; BINDING-SITE; AMINO-ACID; BRAIN; INSECTICIDE; TETRAMINE; RAT AB Use of the highly toxic and easily prepared rodenticide tetramethylenedisulfotetramine (TETS) was banned after thousands of accidental or intentional human poisonings, but it is of continued concern as a chemical threat agent. TETS is a noncompetitive blocker of the GABA type A receptor (GABA(A)R), but its molecular interaction has not been directly established for lack of a suitable radioligand to localize the binding site. We synthesized [C-14]TETS (14 mCi/mmol, radiochemical purity >99%) by reacting sulfamide with (HCHO)-C-14 and s-trioxane then completion of the sequential cyclization with excess HCHO. The outstanding radiocarbon sensitivity of accelerator mass spectrometry (AMS) allowed the use of [C-14] TETS in neuroreceptor binding studies with rat brain membranes in comparison with the standard GABA(A)R radioligand 4'-ethynyl-4-n-[H-3] propylbicycloorthobenzoate ([H-3] EBOB) (46 Ci/mmol), illustrating the use of AMS for characterizing the binding sites of high-affinity C-14 radio-ligands. Fourteen noncompetitive antagonists of widely diverse chemotypes assayed at 1 or 10 mu M inhibited [C-14] TETS and [H-3] EBOB binding to a similar extent (r(2) = 0.71). Molecular dynamics simulations of these 14 toxicants in the pore region of the alpha 1 beta 2 gamma 2 GABA(A)R predict unique and significant polar interactions for TETS with alpha(1)T1' and gamma(2)S2', which are not observed for EBOB or the GABAergic insecticides. Several GABA(A)R modulators similarly inhibited [C-14] TETS and [H-3] EBOB binding, including midazolam, flurazepam, avermectin Ba1, baclofen, isoguvacine, and propofol, at 1 or 10 mu M, providing an in vitro system for recognizing candidate antidotes. C1 [Zhao, Chunqing; Casida, John E.] Univ Calif Berkeley, Environm Chem & Toxicol Lab, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Hwang, Sung Hee; Yang, Jun; Hammock, Bruce D.] Univ Calif Davis, Dept Entomol, Coll Agr & Environm Sci, Davis, CA 95616 USA. [Buchholz, Bruce A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Carpenter, Timothy S.; Lightstone, Felice] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Livermore, CA 94551 USA. RP Buchholz, BA (reprint author), Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. EM buchholz2@llnl.gov; lightstone1@llnl.gov; bdhammock@ucdavis.edu; ectl@berkeley.edu FU China Scholarship Council [2011635139]; National Institutes of Health Office of the Director; CounterACT Program National Institute of Neurological Disorders and Stroke [U54 NS079202]; National Institute of General Medical Sciences Grant [8P41GM103483]; Laboratory Directed Research and Development Grant [13-LW-085]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX C.Z. thanks Prof. Lihong Qiu (China Agricultural University) for academic counsel and Berkeley laboratory colleagues Amanda Ly, Breanna Ford, and Madhur Garg for assistance in manuscript preparation. S.H.H. and B.D.H. thank Jai Woong Seo for the [14C]TETS radio-TLC analysis. We thank the Livermore Computing Grand Challenge for computer time. This work was supported in part by State Scholarship Fund 2011635139 provided by the China Scholarship Council (to C.Z.), National Institutes of Health Office of the Director and the CounterACT Program National Institute of Neurological Disorders and Stroke Grant U54 NS079202 (to S.H.H. and B.D.H.), National Institute of General Medical Sciences Grant 8P41GM103483 (to B.A.B.), and Laboratory Directed Research and Development Grant 13-LW-085 (to T.S.C. and F.L.). Portions of this work were performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, Release LLNL-JRNL-649601. NR 51 TC 13 Z9 14 U1 2 U2 22 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 10 PY 2014 VL 111 IS 23 BP 8607 EP 8612 DI 10.1073/pnas.1407379111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI6IJ UT WOS:000336976000074 PM 24912155 ER PT J AU Ballottari, M Alcocer, MJP D'Andrea, C Viola, D Ahn, TK Petrozza, A Polli, D Fleming, GR Cerullo, G Bassi, R AF Ballottari, Matteo Alcocer, Marcelo J. P. D'Andrea, Cosimo Viola, Daniele Ahn, Tae Kyu Petrozza, Annamaria Polli, Dario Fleming, Graham R. Cerullo, Giulio Bassi, Roberto TI Regulation of photosystem I light harvesting by zeaxanthin SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE photosynthesis; xanthophylls; violaxanthin de-epoxidase; photobleaching ID CHARGE SEPARATION KINETICS; EXCITATION-ENERGY TRANSFER; CAROTENOID-BINDING-SITES; HIGHER-PLANTS; XANTHOPHYLL CYCLE; COMPLEX-II; ARABIDOPSIS-THALIANA; CHLAMYDOMONAS-REINHARDTII; PHOTOOXIDATIVE STRESS; FLUORESCENCE EMISSION AB In oxygenic photosynthetic eukaryotes, the hydroxylated carotenoid zeaxanthin is produced from preexisting violaxanthin upon exposure to excess light conditions. Zeaxanthin binding to components of the photosystem II (PSII) antenna system has been investigated thoroughly and shown to help in the dissipation of excess chlorophyll-excited states and scavenging of oxygen radicals. However, the functional consequences of the accumulation of the light-harvesting complex I (LHCI) proteins in the photosystem I (PSI) antenna have remained unclarified so far. In this work we investigated the effect of zeaxanthin binding on photoprotection of PSI-LHCI by comparing preparations isolated from wild-type Arabidopsis thaliana (i.e., with violaxanthin) and those isolated from the A. thaliana nonphotochemical quenching 2 mutant, in which violaxanthin is replaced by zeaxanthin. Time-resolved fluorescence measurements showed that zeaxanthin binding leads to a previously unrecognized quenching effect on PSI-LHCI fluorescence. The efficiency of energy transfer from the LHCI moiety of the complex to the PSI reaction center was down-regulated, and an enhanced PSI resistance to photoinhibition was observed both in vitro and in vivo. Thus, zeaxanthin was shown to be effective in inducing dissipative states in PSI, similar to its well-known effect on PSII. We propose that, upon acclimation to high light, PSI-LHCI changes its light-harvesting efficiency by a zeaxanthin-dependent quenching of the absorbed excitation energy, whereas in PSII the stoichiometry of LHC antenna proteins per reaction center is reduced directly. C1 [Ballottari, Matteo; Bassi, Roberto] Univ Verona, Dept Biotechnol, I-37134 Verona, Italy. [Alcocer, Marcelo J. P.; D'Andrea, Cosimo; Petrozza, Annamaria; Polli, Dario] Polytech Univ Milan, Italian Inst Technol, Ctr Nanosci & Technol, I-20133 Milan, Italy. [Alcocer, Marcelo J. P.; D'Andrea, Cosimo; Viola, Daniele; Polli, Dario; Cerullo, Giulio] Polytech Univ Milan, Dept Phys, Natl Res Council, Inst Photon & Nanotechnol, I-20133 Milan, Italy. [Ahn, Tae Kyu; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Ahn, Tae Kyu] Sungkyunkwan Univ, Dept Energy Sci, Suwon 440746, South Korea. [Ahn, Tae Kyu; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Bassi, R (reprint author), Univ Verona, Dept Biotechnol, I-37134 Verona, Italy. EM roberto.bassi@univr.it RI Ahn, Tae/A-5838-2013; Petrozza, Annamaria/A-1065-2014; OI Petrozza, Annamaria/0000-0001-6914-4537; Cerullo, Giulio/0000-0002-9534-2702; Ballottari, Matteo/0000-0001-8410-3397; bassi, roberto/0000-0002-4140-8446; Polli, Dario/0000-0002-6960-5708; Alcocer, Marcelo/0000-0002-6600-1335 FU European Union [316427]; Italian Ministry of Agriculture, Food and Forestry [HYDROBIO]; Italian Ministry for Education, Higher Education and Future Research Grant [RBFR08XH0H]; Woo Jang Chun Special Project - Korean Rural Development Agency [PJ00910603201]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences [DE-AC03-76SF000098] FX Research was funded in part through the European Union Seventh Framework Programme for Research Project 316427, Environmental Acclimation of Photosynthesis; the Italian Ministry of Agriculture, Food and Forestry Project HYDROBIO; the Italian Ministry for Education, Higher Education and Future Research Grant RBFR08XH0H; and by Woo Jang Chun Special Project PJ00910603201 financed by the Korean Rural Development Agency. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences through Grant DE-AC03-76SF000098 (at Lawrence Berkeley National Laboratory and University of California, Berkeley). NR 74 TC 16 Z9 16 U1 3 U2 75 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 10 PY 2014 VL 111 IS 23 BP E2431 EP E2438 DI 10.1073/pnas.1404377111 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI6IJ UT WOS:000336976000014 PM 24872450 ER PT J AU Aliu, E Aune, T Behera, B Beilicke, M Benbow, W Berger, K Bird, R Bouvier, A Buckley, JH Bugaev, V Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dumm, J Dwarkadas, VV Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fleischhack, H Fortin, P Fortson, L Furniss, A Galante, N Gillanders, GH Gotthelf, EV Griffin, S Griffiths, ST Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Johnson, CA Kaaret, P Kargaltsev, O Kertzman, M Khassen, Y Kieda, D Krennrich, F Lang, MJ Madhavan, AS Maier, G McArthur, S McCann, A Millis, J Moriarty, P Mukherjee, R Nieto, D de Bhroithe, AO Ong, RA Otte, AN Pandel, D Park, N Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Rajotte, J Reyes, LC Reynolds, PT Richards, GT Roache, E Roberts, M Sembroski, GH Shahinyan, K Smith, AW Staszak, D Telezhinsky, I Tucci, JV Tyler, J Vincent, S Wakely, SP Weinstein, A Welsing, R Wilhelm, A Williams, DA Zitzer, B AF Aliu, E. Aune, T. Behera, B. Beilicke, M. Benbow, W. Berger, K. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dumm, J. Dwarkadas, V. V. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fleischhack, H. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Gotthelf, E. V. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Johnson, C. A. Kaaret, P. Kargaltsev, O. Kertzman, M. Khassen, Y. Kieda, D. Krennrich, F. Lang, M. J. Madhavan, A. S. Maier, G. McArthur, S. McCann, A. Millis, J. Moriarty, P. Mukherjee, R. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Pandel, D. Park, N. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Rajotte, J. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Roberts, M. Sembroski, G. H. Shahinyan, K. Smith, A. W. Staszak, D. Telezhinsky, I. Tucci, J. V. Tyler, J. Vincent, S. Wakely, S. P. Weinstein, A. Welsing, R. Wilhelm, A. Williams, D. A. Zitzer, B. TI SPATIALLY RESOLVING THE VERY HIGH ENERGY EMISSION FROM MGRO J2019+37 WITH VERITAS SO ASTROPHYSICAL JOURNAL LA English DT Article DE gamma rays : stars; pulsars : individual (PSR J2021+3651); supernovae : individual (CTB 87) ID GAMMA-RAY EMISSION; PULSAR WIND NEBULA; GALACTIC PLANE; PSR J2021+3651; CYGNUS REGION; DISCOVERY; MILAGRO; STARS; HESS; ASSOCIATIONS AB We present very high energy (VHE) imaging of MGRO J2019+37 obtained with the VERITAS observatory. The bright extended (similar to 2 degrees) unidentified Milagro source is located toward the rich star formation region Cygnus-X. MGRO J2019+37 is resolved into two VERITAS sources. The faint, point-like source VER J2016+371 overlaps CTB 87, a filled-center remnant (SNR) with no evidence of a supernova remnant shell at the present time. Its spectrum is well fit in the 0.65-10 TeV energy range by a power-law model with photon index 2.3 +/- 0.4. VER J2019+378 is a bright extended (similar to 1 degrees) source that likely accounts for the bulk of the Milagro emission and is notably coincident with PSR J2021+3651 and the star formation region Sh 2-104. Its spectrum in the range 1-30 TeV is well fit with a power-law model of photon index 1.75 +/- 0.3, among the hardest values measured in the VHE band, comparable to that observed near Vela-X. We explore the unusual spectrum and morphology in the radio and X-ray bands to constrain possible emission mechanisms for this source. C1 [Aliu, E.; Errando, M.; Mukherjee, R.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Aune, T.; Ong, R. A.; Popkow, A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Behera, B.; Chen, X.; Federici, S.; Fleischhack, H.; Hughes, G.; Maier, G.; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Vincent, S.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Beilicke, M.; Buckley, J. H.; Bugaev, V.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Fortin, P.; Galante, N.; Roache, E.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Berger, K.; Holder, J.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bird, R.; Khassen, Y.; de Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.; Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Chen, X.; Federici, S.; Pohl, M.; Telezhinsky, I.; Wilhelm, A.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Univ Coll Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Tucci, J. V.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.; Shahinyan, K.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Dwarkadas, V. V.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Gotthelf, E. V.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Griffin, S.; Hanna, D.; Ragan, K.; Rajotte, J.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kargaltsev, O.] George Washington Univ, Dept Phys, Washington, DC 20052 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Krennrich, F.; Madhavan, A. S.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Millis, J.] Anderson Univ, Dept Phys, Anderson, IN 46012 USA. [Millis, J.; Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Pandel, D.] Grand Valley State Univ, Dept Phys, Allendale, MI 49401 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Roberts, M.] Eureka Sci Inc, Oakland, CA 94602 USA. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Aliu, E (reprint author), Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. EM ealiu@astro.columbia.edu; nahee@uchicago.edu RI Khassen, Yerbol/I-3806-2015; Nieto, Daniel/J-7250-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Nieto, Daniel/0000-0003-3343-0755; Cui, Wei/0000-0002-6324-5772; Roberts, Mallory/0000-0002-9396-9720; Pandel, Dirk/0000-0003-2085-5586; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U. K; ESA Member States and NASA; Natural Sciences and Engineering Research Council FX The authors would like to thank Jules Halpern for many useful discussions and help in obtaining and interpreting the Swift data. This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation, and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748), and by STFC in the U. K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. Based on observations obtained with XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States and NASA. This research has made use of data and/or software provided by the High Energy Astrophysics Science Archive Research Center (HEASARC), which is a service of the Astrophysics Science Division at NASA/GSFC and the High Energy Astrophysics Division of the Smithsonian Astrophysical Observatory. The research presented in this paper has used data from the Canadian Galactic Plane Survey, a Canadian project with international partners, supported by the Natural Sciences and Engineering Research Council. NR 56 TC 13 Z9 14 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 78 DI 10.1088/0004-637X/788/1/78 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200078 ER PT J AU Beiersdorfer, P Trabert, E Lepson, JK Brickhouse, NS Golub, L AF Beiersdorfer, Peter Traebert, Elmar Lepson, Jaan K. Brickhouse, Nancy S. Golub, Leon TI HIGH-RESOLUTION LABORATORY MEASUREMENTS OF CORONAL LINES IN THE 198-218 angstrom REGION SO ASTROPHYSICAL JOURNAL LA English DT Article DE atomic data; line&COLFAML identification; stars&COLFAML coronae; Sun&COLFAML corona; X-rays&COLFAML stars ID BEAM ION-TRAP; SOFT-X-RAY; EXTREME-ULTRAVIOLET REGION; AN ATOMIC DATABASE; ELECTRON-BEAM; EMISSION-LINES; CHARGED IONS; FE-XIII; WAVELENGTH MEASUREMENTS; ACTIVE-REGION AB We present high-resolution laboratory measurements of the emission from various ions of C, N, O, F, Ne, S, Ar, Fe, and Ni in the extreme ultraviolet wavelength band centered around the lambda 211 Fe XIV channel of the Atmospheric Imaging Assembly on the Solar Dynamics Observatory. While all of the strong iron lines in this region are well known, we note many weaker lines of iron that are not yet identified. The high resolution of our measurements also allows us to resolve several lines in Fe XI, Fe XII, and Fe XIII between 200 and 205 angstrom, whose identities were in question based on a disagreement between different databases. The spectra of the elements other than iron are much less known, and we find a multitude of lines that are not yet in the databases. For example, the CHIANTI database clearly disagrees with the NIST data listings on several of the argon lines we observe and also it contains only about half of the observed sulfur lines. C1 [Beiersdorfer, Peter; Traebert, Elmar] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Traebert, Elmar] Ruhr Univ Bochum, Astron Inst, D-44801 Bochum, Germany. [Lepson, Jaan K.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Brickhouse, Nancy S.; Golub, Leon] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. FU Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Solar and Heliospherical Physics Program of the National Aeronautics and Space Administration [NNH10AN31I]; German Research Association (DFG) [Tr171/18, Tr171/19] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and was supported by the Solar and Heliospherical Physics Program of the National Aeronautics and Space Administration under award NNH10AN31I. E.T. acknowledges support from the German Research Association (DFG; grants Tr171/18 and Tr171/19). NR 57 TC 11 Z9 12 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 25 DI 10.1088/0004-637X/788/1/25 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200025 ER PT J AU Brenneman, LW Madejski, G Fuerst, F Matt, G Elvis, M Harrison, FA Ballantyne, DR Boggs, SE Christensen, FE Craig, WW Fabian, AC Grefenstette, BW Hailey, CJ Madsen, KK Marinucci, A Rivers, E Stern, D Walton, DJ Zhang, WW AF Brenneman, L. W. Madejski, G. Fuerst, F. Matt, G. Elvis, M. Harrison, F. A. Ballantyne, D. R. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Grefenstette, B. W. Hailey, C. J. Madsen, K. K. Marinucci, A. Rivers, E. Stern, D. Walton, D. J. Zhang, W. W. TI THE BROAD-BAND X-RAY SPECTRUM OF IC 4329A FROM A JOINT NuSTAR/SUZAKU OBSERVATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion; accretion disks; galaxies : active; galaxies : individual (IC 4329A); galaxies : nuclei; galaxies : Seyfert; X-rays : galaxies ID ACTIVE GALACTIC NUCLEI; SEYFERT-GALAXY IC-4329A; K-ALPHA LINES; BLACK-HOLE; XMM-NEWTON; BEPPOSAX OBSERVATIONS; COMPTON REFLECTION; EDDINGTON RATIO; TIMING-EXPLORER; ACCRETION DISK AB We have obtained a deep, simultaneous observation of the bright, nearby Seyfert galaxy IC 4329A with Suzaku and NuSTAR. Through a detailed spectral analysis, we are able to robustly separate the continuum, absorption, and distant reflection components in the spectrum. The absorbing column is found to be modest (similar to 6 x 10(21) cm(-2)), and does not introduce any significant curvature in the Fe K band. We are able to place a strong constraint on the presence of a broadened Fe K alpha line (E-rest = 6.46(-0.07)(+0.08) keV with sigma = 0.33(-0.07)(+0.08) keV and EW = 34(-7)(+8) eV), though we are not able to constrain any of the parameters of a relativistic reflection model. These results highlight the range in broad Fe K line strengths observed in nearby, bright, active galactic nuclei (roughly an order of magnitude), and imply a corresponding range in the physical properties of the inner accretion disk in these sources. We have also updated our previously reported measurement of the high-energy cutoff of the hard X-ray emission using both observatories rather than just NuSTAR alone: E-cut = 186 +/- 14 keV. This high-energy cutoff acts as a proxy for the temperature of the coronal electron plasma, enabling us to further separate this parameter from the plasma's optical depth and to update our results for these parameters as well. We derive kT = 50(-3)(+6) keV with tau = 2.34(-0.11)(+0.16) using a spherical geometry, kT = 61 +/- 1 keV with tau = 0.68 +/- 0.02 for a slab geometry, with both having an equivalent goodness-of-fit. C1 [Brenneman, L. W.; Elvis, M.] Harvard Smithsonian CfA, Cambridge, MA 02138 USA. [Madejski, G.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Fuerst, F.; Harrison, F. A.; Grefenstette, B. W.; Madsen, K. K.; Rivers, E.; Walton, D. J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Matt, G.; Marinucci, A.] Univ Roma Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Ballantyne, D. R.] Georgia Inst Technol, Ctr Relativist Astrophys, Sch Phys, Atlanta, GA 30332 USA. [Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.; Craig, W. W.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fabian, A. C.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Brenneman, LW (reprint author), Harvard Smithsonian CfA, 60 Garden St,MS-67, Cambridge, MA 02138 USA. RI Boggs, Steven/E-4170-2015; XRAY, SUZAKU/A-1808-2009 OI Boggs, Steven/0000-0001-9567-4224; FU NASA [NNG08FD60C, NNX13AE90G]; National Aeronautics and Space Administration; Italian Space Agency [ASI/INAF I/037/12/0-011/13] FX This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). L.B. thanks Koji Mukai and the Suzaku GOF at NASA/GSFC for all their assistance in obtaining and analyzing that data, and also gratefully acknowledges funding from NASA grant NNX13AE90G. G.Matt and A.M. acknowledge financial support from Italian Space Agency under contract ASI/INAF I/037/12/0-011/13. NR 65 TC 29 Z9 29 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 61 DI 10.1088/0004-637X/788/1/61 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200061 ER PT J AU Lee, KG Hennawi, JF White, M Croft, RAC Ozbek, M AF Lee, Khee-Gan Hennawi, Joseph F. White, Martin Croft, Rupert A. C. Ozbek, Melih TI OBSERVATIONAL REQUIREMENTS FOR Ly alpha FOREST TOMOGRAPHIC MAPPING OF LARGE-SCALE STRUCTURE AT z similar to 2 SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: observations; galaxies: high-redshift; intergalactic medium; quasars: absorption lines; surveys; techniques: spectroscopic ID DIGITAL-SKY-SURVEY; OSCILLATION SPECTROSCOPIC SURVEY; STAR-FORMING GALAXIES; COLD DARK-MATTER; HUBBLE-SPACE-TELESCOPE; PROBABILITY-DISTRIBUTION FUNCTION; BARYON ACOUSTIC-OSCILLATIONS; TEMPERATURE-DENSITY RELATION; PRINCIPAL COMPONENT ANALYSIS; EXTRAGALACTIC LEGACY SURVEY AB The z greater than or similar to 2Ly alpha forest traces the underlying dark matter distribution on large scales and, given sufficient sightlines, can be used to create three-dimensional (3D) maps of large-scale structures. We examine the observational requirements to construct such maps and estimate the signal-to-noise as a function of exposure time and sightline density. Sightline densities at z = 2.25 are n(los) approximate to [360, 1200, 3300] deg(-2) at limiting magnitudes of g = [24.0, 24.5, 25.0], resulting in transverse sightline separations of < d(perpendicular to)> approximate to [3.6, 1.9, 1.2] h(-1) Mpc, which roughly sets the reconstruction scale. We simulate these reconstructions using mock spectra with realistic noise properties and find that spectra with S/N approximate to 4 per angstrom can be used to generate maps that clearly trace the underlying dark matter at overdensities of rho/ similar to 1. For the VLT/VIMOS spectrograph, exposure times t(exp) = [4, 6, 10] hr are sufficient for maps with spatial resolution is an element of(3D) = [5.0, 3.2, 2.3] h(-1) Mpc. Assuming similar to 250 h(-1) Mpc is probed along the line of sight, 1 deg(2) of survey area would cover a comoving volume of approximate to 10(6) h(-3) Mpc(3) at < z > similar to 2.3, enabling the efficient mapping of large volumes with 8-10 m telescopes. These maps could be used to study galaxy environments, the topology of large-scale structures at high z, and to detect proto-clusters. C1 [Lee, Khee-Gan; Hennawi, Joseph F.] Max Planck Inst Astron, D-69117 Heidelberg, Germany. [White, Martin] EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Croft, Rupert A. C.; Ozbek, Melih] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. RP Lee, KG (reprint author), Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. EM lee@mpia.de RI White, Martin/I-3880-2015; Croft, Rupert/N-8707-2014 OI White, Martin/0000-0001-9912-5070; Croft, Rupert/0000-0003-0697-2583 FU [NSF-AST 1109730] FX We thank Alberto Rorai for his assistance in creating the simulated Ly alpha forest skewers and Xavier Prochaska for helpful discussions and advice. R.C. and M.O. acknowledge support from the grant NSF-AST 1109730. The Wiener reconstructions discussed in this work were performed on the THEO cluster of the Max-Planck-Institut fur Astronomie at the Rechenzentrum in Garching, Germany. NR 141 TC 16 Z9 16 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 49 DI 10.1088/0004-637X/788/1/49 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200049 ER PT J AU Panaitescu, A Vestrand, WT Wozniak, P AF Panaitescu, A. Vestrand, W. T. Wozniak, P. TI "SELF-ABSORBED" GeV LIGHT CURVES OF GAMMA-RAY BURST AFTERGLOWS SO ASTROPHYSICAL JOURNAL LA English DT Article DE gamma; ray burst : general; radiation mechanisms : non-thermal; relativistic processes; shock waves ID FERMI OBSERVATIONS; GEV EMISSION; GRB 090510; COMPONENT; ONSET AB We investigate the effect that the absorption of high-energy (above 100 MeV) photons produced in gamma-ray burst afterglow shocks has on the light curves and spectra of Fermi Large Area Telescope (LAT) afterglows. Afterglows produced by the interaction of a relativistic outflow with a wind-like medium peak when the blast wave deceleration sets in, and the afterglow spectrum could be hardening before that peak, as the optical thickness to pair formation is decreasing. In contrast, in afterglows produced in the interaction with a homogeneous medium, the optical thickness to pair formation should increase and yield a light curve peak when it reaches unity, followed by a fast light curve decay, accompanied by spectral softening. If energy is injected in the blast wave, then the accelerated increase of the optical thickness yields a convex afterglow light curve. Other features, such as a double-peak light curve or a broad hump, can arise from the evolution of the optical thickness to photon-photon absorption. Fast decays and convex light curves are seen in a few LAT afterglows, but the expected spectral softening is rarely seen in (and difficult to measure with) LAT observations. Furthermore, for the effects of photon-photon attenuation to shape the high-energy afterglow light curve without attenuating it too much, the ejecta initial Lorentz factor must be in a relatively narrow range (50-200), which reduces the chance of observing those effects C1 [Panaitescu, A.; Vestrand, W. T.; Wozniak, P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Panaitescu, A (reprint author), Los Alamos Natl Lab, MS B244, Los Alamos, NM 87545 USA. OI Wozniak, Przemyslaw/0000-0002-9919-3310 FU Laboratory Directed Research and Development program FX This work was supported by an award from the Laboratory Directed Research and Development program at the Los Alamos National Laboratory. NR 16 TC 3 Z9 3 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 70 DI 10.1088/0004-637X/788/1/70 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200070 ER PT J AU Raskin, C Kasen, D Moll, R Schwab, J Woosley, S AF Raskin, Cody Kasen, Daniel Moll, Rainer Schwab, Josiah Woosley, Stan TI TYPE Ia SUPERNOVAE FROM MERGING WHITE DWARFS. II. POST-MERGER DETONATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE hydrodynamics; nuclear reactions, nucleosynthesis, abundances; supernovae: general; white dwarfs ID CHANDRASEKHAR MASS MODELS; DOUBLE DEGENERATE MERGER; RADIATION HYDRODYNAMICS; STELLAR HYDRODYNAMICS; SURFACE DETONATIONS; LIGHT CURVES; EVOLUTION; EXPLOSION; STARS; CONSISTENCY AB Merging carbon-oxygen (CO) white dwarfs are a promising progenitor system for Type Ia supernovae (SNe Ia), but the underlying physics and timing of the detonation are still debated. If an explosion occurs after the secondary star is fully disrupted, the exploding primary will expand into a dense CO medium that may still have a disk-like structure. This interaction will decelerate and distort the ejecta. Here we carry out multidimensional simulations of "tamped" SN Ia models, using both particle and grid-based codes to study the merger and explosion dynamics and a radiative transfer code to calculate synthetic spectra and light curves. We find that post-merger explosions exhibit an hourglass-shaped asymmetry, leading to strong variations in the light curves with viewing angle. The two most important factors affecting the outcome are the scale height of the disk, which depends sensitively on the binary mass ratio, and the total Ni-56 yield, which is governed by the central density of the remnant core. The synthetic broadband light curves rise and decline very slowly, and the spectra generally look peculiar, with weak features from intermediate mass elements but relatively strong carbon absorption. We also consider the effects of the viscous evolution of the remnant and show that a longer time delay between merger and explosion probably leads to larger Ni-56 yields and more symmetrical remnants. We discuss the relevance of this class of aspherical "tamped" SN Ia for explaining the class of "super-Chandrasekhar" SN Ia. C1 [Raskin, Cody; Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Kasen, Daniel; Schwab, Josiah] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, Daniel; Schwab, Josiah] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Moll, Rainer; Woosley, Stan] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Moll, Rainer; Woosley, Stan] Univ Calif Santa Cruz, Dept Astron, Santa Cruz, CA 95064 USA. RP Raskin, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU DOE HEP [DE-SC0010676]; National Science Foundation [AST 0909129, AST-1109896]; NASA Theory Program [NNX09AK36G]; Department of Energy Office of Nuclear Physics Early Career Award [DE-SC0008067]; Alexander von Humboldt Foundation through the Feodor Lynen Research Fellowship program; NSF Graduate Research Fellowship; Office of Science of the U. S. Department of Energy [DE-AC02-05CH11231, DE-AC05-00OR22725] FX This research has been supported by the DOE HEP Program under contract DE-SC0010676; the National Science Foundation (AST 0909129 and AST-1109896) and the NASA Theory Program (NNX09AK36G). D.K. is supported by a Department of Energy Office of Nuclear Physics Early Career Award (DE-SC0008067). Rainer Moll acknowledges support by the Alexander von Humboldt Foundation through the Feodor Lynen Research Fellowship program. J.S. is supported by an NSF Graduate Research Fellowship. We thank John Bell and Ann Almgren for their major roles in developing the CASTRO code. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U. S. Department of Energy under Contract No. DE-AC05-00OR22725. We are grateful for computer time supplied by the Advanced Computing Center at Arizona State University, and to Frank Timmes for technical support and for insightful discussions during the construction of our nuclear network. NR 60 TC 25 Z9 25 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 75 DI 10.1088/0004-637X/788/1/75 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200075 ER PT J AU Todorov, KO Luhman, KL Konopacky, QM McLeod, KK Apai, D Ghez, AM Pascucci, I Robberto, M AF Todorov, K. O. Luhman, K. L. Konopacky, Q. M. McLeod, K. K. Apai, D. Ghez, A. M. Pascucci, I. Robberto, M. TI A SEARCH FOR COMPANIONS TO BROWN DWARFS IN THE TAURUS AND CHAMAELEON STAR-FORMING REGIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: visual; brown dwarfs; stars: formation; stars: low-mass; stars: pre-main sequence ID UPPER SCORPIUS ASSOCIATION; ADAPTIVE OPTICS SYSTEM; PLANETARY-MASS BINARY; DISK POPULATION; WIDE BINARIES; DISCOVERY; MULTIPLICITY; ACCRETION; CANDIDATE; BOUNDARY AB We have used WFPC2 on board the Hubble Space Telescope to obtain images of 47 members of the Taurus and Chamaeleon I star-forming regions that have spectral types of M6-L0 (M similar to 0.01-0.1 M-circle dot). An additional late-type member of Taurus, FU Tau (M7.25+M9.25), was also observed with adaptive optics at Keck Observatory. In these images, we have identified promising candidate companions to 2MASS J04414489+2301513 (rho = 0.'' 105/15 AU), 2MASS J04221332+1934392 (rho = 0.'' 05/7 AU), and ISO 217 (rho = 0.'' 03/5 AU). We reported the first candidate in a previous study, showing that it has a similar proper motion as the primary in images from WFPC2 and Gemini adaptive optics. We have collected an additional epoch of data with Gemini that further supports that result. By combining our survey with previous high-resolution imaging in Taurus, Chamaeleon I, and Upper Sco (tau similar to 10 Myr), we measure binary fractions of 14/93 = 0.15(-0.03)(+0.05) for M4-M6 (M similar to 0.1-0.3 M-circle dot and 4/108 = 0.04+0.03 -0.01 for > M6 (M less than or similar to 0.1 M-circle dot) at separations of > 10 AU. Given the youth and low density of these regions, the lower binary fraction at later types is probably primordial rather than due to dynamical interactions among association members. The widest low-mass binaries (> 100 AU) also appear to be more common in Taurus and Chamaeleon I than in the field, which suggests that the widest low-mass binaries are disrupted by dynamical interactions at > 10 Myr, or that field brown dwarfs have been born predominantly in denser clusters where wide systems are disrupted or inhibited from forming. C1 [Todorov, K. O.; Luhman, K. L.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Luhman, K. L.] Penn State Univ, Ctr Exoplanets & Habitable Worlds, University Pk, PA 16802 USA. [Konopacky, Q. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [McLeod, K. K.] Wellesley Coll, Whitin Observ, Wellesley, MA 02481 USA. [Apai, D.; Pascucci, I.] Univ Arizona, Dept Astron, Tucson, AZ 85721 USA. [Apai, D.; Pascucci, I.] Lunar & Planetary Lab, Tucson, AZ 85721 USA. [Ghez, A. M.] Univ Calif Los Angeles, Div Astron & Astrophys, Los Angeles, CA 90095 USA. [Ghez, A. M.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90095 USA. [Robberto, M.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Robberto, M.] Johns Hopkins Univ, Ctr Astrophys Sci, Baltimore, MD 21218 USA. RP Todorov, KO (reprint author), ETH, Inst Astron, Wolfgang Pauli Str 27, CH-8093 Zurich, Switzerland. EM todorovk@phys.ethz.ch OI Todorov, Kamen/0000-0002-9276-8118; Robberto, Massimo/0000-0002-9573-3199 FU NASA Origins of Solar Systems program [NNX11AG57G]; Pennsylvania State University; Eberly College of Science; Pennsylvania Space Grant Consortium FX We thank Allison Youngblood, Steven Mohammed, Ijeoma Ekeh, and Jaclyn Payne for assistance with the data analysis. We acknowledge support from grant AST-0544588 from the National Science Foundation and grants GO-11203, GO-11204, and GO-11983 from the Space Telescope Science Institute. D. A. also acknowledges support from grant NNX11AG57G from the NASA Origins of Solar Systems program. The Gemini data were obtained through program GN-2011A-Q-10. Gemini Observatory is operated by AURA under a cooperative agreement with the NSF on behalf of the Gemini partnership: the NSF (United States), the Particle Physics and Astronomy Research Council (United Kingdom), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), CNPq (Brazil) and CONICET (Argentina). The Center for Exoplanets and Habitable Worlds is supported by the Pennsylvania State University, the Eberly College of Science, and the Pennsylvania Space Grant Consortium. MultiDrizzle is a product of the Space Telescope Science Institute, which is operated by AURA for NASA. NR 57 TC 11 Z9 11 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 10 PY 2014 VL 788 IS 1 AR 40 DI 10.1088/0004-637X/788/1/40 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AI7RY UT WOS:000337095200040 ER PT J AU Owen, H Holder, D Alonso, J Mackay, R AF Owen, Hywel Holder, David Alonso, Jose Mackay, Ranald TI Technologies for delivery of proton and ion beams for radiotherapy SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Article ID NEUTRON-CAPTURE THERAPY; DIELECTRIC WALL ACCELERATOR; CANCER-THERAPY; COMPUTED-TOMOGRAPHY; RADIATION-THERAPY; HADRON THERAPY; CONCEPTUAL DESIGN; NITROGEN IONS; GANTRY; COMPACT AB Recent developments for the delivery of proton and ion beam therapy have been significant, and a number of technological solutions now exist for the creation and utilisation of these particles for the treatment of cancer. In this paper we review the historical development of particle accelerators used for external beam radiotherapy and discuss the more recent progress towards more capable and cost-effective sources of particles. C1 [Owen, Hywel; Holder, David] Univ Manchester, Cockcroft Inst, Schuster Lab, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Alonso, Jose] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. [Mackay, Ranald] Christie NHS Fdn Trust, Manchester, Lancs, England. RP Owen, H (reprint author), Univ Manchester, Cockcroft Inst, Schuster Lab, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. EM hywel.owen@manchester.ac.uk; david.holder@cockcroft.ac.uk; jralonso@lbl.gov; ranald.mackay@christie.nhs.uk RI Owen, Hywel/G-4548-2014; Mackay, Ranald/M-6941-2015 OI Owen, Hywel/0000-0001-5028-2841; Mackay, Ranald/0000-0002-7329-6127 FU United Kingdom Science and Technology Facilities Council FX This work was supported in part by the United Kingdom Science and Technology Facilities Council. NR 185 TC 6 Z9 6 U1 1 U2 13 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD JUN 10 PY 2014 VL 29 IS 14 SI SI AR 1441002 DI 10.1142/S0217751X14410024 PG 39 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AI5TJ UT WOS:000336931800003 ER PT J AU Egami, T AF Egami, T. TI Elementary excitation and energy landscape in simple liquids SO MODERN PHYSICS LETTERS B LA English DT Review DE Liquid; glass transition; viscosity; fragility ID GLASS-FORMING LIQUIDS; SUPERCOOLED LIQUIDS; POISSONS RATIO; COMPUTER-SIMULATION; METALLIC GLASSES; VISCOUS-LIQUIDS; TRANSITION; FRAGILITY; DYNAMICS; ALLOYS AB The nature of excitations in liquids has been a subject of debate for a long time. In liquids, phonons are extremely short-lived and marginalized. Instead, recent research results indicate that local topological or configurational excitations (anankeons) are the elementary excitations in high temperature metallic liquids. Local topological excitations are those which locally alter the atomic connectivity network by cutting or forming atomic bonds, and are directly tied to the atomistic origin of viscosity in the liquid. The local potential energy landscape (PEL) of anankeons represents the probability weighted projection of the global PEL to a single atom. The original PEL is an insightful concept, but is highly multi-dimensional and difficult to characterize or even to visualize. A description in terms of the local PEL for anankeons appears to offer a simpler and more effective approach toward this complex problem. At the base of these advances, is the recognition that atomic discreteness and the topology of atomic connectivity are the most crucial features of the structure in liquids, which current nonlinear continuum theories cannot fully capture. These discoveries could open the way to the explanation of various complex phenomena in liquids, such as atomic transport, fragility, and the glass transition, in terms of these excitations. C1 [Egami, T.] Univ Tennessee, Dept Mat Sci & Engn, Joint Inst Neutron Sci, Knoxville, TN 37996 USA. [Egami, T.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Egami, T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Egami, T (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Joint Inst Neutron Sci, Knoxville, TN 37996 USA. EM egami@utk.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division FX The author is grateful to S. Sastry, J. S. Langer, J. Bellissard, K. Kelton, T. Iwashita and J. R. Morris for useful discussions. The work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division. NR 55 TC 6 Z9 6 U1 4 U2 42 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-9849 EI 1793-6640 J9 MOD PHYS LETT B JI Mod. Phys. Lett. B PD JUN 10 PY 2014 VL 28 IS 14 AR 1430006 DI 10.1142/S0217984914300063 PG 19 WC Physics, Applied; Physics, Condensed Matter; Physics, Mathematical SC Physics GA AI7RD UT WOS:000337092400001 ER PT J AU Harris, WM Lombardo, JJ Nelson, GJ Lai, B Wang, S Vila-Comamala, J Liu, MF Liu, ML Chiu, WKS AF Harris, William M. Lombardo, Jeffrey J. Nelson, George J. Lai, Barry Wang, Steve Vila-Comamala, Joan Liu, Mingfei Liu, Meilin Chiu, Wilson K. S. TI Three-Dimensional Microstructural Imaging of Sulfur Poisoning-Induced Degradation in a Ni-YSZ Anode of Solid Oxide Fuel Cells SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY NANOTOMOGRAPHY; NICKEL-SULFUR; RECONSTRUCTION; TEMPERATURE; MICROSCOPY; SPECTROSCOPY; SULFIDATION; ELECTRODES; NANOSCALE; KINETICS AB Following exposure to ppm-level hydrogen sulfide at elevated temperatures, a section of a solid oxide fuel cell (SOFC) Ni-YSZ anode was examined using a combination of synchrotron-based x-ray nanotomography and x-ray fluorescence techniques. While fluorescence measurements provided elemental identification and coarse spatial mapping, x-ray nanotomography was used to map the detailed 3-D spatial distribution of Ni, YSZ, and a nickel-sulfur poisoning phase. The nickel-sulfur layer was found to form a scale covering most of the exposed nickel surface, blocking most fuel reformation and hydrogen oxidation reaction sites. Although the exposure conditions precluded the ability to develop a detailed kinetic description of the nickel-sulfur phase formation, the results provide strong evidence of the detrimental effects of 100 ppm hydrogen sulfide on typical Ni-YSZ anode materials. C1 [Harris, William M.; Lombardo, Jeffrey J.; Nelson, George J.; Liu, Mingfei; Liu, Meilin; Chiu, Wilson K. S.] Univ Connecticut, HeteroFoaM Ctr, Storrs, CT 06269 USA. [Harris, William M.; Lombardo, Jeffrey J.; Nelson, George J.; Chiu, Wilson K. S.] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. [Lai, Barry; Wang, Steve; Vila-Comamala, Joan] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Liu, Mingfei; Liu, Meilin] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Chiu, WKS (reprint author), Univ Connecticut, HeteroFoaM Ctr, Storrs, CT 06269 USA. EM wchiu@engr.uconn.edu RI Liu, Meilin/E-5782-2010; Vila-Comamala, Joan/E-2106-2017 OI Liu, Meilin/0000-0002-6188-2372; FU Energy Frontier Research Center on Science Based Nano-Structure Design and Synthesis of Heterogeneous Functional Materials for Energy Systems (HeteroFoaM Center) - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001061]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Financial support from an Energy Frontier Research Center on Science Based Nano-Structure Design and Synthesis of Heterogeneous Functional Materials for Energy Systems (HeteroFoaM Center) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (Award DE-SC0001061) is gratefully acknowledged. Portions of this research were carried out at the Advanced Photon Source supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 43 TC 9 Z9 9 U1 2 U2 61 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 10 PY 2014 VL 4 AR 5246 DI 10.1038/srep05246 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI6EK UT WOS:000336963400004 PM 24912978 ER PT J AU Caro, M Mook, WM Fu, EG Wang, YQ Sheehan, C Martinez, E Baldwin, JK Caro, A AF Caro, M. Mook, W. M. Fu, E. G. Wang, Y. Q. Sheehan, C. Martinez, E. Baldwin, J. K. Caro, A. TI Radiation induced effects on mechanical properties of nanoporous gold foams SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; YIELD STRENGTH; AU; BEHAVIOR; MICROFABRICATION; EVOLUTION AB It has recently been shown that due to a high surface-to-volume ratio, nanoporous materials display radiation tolerance. The abundance of surfaces, which are perfect sinks for defects, and the relation between ligament size, defect diffusion, and time combine to define a window of radiation resistance [Fu et al., Appl. Phys. Lett. 101, 191607 (2012)]. Outside this window, the dominant defect created by irradiation in Au nanofoams are stacking fault tetrahedra (SFT). Molecular dynamics computer simulations of nanopillars, taken as the elemental constituent of foams, predict that SFTs act as dislocation sources inducing softening, in contrast to the usual behavior in bulk materials, where defects are obstacles to dislocation motion, producing hardening. In this work we test that prediction and answer the question whether irradiation actually hardens or softens a nanofam. Ne ion irradiations of gold nanofoams were performed at room temperature for a total dose up to 4 dpa, and their mechanical behavior was measured by nanoindentation. We find that hardness increases after irradiation, a result that we analyze in terms of the role of SFTs on the deformation mode of foams. (C) 2014 AIP Publishing LLC. C1 [Caro, M.; Fu, E. G.; Wang, Y. Q.; Martinez, E.; Caro, A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Mook, W. M.; Sheehan, C.; Baldwin, J. K.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Caro, M (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM magda@lanl.gov; efu@pku.edu.cn OI Martinez Saez, Enrique/0000-0002-2690-2622 FU Los Alamos Laboratory Directed Research and Development (LDRD) Program; DOE Energy Frontier Research Center (EFRC) for Materials under Irradiation and Mechanical Extremes FX Work funded by the Los Alamos Laboratory Directed Research and Development (LDRD) Program. A. C. also acknowledges support from the DOE Energy Frontier Research Center (EFRC) for Materials under Irradiation and Mechanical Extremes. Work performed in part at the Center for Integrated Nanotechnologies (CINT) an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. NR 39 TC 6 Z9 6 U1 6 U2 63 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 233109 DI 10.1063/1.4882275 PG 4 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200079 ER PT J AU de Vries, MA Loving, M McLaren, M Brydson, RMD Liu, X Langridge, S Lewis, LH Marrows, CH AF de Vries, M. A. Loving, M. McLaren, M. Brydson, R. M. D. Liu, X. Langridge, S. Lewis, L. H. Marrows, C. H. TI Asymmetric "melting" and "freezing" kinetics of the magnetostructural phase transition in B2-ordered FeRh epilayers SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROMAGNETIC TRANSITION; ROOM-TEMPERATURE; ALLOY; FILMS AB Synchrotron X-ray diffraction was used to study the phase transformation processes during the magnetostructural transition in a B2-ordered FeRh (001)-oriented epilayer grown on MgO by sputtering. Out-of-plane lattice constant measurements within the hysteretic regime of the transition reveal a microstructure consistent with the coexistence of lattice-expanded and contracted phases in spatially distinct regions. It was found that the phase separation is more pronounced during cooling than heating. Furthermore, whilst lattice-expanded domains that span the height of the film can be undercooled by several kelvins, there is no equivalent superheating. This asymmetry between the cooling and heating processes in FeRh is consistent with the difference in the kinetics of generic freezing and melting transitions. (C) 2014 AIP Publishing LLC. C1 [de Vries, M. A.; Marrows, C. H.] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [de Vries, M. A.] Univ Edinburgh, Sch Chem, Edinburgh EH9 3JJ, Midlothian, Scotland. [Loving, M.; Lewis, L. H.] Northeastern Univ, Dept Chem Engn, Boston, MA 02115 USA. [McLaren, M.; Brydson, R. M. D.] Univ Leeds, Inst Mat Res, Leeds LS2 9JT, W Yorkshire, England. [Liu, X.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Liu, X.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Liu, X.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Liu, X.] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Langridge, S.] Rutherford Appleton Lab, Sci & Technol Facil Council, ISIS, Didcot OX11 0QX, Oxon, England. RP de Vries, MA (reprint author), Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. EM m.a.devries@ed.ac.uk; c.h.marrows@leeds.ac.uk OI Langridge, Sean/0000-0003-1104-0772 FU National Science Foundation [DMR-0908767]; UK Engineering and Physical Sciences Research Council [EP/G065640/1]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We gratefully acknowledge the help and advice from M. Ali, J. S. Weaver, and N. A. Porter in Leeds. This work was supported by a linked grant through the Materials World Network scheme by the National Science Foundation under Grant No. DMR-0908767 and the UK Engineering and Physical Sciences Research Council, Grant No. EP/G065640/1. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We would like to thank Dario Arena for assistance with the experiments at X22C and Jean Jordan-Sweet for the loan of a furnace used there. NR 41 TC 8 Z9 8 U1 1 U2 33 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 232407 DI 10.1063/1.4883369 PG 5 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200056 ER PT J AU Eliseev, EA Morozovska, AN Ievlev, AV Balke, N Maksymovych, P Tselev, A Kalinin, SV AF Eliseev, Eugene A. Morozovska, Anna N. Ievlev, Anton V. Balke, Nina Maksymovych, Peter Tselev, Alexander Kalinin, Sergei V. TI Electrostrictive and electrostatic responses in contact mode voltage modulated scanning probe microscopies SO APPLIED PHYSICS LETTERS LA English DT Article ID PIEZORESPONSE FORCE MICROSCOPY; NANOMETER RESOLUTION; THIN-FILMS; NANOSCALE; POLARIZATION; FERROELECTRICS; CAPACITORS; BEHAVIOR; SURFACE AB Electromechanical response of solids underpins image formation mechanism of several scanning probe microscopy techniques including the piezoresponse force microscopy (PFM) and electrochemical strain microscopy (ESM). While the theory of linear piezoelectric and ionic responses are well developed, the contributions of quadratic effects including electrostriction and capacitive tip-surface forces to measured signal remain poorly understood. Here, we analyze the electrostrictive and capacitive contributions to the PFM and ESM signals and discuss the implications of the dielectric tip-surface gap on these interactions. (C) 2014 AIP Publishing LLC. C1 [Eliseev, Eugene A.] NAS Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Morozovska, Anna N.] NAS Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Ievlev, Anton V.; Balke, Nina; Maksymovych, Peter; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37922 USA. RP Morozovska, AN (reprint author), NAS Ukraine, Inst Phys, 46 Pr Nauki, UA-03028 Kiev, Ukraine. EM anna.n.morozovska@gmail.com; sergei2@ornl.gov RI Tselev, Alexander/L-8579-2015; Balke, Nina/Q-2505-2015; Kalinin, Sergei/I-9096-2012; Maksymovych, Petro/C-3922-2016; Ievlev, Anton/H-3678-2012 OI Tselev, Alexander/0000-0002-0098-6696; Balke, Nina/0000-0001-5865-5892; Kalinin, Sergei/0000-0001-5354-6152; Maksymovych, Petro/0000-0003-0822-8459; Ievlev, Anton/0000-0003-3645-0508 FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program; SFFR-NSF project (US National Science Foundation) [NSF-DMR-1210588]; SFFR-NSF project (State Fund of Fundamental State Fund of Fundamental Research of Ukraine) [UU48/002] FX A part of this research (A. V. I., P. M., A. T., and S. V. K.) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. N.B. acknowledges personal support provided by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program. A.N.M. and E. A. E. are grateful to Professor S. M. Ryabchenko for multiple discussions and acknowledge the support via bilateral SFFR-NSF project (US National Science Foundation under NSF-DMR-1210588 and State Fund of Fundamental State Fund of Fundamental Research of Ukraine, Grant No. UU48/002). NR 42 TC 6 Z9 6 U1 3 U2 70 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 232901 DI 10.1063/1.4882861 PG 5 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200065 ER PT J AU Hunter, A Beyerlein, IJ AF Hunter, A. Beyerlein, I. J. TI Predictions of an alternative pathway for grain-boundary driven twinning SO APPLIED PHYSICS LETTERS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; DEFORMATION MECHANISMS; NANOCRYSTALLINE AL; TEXTURE EVOLUTION; METALS; COPPER; CRYSTALS; SILVER; DISLOCATIONS AB The exceptional strength of nanoscale metallic grains is due to strain-accommodation mechanisms that are uncommon in their coarse-grained counterparts, such as deformation twinning. Using an ab initio density functional theory-phase field dislocation dynamics model, we provide evidence of an unconventional kinetic pathway for twin formation in nano-sized crystals involving two grain boundaries. It corresponds to greater favorability because it accommodates strain yet removes debilitating backstresses. A simple map is presented to relate the associated kinetics of nucleation and propagation to intrinsic material defect formation energies. (C) 2014 AIP Publishing LLC. C1 [Hunter, A.] Los Alamos Natl Lab, Computat Div 10, Los Alamos, NM 87545 USA. [Beyerlein, I. J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Hunter, A (reprint author), Los Alamos Natl Lab, Computat Div 10, POB 1663, Los Alamos, NM 87545 USA. EM ahunter@lanl.gov OI Hunter, Abigail/0000-0002-0443-4020 FU Los Alamos National Laboratory Directed Research and Development (LDRD) [20130745ECR]; Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026] FX A.H. acknowledges support from the Los Alamos National Laboratory Directed Research and Development (LDRD) Project No. 20130745ECR. I.J.B. acknowledges support by the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. 2008LANL1026. NR 36 TC 5 Z9 5 U1 2 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 233112 DI 10.1063/1.4883396 PG 4 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200082 ER PT J AU Li, SQ Zhou, W Buchholz, DB Ketterson, JB Ocola, LE Sakoda, K Chang, RPH AF Li, Shi-Qiang Zhou, Wei Buchholz, D. Bruce Ketterson, John B. Ocola, Leonidas E. Sakoda, Kazuaki Chang, Robert P. H. TI Ultra-sharp plasmonic resonances from monopole optical nanoantenna phased arrays SO APPLIED PHYSICS LETTERS LA English DT Article ID FANO RESONANCES; SPECTROSCOPY; ABSORPTION; SCATTERING; LIGHT AB Diffractively coupled plasmonic resonances possess both ultra-sharp linewidths and giant electric field enhancement around plasmonic nanostructures. They can be applied to create a new generation of sensors, detectors, and nano-optical devices. However, all current designs require stringent index-matching at the resonance condition that limits their applicability. Here, we propose and demonstrate that it is possible to relieve the index-matching requirement and to induce ultra-sharp plasmon resonances in an ordered vertically aligned optical nano-antenna phased array by transforming a dipole resonance to a monopole resonance with a mirror plane. Due to the mirror image effect, the monopole resonance not only retained the dipole features but also enhanced them. The engineered resonances strongly suppressed the radiative decay channel, resulting in a four-order of magnitude enhancement in local electric field and a Q-factor greater than 200. (C) 2014 AIP Publishing LLC. C1 [Li, Shi-Qiang; Buchholz, D. Bruce; Chang, Robert P. H.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Zhou, Wei] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Ketterson, John B.] Northwestern Univ, Dept Phys, Evanston, IL 60208 USA. [Ketterson, John B.; Sakoda, Kazuaki; Chang, Robert P. H.] NU NIMS Mat Innovat Ctr, Evanston, IL 60208 USA. [Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. [Sakoda, Kazuaki] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050047, Japan. RP Chang, RPH (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. EM r-chang@northwestern.edu RI Chang, R.P.H/B-7505-2009; SAKODA, Kazuaki/H-3006-2011; zhou, wei/D-2312-2017; OI zhou, wei/0000-0002-5257-3885; Li, Mike/0000-0002-4095-8606; Ocola, Leonidas/0000-0003-4990-1064 FU NSF [DMR-1121262, DMR 0843962]; QUEST [p20194, p20447]; Center for Nanoscale Materials in Argonne National Laboratory [CNM 25883, CNM 30831]; NSF-NSEC; NSF-MRSEC; Keck Foundation; State of Illinois; Northwestern University; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Supported by NSF funding (DMR-1121262 and DMR 0843962), QUEST computational resources (Project p20194 and Project p20447), and Center for Nanoscale Materials in Argonne National Laboratory (Project CNM 25883 and Project CNM 30831). Various characterizations were done in NUANCE center and KECK II Facilities in Northwestern University. The NUANCE Center and KECK II Facilities are supported by the NSF-NSEC, NSF-MRSEC, Keck Foundation, the State of Illinois, and Northwestern University. E-beam lithography was performed with JEOL-9300 in the Center for Nanoscale materials at Argonne National Laboratory. Use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. S.Q.L. acknowledges Peijun Guo, Yi Hua, and Teri W. Odom for helpful discussions. The parameters for simulation and experiments are in the supplementary materials. NR 32 TC 7 Z9 7 U1 4 U2 41 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 231101 DI 10.1063/1.4881323 PG 5 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200001 ER PT J AU Murphy, RD Torralva, B Adams, DP Yalisove, SM AF Murphy, Ryan D. Torralva, Ben Adams, David P. Yalisove, Steven M. TI Polarization dependent formation of femtosecond laser-induced periodic surface structures near stepped features SO APPLIED PHYSICS LETTERS LA English DT Article ID PULSES; SILICON AB Laser-induced periodic surface structures (LIPSS) are formed near 110 nm-tall Au microstructured edges on Si substrates after single-pulse femtosecond irradiation with a 150 fs pulse centered near a 780 nm wavelength. We investigate the contributions of Fresnel diffraction from step-edges and surface plasmon polariton (SPP) excitation to LIPSS formation on Au and Si surfaces. For certain laser polarization vector orientations, LIPSS formation is dominated by SPP excitation; however, when SPP excitation is minimized, Fresnel diffraction dominates. The LIPSS orientation and period distributions are shown to depend on which mechanism is activated. These results support previous observations of the laser polarization vector influencing LIPSS formation on bulk surfaces. (C) 2014 AIP Publishing LLC. C1 [Murphy, Ryan D.] Univ Michigan, Appl Phys Program, Ann Arbor, MI 48109 USA. [Torralva, Ben] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Adams, David P.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Yalisove, Steven M.] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. RP Murphy, RD (reprint author), Univ Michigan, Appl Phys Program, Ann Arbor, MI 48109 USA. FU Defense Threat Reduction Agency, Basic Research Award [IACRO 12-2026I]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Defense Threat Reduction Agency, Basic Research Award # IACRO 12-2026I. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 14 TC 7 Z9 7 U1 8 U2 36 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 231117 DI 10.1063/1.4882998 PG 5 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200017 ER PT J AU Schaab, J Krug, IP Nickel, F Gottlob, DM Doganay, H Cano, A Hentschel, M Yan, Z Bourret, E Schneider, CM Ramesh, R Meier, D AF Schaab, J. Krug, I. P. Nickel, F. Gottlob, D. M. Doganay, H. Cano, A. Hentschel, M. Yan, Z. Bourret, E. Schneider, C. M. Ramesh, R. Meier, D. TI Imaging and characterization of conducting ferroelectric domain walls by photoemission electron microscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID LITHIUM-NIOBATE; VORTEX DOMAINS; MULTIFERROICS; BATIO3; YMNO3; CONTRAST; DEVICES; FILMS AB High-resolution X-ray photoemission electron microscopy (X-PEEM) is a well-established method for imaging ferroelectric domain structures. Here, we expand the scope of application of X-PEEM and demonstrate its capability for imaging and investigating domain walls in ferroelectrics with high spatial resolution. Using ErMnO3 as test system, we show that ferroelectric domain walls can be visualized based on photo-induced charging effects and local variations in their electronic conductance can be mapped by analyzing the energy distribution of photoelectrons. Our results open the door for non-destructive, contact-free, and element-specific studies of the electronic and chemical structure at domain walls in ferroelectrics. (C) 2014 AIP Publishing LLC. C1 [Schaab, J.; Meier, D.] ETH, Dept Mat, CH-8093 Zurich, Switzerland. [Krug, I. P.] Tech Univ Berlin, Inst Opt & Atomare Phys, D-10623 Berlin, Germany. [Krug, I. P.; Nickel, F.; Gottlob, D. M.; Doganay, H.; Schneider, C. M.] Peter Grunberg Inst PGI 6, Forschungszentrum Julich, D-52425 Julich, Germany. [Cano, A.] Univ Bordeaux, ICMCB, CNRS, UPR 9048, F-33600 Pessac, France. [Hentschel, M.] Univ Suttgart, Phys Inst 4, D-70659 Stuttgart, Germany. [Hentschel, M.] Univ Suttgart, Res Ctr SCoPE, D-70659 Stuttgart, Germany. [Hentschel, M.; Yan, Z.; Bourret, E.; Ramesh, R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ramesh, R.] Univ Calif Berkeley, Dept Mat Sci & Mineral Engn, Berkeley, CA 94720 USA. RP Meier, D (reprint author), ETH, Dept Mat, Vladimir Prelog Weg 4, CH-8093 Zurich, Switzerland. EM dennis.meier@mat.ethz.ch RI Hentschel, Mario/N-2093-2015; Schneider, Claus/H-7453-2012 OI Schneider, Claus/0000-0002-3920-6255 FU Alexander von Humboldt Foundation FX The authors thank M. Fiebig, M. Trassin, Y. Kumagai, and N. A. Spaldin for fruitful discussions, M. Lilienblum for technical assistance, and the BESSY staff and A. Kaiser (Specs GmbH) for support. D. M. acknowledges financial support by the Alexander von Humboldt Foundation. NR 39 TC 9 Z9 9 U1 7 U2 77 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 232904 DI 10.1063/1.4879260 PG 4 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200068 ER PT J AU Shearer, AJ Johns, JE Caplins, BW Suich, DE Hersam, MC Harris, CB AF Shearer, Alex J. Johns, James E. Caplins, Benjamin W. Suich, David E. Hersam, Mark C. Harris, Charles B. TI Electron dynamics of the buffer layer and bilayer graphene on SiC SO APPLIED PHYSICS LETTERS LA English DT Article ID GRAPHITE; GAS; STATES; FEMTOSECOND; SURFACE AB Angle- and time-resolved two-photon photoemission (TPPE) was used to investigate electronic states in the buffer layer of 4H-SiC(0001). An image potential state (IPS) series was observed on this strongly surface-bound buffer layer, and dispersion measurements indicated free-electron-like behavior for all states in this series. These results were compared with TPPE taken on bilayer graphene, which also show the existence of a free-electron-like IPS series. Lifetimes for the n = 2, and n = 3 states were obtained from time-resolved TPPE; slightly increased lifetimes were observed in the bilayer graphene sample for the n = 2 the n = 3 states. Despite the large band gap of graphene at the center of the Brillouin zone, the lifetime results demonstrate that the graphene layers do not behave as a simple tunneling barrier, suggesting that the buffer layer and graphene overlayers play a direct role in the decay of IPS electrons. (C) 2014 AIP Publishing LLC. C1 [Shearer, Alex J.; Caplins, Benjamin W.; Suich, David E.; Harris, Charles B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shearer, Alex J.; Caplins, Benjamin W.; Suich, David E.; Harris, Charles B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Johns, James E.] Univ Minnesota Twin Cities, Dept Chem, Minneapolis, MN 55455 USA. [Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Hersam, Mark C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Harris, CB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM cbharris@berkeley.edu RI Hersam, Mark/B-6739-2009 FU Department of Energy [DE-FG02-09ER16109]; W. M. Keck Foundation Science and Engineering Grant; Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX J.E.J. and M. C. H. acknowledge the Department of Energy (DE-FG02-09ER16109) and a W. M. Keck Foundation Science and Engineering Grant. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 31 TC 3 Z9 3 U1 1 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 9 PY 2014 VL 104 IS 23 AR 231604 DI 10.1063/1.4882236 PG 5 WC Physics, Applied SC Physics GA AJ7QM UT WOS:000337891200023 ER PT J AU DeBord, JD Smith, DF Anderton, CR Heeren, RMA Pasa-Tolic, L Gomer, RH Fernandez-Lima, FA AF DeBord, John Daniel Smith, Donald F. Anderton, Christopher R. Heeren, Ron M. A. Pasa-Tolic, Ljiljana Gomer, Richard H. Fernandez-Lima, Francisco A. TI Secondary Ion Mass Spectrometry Imaging of Dictyostelium discoideum Aggregation Streams SO PLOS ONE LA English DT Article ID TOF-SIMS; LIPID-COMPOSITION; PLASMA-MEMBRANES; DIFFERENTIATION; IDENTIFICATION; PROJECTILES; ACCURACY; SURFACES; C-60(+); ENERGY AB High resolution imaging mass spectrometry could become a valuable tool for cell and developmental biology, but both, high spatial and mass spectral resolution are needed to enable this. In this report, we employed Bi-3 bombardment time-off-light (Bi-3 ToF-SIMS) and C-60 bombardment Fourier transform ion cyclotron resonance secondary ion mass spectrometry (C-60 FTICR-SIMS) to image Dictyostelium discoideum aggregation streams. Nearly 300 lipid species were identified from the aggregation streams. High resolution mass spectrometry imaging (FTICR-SIMS) enabled the generation of multiple molecular ion maps at the nominal mass level and provided good coverage for fatty acyls, prenol lipids, and sterol lipids. The comparison of Bi-3 ToF-SIMS and C-60 FTICR-SIMS suggested that while the first provides fast, high spatial resolution molecular ion images, the chemical complexity of biological samples warrants the use of high resolution analyzers for accurate ion identification. C1 [DeBord, John Daniel; Fernandez-Lima, Francisco A.] Florida Int Univ, Dept Chem & Biochem, Miami, FL 33199 USA. [Smith, Donald F.; Heeren, Ron M. A.] FOM Inst AMOLF, Amsterdam, Netherlands. [Anderton, Christopher R.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Gomer, Richard H.] Texas A&M Univ, Dept Biol, College Stn, TX 77843 USA. RP Fernandez-Lima, FA (reprint author), Florida Int Univ, Dept Chem & Biochem, Miami, FL 33199 USA. EM fernandf@fiu.edu RI Smith, Donald/K-3939-2013; OI Heeren, Ron/0000-0002-6533-7179; Gomer, Richard/0000-0003-2361-4307 FU NIGMS [R00GM106414, GM102280]; Department of Energy's Office of Biological and Environmental Research (DOE-BER) FX The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. This work was supported by NIGMS grants R00GM106414 to FF-L and GM102280 to RHG. A portion of this research was performed at the W. R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research (DOE-BER) and located at Pacific Northwest National Laboratory (PNNL). This work is part of the research program of the Foundation for Fundamental Research on Matter (FOM), which is part of The Netherlands Organization for Scientific Research (NWO). NR 47 TC 3 Z9 3 U1 3 U2 37 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 9 PY 2014 VL 9 IS 6 AR e99319 DI 10.1371/journal.pone.0099319 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AI8LF UT WOS:000337165600073 PM 24911189 ER PT J AU Hiyama, E Ohnishi, S Gibson, BF Rijken, TA AF Hiyama, E. Ohnishi, S. Gibson, B. F. Rijken, Th. A. TI Three-body structure of the nn Lambda system with Lambda N - Sigma N coupling SO PHYSICAL REVIEW C LA English DT Article ID HYPERNUCLEI AB The structure of the three-body nn Lambda system, which has been observed recently by the HypHI Collaboration, is investigated taking Lambda N-Sigma N coupling explicitly into account. The YN and NN interactions employed in this work reproduce the binding energies of (3)(Lambda) H, (4)(Lambda) H, and (4)(Lambda) He. We do not find any (3)(Lambda) n bound state, which contradicts the interpretation of the data reported by the HypHI Collaboration. C1 [Hiyama, E.; Ohnishi, S.] RIKEN, Inst Phys & Chem Res, Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. [Ohnishi, S.] Tokyo Inst Technol, Dept Phys, Meguro 1528551, Japan. [Gibson, B. F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Rijken, Th. A.] Radboud Univ Nijmegen, IMAPP, NL-6525 ED Nijmegen, Netherlands. RP Hiyama, E (reprint author), RIKEN, Inst Phys & Chem Res, Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. RI Hiyama, Emiko/N-6413-2015 OI Hiyama, Emiko/0000-0002-6352-5766 FU Monbukagakusho of Japan; JSPS [23224006]; RIKEN iTHES Project; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The authors thank Dr. T. Saito, Dr. C. Rappold, and Prof. Gal for valuable discussions. This work was supported by a Grant-in-Aid for Scientific Research from Monbukagakusho of Japan. The numerical calculations were performed on the HITACHI SR16000 at KEK and YITP. This work was partly supported by JSPS Grant No. 23224006 and by RIKEN iTHES Project. The work of B.F.G. was performed under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 22 TC 17 Z9 17 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUN 9 PY 2014 VL 89 IS 6 AR 061302 DI 10.1103/PhysRevC.89.061302 PG 5 WC Physics, Nuclear SC Physics GA AI6IT UT WOS:000336977300001 ER PT J AU Acciarri, R Adams, C Asaadi, J Baller, B Bolton, T Bromberg, C Cavanna, F Church, E Edmunds, D Ereditato, A Farooq, S Fleming, B Greenlee, H Hatcher, R Horton-Smith, G James, C Klein, E Lang, K Laurens, P Mehdiyev, R Page, B Palamara, O Partyka, K Rameika, G Rebel, B Soderberg, M Spitz, J Szelc, AM Weber, M Yang, T Zeller, GP AF Acciarri, R. Adams, C. Asaadi, J. Baller, B. Bolton, T. Bromberg, C. Cavanna, F. Church, E. Edmunds, D. Ereditato, A. Farooq, S. Fleming, B. Greenlee, H. Hatcher, R. Horton-Smith, G. James, C. Klein, E. Lang, K. Laurens, P. Mehdiyev, R. Page, B. Palamara, O. Partyka, K. Rameika, G. Rebel, B. Soderberg, M. Spitz, J. Szelc, A. M. Weber, M. Yang, T. Zeller, G. P. CA ArgoNeut Collaboration TI Measurements of inclusive muon neutrino and antineutrino charged current differential cross sections on argon in the NuMI antineutrino beam SO PHYSICAL REVIEW D LA English DT Article AB The ArgoNeuT collaboration presents measurements of inclusive muon neutrino and antineutrino charged current differential cross sections on argon in the Fermilab NuMI beam operating in the low energy antineutrino mode. The results are reported in terms of outgoing muon angle and momentum at a mean neutrino energy of 9.6 GeV (neutrinos) and 3.6 GeV (antineutrinos), in the range 0 degrees < theta(mu) < 36 degrees and 0 < p(mu) < 25 GeV / c, for both neutrinos and antineutrinos. C1 [Acciarri, R.; Baller, B.; Greenlee, H.; Hatcher, R.; James, C.; Rameika, G.; Rebel, B.; Soderberg, M.; Yang, T.; Zeller, G. P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, C.; Cavanna, F.; Church, E.; Klein, E.; Palamara, O.; Partyka, K.; Spitz, J.; Szelc, A. M.] Yale Univ, New Haven, CT 06520 USA. [Asaadi, J.; Soderberg, M.] Syracuse Univ, Syracuse, NY 13244 USA. [Bolton, T.; Farooq, S.; Horton-Smith, G.] Kansas State Univ, Manhattan, KS 66506 USA. [Bromberg, C.; Edmunds, D.; Laurens, P.] Michigan State Univ, E Lansing, MI 48824 USA. [Cavanna, F.] Univ Aquila, I-67100 Laquila, Italy. [Cavanna, F.] Ist Nazl Fis Nucl, I-67100 Laquila, Italy. [Ereditato, A.; Weber, M.] Univ Bern, CH-3012 Bern, Switzerland. [Lang, K.; Mehdiyev, R.] Univ Texas Austin, Austin, TX 78712 USA. [Palamara, O.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67100 Assergi, Italy. RP Acciarri, R (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Horton-Smith, Glenn/A-4409-2011; OI Horton-Smith, Glenn/0000-0001-9677-9167; Spitz, Joshua/0000-0002-6288-7028; Weber, Michele/0000-0002-2770-9031; Cavanna, Flavio/0000-0002-5586-9964 NR 24 TC 15 Z9 15 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUN 9 PY 2014 VL 89 IS 11 AR 112003 DI 10.1103/PhysRevD.89.112003 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AI6IY UT WOS:000336977900001 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M De Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Ranjan, N Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Vazquez, F Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. Datta, M. De Barbaro, P. Demortier, L. Deninno, M. D'Errico, M. Devoto, F. Di Canto, A. Di Ruzza, B. Dittmann, J. R. Donati, S. D'Onofrio, M. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Elagin, A. Erbacher, R. Errede, S. Esham, B. Farrington, S. Ramos, J. P. Fernandez Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Galloni, C. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Giurgiu, G. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Lopez, O. Gonzalez Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grinstein, S. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, W. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. H. Kim, S. B. Kim, Y. J. Kim, Y. K. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, H. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Lucchesi, D. Luca, A. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Martinez, M. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. Moore, R. Morello, M. J. Mukherjee, A. Muller, Th. Murat, P. Mussini, M. Nachtman, J. Nagai, Y. Naganoma, J. Nakano, I. Napier, A. Nett, J. Neu, C. Nigmanov, T. Nodulman, L. Noh, S. Y. Norniella, O. Oakes, L. Oh, S. H. Oh, Y. D. Oksuzian, I. Okusawa, T. Orava, R. Ortolan, L. Pagliarone, C. Palencia, E. Palni, P. Papadimitriou, V. Parker, W. Pauletta, G. Paulini, M. Paus, C. Phillips, T. J. Piacentino, G. Pianori, E. Pilot, J. Pitts, K. Plager, C. Pondrom, L. Poprocki, S. Potamianos, K. Pranko, A. Prokoshin, F. Ptohos, F. Punzi, G. Ranjan, N. Fernandez, I. Redondo Renton, P. Rescigno, M. Rimondi, F. Ristori, L. Robson, A. Rodriguez, T. Rolli, S. Ronzani, M. Roser, R. Rosner, J. L. Ruffini, F. Ruiz, A. Russ, J. Rusu, V. Sakumoto, W. K. Sakurai, Y. Santi, L. Sato, K. Saveliev, V. Savoy-Navarro, A. Schlabach, P. Schmidt, E. E. Schwarz, T. Scodellaro, L. Scuri, F. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shochet, M. Shreyber-Tecker, I. Simonenko, A. Sliwa, K. Smith, J. R. Snider, F. D. Song, H. Sorin, V. Denis, R. St. Stancari, M. Stentz, D. Strologas, J. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thomson, E. Thukral, V. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Ukegawa, F. Uozumi, S. Velev, G. Vellidis, C. Vernieri, C. Vidal, M. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Vazquez, F. Wagner, P. Wallny, R. Wang, S. M. Waters, D. Wester, W. C., III Whiteson, D. Wicklund, A. B. Wilbur, S. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamato, D. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Zanetti, A. M. Zeng, Y. Zhou, C. Zucchelli, S. CA CDF Collaboration TI Search for s-Channel Single-Top-Quark Production in Events with Missing Energy Plus Jets in p(p)over-bar Collisions at root s=1.96 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLLIDER DETECTOR; FERMILAB AB The first search for single-top-quark production from the exchange of an s-channel virtual W boson using events with an imbalance in the total transverse energy, b-tagged jets, and no identified leptons is presented. Assuming the electroweak production of top quarks of mass 172.5 GeV/c(2) in the s channel, a cross section of 1.12(-0.57)(+0.61) (stat + syst) pb with a significance of 1.9 standard deviations is measured. This measurement is combined with the result obtained from events with an imbalance in total transverse momentum, b-tagged jets, and exactly one identified lepton, yielding a cross section of 1.36(-0.32)(+0.37) (stat + syst) pb, with a significance of 4.2 standard deviations. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.; Yoshida, T.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Manca, G.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece. [Camarda, S.; Cavalli-Sforza, M.; Grinstein, S.; Martinez, M.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, ICREA, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Bland, K. R.; Dittmann, J. R.; Hatakeyama, K.; Kasmi, A.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Castro, A.; Deninno, M.; Gramellini, E.; Marchese, L.; Mazzanti, P.; Moggi, N.; Mussini, M.; Rimondi, F.] Ist Nazl Fis Nucl, I-40126 Bologna, Italy. [Brigliadori, L.; Zucchelli, S.] Univ Bologna, I-40127 Bologna, Italy. [Chertok, M.; Conway, J.; Cox, C. A.; Cox, D. J.; Erbacher, R.; Forrest, R.; Ivanov, A.; Pilot, J.; Shalhout, S. Z.; Smith, J. R.; Wilbur, S.] Univ Calif Davis, Davis, CA 95616 USA. [Plager, C.] Univ Calif Los Angeles, Los Angeles, CA 90024 USA. [Casal, B.; Cuevas, J.; Gomez, G.; Palencia, E.; Ruiz, A.; Scodellaro, L.; Vilar, R.; Vizan, J.] Univ Cantabria, CSIC, Inst Fis Cantabria, E-39005 Santander, Spain. [Calamba, A.; Jang, D.; Jun, S. Y.; Paulini, M.; Russ, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Boveia, A.; Canelli, F.; Frisch, H.; Grosso-Pilcher, C.; Ketchum, W.; Kim, Y. K.; Rosner, J. L.; Shochet, M.; Tang, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Comenius Univ, Bratislava 84248, Slovakia. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Inst Expt Vet Med, Kosice 04001, Slovakia. [Artikov, A.; Budagov, J.; Chokheli, D.; Glagolev, V.; Prokoshin, F.; Semenov, A.; Simonenko, A.; Suslov, I.] Joint Inst Nucl Res, RU-141980 Dubna, Russia. [Benjamin, D.; Bocci, A.; Goshaw, A. T.; Kotwal, A. V.; Kruse, M.; Limosani, A.; Oh, S. H.; Phillips, T. J.; Yu, G. B.; Zeng, Y.; Zhou, C.] Duke Univ, Durham, NC 27708 USA. [Anastassov, A.; Apollinari, G.; Appel, J. A.; Ashmanskas, W.; Badgett, W.; Behari, S.; Beretvas, A.; Burkett, K.; Chlachidze, G.; Convery, M. E.; Corbo, M.; Culbertson, R.; d'Ascenzo, N.; Datta, M.; Di Ruzza, B.; Flanagan, G.; Freeman, J. C.; Gerchtein, E.; Ginsburg, C. M.; Glenzinski, D.; Golossanov, A.; Group, R. C.; Hahn, S. R.; Harrington-Taber, T.; Hocker, A.; Hopkins, W.; James, E.; Jayatilaka, B.; Jindariani, S.; Junk, T. R.; Kilminster, B.; Kirby, M.; Knoepfel, K.; Lammel, S.; Lewis, J. D.; Liu, T.; Lukens, P.; Madrak, R.; Mazzacane, A.; Miao, T.; Moed, S.; Moon, C. S.; Moore, R.; Mukherjee, A.; Murat, P.; Nachtman, J.; Papadimitriou, V.; Poprocki, S.; Ristori, L.; Roser, R.; Rusu, V.; Saveliev, V.; Savoy-Navarro, A.; Schlabach, P.; Schmidt, E. E.; Snider, F. D.; Stancari, M.; Stentz, D.; Sukhanov, A.; Thom, J.; Tonelli, D.; Torretta, D.; Velev, G.; Vellidis, C.; Wallny, R.; Wester, W. 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[Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Piacentino, Giovanni/K-3269-2015; Liu, Qiuguang/I-8258-2014; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Chiarelli, Giorgio/E-8953-2012; Cavalli-Sforza, Matteo/H-7102-2015; Introzzi, Gianluca/K-2497-2015 OI Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; Chiarelli, Giorgio/0000-0001-9851-4816; Introzzi, Gianluca/0000-0002-1314-2580 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation, the Italian Istituto Nazionale di Fisica Nucleare, the Ministry of Education, Culture, Sports, Science and Technology of Japan, the Natural Sciences and Engineering Research Council of Canada, the National Science Council of the Republic of China, the Swiss National Science Foundation, the A. P. Sloan Foundation, the Bundesministerium fur Bildung und Forschung, Germany, the Korean World Class University Program, the National Research Foundation of Korea, the Science and Technology Facilities Council and the Royal Society, United Kingdom, the Russian Foundation for Basic Research, the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain, the Slovak R&D Agency, the Academy of Finland, the Australian Research Council (ARC), and the EU community Marie Curie Fellowship Contract No. 302103. NR 34 TC 8 Z9 8 U1 1 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 9 PY 2014 VL 112 IS 23 AR 231805 DI 10.1103/PhysRevLett.112.231805 PG 8 WC Physics, Multidisciplinary SC Physics GA AI6JY UT WOS:000336981200006 PM 24972199 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M De Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Ranjan, N Redondo, I Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Vazquez, F Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. 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CA CDF Collaboration TI Evidence for s-Channel Single-Top-Quark Production in Events with One Charged Lepton and Two Jets at CDF SO PHYSICAL REVIEW LETTERS LA English DT Article ID P(P)OVER-BAR COLLISIONS; ROOT-S=7 TEV; BOSON; ATLAS AB We report evidence for s-channel single-top-quark production in proton-antiproton collisions at center-of-mass energy root s = 1.96 TeV using a data set that corresponds to an integrated luminosity of 9.4 fb(-1) collected by the Collider Detector at Fermilab. We select events consistent with the s-channel process including two jets and one leptonically decaying W boson. The observed significance is 3.8 standard deviations with respect to the background-only prediction. Assuming a top-quark mass of 172.5 GeV/c(2), we measure the s-channel cross section to be 1.41(-0.42)(+0.44) pb. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Wang, S. M.; Yoshida, T.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Nodulman, L.; Wicklund, A. 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RI Cavalli-Sforza, Matteo/H-7102-2015; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Chiarelli, Giorgio/E-8953-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; OI Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756; Torre, Stefano/0000-0002-7565-0118; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; Chiarelli, Giorgio/0000-0001-9851-4816; Casarsa, Massimo/0000-0002-1353-8964; Margaroli, Fabrizio/0000-0002-3869-0153; Latino, Giuseppe/0000-0002-4098-3502; iori, maurizio/0000-0002-6349-0380; Jun, Soon Yung/0000-0003-3370-6109; Toback, David/0000-0003-3457-4144; Vidal Marono, Miguel/0000-0002-2590-5987; Hays, Chris/0000-0003-2371-9723; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Group, Robert/0000-0002-4097-5254; Simonenko, Alexander/0000-0001-6580-3638; Lancaster, Mark/0000-0002-8872-7292 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation, the Italian Istituto Nazionale di Fisica Nucleare, the Ministry of Education, Culture, Sports, Science and Technology of Japan, the Natural Sciences and Engineering Research Council of Canada, the National Science Council of the Republic of China, the Swiss National Science Foundation, the A. P. Sloan Foundation, the Bundesministerium fur Bildung und Forschung, Germany, the Korean World Class University Program, the National Research Foundation of Korea, the Science and Technology Facilities Council and the Royal Society, United Kingdom, the Russian Foundation for Basic Research, the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain, the Slovak R&D Agency, the Academy of Finland, the Australian Research Council (ARC), and the EU community Marie Curie Fellowship Contract No. 302103. NR 29 TC 15 Z9 15 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 9 PY 2014 VL 112 IS 23 AR 231804 DI 10.1103/PhysRevLett.112.231804 PG 8 WC Physics, Multidisciplinary SC Physics GA AI6JY UT WOS:000336981200005 PM 24972198 ER PT J AU Aaltonen, T Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Askew, A Atkins, S Auerbach, B Augsten, K Aurisano, A Avila, C Azfar, F Badaud, F Badgett, W Bae, T Bagby, L Baldin, B Bandurin, DV Banerjee, S Barbaro-Galtieri, A Barberis, E Baringer, P Barnes, VE Barnett, BA Barria, P Bartlett, JF Bartos, P Bassler, U Bauce, M Bazterra, V Bean, A Bedeschi, F Begalli, M Behari, S Bellantoni, L Bellettini, G Bellinger, J Benjamin, D Beretvas, A Beri, SB Bernardi, G Bernhard, R Bertram, I Besanon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Bhatti, A Bland, KR Blazey, G Blessing, S Bloom, K Blumenfeld, B Bocci, A Bodek, A Boehnlein, A Boline, D Boos, EE Borissov, G Bortoletto, D Borysova, M Boudreau, J Boveia, A Brandt, A Brandt, O Brigliadori, L Brock, R Bromberg, C Bross, A Brown, D Brucken, E Bu, XB Budagov, J Budd, HS Buehler, M Buescher, V Bunichev, V Burdin, S Burkett, K Busetto, G Bussey, P Buszello, CP Butti, P Buzatu, A Calamba, A Camacho-Perez, E Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Casey, BCK Castilla-Valdez, H Castro, A Catastini, P Caughron, S Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Cho, SW Choi, S Chokheli, D Choudhary, B Cihangir, S Claes, D Clark, A Clarke, C Clutter, J Convery, ME Conway, J Cooke, M Cooper, WE Corbo, M Corcoran, M Cordelli, M Couderc, F Cousinou, MC Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R Cutts, D Das, A d'Ascenzo, N Datta, M Davies, G De Barbaro, P De Jong, SJ De la Cruz-Burelo, E Deliot, F Demina, R Demortier, L Deninno, M Denisov, D Denisov, SP D'Errico, M Desai, S Deterre, C DeVaughan, K Devoto, F Di Canto, A Di Ruzza, B Diehl, HT Diesburg, M Ding, PF Dittmann, JR Dominguez, A Donati, S D'Onofrio, M Dorigo, M Driutti, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Ebina, K Edgar, R Edmunds, D Elagin, A Ellison, J Elvira, VD Enari, Y Erbacher, R Errede, S Esham, B Evans, H Evdokimov, VN Farrington, S Feng, L Ferbel, T Ramos, JPF Fiedler, F Field, R Filthaut, F Fisher, W Fisk, HE Flanagan, G Forrest, R Fortner, M Fox, H Franklin, M Freeman, JC Frisch, H Fuess, S Funakoshi, Y Galloni, C Garbincius, PH Garcia-Bellido, A Garca-Gonzalez, JA Garfinkel, AF Garosi, P Gavrilov, V Geng, W Gerber, CE Gerberich, H Gerchtein, E Gershtein, Y Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Ginther, G Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Golovanov, G Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grannis, PD Greder, S Greenlee, H Grenier, G Grinstein, S Gris, P Grivaz, JF Grohsjean, A Grosso-Pilcher, C Group, RC Grunendahl, S Grunewald, MW Guillemin, T Da Costa, JG Gutierrez, G Gutierrez, P Hahn, SR Haley, J Han, JY Han, L Happacher, F Hara, K Harder, K Hare, M Harel, A Harr, RF Harrington-Taber, T Hatakeyama, K Hauptman, JM Hays, C Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinrich, J Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herndon, M Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hocker, A Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Hong, Z Hopkins, W Hou, S Howley, I Hubacek, Z Hughes, RE Husemann, U Hussein, M Huston, J Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Introzzi, G Iori, M Ito, AS Ivanov, A Jabeen, S Jaffre, M James, E Jang, D Jayasinghe, A Jayatilaka, B Jeon, EJ Jeong, MS Jesik, R Jiang, P Jindariani, S Johns, K Johnson, E Johnson, M Jonckheere, A Jones, M Jonsson, P Joo, KK Joshi, J Jun, SY Jung, AW Junk, TR Juste, A Kajfasz, E Kambeitz, M Kamon, T Karchin, PE Karmanov, D Kasmi, A Kato, Y Katsanos, I Kehoe, R Kermiche, S Ketchum, W Keung, J Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Kiselevich, I Knoepfel, K Kohli, JM Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kozelov, AV Kraus, J Kreps, M Kroll, J Kruse, M Kuhr, T Kumar, A Kupco, A Kurata, M Kurca, T Kuzmin, VA Laasanen, AT Lammel, S Lammers, S Lancaster, M Lannon, K Latino, G Lebrun, P Lee, HS Lee, HS Lee, JS Lee, SW Lee, WM Lei, X Lellouch, J Leo, S Leone, S Lewis, JD Li, D Li, H Li, L Li, QZ Lim, JK Limosani, A Lincoln, D Linnemann, J Lipaev, VV Lipeles, E Lipton, R Lister, A Liu, H Liu, H Liu, Q Liu, T Liu, Y Lobodenko, A Lockwitz, S Loginov, A Lokajicek, M De Sa, RL Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Luna-Garcia, R Lungu, G Lyon, AL Lys, J Lysak, R Maciel, AKA Madar, R Madrak, R Maestro, P Magana-Villalba, R Malik, S Malik, S Malyshev, VL Manca, G Manousakis-Katsikakis, A Mansour, J Marchese, L Margaroli, F Marino, P Martinez-Ortega, J Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McCarthy, R McGivern, CL McNulty, R Mehta, A Mehtala, P Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Mesropian, C Meyer, A Meyer, J Miao, T Miconi, F Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Mondal, NK Moon, CS Moore, R Morello, MJ Mukherjee, A Mulhearn, M Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nagy, E Nakano, I Napier, A Narain, M Nayyar, R Neal, HA Negret, JP Nett, J Neu, C Neustroev, P Nguyen, HT Nigmanov, T Nodulman, L Noh, SY Norniella, O Nunnemann, T Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Orduna, J Ortolan, L Osman, N Osta, J Pagliarone, C Pal, A Palencia, E Palni, P Papadimitriou, V Parashar, N Parihar, V Park, SK Parker, W Partridge, R Parua, N Patwa, A Pauletta, G Paulini, M Paus, C Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pleier, MA Podstavkov, VM Pondrom, L Popov, AV Poprocki, S Potamianos, K Pranko, A Prewitt, M Price, D Prokopenko, N Prokoshin, F Ptohos, F Punzi, G Qian, J Quadt, A Quinn, B Ranjan, N Ratoff, PN Razumov, I Fernandez, IR Renton, P Rescigno, M Rimondi, F Ripp-Baudot, I Ristori, L Rizatdinova, F Robson, A Rodriguez, T Rolli, S Rominsky, M Ronzani, M Roser, R Rosner, JL Ross, A Royon, C Rubinov, P Ruchti, R Ruffini, F Ruiz, A Russ, J Rusu, V Sajot, G Sakumoto, WK Sakurai, Y Sanchez-Hernandez, A Sanders, MP Santi, L Santos, AS Sato, K Savage, G Saveliev, V Savoy-Navarro, A Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schlabach, P Schmidt, EE Schwanenberger, C Schwarz, T Schwienhorst, R Scodellaro, L Scuri, F Seidel, S Seiya, Y Sekaric, J Semenov, A Severini, H Sforza, F Shabalina, E Shalhout, SZ Shary, V Shaw, S Shchukin, AA Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simak, V Simonenko, A Skubic, P Slattery, P Sliwa, K Smirnov, D Smith, JR Snider, FD Snow, GR Snow, J Snyder, S Soldner-Rembold, S Song, H Sonnenschein, L Sorin, V Soustruznik, K Denis, RS Stancari, M Stark, J Stentz, D Stoyanova, DA Strauss, M Strologas, J Sudo, Y Sukhanov, A Suslov, I Suter, L Svoisky, P Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Titov, M Toback, D Tokar, S Tokmenin, VV Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Tsai, YT Tsybychev, D Tuchming, B Tully, C Ukegawa, F Uozumi, S Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R Van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Vazquez, F Velev, G Vellidis, C Verkheev, AY Vernieri, C Vertogradov, LS Verzocchi, M Vesterinen, M Vidal, M Vilanova, D Vilar, R Vizan, J Vogel, M Vokac, P Volpi, G Wagner, P Wahl, HD Wallny, R Wang, MHLS Wang, SM Warchol, J Waters, D Watts, G Wayne, M Weichert, J Welty-Rieger, L Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Williams, MRJ Wilson, GW Wilson, JS Wilson, P Winer, BL Wittich, P Wobisch, M Wolbers, S Wolfe, H Wood, DR Wright, T Wu, X Wu, Z Wyatt, TR Xie, Y Yamada, R Yamamoto, K Yamato, D Yang, S Yang, T Yang, UK Yang, YC Yao, WM Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yeh, GP Yi, K Yin, H Yip, K Yoh, J Yorita, K Yoshida, T Youn, SW Yu, GB Yu, I Yu, JM Zanetti, AM Zeng, Y Zennamo, J Zhao, TG Zhou, B Zhou, C Zhu, J Zielinski, M Zieminska, D Zivkovic, L Zucchelli, S AF Aaltonen, T. 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Winer, B. L. Wittich, P. Wobisch, M. Wolbers, S. Wolfe, H. Wood, D. R. Wright, T. Wu, X. Wu, Z. Wyatt, T. R. Xie, Y. Yamada, R. Yamamoto, K. Yamato, D. Yang, S. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yeh, G. P. Yi, K. Yin, H. Yip, K. Yoh, J. Yorita, K. Yoshida, T. Youn, S. W. Yu, G. B. Yu, I. Yu, J. M. Zanetti, A. M. Zeng, Y. Zennamo, J. Zhao, T. G. Zhou, B. Zhou, C. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. Zucchelli, S. CA CDF Collaboration DO Collaboration TI Observation of s-Channel Production of Single Top Quarks at the Tevatron SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHANGING NEUTRAL CURRENTS; B-JET IDENTIFICATION; P(P)OVER-BAR COLLISIONS; FERMILAB-TEVATRON; ROOT-S=1.96 TEV; COUPLINGS; DETECTOR; SEARCH; FB(-1); DECAYS AB We report the first observation of single-top-quark production in the s channel through the combination of the CDF and D0 measurements of the cross section in proton-antiproton collisions at a center-of-mass energy of 1.96 TeV. The data correspond to total integrated luminosities of up to 9.7 fb(-1) per experiment. The measured cross section is sigma(s) = 1.29(-0.24)(+0.26) pb. The probability of observing a statistical fluctuation of the background to a cross section of the observed size or larger is 1.8 x 10(-10), corresponding to a significance of 6.3 standard deviations for the presence of an s-channel contribution to the production of single-top quarks. 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L.; Peters, Y.; Petridis, K.; Price, D.; Schwanenberger, C.; Soldner-Rembold, S.; Suter, L.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Adams, M.; Bazterra, V.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. 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RI Chiarelli, Giorgio/E-8953-2012; Punzi, Giovanni/J-4947-2012; Cavalli-Sforza, Matteo/H-7102-2015; Lokajicek, Milos/G-7800-2014; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Sharyy, Viatcheslav/F-9057-2014; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Merkin, Mikhail/D-6809-2012; Juste, Aurelio/I-2531-2015; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Li, Liang/O-1107-2015; Yip, Kin/D-6860-2013; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Lei, Xiaowen/O-4348-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Moon, Chang-Seong/J-3619-2014; Kozelov, Alexander/J-3812-2014; Scodellaro, Luca/K-9091-2014; Dudko, Lev/D-7127-2012 OI Chiarelli, Giorgio/0000-0001-9851-4816; Punzi, Giovanni/0000-0002-8346-9052; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Sharyy, Viatcheslav/0000-0002-7161-2616; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Qian, Jianming/0000-0003-4813-8167; Vidal Marono, Miguel/0000-0002-2590-5987; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Grohsjean, Alexander/0000-0003-0748-8494; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756; Chapon, Emilien/0000-0001-6968-9828; Melnychuk, Oleksandr/0000-0002-2089-8685; Juste, Aurelio/0000-0002-1558-3291; de Jong, Sijbrand/0000-0002-3120-3367; Latino, Giuseppe/0000-0002-4098-3502; iori, maurizio/0000-0002-6349-0380; Heinson, Ann/0000-0003-4209-6146; grannis, paul/0000-0003-4692-2142; Margaroli, Fabrizio/0000-0002-3869-0153; Casarsa, Massimo/0000-0002-1353-8964; Malik, Sudhir/0000-0002-6356-2655; Blazey, Gerald/0000-0002-7435-5758; Wahl, Horst/0000-0002-1345-0401; Group, Robert/0000-0002-4097-5254; Gershtein, Yuri/0000-0002-4871-5449; Bean, Alice/0000-0001-5967-8674; Simonenko, Alexander/0000-0001-6580-3638; Lancaster, Mark/0000-0002-8872-7292; Sawyer, Lee/0000-0001-8295-0605; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Li, Liang/0000-0001-6411-6107; Hedin, David/0000-0001-9984-215X; Blessing, Susan/0000-0002-4455-7279; Duperrin, Arnaud/0000-0002-5789-9825; Hoeneisen, Bruce/0000-0002-6059-4256; Yip, Kin/0000-0002-8576-4311; Beuselinck, Raymond/0000-0003-2613-7446; Toback, David/0000-0003-3457-4144; Jun, Soon Yung/0000-0003-3370-6109; Ding, Pengfei/0000-0002-4050-1753; Torre, Stefano/0000-0002-7565-0118; Bassler, Ursula/0000-0002-9041-3057; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; Bertram, Iain/0000-0003-4073-4941; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Lei, Xiaowen/0000-0002-2564-8351; Russ, James/0000-0001-9856-9155; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Dudko, Lev/0000-0002-4462-3192 FU U.S. DOE (U.S.); NSF (U.S.); ARC (Australia); CNPq (Brazil); FAPERJ (Brazil); FAPESP (Brazil); FUNDUNESP (Brazil); NSERC (Canada); NSC (China); CAS (China); CNSF (China); Colciencias (Colombia); MSMT (Czech Republic); GACR (Czech Republic); Academy of Finland (France); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); DAE (India); DST (India); SFI (Ireland); INFN (Italy); MEXT (Japan); Korean World Class University Program (Korea); NRF (Korea); CONACyT (Mexico); FOM (Netherlands); MON (Russia); NRC KI (Russia); RFBR (Russia); Slovak R&D Agency (Spain); Ministerio de Ciencia e Innovacion (Spain); Programa Consolider-Ingenio (Spain); Swedish Research Council (Sweden); SNSF (Switzerland); STFC (United Kingdom); Royal Society (United Kingdom); A. P. Sloan Foundation (U.S.); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and technical staffs of the participating institutions for their vital contributions. We acknowledge support from the U.S. DOE and NSF (U.S.), ARC (Australia), CNPq, FAPERJ, FAPESP, and FUNDUNESP (Brazil), NSERC (Canada), NSC, CAS, and CNSF (China), Colciencias (Colombia), MSMT and GACR (Czech Republic), the Academy of Finland, CEA and CNRS/IN2P3 (France), BMBF and DFG (Germany), DAE and DST (India), SFI (Ireland), INFN (Italy), MEXT (Japan), the Korean World Class University Program and NRF (Korea), CONACyT (Mexico), FOM (Netherlands), MON, NRC KI, and RFBR (Russia), the Slovak R&D Agency, the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010 (Spain), The Swedish Research Council (Sweden), SNSF (Switzerland), STFC and the Royal Society (United Kingdom), the A. P. Sloan Foundation (U.S.), and the EU community Marie Curie Fellowship Contract No. 302103. NR 59 TC 25 Z9 25 U1 2 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 9 PY 2014 VL 112 IS 23 AR 231803 DI 10.1103/PhysRevLett.112.231803 PG 11 WC Physics, Multidisciplinary SC Physics GA AI6JY UT WOS:000336981200004 PM 24972197 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Villella, I 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Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P De Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A De Cassagnac, RG Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P 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