FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Skinner, B Shklovskii, BI Voloshin, MB AF Skinner, Brian Shklovskii, B. I. Voloshin, M. B. TI Bound state energy of a Coulomb impurity in gapped bilayer graphene SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-STRUCTURE; FIELD; TRANSPORT; LAYERS AB Application of a perpendicular electric field induces a band gap in bilayer graphene, and it also creates a "Mexican hat" structure in the dispersion relation. This structure has unusual implications for the hydrogen-like bound state of an electron to a Coulomb impurity. We calculate the ground state energy of this hydrogen-like state as a function of the applied interlayer voltage and the effective fine structure constant. Unlike in the conventional hydrogen atom, the resulting wave function has many nodes even in the ground state. Further, the electron state undergoes "atomic collapse" into the Dirac continuum both at small and large voltage. C1 [Skinner, Brian; Shklovskii, B. I.; Voloshin, M. B.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Skinner, Brian; Shklovskii, B. I.; Voloshin, M. B.] Univ Minnesota, Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. [Skinner, Brian] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Voloshin, M. B.] Inst Theoret & Expt Phys, Moscow 117218, Russia. RP Skinner, B (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. OI Skinner, Brian/0000-0003-0774-3563 FU MRSEC Program of the National Science Foundation [DMR-0819885]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE [DE-FG02-94ER40823] FX We are grateful to V. Cheianov, A. V. Chaplik, V. Fal'ko, V. Gusynin, A. Kamenev, A. Luican-Mayer, K. A. Matveev, and A. F. Young for useful discussions. This work was supported primarily by the MRSEC Program of the National Science Foundation under Award No. DMR-0819885. Work at Argonne National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. M. B. V. is supported, in part, by DOE Grant No. DE-FG02-94ER40823. NR 44 TC 7 Z9 7 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 23 PY 2014 VL 89 IS 4 AR 041405 DI 10.1103/PhysRevB.89.041405 PG 4 WC Physics, Condensed Matter SC Physics GA AC1DH UT WOS:000332233900001 ER PT J AU Yao, YX Liu, J Wang, CZ Ho, KM AF Yao, Y. X. Liu, J. Wang, C. Z. Ho, K. M. TI Correlation matrix renormalization approximation for total-energy calculations of correlated electron systems SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; MEAN-FIELD THEORY; MOLECULAR-ORBITAL METHODS; DENSITY-FUNCTIONAL THEORY; WAVE-FUNCTIONS; INFINITE DIMENSIONS; TRANSITION-METALS; EXCHANGE-ENERGY; THERMOCHEMISTRY; ACCURATE AB We generalized the commonly used Gutzwiller approximation for calculating the electronic structure and total energy of strongly correlated electron systems. In our method, the evaluation of one-body and two-body density matrix elements of the Hamiltonian is simplified using a renormalization approximation to achieve better scaling of the computational effort as a function of system size. To achieve a clear presentation of the concept and methodology, we describe the detailed formalism for a finite hydrogen system with minimal basis set. We applied the correlation matrix renormalization approximation approach to a H-2 dimer and H-8 cubic fragment with minimal basis sets, as well as a H-2 molecule with a large basis set. The results compare favorably with sophisticated quantum chemical calculations. We believe our approach can serve as an alternative way to build up the exchange-correlation energy functional for an improved density functional theory description of systems with strong electron correlations. C1 [Yao, Y. X.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Yao, YX (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RI Liu, Jun/F-1240-2014 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We are grateful to T. K. Ng, J. Schmalian, G. Kotliar, N. Lanata, S. Trickey, and K. Ruedenberg for useful discussions. Research supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 56 TC 4 Z9 4 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 23 PY 2014 VL 89 IS 4 AR 045131 DI 10.1103/PhysRevB.89.045131 PG 11 WC Physics, Condensed Matter SC Physics GA AC1DH UT WOS:000332233900004 ER PT J AU Celis, A Cirigliano, V Passemar, E AF Celis, Alejandro Cirigliano, Vincenzo Passemar, Emilie TI Lepton flavor violation in the Higgs sector and the role of hadronic tau-lepton decays SO PHYSICAL REVIEW D LA English DT Article ID CHIRAL PERTURBATION-THEORY; VECTOR FORM-FACTOR; DISPERSIVE REPRESENTATION; KLOE DETECTOR; FIELD THEORY; ONE LOOP; MESON; SEARCH; PI(+)PI(-)); EQUATION AB It has been pointed out recently that current low-energy constraints still allow for sizable flavor-changing decay rates of the 125 GeV boson into leptons, h -> tau l (l = e, mu). In this work we discuss the role of hadronic tau-lepton decays in probing lepton flavor violating couplings in the Higgs sector. At low energy, the effective Higgs coupling to gluons induced by heavy quarks contributes to hadronic tau decays, establishing a direct connection with the relevant process at the LHC, pp(gg) -> h -> tau l. Semileptonic transitions like tau -> l pi pi are sensitive to flavor-changing scalar couplings, while decays such as tau -> l eta((l)) probe pseudoscalar couplings, thus providing a useful low-energy handle to disentangle possible Higgs flavor violating signals at the LHC. As part of our analysis, we provide an appropriate description of all the relevant hadronic matrix elements needed to describe Higgs mediated tau -> pi pi transitions, improving over previous treatments in the literature. C1 [Celis, Alejandro] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Cirigliano, Vincenzo; Passemar, Emilie] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Celis, A (reprint author), Univ Valencia, CSIC, IFIC, Apartat Correus 22085, E-46071 Valencia, Spain. OI Celis, Alejandro/0000-0002-3045-6696 FU Spanish Ministry MECD through the FPU [AP2010-0308]; DOE Office of Science; LDRD program at Los Alamos National Laboratory FX We are very grateful to Bachir Moussallam for illuminating discussions and for providing us with the solution of the Roy-Steiner equations needed as inputs to determine the scalar form factors. We also thank Gilberto Colangelo, Heinrich Leutwyler, Antonio Pich, and Jorge Portoles for useful discussions and comments. A. C. would like to thank LANL Theoretical Division for its generous hospitality while part of this work was being done. The work of A. C. is supported by the Spanish Ministry MECD through the FPU Grant No. AP2010-0308. The work of V. C. and E. P. is supported by the DOE Office of Science and the LDRD program at Los Alamos National Laboratory. NR 104 TC 36 Z9 37 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 23 PY 2014 VL 89 IS 1 AR 013008 DI 10.1103/PhysRevD.89.013008 PG 19 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB6AA UT WOS:000331868600001 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Balewski, J Banerjee, A Bamovska, Z Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HE Chen, JH Chen, L Cheng, J Chemey, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Corliss, R Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, E Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efmunov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Fatemi, R Fazio, S Fedorisin, J Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, E Gibson, A Girard, M Gliske, S Grosnick, D Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hajkova, O Hamed, A Han, LX Haque, R Harris, JW Hays-Wehle, JP Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Korsch, W Kotchenda, L Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Leight, W LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lima, LM Lisa, MA Liu, F Ljubicic, T Llope, WJ Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Munhoz, MG Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Oliveira, RAN Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Peterson, A Pile, P Planinic, M Pluta, J Plyku, D Poljak, N Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Pujahari, PR Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smimov, D Smimov, N Solanki, D Sorensen, P deSouza, UG Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Suaide, AAP Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM de Toledo, AS Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Tumau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, E Viyogi, YP Vokal, S Voloshin, SA Vossen, A Wada, M Walker, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YE Xiao, Z Xie, W Xin, K Xu, H Xu, N Xu, QH Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkameeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Balewski, J. Banerjee, A. Bamovska, Z. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bueltmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. de la Barca Sanchez, M. Calderon Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. E. Chen, J. H. Chen, L. Cheng, J. Chemey, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Corliss, R. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. de Souza, R. Derradi Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, E. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efmunov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, E. Gibson, A. Girard, M. Gliske, S. Grosnick, D. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hajkova, O. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Hays-Wehle, J. P. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Korsch, W. Kotchenda, L. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Leight, W. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lima, L. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Munhoz, M. G. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Oliveira, R. A. N. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Peterson, A. Pile, P. Planinic, M. Pluta, J. Plyku, D. Poljak, N. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smimov, D. Smimov, N. Solanki, D. Sorensen, P. deSouza, U. G. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Suaide, A. A. P. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szanto de Toledo, A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Tumau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, E. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Vossen, A. Wada, M. Walker, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. E. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, N. Xu, Q. H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkameeva, Y. Zyzak, M. CA STAR Collaboration TI Energy Dependence of Moments of Net-Proton Multiplicity Distributions at RHIC SO PHYSICAL REVIEW LETTERS LA English DT Article ID QUARK-GLUON PLASMA; QCD PHASE-DIAGRAM; QUANTUM CHROMODYNAMICS; CRITICAL-POINT; COLLISIONS; TRANSITION; FLUCTUATIONS; MODEL; COLLABORATION; PERSPECTIVE AB We report the beam energy (root S-NN = 7.7-200 GeV) and collision centrality dependence of the mean (M), standard deviation (sigma), skewness (S), and kurtosis (kappa) of the net-proton multiplicity distributions in Au + Au collisions. The measurements are carried out by the STAR experiment at midrapidity (vertical bar y vertical bar < 0.5) and within the transverse momentum range 0.4 < p(T) < 0.8 GeV/c in the first phase of the Beam Energy Scan program at the Relativistic Heavy Ion Collider. These measurements are important for understanding the quantum chromodynamic phase diagram. The products of the moments, S sigma and K sigma(2), are sensitive to the correlation length of the hot and dense medium created in the collisions and are related to the ratios of baryon number susceptibilities of corresponding orders. The products of moments are found to have values significantly below the Skellam expectation and close to expectations based on independent proton and antiproton production. The measurements are compared to a transport model calculation to understand the effect of acceptance and baryon number conservation and also to a hadron resonance gas model. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, Krakow, Poland. [Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smimov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, E.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Brovko, S. G.; de la Barca Sanchez, M. Calderon; Cebra, D.; Ding, E.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [de Souza, R. Derradi; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil. [Chen, L.; Huck, P.; Ke, H. W.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. E.; Yang, Y.; Zhang, J. B.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Chwastowski, J.; Kycia, R. A.] Cracow Univ Technol, Krakow, Poland. [Chemey, M.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Hajkova, O.; Pachr, M.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Bamovska, Z.; Bielcikova, J.; Rusnak, J.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] FIAS, Frankfurt, Germany. [Das, S.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Mumbai 400076, Maharashtra, India. [Dhamija, S.; Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efmunov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkameeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Keane, D.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.; Vanfossen, J. A., Jr.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Korsch, W.; Ramachandran, S.; Webb, G.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Taejon, South Korea. [Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou, Peoples R China. [Dong, X.; Eun, L.; Masui, H.; Matis, H. S.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Xu, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Balewski, J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Stevens, J. R.; van Nieuwenhuizen, G.; Walker, M.] MIT, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. 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[Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, E.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Lima, L. M.; Munhoz, M. G.; Oliveira, R. A. N.; deSouza, U. G.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, Sao Paulo, Brazil. [Chen, H. E.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zawisza, Y.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, Nantes, France. [Li, X.; Surrow, B.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. 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[Girard, M.; Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Sandacz, A.; Trzeciak, B. A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smimov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Mohanty, B (reprint author), Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. EM bedanga@niser.ac.in RI Derradi de Souza, Rafael/M-4791-2013; Suaide, Alexandre/L-6239-2016; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Yip, Kin/D-6860-2013; Huang, Bingchu/H-6343-2015; Fazio, Salvatore /G-5156-2010; Lednicky, Richard/K-4164-2013; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Takahashi, Jun/B-2946-2012; Alekseev, Igor/J-8070-2014; Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; XIAO, Zhigang/C-3788-2015; Aparecido Negrao de Oliveira, Renato/G-9133-2015; Kycia, Radoslaw/J-4397-2015; Chaloupka, Petr/E-5965-2012 OI Derradi de Souza, Rafael/0000-0002-2084-7001; Suaide, Alexandre/0000-0003-2847-6556; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Fisyak, Yuri/0000-0002-3151-8377; Bhasin, Anju/0000-0002-3687-8179; Yip, Kin/0000-0002-8576-4311; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536; Huang, Bingchu/0000-0002-3253-3210; Takahashi, Jun/0000-0002-4091-1779; Alekseev, Igor/0000-0003-3358-9635; Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Kycia, Radoslaw/0000-0002-6390-4627; FU Office of NP U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of the Government of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia; Renaissance Technologies Corporation; DST Swarna Jayanti Fellowship; Office of HEP within the U.S. DOE Office of Science FX We thank M. Asakawa, R. Gavai, S. Gupta, F. Karsch, K. Rajagopal, K. Redlich, and M. A. Stephanov for discussions related to this work. We thank the RHIC Operations Group and RCF at BNL, and the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST, and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of the Government of India, National Science Centre of Poland, National Research Foundation (NRF-2012004024), Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. Finally, we gratefully acknowledge a sponsored research grant for the 2006 run period from Renaissance Technologies Corporation. BM is supported by DST Swarna Jayanti Fellowship. NR 46 TC 119 Z9 120 U1 4 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 23 PY 2014 VL 112 IS 3 AR 032302 DI 10.1103/PhysRevLett.112.032302 PG 7 WC Physics, Multidisciplinary SC Physics GA AB7BK UT WOS:000331944100006 PM 24484135 ER PT J AU Belous, K Shapkin, M Sokolov, A Adachi, I Aihara, H Asner, DM Aulchenko, V Bakich, AM Bala, A Bhuyan, B Bobrov, A Bondar, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dolezal, Z Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Ferber, T Gaur, V Ganguly, S Garmash, A Gillard, R Goh, YM Golob, B Haba, J Hara, T Hayasaka, K Hayashii, H Hoshi, Y Hou, WS Iijima, T Inami, K Ishikawa, A Itoh, R Iwashita, T Jaegle, I Julius, T Kato, E Kichimi, H Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, MJ Kim, YJ Kinoshita, K Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kuzmin, A Kwon, YJ Lange, JS Lee, SH Libby, J Liventsev, D Lukin, P Matvienko, D Miyata, H Mizuk, R Mohanty, GB Mori, T Mussa, R Nagasaka, Y Nakano, E Nakao, M Nayak, M Nedelkovska, E Ng, C Nisar, NK Nishida, S Nitoh, O Ogawa, S Okuno, S Olsen, SL Ostrowicz, W Pakhlova, G Park, CW Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Ryu, S Sahoo, H Saito, T Sakai, Y Sandilya, S Santel, D Santelj, L Sanuki, T Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Seon, O Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Stanic, S Staric, M Steder, M Sumiyoshi, T Tamponi, U Tatishvili, G Teramoto, Y Trabelsi, K Tsuboyama, T Uchida, M Uehara, S Uglov, T Unno, Y Uno, S Usov, Y Vahsen, SE Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, P Watanabe, M Watanabe, Y Williams, KM Won, E Yamaoka, J Yamashita, Y Yashchenko, S Yook, Y Yuan, CZ Zhang, ZP Zhilich, V Zupanc, A AF Belous, K. Shapkin, M. Sokolov, A. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Bakich, A. M. Bala, A. Bhuyan, B. Bobrov, A. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dolezal, Z. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Ferber, T. Gaur, V. Ganguly, S. Garmash, A. Gillard, R. Goh, Y. M. Golob, B. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. Hoshi, Y. Hou, W. -S. Iijima, T. Inami, K. Ishikawa, A. Itoh, R. Iwashita, T. Jaegle, I. Julius, T. Kato, E. Kichimi, H. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, M. J. Kim, Y. J. Kinoshita, K. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, S. -H. Libby, J. Liventsev, D. Lukin, P. Matvienko, D. Miyata, H. Mizuk, R. Mohanty, G. B. Mori, T. Mussa, R. Nagasaka, Y. Nakano, E. Nakao, M. Nayak, M. Nedelkovska, E. Ng, C. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Olsen, S. L. Ostrowicz, W. Pakhlova, G. Park, C. W. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Ryu, S. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Santel, D. Santelj, L. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Seon, O. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y-S. Stanic, S. Staric, M. Steder, M. Sumiyoshi, T. Tamponi, U. Tatishvili, G. Teramoto, Y. Trabelsi, K. Tsuboyama, T. Uchida, M. Uehara, S. Uglov, T. Unno, Y. Uno, S. Usov, Y. Vahsen, S. E. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, P. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yamaoka, J. Yamashita, Y. Yashchenko, S. Yook, Y. Yuan, C. Z. Zhang, Z. P. Zhilich, V. Zupanc, A. CA Belle Collaboration TI Measurement of the tau-lepton Lifetime at Belle SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-LEPTONS; COLLISIONS; DETECTOR AB The lifetime of the tau lepton is measured using the process e(+) e(-) -> tau(+) tau(-), where both tau leptons decay to 3 pi nu(tau). The result for the mean lifetime, based on 711 fb(-1) of data collected with the Belle detector at the Upsilon(4S) resonance and 60 MeV below, is tau = (290.17 +/- 0.53(stat) +/- 0.33(syst)) x 10(-15) s. The first measurement of the lifetime difference between tau(+) and tau(-) is performed. The upper limit on the relative lifetime difference between positive and negative tau leptons is vertical bar Delta tau vertical bar/tau < 7.0 x 10(-3) at 90% C.L. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Aulchenko, V.; Bobrov, A.; Bondar, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Aulchenko, V.; Bobrov, A.; Bondar, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Kinoshita, K.; Santel, D.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Vahsen, S. E.; Varner, G.; Yamaoka, J.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Kichimi, H.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Tsuboyama, T.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Hiroshima 7315193, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Belous, K.; Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Chilikin, K.; Chistov, R.; Mizuk, R.; Pakhlova, G.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Kuhr, T.; Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kim, H. J.; Kim, M. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Nedelkovska, E.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Mizuk, R.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Inami, K.; Mori, T.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Iwashita, T.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Ostrowicz, W.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Miyata, H.; Watanabe, M.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Olsen, S. L.; Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.; Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Epifanov, D.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Tokyo 1848588, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y-S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Belous, K (reprint author), Inst High Energy Phys, Protvino 142281, Russia. RI Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Uglov, Timofey/B-2406-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Pakhlova, Galina/C-5378-2014; Cervenkov, Daniel/D-2884-2017; OI Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Cervenkov, Daniel/0000-0002-1865-741X; Yuan, Chang-Zheng/0000-0002-1652-6686 FU MEXT (Japan); JSPS (Japan); Nagoya's TLPRC (Japan); ARC (Australia); DIISR (Australia); FWF (Austria); NSFC (China); MSMT (Czechia); CZF (Germany); DFG (Germany); VS (Germany); DST (India); INFN (Italy); MEST (Korea); WCU (Korea); MNiSW (Poland); NCN (Poland); MES (Russia); RFAAE (Russia); ARRS (Slovenia); IKERBASQUE (Spain); UPV/EHU (Spain); SNSF (Switzerland); NSC (Taiwan); MOE (Taiwan); U.S. DOE (U.S.); NSF (U.S.); NRF (Korea); GSDC of KISTI (Korea) FX We thank the KEKB group for excellent operation of the accelerator, the KEK cryogenics group for efficient solenoid operations, and the KEK computer group, the NII, and PNNL/EMSL for valuable computing and SINET4 network support. We acknowledge support from MEXT, JSPS, and Nagoya's TLPRC (Japan): ARC and DIISR (Australia); FWF (Austria); NSFC (China); MSMT (Czechia); CZF, DFG, and VS (Germany); DST (India); INFN (Italy); MEST, NRF, GSDC of KISTI, and WCU (Korea); MNiSW and NCN (Poland); MES and RFAAE (Russia); ARRS (Slovenia); IKERBASQUE and UPV/EHU (Spain); SNSF (Switzerland); NSC and MOE (Taiwan); and U.S. DOE and NSF (U.S.). NR 21 TC 13 Z9 13 U1 1 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 23 PY 2014 VL 112 IS 3 AR 031801 DI 10.1103/PhysRevLett.112.031801 PG 6 WC Physics, Multidisciplinary SC Physics GA AB7BK UT WOS:000331944100005 PM 24484129 ER PT J AU Cheney, CP Vilmercati, P Martin, EW Chiodi, M Gavioli, L Regmi, M Eres, G Callcott, TA Weitering, HH Mannella, N AF Cheney, C. Parks Vilmercati, P. Martin, E. W. Chiodi, M. Gavioli, L. Regmi, M. Eres, G. Callcott, T. A. Weitering, H. H. Mannella, N. TI Origins of Electronic Band Gap Reduction in Cr/N Codoped TiO2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY-ABSORPTION; RESONANT PHOTOEMISSION; CHARGE-TRANSFER; VISIBLE-LIGHT; THIN-FILMS; SPECTROSCOPY; SURFACE; OXIDATION; RUTILE; OXIDE AB Recent studies indicated that noncompensated cation-anion codoping of wide-band-gap oxide semiconductors such as anatase TiO2 significantly reduces the optical band gap and thus strongly enhances the absorption of visible light [W. Zhu et al., Phys. Rev. Lett. 103, 226401 (2009)]. We used soft x-ray spectroscopy to fully determine the location and nature of the impurity levels responsible for the extraordinarily large (similar to 1 eV) band gap reduction of noncompensated codoped rutile TiO2. It is shown that Cr/N codoping strongly enhances the substitutional N content, compared to single element doping. The band gap reduction is due to the formation of Cr 3d(3) levels in the lower half of the gap while the conduction band minimum is comprised of localized Cr 3d and delocalized N 2p states. Band gap reduction and carrier delocalization are critical elements for efficient light-to-current conversion in oxide semiconductors. These findings thus raise the prospect of using codoped oxide semiconductors with specifically engineered electronic properties in a variety of photovoltaic and photocatalytic applications. C1 [Cheney, C. Parks; Vilmercati, P.; Martin, E. W.; Callcott, T. A.; Weitering, H. H.; Mannella, N.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Chiodi, M.; Gavioli, L.] Univ Cattolica Sacro Cuore, Dipartimento Matemat & Fis, I-25121 Brescia, Italy. [Chiodi, M.; Gavioli, L.] Univ Cattolica Sacro Cuore, Interdisciplinary Labs Adv Mat Phys, I-25121 Brescia, Italy. [Regmi, M.; Eres, G.; Weitering, H. H.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Cheney, CP (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM hanno@utk.edu; nmannell@utk.edu RI Gavioli, Luca/G-5268-2010; Chiodi, Mirco/E-4160-2016; Eres, Gyula/C-4656-2017; Vilmercati, Paolo/E-5655-2017 OI Gavioli, Luca/0000-0003-2782-7414; Chiodi, Mirco/0000-0003-0418-0785; Eres, Gyula/0000-0003-2690-5214; Vilmercati, Paolo/0000-0002-3872-8828 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; National Science Foundation [DMR-1151687] FX We thank Professor Z. Y. Zhang and Professor W. G. Zhu for stimulating discussions. This research was partially supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (H. H. W., G. E., and M. R.), and the National Science Foundation Grant No. DMR-1151687 (N.M.). NR 36 TC 20 Z9 20 U1 4 U2 80 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 23 PY 2014 VL 112 IS 3 AR 036404 DI 10.1103/PhysRevLett.112.036404 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7BK UT WOS:000331944100015 ER PT J AU Emma, P Venturini, M Bane, KLF Stupakov, G Kang, HS Chae, MS Hong, J Min, CK Yang, H Ha, T Lee, WW Park, CD Park, SJ Ko, IS AF Emma, P. Venturini, M. Bane, K. L. F. Stupakov, G. Kang, H. -S. Chae, M. S. Hong, J. Min, C. -K. Yang, H. Ha, T. Lee, W. W. Park, C. D. Park, S. J. Ko, I. S. TI Experimental Demonstration of Energy-Chirp Control in Relativistic Electron Bunches Using a Corrugated Pipe SO PHYSICAL REVIEW LETTERS LA English DT Article AB The first experimental study is presented of a corrugated wall device that uses wakefields to remove a linear energy correlation in a relativistic electron beam (a "dechirper"). Time-resolved measurements of both longitudinal and transverse wakefields of the device are presented and compared with simulations. This study demonstrates the feasibility to employ a dechirper for precise control of the beam phase space in the next generation of free-electron-lasers. C1 [Emma, P.; Venturini, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bane, K. L. F.; Stupakov, G.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Kang, H. -S.; Chae, M. S.; Hong, J.; Min, C. -K.; Yang, H.; Ha, T.; Lee, W. W.; Park, C. D.; Park, S. J.; Ko, I. S.] Pohang Accelerator Lab, Pohang 790784, South Korea. RP Emma, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM Emma@SLAC.Stanford.edu FU U.S. Department of Energy [DE-AC02-76SF00515, DE-AC02-05CH11231] FX Work supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-76SF00515 and No. DE-AC02-05CH11231. NR 13 TC 24 Z9 24 U1 3 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 23 PY 2014 VL 112 IS 3 AR 034801 DI 10.1103/PhysRevLett.112.034801 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7BK UT WOS:000331944100010 PM 24484143 ER PT J AU Ryu, C Henderson, KC Boshier, MG AF Ryu, C. Henderson, K. C. Boshier, M. G. TI Creation of matter wave Bessel beams and observation of quantized circulation in a Bose-Einstein condensate SO NEW JOURNAL OF PHYSICS LA English DT Article ID ORBITAL ANGULAR-MOMENTUM; ELECTRON VORTEX BEAMS; ATOMIC-BEAM; LIGHT-BEAM; SOLITONS; MANIPULATION; DIFFRACTION AB Bessel beams are plane waves with amplitude profiles described by Bessel functions. They are important because they propagate 'diffraction-free' and because they can carry orbital angular momentum. Here we report the creation of a Bessel beam of de Broglie matter waves. The Bessel beam is produced by the free evolution of a thin toroidal atomic Bose-Einstein condensate (BEC) which has been set into rotational motion. By attempting to stir it at different rotation rates, we show that the toroidal BEC can only be made to rotate at discrete, equally spaced frequencies, demonstrating that circulation is quantized in atomic BECs. The method used here can be viewed as a form of wavefunction engineering which might be developed to implement cold atom matter wave holography. C1 [Ryu, C.; Henderson, K. C.; Boshier, M. G.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. RP Boshier, MG (reprint author), Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. EM boshier@lanl.gov RI Boshier, Malcolm/A-2128-2017 OI Boshier, Malcolm/0000-0003-0769-1927 FU US Department of Energy through the LANL/LDRD Program FX This work was supported by the US Department of Energy through the LANL/LDRD Program. We acknowledge inspiring conversations with Eddy Timmermans. NR 31 TC 21 Z9 21 U1 0 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 23 PY 2014 VL 16 AR 013046 DI 10.1088/1367-2630/16/1/013046 PG 12 WC Physics, Multidisciplinary SC Physics GA 302SR UT WOS:000330625700007 ER PT J AU Huang, H Zeqiraj, E Dong, BH Jha, BK Duffy, NM Orlicky, S Thevakumaran, N Talukdar, M Pillon, MC Ceccarelli, DF Wan, LCK Juang, YC Mao, DYL Gaughan, C Brinton, MA Perelygin, AA Kourinov, I Guarne, A Silverman, RH Sicheri, F AF Huang, Hao Zeqiraj, Elton Dong, Beihua Jha, Babal Kant Duffy, Nicole M. Orlicky, Stephen Thevakumaran, Neroshan Talukdar, Manisha Pillon, Monica C. Ceccarelli, Derek F. Wan, Leo C. K. Juang, Yu-Chi Mao, Daniel Y. L. Gaughan, Christina Brinton, Margo A. Perelygin, Andrey A. Kourinov, Igor Guarne, Alba Silverman, Robert H. Sicheri, Frank TI Dimeric Structure of Pseudokinase RNase L Bound to 2-5A Reveals a Basis for Interferon-Induced Antiviral Activity SO MOLECULAR CELL LA English DT Article ID UNFOLDED PROTEIN RESPONSE; 2-5A-DEPENDENT RNASE; RIBONUCLEASE-L; ENCEPHALOMYOCARDITIS VIRUS; ENDOPLASMIC-RETICULUM; PROSTATE-CANCER; INNATE IMMUNITY; KINASE; APOPTOSIS; CELLS AB RNase L is an ankyrin repeat domain-containing dual endoribonuclease-pseudokinase that is activated by unusual 2,'5'-oligoadenylate (2-5A) second messengers and which impedes viral infections in higher vertebrates. Despite its importance in interferon-regulated antiviral innate immunity, relatively little is known about its precise mechanism of action. Here we present a functional characterization of 2.5 angstrom and 3.25 angstrom X-ray crystal and small-angle X-ray scattering structures of RNase L bound to a natural 2-5A activator with and without ADP or the non-hydrolysable ATP mimetic AMP-PNP. These studies reveal how recognition of 2-5A through interactions with the ankyrin repeat domain and the pseudokinase domain, together with nucleotide binding, imposes a rigid intertwined dimer configuration that is essential for RNase catalytic and antiviral functions. The involvement of the pseudokinase domain of RNase L in 2-5A sensing, nucleotide binding, dimerization, and ribonuclease functions highlights the evolutionary adaptability of the eukaryotic protein kinase fold. C1 [Huang, Hao; Zeqiraj, Elton; Duffy, Nicole M.; Orlicky, Stephen; Thevakumaran, Neroshan; Talukdar, Manisha; Ceccarelli, Derek F.; Wan, Leo C. K.; Juang, Yu-Chi; Mao, Daniel Y. L.; Sicheri, Frank] Mt Sinai Hosp, Lunenfeld Tanenbaum Res Inst, Program Syst Biol, Toronto, ON M5G 1X5, Canada. [Huang, Hao; Talukdar, Manisha; Wan, Leo C. K.; Sicheri, Frank] Univ Toronto, Dept Mol Genet, Toronto, ON M5S 1A8, Canada. [Zeqiraj, Elton; Thevakumaran, Neroshan; Sicheri, Frank] Univ Toronto, Dept Biochem, Toronto, ON M5S 1A8, Canada. [Dong, Beihua; Jha, Babal Kant; Gaughan, Christina; Silverman, Robert H.] Cleveland Clin, Lerner Res Inst, Dept Canc Biol, Cleveland, OH 44195 USA. [Pillon, Monica C.; Guarne, Alba] McMaster Univ, Dept Biochem & Biomed Sci, Hamilton, ON L8S 4K1, Canada. [Mao, Daniel Y. L.] Ryerson Univ, Dept Chem & Biol, Toronto, ON M5B 2K3, Canada. [Brinton, Margo A.; Perelygin, Andrey A.] Georgia State Univ, Dept Biol, Atlanta, GA 30302 USA. [Kourinov, Igor] Argonne Natl Lab, NE CAT APS, Argonne, IL 60439 USA. RP Silverman, RH (reprint author), Cleveland Clin, Lerner Res Inst, Dept Canc Biol, Cleveland, OH 44195 USA. EM silverr@ccf.org; sicheri@lunenfeld.ca RI Sicheri, Frank/F-8856-2013; OI Jha, Babal/0000-0002-7660-5255; Zeqiraj, Elton/0000-0003-0239-5926 FU National Institute of General Medical Sciences from the National Institutes of Health [P41 GM103403]; U.S. DOE [DE-AC02-06CH11357]; Canadian Institutes of Health Research [MOP-84370]; Canada Research Chair in Structural Biology; National Institutes of Health (NIH) [CA044059]; Centers for Disease Control and Prevention; NIH [AI045135] FX Diffraction experiments performed at the Advanced Photon Source on the Northeastern Collaborative Access Team beamlines were supported by a grant from the National Institute of General Medical Sciences (P41 GM103403) from the National Institutes of Health and by the U.S. DOE under contract number DE-AC02-06CH11357. We thank Dr. Gabor Bunkoczi, a lecturer at the CCP4/APS school on Macromolecular Crystallography, for assistance with the RNase L structure determination. This work was supported by a grant to F.S. from the Canadian Institutes of Health Research (MOP-84370), by a Canada Research Chair in Structural Biology to F.S., by a grant to R.H.S. from the National Institutes of Health (NIH) (grant number CA044059), by a grant to M.A.B. and A.A.P. from the Centers for Disease Control and Prevention, and by NIH grant number AI045135 to M.A.B. NR 49 TC 31 Z9 31 U1 4 U2 13 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD JAN 23 PY 2014 VL 53 IS 2 BP 221 EP 234 DI 10.1016/j.molcel.2013.12.025 PG 14 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 300XD UT WOS:000330496400006 PM 24462203 ER PT J AU Singh, S Plaks, JG Homa, NJ Amrich, CG Heroux, A Hatfull, GF VanDemark, AP AF Singh, Shweta Plaks, Joseph G. Homa, Nicholas J. Amrich, Christopher G. Heroux, Annie Hatfull, Graham F. VanDemark, Andrew P. TI The Structure of Xis Reveals the Basis for Filament Formation and Insight into DNA Bending within a Mycobacteriophage Intasome SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE DNA recombination; mycobacteriophage; DNA bending; structure; Xis ID SITE-SPECIFIC RECOMBINATION; INTEGRATION HOST FACTOR; BACTERIOPHAGE-LAMBDA; PHAGE-LAMBDA; CRYSTAL-STRUCTURE; ATTACHMENT SITE; PROTEIN; EXCISIONASE; L5; COMPLEX AB The recombination directionality factor, Xis, is a DNA bending protein that determines the outcome of integrase-mediated site-specific recombination by redesign of higher-order protein-DNA architectures. Although the attachment site DNA of mycobacteriophage Pukovnik is likely to contain four sites for Xis binding, Xis crystals contain five subunits in the asymmetric unit, four of which align into a Xis filament and a fifth that is generated by an unusual domain swap. Extensive intersubunit contacts stabilize a bent filament-like arrangement with Xis monomers aligned head to tail. The structure implies a DNA bend of similar to 120 degrees, which is in agreement with DNA bending measured in vitro. Formation of attR-containing intasomes requires only Int and Xis, distinguishing Pukovnik from lambda. Therefore, we conclude that, in Pukovnik, Xis-induced DNA bending is sufficient to promote intramolecular Int-mediated bridges during intasome formation. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Singh, Shweta; Plaks, Joseph G.; Homa, Nicholas J.; Amrich, Christopher G.; Hatfull, Graham F.; VanDemark, Andrew P.] Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. [Heroux, Annie] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP VanDemark, AP (reprint author), Univ Pittsburgh, Dept Biol Sci, 4249 5th Ave,360A Langley Hall, Pittsburgh, PA 15260 USA. EM andyv@pitt.edu FU National Institutes of Health [AI59114]; Science Education Grant from the Howard Hughes Medical Institutes to the University of Pittsburgh FX We thank M. Schmidt and J. Sacchettini for sharing resources and helpful advice. This work was supported by National Institutes of Health grant AI59114 to G.F.H and A.P.V. were supported by a Science Education Grant from the Howard Hughes Medical Institutes to the University of Pittsburgh. NR 43 TC 7 Z9 7 U1 0 U2 3 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD JAN 23 PY 2014 VL 426 IS 2 BP 412 EP 422 DI 10.1016/j.jmb.2013.10.002 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 295WW UT WOS:000330148100013 PM 24112940 ER PT J AU Shaya, D Findeisen, F Abderemane-Ali, F Arrigoni, C Wong, S Nurva, SR Loussouarn, G Minor, DL AF Shaya, David Findeisen, Felix Abderemane-Ali, Fayal Arrigoni, Cristina Wong, Stephanie Nurva, Shailika Reddy Loussouarn, Gildas Minor, Daniel L., Jr. TI Structure of a Prokaryotic Sodium Channel Pore Reveals Essential Gating Elements and an Outer Ion Binding Site Common to Eukaryotic Channels SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE voltage-gated sodium channel; X-ray crystallography; electrophysiology; ion binding; voltage-gated calcium channel ID DEPENDENT K+ CHANNEL; CRYSTAL-STRUCTURE; CALCIUM-CHANNEL; POTASSIUM CHANNELS; PROVIDES INSIGHT; PERMEATION; SELECTIVITY; INACTIVATION; NACHBAC; MECHANISMS AB Voltage-gated sodium channels (Nays) are central elements of cellular excitation. Notwithstanding advances from recent bacterial Na-v (BacNa(v)) structures, key questions about gating and ion selectivity remain. Here, we present a closed conformation of Na(v)Ae1p, a pore-only BacNav derived from Na(v)Ae1, a BacNa(v) from the arsenite oxidizer Alkalilimnicola ehrlichei found in Mono Lake, California, that provides insight into both fundamental properties. The structure reveals a pore domain in which the pore-lining S6 helix connects to a helical cytoplasmic tail. Electrophysiological studies of full-length BacNa(v)s show that two elements defined by the NavAe1p structure, an S6 activation gate position and the cytoplasmic tail "neck", are central to BacNav gating. The structure also reveals the selectivity filter ion entry site, termed the "outer ion" site. Comparison with mammalian voltage-gated calcium channel (Ca-v) selectivity filters, together with functional studies, shows that this site forms a previously unknown determinant of Cav high-affinity calcium binding. Our findings underscore commonalities between BacNavs and eukaryotic voltage-gated channels and provide a framework for understanding gating and ion permeation in this superfamily. (C) 2013 The Authors. Published by Elsevier Ltd. All rights reserved. C1 [Shaya, David; Findeisen, Felix; Arrigoni, Cristina; Wong, Stephanie; Nurva, Shailika Reddy; Minor, Daniel L., Jr.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA. [Abderemane-Ali, Fayal; Loussouarn, Gildas] Inst Natl Sante & Rech Med, UMR 1087, F-44000 Nantes, France. [Abderemane-Ali, Fayal; Loussouarn, Gildas] CNRS, UMR 6291, F-44000 Nantes, France. [Abderemane-Ali, Fayal; Loussouarn, Gildas] Univ Nantes, LUNAM, Inst Thorax, F-44000 Nantes, France. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Sci Div, Berkeley, CA 94720 USA. RP Minor, DL (reprint author), Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA. EM daniel.minor@ucsf.edu RI Loussouarn, Gildas/D-3590-2015 FU National Institutes of Health [R01-HL080050, R01-D0007664, U54-GM094625]; American Heart Association [0740019N]; American Heart Association Postdoctoral Fellowship; Fulbright Scholarship and a Monahan Foundation Fellowship; Marie Curie International Outgoing Fellowship; 7th European Community Framework Programme FX We thank Christine Rumpf and Ahmed Rohaim for expert molecular biology assistance and J. Holton and G. Meigs at Advanced Light Source Beamline 8.3.1 for data collection assistance. We thank K. Brejc, L. Jan, and E. Reuveny for helpful manuscript comments and Minor laboratory members for support throughout these studies. This work was supported by National Institutes of Health grants R01-HL080050, R01-D0007664, and U54-GM094625 and the American Heart Association grant 0740019N to D.L.M.; an American Heart Association Postdoctoral Fellowship to D.S.; and Fulbright Scholarship and a Monahan Foundation Fellowship to F.A.-A. G.L. was supported by a Marie Curie International Outgoing Fellowship within the 7th European Community Framework Programme. D.L.M. is an American Heart Association Established Investigator. NR 66 TC 47 Z9 47 U1 7 U2 27 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD JAN 23 PY 2014 VL 426 IS 2 BP 467 EP 483 DI 10.1016/j.jmb.2013.10.010 PG 17 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 295WW UT WOS:000330148100018 PM 24120938 ER PT J AU Datta, AB Hura, GL Wolberger, C AF Datta, Ajit B. Hura, Greg L. Wolberger, Cynthia TI The Structure and Conformation of Lys63-Linked Tetraubiquitin (vol 392, pg 1117, 2009) SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Correction C1 [Datta, Ajit B.; Wolberger, Cynthia] Johns Hopkins Univ, Dept Biophys & Biophys Chem, Sch Med, Baltimore, MD 21205 USA. [Datta, Ajit B.; Wolberger, Cynthia] Johns Hopkins Univ, Howard Hughes Med Inst, Sch Med, Baltimore, MD 21205 USA. [Hura, Greg L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Wolberger, C (reprint author), Johns Hopkins Univ, Dept Biophys & Biophys Chem, Sch Med, Baltimore, MD 21205 USA. NR 1 TC 0 Z9 0 U1 0 U2 2 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD JAN 23 PY 2014 VL 426 IS 2 BP 499 EP 499 DI 10.1016/j.jmb.2013.11.003 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 295WW UT WOS:000330148100020 ER PT J AU Kryvohuz, M AF Kryvohuz, Maksym TI Calculation of Kinetic Isotope Effects for Intramolecular Hydrogen Shift Reactions Using Semiclassical Instanton Approach SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE THEORY; THERMAL RATE CONSTANTS; SIGMATROPIC REARRANGEMENT; POLYATOMIC-MOLECULES; ENZYME CATALYSIS; ATOM TRANSFER; QUANTUM; DYNAMICS; SYSTEMS; FORMULATION AB Primary HID kinetic isotope effects for the [1,5] hydrogen shift reaction in 13-atomic 1,3-pentadiene and [1,7] hydrogen shift reaction in 23-atomic 7-methylocta-1,3,5-triene are calculated using the semiclassical instanton approach. All 33 and 63 internal degrees of freedom, respectively, are treated quantum mechanically with multidimensional tunneling automatically accounted for by the instanton approach. Reactive potential energy surfaces are calculated on-the-fly using mPW1K/6-31+G(d,p) and mPWB1K/6-31+G(d,p) electronic structure methods. The calculated kinetic isotope effects agree well with the previously reported experimental measurements. The analytical expressions of the semiclassical instanton approach allow one to determine quantitative contributions of various physical mechanisms to the calculated kinetic isotope effects. Multidimensional tunneling is found to play important role in both studied hydrogen shift reactions. C1 [Kryvohuz, Maksym] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Kryvohuz, M (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mkryvohuz@anl.gov FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of the Director, Argonne National Laboratory FX I would like to acknowledge the support of this research by a Director's Postdoctoral Fellowship, Office of the Director, Argonne National Laboratory, and Dr. Julius Jellinek for helpful discussions and support. I acknowledge Dr. John D. Thobum for providing the numerical CVT data on KIE in pentadiene. I also acknowledge Dr. Juan M. Lopez-Encarnacion for fruitful discussions on electronic structure methods. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 65 TC 11 Z9 11 U1 2 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 23 PY 2014 VL 118 IS 3 BP 535 EP 544 DI 10.1021/jp4099073 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 297JZ UT WOS:000330253000001 PM 24387202 ER PT J AU Griffin, PJ Holt, AP Wang, YY Novikov, VN Sangoro, JR Kremer, F Sokolov, AP AF Griffin, Philip J. Holt, Adam P. Wang, Yangyang Novikov, Vladimir N. Sangoro, Joshua R. Kremer, Friedrich Sokolov, Alexei P. TI Interplay Between Hydrophobic Aggregation and Charge Transport in the Ionic Liquid Methyltrioctylammonium Bis(trifluoromethylsulfonyl)imide SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID QUATERNARY AMMONIUM ION; SIDE-CHAIN POLYMERS; X-RAY-SCATTERING; NANOPHASE SEPARATION; DISORDERED SOLIDS; GLASS-TRANSITION; AC CONDUCTION; DYNAMICS; SEGREGATION; RELAXATIONS AB In order to understand the nature of the exceedingly low ionic conductivity of aprotic ammonium ionic liquids (ILs), we have measured the charge transport and structural dynamics of methyltrioctylammonium bis(trifluoromethylsulfonyl)imide [m3oa][ntf2] over a broad temperature range using broadband dielectric spectroscopy, depolarized dynamic light scattering (DDLS), rheology, and pulsed field gradient nuclear magnetic resonance. We demonstrate that the low level of ionic conductivity in this material is due to the combined effects of reduced ion mobility as well as reduced free ion concentration relative to other types of ILs. Furthermore, detailed analysis of the DDLS spectra reveals a slow process in addition to the structural a relaxation that we attribute to reorientational motion of alkyl aggregates. These findings indicate that hydrophobic aggregation strongly influences the charge transport mechanism of aprotic ammonium ionic liquids with long aliphatic side chains. C1 [Griffin, Philip J.; Holt, Adam P.; Sokolov, Alexei P.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Novikov, Vladimir N.; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Sangoro, Joshua R.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Wang, Yangyang; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. [Kremer, Friedrich] Univ Leipzig, Inst Expt Phys, D-04103 Leipzig, Germany. RP Sangoro, JR (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. EM jsangoro@utk.edu RI Griffin, Philip/G-8093-2014; Griffin, Philip/K-3976-2013; Wang, Yangyang/A-5925-2010; Sangoro, Joshua/A-6573-2011 OI Wang, Yangyang/0000-0001-7042-9804; Sangoro, Joshua/0000-0002-5483-9528 FU NSF Chemistry program [CHE-1213444]; LDRD program of Oak Ridge National Laboratory; University of Tennessee-Knoxville; German Research Foundation (DFG) FX The authors gratefully acknowledge S. Naumov and J. Karger (University of Leipzig) for help with PFG NMR measurements. The UT team thanks the NSF Chemistry program for funding (Grant CHE-1213444). Y.W. acknowledges funding through the LDRD program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. J.RS. thanks the University of Tennessee-Knoxville for financial support through tenure-track faculty research start-up funds. F.K. acknowledges the German Research Foundation (DFG) for financial support. NR 47 TC 15 Z9 15 U1 6 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 23 PY 2014 VL 118 IS 3 BP 783 EP 790 DI 10.1021/jp412365n PG 8 WC Chemistry, Physical SC Chemistry GA 297JW UT WOS:000330252700015 PM 24387344 ER PT J AU Lopez-Bezanilla, A AF Lopez-Bezanilla, Alejandro TI Electronic and Quantum Transport Properties of Substitutionally Doped Double-Walled Carbon Nanotubes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HIGH-PERFORMANCE ELECTRONICS; AB-INITIO; GRAPHENE; FUNCTIONALIZATION; CONDUCTANCE; MOLECULES; COVERAGE; ROUTE AB A first-principles investigation of the electronic and quantum transport properties of double-walled carbon nanotubes doped with nitrogen and boron atoms is presented. Concentric nanotube sidewalls separated by the typical graphitic van der Waals bond distance are found to strongly interact upon incorporation of doping atoms in the hexagonal networks. The local perturbation caused by the doping atoms extends over both shells due to a hybridization of their electronic states, yielding a reduction of the backscattering efficiency as compared with two independent single-walled nanotubes. A multiscale approach for the study of transport properties of micrometer-long double-walled carbon nanotubes demonstrates that transitions from the ballistic to the localized regime can occur depending on the type of doping and the energy of the charge carrier. These results shed light on the quantum mechanism by which B and N doping represent an efficient method to create mobility gaps in metallic concentric carbon nanotubes. C1 Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM alejandrolb@gmail.com RI Lopez-Bezanilla, Alejandro/B-9125-2015 OI Lopez-Bezanilla, Alejandro/0000-0002-4142-2360 FU Office of Science of the U.S. DOE [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX I gratefully acknowledge the computing resources provided on the Blues compute cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. Research at Argonne National Laboratory, including resources of the Argonne Leadership Computing Facility, is supported by the Office of Science of the U.S. DOE under contract DE-AC02-06CH11357. This research also used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 26 TC 3 Z9 3 U1 3 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 23 PY 2014 VL 118 IS 3 BP 1472 EP 1477 DI 10.1021/jp410648p PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 297JV UT WOS:000330252600008 ER PT J AU Rajput, NN Monk, J Hung, FR AF Rajput, Nay Nidhi Monk, Joshua Hung, Francisco R. TI Ionic Liquids Confined in a Realistic Activated Carbon Model: A Molecular Simulation Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOUBLE-LAYER CAPACITORS; ELECTRICAL DOUBLE-LAYER; SILICA-DERIVED NETWORKS; PORE-SIZE; DIFFERENTIAL CAPACITANCE; COMPUTER-SIMULATION; ELECTROCHEMICAL CAPACITORS; DYNAMICS SIMULATIONS; NANOTUBE ELECTRODES; GRAPHITE-ELECTRODES AB Classical molecular dynamics simulations were performed to study the structure and dynamics of the ionic liquid (IL) [emim(+)] [NTf2-] inside a slit graphitic nanopore and a realistic model of a coconut shell activated carbon (CSAC), which was generated using a reverse Monte Carlo protocol and matches the experimental radial distribution function from the real adsorbent. The CSAC model material consists of semigraphitic carbon sheets with different sizes and shapes, which form irregularly connected pores of roughly rectangular shape. In general, the ions inside the CSAC model material form layers parallel to the walls, as observed for the IL inside slit pores; however, the distribution of pore sizes and the complex pore geometry of the CSAC model materials cause the density profiles and the orientation of the ions to depart significantly from the uniform behavior observed for these properties of the IL inside slit pores. The presence of interconnected pores with a distribution of sizes in the CSAC model materials also causes confinement effects to be weaker than in slit pores of the same size; as a result, the ions inside CSAC model materials have a liquid structure similar to that of the bulk IL and have faster dynamics than those of ions inside slit pores of the same size. The ions near the pore walls of the CSAC model material move slower than the ions that are farther away from the walls, as observed for the IL inside slit pores; however, the complex pore geometry and variations of pore size with position within the CSAC model material cause the dynamics of the confined IL to exhibit significant spatial heterogeneities and depart significantly from the uniform, regular behavior observed in slit nanopores. Our results suggest that the structure and dynamics of ILs confined inside porous materials having heterogeneities in pore size, pore shape, and pore interconnectivity can depart significantly from the properties of ILs confined inside ideal pores of simple geometries. C1 [Rajput, Nay Nidhi; Monk, Joshua; Hung, Francisco R.] Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Rajput, Nay Nidhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Electrochem Technol Grp, Berkeley, CA 94720 USA. [Monk, Joshua] NASA, Thermal Protect Mat Branch, Ames Res Ctr, Moffett Field, CA 94035 USA. [Hung, Francisco R.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. RP Hung, FR (reprint author), Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. EM frhung@lsu.edu FU National Science Foundation [CBET-1253075]; National Science Foundation (EPSCoR) [EPS-1003897]; Louisiana Board of Regents FX We are grateful to Jeremy Palmer (Princeton) for his help in determining the pore size distribution of the carbon models used in this study. This work was partially supported by the National Science Foundation (CAREER Award CBET-1253075, and EPSCoR Cooperative Agreement EPS-1003897) and by the Louisiana Board of Regents. High-performance computational resources for this research were provided by High Performance Computing at Louisiana State University (http://www.hpc.lsu.edu) and the Louisiana Optical Network Initiative (http://www.loni.org). NR 94 TC 17 Z9 17 U1 6 U2 107 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 23 PY 2014 VL 118 IS 3 BP 1540 EP 1553 DI 10.1021/jp408617j PG 14 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 297JV UT WOS:000330252600016 ER PT J AU Muller, K Lu, DY Senanayake, SD Starr, DE AF Mueller, Kathrin Lu, Deyu Senanayake, Sanjaya D. Starr, David E. TI Monoethanolamine Adsorption on TiO2(110): Bonding, Structure, and Implications for Use as a Model Solid-Supported CO2 Capture Material SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; SELECTIVE OXIDATION; ALIPHATIC-ALCOHOLS; TITANIUM-DIOXIDE; HYDROGEN-BOND; TIO2 RUTILE; SURFACE; METHANOL; DECOMPOSITION; CATALYSTS AB We have studied the adsorption of monoethanolamine (MEA, HO(CH2)(2)NH2), a well-known CO2 capture molecule, on the rutile TiO2(110) surface using a combined experimental and theoretical approach. X-ray photoelectron spectroscopy, near-edge X-ray absorption fine structure spectroscopy, and scanning tunneling microscopy measurements indicate that MEA adsorbs with the oxygen atom of the hydroxyl group and the nitrogen atom of the amine group bonded to adjacent 5-fold coordinated Ti-sites (Ti(5f)) in the Ti-troughs, leading to a saturation coverage of 0.5 ML at room temperature. Density functional theory calculations confirm that this adsorption configuration is the most stable one with an adsorption energy of 2.33 eV per MEA molecule. The bonding of MEA to TiO2(110) is dominated by local donor-acceptor bonds between the oxygen and nitrogen atoms of the MEA molecule and surface Ti(5f) sites. Hydrogen bonds between adjacent MEA molecules stabilize the adsorption structure at saturation coverage. The implications of this bonding configuration for the use of MEA/TiO2(110) as a model CO2 capture material will be discussed. C1 [Mueller, Kathrin; Lu, Deyu; Starr, David E.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Lu, DY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM dlu@bnl.gov; david.starr@helmholtz-berlin.de RI Muller, Kathrin/H-1902-2011; Senanayake, Sanjaya/D-4769-2009; Lu, Deyu/O-4418-2016 OI Senanayake, Sanjaya/0000-0003-3991-4232; Lu, Deyu/0000-0003-4351-6085 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge Tsung-Liang Chen, Peter Albrecht, and Dave Mullins for their assistance during the measurements at the National Synchrotron Light Source. In addition, we thank Hendrik Bluhm of the Chemical Sciences Division at Lawrence Berkeley National Laboratory for assistance with the AP-XPS experiments. This work was made possible through the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. The computational resource is partially provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 64 TC 5 Z9 5 U1 1 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 23 PY 2014 VL 118 IS 3 BP 1576 EP 1586 DI 10.1021/jp409098p PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 297JV UT WOS:000330252600020 ER PT J AU Sorescu, DC Civis, S Jordan, KD AF Sorescu, Dan C. Civis, Svatopluk Jordan, Kenneth D. TI Mechanism of Oxygen Exchange between CO2 and TiO2(101) Anatase SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; PLUS U CALCULATIONS; ISOTOPE-EXCHANGE; CARBON-DIOXIDE; TITANIUM-DIOXIDE; TIO2 NANOCRYSTAL; RUTILE TIO2(110); SURFACE DEFECT; BASIS-SET AB The mechanism of oxygen exchange between CO2 and a defective anatase (101) surface was investigated by density functional theory calculations including corrections for long-range dispersion interactions and for on-site Coulomb interactions. The calculations identify a carbonate-like configuration at a surface oxygen defect site as the key intermediate species responsible for the oxygen exchange. The stability of this species, its vibrational frequencies, and the reaction barriers involved in the oxygen exchange mechanism are found to be highly dependent on the specific value of the Hubbard U correction used to describe the on-site Coulomb interactions within the GGA+U procedure. U parameter values that result in CO2 adsorption energies and reaction barriers for oxygen exchange consistent with the results of room-temperature experiments are smaller (U <= 2.5 eV) than those that reproduce the experimental band gap or location of defect states in the band gap of the reduced TiO2 crystal. C1 [Sorescu, Dan C.; Jordan, Kenneth D.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Civis, Svatopluk] Acad Sci Czech Republic, J Heyrovsky Inst Phys Chem, Vvi, CR-18223 Prague 8, Czech Republic. [Jordan, Kenneth D.] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Jordan, Kenneth D.] Univ Pittsburgh, Ctr Mol & Mat Simulat, Pittsburgh, PA 15260 USA. RP Sorescu, DC (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM sorescu@netl.doe.gov FU National Energy Technology Laboratory's Office of Research and Development [DE-FE0004000.2.661.251.001] FX We acknowledge a grant of computer time at Pittsburgh Supercomputer Center and on the NETL HPCEE supercomputer system. The work at University of Pittsburgh was performed in support of the National Energy Technology Laboratory's Office of Research and Development under Contract DE-FE0004000.2.661.251.001. Disclaimer: reference in this work to any specific commercial product is to facilitate understanding and does not necessarily imply endorsement by the United States Department of Energy. NR 74 TC 15 Z9 15 U1 3 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 23 PY 2014 VL 118 IS 3 BP 1628 EP 1639 DI 10.1021/jp410420e PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 297JV UT WOS:000330252600026 ER PT J AU Roederer, M Keele, BF Schmidt, SD Mason, RD Welles, HC Fischer, W Labranche, C Foulds, KE Louder, MK Yang, ZY Todd, JPM Buzby, AP Mach, LV Shen, L Seaton, KE Ward, BM Bailer, RT Gottardo, R Gu, WJ Ferrari, G Alam, SM Denny, TN Montefiori, DC Tomaras, GD Korber, BT Nason, MC Seder, RA Koup, RA Letvin, NL Rao, SS Nabel, GJ Mascola, JR AF Roederer, Mario Keele, Brandon F. Schmidt, Stephen D. Mason, Rosemarie D. Welles, Hugh C. Fischer, Will Labranche, Celia Foulds, Kathryn E. Louder, Mark K. Yang, Zhi-Yong Todd, John-Paul M. Buzby, Adam P. Mach, Linh V. Shen, Ling Seaton, Kelly E. Ward, Brandy M. Bailer, Robert T. Gottardo, Raphael Gu, Wenjuan Ferrari, Guido Alam, S. Munir Denny, Thomas N. Montefiori, David C. Tomaras, Georgia D. Korber, Bette T. Nason, Martha C. Seder, Robert A. Koup, Richard A. Letvin, Norman L. Rao, Srinivas S. Nabel, Gary J. Mascola, John R. TI Immunological and virological mechanisms of vaccine-mediated protection against SIV and HIV SO NATURE LA English DT Article ID SIMIAN IMMUNODEFICIENCY VIRUS; DOSE CHALLENGE EXPERIMENTS; NEUTRALIZING ANTIBODIES; RHESUS MACAQUES; CELL RESPONSES; EFFICACY TRIAL; INFECTION; BINDING; SIVSME660; PREVENTION AB A major challenge for the development of a highly effective AIDS vaccine is the identification of mechanisms of protective immunity. To address this question, we used a nonhuman primate challenge model with simian immunodeficiency virus (SIV). We show that antibodies to the SIV envelope are necessary and sufficient to prevent infection. Moreover, sequencing of viruses from breakthrough infections revealed selective pressure against neutralization-sensitive viruses; we identified a two-amino-acid signature that alters antigenicity and confers neutralization resistance. A similar signature confers resistance of human immunodeficiency virus (HIV)-1 to neutralization by monoclonal antibodies against variable regions 1 and 2 (V1V2), suggesting that SIV and HIV share a fundamental mechanism of immune escape from vaccine-elicited or naturally elicited antibodies. These analyses provide insight into the limited efficacy seen in HIV vaccine trials. C1 [Roederer, Mario; Schmidt, Stephen D.; Mason, Rosemarie D.; Welles, Hugh C.; Foulds, Kathryn E.; Louder, Mark K.; Yang, Zhi-Yong; Todd, John-Paul M.; Bailer, Robert T.; Seder, Robert A.; Koup, Richard A.; Rao, Srinivas S.; Nabel, Gary J.; Mascola, John R.] NIAID, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA. [Keele, Brandon F.] NIH, SAIC Frederick, Frederick Natl Lab, Frederick, MD 21702 USA. [Welles, Hugh C.] George Washington Univ, Washington, DC 20052 USA. [Fischer, Will; Korber, Bette T.] Los Alamos Natl Labs, Los Alamos, NM 87545 USA. [Labranche, Celia; Ward, Brandy M.; Ferrari, Guido; Montefiori, David C.] Duke Univ, Dept Surg, Durham, NC 27710 USA. [Buzby, Adam P.; Mach, Linh V.; Shen, Ling; Letvin, Norman L.] Beth Israel Deaconess Med Ctr, Ctr Virol & Vaccine Res, Boston, MA 02115 USA. [Seaton, Kelly E.; Alam, S. Munir; Denny, Thomas N.; Tomaras, Georgia D.] Duke Univ, Human Vaccine Inst, Durham, NC 27710 USA. [Gottardo, Raphael] Fred Hutchison Canc Res Ctr, Seattle, WA 98109 USA. [Gu, Wenjuan; Nason, Martha C.] NIAID, Biostat Res Branch, NIH, Bethesda, MD 20892 USA. RP Roederer, M (reprint author), NIAID, Vaccine Res Ctr, NIH, 9000 Rockville Pike, Bethesda, MD 20892 USA. EM Roederer@NIH.gov RI Schmidt, Stephen/B-5398-2012; Ferrari, Guido/A-6088-2015; Tomaras, Georgia/J-5041-2016; OI Denny, Thomas/0000-0002-7364-8276; Welles, Hugh/0000-0002-3336-1203; Fischer, Will/0000-0003-4579-4062; Korber, Bette/0000-0002-2026-5757 FU Intramural Research Program of the Vaccine Research Center, NIAID, NIH; NIH [HHSN261200800001E, HHSN27201100016C, AI100645]; Bill and Melinda Gates Foundation [OPP1032317] FX We thank the following individuals: W. Shi, L. Wu, S.-Y. Ko, L. Wang and W.-P. Kong for immunogen construction; M. M. Donaldson, S.-F. Kao, D. Quinn, J. Owuor, K. Denison, H. Balachandran, C. Luedemann, W. T. Williams, G. Overman, A. Deal, C. Brinkley and L. Racz for technical assistance with immunology assays; A. Ault for assistance managing NHP studies; S. O'Connor for deep-sequencing data; M. Seaman for providing plasmids encoding E660 envelopes; F. McCutchan, J. Overbaugh and J. Kim for HIV-1 strains; and P. Gilbert for advice with using the Aalen and Johansen model. This work was supported by the Intramural Research Program of the Vaccine Research Center, NIAID, NIH; by NIH contracts HHSN261200800001E (B. F. K., W. G.) and HHSN27201100016C (D. C. M.); by NIH grant AI100645 (B. T. K., W. F.); and by the Bill and Melinda Gates Foundation grant OPP1032317. NR 39 TC 65 Z9 65 U1 3 U2 48 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 23 PY 2014 VL 505 IS 7484 BP 502 EP + DI 10.1038/nature12893 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 293SW UT WOS:000329995000030 PM 24352234 ER PT J AU Morita, K Skokov, V Friman, B Redlich, K AF Morita, Kenji Skokov, Vladimir Friman, Bengt Redlich, Krzysztof TI Net baryon number probability distribution near the chiral phase transition SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HEAVY-ION COLLISIONS; FINITE-DENSITY; GAUGE-THEORIES; FREEZE-OUT; QCD; FLUCTUATIONS; DECONFINEMENT; PARTICLE AB We discuss the properties of the net baryon number probability distribution near the chiral phase transition to explore the effect of critical fluctuations. Our studies are performed within Landau theory, where the coefficients of the polynomial potential are parametrized, so as to reproduce the mean-field (MF), the Z(2), and the O(4) scaling behaviors of the cumulants of the net baryon number. We show that in the critical region the structure of the probability distribution changes, depending on the values of the critical exponents. In the MF approach, as well as in the Z(2) universality class, the contribution of the singular part of the thermodynamic potential tends to broaden the distribution. By contrast, in the model with O(4) scaling, the contribution of the singular part results in a narrower net baryon number probability distribution with a wide tail. C1 [Morita, Kenji] Frankfurt Inst Adv Studies, D-60438 Frankfurt, Germany. [Morita, Kenji] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Skokov, Vladimir] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Friman, Bengt] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Redlich, Krzysztof] Univ Wroclaw, Inst Theoret Phys, PL-50204 Wroclaw, Poland. [Redlich, Krzysztof] GSI Darmstadt, Extreme Matter Inst EMMI, D-64291 Darmstadt, Germany. RP Morita, K (reprint author), Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. EM morita@fias.uni-frankfurt.de RI Morita, Kenji/R-8116-2016; OI Morita, Kenji/0000-0001-6272-1290; Skokov, Vladimir/0000-0001-7619-1796; Friman, Bengt/0000-0002-3211-7073 FU HIC for FAIR; Yukawa Institute for Theoretical Physics; Yukawa International Program for Quark-Hadron Sciences at Kyoto University; JSPS [24540271]; Polish Ministry of National Education (MEN); U. S. Department of Energy [DE-AC02-98CH10886]; ExtreMe Matter Institute EMMI FX The authors gratefully acknowledge F. Karsch for discussions, particularly on the O(4) scaling function. K.M. would like to thank RIKEN-BNL Research Center for warm hospitality during his visit where part of this work was completed. He also would like to thank P. de Forcrand and A. Ohnishi for fruitful discussions. This work was in part supported by HIC for FAIR, by the young researchers exchange program by the Yukawa Institute for Theoretical Physics, by Yukawa International Program for Quark-Hadron Sciences at Kyoto University and by the Grants-in-Aid for Scientific Research from JSPS No. 24540271. K.R. acknowledges partial support of the Polish Ministry of National Education (MEN). The research of V.S. is supported under Contract No. DE-AC02-98CH10886 with the U. S. Department of Energy. B.F. is supported in part by the ExtreMe Matter Institute EMMI. NR 64 TC 11 Z9 11 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN 23 PY 2014 VL 74 IS 1 AR 2706 DI 10.1140/epjc/s10052-013-2706-1 PG 9 WC Physics, Particles & Fields SC Physics GA CD0BC UT WOS:000350734100001 ER PT J AU Agrawal, P Frugiuele, C AF Agrawal, Prateek Frugiuele, Claudia TI Mixing stops at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID STANDARD MODEL; SCALAR TOP; SEARCH; PARTICLE; BOSON AB We study the phenomenology of a light stop NLSP in the presence of large mixing with either the first or the second generation. R-symmetric models provide a prime setting for this scenario, but our discussion also applies to the MSSM when a significant amount of mixing can be accommodated. In our framework the dominant stop decay is through the flavor violating mode into a light jet and the LSP in an extended region of parameter space. There are currently no limits from ATLAS and CMS in this region. We emulate shape-based hadronic SUSY searches for this topology, and find that they have potential sensitivity. If the extension of these analyses to this region is robust, we find that these searches can set strong exclusion limits on light stops. If not, then the flavor violating decay mode is challenging and may represent a blind spot in stop searches even at 13TeV. Thus, an experimental investigation of this scenario is well motivated. C1 [Agrawal, Prateek; Frugiuele, Claudia] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Agrawal, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM prateek@fnal.gov; claudiaf@fnal.gov OI Agrawal, Prateek/0000-0001-9947-0632 FU United States Department of Energy [DE-AC02-07CH11359] FX We thank Wolfgang Altmannshofer, Joe Lykken, Verena Martinez Outschoorn and Maurizio Pierini for valuable discussions. We are grateful to Zackaria Chacko, Bogdan Dobrescu, Marco Farina, Thomas Gregoire, Roni Harnik and Felix Yu for useful comments on the manuscript. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 68 TC 17 Z9 17 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 22 PY 2014 IS 1 AR 115 DI 10.1007/JHEP01(2014)115 PG 26 WC Physics, Particles & Fields SC Physics GA AW4GL UT WOS:000346239100003 ER PT J AU Nakhimovsky, L AF Nakhimovsky, Lina TI The Peculiarities of the Optical Absorption of Monocrystalline Fluorene and Its Heteroanalogues in the Energy Range Between 3.5 eV and 8.5 eV SO MOLECULAR CRYSTALS AND LIQUID CRYSTALS LA English DT Article; Proceedings Paper CT 9th International Conference on Electronic Processes in Organic Materials (ICEPOM) CY MAY 20-24, 2013 CL Lviv, UKRAINE ID MOLECULAR-STRUCTURE; ELECTRONIC STATES; CARBAZOLE; CRYSTAL; DIBENZOFURAN; PHENANTHRENE; SPECTRA; HYPOCHROMISM; TRANSITIONS; SINGLET AB Electronic absorption spectra of carbazole, dibenzofuran and fluorene were obtained in all three crystallographic directions (energy range 3.5-8.5eV). All electronic transitions with transition dipoles at oblique angles to a and b crystallographic axes can be traced to parental molecular states. Crystal transitions with parallel transition dipoles can be traced to parental molecular states for thin (0.1-0.2) crystals, slow crystallized from melt under uniaxial pressure. For sublimation flakes and crystals fast crystallized from melt, these transitions cannot be traced to parental molecular states since their spectra have continuous, essentially uniform intensity distribution except for such transition at the onset of absorption. C1 Brookhaven Natl Lab, Upton, NY 11973 USA. RP Nakhimovsky, L (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM linanakh@yahoo.com NR 31 TC 0 Z9 0 U1 0 U2 1 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 1542-1406 EI 1563-5287 J9 MOL CRYST LIQ CRYST JI Mol. Cryst. Liquid Cryst. PD JAN 22 PY 2014 VL 589 IS 1 BP 29 EP 47 DI 10.1080/15421406.2013.871883 PG 19 WC Crystallography SC Crystallography GA AE6BQ UT WOS:000334073700004 ER PT J AU Biswal, AK Soeno, K Gandla, ML Immerzeel, P Pattathil, S Lucenius, J Serimaa, R Hahn, MG Moritz, T Jonsson, LJ Israelsson-Nordstrom, M Mellerowicz, EJ AF Biswal, Ajaya K. Soeno, Kazuo Gandla, Madhavi Latha Immerzeel, Peter Pattathil, Sivakumar Lucenius, Jessica Serimaa, Ritva Hahn, Michael G. Moritz, Thomas Jonsson, Leif J. Israelsson-Nordstrom, Maria Mellerowicz, Ewa J. TI Aspen pectate lyase PtxtPL1-27 mobilizes matrix polysaccharides from woody tissues and improves saccharification yield SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Populus; Wood development; Secondary cell wall; Lignocellulose; Biofuel; Pectin ID PLANT-CELL WALLS; MONOCLONAL-ANTIBODIES; PECTIN-METHYLESTERASE; GENE-EXPRESSION; ENZYME-ACTIVITY; LIGNIN CONTENT; HYBRID ASPEN; XYLOGLUCAN; POPLAR; GROWTH AB Background: Wood cell walls are rich in cellulose, hemicellulose and lignin. Hence, they are important sources of renewable biomass for producing energy and green chemicals. However, extracting desired constituents from wood efficiently poses significant challenges because these polymers are highly cross-linked in cell walls and are not easily accessible to enzymes and chemicals. Results: We show that aspen pectate lyase PL1-27, which degrades homogalacturonan and is expressed at the onset of secondary wall formation, can increase the solubility of wood matrix polysaccharides. Overexpression of this enzyme in aspen increased solubility of not only pectins but also xylans and other hemicelluloses, indicating that homogalacturonan limits the solubility of major wood cell wall components. Enzymatic saccharification of wood obtained from PL1-27-overexpressing trees gave higher yields of pentoses and hexoses than similar treatment of wood from wild-type trees, even after acid pretreatment. Conclusions: Thus, the modification of pectins may constitute an important biotechnological target for improved wood processing despite their low abundance in woody biomass. C1 [Biswal, Ajaya K.; Soeno, Kazuo; Moritz, Thomas; Israelsson-Nordstrom, Maria; Mellerowicz, Ewa J.] Swedish Univ Agr Sci, Dept Forest Genet & Plant Physiol, S-90183 Umea, Sweden. [Gandla, Madhavi Latha; Jonsson, Leif J.] Umea Univ, Dept Chem, S-90187 Umea, Sweden. [Lucenius, Jessica; Serimaa, Ritva] Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland. [Biswal, Ajaya K.; Immerzeel, Peter; Pattathil, Sivakumar; Hahn, Michael G.] Univ Georgia, BioEnergy Sci Ctr BESC, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. RP Mellerowicz, EJ (reprint author), Swedish Univ Agr Sci, Dept Forest Genet & Plant Physiol, S-90183 Umea, Sweden. EM Ewa.Mellerowicz@slu.se RI SOENO, Kazuo/B-1571-2010; OI Hahn, Michael/0000-0003-2136-5191; , Sivakumar Pattathil/0000-0003-3870-4137 FU FORMAS; Swedish Research Council; UPSC Berzelii Center of Forest Biotechnology; VR; Vinnova; Biomime Center; Swedish Foundation for Strategic Research; Knut & Alice Wallenberg Foundation; Bio4Energy; SNS; United States Department of Energy [DE-AC05-00OR22725]; NSF Plant Genome Program [DBI-0421683] FX We thank Mattias Holmlund for a gift of pMH1.kana vector and Jesper Harholt for fruitful discussions. The research was funded by FORMAS, the Swedish Research Council, UPSC Berzelii Center of Forest Biotechnology (funded by VR and Vinnova), Biomime Center (funded by the Swedish Foundation for Strategic Research, the Knut & Alice Wallenberg Foundation), Bio4Energy and SNS. The glycome profiling was supported by the BioEnergy Science Center administered by Oak Ridge National Laboratory and funded by a grant (DE-AC05-00OR22725) from the United States Department of Energy. Generation of the CCRC series of plant glycan-directed monoclonal antibodies was supported by the NSF Plant Genome Program (DBI-0421683). NR 49 TC 19 Z9 19 U1 3 U2 36 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JAN 22 PY 2014 VL 7 AR 11 DI 10.1186/1754-6834-7-11 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA AD1ID UT WOS:000332986700001 PM 24450583 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besanon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G De Jong, SJ De la Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Gruenendahl, S Gruenewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M De Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Snchez-Hernndez, A Sanders, MP Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Sldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R Van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besanon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. De Jong, S. J. De la Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De la Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. De Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Snchez-Hernndez, A. Sanders, M. P. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Sldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. Van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Search for the X(4140) state in B+ -> J/psi phi K+ decays with the D0 detector SO PHYSICAL REVIEW D LA English DT Article AB We investigate the decay B+ -> J/psi phi K+ in a search for the X(4140) state, a narrow threshold resonance in the J/psi phi system. The data sample corresponds to an integrated luminosity of 10.4 fb(-1) of p (p) over bar collisions at root s = 1.96 TeV collected by the D0 experiment at the Fermilab Tevatron collider. We observe a mass peak with a statistical significance of 3.1 standard deviations and measure its invariant mass to be M = 4159.0 +/- 4.3(stat) +/- 6.6(syst) MeV and its width to be Gamma = 19.9 +/- 12.6(stat)(-8.0)(+3.0)(syst) MeV. C1 [Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Augsten, K.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, Prague, Czech Republic. [Kupco, A.; Lokajicek, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Hoeneisen, B.] Univ San Francisco Quito, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, LPC, CNRS, IN2P3, Clermont, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, Inst Natl Polytech Grenoble, LPSC,IN2P3, Grenoble, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CPPM, CNRS, IN2P3, Marseille, France. [Grivaz, J. -F.; Guillemin, T.; Jaffre, M.; Petroff, P.] Univ Paris 11, LAL, CNRS, IN2P3, Orsay, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 06, CNRS, LPNHE, IN2P3, Paris, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 07, CNRS, LPNHE, IN2P3, Paris, France. [Bassler, U.; Besanon, M.; Chapon, E.; Couderc, F.; Deliot, F.; Grohsjean, A.; Hubacek, Z.; Royon, C.; Shary, V.; Titov, M.; Tuchming, B.; Vilanova, D.] CEA, Irfu, SPP, Saclay, France. [Greder, S.; Miconi, F.; Ripp-Baudot, I.] Univ Strasbourg, IPHC, CNRS, IN2P3, Strasbourg, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon 1, CNRS, IPNL, IN2P3, F-69622 Villeurbanne, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon, Lyon, France. [Hebbeker, T.; Meyer, A.; Sonnenschein, L.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Bernhard, R.; Madar, R.] Univ Freiburg, Inst Phys, D-79106 Freiburg, Germany. [Brandt, O.; Deterre, C.; Hensel, C.; Mansour, J.; Meyer, J.; Peters, Y.; Quadt, A.; Shabalina, E.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Buescher, V.; Fiedler, F.; Hohlfeld, M.; Weichert, J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Nunnemann, T.; Sanders, M. P.] Univ Munich, Munich, Germany. [Beri, S. B.; Bhatnagar, V.; Dutt, S.; Kohli, J. M.] Panjab Univ, Chandigarh 160014, India. [Choudhary, B.; Dubey, A.] Univ Delhi, Delhi 110007, India. [Acharya, B. S.; Banerjee, S.; Mondal, N. K.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Gruenewald, M. W.] Univ Coll Dublin, Dublin 2, Ireland. [Cho, S. W.; Choi, S.; Jeong, M. S.; Lee, H. S.; Lim, J. K.; Park, S. K.] Korea Univ, Korea Detector Lab, Seoul, South Korea. [Alton, A.; Camacho-Perez, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Garcia-Gonzalez, J. A.; Heredia-De la Cruz, I.; Luna-Garcia, R.; Magana-Villalba, R.; Martinez-Ortega, J.; Snchez-Hernndez, A.] CINVESTAV, Mexico City 14000, DF, Mexico. [De Jong, S. J.; Filthaut, F.; Meijer, M. M.; Van Leeuwen, W. M.] NIKHEF H, NL-1009 DB Amsterdam, Netherlands. [De Jong, S. J.; Filthaut, F.; Meijer, M. M.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Tokmenin, V. V.; Verkheev, A. Y.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Gavrilov, V.; Kiselevich, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E. E.; Bunichev, V.; Dudko, L. V.; Karmanov, D.; Kuzmin, V. A.; Merkin, M.; Perfilov, M.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Denisov, S. P.; Evdokimov, V. N.; Kozelov, A. V.; Lipaev, V. V.; Popov, A. V.; Prokopenko, N.; Razumov, I.; Shchukin, A. A.; Stoyanova, D. A.; Vasilyev, I. A.] Inst High Energy Phys, Protvino, Russia. [Alkhazov, G.; Lobodenko, A.; Neustroev, P.; Scheglov, Y.; Uvarov, L.; Uvarov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Juste, A.] ICREA, Barcelona, Spain. [Juste, A.] IFAE, Barcelona, Spain. [Buszello, C. P.] Uppsala Univ, Uppsala, Sweden. [Bertram, I.; Borissov, G.; Burdin, S.; Fox, H.; Ratoff, P. N.; Ross, A.] Univ Lancaster, Lancaster LA1 4YB, England. [Beuselinck, R.; Davies, G.; Hays, J.; Jesik, R.; Jonsson, P.; Scanlon, T.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Agnew, J. P.; Ding, P. F.; Harder, K.; Head, T.; Hesketh, G.; McGivern, C. L.; Petridis, K.; Price, D.; Schwanenberger, C.; Sldner-Rembold, S.; Suter, L.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Bandurin, D. V.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Bu, X. B.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Garbincius, P. H.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Herner, K.; Illingworth, R.; Ito, A. S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Lee, W. M.; Li, Q. Z.; Lincoln, D.; Lipton, R.; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Verzocchi, M.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.; Shaw, S.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; De Sa, R. Lopes; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Haley, J.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Jabeen, S.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna, Russia. RI Kupco, Alexander/G-9713-2014; Fisher, Wade/N-4491-2013; Santos, Angelo/K-5552-2012; Deliot, Frederic/F-3321-2014; Kozelov, Alexander/J-3812-2014; Lokajicek, Milos/G-7800-2014; Lei, Xiaowen/O-4348-2014; Merkin, Mikhail/D-6809-2012; Li, Liang/O-1107-2015; Sharyy, Viatcheslav/F-9057-2014; Dudko, Lev/D-7127-2012 OI Lei, Xiaowen/0000-0002-2564-8351; Li, Liang/0000-0001-6411-6107; Sharyy, Viatcheslav/0000-0002-7161-2616; Dudko, Lev/0000-0002-4462-3192 FU DOE (USA); NSF (USA); CEA (France); CNRS/IN2P3 (France); MON (Russia); NRC KI (Russia); RFBR (Russia); CNPq (Brazil); FAPERJ (Brazil); FAPESP (Brazil); FUNDUNESP (Brazil); DAE (India); DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (The Netherlands); STFC (United Kingdom); Royal Society (United Kingdom); MSMT (Czech Republic); GACR (Czech Republic); BMBF (Germany); DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS (China); CNSF (China) FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); MON, NRC KI and RFBR (Russia); CNPq, FAPERJ, FAPESP and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (The Netherlands); STFC and the Royal Society (United Kingdom); MSMT and GACR (Czech Republic); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 16 TC 39 Z9 39 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 22 PY 2014 VL 89 IS 1 AR 012004 DI 10.1103/PhysRevD.89.012004 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5ZR UT WOS:000331867700001 ER PT J AU Balakrishnan, K Garcia, AL Donev, A Bell, JB AF Balakrishnan, Kaushik Garcia, Alejandro L. Donev, Aleksandar Bell, John B. TI Fluctuating hydrodynamics of multispecies nonreactive mixtures SO PHYSICAL REVIEW E LA English DT Article ID NONEQUILIBRIUM FLUCTUATIONS; DIFFUSION; GAS; THERMODYNAMICS; EQUILIBRIUM; SIMULATIONS; EQUATIONS; SCHEMES AB In this paper we discuss the formulation of the fluctuating Navier-Stokes equations for multispecies, nonreactive fluids. In particular, we establish a form suitable for numerical solution of the resulting stochastic partial differential equations. An accurate and efficient numerical scheme, based on our previous methods for single species and binary mixtures, is presented and tested at equilibrium as well as for a variety of nonequilibrium problems. These include the study of giant nonequilibrium concentration fluctuations in a ternary mixture in the presence of a diffusion barrier, the triggering of a Rayleigh-Taylor instability by diffusion in a four-species mixture, as well as reverse diffusion in a ternary mixture. Good agreement with theory and experiment demonstrates that the formulation is robust and can serve as a useful tool in the study of thermal fluctuations for multispecies fluids. C1 [Balakrishnan, Kaushik; Bell, John B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Garcia, Alejandro L.] San Jose State Univ, Dept Phys & Astron, San Jose, CA 95192 USA. [Donev, Aleksandar] NYU, Courant Inst Math Sci, New York, NY 10012 USA. RP Balakrishnan, K (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU Applied Mathematics Program of the US DOE Office of Advance Scientifc Computing Research [DE-AC02005CH11231]; National Science Foundation [DMS-1115341]; Office of Science of the US Department of Energy [DE-SC0008271, DE-AC02-05CH11231] FX The work at LBNL was supported by the Applied Mathematics Program of the US DOE Office of Advance Scientifc Computing Research under Contract No. DE-AC02005CH11231. A. Donev was supported in part by the National Science Foundation under Grant No. DMS-1115341 and the Office of Science of the US Department of Energy through Early Career Award No. DE-SC0008271. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 52 TC 11 Z9 11 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 22 PY 2014 VL 89 IS 1 AR 013017 DI 10.1103/PhysRevE.89.013017 PG 16 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AC0EF UT WOS:000332166900007 PM 24580330 ER PT J AU Yu, JF Xie, ZY Meurice, Y Liu, YZ Denbleyker, A Zou, HY Qin, MP Chen, J Xiang, T AF Yu, J. F. Xie, Z. Y. Meurice, Y. Liu, Yuzhi Denbleyker, A. Zou, Haiyuan Qin, M. P. Chen, J. Xiang, T. TI Tensor renormalization group study of classical XY model on the square lattice SO PHYSICAL REVIEW E LA English DT Article ID HIGH-TEMPERATURE EXPANSIONS; CRITICAL-BEHAVIOR; PHASE-TRANSITION; MONTE-CARLO AB Using the tensor renormalization group method based on the higher-order singular value decomposition, we have studied the thermodynamic properties of the continuous XY model on the square lattice. The temperature dependence of the free energy, the internal energy, and the specific heat agree with the Monte Carlo calculations. From the field dependence of the magnetic susceptibility, we find the Kosterlitz-Thouless transition temperature to be 0.8921(19), consistent with the Monte Carlo as well as the high temperature series expansion results. At the transition temperature, the critical exponent delta is estimated as 14.5, close to the analytic value by Kosterlitz. C1 [Yu, J. F.; Xie, Z. Y.; Qin, M. P.; Chen, J.; Xiang, T.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Meurice, Y.; Liu, Yuzhi; Denbleyker, A.; Zou, Haiyuan] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Liu, Yuzhi] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. RP Yu, JF (reprint author), Chinese Acad Sci, Inst Phys, POB 603, Beijing 100190, Peoples R China. RI qin, mingpu/S-1545-2016 OI qin, mingpu/0000-0001-7733-9684 FU Chinese Academy of Sciences [2012013]; Department of Energy [DE-SC0010114, FG02-91ER40664]; URA Visiting Scholars' program; United States Department of Energy [DE-AC02-07CH11359] FX This work was supported by the Chinese Academy of Sciences Fellowship for Young International Scientists (Grant No. 2012013). Y.M. was supported by the Department of Energy under Awards No. DE-SC0010114 and No. FG02-91ER40664. Y.L. is supported by the URA Visiting Scholars' program. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 29 TC 12 Z9 12 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 22 PY 2014 VL 89 IS 1 AR 013308 DI 10.1103/PhysRevE.89.013308 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AC0EF UT WOS:000332166900008 PM 24580361 ER PT J AU Schweitzer, MH Zheng, WX Cleland, TP Goodwin, MB Boatman, E Theil, E Marcus, MA Fakra, SC AF Schweitzer, Mary H. Zheng, Wenxia Cleland, Timothy P. Goodwin, Mark B. Boatman, Elizabeth Theil, Elizabeth Marcus, Matthew A. Fakra, Sirine C. TI A role for iron and oxygen chemistry in preserving soft tissues, cells and molecules from deep time SO PROCEEDINGS OF THE ROYAL SOCIETY B-BIOLOGICAL SCIENCES LA English DT Article DE soft tissue preservation; haemoglobin; iron; goethite; Fenton chemistry; protein cross-linking ID TYRANNOSAURUS-REX; EXCEPTIONAL PRESERVATION; ORGANIC PRESERVATION; DINOSAUR BONES; CELLULAR PRESERVATION; PROTEIN SEQUENCES; ANCIENT DNA; FERRITIN; FOSSIL; HEMOGLOBIN AB The persistence of original soft tissues in Mesozoic fossil bone is not explained by current chemical degradation models. We identified iron particles (goethite-alpha FeO(OH)) associated with soft tissues recovered from two Mesozoic dinosaurs, using transmission electron microscopy, electron energy loss spectroscopy, micro-X-ray diffraction and Fe micro-X-ray absorption near-edge structure. Iron chelators increased fossil tissue immunoreactivity to multiple antibodies dramatically, suggesting a role for iron in both preserving and masking proteins in fossil tissues. Haemoglobin (HB) increased tissue stability more than 200-fold, from approximately 3 days to more than two years at room temperature (25 degrees C) in an ostrich blood vessel model developed to test post-mortem 'tissue fixation' by cross-linking or peroxidation. HB-induced solution hypoxia coupled with iron chelation enhances preservation as follows: HB + O-2 > HB - O-2 > -O-2 >> +O-2. The well-known O-2/haeme interactions in the chemistry of life, such as respiration and bioenergetics, are complemented by O-2/haeme interactions in the preservation of fossil soft tissues. C1 [Schweitzer, Mary H.; Zheng, Wenxia; Cleland, Timothy P.] N Carolina State Univ, Raleigh, NC 27695 USA. [Schweitzer, Mary H.] North Carolina Museum Nat Sci, Raleigh, NC 27601 USA. [Goodwin, Mark B.] Univ Calif Berkeley, Museum Paleontol, Berkeley, CA 94720 USA. [Boatman, Elizabeth] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Theil, Elizabeth] CHORI, Oakland, CA 94609 USA. [Theil, Elizabeth] N Carolina State Univ, Dept Mol & Struct Biochem, Raleigh, NC 27695 USA. [Marcus, Matthew A.; Fakra, Sirine C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Schweitzer, MH (reprint author), N Carolina State Univ, Campus Box 8208, Raleigh, NC 27695 USA. EM mhschwei@ncsu.edu FU National Science Foundation [DGE-0750733, EAR 0541744]; David and Lucile Packard Foundation; Office of Science, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231] FX This research was financially supported by the National Science Foundation (DGE-0750733 to T.P.C. and EAR 0541744 to M.H.S.) and the David and Lucile Packard Foundation to M.H.S. The operations of the Advanced Light Source at Lawrence Berkeley National Laboratory are supported by the Director, Office of Science, Office of Basic Energy Sciences, US Department of Energy under contract number DE-AC02-05CH11231. NR 86 TC 9 Z9 9 U1 6 U2 37 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 0962-8452 EI 1471-2954 J9 P ROY SOC B-BIOL SCI JI Proc. R. Soc. B-Biol. Sci. PD JAN 22 PY 2014 VL 281 IS 1775 AR 20132741 DI 10.1098/rspb.2013.2741 PG 10 WC Biology; Ecology; Evolutionary Biology SC Life Sciences & Biomedicine - Other Topics; Environmental Sciences & Ecology; Evolutionary Biology GA AC2XY UT WOS:000332380800021 PM 24285202 ER PT J AU Taen, T Yagyuda, H Nakajima, Y Tamegai, T Ayala-Valenzuela, O Civale, L Maiorov, B Kambara, T Kanai, Y AF Taen, Toshihiro Yagyuda, Hidenori Nakajima, Yasuyuki Tamegai, Tsuyoshi Ayala-Valenzuela, Oscar Civale, Leonardo Maiorov, Boris Kambara, Tadashi Kanai, Yasuyuki TI Observation of lock-in phenomena in heavy-ion-irradiated single crystal of Ba(Fe0.93Co0.07)(2)As-2 SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; IRREVERSIBLE MAGNETIC-MOMENT; CO-DOPED BAFE2AS2; BOSON LOCALIZATION; COATED CONDUCTORS; COLUMNAR DEFECTS; YBA2CU3O7-DELTA; TRANSITION; DEPENDENCE; VORTICES AB The angular dependence of magnetization was measured in an optimally Co-doped BaFe2As2 single crystal, which is irradiated by 2.6 GeV uranium to introduce columnar defects (CDs). At low fields (H), we observe the irreversible magnetization M-irr insensitive to the angle theta around H parallel to CDs. The field dependence of the angular range 2 theta(L) is proportional to 1/H, quite consistent with the expectation of the lock-in transition. This manifests the first observation of the fingerprint of the Bose glass phase in iron-based superconductors. C1 [Taen, Toshihiro; Yagyuda, Hidenori; Nakajima, Yasuyuki; Tamegai, Tsuyoshi] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Ayala-Valenzuela, Oscar; Civale, Leonardo; Maiorov, Boris] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Kambara, Tadashi] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Kanai, Yasuyuki] RIKEN, Atom Phys Lab, Wako, Saitama 3510198, Japan. RP Taen, T (reprint author), Univ Tokyo, Dept Appl Phys, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan. RI Kanai, Yasuyuki/A-2599-2009; OI Maiorov, Boris/0000-0003-1885-0436; Civale, Leonardo/0000-0003-0806-3113 FU MEXT in Japan; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX This work is partly supported by Grant-in-Aid for JSPS Fellows and a grant-in-aid from MEXT in Japan. Research at LANL was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 39 TC 2 Z9 2 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 22 PY 2014 VL 89 IS 2 AR 024508 DI 10.1103/PhysRevB.89.024508 PG 5 WC Physics, Condensed Matter SC Physics GA AC1AI UT WOS:000332226200003 ER PT J AU Yu, R Zhu, JX Si, QM AF Yu, Rong Zhu, Jian-Xin Si, Qimiao TI Orbital-selective superconductivity, gap anisotropy, and spin resonance excitations in a multiorbital t-J(1)-J(2) model for iron pnictides SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-SCATTERING; BA0.6K0.4FE2AS2; YBA2CU3O7 AB We study the orbital-selective superconducting pairing in a five-orbital t-J(1)-J(2) model for iron pnictides. Depending on the orbital selectivity of electron correlations and the orbital characters along the Fermi surface, the superconducting gap in an A(1g) pairing state may exhibit anisotropy. This anisotropy varies with the degree of J(1)-J(2) magnetic frustration. In the superconducting state, the frequency dependence of the dynamical spin susceptibility at the antiferromagnetic wave vector (pi, 0) shows a resonance, whose width is enhanced by the orbital selectivity of the superconducting gap. When the degree of the orbital selectivity is sufficiently strong, the resonance peak may be split in two. We discuss the implications of our results on the recent angle-resolved photoemission and neutron-scattering measurements in several superconducting iron pnictides. C1 [Yu, Rong] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Yu, Rong; Si, Qimiao] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Yu, R (reprint author), Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. RI Yu, Rong/H-3355-2016 FU NSF [DMR-1309531]; Robert A. Welch Foundation [C-1411]; National Science Foundation of China [11374361]; Alexander von Humboldt Foundation; National Nuclear Security Administration of the U.S. DOE at LANL [DE-AC52-06NA25396]; U.S. DOE Office of Basic Energy Sciences; Aspen Center for Physics (NSF) [1066293] FX We thank P. Dai, D. H. Lu, and C. L. Zhang for useful discussions. This work was supported in part by NSF Grant No. DMR-1309531, the Robert A. Welch Foundation Grant No. C-1411 (R.Y. & Q. S.), the National Science Foundation of China Grant No. 11374361 (R.Y.), the Alexander von Humboldt Foundation (Q. S.), and the National Nuclear Security Administration of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396 and the U.S. DOE Office of Basic Energy Sciences (J.X.Z.). One of us (Q. S.) acknowledges the hospitality of the Aspen Center for Physics (NSF Grant No. 1066293), the Institute of Physics of the Chinese Academy of Sciences, and the Karlsruhe Institute of Technology. NR 62 TC 19 Z9 19 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 22 PY 2014 VL 89 IS 2 AR 024509 DI 10.1103/PhysRevB.89.024509 PG 7 WC Physics, Condensed Matter SC Physics GA AC1AI UT WOS:000332226200004 ER PT J AU Mukherjee, S Thompson, LK Godin, S Schackwitz, W Lipzen, A Martin, J Blanchard, JL AF Mukherjee, Supratim Thompson, Lynmarie K. Godin, Stephen Schackwitz, Wendy Lipzen, Anna Martin, Joel Blanchard, Jeffrey L. TI Population Level Analysis of Evolved Mutations Underlying Improvements in Plant Hemicellulose and Cellulose Fermentation by Clostridium phytofermentans SO PLOS ONE LA English DT Article ID SOIL ORGANIC-MATTER; ESCHERICHIA-COLI; MALTOSE TRANSPORTER; ADAPTIVE EVOLUTION; LITTER DECOMPOSITION; MEMBRANE-COMPONENTS; CRYSTAL-STRUCTURE; ABC TRANSPORTERS; GENOME EVOLUTION; SYSTEMS AB Background: The complexity of plant cell walls creates many challenges for microbial decomposition. Clostridium phytofermentans, an anaerobic bacterium isolated from forest soil, directly breaks down and utilizes many plant cell wall carbohydrates. The objective of this research is to understand constraints on rates of plant decomposition by Clostridium phytofermentans and identify molecular mechanisms that may overcome these limitations. Results: Experimental evolution via repeated serial transfers during exponential growth was used to select for C. phytofermentans genotypes that grow more rapidly on cellobiose, cellulose and xylan. To identify the underlying mutations an average of 13,600,000 paired-end reads were generated per population resulting in,300 fold coverage of each site in the genome. Mutations with allele frequencies of 5% or greater could be identified with statistical confidence. Many mutations are in carbohydrate-related genes including the promoter regions of glycoside hydrolases and amino acid substitutions in ABC transport proteins involved in carbohydrate uptake, signal transduction sensors that detect specific carbohydrates, proteins that affect the export of extracellular enzymes, and regulators of unknown specificity. Structural modeling of the ABC transporter complex proteins suggests that mutations in these genes may alter the recognition of carbohydrates by substrate-binding proteins and communication between the intercellular face of the transmembrane and the ATPase binding proteins. Conclusions: Experimental evolution was effective in identifying molecular constraints on the rate of hemicellulose and cellulose fermentation and selected for putative gain of function mutations that do not typically appear in traditional molecular genetic screens. The results reveal new strategies for evolving and engineering microorganisms for faster growth on plant carbohydrates. C1 [Mukherjee, Supratim; Blanchard, Jeffrey L.] Univ Massachusetts, Dept Microbiol, Amherst, MA 01003 USA. [Thompson, Lynmarie K.] Univ Massachusetts, Dept Chem, Amherst, MA 01003 USA. [Godin, Stephen; Blanchard, Jeffrey L.] Univ Massachusetts, Dept Biol, Amherst, MA 01003 USA. [Schackwitz, Wendy; Lipzen, Anna; Martin, Joel] Joint Genome Inst, Walnut Creek, CA USA. RP Blanchard, JL (reprint author), Joint Genome Inst, Sci Programs, Walnut Creek, CA USA. EM jeffb@bio.umass.edu FU The Isenberg School of Management at the University of Massachusetts Amherst; National Science Foundation-sponsored Institute for Cellular Engineering IGERT Program [DGE-065412]; Life Sciences Junior Fellowship; Howard Hughes Medical Institute Award; The Department of Energy (DOE) Joint Genome Institute (JGI) FX This research was supported by a scholarship from The Isenberg School of Management at the University of Massachusetts Amherst to SM, a student training grant from National Science Foundation-sponsored Institute for Cellular Engineering IGERT Program (DGE-065412) to SM, a Life Sciences Junior Fellowship to SG, a Howard Hughes Medical Institute Award to SG, a Sponsored Research Agreement between Qteros Inc. and JB and a Community Sequencing Award from The Department of Energy (DOE) Joint Genome Institute (JGI) to JB. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 67 TC 5 Z9 5 U1 2 U2 22 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 22 PY 2014 VL 9 IS 1 AR e86731 DI 10.1371/journal.pone.0086731 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 297VL UT WOS:000330283100203 PM 24466216 ER PT J AU Piombino, P Genovese, A Esposito, S Moio, L Cutolo, PP Chambery, A Severino, V Moneta, E Smith, DP Owens, SM Gilbert, JA Ercolini, D AF Piombino, Paola Genovese, Alessandro Esposito, Silvia Moio, Luigi Cutolo, Pier Paolo Chambery, Angela Severino, Valeria Moneta, Elisabetta Smith, Daniel P. Owens, Sarah M. Gilbert, Jack A. Ercolini, Danilo TI Saliva from Obese Individuals Suppresses the Release of Aroma Compounds from Wine SO PLOS ONE LA English DT Article ID VITIS-VINIFERA L.; VOLATILE COMPOUNDS; RETRONASAL AROMA; OXIDATIVE STRESS; FLAVOR COMPOUNDS; FOOD-INTAKE; RED WINES; PERCEPTION; HABITUATION; MICROBIOTA AB Background: Recent evidence suggests that a lower extent of the retronasal aroma release correspond to a higher amount of ad libitum food intake. This has been regarded as one of the bases of behavioral choices towards food consumption in obese people. In this pilot study we investigated the hypothesis that saliva from obese individuals could be responsible for an alteration of the retro-nasal aroma release. We tested this hypothesis in vitro, by comparing the release of volatiles from a liquid food matrix (wine) after its interaction with saliva from 28 obese (O) and 28 normal-weight (N) individuals. Methods and Findings: Amplicon sequencing of the 16S rRNA V4 region indicated that Firmicutes and Actinobacteria were more abundant in O, while Proteobacteria and Fusobacteria dominated in N. Streptococcaceae were significantly more abundant in the O subjects and constituted 34% and 19% on average of the saliva microbiota of O and N subjects, respectively. The Total Antioxidant Capacity was higher in O vs N saliva samples. A model mouth system was used to test whether the in-mouth wine aroma release differs after the interaction with O or N saliva. In O samples, a 18% to 60% significant decrease in the mean concentration of wine volatiles was detected as a result of interaction with saliva, compared with N. This suppression was linked to biochemical differences in O and N saliva composition, which include protein content. Conclusion: Microbiological and biochemical differences were found in O vs N saliva samples. An impaired retronasal aroma release from white wine was detected in vitro and linked to compositional differences between saliva from obese and normal-weight subjects. Additional in vivo investigations on diverse food matrices could contribute to understanding whether a lower olfactory stimulation due to saliva composition can be a co-factor in the development/maintenance of obesity. C1 [Piombino, Paola; Genovese, Alessandro; Esposito, Silvia; Moio, Luigi; Ercolini, Danilo] Univ Naples Federico II, Dept Agr Sci, Portici, Italy. [Cutolo, Pier Paolo] S Giovanni Bosco Hosp, Gen & Laparoscop Surg Unit, Naples, Italy. [Chambery, Angela; Severino, Valeria] Univ Naples 2, Dept Environm Biol & Pharmaceut Sci & Technol, Caserta, Italy. [Chambery, Angela] IRCCS, Milan, Italy. [Moneta, Elisabetta] Agr Res Council, Res Ctr Food & Nutr, Rome, Italy. [Smith, Daniel P.; Owens, Sarah M.; Gilbert, Jack A.] Argonne Natl Lab, Argonne, IL 60439 USA. [Owens, Sarah M.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. RP Piombino, P (reprint author), Univ Naples Federico II, Dept Agr Sci, Portici, Italy. EM paola.piombino@unina.it RI Ercolini, Danilo/B-2431-2009; OI Ercolini, Danilo/0000-0003-3061-9560; Chambery, Angela/0000-0002-5136-0941 FU "Premio Montana alla Ricerca Alimentare 2010''; Italian Ministry of University and Research (MIUR) FX This study was supported by "Premio Montana alla Ricerca Alimentare 2010'' awarded to P. Piombino and D. Ercolini by Montana Alimentari S. p. A, Italy (www.montanafood.it). Microbiological investigations were partially supported by the Italian Ministry of University and Research (MIUR, programme PRIN 2010). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 63 TC 18 Z9 18 U1 3 U2 39 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 22 PY 2014 VL 9 IS 1 AR e85611 DI 10.1371/journal.pone.0085611 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 297VL UT WOS:000330283100052 PM 24465618 ER PT J AU Plank, H Noh, JH Fowlkes, JD Lester, K Lewis, BB Rack, PD AF Plank, Harald Noh, Joo Hyon Fowlkes, Jason D. Lester, Kevin Lewis, Brett B. Rack, Philip D. TI Electron-Beam-Assisted Oxygen Purification at Low Temperatures for Electron-Beam-Induced Pt Deposits: Towards Pure and High-Fidelity Nanostructures SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE focused electron-beam-induced deposition; platinum; nanofabrication; electron-stimulated reactions ID PLATINUM; PRECURSOR; FABRICATION; PT(PF3)(4); NANOTUBES; GOLD; RESOLUTION; DEVICES; PATTERN; GROWTH AB Nanoscale metal deposits written directly by electron-beam-induced deposition, or EBID, are typically contaminated because of the incomplete removal of the original organometallic precursor. This has greatly limited the applicability of EBID materials synthesis, constraining the otherwise powerful direct-write synthesis paradigm. We demonstrate a low-temperature purification method in which platinum-carbon nanostructures deposited from MeCpP-tIVMe(3) are purified by the presence of oxygen gas during a post-electron exposure treatment. Deposit thickness, oxygen pressure, and oxygen temperature studies suggest that the dominant mechanism is the electron-stimulated reaction of oxygen molecules adsorbed at the defective deposit surface. Notably, pure platinum deposits with low resistivity and retain the original deposit fidelity were accomplished at an oxygen temperature of only 50 degrees C. C1 [Plank, Harald] Graz Univ Technol, Inst Electron Microscopy & Nanoanalsis, A-8010 Graz, Austria. [Plank, Harald] Graz Univ Technol, Ctr Electron Microscopy, A-8010 Graz, Austria. [Noh, Joo Hyon; Fowlkes, Jason D.; Lester, Kevin; Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Noh, Joo Hyon; Lewis, Brett B.; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Rack, PD (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM prack@utk.edu OI Rack, Philip/0000-0002-9964-3254 FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Austrian Cooperative Research (ACR); Graz University of Technology in Austria; University of Tennessee Chancellor's Fellowship program; Semiconductor Research Corporation [SRC-2012-In-2310] FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. HP acknowledges the support from Prof. Ferdinand Hofer and the Austrian Cooperative Research (ACR) and the Graz University of Technology in Austria. BBL acknowledges support via the University of Tennessee Chancellor's Fellowship program. JN and HP acknowledge support from Semiconductor Research Corporation (SRC-2012-In-2310). The authors acknowledge Cheryl Hartfield at Omniprobe, Inc. (an Oxford Instruments Company) for assistance with the OmniGIS gas injection system. NR 53 TC 29 Z9 29 U1 3 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 22 PY 2014 VL 6 IS 2 BP 1018 EP 1024 DI 10.1021/am4045458 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 296RA UT WOS:000330201900039 PM 24377304 ER PT J AU Xu, ZL Wang, JB Zhang, K Zheng, H Dai, ZX Gui, JN Yang, XQ AF Xu, Zhongling Wang, Jianbo Zhang, Ke Zheng, He Dai, Zhong-Xu Gui, Jianian Yang, Xiao-Qing TI Nanoscale Lamellar Monoclinic Li2MnO3 Phase with Stacking Disordering in Lithium-Rich and Oxygen-Deficient Li1.07Mn1.93O4-delta Cathode Materials SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE phase transition; lithium manganese oxide; monoclinic; domain; oxygen vacancy; transmission electron microscopy; lithium-ion batteries ID X-RAY-DIFFRACTION; ION BATTERIES; LOCAL-STRUCTURE; ELECTRON-DIFFRACTION; MANGANESE OXIDES; STRUCTURAL-CHANGES; ELECTROCHEMICAL PROPERTIES; POWDER DIFFRACTION; SOLID-SOLUTION; 4 V AB The powdered crystalline samples of nominal composition Li1.07Mn1.93O4-delta have been investigated by transmission electron microscopy (TEM) combined with X-ray powder diffraction (XRD) at room temperature. As suggested by the TEM observation, the dominant phase of the particles is a cubic spinel Li1+aMn2-alpha O4-delta with space group Fd3m. A monoclinic Li2MnO3 phase with C2/m space group was also identified. Furthermore, the occurrence of nanoscale rotational twinning domains in Li2MnO3 with 120 degrees rotation angles, stacked along the [103](m)/[111](c) ("m" and "c" represent the monoclinic and cubic descriptions, respectively) axis was also observed. These nanoscale rotational twining domains are responsible for the pseudo-3-fold axis and their formation is supported by the superstructure reflections in selected-area electron-diffraction (SAED) patterns. Similar patterns were reported in the literature but may have been misinterpreted without the consideration of such domains. Consistent with the TEM observation, the XRD results reveal the increasing percentage of monoclinic Li2MnO3 with increasing annealing time, associated with more oxygen vacancies. In addition, the electron beam irradiation during TEM studies may cause the nucleation of nanoscale cubic spinel Li-Mn-O crystallites on the monoclinic Li2MnO3 grains. These results provide the detailed structural information about the Li1.07Mn1.93O4-delta samples and advance the understanding of corresponding electrochemical properties of this material as well as other layer structured cathode materials for lithium-ion batteries. C1 [Xu, Zhongling; Wang, Jianbo; Zhang, Ke; Zheng, He; Dai, Zhong-Xu; Gui, Jianian] Wuhan Univ, Ctr Electron Microscopy, Sch Phys & Technol, Wuhan 430072, Peoples R China. [Xu, Zhongling; Wang, Jianbo; Zhang, Ke; Zheng, He; Dai, Zhong-Xu; Gui, Jianian] Wuhan Univ, MOE Key Lab Artificial Micro & Nanostruct, Wuhan 430072, Peoples R China. [Yang, Xiao-Qing] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Wang, JB (reprint author), Wuhan Univ, Ctr Electron Microscopy, Sch Phys & Technol, Wuhan 430072, Peoples R China. EM wang@whu.edu.cn RI Zheng, He/E-2964-2012; Wang, Jianbo/D-9991-2011 OI Zheng, He/0000-0002-6476-8524; Wang, Jianbo/0000-0002-3315-3105 FU 973 Program [2011CB933300]; National Natural Science Foundation of China [51071110, 51271134, 40972044, J1210061]; China MOE NCET Program [NCET-07-0640]; MOE Doctoral Fund [20090141110059]; Fundamental Research Funds for the Central Universities; China Postdoctoral Science Foundation [2013M540602]; U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies [DEACO298CH10886] FX This work was supported by the 973 Program (2011CB933300), the National Natural Science Foundation of China (51071110, 51271134, 40972044, J1210061), the China MOE NCET Program (NCET-07-0640), MOE Doctoral Fund (20090141110059), the Fundamental Research Funds for the Central Universities, and the China Postdoctoral Science Foundation (2013M540602). The work was partially supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under Contract DEACO298CH10886. The authors wholeheartedly appreciate the guidance of the late professor Renhui Wang on this work. The authors gratefully acknowledge Prof. Gordon Tat lock from the University of Liverpool for his helpful comments and suggestions. NR 60 TC 8 Z9 8 U1 3 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 22 PY 2014 VL 6 IS 2 BP 1219 EP 1227 DI 10.1021/am404963u PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 296RA UT WOS:000330201900066 PM 24368018 ER PT J AU Wang, C Li, Q Wang, FF Xia, GF Liu, RQ Li, DY Li, N Spendelow, JS Wu, G AF Wang, Chen Li, Qing Wang, Fangfang Xia, Guofeng Liu, Ruiqing Li, Deyu Li, Ning Spendelow, Jacob S. Wu, Gang TI Morphology-Dependent Performance of CuO Anodes via Facile and Controllable Synthesis for Lithium-Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE copper oxide; morphology dependence; electrochemical performance; anode materials; lithium-ion batteries ID ELECTROCHEMICAL PERFORMANCE; HOLLOW MICRO/NANOSTRUCTURES; ENHANCED PERFORMANCE; NEGATIVE ELECTRODES; STORAGE PROPERTIES; MICROSPHERES; FABRICATION; FILM; NANOSTRUCTURES; STABILITY AB Nanostructured CuO anode materials with controllable morphologies have been successfully synthesized via a facile and environmentally friendly approach in the absence of any toxic surfactants or templates. In particular, leaf-like CuO, oatmeal-like CuO, and hollow-spherical CuO were obtained by changing the ligand agents. The structures and electrochemical performance of these as-prepared CuO were fully characterized by various techniques, and the properties were found to be strongly dependent on morphology. As anode materials for lithium-ion batteries, the leaf-like CuO and oatmeal-like CuO electrodes exhibit relatively high reversible capacities, whereas hollow-spherical CuO shows enhanced reversible capacity after initial degradation. Furthermore, an excellent high rate capability was obtained for the leaf-like CuO and hollow-spherical CuO electrodes. These results may provide valuable insights for the development of nanostructured anodes for next-generation high-performance lithium-ion batteries. C1 [Wang, Chen; Wang, Fangfang; Xia, Guofeng; Liu, Ruiqing; Li, Deyu; Li, Ning] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. [Li, Qing; Spendelow, Jacob S.; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, N (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. EM lininghit@263.net; wugang@lanl.gov RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program [20110483ER] FX Financial support from the Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program (20110483ER) for this work is gratefully acknowledged. NR 45 TC 55 Z9 55 U1 5 U2 109 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 22 PY 2014 VL 6 IS 2 BP 1243 EP 1250 DI 10.1021/am405061c PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 296RA UT WOS:000330201900069 PM 24377276 ER PT J AU Li, M Li, D O'Keeffe, M Yaghi, OM AF Li, Mian Li, Dan O'Keeffe, Michael Yaghi, Omar M. TI Topological Analysis of Metal-Organic Frameworks with Polytopic Linkers and/or Multiple Building Units and the Minimal Transitivity Principle SO CHEMICAL REVIEWS LA English DT Review ID SELECTIVE CO2 CAPTURE; HIGH H-2 ADSORPTION; NON-CRYSTALLOGRAPHIC NETS; HIGH METHANE UPTAKE; HIGH-SURFACE-AREA; COORDINATION POLYMERS; MAGNETIC-PROPERTIES; CRYSTAL-STRUCTURES; HYDROGEN STORAGE; ROOM-TEMPERATURE C1 [Li, Mian; Li, Dan] Shantou Univ, Dept Chem, Shantou 515063, Guangdong, Peoples R China. [O'Keeffe, Michael] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [O'Keeffe, Michael; Yaghi, Omar M.] Korea Adv Inst Sci & Technol, Grad Sch EEWS WCU, Taejon 305701, South Korea. [Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP O'Keeffe, M (reprint author), Shantou Univ, Dept Chem, Shantou 515063, Guangdong, Peoples R China. EM mokeeffe@asu.edu RI Li, Dan/F-2708-2014; OI Yaghi, Omar/0000-0002-5611-3325; Li, Mian/0000-0003-1293-3636 FU World Class University program [R-31-2008-000-10055-0]; U.S. National Science Foundation [DMR 1104798]; National Basic Research Program of China (973 Program) [2012CB821706]; National Natural Science Foundation of China [91222202, 21171114] FX M.O'K. is supported by the World Class University program (R-31-2008-000-10055-0) and by the U.S. National Science Foundation (grant DMR 1104798). He also acknowledges helpful correspondence about the structures of TCNQ-based salts with Kim Dunbar and Zhongyue Zhang. D.L. is supported by the National Basic Research Program of China (973 Program, 2012CB821706) and the National Natural Science Foundation of China (91222202 and 21171114). NR 166 TC 358 Z9 361 U1 49 U2 361 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JAN 22 PY 2014 VL 114 IS 2 BP 1343 EP 1370 DI 10.1021/cr400392k PG 28 WC Chemistry, Multidisciplinary SC Chemistry GA 296RX UT WOS:000330204200012 PM 24191753 ER PT J AU Zhang, GH Yi, H Zhang, GT Deng, Y Bai, RP Zhang, H Miller, JT Kropf, AJ Bunel, EE Lei, AW AF Zhang, Guanghui Yi, Hong Zhang, Guoting Deng, Yi Bai, Ruopeng Zhang, Heng Miller, Jeffrey T. Kropf, Arthur J. Bunel, Emilio E. Lei, Aiwen TI Direct Observation of Reduction of Cu(II) to Cu(I) by Terminal Alkynes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID COUPLING REACTIONS; ORGANIC-CHEMISTRY; COPPER; COMPLEXES; MECHANISM; ARYLATION; CATALYSIS AB X-ray absorption spectroscopy and in situ electron paramagnetic resonance evidence were provided for the reduction of Cu(II) to Cu(I) species by alkynes in the presence of tetramethylethylenediamine (TMEDA), in which TMEDA plays dual roles as both ligand and base. The structures of the starting Cu(II) species and the obtained Cu(I) species were determined as (TMEDA)CuCl2 and [(TMEDA)CuCl], dimer, respectively. C1 [Zhang, Guanghui; Yi, Hong; Zhang, Guoting; Deng, Yi; Bai, Ruopeng; Zhang, Heng; Lei, Aiwen] Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China. [Zhang, Guanghui; Miller, Jeffrey T.; Kropf, Arthur J.; Bunel, Emilio E.; Lei, Aiwen] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Lei, AW (reprint author), Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China. EM aiwenlei@whu.edu.cn RI ID, MRCAT/G-7586-2011; Zhang, Guanghui/C-4747-2008; OI Zhang, Guanghui/0000-0002-5854-6909; Lei, Aiwen/0000-0001-8417-3061; Bai, Ruopeng/0000-0002-1097-8526 FU "973" Program [2012CB725302]; National Natural Science Foundation of China [21025206, 21272180]; Fundamental Research Funds for the Central Universities; Program for New Century Excellent Talents in University (NCET); Research Fund for the Doctoral Program of Higher Education of China [20120141130002]; Program for Changjiang Scholars and Innovative Research Team in University [IRT1030]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Chemical Sciences, Geosciences and Bioscience Division, U.S. Department of Energy [DE-AC0-06CH11357]; Chemical Sciences and Engineering Division, Argonne National Laboratory FX This work was supported by the "973" Program (2012CB725302) and the National Natural Science Foundation of China (21025206, 21272180). The authors also thank the support from "the Fundamental Research Funds for the Central Universities", Program for New Century Excellent Talents in University (NCET), the Research Fund for the Doctoral Program of Higher Education of China (20120141130002) and Program for Changjiang Scholars and Innovative Research Team in University (IRT1030). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Partial funding for J.T.M. was provided by the Chemical Sciences, Geosciences and Bioscience Division, U.S. Department of Energy, under Contract No. DE-AC0-06CH11357. This work was also funded by the Chemical Sciences and Engineering Division, Argonne National Laboratory. NR 28 TC 50 Z9 50 U1 10 U2 133 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 22 PY 2014 VL 136 IS 3 BP 924 EP 926 DI 10.1021/ja410756b PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 296RE UT WOS:000330202300027 PM 24392805 ER PT J AU Mayes, HB Broadbelt, LJ Beckham, GT AF Mayes, Heather B. Broadbelt, Linda J. Beckham, Gregg T. TI How Sugars Pucker: Electronic Structure Calculations Map the Kinetic Landscape of Five Biologically Paramount Monosaccharides and Their Implications for Enzymatic Catalysis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MOLECULAR-ORBITAL METHODS; ALPHA-GLUCOSIDASE INHIBITOR; FREE-ENERGY LANDSCAPE; DENSITY FUNCTIONALS; BASIS-SETS; REACTION COORDINATE; BETA-XYLOSIDASE; GEOBACILLUS-STEAROTHERMOPHILUS; NONCOVALENT INTERACTIONS; LIKELIHOOD MAXIMIZATION AB Glycoside hydrolases (GHs) distort carbohydrate ring geometry along particular "catalytic itineraries" during the cleavage of glycosidic bonds, illustrating. the relationship between substrate conformation and reactivity. Previous theoretical studies of thermodynamics of isolated monosaccharides offer insights into the catalytic itineraries of particular sugars. However, kinetic accessibility of carbohydrate puckering conformations and the role of exocyclic groups have not yet been thoroughly addressed. Here we present the first complete library of low-energy local minima and puckering interconversion transition states for five biologically relevant pyranose sugars: beta-xylose, beta-mannose, alpha-glucose, beta-glucose, and beta-N-acetylglucosamine. These were obtained by a thorough theoretical investigation each of the 38 IUPAC designated puckering geometries and all possible conformations of the exocyclic groups. These calculations demonstrate that exocyclic groups must be explicitly considered when examining these interconversion pathways. Furthermore, these data enable evaluation of previous hypotheses of why enzymes perturb ring geometries from the low-energy equatorial chair (C-4(1)) conformation. They show that the relative thermodynamics alone do not universally correlate with GH catalytic itineraries. For some sugars, particular puckers offer both catalytically favorable electronic structure properties, such as anomeric carbon partial charge, and low kinetic barriers to achieve a given puckering conformation. However, different factors correlate with catalytic itineraries for other sugars; for beta-N-acetylglucosamine, the key N-acetyl arm confounds the puckering landscape and appears to be the crucial factor. Overall, this study reveals a more comprehensive understanding of why particular puckering geometries are favored in carbohydrate catalysis concomitant with the complexity of glycobiology. C1 [Mayes, Heather B.; Broadbelt, Linda J.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Mayes, Heather B.; Beckham, Gregg T.] Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Beckham, GT (reprint author), Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. EM gregg.beckham@nrel.gov RI Broadbelt, Linda/B-7640-2009; Mayes, Heather/D-8755-2016 OI Mayes, Heather/0000-0001-9373-0106 FU DOE Computational Science Graduate Fellowship (CSGF) [DEFG02-97ER25308]; Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) through the BioEnergy Technologies Office [DE-EE0003044]; NREL Laboratory Directed Research and Development Program; DOE Office of EERE [DE-AC36-08GO28308]; National Energy Research Scientific Computing Center; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; San Diego Supercomputing Center (SDSC) SDSC under the NSF XSEDE [MCB090159]; ARCS Foundation Inc., Chicago Chapter FX This work was supported by the DOE Computational Science Graduate Fellowship (CSGF) which is provided under Grant No. DEFG02-97ER25308 and the Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) through the BioEnergy Technologies Office, Grant No. DE-EE0003044. G.T.B. also acknowledges the NREL Laboratory Directed Research and Development Program for funding. This research used resources of the following: the NREL Computational Sciences Center supported by the DOE Office of EERE under Contract No. DE-AC36-08GO28308; the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231; and the San Diego Supercomputing Center (SDSC) SDSC under the NSF XSEDE Grant MCB090159. H.B.M. is also supported by an award from the ARCS Foundation Inc., Chicago Chapter. The authors would like to thank Fernando R. Clemente, George R Schatz, Jared M. Clark, Christina M. Payne, Joshua V. Vermaas, and Michael F. Crowley for helpful discussions. The authors also thank Chris Mayes for helpful scripts, available to the public at https://github.com/cmayes. NR 101 TC 35 Z9 35 U1 5 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 22 PY 2014 VL 136 IS 3 BP 1008 EP 1022 DI 10.1021/ja410264d PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA 296RE UT WOS:000330202300037 PM 24368073 ER PT J AU Mehta, VS Maillot, F Wang, ZM Catalano, JG Giammar, DE AF Mehta, Vrajesh S. Maillot, Fabien Wang, Zheming Catalano, Jeffrey G. Giammar, Daniel E. TI Effect of co-solutes on the products and solubility of uranium( VI) precipitated with phosphate SO CHEMICAL GEOLOGY LA English DT Article DE Uranium; Phosphate; In situ immobilization; Environmental remediation; Autunite ID CONTAMINATED HANFORD SEDIMENTS; SULFATE-REDUCING CONDITIONS; META-AUTUNITE; VADOSE ZONE; SUBSURFACE MEDIA; DISSOLVED-OXYGEN; U(VI) REDUCTION; URANYL; REOXIDATION; IMMOBILIZATION AB Uranyl phosphate solids are often found with uranium ores, and their low solubility makes them promising target phases for in situ remediation of uranium-contaminated subsurface environments. The products and solubility of uranium(VI) precipitated with phosphate can be affected by the pH, dissolved inorganic carbon (DIC) concentration, and co-solute composition (e.g. Na+/Ca2+) of the groundwater. Batch experiments were performed to study the effect of these parameters on the products and extent of uranium precipitation induced by phosphate addition. In the absence of co-solute cations, chernikovite [ H3O(UO2)(PO4) center dot 3H(2)O] precipitated despite uranyl orthophosphate [(UO2)(3)(PO4)2 center dot 4H(2)O] being thermodynamically more favorable under certain conditions. As determined using powder X-ray diffraction, electron microscopy, and laser induced fluorescence spectroscopy, the presence of Na+ or Ca2+ as a co-solute led to the precipitation of sodium autunite ([Na-2(UO2)(2)(PO4)(2)] and autunite [Ca(UO2)(2)(PO4)(2)]), which are structurally similar to chernikovite. In the presence of sodium, the dissolved U(VI) concentrations were generally in agreement with equilibrium predictions of sodium autunite solubility. However, in the calcium-containing systems, the observed concentrations were below the predicted solubility of autunite, suggesting the possibility of uranium adsorption to or incorporation in a calcium phosphate precipitate in addition to the precipitation of autunite. (C) 2013 Elsevier B.V. All rights reserved. C1 [Mehta, Vrajesh S.; Giammar, Daniel E.] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. [Maillot, Fabien; Catalano, Jeffrey G.] Washington Univ, Dept Earth & Planetary Sci, St Louis, MO 63130 USA. [Wang, Zheming] Pacific NW Natl Lab, Dept Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Giammar, DE (reprint author), 1 Brookings Dr,Campus Box 1180, St Louis, MO 63130 USA. EM giammar@wustl.edu RI Catalano, Jeffrey/A-8322-2013; Wang, Zheming/E-8244-2010 OI Catalano, Jeffrey/0000-0001-9311-977X; Wang, Zheming/0000-0002-1986-4357 FU U. S. Department of Energy (DOE) Subsurface Biogeochemical Research Program [DE-SC0006857]; Battelle Memorial Institute [DE-AC06-76RLO-1830] FX We are grateful to the McDonnell International Scholars Academy at Washington University for providing the Ameren corporate fellowship for Vrajesh Mehta. This work was supported by the U. S. Department of Energy (DOE) Subsurface Biogeochemical Research Program (Award No. DE-SC0006857). LIFS measurements were performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory. PNNL is operated for DOE by Battelle Memorial Institute under Contract # DE-AC06-76RLO-1830. The comments and suggestions of Co-Editorin-Chief Jeremy Fein and two anonymous reviewers were helpful for improving an earlier version of this manuscript. NR 72 TC 16 Z9 16 U1 4 U2 61 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD JAN 22 PY 2014 VL 364 BP 66 EP 75 DI 10.1016/j.chemgeo.2013.12.002 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 285QV UT WOS:000329409600007 ER PT J AU Chudo, H Koutroulakis, G Yasuoka, H Bauer, ED Tobash, PH Mitchell, JN Thompson, JD AF Chudo, H. Koutroulakis, G. Yasuoka, H. Bauer, E. D. Tobash, P. H. Mitchell, J. N. Thompson, J. D. TI Weak itinerant antiferromagnetism in PuIn3 explored using In-115 nuclear quadrupole resonance SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID MAGNETIC RELAXATION; LATTICE; CEIN3 AB The results of In-115 nuclear quadrupole resonance (NQR) measurements on PuIn3 are reported. Three of the four NQR lines of In-115 expected for nuclear spin I = 9/2 are observed. The equal spacing of these lines at 20 K yields the NQR frequency of nu(Q) = 10.45 MHz, and the asymmetry parameter of the electric field gradient eta = 0. The NQR line profile and the nuclear spin-lattice relaxation rate 1/T-1 display an abrupt change at 14 K, which is associated with the onset of long-range antiferromagnetic order. The temperature dependences of the staggered magnetization M-Q(T), extracted from the NQR spectra, and 1/T-1 below T-N = 14 K are well explained by the self-consistent renormalization (SCR) theory for spin fluctuations. In addition, the scaling between T1T and M-Q(T)/M-Q(0) is also consistent with the predictions of SCR theory, providing further evidence that PuIn3 is a weak itinerant antiferromagnet in which spin fluctuations around the antiferromagnetic wavevector play a major role in the system's behavior at finite temperatures. C1 [Chudo, H.; Koutroulakis, G.; Yasuoka, H.; Bauer, E. D.; Tobash, P. H.; Mitchell, J. N.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Yasuoka, H.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. RP Chudo, H (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM chudo.hiroyuki@jaea.go.jp RI Mitchell, Jeremy/E-2875-2010 OI Mitchell, Jeremy/0000-0001-7109-3505 FU Glenn T Seaborg Institute; Los Alamos Laboratory Directed Research and Development (LDRD) program; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; LANL LDRD program FX We thank Professor H Harima for valuable discussions on the band structure and electric field gradient in Pu-based metallic compounds. H Yasuoka and G Koutroulakis thank the Glenn T Seaborg Institute and the Los Alamos Laboratory Directed Research and Development (LDRD) program for financial support. Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, and supported in part by the LANL LDRD program. NR 20 TC 3 Z9 3 U1 3 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 22 PY 2014 VL 26 IS 3 AR 036001 DI 10.1088/0953-8984/26/3/036001 PG 5 WC Physics, Condensed Matter SC Physics GA 287EX UT WOS:000329525500018 PM 24334529 ER PT J AU Lashley, JC Gofryk, K Mihaila, B Smith, JL Salje, EKH AF Lashley, J. C. Gofryk, K. Mihaila, B. Smith, J. L. Salje, E. K. H. TI Thermal avalanches near a Mott transition SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID ALLOYING ADDITIONS; CERIUM; TRANSFORMATION; BEHAVIOR AB We probe the volume collapse transition (Delta V=V-o similar to 15%) between the isostructural gamma and alpha phases (T similar to 100 K) of Ce0.9Th0.1 using the Hall effect, three-terminal capacitive dilatometry, and electrical resistivity measurements. Hall effect measurements confirm the itinerant ground state as the carrier concentration increases by a factor of 7 in the alpha phase, gamma phase (n(H) = 5.28 x 10(26) m(-3)), and the alpha phase (n(H) = 3.76 x 10(27) m(-3)). We were able to detect a noise spectrum consisting of avalanches while slowly varying the temperature through the hysteretic region. We surmise that the avalanches originate from intergranular stresses at the interfaces between partially transformed high-volume and low-volume phases. The statistical distribution of avalanches obey power laws with energy exponent epsilon similar or equal to 1.5. Hall effect measurements, combined with universal critical exponents, point to short electron mean-free percolation pathways and carrier localization at phase interfaces. Carrier localization was predicted many years ago for elemental cerium by Johansson (1974 Phil. Mag. 30 469). C1 [Lashley, J. C.; Gofryk, K.; Mihaila, B.; Smith, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Salje, E. K. H.] Univ Cambridge, Dept Earth Sci, Cambridge CB2 3EQ, England. RP Lashley, JC (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM J.lash@lanl.gov RI Gofryk, Krzysztof/F-8755-2014; Mihaila, Bogdan/D-8795-2013; OI Mihaila, Bogdan/0000-0002-1489-8814; Gofryk, Krzysztof/0000-0002-8681-6857 FU United States Department of Energy; Liverhulme Foundation [RG66640]; EPSRC [RG66344] FX Work at Los Alamos National Laboratory was performed under the auspices of the United States Department of Energy. E K H Salje thanks the Liverhulme Foundation (RG66640) and EPSRC (RG66344) for financial support. NR 29 TC 2 Z9 2 U1 4 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 22 PY 2014 VL 26 IS 3 AR 035701 DI 10.1088/0953-8984/26/3/035701 PG 4 WC Physics, Condensed Matter SC Physics GA 287EX UT WOS:000329525500016 PM 24351548 ER PT J AU Mitra, C Fishman, RS Okamoto, S Lee, HN Reboredo, FA AF Mitra, Chandrima Fishman, Randy S. Okamoto, Satoshi Lee, Ho Nyung Reboredo, Fernando A. TI Ground-state and spin-wave dynamics in Brownmillerite SrCoO2.5-a combined hybrid functional and LSDA plus U study SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE magnetism; electronic structure; spin-wave ID OXIDE; PEROVSKITES AB We theoretically investigate the ground-state magnetic properties of the brownmillerite phase of SrCoO2.5. Strong correlations between Co d electrons are treated within the local spin density approximations of density functional theory (DFT) with Hubbard U corrections (LSDA + U), and results are compared with those using the Heyd-Scuseria-Ernzerhof (HSE) functional. The parameters computed with a U value of 7.5 eV are found to match closely to those computed within the HSE functional. A G-type antiferromagnetic structure is found to be the most stable one, consistent with experimental observation. By mapping the total energies of different magnetic configurations onto a Heisenberg Hamiltonian, we compute the magnetic exchange interaction parameters, J, between the nearest-neighbor Co atoms. The J values obtained are then used to compute the spin-wave frequencies and inelastic neutron scattering intensities. Among four spin-wave branches, the lowest energy mode was found to have the largest scattering intensity at the magnetic zone center, while the other modes become dominant at different momenta. These predictions can be tested experimentally. C1 [Mitra, Chandrima; Fishman, Randy S.; Okamoto, Satoshi; Lee, Ho Nyung; Reboredo, Fernando A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Mitra, C (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM mhc@ornl.gov RI Okamoto, Satoshi/G-5390-2011; Lee, Ho Nyung/K-2820-2012 OI Okamoto, Satoshi/0000-0002-0493-7568; Lee, Ho Nyung/0000-0002-2180-3975 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 27 TC 4 Z9 4 U1 2 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 22 PY 2014 VL 26 IS 3 AR 036004 DI 10.1088/0953-8984/26/3/036004 PG 7 WC Physics, Condensed Matter SC Physics GA 287EX UT WOS:000329525500021 PM 24355828 ER PT J AU Richard, P Capan, C Ma, J Zhang, P Xu, N Tian, T Denlinger, JD Chen, GF Sefat, AS Fisk, Z Ding, H AF Richard, P. Capan, C. Ma, J. Zhang, P. Xu, N. Tian, T. Denlinger, J. D. Chen, G-F Sefat, A. S. Fisk, Z. Ding, H. TI Angle-resolved photoemission spectroscopy observation of anomalous electronic states in EuFe2As2-xPx SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE Fe-based superconductors; ARPES; EuFe2P2; electronic structure ID MAGNETIC-PROPERTIES AB We used angle-resolved photoemission spectroscopy to investigate the electronic structure and the Fermi surface of EuFe2As2, EuFe2As1.4P0.6 and EuFe2P2. We observed doubled core level peaks associated with the pnictide atoms. Using K atoms evaporated at the surface to affect the surface quality, we show that one component of these doubled peaks is related to a surface state. Nevertheless, strong electronic dispersion along the c-axis, especially pronounced in EuFe2P2, is observed for at least one band, thus indicating that the Fe states, albeit probably affected at the surface, do not form pure two-dimensional surface states. We determine the evolution of the Fermi surface as a function of the P content and reveal that the hole Fermi surface pockets enlarge with increasing P content. We also show that the spectral weight near the Fermi level of EuFe2P2 is reduced as compared to that of EuFe2As2 and EuFe2As1.4P0.6. Finally, we identify the electronic states associated with the Eu2+ f states and show an anomalous jump in EuFe2P2. C1 [Richard, P.; Ma, J.; Zhang, P.; Xu, N.; Tian, T.; Chen, G-F; Ding, H.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Richard, P.; Ma, J.; Zhang, P.; Xu, N.; Tian, T.; Chen, G-F; Ding, H.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Richard, P.; Ding, H.] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. [Capan, C.; Fisk, Z.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Capan, C.] Washington State Univ, Dept Phys, Pullman, WA 99164 USA. [Xu, N.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Denlinger, J. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Sefat, A. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Richard, P (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM p.richard@iphy.ac.cn RI Richard, Pierre/F-7652-2010; Xu, Nan/N-3728-2016; Sefat, Athena/R-5457-2016 OI Richard, Pierre/0000-0003-0544-4551; Xu, Nan/0000-0001-6739-3468; Sefat, Athena/0000-0002-5596-3504 FU CAS [2010Y1JB6]; MOST [2010CB923000, 2011CBA001000, 2011CBA00102, 2012CB821403, 2013CB921703]; NSFC, China [11004232, 11034011/A0402, 11274362]; University of Wisconsin-Madison; University of Wisconsin-Milwaukee; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH112]; Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We acknowledge M Shi, E Razolli and J-X Yin for useful discussions. This work was supported by grants from CAS (2010Y1JB6), MOST (2010CB923000, 2011CBA001000, 2011CBA00102, 2012CB821403 and 2013CB921703) and NSFC (11004232, 11034011/A0402 and 11274362) from China. This work is based in part on research conducted at the Synchrotron Radiation Center, which is primarily funded by the University of Wisconsin-Madison with supplemental support from facility users and the University of Wisconsin-Milwaukee. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH112. The work at ORNL was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 39 TC 6 Z9 6 U1 3 U2 43 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 22 PY 2014 VL 26 IS 3 AR 035702 DI 10.1088/0953-8984/26/3/035702 PG 8 WC Physics, Condensed Matter SC Physics GA 287EX UT WOS:000329525500017 PM 24351570 ER PT J AU Wu, SQ Ji, M Wang, CZ Nguyen, MC Zhao, X Umemoto, K Wentzcovitch, RM Ho, KM AF Wu, S. Q. Ji, M. Wang, C. Z. Nguyen, M. C. Zhao, X. Umemoto, K. Wentzcovitch, R. M. Ho, K. M. TI An adaptive genetic algorithm for crystal structure prediction SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID TOTAL-ENERGY CALCULATIONS; POST-PEROVSKITE PHASE; WAVE BASIS-SET; AB-INITIO DATA; EFFECTIVE POTENTIALS; HIGH-PRESSURE; MGSIO3; OPTIMIZATION; MGO; DISSOCIATION AB We present a genetic algorithm (GA) for structural search that combines the speed of structure exploration by classical potentials with the accuracy of density functional theory (DFT) calculations in an adaptive and iterative way. This strategy increases the efficiency of the DFT-based GA by several orders of magnitude. This gain allows a considerable increase in the size and complexity of systems that can be studied by first principles. The performance of the method is illustrated by successful structure identifications of complex binary and ternary intermetallic compounds with 36 and 54 atoms per cell, respectively. The discovery of a multi-TPa Mg-silicate phase with unit cell containing up to 56 atoms is also reported. Such a phase is likely to be an essential component of terrestrial exoplanetary mantles. C1 [Wu, S. Q.] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Wu, S. Q.; Ji, M.; Wang, C. Z.; Nguyen, M. C.; Zhao, X.; Umemoto, K.; Ho, K. M.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Wu, S. Q.; Ji, M.; Wang, C. Z.; Nguyen, M. C.; Zhao, X.; Umemoto, K.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Umemoto, K.] Univ Minnesota, Dept Earth Sci, Minneapolis, MN 55455 USA. [Wentzcovitch, R. M.] Univ Minnesota, Minnesota Supercomp Inst, Minneapolis, MN 55455 USA. [Wentzcovitch, R. M.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. RP Wu, SQ (reprint author), Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. EM wangcz@ameslab.gov; kmh@ameslab.gov RI Wu, S.Q./G-3992-2010; Nguyen, Manh Cuong/G-2783-2015; Wentzcovitch, Renata/J-8768-2015; OI Wu, S.Q./0000-0002-2545-0054; Nguyen, Manh Cuong/0000-0001-8027-9029; Zhao, Xin/0000-0002-3580-512X FU US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; NSF/EAR [1047629]; National Natural Science Foundation of China [11004165] FX Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Centre (NERSC) in Berkeley, CA. Work at the University of Minnesota was supported by NSF/EAR 1047629. Computations were performed at the Minnesota Supercomputing Institute and at the Laboratory for Scientific Computing and Engineering. SQW also acknowledges financial support from the National Natural Science Foundation of China (No. 11004165). NR 37 TC 23 Z9 24 U1 7 U2 73 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 22 PY 2014 VL 26 IS 3 AR 035402 DI 10.1088/0953-8984/26/3/035402 PG 6 WC Physics, Condensed Matter SC Physics GA 287EX UT WOS:000329525500010 PM 24351274 ER PT J AU Siemons, W Beekman, C MacDougall, GJ Zarestky, JL Nagler, SE Christen, HM AF Siemons, W. Beekman, C. MacDougall, G. J. Zarestky, J. L. Nagler, S. E. Christen, H. M. TI A complete strain-temperature phase diagram for BiFeO3 films on SrTiO3 and LaAlO3 (001) substrates SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID THIN-FILMS; STABILIZATION; TRANSITION; MECHANISM AB BiFeO3 has a complex phase diagram as function of both strain and temperature, undergoing a morphotropic phase transformation under large compressive strain. Epitaxial films, grown by pulsed laser deposition, are ideal for the study of the intricate phase coexistence between multiple polymporphs. Three polymorphs have been identified in the literature. They are carefully described in this paper (labelled R', T', and S'). As both ferroelectric and magnetic properties are typically strongly linked to structural distortions, the structural, ferroelectric and magnetic transition temperatures are expected to differ between the R', T' and S' polymorphs. In this paper we present a complete strain-temperature phase diagram for each of the polymorphs. C1 [Siemons, W.; Beekman, C.; Christen, H. M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [MacDougall, G. J.; Nagler, S. E.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [MacDougall, G. J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [MacDougall, G. J.] Univ Illinois, Federick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Zarestky, J. L.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Zarestky, J. L.] Iowa State Univ, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Nagler, S. E.] Univ Tennessee, CIRE, Knoxville, TN 37996 USA. RP Siemons, W (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM christenhm@ornl.gov RI Nagler, Stephen/E-4908-2010; Christen, Hans/H-6551-2013; OI Nagler, Stephen/0000-0002-7234-2339; Christen, Hans/0000-0001-8187-7469; MacDougall, Gregory/0000-0002-7490-9650 FU US Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division; Scientific User Facilities Division, BES, DOE FX Research supported by the US Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division (WS, CB, JLZ, HMC). The research at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, BES, DOE (GJM, SEN). NR 32 TC 7 Z9 7 U1 8 U2 60 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD JAN 22 PY 2014 VL 47 IS 3 SI SI AR 034011 DI 10.1088/0022-3727/47/3/034011 PG 5 WC Physics, Applied SC Physics GA 281QL UT WOS:000329116000012 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Aimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asmana, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, SW Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazeka, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brost, E Brown, G Brown, J de Renstrom, PAB 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[Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Huang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. 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[Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Goncalves Pinto Firmino Da Costa, J.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Monig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Bunse, M.; Esch, H.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Pasztor, G.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goshaw, A. T.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettinia, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, INFN, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, H Phys Inst, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Monnier, E.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, H Phys Inst, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gorini, B.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN, Sez Lecce, Lecce, Italy. [Bianco, M.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buscher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, P.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favaretoa, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncona, C.; Turra, R.; Volpini, G.] Univ Milan, INFN, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favaretoa, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; della Volpe, D.; Donato, C. Di; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Donato, C. Di; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Marshall, Z.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Ist Nazl Fis Nucl, Sez Pisa, I-56100 Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillip, P. W.; Sanchez, A.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN, Sez Roma 1, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, INFN, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Univ Roma Tre, INFN, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gorisek, A.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Gornicki, E.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondamentales Univ, DSM IRFU, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goessling, C.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazeka, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asmana, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Gorini, E.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Trieste, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Edmonton, AB, Canada. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, P-1200 Lisbon, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, P-1200 Lisbon, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow MV Lomonosov State Univ, Inst Phys & Technol, Dolgoprudnyi, Russia. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Nessi, M.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Peters, R. F. Y.] DESY, Zeuthen, Germany. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Joergensen, Morten/E-6847-2015; Mitsou, Vasiliki/D-1967-2009; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Smirnova, Oxana/A-4401-2013; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; White, Ryan/E-2979-2015; Gladilin, Leonid/B-5226-2011; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Staroba, Pavel/G-8850-2014; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Della Pietra, Massimo/J-5008-2012; Negrini, Matteo/C-8906-2014; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015 OI Joergensen, Morten/0000-0002-6790-9361; Mitsou, Vasiliki/0000-0002-1533-8886; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Smirnova, Oxana/0000-0003-2517-531X; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Gladilin, Leonid/0000-0001-9422-8636; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Pacheco Pages, Andres/0000-0001-8210-1734; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Petrucci, Fabrizio/0000-0002-5278-2206; Della Pietra, Massimo/0000-0003-4446-3368; Negrini, Matteo/0000-0003-0101-6963; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808 NR 1 TC 2 Z9 2 U1 7 U2 52 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 21 PY 2014 IS 1 AR 109 DI 10.1007/JHEP01(2014)109 PG 18 WC Physics, Particles & Fields SC Physics GA AW4GD UT WOS:000346238300003 ER PT J AU Curry, JJ Estupinan, EG Lapatovich, WP Henins, A Shastri, SD Hardis, JE Gibbs, JM AF Curry, J. J. Estupinan, E. G. Lapatovich, W. P. Henins, A. Shastri, S. D. Hardis, J. E. Gibbs, J. M. TI Study of CeI3 evaporation in the presence of group 13 metal-iodides SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID VAPORS AB The influences of GaI3, InI, and TlI on the evaporation characteristics of CeI3 have been studied over the temperature range 900K to 1400K using x-ray induced fluorescence. The total vapor densities, summed over all atomic and molecular species, of Ce, I, In, and Tl were obtained. Measurements of Ce were limited to temperatures above 1033 K, the melting temperature of CeI3. This is the highest temperature range for which measurements of the vapor pressure of CeI3 have been made. The vapor pressure of the CeI3 monomer above the pure CeI3 salt for temperatures exceeding its melting point can be approximated by log(10)p/Pa = 11.24(+/- 0.03) - 10, 690(+/- 40) (T/K)(-1) where the numbers in parentheses are standard uncertainties. InI and TlI were shown to modestly enhance the presence of Ce in the vapor phase, up to a factor of 5. GaI3 produced no enhancement in this temperature range. Numerical simulations of the thermochemical equilibrium suggest the importance of both liquid-phase and vapor-phase complexes. Significant improvement to the method of absolute calibration is discussed. C1 [Curry, J. J.; Lapatovich, W. P.; Henins, A.; Hardis, J. E.] NIST, Gaithersburg, MD 20899 USA. [Estupinan, E. G.; Gibbs, J. M.] OSRAM SYLVANIA Inc, Beverly, MA 01915 USA. [Shastri, S. D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Henins, A.] Henins Enterprises, Gaithersburg, MD 20886 USA. RP Curry, JJ (reprint author), NIST, 100 Bur Dr, Gaithersburg, MD 20899 USA. EM jjcurry@nist.gov FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Ali Mashayekhi and Roger Ranay of the Advanced Photon Source for their help on the beamline; Nick Guise of NIST for computer programming; and Joanne Browne, Victor Perez, Jeff Neil, Michael Quilici, and John Kelso of OSRAM SYLVANIA, Inc., for cell preparation; NR 16 TC 1 Z9 1 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 034509 DI 10.1063/1.4862041 PG 12 WC Physics, Applied SC Physics GA AI9WU UT WOS:000337296400003 ER PT J AU Sanchez-Juan, P Ghosh, PM Hagen, J Gesierich, B Henry, M Grinberg, LT O'Neil, JP Janabi, M Huang, EJ Trojanowski, JQ Vinters, HV Gorno-Tempini, M Seeley, WW Boxer, AL Rosen, HJ Kramer, JH Miller, BL Jagust, WJ Rabinovici, GD AF Sanchez-Juan, Pascual Ghosh, Pia M. Hagen, Jayne Gesierich, Benno Henry, Maya Grinberg, Lea T. O'Neil, James P. Janabi, Mustafa Huang, Eric J. Trojanowski, John Q. Vinters, Harry V. Gorno-Tempini, Marilu Seeley, William W. Boxer, Adam L. Rosen, Howard J. Kramer, Joel H. Miller, Bruce L. Jagust, William J. Rabinovici, Gil D. TI Practical utility of amyloid and FDG-PET in an academic dementia center SO NEUROLOGY LA English DT Article ID FRONTOTEMPORAL LOBAR DEGENERATION; MILD COGNITIVE IMPAIRMENT; ONSET ALZHEIMERS-DISEASE; PITTSBURGH COMPOUND-B; CORTICOBASAL DEGENERATION; DIFFERENTIAL-DIAGNOSIS; IMPACT; NEUROPATHOLOGY; MANAGEMENT; VARIANTS AB Objective:To evaluate the effect of amyloid imaging on clinical decision making.Methods:We conducted a retrospective analysis of 140 cognitively impaired patients (mean age 65.0 years, 46% primary -amyloid (A) diagnosis, mean Mini-Mental State Examination 22.3) who underwent amyloid (Pittsburgh compound B [PiB]) PET as part of observational research studies and were evaluated clinically before and after the scan. One hundred thirty-four concurrently underwent fluorodeoxyglucose (FDG)-PET. We assessed for changes between the pre- and post-PET clinical diagnosis (from A to non-A diagnosis or vice versa) and Alzheimer disease treatment plan. The association between PiB/FDG results and changes in management was evaluated using (2) and multivariate logistic regression. Postmortem diagnosis was available for 24 patients (17%).Results:Concordance between scan results and baseline diagnosis was high (PiB 84%, FDG 82%). The primary diagnosis changed after PET in 13/140 patients (9%) overall but in 5/13 (38%) patients considered pre-PET diagnostic dilemmas. When examined independently, discordant PiB and discordant FDG were both associated with diagnostic change (unadjusted p < 0.0001). However, when examined together in a multivariate logistic regression, only discordant PiB remained significant (adjusted p = 0.00013). Changes in treatment were associated with discordant PiB in patients with non-A diagnoses (adjusted p = 0.028), while FDG had no effect on therapy. Both PiB (96%) and FDG (91%) showed high agreement with autopsy diagnosis.Conclusions:PET had a moderate effect on clinical outcomes. Discordant PiB had a greater effect than discordant FDG, and influence on diagnosis was greater than on treatment. Prospective studies are needed to better characterize the clinical role of amyloid PET. C1 [Sanchez-Juan, Pascual; Ghosh, Pia M.; Hagen, Jayne; Gesierich, Benno; Henry, Maya; Grinberg, Lea T.; Gorno-Tempini, Marilu; Seeley, William W.; Boxer, Adam L.; Rosen, Howard J.; Kramer, Joel H.; Miller, Bruce L.; Jagust, William J.; Rabinovici, Gil D.] Univ Calif San Francisco, Memory & Aging Ctr, San Francisco, CA 94143 USA. [Sanchez-Juan, Pascual; Ghosh, Pia M.; Hagen, Jayne; Gesierich, Benno; Henry, Maya; Grinberg, Lea T.; Gorno-Tempini, Marilu; Seeley, William W.; Boxer, Adam L.; Rosen, Howard J.; Kramer, Joel H.; Miller, Bruce L.; Jagust, William J.; Rabinovici, Gil D.] Univ Calif San Francisco, Dept Neurol, San Francisco, CA 94143 USA. [Huang, Eric J.] Univ Calif San Francisco, Dept Pathol & Lab Med, San Francisco, CA 94143 USA. [Sanchez-Juan, Pascual] Univ Hosp Marques de Valdecilla, IFIMAV, Santander, Spain. [Sanchez-Juan, Pascual] Ctr Invest Biomed Red Enfermedades Neurodegenerat, Santander, Spain. [Ghosh, Pia M.; Jagust, William J.; Rabinovici, Gil D.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Ghosh, Pia M.; O'Neil, James P.; Janabi, Mustafa; Jagust, William J.; Rabinovici, Gil D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Trojanowski, John Q.] Univ Penn, Ctr Neurodegenerat Res, Philadelphia, PA 19104 USA. [Vinters, Harry V.] Univ Calif Los Angeles, Dept Pathol & Lab Med, Los Angeles, CA USA. RP Sanchez-Juan, P (reprint author), Univ Calif San Francisco, Memory & Aging Ctr, San Francisco, CA 94143 USA. EM ifimav.biobanco1@fmdv.org OI Huang, Eric/0000-0002-5381-3801; grinberg, lea/0000-0002-6809-0618 FU Institute for Formation and Research of the Foundation "Marques de Valdecilla," Instituto de Salud Carlos III [PI12/02288]; European Union Joint Programme-Neurodegenerative Disease Research [DEMTEST PI11/03028]; United States NIH [K23-AG031861, R01-AG027859, R01-AG032306, R01-AG038791, P50-AG16570, P01-AG12435, P01-AG1972403, P50-AG023501]; State of California Department of Health Services Alzheimer's Disease Research Center of California [04-33516]; Alzheimer's Association [NIRG-07-59422]; John Douglas French Alzheimer's Foundation; Hellman Family Foundation; Tau Consortium FX This work was supported by grants from: Institute for Formation and Research of the Foundation "Marques de Valdecilla," Instituto de Salud Carlos III (PI12/02288); European Union Joint Programme-Neurodegenerative Disease Research (DEMTEST PI11/03028); United States NIH K23-AG031861, R01-AG027859, R01-AG032306, R01-AG038791, P50-AG16570, P01-AG12435, P01-AG1972403, and P50-AG023501; State of California Department of Health Services Alzheimer's Disease Research Center of California grant 04-33516; Alzheimer's Association grant NIRG-07-59422; John Douglas French Alzheimer's Foundation; Hellman Family Foundation; and Tau Consortium. NR 39 TC 25 Z9 25 U1 0 U2 6 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA SN 0028-3878 EI 1526-632X J9 NEUROLOGY JI Neurology PD JAN 21 PY 2014 VL 82 IS 3 BP 230 EP 238 DI 10.1212/WNL.0000000000000032 PG 9 WC Clinical Neurology SC Neurosciences & Neurology GA AH6SJ UT WOS:000336260700011 PM 24353340 ER PT J AU Darvasi, G Keitel, CH Buth, C AF Darvasi, Gabor Keitel, Christoph H. Buth, Christian TI Optical control of an atomic inner-shell x-ray laser SO PHYSICAL REVIEW A LA English DT Article ID FREE-ELECTRON LASER; EMISSION; PULSE; FIELD; ULTRASHORT; EXCITATION; RADIATION; COHERENT; NEON AB X-ray free-electron lasers have had an enormous impact on x-ray science by achieving femtosecond pulses with unprecedented intensities. However, present-day facilities operating by the self-amplified spontaneous emission principle have a number of shortcomings; namely, their radiation has a chaotic pulse profile and short coherence times. We put forward a scheme for a neon-based atomic inner-shell x-ray laser (XRL) which produces temporally and spatially coherent subfemtosecond pulses that are controlled by and synchronized to an optical laser with femtosecond precision. We envision that such an XRL will allow for numerous applications such as nuclear quantum optics and the study of ultrafast quantum dynamics of atoms, molecules, and condensed matter. C1 [Darvasi, Gabor; Keitel, Christoph H.; Buth, Christian] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Buth, Christian] Argonne Natl Lab, Argonne, IL 60439 USA. RP Buth, C (reprint author), Max Planck Inst Quantum Opt, Hans Kopfermann Str 1, D-85748 Garching, Germany. EM christian.buth@web.de RI Buth, Christian/A-2834-2017 OI Buth, Christian/0000-0002-5866-3443 FU Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-AC02-06CH11357] FX We would like to thank Stefano M. Cavaletto for fruitful discussions. C.B. was supported by the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy, under Contract No. DE-AC02-06CH11357. NR 56 TC 1 Z9 1 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 21 PY 2014 VL 89 IS 1 AR 013823 DI 10.1103/PhysRevA.89.013823 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0UI UT WOS:000332210500022 ER PT J AU Slater, CS Blake, S Brouard, M Lauer, A Vallance, C John, JJ Turchetta, R Nomerotski, A Christensen, L Nielsen, JH Johansson, MP Stapelfeldt, H AF Slater, Craig S. Blake, Sophie Brouard, Mark Lauer, Alexandra Vallance, Claire John, Jaya John Turchetta, Renato Nomerotski, Andrei Christensen, Lauge Nielsen, Jens H. Johansson, Mikael P. Stapelfeldt, Henrik TI Covariance imaging experiments using a pixel-imaging mass-spectrometry camera SO PHYSICAL REVIEW A LA English DT Article ID MULTIPHOTON MULTIPLE IONIZATION; COULOMB EXPLOSION; DATA-ACQUISITION; SMALL MOLECULES; PHOTOELECTRON; DYNAMICS; ION; COINCIDENCE; DETECTOR AB The "pixel imaging mass spectrometry" camera is used to perform femtosecond laser-induced Coulomb explosion imaging of 3,5-dibromo-3',5'- difluoro-4'-cyanobiphenyl molecules prealigned in space. The experiment allows the concurrent detection of the correlated two-dimensional momentum images of all the ionic fragments resulting from fragmentation of multiple molecules in each acquisition cycle. The Coulomb explosion studies provide rich information about the parent molecular structure and fragmentation dynamics, and open new opportunities for real-time imaging of intramolecular processes. C1 [Slater, Craig S.; Blake, Sophie; Brouard, Mark; Lauer, Alexandra] Univ Oxford, Dept Chem, Oxford OX1 3QZ, England. [Slater, Craig S.; Blake, Sophie; Brouard, Mark; Lauer, Alexandra] Theoret Chem Lab, Oxford OX1 3QZ, England. [Vallance, Claire] Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England. [John, Jaya John] Univ Oxford, Dept Phys, Oxford OX1 3RH, England. [Turchetta, Renato] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Nomerotski, Andrei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Christensen, Lauge; Nielsen, Jens H.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Johansson, Mikael P.] Univ Helsinki, Lab Instruct Swedish, Dept Chem, FI-00014 Helsinki, Finland. [Stapelfeldt, Henrik] Aarhus Univ, Dept Chem, DK-8000 Aarhus C, Denmark. [Stapelfeldt, Henrik] Aarhus Univ, Interdisciplinary Nanosci Ctr iNANO, DK-8000 Aarhus C, Denmark. RP Slater, CS (reprint author), Univ Oxford, Dept Chem, S Parks Rd, Oxford OX1 3QZ, England. EM mark.brouard@chem.ox.ac.uk; henriks@chem.au.dk RI Johansson, Mikael/A-5889-2009; Nomerotski, Andrei/A-5169-2010; OI Johansson, Mikael/0000-0002-9793-8235; John, Jaya/0000-0001-6831-6501 FU EPSRC via Programme [EP/G00224X/1]; EU through grant FP7 ITN " ICONIC" [238671]; STFC through a PNPAS award; mini-IPS grant [ST/J002895/1]; Danish Council for Independent Research (Natural Sciences); DFG [La 3209/11] FX The support of the EPSRC via Programme Grant No. EP/G00224X/1 (to M. B. and C. V.), the EU through grant FP7 ITN " ICONIC" (Project Grant No. 238671 to M. B. and C. V.), STFC through a PNPAS award to A. N., M. B., C. V., and R. T., and a mini-IPS grant ST/J002895/1 to A. N. and R. T., ERC through Starting Independent Researcher grant " ImageMS" (C. V.), and a proof of concept grant from ISIS Innovation Ltd. (M. B., C. V., and A. N.) are gratefully acknowledged. A. L. thanks the DFG via Grant No. La 3209/11 for support. The work was supported by the Danish Council for Independent Research (Natural Sciences), The Lundbeck Foundation, and the Carlsberg Foundation. CSC, The Finnish IT Centre for Science, provided computing resources to M. P. J. NR 33 TC 9 Z9 9 U1 2 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 21 PY 2014 VL 89 IS 1 AR 011401 DI 10.1103/PhysRevA.89.011401 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0UI UT WOS:000332210500003 ER PT J AU Ilieva, S Thurauf, M Kroll, T Krucken, R Behrens, T Bildstein, V Blazhev, A Bonig, S Butler, PA Cederkall, J Davinson, T Delahaye, P Diriken, J Ekstroem, A Finke, F Fraile, LM Franchoo, S Fransen, C Georgiev, G Gernhaeuser, R Habs, D Hess, H Hurst, AM Huyse, M Ivanov, O Iwanicki, J Kent, P Kester, O Koster, U Lutter, R Mahgoub, M Martin, D Mayet, P Maierbeck, P Morgan, T Niedermeier, O Pantea, M Reiter, P Rodriguez, TR Rolke, T Scheit, H Scherillo, A Schwalm, D Seidlitz, M Sieber, T Simpson, GS Stefanescu, I Thiel, S Thirolf, PG Van de Walle, J Van Duppen, P Voulot, D Warr, N Weinzierl, W Weisshaar, D Wenander, F Wiens, A Winkler, S AF Ilieva, S. Thuerauf, M. Kroell, Th. Kruecken, R. Behrens, T. Bildstein, V. Blazhev, A. Boenig, S. Butler, P. A. Cederkaell, J. Davinson, T. Delahaye, P. Diriken, J. Ekstroem, A. Finke, F. Fraile, L. M. Franchoo, S. Fransen, Ch. Georgiev, G. Gernhaeuser, R. Habs, D. Hess, H. Hurst, A. M. Huyse, M. Ivanov, O. Iwanicki, J. Kent, P. Kester, O. Koester, U. Lutter, R. Mahgoub, M. Martin, D. Mayet, P. Maierbeck, P. Morgan, T. Niedermeier, O. Pantea, M. Reiter, P. Rodriguez, T. R. Rolke, Th. Scheit, H. Scherillo, A. Schwalm, D. Seidlitz, M. Sieber, T. Simpson, G. S. Stefanescu, I. Thiel, S. Thirolf, P. G. Van de Walle, J. Van Duppen, P. Voulot, D. Warr, N. Weinzierl, W. Weisshaar, D. Wenander, F. Wiens, A. Winkler, S. TI Coulomb excitation of neutron-rich Cd isotopes SO PHYSICAL REVIEW C LA English DT Article ID STATIC QUADRUPOLE-MOMENTS; SHELL STRUCTURE; PD-108; DETECTORS AB The isotopes (122),(124),Cd-126 were studied in a "safe" Coulomb-excitation experiment at the radioactive ion-beam facility REX-ISOLDE at CERN. The reduced transition probabilities B(E2; 0(g. s)(vertical bar) -> 2(1)(+)) and limits for the quadrupole moments of the first 2(+) excited states in the three isotopes were determined. The onset of collectivity in the vicinity of the Z = 50 and N = 82 shell closures is discussed by comparison with shell model and beyond mean-field calculations. C1 [Ilieva, S.; Thuerauf, M.; Kroell, Th.; Boenig, S.; Pantea, M.; Rodriguez, T. R.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Kroell, Th.; Kruecken, R.; Behrens, T.; Bildstein, V.; Gernhaeuser, R.; Mahgoub, M.; Maierbeck, P.; Weinzierl, W.; Winkler, S.] Tech Univ Munich, Phys Dept E12, Garching, Germany. [Bildstein, V.; Niedermeier, O.; Scheit, H.; Schwalm, D.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Blazhev, A.; Finke, F.; Fransen, Ch.; Hess, H.; Martin, D.; Reiter, P.; Rolke, Th.; Scherillo, A.; Seidlitz, M.; Thiel, S.; Warr, N.; Weisshaar, D.; Wiens, A.] Univ Cologne, Inst Kernphys, Cologne, Germany. [Butler, P. A.; Hurst, A. M.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cederkaell, J.; Delahaye, P.; Koester, U.; Sieber, T.; Voulot, D.; Wenander, F.] CERN, Geneva, Switzerland. [Davinson, T.] Univ Edinburgh, Dept Phys & Astron, Edinburgh EH8 9YL, Midlothian, Scotland. [Diriken, J.; Huyse, M.; Ivanov, O.; Mayet, P.; Stefanescu, I.; Van de Walle, J.; Van Duppen, P.] Katholieke Univ Leuven, Inst Kern & Stralingsfys, Louvain, Belgium. [Diriken, J.] Belgian Nucl Res Ctr SCK CEN, Mol, Belgium. [Ekstroem, A.] Lund Univ, Inst Fys, S-22100 Lund, Sweden. [Fraile, L. M.] Univ Complutense Madrid, Grp Fis Nucl, Madrid, Spain. [Franchoo, S.] Inst Phys Nucl, F-91406 Orsay, France. [Georgiev, G.] Univ Paris 11, CSNSM, CNRS IN2P3, F-91405 Orsay, France. [Habs, D.; Kester, O.; Lutter, R.; Morgan, T.; Thirolf, P. G.] Univ Munich, Garching, Germany. [Hurst, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Iwanicki, J.] Uniwersytet Warszawski, Srodowiskowe Lab Ciezkich Jonow, Warsaw, Poland. [Kent, P.] Univ York, Dept Phys, Nucl Phys Grp, York YO10 5DD, N Yorkshire, England. [Scherillo, A.; Simpson, G. S.] Lab Phys Subatom & Cosmol, Grenoble, France. RP Ilieva, S (reprint author), Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. EM silieva@ikp.tu-darmstadt.de RI Fraile, Luis/B-8668-2011; Rodriguez, Tomas/K-8282-2014; Scheit, Heiko/B-4779-2008; Ekstrom, Andreas/D-3782-2014; Georgiev, Georgi/C-5110-2008; Kruecken, Reiner/A-1640-2013; OI Fraile, Luis/0000-0002-6281-3635; Rodriguez, Tomas/0000-0002-3516-8239; Scheit, Heiko/0000-0002-8937-1101; Georgiev, Georgi/0000-0003-1467-1764; Kruecken, Reiner/0000-0002-2755-8042; Butler, Peter/0000-0001-6080-9205 FU German Federal Ministry of Education and Research (BMBF) [06DA9036I, 05P12RDCIA, 06MT190, 06MT238, 05P09PKCI5, 05P12PKFNE]; European Union under EURONS [506065]; ENSAR [262010]; Spanish MINECO [FPA2010-17142]; UK Science and Technology Facilities Council FX This work was partly supported by the German Federal Ministry of Education and Research (BMBF) with Grant Nos. 06DA9036I, 05P12RDCIA, 06MT190, 06MT238, 05P09PKCI5, and 05P12PKFNE, the European Union under EURONS (No. 506065) and ENSAR (No. 262010), Spanish MINECO FPA2010-17142 and the UK Science and Technology Facilities Council. NR 43 TC 6 Z9 7 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 21 PY 2014 VL 89 IS 1 AR 014313 DI 10.1103/PhysRevC.89.014313 PG 10 WC Physics, Nuclear SC Physics GA AB9ZY UT WOS:000332155600001 ER PT J AU Lonardoni, D Pederiva, F Gandolfi, S AF Lonardoni, D. Pederiva, F. Gandolfi, S. TI Accurate determination of the interaction between A hyperons and nucleons from auxiliary field diffusion Monte Carlo calculations SO PHYSICAL REVIEW C LA English DT Article ID S-SHELL HYPERNUCLEI; BINDING-ENERGY VALUES; LAMBDA-HYPERNUCLEI; SCATTERING; NN; SPECTROSCOPY; MODELS; BE-9(LAMBDA); BREAKING; PARTICLE AB Background: An accurate assessment of the hyperon-nucleon interaction is of great interest in view of recent observations of very massive neutron stars. The challenge is to build a realistic interaction that can be used over a wide range of masses and in infinite matter starting from the available experimental data on the binding energy of light hypernuclei. To this end, accurate calculations of the hyperon binding energy in a hypernucleus are necessary. Purpose: We present a quantum Monte Carlo study of Lambda and Lambda Lambda hypernuclei up to A = 91. We investigate the contribution of two- and three-body Lambda-nucleon forces to the Lambda binding energy. Method: Ground state energies are computed solving the Schrodinger equation for nonrelativistic baryons by means of the auxiliary field diffusion Monte Carlo algorithm extended to the hypernuclear sector. Results: We show that a simple adjustment of the parameters of the Lambda NN three-body force yields a very good agreement with available experimental data over a wide range of hypernuclear masses. In some cases no experiments have been performed yet, and we give new predictions. Conclusions: The newly fitted Lambda NN force properly describes the physics of medium-heavy Lambda hypernuclei, correctly reproducing the saturation property of the hyperon separation energy. C1 [Lonardoni, D.; Pederiva, F.] Univ Trento, Dept Phys, I-38123 Trento, Italy. [Lonardoni, D.; Pederiva, F.] INFN TIFPA, Trento Inst Fundamental Phys & Applicat, Trento, Italy. [Gandolfi, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lonardoni, D (reprint author), Univ Trento, Dept Phys, Via Sommarive 14, I-38123 Trento, Italy. EM lonardoni@science.unitn.it; pederiva@science.unitn.it OI Gandolfi, Stefano/0000-0002-0430-9035 FU Autonomous Province of Trento; INFN; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Department of Energy Nuclear Physics Office; NUCLEI SciDAC program; Los Alamos LDRD FX This work has been partially performed at LISC, Interdisciplinary Laboratory for Computational Science, a joint venture of the University of Trento and Bruno Kessler Foundation. Support and computer time were partly made available by the AuroraScience project (funded by the Autonomous Province of Trento and INFN), and by Los Alamos Open Supercomputing. This research used also resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. The work of S. G. was supported by the Department of Energy Nuclear Physics Office, by the NUCLEI SciDAC program, and by a Los Alamos LDRD early career grant. NR 70 TC 26 Z9 26 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 21 PY 2014 VL 89 IS 1 AR 014314 DI 10.1103/PhysRevC.89.014314 PG 11 WC Physics, Nuclear SC Physics GA AB9ZY UT WOS:000332155600002 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Eroe, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hoermann, N Hrubec, J Jeitler, M Kiesenhofer, W Knuenz, V Krammer, M Kraetschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schoefbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Lowette, S Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, X Wang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Sierra, LFC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Abdelalim, AA Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P De Monchenault, GH Jarry, P Locci, E Malcles, J Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A De Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Bontenackels, M Calpas, B Edelhoff, M Feld, L Hindrichs, O Klein, K Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Gueth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bell, AJ Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dooling, S Dorland, T Eckerlin, G Eckstein, D Flucke, G Geiser, A Grebenyuk, A Gunnellini, P Habib, S Hauk, J Hellwig, G Horton, D Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Kramer, M Krucker, D Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Olzem, J Perrey, H Petrukhin, A Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Riedl, C Ron, E Sahin, MO Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Walsh, R Wissing, C Martin, MA Blobel, V Enderle, H Erfle, J Garutti, E Gebbert, U Gorner, M Gosselink, M Haller, J Heine, K Hoing, RS Kaussen, G Kirschenmann, H Klanner, R Kogler, R Lange, J Marchesini, I Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Thomsen, J Troendle, D Usai, E Vanelderen, L Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hartmann, F Hauth, T Held, H Hoffmann, KH Husemann, U Katkov, I Komaragiri, JR Kornmayer, A Kuznetsova, E Pardo, PL Martschei, D Mozer, MU Muller, T Niegel, M Nurnberg, A Oberst, O Ott, J Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Topsis-Giotis, I Gouskos, L Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S Sharan, M Singh, AP Abdulsalam, A Dutta, D Kailas, S Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Chatterjee, RM Ganguly, S Ghosh, S Guchait, M Gurtu, A Kole, G Kumar, S Maity, M Majumder, G Mazumdar, K Mohanty, GB Parida, B Sudhakar, K Wickramage, N Banerjee, S Dugad, S Arfaei, H Bakhshiansohi, H Etesami, SM Fahim, A Jafari, A Khakzad, M Najafabadi, MM Mehdiabadi, SP Safarzadeh, B Zeinali, M Grunewald, M Abbrescia, M Barbone, L Calabria, C Chhibra, SS Colaleo, A Creanza, D De Filippis, N De Palma, M Fiore, L Iaselli, G Maggi, G Maggi, M Marangelli, B My, S Nuzzo, S Pacifico, N Pompili, A Pugliese, G Radogna, R Selvaggi, G Silvestris, L Singh, G Venditti, R Verwilligen, P Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Campanini, R Capiluppi, P Castro, A Cavallo, FR Codispoti, G Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Grandi, C Guiducci, L Marcellini, S Masetti, G Meneghelli, M Montanari, A Navarria, FL Odorici, F Perrotta, A Primavera, F Rossi, AM Rovelli, T Siroli, GP Tosi, N Travaglini, R Albergo, S Cappello, G Chiorboli, M Costa, S Giordano, F Potenza, R Tricomi, A Tuve, C Barbagli, G Ciulli, V Civinini, C D'Alessandro, R Focardi, E Frosali, S Gallo, E Gonzi, S Gori, V Lenzi, P Meschini, M Paoletti, S Sguazzoni, G Tropiano, A Benussi, L Bianco, S Fabbri, F Piccolo, D Fabbricatore, P Ferretti, R Ferro, F Lo Vetere, M Musenich, R Robutti, E Tosi, S Benaglia, A Dinardo, ME Fiorendi, S Gennai, S Ghezzi, A Govoni, P Lucchini, MT Malvezzi, S Manzoni, RA Martelli, A Menasce, D Moroni, L Paganoni, M Pedrini, D Ragazzi, S Redaelli, N De Fatis, TT Buontempo, S Cavallo, N Fabozzi, F Iorio, AOM Lista, L Meola, S Merola, M Paolucci, P Azzi, P Bacchetta, N Bisello, D Branca, A Carlin, R Checchia, P Dorigo, T Dosselli, U Fanzago, F Galanti, M Gasparini, F Gasparini, U Giubilato, P Gonella, F Gozzelino, A Kanishchev, K Lacaprara, S Lazzizzera, I Margoni, 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CA CMS Collaboration TI Search for the standard model Higgs boson produced in association with a W or a Z boson and decaying to bottom quarks SO PHYSICAL REVIEW D LA English DT Article ID PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; ATLAS DETECTOR; LHC; MASSES AB A search for the standard model Higgs boson (H) decaying to b (b) over bar when produced in association with a weak vector boson (V) is reported for the following channels: W(mu nu)H, W(e nu)H, W(tau nu)H, Z(mu mu)H, Z(ee)H and Z(nu nu)H. The search is performed in data samples corresponding to integrated luminosities of up to 5.1 inverse femtobarns at root s = 7 TeV and up to 18.9 fb(-1) at root s = 8 TeV, recorded by the CMS experiment at the LHC. An excess of events is observed above the expected background with a local significance of 2.1 standard deviations for a Higgs boson mass of 125 GeV, consistent with the expectation from the production of the standard model Higgs boson. 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Vander; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Calpas, B.; Edelhoff, M.; Feld, L.; Hindrichs, O.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thuer, S.; Weber, M.] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Flugge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Grebenyuk, A.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Kramer, M.; Krucker, D.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. 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U.; Muller, Th.; Niegel, M.; Nurnberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Rocker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, Milan, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, I-70121 Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, Milan, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, I-40126 Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, Milan, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, I-95124 Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, Milan, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, I-50121 Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Milan, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; De Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Martelli, A.; Paganoni, M.; Ragazzi, S.; De Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, Milan, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.; Meola, S.; Paolucci, P.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Milan, Italy. [Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, I-35100 Padua, Italy. [Bisello, D.; Galanti, M.; Kanishchev, K.; Lazzizzera, I.] Univ Trento, Trento, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, Milan, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, Milan, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Milan, Italy. [Martini, L.; Messineo, A.; Rizzi, A.] Univ Pisa, I-56100 Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Milan, Italy. [Barone, L.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, Milan, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, I-10124 Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Pelliccioni, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Milan, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, I-34127 Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; la Cruz, I. Heredia-De; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.; Almeida, N.; Bargassa, P.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Silva, C. Beirao Da Cruz E.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Abdulsalam, A.; Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Abdulsalam, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Kaminskiy, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Adair, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.; Adzic, P.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Abdulsalam, A.; Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De la Cruz, B.; Peris, A. Delgado; Vazquez, D. Dominguez; Bedoya, C. Fernandez; Ramos, J. P. Fernandez; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Lopez, O. Gonzalez; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; De Martino, E. Navarro; Pelayo, J. Puerta; Olmeda, A. Quintario; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; De Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Menendez, J. Fernandez; Folgueras, S.; Caballero, I. Gonzalez; Iglesias, L. Lloret] Univ Oviedo, Oviedo, Spain. [Cifuentes, J. A. Brochero; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Campderros, J. Duarte; Fernandez, M.; Gomez, G.; Sanchez, J. Gonzalez; Graziano, A.; Virto, A. Lopez; Marco, J.; Marco, R.; Rivero, C. Martinez; Matorras, F.; Sanchez, F. J. Munoz; Gomez, J. Piedra; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Cortabitarte, R. Vilar] CSIC Univ Cantabria, IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y-J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaafer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wohri, H. K.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Konig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Abdulsalam, A.; Bachmair, F.; Bani, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Dunser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; Del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Nageli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Cosa, A.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Abdulsalam, A.; Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, NJ USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wurthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.; Anastassov, A.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stockli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. 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Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Sogut, Kenan/0000-0002-9682-2855; Jacob, Jeson/0000-0001-6895-5493; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Ulrich, Ralf/0000-0002-2535-402X; Lenzi, Piergiulio/0000-0002-6927-8807; Lucchini, Marco Toliman/0000-0002-7497-7450; Gutsche, Oliver/0000-0002-8015-9622; Raval, Amita/0000-0003-0164-4337; Torassa, Ezio/0000-0003-2321-0599; Verdier, Patrice/0000-0003-3090-2948; CHANG, PAO-TI/0000-0003-4064-388X FU Austrian Federal Ministry of Science and Research and the Austrian Science Fund; Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, and National Office for Research and Technology, Hungary; Department of Atomic Energy and the Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education and the National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); National Science Council, Taipei; Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; Science and Technology Facilities Council, UK; U.S. Department of Energy, and the U.S. National Science Foundation; Marie-Curie program and the European Research Council and EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS program of Foundation for Polish Science; EU, Regional Development Fund; Thalis and Aristeia programs; EU-ESF and the Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation.; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS program of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF. NR 66 TC 67 Z9 67 U1 8 U2 103 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 21 PY 2014 VL 89 IS 1 AR 012003 DI 10.1103/PhysRevD.89.012003 PG 36 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5ZG UT WOS:000331866600001 ER PT J AU Dawson, S Furlan, E AF Dawson, S. Furlan, E. TI Yukawa corrections to Higgs production in top partner models SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-FERMION CORRECTIONS; LOW-ENERGY THEOREMS; BOSON PRODUCTION; ELECTROWEAK CORRECTIONS; HADRON COLLIDERS; QCD CORRECTIONS; DECAY; CONNECTION; PHYSICS; QUARKS AB Higgs production from gluon fusion is sensitive to the properties of heavy colored fermions and to the Yukawa couplings, YFMF/v, of these particles to the Higgs boson. We compute the two-loop, O((YFMF/v)(3)) contributions of new high mass fermions to Higgs production. In the Standard Model, these contributions are part of the well-known electroweak corrections and are negligible. However, in models with TeV scale fermions, such as top partner or composite models, Yukawa corrections are enhanced by effects of O((YFMF/v)(3)) and are potentially significant due to the large mass of the new quarks. We examine the size of these top partner Yukawa corrections to Higgs production for parameter choices which are allowed by precision electroweak constraints. C1 [Dawson, S.; Furlan, E.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Furlan, E.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Dawson, S (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. OI Furlan, Elisabetta/0000-0001-7036-9012 FU U. S. Department of Energy [DE-AC02-98CH10886, DE-AC02-07CH11359] FX BNL is supported by the U. S. Department of Energy under Grant No. DE-AC02-98CH10886. Fermilab is operated by the Fermi Research Alliance under Contract No. DE-AC02-07CH11359 with the U. S. Department of Energy. E. F. thanks the Galileo Galilei Institute for the hospitality during the completion of this work. NR 57 TC 8 Z9 8 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 21 PY 2014 VL 89 IS 1 AR 015012 DI 10.1103/PhysRevD.89.015012 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5ZG UT WOS:000331866600005 ER PT J AU Matan, K Nambu, Y Zhao, Y Sato, TJ Fukumoto, Y Ono, T Tanaka, H Broholm, C Podlesnyak, A Ehlers, G AF Matan, K. Nambu, Y. Zhao, Y. Sato, T. J. Fukumoto, Y. Ono, T. Tanaka, H. Broholm, C. Podlesnyak, A. Ehlers, G. TI Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet Rb2Cu3SnF12 SO PHYSICAL REVIEW B LA English DT Article ID HEISENBERG-ANTIFERROMAGNET; EXCITATIONS; STATES AB High-intensity pulsed neutron scattering reveals a new set of magnetic excitations in the pinwheel valence-bond solid state of the distorted kagome lattice antiferromagnet Rb2Cu3SnF12. The polarization of the dominant dispersive modes (2 meV < (h) over bar omega < 7 meV) is determined and found consistent with a dimer series expansion with strong Dzyaloshinskii-Moriya interactions (D/J = 0.18). A weakly dispersive mode near 5 meV and shifted "ghosts" of the main modes are attributed to the enlarged unit cell below a T = 215 K structural transition. Continuum scattering between 8 and 10 meV might be interpreted as a remnant of the kagome spinon continuum [Nature (London) 492, 406 (2012).]. C1 [Matan, K.] Mahidol Univ, Fac Sci, Dept Phys, Bangkok 10400, Thailand. [Matan, K.] Commiss Higher Educ, ThEP, Bangkok 10400, Thailand. [Nambu, Y.; Sato, T. J.] Tohoku Univ, IMRAM, Sendai, Miyagi 9808577, Japan. [Zhao, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Zhao, Y.; Broholm, C.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Fukumoto, Y.] Tokyo Univ Sci, Fac Sci & Technol, Dept Phys, Noda, Chiba 2788510, Japan. [Ono, T.] Osaka Prefecture Univ, Sch Sci, Dept Phys Sci, Sakai, Osaka 5998531, Japan. [Tanaka, H.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Broholm, C.] Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. [Broholm, C.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Broholm, C.; Podlesnyak, A.; Ehlers, G.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Matan, K (reprint author), Mahidol Univ, Fac Sci, Dept Phys, Bangkok 10400, Thailand. EM kittiwit.mat@mahidol.ac.th; tanaka@lee.phys.titech.ac.jp RI Nambu, Yusuke/C-3863-2012; Sato, Taku/I-7664-2015; Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; Podlesnyak, Andrey/A-5593-2013 OI Nambu, Yusuke/0000-0003-1167-7124; Sato, Taku/0000-0003-2511-4998; Ehlers, Georg/0000-0003-3513-508X; Podlesnyak, Andrey/0000-0001-9366-6319 FU Thailand Research Fund [MRG55800]; JPS [23244072, 24740223, 23540395]; Global COE Program; MEXT Japan; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-08ER46544]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The work was supported in part by the Thailand Research Fund under Grant No. MRG55800, a Grant-in-Aid for Scientific Research from JPS (Grants No. 23244072, No. 24740223, and No. 23540395) and a Global COE Program funded by MEXT Japan. Work at the Institute for Quantum Matter was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-08ER46544. The research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 42 TC 7 Z9 7 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 21 PY 2014 VL 89 IS 2 AR 024414 DI 10.1103/PhysRevB.89.024414 PG 7 WC Physics, Condensed Matter SC Physics GA AC0ZH UT WOS:000332223500004 ER PT J AU Vanderhoef, LR Azad, AK Bomberger, CC Chowdhury, DR Chase, DB Taylor, AJ Zide, JMO Doty, MF AF Vanderhoef, Laura R. Azad, Abul K. Bomberger, Cory C. Chowdhury, Dibakar Roy Chase, D. Bruce Taylor, Antoinette J. Zide, Joshua M. O. Doty, Matthew F. TI Charge carrier relaxation processes in TbAs nanoinclusions in GaAs measured by optical-pump THz-probe transient absorption spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID ASSEMBLED ERAS ISLANDS; NANOISLAND SUPERLATTICES; ELECTRONIC-STRUCTURE; QUANTUM DOTS; DYNAMICS; LUMINESCENCE; FEMTOSECOND AB Rare-earth materials epitaxially codeposited with III-V semiconductors form small, spherical rare-earth-monopnictide nanoparticles embedded within the III-V host. The small size of these particles (approximately 1.5 nm diameter) suggests that interesting electronic properties might emerge as a result of both confinement and surface states. However, ErAs nanoparticles do not exhibit any signs of quantum confinement or an emergent band gap, and these experimental observations are understood theoretically. We use ultrafast pump-probe spectroscopy to investigate the electronic structure of TbAs nanoparticles embedded in a GaAs host, which were expected to be similar to ErAs. We study the dynamics of carrier relaxation into the TbAs states, which essentially act as traps, using optical-pump terahertz-probe transient absorption spectroscopy. By analyzing how the carrier relaxation rates depend on pump fluence and sample temperature, we conclude that the TbAs states are saturable. Saturable traps suggest the existence of a band gap for TbAs nanoparticles, in sharp contrast with the results for ErAs. C1 [Vanderhoef, Laura R.; Doty, Matthew F.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Azad, Abul K.; Chowdhury, Dibakar Roy; Taylor, Antoinette J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bomberger, Cory C.; Chase, D. Bruce; Zide, Joshua M. O.; Doty, Matthew F.] Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA. RP Vanderhoef, LR (reprint author), Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. EM doty@udel.edu OI Azad, Abul/0000-0002-7784-7432; Doty, Matthew/0000-0001-7999-3567 FU National Science Foundation [DMR-1105137] FX The authors wish to acknowledge support from the National Science Foundation (DMR-1105137). Additionally, usage of facilities at Los Alamos National Laboratory was made possible by the Center for Integrated Nanotechnology (CINT), a Department of Energy Basic Energy Science user facility. NR 29 TC 7 Z9 7 U1 0 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 21 PY 2014 VL 89 IS 4 AR 045418 DI 10.1103/PhysRevB.89.045418 PG 7 WC Physics, Condensed Matter SC Physics GA AC1AA UT WOS:000332225400010 ER PT J AU Liu, J Haiman, Z Hui, L Kratochvil, JM May, M AF Liu, Jia Haiman, Zoltan Hui, Lam Kratochvil, Jan M. May, Morgan TI Impact of magnification and size bias on the weak lensing power spectrum and peak statistics SO PHYSICAL REVIEW D LA English DT Article ID FORS DEEP FIELD; COSMOLOGICAL CONSTRAINTS; HIGH-REDSHIFT; LUMINOSITY FUNCTIONS; COSMIC SHEAR; GALAXIES; TELESCOPE; QUASARS; MODEL; DISTRIBUTIONS AB The weak lensing power spectrum is a powerful tool to probe cosmological parameters. Additionally, lensing peak counts contain cosmological information beyond the power spectrum. Both of these statistics can be affected by the preferential selection of source galaxies in patches of the sky with high magnification, as well as by the dilution in the source galaxy surface density in such regions. If not accounted for, these biases introduce systematic errors for cosmological measurements. Here we quantify these systematic errors, using convergence maps from a suite of ray-tracing N-body simulations. At the cutoff magnitude m of ongoing and planned major weak lensing surveys, the logarithmic slope of the cumulative number counts s d log n(> m)/d log m is in the range 0.1 less than or similar to s less than or similar to 0.5. At s approximate to 0.2, expected in the I band for Large Synoptic Survey Telescope, the inferred values of Omega(m), w, and sigma(8) are biased by many sigma (where sigma denotes the marginalized error), and therefore the biases will need to be carefully modeled. We also find that the parameters are biased differently in the (Omega(m), w, sigma(8)) parameter space when the power spectrum and the peak counts are used. In particular, w derived from the power spectrum is less affected than w derived from peak counts, while the opposite is true for the best-constrained combination of sigma(8)Omega(gamma)(m) (with gamma = 0.62 from the power spectrum and gamma = 0.48 from peak counts). This suggests that the combination of the power spectrum and peak counts can help mitigate the impact of magnification and size biases. C1 [Liu, Jia; Haiman, Zoltan] Columbia Univ, Dept Astron & Astrophys, New York, NY 10027 USA. [Haiman, Zoltan; Hui, Lam] Columbia Univ, Inst Strings Cosmol & Astroparticle Phys ISCAP, New York, NY 10027 USA. [Hui, Lam] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kratochvil, Jan M.] Univ Miami, Dept Phys, Coral Gables, FL 33146 USA. [Kratochvil, Jan M.] Univ KwaZulu Natal, Astrophys & Cosmol Res Unit, ZA-4000 Durban, South Africa. [May, Morgan] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Liu, J (reprint author), Columbia Univ, Dept Astron & Astrophys, New York, NY 10027 USA. EM jia@astro.columbia.edu; zoltan@astro.columbia.edu; lhui@astro.columbia.edu; jank@physics.miami.edu; may@bnl.gov OI Liu, Jia/0000-0001-8219-1995 FU State of New York; U.S. Department of Energy [DE-AC02-98CH10886]; NSF [AST-1210877] FX We thank Kevin Huffenberger for useful discussions. This research used resources at the New York Center for Computational Sciences, a cooperative effort between Brookhaven National Laboratory and Stony Brook University, supported in part by the State of New York. This work is supported in part by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886 and by the NSF under Grant No. AST-1210877. The simulations were created on the IBM Blue Gene/L and /P New York Blue computer, and the maps were created and analyzed on the LSST/Astro Linux cluster at BNL. NR 68 TC 11 Z9 11 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 21 PY 2014 VL 89 IS 2 AR 023515 DI 10.1103/PhysRevD.89.023515 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5ZL UT WOS:000331867100002 ER PT J AU Freund, HP Yampolsky, NA Marksteiner, Q AF Freund, H. P. Yampolsky, N. A. Marksteiner, Q. TI Enhanced harmonic generation in x-ray free-electron lasers SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID OPERATION AB Harmonic generation becomes increasingly important as x-ray free-electron lasers push to shorter wavelengths. Recent studies have pointed to the possibility of enhancing harmonic generation by detuning the fundamental. In x-ray free-electron lasers, the wiggler line is composed of multiple wiggler segments with magnetic quadrupoles in the gaps to provide for increased focusing. In this paper, we study the effect on harmonic generation in simulation by (1) varying the gap lengths between the wiggler segments and (2) varying the electron beam beta function. In studying the harmonic we find enhanced harmonic generation is periodic in the gap length and peaks are found as the wiggler separation varies by lambda/3 (where lambda is the fundamental wavelength), which corresponds to a phase shift of 2 pi/3. As a consequence, enhanced harmonic generation is found both when the fundamental emission is strong by the nonlinear harmonic generation mechanism and by linear harmonic generation when the fundamental is detuned. C1 [Freund, H. P.; Yampolsky, N. A.; Marksteiner, Q.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Freund, HP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM henryf@lanl.gov RI Yampolsky, Nikolai/A-7521-2011 FU U.S. Department of Energy through the LANL/LDRD Program; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396] FX We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program for this work. This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. NR 22 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD JAN 21 PY 2014 VL 17 IS 1 AR 010702 DI 10.1103/PhysRevSTAB.17.010702 PG 6 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AC0GU UT WOS:000332173600001 ER PT J AU Schneider, AR Geissler, PL AF Schneider, Anna R. Geissler, Phillip L. TI Coarse-grained computer simulation of dynamics in thylakoid membranes: methods and opportunities SO FRONTIERS IN PLANT SCIENCE LA English DT Review DE simulation; coarse-grained modeling; nanoscale; thylakoid membrane; photosystem; Monte Carlo; Brownian dynamics ID HARVESTING COMPLEX-II; PHOTOSYSTEM-II; LIPID-BILAYERS; SUPRAMOLECULAR ORGANIZATION; PHOTOSYNTHETIC MEMBRANES; PROTEIN INTERACTIONS; GREEN PLANTS; DIFFUSION; CURVATURE; FORCES AB Coarse-grained simulation is a powerful and well-established suite of computational methods for studying structure and dynamics in nanoscale biophysical systems. As our understanding of the plant photosynthetic apparatus has become increasingly nuanced, opportunities have arisen for coarse-grained simulation to complement experiment by testing hypotheses and making predictions. Here, we give an overview of best practices in coarse-grained simulation, with a focus on techniques and results that are applicable to the plant thylakoid membraneprotein system. We also discuss current research topics for which coarse-grained simulation has the potential to play a key role in advancing the field. C1 [Schneider, Anna R.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Schneider, Anna R.; Geissler, Phillip L.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Geissler, Phillip L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Geissler, Phillip L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Geissler, PL (reprint author), Univ Calif Berkeley, Dept Chem, 207 Gilman Hall, Berkeley, CA 94720 USA. EM geissler@berkeley.edu FU National Science Foundation [CHE-7178966] FX Anna R. Schneider was supported by National Science Foundation Grant CHE-7178966. NR 61 TC 1 Z9 1 U1 5 U2 25 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JAN 21 PY 2014 VL 4 AR 555 DI 10.3389/fpls.2013.00555 PG 6 WC Plant Sciences SC Plant Sciences GA AB1AW UT WOS:000331524700001 ER PT J AU Kim, JB Weichman, ML Neumark, DM AF Kim, Jongjin B. Weichman, Marissa L. Neumark, Daniel M. TI Vibronic structure of VO2 probed by slow photoelectron velocity-map imaging spectroscopy SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID VANADIUM-OXIDE CLUSTERS; EFFECTIVE CORE POTENTIALS; GAS-PHASE; PHOTODETACHMENT MICROSCOPE; VIBRATIONAL SPECTROSCOPY; INFRARED-SPECTROSCOPY; ELECTRONIC-STRUCTURE; DIOXIDE MOLECULES; METAL-CLUSTERS; EXCITED-STATES AB We report high-resolution anion photoelectron spectra of vanadium dioxide (VO2(-)) obtained by slow electron velocity-map imaging of trapped and cryogenically cooled anions. Vibrationally resolved spectra are obtained for photodetachment to the first three neutral electronic states, giving an electron affinity of 1.8357(5) eV for the (X) over tilde (2)A(1) ground state and term energies of 0.1845(8) eV and 0.8130(5) eV for the (A) over tilde B-2(1) and (B) over tilde (2)A(1) excited states, respectively. The vibrational fundamentals v(1) and v(2) are obtained for all three states. Experimental assignments are confirmed by energies from electronic structure calculations and Franck-Condon spectral simulations. These simulations support assigning the anion ground state as the (X) over tilde B-3(1) state. With this assignment, photodetachment to the (B) over tilde (2)A(1) state involves a nominally forbidden two-electron transition, suggesting extensive configuration interaction in neutral VO2. (C) 2014 AIP Publishing LLC. C1 [Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu OI Weichman, Marissa/0000-0002-2551-9146 FU Air Force Office of Scientific Research [FA9550-12-1-0160]; Defense University Research Instrumentation Program [FA9550-11-1-0330]; National Science Foundation FX This work is funded by the Air Force Office of Scientific Research under Grant No. FA9550-12-1-0160 and the Defense University Research Instrumentation Program under Grant No. FA9550-11-1-0330. M.L.W. thanks the National Science Foundation for a graduate research fellowship. NR 80 TC 4 Z9 4 U1 1 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2014 VL 140 IS 3 AR 034307 DI 10.1063/1.4861667 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 302OM UT WOS:000330614400025 PM 25669379 ER PT J AU Kryvohuz, M Mukamel, S AF Kryvohuz, Maksym Mukamel, Shaul TI Nonlinear response theory in chemical kinetics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID STRATOSPHERIC OZONE; CLASSICAL MECHANICS; SYSTEMS; PERTURBATIONS; STABILITY AB A theory of nonlinear response of chemical kinetics, in which multiple perturbations are used to probe the time evolution of nonlinear chemical systems, is developed. Expressions for nonlinear chemical response functions and susceptibilities, which can serve as multidimensional measures of the kinetic pathways and rates, are derived. A new class of multidimensional measures that combine multiple perturbations and measurements is also introduced. Nonlinear fluctuation-dissipation relations for steady-state chemical systems, which replace operations of concentration measurement and perturbations, are proposed. Several applications to the analysis of complex reaction mechanisms are provided. (C) 2014 AIP Publishing LLC. C1 [Kryvohuz, Maksym] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Mukamel, Shaul] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. RP Kryvohuz, M (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mkryvohuz@anl.gov; smukamel@uci.edu FU National Science Foundation (NSF) [CHE-1058791]; Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE); NIH [GM-59230] FX We gratefully acknowledge the support of the National Science Foundation (NSF) through Grant No. CHE-1058791, from Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) and from NIH GM-59230. NR 33 TC 4 Z9 4 U1 0 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2014 VL 140 IS 3 AR 034111 DI 10.1063/1.4861588 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 302OM UT WOS:000330614400013 PM 25669367 ER PT J AU Leiding, J Coe, JD AF Leiding, Jeff Coe, Joshua D. TI An efficient approach to ab initio Monte Carlo simulation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; 1ST PRINCIPLES; MOLECULAR-DYNAMICS; PHASE-EQUILIBRIA; SHOCK COMPRESSION; LIQUID LITHIUM; BASIS-SET; WATER AB We present a Nested Markov chain Monte Carlo (NMC) scheme for building equilibrium averages based on accurate potentials such as density functional theory. Metropolis sampling of a reference system, defined by an inexpensive but approximate potential, was used to substantially decorrelate configurations at which the potential of interest was evaluated, thereby dramatically reducing the number needed to build ensemble averages at a given level of precision. The efficiency of this procedure was maximized on-the-fly through variation of the reference system thermodynamic state (characterized here by its inverse temperature beta(0)), which was otherwise unconstrained. Local density approximation results are presented for shocked states of argon at pressures from 4 to 60 GPa, where-depending on the quality of the reference system potential-acceptance probabilities were enhanced by factors of 1.2-28 relative to unoptimized NMC. The optimization procedure compensated strongly for reference potential shortcomings, as evidenced by significantly higher speedups when using a reference potential of lower quality. The efficiency of optimized NMC is shown to be competitive with that of standard ab initio molecular dynamics in the canonical ensemble. (C) 2014 AIP Publishing LLC. C1 [Leiding, Jeff; Coe, Joshua D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Leiding, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jcoe@lanl.gov FU Advanced Simulation and Computing (ASC); Los Alamos National Security, LLC, for the NNSA; U.S. DOE [DE-AC52-06NA25396] FX We thank the Advanced Simulation and Computing (ASC) program for funding, Joel Kress for technical assistance, and Carl Greeff and Sam Shaw for helpful comments on the manuscript. LANL is operated by Los Alamos National Security, LLC, for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. NR 53 TC 1 Z9 1 U1 3 U2 14 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2014 VL 140 IS 3 AR 034106 DI 10.1063/1.4855755 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 302OM UT WOS:000330614400008 PM 25669362 ER PT J AU Pascal, TA Boesenberg, U Kostecki, R Richardson, TJ Weng, TC Sokaras, D Nordlund, D McDermott, E Moewes, A Cabana, J Prendergast, D AF Pascal, Tod A. Boesenberg, Ulrike Kostecki, Robert Richardson, Thomas J. Weng, Tsu-Chien Sokaras, Dimosthenis Nordlund, Dennis McDermott, Eamon Moewes, Alexander Cabana, Jordi Prendergast, David TI Finite temperature effects on the X-ray absorption spectra of lithium compounds: First-principles interpretation of X-ray Raman measurements SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SOLID-ELECTROLYTE INTERPHASE; LI-ION BATTERIES; ALKALI-HALIDE CRYSTALS; HYDROGEN STORAGE; FINE-STRUCTURE; K-EDGE; SCATTERING; SPECTROSCOPY; PSEUDOPOTENTIALS; MODEL AB We elucidate the role of room-temperature-induced instantaneous structural distortions in the Li K-edge X-ray absorption spectra (XAS) of crystalline LiF, Li2SO4, Li2O, Li3N, and Li2CO3 using high resolution X-ray Raman spectroscopy (XRS) measurements and first-principles density functional theory calculations within the eXcited electron and Core Hole approach. Based on thermodynamic sampling via ab initio molecular dynamics simulations, we find calculated XAS in much better agreement with experiment than those computed using the rigid crystal structure alone. We show that local instantaneous distortion of the atomic lattice perturbs the symmetry of the Li 1s core-excited-state electronic structure, broadening spectral line-shapes and, in some cases, producing additional spectral features. The excellent agreement with high-resolution XRS measurements validates the accuracy of our first-principles approach to simulating XAS, and provides both accurate benchmarks for model compounds and a predictive theoretical capability for identification and characterization of multi-component systems, such as lithium-ion batteries, under working conditions. (C) 2014 AIP Publishing LLC. C1 [Pascal, Tod A.; Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Div Mat Sci, Berkeley, CA 94720 USA. [Boesenberg, Ulrike; Kostecki, Robert; Richardson, Thomas J.; Cabana, Jordi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Weng, Tsu-Chien; Sokaras, Dimosthenis; Nordlund, Dennis] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Stanford, CA 94720 USA. [McDermott, Eamon; Moewes, Alexander] Univ Saskatchewan, Dept Phys & Engn Phys, Saskatoon, SK S7N 5E2, Canada. [Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60605 USA. RP Prendergast, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Div Mat Sci, Berkeley, CA 94720 USA. EM dgprendergast@lbl.gov RI Nordlund, Dennis/A-8902-2008; Cabana, Jordi/G-6548-2012; Foundry, Molecular/G-9968-2014 OI Nordlund, Dennis/0000-0001-9524-6908; Cabana, Jordi/0000-0002-2353-5986; FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC0205CH11231, DE-SC0001294]; Laboratory Directed Research and Development Program of the Lawrence Berkeley National Laboratory; Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center; National Sciences and Engineering Research Council of Canada; Canada Research Chair Program; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [AC02-05CH11231]; Batteries for Advanced Transportation Technologies (BATT) Program FX T.A.P. and D. P. acknowledge invaluable discussions with Dr. Das Pemmaraju and the use of the WebXS online XAS simulation tool being created by James Wonsever. We thank the reviewers for bringing the possibility of singlet-repulsion effects in LiF to our attention. Theoretical portions of this work were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The experimental XRS portion of this research was carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory, and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by the Stanford University. T.A.P. was supported by the Laboratory Directed Research and Development Program of the Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. U.B. was supported as part of the Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001294. A.M. and E.M. acknowledge funding from the National Sciences and Engineering Research Council of Canada and the Canada Research Chair Program. Portions of this work were supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, under the Batteries for Advanced Transportation Technologies (BATT) Program. NR 88 TC 11 Z9 11 U1 9 U2 76 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2014 VL 140 IS 3 AR 034107 DI 10.1063/1.4856835 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 302OM UT WOS:000330614400009 PM 25669363 ER PT J AU Smith, KKG Poulsen, JA Cunsolo, A Rossky, PJ AF Smith, Kyle K. G. Poulsen, Jens Aage Cunsolo, A. Rossky, Peter J. TI Refinement of the experimental dynamic structure factor for liquid para-hydrogen and ortho-deuterium using semi-classical quantum simulation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID POLYMER MOLECULAR-DYNAMICS; PHASE-SPACE; SCATTERING; HE(4) AB The dynamic structure factor of liquid para-hydrogen and ortho-deuterium in corresponding thermodynamic states (T = 20.0 K, n = 21.24 nm(-3)) and (T = 23.0 K, n = 24.61 nm(-3)), respectively, has been computed by both the Feynman-Kleinert linearized path-integral (FK-LPI) and Ring-Polymer Molecular Dynamics (RPMD) methods and compared with Inelastic X Ray Scattering spectra. The combined use of computational and experimental methods enabled us to reduce experimental uncertainties in the determination of the true sample spectrum. Furthermore, the refined experimental spectrum of para-hydrogen and ortho-deuterium is consistently reproduced by both FK-LPI and RPMD results at momentum transfers lower than 12.8 nm(-1). At larger momentum transfers the FK-LPI results agree with experiment much better for ortho-deuterium than for para-hydrogen. More specifically we found that for k similar to 20.0 nm(-1) para-hydrogen provides a test case for improved approximations to quantum dynamics. (C) 2014 AIP Publishing LLC. C1 [Smith, Kyle K. G.; Rossky, Peter J.] Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Smith, Kyle K. G.; Rossky, Peter J.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Poulsen, Jens Aage] Gothenburg Univ, Dept Phys Chem, S-41296 Gothenburg, Sweden. [Cunsolo, A.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Smith, KKG (reprint author), Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. EM kylesmith@utexas.edu; jens72@chem.gu.se; acunsolo@bnl.gov; peter.rossky@austin.utexas.edu RI Poulsen, Jens/A-6867-2010 FU U. S. National Science Foundation [CHE-0910499]; R. A. Welch Foundation [F-0019] FX P.J.R. acknowledges the support of this research by the U. S. National Science Foundation (CHE-0910499), with additional support provided by the R. A. Welch Foundation (F-0019). NR 33 TC 7 Z9 7 U1 1 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2014 VL 140 IS 3 AR 034501 DI 10.1063/1.4851997 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 302OM UT WOS:000330614400040 PM 25669394 ER PT J AU Ovchinnikova, OS Kjoller, K Hurst, GB Pelletier, DA Van Berkel, GJ AF Ovchinnikova, Olga S. Kjoller, Kevin Hurst, Gregory B. Pelletier, Dale A. Van Berkel, Gary J. TI Atomic Force Microscope Controlled Topographical Imaging and Proximal Probe Thermal Desorption/Ionization Mass Spectrometry Imaging SO ANALYTICAL CHEMISTRY LA English DT Article ID PSEUDOMONAS-CHLORORAPHIS PCL1391; EVOLVED GAS-ANALYSIS; ELECTROSPRAY-IONIZATION; ATMOSPHERIC-PRESSURE; IN-VIVO; BIOCONTROL; PHENAZINES; AERUGINOSA; BACTERIA; STRAIN AB This paper reports on the development of a hybrid atmospheric pressure atomic force microscopy/mass spectrometry imaging system utilizing nanothermal analysis probes for thermal desorption surface sampling with subsequent atmospheric pressure chemical ionization and mass analysis. The basic instrumental setup and the general operation of the system were discussed, and optimized performance metrics were presented. The ability to correlate topographic images of a surface with atomic force microscopy and a mass spectral chemical image of the same surface, utilizing the same probe without moving the sample from the system, was demonstrated. Co-registered mass spectral chemical images and atomic force microscopy topographical images were obtained from inked patterns on paper as well as from a living bacterial colony on an agar gel. Spatial resolution of the topography images based on pixel size (0.2 mu m x 0.8 mu m) was better than the resolution of the mass spectral images (2.5 mu m x 2.0 mu m), which were limited by current mass spectral data acquisition rate and system detection levels. C1 [Ovchinnikova, Olga S.; Hurst, Gregory B.; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. [Kjoller, Kevin] Anasys Instruments, Santa Barbara, CA 93101 USA. [Pelletier, Dale A.] Oak Ridge Natl Lab, Biosci Div, Biol & Nanoscale Syst Grp, Oak Ridge, TN 37831 USA. RP Van Berkel, GJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. EM vanberkelgj@ornl.gov OI Hurst, Gregory/0000-0002-7650-8009 FU U.S. Government [DE-AC05-00OR22725]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, United States Department of Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory (ORNL); Laboratory Directed Research and Development (LDRD) Program of ORNL FX This manuscript has been authored by a contractor of the U.S. Government under contract No. DE-AC05-00OR22725. Accordingly, the U.S. Government retains a paid-up, nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this contribution, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U.S. Government purposes.; Instrumental implementation, fundamental and metric studies were supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, United States Department of Energy under Contract DE-AC05-00OR22725 with Oak Ridge National Laboratory (ORNL), managed and operated by UT-Battelle, LLC. The work with and analysis of Pseudomonas species GM17 was funded by the Laboratory Directed Research and Development (LDRD) Program of ORNL. NR 47 TC 16 Z9 16 U1 4 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 21 PY 2014 VL 86 IS 2 BP 1083 EP 1090 DI 10.1021/ac4026576 PG 8 WC Chemistry, Analytical SC Chemistry GA 296SA UT WOS:000330204500018 PM 24377265 ER PT J AU Furnish, MD Alexander, CS Brown, JL Reinhart, WD AF Furnish, M. D. Alexander, C. S. Brown, J. L. Reinhart, W. D. TI 2169 steel waveform measurements for equation of state and strength determination SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FUSED-SILICA; SHOCK; SAPPHIRE; ALUMINUM AB In support of efforts to develop multiscale models of a variety of materials, we have performed a set of eleven gas gun impact experiments on 2169 steel, a high-strength austenitic stainless steel. These experiments provided carefully controlled shock, reshock, and release velocimetry data, with initial shock stresses ranging from 10 to 50 GPa. Both windowed and free-surface measurements on samples ranging in thickness from 1 to 5mm were made to increase the utility of the data set. Target physical phenomena included the elastic/plastic transition (Hugoniot elastic limit), the Hugoniot, any phase transition phenomena, and the release/reshock paths (windowed and free-surface), with associated strength information. The Hugoniot is nearly linear in U-S-u(p) space. Reshock tests with explosively welded impactors produced clean results, by contrast with earlier reshock tests with glued impactors which showed gap signatures. The free-surface samples, which were steps on a single piece of steel, showed lower wavespeeds for thin (1 mm) samples than for thicker (2 or 4 mm) samples. A preliminary strength analysis suggests the flow strength increases with stress from similar to 1 GPa to similar to 2.5 GPa over this range, consistent with other recent work but about 25% above the Steinberg model. (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Furnish, M. D.; Alexander, C. S.; Brown, J. L.; Reinhart, W. D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Furnish, MD (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We gratefully acknowledge the assistance of Tom Thornhill in fielding these shots at the Sandia STAR Facility, and of Heidi Anderson in building up the experiment hardware. Tom Thornhill and Keith Hodge set up the 19-beam VISAR system required for the optical timing method used in those same three shots. This work was performed in collaboration with Lawrence Livermore National Laboratory, and we gratefully acknowledge Mukul Kumar, Bryan Reed, and Jeff Florando of LLNL for helpful discussions. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 20 TC 2 Z9 3 U1 1 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 033511 DI 10.1063/1.4862277 PG 9 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500028 ER PT J AU Guss, P Foster, ME Wong, BM Doty, FP Shah, K Squillante, MR Shirwadkar, U Hawrami, R Tower, J Yuan, D AF Guss, Paul Foster, Michael E. Wong, Bryan M. Doty, F. Patrick Shah, Kanai Squillante, Michael R. Shirwadkar, Urmila Hawrami, Rastgo Tower, Joshua Yuan, Ding TI Results for aliovalent doping of CeBr3 with Ca2+ SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; GENERALIZED GRADIENT APPROXIMATION; ENERGY-RESOLUTION SCINTILLATOR; AUGMENTED-WAVE METHOD; OPTICAL-PROPERTIES; PIEZOELECTRIC PROPERTIES; ELECTRONIC-STRUCTURE; AB-INITIO; SPECTRA; CERAMICS AB Despite the outstanding scintillation performance characteristics of cerium tribromide (CeBr3) and cerium-activated lanthanum tribromide, their commercial availability and application are limited due to the difficulties of growing large, crack-free single crystals from these fragile materials. This investigation employed aliovalent doping to increase crystal strength while maintaining the optical properties of the crystal. One divalent dopant (Ca2+) was used as a dopant to strengthen CeBr3 without negatively impacting scintillation performance. Ingots containing nominal concentrations of 1.9% of the Ca2+ dopant were grown, i.e., 1.9% of the CeBr3 molecules were replaced by CaBr2 molecules, to match our target replacement of 1 out of 54 cerium atoms be replaced by a calcium atom. Precisely the mixture was composed of 2.26 g of CaBr2 added to 222.14 g of CeBr3. Preliminary scintillation measurements are presented for this aliovalently doped scintillator. Ca2+-doped CeBr3 exhibited little or no change in the peak fluorescence emission for 371 nm optical excitation for CeBr3. The structural, electronic, and optical properties of CeBr3 crystals were studied using the density functional theory within the generalized gradient approximation. Calculated lattice parameters are in agreement with the experimental data. The energy band structures and density of states were obtained. The optical properties of CeBr3, including the dielectric function, were calculated. (C) 2014 AIP Publishing LLC. C1 [Guss, Paul] Remote Sensing Lab Nellis, Las Vegas, NV 89193 USA. [Foster, Michael E.; Wong, Bryan M.; Doty, F. Patrick] Sandia Natl Labs, Dept Chem Mat, Livermore, CA 94551 USA. [Shah, Kanai; Squillante, Michael R.; Shirwadkar, Urmila; Hawrami, Rastgo; Tower, Joshua] Radiat Monitoring Devices Inc, Watertown, MA 02472 USA. [Yuan, Ding] Natl Secur Technol LLC, Los Alamos Operat, Los Alamos, NM 87544 USA. RP Guss, P (reprint author), Remote Sensing Lab Nellis, POB 98521, Las Vegas, NV 89193 USA. EM gusspp@nv.doe.gov RI Wong, Bryan/B-1663-2009 OI Wong, Bryan/0000-0002-3477-8043 FU U.S. Department of Energy [DE-AC52-06NA25946]; Site-Directed Research and Development Program FX This manuscript has been authored by National Security Technologies, LLC, under Contract No. DE-AC52-06NA25946 with the U.S. Department of Energy and supported by the Site-Directed Research and Development Program. The United States Government retains and the publisher, by accepting the article for publication, acknowledges a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 77 TC 21 Z9 21 U1 0 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 034908 DI 10.1063/1.4861647 PG 10 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500081 ER PT J AU Hui, ZZ Tang, XW Wei, RH Lei, HC Gao, GY Hu, L Yang, J Yang, ZR Song, WH Zhu, XB Sun, YP AF Hui, Zhenzhen Tang, Xianwu Wei, Renhuai Lei, Hechang Gao, Guanyin Hu, Ling Yang, Jie Yang, Zhaorong Song, Wenhai Zhu, Xuebin Sun, Yuping TI Upper critical field and vortex phase diagram of polycrystalline delta-Mo1-xZrxN thin films by sol-gel SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID CRITICAL-CURRENT-DENSITY; CHEMICAL SOLUTION DEPOSITION; HIGH-PRESSURE; GRAIN-GROWTH; FLUX JUMPS; MON FILMS; DELTA-MON; NITRIDES; SUPERCONDUCTIVITY; DEPENDENCE AB Upper critical field of polycrystalline delta-Mo1-xZrxN (0 <= x <= 0.3) thin films by sol-gel was investigated. It showed that the upper critical field was continuously improved with Zr doping content, and the improvement of similar to 10 T in upper critical field was mainly attributed to the combined effects of obvious enhancements in normal-state resistivity with slight changes in T-c, obvious decrease in crystallite/grain size and enhanced microstrains. Flux jump was observed in low-level doped thin films due to enhanced critical current density by Zr doping. Finally, the vortex phase diagram of delta-Mo0.95Zr0.05N thin films was presented, which will provide guidance for investigation about the vortex mechanisms of delta-Mo1-xZrxN thin films. (C) 2014 AIP Publishing LLC. C1 [Hui, Zhenzhen; Tang, Xianwu; Wei, Renhuai; Hu, Ling; Yang, Jie; Yang, Zhaorong; Song, Wenhai; Zhu, Xuebin; Sun, Yuping] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China. [Lei, Hechang] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Gao, Guanyin] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China. [Sun, Yuping] Chinese Acad Sci, High Field Magnet Lab, Hefei 230031, Peoples R China. RP Zhu, XB (reprint author), Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China. EM xbzhu@issp.ac.cn; ypsun@issp.ac.cn RI Yang, Jie/C-5109-2008; Zhu, Xuebin/B-1592-2010; 汤, 现武/J-8860-2014; LEI, Hechang/H-3278-2016; Wei, Renhuai/S-8414-2016; Gao, Guanyin/A-5686-2010 OI Yang, Jie/0000-0003-0641-6296; 汤, 现武/0000-0002-2287-699X; Wei, Renhuai/0000-0002-6090-9561; FU National Key Basic Research [2011CBA00111]; National Nature Science Foundation of China [11104001, 50802096, 11174288] FX This work is supported by the National Key Basic Research under Contract No. 2011CBA00111, and the National Nature Science Foundation of China under Contract Nos. 11104001, 50802096, and 11174288. NR 29 TC 0 Z9 0 U1 3 U2 32 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 033905 DI 10.1063/1.4862860 PG 6 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500053 ER PT J AU Liu, P Zhang, YW Xiao, HY Xiang, X Wang, XL Weber, WJ AF Liu, Peng Zhang, Yanwen Xiao, Haiyan Xiang, Xia Wang, Xuelin Weber, William J. TI Nonlinear luminescence response of CaF2:Eu and YAlO3:Ce to single-ion excitation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SCINTILLATION RESPONSE; CALCIUM-FLUORIDE; INORGANIC-SCINTILLATOR; PLASTIC SCINTILLATORS; ENERGY; RADIATION; CRYSTALS; DETECTOR; NONPROPORTIONALITY; MODEL AB Understanding scintillation physics and nonproportionality is essential to accelerate materials discovery that has been restricted due to the difficulties inherent to large crystal growth and complex nature of gamma-solid interaction. Taking advantage of less restrictive growth and deposition techniques for smaller crystal sizes or thin films and better fundamental understanding of ion-solid interactions, a unique ion approach is demonstrated to effectively screen candidate scintillators with relatively small size and evaluate their nonlinear scintillation response. Response of CaF2:Eu and YAlO3:Ce scintillators to single ions of H+, He+, and O3+ are measured by the corresponding pulse height over a continuous energy range using a time-of-flight-scintillator-photoelectric multiplier tube apparatus. Nonlinear response of the scintillators under ionizing ion irradiation is quantitatively evaluated by considering the energy partitioning process. In a differential energy deposition region with negligible displacement damage, the low, medium and high excitation energy deposition density (D-exci) can be produced by energetic H+, He+ and O3+ ions, respectively, and significantly different impacts on the response characteristics of these two benchmark scintillators are observed. For CaF2:Eu, the scintillation efficiency under ion irradiation monotonically decreases with increasing excitation-energy density. In contrast, the response efficiency of YAlO3:Ce scintillation initially increases with excitation-energy density at low excitation-energy densities, goes through a maximum, and then decreases with further increasing excitation-energy density. The fundamental mechanism causing these different response behaviours in the scintillators is based on the competition between the scintillation response and the nonradiative quenching process under different excitation densities, which is also the main origin of the nonlinear response of the scintillators to irradiation. (C) 2014 AIP Publishing LLC. C1 [Liu, Peng; Zhang, Yanwen; Xiao, Haiyan; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Liu, Peng; Wang, Xuelin] Shandong Univ, Sch Phys, Key Lab Particle Phys & Particle Irradiat MOE, Jinan 250100, Peoples R China. [Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Xiang, Xia] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. RP Liu, P (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM Zhangy1@ornl.gov RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division; China Scholarship Council (CSC); DOE Office of Biological and Environmental Research FX W. J. Weber, H. Xiao, and Y. Zhang were supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division. P. Liu was supported by the China Scholarship Council (CSC) overseas scholarship program. A portion of research was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 26 TC 3 Z9 3 U1 2 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 033108 DI 10.1063/1.4861152 PG 8 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500008 ER PT J AU Tschopp, MA Gao, F Yang, L Solanki, KN AF Tschopp, M. A. Gao, F. Yang, L. Solanki, K. N. TI Binding energetics of substitutional and interstitial helium and di-helium defects with grain boundary structure in alpha-Fe SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MONTE-CARLO SIMULATIONS; HE-VACANCY CLUSTERS; BCC IRON; MOLECULAR-DYNAMICS; DISPLACEMENT CASCADES; TENSILE-STRENGTH; ENERGY; FUSION; COPPER; IRRADIATION AB The formation/binding energetics and length scales associated with the interaction between He atoms and grain boundaries in BCC alpha-Fe were explored. Ten different low R grain boundaries from the < 100 > and < 110 > symmetric tilt grain boundary systems were used. In this work, we then calculated formation/binding energies for 1-2 He atoms in the substitutional and interstitial sites (HeV, He2V, HeInt, He(2)Int) at all potential grain boundary sites within 15 angstrom of the boundary (52 826 simulations total). The present results provide detailed information about the interaction energies and length scales of 1-2 He atoms with grain boundaries for the structures examined. A number of interesting new findings emerge from the present study. For instance, the Sigma 3(112) twin boundary in BCC Fe possesses a much smaller binding energy than other boundaries, which corresponds in long time dynamics simulations to the ability of an interstitial He defect to break away from the boundary in simulations on the order of nanoseconds. Additionally, positive correlations between the calculated formation/binding energies of the He defects (R>0.9) asserts that the local environment surrounding each site strongly influences the He defect energies and that highly accurate quantum mechanics calculations of lower order defects may be an adequate predictor of higher order defects. Various metrics to quantify or classify the local environment were compared with the He defect binding energies. The present work shows that the binding and formation energies for He defects are important for understanding the physics of He diffusion and trapping by grain boundaries, which can be important for modeling He interactions in polycrystalline steels. (C) 2014 AIP Publishing LLC. C1 [Tschopp, M. A.] US Army Res Lab, Dynam Res Corp, Aberdeen Proving Ground, MD 21005 USA. [Tschopp, M. A.] Mississippi State Univ, Ctr Adv Vehicular Syst, Starkville, MS 39762 USA. [Gao, F.; Yang, L.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Solanki, K. N.] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. RP Tschopp, MA (reprint author), US Army Res Lab, Dynam Res Corp, Aberdeen Proving Ground, MD 21005 USA. EM mark.tschopp@gatech.edu RI Solanki, Kiran/E-8337-2010; Tschopp, Mark/B-1594-2008 OI Tschopp, Mark/0000-0001-8471-5035 FU U.S. Department of Energy, Office of Fusion Energy Science [DE-AC06-76RLO 1830]; Alternate Sponsored Fellowship (ASF) at PNNL FX F. G. and L. Y. are grateful for the support by the U.S. Department of Energy, Office of Fusion Energy Science, under Contract No. DE-AC06-76RLO 1830. The authors would like to acknowledge the support and discussions with Xin Sun and Moe Khaleel at Pacific Northwest National Laboratory. The authors would also like to acknowledge G. Henkelman for aiding in implementing the long time dynamics algorithm into the molecular dynamics code utilized within. Last, the authors would like to acknowledge Joanna Sun, high school student supported by Alternate Sponsored Fellowship (ASF) at PNNL, for her contributions to this work. NR 83 TC 10 Z9 11 U1 6 U2 36 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 033503 DI 10.1063/1.4861719 PG 16 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500020 ER PT J AU Zhu, Q Ma, Q Buchholz, DB Chang, RPH Bedzyk, MJ Mason, TO AF Zhu, Q. Ma, Q. Buchholz, D. B. Chang, R. P. H. Bedzyk, M. J. Mason, T. O. TI Structural and physical properties of transparent conducting, amorphous Zn-doped SnO2 films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID OXIDE THIN-FILMS; PULSED-LASER DEPOSITION; ZINC-STANNATE; ELECTRICAL-PROPERTIES; COMBINATORIAL; TRANSISTORS AB The structural and physical properties of conducting amorphous Zn-doped SnO2 (a-ZTO) films, prepared by pulsed laser deposition, were investigated as functions of oxygen deposition pressure (pO(2)), composition, and thermal annealing. X-ray scattering and X-ray absorption spectroscopy measurements reveal that at higher pO(2), the a-ZTO films are highly transparent and have a structural framework similar to that found in crystalline (c-), rutile SnO2 in which the Sn4+ ion is octahedrally coordinated by 6 O2- ions. The Sn4+ ion in these films however has a coordination number (CN) smaller by 2%-3% than that in c-SnO2, indicating the presence of oxygen vacancies, which are the likely source of charge carriers. At lower pO(2), the a-ZTO films show a brownish tint and contain some 4-fold coordinated Sn2+ ions. Under no circumstances is the CN around the Zn2+ ion larger than 4, and the Zn-O bond is shorter than the Sn-O bond by 0.07 angstrom. The addition of Zn has no impact on the electroneutrality but improves significantly the thermal stability of the films. Structural changes due to pO(2), composition, and thermal annealing account well for the changes in the physical properties of a-ZTO films. (C) 2014 AIP Publishing LLC. C1 [Zhu, Q.; Buchholz, D. B.; Chang, R. P. H.; Bedzyk, M. J.; Mason, T. O.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ma, Q.] Argonne Natl Lab, Adv Photon Source, Northwestern Synchrotron Res Ctr, DND CAT, Argonne, IL 60439 USA. RP Ma, Q (reprint author), Argonne Natl Lab, Adv Photon Source, Northwestern Synchrotron Res Ctr, DND CAT, Argonne, IL 60439 USA. EM q-ma@northwestern.edu RI Chang, R.P.H/B-7505-2009; Bedzyk, Michael/B-7503-2009; Mason, Thomas/B-7528-2009 FU NSF [DMR-1121262]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001059]; NU Office of Research; E.I. DuPont de Nemours Co.; Dow Chemical Company; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Film growth, electrical characterization, GIXRD, and X-ray absorption measurements were supported by the NSF funded Materials Research Science and Engineering Center (MRSEC) at Northwestern under Grant No. DMR-1121262. Optical characterization and structural analysis was supported by the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award No. DE-SC0001059. GIXRD measurements used the NU-MRSEC supported X-ray Diffraction Facility. X-ray absorption and scattering measurements were conducted at the DND-CAT at the Advanced Photon Source (APS). DND-CAT is supported by the NU Office of Research, E.I. DuPont de Nemours & Co., and The Dow Chemical Company. Use of the APS was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 39 TC 10 Z9 10 U1 2 U2 57 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2014 VL 115 IS 3 AR 033512 DI 10.1063/1.4861378 PG 9 WC Physics, Applied SC Physics GA 302OV UT WOS:000330615500029 ER PT J AU Amole, C Ashkezari, MD Baquero-Ruiz, M Bertsche, W Butler, E Capra, A Cesar, CL Charlton, M Deller, A Evetts, N Eriksson, S Fajans, J Friesen, T Fujiwara, MC Gill, DR Gutierrez, A Hangst, JS Hardy, WN Hayden, ME Isaac, CA Jonsell, S Kurchaninov, L Little, A Madsen, N McKenna, JTK Menary, S Napoli, SC Olchanski, K Olin, A Pusa, P Rasmussen, CO Robicheaux, F Sarid, E Silveira, DM So, C Stracka, S Tharp, T Thompson, RI van der Werf, DP Wurtele, JS AF Amole, C. Ashkezari, M. D. Baquero-Ruiz, M. Bertsche, W. Butler, E. Capra, A. Cesar, C. L. Charlton, M. Deller, A. Evetts, N. Eriksson, S. Fajans, J. Friesen, T. Fujiwara, M. C. Gill, D. R. Gutierrez, A. Hangst, J. S. Hardy, W. N. Hayden, M. E. Isaac, C. A. Jonsell, S. Kurchaninov, L. Little, A. Madsen, N. McKenna, J. T. K. Menary, S. Napoli, S. C. Olchanski, K. Olin, A. Pusa, P. Rasmussen, C. O. Robicheaux, F. Sarid, E. Silveira, D. M. So, C. Stracka, S. Tharp, T. Thompson, R. I. van der Werf, D. P. Wurtele, J. S. TI In situ electromagnetic field diagnostics with an electron plasma in a Penning-Malmberg trap SO NEW JOURNAL OF PHYSICS LA English DT Article ID SINGLE-COMPONENT PLASMAS; MULTISPECIES ION-PLASMA; CYCLOTRON-RESONANCE; NONNEUTRAL PLASMAS; MASS MEASUREMENTS; MAGNETIC TRAP; ANTIHYDROGEN; SPECTROSCOPY; PRECISION; MODES AB We demonstrate a novel detection method for the cyclotron resonance frequency of an electron plasma in a Penning-Malmberg trap. With this technique, the electron plasma is used as an in situ diagnostic tool for the measurement of the static magnetic field and the microwave electric field in the trap. The cyclotron motion of the electron plasma is excited by microwave radiation and the temperature change of the plasma is measured non-destructively by monitoring the plasma's quadrupole mode frequency. The spatially resolved microwave electric field strength can be inferred from the plasma temperature change and the magnetic field is found through the cyclotron resonance frequency. These measurements were used extensively in the recently reported demonstration of resonant quantum interactions with antihydrogen. C1 [Amole, C.; Capra, A.; Menary, S.] York Univ, Dept Phys & Astron, Toronto, ON M3J 1P3, Canada. [Ashkezari, M. D.; Hayden, M. E.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Baquero-Ruiz, M.; Fajans, J.; Little, A.; So, C.; Tharp, T.; Wurtele, J. S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bertsche, W.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Bertsche, W.] Cockcroft Inst, Warrington WA4 4AD, Cheshire, England. [Butler, E.] CERN, Dept Phys, CH-1211 Geneva 23, Switzerland. [Cesar, C. L.; Silveira, D. M.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, Brazil. [Charlton, M.; Deller, A.; Eriksson, S.; Isaac, C. A.; Madsen, N.; van der Werf, D. P.] Swansea Univ, Coll Sci, Dept Phys, Swansea SA2 8PP, W Glam, Wales. [Evetts, N.; Gutierrez, A.; Hardy, W. N.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Fajans, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Friesen, T.; Thompson, R. I.] Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. [Fujiwara, M. C.; Gill, D. R.; Kurchaninov, L.; Olchanski, K.; Olin, A.; Stracka, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Hangst, J. S.; Rasmussen, C. O.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Jonsell, S.; Napoli, S. C.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [McKenna, J. T. K.; Pusa, P.] Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England. [Robicheaux, F.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Sarid, E.] NRCN Nucl Res Ctr, Dept Phys, IL-84190 Beer Sheva, Israel. RP Friesen, T (reprint author), Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. EM tim.friesen@ucalgary.ca RI Bertsche, William/A-3678-2012; Stracka, Simone/M-3931-2015; Jonsell, Svante/J-2251-2016; wurtele, Jonathan/J-6278-2016; Fajans, Joel/J-6597-2016; Robicheaux, Francis/F-4343-2014 OI Bertsche, William/0000-0002-6565-9282; Stracka, Simone/0000-0003-0013-4714; Jonsell, Svante/0000-0003-4969-1714; wurtele, Jonathan/0000-0001-8401-0297; Butler, Eoin/0000-0003-0947-7166; van der Werf, Dirk/0000-0001-5436-5214; Fajans, Joel/0000-0002-4403-6027; Robicheaux, Francis/0000-0002-8054-6040 FU CNPq, FINEP/RENAFAE (Brazil); ISF (Israel); FNU (Denmark); VR (Sweden); NSERC, NRC/TRIUMF, AITF, FQRNT (Canada); DOE, NSF (USA); EPSRC; Royal Society and the Leverhulme Trust (UK) FX This work was supported by CNPq, FINEP/RENAFAE (Brazil), ISF (Israel), FNU (Denmark), VR (Sweden), NSERC, NRC/TRIUMF, AITF, FQRNT (Canada), DOE, NSF (USA), EPSRC, the Royal Society and the Leverhulme Trust (UK). NR 29 TC 5 Z9 5 U1 0 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 21 PY 2014 VL 16 AR 013037 DI 10.1088/1367-2630/16/1/013037 PG 19 WC Physics, Multidisciplinary SC Physics GA 302SM UT WOS:000330625200004 ER PT J AU Matzke, NJ Shih, PM Kerfeld, CA AF Matzke, Nicholas J. Shih, Patrick M. Kerfeld, Cheryl A. TI Bayesian Analysis of Congruence of Core Genes in Prochlorococcus and Synechococcus and Implications on Horizontal Gene Transfer SO PLOS ONE LA English DT Article ID PHYLOGENETIC TREE SELECTION; GENOME EVOLUTION; PHOTOSYNTHESIS; CYANOBACTERIA; MODELS; CONFIDENCE; INFERENCE; ACCURACY; BACTERIA; SEQUENCE AB It is often suggested that horizontal gene transfer is so ubiquitous in microbes that the concept of a phylogenetic tree representing the pattern of vertical inheritance is oversimplified or even positively misleading. "Universal proteins" have been used to infer the organismal phylogeny, but have been criticized as being only the "tree of one percent." Currently, few options exist for those wishing to rigorously assess how well a universal protein phylogeny, based on a relative handful of well-conserved genes, represents the phylogenetic histories of hundreds of genes. Here, we address this problem by proposing a visualization method and a statistical test within a Bayesian framework. We use the genomes of marine cyanobacteria, a group thought to exhibit substantial amounts of HGT, as a test case. We take 379 orthologous gene families from 28 cyanobacteria genomes and estimate the Bayesian posterior distributions of trees - a "treecloud" - for each, as well as for a concatenated dataset based on putative "universal proteins." We then calculate the average distance between trees within and between all treeclouds on various metrics and visualize this high-dimensional space with non-metric multidimensional scaling (NMMDS). We show that the tree space is strongly clustered and that the universal protein treecloud is statistically significantly closer to the center of this tree space than any individual gene treecloud. We apply several commonly-used tests for incongruence/HGT and show that they agree HGT is rare in this dataset, but make different choices about which genes were subject to HGT. Our results show that the question of the representativeness of the "tree of one percent" is a quantitative empirical question, and that the phylogenetic central tendency is a meaningful observation even if many individual genes disagree due to the various sources of incongruence. C1 [Matzke, Nicholas J.] Univ Calif Berkeley, Dept Integrat Biol, Berkeley, CA 94720 USA. [Shih, Patrick M.; Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Kerfeld, Cheryl A.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. RP Kerfeld, CA (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM ckerfeld@lbl.gov RI Matzke, Nicholas/L-4109-2015 OI Matzke, Nicholas/0000-0002-8698-7656 FU National Science Foundation (NSF) [DEB-0919451]; Wang Fellowship; Tien Fellowship; Google Summer of Code grant; U.C. Berkeley; Department of Integrative Biology; Center for Theoretical and Evolutionary Genetics; John Huelsenbeck; NSF [MCB-0851070] FX NJM was supported by National Science Foundation (NSF) Grant DEB-0919451, a Wang Fellowship, and a Tien Fellowship, and a Google Summer of Code grant, as well as U.C. Berkeley, the Department of Integrative Biology, the Center for Theoretical and Evolutionary Genetics, and John Huelsenbeck. PMS and CAK were funded by NSF Grant MCB-0851070. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 45 TC 4 Z9 4 U1 2 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 21 PY 2014 VL 9 IS 1 AR e85103 DI 10.1371/journal.pone.0085103 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 297GT UT WOS:000330244500036 PM 24465485 ER PT J AU Ramanathan, A Savol, A Burger, V Chennubhotla, CS Agarwal, PK AF Ramanathan, Arvind Savol, Andrej Burger, Virginia Chennubhotla, Chakra S. Agarwal, Pratul K. TI Protein Conformational Populations and Functionally Relevant Substates SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID DIHYDROFOLATE-REDUCTASE; MOLECULAR-DYNAMICS; ENZYME CATALYSIS; BIOMOLECULAR SIMULATIONS; ENERGY LANDSCAPE; DRUG DISCOVERY; CHEMICAL STEP; STATES; COOPERATIVITY; FLUCTUATIONS AB Functioning proteins do not remain fixed in a unique structure, hut instead they sample a range of conformations facilitated by motions within the protein. Even in the native state, a protein exists as a collection of interconverting conformations driven by thermodynamic fluctuations. Motions on the fast time scale allow a protein to sample conformations in the nearby area of Its conformational landscape, while motions on slower time scales give it access to conformations In distal areas of the landscape. Emerging evidence indicates that protein landscapes contain conformational substates with dynamic and structural features that Support the designated function of the protein. Nuclear magnetic resonance (NMR) experiments provide information about conformational ensembles of proteins. X-ray crystallography allows researchers to identify the most populated states along the landscape, and computational simulations give atom-level information about the conformational substates of different proteins. This ability to characterize and obtain quantitative information about the conformational substates and the populations of proteins within them is allowing researchers to better understand the relationship between protein structure and dynamics and the mechanisms of protein function. In this Account, we discuss recent developments and challenges In the characterization of functionally relevant conformational populations and substates of proteins. In some enzymes, the sampling of functionally relevant conformational substates is connected to promoting the overall mechanism of catalysis. For example, the conformational landscape of the enzyme dihydrofolate reductase has multiple substates, which facilitate the binding and the release of the cofactor and substrate and catalyze the hydride transfer. For the enzyme cyclophilin A, computational simulations reveal that the long time scale Conformational fluctuations enable the enzyme to access conformational substates that allow it to attain the transition state, therefore promoting the reaction mechanism. In the long term, this emerging view Of proteins with conformational substates has broad implications for Improving our understanding of enzymes, enzyme engineering, and better drug design. Researchers have already used photoactivation to modulate protein conformations as a strategy to develop a hypercatalytic enzyme. In addition, the alteration of the conformational substates through binding of ligands at locations other than the active site provides the basis for the design of new medicines through allosteric modulation. C1 [Ramanathan, Arvind] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. [Savol, Andrej; Burger, Virginia] Univ Pittsburgh, Joint Carnegie Mellon Univ, PhD Program Computat Biol, Pittsburgh, PA 15260 USA. [Savol, Andrej; Burger, Virginia; Chennubhotla, Chakra S.] Univ Pittsburgh, Dept Computat & Syst Biol, Pittsburgh, PA 15260 USA. [Agarwal, Pratul K.] Annavitas Biosci, Knoxville, TN 37932 USA. [Agarwal, Pratul K.] Oak Ridge Natl Lab, Computat Biol Inst, Oak Ridge, TN 37831 USA. [Agarwal, Pratul K.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Chennubhotla, CS (reprint author), Univ Pittsburgh, Dept Computat & Syst Biol, Pittsburgh, PA 15260 USA. EM chakracs@pitt.edu; agarwalpk@ornl.gov OI /0000-0002-8612-4797 NR 54 TC 22 Z9 22 U1 3 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JAN 21 PY 2014 VL 47 IS 1 BP 149 EP 156 DI 10.1021/ar400084s PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 296RZ UT WOS:000330204400015 PM 23988159 ER PT J AU Milliron, DJ Buonsanti, R Llordes, A Helms, BA AF Milliron, Delia J. Buonsanti, Raffaella Llordes, Anna Helms, Brett A. TI Constructing Functional Mesostructured Materials from Colloidal Nanocrystal Building Blocks SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID FIELD-EFFECT TRANSISTORS; SOLAR-CELLS; MESOPOROUS MATERIALS; SUPERLATTICES; HETEROSTRUCTURES; FILMS; CONDUCTIVITY; COMPOSITES; ARCHITECTURES; TEMPERATURE AB Through synthesizing colloidal nanocrystals (NCs) in the organic phase, chemists gain fine control over their composition, size, and shape. Strategies for arranging them into ordered superlattices have followed closely behind synthetic advances. Nonetheless, the same hydrophobic ligands that help their assembly also severely limit interactions between adjacent nanocrystals. As a result, examples of nanocrystal-based materials whose functionality derives from their mesoscale structure have lagged well behind advances in synthesis and assembly. In this Account, we describe how recent insights into NC surface chemistry have fueled dramatic progress In functional mesostructures. In these constructs, intimate contact between NCs as well as with heterogeneous components is key In determining macroscopic behavior. The simplest mesoscale assemblies we consider are networks of NCs constructed by in situ replacement of their bulky, Insulating surface ligands with small molecules. Transistors are a test bed for understanding conductivity, setting the stage for new functionality. For instance, we demonstrated that by electrochemically charging and discharging networks of plasmonic metal oxide NCs, the transmittance of near infrared light can be strongly and reversibly modulated. When we assemble NCs with heterogeneous components, there is an even greater potential for generating complex functionality. Nanocomposites can exhibit favorable characteristics of their component materials, yet the interaction between components can also have a strong influence. Realizing such opportunities requires an intimate linking of embedded NCs to the surrounding matrix phase. We accomplish this link by coordinating inorganic anionic dusters directly to NC surfaces. By exploiting this connection, we found enhanced ionic conductivity in Ag2S-in-GeS2 nanocrystal-in-glass electrodes. In another example, we also found enhanced optical contrast when linking electrochromic niobium oxide to embedded tin-doped indium oxide (ITO) NCs. These dramatic effects emerge from reconstruction of the inorganic glass immediately adjacent to the NC interface. When co-assembling NCs with block copolymers, direct coordination of the Polymer to NC surfaces again opens new opportunities for functional mesoscale constructs. We strip NCs of their native ligands and: design block copolymers containing a NC tethering domain that bonds strongly, yet dynamically, to the resulting open. coordination sites. This strategy enables their co-assembly at high volume fractions of NCs and leads to well ordered mesoporus NC networks. We find these architectures to be exceptionally stable under chemical transformations. driven by cation. insertion, removal and exchange. These developments offer a modular toolbox for arranging NCs deliberately with respect to heterogeneous elements and open space. We have control over metrics that define such architectures from the atomic sole bonding and crystal structure through the mesoscale shapes and sizes and pore dimensions. By tuning these parameters and better understanding the interactions between components, we look forward to boundless opportunities to employ mesoscale structure; in tandem with composition, to develop functional materials. C1 [Milliron, Delia J.; Buonsanti, Raffaella; Llordes, Anna; Helms, Brett A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Milliron, DJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM dmilliron@lbl.gov RI Milliron, Delia/D-6002-2012; Llordes, Anna/H-2370-2015; Foundry, Molecular/G-9968-2014; OI Llordes, Anna/0000-0003-4169-9156; Helms, Brett/0000-0003-3925-4174 FU DOE Early Career Research Program [DE-ACO2-05CH11231]; Molecular Foundry, Lawrence Berkeley National Laboratory [DE-ACO2-05CH11231] FX Work was carried out at the Molecular Foundry, Lawrence Berkeley National Laboratory, and D.J.M. was' supported by a DOE Early Career Research Program, both under contract DE-ACO2-05CH11231. NR 52 TC 22 Z9 22 U1 16 U2 248 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD JAN 21 PY 2014 VL 47 IS 1 BP 236 EP 246 DI 10.1021/ar400133k PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA 296RZ UT WOS:000330204400023 PM 24004254 ER PT J AU McDonald, LW Campbell, JA Clark, SB AF McDonald, Luther W. Campbell, James A. Clark, Sue B. TI Failure of ESI Spectra to Represent Metal-Complex Solution Composition: A Study of Lanthanide-Carboxylate Complexes SO ANALYTICAL CHEMISTRY LA English DT Article ID ELECTROSPRAY MASS-SPECTROMETRY; LASER-INDUCED FLUORESCENCE; LIGAND SOLUTION EQUILIBRIA; NUCLEAR-FUEL SAMPLES; GAS-PHASE; CHARGED DROPLETS; ORGANOMETALLIC COMPOUNDS; ELEMENTAL SPECIATION; ION-SOURCE; IONIZATION AB Electrospray ionization-mass spectrometry (ESI-MS) shows great promise as a rapid method to identify metal ligand complexes in solution. However, its application for quantitative determination of the distribution of species present in complicated equilibria is still in its infancy, and a direct correlation between ions observed in the gas phase and species expected in solution must be made with caution. The present work focuses on a seemingly simple system; the complexation of lanthanide cations with the acetate ligand. Using a high resolution quadrupole time-of-flight mass spectrometer, ions created by electrospray of solutions containing trivalent neodymium and acetate were identified. The gas phase distribution of species was compared to the solution phase speciation predicted using thermodynamic complexation constants. Apparent gas phase speciation diagrams were constructed as a function of solution conditions and fragmentation potential. Despite the expected variability of metal ligand complexes as solution conditions change, the observed gas phase speciation was independent of the metal to ligand ratio but dependent on the operating conditions of the ESI-MS. C1 [McDonald, Luther W.; Clark, Sue B.] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [McDonald, Luther W.; Campbell, James A.] Pacific NW Natl Lab, Chem & Biol Signature Sci Grp, Richland, WA 99352 USA. RP Clark, SB (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. EM s_clark@wsu.edu FU Defense Threat Reduction Agency [HDTRA11010111]; U.S. Department of Energy, National Nuclear Security Administration [NA0000582]; Basic Energy Sciences [SC0004102] FX We gratefully acknowledge the Defense Threat Reduction Agency (Grant HDTRA11010111), the U.S. Department of Energy, National Nuclear Security Administration (Grant NA0000582), and Basic Energy Sciences (Grant SC0004102). NR 84 TC 11 Z9 11 U1 8 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 21 PY 2014 VL 86 IS 2 BP 1023 EP 1029 DI 10.1021/ac401751r PG 7 WC Chemistry, Analytical SC Chemistry GA 296SA UT WOS:000330204500010 PM 24350789 ER PT J AU Hanson, SK Mueller, AH Oldham, WJ AF Hanson, Susan K. Mueller, Alexander H. Oldham, Warren J., Jr. TI Klaui Ligand Thin Films for Rapid Plutonium Analysis by Alpha Spectrometry SO ANALYTICAL CHEMISTRY LA English DT Article ID EXTRACTION CHROMATOGRAPHY RESIN; NUCLEAR FORENSICS; ORGANOMETALLIC CHEMISTRY; MASS-SPECTROMETRY; CRYSTAL-STRUCTURE; OXYGEN; COMPLEXES; IDENTIFICATION; RADIONUCLIDES; COORDINATION AB As part of a nuclear forensics capability, rapid and effective methods to analyze for plutonium and other actinide metals are needed. A key requirement of these methods is that they afford a high chemical yield while still providing isotopic information necessary for forensic evaluation. Toward this objective, a new method for binding plutonium for analysis by alpha spectrometry has been developed. Thin films of Klaui-type tripodal oxygen donor ligands were prepared by spin-casting solutions onto glass substrates. Three different ligands were evaluated for plutonium binding, and the best results were obtained using the ethyl-substituted complex Na[Cp*Co(P(O)(OEt)(2))(3)], which bound 80-88% of the dissolved Pu under equilibrium conditions. The thin films are simple and inexpensive to prepare and exhibit excellent alpha spectral resolution, having line widths of similar to 33 keV. The method has been successfully applied to analyze for plutonium in both an archived nuclear debris sample and a certified environmental soil sample. The results obtained from the soil analysis are in good agreement with the certified values, demonstrating the effectiveness of the method for rapid plutonium analysis. C1 [Hanson, Susan K.; Mueller, Alexander H.; Oldham, Warren J., Jr.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Hanson, SK (reprint author), Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. EM skhanson@lanl.gov; woldham@lanl.gov FU National Center for Nuclear Security FX We are grateful to the LANL National Technical Nuclear Forensics program manager, George H. Brooks, Jr., for encouragement of this work and the National Center for Nuclear Security managed by NSTech for financial support. NR 32 TC 7 Z9 7 U1 3 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 21 PY 2014 VL 86 IS 2 BP 1153 EP 1159 DI 10.1021/ac402997e PG 7 WC Chemistry, Analytical SC Chemistry GA 296SA UT WOS:000330204500027 PM 24397315 ER PT J AU Augspurger, AE Stender, AS Han, R Fang, N AF Augspurger, Ashley E. Stender, Anthony S. Han, Rui Fang, Ning TI Detecting Plasmon Resonance Energy Transfer with Differential Interference Contrast Microscopy SO ANALYTICAL CHEMISTRY LA English DT Article ID CYTOCHROME-C; NANOPARTICLES; SPECTROSCOPY; NANOSENSORS; CELLS AB Gold nanoparticles are ideal probes for studying intracellular environments and energy transfer mechanisms due to their plasmonic properties. Plasmon resonance energy transfer (PRET) relies on a plasmonic nanoparticle to donate energy to a nearby resonant acceptor molecule, a process which can be observed due to the plasmonic quenching of the donor nanoparticle. In this study, a gold nanosphere was used as the plasmonic donor, while the metalloprotein cytochrome c was used as the acceptor molecule. Differential interference contrast (DIC) microscopy allows for simultaneous monitoring of complex environments and noble metal nanoparticles in real time. Using DIC and specially designed microfluidic channels, we were able to monitor PRET at the single gold particle level and observe the reversibility of PRET upon the introduction of phosphate-buffered saline to the channel. In an additional experiment, single gold particles were internalized by He La cells and were subsequently observed undergoing PRET as the cell hosts underwent morphological changes brought about by ethanol-induced apoptosis. C1 [Augspurger, Ashley E.; Stender, Anthony S.; Han, Rui; Fang, Ning] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Augspurger, Ashley E.; Stender, Anthony S.; Han, Rui; Fang, Ning] US DOE, Ames Lab, Ames, IA 50011 USA. RP Fang, N (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM nfang@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Ames Laboratory; Plant Sciences Institute at Iowa State University (bioimaging); U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This work was supported by U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Ames Laboratory (instrumentation) and the Plant Sciences Institute at Iowa State University (bioimaging). The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under contract no. DE-AC02-07CH11358. NR 22 TC 9 Z9 9 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 21 PY 2014 VL 86 IS 2 BP 1196 EP 1201 DI 10.1021/ac403347e PG 6 WC Chemistry, Analytical SC Chemistry GA 296SA UT WOS:000330204500032 PM 24377308 ER PT J AU Tran, TN Kosaraju, MG Tamamizu-Kato, S Akintunde, O Zheng, Y Bieicki, JK Pinkerton, K Uchida, K Lee, YY Narayanaswami, V AF Tran, Tuyen N. Kosaraju, Malathi G. Tamamizu-Kato, Shiori Akintunde, Olayemi Zheng, Ying Bieicki, John K. Pinkerton, Kent Uchida, Koji Lee, Yuan Yu Narayanaswami, Vasanthy TI Acrolein Modification Impairs Key Functional Features of Rat Apolipoprotein E: Identification of Modified Sites by Mass Spectrometry SO BIOCHEMISTRY LA English DT Article ID LOW-DENSITY-LIPOPROTEIN; REVERSE CHOLESTEROL TRANSPORT; HEPARAN-SULFATE PROTEOGLYCANS; RECEPTOR-BINDING DOMAIN; CORONARY-HEART-DISEASE; C-TERMINAL DOMAIN; OXIDATIVE STRESS; LIPID-BINDING; E DEFICIENCY; CELLULAR CHOLESTEROL AB Apolipoprotein E (apoE), an antiatherogenic apolipoprotein, plays a significant role in the metabolism of lipoproteins. It lowers plasma lipid levels by acting as a ligand for the low-density lipoprotein receptor (LDLr) family of proteins, in addition to playing a role in promoting macrophage cholesterol efflux in atherosclerotic lesions. The objective Of this study is to examine the effect of acrolein modification on the structure and function of rat apoE and to determine the sites and nature of modification by mass spectrometry. Acrolein is. a highly reactive aldehyde, which is generated endogenously as one of the products. of lipid peroxidation and is present in the environment in pollutants such as tobacco smoke and heated oils. In initial studies,. acrolein-modified apoE was identified by immunoprecipitation using an acrolein-lysine specific antibody in the plasma of 10-week old male rats that were exposed to filtered air (FA) or low doses of environmental tobacco smoke (ETS). While both groups displayed acrolein-modified apoE in the lipoprotein fraction, the ETS group had higher levels in the lipid-free fraction compared with the FA group. This observation provided the rationale to further investigate the effect of acrolein modification on rat apoE at a molecular level. Treatment of recombinant rat apoE with a 10-fold molar excess of acrolein resulted in (i) a significant decrease in lipid-binding and cholesterol efflux abilities, (ii) impairment in the LDLr- and heparin-binding capabilities, and (iii) significant alterations,in the overall stability of the protein. The disruption in the functional abilities is attributed directly, or indirectly to acrolein modification yielding an aldimine adduct at K149 and K155 (+38); a propanal adduct at K135 and K138 (+56); an N-epsilon-(3-methylpyridinium)lysine (MP-lysine). at K64, K67, and K254 (+76), and an N-epsilon-(3-formyl-3,4-dehydropiperidino)lysine (FDP-lysine) derivative at position K68 (+94), as determined by matrix-assisted laser desorption/ionization time of flight/time of flight mass spectrometry (MALDI-TOF/TOF MS). The loss of function may also be attributed to alterations in the overall fold of the protein as noted by changes in the guanidine HCl-induced unfolding pattern and to protein cross-linking. Overall, disruption of the structural and functional integrity of apoE by oxidative modification of essential lysine residues by acrolein is expected to affect its role in maintaining plasma cholesterol homeostasis and lead to dysregulation in lipid metabolism. C1 [Tran, Tuyen N.; Narayanaswami, Vasanthy] Calif State Univ Long Beach, Dept Chem & Biochem, Long Beach, CA 90840 USA. [Kosaraju, Malathi G.; Tamamizu-Kato, Shiori; Akintunde, Olayemi; Narayanaswami, Vasanthy] Childrens Hosp Oakland Res Inst, Ctr Prevent Obes Cardiovasc Dis & Diabet, Oakland, CA 94609 USA. [Zheng, Ying; Bieicki, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Donner Lab, Berkeley, CA 94720 USA. [Pinkerton, Kent] Univ Calif Davis, Ctr Hlth & Environm, Davis, CA 95601 USA. [Uchida, Koji] Nagoya Univ, Grad Sch Bioagr Sci, Nagoya, Aichi 4648601, Japan. [Lee, Yuan Yu] Calif State Univ Long Beach, Ctr Educ Prote Anal, Long Beach, CA 90840 USA. [Lee, Yuan Yu] Calif State Univ Long Beach, Inst Integrated Res Mat Environm & Soc, Long Beach, CA 90840 USA. RP Lee, YY (reprint author), Calif State Univ Long Beach, Ctr Educ Prote Anal, Long Beach, CA 90840 USA. EM YuanYu.lee@csulb.edu; vas.narayanaswami@csulb.edu FU Tobacco Related Disease Research Program. [TRDRP 17RT-0165]; NIH [GM105561, HL096365]; Drake Family Trust; American Heart Association; NSF/CSU-LSAMP [HRD-0802628]; Women & Philanthropy Scholarship; CSULB Ronald E. McNair Post-Baccalaureate Achievement Program FX This work was funded by the Tobacco Related Disease Research Program. (TRDRP 17RT-0165), NIH-GM105561 and HL096365, the Drake Family Trust (V.N.), American Heart Association (S.T.K.), NSF/CSU-LSAMP (HRD-0802628), Women & Philanthropy Scholarship, and the CSULB Ronald E. McNair Post-Baccalaureate Achievement Program (T.N.T.). NR 83 TC 3 Z9 3 U1 0 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JAN 21 PY 2014 VL 53 IS 2 BP 361 EP 375 DI 10.1021/bi401404u PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 296SD UT WOS:000330204800010 PM 24325674 ER PT J AU Ly, S Bourguet, F Fischer, NO Lau, EY Coleman, MA Laurence, TA AF Ly, Sonny Bourguet, Feliza Fischer, Nicholas O. Lau, Edmond Y. Coleman, Matthew A. Laurence, Ted A. TI Quantifying Interactions of a Membrane Protein Embedded in a Lipid Nanodisc using Fluorescence Correlation Spectroscopy SO BIOPHYSICAL JOURNAL LA English DT Article ID PHOSPHOLIPID-BILAYER NANODISCS; YERSINIA; MODEL; YOPB AB Using fluorescence correlation spectroscopy, we measured a dissociation constant of 20 nM between EGFP-labeled LcrV from Yersinia pestis and its cognate membrane-bound protein YopB inserted into a lipid nanodisc. The combination of fluorescence correlation spectroscopy and nanodisc technologies provides a powerful approach to accurately measure binding constants of interactions between membrane bound and soluble proteins in solution. Straightforward sample preparation, acquisition, and analysis procedures make this combined technology attractive for accurately measuring binding kinetics for this important class of protein-protein interactions. C1 [Ly, Sonny; Bourguet, Feliza; Fischer, Nicholas O.; Lau, Edmond Y.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Coleman, Matthew A.; Laurence, Ted A.] Univ Calif Davis, Dept Radiat Oncol, Sacramento, CA 95817 USA. RP Laurence, TA (reprint author), Univ Calif Davis, Dept Radiat Oncol, Sacramento, CA 95817 USA. EM coleman16@llnl.gov; laurence2@llnl.gov RI Laurence, Ted/E-4791-2011; OI Laurence, Ted/0000-0003-1474-779X; Coleman, Matthew/0000-0003-1389-4018 FU U.S. Department of Energy [DE-AC52-07NA27344] FX Work was performed under the auspices of the U.S. Department of Energy under contract No. DE-AC52-07NA27344 to the Lawrence Livermore National Laboratory. NR 13 TC 5 Z9 5 U1 0 U2 24 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 21 PY 2014 VL 106 IS 2 BP L5 EP L8 DI 10.1016/j.bpj.2013.12.014 PG 4 WC Biophysics SC Biophysics GA 295RF UT WOS:000330132500001 PM 24461026 ER PT J AU Heath, JE McKenna, SA Dewers, TA Roach, JD Kohos, PH AF Heath, Jason E. McKenna, Sean A. Dewers, Thomas A. Roach, Jesse D. Kohos, Peter H. TI Multiwell CO2 Injectivity: Impact of Boundary Conditions and Brine Extraction on Geologic CO2 Storage Efficiency and Pressure Buildup SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CARBON-DIOXIDE; SALINE FORMATIONS; SCALE; MANAGEMENT; CAPACITY; MAGNITUDE; CONSTRAIN; AQUIFERS AB CO2 storage efficiency is a metric that expresses the portion of the pore space of a subsurface geologic formation that is available to store CO2. Estimates of storage efficiency for large-scale geologic CO2 storage depend on a variety of factors including geologic properties and operational design. These factors govern estimates on CO2 storage resources, the longevity of storage sites, and potential pressure buildup in storage reservoirs. This study employs numerical modeling to quantify CO2 injection well numbers, well spacing, and storage efficiency as a function of geologic formation properties, open-versus-closed boundary conditions, and injection with or without brine extraction. The set of modeling runs is important as it allows the comparison of controlling factors on CO2 storage efficiency. Brine extraction in closed domains can result in storage efficiencies that are similar to those of injection in open-boundary domains. Geomechanical constraints on downhole pressure at both injection and extraction wells lower CO2 storage efficiency as compared to the idealized scenario in which the same volumes of CO2 and brine are injected and extracted, respectively. Geomechanical constraints should be taken into account to avoid potential damage to the storage site. C1 [Heath, Jason E.; Dewers, Thomas A.] Sandia Natl Labs, Dept Geomech, Albuquerque, NM 87815 USA. [McKenna, Sean A.] Sandia Natl Labs, Dept Geosci Res & Applicat, Albuquerque, NM 87815 USA. [Roach, Jesse D.; Kohos, Peter H.] Sandia Natl Labs, Dept Earth Syst Anal, Albuquerque, NM 87815 USA. RP Heath, JE (reprint author), Sandia Natl Labs, Dept Geomech, Albuquerque, NM 87815 USA. EM jeheath@sandia.gov FU U.S. Department of Energy's National Energy Technology Laboratory; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The U.S. Department of Energy's National Energy Technology Laboratory funded this research. We thank Andrea McNemar of NETL for a review of this manuscript. Sandia National Laboratories is a multiprogram laboratory managed. and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 35 TC 11 Z9 11 U1 1 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 21 PY 2014 VL 48 IS 2 BP 1067 EP 1074 DI 10.1021/es4017014 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 296SF UT WOS:000330205000030 PM 23971876 ER PT J AU Upadhyayula, VKK Meyer, DE Curran, MA Gonzalez, MA AF Upadhyayula, Venkata K. K. Meyer, David E. Curran, Mary Ann Gonzalez, Michael A. TI Evaluating the Environmental Impacts of a Nano-Enhanced Field Emission Display Using Life Cycle Assessment: A Screening-Level Study SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID WALL CARBON NANOTUBES; FLUIDIZED-BED; TOXICITY; ECOTOXICITY; NANOPARTICLES; RELEASE; SILVER; TIO2; FABRICATION; CATALYSTS AB Carbon nanotube (CNT) field emission displays (FEDs) are currently in the product development stage and are expected to be commercialized in the near future because they offer image quality and viewing angles comparable to a cathode ray tube (CRT) while using a thinner structure, similar to a liquid crystal display (LCD), and enable more efficient power consumption during use. To address concerns regarding the environmental performance of CNT-FEDs, a screening-level, cradle-to-grave life cycle assessment (LCA) was conducted based on a functional unit of 10 000 viewing hours, the viewing lifespan of a CNT-FED. Contribution analysis suggests the impacts for material acquisition and manufacturing are greater, than the combined impacts for use and end-of-life. A scenario analysis of the CNT paste composition identifies the metal components used in the paste are key contributors to the impacts of the upstream stages due to the impacts associated with metal preparation. Further improvement of the manufacturing impacts is possible by considering the use of plant-based oils, such as rapeseed oil, as alternatives to organic solvents for dispersion of CNTs. Given the differences in viewing lifespan, the impacts of the CNT-FED were compared with a LCD and a CRT display to provide more insight on how to improve the CNT-FED to make it a viable product alternative. When compared with CRT technology, CNT-FEDs show better environmental performance, whereas a comparison with LCD technology indicates the environmental impacts are roughly the same. Based on the results, the enhanced viewing capabilities of CNT-FEDs. will be a more viable display option if manufacturers can increase the product's expected viewing lifespan. C1 [Upadhyayula, Venkata K. K.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Meyer, David E.; Curran, Mary Ann; Gonzalez, Michael A.] US EPA, Syst Anal Branch, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. RP Meyer, DE (reprint author), US EPA, Syst Anal Branch, Natl Risk Management Res Lab, 26 West Martin Luther King Dr, Cincinnati, OH 45268 USA. EM Meyer.David@epa.gov OI Curran, Mary Ann/0000-0001-8565-9928 FU U.S. Environmental Protection Agency through its Office of Research and Development FX The U.S. Environmental Protection Agency through its Office of Research and Development funded the research described here. It has not been subjected to full Agency review and therefore does not necessarily reflect the views of the Agency, and no official endorsement should be inferred. This research was supported in part by an appointment of Dr. Venkata K.K. Upadhyayula in the Postdoctoral Research Program at the National Risk Management Research Laboratory, administered by the Oak Ridge Institute for Science and Education through Interagency Agreement No. DW 89- 92298301-0 between the U.S. Department of Energy and the U.S. Environmental Protection Agency. NR 65 TC 5 Z9 5 U1 7 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 21 PY 2014 VL 48 IS 2 BP 1194 EP 1205 DI 10.1021/es4034638 PG 12 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 296SF UT WOS:000330205000044 PM 24328392 ER PT J AU Luo, SS AF Luo, Shishi TI A unifying framework reveals key properties of multilevel selection SO JOURNAL OF THEORETICAL BIOLOGY LA English DT Article DE Stochastic processes; Group selection; Moran process; Public goods game ID EVOLUTIONARY DYNAMICS; INCLUSIVE FITNESS; SEXUAL CONFLICT; PRICE EQUATION; COOPERATION; VIRULENCE; HOST; EUSOCIALITY; POPULATIONS; COMPETITION AB Natural selection can act at multiple biological levels, often in opposing directions. Viral evolution is an important example, with selection occurring both within infected hosts and between hosts via transmission. A fast-replicating virus may outcompete a slower strain within the same host, however, if rapid viral replication incapacitates the host, this fast-replicating virus may not be transmitted as frequently as its slower counterpart. Such examples of antagonistic multilevel selection arise across biological taxa and scales, from microbial public goods production to male mating strategies. A general formalism for describing and analyzing these diverse systems can identify their common underlying properties. Here I introduce such a unifying framework, which can be intuitively visualized as a stochastic ball-and-urn process. This ball-and-urn process illustrates the dynamics of antagonistic selective forces and allows the systematic derivation of properties with little or no dependence on model parameterization. These properties are consistent with previous studies, both theoretical and empirical, of multilevel selection. In particular I show that selection at the group level is favored when group-level events occur frequently relative to individual-level events, when there is little or no mutation, and when there are many groups relative to the number of individuals in each group. This approach demonstrates how multilevel selection can be understood as a general biological phenomenon, and identifies recurring characteristics that may be independent of specific biological contexts. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Luo, Shishi] Duke Univ, Dept Math, Durham, NC 27708 USA. RP Luo, SS (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies CNLS & Theoret Biol & Bioph, MS B258, Los Alamos, NM 87545 USA. EM szl@math.duke.edu FU Duke Stern Fellowship; [NSF-EF-08-27416] FX Thanks to Katia Koelle, Rick Durrett, and Anand Pai for feedback on the manuscript, and Jonathan Mattingly, Mike Reed, and the Koelle Lab for helpful discussions. This work was supported by grant NSF-EF-08-27416 and the Duke Stern Fellowship. NR 47 TC 6 Z9 6 U1 2 U2 29 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-5193 EI 1095-8541 J9 J THEOR BIOL JI J. Theor. Biol. PD JAN 21 PY 2014 VL 341 BP 41 EP 52 DI 10.1016/j.jtbi.2013.09.024 PG 12 WC Biology; Mathematical & Computational Biology SC Life Sciences & Biomedicine - Other Topics; Mathematical & Computational Biology GA 295XL UT WOS:000330149600005 PM 24096098 ER PT J AU Ranitovic, P Hogle, CW Riviere, P Palacios, A Tong, XM Toshima, N Gonzalez-Castrillo, A Martin, L Martin, F Murnane, MM Kapteyn, H AF Ranitovic, Predrag Hogle, Craig W. Riviere, Paula Palacios, Alicia Tong, Xiao-Ming Toshima, Nobuyuki Gonzalez-Castrillo, Alberto Martin, Leigh Martin, Fernando Murnane, Margaret M. Kapteyn, Henry TI Attosecond vacuum UV coherent control of molecular dynamics SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE chemical dynamics; electron dynamics; ultrafast ID LASER CONTROL; 2-PHOTON TRANSITIONS; DOUBLE-SLIT; PHOTOIONIZATION; H-2; INTERFERENCES; DISSOCIATION; GENERATION; PULSES AB High harmonic light sources make it possible to access attosecond timescales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics, the concept of attosecond chemistry has not yet been realized; this is because excitation and manipulation of molecular orbitals requires precisely controlled attosecond waveforms in the deep UV, which have not yet been synthesized. Here, we present a unique approach using attosecond vacuum UV pulse-trains to coherently excite and control the outcome of a simple chemical reaction in a deuterium molecule in a non-Born-Oppenheimer regime. By controlling the interfering pathways of electron wave packets in the excited neutral and singly ionized molecule, we unambiguously show that we can switch the excited electronic state on attosecond timescales, coherently guide the nuclear wave packets to dictate the way a neutral molecule vibrates, and steer and manipulate the ionization and dissociation channels. Furthermore, through advanced theory, we succeed in rigorously modeling multiscale electron and nuclear quantum control in a molecule. The observed richness and complexity of the dynamics, even in this very simplest of molecules, is both remarkable and daunting, and presents intriguing new possibilities for bridging the gap between attosecond physics and attochemistry. C1 [Ranitovic, Predrag; Hogle, Craig W.; Martin, Leigh; Murnane, Margaret M.; Kapteyn, Henry] Univ Colorado, JILA, Boulder, CO 80309 USA. [Ranitovic, Predrag; Hogle, Craig W.; Martin, Leigh; Murnane, Margaret M.; Kapteyn, Henry] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Ranitovic, Predrag; Hogle, Craig W.; Martin, Leigh; Murnane, Margaret M.; Kapteyn, Henry] NIST, Boulder, CO 80309 USA. [Tong, Xiao-Ming; Toshima, Nobuyuki] Univ Tsukuba, Div Mat Sci, Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan. [Riviere, Paula; Palacios, Alicia; Gonzalez-Castrillo, Alberto; Martin, Fernando] Univ Autonoma Madrid, Dept Quim, E-28049 Madrid, Spain. [Ranitovic, Predrag] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Martin, Fernando] IMDEA Nanosci, Inst Madrileno Estudios Avanzados Nanociencia, Madrid, Spain. RP Murnane, MM (reprint author), Univ Colorado, JILA, Boulder, CO 80309 USA. EM murnane@jila.colorado.edu RI Tong, Xiao-Min/A-2748-2011; Martin, Fernando/C-3972-2014; Riviere, Paula/L-7373-2014; Xlic, Cost/N-2439-2014; Palacios, Alicia/J-6823-2012 OI Tong, Xiao-Min/0000-0003-4898-3491; Martin, Fernando/0000-0002-7529-925X; Riviere, Paula/0000-0002-8866-5845; Palacios, Alicia/0000-0001-6531-9926 FU Army Research Office; National Science Foundation Physics Frontier Center; European Research Council Advanced Grant [XCHEM 290853]; European Marie Curie Reintegration Grant [ATTOTREND]; European COST Actions [CM0702, CM1204]; European Initial Training Network CORINF, Ministerio de Ciencia e Innovacion Project (Spain) [FIS2010-15127, CSD 2007-00010]; ERA-Chemistry Project [PIM2010EEC-00751]; Japan Society for the Promotion of Science [C24540421]; HA-PACS (Highly Accelerated Parallel Advanced system for Computational Sciences) FX The experimental work was performed at JILA with support from the Army Research Office and the National Science Foundation Physics Frontier Center. The theoretical work was supported by the European Research Council Advanced Grant XCHEM 290853, European Marie Curie Reintegration Grant ATTOTREND, European COST Actions CM0702 and CM1204, European Initial Training Network CORINF, Ministerio de Ciencia e Innovacion Projects FIS2010-15127 and CSD 2007-00010 (Spain), and ERA-Chemistry Project PIM2010EEC-00751. X.-M.T. was supported by Japan Society for the Promotion of Science Grant-in-Aid for Scientific Research C24540421 and HA-PACS (Highly Accelerated Parallel Advanced system for Computational Sciences) Project for advanced interdisciplinary computational sciences by exascale computing technology. NR 29 TC 37 Z9 37 U1 7 U2 60 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 21 PY 2014 VL 111 IS 3 BP 912 EP 917 DI 10.1073/pnas.1321999111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 292UQ UT WOS:000329928400025 PM 24395768 ER PT J AU Chen, HH Cartmell, S Wang, Q Lozano, T Deng, ZD Li, HD Chen, XL Yuan, Y Gross, ME Carlson, TJ Xiao, J AF Chen, Honghao Cartmell, Samuel Wang, Qiang Lozano, Terence Deng, Z. Daniel Li, Huidong Chen, Xilin Yuan, Yong Gross, Mark E. Carlson, Thomas J. Xiao, Jie TI Micro-battery Development for Juvenile Salmon Acoustic Telemetry System Applications SO SCIENTIFIC REPORTS LA English DT Article ID THIONYL CHLORIDE BATTERY; LITHIUM BATTERIES; DISCHARGE CHARACTERISTICS; CELLS; PERFORMANCE; IMPEDANCE; TRACKING; DAMS AB The Endangered Species Act requires actions that improve the passage and survival rates for migrating salmonoids and other fish species that sustain injury and mortality when passing through hydroelectric dams. To develop a low-cost revolutionary acoustic transmitter that may be injected instead of surgically implanted into the fish, one major challenge that needs to be addressed is the micro-battery power source. This work focuses on the design and fabrication of micro-batteries for injectable fish tags. High pulse current and required service life have both been achieved as well as doubling the gravimetric energy density of the battery. The newly designed micro-batteries have intrinsically low impedance, leading to significantly improved electrochemical performances at low temperatures as compared with commercial SR416 batteries. Successful field trial by using the micro-battery powered transmitters injected into fish has been demonstrated, providing an exemplary model of transferring fundamental research into practical devices with controlled qualities. C1 [Chen, Honghao; Cartmell, Samuel; Wang, Qiang; Lozano, Terence; Deng, Z. Daniel; Li, Huidong; Chen, Xilin; Yuan, Yong; Gross, Mark E.; Carlson, Thomas J.; Xiao, Jie] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Deng, ZD (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99352 USA. EM zhiqun.deng@pnnl.gov; jie.xiao@pnnl.gov RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU U.S. Army Corps of Engineers, Portland District FX The work described in this article was funded by the U.S. Army Corps of Engineers, Portland District. Brad Eppard is the technical lead for the USACE, and we greatly appreciate his leadership and support of this research. The authors are also grateful to many staff of the Pacific Northwest National Laboratory for their technical help-including Tylor Abel, Duane Balvage, Andrea Currie, Jayson Martinez, Praveen Meduri, Mitchell Myjak and Jinshan Xu. The study was conducted at PNNL, operated in Richland, Washington, by Battelle for the U.S. Department of Energy. NR 29 TC 10 Z9 10 U1 4 U2 39 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 21 PY 2014 VL 4 AR 3790 DI 10.1038/srep03790 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 293SV UT WOS:000329994900002 PM 24445689 ER PT J AU Ishikawa, R Lupini, AR Oba, F Findlay, SD Shibata, N Taniguchi, T Watanabe, K Hayashi, H Sakai, T Tanaka, I Ikuhara, Y Pennycook, SJ AF Ishikawa, Ryo Lupini, Andrew R. Oba, Fumiyasu Findlay, Scott D. Shibata, Naoya Taniguchi, Takashi Watanabe, Kenji Hayashi, Hiroyuki Sakai, Toshifumi Tanaka, Isao Ikuhara, Yuichi Pennycook, Stephen J. TI Atomic Structure of Luminescent Centers in High-Efficiency Ce-doped w-AlN Single Crystal SO SCIENTIFIC REPORTS LA English DT Article ID AUGMENTED-WAVE METHOD; HIGH-PRESSURE; ELECTROLUMINESCENCE; CATHODOLUMINESCENCE; GROWTH; EARTH; AIN AB Rare-earth doped wurtzite-type aluminum nitride (w-AlN) has great potential for high-efficiency electroluminescent applications over a wide wavelength range. However, because of their large atomic size, it has been difficult to stably dope individual rare-earth atoms into the w-AlN host lattice. Here we use a reactive flux method under high pressure and high temperature to obtain cerium (Ce) doped w-AlN single crystals with pink-colored luminescence. In order to elucidate the atomic structure of the luminescent centers, we directly observe individual Ce dopants in w-AlN using annular dark-field scanning transmission electron microscopy. We find that Ce is incorporated as single, isolated atoms inside the w-AlN lattice occupying Al substitutional sites. This new synthesis method represents a new alternative strategy for doping size-mismatched functional atoms into wide band-gap materials. C1 [Ishikawa, Ryo; Lupini, Andrew R.; Pennycook, Stephen J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Oba, Fumiyasu; Hayashi, Hiroyuki; Sakai, Toshifumi; Tanaka, Isao] Kyoto Univ, Dept Mat Sci & Engn, Sakyo Ku, Kyoto 6068501, Japan. [Oba, Fumiyasu] Tokyo Inst Technol, Mat Res Ctr Element Strategy, Yokohama, Kanagawa 2268503, Japan. [Findlay, Scott D.] Monash Univ, Sch Phys, Clayton, Vic 3800, Australia. [Shibata, Naoya; Ikuhara, Yuichi] Univ Tokyo, Inst Engn Innovat, Bunkyo Ku, Tokyo 1138656, Japan. [Shibata, Naoya] Japan Sci & Technol Agcy, PRESTO, Kawaguchi, Saitama 3320012, Japan. [Taniguchi, Takashi; Watanabe, Kenji] Natl Inst Mat Sci, Adv Key Technol Div, Tsukuba, Ibaraki 3050044, Japan. [Tanaka, Isao; Ikuhara, Yuichi] Japan Fine Ceram Ctr, Nanostruct Res Lab, Atsuta Ku, Nagoya, Aichi 4568587, Japan. RP Ishikawa, R (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM ishikawa@sigma.t.u-tokyo.ac.jp RI Shibata, Naoya/E-5327-2013; Oba, Fumiyasu/J-9723-2014; Ishikawa, Ryo/M-4206-2014; Tanaka, Isao/B-5941-2009; Ikuhara, Yuichi/N-1001-2015; Ikuhara, Yuichi/F-3066-2010; TANIGUCHI, Takashi/H-2718-2011; WATANABE, Kenji/H-2825-2011; OI Ishikawa, Ryo/0000-0001-5801-0971; Ikuhara, Yuichi/0000-0003-3886-005X; WATANABE, Kenji/0000-0003-3701-8119; Findlay, Scott/0000-0003-4862-4827 FU JSPS [25106003, 25106005, 25106006]; Funding Program for World-Leading Innovation R&D on Science and Technology (FIRST Program); MEXT, Japan [12024046]; JSPS; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; MEXT Elements Strategy Initiative; Australian Research Council [DP110101570]; JSPS KAKENHI [23686093] FX This research was supported by a Grant-in-Aid for Scientific Research on Innovative Areas, "Nano Informatics" (Grant Nos. 25106003, 25106005, and 25106006) from JSPS, and "Funding Program for World-Leading Innovation R&D on Science and Technology (FIRST Program)." A part of this research was conducted in "Research Hub for Advanced Nano Characterization, The University of Tokyo," supported under "Nanotechnology Platform" (Project No. 12024046) by MEXT, Japan. R. I. acknowledges support from JSPS Postdoctoral Fellowship for Research Abroad. A. R. L. and S.J.P. acknowledge support by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. F.O. acknowledges support from MEXT Elements Strategy Initiative to Form Core Research Center. S. D. F acknowledges support under the Discovery Projects funding scheme of the Australian Research Council (Projects No DP110101570). N.S. acknowledges support from JSPS KAKENHI (Grant No. 23686093). The XANES measurements were carried out under the approval of the Photon Factory Program Advisory Committee (Proposal No. 2007G194). Computing resources of ACCMS at Kyoto University were used for the first-principles calculations. NR 30 TC 13 Z9 13 U1 2 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 21 PY 2014 VL 4 AR 3778 DI 10.1038/srep03778 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 293SO UT WOS:000329994200002 PM 24445335 ER PT J AU Leviner, LE Aalseth, CE Ahmed, MW Avignone, FT Back, HO Barabash, AS Boswell, M De Braeckeleer, L Brudanin, VB Chan, YD Egorov, VG Elliott, SR Gehman, VM Hossbach, TW Kephart, JD Kidd, MF Konovalov, SI Lesko, KT Li, JY Mei, DM Mikhailov, S Miley, H Radford, DC Reeves, J Sandukovsky, VG Umatov, VI Underwood, TA Tornow, W Wu, YK Young, AR AF Leviner, L. E. Aalseth, C. E. Ahmed, M. W. Avignone, F. T., III Back, H. O. Barabash, A. S. Boswell, M. De Braeckeleer, L. Brudanin, V. B. Chan, Y. -D. Egorov, V. G. Elliott, S. R. Gehman, V. M. Hossbach, T. W. Kephart, J. D. Kidd, M. F. Konovalov, S. I. Lesko, K. T. Li, Jingyi Mei, D. -M. Mikhailov, S. Miley, H. Radford, D. C. Reeves, J. Sandukovsky, V. G. Umatov, V. I. Underwood, T. A. Tornow, W. Wu, Y. K. Young, A. R. TI A segmented, enriched N-type germanium detector for neutrinoless double beta-decay experiments SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Double beta decay; Segmented; Germanium; Detector; Majorana; Neutrinoless ID RADIATION DETECTORS; RESOLUTION AB We present data characterizing the performance of the first segmented, N-type Ge detector, isotopically enriched to 85% Ge-76. This detector, based on the Ortec PT6 x 2 design and referred to as SEGA (Segmented, Enriched Germanium Assembly), was developed as a possible prototype for neutrinoless double beta-decay measurements by the MAJORANA collaboration. We present some of the general characteristics (including bias potential, efficiency, leakage current, and integral cross-talk) for this detector in its temporary cryostat. We also present an analysis of this resolution of the detector, and demonstrate that for all but two segments there is at least one channel that reaches the MAJORANA resolution goal below 4 keV FWHM at 2039 keV, and all channels are below 4.5 keV FWHM. (C) 2013 Elsevier B.V. All rights reserved. C1 [Leviner, L. E.; Back, H. O.; Kephart, J. D.; Young, A. R.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Leviner, L. E.; Ahmed, M. W.; Back, H. O.; De Braeckeleer, L.; Kephart, J. D.; Kidd, M. F.; Tornow, W.; Young, A. R.] Triangle Univ Nucl Lab, Durham, NC 27706 USA. [Ahmed, M. W.; De Braeckeleer, L.; Kidd, M. F.; Tornow, W.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Ahmed, M. W.] N Carolina Cent Univ, Dept Phys, Durham, NC USA. [Aalseth, C. E.; Avignone, F. T., III; Hossbach, T. W.; Kephart, J. D.; Miley, H.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Boswell, M.; Elliott, S. R.; Gehman, V. M.; Mei, D. -M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Chan, Y. -D.; Gehman, V. M.; Lesko, K. T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Radford, D. C.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Avignone, F. T., III] Univ S Carolina, Dept Phys, Columbia, SC 29208 USA. [Underwood, T. A.] AMETEK ORTEC, Oak Ridge, TN USA. [Reeves, J.] Reeves & Sons LLC, Richland, WA USA. [Li, Jingyi; Mikhailov, S.; Wu, Y. K.] Duke Univ, Free Electron Laser Lab, Durham, NC USA. [Barabash, A. S.; Konovalov, S. I.; Umatov, V. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Brudanin, V. B.; Egorov, V. G.; Sandukovsky, V. G.] Joint Inst Nucl Res Dubna, Dubna 141980, Moscow Oblast, Russia. [Kidd, M. F.] Tennessee Technol Univ, Cookeville, TN USA. [Mei, D. -M.] Univ S Dakota, Vermillion, SD 57069 USA. [Back, H. O.] Princeton Univ, Princeton, NJ 08544 USA. RP Leviner, LE (reprint author), N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. EM lelevine@ncsu.edu RI radford, David/A-3928-2015; Barabash, Alexander/S-8851-2016 FU Office of Science of the US Department of Energy (DOE) [DE-FG02-97ER41042] FX We would like to thank the TUNL technical staff for their many contributions towards this project. We would also like to acknowledge helpful discussion and feedback from A.W. Poon and R.D. Martin in the process of preparing this paper. This work was supported in part by the Office of Science of the US Department of Energy (DOE) under grant number DE-FG02-97ER41042. NR 33 TC 1 Z9 1 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 66 EP 77 DI 10.1016/j.nima.2013.08.081 PG 12 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600010 ER PT J AU Yan, ZW Gundiah, G Bizarri, GA Samulon, EC Derenzo, SE Bourret-Courchesne, ED AF Yan, Zewu Gundiah, Gautam Bizarri, Gregory A. Samulon, Eric C. Derenzo, Stephen E. Bourret-Courchesne, Edith D. TI Eu2+-activated BaCl2, BaBr2 and BaI2 scintillators revisited SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Barium iodide; Barium bromide; Barium chloride; gamma-Ray detectors; X-ray detectors; Scintillation properties ID COMMON INORGANIC SCINTILLATORS; HALIDE SCINTILLATORS; X-RAY; LUMINESCENCE; RADIATION; CRYSTAL; LIGHT AB We present new results obtained from single crystals of Ba binary halides of BaCl2, BaBr2 and BaI2 activated with Eu2+. While these compounds were known as scintillator materials, clue to improvements in the crystal growth process and availability of higher purity compounds, we obtained crystals with better performances than what have been reported before. The luminosities of BaCl2:5%Eu2+, BaBr2:5%Eu2+ and Bal(2):5%Eu2+ are about 90%, 70% and 60%, respectively, of their theoretical limit. (C) 2013 Elsevier B.V. All rights reserved. C1 [Yan, Zewu; Samulon, Eric C.; Bourret-Courchesne, Edith D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Gundiah, Gautam; Bizarri, Gregory A.; Derenzo, Stephen E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Yan, ZW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM zyan@lbl.gov FU U.S. Department of Homeland Security/DNDO; U.S. Department of Energy/NNSA/NA22; Lawrence Berkeley National Laboratory [DE-ACO2-05CH11231] FX This work was supported by the U.S. Department of Homeland Security/DNDO and the U.S. Department of Energy/NNSA/NA22 and was carried out at the Lawrence Berkeley National Laboratory under Contract No. DE-ACO2-05CH11231. NR 18 TC 10 Z9 11 U1 2 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 83 EP 87 DI 10.1016/j.nima.2013.09.021 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600012 ER PT J AU Zhang, F Muller, H Awes, TC Martoiu, S Kral, J Silvermyr, D Martinez, AT Huang, GM Zhou, DC AF Zhang, Fan Muller, Hans Awes, Terry. C. Martoiu, Sorin Kral, Jiri Silvermyr, David Martinez, Alfonso Tarazona Huang, Guangming Zhou, Daicui TI Point-to-point readout for the ALICE EMCal detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE ALICE calorimeter; GTL bus; Point-to-point links; Scalable Readout Unit; Event readout rate AB It is anticipated that the LHC will deliver Pb + Pb collisions at a minimum bias interaction rate of about 50 kHz after the second long shutdown of the LHC in 2018. This will be roughly two orders of magnitude greater than the current data recording rate capability of the ALICE experiment. Therefore a major upgrade of the ALICE detector is planned for the next shutdown to enable ALICE to record data at the full Pb + Pb minimum bias interaction rate delivered by the LHC. A new point-to-point readout system for the electromagnetic calorimeter (EMCal) of ALICE has been developed, to replace the legacy readout bus, that essentially accomplishes this goal, and is being installed during the current LHC shutdown (2013-2014). The new readout uses the existing EMCal front end electronics yet provides more than an order of magnitude decrease in the readout Lime, to about 21 mu s, with modest cost and effort. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhang, Fan; Zhou, Daicui] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Zhang, Fan; Zhou, Daicui] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Zhang, Fan; Huang, Guangming] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Zhang, Fan; Huang, Guangming] Cent China Normal Univ, Coll Phys Sci & Technol, Wuhan 430079, Peoples R China. [Muller, Hans; Martoiu, Sorin; Martinez, Alfonso Tarazona] CERN, PH Dept, CH-1211 Geneva 23, Switzerland. [Awes, Terry. C.; Silvermyr, David] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Kral, Jiri] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. RP Zhang, F (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. EM fanzhang.ccnu@gmail.com FU NSFC [11020101060, IRG11221504, 1005044]; 973 Grant of MOST of China [2013CB3837803]; CCNU [CCNU13F026, QLPL2011, P01]; China Scholarship Council; LHC ALICE project; RD51 WG5 group at CERN FX This work is supported by the LHC ALICE project and the RD51 WG5 group at CERN, the NSFC key Grant 11020101060, IRG11221504 and 1005044, the 973 Grant of MOST of China 2013CB3837803, CCNU key Grant CCNU13F026, the QLPL2011, P01, and the China Scholarship Council. We wish to thank Filippo Costa, from the DATE team at CERN, for his constant and patient support on the DATE configuration and DDL protocol. NR 18 TC 2 Z9 2 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 157 EP 162 DI 10.1016/j.nima.2013.09.023 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600022 ER PT J AU Perry, A Dickerson, C Ostroumov, PN Zinkann, G AF Perry, A. Dickerson, C. Ostroumov, P. N. Zinkann, G. TI Beam characterization of a new continuous wave radio frequency quadrupole accelerator SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Radio frequency quadrupole; Argonne tandem linac accelerator system; Bunch shape monitor; Transverse beam halo; Energy distribution ID PROBE AB A new Continuous Wave (CW) Radio Frequency Quadrupole (RFQ) for the ATLAS (Argonne Tandem Linac Accelerator System) Intensity Upgrade was developed, built and tested at Argonne National Laboratory. We present here a characterization of the RFQ output beam in the longitudinal phase space, as well as a measurement of the transverse beam halo. Measurement results are compared to simulations performed using the beam dynamics code TRACK. (C) 2013 Elsevier B.V. All rights reserved C1 [Perry, A.; Dickerson, C.; Ostroumov, P. N.; Zinkann, G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Perry, A.] IIT, Chicago, IL 60616 USA. RP Perry, A (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aperry4@hawk.iit.edu FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract no. DE-AC02-06CH11357. NR 10 TC 2 Z9 2 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 163 EP 168 DI 10.1016/j.nima.2013.08.002 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600023 ER PT J AU Amole, C Andresen, GB Ashkezari, MD Baquero-Ruiz, M Bertsche, W Bowe, PD Butler, E Capra, A Carpenter, PT Cesar, CL Chapman, S Charlton, M Deller, A Eriksson, S Escallier, J Fajans, J Friesen, T Fujiwara, MC Gill, DR Gutierrez, A Hangst, JS Hardy, WN Hayano, RS Hayden, ME Humphries, AJ Hurt, JL Hydomako, R Isaac, CA Jenkins, MJ Jonsell, S Jorgensen, LV Kerrigan, SJ Kurchaninov, L Madsen, N Morone, A McKenna, JTK Menary, S Nolan, P Olchanski, K Olin, A Parker, B Povilus, A Pusa, P Robicheaux, F Sarid, E Seddon, D El Nasr, SS Silveira, DM So, C Storey, JW Thompson, RI Thornhill, J Wells, D van der Werf, DP Wurtele, JS Yamazaki, Y AF Amole, C. Andresen, G. B. Ashkezari, M. D. Baquero-Ruiz, M. Bertsche, W. Bowe, P. D. Butler, E. Capra, A. Carpenter, P. T. Cesar, C. L. Chapman, S. Charlton, M. Deller, A. Eriksson, S. Escallier, J. Fajans, J. Friesen, T. Fujiwara, M. C. Gill, D. R. Gutierrez, A. Hangst, J. S. Hardy, W. N. Hayano, R. S. Hayden, M. E. Humphries, A. J. Hurt, J. L. Hydomako, R. Isaac, C. A. Jenkins, M. J. Jonsell, S. Jorgensen, L. V. Kerrigan, S. J. Kurchaninov, L. Madsen, N. Morone, A. McKenna, J. T. K. Menary, S. Nolan, P. Olchanski, K. Olin, A. Parker, B. Povilus, A. Pusa, P. Robicheaux, F. Sarid, E. Seddon, D. El Nasr, S. Seif Silveira, D. M. So, C. Storey, J. W. Thompson, R. I. Thornhill, J. Wells, D. van der Werf, D. P. Wurtele, J. S. Yamazaki, Y. CA ALPHA Collaboration TI The ALPHA antihydrogen trapping apparatus SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Antihydrogen; Antiprotons; Positrons; Neutral atom trap; Microwaves; Silicon Vertex Detector ID PURE ELECTRON-PLASMA; AUTORESONANT NONSTATIONARY EXCITATION; NONNEUTRAL PLASMAS; CONFINEMENT; ATOMS; MOLECULES; MODES; FIELD AB The ALPHA collaboration, based at CERN, has recently succeeded in confining cold antihydrogen atoms in a magnetic minimum neutral atom trap and has performed the first study of a resonant transition of the anti-atoms. The ALPHA apparatus will be described herein, with emphasis on the structural aspects, diagnostic methods and techniques that have enabled antihydrogen trapping and experimentation to be achieved. (C) 2013 Elsevier B.V. All rights reserved. C1 [Amole, C.; Capra, A.; Menary, S.] York Univ, Dept Phys & Astron, Toronto, ON M3J 1P3, Canada. [Andresen, G. B.; Bowe, P. D.; Hangst, J. S.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Ashkezari, M. D.; Hayden, M. E.; Kerrigan, S. J.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Baquero-Ruiz, M.; Chapman, S.; Fajans, J.; Povilus, A.; So, C.; Wurtele, J. S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bertsche, W.; Charlton, M.; Deller, A.; Eriksson, S.; Humphries, A. J.; Isaac, C. A.; Jenkins, M. J.; Jorgensen, L. V.; Madsen, N.; van der Werf, D. P.] Swansea Univ, Dept Phys, Coll Sci, Swansea SA2 8PP, W Glam, Wales. [Bertsche, W.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Bertsche, W.] Cockcroft Inst, Warrington WA4 4AD, Cheshire, England. [Butler, E.] CERN, Dept Phys, CH-1211 Geneva 23, Switzerland. [Carpenter, P. T.; Hurt, J. L.; Robicheaux, F.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Cesar, C. L.; Silveira, D. M.] Univ Fed Rio de Janeiro, Inst Fis, BR-21941972 Rio De Janeiro, Brazil. [Escallier, J.; Morone, A.; Parker, B.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Friesen, T.; Hydomako, R.; Thompson, R. I.] Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. [Fujiwara, M. C.; Gill, D. R.; Kurchaninov, L.; Olchanski, K.; Olin, A.; Storey, J. W.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Gutierrez, A.; Hardy, W. N.; El Nasr, S. Seif] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Hayano, R. S.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Jonsell, S.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [McKenna, J. T. K.; Nolan, P.; Pusa, P.; Seddon, D.; Thornhill, J.; Wells, D.] Univ Liverpool, Dept Phys, Liverpool L6P 7ZE, Merseyside, England. [Sarid, E.] Nucl Res Ctr Negev, Dept Phys, IL-84190 Beer Sheva, Israel. [Yamazaki, Y.] RIKEN, Atom Phys Lab, Adv Sci Inst, Wako, Saitama 3510198, Japan. [Wurtele, J. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Yamazaki, Y.] Univ Tokyo, Grad Sch Arts & Sci, Tokyo 1538902, Japan. RP Amole, C (reprint author), York Univ, Dept Phys & Astron, Toronto, ON M3J 1P3, Canada. RI Bertsche, William/A-3678-2012; Hayano, Ryugo/F-7889-2012; Yamazaki, Yasunori/N-8018-2015; Jonsell, Svante/J-2251-2016; wurtele, Jonathan/J-6278-2016; Fajans, Joel/J-6597-2016; Robicheaux, Francis/F-4343-2014; OI Bertsche, William/0000-0002-6565-9282; Hayano, Ryugo/0000-0002-1214-7806; Yamazaki, Yasunori/0000-0001-5712-0853; Jonsell, Svante/0000-0003-4969-1714; wurtele, Jonathan/0000-0001-8401-0297; Fajans, Joel/0000-0002-4403-6027; van der Werf, Dirk/0000-0001-5436-5214; Robicheaux, Francis/0000-0002-8054-6040; Deller, Adam/0000-0002-3430-1501; Andresen, Gorm Bruun/0000-0002-4820-020X FU EPSRC (UK); Royal Society (UK); Leverhulme Trust (UK); CNPq (Brazil); FINEP (Brazil); ISF (Israel); FNU (Denmark); VR (Sweden); NSERC (Canada); NRC/TRIUMF (Canada); AIF (Canada); CIFAR (Canada); DOE (USA); NSF (USA); MEXT (Japan) FX Our work has been supported by a number of national funding agencies. We are grateful to: EPSRC, the Royal Society and the Leverhulme Trust (UK); CNPq and FINEP (Brazil); ISF (Israel); FNU (Denmark); VR (Sweden); NSERC, NRC/TRIUMF, AIF and CIFAR (Canada); DOE and NSF (USA); MEXT (Japan). We are very appreciative of the support we receive at CERN. NR 59 TC 19 Z9 19 U1 2 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 319 EP 340 DI 10.1016/j.nima.2013.09.043 PG 22 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600044 ER PT J AU Antolak, AJ Chen, AX Leung, KN Morse, DH Raber, TN AF Antolak, A. J. Chen, A. X. Leung, K. -N. Morse, D. H. Raber, T. N. TI Radiatively heated high voltage pyroelectric crystal pulser SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Pulser; High voltage; Pyroelectric crystal AB Thin lithium tantalate pyroelectric crystals in a multi stage pulser were heated by quartz lamps during their charging phase to generate high voltage pulses. The charging voltage was determined empirically based on the measured breakdown voltage in air and verified by the induced breakdown voltage of an external high voltage power supply. A four-stage pyroelectric crystal device generated pulse discharges of up to 86 kV using both quartz lamps (radiative) and thermoelectric (conductive) heating. Approximately 50 mJ of electrical energy was harvested from the crystals when radiatively heated in air, and up to 720 mJ was produced when the crystals were submerged in a dielectric fluid. It is anticipated that joule-level pulse discharges could be obtained by employing additional stages and optimizing the heating configuration. (C) 2013 Elsevier B.V. All rights reserved. C1 [Antolak, A. J.; Chen, A. X.; Leung, K. -N.; Morse, D. H.; Raber, T. N.] Sandia Natl Labs, Livermore, CA 94550 USA. [Leung, K. -N.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Antolak, AJ (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM antolak@sandia.gov FU Office of Nonproliferation Research and Development [DOE/NA-22]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by DOE/NA-22 Office of Nonproliferation Research and Development. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000, NR 8 TC 0 Z9 0 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 379 EP 381 DI 10.1016/j.nima.2013.09.040 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600049 ER PT J AU Salas-Bacci, A McGaughey, PL Baessler, S Broussard, L Makela, MF Mirabal, J Pattie, RW Pocanic, D Sjue, SKL Penttila, SI Wilburn, WS Young, AR Zeck, BA Wang, Z AF Salas-Bacci, A. McGaughey, P. L. Baessler, S. Broussard, L. Makela, M. F. Mirabal, J. Pattie, R. W. Pocanic, D. Sjue, S. K. L. Penttila, S. I. Wilburn, W. S. Young, A. R. Zeck, B. A. Wang, Z. TI Characterization of large area, thick, and segmented silicon detectors for neutron beta-decay experiments SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Neutron beta decay; Silicon detector; Pulse height defect; Nuclear defect; Dead layer ID SURFACE-BARRIER DETECTOR; PULSE-HEIGHT DEFECTS; ALPHA-PARTICLES; STOPPING POWER; ENERGY-LOSS; HEAVY-IONS; SI; PROTONS; NUCLEAR AB The "Nab" and "UCNB" col laborations have proposed to measure the correlation parameters in neutron p decay at Oak Ridge and Los Alamos National Laboratory, using a novel detector design. Two large area, thick, hexagonal-segmented silicon detectors containing 127 pixels per detector will be used to detect the proton and electron from neutron decay. Both silicon detectors are connected by magnetic field lines of a few Tesla field strength, and set on an electrostatic potential, such that protons can be accelerated up to 30 key in order to be detected. Characteristics of the detector response to low energy conversion electrons and protons from 15 key to 35 key, including the evaluation of the dead layer thickness and other contributions to the pulse height defect for proton detection are presented for Si detectors of 0.5 mm and 1 mm of thickness. (C) 2013 Elsevier B.V. All rights reserved, C1 [Salas-Bacci, A.; Baessler, S.; Pocanic, D.] Univ Virginia, Charlottesville, VA 22904 USA. [Salas-Bacci, A.; McGaughey, P. L.; Makela, M. F.; Mirabal, J.; Sjue, S. K. L.; Wilburn, W. S.; Wang, Z.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Pattie, R. W.; Young, A. R.; Zeck, B. A.] N Carolina State Univ, Raleigh, NC 27695 USA. [Baessler, S.; Penttila, S. I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Broussard, L.] Duke Univ, Durham, NC 27708 USA. RP Salas-Bacci, A (reprint author), Univ Virginia, Charlottesville, VA 22904 USA. EM americo.salas.bacci.1@ohio.edu NR 39 TC 6 Z9 6 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 408 EP 415 DI 10.1010/j.nima.2013.09.059 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600053 ER PT J AU Doron, O Wielopolski, L Mitra, S Biegalski, S AF Doron, Oded Wielopolski, Lucian Mitra, Sudeep Biegalski, Steven TI MCNP benchmarking of an inelastic neutron scattering system for soil carbon analysis SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Monte Carlo; Soil analysis; Carbon; Benchmarking; Gamma-ray neutron transport ID RANGE AB We benchmark here a Monte Carlo model simulating an inelastic neutron scattering (INS) system for quantitative analysis of carbon in soil. Specifically, we compare the simulations with experimental results of copper foils activations, INS system calibration, INS system optimization of the height above the ground and comparing pulse height distributions due to Cs-137 and Co-60 sources. Most of the simulations and the measurements agree better than 10%, although some of them registered discrepancies larger than 20%. (C) 2013 Elsevier B.V. All rights reserved. C1 [Doron, Oded] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Wielopolski, Lucian; Mitra, Sudeep] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Biegalski, Steven] Univ Texas Austin, Austin, TX 78759 USA. RP Doron, O (reprint author), Sandia Natl Labs, 1515 Eubank,Bldg 758,MS 0406, Albuquerque, NM 87123 USA. EM odeddo@yahoo.com; lwielo@bnl.gov; smitra@bnl.gov; biegalski@mail.utexas.edu NR 18 TC 2 Z9 2 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 431 EP 436 DI 10.1010/j.nima.2013.09.049 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600056 ER PT J AU Liu, C Talman, R Krafft, G AF Liu, C. Talman, R. Krafft, G. TI Optics matching schemes for linac-based light source SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Optics matching; Linac-based light source; Undulator; Flux density; X-ray source ID CEBAF AB Despite its small average beam current limit, a linac has features that make it attractive as an X-ray source: high energy, ultra-low emittance and energy spread, and flexible beamline optics. Unlike a storage ring, in which an undulator radiation source necessarily is short and positioned at the electron beam waist, in a linac the undulator can be long and the electron beam can be adjustable to have a virtual waist far downstream towards the X-ray target to produce a convergent X-ray beam. Using a planned CEBAF beamline as an example, we show here that we can overcome a factor of 2000 in the beam current to produce a monochromatic hard X-ray source comparable with, or even exceeding, the performance of an X-ray line at a third-generation storage ring. Even with no monochromator, the X-ray energy bandwidth can be as small as 0.1%. We discuss the optimal conditions which produce maximum X-ray flux density by focusing the electron beam for twocases: one is based on the waist-at-target (WAT) scheme, while the other goes beyond the WAT scheme. Both cases were verified by simulations using the SRW code. (C) 2013 Elsevier B.V. All rights reserved. C1 [Liu, C.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Talman, R.] Cornell Univ, Ithaca, NY USA. [Krafft, G.] Jefferson Lab, Newport News, VA USA. [Krafft, G.] Old Dominion Univ, Norfolk, VA USA. RP Liu, C (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM cliu1@bnl.gov NR 18 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 512 EP 520 DI 10.1016/j.nima.2013.08.082 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600067 ER PT J AU Murokh, A Solovyov, V Agustsson, R O'Shea, FH Chubar, O Chen, Y Grandsaert, T AF Murokh, Alex Solovyov, Vyacheslav Agustsson, Ron O'Shea, Finn H. Chubar, Oleg Chen, Yung Grandsaert, Thomas, II TI Textured dysprosium and gadolinium poles for high-field, short-period hybrid undulators SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Dysprosium; Undulator; Material science ID MAGNETIC-PROPERTIES AB We discuss the feasibility of enhancement of the gap field in a short period hybrid undulator by using pole inserts with the saturation inductance B-s, over that of iron, 2 T. Dysprosium metal, with the saturation inductance of 34 T below 90 K, and Gadolinium with B-s=2.7 T, appear as good candidates as the optimized pole material. However, due to the high magnetic anisotropy of Dy, such a high level of magnetization can only be realized when the external field lies in the basal plane. This implies that the pole has to be single crystalline or highly textured. Considering that growing large, > 10 mm, Dy single crystals is difficult, we propose secondary recrystallization as a method to induce the required texture in thin Dy and Grl foils. The textured foils can be stacked to produce pole inserts of the desired geometry and orientation. Results of small-scale processing and magnetic measurements of thin (20-60 mu) foils provide evidence that the required texture quality can be achieved by a relatively simple sequence of heat treatments and cold rolling. The advantage of textured Dy and Grl poles is demonstrated in a several period Lest undulator. (C) 2013 Elsevier BM. All rights reserved. C1 [Murokh, Alex; Agustsson, Ron; O'Shea, Finn H.; Chen, Yung; Grandsaert, Thomas, II] RadiaBeam Technol Inc, Santa Monica, CA 90404 USA. [Solovyov, Vyacheslav; Chubar, Oleg] Brookhaven Natl Lab, Upton, NY 11973 USA. [O'Shea, Finn H.] Univ Calif Los Angeles, Dept Phys, Los Angeles, CA 90095 USA. RP O'Shea, FH (reprint author), RadiaBeam Technol Inc, 1717 Stewart St, Santa Monica, CA 90404 USA. EM oshea@radiabeam.com RI Chubar, Oleg/B-6286-2014; OI Solovyov, Vyacheslav/0000-0003-1879-9802 NR 21 TC 2 Z9 2 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 521 EP 527 DI 10.1016/j.nima.2013.10.020 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600068 ER PT J AU Dayman, KJ Coble, JB Orton, CR Schwantes, JM AF Dayman, Kenneth J. Coble, Jamie B. Orton, Christopher R. Schwantes, Jon M. TI Characterization of used nuclear fuel with multivariate analysis for process monitoring SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Burnup; Multivariate analysis; Process monitoring; Used nuclear fuel ID PARTIAL LEAST-SQUARES; FINANCIAL DISTRESS PREDICTION; SUPPORT VECTOR MACHINE; REPROCESSING FACILITIES; CLASSIFICATION; SPECTROSCOPY; CLASSIFIERS AB This paper presents initial development of a reactor type classifier that is used to select a reactor specific partial least squares model to predict used nuclear fuel burnup. Nuclide activities for prototypic used fuel samples were generated in ORIGEN-ARP and used to investigate techniques to characterize used nuclear Fuel in terms of reactor type (pressurized or boiling water reactor) and burnup. A variety of reactor type classification algorithms, including k-nearest neighbors, linear and quadratic discriminant analyses, and support vector machines, were evaluated to differentiate used fuel from pressurized and boiling water reactors. Then, reactor type-specific partial least squares models were developed to predict the burnup of the fuel. Using these reactor type-specific models instead of a model trained for all light water reactors improved the accuracy of burnup predictions. The developed classification and prediction models were combined and applied to a large dataset that included eight fuel assembly designs, two of which were not used in training the models, and spanned the range of the initial U-235 enrichment, cooling Lime, and burnup values expected of future commercial used fuel for reprocessing. Error rates were consistent across the range of considered enrichment, cooling time, and burnup values. Average absolute relative errors in burnup predictions for validation data both within and outside the training space were 0.0574% and 0.0597%, respectively. The errors seen in this work are artificially low, because the models were trained, optimized, and tested on simulated, noise-free data. However, these results indicate that the developed models may generalize well to new data and that the proposed approach constitutes a viable first step in developing a fuel characterization algorithm based on gamma spectra. (C) 2013 Elsevier B.V. All rights reserved, C1 [Dayman, Kenneth J.] Univ Texas Austin, Austin, TX 78758 USA. [Coble, Jamie B.; Orton, Christopher R.; Schwantes, Jon M.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Dayman, KJ (reprint author), Univ Texas Austin, Austin, TX 78758 USA. EM kenneth.dayman@gmail.com FU U.S. Department of Homeland Security [2012-DN-130-NF0001-02] FX This material is based upon work supported by the U.S. Department of Homeland Security under Grant Award Number, 2012-DN-130-NF0001-02. The views and conclusions contained in this document are those of the authors and should not be interpreted as necessarily representing the official policies, either expressed or implied, of the U.S. Department of Homeland Security. NR 38 TC 1 Z9 1 U1 0 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2014 VL 735 BP 624 EP 632 DI 10.1016/j.nima.2013.09.056 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258YM UT WOS:000327494600085 ER PT J AU Tran, T McCormac, K Li, JL Bi, ZH Wu, J AF Tran, Toan McCormac, Kathleen Li, Jianlin Bi, Zhonghe Wu, Ji TI Electrospun SnO2 and TiO2 Composite Nanofibers for Lithium Ion Batteries SO ELECTROCHIMICA ACTA LA English DT Article DE Titanium Oxide; Tin Oxide; Composite Nanofiber; Electrospin; Lithium ion battery ID NANOSTRUCTURES; GERMANIUM; CAPACITY; STORAGE; ANODES AB Three types of SnO2/TiO2 composite nanofibers (homogeneous SnO2/TiO2, heterogeneous SnO2/TiO2 and SnO2 NPs/TiO2) have been prepared via a facile electrospinning method combined with a sol-gel chemistry, whose electrochemical performance as anode materials in lithium-ion battery was evaluated and compared to that of pure TiO2 and SnO(2)electrospunnanofibers (NFs). Rutile phase TiO(2)nanofibers demonstrated an extremely stable but relatively low gravimetric specific capacity of similar to 80 mAh g(-1) when discharged at 100 mAg(-1). In contrast, rutile phase SnO(2)nanofibers showed a much more unstable but higher specific capacity, which dropped from initial 800 to similar to 35 mAh g(-1) after 50 cycles. The incorporation of structurally unstable SnO2 into stable TiO2 matrix can significantly improve both the cycling performance and specific capacity. These composite nanofibers possess a much higher initial gravimetric specific capacity (>500 mAh g(-1)) than rutile phase TiO(2)nanofibers and maintain superior capacity retention to pure SnO2 NFs. The enhanced cycling stability is attributed to the space confinement provided by the structurally stable TiO2, which finding can provide a beneficial guidance for future lithium ion battery electrode development. Published by Elsevier Ltd. C1 [Tran, Toan; McCormac, Kathleen; Wu, Ji] Georgia So Univ, Dept Chem, Statesboro, GA 30460 USA. [Li, Jianlin] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Bi, Zhonghe] Oak Ridge Natl Lab, Div Chem, Oak Ridge, TN 37831 USA. RP Wu, J (reprint author), Georgia So Univ, Dept Chem, 250 Forest Dr, Statesboro, GA 30460 USA. EM tt01505@georgiasouthern.edu; km07207@georgiasouthern.edu; lij4@ornl.gov; Biz1@ornl.gov RI WU, JI/J-4580-2016; OI Li, Jianlin/0000-0002-8710-9847 FU Georgia Southern University; U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Office of Energy Efficiency and Renewable Energy's Vehicle Technologies and Advanced Manufacturing Offices; ORNL's Laboratory Director's Research and Development Funds FX JW sincerely acknowledges the generous Start-up Funding provided by Georgia Southern University. KM deeply appreciates the financial support from Georgia Southern University for her Master's program. We thank Prof. Rafael Quirino for allowing us to use the micro-Raman spectroscope in his research lab at Georgia Southern University. Part of this research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the U.S. Department of Energy (DOE) under contract DE-AC05-00OR22725, was done in its Battery Manufacturing R&D Facility which has been sponsored by the Office of Energy Efficiency and Renewable Energy's Vehicle Technologies and Advanced Manufacturing Offices and by ORNL's Laboratory Director's Research and Development Funds. JL appreciates the instructive discussion and great help from Drs Claus Daniel and David Wood. NR 33 TC 18 Z9 18 U1 12 U2 169 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 20 PY 2014 VL 117 BP 68 EP 75 DI 10.1016/j.electacta.2013.11.101 PG 8 WC Electrochemistry SC Electrochemistry GA AC8VD UT WOS:000332812300010 ER PT J AU Zhang, N Zhang, S Du, CY Wang, ZB Shao, YY Kong, FD Lin, YH Yin, GP AF Zhang, Na Zhang, Sheng Du, Chunyu Wang, Zhenbo Shao, Yuyan Kong, Fandong Lin, Yuehe Yin, Geping TI Pt/Tin Oxide/Carbon Nanocomposites as Promising Oxygen Reduction Electrocatalyst with Improved Stability and Activity SO ELECTROCHIMICA ACTA LA English DT Article DE Fuel cel ls; Oxygen reduction reaction; Pt/SnO2/C triple junction nanostructures; Pt nanoparticles; Stability ID PROTON-EXCHANGE MEMBRANE; PEM FUEL-CELLS; MONOLAYER ELECTROCATALYSTS; METHANOL OXIDATION; SNO2 NANOPARTICLES; ENHANCED ACTIVITY; CARBON NANOTUBES; CATALYST; ELECTRODES; SUPPORT AB In this report, a novel nanostructural Pt/SnO2/C catalyst was synthesized by depositing Pt nanoparticles on the SnO2/C surface. X-Ray Diffraction and Transmission Electron Microscopy characterizations showed that Pt nanoparticles with an average size of 2.7 nm were uniformly dispersed on the Pt/SnO2/C catalysts. High Resolution Transmission Electron Microscopy images revealed that Pt nanoparticles were bonded with both SnO2 and Cat the SnO2/C junctions, forming Pt/SnO2/C triple junction nanostructures in Pt/SnO2/C catalysts. Electrochemical measurements showed that specific activity towards oxygen reduction reaction (ORR) of Pt/SnO2/C catalysts was 2.3 times as high as that of conventional Pt/C catalysts. Accelerated degradation test (ADT) indicated that electrochemical stability of Pt/SnO2/C was twice as high as that of conventional Pt/C catalysts. The improved performance can be attributed to the presence of Pt/SnO2/C triple junction nanostructures, in which Pt nanoparticles were thermodynamically favored to deposit at the SnO2/C junctions, and then be anchored simultaneously by both SnO2 and C. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Zhang, Na; Zhang, Sheng; Du, Chunyu; Wang, Zhenbo; Kong, Fandong; Yin, Geping] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. [Shao, Yuyan; Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. [Lin, Yuehe] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Yin, GP (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. EM yingeping@hit.edu.cn RI Zhang, Sheng/H-2452-2011; Shao, Yuyan/A-9911-2008; Lin, Yuehe/D-9762-2011 OI Zhang, Sheng/0000-0001-7532-1923; Shao, Yuyan/0000-0001-5735-2670; Lin, Yuehe/0000-0003-3791-7587 FU National Natural Science Foundation of China [50872027, 21106024, 21173062]; Fundamental Research Funds for the Central Universities [HIT.ICRST.2010006]; U.S. Department of Energy [DE-AC05-76RL01830] FX This work is financially supported by National Natural Science Foundation of China (Grant No. 50872027, 21106024, and 21173062), and Fundamental Research Funds for the Central Universities (HIT.ICRST.2010006). Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. NR 56 TC 12 Z9 12 U1 10 U2 98 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 20 PY 2014 VL 117 BP 413 EP 419 DI 10.1016/j.electacta.2013.11.139 PG 7 WC Electrochemistry SC Electrochemistry GA AC8VD UT WOS:000332812300052 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, YZ Ahmad, N Masoodi, AA Ahmed, I Ahn, SU Ahn, SA Aimo, I Aiola, S Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Awes, TC Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bairathi, V Bala, R Baldisseri, A Pedrosa, EBD Ban, J Baral, RC Barbera, R Barile, E Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, L Bianchi, N Bielcik, J Bielcikova, J Bilandzi, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bornschein, J Botje, M Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Caliva, A Villar, EC Camerini, P Roman, VC Romeo, GC Carena, F Carena, W Carminati, F Diaz, AC Castellanos, JC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contin, G Contreras, JG Cormier, TM Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dainese, A Dang, R Danu, A Das, K Das, D Das, I Dash, A Dash, S De, S Delagrange, H Deloff, A Denes, E Deppman, A de Barros, GOV De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S de Rooij, R Corchero, MAD Dietel, T Divia, R Di Bari, D Di Giglio, C Di Liberto, S Di Mauro, A Di Nezza, P Djuvsland, O Dobrin, A Dobrowolski, T Donigus, B Dordic, O Dubey, AK Dubla, A Ducroux, L Dupieux, P Majumdar, AKD Erasmo, GD Elia, D Emschermann, D Engel, H Erazmus, B Erdal, HA Eschweiler, D Espagnon, B Estienne, M Esumi, S Evans, D Evdokimov, S Eyyubova, G Fabris, D Faivre, J Falchieri, D Fantoni, A Fasel, M Fehlker, D Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floratos, E Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Girard, MF Gaardhoje, JJ Gagliardi, M Gago, A Gallio, M Gangadharan, DR Ganoti, R Garabatos, C Garcia-Solis, E Gargiulo, C Garishvili, I Gerhard, J Germain, M Gheata, A Gheata, M Ghidini, B Ghosh, P Gianotti, P Giubellino, P Gladysz-Dziadus, E Glassel, R Goerlich, L Gomez, R Gonzalez-Zamora, P Gorbunov, S Gotovac, S Graczykowski, LK Grajcarek, R Grelli, A Grigoras, C Grigoras, A Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Guilbaud, M Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Khan, KH Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hanratty, LD Hansen, A Harris, JW Hartmann, H Harton, A Hatzifotiadou, D Hayashi, S Hayrapetyan, A Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Herrmann, N Hess, BA Hetland, KF Hicks, B Hippolyte, B Hori, Y Hristov, R Hrivnacova, I Huang, M Humanic, TJ Hutter, D Hwang, DS Ilkaev, R Ilkiv, I Inaba, M Incani, E Innocenti, GM Ionita, C Ippolitov, M Irfan, M Ivanov, M Ivanov, V Ivanytskyi, O Jacholkowski, A Jacobs, PM Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalcher, S Kalinak, P Kalweit, A Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karpechev, E Kazantsev, A Kebschull, U Keidel, R Ketzer, B Khan, MM Khan, R Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, T Kim, B Kim, DJ Kim, DW Kim, JS Kim, M Kim, M Kim, S Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, J Klein-Bosingav, C Kluge, A Knichel, ML Knospe, AG Kobdaj, C Kohler, MK Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Konevskikh, A Kovalenko, V Kowalski, 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Zaviyalov, N. Zbroszczyk, H. Zelnicek, P. Zgura, I. S. Zhalov, M. Zhang, F. Zhang, Y. Zhang, H. Zhang, X. Zhou, D. Zhou, Y. Zhou, F. Zhu, X. Zhu, J. Zhu, J. Zhu, H. Zichichi, A. Zimmermann, M. B. Zimmermann, A. Zinoyjev, G. Zoccarato, Y. Zynovyey, M. Zyzak, M. CA ALICE Collaboration TI Multiplicity dependence of pion, kaon, proton and lambda production in p-Pb collisions at root s(NN)=5.02 TeV SO PHYSICS LETTERS B LA English DT Article ID FINITE-TEMPERATURE; PPB COLLISIONS; LHC; ALICE; QUARK; QCD; ROOT-S=0.9; SPECTRUM; DETECTOR; NUCLEI AB In this Letter, comprehensive results on pi(+/-), K-+/-, K-S(0), p((p) over bar) and A((A) over bar) production at mid-rapidity (0 < y(CMS) < 0.5) in p-Pb collisions at root s(NN) = 5.02 TeV, measured by the ALICE detector at the LHC, are reported. The transverse momentum distributions exhibit a hardening as a function of event multiplicity, which is stronger for heavier particles. This behavior is similar to what has been observed in pp and Pb-Pb collisions at the LHC. The measured pr distributions are compared to d-Au, Au-Au and Pb-Pb results at lower energy and with predictions based on QCD-inspired and hydrodynamic models. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Grigoryan, A.; Gulkanyan, H.; Hayrapetyan, A.; Papikyan, V.] Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab Fdn, Yerevan 375036, Armenia. [Cortes Maldonado, I.; Fernandez Tellez, A.; Martinez, M. I.; Rodriguez Cahuantzi, M.; Tejeda Munoz, G.; Vargas, A.; Vergara, S.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Grinyov, B.; Ivanytskyi, O.; Martynov, Y.; Trubnikov, V.; Zinoyjev, G.; Zynovyey, M.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. [Pestov, Y.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. 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RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Castillo Castellanos, Javier/G-8915-2013; Guber, Fedor/I-4271-2013; Kucera, Vit/G-8459-2014; Vajzer, Michal/G-8469-2014; Krizek, Filip/G-8967-2014; Kovalenko, Vladimir/C-5709-2013; Bielcikova, Jana/G-9342-2014; Adamova, Dagmar/G-9789-2014; Bregant, Marco/I-7663-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Hladky, Jan/G-7953-2014; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vechernin, Vladimir/J-5832-2013; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; Pop, Petru /B-1895-2010; feofilov, grigory/A-2549-2013; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Takahashi, Jun/B-2946-2012; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Ahmed, Ijaz/E-9144-2015 OI Castillo Castellanos, Javier/0000-0002-5187-2779; Guber, Fedor/0000-0001-8790-3218; Kovalenko, Vladimir/0000-0001-6012-6615; Sevcenco, Adrian/0000-0002-4151-1056; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Gago Medina, Alberto Martin/0000-0002-0019-9692; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Bhasin, Anju/0000-0002-3687-8179; Turrisi, Rosario/0000-0002-5272-337X; D'Erasmo, Ginevra/0000-0003-3407-6962; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Takahashi, Jun/0000-0002-4091-1779; Barnby, Lee/0000-0001-7357-9904; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico; ALFA-EC; EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR (Autoritatea Nationala pentru Cercetare Stiintifica - ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas, and the State of Ohio FX The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR (Autoritatea Nationala pentru Cercetare Stiintifica - ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 68 TC 101 Z9 101 U1 8 U2 106 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 25 EP 38 DI 10.1016/j.physletb.2013.11.020 PG 14 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000006 ER PT J AU Eichten, E Martin, A AF Eichten, Estia Martin, Adam TI The muon collider as a H/A factory SO PHYSICS LETTERS B LA English DT Article ID MU(+)MU(-) COLLIDERS; ATLAS DETECTOR; HIGGS-BOSON; DARK-MATTER; SCALAR; SEARCH; MODEL; LHC; CP AB We show that a muon collider is ideally suited for the study of heavy H/A scalars, cousins of the Higgs boson found in two-Higgs-doublet models and required in supersymmetric models. The key aspects of H/A are: (1) they are narrow, yet have a width-to-mass ratio far larger than the expected muon collider beam-energy resolution, and (2) the larger muon Yukawa allows efficient s-channel production. We study in detail a representative Natural Supersymmetry model which has a 1.5 TeV H/A with m(H) - m(A) = 10 GeV. The large event rates at resonant peak allow the determination of the individual H and A resonance parameters (including CP) and the decays into electroweakinos provide a wealth of information unavailable to any other present or planned collider. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Eichten, Estia] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Martin, Adam] CERN, PH TH Dept, CH-1211 Geneva 23, Switzerland. [Martin, Adam] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. RP Martin, A (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. FU Fermilab by Fermi Research Alliance, LLC, U.S. Department of Energy [DE-AC02-07CH11359] FX We thank N. Craig for helpful discussions. This work was supported by Fermilab operated by Fermi Research Alliance, LLC, U.S. Department of Energy Contract DE-AC02-07CH11359 (EE). NR 51 TC 1 Z9 1 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 125 EP 130 DI 10.1016/j.physletb.2013.11.035 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000022 ER PT J AU Airapetian, A Akopov, N Akopov, Z Aschenauer, EC Augustyniak, W Avakian, R Avetissian, A Avetisyan, E Belostotski, S Bianchi, N Blok, HP Borissov, A Bowles, J Bryzgalov, V Burns, J Capiluppi, M Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Nardo, L De Sanctis, E Diefenthaler, M Di Nezza, P Duren, M Ehrenfried, M Elbakian, G Ellinghaus, F Fabbri, R Fantoni, A Felawka, L Frullani, S Gabbert, D Gapienko, G Gapienko, V Gavrilov, G Gharibyan, V Giordano, F Gliske, S Golembiovskaya, M Hadjidakis, C Hartig, M Hasch, D Hillenbrand, A Hoek, M Holler, Y Hristova, I Ivanilov, A Jackson, HE Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Korotkov, V Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lapikas, L Lehmann, I Lenisa, P Ruiz, AL Lorenzon, W Ma, BQ Mahon, D Makins, NCR Manaenkov, SI Mao, Y Marianski, B de la Ossa, AM Marukyan, H Miller, CA Miyachi, Y Movsisyan, A Murray, M Mussgiller, A Nappi, E Naryshkin, Y Negodaev, M Nowak, WD Pappalardo, LL Perez-Benito, R Petrosyan, A Raithel, M Reimer, PE Reolon, AR Riedl, C Rith, K Rosner, G Rostomyan, A Rubin, J Ryckbosch, D Salomatin, Y Sanftl, F Schafer, A Schnell, G Seitz, B Shibata, TA Shutov, V Stancari, M Statera, M Steffens, E Steiter, JJM Stewart, J Stinzing, F Taroian, S Terkulov, A Truty, R Trzcinski, A Tytgat, M Van Haarlem, Y Van Hulse, C Veretennikov, D Vikhrov, V Vilardi, I Wang, S Yaschenko, S Ye, Z Yen, S Yu, W Zagrebelnyy, V Zeiler, D Zihlmann, B Zupranski, P AF Airapetian, A. Akopov, N. Akopov, Z. Aschenauer, E. C. Augustyniak, W. Avakian, R. Avetissian, A. Avetisyan, E. Belostotski, S. Bianchi, N. Blok, H. P. Borissov, A. Bowles, J. Bryzgalov, V. Burns, J. Capiluppi, M. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Nardo, L. De Sanctis, E. Diefenthaler, M. Di Nezza, P. Dueren, M. Ehrenfried, M. Elbakian, G. Ellinghaus, F. Fabbri, R. Fantoni, A. Felawka, L. Frullani, S. Gabbert, D. Gapienko, G. Gapienko, V. Gavrilov, G. Gharibyan, V. Giordano, F. Gliske, S. Golembiovskaya, M. Hadjidakis, C. Hartig, M. Hasch, D. Hillenbrand, A. Hoek, M. Holler, Y. Hristova, I. Ivanilov, A. Jackson, H. E. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Korotkov, V. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lapikas, L. Lehmann, I. Lenisa, P. Lopez Ruiz, A. Lorenzon, W. Ma, B. -Q. Mahon, D. Makins, N. C. R. Manaenkov, S. I. Mao, Y. Marianski, B. Martinez de la Ossa, A. Marukyan, H. Miller, C. A. Miyachi, Y. Movsisyan, A. Murray, M. Mussgiller, A. Nappi, E. Naryshkin, Y. Negodaev, M. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Petrosyan, A. Raithel, M. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rosner, G. Rostomyan, A. Rubin, J. Ryckbosch, D. Salomatin, Y. Sanftl, F. Schaefer, A. Schnell, G. Seitz, B. Shibata, T. -A. Shutov, V. Stancari, M. Statera, M. Steffens, E. Steiter, J. J. M. Stewart, J. Stinzing, F. Taroian, S. Terkulov, A. Truty, R. Trzcinski, A. Tytgat, M. Van Haarlem, Y. Van Hulse, C. Veretennikov, D. Vikhrov, V. Vilardi, I. Wang, S. Yaschenko, S. Ye, Z. Yen, S. Yu, W. Zagrebelnyy, V. Zeiler, D. Zihlmann, B. Zupranski, P. CA HERMES Collaboration TI Transverse target single-spin asymmetry in inclusive electroproduction of charged pions and kaons SO PHYSICS LETTERS B LA English DT Article ID DEEP-INELASTIC SCATTERING; POLARIZED PROTON-BEAM; CHIRAL-ODD CONTRIBUTION; SIVERS ASYMMETRIES; ANALYZING POWER; 200 GEV/C; PI(0) PRODUCTION; HARD SCATTERING; CROSS-SECTIONS; ARROW-P AB Single-spin asymmetries were investigated in inclusive electroproduction of charged pions and kaons from transversely polarized protons at the HERMES experiment. The asymmetries were studied as a function of the azimuthal angle psi about the beam direction between the target-spin direction and the hadron production plane, the transverse hadron momentum P-T relative to the direction of the incident beam, and the Feynman variable x(F). The sin psi* amplitudes are positive for pi(+) and K+ slightly negative for pi(-) and consistent with zero for K-, with particular P-T but weak x(F) dependences. Especially large asymmetries are observed for two small subsamples of events, where also the scattered electron was recorded by the spectrometer. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Jackson, H. E.; Reimer, P. E.; Rubin, J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Nappi, E.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48011, Spain. [Ellinghaus, F.; Kinney, E.; Martinez de la Ossa, A.] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Akopov, Z.; Avetisyan, E.; Borissov, A.; Deconinck, W.; De Nardo, L.; Gavrilov, G.; Hartig, M.; Holler, Y.; Martinez de la Ossa, A.; Rostomyan, A.; Ye, Z.; Zagrebelnyy, V.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Fabbri, R.; Gabbert, D.; Golembiovskaya, M.; Hasch, D.; Hillenbrand, A.; Hristova, I.; Negodaev, M.; Nowak, W. -D.; Riedl, C.; Stewart, J.; Yaschenko, S.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.; Shutov, V.] Joint Inst Nucl Res, Dubna 141980, Russia. [Diefenthaler, M.; Kravchenko, P.; Mussgiller, A.; Raithel, M.; Rith, K.; Steffens, E.; Stinzing, F.; Yaschenko, S.; Zeiler, D.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Ist Nazl Fis Nucl, Sez Ferrara, I-44122 Ferrara, Italy. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Dipartimento Fis & Sci Terra, I-44122 Ferrara, Italy. [Belostotski, S.; Bianchi, N.; Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Fantoni, A.; Hadjidakis, C.; Hasch, D.; Reolon, A. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [De Nardo, L.; Lopez Ruiz, A.; Ryckbosch, D.; Schnell, G.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Airapetian, A.; Dueren, M.; Ehrenfried, M.; Keri, T.; Perez-Benito, R.; Yu, W.; Zagrebelnyy, V.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Bowles, J.; Burns, J.; Hoek, M.; Kaiser, R.; Keri, T.; Lehmann, I.; Mahon, D.; Murray, M.; Rosner, G.; Seitz, B.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Diefenthaler, M.; Giordano, F.; Joosten, S.; Makins, N. C. R.; Riedl, C.; Rubin, J.; Truty, R.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Airapetian, A.; Gliske, S.; Lorenzon, W.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.; Terkulov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Blok, H. P.; Lapikas, L.; Steiter, J. J. M.] Natl Inst Subat Phys Nikhef, NL-1009 DB Amsterdam, Netherlands. [Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Manaenkov, S. I.; Naryshkin, Y.; Veretennikov, D.; Vikhrov, V.] KP Konstantinov Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Bryzgalov, V.; Gapienko, G.; Gapienko, V.; Ivanilov, A.; Korotkov, V.; Salomatin, Y.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Sanftl, F.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Cisbani, E.; Frullani, S.] Ist Nazl Fis Nucl, Grp Collegato Saulta, Sez Roma, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.] Ist Super Sanita, I-00161 Rome, Italy. [De Nardo, L.; Felawka, L.; Gavrilov, G.; Miller, C. A.; Yen, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Sanftl, F.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Natl Ctr Nucl Res, PL-00689 Warsaw, Poland. [Akopov, N.; Avakian, R.; Avetissian, A.; Elbakian, G.; Gharibyan, V.; Karyan, G.; Marukyan, H.; Movsisyan, A.; Petrosyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Schnell, G (reprint author), Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. RI Negodaev, Mikhail/A-7026-2014; Taroian, Sarkis/E-1668-2014; Cisbani, Evaristo/C-9249-2011; Kozlov, Valentin/M-8000-2015; Terkulov, Adel/M-8581-2015; OI Cisbani, Evaristo/0000-0002-6774-8473; Lagamba, Luigi/0000-0002-0233-9812; Deconinck, Wouter/0000-0003-4033-6716 FU Ministry of Economy; Ministry of Education and Science of Armenia; FWO-Flanders; IWT, Belgium; Natural Sciences and Engineering Research Council of Canada; National Natural Science Foundation of China; Alexander von Humboldt Stiftung; German Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Italian Istituto Nazionale di Fisica Nucleare (INFN); MEXT; JSPS; G-COE of Japan; Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); Russian Academy of Science; Russian Federal Agency for Science and Innovations; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; U.K. Engineering and Physical Sciences Research Council; Science and Technology Facilities Council; Scottish Universities Physics Alliance; U.S. Department of Energy (DOE); National Science Foundation (NSF); European Community Research Infrastructure Integrating Activity [283286] FX We gratefully acknowledge the DESY management for its support and the staff at DESY and the collaborating institutions for their significant effort. This work was supported by the Ministry of Economy and the Ministry of Education and Science of Armenia; the FWO-Flanders and IWT, Belgium; the Natural Sciences and Engineering Research Council of Canada; the National Natural Science Foundation of China; the Alexander von Humboldt Stiftung, the German Bundesministerium fur Bildung und Forschung (BMBF), and the Deutsche Forschungsgemeinschaft (DFG); the Italian Istituto Nazionale di Fisica Nucleare (INFN); the MEXT, JSPS, and G-COE of Japan; the Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); the Russian Academy of Science and the Russian Federal Agency for Science and Innovations; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the U.K. Engineering and Physical Sciences Research Council, the Science and Technology Facilities Council, and the Scottish Universities Physics Alliance; the U.S. Department of Energy (DOE) and the National Science Foundation (NSF); as well as the European Community Research Infrastructure Integrating Activity under the FP7 "Study of strongly interacting matter (HadronPhysics3, Grant Agreement number 283286)". NR 72 TC 20 Z9 20 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 183 EP 190 DI 10.1016/j.physletb.2013.11.021 PG 8 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000031 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Ahmad, N Masoodi, AA Ahmed, I Ahn, SU Ahn, SA Aimo, I Aiola, S Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alexandre, D Alici, A Alkin, A Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Prado, CGA Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Awes, TC Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bairathi, V Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bornschein, J Botje, M Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Caliva, A Villa, EC Camerini, P Roman, VC Carena, F Carena, W Carminati, F Diaz, AC Castellanos, JC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contin, G Contreras, JG Cormier, TM Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Crochet, P Albinos, RC Cuautle, E Cunqueiro, L D'Erasmo, G Dainese, A Dang, R Danu, A Das, K Das, D Das, I Dash, A Dash, S De, S Delagrange, H Deloff, A Denes, E Deppman, A de Barros, GOV De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S de Rooij, R Corchero, MAD Dietel, T Divia, R Di Bari, D Di Giglio, C Di Liberto, S Di Mauro, A Di Nezza, P Djuvsland, O Dobrin, A Dobrowolski, T Donigus, B Dordic, O Dubey, AK Dubla, A Ducroux, L Dupieux, P Majumdar, AKD Elia, D Emschermann, D Engel, H Erazmus, B Erdal, HA Eschweiler, D Espagnon, B Estienne, M Esumi, S Evans, D Evdokimov, S Eyyubova, G Fabris, D Faivre, J Falchieri, D Fantoni, A Fasel, M Fehlker, D Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floratos, E Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Girard, MF Gaardhoje, JJ Gagliardi, M Gago, A Gallio, M Gangadharan, DR Ganoti, P Garabatos, C Garcia-Solis, E Gargiulo, C Garishvili, I Gerhard, J Germain, M Gheata, A Gheata, M Ghidini, B Ghosh, P Gianotti, P Giubellino, P Gladysz-Dziadus, E Glassel, P Goerlich, L Gomez, R Gonzalez-Zamora, P Gorbunov, S Gotovac, S Graczykowski, LK Grajcarek, R Grelli, A Grigoras, C Grigoras, A Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Guilbaud, M Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Khan, KH Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hanratty, LD Hansen, A Harris, JW Hartmann, H Harton, A Hatzifotiadou, D Hayashi, S Hayrapetyan, A Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Herrmann, N Hess, BA Hetland, KF Hicks, B Hippolyte, B Hori, Y Hristov, P Hrivnacova, I Huang, M Humanic, TJ Hutter, D Hwang, DS Ilkaev, R Ilkiv, I Inaba, M Incani, E Innocenti, GM Ionita, C Ippolitov, M Irfan, M Ivanov, M Ivanov, V Ivanytskyi, O Jacholkowski, A Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalcher, S Kalinak, P Kalweit, A Kang, JH Kaplin, V Kan, S Uysal, AK Karavichev, O Karavicheva, T Karpechev, E Kazantsev, A Kebschull, U Keidel, R Ketzer, B Khan, SA Khan, MM Khan, P Khanzadeev, A Kharlov, Y Kileng, B Kim, M Kim, M Kim, T Kim, JS Kim, DW Kim, DJ Kim, B Kim, S Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, J Klein-Bosing, C Kluge, A Knichel, ML Knospe, AG Kobdaj, C Kohler, MK Kollegger, T Kolojvari, A Kondratiev, V 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Uras, A. Urciuoli, G. M. Usai, G. L. Vajzer, M. Vala, M. Palomo, L. Valencia Vande Vyvre, P. Vannucci, L. Van Hoorne, J. W. van Leeuwen, M. Vargas, A. Varma, R. Vasileiou, M. Vasiliev, A. Vechernin, V. Veldhoen, M. Venaruzzov, M. Vercellin, E. Vergara, S. Vernet, R. Verweij, M. Vickovic, L. Viesti, G. Viinikainen, J. Vilakazi, Z. Baillie, O. Villalobos Vinogradov, A. Vinogradov, L. Vinogradov, Y. Virgili, T. Viyogi, Y. P. Vodopyanov, A. Voelkl, M. A. Voloshin, S. Voloshin, K. Volpe, G. von Haller, B. Vorobyev, I. Vranic, D. Vrlakova, J. Vulpescu, B. Vyushin, A. Wagner, B. Wagner, V. Wagner, J. Wang, Y. Wang, Y. Wang, M. Watanabe, D. Watanabe, K. Weber, M. Wessels, J. P. Westerhoff, U. Wiechula, J. Wiknet, J. Wilde, M. Wilk, G. Wilkinson, J. Williams, M. C. S. Windelband, B. Winn, M. Xiang, C. Yaldo, C. G. Yamaguchi, Y. Yang, H. Yang, P. Yang, S. Yano, S. Yasnopolskiy, S. Yi, J. Yin, Z. Yoo, I. -K. Yushmanov, I. Zaccolo, V. Zach, C. Zampolli, C. Zaporozhets, S. Zarochentsev, A. Zavada, P. Zaviyalov, N. Zbroszczyk, H. Zelnicek, P. Zgura, I. S. Zhalov, M. Zhang, F. Zhang, Y. Zhang, H. Zhang, X. Zhou, D. Zhou, Y. Zhou, F. Zhu, X. Zhu, J. Zhu, J. Zhu, H. Zichichi, A. Zimmermann, M. B. Zimmermann, A. Zinovjev, G. Zoccarato, Y. Zynovyev, M. Zyzak, M. CA ALICE Collaboration TI Multi-strange baryon production at mid-rapidity in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICS LETTERS B LA English DT Article ID QUARK-GLUON PLASMA; PROTON-PROTON COLLISIONS; HEAVY-ION COLLISIONS; NUCLEAR COLLISIONS; PP COLLISIONS; ALICE; ENERGY; LHC; ENHANCEMENT; DEPENDENCE AB The production of Xi(-) and Omega(-) baryons and their anti-particles in Pb-Pb collisions root s(NN) = 2.76 TeV has been measured using the ALICE detector. The transverse momentum spectra at mid-rapidity (vertical bar y vertical bar < 0.5) for charged Xi and Omega hyperons have been studied in the range 0.6 < P-T < 8.0 GeV/c and 1.2 < p(T) < 7.0 GeV/c, respectively, and in several centrality intervals (from the most central 0-.10% to the most peripheral 60-80% collisions). These spectra have been compared with the predictions of recent hydrodynamic models. In particular, the Krakow and EPOS models give a satisfactory description of the data, with the latter covering a wider P-T range. Mid-rapidity yields, integrated over p(T), have been determined. The hyperon-to-pion ratios are similar to those at RHIC: they rise smoothly with centrality up to < N-part > similar to 150 and saturate thereafter. The enhancements (yields per participant nucleon relative to those in pp collisions) increase both with the strangeness content of the baryon and with centrality, but are less pronounced than at lower energies. (C) 2013 The Authors. 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Martin; Mas, A.; Massacrier, L.; Pillot, P.; Schutz, Y.; Shabetai, A.; Stocco, D.] Univ Nantes, SUBATECH, Ecole Mines Nantes, CNRS IN2P3, Nantes, France. [Kobdaj, C.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Gomez, R.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Cosentino, M. R.; Deppman, A.; de Barros, G. O. V.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Moreira De Godoy, D. A.; Munhoz, M. G.; Oliveira Da Silva, A. C.; Pereira De Oliveira Filho, E.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas, UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Blanco, F.; Chinellato, D. D.; Jayarathna, P. H. S. Y.; Jena, S.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.; Weber, M.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Kral, J.; Morreale, A.; Rak, J.; Trzaska, W. H.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Figueredo, M. A. S.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Miake, Y.; Sakata, D.; Sano, M.; Watanabe, D.; Watanabe, K.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Planinic, M.; Simatovic, G.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Guilbaud, M.; Tieulent, R.; Uras, A.; Zoccarato, Y.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Vorobyev, I.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; De, S.; Dubey, A. K.; Ghosh, P.; Khan, S. A.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Langoy, R.; Lien, J.] Vestfold Univ Coll, Tonsberg, Norway. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pawlak, T.; Peryt, W.; Pluta, J.; Szymanski, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Agocs, A. G.; Barnaefoeldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Borissov, A.; Cormier, T. M.; Denes, E.; Dobrin, A.; Hamar, G.; Kiss, G.; Levai, P.; Loggins, V. R.; Mlynarz, J.; Molnar, L.; Olah, L.; Pochybova, S.; Prasad, S. K.; Pruneau, C. A.; Putschke, J.; Verweij, M.; Voloshin, S.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Adare, A. M.; Aiola, S.; Aronsson, T.; Caines, H.; Connors, M. E.; Harris, J. W.; Hicks, B.; Ma, R.; Oh, S.; Reed, R. J.; Schuster, T.; Smirnov, N.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Adare, A. M.; Aiola, S.; Aronsson, T.; Caines, H.; Connors, M. E.; Harris, J. W.; Ma, R.; Oh, S.; Reed, R. J.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, M.; Kim, T.; Kim, B.; Kwon, Y.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Zentrum Technol Transfer & Telekommunikat ZTT, Fachhsch Worms, Worms, Germany. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; Pop, Petru /B-1895-2010; feofilov, grigory/A-2549-2013; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Ahmed, Ijaz/E-9144-2015; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Kucera, Vit/G-8459-2014; Vajzer, Michal/G-8469-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Adamova, Dagmar/G-9789-2014; Takahashi, Jun/B-2946-2012; Castillo Castellanos, Javier/G-8915-2013; Guber, Fedor/I-4271-2013; Kovalenko, Vladimir/C-5709-2013; Bregant, Marco/I-7663-2012; OI Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Barnby, Lee/0000-0001-7357-9904; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Sevcenco, Adrian/0000-0002-4151-1056; Takahashi, Jun/0000-0002-4091-1779; Castillo Castellanos, Javier/0000-0002-5187-2779; Guber, Fedor/0000-0001-8790-3218; Kovalenko, Vladimir/0000-0001-6012-6615; D'Erasmo, Ginevra/0000-0003-3407-6962; Dainese, Andrea/0000-0002-2166-1874; Gago Medina, Alberto Martin/0000-0002-0019-9692; Paticchio, Vincenzo/0000-0002-2916-1671; Bhasin, Anju/0000-0002-3687-8179; Turrisi, Rosario/0000-0002-5272-337X FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT; DGAPA, Mexico; ALFA-EC; EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR (Autoritatea Nationala pentru Cercetare Stiintifica - ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Economia y Cornpetitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia; Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR (Autoritatea Nationala pentru Cercetare Stiintifica - ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Cornpetitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 65 TC 51 Z9 51 U1 3 U2 88 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 216 EP 227 DI 10.1016/j.physletb.2013.11.048 PG 12 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000037 ER PT J AU Naqvi, F Werner, V Petkov, P Ahn, T Cooper, N Ilie, G Radeck, D Bernards, C Carpenter, MP Chiara, CJ Janssens, RVF Kondev, FG Lauritsen, T Seweryniak, D Stoyanov, C Zhu, S AF Naqvi, F. Werner, V. Petkov, P. Ahn, T. Cooper, N. Ilie, G. Radeck, D. Bernards, C. Carpenter, M. P. Chiara, C. J. Janssens, R. V. F. Kondev, F. G. Lauritsen, T. Seweryniak, D. Stoyanov, Ch. Zhu, S. TI Test of the pi g(7/2) subshell closure at Z=58 SO PHYSICS LETTERS B LA English DT Article DE Nuclear g factors; Lifetimes; Coulomb excitation; Angular distributions ID MIXED-SYMMETRY; RECOIL; STATES; VACUUM; BA-128; BAND AB A simultaneous lifetime and relative g-factor measurement of the 2(1)(+) levels in Ce-138.142 was was performed using the Time Dependent Recoil Into Vacuum (TDRIV) technique. The excitation mechanism was Coulomb excitation in inverse kinematics, and the experimental setup included the Yale plunger device and the Gammasphere array. The latter was used to extract angular distributions for the 2(1)(+) -> 0(+) gamma-ray transitions at various target-to-stopper distances. A g(2(1)(+)) factor of 0.26(8) for Ce-138 was obtained relative to the literature value of g(2(1)(+)) = 0.21(5) in Ce-142. In addition, high-precision values of the B(E2; 2(1)(+) -> 0(+)) strengths were obtained. The new data support a proposed subshell closure for the pi g(7/2) orbital at Z = 58. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. Pi C1 [Naqvi, F.; Werner, V.; Ahn, T.; Cooper, N.; Ilie, G.; Bernards, C.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06511 USA. [Petkov, P.; Stoyanov, Ch.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, BU-1784 Sofia, Bulgaria. [Petkov, P.; Radeck, D.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Carpenter, M. P.; Chiara, C. J.; Janssens, R. V. F.; Kondev, F. G.; Lauritsen, T.; Seweryniak, D.; Zhu, S.] Argonne Natl Lab, Argonne, IL 60439 USA. [Chiara, C. J.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. RP Naqvi, F (reprint author), Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06511 USA. EM Farheen.Naqvi@yale.edu RI Bernards, Christian/C-4879-2013; Carpenter, Michael/E-4287-2015; Ahn, Tan/C-9158-2016; Werner, Volker/C-1181-2017 OI Bernards, Christian/0000-0001-5346-1415; Carpenter, Michael/0000-0002-3237-5734; Ahn, Tan/0000-0003-2249-7399; Werner, Volker/0000-0003-4001-0150 FU U.S. DOE, Office of Nuclear Physics [DE-FG02-91ER-40609, DE-AC02-06CH11357]; Bulgarian Science Foundation [DFNI-E 01/2]; DAAD German-Bulgarian exchange program [PPP 50751591, DNTS/01/2/2011] FX This work is supported by the U.S. DOE, Office of Nuclear Physics, under Grant No. DE-FG02-91ER-40609 and Contract No. DE-AC02-06CH11357. The support of Bulgarian Science Foundation under Contract No. DFNI-E 01/2 and NuPNET-SARFEN pi HC7P Pi 01/0003 is appreciated. Ch.S. acknowledges support by the DAAD German-Bulgarian exchange program under Grant Nos. PPP 50751591 and DNTS/01/2/2011. Discussions with A. Stuchbery are acknowledged. The authors are indebted to the ATLAS staff for providing excellent beam NR 34 TC 2 Z9 2 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 303 EP 307 DI 10.1016/j.physletb.2013.11.057 PG 5 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000049 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apollee, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T 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Zengel, K. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the mass difference between top and anti-top quarks in pp collisions at root s=7 TeV using the ATLAS detector SO PHYSICS LETTERS B LA English DT Article ID PARTON DISTRIBUTIONS; LHC AB A measurement of the mass difference between top and anti-top quarks is presented. In a 4.7 fb(-1) data sample of proton-proton collisions at root s = 7 TeV recorded with the ATLAS detector at the LHC, events consistent with t (t) over bar production and decay into a single charged lepton final state are reconstructed. For each event, the mass difference between the top and anti-top quark candidate is calculated. A two b-tag requirement is used in order to reduce the background contribution. A maximum likelihood fit to these per-event mass differences yields Delta m = m(t) - m((t) over bar) = 0.67 +/- 0.61 (stat) +/- 0.41 (syst) GeV, consistent with CPT invariance. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Jackson, B.; Soni, N.; White, M. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vaque, F. 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[Abajyan, T.; Arslan, O.; Backhaus, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Hageboeck, S.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, R.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; y Garzon, G. Otero; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duhrssen, M.; Ellis, N.; Elsing, M.; Facini, G.; Farthouat, P.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, R.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, A.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kueshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, R.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Willis, W.; Wulf, E.; Zhou, L.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Hoffmann, M. Dano; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, R.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, R.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, R.; Friedrich, E.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Ludwig, I.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Winklmeier, F.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, E.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, E.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Kei, M.; Knue, A.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Nadal, J.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subat & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzeel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Konoplich, R.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, E.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, E.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, Wj; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Donini, J.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mika, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mika, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, A.; Spano, F.; Teixeira-Dias, R.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, R.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, E.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, E.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, E.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Melrose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. 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G.; Schoening, A.; Schwienhorst, R.; Stelzer, B.; Ta, D.; Tollefson, K.; True, P.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, E.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, E.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. 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E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schweglerw, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, E.; de Asmundisa, R.; Della Pietra, M.; Della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengoa, R.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, S.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, R.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Oussoren, K. P.; Pani, R.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, R.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, E.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, B.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, E.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tanasijczuk, A. J.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apollee, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C. -L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dottiab, A.; Giannetti, P.; Roda, C.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dottiab, A.; Giannetti, P.; Roda, C.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Donini, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Batalha Pedro, R. Costa; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Tavares Delgado, A.; Veloso, E.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, R.; Staroba, R.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, R.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, R.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apollee, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazioab, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, R.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazioab, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, R.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Mijovic, L.; Mountricha, E.; Nguyen Thi Hong, V.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffe, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, DSM IRFU, Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Reece, R.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, M.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Backhaus, M.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, J.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, R.; Batkova, L.; Blazek, T.; Federic, R.; Stavina, R.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Seman, M.; Strizenec, R.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khanov, A.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, J.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, J.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, R.; Schramm, S.; Sinervo, R.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, R.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, 'I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J. -R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, R.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, E.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Research, Sch Phys Sci, Bhubaneswar, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Moscow, Russia. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Tikhomirova, V. O.] Moscow Engn & Phys Inst MEPh1, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Yang, Haijun/O-1055-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Lokajicek, Milos/G-7800-2014; Grinstein, Sebastian/N-3988-2014; Lei, Xiaowen/O-4348-2014; Wemans, Andre/A-6738-2012; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Boldyrev, Alexey/K-6303-2012; Moraes, Arthur/F-6478-2010; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Boyko, Igor/J-3659-2013; Fabbri, Laura/H-3442-2012; Ferrando, James/A-9192-2012; Deliot, Frederic/F-3321-2014; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Jakoubek, Tomas/G-8644-2014; Kupco, Alexander/G-9713-2014; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Solfaroli Camillocci, Elena/J-1596-2012; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016 OI Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Fassi, Farida/0000-0002-6423-7213; 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Lett. B PD JAN 20 PY 2014 VL 728 BP 363 EP 379 DI 10.1016/j.physletb.2013.12.010 PG 17 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000059 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, 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CA CMS Collaboration TI Determination of the top-quark pole mass and strong coupling constant from the t(t)over-bar production cross section in pp collisions at root s=7 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Top; Quark; Pair; Cross section; Mass; QCD; Strong; Coupling; Constant ID PARTON DISTRIBUTIONS; (MS)OVER-BAR MASSES; HIGGS-BOSON; LHC; JETS AB The inclusive cross section for top-quark pair production measured by the CMS experiment in protonproton collisions at a center-of-mass energy of 7 TeV is compared to the QCD prediction at next-to-next-to-leading order with various parton distribution functions to determine the top-quark pole mass, m(t)(pole), or the strong coupling constant, alpha(S). With the parton distribution function set NNPDF2.3, a pole mass of 176.7(-3.4)(+3.8) GeV is obtained when constraining alpha(S) at the scale of the Z boson mass, m(Z), to the current world average. Alternatively, by constraining m(t)(pole) to the latest average from direct mass measurements, a value of alpha(S)(m(Z)) = 0.1151(-0.0032)(+0.0033) is extracted. This is the first determination of alpha(S) using events from top-quark production. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [De Guio, F.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Bacchetta, N.; Bellato, M.; Biasotto, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Fanzago, E.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, R.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, R.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, R.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. I.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. I.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientate Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Lbarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.; Gonzalez Caballero, I.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Labo Instrumentac & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Laney, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Gavrilenko, M.; Epshteyn, V.; Erofeeva, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Savrin, V.; Tsirova, N.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, R.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Cifuentes, J. A. Brochero; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; David, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rojo, J.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.; Pieri, M.; George, C.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. 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H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, R.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, R.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Calderon, A.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Ricci-Tam, E.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Jandir, P.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Pierini, M.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT USA. [Ratnikov, F.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, E.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, R.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sander, C.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Stringer, R.; Wood, D.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, D.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. 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RI Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Yazgan, Efe/A-4915-2015; Ferguson, Thomas/O-3444-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Stahl, Achim/E-8846-2011; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Hill, Christopher/B-5371-2012; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Ragazzi, Stefano/D-2463-2009; Bartalini, Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Bonacorsi, Daniele/F-1505-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Codispoti, Giuseppe/F-6574-2014; Dudko, Lev/D-7127-2012; Bellan, Riccardo/G-2139-2014; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Novaes, Sergio/D-3532-2012; Torassa, Ezio/I-1788-2012; Da Silveira, Gustavo Gil/N-7279-2014; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Paulini, Manfred/N-7794-2014; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015 OI Ferguson, Thomas/0000-0001-5822-3731; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Stahl, Achim/0000-0002-8369-7506; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hill, Christopher/0000-0003-0059-0779; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Codispoti, Giuseppe/0000-0003-0217-7021; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Novaes, Sergio/0000-0003-0471-8549; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; TUVE', Cristina/0000-0003-0739-3153; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Rovelli, Tiziano/0000-0002-9746-4842; FU BMWF; FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP (Brazil); MES (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland; MEC; HIP (Finland); CEA; CNRS/IN2P3 (France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NKTH (Hungary); DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU (Republic of Korea); LAS (Lithuania); CINVESTAV; SEP; UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); NSC (Poland); FCT (Portugal); JINR (Dubna); MON; RosAtom; RAS; RFBR (Russia); MESTD (Serbia); SEIDI; CPAN (Spain); NSC (Taipei); ThEPCenter; IPST; STAR; NSTDA (Thailand); TUBITAK; TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE; NSF (USA) FX We thank Alexander Mitov for his help with the NNLO calculations. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 60 TC 44 Z9 45 U1 7 U2 91 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 496 EP 517 DI 10.1016/j.physletb.2013.12.009 PG 22 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000078 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, .S Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorima, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, E Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Lay, NBA Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansi, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, E da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJL Beermann, TA Bege, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J 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Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena in photon plus jet events collected in proton-proton collisions at root s=8 TeV with the ATLAS detector SO PHYSICS LETTERS B LA English DT Article ID EXCITED FERMIONS; HADRON COLLIDERS; MILLIMETER; DIMENSIONS; HERA AB This Letter describes a model-independent search for the production of new resonances in photon + jet (gamma + jet) events using 20 fb(-1) of proton-proton LHC data recorded with the ATLAS detector at a centre-of-mass energy of root s = 8 TeV. The gamma + jet mass distribution is compared to a background model fit from data; no significant deviation from the background-only hypothesis is found. Limits are set at 95% credibility level on generic Gaussian-shaped signals and two benchmark phenomena beyond the Standard Model: non-thermal quantum black holes and excited quarks. Non-thermal quantum black holes are excluded below masses of 4.6 TeV and excited quarks are excluded below masses of 3.5 TeV. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vague, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. [Berger, N.; Colas, J.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Petit, E.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Zitoun, R.] CNRS, LAPP, IN2P3, Annecy Le Vieux, France. [Berger, N.; Colas, J.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Petit, E.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Zitoun, R.] Univ Savoie, Annecy Le Vieux, France. [Asquith, L.; Auerbach, B.; Blair, R. E.; Chekanov, S.; Feng, E. J.; Fernando, W.; Goshaw, A. T.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Ferrando, B. M. Salvachua; Stanek, R. W.; van Gemmeren, P.; Vaniachine, A.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Kaushik, V.; Lampen, C. L.; Lamp, W.; Leone, R.; Loch, P.; O'grady, F.; Paleari, C. P.; Ruehr, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Cote, D.; Darmora, S.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Hernandez, C. M.; Maeno, M.; Nilsson, P.; Ozturk, N.; Sarkisyan-Grinbaum, E.; Sosebee, M.; Spurlock, B.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Antonaki, A.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Byszewski, M.; Dris, M.; Gazisl, E. N.; Lakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezosl, S.; Mountricha, E.; Ntekas, K.; Panagiotopoulou, E.; Papadopouloul, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Huseynov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Abdallah, J.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Demirkoz, B.; Espinal Curull, X.; Francavilla, P.; Giangiobbe, V.; Larra, G. Gonzalez; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Pacheco Pages, A.; Padilla Aranda, C.; Portell Bueso, X.; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Cortes-Gonzalez, A.; Demirkoz, B.; Espinal Curull, X.; Francavilla, P.; Giangiobbe, V.; Larra, G. Gonzalez; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Pacheco Pages, A.; Padilla Aranda, C.; Portell Bueso, X.; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Agatonovic-Jovin, T.; Bozovic-Jelisavcic, I.; Cirkovic, P.; Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Burgess, T.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Stugu, B.; Tonoyan, A.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Bach, A. M.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Calafiura, R.; Caminada, L. M.; Cerri, A.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Marshall, Z.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Bach, A. M.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Calafiura, R.; Caminada, L. M.; Cerri, A.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Marshall, Z.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Aliev, M.; Kuutmann, E. Bergeaas; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Nikiforov, A.; Rieck, R.; Schulz, H.; Wendland, D.; Nedden, M. Zur] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Borer, C.; Cervelli, A.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Topfe, C.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Borer, C.; Cervelli, A.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Topfe, C.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansi, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mahout, G.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Grafstroem, R.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bindi, M.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, R.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Backhaus, M.; Bechtle, P.; Brock, R.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbe, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Hageboeck, S.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, R.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, R.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [Do Vale, M. A. B.] Fed Univ Sao Joao Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Bege, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, R.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cucitic, C. -M; Dinutzsa, F.; Dita, R.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, R.; Fassnacht, R.; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, E.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, A.; Salek, D.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. 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B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, R.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, R.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, R.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, R.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijtnans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thomson, E.; Tian, R.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pinge, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcy, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Hemyk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, R.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildtt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, R.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildtt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, R.; Friedrich, E.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, R.; Steinbach, R.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teikhenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J. V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, E.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flech, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, D.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, R.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; De Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Gutierrez Ortiz, N. G.; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Kei, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; More, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subat & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, R.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetze, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZIT1 Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, R.; Luehring, R.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, E.; Krumnack, N.; Pre, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] Natl Lab High Energy Phys, KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 305, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J. J.] Univ Lancaster, Dept Phys, Lancaster, England. [Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, R.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jofef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snider, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, R.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, E.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Hande, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevski, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J. J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Born, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howard, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, E.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, E.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M. -A.; Keyes, R. A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Haman, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, R.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, R.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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[Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J. L.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, R.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, A.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, R.; Hessey, N. P.; Hod, N.; Igonkina, O.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. 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[Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Koro, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, R.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, E.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hama, R.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, V. J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, R.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, V. J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, R.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajche, K.; Pedersen, M.; Read, A. 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[Brendlinger, K.; Degenhardt, J. J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarria, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarria, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorima, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, R.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J. J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejba, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Schovancova, J. J.; Sicho, R.; Staroba, R.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, Sj.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, E.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, R.; Luci, C.; Luminari, L.; Marzano, R.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, R.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Donato, C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciacci, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, Fr.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. 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R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybe, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, R.; Stavina, R.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Mellado Garcia, B. R.; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, R.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, R.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, R.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, R.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Guest, D.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, R.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farre, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobailac, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobailac, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshal, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, G.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J. -R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M. M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. C.; Ji, H.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, R.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Beermann, T. A.; Boek, J. J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, R.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, R.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J. J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, E.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, R.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Kings Coll London, Dept Phys, London, England. [Bawa, H. S.; Gao, Y. S.; Rahal, G.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Kono, T.; Wildtt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Pasztor, G.; Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Amorima, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorima, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Sci & Tecnol, Caparica, Portugal. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Do Valle Wemans, A.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Kuleshov, Sergey/D-9940-2013; Lokajicek, Milos/G-7800-2014; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Villa, Mauro/C-9883-2009; Ferrando, James/A-9192-2012; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Jakoubek, Tomas/G-8644-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Boyko, Igor/J-3659-2013; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Solfaroli Camillocci, Elena/J-1596-2012; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Tikhomirov, Vladimir/M-6194-2015; Yang, Haijun/O-1055-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016 OI Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Kuleshov, Sergey/0000-0002-3065-326X; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Villa, Mauro/0000-0002-9181-8048; Ferrando, James/0000-0002-1007-7816; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Boyko, Igor/0000-0002-3355-4662; Fabbri, Laura/0000-0002-4002-8353; Brooks, William/0000-0001-6161-3570; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Pacheco Pages, Andres/0000-0001-8210-1734; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920 FU ANPCyT, Argentina; YerPhl, Armenia; ARC, Australia; BMWF; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; VSC CR; Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT; NSRF, Greece; ISF; MINERVA; GIF; DIP; Benoziyo Center, Israel; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, Netherlands; BRF; RCN, Norway; MNiSW, Poland; GRICES; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC; Wallenberg Foundation, Sweden; SER; SNSF; Cantons of Bern; Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC; Royal Society; Leverhulme Trust, United Kingdom; DOE; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhl, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 52 TC 29 Z9 29 U1 7 U2 120 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 562 EP 578 DI 10.1016/j.physletb.2013.12.029 PG 17 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000086 ER PT J AU Stefanini, AM Montagnoli, G Esbensen, H Corradi, L Courtin, S Fioretto, E Goasduff, A Grebosz, J Haas, F Mazzocco, M Michelagnoli, C Mijatovic, T Montanari, D Pasqualato, G Parascandolo, C Scarlassara, F Strano, E Szilner, S Torresi, D AF Stefanini, A. M. Montagnoli, G. Esbensen, H. Corradi, L. Courtin, S. Fioretto, E. Goasduff, A. Grebosz, J. Haas, F. Mazzocco, M. Michelagnoli, C. Mijatovic, T. Montanari, D. Pasqualato, G. Parascandolo, C. Scarlassara, F. Strano, E. Szilner, S. Torresi, D. TI Fusion of Ca-40+Zr-96 revisited: Transfer couplings and hindrance far below the barrier SO PHYSICS LETTERS B LA English DT Article DE Heavy-ion fusion; Sub-barrier cross sections; Coupled-channels model ID COUPLED-CHANNELS CALCULATIONS; SUBBARRIER FUSION; DEPENDENCE; COLLISIONS AB The sub-barrier fusion excitation function of Ca-40 + Zr-96 has been measured down to cross sections similar or equal to 2.4 mu b, i.e. two orders of magnitude smaller than obtained in a previous experiment, where the sub-barrier fusion of this system was found to be greatly enhanced with respect to Ca-40 + Zr-90, and the need of coupling to transfer channels was suggested relying on coupled-channels calculations. The purpose of this work has been to investigate the behavior of Ca-40 + Zr-96 fusion far below the barrier, thereby disentangling the elusive interplay of effects due to inelastic couplings, transfer couplings and, possibly, the appearance of the fusion hindrance. The smooth trend of the excitation function has been found to continue, and the logarithmic slope increases very slowly. No indication of hindrance shows up, and a comparison with Ca-48 + Zr-96 is illuminating in this respect. A new CC analysis of the complete excitation function has been performed, including explicitly one- and two-nucleon Q > 0 transfer channels. Such transfer couplings bring significant cross section enhancements, even at the level of a few mu b. Locating the hindrance threshold, if any, in Ca-40 + Zr-96 would require challenging measurements of cross sections in the sub-mu b range. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Stefanini, A. M.; Corradi, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. [Montagnoli, G.; Fioretto, E.; Mazzocco, M.; Michelagnoli, C.; Montanari, D.; Pasqualato, G.; Parascandolo, C.; Scarlassara, F.; Strano, E.; Torresi, D.] Univ Padua, Dipartimento Fis & Astron, Padua, Italy. [Montagnoli, G.; Fioretto, E.; Mazzocco, M.; Michelagnoli, C.; Montanari, D.; Pasqualato, G.; Parascandolo, C.; Scarlassara, F.; Strano, E.; Torresi, D.] Ist Nazl Fis Nucl, Sez Padova, I-35020 Padua, Italy. [Esbensen, H.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Courtin, S.; Haas, F.] Univ Strasbourg, CNRS, IN2P3, IPHC, F-67037 Strasbourg, France. [Goasduff, A.] CNRS, IN2P3, CSNSM, F-91405 Orsay, France. [Goasduff, A.] Univ Paris 11, F-91405 Orsay, France. [Grebosz, J.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Mijatovic, T.; Szilner, S.] Rudjer Boskovic Inst, HR-10002 Zagreb, Croatia. RP Stefanini, AM (reprint author), Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. EM alberto.stefanini@lnl.infn.it RI Montanari, Daniele/E-2192-2015; Goasduff, Alain/F-1749-2016; OI Montanari, Daniele/0000-0002-1980-7686; Goasduff, Alain/0000-0003-3453-3297; Esbensen, Henning/0000-0002-2483-7708; Strano, Emanuele/0000-0001-8044-8136 FU European Union Seventh Framework Programme [262010-ENSAR]; Croatian Ministry of Science, Education and Sports [0098-1191005-2890]; US Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX Thanks are due to V.V. Sargsyan for providing us with his calculations. We are very grateful to the XTU Tandem staff, to N. Toniolo for developing the new DAQ and to M. Loriggiola for preparing targets of excellent quality. The research leading to these results has received funding from the European Union Seventh Framework Programme FP7/2007-2013 under Grant Agreement No: 262010-ENSAR. T.M. and S.S. were partially supported by the Croatian Ministry of Science, Education and Sports (Grant No. 0098-1191005-2890). H.E. is supported by the US Department of Energy, Office of Nuclear Physics, Contract No. DE-AC02-06CH11357. NR 45 TC 32 Z9 33 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 639 EP 644 DI 10.1016/j.physletb.2013.12.048 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000097 ER PT J AU Bozek, P Bzdak, A Skokov, V AF Bozek, Piotr Bzdak, Adam Skokov, Vladimir TI The rapidity dependence of the average transverse momentum in p + Pb collisions at the LHC: The Color Glass Condensate versus hydrodynamics SO PHYSICS LETTERS B LA English DT Article ID RANGE ANGULAR-CORRELATIONS; COLOR GLASS CONDENSATE; WOUNDED NUCLEON MODEL; LONG-RANGE; ROOT-S(NN)=5.02 TEV; COLLISIONS; MULTIPLICITY; PROTONS; SIDE; PPB AB We show that in proton-lead (p + Pb) collisions at the LHC, the Color Glass Condensate (CGC) and hydrodynamics lead to qualitatively different behavior of the average transverse momentum, (p perpendicular to), with the particle rapidity. In hydrodynamics, the (p perpendicular to) decreases as one goes from zero rapidity, y = 0, to the proton fragmentation region since the number of particles decreases. In contrast, in the CGC the saturation momentum increases as one goes from y = 0 to the proton fragmentation region, and so the (p perpendicular to) increases. At the LHC, the difference between the two models may be large enough to be tested experimentally. (C) 2014 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Bozek, Piotr] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Bozek, Piotr] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Bzdak, Adam] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Bzdak, A (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM piotr.bozek@ifj.edu.pl; abzdak@bnl.gov; vskokov@quark.phy.bnl.gov RI Bozek, Piotr/A-5031-2012; OI Bozek, Piotr/0000-0001-6050-4380; Skokov, Vladimir/0000-0001-7619-1796 FU National Science Centre, Poland [2012/05/B/ST2/02528]; RIKEN-BNL Research Center FX We thank A. Dumitru and L. McLerran for helpful discussions. P.B. is partly supported by the National Science Centre, Poland, grant DEC-2012/05/B/ST2/02528, and PL-Grid infrastructure. A.B. is supported through the RIKEN-BNL Research Center. NR 36 TC 16 Z9 16 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JAN 20 PY 2014 VL 728 BP 662 EP 665 DI 10.1016/j.physletb.2013.12.034 PG 4 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 301TW UT WOS:000330556000101 ER PT J AU Bohlin, A Kliewer, CJ AF Bohlin, Alexis Kliewer, Christopher J. TI Two-beam ultrabroadband coherent anti-Stokes Raman spectroscopy for high resolution gas-phase multiplex imaging SO APPLIED PHYSICS LETTERS LA English DT Article ID SCATTERING MEASUREMENTS; ROTATIONAL CARS; NITROGEN; TEMPERATURE; METHANE; FLAMES; OXYGEN; CO2 AB We propose and develop a method for wideband coherent anti-Stokes Raman spectroscopy (CARS) in the gas phase and demonstrate the single-shot measurement of N-2, H-2, CO2, O-2, and CH4. Pure-rotational and vibrational O-, Q-, and S- branch spectra are collected simultaneously, with high spectral and spatial resolution, and within a single-laser-shot. The relative intensity of the rotational and vibrational signals can be tuned arbitrarily using polarization techniques. The ultrashort 7 fs pump and Stokes pulses are automatically overlapped temporally and spatially using a two-beam CARS technique, and the crossed probe beam allows for excellent spatial sectioning of the probed location. (C) 2014 AIP Publishing LLC. C1 [Bohlin, Alexis; Kliewer, Christopher J.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. RP Kliewer, CJ (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. EM cjkliew@sandia.gov RI Kliewer, Christopher/E-4070-2010; Bohlin, Alexis/L-8973-2015 OI Kliewer, Christopher/0000-0002-2661-1753; Bohlin, Alexis/0000-0003-4383-8332 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Brian D. Patterson of Sandia for technical assistance. Funding provided by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 28 TC 11 Z9 11 U1 2 U2 32 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 20 PY 2014 VL 104 IS 3 AR 031107 DI 10.1063/1.4862980 PG 5 WC Physics, Applied SC Physics GA AA1EQ UT WOS:000330839700007 ER PT J AU Demos, SG Negres, RA Rubenchik, AM AF Demos, Stavros G. Negres, Raluca A. Rubenchik, Alexander M. TI Dynamics of the plume containing nanometric-sized particles ejected into the atmospheric air following laser-induced breakdown on the exit surface of a CaF2 optical window SO APPLIED PHYSICS LETTERS LA English DT Article ID FUSED-SILICA; AMBIENT AIR; ABLATION; POLYMERS; DEBRIS AB Laser induced breakdown on the output surface of calcium fluoride produces distinctive visualization of the gaseous material ejection via time-resolved shadowgraphy microscopy. This characteristic behavior allowed a detailed investigation of the directional expansion of the plume at ambient atmospheric conditions and its spatial separation and influence on the forming shockwave. The results also suggest that the material ejection is prolonged, extending more than 300 ns after the termination of the laser pulse. The dynamics of the backward motion of the gaseous material following its initial expansion is also resolved. (C) 2014 AIP Publishing LLC. C1 [Demos, Stavros G.; Negres, Raluca A.; Rubenchik, Alexander M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Demos, SG (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM demos1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Rajesh N. Raman and Michael D. Feit for stimulating discussions that helped improve the manuscript. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 25 TC 3 Z9 3 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 20 PY 2014 VL 104 IS 3 AR 031603 DI 10.1063/1.4862815 PG 4 WC Physics, Applied SC Physics GA AA1EQ UT WOS:000330839700021 ER PT J AU Zhou, J Riccardi, D Beste, A Smith, JC Parks, JM AF Zhou, Jing Riccardi, Demian Beste, Ariana Smith, Jeremy C. Parks, Jerry M. TI Mercury Methylation by HgcA: Theory Supports Carbanion Transfer to Hg(II) SO INORGANIC CHEMISTRY LA English DT Article ID CO-C BOND; DESULFOVIBRIO-DESULFURICANS ND132; SULFATE-REDUCING BACTERIA; ELECTRONIC-PROPERTIES; SULFUR PROTEIN; DEPENDENT ENZYMES; ACETYL-COENZYME; B-12 COFACTORS; AXIAL LIGAND; COBALAMIN AB Many proteins use corrinoid cofactors to facilitate methyl transfer reactions. Recently, a corrinoid protein, HgcA, has been shown to be required for the production of the neurotoxin methylmercury by anaerobic bacteria. A strictly conserved Cys residue in HgcA was predicted to be a lower-axial ligand to Co(III), which has never been observed in a corrinoid protein. Here, we use density functional theory to study homolytic and heterolytic Co-C bond dissociation and methyl transfer to Hg(II) substrates with model methylcobalamin complexes containing a lower-axial Cys or His ligand to cobalt, the latter of which is commonly found in other corrinoid proteins. We find that Cys thiolate coordination to Co facilitates both methyl radical and methyl carbanion transfer to Hg(II) substrates, but carbanion transfer is more favorable overall in the condensed phase. Thus, our findings are consistent with HgcA representing a new class of corrinoid protein capable of transferring methyl groups to electrophilic substrates. C1 [Zhou, Jing] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA. [Zhou, Jing; Riccardi, Demian; Smith, Jeremy C.; Parks, Jerry M.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. [Beste, Ariana] Univ Tennessee, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Beste, Ariana] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. RP Parks, JM (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. EM parksjm@ornl.gov RI Parks, Jerry/B-7488-2009; smith, jeremy/B-7287-2012; OI Parks, Jerry/0000-0002-3103-9333; smith, jeremy/0000-0002-2978-3227; Beste, Ariana/0000-0001-9132-792X FU U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program [DE-SC0004895]; U.S. DOE [DE-AC05-00OR22725]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE; National Energy Research Scientific Computing Center [m906]; Office of Science of the U.S. DOE [DE-AC02-05CH11231] FX This work was supported by Grant DE-SC0004895 from the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research, Subsurface Biogeochemical Research Program. ORNL is managed by UT-Battelle, LLC. for the U.S. DOE under contract DE-AC05-00OR22725. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE. This research used resources of the National Energy Research Scientific Computing Center (Grant m906), which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC02-05CH11231. NR 66 TC 7 Z9 7 U1 5 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JAN 20 PY 2014 VL 53 IS 2 BP 772 EP 777 DI 10.1021/ic401992y PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 296RV UT WOS:000330204000021 PM 24377658 ER PT J AU Thompson, CM Greedan, JE Garlea, VO Flacau, R Tan, M Nguyen, PHT Wrobel, F Derakhshan, S AF Thompson, Corey M. Greedan, John E. Garlea, V. Ovidiu Flacau, Roxana Tan, Malinda Nguyen, Phuong-Hieu T. Wrobel, Friederike Derakhshan, Shahab TI Partial Spin Ordering and Complex Magnetic Structure in BaYFeO4: A Neutron Diffraction and High Temperature Susceptibility Study SO INORGANIC CHEMISTRY LA English DT Article ID POWDER-DIFFRACTION; MIXED-VALENCE; YBA2FE3O8; NUCLEAR; PHASES AB The novel iron-based compound, BaYFeO4, crystallizes in the Pnma space group with two distinct Fe3+ sites, that are alternately corner-shared [FeO5](7-) square pyramids and [FeO6](9-) octahedra, forming into [Fe4O18](24-) rings, which propagate as columns along the b-axis. A recent report shows two discernible antiferromagnetic (AFM) transitions at 36 and 48 K in the susceptibility, yet heat capacity measurements reveal no magnetic phase transitions at these temperatures. An upturn in the magnetic susceptibility measurements up to 400 K suggests the presence of short-range magnetic behavior at higher temperatures. In this Article, variable-temperature neutron powder diffraction and high-temperature magnetic susceptibility measurements were performed to clarify the magnetic behavior. Neutron powder diffraction confirmed that the two magnetic transitions observed at 36 and 48 K are due to long-range magnetic order. Below 48 K, the magnetic structure was determined as a spin-density wave (SDW) with a propagation vector, k = (0, 0, 1/3), and the moments along the b-axis, whereas the structure becomes an incommensurate cycloid [k = (0, 0, 0.35)] below 36 K with the moments within the bc-plane. However, for both cases the ordered moments on Fe3+ are only of the order similar to 3.0 mu(B), smaller than the expected values near 4.5 mu(B), indicating that significant components of the Fe moments remain paramagnetic to the lowest temperature studied, 6 K. Moreover, new high-temperature magnetic susceptibility measurements revealed a peak maximum at similar to 550 K indicative of short-range spin correlations. It is postulated that most of the magnetic entropy is thus removed at high temperatures which could explain the absence of heat capacity anomalies at the long-range ordering temperatures. Published spin dimer calculations, which appear to suggest a k = (0, 0, 0) magnetic structure, and allow for neither low dimensionality nor geometric frustration, are inadequate to explain the observed complex magnetic structure. C1 [Thompson, Corey M.; Greedan, John E.] McMaster Univ, Dept Chem, Hamilton, ON L8S 4M1, Canada. [Thompson, Corey M.; Greedan, John E.] McMaster Univ, Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. [Garlea, V. Ovidiu] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Flacau, Roxana] Canadian Neutron Beam Ctr, Natl Res Council, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. [Tan, Malinda; Nguyen, Phuong-Hieu T.; Wrobel, Friederike; Derakhshan, Shahab] Calif State Univ Long Beach, Dept Chem & Biochem, Long Beach, CA 90840 USA. RP Thompson, CM (reprint author), McMaster Univ, Dept Chem, Hamilton, ON L8S 4M1, Canada. EM thompco@mcmaster.ca RI Garlea, Vasile/A-4994-2016 OI Garlea, Vasile/0000-0002-5322-7271 FU Natural Sciences and Engineering Research Council (NSERC) of Canada; U.S. DOE, Office of Basic Energy Sciences, Scientific User Facilities Division; U.S. Army Research Office [W911NF1210076]; Research Corporation for Science Advancement (Cottrell College Science Award) [19761] FX J.E.G. acknowledges the support of the Natural Sciences and Engineering Research Council (NSERC) of Canada in the form of a Discovery Grant. V.O.G acknowledges the support by the U.S. DOE, Office of Basic Energy Sciences, Scientific User Facilities Division. S.D. is grateful for financial support from the U.S. Army Research Office under Contract/Grant W911NF1210076 and the Research Corporation for Science Advancement (Cottrell College Science Award #19761). We thank Dr. Paul Dube for assistance in collecting the high temperature magnetic susceptibility data. NR 15 TC 2 Z9 2 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JAN 20 PY 2014 VL 53 IS 2 BP 1122 EP 1127 DI 10.1021/ic4026798 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 296RV UT WOS:000330204000060 PM 24405325 ER PT J AU Langley, SK Helliwell, M Teat, SJ Winpenny, REP AF Langley, Stuart K. Helliwell, Madeleine Teat, Simon J. Winpenny, Richard E. P. TI Synthesis and Characterization of Nickel(II) Phosphonate Complexes Utilizing Pyridonates and Carboxylates as Co-ligands SO INORGANIC CHEMISTRY LA English DT Article ID CAGE COMPLEXES; CLUSTERS; TETRANUCLEAR; COBALT(II); REFRIGERANTS; RELAXATION; CHEMISTRY; NUCLEAR; FAMILY AB The synthesis and structures of five new nickel complexes containing phosphonate ligands are reported. The compounds utilize pivalic acid (HPiv) and 6-chloro-2-pyridonate (Hchp) as co-ligands with the resulting complexes being of formulas [Ni-10(chp)(4)(Hchp)(4.5)((O3PBu)-Bu-t)(3)(Piv)(5)(HPiv)(2)(OH)(6)(H2O)(4.5)](HNEt3)center dot 0.5MeCN center dot 2.5H(2)O 1, [Ni-12(chp)(12)(Hchp)(2)(PhPO3)(2)(Piv)(5)(HPiv)(2)(OH)(2)(H2O)(6)](F)center dot 4.5MeCN center dot 2H(2)O 2, [Ni-10(chp)(6)(O3PCH2Ph)(2)(Piv)(8)(F)(2)(MeCN)(4)] 3, [Ni-10(chp)(6)(O3PMe)(2)(Piv)(8)(F)(2) (MeCN)(4)]center dot 5MeCN center dot 2H(2)O 4, and [Ni-10(chp)(6)(O(3)PCH(2)Nap)(2)(Piv)(8)(F)(2)(MeCN)(2)(H2O)(2)] 5. The metallic core of compounds 1 and 2 display tetra- and hexa-capped trigonal prismatic arrangements, while the metallic and phosphorus core of 3, 4, and 5 display three face-sharing octahedra. Variable temperature direct current (dc) magnetic susceptibility measurements reveal dominant antiferromagnetic exchange interactions within each cluster, with diamagnetic spin ground states found. C1 [Langley, Stuart K.; Helliwell, Madeleine; Winpenny, Richard E. P.] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England. [Teat, Simon J.] Univ Manchester, Photon Sci Inst, Manchester M13 9PL, Lancs, England. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Winpenny, REP (reprint author), Univ Manchester, Sch Chem, Oxford Rd, Manchester M13 9PL, Lancs, England. EM richard.winpenny@man.ac.uk RI Langley, Stuart/G-4973-2011 OI Langley, Stuart/0000-0002-2241-1551 FU EPSRC(U.K.); EC-TMR "QueMolNa"; Royal Society; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the EPSRC(U.K.) for funding for a studentship (S.L.). We are also grateful to the EC-TMR "QueMolNa" for support. R.E.P.W. is grateful to The Royal Society for a Wolfson Merit Award. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 57 TC 17 Z9 17 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JAN 20 PY 2014 VL 53 IS 2 BP 1128 EP 1134 DI 10.1021/ic4026816 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 296RV UT WOS:000330204000061 PM 24392684 ER PT J AU Velazquez-Salinas, L Pauszek, SJ Zarate, S Basurto-Alcantara, FJ Verdugo-Rodriguez, A Perez, AM Rodriguez, LL AF Velazquez-Salinas, Lauro Pauszek, Steven J. Zarate, Selene Basurto-Alcantara, Francisco J. Verdugo-Rodriguez, Antonio Perez, Andres M. Rodriguez, Luis L. TI Phylogeographic characteristics of vesicular stomatitis New Jersey viruses circulating in Mexico from 2005 to 2011 and their relationship to epidemics in the United States SO VIROLOGY LA English DT Article DE Vesicular stomatitis virus; Epidemiology; Spatial clustering; Phylogeny; Phylodynamics; Mexico; United States; Outbreak ID EQUINE ENCEPHALITIS-VIRUS; E2 ENVELOPE GLYCOPROTEIN; EVOLUTION; REEMERGENCE; EMERGENCE; OUTBREAKS; SEQUENCE; VECTORS; STRAINS AB We analyzed the phylogenetic and time-space relationships (phylodynamics) of 181 isolates of vesicular stomatitis New Jersey virus (VSNJV) causing disease in Mexico and the United States (US) from 2005 through 2012. We detail the emergence of a genetic lineage in southern Mexico causing outbreaks in central Mexico spreading into northern Mexico and eventually into the US. That emerging lineage showed higher nucleotide sequence identity (99.5%) than that observed for multiple lineages circulating concurrently in southern Mexico (96.8%). Additionally, we identified 58 isolates from Mexico that, unlike previous isolates from Mexico, grouped with northern Central America clade II viruses. This study provides the first direct evidence for the emergence and northward migration of a specific VSNJV genetic lineage from endemic areas in Mexico causing VS outbreaks in the US. In addition we document the emergence of a Central American VSNJV genetic lineage moving northward and causing outbreaks in central Mexico. Published by Elsevier Inc. C1 [Velazquez-Salinas, Lauro; Pauszek, Steven J.; Rodriguez, Luis L.] USDA ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, Greenport, NY 11944 USA. [Zarate, Selene] Autonomous Univ Mexico, Dept Genom Sci, Mexico City, DF, Mexico. [Basurto-Alcantara, Francisco J.; Verdugo-Rodriguez, Antonio] Univ Nacl Autonoma Mexico, Coll Vet Med & Anim Sci, Mexico City, DF, Mexico. [Perez, Andres M.] Univ Calif Davis, Sch Vet Med, Davis, CA 95616 USA. [Velazquez-Salinas, Lauro] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. RP Rodriguez, LL (reprint author), USDA ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, POB 848, Greenport, NY 11944 USA. EM luis.rodriguez@ars.usda.gov NR 32 TC 1 Z9 2 U1 1 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0042-6822 J9 VIROLOGY JI Virology PD JAN 20 PY 2014 VL 449 BP 17 EP 24 DI 10.1016/j.virol.2013.10.025 PG 8 WC Virology SC Virology GA 295CL UT WOS:000330094100002 PM 24418533 ER PT J AU Obermeyer, AC Jarman, JB Netirojjanakul, C El Muslemany, K Francis, MB AF Obermeyer, Allie C. Jarman, John B. Netirojjanakul, Chawita El Muslemany, Kareem Francis, Matthew B. TI Mild Bioconjugation Through the Oxidative Coupling of ortho-Aminophenols and Anilines with Ferricyanide SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE amines; bioconjugation; iron; oxidation; proteins ID UNNATURAL AMINO-ACIDS; TOBACCO-MOSAIC-VIRUS; CHEMICAL-MODIFICATION; PROTEIN MODIFICATION; ESCHERICHIA-COLI; GENETIC-CODE; CHEMISTRY; LIGATION; SYSTEMS; BACTERIOPHAGE-MS2 AB Using a small-molecule-based screen, ferricyanide was identified as a mild and efficient oxidant for the coupling of anilines and o-aminophenols on protein substrates. This reaction is compatible with thiols and 1,2-diols, allowing its use in the creation of complex bioconjugates for use in biotechnology and materials applications. C1 [Obermeyer, Allie C.; Jarman, John B.; Netirojjanakul, Chawita; El Muslemany, Kareem; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Francis, Matthew B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mbfrancis@berkeley.edu FU NSF [CHE 1059083]; UC Berkeley Chemical Biology Program (NRSA) [1 T32 GMO66698]; SURF Rose-Hills summer research fellowship; HHMI International Student Fellowship; NSF graduate research fellowship FX This work was supported by a grant from the NSF (CHE 1059083). A.C.O was supported by an NSF graduate research fellowship and the UC Berkeley Chemical Biology Program (NRSA Training Grant 1 T32 GMO66698). J.B.J. was supported by a SURF Rose-Hills summer research fellowship, and C.N. was supported by an HHMI International Student Fellowship. NR 50 TC 13 Z9 13 U1 1 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 20 PY 2014 VL 53 IS 4 BP 1057 EP 1061 DI 10.1002/anie.201307386 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 292CL UT WOS:000329879500026 PM 24311449 ER PT J AU Inouye, H Zhang, Y Yang, L Venugopalan, N Fischetti, RF Gleber, SC Vogt, S Fowle, W Makowski, B Tucker, M Ciesielski, P Donohoe, B Matthews, J Himmel, ME Makowski, L AF Inouye, Hideyo Zhang, Yan Yang, Lin Venugopalan, Nagarajan Fischetti, Robert F. Gleber, S. Charlotte Vogt, Stefan Fowle, W. Makowski, Bryan Tucker, Melvin Ciesielski, Peter Donohoe, Bryon Matthews, James Himmel, Michael E. Makowski, Lee TI Multiscale deconstruction of molecular architecture in corn stover SO SCIENTIFIC REPORTS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; X-RAY-SCATTERING; ACID-HYDROLYSIS; CELLULOSE MICROFIBRILS; PRETREATED BIOMASS; RADIAL GROWTH; CELL-WALLS; NANOSTRUCTURE; DIGESTIBILITY; COLLENCHYMA AB Lignocellulosic composite in corn stover is a candidate biofuel feedstock of substantial abundance and sustainability. Its utilization is hampered by resistance of constituent cellulose fibrils to deconstruction. Here we use multi-scale studies of pretreated corn stover to elucidate the molecular mechanism of deconstruction and investigate the basis of recalcitrance. Dilute acid pretreatment has modest impact on fibrillar bundles at 0.1 micron length scales while leading to significant disorientation of individual fibrils. It disintegrates many fibrils into monomeric cellulose chains or small side-by-side aggregates. Residual crystalline fibrils lose amorphous surface material, change twist and where still cross-linked, coil around one another. Yields from enzymatic digestion are largely due to hydrolysis of individual cellulose chains and fragments generated during pretreatments. Fibrils that remain intact after pretreatment display substantial resistance to enzymatic digestion. Optimization of yield will require strategies that maximize generation of fragments and minimize preservation of intact cellulosic fibrils. C1 [Inouye, Hideyo; Zhang, Yan; Makowski, Lee] Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. [Yang, Lin] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Venugopalan, Nagarajan; Fischetti, Robert F.] Argonne Natl Lab, Adv Photon Source, XSD, GM CA CAT, Argonne, IL 60439 USA. [Gleber, S. Charlotte; Vogt, Stefan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Fowle, W.] Northeastern Univ, Dept Biol, Boston, MA 02115 USA. [Makowski, Bryan] Rensselaer Polytech Inst, Dept Phys, Troy, NY 12180 USA. [Tucker, Melvin; Ciesielski, Peter; Donohoe, Bryon; Matthews, James; Himmel, Michael E.] Natl Renewable Energy Lab, Chem & Biosci Ctr, Golden, CO 80401 USA. [Makowski, Lee] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. RP Makowski, L (reprint author), Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. EM makowski@ece.neu.edu RI Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013 OI Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513 FU Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio); Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0000997, DE-AC02-98CH10886]; U.S. DOE [DE-AC02-06CH11357]; National Institutes of Health, National Cancer Institute [Y1-CO-1020]; National Institute of General Medical Science [Y1-GM-1104] FX This work was supported as part of the Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award # DE-SC0000997. Use of the National Synchrotron Light Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Use of GM/CA at the APS was supported by the National Institutes of Health, National Cancer Institute (Y1-CO-1020) and National Institute of General Medical Science (Y1-GM-1104). NR 34 TC 10 Z9 10 U1 2 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 20 PY 2014 VL 4 AR 3756 DI 10.1038/srep03756 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291SP UT WOS:000329850100002 PM 24441444 ER PT J AU Ammons, SM Wong, KC Zabludoff, AI Keeton, CR AF Ammons, S. Mark Wong, Kenneth C. Zabludoff, Ann I. Keeton, Charles R. TI MAPPING COMPOUND COSMIC TELESCOPES CONTAINING MULTIPLE PROJECTED CLUSTER-SCALE HALOS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: clusters: general; galaxies: high-redshift; galaxies: kinematics and dynamics; gravitational lensing: strong; techniques: radial velocities ID DIGITAL SKY SURVEY; MASSIVE GALAXY CLUSTERS; SIMILAR-TO 7; HIGH-REDSHIFT GALAXIES; LYMAN BREAK GALAXIES; ULTRA-DEEP-FIELD; LUMINOSITY FUNCTIONS; LENSED GALAXIES; RICH CLUSTERS; VELOCITY DISPERSIONS AB Lines of sight with multiple projected cluster-scale gravitational lenses have high total masses and complex lens plane interactions that can boost the area of magnification, or etendue, making detection of faint background sources more likely than elsewhere. To identify these new "compound" cosmic telescopes, we have found directions in the sky with the highest integrated mass densities, as traced by the projected concentrations of luminous red galaxies (LRGs). We use new galaxy spectroscopy to derive preliminary magnification maps for two such lines of sight with total mass exceeding similar to 3 x 10(15) M-circle dot. From 1151 MMT Hectospec spectra of galaxies down to i(AB) = 21.2, we identify two to three group-and cluster-scale halos in each beam. These are well traced by LRGs. The majority of the mass in beam J085007.6+360428 (0850) is contributed by Zwicky 1953, a massive cluster at z = 0.3774, whereas beam J130657.5+463219 (1306) is composed of three halos with virial masses of 6 x 10(14)-2 x 10(15) M-circle dot, one of which is A1682. The magnification maps derived from our mass models based on spectroscopy and Sloan Digital Sky Survey photometry alone display substantial etendue: the 68% confidence bands on the lens plane area with magnification exceeding 10 for a source plane of z(s) = 10 are [1.2, 3.8] arcmin(2) for 0850 and [2.3, 6.7] arcmin(2) for 1306. In deep Subaru Suprime-Cam imaging of beam 0850, we serendipitously discover a candidate multiply imaged V-dropout source at z(phot) = 5.03. The location of the candidate multiply imaged arcs is consistent with the critical curves for a source plane of z = 5.03 predicted by our mass model. Incorporating the position of the candidate multiply imaged galaxy as a constraint on the critical curve location in 0850 narrows the 68% confidence band on the lens plane area with mu > 10 and z(s) = 10 to [1.8, 4.2] arcmin(2), an etendue range comparable to that of MACS 0717+3745 and El Gordo, two of the most powerful single cluster lenses known. The significant lensing power of our beams makes them powerful probes of reionization and galaxy formation in the early universe. C1 [Ammons, S. Mark] Lawrence Livermore Natl Lab, Phys Div L 210, Livermore, CA 94550 USA. [Wong, Kenneth C.] Acad Sinica ASIAA, Inst Astron & Astrophys, EACOA, Taipei 10641, Taiwan. [Zabludoff, Ann I.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [Keeton, Charles R.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. RP Ammons, SM (reprint author), Lawrence Livermore Natl Lab, Phys Div L 210, 7000 East Ave, Livermore, CA 94550 USA. EM ammons1@llnl.gov; kwong@as.arizona.edu; aiz@email.arizona.edu; keeton@physics.rutgers.edu FU NASA through a Hubble Fellowship grant from the Space Telescope Science Institute [HST-HF-51250.01-A]; NASA [NAS5-26555, NNX10AD47G, NNX10AE88G]; NSF [1211874, 121385]; Smithsonian Astrophysical Observatory; U.S. Department of Energy [DE-AC52-07NA27344]; EACOA Fellowship; East Asia Core Observatories Association; Academia Sinica Institute of Astronomy and Astrophysics; National Observatory of Japan; National Astronomical Observatory of China; Korea Astronomy and Space Science Institute; [LLNL-JRNL-609412] FX We thank Chang You and Decker French for assistance in gathering MMT Hectospec data and to Fuyan Bian for assistance in obtaining and reducing LBT/LUCI imaging. We thank Adi Zitrin for providing sigmamu values for other clusters. We also thank Dan Coe, Adi Zitrin, Dan Marrone, Brant Robertson, Sandy Faber, Pascal Oesch, Greg Walth, Michael Schneider, and Kristian Finlator for productive conversations. Support for Program number HST-HF-51250.01-A was provided by NASA through a Hubble Fellowship grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated under NASA contract NAS5-26555. A.I.Z., C. R. K., and K. C. W. acknowledge support from NASA through programs NNX10AD47G and NNX10AE88G and NSF support through AAG programs 1211874 and 121385. This work is based in part on data collected at Subaru Telescope and obtained from the SMOKA, which is operated by the Astronomy Data Center, National Astronomical Observatory of Japan. Observations reported here were obtained at the MMT Observatory, a joint facility of the University of Arizona, and the Smithsonian Institution. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. This paper uses data products produced by the OIR Telescope Data Center, supported by the Smithsonian Astrophysical Observatory. This work is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 with document release number LLNL-JRNL-609412. K. C. W. is supported by an EACOA Fellowship awarded by the East Asia Core Observatories Association, which consists of the Academia Sinica Institute of Astronomy and Astrophysics, the National Observatory of Japan, the National Astronomical Observatory of China, and the Korea Astronomy and Space Science Institute. NR 106 TC 5 Z9 5 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2014 VL 781 IS 1 AR 2 DI 10.1088/0004-637X/781/1/2 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 286AE UT WOS:000329436100002 ER PT J AU Guan, XY Li, H Li, ST AF Guan, Xiaoyue Li, Hui Li, Shengtai TI RELATIVISTIC MHD SIMULATIONS OF POYNTING FLUX-DRIVEN JETS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: jets; instabilities; magnetic fields; magnetohydrodynamics (MHD); methods: numerical ID MAGNETIC TOWER JETS; BLACK-HOLE; MAGNETOHYDRODYNAMIC SIMULATIONS; NUMERICAL SIMULATIONS; STABILITY PROPERTIES; ASTROPHYSICAL JETS; ACCRETION FLOWS; INSTABILITY; ENERGY; FIELD AB Relativistic, magnetized jets are observed to propagate to very large distances in many active galactic nuclei (AGNs). We use three-dimensional relativistic MHD simulations to study the propagation of Poynting flux-driven jets in AGNs. These jets are already assumed to be being launched from the vicinity (similar to 10(3) gravitational radii) of supermassive black holes. Jet injections are characterized by a model described in Li et al., and we follow the propagation of these jets to similar to parsec scales. We find that these current-carrying jets are always collimated and mildly relativistic. When alpha, the ratio of toroidal-to-poloidal magnetic flux injection, is large the jet is subject to nonaxisymmetric current-driven instabilities (CDI) which lead to substantial dissipation and reduced jet speed. However, even with the presence of instabilities, the jet is not disrupted and will continue to propagate to large distances. We suggest that the relatively weak impact by the instability is due to the nature of the instability being convective and the fact that the jet magnetic fields are rapidly evolving on Alfvenic time scales. We present the detailed jet properties and show that far from the jet launching region, a substantial amount of magnetic energy has been transformed into kinetic energy and thermal energy, producing a jet magnetization number sigma < 1. In addition, we have also studied the effects of a gas pressure supported "disk" surrounding the injection region, and qualitatively similar global jet behaviors were observed. We stress that jet collimation, CDIs, and the subsequent energy transitions are intrinsic features of current-carrying jets. C1 [Guan, Xiaoyue; Li, Hui; Li, Shengtai] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Guan, XY (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM guan@lanl.gov OI Li, Shengtai/0000-0002-4142-3080 FU LDRD and Institutional Computing Programs at LANL; DOE/Office of Fusion Energy Science through CMSO FX The authors are grateful to Stirling Colgate, Brenda Dingus, Ken Fowler, John Hawley, Philipp Kronberg, and Masanori Nakamura for discussions. We also thank the anonymous referee for insightful suggestions. This work is supported by the LDRD and Institutional Computing Programs at LANL and by DOE/Office of Fusion Energy Science through CMSO. NR 43 TC 9 Z9 9 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2014 VL 781 IS 1 AR 48 DI 10.1088/0004-637X/781/1/48 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 286AE UT WOS:000329436100048 ER PT J AU Ofek, EO Zoglauer, A Boggs, SE Barriere, NM Reynolds, SP Fryer, CL Harrison, FA Cenko, SB Kulkarni, SR Gal-Yam, A Arcavi, I Bellm, E Bloom, JS Christensen, F Craig, WW Even, W Filippenko, AV Grefenstette, B Hailey, CJ Laher, R Madsen, K Nakar, E Nugent, PE Stern, D Sullivan, M Surace, J Zhang, WW AF Ofek, Eran O. Zoglauer, Andreas Boggs, Steven E. Barriere, Nicolas M. Reynolds, Stephen P. Fryer, Chris L. Harrison, Fiona A. Cenko, S. Bradley Kulkarni, Shrinivas R. Gal-Yam, Avishay Arcavi, Iair Bellm, Eric Bloom, Joshua S. Christensen, Finn Craig, William W. Even, Wesley Filippenko, Alexei V. Grefenstette, Brian Hailey, Charles J. Laher, Russ Madsen, Kristin Nakar, Ehud Nugent, Peter E. Stern, Daniel Sullivan, Mark Surace, Jason Zhang, William W. TI SN 2010jl: OPTICAL TO HARD X-RAY OBSERVATIONS REVEAL AN EXPLOSION EMBEDDED IN A TEN SOLAR MASS COCOON SO ASTROPHYSICAL JOURNAL LA English DT Article DE stars: mass-loss; supernovae: general; supernovae: individual (SN 2010jl) ID SUPERNOVA LIGHT CURVES; SWIFT ULTRAVIOLET/OPTICAL TELESCOPE; CORE-COLLAPSE SUPERNOVAE; IIN SUPERNOVA; SHOCK BREAKOUT; LUMINOUS SUPERNOVAE; PHOTOMETRIC CALIBRATION; COLLISIONLESS SHOCKS; DUST FORMATION; STAR AB Some supernovae (SNe) may be powered by the interaction of the SN ejecta with a large amount of circumstellar matter (CSM). However, quantitative estimates of the CSM mass around such SNe are missing when the CSM material is optically thick. Specifically, current estimators are sensitive to uncertainties regarding the CSM density profile and the ejecta velocity. Here we outline a method to measure the mass of the optically thick CSM around such SNe. We present new visible-light and X-ray observations of SN 2010jl (PTF 10aaxf), including the first detection of an SN in the hard X-ray band using NuSTAR. The total radiated luminosity of SN 2010jl is extreme-at least 9 x 10(50) erg. By modeling the visible-light data, we robustly show that the mass of the circumstellar material within similar to 10(16) cm of the progenitor of SN 2010jl was in excess of 10 M-circle dot. This mass was likely ejected tens of years prior to the SN explosion. Our modeling suggests that the shock velocity during shock breakout was similar to 6000 km s(-1), decelerating to similar to 2600 km s(-1) about 2 yr after maximum light. Furthermore, our late-time NuSTAR and XMM spectra of the SN presumably provide the first direct measurement of SN shock velocity 2 yr after the SN maximum light-measured to be in the range of 2000-4500 km s(-1) if the ions and electrons are in equilibrium, and greater than or similar to 2000 km s(-1) if they are not in equilibrium. This measurement is in agreement with the shock velocity predicted by our modeling of the visible-light data. Our observations also show that the average radial density distribution of the CSM roughly follows an r(-2) law. A possible explanation for the greater than or similar to 10 M-circle dot of CSM and the wind-like profile is that they are the result of multiple pulsational pair instability events prior to the SN explosion, separated from each other by years. C1 [Ofek, Eran O.; Gal-Yam, Avishay; Arcavi, Iair] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Zoglauer, Andreas; Boggs, Steven E.; Barriere, Nicolas M.] Univ Calif Berkeley, Dept Phys, Space Sci Lab, Berkeley, CA 94720 USA. [Reynolds, Stephen P.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Fryer, Chris L.; Even, Wesley] Los Alamos Natl Lab, CCS Div, Los Alamos, NM 87545 USA. [Harrison, Fiona A.; Kulkarni, Shrinivas R.; Bellm, Eric; Grefenstette, Brian; Madsen, Kristin] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Cenko, S. Bradley; Bloom, Joshua S.; Filippenko, Alexei V.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Cenko, S. Bradley; Zhang, William W.] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Christensen, Finn] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, William W.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Laher, Russ; Surace, Jason] CALTECH, Spitzer Sci Ctr, Pasadena, CA 91125 USA. [Nakar, Ehud] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. RP Ofek, EO (reprint author), Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bellm, Eric/0000-0001-8018-5348; Madsen, Kristin/0000-0003-1252-4891; Sullivan, Mark/0000-0001-9053-4820; Even, Wesley/0000-0002-5412-3618 FU NASA [NNG08FD60C]; NASA; W. M. Keck Foundation; Israeli Ministry of Science; Israel Science Foundation; Minerva; I-CORE Program of the Planning and Budgeting Committee; Israel Science Foundation [1829/12]; Christopher R. Redlich Fund; Richard and Rhoda Goldman Fund; TABASGO Foundation; NSF [AST-1211916] FX We thank an anonymous referee for a constructive report. E.O.O. thanks Roni Waldman, Nir Sapir, and Orly Gnat for discussions. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This paper is based on observations obtained with the Samuel Oschin Telescope as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, Las Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford, and the Weizmann Institute of Science. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the Observatory was made possible by the generous financial support of the W. M. Keck Foundation. We are grateful for excellent staff assistance at Palomar, Lick, and Keck Observatories. E.O.O. is incumbent of the Arye Dissentshik career development chair and is grateful to support by a grant from the Israeli Ministry of Science, Israel Science Foundation, Minerva, and the I-CORE Program of the Planning and Budgeting Committee and The Israel Science Foundation (grant No 1829/12). A.V.F.'s SN group at UC Berkeley has received generous financial assistance from Gary and Cynthia Bengier, the Christopher R. Redlich Fund, the Richard and Rhoda Goldman Fund, the TABASGO Foundation, and NSF grant AST-1211916. NR 95 TC 37 Z9 37 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2014 VL 781 IS 1 AR 42 DI 10.1088/0004-637X/781/1/42 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 286AE UT WOS:000329436100042 ER PT J AU Wu, Z Chen, Y Li, G Zhao, LL Ebert, RW Desai, MI Mason, GM Lavraud, B Zhao, L Liu, YCM Guo, F Tang, CL Landi, E Sauvaud, J AF Wu, Z. Chen, Y. Li, G. Zhao, L. L. Ebert, R. W. Desai, M. I. Mason, G. M. Lavraud, B. Zhao, L. Liu, Y. C. -M. Guo, F. Tang, C. L. Landi, E. Sauvaud, J. TI OBSERVATIONS OF ENERGETIC PARTICLES BETWEEN A PAIR OF COROTATING INTERACTION REGIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; magnetohydrodynamics (MHD); shock waves; solar wind; Sun: rotation ID ADVANCED COMPOSITION EXPLORER; SOLAR-WIND; STEREO OBSERVATIONS; CORONAL STREAMERS; 1 AU; INTERPLANETARY MEDIUM; COMPRESSION REGIONS; SHOCK ACCELERATION; ION ENHANCEMENTS; ALPHA MONITOR AB We report observations of the acceleration and trapping of energetic ions and electrons between a pair of corotating interaction regions (CIRs). The event occurred in Carrington Rotation 2060. Observed by the STEREO-B spacecraft, the two CIRs were separated by less than 5 days. In contrast to other CIR events, the fluxes of the energetic ions and electrons in this event reached their maxima between the trailing edge of the first CIR and the leading edge of the second CIR. The radial magnetic field (B-r) reversed its sense and the anisotropy of the flux also changed from Sunward to anti-Sunward between the two CIRs. Furthermore, there was an extended period of counterstreaming suprathermal electrons between the two CIRs. Similar observations for this event were also obtained with the Advanced Composition Explorer and STEREO-A. We conjecture that these observations were due to a U-shaped, large-scale magnetic field topology connecting the reverse shock of the first CIR and the forward shock of the second CIR. Such a disconnected U-shaped magnetic field topology may have formed due to magnetic reconnection in the upper corona. C1 [Wu, Z.; Chen, Y.; Tang, C. L.] Shandong Univ Weihai, Inst Space Sci, Weihai 264209, Peoples R China. [Wu, Z.; Chen, Y.; Tang, C. L.] Shandong Univ Weihai, Sch Space Sci & Phys, Weihai 264209, Peoples R China. [Li, G.; Zhao, L. L.] Univ Alabama, Dept Space Sci, Huntsville, AL 35899 USA. [Li, G.; Zhao, L. L.] Univ Alabama, CSPAR, Huntsville, AL 35899 USA. [Ebert, R. W.; Desai, M. I.] SW Res Inst, San Antonio, TX 78228 USA. [Desai, M. I.] Univ Texas San Antonio, San Antonio, TX 78249 USA. [Mason, G. M.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Lavraud, B.; Sauvaud, J.] Univ Toulouse UPS, Inst Rech Astrophys & Planetol, Toulouse, France. [Lavraud, B.; Sauvaud, J.] CNRS, UMR 5277, Toulouse, France. [Zhao, L.; Landi, E.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48105 USA. [Liu, Y. C. -M.] Chinese Acad Sci, Natl Space Sci Ctr, State Key Lab Space Weather, Beijing 100190, Peoples R China. [Guo, F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Wu, Z (reprint author), Shandong Univ Weihai, Inst Space Sci, Weihai 264209, Peoples R China. EM gang.li@uah.edu RI Guo, Fan/H-1723-2013; Chen, Yao/B-7255-2011; Wu, Zhao/H-2359-2016; OI Guo, Fan/0000-0003-4315-3755; Zhao, Liang/0000-0002-5975-7476 FU NSF [AGS0962658, AGS1135432, ATM0847719, AGS-0962666]; NASA grant at UAH [NNX13AE07G, NNSFC41331068, 41274175, 41028004]; NSBRSF grant at SDUWH [2012CB825601]; NNSFC grant at NSSC [Y2503BA110]; University of California Berkeley at APL [SA4889-26309]; NSF grant at SWRI [AGS-0962666] FX This work is supported in part by NSF grants AGS0962658, AGS1135432 and ATM0847719 and NASA grant NNX13AE07G at UAH, NNSFC41331068, 41274175, 41028004, and NSBRSF 2012CB825601 at SDUWH, NNSFC Y2503BA110 at NSSC, NSF grant AGS-0962653, and contract SA4889-26309 from the University of California Berkeley at APL, and NSF grant AGS-0962666 at SWRI. We thank the referee for very useful suggestions. NR 70 TC 5 Z9 7 U1 2 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2014 VL 781 IS 1 AR 17 DI 10.1088/0004-637X/781/1/17 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 286AE UT WOS:000329436100017 ER PT J AU Aliu, E Archambault, S Aune, T Benbow, W Berger, K Bird, R Bouvier, A Buckley, JH Bugaev, V Byrum, K Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dumm, J Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortin, P Fortson, L Furniss, A Galante, N Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krennrich, F Kumar, S Lang, MJ Lyutikov, M Maier, G McArthur, S McCann, A Meagher, K Millis, J Moriarty, P Mukherjee, R de Bhroithe, AO Ong, RA Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Quinn, J Ragan, K Rajotte, J Reyes, LC Reynolds, PT Richards, GT Roache, E Sembroski, GH Sheidaei, F Smith, AW Staszak, D Telezhinsky, I Theiling, M Tucci, JV Tyler, J Varlotta, A Wakely, SP Weekes, TC Weinstein, A Welsing, R Williams, DA Zajczyk, A Zitzer, B AF Aliu, E. Archambault, S. Aune, T. Benbow, W. Berger, K. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Byrum, K. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dumm, J. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krennrich, F. Kumar, S. Lang, M. J. Lyutikov, M. Maier, G. McArthur, S. McCann, A. Meagher, K. Millis, J. Moriarty, P. Mukherjee, R. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Quinn, J. Ragan, K. Rajotte, J. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Sembroski, G. H. Sheidaei, F. Smith, A. W. Staszak, D. Telezhinsky, I. Theiling, M. Tucci, J. V. Tyler, J. Varlotta, A. Wakely, S. P. Weekes, T. C. Weinstein, A. Welsing, R. Williams, D. A. Zajczyk, A. Zitzer, B. TI A SEARCH FOR ENHANCED VERY HIGH ENERGY GAMMA-RAY EMISSION FROM THE 2013 MARCH CRAB NEBULA FLARE SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE gamma rays: general; ISM: individual objects (Crab Nebula) ID LARGE-AREA TELESCOPE; VARIABILITY; APRIL AB In 2013 March, a flaring episode from the Crab Nebula lasting similar to 2 weeks was detected by Fermi-LAT (Large Area Telescope on board the Fermi Gamma-ray Space Telescope). The Very Energetic Radiation Imaging Telescope Array System (VERITAS) provides simultaneous observations throughout this period. During the flare, Fermi-LAT detected a 20 fold increase in flux above the average synchrotron flux >100 MeV seen from the Crab Nebula. Simultaneous measurements with VERITAS are consistent with the non-variable long-term average Crab Nebula flux at TeV energies. Assuming a linear correlation between the very high energy flux change >1 TeV and the flux change seen in the Fermi-LAT band >100 MeV during the period of simultaneous observations, the linear correlation factor can be constrained to be at most 8.6 x 10(-3) with 95% confidence. C1 [Aliu, E.; Errando, M.; Mukherjee, R.] Columbia Univ, Dept Phys & Astron, Barnard Coll, New York, NY 10027 USA. [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Rajotte, J.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Aune, T.; Ong, R. A.; Popkow, A.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Benbow, W.; Cerruti, M.; Fortin, P.; Galante, N.; Roache, E.; Weekes, T. C.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bird, R.; Khassen, Y.; de Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Buckley, J. H.; Bugaev, V.; Zajczyk, A.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Byrum, K.; Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Chen, X.; Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, X.; Federici, S.; Hughes, G.; Maier, G.; Pohl, M.; Telezhinsky, I.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Lyutikov, M.; Sembroski, G. H.; Theiling, M.; Tucci, J. V.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Humensky, T. B.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Sheidaei, F.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Krennrich, F.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Millis, J.] Anderson Univ, Dept Phys, Anderson, IN 46012 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. RP Aliu, E (reprint author), Columbia Univ, Dept Phys & Astron, Barnard Coll, New York, NY 10027 USA. RI Khassen, Yerbol/I-3806-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Cui, Wei/0000-0002-6324-5772; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; STFC in the U.K. FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. NR 36 TC 6 Z9 6 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JAN 20 PY 2014 VL 781 IS 1 AR L11 DI 10.1088/2041-8205/781/1/L11 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 287ZY UT WOS:000329582400011 ER PT J AU Zhou, J AF Zhou, Jia TI Stacking interactions of nickel bis(dithiolene) with benzene SO CHEMICAL PHYSICS LETTERS LA English DT Article ID DENSITY FUNCTIONALS; METAL-COMPLEXES; THERMOCHEMISTRY; ACCURACY; ENERGIES; CHELATE AB Density functional theory with dispersion correction has been used to letter the stacking interactions of nickel bis(dithiolene) and benzene. Two different orientations of benzene molecule towards nickel bis(dithiolene) are considered, and they are close in energy. Detailed investigations discover that these two orientations could change from one to the other when benzene moving along the nickel bis(dithiolene). The stacking interaction energy is found to be very high, compared with other similar systems. This stacking complex as one building unit could stimulate further letter on the bilayer of 2D nickel bis(dithiolene) nanosheet and graphene, which is useful in the molecular electronics. (C) 2013 Elsevier B.V. All rights reserved. C1 Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhou, J (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM zhouj1@ornl.gov FU Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This research in part used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. The author thanks Prof. Schlegel for helpful comments. NR 34 TC 0 Z9 0 U1 3 U2 43 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD JAN 20 PY 2014 VL 591 BP 29 EP 31 DI 10.1016/j.cplett.2013.10.088 PG 3 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 282YG UT WOS:000329210200007 ER PT J AU Zhang, C Song, C Fry, HC Rosi, NL AF Zhang, Chen Song, Chengyi Fry, H. Christopher Rosi, Nathaniel L. TI Peptide Conjugates for Directing the Morphology and Assembly of 1D Nanoparticle Superstructures SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE gold; nanoparticles; peptides; self-assembly; superstructures ID AMPHIPHILE NANOFIBERS; GOLD NANOPARTICLES; AROMATIC INTERACTIONS; INORGANIC MATERIALS; SIZE; NANOMATERIALS; NANOCRYSTALS; CHEMISTRY; DESIGN AB Designed peptide conjugates molecules are used to direct the synthesis and assembly of gold nanoparticles into complex 1D nanoparticle superstructures with various morphologies. Four peptide conjugates, each based on the gold-binding peptide (AYSSGAPPMPPF; PEPAu), are prepared: C12H23O-AYSSGAPPMPP (1), C12H23O-AYSSGAPPMPPF (2), C12H23O-AYSSGAPPMPPFF (3), and C12H23O-AYSSGAPPMPPFFF (4). The affect that C-terminal hydrophobic F residues have on both the soft-assembly of the peptide conjugates and the resulting assembly of gold nanoparticle superstructures is examined. It is shown that the addition of two C-terminal F residues (3) leads to thick, branched 1D gold nanoparticle superstructures, whereas the addition of three C-terminal F residues (4) leads to bundling of thin 1D nanoparticle superstructures. C1 [Zhang, Chen; Song, Chengyi; Rosi, Nathaniel L.] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Fry, H. Christopher] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Rosi, NL (reprint author), Univ Pittsburgh, Dept Chem, 219 Parkman Ave, Pittsburgh, PA 15260 USA. EM nrosi@pitt.edu FU National Science Foundation [DMR-0954380]; Air Force Office of Scientific Research [FA9550-11-1-0275]; U. S. Department of Energy, Office of Science, and Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX Support for this work was provided in part by the National Science Foundation (DMR-0954380, N.L.R.) and in part by the Air Force Office of Scientific Research (FA9550-11-1-0275, N.L.R.). A portion of the peptide synthesis was performed at the Center for Nanoscale Materials, a U. S. Department of Energy, Office of Science, and Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. The authors thank the Peterson NFCF, the MEMS Department and Department of Biological Sciences for provision of access to TEM. NR 39 TC 7 Z9 7 U1 2 U2 53 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JAN 20 PY 2014 VL 20 IS 4 BP 941 EP 945 DI 10.1002/chem.201304074 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 287NG UT WOS:000329548000003 PM 24356987 ER PT J AU Berlin, A Hooper, D AF Berlin, Asher Hooper, Dan TI Stringent constraints on the dark matter annihilation cross section from subhalo searches with the Fermi Gamma-Ray Space Telescope SO PHYSICAL REVIEW D LA English DT Article ID EVOLUTION; HALOES AB The dark matter halo of the Milky Way is predicted to contain a very large number of smaller subhalos. As a result of the dark matter annihilations taking place within such objects, the most nearby and massive subhalos could appear as pointlike or spatially extended gamma-ray sources, without observable counterparts at other wavelengths. In this paper, we use the results of the Aquarius simulation to predict the distribution of nearby subhalos and compare this to the characteristics of the unidentified gamma-ray sources observed by the Fermi Gamma-Ray Space Telescope. Focusing on the brightest high latitude sources, we use this comparison to derive limits on the dark matter annihilation cross section. For dark matter particles lighter than similar to 200 GeV, the resulting limits are the strongest obtained to date, being modestly more stringent than those derived from observations of dwarf galaxies or the Galactic center. We also derive independent limits based on the lack of unidentified gamma-ray sources with discernible spatial extension, but these limits are a factor of similar to 2-10 weaker than those based on pointlike subhalos. Lastly, we note that four of the ten brightest high-latitude sources exhibit a similar spectral shape, consistent with 30-60 GeV dark matter particles annihilating to b (b) over bar with an annihilation cross section on the order of sigma nu similar to (5-10) x 10(-27) cm(3)/s or 8-10 GeV dark matter particles annihilating to tau(+)tau(-) with sigma nu similar to (1.5-3.0) x 10(-27) cm(3)/s. C1 [Berlin, Asher] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Hooper, Dan] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. RP Berlin, A (reprint author), Univ Chicago, Dept Phys, 5720 S Ellis Ave, Chicago, IL 60637 USA. FU US Department of Energy; Kavli Institute for Cosmological Physics FX We would like to thank Andrew Hearin, Keith Bechtol, and Tongyan Lin for valuable discussions. We would also like to acknowledge the hospitality of the Aspen Center for Physics, where this work was in part completed. This work has been supported by the US Department of Energy and by the Kavli Institute for Cosmological Physics. NR 32 TC 27 Z9 27 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 17 PY 2014 VL 89 IS 1 AR 016014 DI 10.1103/PhysRevD.89.016014 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5YW UT WOS:000331865600002 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Heracleous, N Kalogeropoulos, A Keaveney, J Kim, TJ Lowette, S Maes, M Olbrechts, A Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Favart, L Gay, APR Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jez, P Komm, M Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A 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CA CMS Collaboration TI Measurement of Higgs boson production and properties in the WW decay channel with leptonic final states SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Higgs physics ID STANDARD MODEL; HADRON COLLIDERS; ROOT-S=7 TEV; ELECTROWEAK CORRECTIONS; PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; QCD CORRECTIONS; ATLAS DETECTOR; PP COLLISIONS AB A search for the standard model Higgs boson decaying to a W-boson pair at the LHC is reported. The event sample corresponds to an integrated luminosity of 4.9 fb(-1) and 19.4 fb(-1) collected with the CMS detector in pp collisions at = 7 and 8 TeV, respectively. The Higgs boson candidates are selected in events with two or three charged leptons. An excess of events above background is observed, consistent with the expectation from the standard model Higgs boson with a mass of around 125 GeV. The probability to observe an excess equal or larger than the one seen, under the background-only hypothesis, corresponds to a significance of 4.3 standard deviations for m (H) = 125.6 GeV. The observed signal cross section times the branching fraction to WW for m (H) = 125.6 GeV is times the standard model expectation. The spin-parity J (P) = 0(+) hypothesis is favored against a narrow resonance with J (P) = 2(+) or J (P) = 0(-) that decays to a W-boson pair. This result provides strong evidence for a Higgs-like boson decaying to a W-boson pair. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.; Tosi, M.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.; Campagnari, C.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Barbagli, G.; Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Costa, S.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Lee, S.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.] Univ Malaya Jabatan Fiz, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autnoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. 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[Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Milosevic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Papacz, P.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Giffels, M.; Gigi, D.; Gill, K.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Mulders, M.; Musella, P.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. 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Millan; Ngadiuba, J.; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yuecel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St. John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Kovalskyi, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. 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Petrushanko, Sergey/D-6880-2012; Santoro, Alberto/E-7932-2014; Bonacorsi, Daniele/F-1505-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Codispoti, Giuseppe/F-6574-2014; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Popov, Andrey/E-1052-2012; Ligabue, Franco/F-3432-2014; OI Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hill, Christopher/0000-0003-0059-0779; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ragazzi, Stefano/0000-0001-8219-2074; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Novaes, Sergio/0000-0003-0471-8549; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Codispoti, Giuseppe/0000-0003-0217-7021; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Lo Vetere, Maurizio/0000-0002-6520-4480; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Costa, Salvatore/0000-0001-9919-0569; Kasemann, Matthias/0000-0002-0429-2448; Tosi, Nicolo/0000-0002-0474-0247; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; WANG, MIN-ZU/0000-0002-0979-8341; Popov, Andrey/0000-0002-1207-0984; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Margaroli, Fabrizio/0000-0002-3869-0153; Landsberg, Greg/0000-0002-4184-9380; Rizzi, Andrea/0000-0002-4543-2718; Gershtein, Yuri/0000-0002-4871-5449; Tricomi, Alessia Rita/0000-0002-5071-5501; Malik, Sudhir/0000-0002-6356-2655; Blekman, Freya/0000-0002-7366-7098; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Barbieri, Richard/0000-0002-7945-005X; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Staiano, Amedeo/0000-0003-1803-624X; Ciulli, Vitaliano/0000-0003-1947-3396; Tonelli, Guido Emilio/0000-0003-2606-9156; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Toback, David/0000-0003-3457-4144; Martelli, Arabella/0000-0003-3530-2255; Abbiendi, Giovanni/0000-0003-4499-7562; Gonzi, Sandro/0000-0003-4754-645X; HSIUNG, YEE/0000-0003-4801-1238; Levchenko, Petr/0000-0003-4913-0538; Vidal Marono, Miguel/0000-0002-2590-5987; Goldstein, Joel/0000-0003-1591-6014; Heath, Helen/0000-0001-6576-9740; Grassi, Marco/0000-0003-2422-6736; ORTONA, Giacomo/0000-0001-8411-2971; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Ulrich, Ralf/0000-0002-2535-402X; Verdier, Patrice/0000-0003-3090-2948; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Sogut, Kenan/0000-0002-9682-2855; Jacob, Jeson/0000-0001-6895-5493 FU Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; COLCIENCIAS; Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology, Republic of Korea; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; EU-ESF; Greek NSRF; Austrian Federal Ministry of Science and Research; SEP; European Research Council (European Union); Aristeia programme FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 105 TC 51 Z9 51 U1 5 U2 108 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 17 PY 2014 IS 1 AR 096 DI 10.1007/JHEP01(2014)096 PG 86 WC Physics, Particles & Fields SC Physics GA AA0NV UT WOS:000330792800001 ER PT J AU Granados, C Weiss, C AF Granados, C. Weiss, C. TI Chiral dynamics and peripheral transverse densities SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Chiral Lagrangians; Parton Model; 1/N Expansion ID GENERALIZED PARTON DISTRIBUTIONS; ELECTROMAGNETIC FORM-FACTORS; IMPACT PARAMETER SPACE; PERTURBATION-THEORY; INFINITE-MOMENTUM; QUANTUM ELECTRODYNAMICS; RESONANCE PHYSICS; SKYRME MODEL; NULL-PLANE; NUCLEON AB In the partonic (or light-front) description of relativistic systems the electromagnetic form factors are expressed in terms of frame-independent charge and magnetization densities in transverse space. This formulation allows one to identify the chiral components of nucleon structure as the peripheral densities at transverse distances b = O(M-pi(-1)) and compute them in a parametrically controlled manner. A dispersion relation connects the large-distance behavior of the transverse charge and magnetization densities to the spectral functions of the Dirac and Pauli form factors near the two-pion threshold at time-like t = 4M(pi)(2), which can be computed in relativistic chiral effective field theory. Using the leading-order approximation we (a) derive the asymptotic behavior (Yukawa tail) of the isovector transverse densities in the "chiral" region b = O(M-pi(-1)) and the "molecular" region b = O(M-N(2)/M-pi(3)); (b) perform the heavy-baryon expansion of the transverse densities; (c) explain the relative magnitude of the peripheral charge and magnetization densities in a simple mechanical picture; (d) include Delta isobar intermediate states and study the peripheral transverse densities in the large-N-c limit of QCD; (e) quantify the region of transverse distances where the chiral components of the densities are numerically dominant; (f) calculate the chiral divergences of the b(2)-weighted moments of the isovector transverse densities (charge and anomalous magnetic radii) in the limit M-pi -> 0 and determine their spatial support. Our approach provides a concise formulation of the spatial structure of the nucleon's chiral component and offers new insights into basic properties of the chiral expansion. It relates the information extracted from low-t elastic form factors to the generalized parton distributions probed in peripheral high-energy scattering processes. C1 [Granados, C.; Weiss, C.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. RP Granados, C (reprint author), Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden. EM carlos.granados@physics.uu.se; weiss@jlab.org FU Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX Authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. The U.S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce this manuscript for U.S. Government purposes. NR 90 TC 6 Z9 6 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 17 PY 2014 IS 1 AR 092 DI 10.1007/JHEP01(2014)092 PG 81 WC Physics, Particles & Fields SC Physics GA 303AG UT WOS:000330646000005 ER PT J AU Bracht, H Eon, S Frieling, R Plech, A Issenmann, D Wolf, D Hansen, JL Larsen, AN Ager, JW Haller, EE AF Bracht, H. Eon, S. Frieling, R. Plech, A. Issenmann, D. Wolf, D. Hansen, J. Lundsgaard Larsen, A. Nylandsted Ager, J. W., III Haller, E. E. TI Thermal conductivity of isotopically controlled silicon nanostructures SO NEW JOURNAL OF PHYSICS LA English DT Article ID ENRICHED SILICON; MOLECULAR-DYNAMICS; SUPERLATTICES; NANOWIRES; ISOTOPE AB Nanostructured semiconductors open the opportunity to independently tailor electric and thermal conductivity by manipulation of the phonon transport. Nanostructuring of materials is a highly promising strategy for engineering thermoelectric devices with improved efficiency. The concept of reducing the thermal conductivity without degrading the electrical conductivity is most ideally realized by controlled isotope doping. This work reports on experimental and theoretical investigations on the thermal conductivity of isotopically modulated silicon nanostructures. State-of-the-art pump-and-probe experiments are conducted to determine the thermal conductivity of the different nanostructures of isotopically enriched silicon layers epitaxially grown on natural silicon substrates. Concomitant molecular dynamics calculations are performed to study the impact of the silicon isotope mass, isotope interfaces, and of the isotope layer ordering and thickness on the thermal conductivity. Engineering the isotope distribution is a striking concept to reduce the thermal conductivity of silicon without affecting its electronic properties. This approach, using isotopically engineered silicon, might pave the way for future commercial thermoelectric devices. C1 [Bracht, H.; Eon, S.; Frieling, R.] Univ Munster, Inst Mat Phys, D-48149 Munster, Germany. [Plech, A.; Issenmann, D.] ANKA, Karlsruher Inst Technol, Inst Photon Sci & Synchrotron Radiat, D-76344 Eggenstein Leopoldshafen, Germany. [Wolf, D.] Univ Duisburg Essen, Fac Phys, D-47048 Duisburg, Germany. [Hansen, J. Lundsgaard; Larsen, A. Nylandsted] Univ Aarhus, Dept Phys & Astron, DK-8000 Aarhus, Denmark. [Ager, J. W., III; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bracht, H (reprint author), Univ Munster, Inst Mat Phys, Wilhelm Klemm Str 10, D-48149 Munster, Germany. EM bracht@uni-muenster.de RI Plech, Anton/E-4895-2010; OI Ager, Joel/0000-0001-9334-9751; Plech, Anton/0000-0002-6290-9303 FU Deutsche Forschungsgemeinschaft [SPP1386, BR 1520/13-1, BR 1520/15-1, BR 1520/10-2]; Initiatives for Proliferation Prevention Program of the Office of Nonproliferation Research and Engineering of the U.S. Department of Energy [DE-LambdaC03-76SF00098] FX Provision of beamtime at the facilities ANKA and ESRF is gratefully acknowledged. We wish to thank for the excellent support by M Khakulin, M Wulff and G Buth. This work was funded by the Deutsche Forschungsgemeinschaft via the priority program SPP1386 'Nanostructured Thermoelectric Materials: Theory, Model Systems and Controlled Synthesis' (BR 1520/13-1 and BR 1520/15-1) and individual grants for AP and within the Heisenberg program for HB (BR 1520/10-2). The isotopically enriched Si was developed by the Initiatives for Proliferation Prevention Program of the Office of Nonproliferation Research and Engineering (NN-20) of the U.S. Department of Energy under contract DE-Lambda C03-76SF00098. Stimulating discussions with G Bastian, A Vogelsang and C Heiliger are acknowledged. NR 36 TC 10 Z9 10 U1 0 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 17 PY 2014 VL 16 AR 015021 DI 10.1088/1367-2630/16/1/015021 PG 18 WC Physics, Multidisciplinary SC Physics GA 302SA UT WOS:000330624000001 ER PT J AU Creeth, GL Strudwick, AJ Sadowski, JT Marrows, CH AF Creeth, G. L. Strudwick, A. J. Sadowski, J. T. Marrows, C. H. TI Quantum corrections to the conductivity of disordered graphene on SiC (000(1)over-bar): weak localization and current-bias dependent electron-electron interactions SO NEW JOURNAL OF PHYSICS LA English DT Article ID SUSPENDED GRAPHENE; BILAYER GRAPHENE; BERRYS PHASE; GRAPHITE; MAGNETORESISTANCE; TEMPERATURE; FIELDS; GAS AB The properties of epitaxial graphene grown via thermal decomposition of silicon carbide are extremely sensitive to annealing conditions. Here we show how the surface morphologies resulting from a range of UHV growth protocols affect the electron scattering rates associated with various quantum corrections to the conductivity. Detailed analysis of magnetotransport data provides insight into the degree of disorder via fits to weak localization and weak antilocalization models, while additional fitting is used to identify more subtle contributions from electron-electron (e-e) interaction effects. This second contribution is found to be current-bias dependent, and is seen only for more disordered samples, which is attributed to the shorter mean free path in these materials. C1 [Creeth, G. L.; Strudwick, A. J.; Marrows, C. H.] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [Sadowski, J. T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Creeth, GL (reprint author), UCL, London Ctr Nanotechnol, London WC1H 0AH, England. EM g.creeth@ucl.ac.uk; c.h.marrows@leeds.ac.uk FU United Kingdom EPSRC [EP/G009104/1, EP/G005176/1]; Intel Ireland; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We acknowledge useful discussions with N A Porter. The authors acknowledge financial support from the United Kingdom EPSRC (grant numbers EP/G009104/1 and EP/G005176/1) and Intel Ireland. This research was carried out in part at the National Synchrotron Light Source and the Center for Functional Nanomaterials, both at Brookhaven National Laboratory, which is supported by the US Department of Energy, Office of Basic Energy Sciences, under contract number DE-AC02-98CH10886. NR 48 TC 1 Z9 1 U1 3 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 17 PY 2014 VL 16 AR 013024 DI 10.1088/1367-2630/16/1/013024 PG 11 WC Physics, Multidisciplinary SC Physics GA 302RW UT WOS:000330623600001 ER PT J AU Chernyak, VY Chertkov, M Bierkens, J Kappen, HJ AF Chernyak, Vladimir Y. Chertkov, Michael Bierkens, Joris Kappen, Hilbert J. TI Stochastic optimal control as non-equilibrium statistical mechanics: calculus of variations over density and current SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE stochastic optimal control; non-equilibrium statistical physics; Bellman-Hamilton-Jacobi equation; gauge transformations ID MODELS AB In stochastic optimal control (SOC) one minimizes the average cost-to-go, that consists of the cost-of-control (amount of efforts), cost-of-space (where one wants the system to be) and the target cost (where one wants the system to arrive), for a system participating in forced and controlled Langevin dynamics. We extend the SOC problem by introducing an additional cost-of-dynamics, characterized by a vector potential. We propose derivation of the generalized gauge-invariant Hamilton-Jacobi-Bellman equation as a variation over density and current, suggest hydrodynamic interpretation and discuss examples, e. g., ergodic control of a particle-within-a-circle, illustrating non-equilibrium spacetime complexity. C1 [Chernyak, Vladimir Y.] Wayne State Univ, Dept Chem, Detroit, MI 48202 USA. [Chernyak, Vladimir Y.; Chertkov, Michael] LANL, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Chernyak, Vladimir Y.; Chertkov, Michael] LANL, Div Theoret, Los Alamos, NM 87545 USA. [Bierkens, Joris; Kappen, Hilbert J.] Radboud Univ Nijmegen, SNN Adapt Intelligence, NL-6500 HB Nijmegen, Netherlands. RP Chernyak, VY (reprint author), Wayne State Univ, Dept Chem, 5101 Cass Ave, Detroit, MI 48202 USA. EM chertkov@lanl.gov RI Kappen, H.J./L-4425-2015; Chertkov, Michael/O-8828-2015; Chernyak, Vladimir/F-5842-2016; OI Chernyak, Vladimir/0000-0003-4389-4238; Chertkov, Michael/0000-0002-6758-515X FU NSF [CHE-1111350]; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; [231495] FX In this communication we focused on the physics analysis and interpretations of the density/current variational formulation of the SOC. A reader interested in related mathematically rigorous results is advised to consult [39]. The research of VYC has received support from the NSF under grant agreement no. CHE-1111350. The work at LANL was carried out under the auspices of the National Nuclear Security Administration of the US Department of Energy under contract no. DE-AC52-06NA25396. The research of JB and HJK was funded by the FP7/2007-2013 program under the grant no. 231495. NR 39 TC 2 Z9 2 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD JAN 17 PY 2014 VL 47 IS 2 AR 022001 DI 10.1088/1751-8113/47/2/022001 PG 8 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA 280OV UT WOS:000329041500002 ER PT J AU Chou, YC Hillerich, K Tersoff, J Reuter, MC Dick, KA Ross, FM AF Chou, Y. -C. Hillerich, K. Tersoff, J. Reuter, M. C. Dick, K. A. Ross, F. M. TI Atomic-Scale Variability and Control of III-V Nanowire Growth Kinetics SO SCIENCE LA English DT Article ID SUPERLATTICES; MORPHOLOGY AB In the growth of nanoscale device structures, the ultimate goal is atomic-level precision. By growing III-V nanowires in a transmission electron microscope, we measured the local kinetics in situ as each atomic plane was added at the catalyst-nanowire growth interface by the vapor-liquid-solid process. During growth of gallium phosphide nanowires at typical V/III ratios, we found surprising fluctuations in growth rate, even under steady growth conditions. We correlated these fluctuations with the formation of twin defects in the nanowire, and found that these variations can be suppressed by switching to growth conditions with a low V/III ratio. We derive a growth model showing that this unexpected variation in local growth kinetics reflects the very different supply pathways of the V and III species. The model explains under which conditions the growth rate can be controlled precisely at the atomic level. C1 [Chou, Y. -C.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Chou, Y. -C.] Natl Chiao Tung Univ, Dept Electrophys, Hsinchu 300, Taiwan. [Hillerich, K.; Dick, K. A.] Lund Univ, S-22100 Lund, Sweden. [Tersoff, J.; Reuter, M. C.; Ross, F. M.] IBM Corp, Div Res, TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. RP Ross, FM (reprint author), IBM Corp, Div Res, TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. EM fmross@us.ibm.com RI Dick, Kimberly/A-8579-2008; OI Dick, Kimberly/0000-0003-4125-2039; /0000-0002-7775-2927 FU Center for Functional Nanomaterials, Brookhaven National Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; NSF [DMR-0907483]; Nanometer Structure Consortium at Lund University; Swedish Research Council; Swedish Foundation for Strategic Research; Knut and Alice Wallenberg Foundation FX Supported by the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract DE-AC02-98CH10886 (Y.-C.C.); NSF grant DMR-0907483; and the Nanometer Structure Consortium at Lund University, the Swedish Research Council, the Swedish Foundation for Strategic Research, and the Knut and Alice Wallenberg Foundation. Y.-C.C. and K. H. performed experiments and data analysis, J.T. developed the growth model, M. C. R. developed the experimental techniques, and K. A. D. and F. M. R. designed the experiments and coordinated the analysis. NR 28 TC 30 Z9 31 U1 11 U2 149 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 17 PY 2014 VL 343 IS 6168 BP 281 EP 284 DI 10.1126/science.1244623 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 289YN UT WOS:000329718600031 PM 24436416 ER PT J AU Sun, C Bufford, D Chen, Y Kirk, MA Wang, YQ Li, M Wang, H Maloy, SA Zhang, X AF Sun, C. Bufford, D. Chen, Y. Kirk, M. A. Wang, Y. Q. Li, M. Wang, H. Maloy, S. A. Zhang, X. TI In situ study of defect migration kinetics in nanoporous Ag with enhanced radiation tolerance SO SCIENTIFIC REPORTS LA English DT Article ID MECHANICAL-PROPERTIES; IRRADIATED MATERIALS; METALS; DAMAGE; CLUSTERS; HELIUM; IRON; CHALLENGES; NANOSCALE; SURFACE AB Defect sinks, such as grain boundaries and phase boundaries, have been widely accepted to improve the irradiation resistance of metallic materials. However, free surface, an ideal defect sink, has received little attention in bulk materials as surface-to-volume ratio is typically low. Here by using in situ Kr ion irradiation technique in a transmission electron microscope, we show that nanoporous (NP) Ag has enhanced radiation tolerance. Besides direct evidence of free surface induced frequent removal of various types of defect clusters, we determined, for the first time, the global and instantaneous diffusivity of defect clusters in both coarse-grained (CG) and NP Ag. Opposite to conventional wisdom, both types of diffusivities are lower in NP Ag. Such a surprise is largely related to the reduced interaction energy between isolated defect clusters in NP Ag. Determination of kinetics of defect clusters is essential to understand and model their migration and clustering in irradiated materials. C1 [Sun, C.; Bufford, D.; Chen, Y.; Wang, H.; Zhang, X.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sun, C.; Wang, Y. Q.; Maloy, S. A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Kirk, M. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, M.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Wang, H.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Zhang, X.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RP Zhang, X (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. EM zhangx@tamu.edu RI Zhang, Xinghang/H-6764-2013; Wang, Haiyan/P-3550-2014; Maloy, Stuart/A-8672-2009; Chen, Youxing/P-5006-2016 OI Zhang, Xinghang/0000-0002-8380-8667; Wang, Haiyan/0000-0002-7397-1209; Maloy, Stuart/0000-0001-8037-1319; Chen, Youxing/0000-0003-1111-4495 FU NSF-DMR-Metallic Materials and Nanostructures Program [1304101]; DOE-NEUP [DE-AC07-05ID14517-00088120]; US Army Research Office - Materials Science Division [W911NF-09-1-0223]; DOE-BES FX We acknowledge financial support by NSF-DMR-Metallic Materials and Nanostructures Program under grant no. 1304101. C. Sun was partially supported by DOE-NEUP under contract no. DE-AC07-05ID14517-00088120. Y. Chen was partially supported by US Army Research Office - Materials Science Division under contract no. W911NF-09-1-0223. We also thank Peter M. Baldo and Edward A. Ryan at Argonne National Laboratory for their help during in situ irradiation experiments. The IVEM facility at Argonne National Laboratory is supported by DOE-BES. Access to the DOE - Center for Integrated Nanotechnologies (CINT) at Los Alamos and Sandia National Laboratories and Microscopy and Imaging Center at Texas A&M University is also acknowledged. NR 43 TC 17 Z9 17 U1 0 U2 55 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 17 PY 2014 VL 4 AR 3737 DI 10.1038/srep03737 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291SH UT WOS:000329849100003 PM 24435181 ER PT J AU Schiller, QT Li, XL Blum, L Tu, WC Turner, DL Blake, JB AF Schiller, Quintin Li, Xinlin Blum, Lauren Tu, Weichao Turner, Drew L. Blake, J. B. TI A nonstorm time enhancement of relativistic electrons in the outer radiation belt SO GEOPHYSICAL RESEARCH LETTERS LA English DT Letter DE relativistic electrons; outer radiation belt; enhancement; phase space density; internal acceleration; rapid radial transport ID VAN-ALLEN RADIATION; SOLAR-WIND; MAGNETIC STORMS; GEOMAGNETIC STORMS; GEOSYNCHRONOUS ORBIT; ENERGETIC PARTICLE; ACCELERATION; MODEL; MAGNETOSPHERE; ENERGIZATION AB Despite the lack of a geomagnetic storm (based on the Dst index), relativistic electron fluxes were enhanced over 2.5 orders of magnitude in the outer radiation belt in 13h on 13-14 January 2013. The unusual enhancement was observed by Magnetic Electron Ion Spectrometer (MagEIS), onboard the Van Allen Probes; Relativistic Electron and Proton Telescope Integrated Little Experiment, onboard the Colorado Student Space Weather Experiment; and Solid State Telescope, onboard Time History of Events and Macroscale Interactions during Substorms (THEMIS). Analyses of MagEIS phase space density (PSD) profiles show a positive outward radial gradient from 4 Extreme relativistic electron enhancements do not require a geomagnetic storm This enhancement is caused by internal acceleration and rapid radial transport Conjunctive measurements are required to better understand system dynamics C1 [Schiller, Quintin; Li, Xinlin; Blum, Lauren] Univ Colorado, Dept Aerosp Engn Sci, Boulder, CO 80303 USA. [Schiller, Quintin; Li, Xinlin; Blum, Lauren] Univ Colorado, Atmospher & Space Phys Lab, Boulder, CO 80303 USA. [Tu, Weichao] Los Alamos Natl Lab, ISR 1, Space Sci & Applicat, Los Alamos, NM USA. [Turner, Drew L.] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA USA. [Blake, J. B.] Aerosp Corp, Dept Space Sci, Los Angeles, CA 90009 USA. RP Schiller, QT (reprint author), Univ Colorado, Dept Aerosp Engn Sci, Boulder, CO 80303 USA. EM quintinschiller@gmail.com RI Tu, Weichao/B-6507-2011; OI Tu, Weichao/0000-0003-4547-3269; Blum, Lauren/0000-0002-4797-5476 NR 37 TC 8 Z9 8 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 16 PY 2014 VL 41 IS 1 BP 7 EP 12 DI 10.1002/2013GL058485 PG 6 WC Geosciences, Multidisciplinary SC Geology GA AD1JL UT WOS:000332990200002 ER PT J AU Foster, JC Erickson, PJ Baker, DN Claudepierre, SG Kletzing, CA Kurth, W Reeves, GD Thaller, SA Spence, HE Shprits, YY Wygant, JR AF Foster, J. C. Erickson, P. J. Baker, D. N. Claudepierre, S. G. Kletzing, C. A. Kurth, W. Reeves, G. D. Thaller, S. A. Spence, H. E. Shprits, Y. Y. Wygant, J. R. TI Prompt energization of relativistic and highly relativistic electrons during a substorm interval: Van Allen Probes observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Letter DE Relativistic Electrons; Substorm; Radiation Belts; Prompt Energizations ID INNER MAGNETOSPHERE; ENERGETIC PARTICLE; RADIATION BELTS; ACCELERATION; TRANSPORT AB On 17 March 2013, a large magnetic storm significantly depleted the multi-MeV radiation belt. We present multi-instrument observations from the Van Allen Probes spacecraft Radiation Belt Storm Probe A and Radiation Belt Storm Probe B at similar to 6Re in the midnight sector magnetosphere and from ground-based ionospheric sensors during a substorm dipolarization followed by rapid reenergization of multi-MeV electrons. A 50% increase in magnetic field magnitude occurred simultaneously with dramatic increases in 100keV electron fluxes and a 100 times increase in VLF wave intensity. The 100keV electrons and intense VLF waves provide a seed population and energy source for subsequent radiation belt enhancements. Highly relativistic (>2MeV) electron fluxes increased immediately at L*similar to 4.5 and 4.5MeV flux increased >90 times at L*=4 over 5h. Although plasmasphere expansion brings the enhanced radiation belt multi-MeV fluxes inside the plasmasphere several hours postsubstorm, we localize their prompt reenergization during the event to regions outside the plasmasphere. Key Points Substorm dynamics are important for highly relativistic electron energization Cold plasma preconditioning is significant for rapid relativistic energization Relativistic / highly relativistic electron energization can occur in < 5 hrs C1 [Foster, J. C.; Erickson, P. J.] MIT, Haystack Observ, Atmospher Sci Grp, Westford, MA 01886 USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Boulder, CO 80309 USA. [Claudepierre, S. G.] Aerosp Corp, Dept Space Sci, Los Angeles, CA 90009 USA. [Kletzing, C. A.; Kurth, W.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Thaller, S. A.; Wygant, J. R.] Univ Minnesota, Dept Phys & Astron, Minneapolis, MN USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Shprits, Y. Y.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90024 USA. RP Erickson, PJ (reprint author), MIT, Haystack Observ, Atmospher Sci Grp, Westford, MA 01886 USA. EM pje@haystack.mit.edu RI Reeves, Geoffrey/E-8101-2011; OI Reeves, Geoffrey/0000-0002-7985-8098; Kletzing, Craig/0000-0002-4136-3348; Spence, Harlan/0000-0002-2526-2205; Kurth, William/0000-0002-5471-6202 NR 20 TC 21 Z9 21 U1 0 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 16 PY 2014 VL 41 IS 1 BP 20 EP 25 DI 10.1002/2013GL058438 PG 6 WC Geosciences, Multidisciplinary SC Geology GA AD1JL UT WOS:000332990200004 ER PT J AU Jethva, H Torres, O Waquet, F Chand, D Hu, YX AF Jethva, Hiren Torres, Omar Waquet, Fabien Chand, Duli Hu, Yongxiang TI How doA- train sensors intercompare in the retrieval of above- cloud aerosol optical depth? A case study- based assessment SO GEOPHYSICAL RESEARCH LETTERS LA English DT Letter DE Above-cloud Aerosol Optical Depth; A-train; Passive and Active Sensors ID EXTINCTION; CALIOP; LAYERS AB We intercompare the above-cloud aerosol optical depth (ACAOD) of biomass burning plumes retrieved from A-train sensors, i.e., Moderate Resolution Imaging Spectroradiometer (MODIS), Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Polarization and Directionality of Earth Reflectances (POLDER), and Ozone Monitoring Instrument (OMI). These sensors have shown independent capabilities to retrieve aerosol loading above marine boundary layer cloudsa kind of situation often found over the southeast Atlantic Ocean during dry burning season. A systematic comparison reveals that all passive sensors and CALIOP-based research methods derive comparable ACAOD with differences mostly within 0.2 over homogeneous cloud fields. The 532nm ACAOD retrieved by CALIOP operational algorithm is underestimated. The retrieved 1064nm AOD however shows closer agreement with passive sensors. Given the different types of measurements processed with different algorithms, the reported close agreement between them is encouraging. Due to unavailability of direct measurements above cloud, the validation of satellite-based ACAOD remains an open challenge. The intersatellite comparison however can be useful for the relative evaluation and consistency check. Key Points Above-cloud aerosol optical depths derived from A-train sensors are compared Agreement between sensors is robust over homogeneous cloud fields CALIOP 532nm retrieval was underestimated but its 1064nm is in close agreement C1 [Jethva, Hiren] Univ Space Res Assoc, Columbia, MD USA. [Jethva, Hiren; Torres, Omar] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Waquet, Fabien] Univ Lille, Lab Opt Atmospher, Villeneuve Dascq, France. [Chand, Duli] Pacific NW Natl Lab, Richland, WA 99352 USA. [Hu, Yongxiang] NASA, Langley Res Ctr, Hampton, VA 23665 USA. RP Jethva, H (reprint author), Univ Space Res Assoc, Columbia, MD USA. EM hiren.t.jethva@nasa.gov RI Hu, Yongxiang/K-4426-2012; Torres, Omar/G-4929-2013 NR 14 TC 16 Z9 16 U1 1 U2 13 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 16 PY 2014 VL 41 IS 1 BP 186 EP 192 DI 10.1002/2013GL058405 PG 7 WC Geosciences, Multidisciplinary SC Geology GA AD1JL UT WOS:000332990200031 ER PT J AU Sheng, F Liu, HH Wang, K Zhang, RD Tang, ZH AF Sheng, Feng Liu, Huihai Wang, Kang Zhang, Renduo Tang, Zehua TI Investigation into preferential flow in natural unsaturated soils with field multiple-tracer infiltration experiments and the active region model SO JOURNAL OF HYDROLOGY LA English DT Article DE Preferential flow; Multiple-tracer infiltration experiment; Solute transport; Macropore flow; Unstable flow; Active region model ID SOLUTE TRANSPORT; POROUS-MEDIA; MACROPORE CHARACTERISTICS; HYDRAULIC CONDUCTIVITY; FRACTURED ROCKS; BRILLIANT BLUE; CLAY SOIL; WATER; DYE; IRRIGATION AB Preferential flow in natural unsaturated soils is common, but difficult to characterize and predict. The major objective of this research is to investigate the preferential flow patterns with field-scale multiple-tracer infiltration experiments and to evaluate the capability of the active region model (ARM) in predicting the field-scale preferential flow and transport processes. For this purpose, the mixture solutions of iodine and bromide, iodine and nitrate, and again iodine and bromide, as the tracing solutes, were applied sequentially in two plots in natural unsaturated loam soil to illustrate the flow and transport processes. The distributions of soil water content and concentrations of applied tracing solutes (NO3- and Br-) were measured after experiments and predicted using ARM and the mobile-immobile region model (MIM). The relative root mean square errors (RRMSE) between those predictions (from ARM and MIM) and measured results were calculated for quantitatively evaluating the prediction accuracy and comparing the modeling efficiency of the two models. Both field observations and the ARM predictions indicated that there were macropores in Plot 1 but not in Plot 2, and the macropores in Plot 1 were mainly in the top 20 cm soil layer. The mixture solutions transported in the top 20 cm soil layer in Plot 1 were mainly from the soil surface directly and less affected by the macropore flow, while the preferential flow in the soil layer below 20 cm was considerably affected by the macropores and more applied mixture solutions were delivered into the deep soil layer quickly. Compared to the mixture solutions applied in the first and third steps, more mixture solution applied in the second step was transported to the deep soil layer by macropores, corresponding to obvious peaks of soil water content and NO3- concentration distributions observed in the deep soil layer in Plot 1. On the other hand, unstable flow was the major preferential flow behavior in Plot 2, inducing no obvious peaks of soil water content and solutes (NO3- and Br-) concentrations observed in the infiltrated soil profile. The comparisons between predicted and observed results in Plot 2 indicated that the ARM captured the overall behavior of unstable flow and associated tracer transport better than the MIM; however, to well characterize the macropore flow process, the ARM needs to be improved to include the effects of macropores. (C) 2013 Elsevier B.V. All rights reserved. C1 [Sheng, Feng; Tang, Zehua] Changsha Univ Sci & Technol, Sch Hydraul Engn, Changsha 410114, Hunan, Peoples R China. [Liu, Huihai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Wang, Kang] Wuhan Univ, State Key Lab Water Resources & Hydropower Engn S, Wuhan 430072, Peoples R China. [Zhang, Renduo] Sun Yat Sen Zhongshan Univ, Sch Environm Sci & Engn, Guangzhou 510275, Guangdong, Peoples R China. RP Sheng, F (reprint author), Changsha Univ Sci & Technol, Sch Hydraul Engn, Changsha 410114, Hunan, Peoples R China. EM shengf.china@gmail.com FU National Science Foundation of China [51109017, 51039007]; Hunan Provincial Natural Science Foundation of China [13JJ3069]; Open Research Fund Program of State Key Laboratory of Water Resources and Hydropower Engineering Science [2012B097] FX This research was financially supported in part by grants of the National Science Foundation of China (Nos. 51109017 and 51039007), Hunan Provincial Natural Science Foundation of China (No. 13JJ3069), and the Open Research Fund Program of State Key Laboratory of Water Resources and Hydropower Engineering Science (2012B097). We also appreciate the constructive comments from the editors and the anonymous reviewers. NR 73 TC 2 Z9 4 U1 7 U2 53 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD JAN 16 PY 2014 VL 508 BP 137 EP 146 DI 10.1016/j.jhydrol.2013.10.048 PG 10 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA AB9SI UT WOS:000332135600012 ER PT J AU Cosyn, W Melnitchouk, W Sargsian, M AF Cosyn, W. Melnitchouk, W. Sargsian, M. TI Final-state interactions in inclusive deep-inelastic scattering from the deuteron SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON STRUCTURE-FUNCTION; ELECTRON-SCATTERING; NUCLEAR-STRUCTURE; PROTON; COLLABORATION; TRANSPARENCY; BINDING; GLAUBER; GRAPHS; RATIO AB We explore the role of final-state interactions (FSIs) in inclusive deep-inelastic scattering from the deuteron. Relating the inclusive cross section to the deuteron forward virtual Compton scattering amplitude, a general formula for the FSI contribution is derived in the generalized eikonal approximation, utilizing the diffractive nature of the effective hadron-nucleon interaction. The calculation uses a factorized model with a basis of three resonances with mass W < 2 GeV and a continuum contribution for larger W as the relevant set of effective hadron states entering the final-state interaction amplitude. The results show sizeable on-shell FSI contributions for Bjorken x greater than or similar to 0.6 and Q(2) less than or similar to 10 GeV2, increasing in magnitude for lower Q(2), but vanishing in the high-Q(2) limit because of phase-space constraints. The off-shell rescattering contributes at x greater than or similar to 0.8 and is taken as an uncertainty on the on-shell result. C1 [Cosyn, W.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Cosyn, W.; Sargsian, M.] Florida Int Univ, Dept Phys, Miami, FL 33199 USA. [Melnitchouk, W.] Jefferson Lab, Newport News, VA 23606 USA. RP Cosyn, W (reprint author), Univ Ghent, Dept Phys & Astron, Proeftuinstr 86, B-9000 Ghent, Belgium. EM Wim.Cosyn@UGent.be FU Research Foundation Flanders (FWO-Flanders); DOE under Jefferson Science Associates, LLC,operates Jefferson Lab [DE-AC05-06OR23177]; US Department of Energy [DE-FG02-01ER41172]; Ghent University; Hercules Foundation; Flemish Government, department EWI FX W.C. is supported by the Research Foundation Flanders (FWO-Flanders). W.M. is supported by DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, operates Jefferson Lab. M.S. is supported by US Department of Energy grant under Contract No. DE-FG02-01ER41172. The computational resources (Stevin Supercomputer Infrastructure) and services used in this work were provided by Ghent University, the Hercules Foundation and the Flemish Government, department EWI. NR 61 TC 8 Z9 8 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JAN 16 PY 2014 VL 89 IS 1 AR 014612 DI 10.1103/PhysRevC.89.014612 PG 13 WC Physics, Nuclear SC Physics GA AB9ZQ UT WOS:000332154700003 ER PT J AU Maiti, A Small, W Gee, RH Weisgraber, TH Chinn, SC Wilson, TS Maxwell, RS AF Maiti, A. Small, W. Gee, R. H. Weisgraber, T. H. Chinn, S. C. Wilson, T. S. Maxwell, R. S. TI Mullins effect in a filled elastomer under uniaxial tension SO PHYSICAL REVIEW E LA English DT Article ID SURFACE MODIFICATION; NETWORK ALTERATION; SILICONE-RUBBER; STRESS; DEFORMATION; BEHAVIOR; MODEL; MECHANISM; POLYMERS; DAMAGE AB Modulus softening and permanent set in filled polymeric materials due to cyclic loading and unloading, commonly known as the Mullins effect, can have a significant impact on their use as support cushions. A quantitative analysis of such behavior is essential to ensure the effectiveness of such materials in long-term deployment. In this work we combine existing ideas of filler-induced modulus enhancement, strain amplification, and irreversible deformation within a simple non-Gaussian constitutive model to quantitatively interpret recent measurements on a relevant PDMS-based elastomeric cushion. We find that the experimental stress-strain data is consistent with the picture that during stretching (loading) two effects take place simultaneously: (1) the physical constraints (entanglements) initially present in the polymer network get disentangled, thus leading to a gradual decrease in the effective cross-link density, and (2) the effective filler volume fraction gradually decreases with increasing strain due to the irreversible pulling out of an initially occluded volume of the soft polymer domain. C1 [Maiti, A.; Small, W.; Gee, R. H.; Weisgraber, T. H.; Chinn, S. C.; Wilson, T. S.; Maxwell, R. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Maiti, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM amaiti@llnl.gov FU US Department of Energy [DE-AC52-07NA27344]; Lawrence Livermore National Laboratory FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 50 TC 3 Z9 3 U1 1 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 16 PY 2014 VL 89 IS 1 AR 012602 DI 10.1103/PhysRevE.89.012602 PG 6 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AC0DC UT WOS:000332164000004 PM 24580250 ER PT J AU Bud'ko, SL Chung, DY Bugaris, D Claus, H Kanatzidis, MG Canfield, PC AF Bud'ko, Sergey L. Chung, Duck Young Bugaris, Daniel Claus, Helmut Kanatzidis, Mercouri G. Canfield, Paul C. TI Heat capacity jump at T-c and pressure derivatives of superconducting transition temperature in the Ba1-xNaxFe2As2 (0.1 <= x <= 0.9) series SO PHYSICAL REVIEW B LA English DT Article ID IRON ARSENIDE SUPERCONDUCTORS; BAFE2AS2; CHEMISTRY AB We present the evolution of the initial (up to similar to 10 kbar) hydrostatic pressure dependencies of T-c and of the ambient pressure, and the jump in the heat capacity associated with the superconducting transition as a function of Na doping in the Ba1-xNaxFe2As2 family of iron-based superconductors. For Na concentrations 0.15 <= x <= 0.9, the jump in specific heat at T-c, Delta C-p|(Tc), follows the Delta C-p proportional to T-3 (the so-called BNC scaling) found for most BaFe2As2-based superconductors. This finding suggests that, unlike the related Ba1-xKxFe2As2 series, there is no significant modification of the superconducting state (e. g., change in superconducting gap symmetry) in the Ba1-xNaxFe2As2 series over the whole studied Na concentration range. Pressure dependencies are nonmonotonic for x = 0.2 and 0.24. For other Na concentrations, T-c decreases under pressure in an almost linear fashion. The anomalous behavior of the x = 0.2 and 0.24 samples under pressure is possibly due to the crossing of the phase boundaries of the narrow antiferromagnetic tetragonal phase, unique for the Ba1-xNaxFe2As2 series, with the application of pressure. The negative sign of the pressure derivatives of T-c across the whole superconducting dome (except for x = 0.2) is a clear indication of the nonequivalence of substitution and pressure for the Ba1-xNaxFe2As2 series. C1 [Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chung, Duck Young; Bugaris, Daniel; Claus, Helmut; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Bud'ko, SL (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RI Canfield, Paul/H-2698-2014 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX We would like to thank Xiao Lin for assistance in the handling of the samples, Adam Kaminski for discussion of published ARPES data, and S. Wurmehl and V. Grinenko for sharing their data from Ref. [48]. Work at the Ames Laboratory was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 54 TC 13 Z9 13 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 16 PY 2014 VL 89 IS 1 AR 014510 DI 10.1103/PhysRevB.89.014510 PG 7 WC Physics, Condensed Matter SC Physics GA AC0XU UT WOS:000332219600002 ER PT J AU Melikyan, A Norman, MR AF Melikyan, Ashot Norman, M. R. TI Symmetry of the charge density wave in cuprates SO PHYSICAL REVIEW B LA English DT Article ID FLUCTUATING STRIPES; BI2SR2CACU2O8+DELTA; SUPERCONDUCTORS; PSEUDOGAP; STATE AB We derive and analyze an effective Ginzburg-Landau (GL) functional for a charge density wave for a model of electrons on a tight-binding square lattice with density-density interactions. We show, using realistic electronic dispersions for the cuprates, that for the simplest GL theory, the preferred symmetry is typically unidirectional (stripe) type, but inclusion of third-order terms tends to destabilize this in favor of a checkerboard pattern depending on the strength and range of the interaction. This is of interest given the recent observation of such charge order in underdoped YBa2Cu3O6+x. C1 [Melikyan, Ashot; Norman, M. R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Melikyan, Ashot] Amer Phys Soc, Ridge, NY 11961 USA. RP Melikyan, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM norman@anl.gov RI Norman, Michael/C-3644-2013 FU Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, US DOE FX We would like to thank S. Davis, O. Vafek, and H. Yao for discussions and correspondence. This work was supported by the Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, US DOE. NR 27 TC 16 Z9 16 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 16 PY 2014 VL 89 IS 2 AR 024507 DI 10.1103/PhysRevB.89.024507 PG 7 WC Physics, Condensed Matter SC Physics GA AC0YA UT WOS:000332220200003 ER PT J AU James, CW Brinkman, KS Gray, JR Cortes-Concepcion, JA Anton, DL AF James, Charles W., Jr. Brinkman, Kyle S. Gray, Joshua R. Cortes-Concepcion, Jose A. Anton, Donald L. TI Fundamental environmental reactivity testing and analysis of the hydrogen storage material 2LiBH(4)center dot MgH2 SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen storage; Environmental reactivity; Lithium borohydride; Magnesium hydride; Calorimetry ID NAALH4; LIBH4; MECHANISM; KINETICS; AMIDE AB While the storage of hydrogen for portable and stationary applications is regarded as critical in bringing PEM fuel cells to commercial acceptance, little is known of the environmental exposure risks posed in utilizing condensed phase chemical storage options as in complex hydrides. It is thus important to understand the effect of environmental exposure of metal hydrides in the case of accident scenarios. Simulated tests were performed following the United Nations standards to test for flammability and water reactivity in air for a destabilized lithium borohydride and magnesium hydride system in a 2 to 1 molar ratio respectively. It was determined that the mixture acted similarly to the parent, lithium borohydride, but at slower rate of reaction seen in magnesium hydride. To quantify environmental exposure kinetics, isothermal calorimetry was utilized to measure the enthalpy of reaction as a function of exposure time to dry and humid air, and liquid water. The reaction with liquid water was found to increase the heat flow significantly during exposure compared to exposure in dry or humid air environments. Calorimetric results showed the maximum normalized heat flow of the fully charged material was 6 mW/mg under liquid phase hydrolysis; and 14 mW/mg for the fully discharged material also occurring under liquid phase hydrolysis conditions. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [James, Charles W., Jr.; Brinkman, Kyle S.; Gray, Joshua R.; Cortes-Concepcion, Jose A.; Anton, Donald L.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Anton, DL (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA. EM donald.anton@srnl.doe.gov FU U.S. Department of Energy Hydrogen Storage Program FX The authors would like to thank David Missimer and Joseph Wheeler for their XRD and laboratory support, respectively. This work was funded under the U.S. Department of Energy Hydrogen Storage Program managed by Dr. Ned Stetson with whom many helpful and insightful discussions were held. NR 18 TC 2 Z9 2 U1 2 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 16 PY 2014 VL 39 IS 3 BP 1371 EP 1381 DI 10.1016/j.ijhydene.2013.01.139 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA AA9OG UT WOS:000331422200019 ER PT J AU Bulgac, A Forbes, MM Kelley, MM Roche, KJ Wlazlowski, G AF Bulgac, Aurel Forbes, Michael McNeil Kelley, Michelle M. Roche, Kenneth J. Wlazlowski, Gabriel TI Quantized Superfluid Vortex Rings in the Unitary Fermi Gas SO PHYSICAL REVIEW LETTERS LA English DT Article ID REAL-TIME DYNAMICS; QUANTUM TURBULENCE; VORTICES; SOLITONS; ATOMS AB In a recent article, Yefsah et al. [Nature (London) 499, 426 (2013)] report the observation of an unusual excitation in an elongated harmonically trapped unitary Fermi gas. After phase imprinting a domain wall, they observe oscillations almost an order of magnitude slower than predicted by any theory of domain walls which they interpret as a "heavy soliton" of inertial mass some 200 times larger than the free fermion mass or 50 times larger than expected for a domain wall. We present compelling evidence that this "soliton" is instead a quantized vortex ring, by showing that the main aspects of the experiment can be naturally explained within the framework of time-dependent superfluid density functional theories. C1 [Bulgac, Aurel; Forbes, Michael McNeil; Roche, Kenneth J.; Wlazlowski, Gabriel] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Forbes, Michael McNeil] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Forbes, Michael McNeil] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Kelley, Michelle M.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Roche, Kenneth J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Wlazlowski, Gabriel] Warsaw Univ Technol, Fac Phys, PL-00662 Warsaw, Poland. RP Bulgac, A (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA. OI Forbes, Michael/0000-0002-8136-0336 FU U.S. Department of Energy (DoE) [DE-FG02-97ER41014, DE-FG02-00ER41132]; REU NSF fellowship; Polish Ministry of Science [N N202 128439, 628/MOB/2011/0]; Polish National Science Center (NCN) [DEC-2013/08/A/ST3/00708]; NSF MRI [PHY-0922770]; Office of Science of the DOE [DE-AC05-00OR22725] FX We acknowledge support under U.S. Department of Energy (DoE) Grants No. DE-FG02-97ER41014 and No. DE-FG02-00ER41132. M. M. K. acknowledges the support provided by an REU NSF fellowship. G. W. acknowledges the Polish Ministry of Science for the support under Contract No. N N202 128439, within the program "Mobility Plus-I edition" under Contract No. 628/MOB/2011/0, and the Polish National Science Center (NCN) decision No. DEC-2013/08/A/ST3/00708. Some of the calculations reported here have been performed at the University of Washington Hyak cluster funded by the NSF MRI Grant No. PHY-0922770. This research also used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the DOE under Contract No. DE-AC05-00OR22725. We thank R. Sharma and M. Zwierlein for discussions. NR 45 TC 23 Z9 23 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 16 PY 2014 VL 112 IS 2 AR 025301 DI 10.1103/PhysRevLett.112.025301 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7AO UT WOS:000331941900002 PM 24484022 ER PT J AU Converse, AD Riscassi, AL Scanlon, TM AF Converse, Amber D. Riscassi, Ami L. Scanlon, Todd M. TI Seasonal contribution of dewfall to mercury deposition determined using a micrometeorological technique and dew chemistry SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE mercury; dew; deposition; micrometeorology; gaseous ID GASEOUS MERCURY; ATMOSPHERIC MERCURY; SURFACE FLUXES; TRACE-ELEMENTS; VARIABILITY; ECOSYSTEM; EXCHANGE; SYSTEM; VAPOR AB Deposition of mercury (Hg) to dew is thought to influence the diurnal dynamics of Hg species in the near-surface air, yet this depositional pathway is not well characterized and is seldom accounted for in Hg budgets. This study quantifies Hg deposition to dew on a seasonal basis at a high-elevation meadow in Shenandoah National Park, Virginia, and compares these rates with those for wet deposition and other forms of dry deposition. Dew samples were collected on a surrogate surface and analyzed for Hg concentrations (ngL(-1)), and dew depths (mm) were calculated using a micrometeorological approach based on the surface energy budget over 1 week period during each of the four seasons. Concentrations of Hg in dew (mean: 5.57ngL(-1)) were lower than those observed in precipitation (mean weekly composite samples: 8.80ngL(-1)). When dew deposition was scaled to the seasonal and annual levels, Hg deposition in dew was estimated to be 2-3 orders of magnitude smaller than wet deposition (estimated annual Hg deposition to dew/frost: similar to 120ngm(-2); 2008 annual precipitation deposition: similar to 12400ngm(-2)). This disparity is attributed to the much lower dewfall amounts. Rates of Hg accumulation in dew were not related to gaseous elemental mercury (GEM) concentrations in the atmosphere nor were they related to measured GEM fluxes. They were, however, found to be similar to independently estimated rates of gaseous oxidized mercury (GOM) and particulate mercury (Hg-p) deposition during the nighttime, suggesting that dew scavenges GOM and Hg-P from the atmosphere at the study site. C1 [Converse, Amber D.; Scanlon, Todd M.] Univ Virginia, Dept Environm Sci, Charlottesville, VA 22904 USA. [Riscassi, Ami L.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Scanlon, TM (reprint author), Univ Virginia, Dept Environm Sci, 291 McCormick Rd, Charlottesville, VA 22904 USA. EM tms2v@virginia.edu FU U.S. Department of Education; National Science Foundation Hydrologic Science Program [EAR-0645697]; Dominion Foundation; University of Virginia FX Funding for this project was provided by the U.S. Department of Education's program for Graduate Assistance in Areas of National Need and the National Science Foundation Hydrologic Science Program (EAR-0645697). Aqueous mercury analysis instrumentation was funded by the Dominion Foundation and the University of Virginia. We would like to thank the Shenandoah National Park Service staff for their support and advice, specifically Julena Campbell, Liz Garcia, and Jim Schaberl. We also thank Michael Tate of the USGS for sharing modeled dry deposition estimates from Big Meadows. The thoughtful comments and suggestions from three anonymous reviewers led to significant improvements to this manuscript. NR 36 TC 0 Z9 0 U1 3 U2 15 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JAN 16 PY 2014 VL 119 IS 1 BP 284 EP 292 DI 10.1002/2013JD020491 PG 9 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AA2NF UT WOS:000330930600023 ER PT J AU Airapetian, A Akopov, N Aschenauer, EC Augustyniak, W Avakian, R Avetissian, A Avetisyan, E Blok, HP Bottcher, H Borissov, A Bowles, J Brodski, I Bryzgalov, V Burns, J Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Sanctis, E Diefenthaler, M Di Nezza, P Duren, M Ehrenfried, M Elbakian, G Ellinghaus, F Etzelmuller, E Fabbri, R Frullani, S Gapienko, G Gapienko, V Garcia, JG Garibaldi, F Gavrilov, G Gharibyan, V Giordano, F Gliske, S Hartig, M Hasch, D Holler, Y Hristova, I Ivanilov, A Jackson, HE Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Korotkov, V Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lapikas, L Lehmann, I Lenisa, P Lorenzon, W Lu, XG Ma, BQ Mahon, D Makins, NCR Manaenkov, SI Mao, Y Marianski, B Marukyan, H Miller, CA Miyachi, Y Movsisyan, A Muccifora, V Murray, M Mussgiller, A Naryshkin, Y Nass, A Negodaev, M Nowak, WD Pappalardo, LL Perez-Benito, R Petrosyan, A Reimer, PE Reolon, AR Riedl, C Rith, K Rosner, G Rostomyan Rubin, J Ryckbosch, D Salomatin, Y Schafer, A Schnell, G Seitz, B Shibata, TA Stahl, M Statera, M Steffens, E Steijger, JJM Stewart, J Stinzing, F Taroian, S Terkulov, A Truty, R Trzcinski, A Tytgat, M Van Haarlem, Y Van Hulse, C Vikhrov, V Vilardi, I Wang, S Yaschenko, S Ye, Z Yen, S Zagrebelnyy, V Zihlmann, B Zupranski, P AF Airapetian, A. Akopov, N. Aschenauer, E. C. Augustyniak, W. Avakian, R. Avetissian, A. Avetisyan, E. Blok, H. P. Boettcher, H. Borissov, A. Bowles, J. Brodski, I. Bryzgalov, V. Burns, J. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Sanctis, E. Diefenthaler, M. Di Nezza, P. Dueren, M. Ehrenfried, M. Elbakian, G. Ellinghaus, F. Etzelmueller, E. Fabbri, R. Frullani, S. Gapienko, G. Gapienko, V. Garcia, J. Garay Garibaldi, F. Gavrilov, G. Gharibyan, V. Giordano, F. Gliske, S. Hartig, M. Hasch, D. Holler, Y. Hristova, I. Ivanilov, A. Jackson, H. E. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Korotkov, V. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lapikas, L. Lehmann, I. Lenisa, P. Lorenzon, W. Lu, X. -G. Ma, B. -Q. Mahon, D. Makins, N. C. R. Manaenkov, S. I. Mao, Y. Marianski, B. Marukyan, H. Miller, C. A. Miyachi, Y. Movsisyan, A. Muccifora, V. Murray, M. Mussgiller, A. Naryshkin, Y. Nass, A. Negodaev, M. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Petrosyan, A. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rosner, G. Rostomyan Rubin, J. Ryckbosch, D. Salomatin, Y. Schaefer, A. Schnell, G. Seitz, B. Shibata, T. -A. Stahl, M. Statera, M. Steffens, E. Steijger, J. J. M. Stewart, J. Stinzing, F. Taroian, S. Terkulov, A. Truty, R. Trzcinski, A. Tytgat, M. Van Haarlem, Y. Van Hulse, C. Vikhrov, V. Vilardi, I. Wang, S. Yaschenko, S. Ye, Z. Yen, S. Zagrebelnyy, V. Zihlmann, B. Zupranski, P. CA HERMES Collaboration TI Beam-helicity asymmetry in associated electroproduction of real photons ep -> aEuro parts per thousand e gamma pi N in the Delta-resonance region SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Lepton-Nucleon Scattering; QCD; Polarization; Photon production ID VIRTUAL COMPTON-SCATTERING; CROSS-SECTIONS; SPIN; HERA; DEPENDENCE; LIMIT AB The beam-helicity asymmetry in associated electroproduction of real photons, ep -> aEuro parts per thousand e gamma pi N , in the Delta(1232)-resonance region is measured using the longitudinally polarized Hera positron beam and an unpolarized hydrogen target. Azimuthal Fourier amplitudes of this asymmetry are extracted separately for two channels, ep -> aEuro parts per thousand e gamma pi(0) p and ep -> aEuro parts per thousand e gamma pi(+) n, from a data set collected with a recoil detector. All asymmetry amplitudes are found to be consistent with zero. C1 [Jackson, H. E.; Reimer, P. E.; Rubin, J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Garcia, J. Garay; Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. [Garcia, J. Garay; Schnell, G.; Van Hulse, C.] Basque Fdn Sci, IKERBASQUE, Bilbao 48011, Spain. [Airapetian, A.; Ellinghaus, F.; Kinney, E.] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Avetisyan, E.; Borissov, A.; Deconinck, W.; Gavrilov, G.; Hartig, M.; Holler, Y.; Lu, X. -G.; Mussgiller, A.; Rostomyan; Yaschenko, S.; Ye, Z.; Zagrebelnyy, V.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Aschenauer, E. C.; Boettcher, H.; Fabbri, R.; Hristova, I.; Negodaev, M.; Nowak, W. -D.; Riedl, C.; Stewart, J.; Yaschenko, S.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.] Joint Inst Nucl Res, Dubna 141980, Russia. [Diefenthaler, M.; Kravchenko, P.; Mussgiller, A.; Nass, A.; Rith, K.; Steffens, E.; Stinzing, F.; Yaschenko, S.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Statera, M.] Univ Ferrara, Ist Nazl Fis Nucl, Sez Ferrara, I-44122 Ferrara, Italy. [Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Statera, M.] Univ Ferrara, Dipartimento Fis & Sci Terra, I-44122 Ferrara, Italy. [Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Hasch, D.; Muccifora, V.; Reolon, A. R.] Ist Nazl Fis Nucl, Nazl Frascati Lab, I-00044 Frascati, Italy. [Joosten, S.; Ryckbosch, D.; Schnell, G.; Tytgat, M.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Airapetian, A.; Brodski, I.; Dueren, M.; Ehrenfried, M.; Etzelmueller, E.; Keri, T.; Perez-Benito, R.; Stahl, M.; Zagrebelnyy, V.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Bowles, J.; Burns, J.; Kaiser, R.; Keri, T.; Lehmann, I.; Mahon, D.; Murray, M.; Rosner, G.; Seitz, B.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Diefenthaler, M.; Giordano, F.; Joosten, S.; Makins, N. C. R.; Riedl, C.; Rubin, J.; Truty, R.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Airapetian, A.; Gliske, S.; Lorenzon, W.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.; Terkulov, A.] Lebedev Phys Inst, Moscow 117924, Russia. [Blok, H. P.; Lapikas, L.; Steijger, J. J. M.] Natl Inst Subatom Phys Nikhef, NL-1009 DB Amsterdam, Netherlands. [Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Manaenkov, S. I.; Naryshkin, Y.; Vikhrov, V.] BP Konstantinov Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Bryzgalov, V.; Gapienko, G.; Gapienko, V.; Ivanilov, A.; Korotkov, V.; Salomatin, Y.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Nazl Fis Nucl, Sez Roma, Grp Collegato Sanita, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Super Sanita, I-00161 Rome, Italy. [Gavrilov, G.; Miller, C. A.; Yen, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Miyachi, Y.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Natl Ctr Nucl Res, PL-00689 Warsaw, Poland. [Akopov, N.; Avakian, R.; Avetissian, A.; Elbakian, G.; Gharibyan, V.; Karyan, G.; Marukyan, H.; Petrosyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Airapetian, A (reprint author), Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. EM management@hermes.desy.de RI Negodaev, Mikhail/A-7026-2014; Taroian, Sarkis/E-1668-2014; Kozlov, Valentin/M-8000-2015; Terkulov, Adel/M-8581-2015; Cisbani, Evaristo/C-9249-2011 OI Cisbani, Evaristo/0000-0002-6774-8473 FU Ministry of Economy and the Ministry of Education and Science of Armenia; FWO-Flanders; IWT, Belgium; Natural Sciences and Engineering Research Council of Canada; National Natural Science Foundation of China; Alexander von Humboldt Stiftung; German Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Italian Istituto Nazionale di Fisica Nucleare (INFN); MEXT; JSPS; G-COE of Japan; Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); Russian Academy of Science; Russian Federal Agency for Science and Innovations; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; U.K. Engineering and Physical Sciences Research Council; Science and Technology Facilities Council; Scottish Universities Physics Alliance; U.S. Department of Energy (DOE); National Science Foundation (NSF); European Community [283286] FX We gratefully acknowledge the Desy management for its support and the staff at Desy and the collaborating institutions for their significant effort. This work was supported by the Ministry of Economy and the Ministry of Education and Science of Armenia; the FWO-Flanders and IWT, Belgium; the Natural Sciences and Engineering Research Council of Canada; the National Natural Science Foundation of China; the Alexander von Humboldt Stiftung, the German Bundesministerium fur Bildung und Forschung (BMBF), and the Deutsche Forschungsgemeinschaft (DFG); the Italian Istituto Nazionale di Fisica Nucleare (INFN); the MEXT, JSPS, and G-COE of Japan; the Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); the Russian Academy of Science and the Russian Federal Agency for Science and Innovations; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the U.K. Engineering and Physical Sciences Research Council, the Science and Technology Facilities Council, and the Scottish Universities Physics Alliance; the U.S. Department of Energy (DOE) and the National Science Foundation (NSF); as well as the European Community Research Infrastructure Integrating Activity under the FP7 "Study of strongly interacting matter (HadronPhysics3, Grant Agreement number 283286)". NR 39 TC 0 Z9 0 U1 1 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 16 PY 2014 IS 1 DI 10.1007/JHEP01(2014)077 PG 17 WC Physics, Particles & Fields SC Physics GA 296FX UT WOS:000330171700001 ER PT J AU Lu, P Li, C Schneider, EW Harris, SJ AF Lu, Peng Li, Chen Schneider, Eric W. Harris, Stephen J. TI Chemistry, Impedance, and Morphology Evolution in Solid Electrolyte Interphase Films during Formation in Lithium Ion Batteries SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RECHARGEABLE LI BATTERIES; GRAPHITE-ELECTRODES; ENERGY-STORAGE; PERFORMANCE; IDENTIFICATION; SPECTROSCOPY; DEGRADATION; MECHANISMS; CHALLENGES; TRANSPORT AB The solid electrolyte interphase (SEI) forms during the initial cycles in lithium ion batteries and evolves throughout the battery life. By protecting the electrode and passing lithium ions, the SEI plays an important role in the performance and degradation of lithium ion batteries. Identifying how the SEI forms and evolves during battery cycling helps us understand and mitigate battery degradation. In this work, we address the SEI chemical and electrochemical evolution during its formation process and provide a correlation between these properties. It is found that the SEI chemistry, not just its thickness, has a distinct influence on its impedance, which may ultimately impact the battery performance. C1 [Lu, Peng; Schneider, Eric W.] Gen Motors R&D Ctr, Chem & Mat Syst Lab, Warren, MI 48090 USA. [Li, Chen] ZeeAero Inc, Mountain View, CA 94043 USA. [Harris, Stephen J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Lu, P (reprint author), Gen Motors R&D Ctr, Chem & Mat Syst Lab, Warren, MI 48090 USA. EM peng.lu@gm.com NR 35 TC 58 Z9 58 U1 12 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 16 PY 2014 VL 118 IS 2 BP 896 EP 903 DI 10.1021/jp4111019 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 299SX UT WOS:000330417100018 ER PT J AU Das, S Wu, QL Garlapalli, RK Nagpure, S Strzalka, J Jiang, Z Rankin, SE AF Das, Saikat Wu, Qingliu Garlapalli, Ravinder K. Nagpure, Suraj Strzalka, Joseph Jiang, Zhang Rankin, Stephen E. TI In-Situ GISAXS Investigation of Pore Orientation Effects on the Thermal Transformation Mechanism in Mesoporous Titania Thin Films SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY-SCATTERING; NANOCRYSTALLINE ANATASE; PHASE-SEPARATION; TIO2 FILMS; SILICA; CRYSTALLIZATION; PHOTOCATALYSIS; TEMPERATURE; SOL; ROUTE AB This study addresses the effects of mesopore orientation on mesostructural stability and crystallization of titania thin films during calcination based on measurements with in-situ grazing incidence small angle X-ray scattering (GISAXS). Complementary supporting information is provided by ex-situ electron microscopy. Pluronic surfactant P123 (with average structure (EO)(20)(PO)(70)(EO)(20) where EO is an ethylene oxide unit and PO is a propylene oxide unit) serves as the template to synthesize titania thin films on P123-modified glass slides with 2D hexagonally close-packed cylindrical mesopores. The orientation of the pores at the top surface is controlled by sandwiching another P123-modified glass slide on top of the titania thin film to completely orient the pores orthogonal to the films in some samples. This provides the opportunity to directly observe how pore orientation affects the evolution of pore order and crystallinity during calcination. The results show that when the pores are oriented parallel to the substrate at the top surface (for unsandwiched films), the pore structure is stable upon calcination at 400 degrees C but that the structure is quickly lost due to crystallization throughout the film during calcination at 500 degrees C. Films with pores oriented orthogonal to the substrate at the top surface (sandwiched films) retain their long-range pore order even after calcination at 500 degrees C. The reasons for this difference are ascribed to greater resistance to anisotropic stress during heating of the orthogonally oriented pores and titania crystallization nucleation at the top surface of the films with orthogonally oriented pores. C1 [Das, Saikat; Garlapalli, Ravinder K.; Nagpure, Suraj; Rankin, Stephen E.] Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. [Wu, Qingliu] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Strzalka, Joseph; Jiang, Zhang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Rankin, SE (reprint author), Univ Kentucky, Dept Chem & Mat Engn, 177 FP Anderson Tower, Lexington, KY 40506 USA. EM srankin@engr.uky.edu RI Jiang, Zhang/A-3297-2012; OI Jiang, Zhang/0000-0003-3503-8909; Rankin, Stephen/0000-0002-8615-7564 FU U.S. Department of Energy EPSCoR Implementation award [DE-FG02-07-ER46375]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Titania thin film synthesis and characterization work was performed as part of a U.S. Department of Energy EPSCoR Implementation award supported by grant no. DE-FG02-07-ER46375. Use of the Advanced Photon Source at Argonne National Laboratory for GISAXS measurements was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 56 TC 9 Z9 9 U1 0 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 16 PY 2014 VL 118 IS 2 BP 968 EP 976 DI 10.1021/jp406165v PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 299SX UT WOS:000330417100026 ER PT J AU Holmboe, M Bourg, IC AF Holmboe, Michael Bourg, Ian C. TI Molecular Dynamics Simulations of Water and Sodium Diffusion in Smectite Interlayer Nanopores as a Function of Pore Size and Temperature SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELASTIC NEUTRON-SCATTERING; X-RAY-DIFFRACTION; SWELLING CLAY-MINERALS; MONTE-CARLO-SIMULATION; COMPACTED MONTMORILLONITE; SELF-DIFFUSION; NA-MONTMORILLONITE; ACTIVATION-ENERGY; TRACER DIFFUSION; MICROSCOPIC SIMULATION AB The diffusion coefficients (D) of water and solutes in nanoporous Na-smectite clay barriers have been widely studied because of their importance in high-level radioactive waste (HLRW) management and in the isolation of contaminated sites. However, few measurements have been carried out at the high temperatures that are expected to occur in HLRW repositories. We address this knowledge gap by using molecular dynamics (MD) simulations to predict the temperature dependence of diffusion in clay interlayer nanopores, expressed as a pore scale activation energy of diffusion (E-a). Our sensitivity analysis shows that accurate prediction of pore scale D and E-a values requires careful consideration of the influence of pore size, simulation cell size, and clay structure flexibility on MD simulation results. We find that predicted D values in clay interlayer nanopores are insensitive to the size of the simulation cell (contrary to the behavior observed in simulation of bulk liquid water) but sensitive to the vibrational motions of clay atoms (particularly in the smallest pores investigated here, the one-, two-, and three-layer hydrates). Our predicted D and E-a values are consistent with experimental data. They reveal, for both water and Na+, that E-a increases by similar to 6 kJ mol(-1) with increasing confinement, when going from bulk liquid water to the one-layer hydrate of Na-montmorillonite. C1 [Holmboe, Michael] Royal Inst Technol, Sch Engn Sci, Dept Theoret Phys, S-10691 Stockholm, Sweden. [Holmboe, Michael; Bourg, Ian C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Geochem, Berkeley, CA 94720 USA. RP Holmboe, M (reprint author), Royal Inst Technol, Sch Engn Sci, Dept Theoret Phys, S-10691 Stockholm, Sweden. EM holmboe@kth.se RI Bourg, Ian/A-6405-2013; OI Bourg, Ian/0000-0002-5265-7229 FU U.S. Department of Energy [DE-AC02-05CH11231]; Geosciences program (Office of Science, Office of Basic Energy Sciences); Carl Tryggers Foundation; Galo foundation; foundation BLANCEFLOR FX The research reported in this paper was supported by U.S. Department of Energy under Contract DE-AC02-05CH11231 under the auspices of the Used Fuel Disposition program (Office of Nuclear Energy) and the Geosciences program (Office of Science, Office of Basic Energy Sciences). It used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. Financial support to M.H. by the Carl Tryggers Foundation, the Galo foundation and the foundation BLANCEFLOR is gratefully acknowledged. Two anonymous reviewers and Dr. Virginie Marry provided helpful comments on the manuscript. NR 116 TC 27 Z9 27 U1 7 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 16 PY 2014 VL 118 IS 2 BP 1001 EP 1013 DI 10.1021/jp408884g PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 299SX UT WOS:000330417100030 ER PT J AU Wood, BC Schwegler, E Choi, WI Ogitsu, T AF Wood, Brandon C. Schwegler, Eric Choi, Woon Ih Ogitsu, Tadashi TI Surface Chemistry of GaP(001) and InP(001) in Contact with Water SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DENSITY-FUNCTIONAL THEORY; HYDROGEN-BOND; MOLECULAR-DYNAMICS; 1ST PRINCIPLES; SOLAR-CELLS; INTERFACE; PROTON; DECOMPOSITION; SPECTROSCOPY; SIMULATIONS AB We report the results of total-energy density functional theory and ab initio molecular dynamics simulations of (001) surfaces of InP and GaP in contact with gas-phase and liquid water. Both pristine and oxygen-rich surfaces (representing a submonolayer native surface oxide) are considered. We find that gas-phase binding of water on pristine mixed-dimer delta(2x4) reconstructions of InP/GaP(001) is comparable to the solvation energy of liquid water, and that the barriers for room-temperature dissociation are high. In the presence of a submonolayer surface oxide, water binding and dissociation instead become strongly exothermic and proceed with almost no barrier. In this case, the surface chemistry at the interface with liquid water differs significantly from that of gas-phase water adsorption due to the formation of strong, low-barrier hydrogen bonds between surface adsorbates and water molecules. Water dissociation on the oxygen-rich surface is accompanied by extremely rapid local proton hopping between hydrogen-bonded surface adsorbates. C1 [Wood, Brandon C.; Schwegler, Eric; Choi, Woon Ih; Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. RP Wood, BC (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. EM brandonwood@llnl.gov RI Schwegler, Eric/A-2436-2016; OI Schwegler, Eric/0000-0003-3635-7418; Choi, Woon Ih/0000-0002-7183-3400 FU U.S. Department of Energy; Laboratory Directed Research and Development (LDRD) Program at Lawrence Livermore National Laboratory (LLNL); U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX The authors acknowledge helpful discussions with J. Turner, T. Deutsch, and H. Wang (NREL). Funding was provided by the U.S. Department of Energy Fuel Cell Technologies Program and the Laboratory Directed Research and Development (LDRD) Program at Lawrence Livermore National Laboratory (LLNL). Computing support came from the LLNL Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 60 TC 13 Z9 13 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 16 PY 2014 VL 118 IS 2 BP 1062 EP 1070 DI 10.1021/jp4098843 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 299SX UT WOS:000330417100037 ER PT J AU Cheng, TL Wen, YH Hawk, JA AF Cheng, Tian-Le Wen, You-Hai Hawk, Jeffrey A. TI Diffuse-Interface Modeling and Multiscale-Relay Simulation of Metal Oxidation Kinetics-With Revisit on Wagner's Theory SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID THERMAL-OXIDATION; FIELD; GROWTH; CHARGE; TRANSPORT; TEMPERATURE; SILICON; SOLIDIFICATION; TRANSITION; CHROMIUM AB Oxidation of metals generally involves coupling between chemical reactions, mass transport, and electrostatic interaction, and oxidation kinetics is usually a multiscale problem. Existing theories mostly work for either a very thin oxide film or a thick one, leaving a length scale gap for oxidation kinetics. An electrochemistry based diffuse-interface model plus a multiscale-relay scheme are developed to study oxidation kinetics in a gas-oxide-metal environment. The multiscale-relay scheme allows the model to coherently cover a wide range of lengths and times and study the transition stage oxidation kinetics. The coupling between interfacial reactions and ionic transport with the moving boundary problem is solved, without using assumptions such as steady state, coupled currents, local charge neutrality, or local chemical equilibrium. For the model oxidation system, in the thick film limit perfect parabolic growth law is obtained with the rate constant in agreement with Wagner's theory. Nevertheless, the Wagner-parabolic law is violated either when the oxide film thickness is on the order of the Debye length Or when the interfacial reaction is rate-limiting. In addition, computer simulations reveal two space charge related effects in different situations and their linkage to experimental observations is discussed. C1 [Cheng, Tian-Le; Wen, You-Hai; Hawk, Jeffrey A.] Natl Energy Technol Lab, Albany, OR 97321 USA. RP Cheng, TL (reprint author), Natl Energy Technol Lab, 1450 Queen Ave SW, Albany, OR 97321 USA. EM tianle.cheng@contr.netl.doe.gov; youhai.wen@netl.doe.gov FU Postgraduate Research Program; National Science Foundation [OCI-1053575]; United States Government FX We acknowledge the Strategic Center for Coal, NETL, for supporting this ORD activity through the Innovative Process Technologies Program, and in particular Robert Romanosky as Technology Manager, Patricia Rawls as Project Manager, and David Alman as ORD Technical Coordinator. We also thank Michael C. Gao and De Nyago Tafen for helpful discussions. T.-L.C. acknowledges support from the Postgraduate Research Program operated by Oak Ridge Institute for Science and Education (ORISE). This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation Grant No. OCI-1053575. Disclaimer: This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 53 TC 6 Z9 6 U1 5 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 16 PY 2014 VL 118 IS 2 BP 1269 EP 1284 DI 10.1021/jp409811e PG 16 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 299SX UT WOS:000330417100061 ER PT J AU Velaga, SC Anderson, BJ AF Velaga, Srinath C. Anderson, Brian J. TI Carbon Dioxide Hydrate Phase Equilibrium and Cage Occupancy Calculations Using Ab Initio Intermolecular Potentials SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID CARLO MOLECULAR SIMULATIONS; VAN-DER-WAALS; MONTE-CARLO; CO2 HYDRATE; NEUTRON-DIFFRACTION; LANGMUIR CONSTANTS; WATER INTERACTIONS; CLATHRATE HYDRATE; HYDROGEN-SULFIDE; DYNAMICS METHOD AB Gas hydrate deposits are receiving increased attention as potential locations for CO2 sequestration, with CO2 replacing the methane that is recovered as an energy source. In this scenario, it is very important to correctly characterize the cage occupancies of CO2 to correctly assess the sequestration potential as well as the methane recoverability. In order to predict accurate cage occupancies, the guest-host interaction potential must be represented properly. Earlier, these potential parameters were obtained by fitting to experimental equilibrium data and these fitted parameters do not match with those obtained by second virial coefficient or gas viscosity data. Ab initio quantum mechanical calculations provide an independent means to directly obtain accurate intermolecular potentials. A potential energy surface (PES) between H2O and CO2 was computed at the MP2/aug-cc-pVTZ level and corrected for basis set superposition error (BSSE), an error caused due to the lower basis set, by using the half counterpoise method. Intermolecular potentials were obtained by fitting Exponential-6 and Lennard-Jones 6-12 models to the ab initio PES, correcting for many-body interactions. We denoted this model as the "VAS" model. Reference parameters for structure I carbon dioxide hydrate were calculated using the VAS model (site site ab initio intermolecular potentials) as Delta mu(0)(w) = 1206 +/- 2 J/mol and Delta H-w(0) = 1260 +/- 12 J/mol. With these reference parameters and the VAS model, pure CO2 hydrate equilibrium pressure was predicted with an average absolute deviation of less than 3.2% from the experimental data. Predictions of the small cage occupancy ranged from 32 to 51%, and the large cage is more than 98% occupied. The intermolecular potentials were also tested by calculating the pure CO2 density and diffusion of CO2 in water using molecular dynamics simulations. C1 [Velaga, Srinath C.; Anderson, Brian J.] Natl Energy Technol Lab, Morgantown, WV 26506 USA. [Velaga, Srinath C.; Anderson, Brian J.] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. RP Anderson, BJ (reprint author), Natl Energy Technol Lab, Morgantown, WV 26506 USA. EM Brian.Anderson@mail.wvu.edu NR 66 TC 6 Z9 6 U1 2 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 16 PY 2014 VL 118 IS 2 BP 577 EP 589 DI 10.1021/jp410306v PG 13 WC Chemistry, Physical SC Chemistry GA 294BR UT WOS:000330017900020 PM 24328234 ER PT J AU Atalla, RS Crowley, MF Himmel, ME Atalla, RH AF Atalla, R. S. Crowley, M. F. Himmel, M. E. Atalla, R. H. TI Irreversible transformations of native celluloses, upon exposure to elevated temperatures SO CARBOHYDRATE POLYMERS LA English DT Article DE Transformation; Irreversible; Celluloses; Elevated; Temperatures; Native; Accessibility; Aggregation ID NEUTRON FIBER DIFFRACTION; HYDROGEN-BONDING SYSTEM; SYNCHROTRON X-RAY; CRYSTAL-STRUCTURE; COMPLEX; IODINE AB Current research, basic and applied, assumes that observed recalcitrance of celluloses is an inherent characteristic associated with their state of aggregation in their native state; it is thought that processes of isolation remove other components of plant cell walls leaving the celluloses unchanged, even though elevated temperatures are routinely used during isolation. Since temperature elevation is known to influence the structures of all polymers, it is important to explore its influence on the character of isolated celluloses, almost always assumed to be still in their native state. Deuterium exchange is a measure of accessibility of reactive sites in celluloses. We report significant reduction in accessibility to deuterium and other probe molecules for celluloses isolated at ambient temperature and then exposed to elevated temperatures. Our results indicate that native celluloses, which are highly ordered biological structures, are irreversibly transformed and develop polymeric semi-crystalline character upon isolation at elevated temperatures. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Atalla, R. S.; Atalla, R. H.] Cellulose Sci Int, Madison, WI USA. [Crowley, M. F.; Himmel, M. E.] Natl Renewable Energy Lab, Golden, CO USA. [Atalla, R. H.] Univ Wisconsin, Madison, WI 53706 USA. RP Atalla, RH (reprint author), Univ Wisconsin, Madison, WI 53706 USA. EM rhatalla@wisc.edu FU BioEnergy Science Center (BESC); DOE Office of Biological and Environmental Research (BER) under the Genomes to Life (GTL) program; DOE Office of Science ASCR SciDAC program award [DE-AC36-080028303]; Wisconsin Energy Independence Fund FX This work was supported partially by the BioEnergy Science Center (BESC) funded by the DOE Office of Biological and Environmental Research (BER) under the Genomes to Life (GTL) program; the DOE Office of Science ASCR SciDAC program award (DE-AC36-080028303); and the Wisconsin Energy Independence Fund for a grant for purchase of the Xplora Raman Microspectrometer. NR 29 TC 10 Z9 10 U1 3 U2 39 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0144-8617 EI 1879-1344 J9 CARBOHYD POLYM JI Carbohydr. Polym. PD JAN 16 PY 2014 VL 100 SI SI BP 2 EP 8 DI 10.1016/j.carbpol.2013.06.007 PG 7 WC Chemistry, Applied; Chemistry, Organic; Polymer Science SC Chemistry; Polymer Science GA 295BQ UT WOS:000330092000002 PM 24188831 ER PT J AU Santhanagopalan, D Qian, D McGilvray, T Wang, ZY Wang, F Camino, F Graetz, J Dudney, N Meng, YS AF Santhanagopalan, Dhamodaran Qian, Danna McGilvray, Thomas Wang, Ziying Wang, Feng Camino, Fernando Graetz, Jason Dudney, Nancy Meng, Ying Shirley TI Interface Limited Lithium Transport in Solid-State Batteries SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; THIN-FILM; ELECTROCHEMICAL LITHIATION; ION BATTERIES; AMORPHOUS-SILICON; SNO2 NANOWIRE; BEHAVIOR; ANODES AB Understanding the role of interfaces is important for improving the performance of all-solid-state lithium ion batteries. To study these interfaces, we present a novel approach for fabrication of electrochemically active nanobatteries using focused ion beams and their characterization by analytical electron microscopy. Morphological changes by scanning transmission electron microscopy imaging and correlated elemental concentration changes by electron energy loss spectroscopy mapping are presented. We provide first evidence of lithium accumulation at the anode/current collector (Si/Cu) and cathode/electrolyte (LixCoO2/LiPON) interfaces, which can be accounted for the irreversible capacity losses. Interdiffusion of elements at the Si/LiPON interface was also witnessed with a distinct contrast layer. These results highlight that the interfaces may limit the lithium transport significantly in solid-state batteries. Fabrication of electrochemically active nanobatteries also enables in situ electron microscopy observation of electrochemical phenomena in a variety of solid-state battery chemistries. C1 [Santhanagopalan, Dhamodaran; Qian, Danna; McGilvray, Thomas; Wang, Ziying; Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Wang, Feng; Camino, Fernando; Graetz, Jason] Brookhaven Natl Lab, Upton, NY 11973 USA. [Dudney, Nancy] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. RP Meng, YS (reprint author), Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM shirleymeng@ucsd.edu RI Qian, Danna/H-6580-2015; Wang, Feng/C-1443-2016 OI Wang, Feng/0000-0003-4068-9212 FU Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001294, DE-SC0002357, DE-AC02-98CH10886] FX This research is conducted through the partial support of the Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award Number DE-SC0001294. D.S. and Y.S.M. acknowledge the funding support for the development of the all-solid-state battery and the in situ FIB and TEM biasing design by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award Number DE-SC0002357. TEM studies and part of the FIB work were carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. N.J.D. acknowledges U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division for fabrication of the Microbatteries. We would also like to acknowledge the support of Dr. Michael DiBattista, QCT Failure Analysis Lab, Qualcomm, Inc., for providing us with access to several focused ion beam tools for this work. NR 24 TC 33 Z9 33 U1 22 U2 253 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JAN 16 PY 2014 VL 5 IS 2 BP 298 EP 303 DI 10.1021/jz402467x PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 294BQ UT WOS:000330017800007 PM 26270703 ER PT J AU Stolle, CJ Harvey, TB Pernik, DR Hibbert, JI Du, J Rhee, DJ Akhavan, VA Schaller, RD Korgel, BA AF Stolle, C. Jackson Harvey, Taylor B. Pernik, Douglas R. Hibbert, Jarett I. Du, Jiang Rhee, Dong Joon Akhavan, Vahid A. Schaller, Richard D. Korgel, Brian A. TI Multiexciton Solar Cells of CuInSe2 Nanocrystals SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MULTIPLE EXCITON GENERATION; CARRIER MULTIPLICATION YIELDS; APPARENT QUANTUM EFFICIENCY; SEMICONDUCTOR NANOCRYSTALS; PHOTOVOLTAIC DEVICES; SILICON NANOCRYSTALS; FILMS; DOTS; PHOTODETECTORS; 100-PERCENT AB Peak external quantum efficiencies (EQEs) of just over 120% were observed in photovoltaic (PV) devices of CuInSe2 nanocrystals prepared with a photonic curing process. The extraction of more than one electron/hole pair as a result of the absorption of a single photon can occur if multiple excitons are generated and extracted. Multiexciton generation (MEG) in the nanocrystal films was substantiated by transient absorption spectroscopy. We propose that photonic curing leads to sufficient electronic coupling between nanocrystals to enable multiexciton extraction under typical solar illumination conditions. Under low light conditions, however, the EQE drops significantly, indicating that photonic curing-induced ligand desorption creates a significant amount of traps in the film that limit the overall power conversion efficiency of the device. C1 [Stolle, C. Jackson; Harvey, Taylor B.; Pernik, Douglas R.; Hibbert, Jarett I.; Du, Jiang; Rhee, Dong Joon; Korgel, Brian A.] Univ Texas Austin, McKetta Dept Chem Engn, Texas Mat Inst, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA. [Akhavan, Vahid A.] NovaCentrix, Austin, TX 78728 USA. [Schaller, Richard D.] Argonne Natl Labs, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Korgel, BA (reprint author), Univ Texas Austin, McKetta Dept Chem Engn, Texas Mat Inst, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA. EM korgel@che.utexas.edu FU Robert A. Welch Foundation [F-1464]; National Science Foundation Industry/University Cooperative Research Center on Next Generation Photovoltaics [IIP-1134849]; National Science Foundation Graduate Research Fellowship program [DGE-1110007]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Financial support of this work was provided by the Robert A. Welch Foundation (F-1464) and the National Science Foundation Industry/University Cooperative Research Center on Next Generation Photovoltaics (IIP-1134849). Financial support was also provided for C.J.S. and D.RP. by the National Science Foundation Graduate Research Fellowship program under Grant No. DGE-1110007. Use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors also thank Sayan Saha and Sanjay Banerjee for use of their QEXIO Solar Cell Spectral Response Measurement System. NR 40 TC 37 Z9 37 U1 5 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JAN 16 PY 2014 VL 5 IS 2 BP 304 EP 309 DI 10.1021/jz402596v PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 294BQ UT WOS:000330017800008 PM 26270704 ER PT J AU Wang, B Xin, HL Li, XD Cheng, JL Yang, GC Nie, FD AF Wang, Bin Xin, Huolin Li, Xiaodong Cheng, Jianli Yang, Guangcheng Nie, Fude TI Mesoporous CNT@TiO2-C Nanocable with Extremely Durable High Rate Capability for Lithium-Ion Battery Anodes SO SCIENTIFIC REPORTS LA English DT Article ID CARBON NANOTUBES; TIO2 ANATASE; TITANIUM-DIOXIDE; HYBRID MATERIALS; ENERGY-STORAGE; SANDWICH-LIKE; PERFORMANCE; NANOSTRUCTURES; NANOPARTICLES; SPHERES AB A well-designed nanostructure CNT@TiO2-C with fine anatase TiO2 particle (<8 nm), good electronic conducting network (inner CNT core and outer carbon layer), and mesoporous structure was prepared by a simple and green one-pot hydrothermal reaction. The utilization of glucose in the hydrothermal process not only solves the interfacial incompatibility between CNTs and titanate sol and controls the nucleation and growth of TiO2 particles, but also introduces a uniform, glucose-derived, carbon-layer on the TiO2 particles. The nanosized TiO2 particle, high conducting network, and interconnected nanopores of the CNT@TiO2-C nanocable greatly improve its electrochemical performances, especially rate capability. The CNT@TiO2-C nanocables show remarkable rate capability with reversible charge capacity of 297, 240, 210,178 and 127 mAh g(-1) at 1C, 5C, 10C, 20C and 50C, respectively, as well as excellent high rate cycling stability with capacity retention of 87% after 2000 cycles at 50C. C1 [Wang, Bin; Li, Xiaodong; Cheng, Jianli; Yang, Guangcheng; Nie, Fude] China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Sichuan, Peoples R China. [Wang, Bin; Li, Xiaodong; Cheng, Jianli] Sichuan Res Ctr New Mat, Chengdu 610207, Sichuan, Peoples R China. [Xin, Huolin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wang, B (reprint author), China Acad Engn Phys, Inst Chem Mat, POB 919-328, Mianyang 621900, Sichuan, Peoples R China. EM edward.bwang@gmail.com; jenny.jlcheng@gmail.com RI cheng, Jianli/K-1496-2014; Xin, Huolin/E-2747-2010; Wang, Bin/F-9677-2012 OI Xin, Huolin/0000-0002-6521-868X; Wang, Bin/0000-0001-7104-4543 FU Startup Foundation of China Academy of Engineering Physics, Institute of Chemical Materials [KJCX201301, KJCX201306]; National High-tech Research and Development Program (863 Program) [2013AA050905]; National Center for Electron Microscopy, Lawrence Berkeley Lab; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Startup Foundation of China Academy of Engineering Physics, Institute of Chemical Materials (KJCX201301 and KJCX201306) and National High-tech Research and Development Program (863 Program: No. 2013AA050905). The authors acknowledge support of the National Center for Electron Microscopy, Lawrence Berkeley Lab, which is supported by the U.S. Department of Energy under Contract # DE-AC02-05CH11231. NR 43 TC 44 Z9 44 U1 8 U2 165 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 16 PY 2014 VL 4 AR 3729 DI 10.1038/srep03729 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RY UT WOS:000329848100019 PM 24429419 ER PT J AU Makarov, NS McDaniel, H Fuke, N Robel, I Klimov, VI AF Makarov, Nikolay S. McDaniel, Hunter Fuke, Nobuhiro Robel, Istvan Klimov, Victor I. TI Photocharging Artifacts in Measurements of Electron Transfer in Quantum-Dot-Sensitized Mesoporous Titania Films SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID LIGHT-EMITTING-DIODES; HOT-CARRIER TRANSFER; SEMICONDUCTOR NANOCRYSTALS; SOLAR-CELLS; METAL-OXIDE; PERFORMANCE; INJECTION; DYNAMICS; RATES; TIO2 AB Transient absorption and time-resolved photoluminescence measurements of high-performance mesoporous TiO2 photoanodes sensitized with CuInSexS2-x quantum dots reveal the importance of hole scavenging in the characterization of photoinduced electron transfer. The apparent characteristic time of this process strongly depends on the local environment of the quantum dot/TiO2 junction due to accumulation of long-lived positive charges in the quantum dots. The presence of long-lived photoexcited holes introduces artifacts due to fast positive-trion Auger decay (60 ps time constant), which can dominate electron dynamics and thus mask true electron transfer. We show that the presence of a redox electrolyte is critical to the accurate characterization of charge transfer, since it enables fast extraction of holes and helps maintain charge neutrality of the quantum dots. Although electron transfer is observed to be relatively slow (19 ns time constant), a high electron extraction efficiency (>95%) can be achieved because in well-passivated CuInSexS2-x quantum dots neutral excitons have significantly longer lifetimes of hundreds of nanoseconds. C1 [Makarov, Nikolay S.; McDaniel, Hunter; Robel, Istvan; Klimov, Victor I.] Los Alamos Natl Lab, Div Chem, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. [Fuke, Nobuhiro] Sharp Co Ltd, Corp Res & Dev Grp, Mat & Energy Technol Labs, Nara 6392198, Japan. RP Klimov, VI (reprint author), Los Alamos Natl Lab, Div Chem, Ctr Adv Solar Photophys, POB 1663, Los Alamos, NM 87545 USA. EM klimov@lanl.gov RI Robel, Istvan/D-4124-2011; OI Robel, Istvan/0000-0002-9738-7728; Klimov, Victor/0000-0003-1158-3179 FU Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center (EFRC); U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES); LANL FX Authors acknowledge the support of the Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES). N.S.M. is a CASP member supported by a LANL Director's Fellowship. NR 37 TC 12 Z9 13 U1 4 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JAN 16 PY 2014 VL 5 IS 1 BP 111 EP 118 DI 10.1021/jz402338b PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 284PD UT WOS:000329331400019 PM 26276189 ER PT J AU Rao, MJ Shibata, T Chattopadhyay, S Nag, A AF Rao, M. Jagadeeswara Shibata, Tomohiro Chattopadhyay, Soma Nag, Angshuman TI Origin of Photoluminescence and XAFS Study of (ZnS)(1-x)(AgInS2)(x) Nanocrystals SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SOLID-SOLUTION NANOPARTICLES; QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; AGINS2 NANOCRYSTALS; FACILE SYNTHESIS; CHALCOGENIDES; SPECTROSCOPY; TRANSPORT; CDSE; ZNSE AB Donor-Acceptor transition was previously suggested as a mechanism for luminescence in (ZnS)(1-x)(AgInS2)(x) nanocrystals. Here we show the participation of delocalized valence/conduction band in the luminescence. Two emission pathways are observed: Path-1 involves transition between a delocalized state and a localized state exhibiting higher energy and shorter lifetime (similar to 25 ns) and Path-2 (donor-acceptor) involves two localized defect states exhibiting lower emission energy and longer lifetime (>185 ns). Surprisingly, Path-1 dominates (82% for x = 0.33) for nanocrystals with lower x, in sharp difference with prior assignment. Luminescence peak blue shifts systematically by 0.57 eV with decreasing x because of this large contribution from Path-1. X-ray absorption fine structure (XAFS) study of (ZnS)(1-x)(AgInS2)(x) nanocrystals shows larger AgS4 tetrahedra compared with InS4 tetrahedra with Ag-S and In-S bond lengths 2.52 and 2.45 angstrom respectively, whereas Zn-S bond length is 2.33 angstrom along with the absence of second nearest-neighbor Zn-S-metal correlation. C1 [Rao, M. Jagadeeswara; Nag, Angshuman] Indian Inst Sci Educ & Res, Dept Chem, Pune 411008, Maharashtra, India. [Shibata, Tomohiro; Chattopadhyay, Soma] Argonne Natl Lab, MRCAT, Sect 10, Argonne, IL 60439 USA. [Shibata, Tomohiro; Chattopadhyay, Soma] IIT, CSRRI, Chicago, IL 60616 USA. [Shibata, Tomohiro; Chattopadhyay, Soma] IIT, Dept Phys, Adv Mat Grp, Chicago, IL 60616 USA. RP Nag, A (reprint author), Indian Inst Sci Educ & Res, Dept Chem, Dr Homi Bhabha Rd, Pune 411008, Maharashtra, India. EM angshuman@iiserpune.ac.in RI ID, MRCAT/G-7586-2011 FU IISER Pune; Department of Science and Technology (DST); DAE-BRNS grant Govt. of India [2013/20/37C/1/BRNS/954]; Nanoscience Unit Grant of DST, Govt. of India [SR/NM/NS-42/2009]; CSIR, Govt. of India; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank the Director of IISER Pune for financial support and encouragement. A.N. acknowledges Department of Science and Technology (DST) for Ramanujan Fellowship and DAE-BRNS grant (2013/20/37C/1/BRNS/954) Govt. of India. We thank Nanoscience Unit Grant (SR/NM/NS-42/2009) of DST, Govt. of India. M.J.R. acknowledges CSIR, Govt. of India, for a junior research fellowship. MRCAT operations are supported by the Department of Energy and MRCAT host institutions. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 41 TC 20 Z9 20 U1 5 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JAN 16 PY 2014 VL 5 IS 1 BP 167 EP 173 DI 10.1021/jz402443y PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 284PD UT WOS:000329331400027 PM 26276197 ER PT J AU Gu, XD Gunkel, I Hexemer, A Gu, WY Russell, TP AF Gu, Xiaodan Gunkel, Ilja Hexemer, Alexander Gu, Weiyin Russell, Thomas P. TI An In Situ Grazing Incidence X-Ray Scatterings Study of Block Copolymer Thin Films During Solvent Vapor Annealing SO ADVANCED MATERIALS LA English DT Article ID ORDER-DISORDER TRANSITION; MOLECULAR-WEIGHT; NANOPOROUS MEMBRANES; IMMISCIBLE POLYMERS; DIBLOCK COPOLYMERS; SELECTIVE SOLVENTS; PHASE-BEHAVIOR; ARRAYS; NANOSTRUCTURES; LITHOGRAPHY AB In situ grazing-incidence small-angle X-ray scattering experiments on thin films of block copolymers during annealing in neutral solvent vapors are reported. By removing the solvent in a controlled manner, the period of the microphase separated morphology is found to increase with increasing block copolymer concentration in a power law manner with an exponent similar to 2/3. By venting the systems at different rates during the solvent removal process, kinetically arresting the system, the period of the microphase separated morphology in the dried film can be varied. C1 [Gu, Xiaodan; Gunkel, Ilja; Gu, Weiyin; Russell, Thomas P.] Univ Massachusetts, Polymer Sci & Engn Dept, Amherst, MA 01003 USA. [Gunkel, Ilja; Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Russell, TP (reprint author), Univ Massachusetts, Polymer Sci & Engn Dept, 120 Governors Dr, Amherst, MA 01003 USA. EM russell@mail.pse.umass.edu RI Gu, Xiaodan/E-9379-2015; Gu, Xiaodan/G-4029-2015; Foundry, Molecular/G-9968-2014 FU U.S. Department of Energy BES [BES-DE-FG02-96ER45612]; ALS Doctoral Fellowship program; ALS Postdoctoral Fellowship program; DOE; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05ch11231] FX This work was supported by the U.S. Department of Energy BES under contract BES-DE-FG02-96ER45612, X.G. acknowledges the ALS Doctoral Fellowship program for providing partial financial support. I. G. acknowledges the support by the ALS Postdoctoral Fellowship program. A. H. was supported by a DOE Early Career Research Program grant. We would like to thank Prof. T. Xu for the use of the SFM and laboratory facilities. We also would like to acknowledge E. Schaible and E. Lim for assistance during GISAXS measurments. Part of this work was performed as a user project at the Molecular Foundry, Lawrence Berkeley National Laboratory. GISAXS measurements were performed at the Beamline 7.3.3 at the Advanced Light Source, Lawrence Berkeley National Laboratory, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract No. DE-AC02-05ch11231. NR 57 TC 60 Z9 60 U1 10 U2 132 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JAN 15 PY 2014 VL 26 IS 2 BP 273 EP 281 DI 10.1002/adma.201302562 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH3QZ UT WOS:000336041400006 PM 24282077 ER PT J AU Schmidt, K Tassone, CJ Niskala, JR Yiu, AT Lee, OP Weiss, TM Wang, C Frechet, JMJ Beaujuge, PM Toney, MF AF Schmidt, Kristin Tassone, Christopher J. Niskala, Jeremy R. Yiu, Alan T. Lee, Olivia P. Weiss, Thomas M. Wang, Cheng Frechet, Jean M. J. Beaujuge, Pierre M. Toney, Michael F. TI A Mechanistic Understanding of Processing Additive-Induced Efficiency Enhancement in Bulk Heterojunction Organic Solar Cells SO ADVANCED MATERIALS LA English DT Article ID SMALL-ANGLE SCATTERING; SOLVENT ADDITIVES; ALKANE DITHIOLS; THIN-FILMS; POLYMER; MORPHOLOGY; PERFORMANCE; CRYSTALLIZATION; PHOTOVOLTAICS; NETWORK AB The addition of processing additives is a widely used approach to increase power conversion efficiencies for many organic solar cells. We present how additives change the polymer conformation in the casting solution leading to a more intermixed phase-segregated network structure of the active layer which in turn results in a 5-fold enhancement in efficiency. C1 [Schmidt, Kristin; Tassone, Christopher J.; Weiss, Thomas M.; Toney, Michael F.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Niskala, Jeremy R.; Yiu, Alan T.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Niskala, Jeremy R.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Niskala, Jeremy R.; Yiu, Alan T.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Wang, Cheng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Frechet, Jean M. J.; Beaujuge, Pierre M.] King Abdullah Univ Sci & Technol, Thuwal 239556900, Saudi Arabia. RP Toney, MF (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. EM mftoney@slac.stanford.edu RI Wang, Cheng/A-9815-2014; OI Frechet, Jean /0000-0001-6419-0163 FU Center for Advanced Molecular Photovoltaics [KUS-C1-015-21]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393]; National Center for Research Resources [P41RR001209]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This publication was based on work supported by the Center for Advanced Molecular Photovoltaics, Award No KUS-C1-015-21, made by King Abdullah University of Science and Technology (KAUST). Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. The beam line 4-2 is part of the SSRL Structural Molecular Biology Program which is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393) and the National Center for Research Resources (P41RR001209). The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of NIGMS, NCRR or NIH. Scattering experiments were performed at the Advanced Light Source which is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 46 TC 65 Z9 67 U1 4 U2 75 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JAN 15 PY 2014 VL 26 IS 2 BP 300 EP 305 DI 10.1002/adma.201303622 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH3QZ UT WOS:000336041400010 PM 24174401 ER PT J AU Chen, SY Narang, P Atwater, HA Wang, LW AF Chen, Shiyou Narang, Prineha Atwater, Harry A. Wang, Lin-Wang TI Phase Stability and Defect Physics of a Ternary ZnSnN2 Semiconductor: First Principles Insights SO ADVANCED MATERIALS LA English DT Article ID OPTICAL-PROPERTIES; SOLAR-CELLS; NITRIDES; PREDICTION AB First-principles calculations show that ZnSnN2 has a very small formation enthalpy, and the donor defects such as Sn-Zn antisites and O-N impurities have high concentration, making the material degenerately n-type, which explains the observ(e)d high electron concentration. ZnSnN2 can be regarded as a new material that combines a metal-like conductivity with an optical bandgap around 2 eV. C1 [Chen, Shiyou; Narang, Prineha; Atwater, Harry A.; Wang, Lin-Wang] Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Chen, Shiyou; Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Narang, Prineha; Atwater, Harry A.] CALTECH, Thomas J Watson Labs Appl Phys, Pasadena, CA 91125 USA. RP Chen, SY (reprint author), Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM cshiyou@gmail.com; haa@caltech.edu; lwwang@lbl.gov FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation Graduate Research Fellowship; Resnick Sustainability Institute FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. Prineha Narang is supported by the National Science Foundation Graduate Research Fellowship and the Resnick Sustainability Institute. NR 38 TC 10 Z9 10 U1 7 U2 71 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JAN 15 PY 2014 VL 26 IS 2 BP 311 EP 315 DI 10.1002/adma.201302727 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH3QZ UT WOS:000336041400012 PM 24403116 ER PT J AU Streubel, R Lee, J Makarov, D Im, MY Karnaushenko, D Han, L Schafer, R Fischer, P Kim, SK Schmidt, OG AF Streubel, Robert Lee, Jehyun Makarov, Denys Im, Mi-Young Karnaushenko, Daniil Han, Luyang Schaefer, Rudolf Fischer, Peter Kim, Sang-Koog Schmidt, Oliver G. TI Magnetic Microstructure of Rolled-Up Single-Layer Ferromagnetic Nanomembranes SO ADVANCED MATERIALS LA English DT Article ID X-RAY MICROSCOPY; PERMALLOY-FILMS; DOMAIN-WALL; ELECTRONICS; NANOTUBES; MAGNETOELECTRONICS; MAGNETORESISTANCE; MAGNETOSTRICTION; MULTILAYERS AB The magnetic microstructure of rolled-up magnetic nanomembranes is revealed both theoretically and experimentally. Two types of nanomembranes are considered, one with a non-magnetic spacer layer and the other without. Experimentally, by using different materials and tuning the dimensions of the rolled-up nanomembranes, domain patterns consisting of spiral-like and azimuthally magnetized domains are observed, which are in qualitative agreement with the theoretical predictions. C1 [Streubel, Robert; Makarov, Denys; Karnaushenko, Daniil; Han, Luyang; Schmidt, Oliver G.] IFW Dresden, Inst Integrat Nanosci, D-01069 Dresden, Germany. [Streubel, Robert; Schmidt, Oliver G.] Tech Univ Chemnitz, D-09107 Chemnitz, Germany. [Lee, Jehyun; Kim, Sang-Koog] Seoul Natl Univ, Dept Mat Sci & Engn, Res Inst Adv Mat,Nanospin Lab, Natl Creat Res Initiat Ctr Spin Dynam & Spin Wave, Seoul 151744, South Korea. [Schaefer, Rudolf] IFW Dresden, Inst Metall Mat, D-01069 Dresden, Germany. [Schaefer, Rudolf] Tech Univ Dresden, Inst Mat Sci, D-01069 Dresden, Germany. [Im, Mi-Young; Fischer, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. RP Makarov, D (reprint author), IFW Dresden, Inst Integrat Nanosci, D-01069 Dresden, Germany. EM d.makarov@ifw-dresden.de RI Makarov, Denys/G-1025-2011; Fischer, Peter/A-3020-2010; Streubel, Robert/D-9686-2012 OI Fischer, Peter/0000-0002-9824-9343; FU Basic Science Research Program through a National Research Foundation of Korea; Ministry of Science, ICT & Future Planning [2013003460]; German Science Foundation (DFG) [MA 5144/2-1]; DFG Research Unit [1713]; European Research Council under the European Union [306277]; Office of Science, Office of Basic Energy Sciences, Materials Sciences, and Engineering Division, of the U.S. Department of Energy [DE-AC02-05-CH11231] FX This work was supported in part by the Basic Science Research Program through a National Research Foundation of Korea funded by the Ministry of Science, ICT & Future Planning (Grant No. 2013003460) and via the German Science Foundation (DFG) grant MA 5144/2-1, DFG Research Unit 1713 and European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement no. 306277. The operation of the soft X-ray microscope was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences, and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231. NR 46 TC 32 Z9 32 U1 2 U2 50 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JAN 15 PY 2014 VL 26 IS 2 BP 316 EP 323 DI 10.1002/adma.201303003 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AH3QZ UT WOS:000336041400013 PM 24136680 ER PT J AU Chiang, HT Xu, GL Somma, RD AF Chiang, Hao-Tien Xu, Guanglei Somma, Rolando D. TI Improved bounds for eigenpath traversal SO PHYSICAL REVIEW A LA English DT Article ID ADIABATIC EVOLUTION; QUANTUM COMPUTATION; SPIN SYSTEMS; HAMILTONIANS; OPTIMIZATION; COMPLEXITY AB We present a bound on the length of the path defined by the ground states of a continuous family of Hamiltonians in terms of the spectral gap Delta. We use this bound to obtain a significant improvement over the cost of recently proposed methods for quantum adiabatic state transformations and eigenpath traversal. In particular, we prove that a method based on evolution randomization, which is a simple extension of adiabatic quantum computation, has an average cost of order 1/Delta(2), and amethod based on fixed-point search has a maximum cost of order 1/Delta(3/2). Additionally, if the Hamiltonians satisfy a frustration-free property, such costs can be further improved to order 1/Delta(3/2) and 1/Delta, respectively. Our methods offer an important advantage over adiabatic quantum computation when the gap is small, where the cost is of order 1/Delta(3). C1 [Chiang, Hao-Tien] Univ New Mexico, Albuquerque, NM 87185 USA. [Xu, Guanglei] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Somma, Rolando D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chiang, HT (reprint author), Univ New Mexico, Albuquerque, NM 87185 USA. EM lewis.prometheus@gmail.com; glxu.leo@gmail.com; somma@lanl.gov FU National Science Foundation through the CCF program; AFOSR [FA9550-12-1-0057]; Sandia National Laboratories; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX H.-T.C. acknowledges support from the National Science Foundation through the CCF program. G.X. and R.S. acknowledge support from AFOSR through Grant No. FA9550-12-1-0057. R.S. thanks Sandia National Laboratories, where the initial ideas of this work were developed. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. We thank Sergio Boixo, Andrew Daley, and Andrew Landahl for discussions. NR 44 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JAN 15 PY 2014 VL 89 IS 1 AR 012314 DI 10.1103/PhysRevA.89.012314 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0GW UT WOS:000332173800005 ER PT J AU Naginey, TC Pollock, BB Stacy, EW Walters, HRJ Whelan, CT AF Naginey, T. C. Pollock, B. B. Stacy, Eric W. Walters, H. R. J. Whelan, Colm T. TI Estimating positronium formation for plasma applications SO PHYSICAL REVIEW A LA English DT Article ID HYDROGEN-ATOMS; CROSS-SECTIONS; IMPACT-IONIZATION; CHARGE-TRANSFER; COLLISIONS; ANNIHILATION; ELECTRONS; PROTONS; SCATTERING; PAIR AB The basic physics of e(+), e(-) creation and annihilation is overviewed. It is shown that for atomic hydrogen targets electron capture by a free positron to form positronium is vastly more probable than in-flight annihilation. Cross sections are presented using the classical trajectory Monte Carlo (CTMC) approach for the charge-exchange process: e(+) + A(q+) -> Ps + A((q+1)+), where A(q+) is some target ion of charge q. Charge-exchange cross sections for hydrogenic ion targets are presented. It is found that while the CTMC gives adequate results for positronium formation for e(+)-hydrogen and e(+)-cesium collisions, its high-energy behavior for hydrogenic ions is not in agreement with quantum mechanical predictions. Since we are interested in situations where many multicharged ions will be present we have looked for an alternative approach. Scaling rules are proposed and used to estimate the charge-exchange cross sections for both neutral atoms and multicharged ions. C1 [Naginey, T. C.; Stacy, Eric W.; Whelan, Colm T.] Old Dominion Univ, Dept Phys, Norfolk, VA 23323 USA. [Pollock, B. B.; Whelan, Colm T.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Walters, H. R. J.] Queens Univ, Dept Appl Math & Theoret Phys, Belfast BT7 1NN, Antrim, North Ireland. RP Naginey, TC (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23323 USA. FU Department of Energy by the Lawrence Livermore National Laboratory [AC52-07NA-27344]; LLNL's Institute for Laser Science Applications (ILSA) FX We are grateful to Professor Gaetana Laricchia for supplying us with her experimental data and to an unnamed referee for most helpful comments on positron-atom annihilation near the positronium formation threshold. This work was performed under the auspices of the Department of Energy by the Lawrence Livermore National Laboratory under Contract No. AC52-07NA-27344. The authors acknowledge support from LLNL's Institute for Laser Science Applications (ILSA). NR 41 TC 3 Z9 3 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 15 PY 2014 VL 89 IS 1 AR 012708 DI 10.1103/PhysRevA.89.012708 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0GW UT WOS:000332173800009 ER PT J AU Kimchi, I Vishwanath, A AF Kimchi, Itamar Vishwanath, Ashvin TI Kitaev-Heisenberg models for iridates on the triangular, hyperkagome, kagome, fcc, and pyrochlore lattices SO PHYSICAL REVIEW B LA English DT Article ID TOPOLOGICAL INSULATORS; FLUCTUATIONS; STATE; ORDER AB The Kitaev-Heisenberg (KH) model has been proposed to capture magnetic interactions in iridate Mott insulators on the honeycomb lattice. We show that analogous interactions arise in many other geometries built from edge-sharing IrO6 octahedra, including the pyrochlore and hyperkagome lattices relevant to Ir2O4 and Na4Ir3O8, respectively. The Kitaev spin liquid exact solution does not generalize to these lattices. However, a different, exactly soluble point of the honeycomb lattice KH model, obtained by a four-sublattice transformation to a ferromagnet, generalizes to all of these lattices and even to certain additional further neighbor Heisenberg couplings. A Klein four-group congruent to Z(2) x Z(2) structure is associated with this mapping (hence Klein duality). A finite lattice admits the duality if a simple geometrical condition is met. This duality predicts fluctuation-free ordered states on these different 2D and 3D lattices, which are analogues of the honeycomb lattice KH stripy order. This result is used in conjunction with a semiclassical Luttinger-Tisza approximation to obtain phase diagrams for KH models on the different lattices. We also discuss a Majorana fermion based mean-field theory at the Kitaev point, which is exact on the honeycomb lattice, for the KH models on the different lattices. We attribute the rich behavior of these models to the interplay of geometric frustration and frustration induced by spin-orbit coupling. C1 [Kimchi, Itamar; Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Vishwanath, Ashvin] Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA 94720 USA. RP Kimchi, I (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. FU NSF [DGE 1106400, PHY11-25915]; ARO MURI [W911NF-12-0461] FX We thank Yi-Zhuang You, Yuan-Ming Lu, George Jackeli, and Christopher Henley for useful discussions. We are also grateful for the hospitality of the Kavli Institute for Theoretical Physics, where part of this work was written. This research is supported in part by the NSF under Grants No. DGE 1106400 and NSF PHY11-25915 for the KITP Graduate Fellowship Program (IK), and ARO MURI grant W911NF-12-0461 (AV). NR 64 TC 40 Z9 40 U1 7 U2 64 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 15 PY 2014 VL 89 IS 1 AR 014414 DI 10.1103/PhysRevB.89.014414 PG 13 WC Physics, Condensed Matter SC Physics GA AC0WS UT WOS:000332216800001 ER PT J AU Chatillon, A Belier, G Granier, T Laurent, B Morillon, B Taieb, J Haight, RC Devlin, M Nelson, RO Noda, S O'Donnell, JM AF Chatillon, A. Belier, G. Granier, T. Laurent, B. Morillon, B. Taieb, J. Haight, R. C. Devlin, M. Nelson, R. O. Noda, S. O'Donnell, J. M. TI Measurement of prompt neutron spectra from the Pu-239(n, f) fission reaction for incident neutron energies from 1 to 200 MeV SO PHYSICAL REVIEW C LA English DT Article AB Prompt fission neutron spectra in the neutron-induced fission of Pu-239 have been measured for incident neutron energies from 1 to 200 MeV at the Los Alamos Neutron Science Center. Mean energies deduced from the prompt fission neutron spectra (PFNS) lead to the observation of the opening of the second chance fission at 7 MeV and to indications for the openings of fission channels of third and fourth chances. Moreover, the general trend of the measured PFNS is well reproduced by the different models. The comparison between data and models presents, however, two discrepancies. First, the prompt neutron mean energy seems constant for neutron energy, at least up to 7 MeV, whereas in the theoretical calculations it is continuously increasing. Second, data disagree with models on the shape of the high energy part of the PFNS, where our data suggest a softer spectrum than the predictions. C1 [Chatillon, A.; Belier, G.; Granier, T.; Laurent, B.; Morillon, B.; Taieb, J.] CEA, DAM, DIF, F-91297 Arpajon, France. [Haight, R. C.; Devlin, M.; Nelson, R. O.; Noda, S.; O'Donnell, J. M.] Los Alamos Natl Lab, LANSCE, Los Alamos, NM 87545 USA. RP Chatillon, A (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM audrey.chatillon@cea.fr RI Devlin, Matthew/B-5089-2013 OI Devlin, Matthew/0000-0002-6948-2154 FU DOE [DE-AC52-06NA25396] FX This work was performed under the auspices of a cooperation agreement between CEA/DAM and DOE/NNSA on fundamental sciences and benefited from the use of the LANSCE accelerator facility, supported under DOE Contract No. DE-AC52-06NA25396. NR 21 TC 8 Z9 8 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 15 PY 2014 VL 89 IS 1 AR 014611 DI 10.1103/PhysRevC.89.014611 PG 9 WC Physics, Nuclear SC Physics GA AB9ZE UT WOS:000332153500003 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Balewski, J Banerjee, A Barber, B Barnovska, Z Beavis, DR Bellwied, R Betancourt, MJ Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Bridgeman, A Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Corliss, R Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, F Dion, A Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Fatemi, R Fazio, S Fedorisin, J Fersch, RG Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Grosnick, D Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hajkova, O Hamed, A Han, LX Haque, R Harris, JW Hays-Wehle, JP He, W Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Jena, C Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Korsch, W Kotchenda, L Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Leight, W LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lima, LM Lisa, MA Liu, F Ljubicic, T Llope, WJ Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Manweiler, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Munhoz, MG Mustafa, MK Naglis, M Nandi, BK Nasim, M Nayak, TK Nelson, JM Nogach, LV Noh, SY Nord, PM Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Oliveira, RAN Olson, D Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Peterson, A Pile, P Planinic, M Pluta, J Plyku, D Pochron, W Poljak, N Porter, J Poskanzer, AM Powell, CB Pruneau, C Pruthi, NK Przybycien, M Pujahari, PR Putschke, J Qiu, H Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schaub, J Schmah, AM Schmidke, WB Schmitz, N Seger, J Selyuzhenkov, I Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P deSouza, UG Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Suaide, AAP Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM de Toledo, AS Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbk, F Viyogi, YP Vokal, S Voloshin, SA Vossen, A Wada, M Walker, M Wang, F Wang, G Wang, H Wang, JS Wang, Q Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, N Xu, QH Xu, W Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Balewski, J. Banerjee, A. Barber, B. Barnovska, Z. Beavis, D. R. Bellwied, R. Betancourt, M. J. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Bridgeman, A. Brovko, S. G. Bultmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. de la Barca Sanchez, M. Calderon Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Corliss, R. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Derradi de Souza, R. Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Dion, A. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Fatemi, R. Fazio, S. Fedorisin, J. Fersch, R. G. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Grosnick, D. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hajkova, O. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Hays-Wehle, J. P. He, W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Jena, C. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Korsch, W. Kotchenda, L. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Leight, W. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lima, L. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Manweiler, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Munhoz, M. G. Mustafa, M. K. Naglis, M. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nogach, L. V. Noh, S. Y. Nord, P. M. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Oliveira, R. A. N. Olson, D. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Peterson, A. Pile, P. Planinic, M. Pluta, J. Plyku, D. Pochron, W. Poljak, N. Porter, J. Poskanzer, A. M. Powell, C. B. Pruneau, C. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Putschke, J. Qiu, H. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schaub, J. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Selyuzhenkov, I. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. deSouza, U. G. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Suaide, A. A. P. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szanto de Toledo, A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbk, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Vossen, A. Wada, M. Walker, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, Q. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, N. Xu, Q. H. Xu, W. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Neutral pion cross section and spin asymmetries at intermediate pseudorapidity in polarized proton collisions at root s=200 GeV SO PHYSICAL REVIEW D LA English DT Article ID PLUS P COLLISIONS; PI-0 PRODUCTION; PARTON DISTRIBUTIONS; TRANSVERSE-MOMENTUM; STAR; FRAGMENTATION; ANTIPROTONS; QCD AB The differential cross section and spin asymmetries for neutral pions produced within the intermediate pseudorapidity range 0.8 < eta < 2.0 in polarized proton-proton collisions at root s = 200 GeV are presented. Neutral pions were detected using the end cap electromagnetic calorimeter in the STAR detector at RHIC. The cross section was measured over a transverse momentum range of 5 < p(T) < 16 GeV/c and is found to agree with a next-to-leading order perturbative QCD calculation. The longitudinal double-spin asymmetry A(LL) is measured in the same pseudorapidity range and spans a range of Bjorken-x down to x approximate to 0.01. The measured A(LL) is consistent with model predictions for varying degrees of gluon polarization. The parity-violating asymmetry A(L) is also measured and found to be consistent with zero. The transverse single-spin asymmetry A(N) is measured over a previously unexplored kinematic range in Feynman-x and p(T). Such measurements may aid our understanding of the onset and kinematic dependence of the large asymmetries observed at more forward pseudorapidity (eta approximate to 3) and their underlying mechanisms. The A(N) results presented are consistent with a twist-3 model prediction of a small asymmetry over the present kinematic range. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, Krakow, Poland. [Bridgeman, A.; Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dion, A.; Dunlop, J. C.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbk, F.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Brovko, S. G.; de la Barca Sanchez, M. Calderon; Cebra, D.; Ding, F.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Xu, W.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil. [Chen, L.; Huck, P.; Ke, H. W.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. F.; Yang, Y.; Zhang, J. B.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Chwastowski, J.; Kycia, R. A.] Cracow Univ Technol, Krakow, Poland. [Cherney, M.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Hajkova, O.; Pachr, M.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Barnovska, Z.; Bielcikova, J.; Rusnak, J.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] Frankfurt Inst Adv Studies FIAS, Frankfurt, Germany. [Das, S.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Mumbai 400076, Maharashtra, India. [Dhamija, S.; He, W.; Jacobs, W. W.; Page, B. S.; Selyuzhenkov, I.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Keane, D.; Kumar, L.; Margetis, S.; Shanmuganathan, P. V.; Vanfossen, J. A., Jr.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Fersch, R. G.; Korsch, W.; Ramachandran, S.; Webb, G.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Taejon, South Korea. [Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou, Peoples R China. [Dong, X.; Eun, L.; Masui, H.; Matis, H. S.; Naglis, M.; Odyniec, G.; Olson, D.; Porter, J.; Poskanzer, A. M.; Powell, C. B.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Xu, N.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Balewski, J.; Betancourt, M. J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Stevens, J. R.; van Nieuwenhuizen, G.; Walker, M.] MIT, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Jena, C.; Mohanty, B.; Nasim, Md.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Anson, C. D.; Gangadharan, D. R.; Humanic, T. J.; Lisa, M. A.; Peterson, A.] Ohio State Univ, Columbus, OH 43210 USA. [Bultmann, S.; Koralt, I.; Plyku, D.] Old Dominion Univ, Norfolk, VA 23529 USA. [Pawlik, B.; Turnau, J.] Inst Nucl Phys PAN, Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Cendejas, R.; Dilks, C.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino, Russia. [Garand, D.; Hirsch, A.; Kikola, D. P.; Konzer, J.; Li, X.; Mustafa, M. K.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Wang, Q.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Lima, L. M.; Munhoz, M. G.; Oliveira, R. A. N.; deSouza, U. G.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, Sao Paulo, Brazil. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zawisza, Y.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, Nantes, France. [Li, X.; Surrow, B.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; De Silva, L. C.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Engle, K. S.; Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Barber, B.; Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Manweiler, R.; Nord, P. M.; Pochron, W.; Schaub, J.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Pal, S. K.; Roy, A.; Sahoo, N. R.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Sandacz, A.; Trzeciak, B. A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Pruneau, C.; Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, Krakow, Poland. RI Derradi de Souza, Rafael/M-4791-2013; Suaide, Alexandre/L-6239-2016; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Fazio, Salvatore /G-5156-2010; Lednicky, Richard/K-4164-2013; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Takahashi, Jun/B-2946-2012; Alekseev, Igor/J-8070-2014; Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; Xu, Wenqin/H-7553-2014; Aparecido Negrao de Oliveira, Renato/G-9133-2015; Kycia, Radoslaw/J-4397-2015; Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015 OI Derradi de Souza, Rafael/0000-0002-2084-7001; Suaide, Alexandre/0000-0003-2847-6556; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Bhasin, Anju/0000-0002-3687-8179; Ke, Hongwei/0000-0003-1463-7291; Takahashi, Jun/0000-0002-4091-1779; Alekseev, Igor/0000-0003-3358-9635; Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Xu, Wenqin/0000-0002-5976-4991; Kycia, Radoslaw/0000-0002-6390-4627; Huang, Bingchu/0000-0002-3253-3210 FU Office of NP within the U.S. DOE Office of Science; Office of HEP within the U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA of the Czech Republic; MSMT of the Czech Republic; FIAS of Germany; DAE of India; DST of India; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia; Renaissance Technologies Corporation FX The authors thank M. Stratmann, W. Vogelsang, and K. Kanazawa for providing calculations and discussion. We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, National Science Centre of Poland, National Research Foundation (NRF-2012004024), Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. Finally, we gratefully acknowledge a sponsored research grant for the 2006 run period from Renaissance Technologies Corporation. NR 61 TC 17 Z9 17 U1 1 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 15 PY 2014 VL 89 IS 1 AR 012001 DI 10.1103/PhysRevD.89.012001 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5YO UT WOS:000331864800001 ER PT J AU Chern, GW Wu, CJ AF Chern, Gia-Wei Wu, Congjun TI Four-Coloring Model and Frustrated Superfluidity in the Diamond Lattice SO PHYSICAL REVIEW LETTERS LA English DT Article ID STATE AB We propose a novel four-coloring model which describes "frustrated superfluidity" of p-band bosons in the diamond optical lattice. The superfluid phases of the condensate wave functions on the diamond-lattice bonds are mapped to four distinct colors at low temperatures. The fact that a macroscopic number of states satisfy the constraints that four differently colored bonds meet at the same site leads to an extensive degeneracy in the superfluid ground state at the classical level. We demonstrate that the phase of the superfluid wave function as well as the orbital angular momentum correlations exhibit a power-law decay in the degenerate manifold that is described by an emergent magnetostatic theory with three independent flux fields. Our results thus provide a novel example of critical superfluid phase with algebraic order in three dimensions. We further show that quantum fluctuations favor a Neel ordering of orbital angular moments with broken sublattice symmetry through the order-by-disorder mechanism. C1 [Chern, Gia-Wei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Wu, Congjun] Univ Calif San Diego, Dept Phys, San Diego, CA 92093 USA. RP Chern, GW (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Wu, Congjun/L-1750-2015 FU ICAM; NSF [DMR-0844115]; NSF of China [11328403]; Aspen Center of Physics; [NSF DMR-1105945]; [AFOSR FA9550-11-1-0067] FX We are thankful for useful discussions with R. Moessner, Y. Li, and Zi Cai. G. W. C. acknowledges the support of ICAM and NSF Grant No. DMR-0844115. C. W. is supported by Grants No. NSF DMR-1105945 and No. AFOSR FA9550-11-1-0067 (Young Investigator Research Program). C. W. also acknowledges support from the NSF of China under Grant No. 11328403 and the hospitality of the Aspen Center of Physics. NR 36 TC 1 Z9 1 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 15 PY 2014 VL 112 IS 2 AR 020601 DI 10.1103/PhysRevLett.112.020601 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7AI UT WOS:000331941300004 PM 24483997 ER PT J AU Mourigal, M Fuhrman, WT Sheckelton, JP Wartelle, A Rodriguez-Rivera, JA Abernathy, DL McQueen, TM Broholm, CL AF Mourigal, M. Fuhrman, W. T. Sheckelton, J. P. Wartelle, A. Rodriguez-Rivera, J. A. Abernathy, D. L. McQueen, T. M. Broholm, C. L. TI Molecular Quantum Magnetism in LiZn2Mo3O8 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SPIN-LIQUID; VALENCE; ANTIFERROMAGNET AB Inelastic neutron scattering at low temperatures T <= 30 K from a powder of LiZn2Mo3O8 demonstrates this triangular-lattice antiferromagnet hosts collective magnetic excitations from spin-1/2 Mo3O13 molecules. Apparently gapless (Delta < 0.2 meV) and extending at least up to 2.5 meV, the low-energy magnetic scattering cross section is surprisingly broad in momentum space and involves one-third of the spins present above 100 K. The data are compatible with the presence of valence bonds involving nearest-neighbor and next-nearest-neighbor spins forming a disordered or dynamic state. C1 [Mourigal, M.; Fuhrman, W. T.; Sheckelton, J. P.; Wartelle, A.; McQueen, T. M.; Broholm, C. L.] Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. [Mourigal, M.; Fuhrman, W. T.; Sheckelton, J. P.; Wartelle, A.; McQueen, T. M.; Broholm, C. L.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Sheckelton, J. P.; McQueen, T. M.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [Wartelle, A.] Univ Lyon, Ecole Normale Super Lyon, F-69364 Lyon 07, France. [Rodriguez-Rivera, J. A.; Broholm, C. L.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Rodriguez-Rivera, J. A.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Abernathy, D. L.; Broholm, C. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Mourigal, M (reprint author), Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. RI Abernathy, Douglas/A-3038-2012; Mourigal, Martin/F-4495-2010; Rodriguez-Rivera, Jose/A-4872-2013; BL18, ARCS/A-3000-2012 OI Abernathy, Douglas/0000-0002-3533-003X; Mourigal, Martin/0000-0003-2772-8440; Rodriguez-Rivera, Jose/0000-0002-8633-8314; FU U.S. Department of Energy, office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]; National Science Foundation [DMR-0944772]; U.S. Department of Energy, office of Basic Energy Sciences, Scientific User Facilities Division FX We thank R. Flint, P. A. Lee, O. Tchernyshyov, and Y. Wan for discussion and Y. Qiu for assistance with the MACS experiment and data treatment. The work at IQM was supported by the U.S. Department of Energy, office of Basic Energy Sciences, Division of Material Sciences and Engineering under Grant No. DE-FG02-08ER46544. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. Research at Oak Ridge National Laboratory's Spallation Neutron Source is sponsored by the U.S. Department of Energy, office of Basic Energy Sciences, Scientific User Facilities Division. NR 31 TC 17 Z9 17 U1 5 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 15 PY 2014 VL 112 IS 2 AR 027202 DI 10.1103/PhysRevLett.112.027202 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7AI UT WOS:000331941300026 PM 24484043 ER PT J AU Vaikuntanathan, S Geissler, PL AF Vaikuntanathan, Suriyanarayanan Geissler, Phillip L. TI Putting Water on a Lattice: The Importance of Long Wavelength Density Fluctuations in Theories of Hydrophobic and Interfacial Phenomena SO PHYSICAL REVIEW LETTERS LA English DT Article ID 3-DIMENSIONAL ISING-MODEL; LIQUID-VAPOR INTERFACES; SURFACE-TENSION; SOLVENT FLUCTUATIONS; FREE-ENERGIES; TRANSITION; ADSORPTION; SOLUTES AB The physics of air-water interfaces plays a central role in modern theories of the hydrophobic effect. Implementing these theories, however, has been hampered by the difficulty of addressing fluctuations in the shape of such soft interfaces. We show that this challenge is a fundamental consequence of mapping long wavelength density variations onto discrete degrees of freedom. Drawing from studies of surface roughness in lattice models, we account for the resulting nonlinearities simply but accurately. Simulations show that this approach captures complex solvation behaviors quantitatively. C1 [Vaikuntanathan, Suriyanarayanan; Geissler, Phillip L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Geissler, Phillip L.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Vaikuntanathan, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. FU U.S. Department of Energy, Office of Basic Energy Sciences, through the Chemical Sciences Division (CSD) of the Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231] FX We gratefully acknowledge extremely useful discussions with John D. Weeks, Gerhard Hummer, David Chandler, and David Limmer. This project was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, through the Chemical Sciences Division (CSD) of the Lawrence Berkeley National Laboratory (LBNL), under Contract DE-AC02-05CH11231. NR 34 TC 11 Z9 11 U1 0 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 15 PY 2014 VL 112 IS 2 AR 020603 DI 10.1103/PhysRevLett.112.020603 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7AI UT WOS:000331941300005 PM 24483999 ER PT J AU Miao, L Wu, WT Aubry, N Massoudi, M AF Miao, Ling Wu, Wei-Tao Aubry, Nadine Massoudi, Mehrdad TI Heat transfer and flow of a slag-type non-linear fluid: Effects of variable thermal conductivity SO APPLIED MATHEMATICS AND COMPUTATION LA English DT Article DE Slag; Non-linear fluids; Variable viscosity; Variable thermal conductivity; Falling film; Viscous dissipation; Radiation boundary condition; Gasification ID GRANULAR-MATERIALS; PART II; VECTOR; BEHAVIOR; SPHERES; FOURIER AB In this paper, we study the effects of variable thermal conductivity on the flow and heat transfer in a slag-type non-linear fluid down a vertical wall. The constitutive relation for the heat flux vector is assumed to be the Fourier's law of conduction with a variable thermal conductivity which includes the second order effects of the volume fraction. We numerically solve the non-dimensional form of the governing equations to study the effects of various dimensionless numbers on the velocity, temperature and volume fraction. The results indicate that the thermal conductivity plays a major role in the temperature distribution. Also, for certain values of the dimensionless numbers, minor differences are observed in the velocity and volume fraction distribution compared with the case of constant thermal conductivity. Published by Elsevier Inc. C1 [Miao, Ling; Wu, Wei-Tao] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. [Aubry, Nadine] Northeastern Univ, Dept Mech Engn, Boston, MA 02115 USA. [Massoudi, Mehrdad] US DOE, NETL, Pittsburgh, PA 15236 USA. RP Massoudi, M (reprint author), US DOE, NETL, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. EM MASSOUDI@NETL.DOE.GOV NR 34 TC 3 Z9 3 U1 2 U2 6 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0096-3003 EI 1873-5649 J9 APPL MATH COMPUT JI Appl. Math. Comput. PD JAN 15 PY 2014 VL 227 BP 77 EP 91 DI 10.1016/j.amc.2013.11.010 PG 15 WC Mathematics, Applied SC Mathematics GA AB0QE UT WOS:000331496400008 ER PT J AU Hay, BP Jia, CD Nadas, J AF Hay, Benjamin P. Jia, Chuandong Nadas, Janos TI Computer-aided design of host molecules for recognition of organic guests SO COMPUTATIONAL AND THEORETICAL CHEMISTRY LA English DT Article DE Computer-aided molecular design; Host; Receptor; Oxygen mustard; HostDesigner ID MM3 FORCE-FIELD; SULFUR MUSTARD; CHIRAL LIGANDS; OXYGEN ANALOG; GUIDED DESIGN; COMPLEXES; MECHANICS; RECEPTOR; HYDROCARBONS; DIFFUSION AB This paper presents an overview of a computational approach to design molecular host architectures. After positioning donor groups about a targeted guest molecule, the donor groups are connected with hydrocarbon linkages taken from an extensive database of molecular fragments. Initial ranking of the host structures is based on how well bond vectors on the donor groups match bond vectors on the linkages. The top candidates are then subjected to further evaluation with molecular mechanics identifying host architectures that are both complementary and preorganized for binding the guest. The efficacy of this computer-aided design methodology is illustrated with a search for hydrogen bonding receptors that are structurally organized for complexation with oxygen mustard. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hay, Benjamin P.; Jia, Chuandong; Nadas, Janos] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Hay, BP (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,POB 2008,Bldg 4100, Oak Ridge, TN 37831 USA. EM haybp@ornl.gov RI Jia, Chuandong/G-3779-2012 FU Defense Threat Reduction Agency-joint Science and Technology Office for Chemical and Biological Defense [DTRA10027-8137] FX This project received support from the Defense Threat Reduction Agency-joint Science and Technology Office for Chemical and Biological Defense (DTRA10027-8137). NR 44 TC 6 Z9 6 U1 1 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2210-271X EI 1872-7999 J9 COMPUT THEOR CHEM JI Comput. Theor. Chem. PD JAN 15 PY 2014 VL 1028 BP 72 EP 80 DI 10.1016/j.comptc.2013.12.003 PG 9 WC Chemistry, Physical SC Chemistry GA AB3JY UT WOS:000331688300009 ER PT J AU Datko-Williams, L Wilkie, A Richmond-Bryant, J AF Datko-Williams, Laura Wilkie, Adrien Richmond-Bryant, Jennifer TI Analysis of U.S. soil lead (Pb) studies from 1970 to 2012 SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Soil lead; Pb storage; United States; Urbanized area; Population density ID CHILDRENS BLOOD LEAD; HEAVY-METAL CONTAMINATION; NEW-ORLEANS; ENVIRONMENTAL LEAD; URBAN SOILS; HURRICANE-KATRINA; INNER-CITY; GASTROINTESTINAL-TRACT; RESIDENTIAL SOILS; SURFACE SOILS AB Although lead (Pb) emissions to the air have substantially decreased in the United States since the phase-out of leaded gasoline by 1995, amounts of lead in some soils remain elevated. Lead concentrations in residential and recreational soils are of concern because health effects have been associated with Pb exposure. Elevated soil Pb is especially harmful to young children due to their higher likelihood of soil ingestion. The purpose of this study is to create a comprehensive compilation of U.S. soil Pb data published from 1970 through 2012 as well as to analyze the collected data to reveal spatial and/or temporal soil Pb trends in the U.S. over the past 40 years. A total of 84 soil Pb studies across 62 U.S. cities were evaluated. Median soil Pb values from the studies were analyzed with respect to year of sampling, residential location type (e.g., urban, suburban), and population density. In aggregate, there was no statistically significant correlation between year and median soil Pb; however, within single cities, soil Pb generally declined overtime. Our analysis shows that soil Pb quantities in city centers were generally highest and declined towards the suburbs and exurbs of the city. In addition, there was a statistically significant, positive relationship between median soil Pb and population density. In general, the trends examined here align with previously reported conclusions that soil Pb levels are higher in larger urban areas and Pb tends to remain in soil for long periods of time. (C) 2013 Elsevier B.V. All rights reserved. C1 [Datko-Williams, Laura; Wilkie, Adrien] US EPA, Oak Ridge Inst Sci & Educ, Environm Media Assessment Grp, Natl Ctr Environm Assessment, Res Triangle Pk, NC 27711 USA. [Richmond-Bryant, Jennifer] US EPA, Environm Media Assessment Grp, Natl Ctr Environm Assessment, Res Triangle Pk, NC 27711 USA. RP Datko-Williams, L (reprint author), US EPA, Oak Ridge Inst Sci & Educ, Environm Media Assessment Grp, Natl Ctr Environm Assessment, Mail Drop B243-01, Res Triangle Pk, NC 27711 USA. EM Datko-Williams.Laura@epa.gov NR 113 TC 18 Z9 19 U1 3 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD JAN 15 PY 2014 VL 468 BP 854 EP 863 DI 10.1016/j.scitotenv.2013.08.089 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA AB4QW UT WOS:000331776000091 PM 24076506 ER PT J AU Zhang, C Malhotra, SV Francis, AJ AF Zhang, C. Malhotra, S. V. Francis, A. J. TI Toxicity of ionic liquids to Clostridium sp. and effects on uranium biosorption SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Ionic liquids; Uranium; Biosorption; Clostridium sp.; Toxicity ID WHOLE-CELL BIOCATALYSIS; MEMBRANE DAMAGE; BIOREDUCTION; REMEDIATION; HYDROLYSIS; ACTINIDES; BACTERIA; BEHAVIOR; SOLVENTS; ARCHAEA AB As green solvents ionic liquids (ILs) show high potential in nuclear industry for extraction and purification of actinides. However, to date relatively little information has been gained on ILs application in microbial processes, for example biosorption of radionuclides. We investigated the effects of three ILs, 1-butyl-3-methylimidazolium hexafluorophosphate (BMIMPF6), N-ethylpyridinium trifluoroacetate (EtPyCF3COO) and N-ethylpyridinium tetrafluoroborate (EtPyBF4) on the growth and biosorption of uranium by Clostridium sp. The ILs affected the growth of the bacterium as evidenced by decreases in optical density, total gas production, and organic acids production from glucose metabolism. The IC50-48 h of three ILs decreased in the order of BMIMPF6 (8.26 mM)> EtPyBF4 (7.04 mM)> EtPyCF3COO (4.05 mM). Uranium biosorption by the bacterial cells decreased by 75% in the presence of 1% (v/v) BMIMPF6 and by about 90% with 1% (v/v) EtPyBF4 or EtPyCF3COO, in comparison to the control without ILs. The diminished biosorption may be attributed to the membrane damages induced by EtPyBF4 and EtPyCF3COO, which can be visualized by Transmission Electron Microscope (TEM) analysis. Energy-dispersive X-ray spectroscopy (EDS) analysis revealed the accumulation of uranium inside peripheral membrane of the cells exposed to uranium alone or with BMIMPF6, while little or no accumulation was observed in the presence of EtPyBF4 and EtPyCF3COO. These results imply that potential toxicity of ILs towards microorganisms is a particularly important issue in limiting its biotechnological applications. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhang, C.] Nankai Univ, Coll Environm Sci & Engn, Tianjin 300071, Peoples R China. [Zhang, C.; Malhotra, S. V.] New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07104 USA. [Francis, A. J.] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Francis, A. J.] Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang 790784, South Korea. RP Zhang, C (reprint author), Nankai Univ, Coll Environm Sci & Engn, 94 Weijin Rd, Tianjin 300457, Peoples R China. EM zhangchengdong@nankai.edu.cn FU Brookhaven National Laboratory, Laboratory Directed Research and Development (LDRD), U.S. Department of Energy [DE-AC02-98CH10886]; BK21+ program through the National Research Foundation of Korea; Ministry of Education, Science and Technology FX We thank R. Harris, University of Guelph, for SEM and TEM analysis, and J.B. Gillow, for assistance. This work was supported by Brookhaven National Laboratory, Laboratory Directed Research and Development (LDRD), U.S. Department of Energy under contract No. DE-AC02-98CH10886; and in part by the BK21+ program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology. The authors have no conflict of interest to declare. NR 33 TC 12 Z9 13 U1 7 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JAN 15 PY 2014 VL 264 BP 246 EP 253 DI 10.1016/j.jhazmat.2013.11.003 PG 8 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AA3UW UT WOS:000331021200030 PM 24316798 ER PT J AU Roostapour, A Lee, G Zhong, L Kam, SI AF Roostapour, A. Lee, G. Zhong, L. Kam, S. I. TI Model fit to experimental data for foam-assisted deep vadose zone remediation SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Foams; Remediation; Deep vadose zone; Fractional flow method ID DELIVERY AB This study investigates how a foam model, developed in Roostapour and Kam [1], can be applied to make a fit to a set of existing laboratory flow experiments in an application relevant to deep vadose zone remediation. This study reveals a few important insights regarding foam-assisted deep vadose zone remediation: (i) the mathematical framework established for foam modeling can fit typical flow experiments matching wave velocities, saturation history, and pressure responses; (ii) the set of input parameters may not be unique for the fit, and therefore conducting experiments to measure basic model parameters related to relative permeability, initial and residual saturations, surfactant adsorption and so on should not be overlooked; and (iii) gas compressibility plays an important role for data analysis, thus should be handled carefully in laboratory flow experiments. Foam kinetics, causing foam texture to reach its steady-state value slowly, may impose additional complications. (C) 2013 Elsevier B.V. All rights reserved. C1 [Roostapour, A.; Kam, S. I.] Louisiana State Univ, Craft & Hawkins Dept Petr Engn, Baton Rouge, LA 70803 USA. [Zhong, L.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Kam, SI (reprint author), Louisiana State Univ, Craft & Hawkins Dept Petr Engn, Baton Rouge, LA 70803 USA. EM kam@lsu.edu NR 17 TC 3 Z9 3 U1 3 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JAN 15 PY 2014 VL 264 BP 460 EP 473 DI 10.1016/j.jhazmat.2013.09.016 PG 14 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AA3UW UT WOS:000331021200054 PM 24295900 ER PT J AU Saat, MR Werth, CJ Schaeffer, D Yoon, H Barkan, CPL AF Saat, Mohd Rapik Werth, Charles J. Schaeffer, David Yoon, Hongkyu Barkan, Christopher P. L. TI Environmental risk analysis of hazardous material rail transportation SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Risk analysis; Environmental cleanup; Rail transportation; Hazardous material AB An important aspect of railroad environmental risk management involves tank car transportation of hazardous materials. This paper describes a quantitative, environmental risk analysis of rail transportation of a group of light, non-aqueous-phase liquid (LNAPL) chemicals commonly transported by rail in North America. The Hazardous Materials Transportation Environmental Consequence Model (HMTECM) was used in conjunction with a geographic information system (GIS) analysis of environmental characteristics to develop probabilistic estimates of exposure to different spill scenarios along the North American rail network. The risk analysis incorporated the estimated clean-up cost developed using the HMTECM, route-specific probability distributions of soil type and depth to groundwater, annual traffic volume, railcar accident rate, and tank car safety features, to estimate the nationwide annual risk of transporting each product. The annual risk per car-mile (car-km) and per ton-mile (ton-km) was also calculated to enable comparison between chemicals and to provide information on the risk cost associated with shipments of these products. The analysis and the methodology provide a quantitative approach that will enable more effective management of the environmental risk of transporting hazardous materials. Published by Elsevier B.V. C1 [Saat, Mohd Rapik; Werth, Charles J.; Schaeffer, David; Barkan, Christopher P. L.] Univ Illinois, Dept Civil & Environm Engn, Newmark Civil Engn Lab 1243, Urbana, IL 61801 USA. [Yoon, Hongkyu] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Saat, MR (reprint author), Univ Illinois, Dept Civil & Environm Engn, Newmark Civil Engn Lab 1243, 205 North Mathews Ave, Urbana, IL 61801 USA. EM mohdsaat@illinois.edu FU Association of American Railroads FX The authors would like to thank the Association of American Railroads for their ongoing support of tank car safety and risk research in general, and this project in particular. The opinions expressed here do not necessarily represent the views of the AAR. NR 20 TC 9 Z9 9 U1 8 U2 62 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JAN 15 PY 2014 VL 264 BP 560 EP 569 DI 10.1016/j.jhazmat.2013.10.051 PG 10 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AA3UW UT WOS:000331021200066 PM 24239259 ER PT J AU Pakarinen, J He, L Gupta, M Gan, J Nelson, A El-Azab, A Allen, TR AF Pakarinen, J. He, L. Gupta, M. Gan, J. Nelson, A. El-Azab, A. Allen, T. R. TI 2.6 MeV proton irradiation effects on the surface integrity of depleted UO2 SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Uranium dioxide; Proton irradiation; Surface flaking; Crystal damage ID URANIUM-DIOXIDE; SINGLE-CRYSTALS; BURN-UP; DIFFUSION; HYDROGEN AB The effect of low temperature proton irradiation in depleted uranium dioxide was examined as a function of fluence. With 2.6 MeV protons, the fluence limit for preserving a good surface quality was found to be relatively low, about 1.4 and 7.0 x 10(17) protons/cm(2) for single and poly crystalline samples, respectively. Upon increasing the fluence above this threshold, severe surface flaking and disintegration of samples was observed. Based on scanning electron microscopy (SEM) and X-ray diffraction (XRD) observations the causes of surface failure were associated to high H atomic percent at the peak damage region due to low solubility of H in UO2. The resulting lattice stress is believed to exceed the fracture stress of the crystal at the observed fluencies. The oxygen point defects from the displacement damage may hinder the H diffusion and further increase the lattice stress, especially at the peak damage region. Published by Elsevier B.V. C1 [Pakarinen, J.; He, L.; Gupta, M.; Allen, T. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Gan, J.; Allen, T. R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Nelson, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [El-Azab, A.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. RP Pakarinen, J (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. EM pakarinen@wisc.edu OI Allen, Todd/0000-0002-2372-7259; He, Lingfeng/0000-0003-2763-1462 FU Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [FWP 1356] FX This work was supported as a part of the Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award number FWP 1356. NR 17 TC 5 Z9 5 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD JAN 15 PY 2014 VL 319 BP 100 EP 106 DI 10.1016/j.nimb.2013.11.014 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AA9QL UT WOS:000331427900018 ER PT J AU Aitken, ZH Jang, DC Weinberger, CR Greer, JR AF Aitken, Zachary H. Jang, Dongchan Weinberger, Christopher R. Greer, Julia R. TI Grain Boundary Sliding in Aluminum Nano-Bi-Crystals Deformed at Room Temperature SO SMALL LA English DT Article DE bicrystals; grain boundary; mechanical properties; nanopillar; aluminum ID DISLOCATION NUCLEATION; SINGLE-CRYSTALS; DEFORMATION; SIZE; NANOPILLARS; PLASTICITY; STRENGTH; BEHAVIOR; SCALE; AL AB Room-temperature uniaxial compressions of 900-nm-diameter aluminum bi-crystals, each containing a high-angle grain boundary with a plane normal inclined at 24 degrees to the loading direction, revealed frictional sliding along the boundary plane to be the dominant deformation mechanism. The top crystallite sheared off as a single unit in the course of compression instead of crystallographic slip and extensive dislocation activity, as would be expected. Compressive stress strain data of deforming nano bicrystals was continuous, in contrast to single crystalline nano structures that show a stochastic stress strain signature, and displayed a peak in stress at the elastic limit of approximate to 176 MPa followed by gradual softening and a plateau centered around approximate to 125 MPa. An energetics-based physical model, which may explain observed room-temperature grain boundary sliding, in presented, and observations are discussed within the framework of crystalline nano-plasticity and defect microstructure evolution. C1 [Aitken, Zachary H.; Jang, Dongchan; Greer, Julia R.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Weinberger, Christopher R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Aitken, ZH (reprint author), CALTECH, Div Engn & Appl Sci, 1200 E Calif Blvd, Pasadena, CA 91125 USA. EM zaitken@caltech.edu RI Jang, Dongchan/C-9510-2012 OI Jang, Dongchan/0000-0002-2814-9734 FU NSF through JRG's CAREER [DMR-1204864]; Office of Naval Research [N000140910883]; Sandia National Laboratories Truman Fellowship in National Security Science and Engineering; Sandia Corporation (a wholly owned subsidiary of Lockheed Martin Corporation); U.S. Department of Energy [DE-AC04-94AL85000] FX The authors gratefully acknowledge the financial support of NSF through JRG's CAREER Grant (DMR-1204864) and the Office of Naval Research (N000140910883). This research was supported in part by an appointment to the Sandia National Laboratories Truman Fellowship in National Security Science and Engineering, sponsored by Sandia Corporation (a wholly owned subsidiary of Lockheed Martin Corporation) as Operator of Sandia National Laboratories under its U.S. Department of Energy Contract No. DE-AC04-94AL85000. The authors also acknowledge the facilities and staff of the Kavli Nanoscience Institute at Caltech. NR 52 TC 8 Z9 8 U1 3 U2 35 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD JAN 15 PY 2014 VL 10 IS 1 BP 100 EP 108 DI 10.1002/smll.201301060 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 302SE UT WOS:000330624400012 PM 23873787 ER PT J AU Ulrich, LE Zhulin, IB AF Ulrich, Luke E. Zhulin, Igor B. TI SeqDepot: streamlined database of biological sequences and precomputed features SO BIOINFORMATICS LA English DT Article ID PROTEIN; PREDICTION; SIGNALP; DOMAINS AB Assembling and/or producing integrated knowledge of sequence features continues to be an onerous and redundant task despite a large number of existing resources. We have developed SeqDepot-a novel database that focuses solely on two primary goals: (i) assimilating known primary sequences with predicted feature data and (ii) providing the most simple and straightforward means to procure and readily use this information. Access to >28.5 million sequences and 300 million features is provided through a well-documented and flexible RESTful interface that supports fetching specific data subsets, bulk queries, visualization and searching by MD5 digests or external database identifiers. We have also developed an HTML5/JavaScript web application exemplifying how to interact with SeqDepot and Perl/Python scripts for use with local processing pipelines. C1 [Ulrich, Luke E.] Agile Genom LLC, Mt Pleasant, MI 29466 USA. [Ulrich, Luke E.; Zhulin, Igor B.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Zhulin, Igor B.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Ulrich, LE (reprint author), Agile Genom LLC, Mt Pleasant, MI 29466 USA. EM ulrich.luke_sci@gmail.com RI Zhulin, Igor/A-2308-2012 OI Zhulin, Igor/0000-0002-6708-5323 FU National Institutes of Health grant [GM072285] FX This work was supported in part by the National Institutes of Health grant [GM072285]. NR 17 TC 3 Z9 3 U1 1 U2 8 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 EI 1460-2059 J9 BIOINFORMATICS JI Bioinformatics PD JAN 15 PY 2014 VL 30 IS 2 BP 295 EP 297 DI 10.1093/bioinformatics/btt658 PG 3 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA 299YV UT WOS:000330432500023 PM 24234005 ER PT J AU Eudes, A Juminaga, D Baidoo, EEK Collins, FW Keasling, JD Loque, D AF Eudes, Aymerick Juminaga, Darmawi Baidoo, Edward E. K. Collins, F. William Keasling, Jay D. Loque, Dominique TI Production of hydroxycinnamoyl anthranilates from glucose in Escherichia coli (vol 12, 62, 2013) SO MICROBIAL CELL FACTORIES LA English DT Correction C1 [Eudes, Aymerick; Juminaga, Darmawi; Baidoo, Edward E. K.; Keasling, Jay D.; Loque, Dominique] Joint BioEnergy Inst, Oakland, CA 94608 USA. [Eudes, Aymerick; Keasling, Jay D.; Loque, Dominique] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Juminaga, Darmawi; Keasling, Jay D.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Juminaga, Darmawi; Keasling, Jay D.] Univ Calif Berkeley, Synthet Biol Inst, Berkeley, CA 94720 USA. [Collins, F. William] Agr & Agri Food Canada, Eastern Cereal & Oilseed Res Ctr, Ottawa, ON K1A 0C5, Canada. [Keasling, Jay D.] Univ Calif Berkeley, Dept Biomol & Chem Engn, Dept Bioengn, Berkeley, CA 94720 USA. RP Loque, D (reprint author), Joint BioEnergy Inst, Oakland, CA 94608 USA. EM dloque@lbl.gov RI Keasling, Jay/J-9162-2012; Loque, Dominique/A-8153-2008 OI Keasling, Jay/0000-0003-4170-6088; NR 2 TC 1 Z9 1 U1 0 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1475-2859 J9 MICROB CELL FACT JI Microb. Cell. Fact. PD JAN 15 PY 2014 VL 13 AR 8 DI 10.1186/1475-2859-13-8 PG 1 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 295UE UT WOS:000330140300001 ER PT J AU Xie, G Lo, CC Scholz, M Chain, PSG AF Xie, Gary Lo, Chien-Chi Scholz, Matthew Chain, Patrick S. G. TI Recruiting Human Microbiome Shotgun Data to Site-Specific Reference Genomes SO PLOS ONE LA English DT Article ID SKIN MICROBIOME; INTESTINAL MICROBIOTA; GUT MICROBIOME; DIVERSITY; COMMUNITY; ECOLOGY; CATALOG; TRACT; CORE AB The human body consists of innumerable multifaceted environments that predispose colonization by a number of distinct microbial communities, which play fundamental roles in human health and disease. In addition to community surveys and shotgun metagenomes that seek to explore the composition and diversity of these microbiomes, there are significant efforts to sequence reference microbial genomes from many body sites of healthy adults. To illustrate the utility of reference genomes when studying more complex metagenomes, we present a reference-based analysis of sequence reads generated from 55 shotgun metagenomes, selected from 5 major body sites, including 16 sub-sites. Interestingly, between 13% and 92% (62.3% average) of these shotgun reads were aligned to a then-complete list of 2780 reference genomes, including 1583 references for the human microbiome. However, no reference genome was universally found in all body sites. For any given metagenome, the body site-specific reference genomes, derived from the same body site as the sample, accounted for an average of 58.8% of the mapped reads. While different body sites did differ in abundant genera, proximal or symmetrical body sites were found to be most similar to one another. The extent of variation observed, both between individuals sampled within the same microenvironment, or at the same site within the same individual over time, calls into question comparative studies across individuals even if sampled at the same body site. This study illustrates the high utility of reference genomes and the need for further site-specific reference microbial genome sequencing, even within the already well-sampled human microbiome. C1 [Xie, Gary; Lo, Chien-Chi; Scholz, Matthew; Chain, Patrick S. G.] Los Alamos Natl Lab, Genome Sci Grp, Los Alamos, NM 87545 USA. [Xie, Gary; Lo, Chien-Chi; Scholz, Matthew; Chain, Patrick S. G.] Joint Genome Inst, Microbial & Metagenome Program, Walnut Creek, CA USA. RP Chain, PSG (reprint author), Los Alamos Natl Lab, Genome Sci Grp, Los Alamos, NM 87545 USA. EM pchain@lanl.gov OI Chain, Patrick/0000-0003-3949-3634; xie, gary/0000-0002-9176-924X FU National Institutes of Health [Y1-DE-6006-02]; U.S. Department of Energy (Office of Science) Joint Genome Institute [DE-AC02-05CH11231] FX This study was supported by grants from National Institutes of Health (Y1-DE-6006-02) and U.S. Department of Energy (Office of Science) Joint Genome Institute (DE-AC02-05CH11231). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 34 TC 2 Z9 2 U1 0 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 15 PY 2014 VL 9 IS 1 AR e84963 DI 10.1371/journal.pone.0084963 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 297DH UT WOS:000330235100044 PM 24454771 ER PT J AU Klippenstein, SJ Pande, VS Truhlar, DG AF Klippenstein, Stephen J. Pande, Vijay S. Truhlar, Donald G. TI Chemical Kinetics and Mechanisms of Complex Systems: A Perspective on Recent Theoretical Advances SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRANSITION-STATE THEORY; POTENTIAL-ENERGY SURFACES; DENSITY-FUNCTIONAL THEORY; PROTEIN-FOLDING KINETICS; ANHARMONIC VIBRATIONAL PROPERTIES; PHENOMENOLOGICAL RATE COEFFICIENTS; MASTER-EQUATION SIMULATION; MAIN-GROUP THERMOCHEMISTRY; STRAIGHT-LINE PATHS; AB-INITIO AB This Perspective presents a personal overview of the current status of the theory of chemical kinetics and mechanisms for complex processes. We attempt to assess the status of the field for reactions in the gas phase, at gas-solid interfaces, in liquid solutions, in enzymes, and for protein folding. Some unifying concepts such as potential energy surfaces, free energy, master equations, and reaction coordinates occur in more than one area. We hope this Perspective will be useful for highlighting recent advances and for identifying important areas for future research. C1 [Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Pande, Vijay S.] Stanford Univ, Dept Chem & Struct Biol, Stanford, CA 94305 USA. [Truhlar, Donald G.] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Truhlar, Donald G.] Univ Minnesota, Inst Supercomp, Minneapolis, MN 55455 USA. RP Truhlar, DG (reprint author), Univ Minnesota, Dept Chem, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM truhlar@umn.edu RI Truhlar, Donald/G-7076-2015; OI Truhlar, Donald/0000-0002-7742-7294; Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-86ER13579, DE-AC02-06CH11357] FX The authors are grateful to Yuri Georgievskii, Bill Green, Jeff Hammond, Amrit Jalan, Ahren Jasper, Geert-Jan Kroes, Larry Harding, Jim Miller, Karsten Reuter, Prasenjit Seal, Arthur Suits, Dave Thirumalai, Al Wagner, Ke Yang, Yan Zhao, and Jingjing Zheng for illuminating discussions or helpful suggestions and to Yan Zhao and Prasenjit Seal for providing Figures 2 and 3, respectively. This work was supported in part by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under grant no. DE-FG02-86ER13579 (D.G.T.) and under contract no. DE-AC02-06CH11357 (S.J.K.). NR 341 TC 56 Z9 56 U1 22 U2 206 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 15 PY 2014 VL 136 IS 2 BP 528 EP 546 DI 10.1021/ja408723a PG 19 WC Chemistry, Multidisciplinary SC Chemistry GA 294BY UT WOS:000330018600001 PM 24283502 ER PT J AU Vu, VV Beeson, WT Phillips, CM Cate, JHD Marletta, MA AF Vu, Van V. Beeson, William T. Phillips, Christopher M. Cate, Jamie H. D. Marletta, Michael A. TI Determinants of Regioselective Hydroxylation in the Fungal Polysaccharide Monooxygenases SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID GLYCOSIDE HYDROLASE FAMILY; NEUROSPORA-CRASSA; CELLOBIOSE DEHYDROGENASE; CELLULOSE DEGRADATION; HYDROLYSIS; ENZYMES AB The ubiquitous fungal polysaccharide monooxygenases (PMOs) (also known as GH61 proteins, LPMOs, and AA9 proteins) are structurally related but have significant variation in sequence. A heterologous expression method in Neurospora crassa was developed as a step toward connecting regioselectivity of the chemistry to PMO phylogeny. Activity assays, as well as sequence and phylogenetic analyses, showed that the majority of fungal PMOs fall into three major groups with distinctive active site surface features. PMO1s and PMO2s hydroxylate glycosidic positions C1 and C4, respectively. PMO3s hydroxylate both C1 and C4. A subgroup of PMO3s (PMO3*) hydroxylate C1. Mutagenesis studies showed that an extra subdomain of about 12 amino acids contribute to C4 oxidation in the PMO3 family. C1 [Vu, Van V.; Marletta, Michael A.] Scripps Res Inst, Dept Chem, La Jolla, CA 92037 USA. [Beeson, William T.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Phillips, Christopher M.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys Biosci, Berkeley, CA 94720 USA. RP Marletta, MA (reprint author), Scripps Res Inst, Dept Chem, La Jolla, CA 92037 USA. EM marletta@scripps.edu FU Energy Biosciences Institute; Scripps Research Institute FX We thank Elise Span and other Marietta group members for experimental support and helpful discussions. This work was funded by grants from the Energy Biosciences Institute to J.H.D.C. and M.A.M. and support from The Scripps Research Institute to M.A.M. NR 19 TC 40 Z9 40 U1 6 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 15 PY 2014 VL 136 IS 2 BP 562 EP 565 DI 10.1021/ja409384b PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 294BY UT WOS:000330018600006 PM 24350607 ER PT J AU Heims, F Pfaff, FF Abram, SL Farquhar, ER Bruschi, M Greco, C Ray, K AF Heims, Florian Pfaff, Florian Felix Abram, Sarah-Luise Farquhar, Erik R. Bruschi, Maurizio Greco, Claudio Ray, Kallol TI Redox Non-Innocence of a N-Heterocyclic Nitrenium Cation Bound to a Nickel-Cyclam Core SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID COUPLING REACTIONS; METAL-COMPLEXES; LIGANDS; REACTIVITY; CARBENES; IONS AB The redox properties of Ni complexes bound to a new ligand, [DMC-nit](+), where a N-heterocyclic nitrenium group is anchored on a 1,4,8,11-tetraazacyclotetradecane backbone, have been examined using spectroscopic and DFT methods. Ligand-based [(DMC-nit)Ni](2+/+) reduction and. metal-based [(DMC-nit)Ni](2+/3+) oxidation processes have been established for the [(DMC-nit)Ni](+/2+/3+) redox series, which represents the first examples of nitrenium nitrogen (N-nit)-bound first-row transition-metal complexes. An unprecedented bent binding mode of N-nit in [(DMC-nit)Ni](2+) is observed, which possibly results from the absence of any N-nit -> Ni sigma-donation. For the corresponding (DMC-nit)Ni(F)](2+) complex, sigma-donation is dominant, and hence a coplanar arrangement at N-nit is predicted by DFT. The binding of the triazolium ion to Ni enables new chemistry (formate oxidation) that is not observed in a derivative that lacks this functional group. Thus the N-heterocyclic nitrenium ligand is a potentially useful and versatile reagent in transition-metal-based catalysis. C1 [Heims, Florian; Pfaff, Florian Felix; Abram, Sarah-Luise; Ray, Kallol] Humboldt Univ, Inst Chem, D-12489 Berlin, Germany. [Farquhar, Erik R.] Case Western Reserve Univ, Ctr Synchrotron Biosci, Upton, NY 11973 USA. [Farquhar, Erik R.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Ctr Prote & Bioinformat, Upton, NY 11973 USA. [Bruschi, Maurizio; Greco, Claudio] Univ Milano Bicocca, Dept Earth & Environm Sci, I-20126 Milan, Italy. RP Ray, K (reprint author), Humboldt Univ, Inst Chem, Brook Taylor Str 2, D-12489 Berlin, Germany. EM kallol.ray@chemie.hu-berlin.de RI greco, claudio/H-7834-2015; OI greco, claudio/0000-0001-9628-7875; BRUSCHI, MAURIZIO/0000-0002-5709-818X FU Cluster of Excellence "Unifying Concepts in Catalysis", Berlin [EXC 314/1]; NIH [P30-EB-009998]; U.S. Department of Energy; BIG-NSE FX We dedicate this paper to Dr. Eckhard Bill on the occasion of his 60th birthday. We gratefully acknowledge financial support of this work from the Cluster of Excellence "Unifying Concepts in Catalysis" (EXC 314/1), Berlin. XAS data were obtained on NSLS beamline X3B (Brookhaven National Laboratory), with support from NIH Grant P30-EB-009998 and the U.S. Department of Energy. F.H. thanks BIG-NSE for a scholarship. We also thank Corinna Matlachowski for help with GC experiments. NR 26 TC 6 Z9 6 U1 4 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 15 PY 2014 VL 136 IS 2 BP 582 EP 585 DI 10.1021/ja4099559 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 294BY UT WOS:000330018600011 PM 24380589 ER PT J AU Knorowski, C Travesset, A AF Knorowski, Christopher Travesset, Alex TI Self-Assembly and Crystallization of Hairy (f-Star) and DNA-Grafted Nanocubes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; PROGRAMMABLE NANOPARTICLE CRYSTALLIZATION; GRAPHICS PROCESSING UNITS; ORIENTATIONAL ORDER; BUILDING-BLOCKS; SUPERLATTICES; BEHAVIOR AB Nanoparticle superlattices are key to realizing many of the materials that will solve current technological challenges. Particularly important for their optical, mechanical or catalytic properties are superlattices of anisotropic (non-spherical) nanoparticles. The key challenge is how to program anisotropic nanoparticles to self-assemble into the relevant structures. In this Article, using numerical simulations, we show that "hairy" (f-star) or DNA grafted on nanocubes provides a general framework to direct the self-assembly into phases with crystalline, liquid crystalline, rotator, or noncrystalline phases with both long-range positional and orientational order. We discuss the relevance of these phases for engineering nanomaterials or micromaterials displaying precise orientational order, realization of dry superlattices as well as for the field of programmed self-assembly of anisotropic nanoparticles in general. C1 [Knorowski, Christopher] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Knorowski, C (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM cdknorow@iastate.edu FU U.S. DOE through the Ames Laboratory [DE-AC02-07CH11358] FX We acknowledge discussions and interest with R. Kamien and O. Gang. We also thank J. Anderson for help with HOOMD-blue as well as Martin Bertrand for help with the Berendsen thermostat. This work is funded by the U.S. DOE through the Ames Laboratory under Contract DE-AC02-07CH11358. NR 35 TC 12 Z9 12 U1 2 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 15 PY 2014 VL 136 IS 2 BP 653 EP 659 DI 10.1021/ja406241n PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 294BY UT WOS:000330018600029 PM 24325673 ER PT J AU Lee, K Isley, WC Dzubak, AL Verma, P Stoneburner, SJ Lin, LC Howe, JD Bloch, ED Reed, DA Hudson, MR Brown, CM Long, JR Neaton, JB Smit, B Cramer, CJ Truhlar, DG Gagliardi, L AF Lee, Kyuho Isley, William C., III Dzubak, Allison L. Verma, Pragya Stoneburner, Samuel J. Lin, Li-Chiang Howe, Joshua D. Bloch, Eric D. Reed, Douglas A. Hudson, Matthew R. Brown, Craig M. Long, Jeffrey R. Neaton, Jeffrey B. Smit, Berend Cramer, Christopher J. Truhlar, Donald G. Gagliardi, Laura TI Design of a Metal-Organic Framework with Enhanced Back Bonding for Separation of N-2 and CH4 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON(II) COORDINATION SITES; MAIN-GROUP THERMOCHEMISTRY; DENSITY-FUNCTIONAL THEORY; NONCOVALENT INTERACTIONS; ELECTRONIC-STRUCTURE; CARBON-DIOXIDE; ADSORPTION; CHEMISTRY; TEMPERATURE; KINETICS AB Gas separations with porous materials are economically important and provide a unique challenge to fundamental materials design, as adsorbent properties can be altered to achieve selective gas adsorption. Metal organic. frameworks represent a rapidly expanding new class of porous adsorbents with a large range of possibilities for designing materials with desired functionalities. Given the large number of possible, framework structures, quantum mechanical computations can provide useful guidance in prioritizing the synthesis of the most useful materials for a given, application. Here, we show that such calculations can predict a new metal-organic framework of potential utility for separation of dinitrogen from methane, a particularly challenging separation of critical value for utilizing natural gas. An open V(II) site incorporated into a metal-organic framework can provide a material with a considerably higher methane, based on strong selective back bonding with the former but not the enthalpy of adsorption for dinitrogen latter. C1 [Lee, Kyuho; Lin, Li-Chiang; Howe, Joshua D.; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Lee, Kyuho; Isley, William C., III; Dzubak, Allison L.; Verma, Pragya; Stoneburner, Samuel J.; Lin, Li-Chiang; Howe, Joshua D.; Bloch, Eric D.; Long, Jeffrey R.; Neaton, Jeffrey B.; Smit, Berend; Cramer, Christopher J.; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Nanoporous Mat Genome Ctr, Minneapolis, MN 55455 USA. [Lee, Kyuho; Howe, Joshua D.; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Isley, William C., III; Dzubak, Allison L.; Verma, Pragya; Stoneburner, Samuel J.; Cramer, Christopher J.; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Chem Theory Ctr, Dept Chem, Minneapolis, MN 55455 USA. [Isley, William C., III; Dzubak, Allison L.; Verma, Pragya; Stoneburner, Samuel J.; Cramer, Christopher J.; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. [Reed, Douglas A.; Long, Jeffrey R.; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hudson, Matthew R.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Long, Jeffrey R.; Neaton, Jeffrey B.; Smit, Berend] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Minnesota, Nanoporous Mat Genome Ctr, 207 Pleasant St Southeast, Minneapolis, MN 55455 USA. EM jrlong@berkeley.edu; jbneaton@lbl.gov; berend-smit@berkeley.edu; cramer@umn.edu; truhlar@umn.edu; gagliard@umn.edu RI Lee, Kyuho/B-9370-2008; Smit, Berend/B-7580-2009; Lin, Li-Chiang/J-8120-2014; Brown, Craig/B-5430-2009; Truhlar, Donald/G-7076-2015; Cramer, Christopher/B-6179-2011; Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; OI Lee, Kyuho/0000-0001-9325-3717; Smit, Berend/0000-0003-4653-8562; Brown, Craig/0000-0002-9637-9355; Truhlar, Donald/0000-0002-7742-7294; Cramer, Christopher/0000-0001-5048-1859; Neaton, Jeffrey/0000-0001-7585-6135; Lin, Li-Chiang/0000-0002-2821-9501; Isley, William/0000-0002-1887-1221 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-12ER16362]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DEAC02-05CH11231]; Kenneth E. and Marion S. Owens Endowed Fellowship; Louise T. Dosdall Fellowship; NIST NRC; Gerald K. Branch fellowship; Phillips 66 Departmental Excellence Fellowship FX We gratefully acknowledge Xuefei Xu, Joshua Borycz, Remi Maurice, Robert Berger, Roberta Poloni, James Phillips, and Pere Miro for helpful discussions. This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under award DE-FG02-12ER16362. Portions of this work were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DEAC02-05CH11231. Portions of the computations were performed using NERSC. W.C.I. is grateful for a Kenneth E. and Marion S. Owens Endowed Fellowship. A.L.D. is grateful for support through the Louise T. Dosdall Fellowship. M.R.H. acknowledges the NIST NRC Postdoctoral Fellowship research program for support. E.D.B. was supported by a Gerald K. Branch fellowship in chemistry. P.V. acknowledges a Phillips 66 Departmental Excellence Fellowship. NR 46 TC 55 Z9 57 U1 13 U2 177 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 15 PY 2014 VL 136 IS 2 BP 698 EP 704 DI 10.1021/ja4102979 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 294BY UT WOS:000330018600034 PM 24313689 ER PT J AU Howes, SC Alushin, GM Shida, T Nachury, MV Nogales, E AF Howes, Stuart C. Alushin, Gregory M. Shida, Toshinobu Nachury, Maxence V. Nogales, Eva TI Effects of tubulin acetylation and tubulin acetyltransferase binding on microtubule structure SO MOLECULAR BIOLOGY OF THE CELL LA English DT Article ID CHLAMYDOMONAS ALPHA-TUBULIN; POSTTRANSLATIONAL MODIFICATIONS; RESOLUTION STRUCTURE; ELECTRON-MICROSCOPY; PURIFIED TUBULIN; MAMMALIAN-CELLS; DEACETYLASE; PROTEIN; MEC-17; VISUALIZATION AB Tubulin undergoes posttranslational modifications proposed to specify microtubule subpopulations for particular functions. Most of these modifications occur on the C-termini of tubulin and may directly affect the binding of microtubule-associated proteins (MAPs) or motors. Acetylation of Lys-40 on alpha-tubulin is unique in that it is located on the luminal surface of microtubules, away from the interaction sites of most MAPs and motors. We investigate whether acetylation alters the architecture of microtubules or the conformation of tubulin, using cryo-electron microscopy (cryo-EM). No significant changes are observed based on protofilament distributions or microtubule helical lattice parameters. Furthermore, no clear differences in tubulin structure are detected between cryo-EM reconstructions of maximally deacetylated or acetylated microtubules. Our results indicate that the effect of acetylation must be highly localized and affect interaction with proteins that bind directly to the lumen of the microtubule. We also investigate the interaction of the tubulin acetyltransferase, alpha TAT1, with microtubules and find that alpha TAT1 is able to interact with the outside of the microtubule, at least partly through the tubulin C-termini. Binding to the outside surface of the microtubule could facilitate access of alpha TAT1 to its luminal site of action if microtubules undergo lateral opening between protofilaments. C1 [Howes, Stuart C.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Alushin, Gregory M.; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Alushin, Gregory M.; Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Shida, Toshinobu; Nachury, Maxence V.] Stanford Sch Med, Dept Mol & Cellular Physiol, Stanford, CA 94305 USA. [Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. EM enogales@lbl.gov RI Nachury, Maxence/A-8759-2008 OI Nachury, Maxence/0000-0003-4918-1562 FU National Institute of General Medical Sciences [P01GM051487, R01GM089933] FX We thank Erik Jonsson and Ronald Vale (Department of Cellular and Molecular Pharmacology and Howard Hughes Medical Institute, University of California, San Francisco, San Francisco, CA) for the generous gift of monomeric kinesin protein and expression plasmids. We also thank Gabriel Lander and Tom Houweling for computer support and Patricia Grob and Gigi Kemalyan for maintenance of the electron microscope facility. This work was supported by National Institute of General Medical Sciences Grants P01GM051487 to E.N. and R01GM089933 to M.V.N. E.N. is a Howard Hughes Medical Institute Investigator. NR 61 TC 40 Z9 42 U1 1 U2 25 PU AMER SOC CELL BIOLOGY PI BETHESDA PA 8120 WOODMONT AVE, STE 750, BETHESDA, MD 20814-2755 USA SN 1059-1524 EI 1939-4586 J9 MOL BIOL CELL JI Mol. Biol. Cell PD JAN 15 PY 2014 VL 25 IS 2 BP 257 EP 266 DI 10.1091/mbc.E13-07-0387 PG 10 WC Cell Biology SC Cell Biology GA 294DP UT WOS:000330022900005 PM 24227885 ER PT J AU Wang, YS Wen, MX Kwon, Y Xu, YY Liu, YY Zhang, PJ He, XQ Wang, Q Huang, YR Jen, KY LaBarge, MA You, L Kogan, SC Gray, JW Mao, JH Wei, GW AF Wang, Yunshan Wen, Mingxin Kwon, Yongwon Xu, Yangyang Liu, Yueyong Zhang, Pengju He, Xiuquan Wang, Qin Huang, Yurong Jen, Kuang-Yu LaBarge, Mark A. You, Liang Kogan, Scott C. Gray, Joe W. Mao, Jian-Hua Wei, Guangwei TI CUL4A Induces Epithelial-Mesenchymal Transition and Promotes Cancer Metastasis by Regulating ZEB1 Expression SO CANCER RESEARCH LA English DT Article ID COMPARATIVE GENOMIC HYBRIDIZATION; NEGATIVE BREAST-CANCER; HUMAN HOMOLOG; MOLECULAR RECOGNITION; HISTONE H3; GENE; AMPLIFICATION; CARCINOMA; WDR5; OVEREXPRESSION AB The ubiquitin ligase CUL4A has been implicated in tumorigenesis, but its contributions to progression and metastasis have not been evaluated. Here, we show that CUL4A is elevated in breast cancer as well as in ovarian, gastric, and colorectal tumors in which its expression level correlates positively with distant metastasis. CUL4A overexpression in normal or malignant human mammary epithelial cells increased their neoplastic properties in vitro and in vivo, markedly increasing epithelial-mesenchymal transition (EMT) and the metastatic capacity of malignant cells. In contrast, silencing CUL4A in aggressive breast cancer cells inhibited these processes. Mechanistically, we found that CUL4A modulated histone H3K4me3 at the promoter of the EMT regulatory gene ZEB1 in a manner associated with its transcription. ZEB1 silencing blocked CUL4A-driven proliferation, EMT, tumorigenesis, and metastasis. Furthermore, in human breast cancers, ZEB1 expression correlated positively with CUL4A expression and distant metastasis. Taken together, our findings reveal a pivotal role of CUL4A in regulating the metastatic behavior of breast cancer cells. C1 [Wang, Yunshan; Wen, Mingxin; Xu, Yangyang; He, Xiuquan; Wei, Guangwei] Shandong Univ, Sch Med, Dept Human Anat, Jinan 250012, Shandong, Peoples R China. [Wang, Yunshan; Wen, Mingxin; Xu, Yangyang; He, Xiuquan; Wei, Guangwei] Shandong Univ, Sch Med, Key Lab Expt Teratol, Minist Educ, Jinan 250012, Shandong, Peoples R China. [Zhang, Pengju] Shandong Univ, Sch Med, Dept Biochem & Mol Biol, Jinan 250012, Shandong, Peoples R China. [Wang, Qin] Shandong Univ, Qilu Hosp, Dept Resp Med, Jinan 250100, Peoples R China. [Wang, Yunshan] Shandong Univ, Sch Ocean, Int Biotechnol R&D Ctr, Weihai, Shandong, Peoples R China. [Kwon, Yongwon; Liu, Yueyong; Huang, Yurong; LaBarge, Mark A.; Mao, Jian-Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Jen, Kuang-Yu] Univ Calif San Francisco, Dept Pathol, San Francisco, CA 94140 USA. [You, Liang] Univ Calif San Francisco, Dept Surg, Thorac Oncol Lab, San Francisco, CA 94143 USA. [Kogan, Scott C.] Univ Calif San Francisco, Helen Diller Family Comprehens Canc Ctr, San Francisco, CA 94143 USA. [Kogan, Scott C.] Univ Calif San Francisco, Dept Lab Med, San Francisco, CA 94143 USA. [Gray, Joe W.] Oregon Hlth & Sci Univ, Dept Biomed Engn, Portland, OR 97201 USA. RP Wei, GW (reprint author), Shandong Univ, Sch Med, Dept Human Anat, 44 Wenhua Xi Rd, Jinan 250012, Shandong, Peoples R China. EM JHMao@lbl.gov; gwwei@yahoo.com FU National Natural Science Foundation of China [81172528, 31271461]; Doctoral Fund of Ministry of Education of China [20110131110035]; Natural Science Foundation of Shandong Province [ZR2011HM034]; Taishan Scholar Program of Shandong Province; NIH, National Cancer Institute [R01 CA116481]; Low Dose Scientific Focus Area, Office of Biological and Environmental Research, U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Natural Science Foundation of China (grant nos. 81172528 and 31271461), the Doctoral Fund of Ministry of Education of China (grant 20110131110035), the Natural Science Foundation of Shandong Province (grant ZR2011HM034), and the Taishan Scholar Program of Shandong Province (G. Wei); the NIH, National Cancer Institute grant R01 CA116481, and Low Dose Scientific Focus Area, Office of Biological and Environmental Research, U.S. Department of Energy (DE-AC02-05CH11231; J.-H. Mao). NR 33 TC 74 Z9 76 U1 1 U2 15 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD JAN 15 PY 2014 VL 74 IS 2 BP 520 EP 531 DI 10.1158/0008-5472.CAN-13-2182 PG 12 WC Oncology SC Oncology GA 294HB UT WOS:000330034200012 PM 24305877 ER PT J AU Peterson, GW DeCoste, JB Fatollahi-Fard, F Britt, DK AF Peterson, Gregory W. DeCoste, Jared B. Fatollahi-Fard, Farzin Britt, David K. TI Engineering UiO-66-NH2 for Toxic Gas Removal SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID METAL-ORGANIC FRAMEWORKS; ADSORPTION PROPERTIES; COMBINATORIAL METHODS; POSTSYNTHETIC LIGAND; CYANOGEN CHLORIDE; BUILDING UNIT; HIGH-CAPACITY; STABILITY; FUNCTIONALIZATION; AMMONIA AB The metal organic framework UiO-66-NH2 was synthesized in a scaled batch of approximately 100 g. The material was then pressed into small pellets at pressures ranging from 5000 to 100000 psi to determine the effects on porosity and crystal structure. Nitrogen isotherm data and powder X-ray diffraction data indicate that the structure remains intact up to 25000 psi, with only a slight decrease in surface area. The structure exhibits significant degradation at pressures above 25000 psi. Subsequently, the powder was pressed at 5000 psi and then crushed and sieved into 20 X 40 mesh granules for evaluation against ammonia and cyanogen chloride in a breakthrough system simulating individual protection filters and respirator cartridges. The MOF showed capacity similar to that of a broad-spectrum carbon for both ammonia and cyanogen chloride; however, the breakthrough times, especially for cyanogen chloride, were dramatically reduced, likely as a result of mass-transfer limitations from the completely microporous MOF. C1 [Peterson, Gregory W.] Edgewood Chem Biol Ctr, Aberdeen Proving Ground, MD 21010 USA. [DeCoste, Jared B.] Leidos Inc, Gunpowder, MD 21010 USA. [Fatollahi-Fard, Farzin; Britt, David K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Peterson, GW (reprint author), Edgewood Chem Biol Ctr, 5183 Blackhawk Rd, Aberdeen Proving Ground, MD 21010 USA. EM gregory.w.peterson.civ@mail.mil RI Britt, David/D-4675-2009; Foundry, Molecular/G-9968-2014; OI Fatollahi-Fard, Farzin/0000-0003-0744-9196; Peterson, Gregory/0000-0003-3467-5295 FU Defense Threat Reduction Agency (DTRA) Project [BA07PRO104] FX This work was completed under Defense Threat Reduction Agency (DTRA) Project BA07PRO104. The authors thank Paulette Jones, Amedeo Napolitano, and Matt Browe for running the breakthrough experiments and Bryan Schindler for providing nitrogen isotherm data. The authors also thank 3M for providing broad spectrum carbon. NR 37 TC 21 Z9 21 U1 15 U2 151 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JAN 15 PY 2014 VL 53 IS 2 BP 701 EP 707 DI 10.1021/ie403366d PG 7 WC Engineering, Chemical SC Engineering GA 294BX UT WOS:000330018500024 ER PT J AU Altmannshofer, W Bauer, M Carena, M AF Altmannshofer, Wolfgang Bauer, Martin Carena, Marcela TI Exotic leptons: Higgs, flavor and collider phenomenology SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Beyond Standard Model; CP violation ID RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; STANDARD MODEL; ATLAS DETECTOR; PP COLLISIONS; ROOT-S=7 TEV; BOSON; SEARCH; LHC; CONVERSION AB We study extensions of the standard model by one generation of vector-like leptons with non-standard hypercharges, which allow for a sizable modification of the h -> gamma gamma decay rate for new lepton masses in the 300 GeV-1 TeV range. We analyze vacuum stability implications for different hypercharges. Effects in h -> Z gamma are typically much smaller than in h -> gamma gamma, but distinct among the considered hypercharge assignments. Non-standard hypercharges constrain or entirely forbid possible mixing operators with standard model leptons. As a consequence, the leading contributions to the experimentally strongly constrained electric dipole moments of standard model fermions are only generated at the two loop level by the new CP violating sources of the considered setups. We derive the bounds from dipole moments, electro-weak precision observables and lepton flavor violating processes, and discuss their implications. Finally, we examine the production and decay channels of the vector-like leptons at the LHC, and find that signatures with multiple light leptons or taus are already probing interesting regions of parameter space. C1 [Altmannshofer, Wolfgang; Bauer, Martin; Carena, Marcela] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Bauer, Martin; Carena, Marcela] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carena, Marcela] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Altmannshofer, W (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM waltmann@fnal.gov; martinbauer@uchicago.edu; carena@fnal.gov FU National Science Foundation [NSF PHY11-25915]; United States Department of Energy [De-AC02-07CH11359]; Alexander von Humboldt Foundation; Perimeter Institute for Theoretical Physics; Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Economic Development Innovation FX We would like to thank Prateek Agrawal, Stefania Gori, Aurelio Juste, Matthias Neubert, Pedro Schwaller, Carlos Wagner, Lian Tao Wang, and Felix Yu for many useful discussions. We also thank David Straub for useful comments. We would like to thank KITP Santa Barbara for warm hospitality and support during completion of this work. KITP is supported in part by the National Science Foundation under Grant No. NSF PHY11-25915. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. One of us, M. B., is acknowledging the support of the Alexander von Humboldt Foundation. The research of W. A. was supported in part by Perimeter Institute for Theoretical Physics. Research at Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Economic Development & Innovation. NR 94 TC 0 Z9 0 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 15 PY 2014 IS 1 DI 10.1007/JHEP01(2014)060 PG 39 WC Physics, Particles & Fields SC Physics GA 294FD UT WOS:000330027600001 ER PT J AU Zhu, JL Zhang, JZ Xu, HW Vogel, SC Jin, CQ Frantti, J Zhao, YS AF Zhu, Jinlong Zhang, Jianzhong Xu, Hongwu Vogel, Sven C. Jin, Changqing Frantti, Johannes Zhao, Yusheng TI Pressure-induced reversal between thermal contraction and expansion in ferroelectric PbTiO3 SO SCIENTIFIC REPORTS LA English DT Article ID PHASE-TRANSITION; MATERIALS SCIENCE; ZERO-EXPANSION; LEAD TITANATE; X-RAY; PEROVSKITES; TEMPERATURES; STRESS; OXIDES AB Materials with zero/near zero thermal expansion coefficients are technologically important for applications in thermal management and engineering. To date, this class of materials can only be produced by chemical routes, either by changing chemical compositions or by composting materials with positive and negative thermal expansion. Here, we report for the first time a physical route to achieve near zero thermal expansion through application of pressure. In the stability field of tetragonal PbTiO3 we observed pressure-induced reversals between thermal contraction and expansion between ambient pressure and 0.9 GPa. This hybrid behavior leads to a mathematically infinite number of crossover points in the pressure-volume-temperature space and near-zero thermal expansion coefficients comparable to or even smaller than those attained by chemical routes. The observed pressures for this unusual phenomenon are within a small range of 0.1-0.9 GPa, potentially feasible for designing stress-engineered materials, such as thin films and nano-crystals, for thermal management applications. C1 [Zhu, Jinlong; Zhang, Jianzhong; Vogel, Sven C.] Los Alamos Natl Lab, LANSCE, Los Alamos, NM 87545 USA. [Xu, Hongwu] Los Alamos Natl Lab, EES Div, Los Alamos, NM 87545 USA. [Zhu, Jinlong; Jin, Changqing; Zhao, Yusheng] Chinese Acad Sci, Inst Phys, Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Frantti, Johannes] Aalto Univ, Sch Sci, Dept Appl Phys, FI-00076 Aalto, Finland. [Zhao, Yusheng] Univ Nevada, Dept Phys & Astron, HiPSEC, Las Vegas, NV 89154 USA. RP Xu, HW (reprint author), Los Alamos Natl Lab, EES Div, POB 1663, Los Alamos, NM 87545 USA. EM hxu@lanl.gov; jin@iphy.ac.cn; Yusheng.Zhao@unlv.edu OI Xu, Hongwu/0000-0002-0793-6923; Zhang, Jianzhong/0000-0001-5508-1782; Vogel, Sven C./0000-0003-2049-0361 FU Los Alamos National Security LLC under DOE [DE-AC52-06NA25396]; NSF MOST of China; U.S. Department of Energy's Office of Basic Energy Sciences FX This work was supported by the laboratory-directed research and development (LDRD) program of Los Alamos National Laboratory, which is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. The experimental work has benefited from the use of the Lujan Neutron Scattering Center at Los Alamos Neutron Science Center, which is funded by the U.S. Department of Energy's Office of Basic Energy Sciences. We also acknowledge the support from NSF & MOST of China through research projects. NR 40 TC 7 Z9 7 U1 3 U2 65 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 15 PY 2014 VL 4 AR 3700 DI 10.1038/srep03700 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RP UT WOS:000329847100008 PM 24424396 ER PT J AU Han, WZ Cerreta, EK Mara, NA Beyerlein, IJ Carpenter, JS Zheng, SJ Trujillo, CP Dickerson, PO Misra, A AF Han, W. Z. Cerreta, E. K. Mara, N. A. Beyerlein, I. J. Carpenter, J. S. Zheng, S. J. Trujillo, C. P. Dickerson, P. O. Misra, A. TI Deformation and failure of shocked bulk Cu-Nb nanolaminates SO ACTA MATERIALIA LA English DT Article DE Shock wave; Cu-Nb nanolaminates; Voids; Spall; Interface ID SEVERE PLASTIC-DEFORMATION; ULTRA-HIGH STRENGTH; INTERFACE STRUCTURE; BIMETAL INTERFACES; TEXTURE EVOLUTION; COMPOSITES; COMPRESSION; COPPER; ORIENTATION; ALUMINUM AB The deformation and failure of bulk Cu-Nb nanocomposites with a nominal layer thickness of 135 nm was investigated under planar shock loading. It was observed that little substructural evolution was evident after shock compression to a peak stress of 7 GPa, while specimens were fully spalled after loading to 7 GPa under free surface conditions. In these fully spalled specimens, the characteristics of ductile failure that formed on the fracture surface were dependent upon the processing route of the nanocomposite. Specifically, process-induced grain-shape differences due to dissimilar rolling passes are linked with differences in the failure response. In addition, incipient failure was also observed. Numerous nanovoids, 20 nm or less in size, nucleated and aligned in a row in the middle of Cu layers. Due to the reflection of the shock wave at the Cu-Nb interfaces, incipient voids tend to nucleate within the Cu phase, which has a higher impedance and lower spall strength than Nb. This occurs rather than nucleation along the Cu-Nb interfaces or in the Nb phase. This finding contradicts the general thinking of failure starting from interfaces, and indicates that the Cu-Nb interfaces are stable under dynamic loading. It is postulated that numerous voids nucleate in the Cu layers under shock loading, then lead to failure through their growth and coalescence. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Han, W. Z.; Cerreta, E. K.; Mara, N. A.; Beyerlein, I. J.; Carpenter, J. S.; Zheng, S. J.; Trujillo, C. P.; Dickerson, P. O.; Misra, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Han, WZ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM wzhanmail@gmail.com RI zheng, shijian/F-2453-2012; Han, Weizhong/C-9963-2011; Mara, Nathan/J-4509-2014; Misra, Amit/H-1087-2012; Beyerlein, Irene/A-4676-2011; OI Carpenter, John/0000-0001-8821-043X FU National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; Center for Materials in Irradiation and Mechanical Extremes (CMIME); Energy Frontier Research Center (EFRC); US Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL 1026] FX Los Alamos National Laboratory is operated by LANS, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract DE-AC52-06NA25396. This work was supported by the Center for Materials in Irradiation and Mechanical Extremes (CMIME), an Energy Frontier Research Center (EFRC) funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. 2008LANL 1026. NR 50 TC 23 Z9 23 U1 5 U2 83 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JAN 15 PY 2014 VL 63 BP 150 EP 161 DI 10.1016/j.actamat.2013.10.019 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 287OM UT WOS:000329552100014 ER PT J AU Knezevic, M Carpenter, JS Lovato, ML McCabe, RJ AF Knezevic, Marko Carpenter, John S. Lovato, Manuel L. McCabe, Rodney J. TI Deformation behavior of the cobalt-based superalloy Haynes 25: Experimental characterization and crystal plasticity modeling SO ACTA MATERIALIA LA English DT Article DE Cobalt-based superalloys; TEM; EBSD; Texture; Constitutive modeling ID MAGNESIUM SINGLE CRYSTALS; STRAIN-PATH CHANGES; POLYCRYSTAL PLASTICITY; MECHANICAL RESPONSE; TEXTURE EVOLUTION; ALPHA-URANIUM; MICROSTRUCTURE; METALS; ALLOYS; SLIP AB The deformation behavior of a wrought, cobalt-based superalloy, Haynes 25, was studied using a combination of experimental techniques and crystal plasticity modeling. The microstructure was examined by transmission electron microscopy and electron backscattered diffraction to determine the deformation and hardening mechanisms contributing to the mechanical behavior of the alloy. A high density of stacking faults within the grains, consistent with planar glide, was found to be the predominant defect mechanism with no evidence of deformation twinning observed. A strain-rate and temperature-sensitive hardening law that includes effects of planar glide was developed for the material and implemented in a self-consistent homogenization scheme. The hardening of individual crystals is based on the evolution of dislocation densities per plane and includes the effects of strain rate and temperature through thermally activated recovery and dislocation interactions. The model is validated on a comprehensive set of compression tests performed at temperatures ranging from 298 to 673 K and strain rates ranging from 10(-3) to 2600 s(-1) and found capable of reproducing the stress-strain response and texture for all tests with a unique set of single-crystal hardening parameters. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Knezevic, Marko] Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. [Carpenter, John S.; Lovato, Manuel L.; McCabe, Rodney J.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. EM marko.knezevic@unh.edu OI McCabe, Rodney /0000-0002-6684-7410; Carpenter, John/0000-0001-8821-043X FU Seaborg Institute; US Department of Energy [DE-AC52-06NA25396] FX M.K. acknowledges the Seaborg Institute for partial financial support under a Post-Doctoral Fellowship through the LANL LDRD Program. Daniel Martinez performed the high-rate dynamic testing and Pallas Papin prepared the TEM foils. The work was supported by the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 30 TC 31 Z9 31 U1 2 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JAN 15 PY 2014 VL 63 BP 162 EP 168 DI 10.1016/j.actamat.2013.10.021 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 287OM UT WOS:000329552100015 ER PT J AU Yang, SH Ramirez-Cuesta, AJ Schroder, M AF Yang, Sihai Ramirez-Cuesta, Anibal J. Schroeder, Martin TI Inelastic neutron scattering study of binding of para-hydrogen in an ultra-microporous metal-organic framework SO CHEMICAL PHYSICS LA English DT Article DE Metal organic framework; Hydrogen adsorption; Inelastic neutron scattering; Neutron spectroscopy; Binding interaction ID ALUMINUM PYROMELLITATE; SORPTION PROPERTIES; CARBON-DIOXIDE; ADSORPTION; STORAGE; MIL-53; SITES; H-2; DIFFRACTION; CAPACITIES AB Metal-organic framework (MOF) materials show promise for H-2 storage and it is widely predicted by computational modelling that MOFs incorporating ultra-micropores are optimal for H-2 binding due to enhanced overlapping potentials. We report the investigation using inelastic neutron scattering of the interaction of H-2 in an ultra-microporous MOF material showing low H-2 uptake capacity. The study has revealed that adsorbed H-2 at 5 K has a liquid recoil motion along the channel with very little interaction with the MOF host, consistent with the observed low uptake. The low H-2 uptake is not due to incomplete activation or decomposition as the desolvated MOF shows CO2 uptake with a measured pore volume close to that of the single crystal pore volume. This study represents a unique example of surprisingly low H-2 uptake within a MOF material, and complements the wide range of studies on systems showing higher uptake capacities and binding interactions. (C) 2013 The Authors. Published by Elsevier B.V. All rights reserved. C1 [Yang, Sihai; Schroeder, Martin] Univ Nottingham, Sch Chem, Nottingham NG7 2RD, England. [Ramirez-Cuesta, Anibal J.] Rutherford Appleton Lab, ISIS Facil, Chilton OX11 0QX, Oxon, England. [Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Yang, SH (reprint author), Univ Nottingham, Sch Chem, Univ Pk, Nottingham NG7 2RD, England. EM Sihai.Yang@nottingham.ac.uk; M.Schroder@nottingham.ac.uk RI Schroder, Martin/I-5432-2013; Ramirez-Cuesta, Timmy/A-4296-2010 OI Schroder, Martin/0000-0001-6992-0700; Ramirez-Cuesta, Timmy/0000-0003-1231-0068 FU Leverhulme Trust Early Career Research Fellowship; Nottingham Research Fellowship; ERC; EPSRC FX SY gratefully acknowledges receipt of a Leverhulme Trust Early Career Research Fellowship and a Nottingham Research Fellowship, and MS receipt of an ERC Advanced Grant and EPSRC Programme Grant. We are especially grateful to the STFC ISIS Neutron Facility for access to the TOSCA Beamline. We thank the user support group at ISIS (Chris Goodway and Mark Kibble) for the technical help at TOSCA beamline. NR 32 TC 5 Z9 5 U1 4 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD JAN 15 PY 2014 VL 428 BP 111 EP 116 DI 10.1016/j.chemphys.2013.11.004 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 287XA UT WOS:000329574400015 ER PT J AU Loukonen, V Kuo, IFW McGrath, MJ Vehkamaki, H AF Loukonen, V. Kuo, I-F. W. McGrath, M. J. Vehkamaki, H. TI On the stability and dynamics of (sulfuric acid) (ammonia) and (sulfuric acid) (dimethylamine) clusters: A first-principles molecular dynamics investigation SO CHEMICAL PHYSICS LA English DT Article DE Weakly bound molecular clusters; First-principles molecular dynamics; Electric dipole moment; Sulfuric acid; Atmospheric new-particle formation ID PARTICLE FORMATION EVENTS; ATMOSPHERIC PARTICLES; AEROSOL FORMATION; NUCLEATION; WATER; AMINE; RATES; NANOPARTICLES; CHEMISTRY; EXCHANGE AB The main pathway of new-particle formation in the atmosphere is likely to begin from small sulfuric acid clusters stabilized by other compounds, such as ammonia or amines. Here, we present the results of first-principles molecular dynamics simulations probing the stability and dynamics of (sulfuric acid)(ammonia/dimethylamine) clusters with two, three and four sulfuric acid molecules and a varying number of the bases. In each of the eight simulated clusters, an energetic equilibrium was reached and 35 ps of equilibrium data was collected in the NVT (T = 300 K) ensemble. The clusters exhibited pronounced thermal motion including rotations of the molecules within the clusters. Regardless of the continuous movement, the clusters stayed bound together. The calculated electric dipole moments were found to be sensitive to the thermal motion and consequently, large fluctuations were observed. In addition, the vibrational spectra for all the clusters were determined, indicating that the thermal motion differs from purely harmonic motion. (C) 2013 Elsevier B.V. All rights reserved. C1 [Loukonen, V.; Vehkamaki, H.] Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland. [Kuo, I-F. W.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94550 USA. [McGrath, M. J.] Kyoto Univ, Grad Sch Sci, Dept Biophys, Kyoto 6068502, Japan. RP Loukonen, V (reprint author), Univ Helsinki, Dept Phys, POB 64, FI-00014 Helsinki, Finland. EM ville.loukonen@helsinki.fi RI Vehkamaki, Hanna/A-8262-2008 OI Vehkamaki, Hanna/0000-0002-5018-1255 FU Maj and Tor Nessling Foundation [2011200]; Academy of Finland (Center of Excellence program) [1118615]; European Research Council [ERC-StG 257360-MOCAPAF]; US Department of Energy [DE-AC52-07NA27344]; Academy of Finland (LASTU program) [135054] FX This work was financially supported by the Maj and Tor Nessling Foundation (project #2011200), the Academy of Finland (Center of Excellence program project #1118615, LASTU program project #135054) and the European Research Council (project ERC-StG 257360-MOCAPAF). We also thank the Livermore Computing and the Grand Challenge scientific computing program and the CSC - IT Center for Science Ltd for kindly providing computer resources. Part of this work was performed under the auspices of the US Department of Energy under contract DE-AC52-07NA27344. NR 39 TC 13 Z9 13 U1 3 U2 70 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD JAN 15 PY 2014 VL 428 BP 164 EP 174 DI 10.1016/j.chemphys.2013.11.014 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 287XA UT WOS:000329574400022 ER PT J AU Grossman, Y Ligeti, Z Robinson, DJ AF Grossman, Yuval Ligeti, Zoltan Robinson, Dean J. TI More flavor SU(3) tests for new physics in CP violating B decays SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE B-Physics; CP violation ID QCD FACTORIZATION; STANDARD MODEL; ASYMMETRIES AB The recent LHCb measurements of the B-s -> K-pi(+) and B-s -> K+K- rates and CP asymmetries are in agreement with U-spin expectations from B-d -> K+pi(-) and B-d -> pi(+)pi(-) results. We derive the complete set of isospin, U-spin, and SU(3) relations among the CP asymmetries in two-body charmless B -> PP and B -> PV decays, some of which are novel. To go beyond the unbroken SU(3) limit, we present relations which are properly defined and normalized to allow incorporation of SU(3) breaking in the simplest manner. We show that there are no CP relations beyond first order in SU(3) and isospin breaking. We also consider the corresponding relations for charm decays. Comparing parametrizations of the leading order sum rules with data can shed light on the applicability and limitations of both the flavor symmetry and factorization-based descriptions of SU(3) breaking. Two factorization relations can already be tested, and we show they agree with current data. C1 [Grossman, Yuval; Robinson, Dean J.] Cornell Univ, Lab Elementary Particle Phys, Ithaca, NY USA. [Ligeti, Zoltan; Robinson, Dean J.] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Robinson, Dean J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Grossman, Y (reprint author), Cornell Univ, Lab Elementary Particle Phys, Ithaca, NY USA. EM yg73@cornell.edu; ligeti@lbl.gov; djrobinson@berkeley.edu FU U.S. National Science Foundation [PHY-0757868, PHY-1002399]; United States-Israel Binational Science Foundation (BSF) [2010221]; Office of High Energy Physics of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Gerhard Buchalla, Iain Stewart and Jure Zupan for helpful conversations. While we were finalizing this work, ref. [28] appeared with U-spin results that partially overlap, and agree, with ours. The work of YG and DR is supported by the U.S. National Science Foundation through grant PHY-0757868 and by the United States-Israel Binational Science Foundation (BSF) under grant No. 2010221. The work of DR is also supported in part by the U.S. National Science Foundation under Grant No. PHY-1002399. ZL was supported in part by the Office of High Energy Physics of the U.S. Department of Energy under contract DE-AC02-05CH11231. ZL thanks the Erwin Schrodinger Institute program "Jets and Quantum Fields for LHC and Future Colliders" for hospitality while portions of this work were completed. NR 29 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 15 PY 2014 IS 1 AR 066 DI 10.1007/JHEP01(2014)066 PG 25 WC Physics, Particles & Fields SC Physics GA 288OH UT WOS:000329620800001 ER PT J AU Hrma, P Riley, BJ Crum, JV Matyas, J AF Hrma, Pavel Riley, Brian J. Crum, Jarrod V. Matyas, Josef TI The effect of high-level waste glass composition on spinel liquidus temperature SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article; Proceedings Paper CT 10th International Symposium on Crystallization in Glasses and Liquids (Crystallization) CY SEP 23-26, 2012 CL Goslar, GERMANY SP Amer Ceram Soc DE Waste glass; Spinel; Liquidus temperature ID BOROSILICATE GLASS; NEPHELINE LIQUIDUS; HLW-GLASSES; CRYSTALLIZATION; EQUILIBRIUM; CRYSTALS; BEHAVIOR; MODEL AB Spinel crystals precipitate in high-level waste glasses containing Fe, Cr, Ni, Mn, Zn, and Ru. The liquidus temperature (T-L) of spinel as the primary crystallization phase is a function of glass composition, and the spinet solubility (c(0)) is a function of both glass composition and temperature (T). Previously reported models of T-L as a function of composition are based on T-L measured directly, which requires laborious experimental procedures. Viewing the curve of c(0) versus T as the liquidus line allows a significant broadening of the composition region for model fitting. This paper estimates T-L, as a function of composition based on c(0) data obtained with the X-ray diffraction technique. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hrma, Pavel; Riley, Brian J.; Crum, Jarrod V.; Matyas, Josef] PNNL, Richland, WA 99354 USA. [Hrma, Pavel] Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang, South Korea. RP Hrma, P (reprint author), PNNL, Richland, WA 99354 USA. EM pavelhrma@postech.ac.kr OI Riley, Brian/0000-0002-7745-6730 NR 37 TC 6 Z9 6 U1 0 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD JAN 15 PY 2014 VL 384 SI SI BP 32 EP 40 DI 10.1016/j.jnonaysol.2013.02.014 PG 9 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA 285VF UT WOS:000329422400006 ER PT J AU Wu, GP Yang, JB Wang, DP Xu, R Amine, K Lu, CX AF Wu, Gang-Ping Yang, Junbing Wang, Dapeng Xu, Rui Amine, Khalil Lu, Chun-Xiang TI A novel route for preparing mesoporous carbon aerogels using inorganic templates under ambient drying SO MATERIALS LETTERS LA English DT Article DE Carbon materials; Porous materials; Carbon aerogel; Ambient drying AB A low-cost approach for mesoporous carbon aerogel synthesis using calcium carbonate particles as templates and ambient pressure drying is reported in this paper. The removal of templates by acid treatment produced additional mesopores that mimic the template particles. The resulting carbon aerogels showed higher mesopore ratio and a significantly larger pore volume compared with those without templates. This study provides a low-cost and easy-to-scale-up method for producing mesoporous carbon aerogels with large pore volumes. (C) 2013 Elsevier B.V. All rights reserved. C1 [Wu, Gang-Ping; Lu, Chun-Xiang] Chinese Acad Sci, Inst Coal Chem, Natl Engn Lab Carbon Fiber Technol, Taiyuan 030001, Shanxi Province, Peoples R China. [Wu, Gang-Ping; Yang, Junbing; Wang, Dapeng; Xu, Rui; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Wu, GP (reprint author), Chinese Acad Sci, Inst Coal Chem, Natl Engn Lab Carbon Fiber Technol, 27 Taoyuan South Rd, Taiyuan 030001, Shanxi Province, Peoples R China. EM wgp@sxicc.ac.cn FU Scholarship Council Foundation of Chinese Academy of Sciences in China; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This work was supported by the Scholarship Council Foundation of Chinese Academy of Sciences in China. Electron microscopy was performed at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 10 TC 10 Z9 10 U1 4 U2 79 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-577X EI 1873-4979 J9 MATER LETT JI Mater. Lett. PD JAN 15 PY 2014 VL 115 BP 1 EP 4 DI 10.1016/j.matlet.2013.10.003 PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 287SV UT WOS:000329563400001 ER PT J AU Jiang, W Bailey, K Lu, ZT Mueller, P O'Connor, TP Purtschert, R AF Jiang, W. Bailey, K. Lu, Z. -T. Mueller, P. O'Connor, T. P. Purtschert, R. TI Ion current as a precise measure of the loading rate of a magneto-optical trap SO OPTICS LETTERS LA English DT Article ID ATOMS; COLLISIONS; COLD AB We have demonstrated that the ion current resulting from collisions between metastable krypton atoms in a magneto-optical trap can be used to precisely measure the trap loading rate. We measured both the ion current of the abundant isotope Kr-83 (isotopic abundance = 11%) and the single-atom counting rate of the rare isotope Kr-85 (isotopic abundance similar to 1 x 10(-11)), and found the two quantities to be proportional at a precision level of 0.9%. This work results in a significant improvement in using the magneto-optical trap as an analytical tool for noble-gas isotope ratio measurements, and will benefit both atomic physics studies and applications in the earth sciences. (C) 2014 Optical Society of America C1 [Jiang, W.; Bailey, K.; Lu, Z. -T.; Mueller, P.; O'Connor, T. P.] Argonne Natl Lab, Div Phys, Lemont, IL 60439 USA. [Lu, Z. -T.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Lu, Z. -T.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Purtschert, R.] Univ Bern, CH-3012 Bern, Switzerland. RP Jiang, W (reprint author), Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Lemont, IL 60439 USA. EM wjiang@phy.anl.gov RI Jiang, Wei/E-5582-2011; Mueller, Peter/E-4408-2011; Purtschert, Roland/N-7108-2016 OI Mueller, Peter/0000-0002-8544-8191; Purtschert, Roland/0000-0002-4734-7664 FU Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX We thank S.-M. Hu and H. Esbensen for stimulating discussions. This work is supported by the Department of Energy, Office of Nuclear Physics, under contract DE-AC02-06CH11357. NR 16 TC 2 Z9 2 U1 0 U2 7 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD JAN 15 PY 2014 VL 39 IS 2 BP 409 EP 412 DI 10.1364/OL.39.000409 PG 4 WC Optics SC Optics GA 292MV UT WOS:000329906900059 PM 24562159 ER PT J AU DiSanti, MA Villanueva, GL Paganini, L Bonev, BP Keane, JV Meech, KJ Mumma, MJ AF DiSanti, Michael A. Villanueva, Geronimo L. Paganini, Lucas Bonev, Boncho P. Keane, Jacqueline V. Meech, Karen J. Mumma, Michael J. TI Pre- and post-perihelion observations of C/2009 P1 (Garradd): Evidence for an oxygen-rich heritage? SO ICARUS LA English DT Article DE Comets, composition; Spectroscopy; Comets, coma; Comets, origin ID O1 HALE-BOPP; C/1996 B2 HYAKUTAKE; CARBON-MONOXIDE; OORT-CLOUD; CHEMICAL-COMPOSITION; VOLATILE COMPOSITION; ORGANIC COMPOSITION; INTERSTELLAR ICES; PARENT VOLATILES; COMET 8P/TUTTLE AB We conducted pre- and post-perihelion observations of Comet C/2009 P1 (Garradd) on UT 2011 October 13 and 2012 January 8, at heliocentric distances of 1.83 and 1.57 AU, respectively, using the high-resolution infrared spectrometer (NIRSPEC) at the Keck II 10-m telescope on Mauna Kea, HI. Pre-perihelion, we obtained production rates for nine primary volatiles (native ices): H2O, CO, CH3OH, CH4, C2H6, HCN, C2H2, H2CO, and NH3. Post-perihelion, we obtained production rates for three of these (H2O, CH4, and HCN) and sensitive upper limits for three others (C2H2, H2CO, and NH3). CO was enriched and C2H2 was depleted, yet C2H6 and CH3OH were close to their current mean values as measured in a dominant group of Oort cloud comets. This may indicate processing of its pre-cometary ices in a relatively oxygen-rich environment. Our measurements indicate consistent pre- and post-perihelion abundance ratios relative to H2O, suggesting we were measuring compositional homogeneity among measured species to the depths in the nucleus sampled. However, the overall gas production was lower post-perihelion despite its smaller heliocentric distance on January 8. This is qualitatively consistent with other studies of C/2009 P1, perhaps due to seasonal differences in the heating of one or more active regions on the nucleus. On October 13, the water profile showed a pronounced excess towards the Sun-facing hemisphere that was not seen in other molecules, including H2O on January 8, nor in the dust continuum. Inter-comparison of profiles from October 13 permitted us to quantify contributions due to release of H2O from the nucleus, and from its release in the coma. This resulted in the latter source contributing 25-30% of the total observed water within our slit, which covered roughly +/- 300 km by +/- 4500 km from the nucleus. We attribute this excess H2O, which peaked at a mean projected distance of 1300-1500 km from the nucleus, to release from water-rich, relatively pure icy grains. Published by Elsevier Inc. C1 [DiSanti, Michael A.; Villanueva, Geronimo L.; Paganini, Lucas; Bonev, Boncho P.; Mumma, Michael J.] NASA, Goddard Space Flight Ctr, Goddard Ctr Astrobiol, Greenbelt, MD 20771 USA. [DiSanti, Michael A.; Mumma, Michael J.] NASA, Goddard Space Flight Ctr, Solar Syst Explorat Div, Greenbelt, MD 20771 USA. [Villanueva, Geronimo L.; Paganini, Lucas; Bonev, Boncho P.] Catholic Univ Amer, Dept Phys, Washington, DC 20064 USA. [Paganini, Lucas] Oak Ridge Associated Univ, NASA, Postdoctoral Program, Oak Ridge, TN 37830 USA. [Keane, Jacqueline V.; Meech, Karen J.] Univ Hawaii, NASA, Astrobiol Inst, Honolulu, HI 96722 USA. [Keane, Jacqueline V.; Meech, Karen J.] Univ Hawaii, Inst Astron, Honolulu, HI 96822 USA. RP DiSanti, MA (reprint author), NASA, Goddard Space Flight Ctr, Goddard Ctr Astrobiol, Mail Stop 693-0, Greenbelt, MD 20771 USA. EM michael.a.disanti@nasa.gov FU NASA Astrobiology Institute [RTOP 344-53-51, NNA09DA77A]; NASA Planetary Astronomy Program [RTOPs 09-PAST09-0034, 344-32-07]; NASA Planetary Atmospheres Program [RTOPs 09-PATM-0080, 12-PATM12-0049]; National Science Foundation Astronomy and Astrophysics [AST-1211362, AST-0807939]; NASA Postdoctoral Program; W.M. Keck Foundation FX We gratefully acknowledge support through the NASA Astrobiology Institute under Cooperative Agreements (RTOP 344-53-51 to GSFC, and NNA09DA77A to U. Hawai'i), the NASA Planetary Astronomy Program (RTOPs 09-PAST09-0034, 344-32-07), the NASA Planetary Atmospheres Program (RTOPs 09-PATM-0080, 12-PATM12-0049), the National Science Foundation Astronomy and Astrophysics Grants Program (AST-1211362, AST-0807939), and the NASA Postdoctoral Program. We thank two anonymous reviewers for comments that improved the paper. M.A.D. thanks S. Charnley for fruitful discussions regarding surface chemistry of interstellar ices, and R. Novak for participating in the January 8 observations. The data presented herein were obtained at the W.M. Keck Observatory, operated as a scientific partnership among CalTech, UCLA, and NASA, and made possible by the generous financial support of the W.M. Keck Foundation. The authors recognize the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate for the opportunity to conduct observations from this mountain. NR 93 TC 14 Z9 14 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD JAN 15 PY 2014 VL 228 BP 167 EP 180 DI 10.1016/j.icarus.2013.09.001 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 275HC UT WOS:000328665900013 ER PT J AU Thomas, CA Emery, JP Trilling, DE Delbo, M Hora, JL Mueller, M AF Thomas, Cristina A. Emery, Joshua P. Trilling, David E. Delbo, Marco Hora, Joseph L. Mueller, Michael TI Physical characterization of Warm Spitzer-observed near-Earth objects SO ICARUS LA English DT Article DE Asteroids; Asteroids, composition; Spectroscopy; Near-Earth objects ID ASTEROID SPECTROSCOPIC SURVEY; INFRARED TELESCOPE FACILITY; S-TYPE ASTEROIDS; REFLECTANCE SPECTRA; ORDINARY CHONDRITE; 433 EROS; MINERALOGICAL CHARACTERIZATION; SPACE-TELESCOPE; SOURCE REGIONS; DAWN MISSION AB Near-infrared spectroscopy of Near-Earth Objects (NEOs) connects diagnostic spectral features to specific surface mineralogies. The combination of spectroscopy with albedos and diameters derived from thermal infrared observations can increase the scientific return beyond that of the individual datasets. For instance, some taxonomic classes can be separated into distinct compositional groupings with albedo and different mineralogies with similar albedos can be distinguished with spectroscopy. To that end, we have completed a spectroscopic observing campaign to complement the ExploreNEOs Warm Spitzer program that obtained albedos and diameters of nearly 600 NEOs (Trilling, D.E. et al. [2010]. Astron. J. 140, 770-784. http://dx.doi.org/10.1088/0004-6256/140/3/770). The spectroscopy campaign included visible and near-infrared observations of ExploreNEOs targets from various observatories. Here we present the results of observations using the low-resolution prism mode (similar to 0.7-2.5 mu m) of the SpeX instrument on the NASA Infrared Telescope Facility (IRTF). We also include near-infrared observations of ExploreNEOs targets from the MIT-UH-IRTF Joint Campaign for Spectral Reconnaissance. Our dataset includes near-infrared spectra of 187 ExploreNEOs targets (125 observations of 92 objects from our survey and 213 observations of 154 objects from the MIT survey). We identify a taxonomic class for each spectrum and use band parameter analysis to investigate the mineralogies for the S-, Q-, and V-complex objects. Our analysis suggests that for spectra that contain near-infrared data but lack the visible wavelength region, the Bus-DeMeo system misidentifies some S-types as Q-types. We find no correlation between spectral band parameters and ExploreNEOs albedos and diameters. We investigate the correlations of phase angle with Band Area Ratio and near-infrared spectral slope. We find slightly negative Band Area Ratio (BAR) correlations with phase angle for Eros and Ivar, but a positive BAR correlation with phase angle for Ganymed. The results of our phase angle study are consistent with those of (Sanchez, J.A., Reddy, V., Nathues, A., Cloutis, E.A., Mann, P., Hiesinger, H. [2012]. Icarus 220, 36-50. http://dx.doi.org/10.1016/j.icarus.2012.04.008, arXiv:1205.0248). We find evidence for spectral phase reddening for Eros, Ganymed, and Ivar. We identify the likely ordinary chondrite type analog for an appropriate subset of our sample. Our resulting proportions of H, L, and LL ordinary chondrites differ from those calculated for meteorite falls and in previous studies of ordinary chondrite-like NEOs. (C) 2013 Elsevier Inc. All rights reserved. C1 [Thomas, Cristina A.; Trilling, David E.] No Arizona Univ, Dept Phys & Astron, Flagstaff, AZ 86011 USA. [Thomas, Cristina A.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Thomas, Cristina A.] Oak Ridge Associated Univ, NASA, Postdoctoral Program, Oak Ridge, TN 37831 USA. [Emery, Joshua P.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Delbo, Marco] Univ Nice Sophia Antipolis, CNRS, Observ Cote Azur, F-06304 Nice 4, France. [Hora, Joseph L.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Mueller, Michael] Univ Groningen, SRON Netherlands Inst Space Res, NL-9700 AV Groningen, Netherlands. RP Thomas, CA (reprint author), NASA, Goddard Space Flight Ctr, 8800 Greenbelt Rd,Code 691, Greenbelt, MD 20771 USA. EM cristina.a.thomas@nasa.gov OI Hora, Joseph/0000-0002-5599-4650; Mueller, Michael/0000-0003-3217-5385 FU NASA Postdoctoral Program at Goddard Space Flight Center; NASA; JPL/Caltech; National Science Foundation [0506716] FX This research was supported by an appointment to the NASA Postdoctoral Program at Goddard Space Flight Center, administered by Oak Ridge Associated Universities through a contract with NASA.; This work is based in part on observations made with the Spitzer Space Telescope, which is operated by JPL/Caltech under a contract with NASA. Support for this work was, provided by NASA through an award issued by JPL/Caltech.; Part of the data utilized in this publication were obtained and made available by the MIT-UH-IRTF Joint Campaign for NEO Reconnaissance. The IRTF is operated by the University of Hawaii under Cooperative Agreement No. NCC 5-538 with the National Aeronautics and Space Administration, Office of Space Science, Planetary Astronomy Program. The MIT component of this work is supported by the National Science Foundation under Grant No. 0506716. NR 71 TC 8 Z9 8 U1 0 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD JAN 15 PY 2014 VL 228 BP 217 EP 246 DI 10.1016/j.icarus.2013.10.004 PG 30 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 275HC UT WOS:000328665900017 ER PT J AU Dover, N Barash, JR Hill, KK Xie, G Arnon, SS AF Dover, Nir Barash, Jason R. Hill, Karen K. Xie, Gary Arnon, Stephen S. TI Molecular Characterization of a Novel Botulinum Neurotoxin Type H Gene SO JOURNAL OF INFECTIOUS DISEASES LA English DT Article DE Clostridium botulinum; botulinum toxin; botulinum toxin type H; botulism ID SEROTYPE-A SUBTYPES; CLOSTRIDIUM-BOTULINUM; INFANT BOTULISM; GENOMIC ANALYSIS; GROUP-II; STRAINS; DIVERSITY; TOXIN; COMPLEX; SEQUENCE AB We sequenced the 2 botulinum toxin gene clusters of Clostridium botulinum strain IBCA10-7060 type Bh. The sequence of bont/H differed substantially from the sequences of the 7 known bont genes for toxin types A-G. The 5' one-third terminus of bont/H that codes for the botulinum toxin light chain differed markedly from the light chain coding sequences of toxin types A-G. The 3' two-thirds terminus of bont/H that codes for the botulinum toxin heavy chain contained a novel Hn translocation domain coding sequence and a nonneutralizing type A-like Hc binding domain coding sequence. bont/H was part of an orfX toxin gene cluster that was located at a unique chromosomal site distant from those used by other botulinum toxin gene clusters. The bont/B sequence was similar to that of subtype bont/B2 and was located within its ha toxin gene cluster at the oppA/brnQ site. Our findings further establish that C. botulinum IBCA10-7060 produces novel BoNT/H. C1 [Dover, Nir; Barash, Jason R.; Arnon, Stephen S.] Calif Dept Publ Hlth, Infant Botulism Treatment & Prevent Program, Richmond, CA 94804 USA. [Hill, Karen K.; Xie, Gary] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. RP Arnon, SS (reprint author), Calif Dept Publ Hlth, Infant Botulism Treatment & Prevent Program, 850 Marina Bay Pkwy,Rm E361, Richmond, CA 94804 USA. EM stephen.arnon@cdph.ca.gov OI xie, gary/0000-0002-9176-924X FU Infant Botulism Treatment and Prevention Fund of the California Department of Public Health FX This work was supported by the Infant Botulism Treatment and Prevention Fund of the California Department of Public Health. NR 31 TC 84 Z9 85 U1 5 U2 34 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0022-1899 EI 1537-6613 J9 J INFECT DIS JI J. Infect. Dis. PD JAN 15 PY 2014 VL 209 IS 2 BP 192 EP 202 DI 10.1093/infdis/jit450 PG 11 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA 282GA UT WOS:000329157200008 PM 24106295 ER PT J AU Billesbach, DP Berry, JA Seibt, U Maseyk, K Torn, MS Fischer, ML Abu-Naser, M Campbell, JE AF Billesbach, D. P. Berry, J. A. Seibt, U. Maseyk, K. Torn, M. S. Fischer, M. L. Abu-Naser, Mohammad Campbell, J. E. TI Growing season eddy covariance measurements of carbonyl sulfide and CO2 fluxes: COS and CO2 relationships in Southern Great Plains winter wheat SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Carbonyl sulfide; COS; GPP; Eddy covariance; Trace gas flux ID STOMATAL CONDUCTANCE; ATMOSPHERE EXCHANGE; SPRUCE FOREST; WATER-VAPOR; SOIL; PHOTOSYNTHESIS; TRANSPIRATION; RESPIRATION; TEMPERATURE; CONSUMPTION AB To test the capabilities of newly available instrumentation and to explore the dynamics of carbonyl sulfide (COS) as a proxy for the measurement of canopy-scale gross primary production (GPP), we conducted an experiment to measure the simultaneous net transfer of COS and CO2 between the atmosphere and a growing wheat canopy, senesced wheat, and the harvested field (located in the Southern Great Plains of the U.S.) using the eddy covariance technique. We found that during the growing season, there was a strong uptake of COS by the canopy (roughly between -10 and -40 pmol m(-2) s(-1)) with a strong diel signal that mirrored net CO2 fluxes. After senescence and over the harvested field, we observed a strong source of COS to the atmosphere (up to +40 pmol m(-2) s(-1)) that exhibited a weaker diel pattern, again similar to CO2. These results suggest that the dynamics of COS are more complicated than once thought, but that it may still be possible to independently derive canopy-scale GPP from direct COS measurements and to use them as model constraints on the atmospheric carbon cycle. To demonstrate this, we computed an average value of leaf relative uptake (LRU) (the scaling factor between GPP and ratios of the fluxes of COS and CO2 and ratios of the atmospheric concentrations of COS and CO2) that is in good agreement with laboratory results. (C) 2013 Elsevier B.V. All rights reserved. C1 [Billesbach, D. P.] Univ Nebraska, Dept Biol Syst Engn, Lincoln, NE 68588 USA. [Berry, J. A.] Stanford Univ, Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA. [Seibt, U.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Maseyk, K.] Univ Paris 06, Paris, France. [Torn, M. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Fischer, M. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Abu-Naser, Mohammad; Campbell, J. E.] Univ Calif, Sierra Nevada Res Inst, Merced, CA USA. RP Billesbach, DP (reprint author), Univ Nebraska, Dept Biol Syst Engn, Lincoln, NE 68588 USA. EM dbillesbach1@unl.edu RI Torn, Margaret/D-2305-2015 FU U.S. Department of Energy, Biological and Environmental Research Division [DE-SC0007094]; Air Liquide Foundation; U.S. National Science Foundation FX We would like to thank the staff of the DOE-ARM Central Facility for hosting and assisting us in completing this project. This work was supported by the U.S. Department of Energy, Biological and Environmental Research Division under Award # DE-SC0007094, The Air Liquide Foundation, and through a major equipment grant from the U.S. National Science Foundation. NR 42 TC 13 Z9 13 U1 4 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD JAN 15 PY 2014 VL 184 BP 48 EP 55 DI 10.1016/j.agrformet.2013.06.007 PG 8 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA 275HH UT WOS:000328666400005 ER PT J AU Hu, YZ Lu, F Nualart, D AF Hu, Yaozhong Lu, Fei Nualart, David TI Convergence of densities of some functionals of Gaussian processes SO JOURNAL OF FUNCTIONAL ANALYSIS LA English DT Article DE Multiple Wiener-Ito integrals; Wiener chaos; Malliavin calculus; Integration by parts; Stein's method; Convergence of densities; Ornstein-Uhlenbeck process; Least squares estimator; Small deviation ID MULTIVARIATE NORMAL APPROXIMATION; MULTIPLE STOCHASTIC INTEGRALS; CENTRAL LIMIT-THEOREMS; STEINS METHOD; MALLIAVIN CALCULUS; EXCHANGEABLE PAIRS; WIENER CHAOS; INEQUALITIES; EXPANSIONS AB The aim of this paper is to establish the uniform convergence of the densities of a sequence of random variables, which are functionals of an underlying Gaussian process, to a normal density. Precise estimates for the uniform distance are derived by using the techniques of Malliavin calculus, combined with Stein's method for normal approximation. We need to assume some non-degeneracy conditions. First, the study is focused on random variables in a fixed Wiener chaos, and later, the results are extended to the uniform convergence of the derivatives of the densities and to the case of random vectors in some fixed chaos, which are uniformly non-degenerate in the sense of Malliavin calculus. Explicit upper bounds for the uniform norm are obtained for random variables in the second Wiener chaos, and an application to the convergence of densities of the least square estimator for the drift parameter in Ornstein-Uhlenbeck processes is discussed. Published by Elsevier Inc. C1 [Hu, Yaozhong; Nualart, David] Univ Kansas, Dept Math, Lawrence, KS 66045 USA. [Lu, Fei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lu, F (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM hu@math.ku.edu; flu@lbl.gov; nualart@math.ku.edu FU Simons Foundation [209206]; NSF [DMS1208625] FX Y. Hu is partially supported by a grant from the Simons Foundation #209206.; D. Nualart is supported by the NSF grant DMS1208625. NR 30 TC 4 Z9 4 U1 1 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-1236 EI 1096-0783 J9 J FUNCT ANAL JI J. Funct. Anal. PD JAN 15 PY 2014 VL 266 IS 2 BP 814 EP 875 DI 10.1016/j.jfa.2013.09.024 PG 62 WC Mathematics SC Mathematics GA 272FM UT WOS:000328445700015 ER PT J AU Mendoza-Mendez, P Lopez-Flores, L Vizcarra-Rendon, A Sanchez-Diaz, LE Medina-Noyola, M AF Mendoza-Mendez, Patricia Lopez-Flores, Leticia Vizcarra-Rendon, Alejandro Sanchez-Diaz, Luis E. Medina-Noyola, Magdaleno TI Generalized Langevin equation for tracer diffusion in atomic liquids SO PHYSICA A-STATISTICAL MECHANICS AND ITS APPLICATIONS LA English DT Article DE Colloidal and atomic liquids; Generalized Langevin equation; Doppler friction ID FLUCTUATION-DISSIPATION THEOREM; MODE-COUPLING THEORY; BROWNIAN-MOTION; STATISTICAL-MECHANICS; COLLOIDAL SUSPENSIONS; MICROSCOPIC DYNAMICS; GLASS-TRANSITION; THERMODYNAMICS; DISPERSIONS; RELAXATION AB We derive the time-evolution equation that describes the Brownian motion of labeled individual tracer particles in a simple model atomic liquid (i.e., a system of N particles whose motion is governed by Newton's second law, and interacting through spherically symmetric pairwise potentials). We base our derivation on the generalized Langevin equation formalism, and find that the resulting time evolution equation is formally identical to the generalized Langevin equation that describes the Brownian motion of individual tracer particles in a colloidal suspension in the absence of hydrodynamic interactions. This formal dynamic equivalence implies the long-time indistinguishability of some dynamic properties of both systems, such as their mean squared displacement, upon a well-defined time scaling. This prediction is tested here by comparing the results of molecular and Brownian dynamics simulations performed on the hard sphere system. (C) 2013 Elsevier B.V. All rights reserved. C1 [Mendoza-Mendez, Patricia; Lopez-Flores, Leticia] Benemerita Univ Autonoma Puebla, Fac Ciencias Fisicomatemat, Puebla 72000, Pue, Mexico. [Vizcarra-Rendon, Alejandro] Univ Autonoma Zacatecas, Unidad Acad Fis, Zacatecas 98600, Zac, Mexico. [Sanchez-Diaz, Luis E.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Medina-Noyola, Magdaleno] Univ Autonoma San Luis Potosi, Inst Fis Manuel Sandoval Vallarta, San Luis Potosi 78000, Slp, Mexico. RP Medina-Noyola, M (reprint author), Univ Autonoma San Luis Potosi, Inst Fis Manuel Sandoval Vallarta, Alvaro Obregon 64, San Luis Potosi 78000, Slp, Mexico. EM medina@ifisica.uaslp.mx FU Consejo Nacional de Ciencia y Tecnologia (CONACYT, Mexico) [132540, 182132] FX The authors are grateful to G. Perez-Angel and M. Chavez-Paez for their advice and assistance with the molecular and Brownian dynamics simulations, and to L. Yeomans-Reyna, for valuable discussions. We also acknowledge the kind hospitality of the Joint Institute for Neutron Sciences (Oak Ridge, TN), where part of this manuscript was written. We are grateful to W.-R. Chen and T. Egami for stimulating discussions. This work was supported by the Consejo Nacional de Ciencia y Tecnologia (CONACYT, Mexico) through grants 132540 and 182132. NR 51 TC 4 Z9 5 U1 1 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-4371 EI 1873-2119 J9 PHYSICA A JI Physica A PD JAN 15 PY 2014 VL 394 BP 1 EP 16 DI 10.1016/j.physa.2013.09.061 PG 16 WC Physics, Multidisciplinary SC Physics GA 273GP UT WOS:000328523600001 ER PT J AU Baumbach, RE Scott, BL Ronning, F Thompson, JD Bauer, ED AF Baumbach, R. E. Scott, B. L. Ronning, F. Thompson, J. D. Bauer, E. D. TI Single crystal study of antiferromagnetic CePd3Al9 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE antiferromagnetism; single ion Kondo effect; molten metal flux growth ID FERMI-LIQUID BEHAVIOR; PHASE-TRANSITIONS; KONDO DISORDER; ELECTRON; SUPERCONDUCTIVITY; TEMPERATURE; ALLOYS; METALS AB Single crystal x-ray diffraction, magnetic susceptibility (M), heat capacity (C), and electrical resistivity (rho) measurements are reported for specimens of the new tetragonal compound CePd3Al9, which forms in a new structure type. X-ray diffraction measurements reveal that the nearest neighbor Ce-Ce distances are large (d(Ce-Ce) = 5.272 angstrom), suggesting that this compound may be described as a stoichiometric dilute Kondo lattice. Thermodynamic and transport measurements reveal antiferromagnetic order near T-N = 0.9 K. The ordered ground state emerges from a lattice of localized Ce ions that are weakly hybridized with the conduction electrons, as revealed by the moderate electronic coefficient of the specific heat gamma approximate to 45 mJ mol(-1) K-2 (extrapolated from above T-N) and the lack of evidence for Kondo coherence in the magnetic susceptibility and electrical resistivity. The application of a magnetic field initially suppresses the magnetic order at a rate of -0.04 K kOe(-1), but Zeeman splitting of the doublet ground state produces a nonmagnetic singlet before T-N reaches zero. The data additionally reveal that chemical/structural disorder plays an important role, as evidenced by results from single crystal x-ray diffraction, the broadness of the peak at TN in the heat capacity, and the small residual resistivity ratio RRR = rho(300 K)/rho(0) = 1.3. C1 [Baumbach, R. E.; Scott, B. L.; Ronning, F.; Thompson, J. D.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Baumbach, RE (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM rbaumbach@lanl.gov RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US DOE, OBES, Division of Material Science and Engineering FX Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, and PECASE funding from the US DOE, OBES, Division of Material Science and Engineering. NR 28 TC 1 Z9 1 U1 0 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 15 PY 2014 VL 26 IS 2 AR 025601 DI 10.1088/0953-8984/26/2/025601 PG 6 WC Physics, Condensed Matter SC Physics GA 270PB UT WOS:000328329700015 PM 24326344 ER PT J AU Smadici, S Lee, JCT Logvenov, G Bozovic, I Abbamonte, P AF Smadici, S. Lee, J. C. T. Logvenov, G. Bozovic, I. Abbamonte, P. TI Form factor dispersion at La M5,4 edges and average density of resonant atoms SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE x-ray scattering; superlattice; resonant; form factor ID X-RAY-SCATTERING; SUPERCONDUCTIVITY; TRANSMISSION; REFLECTION; NEUTRON; LAYER AB Resonant soft x-ray scattering on complex oxide superlattices shows very large variations in the superlattice reflection position and intensity near La M-5,M-4 edges. Resonant dispersion of the La x-ray form factor describes the observations well. We determine the average density of resonant La atoms and the thickness of superlattice layers. C1 [Smadici, S.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Smadici, S.; Lee, J. C. T.; Abbamonte, P.] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Logvenov, G.; Bozovic, I.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Logvenov, G.] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany. RP Smadici, S (reprint author), Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. EM serban.smadici@louisville.edu FU Center for Emergent Superconductivity, an Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences; University of Louisville Research Foundation; DOE [DE-AC02-98CH10886] FX This work was supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. Additional support came from the University of Louisville Research Foundation. Use of the NSLS was supported by DOE grant DE-AC02-98CH10886 and use of Materials Research Laboratory facilities by DE-FG02-07ER46453 and DE-FG02-07ER46471. NR 43 TC 1 Z9 1 U1 2 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 15 PY 2014 VL 26 IS 2 AR 025303 DI 10.1088/0953-8984/26/2/025303 PG 8 WC Physics, Condensed Matter SC Physics GA 270PB UT WOS:000328329700005 PM 24318961 ER PT J AU Xing, YL AF Xing, Yulong TI Exactly well-balanced discontinuous Galerkin methods for the shallow water equations with moving water equilibrium SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Shallow water equations; Discontinuous Galerkin method; Moving water equilibrium; High order accuracy; Well-balanced; Positivity preserving methods ID GEOMETRICAL SOURCE TERMS; VOLUME WENO SCHEMES; COMPUTING HYPERBOLIC SYSTEMS; SAINT-VENANT SYSTEM; CONSERVATION-LAWS; UPWIND SCHEMES; ORDER; RECONSTRUCTION; FLOWS; STATES AB Hyperbolic conservation laws with source terms often admit steady state solutions where the fluxes and source terms balance each other. To capture this balance and near-equilibrium solutions, well-balanced methods have been introduced and performed well in many numerical tests. Shallow water equations have been extensively investigated as a prototype example. In this paper, we develop well-balanced discontinuous Galerkin methods for the shallow water system, which preserve not only the still water at rest steady state, but also the more general moving water equilibrium. The key idea is the recovery of well-balanced states, a special source term approximation, and the approximation of the numerical fluxes based on a generalized hydrostatic reconstruction. We also study the extension of the positivity-preserving limiter presented in [40] in this framework. Numerical examples are provided at the end to verify the well-balanced property and good resolution for smooth and discontinuous solutions. (C) 2013 Elsevier Inc. All rights reserved. C1 [Xing, Yulong] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Xing, Yulong] Univ Tennessee, Dept Math, Knoxville, TN 37996 USA. RP Xing, YL (reprint author), Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. EM xingy@math.utk.edu FU National Science Foundation [DMS-1216454]; ORNL's Laboratory Directed Research and Development funds; U.S. Department of Energy, Office of Advanced Scientific Computing Research; UT-Battelle, LLC [DE-AC05-00OR22725] FX Research is sponsored by the National Science Foundation grant DMS-1216454, ORNL's Laboratory Directed Research and Development funds, and the U.S. Department of Energy, Office of Advanced Scientific Computing Research. The work was partially performed at ORNL, which is managed by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725. NR 41 TC 23 Z9 24 U1 0 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 536 EP 553 DI 10.1016/j.jcp.2013.10.010 PN A PG 18 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UC UT WOS:000327483200026 ER PT J AU Meyer, CD Balsara, DS Aslam, TD AF Meyer, Chad D. Balsara, Dinshaw S. Aslam, Tariq D. TI A stabilized Runge-Kutta-Legendre method for explicit super-time-stepping of parabolic and mixed equations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Numerical methods; Super-time-stepping; Parabolic operators; PDEs ID PARTIAL-DIFFERENTIAL-EQUATIONS; NUMERICAL-METHODS; SCHEMES; CONSTRUCTION; DETONATION; CONDUCTION; DIFFUSION; RADIATION; DYNAMICS; SPEED AB Parabolic partial differential equations appear in several physical problems, including problems that have a dominant hyperbolic part coupled to a sub-dominant parabolic component. Explicit methods for their solution are easy to implement but have very restrictive time step constraints. Implicit solution methods can be unconditionally stable but have the disadvantage of being computationally costly or difficult to implement. Super-time-stepping methods for treating parabolic terms in mixed type partial differential equations occupy an intermediate position. In such methods each superstep takes "s" explicit Runge-Kutta-like time-steps to advance the parabolic terms by a time-step that is s(2) times larger than a single explicit time-step. The expanded stability is usually obtained by mapping the short recursion relation of the explicit Runge-Kutta scheme to the recursion relation of some well-known, stable polynomial. Prior work has built temporally first- and second-order accurate super-time-stepping methods around the recursion relation associated with Chebyshev polynomials. Since their stability is based on the boundedness of the Chebyshev polynomials, these methods have been called RKC1 and RKC2. In this work we build temporally first- and second-order accurate super-time-stepping methods around the recursion relation associated with Legendre polynomials. We call these methods RKL1 and RKL2. The RKL1 method is first-order accurate in time; the RKL2 method is second-order accurate in time. We verify that the newly-designed RKL1 and RKL2 schemes have a very desirable monotonicity preserving property for one-dimensional problems - a solution that is monotone at the beginning of a time step retains that property at the end of that time step. It is shown that RKL1 and RKL2 methods are stable for all values of the diffusion coefficient up to the maximum value. We call this a convex monotonicity preserving property and show by examples that it is very useful in parabolic problems with variable diffusion coefficients. This includes variable coefficient parabolic equations that might give rise to skew symmetric terms. The RKC1 and RKC2 schemes do not share this convex monotonicity preserving property. One-dimensional and two-dimensional von Neumann stability analyses of RKC1, RKC2, RKL1 and RKL2 are also presented, showing that the latter two have some advantages. The paper includes several details to facilitate implementation. A detailed accuracy analysis is presented to show that the methods reach their design accuracies. A stringent set of test problems is also presented. To demonstrate the robustness and versatility of our methods, we show their successful operation on problems involving linear and non-linear heat conduction and viscosity, resistive magnetohydrodynamics, ambipolar diffusion dominated magnetohydrodynamics, level set methods and flux limited radiation diffusion. In a prior paper (Meyer, Balsara and Aslam 2012 [36]) we have also presented an extensive test-suite showing that the RKL2 method works robustly in the presence of shocks in an anisotropically conducting, magnetized plasma. (C) 2013 Elsevier Inc. All rights reserved. C1 [Meyer, Chad D.; Balsara, Dinshaw S.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Aslam, Tariq D.] Los Alamos Natl Lab, WX Grp 9, Los Alamos, NM 87545 USA. RP Meyer, CD (reprint author), Univ Notre Dame, Dept Phys, 225 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. OI Aslam, Tariq/0000-0002-4263-0401 FU NSF [NSF-AST-0947765, NSF-AST-1009091]; NASA grants from the Fermi program; NASA-NNX [12A088G]; US Department of Energy FX DSB acknowledges support via NSF grants NSF-AST-0947765 and NSF-AST-1009091. DSB also acknowledges support via NASA grants from the Fermi program as well as NASA-NNX 12A088G. The majority of simulations were performed on a cluster at UND that is run by the Center for Research Computing. Computer support on NSF's XSEDE computing resources is also acknowledged.; The authors wish to thank Christopher Romick for providing the exact solution to the Argon shock structure. TDA was supported by the US Department of Energy. TDA would like to thank the John Bdzil (LANL), Joseph Powers (Notre Dame), Steve Son (Purdue) and Lori Groven (Purdue) for useful discussions during this work. NR 53 TC 6 Z9 6 U1 1 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 594 EP 626 DI 10.1016/j.jcp.2013.08.021 PN A PG 33 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UC UT WOS:000327483200029 ER PT J AU Roy, UN Bolotnikov, AE Camarda, GS Cui, Y Hossain, A Lee, K Marshall, M Yang, G James, RB AF Roy, U. N. Bolotnikov, A. E. Camarda, G. S. Cui, Y. Hossain, A. Lee, K. Marshall, M. Yang, G. James, R. B. TI Growth of CdTexSe1-x from a Te-rich solution for applications in radiation detection SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Characterization; Defects; Te-inclusions; THM; CdTeSe; Semiconducting II-VI materials ID CADMIUM ZINC TELLURIDE; CDZNTE DETECTORS; CDTE; PERFORMANCE; CRYSTALS; DEFECTS; PHOTOLUMINESCENCE; SEGREGATION; INCLUSIONS AB We grew CdTexSe1-x (CTS) crystals from a Te-rich solution by using the traveling heater method (THM). The average size distribution and concentration of Te inclusions/precipitates in these as-grown samples were measured to be similar to 7 x 10(4) cm(-3), which is much lower than values typical for the present state-of-the-art commercial CdZnTe (CZT) material. Their low-temperature photoluminescence measurement indicates high quality of the material; however the resistivity obtained via I-V curve measurements was similar to 5 x 10(8) Omega-cm, which is low in comparison to that required for gamma detectors. A well resolved alpha response peak can be detected for both planar- and hemispherical detector geometry. The (mu tau)(e), value for our as grown sample at room temperature was found to be similar to 4 x 10(-3) cm(2)/V. (C) 2013 Elsevier B.V. All rights reserved. C1 [Roy, U. N.; Bolotnikov, A. E.; Camarda, G. S.; Cui, Y.; Hossain, A.; Lee, K.; Marshall, M.; Yang, G.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Roy, UN (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM utpalnroy@gmail.com OI Marshall, Matthew/0000-0002-6440-8713 FU U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and development, DNN RD; U.S. Department of Energy [DE-AC02-98CH10886] FX This work was supported by the U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and development, DNN R&D. The manuscript has been authored by Brookhaven Science Associates, LLC under Contract no. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 16 TC 5 Z9 5 U1 1 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD JAN 15 PY 2014 VL 386 BP 43 EP 46 DI 10.1016/j.jcrysgro.2013.09.039 PG 4 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA 259WE UT WOS:000327556200008 ER PT J AU Sugar, JD El Gabaly, F Chueh, WC Fenton, KR Tyliszczak, T Kotula, PG Bartelt, NC AF Sugar, Joshua D. El Gabaly, Farid Chueh, William C. Fenton, Kyle R. Tyliszczak, Tolek Kotula, Paul G. Bartelt, Norman C. TI High-resolution chemical analysis on cycled LiFePO4 battery electrodes using energy-filtered transmission electron microscopy SO JOURNAL OF POWER SOURCES LA English DT Article DE LiFePO4; TEM; Electron energy loss spectroscopy; Phase transformation ID MULTIVARIATE STATISTICAL-ANALYSIS; DOMINO-CASCADE MODEL; SIMS SPECTRUM-IMAGES; X-RAY-DIFFRACTION; LITHIUM BATTERY; LI-INSERTION/EXTRACTION; LOSS SPECTROSCOPY; PHASE-TRANSITION; LIXFEPO4; KINETICS AB We demonstrate an ex situ method for analyzing the chemistry of battery electrode particles after electrochemical cycling using the transmission electron microscope (TEM). The arrangement of particles during our analysis is the same as when the particles are being cycled. We start by sectioning LiFePO4 battery electrodes using an ultramicrotome. We then show that mapping of the Fe2+ and Fe3+ oxidation state using energy-filtered TEM (EFTEM) and multivariate statistical analysis techniques can be used to determine the spatial distribution of Li in the particles. This approach is validated by comparison with scanning transmission X-ray microscopy (STXM) analysis of the same samples [Chueh et al. Nanoletters, 13 (3) (2013) 866-72]. EFTEM uses a parallel electron beam and reduces the electron-beam dose (and potential beam-induced damage) to the sample when compared to alternate techniques that use a focused probe (e.g. STEM-EELS). Our analysis confirms that under the charging conditions of the analyzed battery, mixed phase particles are rare and thus Li intercalation is limited by the nucleation of new phases. (C) 2013 Elsevier B.V. All rights reserved. C1 [Sugar, Joshua D.; El Gabaly, Farid; Bartelt, Norman C.] Sandia Natl Labs, Livermore, CA 94550 USA. [Fenton, Kyle R.; Kotula, Paul G.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chueh, William C.] Stanford Univ, Stanford, CA 94305 USA. RP Sugar, JD (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM jdsugar@sandia.gov RI Kotula, Paul/A-7657-2011 OI Kotula, Paul/0000-0002-7521-2759 FU U.S. Department of Energy through the Sandia Laboratory Directed research and Development program; Office of Basic Energy Science, Division of Materials Sciences and Engineering; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Special thanks to Mark Homer, Ray Twesten, Masashi Watanabe, Bernhard Schaffer, Kevin McCarty, Tony McDaniel, and Helmut Gnaegi. The research was supported by the U.S. Department of Energy through the Sandia Laboratory Directed research and Development program. F.E.G. and N.C.B. acknowledge support from the Office of Basic Energy Science, Division of Materials Sciences and Engineering. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 62 TC 17 Z9 17 U1 10 U2 148 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2014 VL 246 BP 512 EP 521 DI 10.1016/j.jpowsour.2013.08.003 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 247YO UT WOS:000326661100068 ER PT J AU Koren, B Abgrall, R Bochev, P Frank, J Perot, B AF Koren, Barry Abgrall, Remi Bochev, Pavel Frank, Jason Perot, Blair TI Physics-compatible numerical methods SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Editorial Material C1 [Koren, Barry] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. [Abgrall, Remi] INRIA, Paris, France. [Abgrall, Remi] Inst Polytech Bordeaux, Bordeaux, France. [Bochev, Pavel] Sandia Natl Labs, Livermore, CA 94550 USA. [Frank, Jason] Univ Utrecht, NL-3508 TC Utrecht, Netherlands. [Perot, Blair] Univ Massachusetts, Amherst, MA 01003 USA. RP Koren, B (reprint author), Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. NR 0 TC 3 Z9 3 U1 0 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 1039 EP 1039 DI 10.1016/j.jcp.2013.10.015 PN B PG 1 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UH UT WOS:000327483700001 ER PT J AU Dobrev, VA Kolev, TV Rieben, RN AF Dobrev, Veselin A. Kolev, Tzanio V. Rieben, Robert N. TI High order curvilinear finite elements for elastic-plastic Lagrangian dynamics SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Elastic-plastic flow; Lagrangian hydrodynamics; High-order finite element methods ID HYDRODYNAMICS AB This paper presents a high-order finite element method for calculating elastic-plastic flow on moving curvilinear meshes and is an extension of our general high-order curvilinear finite element approach for solving the Euler equations of gas dynamics in a Lagrangian frame [1,2]. In order to handle transition to plastic flow, we formulate the stress-strain relation in rate (or incremental) form and augment our semi-discrete equations for Lagrangian hydrodynamics with an additional evolution equation for the deviatoric stress which is valid for arbitrary order spatial discretizations of the kinematic and thermodynamic variables. The semi-discrete equation for the deviatoric stress rate is developed for 2D planar, 2D axisymmetric and full 3D geometries. For each case, the strain rate is approximated via a collocation method at zone quadrature points while the deviatoric stress is approximated using an L-2 projection onto the thermodynamic basis. We apply high order, energy conserving, explicit time stepping methods to the semi-discrete equations to develop the fully discrete method. We conclude with numerical results from an extensive series of verification tests that demonstrate several practical advantages of using high-order finite elements for elastic-plastic flow. (C) 2013 Elsevier Inc. All rights reserved. C1 [Dobrev, Veselin A.; Kolev, Tzanio V.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA USA. [Rieben, Robert N.] Lawrence Livermore Natl Lab, Div B, Livermore, CA 94550 USA. RP Rieben, RN (reprint author), Lawrence Livermore Natl Lab, Div B, Livermore, CA 94550 USA. EM dobrev1@llnl.gov; kolev1@llnl.gov; rieben1@llnl.gov NR 28 TC 3 Z9 3 U1 0 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 1062 EP 1080 DI 10.1016/j.jcp.2013.01.015 PN B PG 19 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UH UT WOS:000327483700003 ER PT J AU Bochev, P Ridzal, D Peterson, K AF Bochev, Pavel Ridzal, Denis Peterson, Kara TI Optimization-based remap and transport: A divide and conquer strategy for feature-preserving discretizations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Constrained interpolation; Remap; Quadratic programming; Preservation of local bounds; Preservation of linearity; Optimization-based remap; Transport; Spherical geometry; Lat/lon coordinates ID DISCRETE MAXIMUM PRINCIPLE; DIFFUSION-EQUATIONS; GRIDS; ALGORITHMS; SCHEME; MESHES; FLOW; GRADIENT AB This paper examines the application of optimization and control ideas to the formulation of feature-preserving numerical methods, with particular emphasis on the conservative and bound-preserving remap (constrained interpolation) and transport (advection) of a single scalar quantity. We present a general optimization framework for the preservation of physical properties and specialize it to a generic optimization-based remap (OBR) of mass density. The latter casts remap as a quadratic program whose optimal solution minimizes the distance to a suitable target quantity, subject to a system of linear inequality constraints. The approximation of an exact mass update operator defines the target quantity, which provides the best possible accuracy of the new masses without regard to any physical constraints such as conservation of mass or local bounds. The latter are enforced by the system of linear inequalities. In so doing, the generic OBR formulation separates accuracy considerations from the enforcement of physical properties. We proceed to show how the generic OBR formulation yields the recently introduced flux-variable flux-target (FVFT) [1] and mass-variable mass-target (MVMT) [2] formulations of remap and then follow with a formal examination of their relationship. Using an intermediate flux-variable mass-target (FVMT) formulation we show the equivalence of FVFT and MVMT optimal solutions. To underscore the scope and the versatility of the generic OBR formulation we introduce the notion of adaptable targets, i.e., target quantities that reflect local solution properties, extend FVFT and MVMT to remap on the sphere, and use OBR to formulate adaptable, conservative and bound-preserving optimization-based transport algorithms for Cartesian and latitude/longitude coordinate systems. A selection of representative numerical examples on two-dimensional grids demonstrates the computational properties of our approach. (C) 2013 Elsevier Inc. All rights reserved. C1 [Bochev, Pavel; Ridzal, Denis; Peterson, Kara] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ridzal, D (reprint author), Sandia Natl Labs, MS 1320, Albuquerque, NM 87185 USA. EM pbboche@sandia.gov; dridzal@sandia.gov; kjpeter@sandia.gov FU DOE Office of Science Advanced Scientific Computing Research (ASCR) Program; Advanced Simulation & Computing (ASC) Program FX All authors acknowledge funding by the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program. DR and KP also acknowledge funding by the Advanced Simulation & Computing (ASC) Program. Special thanks go to M. Shashkov who introduced us to the remap problem, guided us through its subtleties and prompted our initial interest in the use of optimization in this context. Our colleague J. Young helped with the formulation and implementation of some of the optimization algorithms used in the approach. Technical discussions and informal conversations with R. Abgrall, A. Barlow, E. Cyr, D. Kuzmin, A. Robinson, J. Shadid, G. Scovazzi, and many other colleagues provided useful insights and perspectives. NR 47 TC 4 Z9 4 U1 0 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 1113 EP 1139 DI 10.1016/j.jcp.2013.03.057 PN B PG 27 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UH UT WOS:000327483700005 ER PT J AU Lipnikov, K Manzini, G Shashkov, M AF Lipnikov, Konstantin Manzini, Gianmarco Shashkov, Mikhail TI Mimetic finite difference method SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Mimetic finite difference method; Discrete vector and tensor calculus; Lagrangian hydrodynamics ID SHALLOW-WATER EQUATIONS; ANISOTROPIC DIFFUSION-PROBLEMS; TENSOR ARTIFICIAL VISCOSITY; LOGICALLY RECTANGULAR GRIDS; ELEMENT EXTERIOR CALCULUS; SUPPORT-OPERATOR METHOD; GENERAL 2D MESHES; DIV-CURL PROBLEMS; POLYHEDRAL MESHES; ELLIPTIC PROBLEMS AB The mimetic finite difference (MFD) method mimics fundamental properties of mathematical and physical systems including conservation laws, symmetry and positivity of solutions, duality and self-adjointness of differential operators, and exact mathematical identities of the vector and tensor calculus. This article is the first comprehensive review of the 50-year long history of the mimetic methodology and describes in a systematic way the major mimetic ideas and their relevance to academic and real-life problems. The supporting applications include diffusion, electromagnetics, fluid flow, and Lagrangian hydrodynamics problems. The article provides enough details to build various discrete operators on unstructured polygonal and polyhedral meshes and summarizes the major convergence results for the mimetic approximations. Most of these theoretical results, which are presented here as lemmas, propositions and theorems, are either original or an extension of existing results to a more general formulation using polyhedral meshes. Finally, flexibility and extensibility of the mimetic methodology are shown by deriving higher-order approximations, enforcing discrete maximum principles for diffusion problems, and ensuring the numerical stability for saddle-point systems. (C) 2013 Elsevier Inc. All rights reserved. C1 [Lipnikov, Konstantin; Manzini, Gianmarco] Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87544 USA. [Shashkov, Mikhail] Los Alamos Natl Lab, Methods & Algorithms Grp, XCP 4, X Computat Phys Div, Los Alamos, NM 87544 USA. RP Shashkov, M (reprint author), Los Alamos Natl Lab, Methods & Algorithms Grp, XCP 4, X Computat Phys Div, POB 1663, Los Alamos, NM 87544 USA. EM lipnikov@lanl.gov; gmanzini@lanl.gov; shashkov@lanl.gov OI Manzini, Gianmarco/0000-0003-3626-3112 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research; US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program FX This work was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The authors gratefully acknowledge the partial support of the US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research and the partial support of the US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program. NR 274 TC 60 Z9 64 U1 0 U2 27 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 1163 EP 1227 DI 10.1016/j.jcp.2013.07.031 PN B PG 65 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UH UT WOS:000327483700007 ER PT J AU Brezzi, F Buffa, A Manzini, G AF Brezzi, F. Buffa, A. Manzini, G. TI Mimetic scalar products of discrete differential forms SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Discrete differential form; Mimetic finite difference method; Polyhedral mesh ID FINITE-VOLUME METHOD; CONVECTION-DIFFUSION PROBLEMS; LOGICALLY RECTANGULAR GRIDS; ELEMENT EXTERIOR CALCULUS; ELLIPTIC PROBLEMS; CONVERGENCE ANALYSIS; POLYHEDRAL MESHES; POLYGONAL MESHES; NATURAL DISCRETIZATIONS; MAXWELLS EQUATIONS AB We propose a strategy for the systematic construction of the mimetic inner products on cochain spaces for the numerical approximation of partial differential equations on unstructured polygonal and polyhedral meshes. The mimetic inner products are locally built in a recursive way on each k-cell and, then, globally assembled. This strategy is similar to the implementation of the finite element methods. The effectiveness of this approach is documented by deriving mimetic discretizations and testing their behavior on a set of problems related to the Maxwell equations. Published by Elsevier Inc. C1 [Brezzi, F.] KAU, Jeddah, Saudi Arabia. [Brezzi, F.; Buffa, A.; Manzini, G.] CNR, IMATI, I-27100 Pavia, Italy. [Brezzi, F.; Manzini, G.] IUSS Pavia, Ctr Simulaz Numer Avanzata CeSNA, I-27100 Pavia, Italy. [Manzini, G.] Los Alamos Natl Lab, Div Theoret, Grp T5, Los Alamos, NM 87545 USA. RP Manzini, G (reprint author), Los Alamos Natl Lab, Div Theoret, Grp T5, MS B284, Los Alamos, NM 87545 USA. EM gmanzini@lanl.gov RI Brezzi, Franco/D-4362-2009; Buffa, Annalisa/C-4275-2011; OI Brezzi, Franco/0000-0003-4715-5475; Buffa, Annalisa/0000-0003-0384-0876; Manzini, Gianmarco/0000-0003-3626-3112 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics FX The work of the third author was partially supported by the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics. NR 89 TC 11 Z9 11 U1 0 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2014 VL 257 BP 1228 EP 1259 DI 10.1016/j.jcp.2013.08.017 PN B PG 32 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 258UH UT WOS:000327483700008 ER PT J AU Lienert, TJ Burgardt, P Harada, KL Forsyth, RT DebRoy, T AF Lienert, T. J. Burgardt, P. Harada, K. L. Forsyth, R. T. DebRoy, T. TI Weld bead center line shift during laser welding of austenitic stainless steels with different sulfur content SO SCRIPTA MATERIALIA LA English DT Article DE Laser welding; Stainless steels; Optical microscopy; Arc Welding ID GAS TUNGSTEN ARC; MARANGONI FLOW AB The magnitude of the shift in position of the maximum depth of penetration, the center line shift (CLS), for a laser weld produced between two heats of austenitic stainless steels with large differences in S content was smaller relative to gas tungsten arc (GTA) welds made with both higher and lower heat inputs. The results of this study suggest that both surface tension driven fluid (Marangoni) flow effects and arc shift effects may contribute to the CLS in GTA welding. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Lienert, T. J.; Burgardt, P.; Harada, K. L.; Forsyth, R. T.] Los Alamos Natl Lab, Div Mat Sci, Los Alamos, NM 87545 USA. [DebRoy, T.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Lienert, TJ (reprint author), Los Alamos Natl Lab, Div Mat Sci, POB 1663, Los Alamos, NM 87545 USA. EM lienert@lanl.gov FU Los Alamos National Security, LLC FX The lead author acknowledges Miss Marisa Lienert for inspiration during the course this study. The authors wish to extend their appreciation to William L. Stellwag, Jr., formerly with Los Alamos National Laboratory, for assistance with the laser welding experiments. This work was performed at Los Alamos National Laboratory under the auspices of Los Alamos National Security, LLC, under contract to the US Department of Energy. NR 24 TC 6 Z9 6 U1 6 U2 48 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD JAN 15 PY 2014 VL 71 BP 37 EP 40 DI 10.1016/j.scriptamat.2013.09.029 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 255HM UT WOS:000327230000010 ER PT J AU Zhu, Y Casselman, MD Li, Y Wei, A Abraham, DP AF Zhu, Ye Casselman, Matthew D. Li, Yan Wei, Alexander Abraham, Daniel P. TI Perfluoroalkyl-substituted ethylene carbonates: Novel electrolyte additives for high-voltage lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Polyfluoroalkyl compounds; Electrolyte additives; High voltage, high capacity; Lithium-ion battery; Solid electrolyte interphase (SEI) ID GRAPHITE-ELECTRODES; POSITIVE ELECTRODE; VINYLENE CARBONATE; CELLS; PERFORMANCE; ANODE; CHEMISTRY; STORAGE; SURFACE; LIQUID AB A new family of polyfluoroalkyl-substituted ethylene carbonates is synthesized and tested as additives in lithium-ion cells containing EC:EMC + LiPF6-based electrolyte. The influence of these compounds is investigated in Li1.2Ni0.15Mn0.55Co0.1O2//graphite cells via a combination of galvanostatic cycling and electrochemical impedance spectroscopy (EIS) tests. Among the four additives studied in this work (4-(trifluoromethyl)-1,3-dioxolan-2-one (TFM-EC), 4-(perfluorobutyl)-1,3-dioxolan-2-one (PFB-EC), 4-(perfluorohexyl)-1,3-dioxolan-2-one (PFH-EC), and 4-(perfluorooctyl)-1,3-dioxolan-2-one (PFO-EC)), small amounts (0.5 wt%) of PFO-EC is found to be most effective in lessening cell performance degradation during extended cycling. Linear sweep voltammetiy (LSV), X-ray photoelectron spectroscopy (XPS) and Raman spectroscopy are used to further characterize the effects of PFO-EC on the positive and negative electrodes. LSV data from the electrolyte, and XPS analyses of electrodes harvested after cycling, suggest that PFO-EC is oxidized on the cathode forming surface films that slow electrode/cell impedance rise. Differential capacity (dQ/dV) plots from graphite//Li cells suggest that PFO-EC is involved in solid electrolyte interphase (SEI) formation. Raman data from anodes after cycling suggest that structural disordering of graphite is reduced by the addition of PFO-EC, which may explain the improved cell capacity retention. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhu, Ye; Li, Yan; Abraham, Daniel P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Casselman, Matthew D.; Wei, Alexander] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. [Li, Yan] Univ Rochester, Mat Sci Program, Rochester, NY 14627 USA. RP Abraham, DP (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zhuy@anl.gov; mdcassel@purdue.edu; liy@anl.gov; alexwei@purdue.edu; abraham@anl.gov RI Li, Yan/H-2957-2012 OI Li, Yan/0000-0002-9801-7243 FU U.S. Department of Energy's Vehicle Technologies Program; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; DOE Vehicle Technologies Program (VTP) within Applied Battery Research (ABR) for Transportation Program; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Support from the U.S. Department of Energy's Vehicle Technologies Program, specifically from Dave Howell and Peter Faguy, is gratefully acknowledged. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. We are grateful to B. Polzin, A. Jansen, and S. Trask from the U.S. Department of Energy's (DOE) Cell Fabrication Facility (CFF), Argonne National Laboratory for providing electrodes used in this work. The CFF is fully supported by the DOE Vehicle Technologies Program (VTP) within the core funding of the Applied Battery Research (ABR) for Transportation Program. We acknowledge use of the Center for Microanalysis of Materials (CMM) at the Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign (Illinois). Use of the Center for Nanoscale Materials at Argonne, was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 33 TC 33 Z9 34 U1 13 U2 143 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2014 VL 246 BP 184 EP 191 DI 10.1016/j.jpowsour.2013.07.070 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 247YO UT WOS:000326661100025 ER PT J AU Nelson, GJ Nakajo, A Cassenti, BN DeGostin, MB Bagshaw, KR Peracchio, AA Xiao, GL Wang, S Chen, FL Chiu, WKS AF Nelson, George J. Nakajo, Arata Cassenti, Brice N. DeGostin, Matthew B. Bagshaw, Kyle R. Peracchio, Aldo A. Xiao, Guoliang Wang, Steve Chen, Fanglin Chiu, Wilson K. S. TI A rapid analytical assessment tool for three dimensional electrode microstructural networks with geometric sensitivity SO JOURNAL OF POWER SOURCES LA English DT Article DE Microstructure; Fuel cell; Design; Electrode; Electrochemical fin; Segmentation ID OXIDE FUEL-CELLS; MONTE-CARLO SIMULATIONS; COMPOSITE ELECTRODES; SOFC ELECTRODES; CHARGE-TRANSFER; SPACE-CHARGE; AIR CATHODES; ANODE; PERFORMANCE; TRANSPORT AB Electrochemical fin theory is applied to the microstructural analysis of Sr2Fe1.5Mo0.5O6-delta (SFM), a redox stable solid oxide fuel cell (SOFC) electrode. The electrode microstructure is imaged by X-ray nanotomography, then partitioned into a network of resistive components with distinct geometric characteristics. The network is analyzed using an analytical electrochemical fin network model. The resulting predictions of electrode performance are compared to predictions made using three-dimensional finite element simulations of charge transport with surface electrochemical reactions in the imaged microstructure. For a representative subvolume of the structure, the electrochemical fin and finite element models provide comparable predictions. Analysis of larger representative volume elements extracted from the X-ray nanotomography data demonstrates good agreement with experimental measurements of the electrodes analyzed. Finally, advantages of applying the analytical electrochemical fin network models to real microstructures are addressed, particularly with respect to significant reduction in memory requirements and computational time. The use of the electrochemical fin theory is able to rapidly analyze real microstructures with microstructural details that are comparable to finite element and lattice Boltzmann methods, but at volume sizes that finite element and lattice Boltzmann methods were not able to perform due to limits in memory and computational time. (C) 2013 Elsevier B.V. All rights reserved. C1 [Nelson, George J.; Nakajo, Arata; Cassenti, Brice N.; DeGostin, Matthew B.; Bagshaw, Kyle R.; Peracchio, Aldo A.; Chiu, Wilson K. S.] Univ Connecticut, Dept Mech Engn, Storrs, CT 06260 USA. [Xiao, Guoliang; Chen, Fanglin] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Wang, Steve] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Chiu, WKS (reprint author), Univ Connecticut, Dept Mech Engn, Storrs, CT 06260 USA. EM wchiu@engr.uconn.edu RI Chen, Fanglin/K-1039-2012 OI Chen, Fanglin/0000-0001-9942-8872 FU Energy Frontier Research Center on Science Based Nano-Structure Design and Synthesis of Heterogeneous Functional Materials for Energy Systems (HeteroFoaM Center); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001061, DE-AC02-06CH11357] FX Financial support from an Energy Frontier Research Center on Science Based Nano-Structure Design and Synthesis of Heterogeneous Functional Materials for Energy Systems (HeteroFoaM Center) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (Award DE-SC0001061) is gratefully acknowledged. Portions of this research were carried out at the Advanced Photon Source supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. The authors thank W. M. Harris for comments provided on image processing and analysis. NR 44 TC 12 Z9 13 U1 1 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2014 VL 246 BP 322 EP 334 DI 10.1016/j.jpowsour.2013.07.009 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 247YO UT WOS:000326661100043 ER PT J AU Allu, S Kalnaus, S Elwasif, W Simunovic, S Turner, JA Pannala, S AF Allu, Srikanth Kalnaus, Sergiy Elwasif, Wael Simunovic, Srdjan Turner, John A. Pannala, Sreekanth TI A new open computational framework for highly-resolved coupled three-dimensional multiphysics simulations of Li-ion cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium ion battery; Modeling; Computational framework; Multiphysics simulations ID HYBRID-ELECTRIC VEHICLES; THERMAL MANAGEMENT; DISCHARGE BEHAVIOR; BATTERY SYSTEMS; POLYMER BATTERY; INSERTION CELL; LITHIUM; TEMPERATURE; GENERATION; MODEL AB In this paper we report on the development and demonstration of physically consistent three-dimensional models for Lithium Ion Battery (LIB) cells. The discharge behavior of a LIB is a multi-physics and multiscale problem that is simulated using coupled models for thermal, electrical, and electrochemical phenomena. The individual physics models and software are integrated into a new open computational framework for battery simulations which was designed to support a variety of modeling formulations and computer codes. Several cell configurations (unrolled cell, unrolled cell with current collectors, large capacity pouch cell, and cylindrical cell) that show the importance of coupled simulations are simulated using this approach and discussed. A validation study is presented for the pouch cell discharged under high rates to demonstrate the accuracy of the proposed modeling framework. (C) 2013 Elsevier B.V. All rights reserved, C1 [Allu, Srikanth; Kalnaus, Sergiy; Elwasif, Wael; Simunovic, Srdjan; Turner, John A.; Pannala, Sreekanth] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Allu, S (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM allus@ornl.gov RI Pannala, Sreekanth/F-9507-2010; OI Kalnaus, Sergiy/0000-0002-7465-3034; Turner, John/0000-0003-2521-4091; allu, srikanth/0000-0003-2841-4398 FU Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy [DE-AC05-000R22725] FX This research at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-000R22725, was sponsored by the Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy (with David Howell and Brian Cunningham as program managers). The authors would like to acknowledge that the pouch cell for testing was obtained from Dr. Keith Kepler at Farasis Energy Inc. and the experimental data was obtained from Dr. Hsin Wang at the Oak Ridge National Laboratory. NR 37 TC 14 Z9 14 U1 5 U2 71 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2014 VL 246 BP 876 EP 886 DI 10.1016/j.jpowsour.2013.08.040 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 247YO UT WOS:000326661100109 ER PT J AU Hochgraf, CG Basco, JK Bohn, TP Bloom, I AF Hochgraf, Clark G. Basco, John K. Bohn, Theodore P. Bloom, Ira TI Effect of ultracapacitor-modified PHEV protocol on performance degradation in lithium-ion cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Ultracapacitor-battery hybrid; Battery testing; Cycle life; Electric vehicle; PHEV ID CALENDAR-LIFE; CYCLE-LIFE; BATTERIES; MECHANISM; SPINEL; ENERGY; POWER AB The cycle life of lithium-ion batteries was investigated using a modified USABC electric vehicle testing protocol designed to simulate the effect of a hybrid energy-storage system (ultracapacitor and battery) in a plug-in hybrid electric vehicle. A side-by-side comparison of battery capacity and impedance changes with and without the effect of the ultracapacitor was performed. Calendar-life degradation effects were corrected for using control cells. The battery's rate of cycle-related capacity degradation decreased by a factor of 2 and rate of cycle-related impedance degradation, by a factor of 5.9 when exposed to the ultracapacitor-modified profile. The modified profile avoids exposure to regeneration energy and reduces maximum voltage of the battery. (C) 2012 Elsevier B.V. All rights reserved. C1 [Hochgraf, Clark G.] Rochester Inst Technol, Rochester, NY 14623 USA. [Basco, John K.; Bloom, Ira] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Bohn, Theodore P.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Bloom, I (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ira.bloom@anl.gov FU U.S. Department of Energy, Office of Vehicle Technologies, Hybrid and Electric Systems [DE-AC02-06CH11357] FX The work at Argonne National Laboratory was performed under the auspices of the U.S. Department of Energy, Office of Vehicle Technologies, Hybrid and Electric Systems, under Contract No. DE-AC02-06CH11357. NR 14 TC 17 Z9 17 U1 1 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2014 VL 246 BP 965 EP 969 DI 10.1016/j.jpowsour.2012.09.038 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 247YO UT WOS:000326661100119 ER PT J AU Braun, F Tarditi, AM Miller, JB Cornaglia, LM AF Braun, Fernando Tarditi, Ana M. Miller, James B. Cornaglia, Laura M. TI Pd-based binary and ternary alloy membranes: Morphological and perm-selective characterization in the presence of H2S SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE PdAgAu alloy; Sulfur tolerance; Ternary alloy; Hydrogen separation membrane ID HYDROGEN SEPARATION; COMPOSITE MEMBRANE; CU MEMBRANES; SULFUR; PREDICTION; KINETICS; COAL AB Pd, Pd90Ag10, Pd91Au9, Pd78Ag9Au13 and Pd75Ag16Au9 alloy membranes were prepared on vacuum-assisted ZrO2-modified porous stainless steel supports by sequential electroless deposition. The membranes were evaluated for permeability in pure H-2 and in an H2S/H-2 mixture. The membranes displayed a range of permeabilities in pure H-2: Pd90Ag10 > Pd78Ag9Au13 > Pd similar to Pd75Ag16Au9 > Pd91Au9. On exposure to 100 ppm H2S/H-2 at 673 K for 24 h, all membranes lost a significant fraction of their H-2 permeabilities: Pd (lost the largest fraction, 85%) > Pd90Ag10 > Pd75Ag16Au9 > Pd78Ag9Au13 > Pd91Au9 (60%). When H2S was removed, the membranes recovered the lost permeability to different extents. The Pd91Au9 and Pd78Ag9Au13 membranes displayed the highest fractional recovery of initial H-2 permeability (similar to 80%). But, with its higher initial pure H-2 permeability, Pd78Ag9Au13 had the highest absolute H-2 permeability after recovery. The microstructure, morphology and bulk composition of H2S-exposed samples were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM) and energy-dispersive X-ray spectroscopy (EDS). XRD revealed the presence of a bulk Pd4S phase on both Pd and Pd90Ag10 to, the membranes that recovered the least H-2 relative flux after their exposure to H2S. In contrast, bulk sulfides did not form on Pd91Au9 or on PdAgAu ternary alloys. In agreement with the XRD results, EDS did not detect sulfur in the bulk of Pd91Au9 or in either of the ternary alloy samples. Our results show that the addition of Au to the high permeability PdAg binary membrane results in a PdAgAu ternary membrane that minimizes the permanent H-2 flux loss associated with H2S exposure by preventing the formation of thick stable sulfides. (C) 2013 Elsevier B.V. All rights reserved. C1 [Braun, Fernando; Tarditi, Ana M.; Cornaglia, Laura M.] UNL CONICET, Inst Invest Catalisis & Petroquim FIQ, RA-3000 Santa Fe, Argentina. [Miller, James B.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Miller, James B.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. RP Cornaglia, LM (reprint author), UNL CONICET, Inst Invest Catalisis & Petroquim FIQ, Santiago Estero 2829, RA-3000 Santa Fe, Argentina. EM lmcornag@fiq.unl.edu.ar FU UNL; ANPCyT FX The authors wish to acknowledge the financial support received from UNL and ANPCyT. Elsa Grimaldi is thanked for the English language editing and Fabio Fontanarrosa is hereby thanked for the SEM images acquisition. NR 28 TC 12 Z9 12 U1 0 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 EI 1873-3123 J9 J MEMBRANE SCI JI J. Membr. Sci. PD JAN 15 PY 2014 VL 450 BP 299 EP 307 DI 10.1016/j.memsci.2013.09.026 PG 9 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA 243NY UT WOS:000326324600033 ER PT J AU Singh, DJ AF Singh, David J. TI Superconductivity and magnetism in YFe2Ge2 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-DENSITY-WAVE; SR2RUO4; HEAT AB We report calculations of the electronic structure and magnetic properties of YFe2Ge2 and discuss the results in terms of the observed superconductivity near magnetism. We find that YFe2Ge2 is a material near a magnetic quantum critical point based on comparison of standard density functional results that predict magnetism with experiment. The band structure and Fermi surfaces are very three dimensional and higher conductivity is predicted in the c-axis direction. The magnetism is of Stoner type and is predominately from an in-plane ferromagnetic tendency. The interlayer coupling is weak giving a perhaps two dimensional character to the magnetism, which is in contrast to the conductivity and may be important for suppressing the ordering tendency. This is compatible with a triplet superconducting state mediated by spin fluctuations. C1 Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Singh, DJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 30 TC 16 Z9 16 U1 3 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 14 PY 2014 VL 89 IS 2 AR 024505 DI 10.1103/PhysRevB.89.024505 PG 6 WC Physics, Condensed Matter SC Physics GA AC0UV UT WOS:000332211900004 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soeldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Study of CP-violating charge asymmetries of single muons and like-sign dimuons in p(p)over-bar collisions SO PHYSICAL REVIEW D LA English DT Article ID BARYON ASYMMETRY; DETECTOR AB We measure the inclusive single muon charge asymmetry and the like-sign dimuon charge asymmetry in p (p) over bar collisions using the full data set of 10.4 fb(-1) collected with the D0 detector at the Fermilab Tevatron. The standard model predictions of the charge asymmetries induced by CP violation are small in magnitude compared to the current experimental precision, so nonzero measurements could indicate new sources of CP violation. The measurements differ from the standard model predictions of CP violation in these asymmetries with a significance of 3.6 standard deviations. These results are interpreted in a framework of B meson mixing within the Cabibbo-Kobayashi-Maskawa formalism to measure the relative width difference Delta Gamma(d)/Gamma(d) between the mass eigenstates of the B-0 meson system and the semileptonic charge asymmetries a(sl)(d) and a(sl)(s) of B-0 and B-s(0) mesons, respectively. C1 [Maciel, A. K. A.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Augsten, K.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Kupco, A.; Lokajicek, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Hoeneisen, B.] Univ San Francisco Quito, Quito, Ecuador. [Badaud, F.; Gris, Ph] Univ Clermont Ferrand, LPC, CNRS, IN2P3, Clermont, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, IN2P3, Inst Natl Polytech Grenoble,LPSC, Grenoble, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CNRS, IN2P3, CPPM, Marseille, France. [Grivaz, J. -F.; Guillemin, T.; Jaffre, M.; Petroff, P.] Univ Paris 11, CNRS, IN2P3, LAL, F-91405 Orsay, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 06, CNRS, IN2P3, LPNHE, Paris, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 07, CNRS, IN2P3, LPNHE, Paris, France. [Bassler, U.; Besancon, M.; Chapon, E.; Couderc, F.; Deliot, F.; Hubacek, Z.; Royon, C.; Shary, V.; Titov, M.; Tuchming, B.; Vilanova, D.] SPP, Irfu, CEA, Saclay, France. [Greder, S.; Miconi, F.; Ripp-Baudot, I.] Univ Strasbourg, CNRS, IN2P3, IPHC, Strasbourg, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon 1, CNRS, IN2P3, IPNL, F-69622 Villeurbanne, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon, Lyon, France. [Hebbeker, T.; Meyer, A.; Sonnenschein, L.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Brandt, O.; Hensel, C.; Mansour, J.; Meyer, J.; Peters, Y.; Quadt, A.; Shabalina, E.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Buescher, V.; Fiedler, F.; Hohlfeld, M.; Weichert, J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Nunnemann, T.; Sanders, M. P.] Univ Munich, Munich, Germany. [Beri, S. B.; Bhatnagar, V.; Dutt, S.; Kohli, J. M.] Panjab Univ, Chandigarh 160014, India. [Choudhary, B.; Dubey, A.] Univ Delhi, Delhi 110007, India. [Acharya, B. S.; Banerjee, S.; Mondal, N. K.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Gruenewald, M. W.] Univ Coll Dublin, Dublin 2, Ireland. [Cho, S. W.; Choi, S.; Jeong, M. S.; Lee, H. S.; Lim, J. K.; Park, S. K.] Korea Univ, Korea Detector Lab, Seoul, South Korea. [Camacho-Perez, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Garcia-Gonzalez, J. A.; Magana-Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.] CINVESTAV, Mexico City 14000, DF, Mexico. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.; van Leeuwen, W. M.] NIKHEF H, NL-1009 DB Amsterdam, Netherlands. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Tokmenin, V. V.; Verkheev, A. Y.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Gavrilov, V.; Kiselevich, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E. E.; Bunichev, V.; Dudko, L. V.; Karmanov, D.; Kuzmin, V. A.; Merkin, M.; Perfilov, M.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Denisov, S. P.; Evdokimov, V. N.; Kozelov, A. V.; Lipaev, V. V.; Popov, A. V.; Prokopenko, N.; Razumov, I.; Shchukin, A. A.; Stoyanova, D. A.; Vasilyev, I. A.] Inst High Energy Phys, Protvino, Russia. [Alkhazov, G.; Lobodenko, A.; Neustroev, P.; Scheglov, Y.; Uvarov, L.; Uvarov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Juste, A.] ICREA, Barcelona, Spain. [Juste, A.] IFAE, Barcelona, Spain. [Buszello, C. P.] Uppsala Univ, Uppsala, Sweden. [Bertram, I.; Borissov, G.; Fox, H.; Ratoff, P. N.; Ross, A.] Univ Lancaster, Lancaster LA1 4YB, England. [Beuselinck, R.; Davies, G.; Hays, J.; Jesik, R.; Jonsson, P.; Scanlon, T.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Agnew, J. P.; Ding, P. F.; Harder, K.; Head, T.; McGivern, C. L.; Petridis, K.; Price, D.; Schwanenberger, C.; Soeldner-Rembold, S.; Suter, L.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Bandurin, D. V.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Bu, X. B.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Garbincius, P. H.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Herner, K.; Illingworth, R.; Ito, A. S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Lee, W. M.; Li, Q. Z.; Lincoln, D.; Lipton, R.; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Verzocchi, M.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.; Shaw, S.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; de Sa, R. Lopes; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Haley, J.; Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Jabeen, S.; Narain, M.; Parihar, V.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna, Russia. RI Fisher, Wade/N-4491-2013; Santos, Angelo/K-5552-2012; Deliot, Frederic/F-3321-2014; Li, Liang/O-1107-2015; Sharyy, Viatcheslav/F-9057-2014; Dudko, Lev/D-7127-2012; Kupco, Alexander/G-9713-2014; Kozelov, Alexander/J-3812-2014; Lokajicek, Milos/G-7800-2014; Lei, Xiaowen/O-4348-2014; Merkin, Mikhail/D-6809-2012; OI Li, Liang/0000-0001-6411-6107; Sharyy, Viatcheslav/0000-0002-7161-2616; Dudko, Lev/0000-0002-4462-3192; Lei, Xiaowen/0000-0002-2564-8351; Williams, Mark/0000-0001-5448-4213; Price, Darren/0000-0003-2750-9977; Bertram, Iain/0000-0003-4073-4941 FU DOE (USA); NSF (USA); CEA (France); CNRS/IN2P3 (France); MON (Russia); NRC KI (Russia); RFBR (Russia); CNPq (Brazil); FAPERJ (Brazil); FAPESP (Brazil); FUNDUNESP (Brazil); DAE (India); DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (Netherlands); STFC (United Kingdom); Royal Society (United Kingdom); MSMT (Czech Republic); GACR (Czech Republic); BMBF (Germany); DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS (China); CNSF (China) FX We thank the staffs at Fermilab and collaborating institutions and acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); MON, NRC KI, and RFBR (Russia); CNPq, FAPERJ, FAPESP, and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (Netherlands); STFC and the Royal Society (United Kingdom); MSMT and GACR (Czech Republic); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 28 TC 32 Z9 32 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 14 PY 2014 VL 89 IS 1 AR 012002 DI 10.1103/PhysRevD.89.012002 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5RQ UT WOS:000331846600001 ER PT J AU Smalyuk, VA Tipton, RE Pino, JE Casey, DT Grim, GP Remington, BA Rowley, DP Weber, SV Barrios, M Benedetti, LR Bleuel, DL Bradley, DK Caggiano, JA Callahan, DA Cerjan, CJ Clark, DS Edgell, DH Edwards, MJ Frenje, JA Gatu-Johnson, M Glebov, VY Glenn, S Haan, SW Hamza, A Hatarik, R Hsing, WW Izumi, N Khan, S Kilkenny, JD Kline, J Knauer, J Landen, OL Ma, T McNaney, JM Mintz, M Moore, A Nikroo, A Pak, A Parham, T Petrasso, R Sayre, DB Schneider, MB Tommasini, R Town, RP Widmann, K Wilson, DC Yeamans, CB AF Smalyuk, V. A. Tipton, R. E. Pino, J. E. Casey, D. T. Grim, G. P. Remington, B. A. Rowley, D. P. Weber, S. V. Barrios, M. Benedetti, L. R. Bleuel, D. L. Bradley, D. K. Caggiano, J. A. Callahan, D. A. Cerjan, C. J. Clark, D. S. Edgell, D. H. Edwards, M. J. Frenje, J. A. Gatu-Johnson, M. Glebov, V. Y. Glenn, S. Haan, S. W. Hamza, A. Hatarik, R. Hsing, W. W. Izumi, N. Khan, S. Kilkenny, J. D. Kline, J. Knauer, J. Landen, O. L. Ma, T. McNaney, J. M. Mintz, M. Moore, A. Nikroo, A. Pak, A. Parham, T. Petrasso, R. Sayre, D. B. Schneider, M. B. Tommasini, R. Town, R. P. Widmann, K. Wilson, D. C. Yeamans, C. B. TI Measurements of an Ablator-Gas Atomic Mix in Indirectly Driven Implosions at the National Ignition Facility SO PHYSICAL REVIEW LETTERS LA English DT Article ID PERFORMANCE AB We present the first results from an experimental campaign to measure the atomic ablator-gas mix in the deceleration phase of gas-filled capsule implosions on the National Ignition Facility. Plastic capsules containing CD layers were filled with tritium gas; as the reactants are initially separated, DT fusion yield provides a direct measure of the atomic mix of ablator into the hot spot gas. Capsules were imploded with x rays generated in hohlraums with peak radiation temperatures of similar to 294 eV. While the TT fusion reaction probes conditions in the central part (core) of the implosion hot spot, the DT reaction probes a mixed region on the outer part of the hot spot near the ablator-hot-spot interface. Experimental data were used to develop and validate the atomic-mix model used in two-dimensional simulations. C1 [Smalyuk, V. A.; Tipton, R. E.; Pino, J. E.; Casey, D. T.; Remington, B. A.; Rowley, D. P.; Weber, S. V.; Barrios, M.; Benedetti, L. R.; Bleuel, D. L.; Bradley, D. K.; Caggiano, J. A.; Callahan, D. A.; Cerjan, C. J.; Clark, D. S.; Edwards, M. J.; Glenn, S.; Haan, S. W.; Hamza, A.; Hatarik, R.; Hsing, W. W.; Izumi, N.; Khan, S.; Landen, O. L.; Ma, T.; McNaney, J. M.; Mintz, M.; Pak, A.; Parham, T.; Sayre, D. B.; Schneider, M. B.; Tommasini, R.; Town, R. P.; Widmann, K.; Yeamans, C. B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grim, G. P.; Kline, J.; Wilson, D. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Edgell, D. H.; Glebov, V. Y.; Knauer, J.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Frenje, J. A.; Gatu-Johnson, M.; Petrasso, R.] MIT, Cambridge, MA 02139 USA. [Kilkenny, J. D.; Nikroo, A.] Gen Atom Co, San Diego, CA 92121 USA. [Moore, A.] AWE Aldermaston, Reading RG7 4PR, Berks, England. RP Smalyuk, VA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Ma, Tammy/F-3133-2013; IZUMI, Nobuhiko/J-8487-2016; Tommasini, Riccardo/A-8214-2009; OI Ma, Tammy/0000-0002-6657-9604; IZUMI, Nobuhiko/0000-0003-1114-597X; Tommasini, Riccardo/0000-0002-1070-3565; Kline, John/0000-0002-2271-9919 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 25 TC 21 Z9 21 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 14 PY 2014 VL 112 IS 2 AR 025002 DI 10.1103/PhysRevLett.112.025002 PG 5 WC Physics, Multidisciplinary SC Physics GA AB7AD UT WOS:000331940800008 PM 24484021 ER PT J AU Balachandran, U Lee, TH Park, CY Emerson, JE Picciolo, JJ Dorris, SE AF Balachandran, U. (Balu) Lee, T. H. Park, C. Y. Emerson, J. E. Picciolo, J. J. Dorris, S. E. TI Dense cermet membranes for hydrogen separation SO SEPARATION AND PURIFICATION TECHNOLOGY LA English DT Article DE Hydrogen transport membrane; Cermet; Dense membrane; Hydrogen flux ID CHEMICAL-STABILITY; PERMEABILITY; CONDUCTORS; TRANSPORT; DOPANTS AB Dense cermet (i.e., ceramic-metal composite) membranes have been developed for separating hydrogen from mixed gases, particularly product streams generated during coal gasification and/or steam methane reforming. Hydrogen separation with these membranes yields high-purity hydrogen, thereby eliminating the need for post-separation purification steps. Extensive tests have been conducted with cermet membranes made by mixing approximate to 50-60 vol.% Pd with Y2O3-stabilized ZrO2. Using several feed gas mixtures, the hydrogen permeation rate, or flux, for the membranes was measured in the temperature range 400-900 degrees C. With pure hydrogen at ambient pressure as feed gas, an approximate to 18-mu m-thick membrane on a porous substrate gave a measured flux of approximate to 26 cm(3)[STP]/min-cm(2) at 400 degrees C and approximate to 52 cm(3)[STP]/min-cm(2) at 900 degrees C. We also measured the hydrogen flux through a thicker (approximate to 150 mu m) membrane at 400 degrees C using a mixture of H-2, CO, CO2, H2O, and He at approximate to 200 psig as feed gas. Hydrogen flux measurements in H2S-containing atmospheres showed that the cermet membranes are stable at 900 degrees C in gases that contain approximate to 80% H-2/400 ppm H2S. Because formation of palladium sulfide (Pd4S) can seriously degrade hydrogen permeation through Pd-containing cermet membranes, the Pd/Pd4S stability phase boundary of the cermet membrane was determined in the temperature range 450-650 degrees C using various feed gases that contained 10-73% H-2 and 8-400 ppm H2S. Given these promising results, longer studies using real-world coal gasification conditions should be pursued. (C) 2013 Elsevier B.V. All rights reserved. C1 [Balachandran, U. (Balu); Lee, T. H.; Park, C. Y.; Emerson, J. E.; Picciolo, J. J.; Dorris, S. E.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Balachandran, U (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM balu@anl.gov FU U.S. Department of Energy, Office of Fossil Energy, National Energy Technology Laboratory's Advanced Fuels Program [DE-AC02-06CH11357] FX Work supported by the U.S. Department of Energy, Office of Fossil Energy, National Energy Technology Laboratory's Advanced Fuels Program, under Contract DE-AC02-06CH11357. NR 18 TC 10 Z9 10 U1 2 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-5866 EI 1873-3794 J9 SEP PURIF TECHNOL JI Sep. Purif. Technol. PD JAN 14 PY 2014 VL 121 SI SI BP 54 EP 59 DI 10.1016/j.seppur.2013.10.001 PG 6 WC Engineering, Chemical SC Engineering GA AB3EH UT WOS:000331673600008 ER PT J AU Engel, JH Alivisatos, AP AF Engel, Jesse H. Alivisatos, A. Paul TI Postsynthetic Doping Control of Nanocrystal Thin Films: Balancing Space Charge to Improve Photovoltaic Efficiency SO CHEMISTRY OF MATERIALS LA English DT Article DE quantum dots; nanocrystals; doping; photovoltaics; compensation ID QUANTUM-DOT PHOTOVOLTAICS; FIELD-EFFECT TRANSISTORS; DOPED SEMICONDUCTOR NANOCRYSTALS; LEVEL TRANSIENT SPECTROSCOPY; SOLAR-CELLS; CDSE NANOCRYSTALS; PBSE NANOCRYSTALS; COLLOIDAL NANOCRYSTALS; ELECTRICAL-PROPERTIES; SURFACE-CHEMISTRY AB A semiconductor nanocrystal film is a unique class of nanocomposite, whose collective properties are determined by those of its constituents. Colloidal synthetic methods offer precise size control and finely tuned optical properties via quantum confinement, while recent improvements in charge transport through films have led to a variety of optoelectronic applications. However, understanding the role a, of defects and impurities in doping, crucial for optimizing device performance, has remained more elusive. In this perspective, we review recent progress in understanding and controlling the doping of semiconductor nanocrystal thin films, with a special focus on its relevance to photovoltaic applications. We highlight an array of postsynthetic techniques based on stoichiometric control, metal impurity incorporation, and electrochemical charging. We conclude with a review of the state of the art for nanocrystal photovoltaics, and propose the use of controlled doping and charge balance as a pathway to higher device efficiencies. C1 [Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM alivis@berkeley.edu RI Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU DOE NSET program on the Self-Assembly of Organic/Inorganic Nanocomposite Materials [DE-AC02-05CH11231] FX The authors gratefully acknowledge financial support by DOE NSET program on the Self-Assembly of Organic/Inorganic Nanocomposite Materials (Grant DE-AC02-05CH11231 to A.P.A), under which all work for this publication was supported. NR 113 TC 18 Z9 19 U1 7 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 14 PY 2014 VL 26 IS 1 SI SI BP 153 EP 162 DI 10.1021/cm402383r PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 299SV UT WOS:000330416900014 ER PT J AU Liu, C Dasgupta, NP Yang, PD AF Liu, Chong Dasgupta, Neil P. Yang, Peidong TI Semiconductor Nanowires for Artificial Photosynthesis SO CHEMISTRY OF MATERIALS LA English DT Article DE nanowire; artificial photosynthesis; solar water splitting ID ATOMIC LAYER DEPOSITION; HYDROGEN EVOLUTION REACTION; ENHANCED PHOTOELECTROCHEMICAL PERFORMANCE; OXYGEN-EVOLVING CATALYST; SOLAR-ENERGY-CONVERSION; WATER OXIDATION; SURFACTANT-FREE; CARBON-DIOXIDE; ACID-SOLUTIONS; H-2 EVOLUTION AB In this Perspective, we discuss current challenges in artificial photosynthesis research, with a focus on the benefits of a nanowire morphology. Matching the flux between electrocatalysts and light-absorbers, and between individual semiconducting light-absorbers, are two major issues to design economically viable devices for artificial photosynthesis. With the knowledge that natural photosynthesis is an integrated nanosystem, individual building blocks of biomimetic artificial photosynthesis are discussed. Possible research directions are presented under an integrated device design scheme, with examples of our current progress in these areas. Coupling all of the components together, including electrocatalysts, light-absorbers, and charge transport units, is crucial due to both fundamental and practical considerations. Given the advantages of one-dimensional nanostructures, it is evident that semiconductor nanowires can function as essential building blocks and help to solve many of the issues in artificial photosynthesis. C1 [Liu, Chong; Dasgupta, Neil P.; Yang, Peidong] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Yang, PD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM p_yang@berkeley.edu OI Liu, Chong/0000-0001-5546-3852 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Awards under the SunShot Solar Energy Technologies Program; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX N.P.D. acknowledges support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Awards under the SunShot Solar Energy Technologies Program. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 82 TC 102 Z9 103 U1 21 U2 283 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 14 PY 2014 VL 26 IS 1 SI SI BP 415 EP 422 DI 10.1021/cm4023198 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 299SV UT WOS:000330416900035 ER PT J AU Reid, OG Pensack, RD Song, Y Scholes, GD Rumbles, G AF Reid, Obadiah G. Pensack, Ryan D. Song, Yin Scholes, Gregory D. Rumbles, Garry TI Charge Photogeneration in Neat Conjugated Polymers SO CHEMISTRY OF MATERIALS LA English DT Article DE excimer; polaron; exciplex; microwave conductivity; transient absorption; pump-probe; pump-dump ID FIELD-EFFECT MOBILITY; 2-DIMENSIONAL ELECTRONIC SPECTROSCOPY; EXCITON-EXCITON ANNIHILATION; POWER-CONVERSION EFFICIENCY; HETEROJUNCTION SOLAR-CELLS; ENERGY-TRANSFER PROCESSES; BAND-GAP POLYMERS; MEH-PPV FILMS; INTERCHAIN INTERACTIONS; REGIOREGULAR POLY(3-HEXYLTHIOPHENE) AB The origin and yield of charges in neat conjugated polymers has long been controversial. In this paper, we review the body of literature that has been created over the past three decades of research in this field and provide insight from our own recent work highlighting the importance of polymer microstructure in understanding the photophysics of these materials. We focus primarily on polythiophene, poly(p-phenylene vinylene), and ladder-type poly(p-phenylene) derivatives, as these three prototypical polymer backbone structures have undergone the most complete study. We find compelling evidence that the primary photoexcitations in conjugated polymers include both intrachain excitons and excimers, that charges are produced in a secondary process, primarily from breakup of intrachain excitons, and that the locus of long-lived charge generation is at the interface between amorphous and crystalline domains of the polymer. Interestingly, the existence of interchromophore complexes that we refer to as excimers has largely been ignored in the development of organic photovoltaics based on conjugated polymers. We suggest that the prevalence of this species may help explain certain mysterious features in that body of work, in particular the excess energy offset required for efficient charge separation in donor/acceptor blends and the requirement for intimately mixed phases of the two materials for maximally efficient photocurrent generation. C1 [Reid, Obadiah G.; Rumbles, Garry] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Pensack, Ryan D.; Song, Yin; Scholes, Gregory D.] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada. [Rumbles, Garry] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Rumbles, G (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM garry.rumbles@nrel.gov OI Rumbles, Garry/0000-0003-0776-1462; REID, OBADIAH/0000-0003-0646-3981 FU National Science and Engineering Research Council of Canada; Laboratory Directed Research and Development (LDRD) Program at the National Renewable Energy Laboratory [06RF1201]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX G.D.S. thanks the National Science and Engineering Research Council of Canada for financial support. This work was supported by the Laboratory Directed Research and Development (LDRD) Program at the National Renewable Energy Laboratory under task number 06RF1201 and the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. O.G.R. and G.R. thank Natalie Stingelin for many edifying discussions on the subject of polymer microstructure. NR 174 TC 36 Z9 36 U1 9 U2 150 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 14 PY 2014 VL 26 IS 1 SI SI BP 561 EP 575 DI 10.1021/cm4027144 PG 15 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 299SV UT WOS:000330416900046 ER PT J AU Norris, AL Nickels, J Sokolov, AP Serpersu, EH AF Norris, Adrianne L. Nickels, Jonathan Sokolov, Alexei P. Serpersu, Engin H. TI Protein Dynamics Are Influenced by the Order of Ligand Binding to an Antibiotic Resistance Enzyme SO BIOCHEMISTRY LA English DT Article ID AMINOGLYCOSIDE-MODIFYING ENZYMES; SOLVENT-EXPOSED AMIDES; CORRELATION SPECTROSCOPY; HEAT-CAPACITY; NMR; SENSITIVITY; NUCLEOTIDYLTRANSFERASE(2'')-IA; PHOSPHOTRANSFERASE(3')-IIIA; ULTRACENTRIFUGATION; THERMODYNAMICS AB The aminoglycoside N3 acetyltransferase-IIIb (AAC) is responsible for conferring bacterial resistance to a variety of aminoglycoside antibiotics. Nuclear magnetic resonance spectroscopy and dynamic light scattering analyses revealed a surprising result; the dynamics of the ternary complex between AAC and its two ligands, an antibiotic and coenzyme A, are dependent upon the order in which the ligands are bound. Additionally, two structurally similar aminoglycosides, neomycin and paromomycin, induce strikingly different dynamic properties when they are in their ternary complexes. To the best of our knowledge, this is the first example of a system in which two identically productive pathways of forming a simple ternary complex yield significant differences in dynamic properties. These observations emphasize the importance of the sequence of events in achieving optimal protein ligand interactions and demonstrate that even a minor difference in molecular structure can have a profound effect on biochemical processes. C1 [Norris, Adrianne L.; Serpersu, Engin H.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Nickels, Jonathan; Sokolov, Alexei P.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Knoxville, TN 37831 USA. [Nickels, Jonathan; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Serpersu, Engin H.] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA. [Serpersu, Engin H.] Oak Ridge Natl Lab, Knoxville, TN 37996 USA. RP Serpersu, EH (reprint author), Univ Tennessee, Walters Life Sci Bldg M407, Knoxville, TN 37996 USA. EM serpersu@utk.edu RI Nickels, Jonathan/I-1913-2012 OI Nickels, Jonathan/0000-0001-8351-7846 FU National Science Foundation [MCB-0842743]; U.S. Department of Energy through the EPSCoR program [DOE-DE-FG02-08ER46528] FX This work is supported by a grant from the National Science Foundation (MCB-0842743 to E.H.S.). J.N. and A.P.S. thank the U.S. Department of Energy for financial support through the EPSCoR program (DOE-DE-FG02-08ER46528). NR 38 TC 1 Z9 1 U1 1 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JAN 14 PY 2014 VL 53 IS 1 BP 30 EP 38 DI 10.1021/bi401635r PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 293VI UT WOS:000330001400007 PM 24320996 ER PT J AU Yang, B Ni, HK Huang, JJ Luo, Y AF Yang, Biao Ni, Hongkai Huang, Jijun Luo, Yi TI Effects of Poly(vinyl butyral) as a Macromolecular Nucleating Agent on the Nonisothermal Crystallization and Mechanical Properties of Biodegradable Poly(butylene succinate) SO MACROMOLECULES LA English DT Article ID PHASE-TRANSITION KINETICS; GROWTH SITE IMPINGEMENT; SUCCINATE)/POLY(VINYL PHENOL) BLEND; NON-ISOTHERMAL CRYSTALLIZATION; VITRO BIOLOGICAL PERFORMANCE; POLY(ETHYLENE OXIDE); HOMOGENEOUS NUCLEATION; MISCIBLE BLENDS; BEHAVIOR; NANOCOMPOSITES AB To improve the crystallization and mechanical properties of poly(butylene succinate) (PBS), a series of poly(vinyl butyral) (PVBs) with various degrees of polymerization, have been synthesized as macromolecular nucleating agents. Nonisothermal crystallization kinetics of PBS nucleated by the PVBs has been examined via polarized optical microscopy and differential scanning calorimetry, followed by detailed analysis with theoretical models. The PVBs are found to significantly increase the number of spherulites and crystallization temperatures by 11 degrees C, and to reduce the spherulite size from 80 to 3 pm and the activation energy from 133 to 53 kJ/mol. Only Avrami and Tobin's models are capable of well characterizing the crystallization kinetics. The effects of the PVBs depend on their concentration and the degree of polymerization, coupled with their miscibility/immiscibility with PBS. Meanwhile, the nucleated PBS exhibits a significant enhancement in mechanical properties: 69% in Young's modulus, 26% in tensile strength, and 14% in impact strength. C1 [Yang, Biao; Ni, Hongkai; Luo, Yi] Beijing Technol & Business Univ, Sch Mat Sci & Mech Engn, Beijing 100048, Peoples R China. [Huang, Jijun] Univ Chinese Acad Sci, Coll Mat Sci & Optoelect Technol, Beijing 100049, Peoples R China. [Huang, Jijun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Yang, B (reprint author), Beijing Technol & Business Univ, Sch Mat Sci & Mech Engn, Beijing 100048, Peoples R China. EM ybiao@btbu.edu.cn; jjh06@mit.edu FU Beijing Natural Science Foundation [2132018]; Scientific Research Program of Beijing Municipal Commission of Education of China [KM200910011005]; Funding Project for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipality, China [PHR200907108, PHR201008248]; US National Institutes of Health/National Institute of Dental and Craniofacial Research (NIH/NIDCR) [1 R01 DE015633] FX We specially acknowledge the support by Beijing Natural Science Foundation (2132018), along with the support by the Scientific Research Program of Beijing Municipal Commission of Education (KM200910011005) of China and Funding Project for Academic Human Resources Development in Institutions of Higher Learning under the Jurisdiction of Beijing Municipality (PHR200907108, PHR201008248) of China. This work was partly supported by the US National Institutes of Health/National Institute of Dental and Craniofacial Research (NIH/NIDCR), Grant No. 1 R01 DE015633. NR 85 TC 2 Z9 2 U1 6 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JAN 14 PY 2014 VL 47 IS 1 BP 284 EP 296 DI 10.1021/ma4019894 PG 13 WC Polymer Science SC Polymer Science GA 293VL UT WOS:000330001700034 ER PT J AU Ju, L Zhang, GL Zhang, X Jia, ZY Gao, XJ Jiang, Y Yan, CL Duerksen-Hughes, PJ Chen, FF Li, HJ Zhu, XQ Yang, J AF Ju, Li Zhang, Guanglin Zhang, Xing Jia, Zhenyu Gao, Xiangjing Jiang, Ying Yan, Chunlan Duerksen-Hughes, Penelope J. Chen, Fanqing Frank Li, Hongjuan Zhu, Xinqiang Yang, Jun TI Proteomic Analysis of Cellular Response Induced by Multi-Walled Carbon Nanotubes Exposure in A549 Cells SO PLOS ONE LA English DT Article ID MICROVASCULAR ENDOTHELIAL-CELLS; DNA-DAMAGE; IN-VITRO; INTRATRACHEAL INSTILLATION; INFLAMMATORY RESPONSE; ACTIN CYTOSKELETON; OXIDATIVE STRESS; EPITHELIAL-CELLS; IMMUNE FUNCTION; HEAT-SHOCK AB The wide application of multi-walled carbon nanotubes (MWCNT) has raised serious concerns about their safety on human health and the environment. However, the potential harmful effects of MWCNT remain unclear and contradictory. To clarify the potentially toxic effects of MWCNT and to elucidate the associated underlying mechanisms, the effects of MWCNT on human lung adenocarcinoma A549 cells were examined at both the cellular and the protein level. Cytotoxicity and genotoxicity were examined, followed by a proteomic analysis (2-DE coupled with LC-MS/MS) of the cellular response to MWCNT. Our results demonstrate that MWCNT induces cytotoxicity in A549 cells only at relatively high concentrations and longer exposure time. Within a relatively low dosage range (30 mg/ml) and short time period (24 h), MWCNT treatment does not induce significant cytotoxicity, cell cycle changes, apoptosis, or DNA damage. However, at these low doses and times, MWCNT treatment causes significant changes in protein expression. A total of 106 proteins show altered expression at various time points and dosages, and of these, 52 proteins were further identified by MS. Identified proteins are involved in several cellular processes including proliferation, stress, and cellular skeleton organization. In particular, MWCNT treatment causes increases in actin expression. This increase has the potential to contribute to increased migration capacity and may be mediated by reactive oxygen species (ROS). C1 [Ju, Li; Zhang, Guanglin; Gao, Xiangjing; Jiang, Ying; Yan, Chunlan; Yang, Jun] Zhejiang Univ, Affiliated Hosp 1, Collaborat Innovat Ctr Diag & Treatment Infect Di, State Key Lab Infect Dis Diag & Therapy,Sch Med, Hangzhou 310003, Zhejiang, Peoples R China. [Ju, Li; Zhang, Guanglin; Gao, Xiangjing; Jiang, Ying; Yan, Chunlan; Zhu, Xinqiang] Zhejiang Univ, Sch Publ Hlth, Dept Toxicol, Hangzhou 310003, Zhejiang, Peoples R China. [Ju, Li; Zhang, Xing; Jia, Zhenyu] Zhejiang Acad Med Sci, Hangzhou, Zhejiang, Peoples R China. [Duerksen-Hughes, Penelope J.] Loma Linda Univ, Div Biochem, Dept Basic Sci, Sch Med, Loma Linda, CA USA. [Chen, Fanqing Frank] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Li, Hongjuan] Hangzhou Normal Univ, Sch Publ Hlth, Hangzhou, Zhejiang, Peoples R China. [Yang, Jun] Zhejiang Agr & Forestry Univ, Coll Biotechnol, Hangzhou, Zhejiang, Peoples R China. RP Zhu, XQ (reprint author), Zhejiang Univ, Sch Publ Hlth, Dept Toxicol, Hangzhou 310003, Zhejiang, Peoples R China. EM zhuxq@zju.edu.cn; gastate@zju.edu.cn FU National Natural Science Foundation of China [81172692, 81202241, 81373036, 81302398]; Provincial Natural Science Foundation [LY12H26006]; Zhejiang Provincial Department of Science and Technology [2013C14016]; Zhejiang Medical Support Plan in Discipline Construction [11ZC02]; Zhejiang Provincial Program for the Cultivation of High-level Innovative Health Talents FX This work was supported by grants from the National Natural Science Foundation of China (No. 81172692, 81202241, 81373036 and 81302398; http://isisn.nsfc.gov.cn/egrantindex/funcindex/prjsearch-list); Zhejiang Provincial Natural Science Foundation (No. LY12H26006; http://www.zjnsf.gov.cn/); Zhejiang Provincial Department of Science and Technology (No. 2013C14016; http://www.zjkjt.gov.cn); and Zhejiang Medical Support Plan in Discipline Construction (11ZC02; http://www.zjwst.gov.cn/). JY is a recipient of the Zhejiang Provincial Program for the Cultivation of High-level Innovative Health Talents (http://www.zjwst.gov.cn/). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 77 TC 18 Z9 20 U1 0 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 14 PY 2014 VL 9 IS 1 AR e84974 DI 10.1371/journal.pone.0084974 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 292TQ UT WOS:000329925800019 PM 24454774 ER PT J AU Lee, CS Dadmun, MD AF Lee, Cameron S. Dadmun, Mark D. TI Important thermodynamic characteristics of poly(3-hexyl thiophene) SO POLYMER LA English DT Article DE Conjugated polymer; Melting enthalpy; Density ID ORGANIC SOLAR-CELLS; REGIOREGULAR POLY(3-HEXYLTHIOPHENE); POLY(3-ALKYL THIOPHENE)S; MOLECULAR-WEIGHT; THIN-FILMS; MORPHOLOGY; CRYSTALLIZATION; HETEROJUNCTIONS; SOLIDIFICATION; POLYTHIOPHENES AB Poly(3-hexyl thiophene) (P3HT) is widely studied as a model material in many electrical and photovoltaic applications, and has become the benchmark polymer when studying the physics of these devices. Despite its extensive use, its precise crystalline structure and thermodynamic characteristics, such as its enthalpy of melting of an ideal crystal, crystalline density, and amorphous density, are not well characterized. This work seeks to provide more certainty in defining these thermodynamic characteristics for regioregular P3HT. This is accomplished by determining the density of rr-P3HT with various thermal histories, and thus percent crystallinity. These densities are correlated to their melting enthalpy melting (Delta H-m) via DSC. This relationship estimates that Delta H-0 for P3HT is between 37 and 50 J/g, that the density of the amorphous portion of semicrystalline rr-P3HT is 1.094 g/cc, and that the density of crystalline P3HT is 1.12-1.14 g/cc. Interestingly, the density of the amorphous portion of rr-P3HT differs significantly from that of regio-random P3HT. This result indicates that the local packing of the segments differs in regio-random P3HT from that in the amorphous portions of rr-P3HT and that care must be expended when equating the behavior of these two phases. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Lee, Cameron S.; Dadmun, Mark D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Dadmun, Mark D.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Dadmun, MD (reprint author), Univ Tennessee, Dept Chem, 1420 Circle Dr, Knoxville, TN 37996 USA. EM Dad@utk.edu OI Dadmun, Mark/0000-0003-4304-6087 FU NSF-EPSCOR [EPS-1004083] FX The authors wish to acknowledge the Sustainable Energy Education Research Center and support from TN-SCORE, a multidisciplinary research program sponsored by NSF-EPSCOR (EPS-1004083), and figure development by Tyler Lee. NR 33 TC 10 Z9 10 U1 2 U2 75 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD JAN 14 PY 2014 VL 55 IS 1 SI SI BP 4 EP 7 DI 10.1016/j.polymer.2013.11.033 PG 4 WC Polymer Science SC Polymer Science GA 296TA UT WOS:000330207100001 ER PT J AU Holley, DW Ruppel, M Mays, JW Urban, VS Baskaran, D AF Holley, D. W. Ruppel, M. Mays, J. W. Urban, V. S. Baskaran, D. TI Polystyrene nanoparticles with tunable interfaces and softness SO POLYMER LA English DT Article DE Nanoparticles; Polystyrene; Neutron scattering ID POLYMER NANOCOMPOSITES; SCATTERING; DISPERSIONS; MICROGELS; DILUTE; SIZE AB Polystyrene nanoparticles, cross-linked with divinylbenzene (PS-(DVB)(x)) and having radii, R-p <= 10 nm, have been synthesized using batch and semi-batch radical microemulsion polymerizations. The nanoparticles were characterized thoroughly using H-1 NMR, size exclusion chromatography, differential scanning calorimety, and various small-angle scattering techniques (light, X-rays, and neutrons). Control over network and interface morphologies of the PS-(DVB)(x), nanoparticles is readily achieved by varying the concentration of divinylbenzene and the polymerization technique (batch vs. semi-batch). Small-angle neutron scattering (SANS) allowed us to identify three distinct nanoparticle morphologies: (i) fuzzy soft gels with flexible chain-segments tethered/looped at the interface of a homogeneous core, (ii) smooth soft gels without a fuzzy interfacial layer, and (iii) dendritic glassy gels exhibiting an inhomogeneous core with an ill-defined interface. Atomic force microscopy imaging supports the morphologies and the softness of the nanoparticles as indicated by SANS. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Holley, D. W.; Mays, J. W.; Baskaran, D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ruppel, M.; Mays, J. W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Urban, V. S.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Baskaran, D (reprint author), AZ Elect Mat USA Corp, 70 Meister Ave, Somerville, NJ 08876 USA. EM baskaran@utk.edu RI Urban, Volker/N-5361-2015 OI Urban, Volker/0000-0002-7962-3408 FU US Department of Energy, Basic Energy Sciences, MSE Division [DE-AC05-000R22725]; DOE/BES FX This research was supported by the US Department of Energy, Basic Energy Sciences, MSE Division (DE-AC05-000R22725), and in part performed at the Center for Nanophase Materials Sciences, sponsored at ORNL by DOE/BES. NR 25 TC 8 Z9 9 U1 5 U2 58 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD JAN 14 PY 2014 VL 55 IS 1 SI SI BP 58 EP 65 DI 10.1016/j.polymer.2013.11.028 PG 8 WC Polymer Science SC Polymer Science GA 296TA UT WOS:000330207100008 ER PT J AU Maya, F Svec, F AF Maya, Fernando Svec, Frantisek TI A new approach to the preparation of large surface area poly(styrene-co-divinylbenzene) monoliths via knitting of loose chains using external crosslinkers and application of these monolithic columns for separation of small molecules SO POLYMER LA English DT Article DE Poly(styrene-co-divinylbenzene); Porous monolith; Hypercrosslinked polymer ID PERFORMANCE LIQUID-CHROMATOGRAPHY; MICROPOROUS ORGANIC POLYMERS; SIZE-EXCLUSION CHROMATOGRAPHY; CAPILLARY COLUMNS; HYPERCROSSLINKED POLYSTYRENE; MACROPOROUS POLYMERS; EFFICIENT SEPARATION; MEDIA; ELECTROCHROMATOGRAPHY; DIMETHACRYLATE AB Poly(styrene-divinylbenzene) monoliths have been hypercrosslinked using a Fe3+ catalyzed Friedel Crafts reaction involving three external crosslinkers (1) 4,4'-bis(chloromethyl)-1,1'-biphenyl, (2) axedichloro-p-xylene, and (3) formaldehyde dimethyl acetal. The first crosslinker was found to produce monoliths with the best chromatographic performance. The effects of a number of variables affecting the hypercrosslinking reaction were studied in detail. These variables included: (i) the temperature and time used for polymerization of the precursor monoliths, (ii) the amount and loading procedure of the external crosslinker and catalyst, and, (iii) the temperature and reaction time of the Friedel Crafts alkylation. Polymers with extremely large surface areas reaching up to 900 m(2)/g were obtained using a precursor monolith polymerized for only 2.5 h, and hypercrosslinked with 4,4'-bis(chloromethyl)-1,1'-biphenyl. The increased performance of monoliths modified using this new procedure is comparable to the performance obtained with monolithic polymers containing chloromethylstyrene. However, the preparation of the poly(styrene-divinylbenzene) precursor is simpler than that of conterparts containing chloromethylstyrene. The hypercrosslinked monoliths in capillary columns were tested in an isocratic reversed phase liquid chromatography separation using a mixture comprised of acetone and six alkyl-benzenes. Column efficiencies for retained analytes exceeded 70,000 plates/m. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Maya, Fernando; Svec, Frantisek] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Svec, F (reprint author), EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM fsvec@lbl.gov RI Maya, Fernando/I-3355-2012; Foundry, Molecular/G-9968-2014 OI Maya, Fernando/0000-0003-1458-736X; FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the U.S. Department of Energy [DE-AC02-05CH11231]; ME-Fulbright fellowship FX All work presented in this paper was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory and supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. The financial support of F.M. by a ME-Fulbright fellowship is gratefully acknowledged. NR 46 TC 40 Z9 40 U1 15 U2 118 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD JAN 14 PY 2014 VL 55 IS 1 SI SI BP 340 EP 346 DI 10.1016/j.polymer.2013.08.018 PG 7 WC Polymer Science SC Polymer Science GA 296TA UT WOS:000330207100043 ER PT J AU He, HK Li, WW Lamson, M Zhong, MJ Konkolewicz, D Hui, CM Yaccato, K Rappold, T Sugar, G David, NE Damodaran, K Natesakhawat, S Nulwala, H Matyjaszewski, K AF He, Hongkun Li, Wenwen Lamson, Melissa Zhong, Mingjiang Konkolewicz, Dominik Hui, Chin Ming Yaccato, Karin Rappold, Timothy Sugar, Glenn David, Nathaniel E. Damodaran, Krishnan Natesakhawat, Sittichai Nulwala, Hunaid Matyjaszewski, Krzysztof TI Porous polymers prepared via high internal phase emulsion polymerization for reversible CO2 capture SO POLYMER LA English DT Article DE Porous polymers; PolyHIPEs; CO2 capture ID CARBON-DIOXIDE CAPTURE; SIDE-CHAIN MONOMERS; AMBIENT AIR; MECHANICAL-PROPERTIES; POLYHIPE MATERIALS; ATMOSPHERIC AIR; SURFACE-AREA; FOAMS; NANOPARTICLES; SCAFFOLDS AB A series of porous polymers with different pore volumes, pore sizes, and crosslinking densities were synthesized by high internal phase emulsion (HIPE) polymerization. The crosslinked polymerized HIPEs (polyHIPEs) were formed by the copolymerization of 4-vinylbenzyl chloride and divinylbenzene using water droplets in conventional or Pickering HIPEs as the templates. These porous materials were further modified by quaternization and ion exchange to introduce quaternary ammonium hydroxide groups. The resulting polyHIPEs were utilized as sorbents for reversible CO2 capture from air using the humidity swing. The effect of pore structure on the CO2 adsorption and desorption processes was studied. The polyHIPEs containing large pores and interconnected porous structures showed improved swing sizes and faster adsorption/desorption kinetics of CO2 compared to a commercial Excellion membrane with similar functional groups. (C) 2013 Elsevier Ltd. All rights reserved. C1 [He, Hongkun; Li, Wenwen; Lamson, Melissa; Zhong, Mingjiang; Konkolewicz, Dominik; Hui, Chin Ming; Nulwala, Hunaid; Matyjaszewski, Krzysztof] Carnegie Mellon Univ, Dept Chem, Ctr Macromol Engn, Pittsburgh, PA 15213 USA. [Yaccato, Karin; Rappold, Timothy; Sugar, Glenn; David, Nathaniel E.] Kilimanjaro Energy Inc, San Francisco, CA 94107 USA. [Damodaran, Krishnan] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Natesakhawat, Sittichai] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Natesakhawat, Sittichai] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15260 USA. RP Matyjaszewski, K (reprint author), Carnegie Mellon Univ, Dept Chem, Ctr Macromol Engn, 4400 5th Ave, Pittsburgh, PA 15213 USA. EM km3b@andrew.cmu.edu RI He, Hongkun/B-4759-2011; Zhong, Mingjiang/F-3470-2011; Matyjaszewski, Krzysztof/A-2508-2008; OI He, Hongkun/0000-0002-7214-3313; Zhong, Mingjiang/0000-0001-7533-4708; Matyjaszewski, Krzysztof/0000-0003-1960-3402; Natesakhawat, Sittichai/0000-0003-1272-1238; Nulwala, Hunaid/0000-0001-7481-3723 FU NSF [CHE-1039870, DMR 09-69301]; DoE [ER-45998]; U.S. Department of Energy's National Energy Technology Laboratory [DE-FE0004000] FX The authors thank Joseph P. Suhan for his help on the SEM and TEM imaging. NSF support (CHE-1039870, and DMR 09-69301) and DoE support (ER-45998) is also acknowledged. This technical effort was also performed in support of U.S. Department of Energy's National Energy Technology Laboratory's on-going research on CO2 capture under the contract DE-FE0004000. NR 72 TC 23 Z9 24 U1 13 U2 130 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD JAN 14 PY 2014 VL 55 IS 1 SI SI BP 385 EP 394 DI 10.1016/j.polymer.2013.08.002 PG 10 WC Polymer Science SC Polymer Science GA 296TA UT WOS:000330207100049 ER PT J AU Choi, SG Hillier, GC Adams, JGJ AF Choi, S. G. Hillier, G. C. Adams, J. G. J. TI Ellipsometric studies of AlxGa1-xAs0.5Sb0.5 (0.0 <= x <= 0.6) alloys lattice-matched to InP(100) SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DIELECTRIC FUNCTION; SPECTROSCOPIC ELLIPSOMETRY; OPTICAL-PROPERTIES; BAND-GAPS; INP; PARAMETERS; SPECTRA; RAMAN; GAAS AB We report on the optical properties of AlxGa1-xAs0.5Sb0.5 (0.0 <= x <= 0.6) alloys grown by metal-organic vapor phase epitaxy on InP(100) substrates for InP-based multi-junction photovoltaic device applications. Spectroscopic ellipsometry is used to determine the complex dielectric function epsilon = epsilon(1) + i epsilon(2), complex refractive index N = n+ik, normal-incidence reflectivity R, and absorption coefficients alpha from 0.73 to 6.45 eV at room temperature. The measured spectra exhibit four above-bandgap critical point (CP) structures E-1, E-1+Delta(1), E-0', and E-2, and the CP energies are accurately obtained from the standard lineshape analysis. The fundamental bandgap E-0 CP energies are estimated from the multilayer modeling of ellipsometric data. Dependence of the CP energies on composition x is discussed. (C) 2014 AIP Publishing LLC. C1 [Choi, S. G.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hillier, G. C.; Adams, J. G. J.] MicroLink Devices Inc, Niles, IL 60714 USA. RP Choi, SG (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM sukgeun.choi@nrel.gov RI Choi, Sukgeun/J-2345-2014 FU U.S. Department of Energy as a part of the Non-Proprietary Partnering Program at the National Renewable Energy Laboratory [DE-AC36-08-GO28308] FX This work was supported by the U.S. Department of Energy as a part of the Non-Proprietary Partnering Program at the National Renewable Energy Laboratory under Contract No. DE-AC36-08-GO28308. NR 35 TC 1 Z9 1 U1 0 U2 3 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 023510 DI 10.1063/1.4861614 PG 6 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700022 ER PT J AU Eremeev, G Palczewski, AD AF Eremeev, G. Palczewski, A. D. TI Characterization of superconducting radiofrequency breakdown by two-mode excitation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NIOBIUM; FIELDS AB We show that thermal and magnetic contributions to the breakdown of superconductivity in radiofrequency (RF) fields can be separated by applying two RF modes simultaneously to a superconducting surface. We develop a simple model that illustrates how mode-mixing RF data can be related to properties of the superconductor. Within our model the data can be described by a single parameter, which can be derived either from RF or thermometry data. Our RF and thermometry data are in good agreement with the model. We propose to use mode-mixing technique to decouple thermal and magnetic effects on RF breakdown of superconductors. (C) 2014 AIP Publishing LLC. C1 [Eremeev, G.; Palczewski, A. D.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Eremeev, G (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM grigory@jlab.org FU U.S. Department of Energy [DE-AC05-06OR23177] FX This manuscript has been authored by Jefferson Science Associates, LLC under Contract No. DE-AC05-06OR23177 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 28 TC 0 Z9 0 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 023901 DI 10.1063/1.4861396 PG 6 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700044 ER PT J AU Harrison, SE Collins-McIntyre, LJ Li, S Baker, AA Shelford, LR Huo, Y Pushp, A Parkin, SSP Harris, JS Arenholz, E van der Laan, G Hesjedal, T AF Harrison, S. E. Collins-McIntyre, L. J. Li, S. Baker, A. A. Shelford, L. R. Huo, Y. Pushp, A. Parkin, S. S. P. Harris, J. S. Arenholz, E. van der Laan, G. Hesjedal, T. TI Study of Gd-doped Bi2Te3 thin films: Molecular beam epitaxy growth and magnetic properties SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID RAY CIRCULAR-DICHROISM; TOPOLOGICAL-INSULATOR; ABSORPTION; HETEROSTRUCTURES; TRANSITION; SURFACE AB Incorporation of magnetic dopants into topological insulators to break time-reversal symmetry is a prerequisite for observing the quantum anomalous Hall (QAHE) effect and other novel magnetoelectric phenomena. GdBiTe3 with a Gd:Bi ratio of 1:1 is a proposed QAHE system, however, the reported solubility limit for Gd doping into Bi2Te3 bulk crystals is between similar to 0.01 and 0.05. We present a magnetic study of molecular beam epitaxy grown (GdxBi1-x)(2)Te-3 thin films with a high Gd concentration, up to x approximate to 0.3. Magnetometry reveals that the films are paramagnetic down to 1.5 K. X-ray magnetic circular dichroism at the Gd M-4,M-5 edge at 1.5 K reveals a saturation field of similar to 6 T, and a slow decay of the magnetic moment with temperature up to 200 K. The Gd3+ ions, which are substitutional on Bi sites in the Bi2Te3 lattice, exhibit a large atomic moment of similar to 7 mu(B), as determined by bulk-sensitive superconducting quantum interference device magnetometry. Surface oxidation and the formation of Gd2O3 lead to a reduced moment of similar to 4 mu(B) as determined by surface-sensitive x-ray magnetic circular dichroism. Their large atomic moment makes these films suitable for incorporation into heterostructures, where interface polarization effects can lead to the formation of magnetic order within the topological insulators. (C) 2014 AIP Publishing LLC. C1 [Harrison, S. E.; Huo, Y.; Harris, J. S.] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Collins-McIntyre, L. J.; Baker, A. A.; Hesjedal, T.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Li, S.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Baker, A. A.; Shelford, L. R.; van der Laan, G.] Diamond Light Source, Magnet Spect Grp, Didcot OX11 0DE, Oxon, England. [Pushp, A.; Parkin, S. S. P.] IBM Almaden Res Ctr, San Jose, CA 95120 USA. [Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hesjedal, T (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. EM Thorsten.Hesjedal@physics.ox.ac.uk RI Hesjedal, Thorsten/C-6853-2014; Baker, Alexander/I-4265-2015; van der Laan, Gerrit/Q-1662-2015; Chapon, Laurent/A-1653-2011; OI Hesjedal, Thorsten/0000-0001-7947-3692; Baker, Alexander/0000-0003-0700-0858; van der Laan, Gerrit/0000-0001-6852-2495; Collins-McIntyre, Liam/0000-0002-9397-1986 FU DARPA MESO [N66001-11-1-4105]; Army Research Laboratories; Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; John Fell Fund (University of Oxford); RCaH; EPSRC (UK) FX This work was supported by a DARPA MESO Project (No. N66001-11-1-4105) and the Army Research Laboratories. S. E. Harrison was supported by the Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program. Diamond Light Source was acknowledged for beamtime allocated on I06. The Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. T. H. wishes to acknowledge funding from the John Fell Fund (University of Oxford) and RCaH for their hospitality, and L. C. M. and A. A. B. acknowledge partial financial support from EPSRC (UK). We would like to thank H. Zhang, S.-C. Zhang, X. Zhang, I. Fisher, W. Han, A. Kellock, Y. Chen, B. Zhou, Z. Liu, H. Yuan, D. Kong, D. Liang, A. Lin, and T. Sarmiento for useful discussions throughout the course of this work. NR 41 TC 19 Z9 19 U1 7 U2 67 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 023904 DI 10.1063/1.4861615 PG 7 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700047 ER PT J AU Kaul, AM Ivanovsky, AV Atchison, WL Petrukhin, AA Duday, PV Griego, JR Salazar, M Nadezhin, SS Tyupanova, OA Oro, DM Holtkamp, DB Rodriguez, G Tabaka, LJ Kraev, AI Skobelev, AN Westley, DT Anderson, BG Ivanov, VA Glybin, AM Kuzyaev, AI Stone, JB Payton, JR Goodwin, PM McCulloch, Q Montoya, RR Dudin, VI Zimenkov, AA Randolph, RB Fierro, F Reinovsky, RE Rousculp, CL Balandina, AN Podurets, AM AF Kaul, A. M. Ivanovsky, A. V. Atchison, W. L. Petrukhin, A. A. Duday, P. V. Griego, J. R. Salazar, M. Nadezhin, S. S. Tyupanova, O. A. Oro, D. M. Holtkamp, D. B. Rodriguez, G. Tabaka, L. J. Kraev, A. I. Skobelev, A. N. Westley, D. T. Anderson, B. G. Ivanov, V. A. Glybin, A. M. Kuzyaev, A. I. Stone, J. B. Payton, J. R. Goodwin, P. M. McCulloch, Q. Montoya, R. R. Dudin, V. I. Zimenkov, A. A. Randolph, R. B. Fierro, F. Reinovsky, R. E. Rousculp, C. L. Balandina, A. N. Podurets, A. M. TI Damage growth and recollection in aluminum under axisymmetric convergence using a helical flux compression generator SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SPALL STRENGTH; FRACTURE; DUCTILE; COPPER; METALS; MODEL AB Damage initiation and evolution, failure, and recollection processes under axisymmetric convergence were studied in the Russian-Damage experimental series, a joint effort between the Los Alamos National Laboratory and the All-Russian Institute of Experimental Physics. A helical explosive magnetic generator was used to drive a cylindrical liner shell to produce shock wave loading of a concentric cylindrical target shell. Shock wave amplitude was controlled by the liner-to-target spacing and by the magnetic field amplitude. Variation of the current pulse duration produced either a single impact, to study damage initiation through failure, or a double impact, to study failure with recollection. Both full and partial recollection of the main crack was obtained. By fielding high-precision diagnostics to measure the dynamic drive conditions and material response and by employing post-shot metallographic analysis, this project produced well-characterized experimental data across a range of damage and recollection levels for the chosen material, aluminum. We present selected experimental results to illustrate the methodology and utility of this experimental technique. (C) 2014 AIP Publishing LLC. C1 [Kaul, A. M.; Atchison, W. L.; Griego, J. R.; Salazar, M.; Oro, D. M.; Holtkamp, D. B.; Rodriguez, G.; Tabaka, L. J.; Westley, D. T.; Anderson, B. G.; Stone, J. B.; Payton, J. R.; Goodwin, P. M.; McCulloch, Q.; Montoya, R. R.; Randolph, R. B.; Fierro, F.; Reinovsky, R. E.; Rousculp, C. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ivanovsky, A. V.; Petrukhin, A. A.; Duday, P. V.; Nadezhin, S. S.; Tyupanova, O. A.; Kraev, A. I.; Skobelev, A. N.; Ivanov, V. A.; Glybin, A. M.; Kuzyaev, A. I.; Dudin, V. I.; Zimenkov, A. A.; Balandina, A. N.; Podurets, A. M.] Russian Fed Nucl Ctr, Sarov 607190, Nizhniy Novgoro, Russia. RP Kaul, AM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM akaul@lanl.gov RI Rodriguez, George/G-7571-2012 OI Rodriguez, George/0000-0002-6044-9462 FU U.S. Department of Energy [DE-AC52-06NA25396] FX The authors would like to acknowledge the metallographic analysis contributions of L. V. Lobova, N. Yu. Ilyushkina, and A. V. Tsibikov. Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 33 TC 3 Z9 4 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 023516 DI 10.1063/1.4861411 PG 13 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700028 ER PT J AU Schulze, PA Ivanov, TW Bolme, CA Brown, KE McGrane, SD Moore, DS AF Schulze, Peter A. Ivanov, Trevor W. Bolme, Cynthia A. Brown, Kathryn E. McGrane, Shawn D. Moore, David S. TI Shock Hugoniot equations of state for binary water-alcohol liquid mixtures SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ETHANOL MIXTURES; MOLECULAR-DYNAMICS; REFRACTIVE-INDEX; AQUEOUS-SOLUTION; SOUND SPEED; COMPRESSION; WAVES; SPECTROSCOPY; VELOCITY; METHANOL AB Shock Hugoniot data were obtained using laser generated shock and ultrafast dynamic ellipsometry (UDE) methods for several non-ideal water-alcohol liquid mixtures, with the alcohols being methanol, ethanol, 1-propanol, 2-propanol, 1-butanol, and t-butanol (a.k.a., 2-methyl-2-propanol or tert-butanol). The sound speeds of the mixtures were obtained using Brillouin scattering when not available in the literature. The shock and particle velocities obtained from the UDE data were compared to expectations of the universal liquid Hugoniot (ULH) and to literature shock (plate impact) data where available. The ethanol/water data were presented in a previous publication [Schulze et al., J. Phys. Chem. A 117, 6158-6163 (2013)]. The shock Hugoniot trends for all these mixtures, here represented as deviations from predictions of the ULH, versus fraction of alcohol are quite similar to each other and suggest that complex hydrogen bonding networks in alcohol-water mixtures alter the compressibility of the mixtures. (C) 2014 AIP Publishing LLC. C1 [Schulze, Peter A.; Ivanov, Trevor W.; Bolme, Cynthia A.; Brown, Kathryn E.; McGrane, Shawn D.; Moore, David S.] Los Alamos Natl Lab, Shock & Detonat Phys Grp, Los Alamos, NM 87545 USA. RP Moore, DS (reprint author), Los Alamos Natl Lab, Shock & Detonat Phys Grp, POB 1663, Los Alamos, NM 87545 USA. EM moored@lanl.gov OI Mcgrane, Shawn/0000-0002-2978-3980; Bolme, Cynthia/0000-0002-1880-271X FU National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; Science Campaign 2: HE Science FX Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC52-06NA25396. The authors gratefully acknowledge the support of this study by Rick Martineau through Science Campaign 2: HE Science. The authors also thank Dr. Joshua Coe and Dr. Emeric Bourasseau for useful discussions, and Dr. Bryce Tappan and Maxwell Schulze for the use of their refractometer. NR 43 TC 0 Z9 0 U1 3 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 023512 DI 10.1063/1.4858385 PG 6 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700024 ER PT J AU Sullivan, KT Swift, D Barham, M Stolken, J Kuntz, J Kumar, M AF Sullivan, Kyle T. Swift, Damian Barham, Matthew Stoelken, James Kuntz, Joshua Kumar, Mukul TI Shock compression behavior of bi-material powder composites with disparate melting temperatures SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DYNAMIC FRAGMENTATION; LASER; SPALLATION; SIMULATION; METALS AB Laser driven experiments were used to investigate the shock compression behavior of powder processed Bismuth/Tungsten (Bi/W) composite samples. The constituents provide different functionality to the composite behavior as Bi could be shock melted at the pressures attained in this work, while the W could not. Samples were prepared by uniaxial pressing, and the relative density was measured as a function of particle size, applied pressure, and composition for both hot and cold pressing conditions. This resulted in sample densities between 73% and 99% of the theoretical maximum density, and also noticeable differences in microstructure in the hot and cold pressed samples. The compression waves were generated with a 1.3 x 1.3mm square spot directly onto the surface of the sample, using irradiances between 10(12) and 10(13) W/cm(2), which resulted in calculated peak pressures between 50 and 150 GPa within a few micrometers. Sample recovery and post-mortem analysis revealed the formation of a crater on the laser drive surface, and the depth of this crater corresponded to the depth to which the Bi had been melted. The melt depth was found to be primarily a function of residual porosity and composition, and ranged from 167 to 528 mu m. In general, a higher porosity led to a larger melt depth. Direct numerical simulations were performed, and indicated that the observed increase in melt depth for low-porosity samples could be largely attributed to increased heating associated with work done for pore collapse. However, the relative scaling was sensitive to composition, with low volume fraction Bi samples exhibiting a much stronger dependence on porosity than high Bi content samples. Select samples were repeated using an Al foil ablator, but there were no noticeable differences ensuring that the observed melting was indeed pressure-driven and was not a result of direct laser heating. The resultant microstructures and damage near the spall surface were also investigated qualitatively. (C) 2014 AIP Publishing LLC. C1 [Sullivan, Kyle T.; Swift, Damian; Barham, Matthew; Stoelken, James; Kuntz, Joshua; Kumar, Mukul] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Sullivan, KT (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 10 TC 0 Z9 0 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 14 PY 2014 VL 115 IS 2 AR 024904 DI 10.1063/1.4861872 PG 10 WC Physics, Applied SC Physics GA 292SN UT WOS:000329922700077 ER PT J AU Coutinho, LH Gardenghi, DJ Schlachter, AS de Souza, GGB Stolte, WC AF Coutinho, L. H. Gardenghi, D. J. Schlachter, A. S. de Souza, G. G. B. Stolte, W. C. TI Positive and negative ion formation in deep-core excited molecules: S 1s excitation in dimethyl sulfoxide SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; CHLORINE K EDGE; BIOINORGANIC CHEMISTRY; CHLOROFORM MOLECULE; GALACTOSE-OXIDASE; PHOTOFRAGMENTATION; PHOTOEXCITATION; IONIZATION; SITE; DISSOCIATION AB The photo-fragmentation of the dimethyl sulfoxide (DMSO) molecule was studied using synchrotron radiation and a magnetic mass spectrometer. The total cationic yield spectrum was recorded in the photon energy region around the sulfur K edge. The sulfur composition of the highest occupied molecular orbital's and lowest unoccupied molecular orbital's in the DMSO molecule has been obtained using both ab initio and density functional theory methods. Partial cation and anion-yield measurements were obtained in the same energy range. An intense resonance is observed at 2475.4 eV. Sulfur atomic ions present a richer structure around this resonant feature, as compared to other fragment ions. The yield curves are similar for most of the other ionic species, which we interpret as due to cascade Auger processes leading to multiply charged species which then undergo Coulomb explosion. The anions S-, C-, and O- are observed for the first time in deep-core-level excitation of DMSO. (C) 2014 AIP Publishing LLC. C1 [Coutinho, L. H.] Univ Fed Rio de Janeiro, Inst Phys, BR-21941972 Rio De Janeiro, RJ, Brazil. [Gardenghi, D. J.; Stolte, W. C.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Schlachter, A. S.; Stolte, W. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [de Souza, G. G. B.] Univ Fed Rio de Janeiro, Inst Chem, BR-21949900 Rio De Janeiro, RJ, Brazil. RP Coutinho, LH (reprint author), Univ Fed Rio de Janeiro, Inst Phys, BR-21941972 Rio De Janeiro, RJ, Brazil. EM lucia@if.ufrj.br FU Brazilian agencies CNPq; FAPERJ; National Science Foundation (NSF) under NSF [PHY-09-70125]; U.S. Department of Energy (DOE) [DE-AC03-76SF00098] FX The authors thank the staff of the ALS for their excellent support. We would also like to thank Dr. Maria Novella Piancastelli for all of the suggestions and help towards the preparation of this paper. L.H.C. and G.G.B.S. would like to acknowledge financial support from the Brazilian agencies CNPq and FAPERJ. W.C.S. and D.J.G. would like to acknowledge support from the National Science Foundation (NSF) under NSF Grant No. PHY-09-70125. This work was performed at the Advanced Light Source, which is supported by U.S. Department of Energy (DOE) (DE-AC03-76SF00098). NR 56 TC 1 Z9 1 U1 0 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 14 PY 2014 VL 140 IS 2 AR 024314 DI 10.1063/1.4861050 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 292TL UT WOS:000329925200027 PM 24437884 ER PT J AU Stinson, JL Kathmann, SM Ford, IJ AF Stinson, Jake L. Kathmann, Shawn M. Ford, Ian J. TI Investigating the significance of zero-point motion in small molecular clusters of sulphuric acid and water SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID AB-INITIO; NUCLEATION; SIMULATIONS; BOND AB The nucleation of particles from trace gases in the atmosphere is an important source of cloud condensation nuclei, and these are vital for the formation of clouds in view of the high supersaturations required for homogeneous water droplet nucleation. The methods of quantum chemistry have increasingly been employed to model nucleation due to their high accuracy and efficiency in calculating configurational energies; and nucleation rates can be obtained from the associated free energies of particle formation. However, even in such advanced approaches, it is typically assumed that the nuclei have a classical nature, which is questionable for some systems. The importance of zero-point motion (also known as quantum nuclear dynamics) in modelling small clusters of sulphuric acid and water is tested here using the path integral molecular dynamics method at the density functional level of theory. The general effect of zero-point motion is to distort the mean structure slightly, and to promote the extent of proton transfer with respect to classical behaviour. In a particular configuration of one sulphuric acid molecule with three waters, the range of positions explored by a proton between a sulphuric acid and a water molecule at 300 K (a broad range in contrast to the confinement suggested by geometry optimisation at 0 K) is clearly affected by the inclusion of zero point motion, and similar effects are observed for other configurations. (C) 2014 AIP Publishing LLC. C1 [Stinson, Jake L.; Ford, Ian J.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Stinson, Jake L.; Ford, Ian J.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Kathmann, Shawn M.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Stinson, JL (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM j.stinson@ucl.ac.uk FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; IMPACT scheme at UCL; U.S. Department of Energy, Office of Science [DE-AC02-05CH11231] FX We thank Professor Angelos Michaelides and his group at UCL for practical advice and helpful discussions; and this work benefited from interactions within the Thomas Young Centre. S.M.K. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. J.L.S. was supported by the IMPACT scheme at UCL and by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. We are grateful for use of the UCL Legion High Performance Computing Facility and the resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the U.S. Department of Energy, Office of Science under Contract No. DE-AC02-05CH11231. NR 41 TC 2 Z9 2 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 14 PY 2014 VL 140 IS 2 AR 024306 DI 10.1063/1.4860973 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 292TL UT WOS:000329925200019 PM 24437876 ER PT J AU Liu, WJ Sharp, ID Tilley, TD AF Liu, Wenjun Sharp, Ian D. Tilley, T. Don TI Multifunctional Silicon Surfaces: Reaction of Dichlorocarbene Generated from Seyferth Reagent with Hydrogen-Terminated Silicon (111) Surfaces SO LANGMUIR LA English DT Article ID HALOMETHYL-METAL COMPOUNDS; SI-C PASSIVATION; SI(111) SURFACES; COVALENT ATTACHMENT; POROUS SILICON; MEDIATED HYDROSILYLATION; SEMICONDUCTOR SURFACES; INFRARED-SPECTROSCOPY; THERMAL-REACTIONS; MONOLAYERS AB Insertion of dichlorocarbene (:CCl2), generated by decomposition of the Seyferth reagent PhHgCCl2Br, into the Si-H bond of a tertiary silane to form a Si-CCl2H group is an efficient homogeneous, molecular transformation. A heterogeneous version of this reaction, between PhHgCCl2Br and a silicon (111) surface terminated by tertiary Si-H bonds, was studied using a combination of surface-sensitive infrared and X-ray photoelectron spectroscopies. The insertion of dichlorocarbene into surface Si H bonds parallels the corresponding reaction of silanes in solution, to produce surface-bound dichloromethyl groups (Si-CCl2H) covering similar to 25% of the silicon surface sites. A significant fraction of the remaining Si-H bonds on the surface was converted to Si-Cl/Br groups during the same reaction, with PhHgCCl2Br serving as a halogen atom source. The presence of two distinct environments for the chlorine atoms (Si-CCl2H and Si-Cl) and one type of bromine atom (Si-Br) was confirmed by Cl 2p, Br 3d, and C 1s X-ray photoelectron spectroscopy. The formation of reactive, halogen-terminated atop silicon sites was also verified by reaction with sodium azide or the Grignard reagent (CH3MgBr), to produce Si-N-3 or Si-Me functionalities, respectively. Thus, reaction of a hydrogen-terminated silicon (111) surface with PhHgCCl2 Br provides a facile route to multifunctional surfaces possessing both stable silicon carbon and labile silicon halogen sites, in a single pot synthesis. The reactive silicon halogen groups can be utilized for subsequent transformations and, potentially, the construction of more complex organic silicon hybrid systems. C1 [Liu, Wenjun; Sharp, Ian D.; Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Liu, Wenjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Sharp, ID (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM idsharp@lbl.gov; tdtilley@berkeley.edu RI Liu, Wenjun/J-8679-2012; Sharp, Ian/I-6163-2015 OI Sharp, Ian/0000-0001-5238-7487 FU Office of Science of the U.S. Department of Energy [DE-SC0004993] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. We thank Dr. Jinhui Yang for her help in obtaining AFM images. NR 58 TC 4 Z9 4 U1 0 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JAN 14 PY 2014 VL 30 IS 1 BP 172 EP 178 DI 10.1021/la403789a PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 293VK UT WOS:000330001600022 PM 24328351 ER PT J AU Donatelli, JJ Sethian, JA AF Donatelli, Jeffrey J. Sethian, James A. TI Algorithmic framework for X-ray nanocrystallographic reconstruction in the presence of the indexing ambiguity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID SERIAL FEMTOSECOND CRYSTALLOGRAPHY; PROTEIN NANOCRYSTALLOGRAPHY; FOURIER-TRANSFORM; PHASE; DIFFRACTION; BIOLOGY AB X-ray nanocrystallography allows the structure of a macromolecule to be determined from a large ensemble of nanocrystals. However, several parameters, including crystal sizes, orientations, and incident photon flux densities, are initially unknown and images are highly corrupted with noise. Autoindexing techniques, commonly used in conventional crystallography, can determine orientations using Bragg peak patterns, but only up to crystal lattice symmetry. This limitation results in an ambiguity in the orientations, known as the indexing ambiguity, when the diffraction pattern displays less symmetry than the lattice and leads to data that appear twinned if left unresolved. Furthermore, missing phase information must be recovered to determine the imaged object's structure. We present an algorithmic framework to determine crystal size, incident photon flux density, and orientation in the presence of the indexing ambiguity. We show that phase information can be computed from nanocrystallographic diffraction using an iterative phasing algorithm, without extra experimental requirements, atomicity assumptions, or knowledge of similar structures required by current phasing methods. The feasibility of this approach is tested on simulated data with parameters and noise levels common in current experiments. C1 [Donatelli, Jeffrey J.; Sethian, James A.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Donatelli, Jeffrey J.; Sethian, James A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Sethian, JA (reprint author), Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. EM sethian@math.berkeley.edu FU Applied Mathematical Sciences subprogram of the Office of Energy Research, US Department of Energy (DOE) [DE-AC02-05CH11231]; Division of Mathematical Sciences of the National Science Foundation; Office of Science of the US DOE [DE-AC02-05CH11231]; Einstein Visiting Fellowship of the Einstein Foundation; DOE Computational Science Graduate Fellowship FX We thank Stefano Marchesini for many valuable conversations. This research was supported in part by the Applied Mathematical Sciences subprogram of the Office of Energy Research, US Department of Energy (DOE) under Contract DE-AC02-05CH11231 and by the Division of Mathematical Sciences of the National Science Foundation, and used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US DOE under Contract DE-AC02-05CH11231. J.A.S. was also supported by an Einstein Visiting Fellowship of the Einstein Foundation, Berlin. J.J.D. was also supported by a DOE Computational Science Graduate Fellowship. NR 28 TC 1 Z9 1 U1 2 U2 12 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 14 PY 2014 VL 111 IS 2 BP 593 EP 598 DI 10.1073/pnas.1321790111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 288LW UT WOS:000329614500021 PM 24344317 ER PT J AU Breuer, M Rosso, KM Blumberger, J AF Breuer, Marian Rosso, Kevin M. Blumberger, Jochen TI Electron flow in multiheme bacterial cytochromes is a balancing act between heme electronic interaction and redox potentials SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE respiration; density functional theory ID REORGANIZATION FREE-ENERGIES; SHEWANELLA-ONEIDENSIS MR-1; SELF-EXCHANGE REACTION; CRYSTAL-STRUCTURE; C-OXIDASE; DECAHEME CYTOCHROMES; STRAIN MR-1; TRANSPORT; NANOWIRES; PROTEIN AB The naturally widespread process of electron transfer from metal reducing bacteria to extracellular solid metal oxides entails unique biomolecular machinery optimized for long-range electron transport. To perform this function efficiently, microorganisms have adapted multiheme c-type cytochromes to arrange heme cofactors into wires that cooperatively span the cellular envelope, transmitting electrons along distances greater than 100 angstrom. Implications and opportunities for bionanotechnological device design are self-evident. However, at the molecular level, how these proteins shuttle electrons along their heme wires, navigating intraprotein intersections and interprotein interfaces efficiently, remains a mystery thus far inaccessible to experiment. To shed light on this critical topic, we carried out extensive quantum mechanics/molecular mechanics simulations to calculate stepwise heme-to-heme electron transfer rates in the recently crystallized outer membrane deca-heme cytochrome MtrF. By solving a master equation for electron hopping, we estimate an intrinsic, maximum possible electron flux through solvated MtrF of 10(4)-10(5) s(-1), consistent with recently measured rates for the related multiheme protein complex MtrCAB. Intriguingly, our calculations show that the rapid electron transport through MtrF is the result of a clear correlation between heme redox potential and the strength of electronic coupling along the wire: thermodynamically uphill steps occur only between electronically well-connected stacked heme pairs. This observation suggests that the protein evolved to harbor low-potential hemes without slowing down electron flow. These findings are particularly profound in light of the apparently well-conserved staggered cross-heme wire structural motif in functionally related outer membrane proteins. C1 [Breuer, Marian; Blumberger, Jochen] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Rosso, Kevin M.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Rosso, KM (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM kevin.rosso@pnnl.gov; j.blumberger@ucl.ac.uk FU Materials Chemistry Consortium from the Engineering and Physical Sciences Research Council [EP/F067496]; Department of Energy Office of Biological and Environmental Research; University College London; PNNL through the US Department of Energy Office of Biological and Environmental Research Subsurface Biogeochemistry Research Science Focus Area program at PNNL; University Research fellowship FX We thank Cortland Johnson [Pacific Northwest National Laboratory (PNNL)] and Julian Breuer for helping with the preparation of Figs. 1 and 3. This work was carried out at the UK High Performance Computing Facility, to which access was granted via the Materials Chemistry Consortium (Grant EP/F067496 from the Engineering and Physical Sciences Research Council), and on Chinook at Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy Office of Biological and Environmental Research and located at PNNL. M. B. gratefully acknowledges an IMPACT studentship cosponsored by University College London and PNNL through the US Department of Energy Office of Biological and Environmental Research Subsurface Biogeochemistry Research Science Focus Area program at PNNL (which provided support for K.M.R.). J.B. thanks the Royal Society for a University Research fellowship. NR 47 TC 44 Z9 45 U1 9 U2 98 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 14 PY 2014 VL 111 IS 2 BP 611 EP 616 DI 10.1073/pnas.1316156111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 288LW UT WOS:000329614500024 PM 24385579 ER PT J AU Shi, QM Ghosh, RP Engelke, H Rycroft, CH Cassereau, L Sethian, JA Weaver, VM Liphardt, JT AF Shi, Quanming Ghosh, Rajarshi P. Engelke, Hanna Rycroft, Chris H. Cassereau, Luke Sethian, James A. Weaver, Valerie M. Liphardt, Jan T. TI Rapid disorganization of mechanically interacting systems of mammary acini SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE mechanobiology; cancer ID EPITHELIAL-MESENCHYMAL TRANSITION; BREAST-CANCER; SPATIAL CONTROL; COLLAGEN GELS; MYOSIN-II; INTEGRIN; CELLS; MORPHOGENESIS; CROSSTALK; INHIBITOR AB Cells and multicellular structures can mechanically align and concentrate fibers in their ECM environment and can sense and respond to mechanical cues by differentiating, branching, or disorganizing. Here we show that mammary acini with compromised structural integrity can interconnect by forming long collagen lines. These collagen lines then coordinate and accelerate transition to an invasive phenotype. Interacting acini begin to disorganize within 12.5 +/- 4.7 h in a spatially coordinated manner, whereas acini that do not interact mechanically with other acini disorganize more slowly (in 21.8 +/- 4.1 h) and to a lesser extent (P < 0.0001). When the directed mechanical connections between acini were cut with a laser, the acini reverted to a slowly disorganizing phenotype. When acini were fully mechanically isolated from other acini and also from the bulk gel by box-cuts with a side length <900 mu m, transition to an invasive phenotype was blocked in 20 of 20 experiments, regardless of waiting time. Thus, pairs or groups of mammary acini can interact mechanically over long distances through the collagen matrix, and these directed mechanical interactions facilitate transition to an invasive phenotype. C1 [Shi, Quanming; Ghosh, Rajarshi P.; Engelke, Hanna; Rycroft, Chris H.; Cassereau, Luke; Sethian, James A.; Weaver, Valerie M.; Liphardt, Jan T.] Univ Calif Berkeley, Bay Area Phys Sci Oncol Ctr, Berkeley, CA 94720 USA. [Shi, Quanming; Ghosh, Rajarshi P.; Engelke, Hanna; Liphardt, Jan T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Rycroft, Chris H.; Sethian, James A.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Rycroft, Chris H.; Sethian, James A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. [Cassereau, Luke; Weaver, Valerie M.] Univ Calif San Francisco, Dept Surg, San Francisco, CA 94143 USA. [Cassereau, Luke; Weaver, Valerie M.] Univ Calif San Francisco, Ctr Bioengn & Tissue Regenerat, San Francisco, CA 94143 USA. RP Weaver, VM (reprint author), Univ Calif Berkeley, Bay Area Phys Sci Oncol Ctr, Berkeley, CA 94720 USA. EM Valerie.Weaver@ucsfmedctr.org; jan.liphardt@stanford.edu RI Shi, Quanming/J-8390-2014; OI Shi, Quanming/0000-0003-2109-5048; Rycroft, Chris/0000-0003-4677-6990 FU National Institutes of Health (NIH) [GM77856]; NIH/National Cancer Institute (NCI) [U54CA143836, R01CA138818]; Applied Mathematical Science subprogram of the Office of Energy Research, US Department of Energy [DE-AC02-05CH11231]; Division of Mathematical Sciences of the National Science Foundation; Miller Foundation at University of California, Berkeley FX We thank Robert I. Saye (Mathematics Department, University of California, Berkeley) for comments and suggestions. We thank the anonymous reviewers for numerous excellent suggestions, including comparing MCF-10AT acini to MCF-7 spheroids and the immuno-fluorescence study of cells streaming from their parent acini. We thank Shelley Hwang, MD, MPH (Duke University), for extensive discussions and suggestions. This work was partially supported by the National Institutes of Health (NIH) Grant GM77856 (to J.T.L.) and NIH/National Cancer Institute (NCI) Grants U54CA143836 (to J.T.L.) and R01CA138818 (to V.M.W.), the Applied Mathematical Science subprogram of the Office of Energy Research, US Department of Energy Contract DE-AC02-05CH11231, and the Division of Mathematical Sciences of the National Science Foundation. J.A.S. was supported by the Miller Foundation at University of California, Berkeley and as an Einstein Visiting Fellow of the Einstein Foundation (Berlin). NR 45 TC 31 Z9 31 U1 2 U2 30 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 14 PY 2014 VL 111 IS 2 BP 658 EP 663 DI 10.1073/pnas.1311312110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 288LW UT WOS:000329614500032 PM 24379367 ER PT J AU Cai, DQ Wu, ZY Jiang, J Wu, YJ Feng, HY Brown, IG Chu, PK Yu, ZL AF Cai, Dongqing Wu, Zhengyan Jiang, Jiang Wu, Yuejin Feng, Huiyun Brown, Ian G. Chu, Paul K. Yu, Zengliang TI Controlling nitrogen migration through micro-nano networks SO SCIENTIFIC REPORTS LA English DT Article ID ACIDIFICATION; COMPOSITE; RELEASE; CLAYS; UREA AB Nitrogen fertilizer unabsorbed by crops eventually discharges into the environment through runoff, leaching and volatilization, resulting in three-dimensional (3D) pollution spanning from underground into space. Here we describe an approach for controlling nitrogen loss, developed using loss control fertilizer (LCF) prepared by adding modified natural nanoclay (attapulgite) to traditional fertilizer. In the aqueous phase, LCF self-assembles to form 3D micro/nano networks via hydrogen bonds and other weak interactions, obtaining a higher nitrogen spatial scale so that it is retained by a soil filtering layer. Thus nitrogen loss is reduced and sufficient nutrition for crops is supplied, while the pollution risk of the fertilizer is substantially lowered. As such, self-fabrication of nano-material was used to manipulate the nitrogen spatial scale, which provides a novel and promising approach for the research and control of the migration of other micro-scaled pollutants in environmental medium. C1 [Cai, Dongqing; Wu, Zhengyan; Jiang, Jiang; Wu, Yuejin; Feng, Huiyun; Yu, Zengliang] Chinese Acad Sci & Anhui Prov, Key Lab Ion Beam Bioengn, Hefei 230031, Peoples R China. [Cai, Dongqing; Wu, Zhengyan; Jiang, Jiang; Wu, Yuejin; Feng, Huiyun; Yu, Zengliang] State Forestry Adm, Bioenergy Forest Res Ctr, Hefei 230031, Peoples R China. [Brown, Ian G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chu, Paul K.] City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China. RP Yu, ZL (reprint author), Chinese Acad Sci & Anhui Prov, Key Lab Ion Beam Bioengn, Hefei 230031, Peoples R China. EM zlyu@ipp.ac.cn RI Chu, Paul/B-5923-2013 OI Chu, Paul/0000-0002-5581-4883 FU The Chinese Ministry of science and technology [10975154, 1206c0805014, 08010302117, 10975145, KSZD-EW-Z-022-05, KSCX2-YW-N-080]; National Natural Science Foundation of China, Anhui province; National Natural Science Foundation of China, Ningxia province; Chinese Academy of Sciences FX The authors acknowledge financial support from the National Natural Science Foundation of China, Anhui province, Ningxia province, Chinese Academy of Sciences and The Chinese Ministry of science and technology: No. 10975154, 1206c0805014, 08010302117, 10975145, KSZD-EW-Z-022-05, KSCX2-YW-N-080. The authors also acknowledge the X-ray imaging (BL13W) and the scanning and transmission X-ray microscopy (BL08U) work stations on Shanghai Synchrotron Radiation Facility (SSRF) for the microstructure observation, and the hard X-ray microscopy work station on National Synchrotron Radiation Laboratory (NSRL) of China for the help of the data analysis. Additionally, we thank S. Yu for his kindly revision of this article, L. F. Wu for her contribution to the application of LCF, N. Wang and G. L. Zhang for their constructive suggestions. NR 19 TC 11 Z9 11 U1 10 U2 64 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 14 PY 2014 VL 4 AR 3665 DI 10.1038/srep03665 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RC UT WOS:000329845800001 PM 24419037 ER PT J AU Gu, M Xiao, XC Liu, G Thevuthasan, S Baer, DR Zhang, JG Liu, J Browning, ND Wang, CM AF Gu, Meng Xiao, Xing-Cheng Liu, Gao Thevuthasan, Suntharampillai Baer, Donald R. Zhang, Ji-Guang Liu, Jun Browning, Nigel D. Wang, Chong-Min TI Mesoscale Origin of the Enhanced Cycling-Stability of the Si-Conductive Polymer Anode for Li-ion Batteries SO SCIENTIFIC REPORTS LA English DT Article ID ELECTROCHEMICAL LITHIATION; SILICON NANOPARTICLES; PHASE-TRANSITION; PERFORMANCE; ELECTRODES; NANOWIRES; TEM AB Electrode used in lithium-ion battery is invariably a composite of multifunctional components. The performance of the electrode is controlled by the interactive function of all components at mesoscale. Fundamental understanding of mesoscale phenomenon sets the basis for innovative designing of new materials. Here we report the achievement and origin of a significant performance enhancement of electrode for lithium ion batteries based on Si nanoparticles wrapped with conductive polymer. This new material is in marked contrast with conventional material, which exhibit fast capacity fade. In-situ TEM unveils that the enhanced cycling stability of the conductive polymer-Si composite is associated with mesoscale concordant function of Si nanoparticles and the conductive polymer. Reversible accommodation of the volume changes of Si by the conductive polymer allows good electrical contact between all the particles during the cycling process. In contrast, the failure of the conventional Si-electrode is probed to be the inadequate electrical contact. C1 [Gu, Meng; Thevuthasan, Suntharampillai; Baer, Donald R.; Wang, Chong-Min] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Xiao, Xing-Cheng] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA. [Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zhang, Ji-Guang; Liu, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Browning, Nigel D.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM gliu@lbl.gov; Chongmin.wang@pnnl.gov RI Baer, Donald/J-6191-2013; Gu, Meng/B-8258-2013; OI Baer, Donald/0000-0003-0875-5961; Browning, Nigel/0000-0003-0491-251X FU Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of DOE [DE-AC02-05CH11231]; Batteries for Advanced TransportationTechnologies (BATT) program [18769]; Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL); U. S. Department of Energy (DOE) [DE-AC05-76RLO1830]; Battelle for the Department of Energy [DE-AC05-76RLO1830]; NSF [DMR-1008104, DMR-1120901] FX This work is supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of DOE under Contract No. DE-AC02-05CH11231, Subcontract No. 18769 under the Batteries for Advanced TransportationTechnologies (BATT) program. The in-situ TEM capability and associated technique development is supported by the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi-program national laboratory operated by Battelle under Contract DE-AC05-76RLO1830 for the U. S. Department of Energy (DOE). The work was conducted in theWilliam R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE'sOffice of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the Department of Energy under Contract DE- AC05-76RLO1830. AK and JL acknowledge support by NSF DMR-1008104 and DMR-1120901. NR 21 TC 17 Z9 17 U1 7 U2 110 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 14 PY 2014 VL 4 AR 3684 DI 10.1038/srep03684 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RF UT WOS:000329846100013 PM 24418812 ER PT J AU Wang, CM Genc, A Cheng, HK Pullan, L Baer, DR Bruemmer, SM AF Wang, Chong-Min Genc, Arda Cheng, Huikai Pullan, Lee Baer, Donald R. Bruemmer, Stephen M. TI In-Situ TEM visualization of vacancy injection and chemical partition during oxidation of Ni-Cr nanoparticles SO SCIENTIFIC REPORTS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; HIGH-TEMPERATURE OXIDATION; CORE-SHELL NANOCLUSTERS; IRON NANOPARTICLES; KIRKENDALL; DIFFUSION; TOMOGRAPHY; SURFACE; NICKEL; ALLOYS AB Oxidation of alloy often involves chemical partition and injection of vacancies. Chemical partition is the consequence of selective oxidation, while injection of vacancies is associated with the differences of diffusivity of cations and anions. It is far from clear as how the injected vacancies behave during oxidation of metal. Using in-situ transmission electron microscopy, we captured unprecedented details on the collective behavior of injected vacancies during oxidation of metal, featuring an initial multi-site oxide nucleation, vacancy supersaturation, nucleation of a single cavity, sinking of vacancies into the cavity and accelerated oxidation of the particle. High sensitive energy dispersive x-ray spectroscopy mapping reveals that Cr is preferentially oxidized even at the initial oxidation, leading to a structure that Cr oxide is sandwiched near the inner wall of the hollow particle. The work provides a general guidance on tailoring of nanostructured materials involving multi-ion exchange such as core-shell structured composite nanoparticles. C1 [Wang, Chong-Min; Baer, Donald R.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Genc, Arda; Cheng, Huikai; Pullan, Lee] FEI Co, Hillsboro, OR 97124 USA. [Bruemmer, Stephen M.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Wang, CM (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. EM chongmin.wang@pnnl.gov RI Baer, Donald/J-6191-2013 OI Baer, Donald/0000-0003-0875-5961 FU US Department of Energy (DOE), Office of Basic Energy Sciences; DOE [DE-AC06-76RLO 1830] FX This work was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences. The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a DOE User Facility operated by Battelle for the DOE Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the DOE under Contract DE-AC06-76RLO 1830. The nanoparticles used in this work were prepared by Professor Qian You of University of Idaho. NR 28 TC 14 Z9 14 U1 4 U2 51 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 14 PY 2014 VL 4 AR 3683 DI 10.1038/srep03683 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RF UT WOS:000329846100012 PM 24418778 ER PT J AU Wu, JJ Lin, JF Wang, XC Liu, QQ Zhu, JL Xiao, YM Chow, P Jin, CQ AF Wu, J. J. Lin, J. F. Wang, X. C. Liu, Q. Q. Zhu, J. L. Xiao, Y. M. Chow, P. Jin, C. Q. TI Magnetic and structural transitions of SrFe2As2 at high pressure and low temperature SO SCIENTIFIC REPORTS LA English DT Article ID SUPERCONDUCTIVITY; LAO1-XFXFEAS AB One of key issues in studying iron based superconductors is to understand how the magnetic phase of the parent compounds evolves. Here we report the systematic investigation of paramagnetic to antiferromagnetic and tetragonal to orthorhombic structural transitions of "122'' SrFe2As2 parent compound using combined high resolution synchrotron Mossbauer spectroscopy and x-ray diffraction techniques in a cryogenically cooled high pressure diamond anvil cell. It is found that although the two transitions are coupled at 205 K at ambient pressure, they are concurrently suppressed to much lower temperatures near a quantum critical pressure of approximately 4.8 GPa where the antiferromagnetic state transforms into bulk superconducting state. Our results indicate that the lattice distortions and magnetism jointly play a critical role in inducing superconductivity in iron based compounds. C1 [Wu, J. J.; Wang, X. C.; Liu, Q. Q.; Zhu, J. L.; Jin, C. Q.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Wu, J. J.; Wang, X. C.; Liu, Q. Q.; Zhu, J. L.; Jin, C. Q.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Wu, J. J.; Lin, J. F.] Univ Texas Austin, Jackson Sch Geosci, Dept Geol Sci, Austin, TX 78712 USA. [Xiao, Y. M.; Chow, P.] Argonne Natl Lab, Adv Photon Source, Carnegie Inst Washington, HPCAT, Argonne, IL 60439 USA. RP Jin, CQ (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM Jin@iphy.ac.cn RI Lin, Jung-Fu/B-4917-2011 FU NFS of China; MOST of China; DOE-NNSA; DOE-BES [DE-AC02-06CH11357]; NFS; Energy Frontier Research in Extreme Environments (EFree) FX Work is supported by NFS and MOST of China through research projects. We appreciate C. Kenney-Benson for his assistance in setting up the cryogenic and online ruby systems at HPCAT. This work was performed at HPCAT (sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT is supported by CIW, CDAC, UNLV and LLNL through funding from DOE-NNSA, DOE-BES and NFS. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. Work at UT Austin is supported by Energy Frontier Research in Extreme Environments (EFree). NR 36 TC 10 Z9 11 U1 0 U2 39 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 14 PY 2014 VL 4 AR 3685 DI 10.1038/srep03685 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291RF UT WOS:000329846100014 PM 24418845 ER PT J AU Kang, ZB Ma, YQ Venugopalan, R AF Kang, Zhong-Bo Ma, Yan-Qing Venugopalan, Raju TI Quarkonium production in high energy proton-nucleus collisions: CGC meets NRQCD SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higher Twist Effects; QCD ID COLOR GLASS CONDENSATE; GLUON DISTRIBUTION-FUNCTIONS; PA-COLLISIONS; BFKL POMERON; HEAVY QUARKONIUM; J/PSI-PRODUCTION; EVOLUTION; QCD; ANNIHILATION; SATURATION AB We study the production of heavy quarkonium states in high energy proton-nucleus collisions. Following earlier work of Blaizot, Fujii, Gelis, and Venugopalan, we systematically include both small x evolution and multiple scattering effects on heavy quark pair production within the Color Glass Condensate (CGC) framework. We obtain for the first time expressions in the Non-Relativistic QCD (NRQCD) factorization formalism for heavy quarkonium differential cross sections as a function of transverse momentum and rapidity. We observe that the production of color singlet heavy quark pairs is sensitive to both "quadrupole" and "dipole" Wilson line correlators, whose energy evolution is described by the Balitsky-JIMWLK equations. In contrast, the color octet channel is sensitive to dipole correlators alone. In a quasi-classical approximation, our results for the color singlet channel reduce to those of Dominguez et al. [1]. We compare our results to those obtained combining the CGC with the color evaporation model and point to qualitative differences in the two approaches. C1 [Kang, Zhong-Bo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ma, Yan-Qing; Venugopalan, Raju] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Kang, ZB (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM zkang@lanl.gov; yqma@bnl.gov; raju@bnl.gov RI Kang, Zhongbo/P-3645-2014 FU U.S. Department of Energy [DE-AC52-06NA25396, DE-AC02-98CH10886] FX We would like to thank F. Dominguez, A. Dumitru, K. Dusling, H. Fujii, J. Lansberg, E. Levin, L. McLerran, Y. Nara, J. Qiu, B. Schenke and F. Yuan for useful discussions. This work was supported by the U.S. Department of Energy, under Contract No. DE-AC52-06NA25396 (ZK) and DE-AC02-98CH10886 (YM and RV). The Feynman diagrams were drawn using Jaxodraw [75]. NR 76 TC 13 Z9 13 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 14 PY 2014 IS 1 AR 056 DI 10.1007/JHEP01(2014)056 PG 33 WC Physics, Particles & Fields SC Physics GA 288OA UT WOS:000329620100002 ER PT J AU Hraber, P Seaman, MS Bailer, RT Mascola, JR Montefiori, DC Korber, BT AF Hraber, Peter Seaman, Michael S. Bailer, Robert T. Mascola, John R. Montefiori, David C. Korber, Bette T. TI Prevalence of broadly neutralizing antibody responses during chronic HIV-1 infection SO AIDS LA English DT Article DE HIV-1; immunity; neutralizing antibodies; serum; vaccines ID MUCOSAL SHIV CHALLENGE; MONOCLONAL-ANTIBODIES; VIRUS; VACCINE; PANEL; PROTECTION; BREADTH; INDIVIDUALS; RECOGNITION; MAGNITUDE AB Objective:Studies of neutralizing antibodies in HIV-1 infected individuals provide insights into the quality of the response that should be possible to elicit with vaccines and ways to design effective immunogens. Some individuals make high titres of exceptional broadly reactive neutralizing antibodies that are of particular interest; however, more modest responses may be a reasonable goal for vaccines. We performed a large cross-sectional study to determine the spectrum of neutralization potency and breadth that is seen during chronic HIV-1 infection. Design:Neutralization potency and breadth were assessed with genetically and geographically diverse panels of 205 chronic HIV-1 sera and 219 Env-pseudotyped viruses representing all major genetic subtypes of HIV-1. Methods:Neutralization was measured by using Tat-regulated luciferase reporter gene expression in TZM-bl cells. Serum-neutralizing activity was compared with a diverse set of human mAbs that are widely considered to be broadly neutralizing. Results:We observed a uniform continuum of responses, with most sera displaying some level of cross-neutralization, and approximately 50% of sera neutralizing more than 50% of viruses. Titres of neutralization (potency) were highly correlated with breadth. Many sera had breadth comparable to several of the less potent broadly neutralizing human mAbs. Conclusion:These results help clarify the spectrum of serum-neutralizing activity induced by HIV-1 infection and that should be possible to elicit with vaccines. Importantly, most people appear capable of making low to moderate titres of broadly neutralizing antibodies. Additional studies of these relatively common responses might provide insights for practical and feasible vaccine designs. (c) 2014 Wolters Kluwer Health | Lippincott Williams & Wilkins C1 [Hraber, Peter; Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM USA. [Seaman, Michael S.] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Bailer, Robert T.; Mascola, John R.] NIAID, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA. [Montefiori, David C.] Duke Univ, Med Ctr, Dept Surg, Durham, NC 27710 USA. RP Montefiori, DC (reprint author), Duke Univ, Med Ctr, Durham, NC 27710 USA. EM monte@duke.edu OI Korber, Bette/0000-0002-2026-5757; Hraber, Peter/0000-0002-2920-4897 FU Bill & Melinda Gates Foundation; Intramural Research Program of the Vaccine Research Center, NIAID, NIH FX This work was funded by a grant from the Bill & Melinda Gates Foundation (Collaboration for AIDS Vaccine Discovery) and by the Intramural Research Program of the Vaccine Research Center, NIAID, NIH. NR 38 TC 99 Z9 99 U1 0 U2 8 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA SN 0269-9370 EI 1473-5571 J9 AIDS JI Aids PD JAN 14 PY 2014 VL 28 IS 2 BP 163 EP 169 DI 10.1097/QAD.0000000000000106 PG 7 WC Immunology; Infectious Diseases; Virology SC Immunology; Infectious Diseases; Virology GA 282QZ UT WOS:000329188800002 PM 24361678 ER PT J AU Gaire, B Lee, SY Haxton, DJ Pelz, PM Bocharova, I Sturm, FP Gehrken, N Honig, M Pitzer, M Metz, D Kim, HK Schoffler, M Dorner, R Gassert, H Zeller, S Voigtsberger, J Cao, W Zohrabi, M Williams, J Gatton, A Reedy, D Nook, C Muller, T Landers, AL Cocke, CL Ben-Itzhak, I Jahnke, T Belkacem, A Weber, T AF Gaire, B. Lee, S. Y. Haxton, D. J. Pelz, P. M. Bocharova, I. Sturm, F. P. Gehrken, N. Honig, M. Pitzer, M. Metz, D. Kim, H. -K. Schoeffler, M. Doerner, R. Gassert, H. Zeller, S. Voigtsberger, J. Cao, W. Zohrabi, M. Williams, J. Gatton, A. Reedy, D. Nook, C. Mueller, Thomas Landers, A. L. Cocke, C. L. Ben-Itzhak, I. Jahnke, T. Belkacem, A. Weber, Th. TI Photo-double-ionization of ethylene and acetylene near threshold SO PHYSICAL REVIEW A LA English DT Article ID CHARGE-TRANSFER SPECTROSCOPY; DIPOLE OSCILLATOR-STRENGTHS; X-RAY PHOTOABSORPTION; DOUBLE PHOTOIONIZATION; ELECTRONIC STATES; PROGRAM SYSTEM; DISSOCIATIVE PHOTOIONIZATION; ASYMMETRY PARAMETERS; POLYATOMIC-MOLECULES; DICATION C2H22+ AB We present kinematically complete measurements of the photo-double-ionization of ethylene (double CC bond) and acetylene (triple CC bond) hydrocarbons just above the double-ionization threshold. We discuss the results in terms of the coincident kinetic energy of the photoelectrons and the nuclear kinetic-energy release of the recoiling ions. We have incorporated quantum chemistry calculations to interpret which of the electronic states of the dication have been populated and trace the various subsequent fragmentation channels. We suggest pathways that involve the electronic ground and excited states of the precursor ethylene dication and explore the strong influence of the conical intersections between the different electronic states. The nondissociative ionization yield is small in ethylene and high in acetylene when compared with the dissociative ionization channels. The reason for such a striking difference is explained in part on the basis of a propensity rule that influences the population of states in the photo-double-ionization of a centrosymmetric closed-shell molecule by favoring singlet ungerade and triplet gerade final states. This propensity rule and the calculated potential-energy surfaces clarify a picture of the dynamics leading to the observed dication dissociation products. C1 [Gaire, B.; Lee, S. Y.; Haxton, D. J.; Pelz, P. M.; Bocharova, I.; Sturm, F. P.; Gehrken, N.; Belkacem, A.; Weber, Th.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Haxton, D. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA. [Sturm, F. P.; Gehrken, N.; Honig, M.; Pitzer, M.; Metz, D.; Kim, H. -K.; Schoeffler, M.; Doerner, R.; Gassert, H.; Zeller, S.; Voigtsberger, J.; Jahnke, T.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Cao, W.; Zohrabi, M.; Cocke, C. L.; Ben-Itzhak, I.] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA. [Williams, J.; Gatton, A.; Reedy, D.; Nook, C.; Landers, A. L.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Mueller, Thomas] Forschungszentrum Julich, Julich Supercomp Ctr, Inst Adv Simulat, D-52425 Julich, Germany. RP Gaire, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RI Doerner, Reinhard/A-5340-2008; cao, wei/D-9643-2015; Schoeffler, Markus/B-6261-2008 OI Doerner, Reinhard/0000-0002-3728-4268; Schoeffler, Markus/0000-0001-9214-6848 FU Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at LBNL [DE-AC02-05CH11231, DE-FG02-86ER13491]; DAAD; DFG; US Government under the DOE FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences and by the Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. W. C., M.Z., C. L. C., and I. B. were supported by Grant No. DE-FG02-86ER13491 from the same funding agency. We acknowledge financial support from the DAAD and the DFG. We thank the staff of the Advanced Light Source, in particular A. Aguilar and D. Kilcoyne from beamline 10.0.1, for their outstanding support. This article is based upon work partially supported by the US Government under the DOE. The views and opinions of the authors expressed herein do not necessarily state or reflect those of the US Government or any agency thereof. The US Government is authorized to reproduce and distribute reprints for governmental purposes. NR 68 TC 8 Z9 8 U1 1 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 13 PY 2014 VL 89 IS 1 AR 013403 DI 10.1103/PhysRevA.89.013403 PG 16 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0GL UT WOS:000332172700008 ER PT J AU Zhou, Y Grinstein, FF Wachtor, AJ Haines, BM AF Zhou, Ye Grinstein, Fernando F. Wachtor, Adam J. Haines, Brian M. TI Estimating the effective Reynolds number in implicit large-eddy simulation SO PHYSICAL REVIEW E LA English DT Article ID ENERGY-DISSIPATION RATE; RICHTMYER-MESHKOV INSTABILITIES; TAYLOR-GREEN VORTEX; TURBULENT FLOWS; ISOTROPIC TURBULENCE; INERTIAL-RANGE; 3-DIMENSIONAL TURBULENCE; NUMERICAL SIMULATIONS; SCALES; RESHOCK AB In implicit large-eddy simulation (ILES), energy-containing large scales are resolved, and physics capturing numerics are used to spatially filter out unresolved scales and to implicitly model subgrid scale effects. From an applied perspective, it is highly desirable to estimate a characteristic Reynolds number (Re)-and therefore a relevant effective viscosity-so that the impact of resolution on predicted flow quantities and their macroscopic convergence can usefully be characterized. We argue in favor of obtaining robust Re estimates away from the smallest scales of the simulated flow-where numerically controlled dissipation takes place and propose a theoretical basis and framework to determine such measures. ILES examples include forced turbulence as a steady flow case, the Taylor-Green vortex to address transition and decaying turbulence, and simulations of a laser-driven reshock experiment illustrating a fairly complex turbulence problem of current practical interest. C1 [Zhou, Ye] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Grinstein, Fernando F.; Wachtor, Adam J.; Haines, Brian M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Zhou, Y (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. OI Haines, Brian/0000-0002-3889-7074; Wachtor, Adam/0000-0003-0609-9171 FU U.S. Department of Energy NNSA [DE-AC52-06NA25396]; Lawrence Livermore National Security; LLC [DE-AC52-07NA27344]; LANL-LDRD [20100441ER] FX Los Alamos National Laboratory (LANL) is operated by the Los Alamos National Security, LLC for the U.S. Department of Energy NNSA under Contract No. DE-AC52-06NA25396. This work was performed under the auspices of the Lawrence Livermore National Security, LLC under Contract No. DE-AC52-07NA27344 and was made possible by funding from the LANL-LDRD Project No. 20100441ER on "LES Modeling for Predictive Simulations of Material Mixing." We thank H. Aluie for providing the code and assistance to compute the energy flux functions in Fig. 6. NR 67 TC 18 Z9 18 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 13 PY 2014 VL 89 IS 1 AR 013303 DI 10.1103/PhysRevE.89.013303 PG 13 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AC0CN UT WOS:000332162500024 PM 24580356 ER PT J AU Landa, A Soderlind, P Yang, LH AF Landa, A. Soederlind, P. Yang, L. H. TI Ab initio phase stability at high temperatures and pressures in the V-Cr system SO PHYSICAL REVIEW B LA English DT Article ID ELASTIC-CONSTANTS; VANADIUM; NB AB The phase stability of vanadium metal and vanadium-chromium alloys at high temperatures and pressures is explored by means of first-principles electronic-structure calculations. Utilizing the self-consistent ab initio lattice dynamics approach in conjunction with density-functional theory, we show that pressure-induced mechanical instability of body-centered cubic vanadium metal, which results in formation of a rhombohedral phase at around 60-70 GPa at room temperature, will survive significant heating and compression. Furthermore, alloying with chromium decreases the temperature at which stabilization of the body-centered cubic phase occurs at elevated pressure. C1 [Landa, A.; Soederlind, P.; Yang, L. H.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Condensed Matter & Mat Div, Livermore, CA 94551 USA. RP Landa, A (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Condensed Matter & Mat Div, Livermore, CA 94551 USA. FU U.S. DOE by LLNL [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [11-ER-033] FX Computing support for this work came from the LLNL Computing Grand Challenge program. This work was performed under the auspices of the U.S. DOE by LLNL under Contract No. DE-AC52-07NA27344 and was funded by the Laboratory Directed Research and Development Program at LLNL under Project Tracking Code No. 11-ER-033. NR 20 TC 5 Z9 5 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 13 PY 2014 VL 89 IS 2 AR 020101 DI 10.1103/PhysRevB.89.020101 PG 4 WC Physics, Condensed Matter SC Physics GA AC0TT UT WOS:000332208900001 ER PT J AU Luo, QL Dagotto, E AF Luo, Qinlong Dagotto, Elbio TI Magnetic phase diagram of a five-orbital Hubbard model in the real-space Hartree-Fock approximation varying the electronic density SO PHYSICAL REVIEW B LA English DT Article ID SEPARATION; SUPERCONDUCTORS; MANGANITES AB Using the real-space Hartree-Fock approximation, the magnetic phase diagram of a five-orbital Hubbard model for the iron-based superconductors is studied varying the electronic density n in the range from five to seven electrons per transition metal atom. The Hubbard interaction U is also varied, at a fixed Hund coupling J/U = 0.25. Several qualitative trends and a variety of competing magnetic states are observed. At n = 5, a robust G-type antiferromagnetic insulator is found, in agreement with experimental results for BaMn2As2. As n increases away from 5, magnetic states with an increasing number of nearest-neighbors ferromagnetic links become energetically stable. This includes the well-known C-type antiferromagnetic state at n = 6, the E-phase known to exist in FeTe, and also a variety of novel states not found yet experimentally, some of them involving blocks of ferromagnetically oriented spins. Regions of phase separation, as in Mn oxides, have also been detected. Comparison to previous theoretical investigations indicate that these qualitative trends may be generic characteristics of phase diagrams of multi-orbital Hubbard models. C1 [Luo, Qinlong; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Luo, Qinlong; Dagotto, Elbio] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Luo, QL (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. FU U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; National Science Foundation [DMR-1104386] FX The work of Q.L. was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. The work of E.D. for this project was supported by the National Science Foundation under Grant No. DMR-1104386. NR 38 TC 13 Z9 13 U1 3 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 13 PY 2014 VL 89 IS 4 AR 045115 DI 10.1103/PhysRevB.89.045115 PG 8 WC Physics, Condensed Matter SC Physics GA AC0UK UT WOS:000332210700002 ER PT J AU Skoropata, E Desautels, RD Chi, CC Ouyang, H Freeland, JW van Lierop, J AF Skoropata, E. Desautels, R. D. Chi, C. -C. Ouyang, H. Freeland, J. W. van Lierop, J. TI Magnetism of iron oxide based core-shell nanoparticles from interface mixing with enhanced spin-orbit coupling SO PHYSICAL REVIEW B LA English DT Article ID RAY CIRCULAR-DICHROISM; HIGH-TEMPERATURE PHASE; GAMMA-FE2O3 NANOPARTICLES; MAGHEMITE NANOPARTICLES; SUBSTITUTED MAGNETITES; MOSSBAUER; COBALT; SPECTROSCOPY; MAGNETIZATION; NANOCRYSTALS AB We show that the magnetism of core-shell nanoparticles (made of maghemite, gamma-Fe2O3, cores and transition-metal and metal-oxide shells) is altered substantially by the interface, which is a doped iron-oxide layer formed naturally during the seed-mediated synthesis process, a route used typically to produce core-shell nanoparticles. Characteristics fundamental to useful applications, such as the anisotropy and superparamagnetic blocking temperature, were altered substantially with Cu, CoO, MnO, and NiO shells. To ascertain the origin of this behavior, the prototype gamma-Fe2O3/CoO core-shell nanoparticles are described in detail. We show that the magnetism originates essentially from an interfacial doped iron-oxide layer formed via migration of shell ions, e.g., Co2+, into octahedral site vacancies in the surface layers of the gamma-Fe2O3 core. For this system, an overall Fe m(orb)/m(spin) = 0.15 +/- 0.03 is measured (m(orb) similar to 0 for the Fe-oxides) and an enhanced Co m(orb)/m(spin) = 0.65 +/- 0.03 elucidates the origin of the unexpectedly high overall anisotropy of the nanoparticle. This interfacial layer is responsible for the overall (e.g., bulk) magnetism and provides a perspective on how the magnetism of core-shell nanoparticles manifests from the selected core and shell materials. C1 [Skoropata, E.; Desautels, R. D.; van Lierop, J.] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada. [Chi, C. -C.; Ouyang, H.] Natl Tsing Hua Univ, Hsinchu, Taiwan. [Freeland, J. W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Skoropata, E (reprint author), Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada. EM eskoropata@physics.umanitoba.ca; Johan.van.Lierop@umanitoba.ca OI Desautels, Ryan/0000-0001-5359-3565 FU US DOE [DE-AC02-06CH11357] FX The authors thank NSERC and CFI of Canada, and NSC of Taiwan. Use of the Advanced Photon Source at Argonne National Laboratories was supported by the US DOE under contract DE-AC02-06CH11357. The authors also thank Dr. Shen-Chuan Lo of the Material and Chemical Research Laboratories, Industrial Technology Research Institute, Taiwan for his assistance with the TEM measurements. NR 43 TC 17 Z9 17 U1 4 U2 54 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 13 PY 2014 VL 89 IS 2 AR 024410 DI 10.1103/PhysRevB.89.024410 PG 9 WC Physics, Condensed Matter SC Physics GA AC0TT UT WOS:000332208900006 ER PT J AU Aoki, Y Shintani, E Soni, A AF Aoki, Y. Shintani, E. Soni, A. TI Proton decay matrix elements on the lattice SO PHYSICAL REVIEW D LA English DT Article ID NUCLEON DECAY AB Hadronic matrix elements of proton decays are essential ingredients for bridging the grand unification theory to low-energy observables like the proton lifetime. In this paper we nonperturbatively calculate the matrix elements, relevant for the process of a nucleon decaying into a pseudoscalar meson and an antilepton through generic baryon-number-violating four-fermi operators. Lattice QCD with 2 + 1 flavor dynamical domain-wall fermions with the direct method-which is the direct measurement of the matrix elements from the three-point function without using chiral perturbation theory-is used for this study in order to have good control over the errors due to lattice discretization effects, operator renormalization, and chiral extrapolation. The relevant form factors for possible transition processes from an initial proton or neutron to a final pion or kaon induced by all types of three-quark operators are obtained through three-point functions of the (nucleon)-(three-quark operator)-(meson) with physical kinematics. In this study all the relevant systematic uncertainties of the form factors are taken into account for the first time, and the total error is found to be in the range 30%-40% for the pi and 20%-40% for the K final states. C1 [Aoki, Y.] Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univ KM, Nagoya, Aichi 4648602, Japan. [Aoki, Y.; Shintani, E.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Soni, A.] Brookhaven Natl Lab, High Energy Theory Grp, Upton, NY 11973 USA. RP Aoki, Y (reprint author), Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univ KM, Nagoya, Aichi 4648602, Japan. EM yaoki@kmi.nagoya-u.ac.jp; shintani@riken.jp; adlersoni@gmail.com RI Shintani, Eigo/C-8623-2016 FU U.S. DOE [DE-AC02-98CH10886]; JSPS Kakenhi Grant [21540289, 22224003]; MEXT Kakenhi Grant [23105714] FX We thank the members of the RBC/UKQCD collaborations for their valuable help with comments and encouragement. We especially would like to thank Peter Boyle, Paul Cooney, Chris Dawson, Luigi Del Debbio, Taku Izubuchi, Chulwoo Jung, Adam Lichtle, Chris Maynard, and Robert Tweedie. Numerical calculations were performed on QCDOC computers of the USQCD Collaboration and the RIKEN BNL Research Center, for which we thank the US DOE and RIKEN BNL Research Center. A. S. is supported by U.S. DOE Contract No. DE-AC02-98CH10886. This work is also supported, in part, by JSPS Kakenhi Grant Nos. 21540289, 22224003 (Y. A.), and by MEXT Kakenhi Grant No. 23105714 (E. S.). NR 26 TC 29 Z9 29 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 13 PY 2014 VL 89 IS 1 AR 014505 DI 10.1103/PhysRevD.89.014505 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5QZ UT WOS:000331844800008 ER PT J AU Czernik, S French, R AF Czernik, Stefan French, Richard TI Distributed production of hydrogen by auto-thermal reforming of fast pyrolysis bio-oil SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Fast pyrolysis; Bio-oil; Catalytic reforming ID NOBLE-METAL CATALYSTS; SYNTHESIS GAS; BIOMASS; GASIFICATION AB We demonstrated an auto-thermal reforming process for producing hydrogen from biomass pyrolysis liquids. Using a noble metal catalyst (0.5% Pt/Al2O3 from BASF) at a methane-equivalent space velocity of around 2000 h(-1), a reformer temperature of 800 degrees C-850 degrees C, a steam-to-carbon ratio of 2.8-4.0, and an oxygen-to-carbon ratio of 0.9-1.1, we produced 9-11 g of hydrogen per 100 g of fast pyrolysis bio-oil, which corresponds to 70%-83% of the stoichiometric potential. The elemental composition of bio-oil and the bio-oil carbon-to-gas conversion, which ranged from 70% to 89%, had the most significant impact on the yield of hydrogen. Because of incomplete volatility the remaining 11%-30% of bio-oil carbon formed deposits in the evaporator. Assuming the same process efficiency as that in the laboratory unit, the cost of hydrogen production in a 1500 kg/day plant was estimated at $4.26/kg with the feedstock, fast pyrolysis bio-oil, contributing 56.3% of the production cost. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Czernik, Stefan; French, Richard] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP French, R (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Richard.French@nrel.gov FU U.S. Department of Energy Fuel Cell Technologies Office [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX We thank Tyler Hammock and Samantha Hart for their help in conducting experiments. This work was supported by the U.S. Department of Energy Fuel Cell Technologies Office under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 19 TC 8 Z9 8 U1 1 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 13 PY 2014 VL 39 IS 2 BP 744 EP 750 DI 10.1016/j.ijhydene.2013.10.134 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA AA5RB UT WOS:000331156200012 ER PT J AU Yi, J Miller, JT Zemlyanov, DY Zhang, RH Dietrich, PJ Ribeiro, FH Suslov, S Abu-Omar, MM AF Yi, Jing Miller, Jeffrey T. Zemlyanov, Dmitry Y. Zhang, Ruihong Dietrich, Paul J. Ribeiro, Fabio H. Suslov, Sergey Abu-Omar, Mahdi M. TI A Reusable Unsupported Rhenium Nanocrystalline Catalyst for Acceptorless Dehydrogenation of Alcohols through gamma-C-H Activation SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE alcohols; dehydrogenation; heterogeneous catalysis; nanoparticles; rhenium ID OXIDANT-FREE DEHYDROGENATION; ACID-BASE SITES; HETEROGENEOUS CATALYST; DEOXYDEHYDRATION; ALUMINA; DEOXYGENATION; NANOPARTICLES; COMPLEXES; OXIDATION; GLYCOLS AB Rhenium nanocrystalline particles (Re NPs), of 2 nm size, were prepared from NH4ReO4 under mild conditions in neat alcohol. The unsupported Re NPs convert secondary and benzylic alcohols to ketones and aldehydes, respectively, through catalytic acceptorless dehydrogenation (AD). The oxidant-and acceptor-free neat dehydrogenation of alcohols to obtain dihydrogen gas is a green and atom-economical process for making carbonyl compounds. Secondary aliphatic alcohols give quantitative conversion and yield. Transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), Re K-edge X-ray absorption near-edge structure (XANES), and X-ray absorption fine structure (EXAFS) data confirmed the characterization of the Re NPs as metallic rhenium with surface oxidation to rhenium(IV) oxide (ReO2). Isotope labeling experiments revealed a novel gamma-CH activation mechanism for AD of alcohols. C1 [Abu-Omar, Mahdi M.] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60429 USA. [Zemlyanov, Dmitry Y.; Suslov, Sergey] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Zhang, Ruihong] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Miller, Jeffrey T.; Dietrich, Paul J.; Ribeiro, Fabio H.; Abu-Omar, Mahdi M.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. RP Abu-Omar, MM (reprint author), Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. EM mabuomar@purdue.edu RI ID, MRCAT/G-7586-2011; Suslov, Sergey/M-8390-2015 FU US Department of Energy, Office of Basic Energy Sciences [DE-FG02-06ER15794, DE-AC02-06CH11357]; US Department of Energy, Office of Basic Energy Sciences FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences (DE-FG02-06ER15794); and (DE-AC02-06CH11357) for Advanced Photon Source use. MRCAT operations were supported by the Department of Energy and the MRCAT member institutions. Funding for J.T.M., P.J.D., and F. H. R. was provided as part of the Institute of Atom-efficient Chemical Transformations, an Energy Frontier Research Center funded by the US Department of Energy, Office of Basic Energy Sciences. Dr. Bruce R. Cooper is acknowledged for assistance with GC-MS; and Dr. Kothanda R. Pichaandi, Dr. Benjamin Wegenhart, and Prof. Christopher Uyeda for helpful discussions. NR 31 TC 13 Z9 13 U1 4 U2 91 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 13 PY 2014 VL 53 IS 3 BP 833 EP 836 DI 10.1002/anie.201307665 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AA3HK UT WOS:000330983300035 PM 24282107 ER PT J AU Brons, JG Hardwick, JA Padilla, HA Hattar, K Thompson, GB Boyce, BL AF Brons, J. G. Hardwick, J. A. Padilla, H. A., II Hattar, K. Thompson, G. B. Boyce, B. L. TI The role of copper twin boundaries in cryogenic indentation-induced grain growth SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Microindentation; Grain growth; Twinning; Coincidence lattice; Precession enhanced diffraction ID CENTERED-CUBIC METALS; IN-SITU OBSERVATION; STEEL THIN-FILMS; NANOCRYSTALLINE NICKEL; MOLECULAR-DYNAMICS; ROOM-TEMPERATURE; DEFORMATION; ALUMINUM; STABILITY; RECOVERY AB Nanostructured Cu films with and without a high density of twins were indented at approximately 77 K with a load of 0.5 N. Utilizing precession-enhanced electron diffraction in the transmission electron microscope, the crystallographic texture, grain size, and grain-to-grain misorientation were quantified. In both orientations, the nanotwinned Cu underwent grain growth in the pile-up region of the indent, with the < 100 > oriented nanotwinned Cu having marked increases in the Sigma 3 and Sigma 5 boundary fractions as compared to the < 111 > orientated nanotwinned Cu. The Cu film without twin boundaries predominately experienced grain distortion and refinement. The twinned grain structure seems to facilitate the observed grain growth, either as a result of the increased mobility of the twin boundaries through a complex mechanically-induced detwinning mechanism and/or microstructure dependent dynamic recrystallization. (C) 2013 Elsevier B.V. All rights reserved. C1 [Brons, J. G.; Hardwick, J. A.; Thompson, G. B.] Univ Alabama, Dept Met Engn, Tuscaloosa, AL 35487 USA. [Padilla, H. A., II; Hattar, K.; Boyce, B. L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Thompson, GB (reprint author), Univ Alabama, Dept Met Engn, Tuscaloosa, AL 35487 USA. EM gthompson@eng.ua.edu FU US Department of Energy, Office of Basic Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences. JGB and GBT received additional supplementary support from NSF-EPS-1158862. UA's Central Analytical Facility is also recognized for support in the use of the FIB, TEM and ASTAR PED platform. Additional FIB access was provided by DOE's Center for Integrated NanoTechnology (CINT). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 45 TC 3 Z9 4 U1 4 U2 30 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JAN 13 PY 2014 VL 592 BP 182 EP 188 DI 10.1016/j.msea.2013.11.005 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AA3WN UT WOS:000331026000024 ER PT J AU Chen, ZH Jiang, XW Dong, S Li, JB Li, SS Wang, LW AF Chen, Zhanghui Jiang, Xiangwei Dong, Shan Li, Jingbo Li, Shushen Wang, Linwang TI Insight into the photoelectron angular dependent energy distribution of negative-electron-affinity InP photocathodes SO APPLIED PHYSICS LETTERS LA English DT Article ID INP(100) SURFACES; MONTE-CARLO; PHOTOEMISSION; TRANSPORT; SEMICONDUCTORS; SPECTROSCOPY; GAAS AB Energy distribution and angular distribution of the photoelectrons from InP photocathodes are investigated using a precise Monte Carlo model. It is found that Gamma-valley electrons contribute to the first peak of the energy distribution curve, but the second peak is contributed by both Gamma-valley and L-valley electrons rather than only L-valley electrons. L valley electrons are shown to have a smaller angular spread than Gamma-valley electrons, which is attributed to the much higher potential energy of L-valley minimum. The further simulation indicates that the performance of InP photocathodes can be improved by increasing the hole concentration or decreasing the temperature, but the activation layer thickness variation only has very slight influence on either energy or angular distribution. (C) 2014 AIP Publishing LLC. C1 [Chen, Zhanghui; Jiang, Xiangwei; Dong, Shan; Li, Jingbo; Li, Shushen] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Wang, Linwang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Li, JB (reprint author), Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, POB 912, Beijing 100083, Peoples R China. EM jbli@semi.ac.cn FU National Natural Science Foundation of China [91233120, 61106091]; National Basic Research Program of China [2011CB921901]; Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S. Department of Energy (DOE) [DEAC02-05CH11231]; China Scholarship Council; Graduate Innovation Fund of University of Chinese Academy of Sciences FX J. Li gratefully acknowledges the funds from National Natural Science Foundation of China under Grant No. 91233120 and the National Basic Research Program of China (2011CB921901). The work of X. W. Jiang is supported by the National Natural Science Foundation of China under Grants No. 61106091. The work of L. W. Wang is supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S. Department of Energy (DOE) under Contract No. DEAC02-05CH11231. Z. H. Chen thanks the financial support of China Scholarship Council and Graduate Innovation Fund of University of Chinese Academy of Sciences. NR 29 TC 1 Z9 2 U1 3 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 021120 DI 10.1063/1.4862645 PG 4 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000020 ER PT J AU Dattelbaum, DM Chellappa, RS Bowden, PR Coe, JD Margevicius, MA AF Dattelbaum, Dana M. Chellappa, Raja S. Bowden, Patrick R. Coe, Joshua D. Margevicius, Madeline A. TI Chemical stability of molten 2,4,6-trinitrotoluene at high pressure SO APPLIED PHYSICS LETTERS LA English DT Article ID THERMAL-DECOMPOSITION; KINETIC-PARAMETERS; AMORPHOUS-CARBON; POLYMORPHISM; EXPLOSIVES; TNT; DETONATION; LIQUID; TRINITROTOLUENE; SPECTROSCOPY AB 2,4,6-trinitrotoluene (TNT) is a molecular explosive that exhibits chemical stability in the molten phase at ambient pressure. A combination of visual, spectroscopic, and structural (x-ray diffraction) methods coupled to high pressure, resistively heated diamond anvil cells was used to determine the melt and decomposition boundaries to > 15 GPa. The chemical stability of molten TNT was found to be limited, existing in a small domain of pressure-temperature conditions below 2 GPa. Decomposition dominates the phase diagram at high temperatures beyond 6 GPa. From the calculated bulk temperature rise, we conclude that it is unlikely that TNT melts on its principal Hugoniot. (C) 2014 AIP Publishing LLC. C1 [Dattelbaum, Dana M.; Chellappa, Raja S.; Bowden, Patrick R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Coe, Joshua D.; Margevicius, Madeline A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Dattelbaum, DM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM danadat@lanl.gov FU DOE/NNSA; LDRD program [2011012DR]; DOE/NNSA [DE-NA0001974]; DOE/BES [DE-FG02-00ER45775, DE-AC02-06CH11357]; NSF FX Los Alamos National Laboratory is operated by LANS, LLC for the U. S. Department of Energy. Funding for this work was provided by DOE/NNSA and the LDRD program under Project No. #2011012DR. The authors are grateful to Virginia (Tate) Hamilton for providing the TNT crystals, Zhenxian Liu for assistance at the U2A beamline at NSLS, and to the Carnegie DOE-Alliance Center (CDAC) for beam time at APS Sector 16-ID-B, and NSLS U2A. Portions of this work were performed at HP-CAT (Sector 16), Advanced Photon Source, Argonne National Laboratory. HP-CAT operations are supported by DOE/NNSA under Award No. DE-NA0001974, and DOE/BES under Award No. DE-FG02-00ER45775, with partial instrumentation funding by NSF. APS is supported by DOE/BES, under Contract No. DE-AC02-06CH11357. We acknowledge insightful conversations with Stephen Sheffield, and help with experiments from Jesse Smith and Stas Sinogeikin at HP-CAT. NR 56 TC 2 Z9 2 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 021911 DI 10.1063/1.4860395 PG 5 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000039 ER PT J AU Jiang, XW Gong, J Xu, N Li, SS Zhang, JF Hao, Y Wang, LW AF Jiang, Xiang-Wei Gong, Jian Xu, Nuo Li, Shu-Shen Zhang, Jinfeng Hao, Yue Wang, Lin-Wang TI Enhancement of band-to-band tunneling in mono-layer transition metal dichalcogenides two-dimensional materials by vacancy defects SO APPLIED PHYSICS LETTERS LA English DT Article ID MOS2 TRANSISTORS; PHOTOLUMINESCENCE AB The band-to-band tunneling of monolayer transition metal dichalcogenides nano-junction is investigated using atomistic ab initio quantum transport simulations. From the simulation, it is found that the transition metal vacancy defect in the two-dimensional MX2 (M = Mo, W; X = S, Se) band-to-band tunneling diode can dramatically boost the on-state current up to 10 times while maintaining the device sub-threshold swing. The performance enhancement mechanism is discussed in detail by examining partial density of states of the system. It is found that the transition metal vacancy induces band-gap states, which reduce the effective length of the tunneling transition region. (C) 2014 AIP Publishing LLC. C1 [Jiang, Xiang-Wei; Li, Shu-Shen] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Gong, Jian] Inner Mongolia Univ, Sch Phys Sci & Technol, Hohhot 010021, Peoples R China. [Xu, Nuo] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Zhang, Jinfeng; Hao, Yue] Xidian Univ, Sch Microelect, Key Lab Wide Band Gap Semicond Mat & Devices, Xian 710071, Peoples R China. [Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wang, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM lwwang@lbl.gov RI Xu, Nuo/G-1768-2014 FU Office of Naval Research through Princeton University [00001914]; U.S. Department of Energy [DE-AC02-05CH11231]; National Basic Research Program of China (973 Program) [G2009CB929300]; National Natural Science Foundation of China [61121491, 61106091] FX The authors would like to thank Dr. Jun Kang for helpful discussions. This work was supported by the Office of Naval Research through a sub award from Princeton University under Contract No. 00001914, through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work of X. W. Jiang and S. S. Li was partially supported by the National Basic Research Program of China (973 Program) Grant No. G2009CB929300 and the National Natural Science Foundation of China under Grant Nos. 61121491 and 61106091. NR 20 TC 8 Z9 8 U1 5 U2 66 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 023512 DI 10.1063/1.4862667 PG 4 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000124 ER PT J AU Morris, CL Bacon, J Ban, Y Borozdin, K Fabritius, JM Izumi, M Miyadera, H Mizokami, S Otsuka, Y Perry, J Ramsey, J Sano, Y Sugita, T Yamada, D Yoshida, N Yoshioka, K AF Morris, C. L. Bacon, Jeffery Ban, Yuichiro Borozdin, Konstantin Fabritius, J. M. Izumi, Mikio Miyadera, Haruo Mizokami, Shinya Otsuka, Yasuyuki Perry, John Ramsey, John Sano, Yuji Sugita, Tsukasa Yamada, Daichi Yoshida, Noriyuki Yoshioka, Kenichi TI Analysis of muon radiography of the Toshiba nuclear critical assembly reactor SO APPLIED PHYSICS LETTERS LA English DT Article ID SCATTERING AB A 1.2 x 1.2 m(2) muon tracker was moved from Los Alamos to the Toshiba facility at Kawasaki, Japan, where it was used to take similar to 4 weeks of data radiographing the Toshiba Critical Assembly Reactor with cosmic ray muons. In this paper, we describe the analysis procedure, show results of this experiment, and compare the results to Monte Carlo predictions. The results validate the concept of using cosmic rays to image the damaged cores of the Fukushima Daiichi reactors. (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Morris, C. L.; Bacon, Jeffery; Borozdin, Konstantin; Fabritius, J. M.; Miyadera, Haruo; Perry, John; Ramsey, John] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ban, Yuichiro; Izumi, Mikio; Miyadera, Haruo; Sano, Yuji; Yoshida, Noriyuki] Toshiba Co Ltd, Isogo Ku, Yokohama, Kanagawa 2358523, Japan. [Mizokami, Shinya; Otsuka, Yasuyuki; Yamada, Daichi] Tokyo Elect Power Co Ltd, Chiyoda Ku, Tokyo, Japan. [Sugita, Tsukasa; Yoshioka, Kenichi] Toshiba Co Ltd, Kawasaki Ku, Kawasaki, Kanagawa 2100862, Japan. RP Morris, CL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Morris, Christopher/0000-0003-2141-0255; Perry, John/0000-0003-3639-5617 FU Tokyo Electric Power Company; Toshiba Corporation, Power Systems Company FX This work has been supported by the Tokyo Electric Power Company and by Toshiba Corporation, Power Systems Company. NR 12 TC 5 Z9 5 U1 1 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 024110 DI 10.1063/1.4862475 PG 4 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000141 ER PT J AU Savukov, I Karaulanov, T Boshier, MG AF Savukov, I. Karaulanov, T. Boshier, M. G. TI Ultra-sensitive high-density Rb-87 radio-frequency magnetometer SO APPLIED PHYSICS LETTERS LA English DT Article ID ATOMIC MAGNETOMETER; NMR AB Radio-frequency (RF) atomic magnetometers (AMs) can be used in many applications, such as magnetic resonance imaging and nuclear quadrupole resonance. High-density AMs provide both superior sensitivity and large bandwidth. Previously, high-density potassium AMs were demonstrated, but these magnetometers have various disadvantages, such as high-temperature of operation and bulky design. We demonstrate a rubidium-87 RF AM with 5 fT/Hz(1/2) sensitivity (3 fT Hz(1/2) probe noise), which is comparable to that of the best potassium magnetometers. Our magnetometer also features a simple fiber-optic design, providing maximum flexibility for magnetic-field measurements. (C) 2014 AIP Publishing LLC. C1 [Savukov, I.; Boshier, M. G.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Karaulanov, T.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Savukov, I (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RI Boshier, Malcolm/A-2128-2017; OI Boshier, Malcolm/0000-0003-0769-1927; Savukov, Igor/0000-0003-4190-5335 FU U.S. DOE through the LANL/LDRD program FX This work was supported by the U.S. DOE through the LANL/LDRD program. NR 12 TC 13 Z9 14 U1 6 U2 33 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 023504 DI 10.1063/1.4861657 PG 3 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000116 ER PT J AU Smilowitz, L Henson, BF Romero, JJ Oschwald, D AF Smilowitz, L. Henson, B. F. Romero, J. J. Oschwald, D. TI Thermal decomposition of energetic materials viewed via dynamic x-ray radiography SO APPLIED PHYSICS LETTERS LA English DT Article ID DELTA PHASE-TRANSITION; HIGH EXPLOSIVE LX-04; COOK-OFF; VIOLENCE AB We describe the evolution of solid density, leading up to ignition in the slow thermal decomposition of the solid organic secondary explosive octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine. This work describes an x-ray radiographic diagnostic, allowing the study of solid density in a fully encased explosive heated to thermal explosion. The result of this study is the ability to observe and manipulate the ignition volume in a thermal explosion. (C) 2014 AIP Publishing LLC. C1 [Smilowitz, L.; Henson, B. F.; Romero, J. J.; Oschwald, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Smilowitz, L (reprint author), Los Alamos Natl Lab, C PCS J567, Los Alamos, NM 87545 USA. FU Science Campaign and Surety Programs administered by Los Alamos National Laboratory; Joint Munitions Program administered jointly by the Departments of Energy and Defense FX The authors wish to acknowledge support from the Science Campaign and Surety Programs administered by Los Alamos National Laboratory and the Joint Munitions Program administered jointly by the Departments of Energy and Defense. NR 12 TC 4 Z9 4 U1 3 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 024107 DI 10.1063/1.4858965 PG 4 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000138 ER PT J AU Zhou, X Deeb, C Vincent, R Lerond, T Adam, PM Plain, J Wiederrecht, GP Charra, F Fiorini, C des Francs, GC Soppera, O Bachelot, R AF Zhou, X. Deeb, C. Vincent, R. Lerond, T. Adam, P. -M. Plain, J. Wiederrecht, G. P. Charra, F. Fiorini, C. des Francs, G. Colas Soppera, O. Bachelot, R. TI Polarization-dependent fluorescence from an anisotropic gold/polymer hybrid nano-emitter SO APPLIED PHYSICS LETTERS LA English DT Article ID GOLD NANOPARTICLES; ENERGY-TRANSFER; WATER SOLUTION; NEAR-FIELD; SURFACE; RESONANCE; ENHANCEMENTS; NANOANTENNA; PLASMONS AB Based on nanoscale photopolymerization triggered by the dipolar surface plasmon mode, we developed a light-emitting gold nanoparticle/Eosin Y-doped polymer hybrid nanostructure. Due to the anisotropic spatial distribution of the dipolar surface plasmon mode during photopolymerization, this nano-emitter is anisotropic in both geometry and emission. The trapped dye molecules in the hybrid nanostructure display fluorescence intensity that is dependent upon the polarization of the incident excitation light. This nano-emitter further allows the photo-selection of fluorescence configuration (i.e., molecule concentration and refractive index of active medium) by controlling the incident polarization. (C) 2014 AIP Publishing LLC. C1 [Zhou, X.; Deeb, C.; Vincent, R.; Lerond, T.; Adam, P. -M.; Plain, J.; Bachelot, R.] Univ Technol Troyes, ICD, LNIO, CNRS,UMR 6279, F-10004 Troyes, France. [Wiederrecht, G. P.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Charra, F.; Fiorini, C.] CEA, IRAMIS, Ctr Etud Saclay, Serv Phys & Chim Surfaes & Interfaces, F-91191 Gif Sur Yvette, France. [des Francs, G. Colas] Univ Bourgogne, Lab Interdisciplinaire Carnot Bourgogne ICB, F-21078 Dijon, France. [Soppera, O.] Univ Haute Alsace, CNRS, UMR 7361, IS2M, Mulhouse, France. RP Zhou, X (reprint author), Univ Technol Troyes, ICD, LNIO, CNRS,UMR 6279, 12 Rue Marie Curie CS 42060, F-10004 Troyes, France. EM renaud.bachelot@utt.fr RI Bachelot, Renaud/M-6888-2015; OI Deeb, Claire/0000-0002-1323-0660; Charra, Fabrice/0000-0003-1228-0583 FU Agence Nationale de la Recherche (ANR) [ANR-12-BS10-0016, ANR-10-BLAN-1016, ANR-12-NANO-0019]; Partner University Fund (PUF) program; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; China Scholarship Council (CSC) FX The authors would like to thank the platform Nano'mat, the HAPPLE (ANR-12-BS10-0016), HYNNA (ANR-10-BLAN-1016), and SINPHONIE (ANR-12-NANO-0019) projects funded by Agence Nationale de la Recherche (ANR), as well as the Partner University Fund (PUF) program. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. X.Z. wishes to thank China Scholarship Council (CSC) for funding. NR 34 TC 4 Z9 4 U1 5 U2 51 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 13 PY 2014 VL 104 IS 2 AR 023114 DI 10.1063/1.4861898 PG 5 WC Physics, Applied SC Physics GA 299YG UT WOS:000330431000102 ER PT J AU Lin, YG Hsu, YK Basilio, AM Chen, YT Chen, KH Chen, LC AF Lin, Yan-Gu Hsu, Yu-Kuei Basilio, Antonio M. Chen, Yit-Tsong Chen, Kuei-Hsien Chen, Li-Chyong TI Photoelectrochemical activity on Ga-polar and N-polar GaN surfaces for energy conversion SO OPTICS EXPRESS LA English DT Article ID WATER OXIDATION; VISIBLE-LIGHT; PHOTOANODES; NANOWIRES; HYDROGEN AB Hydrogen generation through direct photoelectrolysis of water was studied using photoelectrochemical cells made of different facets of free-standing polar GaN system. To build the fundamental understanding at the differences of surface photochemistry afforded by the GaN {0001} and {000-1} polar surfaces, we correlated the relationship between the surface structure and photoelectrochemical performance on the different polar facets. The photoelectrochemical measurements clearly revealed that the Ga-polar surface had a more negative onset potential relative to the N-polar surface due to the much negative flat-band potential. At more positive applied voltages, however, the N-polar surface yielded much higher photocurrent with conversion efficiency of 0.61% compared to that of 0.55% by using the Ga-polar surface. The reason could be attributed to the variation in the band structure of the different polar facets via Mott-Schottky analyses. Based on this work, understanding the facet effect on photoelectrochemical activity can provide a blueprint for the design of materials in solar hydrogen applications. (C) 2013 Optical Society of America C1 [Lin, Yan-Gu; Basilio, Antonio M.; Chen, Yit-Tsong; Chen, Kuei-Hsien] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. [Lin, Yan-Gu; Chen, Kuei-Hsien; Chen, Li-Chyong] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Lin, Yan-Gu] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Hsu, Yu-Kuei] Natl Dong Hwa Univ, Dept Optoelect Engn, Hualien 97401, Taiwan. [Basilio, Antonio M.; Chen, Yit-Tsong] Natl Taiwan Univ, Dept Chem, Taipei 10617, Taiwan. [Basilio, Antonio M.] Ateneo de Manila Univ Quezon City, Dept Chem, Quezon City 1108, Philippines. RP Chen, LC (reprint author), Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. EM chenkh@pub.iams.sinica.edu.tw; chenlc@ntu.edu.tw RI Chen, Yit-Tsong/F-7935-2012; Hsu, Yu-Kuei/H-6591-2014; Chen, Kuei-Hsien/F-7924-2012; Chen, Li-Chyong/B-1705-2015 OI Chen, Yit-Tsong/0000-0002-6204-8320; Chen, Li-Chyong/0000-0001-6373-7729 FU National Natural Science Council, Ministry of Education, Taiwan; AOARD under AFSOR, US; NSC; IAMS; NTU FX This work was supported by the National Natural Science Council, Ministry of Education, Taiwan, and AOARD under AFSOR, US. We gratefully thank NSC, IAMS, and NTU for financial support for this project. NR 20 TC 6 Z9 6 U1 5 U2 52 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 13 PY 2014 VL 22 IS 1 BP A21 EP A27 DI 10.1364/OE.22.000A21 PG 7 WC Optics SC Optics GA 302CP UT WOS:000330579300011 PM 24921996 ER PT J AU Pang, YT Bossart, M Eisaman, MD AF Pang, Y. T. Bossart, M. Eisaman, M. D. TI Index-matched IWKB method for the measurement of spatially varying refractive index profiles within thin-film photovoltaics SO OPTICS EXPRESS LA English DT Article ID OPTICAL WAVE-GUIDES; SOLAR-CELLS; CONSTRUCTION AB In many thin-film photovoltaic devices, the photoactive layer has a spatially varying refractive index in the substrate-normal direction, but measurement of this variation with high spatial resolution is difficult due to the thinness of these layers (typically 200 nm for organic photovoltaics). We demonstrate a new method for reconstructing the depth-dependent refractive-index profile with high spatial resolution (similar to 10 nm at a wavelength of 500 nm) in thin (200 nm) photoactive layers by depositing a relatively thick index-matched layer (1-10 mu m) adjacent to the photoactive layer and applying the Inverse Wentzel-Kramers-Brillouin (IWKB) method. This novel technique, which we refer to as index-matched IWKB (IMIWKB), is applicable to any thin film, including the photoactive layers of a broad range of thin-film photovoltaics. (C) 2014 Optical Society of America C1 [Pang, Y. T.; Eisaman, M. D.] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Pang, Y. T.; Eisaman, M. D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bossart, M.] Dartmouth Coll, Hanover, NH 03755 USA. RP Eisaman, MD (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. EM meisaman@bnl.gov FU U.S. Department of Energy, Sustainable Energy Technologies Department [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI) FX This work was partially supported by the U.S. Department of Energy, Sustainable Energy Technologies Department under contract DE-AC02-98CH10886. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. M.B. was partially supported by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI). The authors would like to thank N. Dissanayake for helpful discussions and A. Ashraf for spectroscopic ellipsometry measurements. NR 20 TC 2 Z9 2 U1 0 U2 4 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 13 PY 2014 VL 22 IS 1 BP A188 EP A197 DI 10.1364/OE.22.00A188 PG 10 WC Optics SC Optics GA 302CP UT WOS:000330579300010 PM 24921995 ER PT J AU Sukhanov, A Lunin, A Yakovlev, V Awida, M Champion, M Ginsburg, C Gonin, I Grimm, C Khabiboulline, T Nicol, T Orlov, Y Saini, A Sergatskov, D Solyak, N Vostrikov, A AF Sukhanov, A. Lunin, A. Yakovlev, V. Awida, M. Champion, M. Ginsburg, C. Gonin, I. Grimm, C. Khabiboulline, T. Nicol, T. Orlov, Yu. Saini, A. Sergatskov, D. Solyak, N. Vostrikov, A. TI High order modes in Project-X linac SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Superconducting proton linac; High order modes; Beans dynamics AB Project X, a multi MW proton source, is now under development at Fermilab. In this paper we present study of high order modes (HOM) excited in continues wave (CW) superconducting linac of Project X. We investigate effects of cryogenic losses caused by HOMs and influence of HOMs on beam dynamics. We find that these effects are small. We conclude that HOM couplers/dampers are not needed in the Project-X SC RF cavities. (C) 2013 Elsevier B.V. All rights reserved. C1 [Sukhanov, A.; Lunin, A.; Yakovlev, V.; Awida, M.; Champion, M.; Ginsburg, C.; Gonin, I.; Grimm, C.; Khabiboulline, T.; Nicol, T.; Orlov, Yu.; Saini, A.; Sergatskov, D.; Solyak, N.; Vostrikov, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Sukhanov, A (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM ais@fnal.gov OI Champion, Mark/0000-0002-5742-2568 FU United States Department of Energy [De-AC02-07CH11359] FX Operated by Fermi Research Alliance, LLC under contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 18 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 11 PY 2014 VL 734 BP 9 EP 22 DI 10.1016/j.nima.2013.06.113 PN A PG 14 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258XN UT WOS:000327492100003 ER PT J AU Hahn, H Jain, P Xu, WC AF Hahn, H. Jain, Puneet Xu, Wencan TI Study of split higher order mode resonances in superconducting cavities SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Higher order modes; Bead pull perturbations; Superconducting cavities AB Split resonances are a common appearance in superconducting cavities and are studied here on a specific example. A five cell superconducting cavity suitable for the envisioned electron-hadron collider eRHIC was designed and will be used in the upcoming "Coherent electron Cooling" Proof-of-Principle experiment. The superconducting cavity is intended for high-current applications, and beam stability depends on minimizing the Higher Order Modes (ROM). This was attempted in the design phase and will be done with appropriate mode dampers in operation. The design was implemented as a copper cavity and two Niobium cavities were fabricated. The availability of the copper model provided a convenient opportunity to confirm the design and to study potentially nefarious HOMs. Selected high-Q resonances were investigated via bead pull measurements. The appearance of split resonances impeded their study and suitable methods of HOM identification are presented in this report. (C) 2013 Elsevier B.V. All rights reserved. C1 [Hahn, H.; Xu, Wencan] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Jain, Puneet] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Hahn, H (reprint author), Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. EM hahnh@bnl.gov FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. DOE; [DE-SC0002496] FX The authors acknowledge the advice by Drs. I. Ben-Zvi, V. Litvinenko, S. Belomestnykh, and K. Calaga. This work was supported by the Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH10886 with the U.S. DOE and Award No. DE-SC0002496 to Stony Brook University with the US DOE. NR 15 TC 0 Z9 0 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 11 PY 2014 VL 734 BP 44 EP 50 DI 10.1016/j.nima.2013.06.056 PN A PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258XN UT WOS:000327492100007 ER PT J AU Bermel, P Byer, RL Colby, ER Cowan, BM Dawson, J England, RJ Noble, RJ Qi, MH Yoder, RB AF Bermel, Peter Byer, Robert L. Colby, Eric R. Cowan, Benjamin M. Dawson, Jay England, R. Joel Noble, Robert J. Qi, Minghao Yoder, Rodney B. TI Summary of the 2011 Dielectric Laser Accelerator Workshop SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Acceleration; Laser; Dielectric; Optical; Photonic; Crystal ID HIGH-ENERGY; PHOTONIC CRYSTAL; PEAK-POWER; AMPLIFICATION; FIBERS AB The first ICFA Mini-Workshop on dielectric laser accelerators (DLA) was held on September 15-16,2011 at SLAC National Accelerator Laboratory. We present the results of the workshop, and discuss the main conclusions of the Accelerator Applications, Photonics, and Laser Technologies working groups. Over 50 participants from four countries participated, discussing the state of the art in photonic structures, laser science, and nanofabrication as it pertains to laser-driven particle acceleration in dielectric structures. Applications of this new and promising acceleration concept to discovery science and industrial, medical, and basic energy sciences were explored. The DLA community is presently focused on making demonstrations of high gradient acceleration and a compatible atto-second injector source, two critical steps towards realizing the potential of this technology. Published by Elsevier B.V. C1 [Bermel, Peter; Qi, Minghao] Purdue Univ, W Lafayette, IN 47907 USA. [Byer, Robert L.] Stanford Univ, Stanford, CA 94305 USA. [Colby, Eric R.; England, R. Joel; Noble, Robert J.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Cowan, Benjamin M.] Tech X Corp, Boulder, CO USA. [Dawson, Jay] Lawrence Livermore Natl Lab, Livermore, CA USA. [Yoder, Rodney B.] Manhattanville Coll, Purchase, NY USA. RP England, RJ (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM england@slac.stanford.edu OI Bermel, Peter/0000-0001-7140-0667 FU Department of Energy [DE-AC03-76SF00515]; US Department of Energy FX We thank the organizers of DLA 2011 for putting together the workshop, SLAC for hosting it, and the US Department of Energy for providing funding. We acknowledge support from Department of Energy contract DE-AC03-76SF00515, Tech-X Corporation (BMC) and the Defense Threat Reduction Agency (RBY) for the preparation of this report. NR 45 TC 6 Z9 7 U1 0 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 11 PY 2014 VL 734 BP 51 EP 59 DI 10.1016/j.nima.2013.06.055 PN A PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258XN UT WOS:000327492100008 ER PT J AU Burt, G Wang, H AF Burt, G. Wang, H. TI Damping of unwanted modes in SRF deflecting/crabbing cavities SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Crab cavities; Higher order modes; Deflecting cavities AB As deflecting and crab cavities do not use the fundamental acceleration mode for their operation, the spectrum of unwanted modes is significantly different from that of accelerating cavities. The fundamental acceleration mode is now unwanted and can cause energy spread in the beam; in addition this mode frequency is often close to or lower than that of the deflecting mode, making it difficult to damp. This is made more complex in some of the compact crab cavities as there small beampipes often attenuate the fields very sharply. In addition in some crab cavities there can be an orthogonal transverse mode similar to the deflecting mode, known as the same order mode. The degeneracy of these modes most be split by polarising the cavity and if the polarisation is not large enough, dampers should be placed at either an electric or magnetic held null of the crabbing mode to effectively damp the unwanted polarisation. Various concepts for dealing with unwanted modes in various SRF deflecting cavities will be reviewed. Crown Copyright (C) 2013 Published by Elsevier B.V. All rights reserved. C1 [Burt, G.] Univ Lancaster, Dept Engn, Lancaster, England. [Wang, H.] Jefferson Lab, Newport News, VA USA. RP Burt, G (reprint author), Univ Lancaster, Dept Engn, Lancaster, England. EM graeme.burt@stfc.ac.uk OI Burt, Graeme/0000-0001-8288-1216 FU EU; STFC via the Cockcroft Institute FX The authors would like to thank Amos Dexter (Lancaster), Peter McIntosh, Philippe Goudket (STFC), Leo Bellantoni (FNAL), Bob Rimmer (JLAB), Zenghai Li, Liling Xiao (SLAC), Ali Nassiri, Geoff Waldshmitt (ANL), Derun Li (LBNL), Rama Calaga, Erk Jensen (CERN), Jean Delayen (ODU) and all the crab cavity team at KEK for many useful discussions on couplers for deflecting mode cavities and the use of their work in this paper. This work has been funded by EU FP7 as part of the EUCARD and HiLumi LHC programmes, and by STFC via the Cockcroft Institute grant. NR 22 TC 2 Z9 2 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 11 PY 2014 VL 734 BP 65 EP 71 DI 10.1016/j.nima.2012.12.068 PN A PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258XN UT WOS:000327492100010 ER PT J AU Hahn, H Calaga, R Jain, P Johnson, EC Xu, WC AF Hahn, H. Calaga, R. Jain, Puneet Johnson, Elliott C. Xu, Wencan TI HOM identification by bead pulling in the Brookhaven ERL cavity SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Energy recovery linac; Superconducting five-cell cavity; Higher order modes; Bead pulling AB Exploratory measurements of the Brookhaven Energy Recovery Linac (ERL) cavity at superconducting temperature produced a long list of high order modes (HOMs). The niobium 5-cell cavity is terminated at each end with HOM ferrite dampers that successfully reduce the Q-factors to levels required to avoid beam break up (BBU) instabilities. However, a number of un-damped resonances with Q > 10(6) were found at 4 K and their mode identification forms the focus of this paper. The approach taken here consists of bead pulling on a copper (Cu) replica of the ERL cavity with dampers involving various network analyzer measurements. Several different S-21 transmission measurements are used, including those taken from the fundamental input coupler to the pick-up probe across the cavity, others between beam-position monitor probes in the beam tubes, and also between probes placed into the cells. The bead pull technique suitable for HOM identification with a metallic needle or dielectric bead is detailed. This paper presents the results for HOMs in the first two dipole bands, the tin-clamped modes in the first quadrupole band, and the identification of several high-Q modes beyond. (C) 2012 Elsevier B.V. All rights reserved. C1 [Hahn, H.; Calaga, R.; Xu, Wencan] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Calaga, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Jain, Puneet; Johnson, Elliott C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. RP Hahn, H (reprint author), Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. EM hahnh@bnl.gov FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; US DOE [DE-SC0002496] FX The authors acknowledge the advice by Ilan Ben-Zvi and Sergey Belomestnykh, and thank Scott Seberg, Richard Anderson and Harold Dorr for multi-year technical support. This work was supported by Brookhaven Science Associates, LLC, under Contract no. DE-AC02-98CH10886 with the US DOE and award no. DE-SC0002496 to Stony Brook University with the US DOE. NR 11 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 11 PY 2014 VL 734 BP 72 EP 78 DI 10.1016/j.nima.2012.12.065 PN A PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 258XN UT WOS:000327492100011 ER PT J AU Yang, QG Williams, F Zhao, X Reece, C Krishnan, M AF Yang, Qiguang Williams, Frances Zhao, Xin Reece, Charles Krishnan, Mahadevan TI Investigating crystal microstructure of niobium materials by an x-ray diffraction reciprocal space mapping technique SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID FILMS AB An x-ray diffraction reciprocal spacing mapping (RSM) technique was applied to investigate crystal quality of Nb films and bulk materials, relevant to superconducting radio frequency applications. The RSM study used different x-ray penetration depths to study material processes after two different surface treatments: mechanical polishing or energetic condensation (a plasma process). The study revealed the material's microstructure evolution for the two different processes. The RSM plots revealed crystal quality of the materials at different thickness. The novel, differential-depth RSM technique presented in this study substantiated the following facts: (1) For a heteroepitaxial Nb film Nb(100)/MgO(100), a film thickening process, via a cathodic arc-discharge Nb ion deposition (energetic condensation), created a near-perfect single crystal Nb on the surface top layer. (2) For a fine mechanically polished single-crystal bulk Nb material, the microstructure on the top surface layer is more disordered than that at a greater depth. C1 [Yang, Qiguang; Williams, Frances] Norfolk State Univ, Ctr Mat Res, Norfolk, VA 23504 USA. [Zhao, Xin; Reece, Charles] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Krishnan, Mahadevan] Alameda Appl Sci Corp, San Leandro, CA 94577 USA. RP Yang, QG (reprint author), Norfolk State Univ, Ctr Mat Res, Norfolk, VA 23504 USA. EM xinzhao@jlab.org OI Reece, Charles/0000-0003-1939-8699 FU AASC by DOE [DE-FG02-08ER85162, DE-SC0004994]; Jefferson Science Associates, LLC, under U.S. DOE [DEAC05-06OR23177]; American Recovery and Reinvestment Act FX This research is supported at AASC by DOE via Grants No. DE-FG02-08ER85162 and No. DE-SC0004994. The JLab effort was provided by Jefferson Science Associates, LLC, under U.S. DOE Contract No. DEAC05-06OR23177, including supplemental funding provided by the American Recovery and Reinvestment Act. NR 20 TC 1 Z9 1 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD JAN 10 PY 2014 VL 17 IS 1 AR 013501 DI 10.1103/PhysRevSTAB.17.013501 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AC0GH UT WOS:000332172300001 ER PT J AU Sparks, TD Kemei, MC Barton, PT Seshadri, R Mun, ED Zapf, VS AF Sparks, Taylor D. Kemei, Moureen C. Barton, Phillip T. Seshadri, Ram Mun, Eun-Deok Zapf, Vivien S. TI Magnetocapacitance as a sensitive probe of magnetostructural changes in NiCr2O4 SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIZATION; TEMPERATURE; TRANSITION AB The spinel NiCr2O4 is characterized using dielectric and high-magnetic-field measurements. The trends in the magnetodielectric response fall into three clear temperature regimes corresponding to known magnetic and structural transitions. Above the Neel temperature, weak magnetic field dependence of the dielectric constant is observed with no hysteresis. Below the Neel temperature but above 30 K, a dependence of the dielectric constant on the magnetic field is observed and hysteresis develops, resulting in so-called butterfly loops. Below 30 K, magnetodielectric hysteresis is enhanced. Magnetodielectric hysteresis mirrors magnetic hysteresis, suggesting that spin-spin interactions are the mechanism for the magnetodielectric effect in NiCr2O4. We show that below 40 kOe, the field-dependent permittivity scales linearly with the squared magnetization as described by the Ginzburg-Landau theory. At high fields, however, the magnetization continues to increase while the dielectric constant saturates. Magnetodielectric measurements of NiCr2O4 suggest an additional, previously unobserved, transition at 20 K. Subtle changes in magnetism and structure at 20 K, suggest the completion of ferrimagnetic ordering and the spin-driven structural distortion. We demonstrate that magnetocapacitance is a sensitive probe of magnetostructural distortion and provide the first high-field measurements of NiCr2O4. C1 [Sparks, Taylor D.; Kemei, Moureen C.; Barton, Phillip T.; Seshadri, Ram] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Sparks, Taylor D.; Kemei, Moureen C.; Barton, Phillip T.; Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [Mun, Eun-Deok; Zapf, Vivien S.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. RP Sparks, TD (reprint author), Univ Utah, Dept Mat Sci & Engn, Salt Lake City, UT 84112 USA. EM sparks@eng.utah.edu; kemei@mrl.ucsb.edu; pbarton@mrl.ucsb.edu; seshadri@mrl.ucsb.edu; edmun@lanl.gov; vzapf@lanl.gov RI Seshadri, Ram/C-4205-2013; Barton, Phillip/H-3847-2011 OI Seshadri, Ram/0000-0001-5858-4027; FU NSF [DMR 1105301]; Schlumberger Foundation Faculty for the Future fellowship; National Science Foundation; NSF DMR [1121053]; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC0206CH11357]; National Science Foundation [DMR 1157490]; State of Florida; US Department of Energy FX This project was supported by the NSF through the DMR 1105301. M. C. K. was supported by a Schlumberger Foundation Faculty for the Future fellowship. P. T. B. was supported by a National Science Foundation Graduate Research fellowship. We acknowledge the use of shared experimental facilities of the Materials Research Laboratory, an NSF MRSEC, supported by NSF DMR 1121053. The 11-BM beamline at the Advanced Photon Source was supported by the DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC0206CH11357. The National High Magnetic Field Laboratory was supported by the National Science Foundation through Cooperative Grant No. DMR 1157490, the State of Florida, and the US Department of Energy. We thank B. C. Melot for helpful discussions and assistance in designing and building the magnetocapacitance measurement system. M. C. K. thanks David Poerschke for assistance with the spark plasma sintering process and Bryan A. Myers for insightful discussions. NR 21 TC 14 Z9 14 U1 3 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 10 PY 2014 VL 89 IS 2 AR 024405 DI 10.1103/PhysRevB.89.024405 PG 6 WC Physics, Condensed Matter SC Physics GA AC0TD UT WOS:000332206900002 ER PT J AU Tsetseris, L Wang, B Pantelides, ST AF Tsetseris, L. Wang, B. Pantelides, S. T. TI Substitutional doping of graphene: The role of carbon divacancies SO PHYSICAL REVIEW B LA English DT Article ID DOPED GRAPHENE; OXYGEN REDUCTION; NANOTUBES; VACANCIES; CATALYST; ENERGY AB The most common approach to dope an electronic material is to substitute a constituent atom with a suitable impurity. Here we show with first-principles calculations that this is not the best recipe for doping graphene with Al, P, Ga, or As impurities. Instead, substitution of two C atoms by one of these species is preferred (the ideal choice is phosphorus), as it shifts the Fermi level in the valence band without affecting significant changes in the electronic properties of low-energy carriers. This alternative way of doping could help optimize graphene-based devices and provide analogous doping schemes in other graphenelike materials. C1 [Tsetseris, L.] Natl Tech Univ Athens, Dept Phys, GR-15780 Athens, Greece. [Tsetseris, L.; Wang, B.; Pantelides, S. T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Pantelides, S. T.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA. [Pantelides, S. T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tsetseris, L (reprint author), Natl Tech Univ Athens, Dept Phys, GR-15780 Athens, Greece. RI Wang, Bin/E-8301-2011 OI Wang, Bin/0000-0001-8246-1422 FU McMinn Endowment at Vanderbilt University; [HDTRA 1-10-10016] FX This work was supported by the McMinn Endowment at Vanderbilt University and by Grant No. HDTRA 1-10-10016. The calculations used resources of the EGEE and HellasGrid infrastructures. NR 47 TC 16 Z9 16 U1 3 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 10 PY 2014 VL 89 IS 3 AR 035411 DI 10.1103/PhysRevB.89.035411 PG 4 WC Physics, Condensed Matter SC Physics GA AC0TH UT WOS:000332207400005 ER PT J AU Xiao, N Li, DY Cui, GF Li, N Li, Q Wu, G AF Xiao, Ning Li, Deyu Cui, Guofeng Li, Ning Li, Qing Wu, Gang TI Adsorption behavior of triblock copolymer suppressors during the copper electrodeposition SO ELECTROCHIMICA ACTA LA English DT Article DE Adsorption behavior; Triblock copolymer; Copper electroplating; Cyclic voltammetric stripping; Rotating ring-disk electrode ID CONVECTION-DEPENDENT ADSORPTION; POLYETHYLENE-GLYCOL; ADDITIVE SYSTEM; BUMP FORMATION; CU; PEG; CL; SPS; DEPOSITION; CHLORIDE AB Suppressors play a significant role in microvia filling by copper electrodeposition to achieve electrical interconnection of the adjacent layers in printed circuit boards (PCBs). In this work, in order to investigate the adsorption behaviors of one type of triblock copolymer (with a structure of polyethylene oxide - polypropylene oxide - polyethylene oxide and a molecular weight of 2900, named as EPE2900) on the cathode during the copper electroplating process, electrochemical methods such as cyclic voltammetric stripping (CVS) was employed. The integrated value of the Cu stripping peak was marked as Q, the size of which can reflect the inhibiting strength of EPE2900 on the copper deposition. Then the dependence of Q/Q(0) values on EPE2900 and Cl- concentrations was studied systematically by the CVS measurements. Here Q(0) was the integrated value of the Cu stripping peak measured in the base electrolyte. The obtained results indicated that the inhibiting strength of EPE2900 monotonously increased with its concentrations. However, the inhibiting strength of EPE2900 only increased with Cl- concentration when EPE2900 concentration was higher than 20 ppm. Importantly, the critical concentrations of Cl- and EPE2900 in the solution to form an intact barrier layer adsorbing onto the cathode surface were calculated. Based on the results of CVS measurements, a possible adsorption model of EPE2900 was proposed, which was able to reasonably elucidate the CVS measurements. In the meantime, Cu+-EPE2900-Cl- complexes were formed and very likely involved in the adsorption model, further evidenced by rotating ring-disk electrode (RRDE) techniques. (C) 2013 Published by Elsevier Ltd. C1 [Xiao, Ning; Li, Deyu; Li, Ning] Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. [Cui, Guofeng] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China. [Li, Qing; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, N (reprint author), Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. EM lininghit@263.net; wugang@lanl.gov RI Li, Qing/G-4502-2011; Wu, Gang/E-8536-2010 OI Li, Qing/0000-0003-4807-030X; Wu, Gang/0000-0003-4956-5208 FU Highnic Group (China) FX This work was financially supported by Highnic Group (China). NR 37 TC 8 Z9 8 U1 6 U2 76 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 10 PY 2014 VL 116 BP 284 EP 291 DI 10.1016/j.electacta.2013.11.056 PG 8 WC Electrochemistry SC Electrochemistry GA AB0PK UT WOS:000331494400040 ER PT J AU Mun, ED Chern, GW Pardo, V Rivadulla, F Sinclair, R Zhou, HD Zapf, VS Batista, CD AF Mun, E. D. Chern, Gia-Wei Pardo, V. Rivadulla, F. Sinclair, R. Zhou, H. D. Zapf, V. S. Batista, C. D. TI Magnetic Field Induced Transition in Vanadium Spinels SO PHYSICAL REVIEW LETTERS LA English DT Article ID ZNV2O4; CDV2O4 AB We study vanadium spinels AV(2)O(4) (A = Cd, Mg) in pulsed magnetic fields up to 65 T. A jump in magnetization at mu H-0 approximate to 40 T is observed in the single-crystal MgV2O4 , indicating a field induced quantum phase transition between two distinct magnetic orders. In the multiferroic CdV2O4, the field induced transition is accompanied by a suppression of the electric polarization. By modeling the magnetic properties in the presence of strong spin-orbit coupling characteristic of vanadium spinels, we show that both features of the field induced transition can be successfully explained by including the effects of the local trigonal crystal field. C1 [Mun, E. D.; Zapf, V. S.] Los Alamos Lab LANL, NHMFL Mat Phys & Applicat, Los Alamos, NM 87545 USA. [Mun, E. D.; Zapf, V. S.] Los Alamos Lab LANL, CNLS, Los Alamos, NM 87545 USA. [Chern, Gia-Wei; Batista, C. D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chern, Gia-Wei; Batista, C. D.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. [Pardo, V.] Univ Santiago de Compostela, Dept Fis, Santiago De Compostela 15782, Spain. [Rivadulla, F.] Univ Santiago de Compostela, CIQUS, Santiago De Compostela 15782, Spain. [Sinclair, R.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Mun, ED (reprint author), Los Alamos Lab LANL, NHMFL Mat Phys & Applicat, T-4, Los Alamos, NM 87545 USA. RI Pardo, Victor/C-2700-2009; Batista, Cristian/J-8008-2016; Zhou, Haidong/O-4373-2016; OI Pardo, Victor/0000-0002-4713-3519; Rivadulla, Francisco/0000-0003-3099-0159 FU U.S. DOE through the LDRD program [DE-AC52-06NA25396]; NSF [DMR-1157490, PHY-1066293]; DOE; State of Florida; Ramon y Cajal Program; Xunta de Galicia [2012-CP071] FX We thank N. Perkins and D. Khomskii for useful discussions and Brian Scott for single-crystal orientations. Work at the LANL was performed under the auspices of the U.S. DOE Grant No. DE-AC52-06NA25396 through the LDRD program. The NHMFL facility is funded by the NSF through cooperative Grant No. DMR-1157490, by the DOE, and by the State of Florida. This material is based upon work supported in part by the NSF under Grant No. PHY-1066293 and the hospitality of the ACP. V. P. acknowledges financial support from the Ramon y Cajal Program. F. R. acknowledges support from Xunta de Galicia 2012-CP071. NR 28 TC 9 Z9 9 U1 5 U2 68 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 10 PY 2014 VL 112 IS 1 AR 017207 DI 10.1103/PhysRevLett.112.017207 PG 5 WC Physics, Multidisciplinary SC Physics GA AB6ZR UT WOS:000331939600013 PM 24483929 ER PT J AU Fang, K Fernando, GW Balatsky, AV Kocharian, AN Palandage, K AF Fang, Kun Fernando, G. W. Balatsky, A. V. Kocharian, A. N. Palandage, K. TI Pairing modulations and phase separation instabilities in Bi2Sr2CaCu2O8+delta SO PHYSICS LETTERS A LA English DT Article DE High T-c superconductivity; Phase separation; Charge modulation; Electron pairing; Nanoscale inhomogeneities; Apical atom ID UNDERDOPED BI2212; APICAL-OXYGEN; SUPERCONDUCTIVITY; TEMPERATURE; NANOCLUSTERS; PSEUDOGAP; NEMATICITY; CRYSTAL; IMPACT; ONSET AB There is growing evidence that the unconventional spatial inhomogeneities in the doped high-T-c superconductors are accompanied by the pairing of electrons, subsequent phase transitions and condensation into coherent states. We show that such pairing states can be obtained from phase separation instabilities near level crossings. Conditions for coherent pairing instabilities are examined using exact diagonalization of Hubbard-like pyramid structures under variation of coupling and interaction strengths. We also evaluate the behavior of the energy charge gap in the vicinity of level crossings using a parametrization of coupling to the apical site to represent out-of-plane effects. These results provide a simple microscopic explanation of (correlation induced) supermodulation of the coherent pairing gap observed in scanning tunneling microscopy measurements at atomic scale in Bi2Sr2CaCu2O8+delta. Published by Elsevier B.V. C1 [Fang, Kun; Fernando, G. W.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Balatsky, A. V.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Balatsky, A. V.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Balatsky, A. V.] NORDITA, S-10691 Stockholm, Sweden. [Kocharian, A. N.] Calif State Univ Los Angeles, Dept Phys, Los Angeles, CA 90032 USA. [Palandage, K.] Trinity Coll, Dept Phys, Hartford, CT 06106 USA. RP Kocharian, AN (reprint author), Calif State Univ Los Angeles, Dept Phys, Los Angeles, CA 90032 USA. EM armen.kocharian@calstatela.edu FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000] FX We are grateful to A. Bishop, J.C. Davis, K. Fujita, H. She, I. Zeljkovic, J. Hoffman and J.X. Zhu for useful discussions. The authors acknowledge the computing facilities provided by the Center for Functional Nanomaterials, Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The work was performed also, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences, user facility at Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). NR 28 TC 0 Z9 0 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9601 EI 1873-2429 J9 PHYS LETT A JI Phys. Lett. A PD JAN 10 PY 2014 VL 378 IS 3 BP 243 EP 248 DI 10.1016/j.physleta.2013.11.006 PG 6 WC Physics, Multidisciplinary SC Physics GA 300YV UT WOS:000330500800022 ER PT J AU Aliu, E Archambault, S Aune, T Behera, B Beilicke, M Benbow, W Berger, K Bird, R Bouvier, A Buckley, JH Bugaev, V Byrum, K Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Duke, C Dumm, J Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortin, P Fortson, L Furniss, A Galante, N Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Krennrich, F Lang, MJ Madhavan, AS Maier, G Majumdar, P McCann, A Moriarty, P Mukherjee, R Nieto, D de Bhroithe, AO Ong, RA Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Rajotte, J Reyes, LC Reynolds, PT Richards, GT Roache, E Rousselle, J Sembroski, GH Sheidaei, F Skole, C Smith, AW Staszak, D Stroh, M Telezhinsky, I Theiling, M Tucci, JV Tyler, J Varlotta, A Vincent, S Wakely, SP Weinstein, A Welsing, R Williams, DA Zajczyk, A Zitzer, B Abramowski, A Aharonian, F Benkhali, FA Akhperjanian, AG Anguner, E Anton, G Balenderan, S Balzer, A Barnacka, A Becherini, Y Tjus, JB Bernlohr, K Birsin, E Bissaldi, E Biteau, J Bottcher, M Boisson, C Bolmont, J Bordas, P Brucker, J Brun, F Brun, P Bulik, T Carrigan, S Casanova, S Cerruti, M Chadwick, PM Chalme-Calvet, R Chaves, RCG Cheesebrough, A Chretien, M Colafrancesco, S Cologna, G Conrad, J Couturier, C Dalton, M Daniel, MK Davids, ID Degrange, B Deil, C deWilt, P Dickinson, HJ Djannati-Atai, A Domainko, W Drury, LO Dubus, G Dutson, K Dyks, J Dyrda, M Edwards, T Egberts, K Eger, P Espigat, P Farnier, C Fegan, S Feinstein, F Fernandes, MV Fernandez, D Fiasson, A Fontaine, G Forster, A Fussling, M Gajdus, M Gallant, YA Garrigoux, T Giavitto, G Giebels, B Glicenstein, JF Grondin, MH Grudzinska, M Haffner, S Hahn, J Harris, J Heinzelmann, G Henri, G Hermann, G Hervet, O Hillert, A Hinton, JA Hofmann, W Hofverberg, P Holler, M Horns, D Jacholkowska, A Jahn, C Jamrozy, M Janiak, M Jankowsky, F Jung, I Kastendieck, MA Katarzynski, K Katz, U Kaufmann, S Khelifi, B Kieffer, M Klepser, S Klochkov, D Kluzniak, W Kneiske, T Kolitzus, D Komin, N Kosack, K Krakau, S Krayzel, F Kruger, PP Laffon, H Lamanna, G Lefaucheur, J Lemiere, A Lemoine-Goumard, M Lenain, JP Lennarz, D Lohse, T Lopatin, A Lu, CC Marandon, V Marcowith, A Marx, R Maurin, G Maxted, N Mayer, M McComb, TJL Mehault, J Menzler, U Meyer, M Moderski, R Mohamed, M Moulin, E Murach, T Naumann, CL de Naurois, M Niemiec, J Nolan, SJ Oakes, L Ohm, S Wilhelmi, ED Opitz, B Ostrowski, M Oya, I Panter, M Parsons, RD Arribas, MP Pekeur, NW Pelletier, G Perez, J Petrucci, PO Peyaud, B Pita, S Poon, H Puhlhofer, G Punch, M Quirrenbach, A Raab, S Raue, M Reimer, A Reimer, O Renaud, M de los Reyes, R Rieger, F Rob, L Romoli, C Rosier-Lees, S Rowell, G Rudak, B Rulten, CB Sahakian, V Sanchez, DA Santangelo, A Schlickeiser, R Schussler, F Schulz, A Schwanke, U Schwarzburg, S Schwemmer, S Sol, H Spengler, G Spies, F Stawarz, L Steenkamp, R Stegmann, C Stinzing, F Stycz, K Sushch, I Szostek, A Tavernet, JP Tavernier, T Taylor, AM Terrier, R Tluczykont, M Trichard, C Valerius, K van Eldik, C Vasileiadis, G Venter, C Viana, A Vincent, P Volk, HJ Volpe, F Vorster, M Wagner, SJ Wagner, P Ward, M Weidinger, M Weitzel, Q White, R Wierzcholska, A Willmann, P Wornlein, A Wouters, D Zacharias, M Zajczyk, A Zdziarski, AA Zech, A Zechlin, HS AF Aliu, E. Archambault, S. Aune, T. Behera, B. Beilicke, M. Benbow, W. Berger, K. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Byrum, K. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Duke, C. Dumm, J. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Krennrich, F. Lang, M. J. Madhavan, A. S. Maier, G. Majumdar, P. McCann, A. Moriarty, P. Mukherjee, R. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Rajotte, J. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Rousselle, J. Sembroski, G. H. Sheidaei, F. Skole, C. Smith, A. W. Staszak, D. Stroh, M. Telezhinsky, I. Theiling, M. Tucci, J. V. Tyler, J. Varlotta, A. Vincent, S. Wakely, S. P. Weinstein, A. Welsing, R. Williams, D. A. Zajczyk, A. Zitzer, B. Abramowski, A. Aharonian, F. Benkhali, F. Ait Akhperjanian, A. G. Anguener, E. Anton, G. Balenderan, S. Balzer, A. Barnacka, A. Becherini, Y. Tjus, J. Becker Bernloehr, K. Birsin, E. Bissaldi, E. Biteau, J. Boettcher, M. Boisson, C. Bolmont, J. Bordas, P. Brucker, J. Brun, F. Brun, P. Bulik, T. Carrigan, S. Casanova, S. Cerruti, M. Chadwick, P. M. Chalme-Calvet, R. Chaves, R. C. G. Cheesebrough, A. Chretien, M. Colafrancesco, S. Cologna, G. Conrad, J. Couturier, C. Dalton, M. Daniel, M. K. Davids, I. D. Degrange, B. Deil, C. deWilt, P. Dickinson, H. J. Djannati-Atai, A. Domainko, W. Drury, L. O'C. Dubus, G. Dutson, K. Dyks, J. Dyrda, M. Edwards, T. Egberts, K. Eger, P. Espigat, P. Farnier, C. Fegan, S. Feinstein, F. Fernandes, M. V. Fernandez, D. Fiasson, A. Fontaine, G. Foerster, A. Fuessling, M. Gajdus, M. Gallant, Y. A. Garrigoux, T. Giavitto, G. Giebels, B. Glicenstein, J. F. Grondin, M. -H. Grudzinska, M. Haeffner, S. Hahn, J. Harris, J. Heinzelmann, G. Henri, G. Hermann, G. Hervet, O. Hillert, A. Hinton, J. A. Hofmann, W. Hofverberg, P. Holler, M. Horns, D. Jacholkowska, A. Jahn, C. Jamrozy, M. Janiak, M. Jankowsky, F. Jung, I. Kastendieck, M. A. Katarzynski, K. Katz, U. Kaufmann, S. Khelifi, B. Kieffer, M. Klepser, S. Klochkov, D. Kluzniak, W. Kneiske, T. Kolitzus, D. Komin, Nu. Kosack, K. Krakau, S. Krayzel, F. Krueger, P. P. Laffon, H. Lamanna, G. Lefaucheur, J. Lemiere, A. Lemoine-Goumard, M. Lenain, J. -P. Lennarz, D. Lohse, T. Lopatin, A. Lu, C. -C. Marandon, V. Marcowith, A. Marx, R. Maurin, G. Maxted, N. Mayer, M. McComb, T. J. L. Mehault, J. Menzler, U. Meyer, M. Moderski, R. Mohamed, M. Moulin, E. Murach, T. Naumann, C. L. de Naurois, M. Niemiec, J. Nolan, S. J. Oakes, L. Ohm, S. Wilhelmi, E. de Ona Opitz, B. Ostrowski, M. Oya, I. Panter, M. Parsons, R. D. Arribas, M. Paz Pekeur, N. W. Pelletier, G. Perez, J. Petrucci, P. -O. Peyaud, B. Pita, S. Poon, H. Puehlhofer, G. Punch, M. Quirrenbach, A. Raab, S. Raue, M. Reimer, A. Reimer, O. Renaud, M. de los Reyes, R. Rieger, F. Rob, L. Romoli, C. Rosier-Lees, S. Rowell, G. Rudak, B. Rulten, C. B. Sahakian, V. Sanchez, D. A. Santangelo, A. Schlickeiser, R. Schuessler, F. Schulz, A. Schwanke, U. Schwarzburg, S. Schwemmer, S. Sol, H. Spengler, G. Spies, F. Stawarz, L. Steenkamp, R. Stegmann, C. Stinzing, F. Stycz, K. Sushch, I. Szostek, A. Tavernet, J. -P. Tavernier, T. Taylor, A. M. Terrier, R. Tluczykont, M. Trichard, C. Valerius, K. van Eldik, C. Vasileiadis, G. Venter, C. Viana, A. Vincent, P. Voelk, H. J. Volpe, F. Vorster, M. Wagner, S. J. Wagner, P. Ward, M. Weidinger, M. Weitzel, Q. White, R. Wierzcholska, A. Willmann, P. Woernlein, A. Wouters, D. Zacharias, M. Zajczyk, A. Zdziarski, A. A. Zech, A. Zechlin, H. -S. CA VERITAS Collaboration HESS Collaboration TI LONG-TERM TeV AND X-RAY OBSERVATIONS OF THE GAMMA- RAY BINARY HESS J0632+057 SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; binaries: general; gamma rays: general(HESS J0632+057, VER J0633+057) ID LS-I +61-DEGREES-303; VERITAS OBSERVATIONS; I+61 303; EMISSION; I+61-DEGREES-303; VARIABILITY; DISCOVERY; WINDS; TELESCOPE; CATALOG AB HESS J0632+057 is the only gamma-ray binary known so far whose position in the sky allows observations with ground-based observatories in both the northern and southern hemispheres. Here we report on long-term observations of HESS J0632+057 conducted with the Very Energetic Radiation Imaging Telescope Array System and High Energy Stereoscopic System Cherenkov telescopes and the X-ray satellite Swift, spanning a time range from 2004 to 2012 and covering most of the system's orbit. The very-high-energy (VHE) emission is found to be variable and is correlated with that at X-ray energies. An orbital period of 315(-4)(+6) days is derived from the X-ray data set, which is compatible with previous results, P = (321 +/- 5) days. The VHE light curve shows a distinct maximum at orbital phases close to 0.3, or about 100 days after periastron passage, which coincides with the periodic enhancement of the X-ray emission. Furthermore, the analysis of the TeV data shows for the first time a statistically significant (> 6.5 sigma) detection at orbital phases 0.6-0.9. The obtained gamma-ray and X-ray light curves and the correlation of the source emission at these two energy bands are discussed in the context of the recent ephemeris obtained for the system. Our results are compared to those reported for other gamma-ray binaries. C1 [Aliu, E.; Errando, M.; Mukherjee, R.] Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. 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[deWilt, P.; Maxted, N.; Rowell, G.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Djannati-Atai, A.; Espigat, P.; Lefaucheur, J.; Lemiere, A.; Pita, S.; Punch, M.; Tavernier, T.] Univ Paris Diderot, Sorbonne Paris Cite, Observ Paris, APC,CNRS,IN2P3,CEA Irfu, F-75205 Paris 13, France. [Dubus, G.; Henri, G.; Pelletier, G.; Petrucci, P. -O.] UJF Grenoble 1 CNRS INSU, Inst Planetol & Astrophys Grenoble IPAG UMR 5274, F-38041 Grenoble, France. [Dutson, K.; Hinton, J. A.; Ohm, S.; White, R.] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Dyrda, M.] Inst Fizyki Jadrowej PAN, PL-31342 Krakow, Poland. [Zajczyk, A.; Feinstein, F.; Fernandez, D.; Niemiec, J.; Poon, H.; Renaud, M.; Vasileiadis, G.] Univ Montpellier 2, Lab Univers & Particules Montpellier, CNRS, IN2P3, F-34095 Montpellier 5, France. [Fiasson, A.; Komin, Nu.; Krayzel, F.; Lamanna, G.; Maurin, G.; Trichard, C.] Univ Savoie, CNRS, IN2P3, Lab Annecy le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. [Jamrozy, M.; Stawarz, L.; Szostek, A.; Wierzcholska, A.] Uniwersytet Jagiellonian, Obserwatorium Astron, PL-30244 Krakow, Poland. [Katarzynski, K.] Nicholas Copernicus Univ, Torun Ctr Astron, PL-87100 Torun, Poland. [Ohm, S.; Ostrowski, M.] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [Rob, L.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, CR-18000 Prague 8, Czech Republic. RP Aliu, E (reprint author), Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. EM afalcone@astro.psu.edu; gernot.maier@desy.de; pol.bordas@uni-tuebingen.de RI Nieto, Daniel/J-7250-2015; Meyer, Manuel/E-2697-2016; Bissaldi, Elisabetta/K-7911-2016; Drury, Luke/B-1916-2017; Moulin, Emmanuel/B-5959-2017; Daniel, Michael/A-2903-2010; Khassen, Yerbol/I-3806-2015; Tjus, Julia/G-8145-2012; Fontaine, Gerard/D-6420-2014; van Eldik, Christopher/C-3901-2013; Venter, Christo/E-6884-2011; Reimer, Olaf/A-3117-2013; Schussler, Fabian/G-5313-2013; Katarzynski, Krzysztof/G-4528-2014; Jamrozy, Marek/F-4507-2015; Katz, Uli/E-1925-2013; Casanova, Sabrina/J-8935-2013; Anton, Gisela/C-4840-2013; Komin, Nukri/J-6781-2015; OI Nieto, Daniel/0000-0003-3343-0755; Meyer, Manuel/0000-0002-0738-7581; Bissaldi, Elisabetta/0000-0001-9935-8106; Drury, Luke/0000-0002-9257-2270; Moulin, Emmanuel/0000-0003-4007-0145; Chadwick, Paula/0000-0002-1468-2685; Kneiske, Tanja M./0000-0002-3210-6200; mohamed, mahmoud/0000-0002-4625-6242; Cui, Wei/0000-0002-6324-5772; Daniel, Michael/0000-0002-8053-7910; Khassen, Yerbol/0000-0002-7296-3100; van Eldik, Christopher/0000-0001-9669-645X; Venter, Christo/0000-0002-2666-4812; Reimer, Olaf/0000-0001-6953-1385; Schussler, Fabian/0000-0003-1500-6571; Katz, Uli/0000-0002-7063-4418; Casanova, Sabrina/0000-0002-6144-9122; Anton, Gisela/0000-0003-2039-4724; de Ona Wilhelmi, Emma/0000-0002-5401-0744; Rowell, Gavin/0000-0002-9516-1581; Lenain, Jean-Philippe/0000-0001-7284-9220; de los Reyes Lopez, Raquel/0000-0003-0485-9552; Kruger, Paulus/0000-0003-0664-8521; Komin, Nukri/0000-0003-3280-0582; Errando, Manel/0000-0002-1853-863X; Maxted, Nigel/0000-0003-2762-8378; Punch, Michael/0000-0002-4710-2165; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563; Sushch, Iurii/0000-0002-2814-1257; Bordas, Pol/0000-0002-0266-8536; Oya, Igor/0000-0002-3881-9324 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K; Helmholtz Association; European Community [ERC-StG-259391]; German Ministry for Education and Research (BMBF); Max Planck Society; French Ministry for Research; CNRS-IN2P3; Astroparticle Interdisciplinary Programme of the CNRS; U.K. Particle Physics and Astronomy Research Council (PPARC); IPNP of the Charles University; South African Department of Science and Technology and National Research Foundation; University of Namibia FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. G.M. acknowledges support through the Young Investigators Program of the Helmholtz Association. M.D. is funded by contract ERC-StG-259391 from the European Community.; The support of the Namibian authorities and of the University of Namibia in facilitating the construction and operation of H.E.S.S. is gratefully acknowledged, as is the support by the German Ministry for Education and Research (BMBF), the Max Planck Society, the French Ministry for Research, the CNRS-IN2P3 and the Astroparticle Interdisciplinary Programme of the CNRS, the U.K. Particle Physics and Astronomy Research Council (PPARC), the IPNP of the Charles University, the South African Department of Science and Technology and National Research Foundation, and by the University of Namibia. We appreciate the excellent work of the technical support staff in Berlin, Durham, Hamburg, Heidelberg, Palaiseau, Paris, Saclay, and in Namibia in the construction and operation of the H.E.S.S. equipment. NR 82 TC 11 Z9 11 U1 3 U2 23 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 10 PY 2014 VL 780 IS 2 AR 168 DI 10.1088/0004-637X/780/2/168 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 281JL UT WOS:000329097100055 ER PT J AU de Putter, R Dore, O Das, S AF de Putter, Roland Dore, Olivier Das, Sudeep TI USING CROSS CORRELATIONS TO CALIBRATE LENSING SOURCE REDSHIFT DISTRIBUTIONS: IMPROVING COSMOLOGICAL CONSTRAINTS FROM UPCOMING WEAK LENSING SURVEYS SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmological parameters; cosmology: observations; dark energy; galaxies: photometry; gravitational lensing: weak; large-scale structure of universe ID PHOTOMETRIC REDSHIFT; COSMIC SHEAR; TOMOGRAPHY; ERRORS; REQUIREMENTS; GALAXIES; IMPACT AB Cross correlations between the galaxy number density in a lensing source sample and that in an overlapping spectroscopic sample can in principle be used to calibrate the lensing source redshift distribution. In this paper, we study in detail to what extent this cross-correlation method can mitigate the loss of cosmological information in upcoming weak lensing surveys (combined with a cosmic microwave background prior) due to lack of knowledge of the source distribution. We consider a scenario where photometric redshifts are available and find that, unless the photometric redshift distribution p(z(ph)vertical bar z) is calibrated very accurately a priori (bias and scatter known to similar to 0.002 for, e.g., EUCLID), the additional constraint on p(z(ph)vertical bar z) from the cross-correlation technique to a large extent restores the cosmological information originally lost due to the uncertainty in dn/dz(z). Considering only the gain in photo-z accuracy and not the additional cosmological information, enhancements of the dark energy figure of merit of up to a factor of four (40) can be achieved for a SuMIRe-like (EUCLID-like) combination of lensing and redshift surveys, where SuMIRe stands for Subaru Measurement of Images and Redshifts). However, the success of the method is strongly sensitive to our knowledge of the galaxy bias evolution in the source sample and we find that a percent level bias prior is needed to optimize the gains from the cross-correlation method (i.e., to approach the cosmology constraints attainable if the bias was known exactly). C1 [de Putter, Roland; Dore, Olivier] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [de Putter, Roland; Dore, Olivier] CALTECH, Pasadena, CA 91125 USA. [Das, Sudeep] Argonne Natl Lab, Div High Energy Phys, Lemont, IL 60439 USA. RP de Putter, R (reprint author), CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. FU NASA ATP grant [11-ATP-090] FX The authors thank Carlos Cunha, Patrick MacDonald, Jeffrey Newman, David Schlegel, David Spergel, and Masahiro Takada for useful discussions. Part of the research described in this paper was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. This work is supported by NASA ATP grant 11-ATP-090. NR 49 TC 10 Z9 10 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 10 PY 2014 VL 780 IS 2 AR 185 DI 10.1088/0004-637X/780/2/185 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 281JL UT WOS:000329097100072 ER PT J AU Furst, F Pottschmidt, K Wilms, J Tomsick, JA Bachetti, M Boggs, SE Christensen, FE Craig, WW Grefenstette, BW Hailey, CJ Harrison, F Madsen, KK Miller, JM Stern, D Walton, DJ Zhang, W AF Fuerst, Felix Pottschmidt, Katja Wilms, Joern Tomsick, John A. Bachetti, Matteo Boggs, Steven E. Christensen, Finn E. Craig, William W. Grefenstette, Brian W. Hailey, Charles J. Harrison, Fiona Madsen, Kristin K. Miller, Jon M. Stern, Daniel Walton, Dominic J. Zhang, William TI NuSTAR DISCOVERY OF A LUMINOSITY DEPENDENT CYCLOTRON LINE ENERGY IN VELA X-1 SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; radiation: dynamics; stars: neutron; X-rays: binaries; X-rays: individual (Vela X-1) ID X-RAY BINARIES; SPECTROSCOPIC-TELESCOPE-ARRAY; HOT-STAR WINDS; MAGNETIC-FIELDS; NEUTRON-STAR; RESOLVED SPECTROSCOPY; 2004-2005 OUTBURST; ACCRETING PULSARS; TIMING-EXPLORER; STELLAR WINDS AB We present NuSTAR observations of Vela X-1, a persistent, yet highly variable, neutron star high-mass X-ray binary (HMXB). Two observations were taken at similar orbital phases but separated by nearly a year. They show very different 3-79 keV flux levels as well as strong variability during each observation, covering almost one order of magnitude in flux. These observations allow, for the first time ever, investigations on kilo-second time-scales of how the centroid energies of cyclotron resonant scattering features (CRSFs) depend on flux for a persistent HMXB. We find that the line energy of the harmonic CRSF is correlated with flux, as expected in the sub-critical accretion regime. We argue that Vela X-1 has a very narrow accretion column with a radius of around 0.4 km that sustains a Coulomb interaction dominated shock at the observed luminosities of L-x similar to 3 x 10(36) erg s(-1). Besides the prominent harmonic line at 55 keV the fundamental line around 25 keV is clearly detected. We find that the strengths of the two CRSFs are anti-correlated, which we explain by photon spawning. This anti-correlation is a possible explanation for the debate about the existence of the fundamental line. The ratio of the line energies is variable with time and deviates significantly from 2.0, also a possible consequence of photon spawning, which changes the shape of the line. During the second observation, Vela X-1 showed a short off-state in which the power-law softened and a cut-off was no longer measurable. It is likely that the source switched to a different accretion regime at these low mass accretion rates, explaining the drastic change in spectral shape. C1 [Fuerst, Felix; Grefenstette, Brian W.; Harrison, Fiona; Madsen, Kristin K.; Walton, Dominic J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Pottschmidt, Katja] Univ Maryland Baltimore Cty, Ctr Space Sci & Technol, Baltimore, MD 21250 USA. [Pottschmidt, Katja] CRESST, Greenbelt, MD 20771 USA. [Pottschmidt, Katja; Zhang, William] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Wilms, Joern] Dr Karl Remeis Sternwarte, D-96049 Bamberg, Germany. [Wilms, Joern] ECAP, D-96049 Bamberg, Germany. [Tomsick, John A.; Boggs, Steven E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Bachetti, Matteo] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Bachetti, Matteo] CNRS, Inst Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Furst, F (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. RI Wilms, Joern/C-8116-2013; Boggs, Steven/E-4170-2015; OI Wilms, Joern/0000-0003-2065-5410; Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C]; National Aeronautics and Space Administration; NASA Astrophysics Data Analysis Program [NNX13AE98G]; Centre National d'Etudes Spatiales (CNES) FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). We would like to thank John E. Davis for the slxfig module, which was used to produce all figures in this work. We would like to thank Fritz Schwarm for the helpful discussions about cyclotron line shapes. J.A.T. acknowledges partial support from NASA Astrophysics Data Analysis Program grant NNX13AE98G. M. B. was supported by the Centre National d'Etudes Spatiales (CNES). We would like to thank the anonymous referee for the useful comments. NR 67 TC 24 Z9 24 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 10 PY 2014 VL 780 IS 2 AR 133 DI 10.1088/0004-637X/780/2/133 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 281JL UT WOS:000329097100020 ER PT J AU Yamaguchi, H Eriksen, KA Badenes, C Hughes, JP Brickhouse, NS Foster, AR Patnaude, DJ Petre, R Slane, PO Smith, RK AF Yamaguchi, Hiroya Eriksen, Kristoffer A. Badenes, Carles Hughes, John P. Brickhouse, Nancy S. Foster, Adam R. Patnaude, Daniel J. Petre, Robert Slane, Patrick O. Smith, Randall K. TI NEW EVIDENCE FOR EFFICIENT COLLISIONLESS HEATING OF ELECTRONS AT THE REVERSE SHOCK OF A YOUNG SUPERNOVA REMNANT SO ASTROPHYSICAL JOURNAL LA English DT Article DE atomic data; hydrodynamics; ISM: individual objects (SN 1572, Tycho's SNR); ISM: supernova remnants; shock waves; X-rays: ISM ID X-RAY-EMISSION; TEMPERATURE EQUILIBRATION; PARTICLE-ACCELERATION; NONRADIATIVE SHOCKS; ION EQUILIBRATION; IA SUPERNOVAE; CYGNUS LOOP; SN 1006; SPECTRUM; LIGHT AB Although collisionless shocks are ubiquitous in astrophysics, certain key aspects of them are not well understood. In particular, the process known as collisionless electron heating, whereby electrons are rapidly energized at the shock front, is one of the main open issues in shock physics. Here, we present the first clear evidence for efficient collisionless electron heating at the reverse shock of Tycho's supernova remnant (SNR), revealed by FeK diagnostics using high-quality X-ray data obtained by the Suzaku satellite. We detect K beta (3p -> 1s) fluorescence emission from low-ionization Fe ejecta excited by energetic thermal electrons at the reverse shock front, which peaks at a smaller radius than Fe K alpha (2p -> 1s) emission dominated by a relatively highly ionized component. Comparisons with our hydrodynamical simulations imply instantaneous electron heating to a temperature 1000 times higher than expected from Coulomb collisions alone. The unique environment of the reverse shock, which is propagating with a high Mach number into rarefied ejecta with a low magnetic field strength, puts strong constraints on the physical mechanism responsible for this heating and favors a cross-shock potential created by charge deflection at the shock front. Our sensitive observation also reveals that the reverse shock radius of this SNR is about 10% smaller than the previous measurement using the Fe K alpha morphology from the Chandra observations. Since strong Fe K beta fluorescence is expected only from low-ionization plasma where Fe ions still have many 3p electrons, this feature is key to diagnosing the plasma state and distribution of the immediate postshock ejecta in a young SNR. C1 [Yamaguchi, Hiroya; Petre, Robert] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Yamaguchi, Hiroya] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Yamaguchi, Hiroya; Brickhouse, Nancy S.; Foster, Adam R.; Patnaude, Daniel J.; Slane, Patrick O.; Smith, Randall K.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Eriksen, Kristoffer A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Badenes, Carles] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Badenes, Carles] Univ Pittsburgh, Pittsburgh Particle Phys Astrophys & Cosmol Ctr P, Pittsburgh, PA 15260 USA. [Hughes, John P.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. RP Yamaguchi, H (reprint author), NASA, Goddard Space Flight Ctr, Code 662, Greenbelt, MD 20771 USA. EM hiroya.yamaguchi@nasa.gov RI XRAY, SUZAKU/A-1808-2009; OI Brickhouse, Nancy/0000-0002-8704-4473 FU NASA Suzaku GO grant [NNX08AZ86G]; NASA ADP grant [NNX12AF44G] FX We are thankful to Drs. John D. Raymond and Timothy R. Kallman for useful information and discussion. This work is supported by funding from NASA Suzaku GO grant NNX08AZ86G (J.P.H.) and NASA ADP grant NNX12AF44G (R.K.S.). NR 46 TC 13 Z9 13 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 10 PY 2014 VL 780 IS 2 AR 136 DI 10.1088/0004-637X/780/2/136 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 281JL UT WOS:000329097100023 ER PT J AU McWilliams, B Yu, J Klier, E Yen, CF AF McWilliams, B. Yu, J. Klier, E. Yen, C. -F. TI Mechanical response of discontinuous ceramic fiber reinforced metal matrix composites under quasi-static and dynamic loadings SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Metal matrix composites; Ballistic performance; Mechanical characterization; Failure mechanisms; Digital image correlation ID VISCOPLASTIC DAMAGE MODEL; PARTICLE DISTRIBUTION; BEHAVIOR; COMPRESSION; PENETRATION; PERFORATION; STRENGTH; SAFFIL; IMPACT AB The quasi-static mechanical properties and ballistic impact performance of several discontinuous ceramic fiber (Saffil) reinforced Al-2% Cu metal matrix composites (MMC) are characterized. The ballistic penetration resistance of the materials are determined against a fragment simulating projectile and compared to the performance of the baseline matrix alloy. Digital image correlation with high speed photography is used to measure the full field deflection of the materials during impact. Mechanical behavior and post-mortem fracture analysis are used to relate material properties to performance in penetrating and non-penetrating impact events. It is demonstrated that the MMC materials exhibit a strong asymmetry in their tensile and compressive responses. The MMC materials are stronger in compression and the asymmetry in response increases with increasing volume fraction of fiber. It was found that the ballistic performance (V-50(BL)) decreases when the volume fraction of fiber is greater than 3% due to the decrease in tensile strain to failure at higher volume fractions. In non-penetrating impacts the increased stiffness and strength with higher volume fractions greatly reduces the magnitude and distribution of plate deflection. (C) 2013 Elsevier B.V. All rights reserved. C1 [McWilliams, B.] Oak Ridge Inst Sci & Educ, Aberdeen Proving Ground, MD 21005 USA. [Yu, J.; Klier, E.; Yen, C. -F.] US Army Res Lab, Weap & Mat Res Directorate, Aberdeen Proving Ground, MD USA. RP McWilliams, B (reprint author), Oak Ridge Inst Sci & Educ, ATTN WMM B, Bldg 4600, Aberdeen Proving Ground, MD 21005 USA. EM brandon.a.mcwilliams.ctr@mail.mil NR 26 TC 9 Z9 10 U1 3 U2 18 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JAN 10 PY 2014 VL 590 BP 21 EP 29 DI 10.1016/j.msea.2013.09.068 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 292FV UT WOS:000329888500004 ER PT J AU Brady, MP Magee, J Yamamoto, Y Helmick, D Wang, L AF Brady, M. P. Magee, J. Yamamoto, Y. Helmick, D. Wang, L. TI Co-optimization of wrought alumina-forming austenitic stainless steel composition ranges for high-temperature creep and oxidation/corrosion resistance SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Mechanical characterization; Oxidation; Austenite; Intermetallic; Precipitation ID OXIDATION RESISTANCE; WATER-VAPOR; ALLOYS; BEHAVIOR; ADDITIONS; SCALES AB A series of candidate alumina-forming austenitic (AFA) stainless steels designed to evaluate the effects of variation in Al, C, Cr, Mn, Nb, and Ni content on high-temperature tensile properties, creep, and oxidation/corrosion resistance were studied. The compositions assessed were based on medium Ni (20-25 wt%) and low Ni (12 wt%) AFA variations strengthened primarily by MC and/or M23C6 carbide precipitates, and a high Ni (32 wt%) AFA superalloy variation strengthened primarily by gamma '-Ni3Al intermetallic precipitates. Tensile and creep properties were measured at 650 and 750/760 degrees C, oxidation resistance from 650 to 900 C in air with water vapor and steam environments, and sulfidation-oxidation resistance in Ar-20%H-2-20%H-2(O)-5% H2S at 550 and 650 degrees C. Optimized composition ranges for different use temperatures ranges based on these evaluations are presented. (C) 2013 Elsevier B.V. All rights reserved. C1 [Brady, M. P.; Yamamoto, Y.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Magee, J.; Helmick, D.] Carpenter Technol Corp, Reading, PA 19612 USA. [Wang, L.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Brady, MP (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM bradymp@ornl.gov RI Brady, Michael/A-8122-2008 OI Brady, Michael/0000-0003-1338-4747 FU United States Department of Energy; Energy Efficiency and Renewable Energy Advanced Manufacturing Office FX The authors thank Sebastien Dryepondt, Govindarajan Muralidharan, and Bruce Pint for helpful comments on this manuscript. This work was funded by the United States Department of Energy, Energy Efficiency and Renewable Energy Advanced Manufacturing Office. NR 33 TC 25 Z9 25 U1 3 U2 33 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JAN 10 PY 2014 VL 590 BP 101 EP 115 DI 10.1016/j.msea.2013.10.014 PG 15 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 292FV UT WOS:000329888500015 ER PT J AU Cooper, KK Mandrell, RE Louie, JW Korlach, J Clark, TA Parker, CT Huynh, S Chain, PS Ahmed, S Carter, MQ AF Cooper, Kerry K. Mandrell, Robert E. Louie, Jacqueline W. Korlach, Jonas Clark, Tyson A. Parker, Craig T. Huynh, Steven Chain, Patrick S. Ahmed, Sanaa Carter, Michelle Qiu TI Comparative genomics of enterohemorrhagic Escherichia coli O145:H28 demonstrates a common evolutionary lineage with Escherichia coli O157:H7 SO BMC GENOMICS LA English DT Article DE Comparative genomics; Enterohemorrhagic Escherichia coli; Shiga toxin-producing Escherichia coli; DNA methylation; O145 ID NON-O157 SHIGA TOXIN; HEMOLYTIC-UREMIC SYNDROME; UNITED-STATES; SINGLE-MOLECULE; PARALLEL EVOLUTION; MAXIMUM-LIKELIHOOD; STEPWISE EMERGENCE; DNA METHYLATION; PHASE VARIATION; DIVERSITY AB Background: Although serotype O157:H7 is the predominant enterohemorrhagic Escherichia coli (EHEC), outbreaks of non-O157 EHEC that cause severe foodborne illness, including hemolytic uremic syndrome have increased worldwide. In fact, non-O157 serotypes are now estimated to cause over half of all the Shiga toxin-producing Escherichia coli (STEC) cases, and outbreaks of non-O157 EHEC infections are frequently associated with serotypes O26, O45, O103, O111, O121, and O145. Currently, there are no complete genomes for O145 in public databases. Results: We determined the complete genome sequences of two O145 strains (EcO145), one linked to a US lettuce-associated outbreak (RM13514) and one to a Belgium ice-cream-associated outbreak (RM13516). Both strains contain one chromosome and two large plasmids, with genome sizes of 5,737,294 bp for RM13514 and 5,559,008 bp for RM13516. Comparative analysis of the two EcO145 genomes revealed a large core (5,173 genes) and a considerable amount of strain-specific genes. Additionally, the two EcO145 genomes display distinct chromosomal architecture, virulence gene profile, phylogenetic origin of Stx2a prophage, and methylation profile (methylome). Comparative analysis of EcO145 genomes to other completely sequenced STEC and other E. coli and Shigella genomes revealed that, unlike any other known non-O157 EHEC strain, EcO145 ascended from a common lineage with EcO157/EcO55. This evolutionary relationship was further supported by the pangenome analysis of the 10 EHEC strains. Of the 4,192 EHEC core genes, EcO145 shares more genes with EcO157 than with the any other non-O157 EHEC strains. Conclusions: Our data provide evidence that EcO145 and EcO157 evolved from a common lineage, but ultimately each serotype evolves via a lineage-independent nature to EHEC by acquisition of the core set of EHEC virulence factors, including the genes encoding Shiga toxin and the large virulence plasmid. The large variation between the two EcO145 genomes suggests a distinctive evolutionary path between the two outbreak strains. The distinct methylome between the two EcO145 strains is likely due to the presence of a BsuBI/PstI methyltransferase gene cassette in the Stx2a prophage of the strain RM13514, suggesting a role of horizontal gene transfer-mediated epigenetic alteration in the evolution of individual EHEC strains. C1 [Cooper, Kerry K.; Mandrell, Robert E.; Louie, Jacqueline W.; Parker, Craig T.; Huynh, Steven; Carter, Michelle Qiu] ARS, Produce Safety & Microbiol Res Unit, Western Reg Res Ctr, USDA, Albany, CA 94710 USA. [Korlach, Jonas; Clark, Tyson A.] Pacific Biosci, Menlo Pk, CA USA. [Chain, Patrick S.; Ahmed, Sanaa] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Carter, MQ (reprint author), ARS, Produce Safety & Microbiol Res Unit, Western Reg Res Ctr, USDA, Albany, CA 94710 USA. EM michelle.carter@ars.usda.gov OI Chain, Patrick/0000-0003-3949-3634 FU USDA-ARS CRIS [5325-046, 5325-047]; USDA Research Associate Program funds FX The authors thank Anna Bates and Jaszemyn Yambao for their assistance with bacterial cultures; Gerard Lazo and Yong Gu for their assistance with whole-genome based phylogenetic analysis; Matthew Boitano for assistance with PacBio sample preparation; Khai Luong for assistance with data analysis; Denis Pierard (Brussels, Belgium) for providing the Belgian outbreak strain; and James Rudrik (Lansing, MI) for providing the US outbreak strain. We thank Richard Roberts (New England Biolabs) for bioinformatic analysis of the methyltransferase gene assignments and comparison. This research work is supported by USDA-ARS CRIS 5325-046 and -047. KK Cooper was supported by USDA Research Associate Program funds awarded to M. Q. Carter. NR 75 TC 19 Z9 20 U1 1 U2 28 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD JAN 10 PY 2014 VL 15 AR 17 DI 10.1186/1471-2164-15-17 PG 17 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 288MI UT WOS:000329615700001 PM 24410921 ER PT J AU Ehlen, MA Sun, AC Pepple, MA Eidson, ED Jones, BS AF Ehlen, Mark A. Sun, Amy C. Pepple, Mark A. Eidson, Eric D. Jones, Brian S. TI Chemical supply chain modeling for analysis of homeland security events SO COMPUTERS & CHEMICAL ENGINEERING LA English DT Article DE Agent-based modeling; Supply chains; Linear programming; Economic markets; Transportation networks; Supply chain resilience ID DEMAND UNCERTAINTY; MANAGEMENT; INDUSTRY; OPTIMIZATION; SIMULATION; NETWORKS; SUPPORT; SYSTEM; HEAPS AB The potential impacts of man-made and natural disasters on chemical plants, complexes, and supply chains are of great importance to homeland security. To be able to estimate these impacts, we developed an agent-based chemical supply chain model that includes: chemical plants with enterprise operations such as purchasing, production scheduling, and inventories; merchant chemical markets, and multi-modal chemical shipments. Large-scale simulations of chemical-plant activities and supply chain interactions, running on desktop computers, are used to estimate the scope and duration of disruptive-event impacts, and overall system resilience, based on the extent to which individual chemical plants can adjust their internal operations (e.g., production mixes and levels) versus their external interactions (market sales and purchases, and transportation routes and modes). To illustrate how the model estimates the impacts of a hurricane disruption, a simple example model centered on 1,4-butanediol is presented. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Ehlen, Mark A.; Sun, Amy C.; Pepple, Mark A.; Eidson, Eric D.; Jones, Brian S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Ehlen, MA (reprint author), Sandia Natl Labs, 1515 Eubank St, Albuquerque, NM 87123 USA. EM maehlen@sandia.gov RI Tong, Xun/A-9304-2015 FU U.S. Department of Homeland Security Science & Technology Directorate FX The authors would like to acknowledge financial support from the U.S. Department of Homeland Security Science & Technology Directorate. The authors would also like to thank Margaret Welk and Sue Downes for chemical data model contributions, Greg Mackey for transportation modeling, and Kevin Stamber for discussions on agent-based modeling. NR 52 TC 3 Z9 3 U1 4 U2 25 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0098-1354 EI 1873-4375 J9 COMPUT CHEM ENG JI Comput. Chem. Eng. PD JAN 10 PY 2014 VL 60 BP 102 EP 111 DI 10.1016/j.compchemeng.2013.07.014 PG 10 WC Computer Science, Interdisciplinary Applications; Engineering, Chemical SC Computer Science; Engineering GA 264NO UT WOS:000327885100008 ER PT J AU Liu, L Park, J Siegel, DA McCarty, KF Clark, KW Deng, W Basile, L Idrobo, JC Li, AP Gu, G AF Liu, Lei Park, Jewook Siegel, David A. McCarty, Kevin F. Clark, Kendal W. Deng, Wan Basile, Leonardo Idrobo, Juan Carlos Li, An-Ping Gu, Gong TI Heteroepitaxial Growth of Two-Dimensional Hexagonal Boron Nitride Templated by Graphene Edges SO SCIENCE LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; MOLYBDENUM-DISULFIDE; GRAIN-BOUNDARIES; MONOLAYER; HETEROSTRUCTURES; HYDROGEN; CU; SURFACES; FILMS; FOILS AB By adapting the concept of epitaxy to two-dimensional space, we show the growth of a single-atomic-layer, in-plane heterostructure of a prototypical material system-graphene and hexagonal boron nitride (h-BN). Monolayer crystalline h-BN grew from fresh edges of monolayer graphene with atomic lattice coherence, forming an abrupt one-dimensional interface, or boundary. More important, the h-BN lattice orientation is solely determined by the graphene, forgoing configurations favored by the supporting copper substrate. C1 [Liu, Lei; Deng, Wan; Gu, Gong] Univ Tennessee, Knoxville, TN 37996 USA. [Park, Jewook; Clark, Kendal W.; Basile, Leonardo; Idrobo, Juan Carlos; Li, An-Ping] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Siegel, David A.; McCarty, Kevin F.] Sandia Natl Labs, Livermore, CA 94550 USA. [Basile, Leonardo] Escuela Politec Nacl, Dept Fis, Quito, Ecuador. RP Li, AP (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM apli@ornl.gov; ggu1@utk.edu RI Li, An-Ping/B-3191-2012; Liu, Lei/E-6267-2014; Idrobo, Juan/H-4896-2015; Gu, Gong/L-5919-2015; Park, Jewook/N-2856-2015 OI Li, An-Ping/0000-0003-4400-7493; Idrobo, Juan/0000-0001-7483-9034; Gu, Gong/0000-0002-3888-1427; FU NSF [ECCS-1231808]; Defense Advanced Research Projects Agency; National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy [DE-AC04-94AL85000] FX This work was partially supported by NSF (ECCS-1231808), the Defense Advanced Research Projects Agency (approved for public release; distribution is unlimited), and the National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT). A portion of this research was conducted at the Center for Nanophase Materials Sciences (CNMS), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Work at Sandia was supported by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy, under contract DE-AC04-94AL85000. We thank R. M. Feenstra for discussions on LEEM. Authors declare no conflicts of interest. NR 24 TC 138 Z9 138 U1 44 U2 440 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 10 PY 2014 VL 343 IS 6167 BP 163 EP 167 DI 10.1126/science.1246137 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 286BZ UT WOS:000329440800037 PM 24408431 ER PT J AU Lin, J Sinitsyn, NA AF Lin, J. Sinitsyn, N. A. TI Exact transition probabilities in the three-state Landau-Zener-Coulomb model SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE nonadiabatic transitions; Landau-Zener; exactly solvable model; nonstationary quantum mechanics ID BOW-TIE MODEL; SURVIVAL PROBABILITY; POTENTIAL CURVES; CROSSINGS; DYNAMICS; ATOMS; BANDS; FE-8 AB We obtain the exact expression for the matrix of nonadiabatic transition probabilities in the model of three interacting states with a time-dependent Hamiltonian. Unlike other known solvable Landau-Zener-like problems, our solution is generally expressed in terms of hypergeometric functions that have relatively complex behavior, e.g. the obtained transition probabilitiesmay show multiple oscillations as functions of parameters of the model Hamiltonian. C1 [Lin, J.] Princeton Univ, Dept Math, Princeton, NJ 08544 USA. [Lin, J.; Sinitsyn, N. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, J (reprint author), Princeton Univ, Dept Math, Princeton, NJ 08544 USA. EM jeffminl@princeton.edu; nsinitsyn@lanl.gov FU US DOE [DE-AC52-06NA25396] FX This work was funded by the US DOE under contract no. DE-AC52-06NA25396. NR 56 TC 2 Z9 2 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD JAN 10 PY 2014 VL 47 IS 1 AR 015301 DI 10.1088/1751-8113/47/1/015301 PG 10 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA 274RU UT WOS:000328624700010 ER PT J AU Hurst, AM Firestone, RB Sleaford, BW Summers, NC Revay, Z Szentmiklosi, L Basunia, MS Belgya, T Escher, JE Krticka, M AF Hurst, A. M. Firestone, R. B. Sleaford, B. W. Summers, N. C. Revay, Zs. Szentmiklosi, L. Basunia, M. S. Belgya, T. Escher, J. E. Krticka, M. TI Investigation of the tungsten isotopes via thermal neutron capture SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; GAMMA ACTIVATION-ANALYSIS; BUDAPEST RESEARCH REACTOR; CROSS-SECTIONS; GIANT-RESONANCE; W-186(N,GAMMA)W-187 REACTION; N,GAMMA REACTION; DEFORMED-NUCLEI; STRENGTH; STATES AB Total radiative thermal neutron-capture gamma-ray cross sections for the W-182,W-183,W-184,W-186 isotopes were measured using guided neutron beams from the Budapest Research Reactor to induce prompt and delayed gamma rays from natural and isotopically-enriched tungsten targets. These cross sections were determined from the sum of measured gamma-ray cross sections feeding the ground state from low-lying levels below a cutoff energy, E-crit, where the level scheme is completely known, and continuum gamma rays from levels above E-crit, calculated using the Monte Carlo statistical-decay code DICEBOX. The new cross sections determined in this work for the tungsten nuclides are sigma(0)(W-182) = 20.5(14) b and sigma(11/2+) (W-183(m), 5.2 s) = 0.177(18) b; sigma(0)(W-183) = 9.37(38) b and sigma(5)-(W-184(m), 8.33 mu s) = 0.0247(55) b; sigma(0)(W-184) = 1.43(10) b and sigma(11/2+) (W-185(m), 1.67 min) = 0.0062(16) b; and, sigma(0)(W-186) = 33.33(62) b and sigma(9/2+) (W-187(m), 1.38 mu s) = 0.400(16) b. These results are consistent with earlier measurements in the literature. The W-186 cross section was also independently confirmed from an activation measurement, following the decay of W-187, yielding values for sigma(0)(W-186) that are consistent with our prompt gamma-ray measurement. The cross-section measurements were found to be insensitive to choice of level density or photon strength model and only weakly dependent on E-crit. Total radiative-capture widths calculated with DICEBOX showed much greater model dependence; however, the recommended values could be reproduced with selected model choices. The decay schemes for all tungsten isotopes were improved in these analyses. We were also able to determine new neutron-separation energies from our primary gamma-ray measurements for the respective (n,gamma) compounds: W-183 [S-n = 6190.88(6) keV]; W-184 [S-n = 7411.11(13) keV]; W-185 [S-n = 5753.74(5) keV]; and, W-187 [S-n = 5466.62(7) keV]. C1 [Hurst, A. M.; Firestone, R. B.; Basunia, M. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sleaford, B. W.; Summers, N. C.; Escher, J. E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Revay, Zs.; Szentmiklosi, L.; Belgya, T.] Hungarian Acad Sci, Energy Res Ctr, H-1525 Budapest, Hungary. [Revay, Zs.] Tech Univ Munich, Forsch Neutronenquelle Heinz Maier Leibnitz FRM 2, Garching, Germany. [Krticka, M.] Charles Univ Prague, Fac Math & Phys, CR-18000 Prague, Czech Republic. RP Hurst, AM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM AMHurst@lbl.gov RI Szentmiklosi, Laszlo/F-5362-2015; OI Szentmiklosi, Laszlo/0000-0001-7747-8545; Firestone, Richard/0000-0003-3833-5546 FU University of California; Director, Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U. S. Department of Energy at the Lawrence LivermoreNational Laboratory [DE-AC52-07NA27344]; NAP [VENEUS08, OMFB-00184/2006]; Ministry of Education of the Czech Republic [MSM 002 162 0859]; Czech Science Foundation [13-07117S] FX This work was performed under the auspices of the University of California, supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, and by the U. S. Department of Energy at the Lawrence LivermoreNational Laboratory under Contract No. DE-AC52-07NA27344. The access to the Budapest PGAA facility was financially supported by the NAP VENEUS08 grant under Contract No. OMFB-00184/2006. Additional support was received through Research Plan No. MSM 002 162 0859 supplied by the Ministry of Education of the Czech Republic and Grant No. 13-07117S of the Czech Science Foundation. The operations staff at the Budapest Research Reactor is gratefully acknowledged. NR 79 TC 8 Z9 8 U1 1 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 9 PY 2014 VL 89 IS 1 AR 014606 DI 10.1103/PhysRevC.89.014606 PG 22 WC Physics, Nuclear SC Physics GA AB9YH UT WOS:000332151100003 ER PT J AU Lin, CY McCurdy, CW Rescigno, TN AF Lin, Chih-Yuan McCurdy, C. W. Rescigno, T. N. TI Complex Kohn approach to molecular ionization by high-energy electrons: Application to H2O SO PHYSICAL REVIEW A LA English DT Article ID IMPACT IONIZATION; CROSS-SECTIONS; WATER-MOLECULES; COLLISIONS; HELIUM; EXCITATION; SCATTERING; STATE AB The complex Kohn variational method, which has been extensively applied to low-energy molecule scattering, is extended to treat molecular ionization by fast electrons under the assumption that the incident and scattered electrons can be described by plane waves. The formulation reduces to the computation of the continuum generalized oscillation strength, which amounts to a generalization of the molecular photoionization problem to which the Kohn method has been successfully applied. To illustrate the approach, we present fully differential cross sections for the case of water, where good experimental data is available for comparison. C1 [Lin, Chih-Yuan; McCurdy, C. W.; Rescigno, T. N.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [McCurdy, C. W.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. RP Lin, CY (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. FU US Department of Energy by the University of California Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US DOE Office of Basic Energy Sciences, Division of Chemical Sciences FX This work was performed under the auspices of the US Department of Energy by the University of California Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231 and was supported by the US DOE Office of Basic Energy Sciences, Division of Chemical Sciences. NR 25 TC 8 Z9 8 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JAN 9 PY 2014 VL 89 IS 1 AR 012703 DI 10.1103/PhysRevA.89.012703 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AC0FH UT WOS:000332169700005 ER PT J AU Denbleyker, A Liu, YZ Meurice, Y Qin, MP Xiang, T Xie, ZY Yu, JF Zou, HY AF Denbleyker, Alan Liu, Yuzhi Meurice, Y. Qin, M. P. Xiang, T. Xie, Z. Y. Yu, J. F. Zou, Haiyuan TI Controlling sign problems in spin models using tensor renormalization SO PHYSICAL REVIEW D LA English DT Article ID 2-DIMENSIONAL XY-MODEL; PHASE-TRANSITIONS; TEMPERATURE; EXPANSIONS; STRENGTH; DENSITY; ZEROS AB We consider the sign problem for classical spin models at complex beta = 1/g(0)(2) on L x L lattices. We show that the tensor renormalization group method allows reliable calculations for larger Im beta than the reweighting Monte Carlo method. For the Ising model with complex beta we compare our results with the exact Onsager-Kaufman solution at finite volume. The Fisher zeros can be determined precisely with the tensor renormalization group method. We check the convergence of the tensor renormalization group method for the O(2) model on L x L lattices when the number of states D-s increases. We show that the finite size scaling of the calculated Fisher zeros agrees very well with the Kosterlitz-Thouless transition assumption and predict the locations for larger volume. The location of these zeros agree with Monte Carlo reweighting calculation for small volume. The application of the method for the O(2) model with a chemical potential is briefly discussed. C1 [Denbleyker, Alan; Liu, Yuzhi; Meurice, Y.; Zou, Haiyuan] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Liu, Yuzhi] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Qin, M. P.; Xiang, T.; Xie, Z. Y.; Yu, J. F.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Liu, Yuzhi] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. RP Zou, HY (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. EM haiyuan-zou@uiowa.edu RI qin, mingpu/S-1545-2016 OI qin, mingpu/0000-0001-7733-9684 FU Department of Energy [DE-SC0010114, FG02-91ER40664]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; University of Iowa's Helium Cluster; URA Visiting Scholars' program; United States Department of Energy [DE-AC02-07CH11359]; National Natural Science Foundation of China [10934008, 10874215]; MOST 973 Project [2011CB309703]; NSF [1066293] FX This research was supported in part by the Department of Energy under Grant Nos. DE-SC0010114 and FG02-91ER40664. We have used resources of the National Energy Research Scientific Computing Center which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and The University of Iowa's Helium Cluster. Y. L. was supported by the URA Visiting Scholars' program. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. T. X., Z. X, J. Y, and M. Q. were supported by the National Natural Science Foundation of China (Grants No. 10934008 and No. 10874215) and MOST 973 Project (Grant No. 2011CB309703). Our work on the subject started while attending the KITPC workshop "Critical Properties of Lattice Models" in summer 2012. Y. M. did part of the work while at the workshop "LGT in the LHC Era" in summer 2013 at the Aspen Center for Physics supported by NSF Grant No. 1066293. NR 30 TC 12 Z9 12 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 9 PY 2014 VL 89 IS 1 AR 016008 DI 10.1103/PhysRevD.89.016008 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5PP UT WOS:000331841100009 ER PT J AU Tien, KJ Wang, MZ Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Bakich, AM Bala, A Bhuyan, B Bozek, A Bracko, M Browder, TE Chang, P Chekelian, V Chen, A Chen, P Cheon, BG Chilikin, K Chistov, R Cho, IS Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Danilov, M Dolezal, Z Drasal, Z Dutta, D Eidelman, S Farhat, H Fast, JE Ferber, T Gaur, V Ganguly, S Gillard, R Goh, YM Golob, B Haba, J Hayashii, H Horii, Y Hoshi, Y Hou, WS Hsiung, YB Huschle, M Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Julius, T Kah, DH Kang, JH Kato, E Kawasaki, T Kichimi, H Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, JH Kim, YJ Klucar, J Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kronenbitter, B Kuhr, T Kumita, T Kuzmin, A Kwon, YJ Lee, SH Li, J Li, Y Libby, J Liu, C Liu, Y Liventsev, D Lukin, P Miyabayashi, K Miyata, H Mohanty, GB Moll, A Mussa, R Nakano, E Nakao, M Natkaniec, Z Nayak, M Nedelkovska, E Ng, C Nisar, NK Nishida, S Nitoh, O Ogawa, S Okuno, S Olsen, SL Ostrowicz, W Oswald, C Park, CW Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Sahoo, H Saito, T Sakai, Y Sandilya, S Santel, D Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Seon, O Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Sibidanov, A Sohn, YS Sokolov, A Stanic, S Staric, M Steder, M Sumihama, M Sumiyoshi, T Tanida, K Tatishvili, G Teramoto, Y Uchida, M Uehara, S Uglov, T Unno, Y Uno, S Urquijo, P Vahsen, SE Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, P Watanabe, M Watanabe, Y Williams, KM Won, E Yamaoka, J Yamashita, Y Yashchenko, S Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Tien, K. -J. Wang, M. -Z. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Bakich, A. M. Bala, A. Bhuyan, B. Bozek, A. Bracko, M. Browder, T. E. Chang, P. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chilikin, K. Chistov, R. Cho, I. -S. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Danilov, M. Dolezal, Z. Drasal, Z. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Gaur, V. Ganguly, S. Gillard, R. Goh, Y. M. Golob, B. Haba, J. Hayashii, H. Horii, Y. Hoshi, Y. Hou, W. -S. Hsiung, Y. B. Huschle, M. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Julius, T. Kah, D. H. Kang, J. H. Kato, E. Kawasaki, T. Kichimi, H. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, J. H. Kim, Y. J. Klucar, J. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kronenbitter, B. Kuhr, T. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lee, S. -H. Li, J. Li, Y. Libby, J. Liu, C. Liu, Y. Liventsev, D. Lukin, P. Miyabayashi, K. Miyata, H. Mohanty, G. B. Moll, A. Mussa, R. Nakano, E. Nakao, M. Natkaniec, Z. Nayak, M. Nedelkovska, E. Ng, C. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Olsen, S. L. Ostrowicz, W. Oswald, C. Park, C. W. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Santel, D. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Sibidanov, A. Sohn, Y. -S. Sokolov, A. Stanic, S. Staric, M. Steder, M. Sumihama, M. Sumiyoshi, T. Tanida, K. Tatishvili, G. Teramoto, Y. Uchida, M. Uehara, S. Uglov, T. Unno, Y. Uno, S. Urquijo, P. Vahsen, S. E. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, P. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yamaoka, J. Yamashita, Y. Yashchenko, S. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Evidence for semileptonic B- -> p(p)over-barl(-)(nu)over-bar(l) decays SO PHYSICAL REVIEW D LA English DT Article AB We find evidence for the semileptonic baryonic decay B- -> p (p) over barl(-)(nu) over bar (l) (l = e, mu), based on a data sample of 772 million B (B) over bar pairs collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy electron-positron collider. A neural-network based hadronic B-meson tagging method is used in this study. The branching fraction of B- -> p (p) over barl(-)(nu) over bar (l) is measured to be (5.8(-2.1)(+2.4)(stat) +/- 0.9(syst)) x 10(-6) with a significance of 3.2 sigma s, where lepton universality is assumed. We also estimate the corresponding upper limit: B(B- -> p (p) over barl(-)(nu) over bar (l)) < 9.6 x 10(-6) at the 90% confidence level. This measurement helps constrain the baryonic transition form factor in B decays. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Oswald, C.; Urquijo, P.] Univ Bonn, D-53115 Bonn, Germany. [Aulchenko, V.; Eidelman, S.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Aulchenko, V.; Eidelman, S.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Liu, Y.; Santel, D.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Sahoo, H.; Vahsen, S. E.; Varner, G.; Yamaoka, J.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Itoh, R.; Iwasaki, Y.; Kichimi, H.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Uehara, S.; Uno, S.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Chistov, R.; Danilov, M.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Korpar, S.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Huschle, M.; Kronenbitter, B.; Kuhr, T.; Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kah, D. H.; Kim, H. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Moll, A.; Nedelkovska, E.; Ritter, M.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Danilov, M.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Seon, O.; Shen, C. P.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Horii, Y.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Tien, K. -J.; Wang, M. -Z.; Chang, P.; Chen, P.; Hou, W. -S.; Hsiung, Y. B.; Shiu, J. -G.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Natkaniec, Z.; Ostrowicz, W.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Kawasaki, T.; Miyata, H.; Watanabe, M.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Liu, C.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Li, J.; Olsen, S. L.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.; Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.; Sato, Y.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Tokyo 1848588, Japan. [Li, Y.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Cho, I. -S.; Kang, J. H.; Kwon, Y. -J.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. RP Tien, KJ (reprint author), Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. RI Danilov, Mikhail/C-5380-2014; Krokovny, Pavel/G-4421-2016; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Uglov, Timofey/B-2406-2014; Chilikin, Kirill/B-4402-2014 OI Danilov, Mikhail/0000-0001-9227-5164; Krokovny, Pavel/0000-0002-1236-4667; Chistov, Ruslan/0000-0003-1439-8390; Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Chilikin, Kirill/0000-0001-7620-2053 FU MEXT (Japan); JSPS (Japan); Nagoya's TLPRC (Japan); ARC (Australia); DIISR (Australia); NSFC (China); MSMT (Czechia); CZF (Germany); DFG (Germany); VS (Germany); DST (India); INFN (Italy); MEST (Korea); NRF (Korea); GSDC of KISTI (Korea); WCU (Korea); MNiSW (Poland); NCN (Poland); MES (Russia); RFAAE (Russia); ARRS (Slovenia); IKERBASQUE (Spain); UPV/EHU (Spain); NSC (Taiwan); MOE (Taiwan); DOE (USA); NSF (USA) FX We thank the KEKB group for excellent operation of the accelerator; the KEK cryogenics group for efficient solenoid operations; and the KEK computer group, the NII, and PNNL/EMSL for valuable computing and SINET4 network support. We acknowledge support from MEXT, JSPS and Nagoya's TLPRC (Japan); ARC and DIISR (Australia); NSFC (China); MSMT (Czechia); CZF, DFG, and VS (Germany); DST (India); INFN (Italy); MEST, NRF, GSDC of KISTI, and WCU (Korea); MNiSW and NCN (Poland); MES and RFAAE (Russia); ARRS (Slovenia); IKERBASQUE and UPV/EHU (Spain); SNSF (Switzerland); NSC and MOE (Taiwan); and DOE and NSF (USA). NR 24 TC 4 Z9 4 U1 0 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 9 PY 2014 VL 89 IS 1 AR 011101 DI 10.1103/PhysRevD.89.011101 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5PP UT WOS:000331841100001 ER PT J AU Moser, S Moreschini, L Ebrahimi, A Dalla Piazza, B Isobe, M Okabe, H Akimitsu, J Mazurenko, VV Kim, KS Bostwick, A Rotenberg, E Chang, J Ronnow, HM Grioni, M AF Moser, S. Moreschini, L. Ebrahimi, A. Dalla Piazza, B. Isobe, M. Okabe, H. Akimitsu, J. Mazurenko, V. V. Kim, K. S. Bostwick, A. Rotenberg, E. Chang, J. Ronnow, H. M. Grioni, M. TI The electronic structure of the high-symmetry perovskite iridate Ba2IrO4 SO NEW JOURNAL OF PHYSICS LA English DT Article ID SR2IRO4 AB We report angle-resolved photoemission (ARPES) measurements, density functional and model tight-binding calculations on Ba2IrO4 (Ba-214), an antiferromagnetic (T-N = 230 K) insulator. Ba-214 does not exhibit the rotational distortion of the IrO6 octahedra that is present in its sister compound Sr2IrO4 (Sr-214), and is therefore an attractive reference material to study the electronic structure of layered iridates. We find that the band structures of Ba-214 and Sr214 are qualitatively similar, hinting at the predominant role of the spin-orbit interaction in these materials. Temperature-dependent ARPES data show that the energy gap persists well above TN, and favor a Mott over a Slater scenario for this compound. C1 [Moser, S.; Ebrahimi, A.; Dalla Piazza, B.; Chang, J.; Ronnow, H. M.; Grioni, M.] Ecole Polytech Fed Lausanne, ICMP, CH-1015 Lausanne, Switzerland. [Moser, S.; Moreschini, L.; Bostwick, A.; Rotenberg, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. [Isobe, M.; Okabe, H.] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Akimitsu, J.] Aoyama Gakuin Univ, Dept Math & Phys, Chuo Ku, Sagamihara, Kanagawa 2525258, Japan. [Mazurenko, V. V.] Ural Fed Univ, Theoret Phys & Appl Math Dept, Ekaterinburg 620002, Russia. RP Moser, S (reprint author), Ecole Polytech Fed Lausanne, ICMP, CH-1015 Lausanne, Switzerland. EM simon.moser@epfl.ch RI Chang, Johan/F-1506-2014; Rotenberg, Eli/B-3700-2009; Dalla Piazza, Bastien/M-6954-2014; EPFL, Physics/O-6514-2016 OI Chang, Johan/0000-0002-4655-1516; Rotenberg, Eli/0000-0002-3979-8844; Dalla Piazza, Bastien/0000-0003-4997-7165; FU Swiss NSF LM; Swiss NSF [N PA00P21-36420]; grant program of President of Russian Federation [MK-5565.2013.2]; contract of the Ministry of Education and Science of Russia [N 14.A18.21.0076]; Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge insightful discussions with V I Anisimov, A O Shorikov, B J Kim, D F McMorrow, S Boseggia and C Tournier-Colletta. Special thanks are due to K M Shen for sharing with us his unpublished data. The work at Lausanne is supported by the Swiss NSF LM was supported by the Swiss NSF Grant N PA00P21-36420. The work of VVM is supported by the grant program of President of Russian Federation MK-5565.2013.2 and the contract of the Ministry of Education and Science of Russia N 14.A18.21.0076. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 33 TC 18 Z9 18 U1 6 U2 90 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 9 PY 2014 VL 16 DI 10.1088/1367-2630/16/1/013008 PG 13 WC Physics, Multidisciplinary SC Physics GA 302AY UT WOS:000330574800003 ER PT J AU Wood, BC Ogitsu, T Otani, M Biener, J AF Wood, Brandon C. Ogitsu, Tadashi Otani, Minoru Biener, Juergen TI First-Principles-Inspired Design Strategies for Graphene-Based Supercapacitor Electrodes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOUBLE-LAYER CAPACITANCES; IMPEDANCE MEASUREMENTS; INTRINSIC LIMITATIONS; QUANTUM CAPACITANCE; INTERFACIAL CAPACITANCE; ACTIVATED CARBONS; H. WANG; GRAPHITE; DENSITY; STATES AB Using density-functional theory calculations on a variety of model surfaces, we demonstrate that the low theoretical quantum capacitance of graphene-based electrodes can be significantly improved by altering local structural and morphological features. Common point defects, dopants, strain, and surface rippling are considered, as well as differences between locally single-layer and multilayer configurations. Local curvature is particularly effective at improving quantum capacitance, as is the inclusion of certain point defects and substitutional dopants at sufficiently high concentrations. We also show that single-layer graphene exhibits poor screening behavior of the double-layer potential when compared with multilayer samples, which suggests that higher area-specific capacitance can be obtained with samples a few layers thick. Overall, our results demonstrate the viability of local structural engineering as a tool to optimize graphene derivatives for use as supercapacitor electrodes, potentially increasing their theoretical charge storage capacity by severalfold. C1 [Wood, Brandon C.; Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. [Otani, Minoru] AIST, Nanosyst Res Inst, Tsukuba, Ibaraki, Japan. [Biener, Juergen] Lawrence Livermore Natl Lab, Nanoscale Synth & Characterizat Lab, Livermore, CA 94550 USA. RP Wood, BC (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, POB 5508, Livermore, CA 94550 USA. EM brandonwood@llnl.gov RI Otani, Minoru/G-2270-2012; Mohd Jasni, Mohamad Redwani/E-7555-2015 OI Mohd Jasni, Mohamad Redwani/0000-0003-4036-4856 FU Lawrence Livermore National Laboratory Directed Research and Development (LDRD) Grant [12-ERD-035]; Japan-U.S. Cooperation Project for Research and Standardization of Clean Energy Technologies; U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX Funding was provided by Lawrence Livermore National Laboratory Directed Research and Development (LDRD) Grant 12-ERD-035 and the Japan-U.S. Cooperation Project for Research and Standardization of Clean Energy Technologies. Computing support came from the LLNL Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 66 TC 36 Z9 36 U1 13 U2 129 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 4 EP 15 DI 10.1021/jp4044013 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200002 ER PT J AU Ferrari, D Celardo, GL Berman, GP Sayre, RT Borgonovi, F AF Ferrari, D. Celardo, G. L. Berman, G. P. Sayre, R. T. Borgonovi, F. TI Quantum Biological Switch Based on Superradiance Transitions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOSYNTHETIC REACTION-CENTER; PRIMARY CHARGE SEPARATION; LIGHT-HARVESTING COMPLEXES; II REACTION CENTERS; PHOTOSYSTEM-II; ENERGY-TRANSFER; PHYSIOLOGICAL TEMPERATURE; MULTIMER MODEL; WILD-TYPE; COHERENCE AB A linear chain of connected sites with two asymmetric sinks, one attached to each end, is used as a simple model of quantum (excitonic and/or electron) transport in photosynthetic biocomplexes. For a symmetric initial population in the middle of the chain, it is expected that transport is mainly directed toward the strongly coupled sink. However, we show that quantum effects radically change this intuitive "classical" mechanism so that transport can occur through the weakly coupled sink with maximal efficiency. Using this capability, we show how to design a quantum switch that can transfer energy or charge to the strongly or weakly coupled branch of the chain, by changing the coupling to the sinks. The operational principles of this quantum device can be understood in terms of superradiance transitions and subradiant states. This switching, being a pure quantum effect, can be used as a witness of wavelike behavior in molecular chains. When realistic data are used for the photosystem II reaction center, this quantum biological switch is shown to retain its reliability, even at room temperature. C1 [Ferrari, D.; Celardo, G. L.; Borgonovi, F.] Univ Cattolica Sacro Cuore, Dept Math & Phys, I-25121 Brescia, Italy. [Ferrari, D.; Celardo, G. L.; Borgonovi, F.] Univ Cattolica Sacro Cuore, Interdisciplinary Labs Adv Mat Phys, I-25121 Brescia, Italy. [Celardo, G. L.; Borgonovi, F.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Berman, G. P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Sayre, R. T.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Sayre, R. T.] New Mexico Consortium, Los Alamos, NM 87544 USA. RP Borgonovi, F (reprint author), Univ Cattolica Sacro Cuore, Dept Math & Phys, Via Musei 41, I-25121 Brescia, Italy. EM fausto.borgonovi@unicatt.it RI celardo, giuseppe/J-3629-2015; OI celardo, giuseppe/0000-0002-3679-1954; Sayre, Richard/0000-0002-3153-7084 FU Regione Lombardia; CILEA Consortium through a LISA Initiative (Laboratory for Interdisciplinary Advanced Simulation); Universita Cattolica [D.2.2 2011]; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work has been supported by Regione Lombardia and CILEA Consortium through a LISA Initiative (Laboratory for Interdisciplinary Advanced Simulation) 2011 grant available at http://lisa.cilea.it. Support by the grant D.2.2 2011 (Calcolo ad alte prestazioni) from Universita Cattolica is also acknowledged. The work by GPB and RTS was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. We also thank Gary Doolen for useful comments. NR 56 TC 16 Z9 16 U1 1 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 20 EP 26 DI 10.1021/jp4092909 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200004 ER PT J AU Callini, E Borgschulte, A Hugelshofer, CL Ramirez-Cuesta, AJ Zuttel, A AF Callini, Elsa Borgschulte, Andreas Hugelshofer, Cedric L. Ramirez-Cuesta, Anibal J. Zuettel, Andreas TI The Role of Ti in Alanates and Borohydrides: Catalysis and Metathesis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID REVERSIBLE HYDROGEN STORAGE; DENSITY-FUNCTIONAL THEORY; SODIUM ALANATE; DEUTERIUM EXCHANGE; ALUMINUM HYDRIDES; COMPLEX HYDRIDES; NAALH4; DECOMPOSITION; LIBH4; DEHYDROGENATION AB Ti catalyzes the hydrogen sorption reaction in alanates and allows the measurement of pressure composition isotherms, that is, the reaction equilibrates at each point of the isotherm. Although some effects of Ti compounds addition to borohydrides have been shown, our measurements show that the hydrogen desorption reaction from borohydrides is not catalyzed by Ti, when the system is exposed to a gas flow. The reabsorption of hydrogen by the products of the desorption reaction requires high temperatures and high pressures. Furthermore, the reaction pathway for the hydrogen desorption is different from the absorption one and as a consequence the borohydrides do not equilibrate with the gas phase during the hydrogen sorption reactions. Ti in borohydrides leads to the formation of stable and volatile Ti-containing species, for example, (Ti(BH4)(3)). This is a metathesis reaction, that is, a bimolecular process involving the exchange of bonds between the two reacting chemical species. In this paper, we have investigated via spectroscopy measurements the hydrogen sorption reactions of NaAlH4 and LiBH4 with Ti catalyst in view of the changes in the solid phase as well as in the gas phase. C1 [Callini, Elsa; Borgschulte, Andreas; Hugelshofer, Cedric L.; Zuettel, Andreas] Empa, Swiss Fed Labs Mat Testing & Res, CH-8600 Dubendorf, Switzerland. [Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Callini, E (reprint author), Empa, Swiss Fed Labs Mat Testing & Res, CH-8600 Dubendorf, Switzerland. EM elsa.callini@empa.ch RI Ramirez-Cuesta, Timmy/A-4296-2010; Borgschulte, Andreas/D-5168-2016 OI Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Borgschulte, Andreas/0000-0001-6250-4667 FU Swiss Federal Office of Energy through the project ACH; CCEM and Swisselectric research through the HyTech project; Fuel Cells and Hydrogen Joint Undertaking [303428] FX This work was financially supported by the Swiss Federal Office of Energy through the project ACH and by CCEM and Swisselectric research through the HyTech project. The research leading to these results has received funding from the Fuel Cells and Hydrogen Joint Undertaking under BOR4STORE Grant 303428. NR 54 TC 9 Z9 9 U1 4 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 77 EP 84 DI 10.1021/jp407999r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200011 ER PT J AU Bakalis, J Cook, AR Asaoka, S Forster, M Scherf, U Miller, JR AF Bakalis, Jin Cook, Andrew R. Asaoka, Sadayuki Forster, Michael Scherf, Ulrich Miller, John R. TI Polarons, Compressed Polarons, and Bipolarons in Conjugated Polymers SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CHARGE-TRANSPORT; CONDUCTING POLYMERS; ABSORPTION-SPECTRA; ELECTRON-TRANSFER; PULSE-RADIOLYSIS; OPTICAL-PROPERTIES; EXCITED-STATES; METALLIC STATE; SODIUM-CATION; AB-INITIO AB Extensive reductive chemical doping in four conjugated polymers showed evolution of optical spectra for negative polarons and more reduced species. Delocalization lengths of the polarons, which ranged from 2 to 6 nm, were determined from measurements of bleaching of the neutrals, with the extinction coefficients measured by pulse radiolysis. A particular advantage of reductive doping is the ability to encapsulate the Na+ counterions in the C-222 cryptand to control the interaction of charges with counterions. For lightly doped chains C-222 had little effect on the delocalization lengths or spectra of the two polaron transitions P-1 and P-2, perhaps because most were completely dissociated to free ions. C-222 did strongly alter the spectra when many electrons were added to a chain. For the shortest polarons, 2 nm in poly(phenylene-vinylene) (PPV), energies of the P-1 and P-2 transitions increased with the extent of reduction. The effect on the P, transition was greater in the absence of C-222 indicating ion-pairing equilibria for the short PPV polarons. Highly reduced ions formed upon injection of multiple electrons included polarons compressed by factors of four or more from their normal lengths to similar to 1 charge/nm: a highly reduced 60 nm long chain contained similar to 60 electrons. For compressed polarons the transitions shifted with increasing reduction indicating sensitivity to counterions: ion pairing is an important determinant of the behavior upon multiple reductions. C1 [Bakalis, Jin; Cook, Andrew R.; Miller, John R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Bakalis, Jin] CUNY City Coll, Dept Phys, New York, NY 10031 USA. [Asaoka, Sadayuki] Kyoto Inst Technol, Dept Biomol Engn, Sakyo Ku, Kyoto 6068585, Japan. [Forster, Michael; Scherf, Ulrich] Berg Univ Wuppertal, Macromol Chem Grp, D-42119 Wuppertal, Germany. RP Miller, JR (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM jrmiller@bnl.gov RI Scherf, Ullrich/G-1552-2012; OI Cook, Andrew/0000-0001-6633-3447 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-98-CH10886]; National Science Foundation [0652963]; QCC CUNY; FAST Program at BNL FX The authors gratefully acknowledge support of the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through Grant #DE-AC02-98-CH10886, and use of the LEAF Facility of the BNL Accelerator Center for Energy Research. We thank Dr. Seogjoo Jang for collaborative encouragement, and J.B. thanks National Science Foundation Grant #0652963 titled Queens Borough Bridge to QC and QCC CUNY, and the FAST Program at BNL for partial support. NR 67 TC 4 Z9 4 U1 1 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 114 EP 125 DI 10.1021/jp408910a PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200015 ER PT J AU Horan, JL Lingutla, A Ren, H Kuo, MC Sachdeva, S Yang, Y Seifert, S Greenlee, LF Yandrasits, MA Hamrock, SJ Frey, MH Herring, AM AF Horan, James L. Lingutla, Anitha Ren, Hui Kuo, Mei-Chen Sachdeva, Sonny Yang, Yuan Seifert, Soenke Greenlee, Lauren F. Yandrasits, Michael A. Hamrock, Steven J. Frey, Matthew H. Herring, Andrew M. TI Fast Proton Conduction Facilitated by Minimum Water in a Series of Divinylsilyl-11-silicotungstic. Acid-co-Butyl Acrylate-co-Hexanediol Diacrylate Polymers SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FUEL-CELL APPLICATIONS; COMPOSITE MEMBRANES; HETEROPOLY ACIDS; FIELD GRADIENT; DODECAMOLYBDOPHOSPHORIC ACID; 12-TUNGSTOPHOSPHORIC ACID; NANOCOMPOSITE MEMBRANES; DIFFUSION MEASUREMENTS; ELEVATED-TEMPERATURES; SILICOTUNGSTIC ACID AB Studies of proton transport in novel materials are important to enable a large array of electrochemical devices. In this study, we show that heteropoly acids (HPAs) when immobilized in polymer matrixes have highly mobile protons. Divinyl-11-silicotungstic acid, an HPA, was copolymerized with butyl acrylate and hexanediol diacrylate at various weight percentage loadings from 25% to 85% using UV initiated polymerizations. The resultant films were tan colored flexible sheets of ca. 120 mu m thickness. The morphology of these films varied with loading, showing phase separation into clustered HPA above a 50 wt % loading and lamella morphologies above an 80 wt % loading. Water uptake was strongly associated with the HPA clusters, which facilitated transport of protons. This was realized by proton conductivities as high as 0.4 S cm(-1) at 95 degrees C and 95% RH and 0.1 S cm(-1) at 85 degrees C and 50% RH. Pulse field gradient spin echo NMR measurements indicated that water self-diffusion was fast (1.4 x 10(-5) and 4.4 x 10(-5) cm(2) s(-1) for 50% and 100% RH, respectively) at 80 degrees C. We show that the water in these systems is highly associated with the HPA clusters and that fast proton transport is facilitated by as few as 3 water molecules per proton. C1 [Horan, James L.; Kuo, Mei-Chen; Sachdeva, Sonny; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Horan, James L.; Kuo, Mei-Chen; Sachdeva, Sonny; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Lingutla, Anitha; Ren, Hui; Frey, Matthew H.] 3M Co, Corp Res Mat Lab 3M, St Paul, MN 55144 USA. [Yandrasits, Michael A.; Hamrock, Steven J.] 3M Co, Component Fuel Cell Program 3M, St Paul, MN 55144 USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Greenlee, Lauren F.] NIST, Appl Chem & Mat Div, Boulder, CO 80305 USA. RP Herring, AM (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM aherring@mines.edu OI Sachdeva, Sonny/0000-0002-1239-2684; Greenlee, Lauren/0000-0001-6147-1533; Herring, Andrew/0000-0001-7318-5999 FU U.S. DOE office of energy efficiency and renewable energy [DE-FG36-06GO16032]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ARO DURIP [W911NF-NF-1-0462]; NSF MRI program [0923537] FX This work was supported by the U.S. DOE office of energy efficiency and renewable energy under contract no. DE-FG36-06GO16032. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. The IR microscope was obtained from an ARO DURIP under contract no. W911NF-NF-1-0462. The CSM NMR facility was supported by the NSF MRI program under contract no. 0923537. NR 64 TC 5 Z9 5 U1 3 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 135 EP 144 DI 10.1021/jp4089657 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200017 ER PT J AU Hong, MK Lee, DH Phillpot, SR Sinnott, SB AF Hong, Minki Lee, Dong-Hwa Phillpot, Simon R. Sinnott, Susan B. TI A Mechanism for TiO2 Formation on Stepped TiN(001) from First-Principles Calculations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TITANIUM NITRIDE; PHOTOELECTRON-SPECTROSCOPY; MOLECULAR PRECURSORS; INTRINSIC DEFECTS; SURFACE; OXIDATION; DISSOCIATION; ADSORPTION; OXYGEN; SITES AB The adsorption of O-2 on the TiN(001) stepped surface and the consequent formation of surface oxide have been characterized using first-principles calculations. The adsorption and dissociation of O-2 on both the flat and the stepped surface are predicted to be spontaneous. Compared with the flat surface, however, the dissociation of O-2 on the stepped surface is predicted to be more exothermic. A formation mechanism for TiO2 at the step is proposed that includes a nitrogen exit channel that enables further oxidation. C1 [Hong, Minki; Phillpot, Simon R.; Sinnott, Susan B.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Lee, Dong-Hwa] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Sinnott, SB (reprint author), Univ Florida, POB 116400, Gainesville, FL 32611 USA. EM ssinn@mse.ufl.edu RI Lee, Donghwa/G-7934-2012; Sinnott, Susan/P-8523-2014; OI Lee, Donghwa/0000-0002-8956-3648; Sinnott, Susan/0000-0002-3598-0403; Phillpot, Simon/0000-0002-7774-6535 FU National Science Foundation [DMR-1005779] FX We gratefully acknowledge the support of the National Science Foundation (DMR-1005779). NR 34 TC 2 Z9 2 U1 1 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 384 EP 388 DI 10.1021/jp409494q PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200042 ER PT J AU Uysal, A Zhou, H Feng, G Lee, SS Li, S Fenter, P Cummings, PT Fulvio, PF Dai, S McDonough, JK Gogotsi, Y AF Uysal, Ahmet Zhou, Hua Feng, Guang Lee, Sang Soo Li, Song Fenter, Paul Cummings, Peter T. Fulvio, Pasquale F. Dai, Sheng McDonough, John K. Gogotsi, Yury TI Structural Origins of Potential Dependent Hysteresis at the Electrified Graphene/Ionic Liquid Interface SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY REFLECTIVITY; TEMPERATURE IONIC LIQUID; MOLECULAR-DYNAMICS SIMULATIONS; DOUBLE-LAYER; DIFFERENTIAL CAPACITANCE; SURFACE; ELECTRODE; SLOW; TIME; RELAXATION AB We studied the potential and time-dependent changes in the electric double layer (EDL) structure of an imidazolium-based room temperature ionic liquid (RTIL) electrolyte at an epitaxial graphene (EG) surface. We used in situ X-ray reflectivity (XR) to determine the EDL structure at static potentials, during cyclic voltammetry (CV) and potential step measurements. The static potential structures were also investigated with fully atomistic molecular dynamics (MD) simulations. Combined XR and MD results show that the EDL structure has alternating anion/cation layers within the first nanometer of the interface and that these structures are distinct at the most positive and negative static potentials (1.0 and -0.4 V, respectively) applied in this study. The dynamical response of the EDL to potential steps has a slow component (>10 s) and the RTIL structure shows hysteresis during CV scans (e.g., at 100 mV/s scan rate). Our results reveal that both the slow kinetics and hysteresis are due to the reorganization of the distinct EDL structures found at the extreme potentials. C1 [Uysal, Ahmet; Lee, Sang Soo; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Zhou, Hua] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Feng, Guang; Li, Song; Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Fulvio, Pasquale F.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [McDonough, John K.; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [McDonough, John K.; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanotechnol Inst, Philadelphia, PA 19104 USA. RP Feng, G (reprint author), Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. EM ahmet@anl.gov; guang.feng@vanderbilt.edu; fenter@anl.gov RI Feng, Guang/D-8989-2011; Gogotsi, Yury/B-2167-2008; Fulvio, Pasquale/B-2968-2014; Uysal, Ahmet/E-7638-2010; Dai, Sheng/K-8411-2015; OI Gogotsi, Yury/0000-0001-9423-4032; Fulvio, Pasquale/0000-0001-7580-727X; Uysal, Ahmet/0000-0003-3278-5570; Dai, Sheng/0000-0002-8046-3931; Feng, Guang/0000-0001-6659-9181 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center; U.S. Department of Energy (DOE), Office of Science (SC), Office of Basic Energy Sciences (BES); DOE-SC-BES [DE-AC02-06CH11357]; DOE-SC [DE-AC02-05CH11231] FX We thank Tim T. Fister, Francesco Bellucci, and Nouamane Laanait for technical and intellectual support at various stages of the experiments. This material is based on work supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science (SC), Office of Basic Energy Sciences (BES). Use of the beamlines 6ID, 12ID, and 33ID at the Advanced Photon Source was supported by DOE-SC-BES under Contract DE-AC02-06CH11357 to UChicago Argonne, LLC, as operator of Argonne National Laboratory. This research used resources of the National Energy Research Scientific Computing Center, which is supported by DOE-SC under Contract No. DE-AC02-05CH11231, and the Palmetto cluster at Clemson University. NR 53 TC 33 Z9 33 U1 11 U2 129 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 9 PY 2014 VL 118 IS 1 BP 569 EP 574 DI 10.1021/jp4111025 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 289JL UT WOS:000329678200061 ER PT J AU Altinay, G Macdonald, RG AF Altinay, Gokhan Macdonald, R. Glen TI Determination of the Rate Constant for the OH((XII)-I-2) + OH((XII)-I-2) -> H2O + O(P-3) Reaction Over the Temperature Range 295 to 701 K SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DIPOLE-MOMENT FUNCTION; OH PLUS OH; PRESSURE-DEPENDENCE; TRANSITION INTENSITIES; TEMPERATURE-DEPENDENCE; MOLECULAR-CONSTANTS; HYDROXYL RADICALS; TERM VALUES; KINETICS; O(D-1) AB The rate constant for the radical-radical reaction OH((XII)-I-2) + OH((XII)-I-2) -> H2O + O(P-3) has been measured over the temperature and pressure ranges 295-701 K and 2-12 Torr, respectively, in mixtures of CF4, N-20,N- and H2O. The OH radical was produced by the 193 nm laser photolysis of N2O. The resulting O(D-1) atoms reacted rapidly with H2O to produce the OH radical. The OH radical was detected by high-resolution time-resolved infrared absorption spectroscopy using a single A-doublet component of the OH(1,0) P-1e/(f)(4.5) fundamental vibrational transition. A detailed kinetic model was used to determine the reaction rate constant as a function of temperature. These experiments were conducted in a new temperature controlled reaction chamber. The values of the measured rate constants are quite similar to the previous measurements from this laboratory of Bahng and Macdonald (J. Phys. Chem. A 2007, 111, 3850-3861); however, they cover a much larger temperature range. The results of the present work do not agree with recent measurements of Sangwan and Krasnoperov (J. Phys. Chem. A 2012, 116, 11817-11822). At 295 K the rate constant of the title reaction was found to be (2.52 +/- 0.63) X 10(-12) cm(3) molecule(-1) s(-1), where the uncertainty includes both experimental scatter and an estimate of systematic errors at the temperature range of the experiments, the rate constant can be represented by k(1a) = 4.79 x 10(-18)T(1.79) exp (879.0/T) cm(3) molecule(-1) s(-1) a uncertainty of +/- 24% at the 2 sigma level, including experimental scatter and systematic error. C1 [Altinay, Gokhan; Macdonald, R. Glen] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Macdonald, RG (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rgmacdonald@anl.gov FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy [DE-AC02-06CH11357] FX The authors thank Dr. S. Klippenstein and Dr. L. Harding of Argonne National Laboratory for valuable discussions on the OH + OH reaction. This work was performed under the auspices of the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy under Contract Number DE-AC02-06CH11357. NR 67 TC 6 Z9 6 U1 0 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 9 PY 2014 VL 118 IS 1 BP 38 EP 54 DI 10.1021/jp409344q PG 17 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 289JK UT WOS:000329678100005 PM 24328281 ER PT J AU Clark, JM Nimlos, MR Robichaud, DJ AF Clark, Jared M. Nimlos, Mark R. Robichaud, David J. TI Comparison of Unimolecular Decomposition Pathways for Carboxylic Acids of Relevance to Biofuels SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID BETAGAMMA-UNSATURATED ACIDS; GAS-PHASE DECARBOXYLATION; SET MODEL CHEMISTRY; THERMAL-DECOMPOSITION; ACETIC-ACID; FORMIC-ACID; EICOSAPENTAENOIC ACID; HYDROGEN ABSTRACTION; DENSITY FUNCTIONALS; KINETIC-PARAMETERS AB Quantum mechanical molecular modeling is used [M06-2X/6-311++G(2df,p)] to compare activation energies and rate constants for unimolecular decomposition pathways of saturated and unsaturated carboxylic acids that are important in the production of biofuels and that are models for plant and algae-derived intermediates. Dehydration and decarboxylation reactions are considered. The barrier heights to decarboxylation and dehydration are similar in magnitude for saturated acids (similar to 71 kcal mol(-1)), with an approximate 1:1 [H2O]/[CO2] branching ratio over the temperature range studied (500-2000 K). alpha,beta-Unsaturation lowers the barrier to decarboxylation between 2.2 and 12.2 kcal mol(-1) while increasing the barriers to dehydration by similar to 3 kcal mol(-1). The branching ratio, as a result, is an order of magnitude smaller, [H2O]/[CO2] = 0.07. For some alpha,beta-unsaturated acids, six-center transition states are available for dehydration, with barrier heights of similar to 35.0 kcal mol(-1). The branching ratio for these acids can be as high as 370:1. beta,gamma-Unsaturation results in a small lowering in the barrier height to decarboxylation (similar to 70.0 kcal mol(-1)). beta,gamma-Unsaturation also leads to a lowering in the dehydration pathway from 1.7 to 5.1 kcal mol(-1). These results are discussed with respect to predicted kinetic values for adds of importance in biofuels production. C1 [Clark, Jared M.; Nimlos, Mark R.; Robichaud, David J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Robichaud, DJ (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM David.Robichaud@nrel.gov FU Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE); DOE [DE-AC05-06OR23100]; DOE Bioenergy Technology Office [DE-AC36-99GO100337] FX This research was supported in part by the Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Awards under the EERE Biomass Program administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. ORISE is managed by Oak Ridge Associated Universities (ORAU) under DOE Contract Number DE-AC05-06OR23100. Additional funding was provided from the DOE Bioenergy Technology Office under Contract Number DE-AC36-99GO100337. All opinions expressed in this paper are the authors' and do not necessarily reflect the policies and views of DOE, ORAU, or ORISE. NR 74 TC 9 Z9 9 U1 2 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 9 PY 2014 VL 118 IS 1 BP 260 EP 274 DI 10.1021/jp4095485 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 289JK UT WOS:000329678100030 PM 24295398 ER PT J AU Gong, Y Vallet, V Michelini, MD Rios, D Gibson, JK AF Gong, Yu Vallet, Valerie Michelini, Maria del Carmen Rios, Daniel Gibson, John K. TI Activation of Gas-Phase Uranyl: From an Oxo to a Nitrido Complex SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID BASIS-SETS; COORDINATION-COMPLEXES; INFRARED-SPECTRA; URANIUM; ION; EXCHANGE; DENSITY; TRIPLE; LIGAND; PSEUDOPOTENTIALS AB The uranyl moiety, UO22+; is ubiquitous in the chemistry of uranium, the most prevalent actinide. Replacing the strong uranium-oxygen bonds in uranyl with other ligands is very challenging, having met with only limited success. We report here uranyl oxo bond activation in the gas phase to form a terminal nitrido complex, a previously elusive transformation. Collision induced dissociation of gas-phase UO2(NCO)Cl-2(-) in an ion trap produced the nitrido oxo complex, NUOCl2-, and CO2. NUOCl2- was computed by DFT to have C-s symmetry and a singlet ground state. The computed bond length and order indicate a triple U-N bond. Endothermic activation of UO2(NCO)Cl-2(-) to produce NUOCl2- and neutral CO2 was computed to be thermodynamically more favorable than NCO ligand loss. Complete reaction pathways for the CO2 elimination process were computed at the DFT level. C1 [Gong, Yu; Rios, Daniel; Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Vallet, Valerie] Univ Lille 1 Sci & Technol, Lab PhLAM, CNRS UMR 8523, F-59655 Villeneuve Dascq, France. [Michelini, Maria del Carmen] Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. RP Gibson, JK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jkgibson@lbl.gov RI Vallet, Valerie/G-8491-2012 OI Vallet, Valerie/0000-0002-2202-3858 FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; CNRS; French Ministere de l'Enseignement Superieur et de la Recherche; Universita della Calabria; National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05C1411231]; GENCI-CCRT [2012-081859, 2013-081859] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract No. DE-AC02-05CH11231 [Y.G., D.R, J.K.G.], by CNRS and French Ministere de l'Enseignement Superieur et de la Recherche [V.V.], and by the Universita della Calabria [M.C.M.]. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05C1411231, as well as the use of HPC resources from GENCI-CCRT (Grants 2012-081859 and 2013-081859). NR 55 TC 7 Z9 7 U1 8 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 9 PY 2014 VL 118 IS 1 BP 325 EP 330 DI 10.1021/jp4113798 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 289JK UT WOS:000329678100036 PM 24354492 ER PT J AU Teran, AA Balsara, NP AF Teran, Alexander A. Balsara, Nitash P. TI Thermodynamics of Block Copolymers with and without Salt SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MICROPHASE SEPARATION TRANSITION; SATURATED-HYDROCARBON POLYMERS; ORDER-DISORDER TRANSITION; INTEGRAL-EQUATION THEORY; MOLECULAR-WEIGHT; MONTE-CARLO; IONIC-CONDUCTIVITY; LIQUID STRUCTURE; PHASE-DIAGRAM; CHI-PARAMETER AB Ion-containing block copolymers are of interest for applications such as electrolytes in rechargeable lithium batteries. The addition of salt to these materials is necessary to make them conductive; however, even small amounts of salt can have significant effects on the phase behavior of these materials and consequently on their ion-transport and mechanical properties. As a result, the effect of salt addition on block copolymer thermodynamics has been the subject of significant interest over the past decade. This feature article describes a comprehensive study of the thermodynamics of block copolymer/salt mixtures over a wide range of molecular weights, compositions, salt concentrations, and temperatures. The Flory-Huggins interaction parameter was determined by fitting small-angle X-ray scattering data of disordered systems to predictions based on the random phase approximation. Experiments on neat block copolymers revealed that the Flory-Huggins parameter is a strong function of chain length. Experiments on block copolymer/salt mixtures revealed a highly nonlinear dependence of the Flory-Huggins parameter on salt concentration. These findings are a significant departure from previous results and indicate the need for improved theories for describing thermodynamic interactions in neat and salt-containing block copolymers. C1 [Teran, Alexander A.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Teran, Alexander A.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank Dr. Frances Allen and Dr. Andrew Minor for providing the TEM micrograph of the SEO/salt mixture. The synthesis and characterization of the polymer was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under contract DE-AC02-05CH11231 under the Batteries for Advanced Transportation Technologies (BATT) Program. A.A.T. was supported by a National Science Foundation Graduate Research Fellowship. SAXS experiments were performed at the Advanced Light Source, a user facilities at Lawrence Berkeley National Laboratory supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 42 TC 32 Z9 32 U1 6 U2 101 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 9 PY 2014 VL 118 IS 1 BP 4 EP 17 DI 10.1021/jp408079z PG 14 WC Chemistry, Physical SC Chemistry GA 289JJ UT WOS:000329678000002 PM 24229067 ER PT J AU Sangha, AK Davison, BH Standaert, RF Davis, MF Smith, JC Parks, JM AF Sangha, Amandeep K. Davison, Brian H. Standaert, Robert F. Davis, Mark F. Smith, Jeremy C. Parks, Jerry M. TI Chemical Factors that Control Lignin Polymerization SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID HORSERADISH-PEROXIDASE; BIOMASS RECALCITRANCE; MOLECULAR-MECHANICS; OXIDATION; DENSITY; BIOSYNTHESIS; LIGNIFICATION; ENERGIES; BIOFUELS; ALCOHOL AB Lignin is a complex, branched polymer that reinforces plant tissue. Understanding the factors that govern lignin structure is of central importance to the development of technologies for converting lignocellulosic biomass into fuels because lignin imparts resistance to chemical, enzymatic, and mechanical, deconstruction. Lignin is formed by enzymatic oxidation of phenolic monomers (monolignols) of three main types, guaiacyl (G), syringyl (S), and p-hydroxyphenyl (H) subunits. It is known that increasing the relative abundance of H subunits results in lower molecular weight lignin polymers and hence more easily deconstructed biomass, but it is not known why. Here, we report an analysis of frontier molecular orbitals in mono-, di-, and trilignols, calculated using density functional theory, which points to a requirement of strong p-electron density on the reacting phenolic oxygen atom of the neutral precursor for enzymatic oxidation to occur. This model is consistent with a proton-coupled electron transfer (PCET) mechanism and for the first time explains why H subunits in certain linkages (beta-beta or beta-5) react poorly and tend to "cap" the polymer. In general, beta-5 linkages with either a G or H terminus are predicted to inhibit elongation. More broadly, the model correctly accounts for the reactivity of the phenolic groups in a diverse set of dilignols comprising H and G subunits. Thus, we provide a coherent framework for understanding the propensity toward growth or termination of different terminal subunits in lignin. C1 [Sangha, Amandeep K.; Smith, Jeremy C.; Parks, Jerry M.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. [Davison, Brian H.; Smith, Jeremy C.; Parks, Jerry M.] Oak Ridge Natl Lab, Bioenergy Sci Ctr, Oak Ridge, TN 37831 USA. [Davison, Brian H.; Standaert, Robert F.; Parks, Jerry M.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Standaert, Robert F.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Davis, Mark F.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Davis, Mark F.] Natl Renewable Energy Lab, Bioenergy Sci Ctr, Golden, CO 80401 USA. [Standaert, Robert F.; Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. RP Parks, JM (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. EM parksjm@ornl.gov RI Parks, Jerry/B-7488-2009; Davison, Brian/D-7617-2013; smith, jeremy/B-7287-2012; Standaert, Robert/D-9467-2013; OI Parks, Jerry/0000-0002-3103-9333; Davison, Brian/0000-0002-7408-3609; smith, jeremy/0000-0002-2978-3227; Standaert, Robert/0000-0002-5684-1322; davis, mark/0000-0003-4541-9852 FU Bioenergy Science Center, a U.S. Department of Energy Bioenergy Research Center; office of Biological and Environmental Research in the Department of Energy Office of Science; National Energy Research Scientific Computing Center (NERSC) [m906, m1305] FX The authors thank Ariana Beste and Arthur J. Ragauskas for helpful discussions. This research was supported by the Bioenergy Science Center, which is a U.S. Department of Energy Bioenergy Research Center supported by the office of Biological and Environmental Research in the Department of Energy Office of Science. This work was conducted using the resources at the National Energy Research Scientific Computing Center (NERSC) under Grant Numbers m906 and m1305. NR 42 TC 16 Z9 16 U1 5 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 9 PY 2014 VL 118 IS 1 BP 164 EP 170 DI 10.1021/jp411998t PG 7 WC Chemistry, Physical SC Chemistry GA 289JJ UT WOS:000329678000017 PM 24341896 ER PT J AU Ellis, RJ AF Ellis, Ross J. TI Critical Exponents for Solvent Extraction Resolved Using SAXS SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID SMALL-ANGLE SCATTERING; STICKY SPHERES MODEL; N-DODECANE SYSTEM; CRITICAL-BEHAVIOR; REVERSE MICELLES; NEUTRON-SCATTERING; MICROEMULSION SYSTEMS; BUTYL PHOSPHATE; PHASE; OCTANE AB The solvent extraction of an ionizable solute (H3PO4) from water into a water-in-oil microemulsion, and subsequent organic phase splitting (known as third phase formation), has been recast as a critical phenomenon by linking system structure to solute concentration via a critical exponent. The transuranic extraction (TRUEX) system was investigated by extracting increasing concentrations of H3PO4 into a microemulsion consisting of two extractant amphiphiles (CMPO and TBP) and water in n-dodecane and taking small-angle X-ray scattering (SAXS) measurements from the resulting solutions. The H3PO4 concentration at which phase splitting occurred was defined as the critical concentration (X-C), and this was related to the precritical concentrations (X) by the reduced parameter epsilon = (X-C - X)/X-C. The scattering intensity at the zero angle I(0), relating to the interaction between reverse micellar aggregates, conformed to the relation I(0) = I-0 epsilon(-gamma), with critical exponent gamma = 2.20. To check gamma, SAXS measurements were taken from the organic phase in situ with variable temperature through the point at which third phase formation initiates (the critical temperature), giving I(0) = I(0)t(-gamma), where t = (T - T-C)/T-C and T-C and T are the critical and precritical temperatures, with critical exponent gamma = 2.55. These gamma values suggest third phase formation is a universal phenomenon manifest from a critical double point. Thus, solvent extraction is reduced to its fundamental physical roots where the system is not defined by detailed analysis of metrical properties but by linking the fundamental order to thermodynamic parameters via an exponent, working toward a more predictive understanding of third phase formation. C1 Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Ellis, RJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rellis@anl.gov RI ellis, ross/J-1981-2016 OI ellis, ross/0000-0001-7691-5205 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences [DE-AC02-06CH11357] FX This work and the use of the Advanced Photon Source are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, under Contract DE-AC02-06CH11357. NR 59 TC 4 Z9 4 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 9 PY 2014 VL 118 IS 1 BP 315 EP 322 DI 10.1021/jp408078v PG 8 WC Chemistry, Physical SC Chemistry GA 289JJ UT WOS:000329678000032 PM 24328275 ER PT J AU Gillis, KM Snow, JE Klaus, A Abe, N Adriao, AB Akizawa, N Ceuleneer, G Cheadle, MJ Faak, K Falloon, TJ Friedman, SA Godard, M Guerin, G Harigane, Y Horst, AJ Hoshide, T Ildefonse, B Jean, MM John, BE Koepke, J Machi, S Maeda, J Marks, NE McCaig, AM Meyer, R Morris, A Nozaka, T Python, M Saha, A Wintsch, RP AF Gillis, Kathryn M. Snow, Jonathan E. Klaus, Adam Abe, Natsue Adriao, Alden B. Akizawa, Norikatsu Ceuleneer, Georges Cheadle, Michael J. Faak, Kathrin Falloon, Trevor J. Friedman, Sarah A. Godard, Marguerite Guerin, Gilles Harigane, Yumiko Horst, Andrew J. Hoshide, Takashi Ildefonse, Benoit Jean, Marlon M. John, Barbara E. Koepke, Juergen Machi, Sumiaki Maeda, Jinichiro Marks, Naomi E. McCaig, Andrew M. Meyer, Romain Morris, Antony Nozaka, Toshio Python, Marie Saha, Abhishek Wintsch, Robert P. TI Primitive layered gabbros from fast-spreading lower oceanic crust SO NATURE LA English DT Article ID EAST PACIFIC RISE; MIDOCEAN RIDGE BASALTS; HESS DEEP RIFT; EQUATORIAL PACIFIC; OMAN OPHIOLITE; UPPER-MANTLE; LIQUID EQUILIBRIA; MAGMA CHAMBERS; FLOOR BASALTS; MELT AB Three-quarters of the oceanic crust formed at fast-spreading ridges is composed of plutonic rocks whose mineral assemblages, textures and compositions record the history of melt transport and crystallization between the mantle and the sea floor. Despite the importance of these rocks, sampling them in situ is extremely challenging owing to the overlying dykes and lavas. This means that models for understanding the formation of the lower crust are based largely on geophysical studies(1) and ancient analogues (ophiolites)(2-5) that did not form at typical mid-ocean ridges. Here we describe cored intervals of primitive, modally layered gabbroic rocks from the lower plutonic crust formed at a fast-spreading ridge, sampled by the Integrated Ocean Drilling Program at the Hess Deep rift. Centimetre-scale, modally layered rocks, some of which have a strong layering-parallel foliation, confirm a long-held belief that such rocks are a key constituent of the lower oceanic crust formed at fast-spreading ridges(3,6). Geochemical analysis of these primitive lower plutonic rocks-in combination with previous geochemical data for shallow-level plutonic rocks, sheeted dykes and lavas-provides the most completely constrained estimate of the bulk composition of fast-spreading oceanic crust so far. Simple crystallization models using this bulk crustal composition as the parental melt accurately predict the bulk composition of both the lavas and the plutonic rocks. However, the recovered plutonic rocks show early crystallization of orthopyroxene, which is not predicted by current models of melt extraction from the mantle(7) and mid-ocean-ridge basalt differentiation(8,9). The simplest explanation of this observation is that compositionally diverse melts are extracted from the mantle and partly crystallize before mixing to produce the more homogeneous magmas that erupt. C1 [Gillis, Kathryn M.; Faak, Kathrin] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC V8W 2Y2, Canada. [Snow, Jonathan E.] Univ Houston, Houston, TX 77204 USA. [Klaus, Adam] Texas A&M Univ, Integrated Ocean Drilling Program, US Implementing Org, College Stn, TX 77845 USA. [Abe, Natsue] Japan Agcy Marine Earth Sci & Technol, Inst Res Earth Evolut, Yokosuka, Kanagawa 2370061, Japan. [Adriao, Alden B.] Univ Fed Rio Grande do Sul, Inst Geosci, BR-91501970 Porto Alegre, RS, Brazil. [Akizawa, Norikatsu; Machi, Sumiaki] Kanazawa Univ, Dept Earth Sci, Kanazawa, Ishikawa 9201192, Japan. [Ceuleneer, Georges] Univ Toulouse 3, CNRS, UMS 831, Observ Midipyrenees, F-31400 Toulouse, France. [Cheadle, Michael J.; John, Barbara E.] Univ Wyoming, Dept 3006, Dept Geol & Geophys, Laramie, WY 82071 USA. [Faak, Kathrin] Ruhr Univ Bochum, Inst Geol Mineral & Geophys, D-44780 Bochum, Germany. [Falloon, Trevor J.] Univ Tasmania, Inst Marine & Antarctic Studies, Hobart, Tas, Australia. [Falloon, Trevor J.] Univ Tasmania, Sch Earth Sci, Hobart, Tas, Australia. [Friedman, Sarah A.] So Illinois Univ, Dept Geol, Carbondale, IL 62901 USA. [Godard, Marguerite; Ildefonse, Benoit] Univ Montpellier 2, CNRS UMR5243, Geosci Montpellier, CC 60, F-34095 Montpellier 5, France. [Guerin, Gilles] Columbia Univ, Lamont Doherty Earth Observ, Borehole Res Grp, Palisades, NY USA. [Harigane, Yumiko] Geol Survey Japan, Natl Inst Adv Ind Sci & Technol, Inst Geol & Geoinformat, Tsukuba, Ibaraki 3058567, Japan. [Horst, Andrew J.] Oberlin Coll, Dept Geol, Oberlin, OH 44074 USA. [Hoshide, Takashi] Tohoku Univ, Grad Sch Sci, Aoba Ku, Sendai, Miyagi 9808578, Japan. [Jean, Marlon M.] No Illinois Univ, Dept Geol & Environm, De Kalb, IL 60115 USA. [Koepke, Juergen] Leibniz Univ Hannover, Inst Mineral, D-30167 Hannover, Germany. [Maeda, Jinichiro; Python, Marie] Hokkaido Univ, Dept Nat Hist Sci, Kita Ku, Sapporo, Hokkaido 0600810, Japan. [Marks, Naomi E.] Lawrence Livermore Natl Lab, Chem & Mat Sci Dept, Livermore, CA 94551 USA. [McCaig, Andrew M.] Univ Leeds, Sch Earth & Environm, Leeds LS2 9JT, W Yorkshire, England. [Meyer, Romain] Univ Bergen, Ctr Geobiol, N-5007 Bergen, Norway. [Meyer, Romain] Univ Bergen, Dept Earth Sci, N-5007 Bergen, Norway. [Morris, Antony] Univ Plymouth, Sch Geog Earth & Environm Sci, Plymouth PL4 8AA, Devon, England. [Nozaka, Toshio] Okayama Univ, Dept Earth Sci, Okayama 7008530, Japan. [Saha, Abhishek] Univ Calcutta, Dept Geol, Kolkata 700019, India. [Wintsch, Robert P.] Indiana Univ, Dept Geol Sci, Bloomington, IN 47405 USA. RP Gillis, KM (reprint author), Univ Victoria, Sch Earth & Ocean Sci, POB 1700 Stn CSC, Victoria, BC V8W 2Y2, Canada. EM kgillis@uvic.ca RI Godard, Marguerite/A-7127-2008; Snow, Jonathan/E-5591-2011; ildefonse, benoit/A-6205-2009; NOZAKA, Toshio/B-2096-2011; McCaig, Andrew/C-1066-2014 OI Godard, Marguerite/0000-0003-3097-5135; ildefonse, benoit/0000-0001-7635-9288; McCaig, Andrew/0000-0001-7416-4911 NR 45 TC 16 Z9 18 U1 6 U2 91 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 9 PY 2014 VL 505 IS 7482 BP 204 EP + DI 10.1038/nature12778 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 286CG UT WOS:000329441500036 PM 24291793 ER PT J AU Retinskaya, E Luzum, M Ollitrault, JY AF Retinskaya, Ekaterina Luzum, Matthew Ollitrault, Jean-Yves TI Constraining models of initial conditions with elliptic and triangular flow data SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; NUCLEAR COLLISIONS; COLLECTIVE FLOW; ANISOTROPY; VISCOSITY; SIGNATURE; QCD AB We carry out a combined analysis of elliptic and triangular flow data using viscous relativistic hydrodynamics. We show that these data allow us to put tight constraints on models of the early dynamics of a nucleus-nucleus collision. Specifically, the rms values of the initial ellipticity epsilon(2) and the initial triangularity epsilon(3) are constrained to lie within a narrow band for each centrality. We use these constraints as a filter for existing Monte Carlo models of initial state, and provide a simple test that can be performed on any candidate model to determine its compatibility with data. C1 [Retinskaya, Ekaterina] CEA, IPhT, Inst Phys Theor Saclay, F-91191 Gif Sur Yvette, France. [Luzum, Matthew] McGill Univ, Montreal, PQ H3A 2TS, Canada. [Luzum, Matthew] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ollitrault, Jean-Yves] CNRS, IPhT, Inst Phys Theor Saclay, URA2306, F-91191 Gif Sur Yvette, France. RP Retinskaya, E (reprint author), CEA, IPhT, Inst Phys Theor Saclay, F-91191 Gif Sur Yvette, France. RI Luzum, Matthew/C-4986-2015 OI Luzum, Matthew/0000-0002-0367-7055 FU European Research Council under the Advanced Investigator Grant [ERC-AD-267258] FX We thank the ALICE Collaboration for providing experimental data, and Jurgen Schukraft for helpful discussion. We also thank Christoffer Flensburg and Bjorn Schenke, for providing results from the DIPSY and IP-Glasmamodels. This work is funded by the European Research Council under the Advanced Investigator Grant ERC-AD-267258. NR 85 TC 26 Z9 26 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 8 PY 2014 VL 89 IS 1 AR 014902 DI 10.1103/PhysRevC.89.014902 PG 7 WC Physics, Nuclear SC Physics GA AB9XZ UT WOS:000332150300002 ER PT J AU Mahyari, ZL Cannell, A Gomez, C Tezok, S Zelati, A de Mello, EVL Yan, JQ Mandrus, DG Sonier, JE AF Mahyari, Z. Lotfi Cannell, A. Gomez, C. Tezok, S. Zelati, A. de Mello, E. V. L. Yan, J. -Q. Mandrus, D. G. Sonier, J. E. TI Zero-field mu SR search for a time-reversal-symmetry-breaking mixed pairing state in superconducting Ba1-xKxFe2As2 SO PHYSICAL REVIEW B LA English DT Article AB We report the results of a zero-field muon-spin relaxation (ZF-mu SR) study of superconducting Ba1-xKxFe2As2 (0.5 <= x <= 0.9) in search of weak spontaneous internal magnetic fields associated with proposed time-reversal-symmetry-breaking mixed pairing states. The measurements were performed on polycrystalline samples, which do not exhibit the mesoscopic phase separation previously observed in single crystals of Ba1-xKxFe2As2. No evidence of spontaneous internal magnetic fields is found in any of the samples at temperatures down to T similar to 0.02 K. C1 [Mahyari, Z. Lotfi; Cannell, A.; Gomez, C.; Tezok, S.; Zelati, A.; Sonier, J. E.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [de Mello, E. V. L.] Univ Fed Fluminense, Inst Fis, BR-24210340 Niteroi, RJ, Brazil. [Yan, J. -Q.; Mandrus, D. G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Yan, J. -Q.; Mandrus, D. G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Sonier, J. E.] Canadian Inst Adv Res, Toronto, ON, Canada. RP Mahyari, ZL (reprint author), Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. RI Mandrus, David/H-3090-2014; de Mello, Evandro /C-5828-2015; OI de Mello, Evandro /0000-0001-5793-0506; Zelati, Amir/0000-0002-7895-3149 FU Canadian Institute of Advanced Research; Natural Sciences and Engineering Research Council of Canada; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank the staff of TRIUMF's Centre for Molecular and Materials Science for technical assistance, and C. Wu, R. M. Fernandes, R. F. Kiefl, L. Taillefer, C. Kallin, A. Chubukov, and M. Sigrist for informative discussions. The work at TRIUMF was supported by the Canadian Institute of Advanced Research, and the Natural Sciences and Engineering Research Council of Canada. J.Q.Y. and D.G.M. thank Dr. Chenglin Zhang for his help in synthesis. Work at ORNL was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. NR 37 TC 3 Z9 3 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 8 PY 2014 VL 89 IS 2 AR 020502 DI 10.1103/PhysRevB.89.020502 PG 5 WC Physics, Condensed Matter SC Physics GA AC0QO UT WOS:000332200000002 ER PT J AU Dumitru, A Guo, Y Altes, CPK AF Dumitru, Adrian Guo, Yun Altes, Chris P. Korthals TI Two-loop perturbative corrections to the thermal effective potential in gluodynamics SO PHYSICAL REVIEW D LA English DT Article ID T-HOOFT LOOP; HOT QCD; FINITE TEMPERATURE; ORDER-PARAMETER; GAUGE-THEORY; CUBIC ORDER AB The thermodynamics of pure glue theories can be described in terms of an effective action for the Polyakov loop. This effective action is of the Landau-Ginzburg type, and its variables are the angles parametrizing the loop. In this paper we compute perturbative corrections to this action. Remarkably, two-loop corrections turn out to be proportional to the one-loop action, independent of the eigenvalues of the loop. By a straightforward generalization of the 't Hooft coupling, this surprisingly simple result holds for any of the classical and exceptional groups. C1 [Dumitru, Adrian] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Dumitru, Adrian] CUNY, Baruch Coll, Dept Nat Sci, New York, NY 10010 USA. [Dumitru, Adrian] CUNY, Grad Sch, New York, NY 10016 USA. [Dumitru, Adrian] CUNY, Univ Ctr, New York, NY 10016 USA. [Guo, Yun] Univ Santiago de Compostela, Dept Fis Particulas, E-15782 Santiago De Compostela, Galicia, Spain. [Guo, Yun] Guangxi Normal Univ, Dept Phys, Guilin 541004, Peoples R China. [Altes, Chris P. Korthals] CNRS Case 907, Ctr Phys Theor, F-13288 Marseille, France. [Altes, Chris P. Korthals] NIKHEF Theory Grp, NL-1098 XG Amsterdam, Netherlands. RP Dumitru, A (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM dumitru@quark.phy.bnl.gov; yun.guo@usc.es; altes@cpt.univ-mrs.fr FU DOE Office of Nuclear Physics [DE-FG02-09ER41620]; City University of New York through the PSC-CUNY Research Award Program [65041-00 43, 66514-00 44]; European Research Council [HotLHC ERC-2001-StG-279579]; NSFC of China [11205035]; Guangxi Normal University [2011ZD004] FX We thank Rob Pisarski and Nan Su for useful discussions. A. D. gratefully acknowledges support by the DOE Office of Nuclear Physics through Grant No. DE-FG02-09ER41620 and by The City University of New York through the PSC-CUNY Research Award Program, Grants No. 65041-00 43 and No. 66514-00 44. Y. G. gratefully acknowledges support by the European Research Council Grant No. HotLHC ERC-2001-StG-279579, a grant from the NSFC of China with Project No. 11205035 and by Guangxi Normal University with Project No. 2011ZD004. NR 25 TC 7 Z9 7 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 8 PY 2014 VL 89 IS 1 AR 016009 DI 10.1103/PhysRevD.89.016009 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5OY UT WOS:000331839400003 ER PT J AU Martin, SP AF Martin, Stephen P. TI Three-loop Standard Model effective potential at leading order in strong and top Yukawa couplings SO PHYSICAL REVIEW D LA English DT Article ID RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; HIGGS MASS; ELECTROWEAK VACUUM; STABILITY BOUNDS; 2-LOOP; REGULARIZATION; DIAGRAMS; BOSON; LHC AB I find the three-loop contribution to the effective potential for the Standard Model Higgs field, in the approximation that the strong and top Yukawa couplings are large compared to all other couplings, using dimensional regularization with modified minimal subtraction. Checks follow from gauge invariance and renormalization group invariance. I also briefly comment on the special problems posed by Goldstone boson contributions to the effective potential, and on the numerical impact of the result on the relations between the Higgs vacuum expectation value, mass, and self-interaction coupling. C1 [Martin, Stephen P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Martin, Stephen P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Martin, Stephen P.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA USA. RP Martin, SP (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. FU National Science Foundation [PHY-1068369, NSF PHY11-25915] FX This work was supported in part by the National Science Foundation Grant No. PHY-1068369. This research was supported in part by the National Science Foundation under Grant No. NSF PHY11-25915. NR 56 TC 19 Z9 19 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 8 PY 2014 VL 89 IS 1 AR 013003 DI 10.1103/PhysRevD.89.013003 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5OY UT WOS:000331839400001 ER PT J AU Arpino, KE Wallace, DC Nie, YF Birol, T King, PDC Chatterjee, S Uchida, M Koohpayeh, SM Wen, JJ Page, K Fennie, CJ Shen, KM McQueen, TM AF Arpino, K. E. Wallace, D. C. Nie, Y. F. Birol, T. King, P. D. C. Chatterjee, S. Uchida, M. Koohpayeh, S. M. Wen, J-J Page, K. Fennie, C. J. Shen, K. M. McQueen, T. M. TI Evidence for Topologically Protected Surface States and a Superconducting Phase in [Tl-4](Tl1-xSnx)Te(3)Using Photoemission, Specific Heat, and Magnetization Measurements, and Density Functional Theory SO PHYSICAL REVIEW LETTERS LA English DT Article ID CRYSTAL; BI2SE3; BI2TE3 AB We report the discovery of surface states in the perovskite superconductor [Tl-4]TlTe3 (Tl5Te3) and its nonsuperconducting tin-doped derivative [Tl-4](Tl0.4Sn0.6)Te-3 as observed by angle-resolved photoemission spectroscopy. Density functional theory calculations predict that the surface states are protected by a Z(2) topology of the bulk band structure. Specific heat and magnetization measurements show that Tl5Te3 has a superconducting volume fraction in excess of 95%. Thus Tl5Te3 is an ideal material in which to study the interplay of bulk band topology and superconductivity. C1 [Arpino, K. E.; Wallace, D. C.; McQueen, T. M.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [Arpino, K. E.; Wallace, D. C.; Koohpayeh, S. M.; Wen, J-J; McQueen, T. M.] Johns Hopkins Univ, Inst Quantum Matter, Dept Phys & Astron, Baltimore, MD 21218 USA. [Nie, Y. F.; King, P. D. C.; Chatterjee, S.; Uchida, M.; Shen, K. M.] Cornell Univ, Dept Phys, Lab Atom & Solid State Phys, Ithaca, NY 14853 USA. [Nie, Y. F.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Birol, T.; Fennie, C. J.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [King, P. D. C.; Shen, K. M.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. [Page, K.] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Arpino, KE (reprint author), Johns Hopkins Univ, Dept Chem, Charles & 34Th St, Baltimore, MD 21218 USA. EM mcqueen@jhu.edu RI King, Philip/D-3809-2014; Uchida, Masaki/D-3710-2012; Nie, Yuefeng/L-8071-2013; Birol, Turan/D-1948-2012; Page, Katharine/C-9726-2009; Uchida, Masaki/I-1660-2014; Wen, Jiajia/C-5370-2013 OI King, Philip/0000-0002-6523-9034; Uchida, Masaki/0000-0002-0735-8844; Nie, Yuefeng/0000-0002-3449-5393; Birol, Turan/0000-0001-5174-3320; Page, Katharine/0000-0002-9071-3383; Uchida, Masaki/0000-0002-0735-8844; Wen, Jiajia/0000-0002-1651-3578 FU Johns Hopkins University; David and Lucile Packard Foundation; NSF Materials Research Science and Engineering Centers (MRSEC) program Grant [DMR-1120296]; AFOSR [FA9550-11-1-0033, FA9550-12-1-0335]; NSF CAREER Grant [DMR-0847385]; Energy Materials Center at Cornell (EMC2), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001086]; Cornell Center for Materials Research; NSF MRSEC program [DMR-1120296]; DOE, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering (The Institute for Quantum Matter) [DE-FG02-08ER46544]; U.S. DOE Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396]; National Science Foundation Major Research Instrumentation Program [DMR-0821005] FX T. M. M. acknowledges support of startup funds from the Johns Hopkins University as well as the David and Lucile Packard Foundation. K. M. S. acknowledges the NSF Materials Research Science and Engineering Centers (MRSEC) program Grant No. DMR-1120296, AFOSR Grants No. FA9550-11-1-0033 and No. FA9550-12-1-0335, and the NSF CAREER Grant No. DMR-0847385. T. B. was supported as part of the Energy Materials Center at Cornell (EMC2), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001086. C. J. F. was supported by the Cornell Center for Materials Research with funding from the NSF MRSEC program (DMR-1120296). Crystal growth supported by DOE, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering (The Institute for Quantum Matter, Award No. DE-FG02-08ER46544). This work has benefited from the use of the NPDF beam line at the Lujan Center at Los Alamos Neutron Science Center, funded by the U.S. DOE Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. The dilution refrigerator used in this study was funded through the National Science Foundation Major Research Instrumentation Program, Grant No. DMR-0821005. K. E. A., D. C. W., and Y. F. N. contributed equally to this work. NR 28 TC 12 Z9 12 U1 1 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 8 PY 2014 VL 112 IS 1 AR 017002 DI 10.1103/PhysRevLett.112.017002 PG 5 WC Physics, Multidisciplinary SC Physics GA AB6ZK UT WOS:000331938800008 PM 24483920 ER PT J AU Stasto, AM Xiao, BW Zaslavsky, D AF Stasto, Anna M. Xiao, Bo-Wen Zaslavsky, David TI Towards the Test of Saturation Physics Beyond Leading Logarithm SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLOR GLASS CONDENSATE; NONLINEAR GLUON EVOLUTION; HADRON-PRODUCTION; PB COLLISIONS; LHC; REGION AB We present results from the first next-to-leading-order (NLO) numerical analysis of forward hadron production in pA and dA collisions in the small-x saturation formalism. Using parton distributions and fragmentation functions at NLO, as well as the dipole amplitude from the solution to the Balitsky-Kovchegov equation with running coupling, together with the NLO corrections to the hard coefficients, we obtain a good description of the available RHIC data in dAu collisions. In the large p(perpendicular to) region beyond the saturation scale, we find that the NLO correction becomes dominant and negative, which indicates that other physics beyond NLO becomes important and should also be taken into account. Furthermore, we make predictions for forward hadron production in pPb collisions at the LHC. This analysis not only incorporates the important NLO corrections for all partonic channels, but also reduces the renormalization scale dependence and helps to significantly reduce the theoretical uncertainties. It therefore provides a precise test of saturation physics beyond the leading logarithmic approximation. C1 [Stasto, Anna M.; Zaslavsky, David] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Stasto, Anna M.] Brookhaven Natl Lab, RIKEN Ctr, Upton, NY 11973 USA. [Stasto, Anna M.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Xiao, Bo-Wen] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Xiao, Bo-Wen] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. RP Stasto, AM (reprint author), Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA. EM astasto@phys.psu.edu OI Zaslavsky, David/0000-0002-6404-2205 FU DOE OJI Grant [DE-SC0002145]; Polish NCN [DEC-2011/01/B/ST2/03915]; Sloan Foundation FX We thank C. Marquet, A. Mueller, S. Munier, B. Pire, L. Szymanowski, and F. Yuan for their stimulating comments. This work was supported in part by the DOE OJI Grant No. DE-SC0002145 and by the Polish NCN Grant No. DEC-2011/01/B/ST2/03915. A. M. S. is supported by the Sloan Foundation. NR 43 TC 22 Z9 22 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 8 PY 2014 VL 112 IS 1 AR 012302 DI 10.1103/PhysRevLett.112.012302 PG 5 WC Physics, Multidisciplinary SC Physics GA AB6ZK UT WOS:000331938800002 PM 24483891 ER PT J AU Zahran, EM Bedford, NM Nguyen, MA Chang, YJ Guiton, BS Naik, RR Bachas, LG Knecht, MR AF Zahran, Elsayed M. Bedford, Nicholas M. Nguyen, Michelle A. Chang, Yao-Jen Guiton, Beth S. Naik, Rajesh R. Bachas, Leonidas G. Knecht, Marc R. TI Light-Activated Tandem Catalysis Driven by Multicomponent Nanomaterials SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PD/FE BIMETALLIC NANOTUBES; PHOTOCATALYTIC ACTIVITY; TITANIUM-DIOXIDE; VISIBLE-LIGHT; WATER; MECHANISM; HYDROGEN; DECHLORINATION; DEGRADATION; TEMPERATURE AB Transitioning energy-intensive and environmentally intensive processes toward sustainable conditions is necessary in light of the current global condition. To this end, photocatalytic processes represent new approaches for H-2 generation; however, their application toward tandem catalytic reactivity remains challenging. Here, we demonstrate that metal oxide materials decorated with noble metal nanoparticles advance visible light photocatalytic activity toward new reactions not typically driven by light. For this, Pd nanoparticles were deposited onto Cu2O cubes to generate a composite structure. Once characterized, their hydrodehalogenation activity was studied via the reductive dechlorination of polychlorinated biphenyls. To this end, tandem catalytic reactivity was observed with H-2 generation via H2O reduction at the Cu2O surface, followed by dehalogenation at the Pd using the in situ generated H-2. Such results present methods to achieve sustainable catalytic technologies by advancing photocatalytic approaches toward new reaction systems. C1 [Zahran, Elsayed M.; Bedford, Nicholas M.; Nguyen, Michelle A.; Bachas, Leonidas G.; Knecht, Marc R.] Univ Miami, Dept Chem, Coral Gables, FL 33146 USA. [Bedford, Nicholas M.; Naik, Rajesh R.] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. [Chang, Yao-Jen; Guiton, Beth S.] Univ Kentucky, Dept Chem, Lexington, KY 40506 USA. [Guiton, Beth S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Bachas, LG (reprint author), Univ Miami, Dept Chem, Coral Gables, FL 33146 USA. EM bachas@miami.edu; knecht@miami.edu RI Bachas, Leonidas/G-2479-2015; Chang, Yao-Jen/E-6766-2017; OI Bachas, Leonidas/0000-0002-3308-6264; Zahran, Elsayed/0000-0003-3456-515X FU University of Miami; Air Force Office of Scientific Research; Office of Basic Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy; NASA Kentucky EPSCoR; National Research Council FX This work was supported by University of Miami (L.G.B. and M.R.K.), the Air Force Office of Scientific Research (R.R.N.), the Office of Basic Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy (B.S.G), and the NASA Kentucky EPSCoR Program (Y.-J.C. and B.S.G.). E.M.Z. acknowledges the National Research Center, Egypt, for granting an academic leave, N.M.B acknowledges fellowship support from the National Research Council Research Associateship award, and M.A.N. acknowledges a fellowship from the Science Made Sensible program at University of Miami. NR 26 TC 21 Z9 21 U1 10 U2 141 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 32 EP 35 DI 10.1021/ja410465s PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600009 PM 24397770 ER PT J AU Li, Z Assary, RS Atesin, AC Curtiss, LA Marks, TJ AF Li, Zhi Assary, Rajeev S. Atesin, Abdurrahman C. Curtiss, Larry A. Marks, Tobin J. TI Rapid Ether and Alcohol C-O Bond Hydrogenolysis Catalyzed by Tandem High-Valent Metal Triflate plus Supported Pd Catalysts SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HIGH-QUALITY DIESEL; AQUEOUS-PHASE HYDRODEOXYGENATION; IONIC LIQUIDS; ORGANIC-SYNTHESIS; BIOMASS; CONVERSION; ALKANES; CHEMICALS; CELLULOSE; ACID AB The thermodynamically leveraged conversion of ethers and alcohols to saturated hydrocarbons is achieved efficiently with low loadings of homogeneous M(OTf)(n) + heterogeneous Pd tandem catalysts (M = transition metal; OTf = triflate; n = 4). For example, Hf(OTf)(4) mediates rapid endothermic ether reversible arrow alcohol and alcohol reversible arrow alkene equilibria, while Pd/C catalyzes the subsequent, exothermic alkene hydrogenation. The relative C-O cleavage rates scale as 30 degrees > 20 degrees > 1 degrees. The reaction scope extends to efficient conversion of biomass-derived ethers, such as THF derivatives, to the corresponding alkanes. C1 [Li, Zhi; Atesin, Abdurrahman C.; Marks, Tobin J.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Curtiss, Larry A.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Marks, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM t-marks@northwestern.edu RI Surendran Assary, Rajeev/E-6833-2012; Li, Zhi/D-8662-2011 OI Surendran Assary, Rajeev/0000-0002-9571-3307; Li, Zhi/0000-0003-2770-6364 FU U.S. Department of Energy [DE-AC0206CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; NSF [CHE-1213235]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy under contract DE-AC0206CH11357. This material is based upon work supported as part of the Institute of Atom Efficient Chemical Transformation (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NSF grant CHE-1213235 on basic f-element chemistry supported Z.L. and provided reactor equipment. We gratefully acknowledge the computing resources provided on "Fusion", a 320-node computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 52 TC 31 Z9 31 U1 10 U2 159 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 104 EP 107 DI 10.1021/ja411546r PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600027 PM 24354599 ER PT J AU Garimella, PD Meldrum, T Witus, LS Smith, M Bajaj, VS Wemmer, DE Francis, MB Pines, A AF Garimella, Praveena D. Meldrum, Tyler Witus, Leah S. Smith, Monica Bajaj, Vikram S. Wemmer, David E. Francis, Matthew B. Pines, Alexander TI Hyperpolarized Xenon-Based Molecular Sensors for Label-Free Detection of analytes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NUCLEAR-MAGNETIC-RESONANCE; FUNCTIONALIZED XENON; PEPTIDE LIBRARY; BETA-HAIRPIN; BIOSENSOR; SEQUENCES; XE-129; MRI AB Nuclear magnetic resonance (NMR) can reveal the chemical constituents of a complex mixture without resorting to chemical modification, separation, or other perturbation. Recently, we and others have developed magnetic resonance agents that report on the presence of dilute analytes by proportionately altering the response of a more abundant or easily detected species, a form of amplification. One example of such a sensing medium is xenon gas, which is chemically inert and can be optically hyperpolarized, a process that enhances its NMR signal by up to 5 orders of magnitude. Here, we use a combinatorial synthetic approach to produce xenon magnetic resonance sensors that respond to small molecule analytes. The sensor responds to the ligand by producing a small chemical shift change in the Xe NMR spectrum. We demonstrate this technique for the dye, Rhodamine 6G, for which we have an independent optical assay to verify binding. We thus demonstrate that specific binding of a small molecule can produce a xenon chemical shift change, suggesting a general approach to the production of xenon sensors targeted to small molecule analytes for in vitro assays or molecular imaging in vivo. C1 [Garimella, Praveena D.; Meldrum, Tyler; Witus, Leah S.; Bajaj, Vikram S.; Wemmer, David E.; Francis, Matthew B.; Pines, Alexander] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Garimella, Praveena D.; Meldrum, Tyler; Witus, Leah S.; Smith, Monica; Bajaj, Vikram S.; Wemmer, David E.; Francis, Matthew B.; Pines, Alexander] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Smith, Monica; Wemmer, David E.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Garimella, Praveena D.; Meldrum, Tyler; Witus, Leah S.; Bajaj, Vikram S.; Francis, Matthew B.; Pines, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Smith, Monica; Wemmer, David E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Bajaj, VS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM vikbajaj@gmail.com; francis@cchem.berkeley.edu RI Meldrum, Tyler/P-7420-2015 OI Meldrum, Tyler/0000-0002-5954-0795 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 38 TC 11 Z9 11 U1 1 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 164 EP 168 DI 10.1021/ja406760r PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600037 PM 24313335 ER PT J AU Marquardt, D Williams, JA Kinnun, JJ Kucerka, N Atkinson, J Wassall, SR Katsaras, J Harroun, TA AF Marquardt, Drew Williams, Justin A. Kinnun, Jacob J. Kucerka, Norbert Atkinson, Jeffrey Wassall, Stephen R. Katsaras, John Harroun, Thad A. TI Dimyristoyl Phosphatidylcholine: A Remarkable Exception to alpha-Tocopherol's Membrane Presence SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID POLYUNSATURATED LIPID-MEMBRANE; PHOSPHOLIPID MODEL MEMBRANES; VITAMIN-E; MAGNETIC-RESONANCE; MOLECULAR-MECHANISM; HYDROCARBON CHAINS; FATTY-ACID; DYNAMICS; ANTIOXIDANT; VESICLES AB Using data obtained from different physical techniques (i.e., neutron diffraction, NMR and UV spectroscopy), we present evidence which explains some of the conflicting and inexplicable data found in the literature regarding alpha-tocopherol's (aToc's) behavior in dimyristoyl phosphatidylcholine (di-14:0PC) bilayers. Without exception, the data point to aToc's active chromanol moiety residing deep in the hydrophobic core of di-14:0PC bilayers, a location that is in stark contrast to aToc's location in other PC bilayers. Our result is a clear example of the importance of lipid species diversity in biological membranes and importantly, it suggests that measurements of aToc's oxidation kinetics, and its associated byproducts observed in di-14:0PC bilayers, should be reexamined, this time taking into account its noncanonical location in this bilayer. C1 [Marquardt, Drew; Katsaras, John; Harroun, Thad A.] Brock Univ, Dept Phys, St Catharines, ON L2S 3A1, Canada. [Williams, Justin A.; Kinnun, Jacob J.; Wassall, Stephen R.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46202 USA. [Kucerka, Norbert] Canadian Neutron Beam Ctr, Natl Res Council, Chalk River, ON K0J 1J0, Canada. [Atkinson, Jeffrey] Brock Univ, Dept Chem, St Catharines, ON L2S 3A1, Canada. [Katsaras, John] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Katsaras, John] Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Katsaras, John] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. RP Marquardt, D (reprint author), Brock Univ, Dept Phys, St Catharines, ON L2S 3A1, Canada. OI Harroun, Thad/0000-0001-9816-2590; Marquardt, Drew/0000-0001-6848-2497 FU NSERC Vanier Canada Graduate Scholarship; National Science and Engineering Research Council of Canada (NSERC); Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); U.S. Department of Energy (DOE) [DE-AC05-00OR2275]; Scientific User Facilities Division of the Office of Basic Energy Sciences (BES) FX We acknowledge the Canadian Neutron Beam Centre (CNBC, Chalk River, ON) for providing generous amounts of neutron beamtime. D.M. is supported by a NSERC Vanier Canada Graduate Scholarship. T.A.H. and J.A. are partially supported by the National Science and Engineering Research Council of Canada (NSERC). J.K. is partially supported from the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) under contract no. DE-AC05-00OR2275. Support for J.K. from the Scientific User Facilities Division of the Office of Basic Energy Sciences (BES) is also acknowledged. NR 52 TC 16 Z9 16 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 203 EP 210 DI 10.1021/ja408288f PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600042 PM 24308426 ER PT J AU Knott, BC Momeni, MH Crowley, MF Mackenzie, LF Gotz, AW Sandgren, M Withers, SG Stahlberg, J Beckham, GT AF Knott, Brandon C. Momeni, Majid Haddad Crowley, Michael F. Mackenzie, Lloyd F. Goetz, Andreas W. Sandgren, Mats Withers, Stephen G. Stahlberg, Jerry Beckham, Gregg T. TI The Mechanism of Cellulose Hydrolysis by a Two-Step, Retaining Cellobiohydrolase Elucidated by Structural and Transition Path Sampling Studies SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PHANEROCHAETE-CHRYSOSPORIUM CEL7D; TRICHODERMA-REESEI; CRYSTAL-STRUCTURE; ENDOGLUCANASE I; CATALYTIC MECHANISM; ANGSTROM RESOLUTION; FUSARIUM-OXYSPORUM; REACTION COORDINATE; PROVIDES INSIGHT; COMPLEX AB Glycoside hydrolases (GHs) cleave glycosidic linkages in carbohydrates, typically via inverting or retaining mechanisms, the latter of which proceeds via a two-step mechanism that includes formation of a glycosyl-enzyme intermediate. We present two new structures of the catalytic domain of Hypocrea jecorina GH Family 7 cellobiohydrolase Cel7A, namely a Michaelis complex with a full cellononaose ligand and a glycosyl-enzyme intermediate, that reveal details of the 'static' reaction coordinate. We also employ transition path sampling to determine the 'dynamic' reaction coordinate for the catalytic cycle. The glycosylation reaction coordinate contains components of forming and breaking bonds and a conformational change in the nucleophile. Deglycosylation proceeds via a product-assisted mechanism wherein the glycosylation product, cellobiose, positions a water molecule for nucleophilic attack on the anomeric carbon of the glycosyl-enzyme intermediate. In concert with previous structures, the present results reveal the complete hydrolytic reaction coordinate for this naturally and industrially important enzyme family. C1 [Knott, Brandon C.; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Crowley, Michael F.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Momeni, Majid Haddad; Sandgren, Mats; Stahlberg, Jerry] Swedish Univ Agr Sci, Dept Mol Biol, SE-75007 Uppsala, Sweden. [Mackenzie, Lloyd F.; Withers, Stephen G.] Univ British Columbia, Dept Chem, Vancouver, BC V6T 1Z1, Canada. [Goetz, Andreas W.] Univ Calif San Diego, San Diego Supercomp Ctr, La Jolla, CA 92093 USA. RP Stahlberg, J (reprint author), Swedish Univ Agr Sci, Dept Mol Biol, SE-75007 Uppsala, Sweden. EM Jerry.Stahlberg@slu.se; Gregg.Beckham@nrel.gov RI Stahlberg, Jerry/D-4163-2013 OI Stahlberg, Jerry/0000-0003-4059-8580 FU NREL; Department of Energy BioEnergy Technologies Office; NREL Laboratory Directed Research and Development funds; US Department of Energy SciDAC program; European Commission [DG-12 (BIO4-CT96-0580)]; Swedish Foundation for Strategic Research; Swedish Structural Biology Network (SBNet); Swedish Natural Science Research Council (NFR); Swedish Council for Forestry and Agricultural Research (SJFR); Bo Rydin's Foundation for Scientific Research; Faculty for Natural Resources and Agriculture at the Swedish University of Agricultural Sciences; Natural Sciences and Engineering Research Council of Canada (NSERC) FX B.C.K. and G.T.B. thank the NREL Director's Fellowship Program for funding. G.T.B. also acknowledges funding from the Department of Energy BioEnergy Technologies Office and NREL Laboratory Directed Research and Development funds. M.F.C. and A.W.G. acknowledge the US Department of Energy SciDAC program for funding. J.S., M.S., and M.H.M. acknowledge financial support from the European Commission DG-12 (BIO4-CT96-0580), Swedish Foundation for Strategic Research, Swedish Structural Biology Network (SBNet), Swedish Natural Science Research Council (NFR), Swedish Council for Forestry and Agricultural Research (SJFR), Bo Rydin's Foundation for Scientific Research, and the Faculty for Natural Resources and Agriculture at the Swedish University of Agricultural Sciences through the research program 'Micro-DrivE' S.G.W. and L.M. thank the Natural Sciences and Engineering Research Council of Canada (NSERC) for financial support. Computer time was provided by the Kraken cluster at the National Institute of Computational Sciences through the XSEDE allocation MCB09159. The authors thank Heather B. Mayes for assistance with figures, Prof. Jurgen Puls for providing the insoluble cellooligosaccharides, and Maria Bostrom, Sabah Mahdi, Dr. Mark Harris, Dr. Christina Divne, and Prof. T. Alwyn Jones for help in association with protein crystallization and structure determination. The authors are also grateful to Prof. John Brady and Dr. Udo Schnupf for sharing preliminary results from an independent study of HjeCel7A. NR 49 TC 49 Z9 50 U1 9 U2 84 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 321 EP 329 DI 10.1021/ja410291u PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600055 PM 24341799 ER PT J AU Chen, WY Hartwig, JF AF Chen, Wenyong Hartwig, John F. TI Cation Control of Diastereoselectivity in Iridium-Catalyzed Allylic Substitutions. Formation of Enantioenriched Tertiary Alcohols and Thioethers by Allylation of 5H-Oxazol-4-ones and 5H-Thiazol-4-ones SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ACID-DERIVATIVES; MICHAEL ADDITION; ENANTIOSELECTIVE SYNTHESIS; QUATERNARY STEREOCENTERS; 1,4-ADDITION REACTION; ASYMMETRIC-SYNTHESIS; ALKYLATION REACTION; N-ALLYLATION; VINYLATION; COMPLEXES AB We report highly diastereo- and enantioselective allylations of substituted 5H-oxazol-4-ones and 5H-thiazol-4-ones catalyzed by a metallacyclic iridium complex. Enantioselective Ir-catalyzed allylation of substituted 5H-oxazol-4-ones occurs with high diastereoselectivity by employing the corresponding zinc enolates; enantioselective Ir-catalyzed allylation of substituted 5H-thiazol-4-ones occurs with the corresponding magnesium enolates with high diastereoselectivity. The allylation of substituted 5H-oxazol-4-ones provides rapid access to enantioenriched tertiary alpha-hydroxy acid derivatives unavailable through Mo-catalyzed allylic substitution. The allylation of substituted 5H-thiazol-4-ones provides a novel method to synthesize enantioenriched tertiary thiols and thioethers. The observed cation effect implies a novel method to control the diastereoselectivity in Ir-catalyzed allylic substitution. C1 [Hartwig, John F.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Hartwig, JF (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jhartwig@berkeley.edu RI chen, wy/E-3832-2014 FU NIH [GM-58108]; Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the NIH (GM-58108) for work on methods development, the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 for support of our studies on effects of the outer coordination sphere, Johnson-Matthey for gifts of [Ir(cod)Cl]2, and Dr. Klaus Ditrich and BASF for a generous gift of chiral amines. NR 56 TC 52 Z9 52 U1 6 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 377 EP 382 DI 10.1021/ja410650e PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600061 PM 24295427 ER PT J AU Lu, XJ Yang, WG Quan, ZW Lin, TQ Bai, LG Wang, L Huang, FQ Zhao, YS AF Lu, Xujie Yang, Wenge Quan, Zewei Lin, Tianquan Bai, Ligang Wang, Lin Huang, Fuqiang Zhao, Yusheng TI Enhanced Electron Transport in Nb-Doped TiO2 Nanoparticles via Pressure-Induced Phase Transitions SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SENSITIZED SOLAR-CELLS; ANATASE TIO2; INDUCED AMORPHIZATION; HIERARCHICAL SPHERES; LITHIUM STORAGE; 001 FACETS; RUTILE; FILMS; PHOTOCATALYSIS; EFFICIENCY AB Anatase TiO2 is one of the most important energy materials but suffers from poor electrical conductivity. Nb doping has been considered as an effective way to improve its performance in the applications of photocatalysis, solar cells, Li batteries, and transparent conducting oxide films. Here, we report the further enhancement of electron transport in Nb-doped TiO2 nanoparticles via pressure-induced phase transitions. The phase transition behavior and influence of Nb doping in anatase Nb-TiO2 have been systematically investigated by in situ synchrotron X-ray diffraction and Raman spectroscopy. The bulk moduli are determined to be 179.5, 163.3, 148.3, and 139.0 GPa for 0, 2.5, 5.0, and 10.0 mol % Nb-doped TiO2, respectively. The Nb-concentration-dependent stiffness variation has been demonstrated: samples with higher Nb concentrations have lower stiffness. In situ resistance measurements reveal an increase of 40% in conductivity of quenched Nb-TiO2 in comparison to the pristine anatase phase. The pressure-induced conductivity evolution is discussed in detail in terms of the packing factor model, which provides direct evidence for the rationality of the correlation of packing factors with electron transport in semiconductors. Pressure-treated Nb-doped TiO2 with unique properties surpassing those in the anatase phase holds great promise for energy-related applications. C1 [Lu, Xujie; Bai, Ligang; Zhao, Yusheng] Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. [Lu, Xujie; Yang, Wenge; Wang, Lin] Carnegie Inst Sci, Geophys Lab, High Pressure Synerget Consortium, Argonne, IL 60439 USA. [Yang, Wenge; Wang, Lin] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Quan, Zewei] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Lin, Tianquan; Huang, Fuqiang] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China. RP Lu, XJ (reprint author), Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. EM xujie@aps.anl.gov; wyang@ciw.edu; yusheng.zhao@unlv.edu RI WANG, LIN/G-7884-2012; Quan, Zewei/G-4759-2011; Bai, Ligang/E-9371-2015; Lu, Xujie/L-9672-2014; Lin, Tianquan/I-3030-2012 OI Lu, Xujie/0000-0001-8402-7160; FU EFree, an Energy Frontier Research Center; DOE-BES [DE-SC0001057, DE-FG02-99ER45775]; DOE-NNSA [DE-NA0001974]; NSF; NSF of China [51125006, 91122034]; [DE-NA0001982]; [EAR-1128799]; [DE-FG02-94ER14466] FX The UNLV High Pressure Science and Engineering Center (HiPSEC) is a DOE-NNSA Center of Excellence supported by Cooperative Agreement DE-NA0001982. HPSynC is supported by the EFree, an Energy Frontier Research Center funded by the DOE-BES under Grant DE-SC0001057. HPCAT operations are supported by the DOE-NNSA under Award DE-NA0001974 and DOE-BES under Award DE-FG02-99ER45775, with partial instrumentation funding by the NSF. The gas loading was performed at GeoSoilEnviroCARS, APS, ANL, supported by EAR-1128799 and DE-FG02-94ER14466. The samples synthesis was conducted at Shanghai Institute of Ceramics, Chinese Academy of Sciences, supported by NSF of China Grant No. 51125006 and 91122034. The authors thank H. K Mao, Y. Ding, M. Baldini, J. Y. Wang, K. Li, R. Ferry, G. Y. Shen, Y. Meng, C. Park, J. Smith, S. Sinogeikin, E. Rod, Q S. Zeng, B. Lavina, and S. Tkachev for their valuable suggestions and technical support. NR 45 TC 44 Z9 46 U1 22 U2 203 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 8 PY 2014 VL 136 IS 1 BP 419 EP 426 DI 10.1021/ja410810w PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 288BI UT WOS:000329586600066 PM 24320708 ER PT J AU Donaldson, TM Ting, LM Zhan, CY Shi, WX Zheng, RJ Almo, SC Kim, K AF Donaldson, Teraya M. Ting, Li-Min Zhan, Chenyang Shi, Wuxian Zheng, Renjian Almo, Steven C. Kim, Kami TI Structural Determinants of the 5 '-Methylthioinosine Specificity of Plasmodium Purine Nucleoside Phosphorylase SO PLOS ONE LA English DT Article ID TRANSITION-STATE ANALOG; TRICHOMONAS-VAGINALIS; TOXOPLASMA-GONDII; IMMUCILLIN-H; FALCIPARUM; INHIBITORS; PATHWAY AB Plasmodium parasites rely upon purine salvage for survival. Plasmodium purine nucleoside phosphorylase is part of the streamlined Plasmodium purine salvage pathway that leads to the phosphorylysis of both purines and 5 '-methylthiopurines, byproducts of polyamine synthesis. We have explored structural features in Plasmodium falciparum purine nucleoside phosphorylase ( PfPNP) that affect efficiency of catalysis as well as those that make it suitable for dual specificity. We used site directed mutagenesis to identify residues critical for PfPNP catalytic activity as well as critical residues within a hydrophobic pocket required for accommodation of the 5 '-methylthio group. Kinetic analysis data shows that several mutants had disrupted binding of the 5 '-methylthio group while retaining activity for inosine. A triple PfPNP mutant that mimics Toxoplasma gondii PNP had significant loss of 5 '-methylthio activity with retention of inosine activity. Crystallographic investigation of the triple mutant PfPNP with Tyr160Phe, Val66Ile, andVal73Ile in complex with the transition state inhibitor immucillin H reveals fewer hydrogen bond interactions for the inhibitor in the hydrophobic pocket. C1 [Donaldson, Teraya M.; Ting, Li-Min; Kim, Kami] Albert Einstein Coll Med, Dept Med, Bronx, NY 10467 USA. [Donaldson, Teraya M.; Ting, Li-Min; Kim, Kami] Albert Einstein Coll Med, Dept Pathol, Bronx, NY 10467 USA. [Donaldson, Teraya M.; Ting, Li-Min; Kim, Kami] Albert Einstein Coll Med, Dept Microbiol & Immunol, Bronx, NY 10467 USA. [Zhan, Chenyang; Almo, Steven C.] Albert Einstein Coll Med, Dept Biochem, Bronx, NY 10467 USA. [Shi, Wuxian] Brookhaven Natl Lab, Natl Synchrotron Light Source, Brookhaven, NY USA. [Zheng, Renjian] Albert Einstein Coll Med, Dept Mol Pharmacol, Bronx, NY 10467 USA. RP Kim, K (reprint author), Albert Einstein Coll Med, Dept Med, Bronx, NY 10467 USA. EM kami.kim@einstein.yu.edu OI Zucker-Scharff, Thomas/0000-0002-1790-7405; Kim, Kami/0000-0003-3384-152X FU US Army Research [W81XWH-05-2-0025]; National Synchrotron Light Source comes principally from the Offices of Biological and Environmental Research; Basic Energy Sciences of the US Department of Energy; National Center for Research Resources of the National Institutes of Health; National Center for Research Resources at the National Institute of Health [RR-15301]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02_06CH11357] FX Part of this work was supported by US Army Research Grant W81XWH-05-2-0025 (to K. K.). Financial support of beamline X29A of the National Synchrotron Light Source comes principally from the Offices of Biological and Environmental Research and of Basic Energy Sciences of the US Department of Energy and from the National Center for Research Resources of the National Institutes of Health. The Northeastern Collaborative Access Team beamlines of the Advanced Photon Source are supported by award RR-15301 from the National Center for Research Resources at the National Institute of Health. Use of the Advanced Photon Source is supported by the US Department of Energy, Office of Basic Energy Sciences, under contract number DE-AC02_06CH11357. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 38 TC 2 Z9 2 U1 0 U2 2 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 8 PY 2014 VL 9 IS 1 AR e84384 DI 10.1371/journal.pone.0084384 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291WL UT WOS:000329862500121 PM 24416224 ER PT J AU Fagen, JR Leonard, MT McCullough, CM Edirisinghe, JN Henry, CS Davis, MJ Triplett, EW AF Fagen, Jennie R. Leonard, Michael T. McCullough, Connor M. Edirisinghe, Janaka N. Henry, Christopher S. Davis, Michael J. Triplett, Eric W. TI Comparative Genomics of Cultured and Uncultured Strains Suggests Genes Essential for Free-Living Growth of Liberibacter SO PLOS ONE LA English DT Article ID ESCHERICHIA-COLI; CAULOBACTER-CRESCENTUS; SINORHIZOBIUM-MELILOTI; GREENING DISEASE; CELL-DIVISION; UPTAKE SYSTEM; LOW-PH; ASIATICUS; TRANSPORT; CITRUS AB The full genomes of two uncultured plant pathogenic Liberibacter, Ca. Liberibacter asiaticus and Ca. Liberibacter solanacearum, are publicly available. Recently, the larger genome of a closely related cultured strain, Liberibacter crescens BT-1, was described. To gain insights into our current inability to culture most Liberibacter, a comparative genomics analysis was done based on the RAST, KEGG, and manual annotations of these three organisms. In addition, pathogenicity genes were examined in all three bacteria. Key deficiencies were identified in Ca. L. asiaticus and Ca. L. solanacearum that might suggest why these organisms have not yet been cultured. Over 100 genes involved in amino acid and vitamin synthesis were annotated exclusively in L. crescens BT-1. However, none of these deficiencies are limiting in the rich media used to date. Other genes exclusive to L. crescens BT-1 include those involved in cell division, the stringent response regulatory pathway, and multiple two component regulatory systems. These results indicate that L. crescens is capable of growth under a much wider range of conditions than the uncultured Liberibacter strains. No outstanding differences were noted in pathogenicity-associated systems, suggesting that L. crescens BT-1 may be a plant pathogen on an as yet unidentified host. C1 [Fagen, Jennie R.; Leonard, Michael T.; McCullough, Connor M.; Triplett, Eric W.] Univ Florida, Inst Food & Agr Sci, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA. [Edirisinghe, Janaka N.; Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Davis, Michael J.] Univ Florida, Inst Food & Agr Sci, Dept Plant Pathol, Citrus Res & Dev Ctr, Lake Alfred, FL USA. RP Triplett, EW (reprint author), Univ Florida, Inst Food & Agr Sci, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA. EM ewt@ufl.edu FU Citrus Research and Development Foundation [336] FX This work was funded by the Citrus Research and Development Foundation grant number 336. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 61 TC 10 Z9 10 U1 0 U2 17 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 8 PY 2014 VL 9 IS 1 AR e84469 DI 10.1371/journal.pone.0084469 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291WL UT WOS:000329862500128 PM 24416233 ER PT J AU Boland, KS Hobart, DE Kozimor, SA MacInnes, MM Scott, BL AF Boland, Kevin S. Hobart, David E. Kozimor, Stosh A. MacInnes, Molly M. Scott, Brian L. TI The coordination chemistry of trivalent lanthanides (Ce, Nd, Sm, Eu, Gd, Dy, Yb) with diphenyldithiophosphinate anions SO POLYHEDRON LA English DT Article DE Lanthanide; Coordination chemistry; Dithiophosphinate; Extractant ID NUCLEAR-MAGNETIC-RESONANCE; MINOR ACTINIDE EXTRACTION; DITHIOPHOSPHINATE-COMPLEXES; SELECTIVE EXTRACTION; CRYSTAL-STRUCTURES; MOLECULAR-STRUCTURES; ELECTRONIC-STRUCTURE; SEPARATION; ACIDS; SPECTROSCOPY AB Understanding the coordination chemistry between lanthanide elements and dithiophosphinate ligands is important given prospects for using dithiophosphinate ligands to separate trivalent minor actinides from lanthanides in advanced nuclear fuel cycles. Reported here is the coordination chemistry of a series of lanthanide elements (Ce, Nd, Sm, Eu, Gd, Dy, and Yb) with diphenyldithiophosphinate anions, S2PPh21- In all cases, LnCl(3) was reacted with 4 equivalents of S2PPh21-. The large lanthanides (Ce3+, Nd3+, Sm3+, Eu3+) formed eight coordinate anions of the general formula Ln(S2PPh2)(4)(1-) and were characterized by H-1 and P-31 NMR, IR, UV-Vis, elemental analysis, and single crystal X-ray crystallography. For the slightly smaller Gd3+ and Dy3+ ions, a break in reactivity was observed. Here, analyses of reaction solutions by H-1 and P-31 NMR spectroscopy suggested that a complicated mixture formed from which single crystals of eight coordinate and neutral Gd(S2PPh2)(3)(NCMe)(2) and Dy(S2PPh2)(3)(NCMe)(2) complexes were isolated. Reactions involving even smaller Yb3+ ions provided similar results to Gd3+ and Dy3+, in that reaction solutions also contained a mixture of products. In the Yb3+ case a new heteroleptic species [Ph4P][Yb(S2PPh2)(3)Cl], was isolated in single crystal form. The structural data have been presented in comparison to that of [Ph4P][Sm(S2PMe2)(4)] and [Ph4P][Eu(S2PMe2)(4)], which were also structurally characterized for the first time. Overall, these results demonstrate how subtle differences in lanthanide ionic radii can drastically affect the coordination number, ligand stoichiometry, and charge on the resulting diphenyldithiophosphinate complex. Published by Elsevier Ltd. C1 [Boland, Kevin S.; Hobart, David E.; Kozimor, Stosh A.; MacInnes, Molly M.; Scott, Brian L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Kozimor, SA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM stosh@lanl.gov RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (Heavy Element Chemistry Program); US Department of Energy, Office of Nuclear Energy (Fuel Cycle RD Program); Heavy Element Chemistry Program at LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; DOE Science Undergraduate Laboratory Internship (Maclnnes); National Nuclear Security Administration of US Department of Energy [DE-AC52-06NA25396] FX The research involving 1-6 were supported by US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (Heavy Element Chemistry Program), the US Department of Energy, Office of Nuclear Energy (Fuel Cycle R&D Program). Studies focused on 7-9 were funded under the Heavy Element Chemistry Program at LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Additionally support was provided by the DOE Science Undergraduate Laboratory Internship (Maclnnes). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of US Department of Energy under contract DE-AC52-06NA25396. NR 73 TC 8 Z9 8 U1 1 U2 45 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD JAN 8 PY 2014 VL 67 BP 540 EP 548 DI 10.1016/j.poly.2013.09.019 PG 9 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA 287QL UT WOS:000329557200067 ER PT J AU Tian, H Yang, Y Xie, D Cui, YL Mi, WT Zhang, YG Ren, TL AF Tian, He Yang, Yi Xie, Dan Cui, Ya-Long Mi, Wen-Tian Zhang, Yuegang Ren, Tian-Ling TI Wafer-Scale Integration of Graphene-based Electronic, Optoelectronic and Electroacoustic Devices SO SCIENTIFIC REPORTS LA English DT Article ID SINGLE-LAYER GRAPHENE; MICRO-SUPERCAPACITORS; SCALABLE FABRICATION; MONOLAYER GRAPHENE; LARGE-AREA; FILMS; OXIDE; PHOTODETECTORS; TRANSPARENT; TRANSISTORS AB In virtue of its superior properties, the graphene-based device has enormous potential to be a supplement or an alternative to the conventional silicon-based device in varies applications. However, the functionality of the graphene devices is still limited due to the restriction of the high cost, the low efficiency and the low quality of the graphene growth and patterning techniques. We proposed a simple one-step laser scribing fabrication method to integrate wafer-scale high-performance graphene-based in-plane transistors, photodetectors, and loudspeakers. The in-plane graphene transistors have a large on/off ratio up to 5.34. And the graphene photodetector arrays were achieved with photo responsivity as high as 0.32 A/W. The graphene loudspeakers realize wide-band sound generation from 1 to 50 kHz. These results demonstrated that the laser scribed graphene could be used for wafer-scale integration of a variety of graphene-based electronic, optoelectronic and electroacoustic devices. C1 [Tian, He; Yang, Yi; Xie, Dan; Cui, Ya-Long; Mi, Wen-Tian; Ren, Tian-Ling] Tsinghua Univ, Inst Microelect, Beijing 100084, Peoples R China. [Tian, He; Yang, Yi; Cui, Ya-Long; Mi, Wen-Tian; Ren, Tian-Ling] Tsinghua Univ, TNList, Beijing 100084, Peoples R China. [Zhang, Yuegang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Zhang, Yuegang] Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Suzhou 215123, Peoples R China. RP Zhang, YG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM yzhang5@lbl.gov; RenTL@tsinghua.edu.cn RI Mi, Wentian/K-4112-2013; Tian, He/I-1299-2014; Zhang, Y/E-6600-2011 OI Mi, Wentian/0000-0001-5416-2716; Tian, He/0000-0001-7328-2182; Zhang, Y/0000-0003-0344-8399 FU National Natural Science Foundation of China [61025021, 60936002, 51072089, 61020106006]; National Key Project of Science and Technology [2011ZX02403-002]; Special Fund for Agro-scientific Research in the Public Interest [201303107]; Ministry of Education Scholarship of China FX This work was supported by the National Natural Science Foundation of China (61025021, 60936002, 51072089, and 61020106006), the National Key Project of Science and Technology (2011ZX02403-002) the Special Fund for Agro-scientific Research in the Public Interest (201303107). He Tian is additionally supported by the Ministry of Education Scholarship of China. Thanks for the valuable discussions with Prof. Z. Bao from Stanford University. NR 35 TC 23 Z9 23 U1 9 U2 105 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 8 PY 2014 VL 4 AR 3598 DI 10.1038/srep03598 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 291OU UT WOS:000329839000006 PM 24398542 ER PT J AU Delattre, B Bai, H Ritchie, RO De Coninck, J Tomsia, AP AF Delattre, Benjamin Bai, Hao Ritchie, Robert O. De Coninck, Joel Tomsia, Antoni P. TI Unidirectional Freezing of Ceramic Suspensions: In Situ X-ray Investigation of the Effects of Additives SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE freeze-casting; ice-templating; ice lens; unidirectional freezing; ice growth; freezing dynamics ID HYDROXYAPATITE SCAFFOLDS; PARTICLE REDISTRIBUTION; TOMOGRAPHY OBSERVATIONS; COLLOIDAL DISPERSIONS; POROUS CERAMICS; CRYSTAL-GROWTH; SOLIDIFICATION; BIOMATERIALS; RADIOGRAPHY AB Using in situ X-ray radiography, we investigated unidirectional freezing of titanium dioxide suspensions. We showed how processing additives, which are generally used for ice-templating, strongly modified freezing dynamics during the solidification process. We observed and identified different freezing regimes by varying the amount of dispersant, binder, or poly(ethylene glycol) (PEG). We demonstrated that because each regime corresponds to a given final structure understanding the particle motion and redistribution at the ice-front level was essential. We also examined the transition from a random particles-entrapment regime to a well-defined lamellar regime and proposed and discussed two mechanisms by which additives might affect the solidification process. C1 [Delattre, Benjamin; Bai, Hao; Ritchie, Robert O.; Tomsia, Antoni P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Delattre, Benjamin; De Coninck, Joel] Univ Mons, Lab Phys Surfaces & Interfaces, B-7000 Mons, Belgium. RP Delattre, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM bdelattre@lbl.gov RI Ritchie, Robert/A-8066-2008; Bai, Hao/J-5255-2012; Bai, Hao/D-1713-2017 OI Ritchie, Robert/0000-0002-0501-6998; Bai, Hao/0000-0002-1707-4976; Bai, Hao/0000-0002-3348-6129 FU Mechanical Behavior of Materials Program at Lawrence Berkeley National Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]; DOE's Office of Basic Energy Sciences FX This work was supported by the Mechanical Behavior of Materials Program at Lawrence Berkeley National Laboratory and by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under contract no. DE-AC02-05CH11231. We acknowledge support of the X-ray tomography beamline 8.3.2 at the Advanced Light Source (ALS) at Lawrence Berkeley National Laboratory, which is also supported by the DOE's Office of Basic Energy Sciences under the same contract number. NR 28 TC 8 Z9 8 U1 6 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 8 PY 2014 VL 6 IS 1 BP 159 EP 166 DI 10.1021/am403793x PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 288BG UT WOS:000329586300024 PM 24341868 ER PT J AU Maeng, S Kim, SW Lee, DH Moon, SE Kim, KC Maiti, A AF Maeng, Sunglyul Kim, Sang-Woo Lee, Deuk-Hee Moon, Seung-Eon Kim, Ki-Chul Maiti, Amitesh TI SnO2 Nanoslab as NO2 Sensor: Identification of the NO2 Sensing Mechanism on a SnO2 Surface SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE SnO2 nanoslab; NO2 sensor; gas sensing mechanism; flat band condition ID SEMICONDUCTOR GAS SENSORS; LOW-POWER CONSUMPTION; TIN OXIDE; NANOWIRE; CO; NANOSTRUCTURES; NANOCRYSTALS; TEMPERATURE; SENSITIVITY; FABRICATION AB Among the various metal oxides, SnO2 has been most widely exploited as a semiconductor gas sensor for its excellent functionalities. Models illustrating the sensing mechanism of SnO2 have been proposed and tested to explain experimentally derived "power laws". The models, however, are often based on somewhat simplistic assumptions; for instance, the net charge transfer from an adsorbate to a sensor surface site is assumed to occur only by integer values independent of the crystallographic planes. In this work, we use layer-shaped SnO2 crystallites with one nanodimension (1ND-crystallites) as NO2 gas sensing elements under flat band conditions, and derive appropriate "power laws" by combining the dynamics of gas molecules on the sensor surface with a depletion theory of semiconductor. Our experimentally measured sensor response as a function of NO2 concentration when compared with the theoretically derived power law indicates that sensing occurs primarily through the chemisorption of single NO2 molecules at oxygen vacancy sites on the sensor surface. C1 [Maeng, Sunglyul] Woosuk Univ, Dept Elect & Elect Engn, Wanju Gun 565701, Jeonbuk, South Korea. [Kim, Sang-Woo] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, SKKU Adv Inst Nanotechnol SAINT, Ctr Human Interface Nanotechnol HINT, Suwon 440746, South Korea. [Lee, Deuk-Hee] Korea Univ, Dept Elect Engn, Seoul 136701, South Korea. [Lee, Deuk-Hee] Korea Univ, Inst Nano Sci, Seoul 136701, South Korea. [Moon, Seung-Eon] Elect & Telecommun Res Inst, IT Convergence Technol Res Lab, Taejon 305700, South Korea. [Kim, Ki-Chul] Mokwon Univ, Dept Adv Chem Engn, Taejon 302729, South Korea. [Maiti, Amitesh] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Maeng, S (reprint author), Woosuk Univ, Dept Elect & Elect Engn, Wanju Gun 565701, Jeonbuk, South Korea. EM sunglyulm@gmail.com; kimsw1@skku.edu; maiti2@llnl.gov RI Kim, Sang-Woo/I-7769-2014; Kim, Ki-Chul/K-6312-2016 OI Kim, Sang-Woo/0000-0002-0079-5806; FU Program of Regional Innovation Center (Woosuk University); National Research Foundation of Korea (NRF) [2009-0083540]; Ministry of Science, ICT & Future Planning (MSIP); U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the Program of Regional Innovation Center (Woosuk University) which was conducted by the Ministry of Trade, Industry and Energy of the Korean Government. This work was also supported by the Basic Research Program (2009-0083540) of the National Research Foundation of Korea (NRF) grant funded by the Ministry of Science, ICT & Future Planning (MSIP). The work by one of the authors (AM.) was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 41 TC 31 Z9 31 U1 7 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 8 PY 2014 VL 6 IS 1 BP 357 EP 363 DI 10.1021/am404397f PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 288BG UT WOS:000329586300048 PM 24309131 ER PT J AU Fang, SM Brinkman, K Chen, FL AF Fang, Shumin Brinkman, Kyle Chen, Fanglin TI Unprecedented CO2-Promoted Hydrogen Permeation in Ni-BaZr0.1Ce0.7Y0.1Yb0.1O3-delta Membrane SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE hydrogen permeation; composite membrane; high temperature proton conductor; barium cerate; chemical stability ID BACEO3-BASED PROTON CONDUCTORS; CHEMICAL-STABILITY; FUEL-CELLS; CO2; PERFORMANCE; CATHODE; CERMET; BACE0.9Y0.1O3-DELTA; PERMEABILITY; ATMOSPHERES AB Conventional Ni-BaCeO3-based membranes possess high hydrogen permeation flux but suffer serious flux degradation in CO2-containing atmosphere because of the formation of BaCO3 insulating layer. In this work, we report a novel Ni-BaZr0.1Ce0.7Y0.1Yb0.1O3-delta (Ni-BZCYYb) membrane, capable of both high hydrogen permeation flux and stable performance in CO2-containing atmosphere at 900 degrees C. Most importantly, the flux is found to be promoted rather than being diminished by CO2 normally observed for other high temperature proton conductors. The flux enhancement in Ni-BZCYYb membrane is attributed to the increase of moisture content in feed gas. When CO2 is introduced, the reverse water-gas shift reaction takes place generating H2O and CO. This work demonstrates that CO2 can be beneficial rather than detrimental for hydrogen permeation membranes that possess high chemical stability. C1 [Fang, Shumin; Chen, Fanglin] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Brinkman, Kyle] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Chen, FL (reprint author), Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. EM chenfa@cec.sc.edu RI Fang, Shumin/I-3264-2012; Chen, Fanglin/K-1039-2012 OI Chen, Fanglin/0000-0001-9942-8872 FU HeteroFoaM Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DESC0001061]; DOE Office of Nuclear Energy's Nuclear Energy University Programs FX We gratefully acknowledge the financial support from the HeteroFoaM Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award DESC0001061 and the DOE Office of Nuclear Energy's Nuclear Energy University Programs. NR 42 TC 9 Z9 9 U1 2 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 8 PY 2014 VL 6 IS 1 BP 725 EP 730 DI 10.1021/am405169d PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 288BG UT WOS:000329586300096 PM 24328190 ER PT J AU Park, JY Salmeron, M AF Park, Jeong Young Salmeron, Miguel TI Fundamental Aspects of Energy Dissipation in Friction SO CHEMICAL REVIEWS LA English DT Review ID ATOMIC-FORCE MICROSCOPY; DEPENDENT SLIDING FRICTION; SELF-ASSEMBLED MONOLAYERS; TRANSMISSION ELECTRON-MICROSCOPE; QUARTZ-CRYSTAL MICROBALANCE; DECAGONAL QUASI-CRYSTALS; MOLECULARLY THIN-FILMS; STICK-SLIP MOTION; ADSORBATE VIBRATIONAL-RELAXATION; INTERFACIAL SHEAR-STRENGTH C1 [Park, Jeong Young] Inst for Basic Sci Korea, Ctr Nanomat & Chem React, Taejon 305701, South Korea. [Park, Jeong Young] Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea. [Salmeron, Miguel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Salmeron, Miguel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci & Engn Dept, Berkeley, CA 94720 USA. RP Park, JY (reprint author), Inst for Basic Sci Korea, Ctr Nanomat & Chem React, Taejon 305701, South Korea. EM jeongypark@kaist.ac.kr; mbsalmeron@lbl.gov RI Park, Jeong Young/A-2999-2008 FU Institute for Basic Science (IBS); National Research Foundation (NRF) [2012R1A2A1A01009249]; Ministry of Education, Science and Technology (MEST), Republic of Korea; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-AC02-05CH11231] FX J.Y.P. was supported by Institute for Basic Science (IBS) and 2012R1A2A1A01009249 through the National Research Foundation (NRF) funded by the Ministry of Education, Science and Technology (MEST), Republic of Korea. M.B.S. was supported by the "Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures" program, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 315 TC 25 Z9 25 U1 19 U2 132 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JAN 8 PY 2014 VL 114 IS 1 BP 677 EP 711 DI 10.1021/cr200431y PG 35 WC Chemistry, Multidisciplinary SC Chemistry GA 288BE UT WOS:000329586000015 PM 24050522 ER PT J AU Liu, XY Ruiz, E Afzal, W Ferro, V Palomar, J Prausnitz, JM AF Liu, Xiangyang Ruiz, Elia Afzal, Waheed Ferro, Victor Palomar, Jose Prausnitz, John M. TI High Solubilities for Methane, Ethane, Ethylene, and Propane in Trimethyloctylphosphonium Bis(2,4,4-trimethylpentyl) Phosphinate ([P8111][TMPP]) SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID COSMO-RS; HYDROCARBONS; SEPARATION AB Solubilities are reported for methane, ethane, ethylene, and propane in trimethyloctylphosphonium bis(2,4,4-trimethylpentyl) phosphinate [P8111] [TMPP] from 299 to 323 K up to 4 MPa. Consistent with prediction of COSMO-RS, [P8111] [TMPP] shows large solubilities for all four hydrocarbons. Contrary to solubility data in conventional ionic liquids, in [P8111] [TMPP] the solubility for ethane is higher than that for ethylene. When compared with solubilities in other similar phosphonium-based ionic liquids, the cation has only a small influence on the solubilities of small hydrocarbons. Ionic liquid [P8111][TMPP] may be useful for storage or separation of small hydrocarbons. C1 [Liu, Xiangyang; Ruiz, Elia; Afzal, Waheed; Prausnitz, John M.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Afzal, Waheed; Prausnitz, John M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Liu, Xiangyang] Xi An Jiao Tong Univ, MOE Key Lab Thermofluid Sci & Engn, Xian 710049, Shaanxi, Peoples R China. [Ruiz, Elia; Ferro, Victor; Palomar, Jose] Univ Autonoma Madrid, Dept Quim Fis Aplicada, Secc Ingn Quim, E-28049 Madrid, Spain. [Afzal, Waheed] Univ Punjab, Inst Chem Engn & Technol, Lahore 54590, Pakistan. RP Prausnitz, JM (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM prausnit@cchem.berkeley.edu RI Ferro, Victor/I-2462-2015; OI Ferro, Victor/0000-0002-2268-5595; Afzal, Waheed/0000-0002-2927-0114 FU Environmental Energy Technologies Division of the Lawrence Berkeley National Laboratory FX The authors are grateful to the Environmental Energy Technologies Division of the Lawrence Berkeley National Laboratory, for financial support and to Prof. Alexis Bell and co-workers for general assistance. NR 12 TC 9 Z9 11 U1 4 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JAN 8 PY 2014 VL 53 IS 1 BP 363 EP 368 DI 10.1021/ie402677t PG 6 WC Engineering, Chemical SC Engineering GA 288BF UT WOS:000329586100041 ER PT J AU Lei, HC Abeykoon, M Wang, KF Bozin, ES Ryu, H Graf, D Warren, JB Petrovic, C AF Lei, Hechang Abeykoon, Milinda Wang, Kefeng Bozin, Emil S. Ryu, Hyejin Graf, D. Warren, J. B. Petrovic, C. TI Physical properties of KxNi2-ySe2 single crystals SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID LAYERED SUPERCONDUCTOR; MAGNETIZATION AB We have synthesized K0.95(1)Ni1.86(2)Se2 single crystals. The single crystals contain K and Ni deficiencies not observed in KNi2Se2 polycrystals. Unlike KNi2Se2 polycrystals, the superconductivity is absent in single crystals. The detailed physical property study indicates that the K0.95Ni1.86Se2 single crystals exhibit heavy-fermion-like characteristics. The transition to a heavy fermion state below T similar to 30 K results in an enhancement of the electron-like carrier density whereas the magnetic susceptibility shows little anisotropy and suggests the presence of both itinerant and localized Ni orbitals. C1 [Lei, Hechang; Abeykoon, Milinda; Wang, Kefeng; Bozin, Emil S.; Ryu, Hyejin; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Ryu, Hyejin; Petrovic, C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Graf, D.] Florida State Univ, NHMFL Phys, Tallahassee, FL 32310 USA. [Warren, J. B.] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. RP Lei, HC (reprint author), Tokyo Inst Technol, Frontier Res Ctr, Midori Ku, 4259 Nagatsuta, Yokohama, Kanagawa 2268503, Japan. EM petrovic@bnl.gov RI Wang, Kefeng/E-7683-2011; Petrovic, Cedomir/A-8789-2009; LEI, Hechang/H-3278-2016 OI Wang, Kefeng/0000-0002-8449-9720; Petrovic, Cedomir/0000-0001-6063-1881; FU US DOE [DE-AC02-98CH10886]; DOE NNSA [DEFG52-10NA29659]; NSF [DMR-0654118]; State of Florida FX Work at Brookhaven is supported by the US DOE under Contract No. DE-AC02-98CH10886. This work has benefited from using the X7B beamline of the National Synchrotron Light Source at Brookhaven National Laboratory (MA and EB). Work at the National High Magnetic Field Laboratory is supported by the DOE NNSA DEFG52-10NA29659 (DG), by the NSF Cooperative Agreement No. DMR-0654118, and by the State of Florida. NR 41 TC 5 Z9 5 U1 10 U2 55 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 8 PY 2014 VL 26 IS 1 AR 015701 DI 10.1088/0953-8984/26/1/015701 PG 7 WC Physics, Condensed Matter SC Physics GA 268TX UT WOS:000328194600022 PM 24292376 ER PT J AU Berlijn, T Cheng, HP Hirschfeld, PJ Ku, W AF Berlijn, Tom Cheng, Hai-Ping Hirschfeld, P. J. Ku, Wei TI Doping effects of Se vacancies in monolayer FeSe SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; IRON PNICTIDES; FILMS AB Following the discovery of the potentially very high-temperature superconductivity in monolayer FeSe, we investigate the doping effect of Se vacancies in these materials. We find that Se vacancies pull a vacancy-centered orbital below the Fermi energy that absorbs most of the doped electrons. Furthermore, we find that the disorder-induced broadening causes an effective hole doping. The surprising net result is that, in terms of the Fe-d bands, Se vacancies behave like hole dopants rather than electron dopants. Our results exclude Se vacancies as the origin of the large electron pockets measured by angle-resolved photoemission spectroscopy. Furthermore, the unexpected doping effects not only lead to numerous consequences for the debated role of anion vacancies in the iron-based superconductors, but also demonstrate the surprisingly rich physics of vacancies in materials in general. C1 [Berlijn, Tom; Cheng, Hai-Ping; Hirschfeld, P. J.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Berlijn, Tom; Cheng, Hai-Ping] Univ Florida, Quantum Theory Project, Gainesville, FL 32611 USA. [Berlijn, Tom] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Ku, Wei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Ku, Wei] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11790 USA. RP Berlijn, T (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RI Berlijn, Tom/A-3859-2016 OI Berlijn, Tom/0000-0002-1001-2238 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE-CMSN [DE-AC02-98CH10886]; DOE [DE-FG02-05ER46236, DE-FG02-02ER45995]; DOE CMCSN; Oak Ridge National Laboratory FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division and DOE-CMSN Grant No. DE-AC02-98CH10886. P.J.H. was supported by DOE Grant No. DE-FG02-05ER46236. H.-P. C. was supported by DOE Grant No. DE-FG02-02ER45995. T. B. was supported by DOE CMCSN and, as a Wigner Fellow, by the Oak Ridge National Laboratory. NR 47 TC 18 Z9 18 U1 6 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 7 PY 2014 VL 89 IS 2 AR 020501 DI 10.1103/PhysRevB.89.020501 PG 5 WC Physics, Condensed Matter SC Physics GA AC0KZ UT WOS:000332184500002 ER PT J AU Yan, HF Li, L AF Yan, Hanfei Li, Li TI X-ray dynamical diffraction from single crystals with arbitrary shape and strain field: A universal approach to modeling SO PHYSICAL REVIEW B LA English DT Article ID PENDELLOSUNG FRINGES; DISTORTED CRYSTALS; PROPAGATION; TOPOGRAPHS; BEAMS AB The effects of dynamical diffraction in single crystals engender many unique diffraction phenomena that cannot be interpreted by the kinematical-diffraction theory, yet knowledge of them is vital to resolving a vast variety of scientific problems ranging from crystal optics to strain measurements in crystalline specimens. Although the fundamental dynamical-diffraction theory was established decades ago, modeling it remains a challenge in a general case wherein the crystal has complex boundaries and mixed diffraction geometries (Bragg or Laue). Here, we propose a universal approach for modeling x-ray dynamical diffraction from a single crystal with arbitrary shape and strain field that is based on the integral representation of the Takagi-Taupin equations. Using it, we can construct the solution iteratively via a converging series, independent of the diffraction geometry. Moreover, the integral equations offer additional insights into the diffraction physics that are not readily apparent in its differential counterparts. To demonstrate this approach, we studied the dynamical diffraction from a slab of single crystal with both Bragg and Laue diffraction excited on the entrance boundaries, a problem that is difficult to model by other methods. We also explored the mirage effect caused by the presence of a linear strain field and compared it to the Eikonal theory. Lastly, we derived a dynamical-diffraction equation correlating the structural properties of a particle to its far-field Bragg-diffraction pattern, shedding light on how dynamical diffraction affects these kinematical-diffraction-based inverse techniques for reconstructing the shape and the strain field. C1 [Yan, Hanfei; Li, Li] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Yan, HF (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM hyan@bnl.gov RI Yan, Hanfei/F-7993-2011 OI Yan, Hanfei/0000-0001-6824-0367 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC-02-98CH10886] FX H.Y. thanks I. K. Robinson for a fruitful discussion on BCDI. This paper was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC-02-98CH10886. NR 29 TC 4 Z9 4 U1 3 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 7 PY 2014 VL 89 IS 1 AR 014104 DI 10.1103/PhysRevB.89.014104 PG 6 WC Physics, Condensed Matter SC Physics GA AC0KX UT WOS:000332184300002 ER PT J AU Kashiwa, K Monnai, A AF Kashiwa, Kouji Monnai, Akihiko TI Quark contribution for center domain in heavy ion collisions SO PHYSICAL REVIEW D LA English DT Article ID FINITE TEMPERATURE; GAUGE-THEORIES; PP AB The center domain structure is revisited with the introduction of a quark contribution to understand the phenomenology in high-energy heavy-ion collisions. We show that the quark contribution may allow metastable states that would lead to a natural and consistent explanation for the temperature dependencies of color opacity and viscosity. We also argue the possibility of indirect observations of the center domain structure in experiments due to a topological critical temperature. C1 [Kashiwa, Kouji; Monnai, Akihiko] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Kashiwa, K (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM kashiwa@ribf.riken.jp; amonnai@riken.jp FU RIKEN Special Postdoctoral Researchers Program FX The authors are grateful for encouragements and valuable comments by B. Muller, R. Pisarski, and R. Venugopalan. This work is supported by the RIKEN Special Postdoctoral Researchers Program. NR 23 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 7 PY 2014 VL 89 IS 1 AR 011501 DI 10.1103/PhysRevD.89.011501 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5OP UT WOS:000331838400002 ER PT J AU Lee, D DuBois, JL Lordi, V AF Lee, Donghwa DuBois, Jonathan L. Lordi, Vincenzo TI Identification of the Local Sources of Paramagnetic Noise in Superconducting Qubit Devices Fabricated on alpha-Al2O3 Substrates Using Density-Functional Calculations SO PHYSICAL REVIEW LETTERS LA English DT Article ID DYNAMICS; ALUMINUM; SURFACES AB Effective methods for decoupling superconducting qubits (SQs) from parasitic environmental noise sources are critical for increasing their lifetime and phase fidelity. While considerable progress has been made in this area, the microscopic origin of noise remains largely unknown. In this work, first principles density functional theory calculations are employed to identify the microscopic origins of magnetic noise sources in SQs on an alpha-Al2O3 substrate. The results indicate that it is unlikely that the existence of intrinsic point defects and defect complexes in the substrate are responsible for low frequency noise in these systems. Rather, a comprehensive analysis of extrinsic defects shows that surface aluminum ions interacting with ambient molecules will form a bath of magnetic moments that can couple to the SQ paramagnetically. The microscopic origin of this magnetic noise source is discussed and strategies for ameliorating the effects of these magnetic defects are proposed. C1 [Lee, Donghwa; DuBois, Jonathan L.; Lordi, Vincenzo] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. RP Lee, D (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. EM lee1004@llnl.gov; lordi2@llnl.gov RI dubois, julie/I-9488-2014; Lee, Donghwa/G-7934-2012; OI Lee, Donghwa/0000-0002-8956-3648; DuBois, Jonathan/0000-0003-3154-4273 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [12-ERD-020] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, funded by the Laboratory Directed Research and Development Program at LLNL under project tracking code 12-ERD-020. The LLNL Computing Grand Challenge Program is acknowledged for computational support. NR 36 TC 12 Z9 12 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 7 PY 2014 VL 112 IS 1 AR 017001 DI 10.1103/PhysRevLett.112.017001 PG 5 WC Physics, Multidisciplinary SC Physics GA AB6ZC UT WOS:000331937900022 PM 24483919 ER PT J AU Kakoulli, I Prikhodko, SV Fischer, C Cilluffo, M Uribe, M Bechtel, HA Fakra, SC Marcus, MA AF Kakoulli, Ioanna Prikhodko, Sergey V. Fischer, Christian Cilluffo, Marianne Uribe, Mauricio Bechtel, Hans A. Fakra, Sirine C. Marcus, Matthew A. TI Distribution and Chemical Speciation of Arsenic in Ancient Human Hair Using Synchrotron Radiation SO ANALYTICAL CHEMISTRY LA English DT Article ID INDUCED SKIN-LESIONS; ATACAMA DESERT; CHRONIC EXPOSURE; DRINKING-WATER; NORTHERN CHILE; NAPOLEON HAIR; 2 SPECIMENS; METABOLISM; OXIDATION; ORIGIN AB Pre-Columbian populations that inhabited the Tarapaci mid river valley in the Atacama Desert in Chile during the Middle Horizon and Late Intermediate Period (AD 500-1450) show patterns of chronic poisoning due to exposure to geogenic arsenic. Exposure of these people to arsenic was assessed using synchrotron-based elemental X-ray fluorescence mapping, X-ray absorption spectroscopy, X-ray diffraction and Fourier transform infrared spectromicroscopy measurements on ancient human hair.- These combined techniques of high sensitivity and specificity enabled the discrimination between endogenous and exogenous processes that has been an analytical challenge for archeological studies and criminal investigations in which hair is used as a proxy of premortem metabolism. The high concentration of arsenic mainly in the form of inorganic As(III) and As(V) detected in the hair suggests chronic arsenicism through ingestion of As-polluted water rather than external contamination by the deposition of heavy metals due to metallophilic soil microbes or diffusion of arsenic from the soil. A decrease in arsenic concentration from the proximal to the distal end of the hair shaft analyzed may indicate a change in the diet due to mobility, though chemical or microbiologically induced processes during burial cannot be entirely ruled out. C1 [Kakoulli, Ioanna; Prikhodko, Sergey V.; Fischer, Christian] Univ Calif Los Angeles, Mat Sci & Engn Dept, Los Angeles, CA 90095 USA. [Kakoulli, Ioanna; Fischer, Christian] Univ Calif Los Angeles, Cotsen Inst Archaeol, Los Angeles, CA 90095 USA. [Cilluffo, Marianne] Univ Calif Los Angeles, Dept Integrat Biol & Physiol, Los Angeles, CA 90095 USA. [Uribe, Mauricio] Univ Chile, Fac Ciencias Sociales, Nunoa, Santiago De Chi, Chile. [Bechtel, Hans A.; Fakra, Sirine C.; Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kakoulli, I (reprint author), Univ Calif Los Angeles, Mat Sci & Engn Dept, POB 951595, Los Angeles, CA 90095 USA. EM kakoulli@ucla.edu FU Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-ACO2-05CH11231]; NSF [0813649]; Senate Faculty Awards at the University of California Los Angeles (UCLA) FX We thank the Consejo de Monumentos Nacionales de Chile for site access and permissions for sampling and analysis and Ran Boytner and Maria Cecilia Lozada codirectors of the Tarapaci Valley Archaeological Project for providing information on the archaeology and ethnography of the area. The operations of the Advanced Light Source at Lawrence Berkeley National Laboratory are supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under contract number DE-AC02-05CH11231. FEGVPSEM-EDS analysis was conducted at the Molecular and Nano Archaeology Laboratory at UCLA on the FEI Nova NanoSEM 230 purchased with NSF award no. 0813649. Travel funding to the synchrotron facility was provided by the Senate Faculty Awards at the University of California Los Angeles (UCLA). Physical microsamples used for the analysis and analytical data are stored and accessed through the Molecular and Nano Archaeology Laboratory, UCLA. NR 47 TC 5 Z9 5 U1 3 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 7 PY 2014 VL 86 IS 1 SI SI BP 521 EP 526 DI 10.1021/ac4024439 PG 6 WC Chemistry, Analytical SC Chemistry GA 287NM UT WOS:000329548700052 PM 24320096 ER PT J AU VanDelinder, V Bachand, GD AF VanDelinder, Virginia Bachand, George D. TI Photodamage and the Importance of Photoprotection in Biomolecular-Powered Device Applications SO ANALYTICAL CHEMISTRY LA English DT Article ID SINGLE-MOLECULE FLUORESCENCE; OXYGEN SCAVENGING SYSTEM; SOFT LITHOGRAPHY; KINESIN; MICROTUBULES; MOTOR; MECHANISM; TRANSPORT; MOVEMENT; PROTEINS AB In recent years, an enhanced understanding of the mechanisms underlying photobleaching and photoblinking of fluorescent dyes has led to improved photoprotection strategies, such as reducing and oxidizing systems (ROXS) that reduce blinking and oxygen scavenging systems to reduce bleaching. Excitation of fluorescent dyes can also result in damage to catalytic proteins (e.g., biomolecular motors), affecting the performance of integrated devices. Here, we characterized the motility of microtubules driven by kinesin motor proteins using various photoprotection strategies, including a microfluidic deoxygenation device. Impaired motility of microtubules was observed at high excitation intensities in the absence of photoprotection as well as in the presence of an enzymatic oxygen scavenging system. In contrast, using a polydimethylsiloxane (PDMS) microfluidic deoxygenation device and ROXS, not only were the fluorophores slower to bleach but also moving the velocity and fraction of microtubules over time remained unaffected even at high excitation intensities. Further, we demonstrate the importance of photoprotection by examining the effect of photodamage on the behavior of a switchable mutant of kinesin. Overall, these results demonstrate that improved photoprotection strategies may have a profound impact on functional fluorescently labeled biomolecules in integrated devices. C1 [VanDelinder, Virginia; Bachand, George D.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Bachand, GD (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM gdbacha@sandia.gov OI Bachand, George/0000-0002-3169-9980 FU U.S. Department of Energy; Office of Basic Energy Sciences; Division of Materials Sciences and Engineering [KC0203010]; Center for Integrated Nanotechnologies [RA2013A0021]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported from the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, Project KC0203010. Fabrication of the microfluidic device was performed at the Center for Integrated Nanotechnologies (V.V., user project RA2013A0021), an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 38 TC 7 Z9 7 U1 2 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 7 PY 2014 VL 86 IS 1 SI SI BP 721 EP 728 DI 10.1021/ac403187g PG 8 WC Chemistry, Analytical SC Chemistry GA 287NM UT WOS:000329548700077 PM 24350711 ER PT J AU Petridis, L Arnbaye, H Jagadamma, S Kilbey, SM Lokitz, BS Lauter, V Mayes, MA AF Petridis, Loukas Arnbaye, Haile Jagadamma, Sindhu Kilbey, S. Michael, II Lokitz, Bradley S. Lauter, Valeria Mayes, Melanie A. TI Spatial Arrangement of Organic Compounds on a Model Mineral Surface: Implications for Soil Organic Matter Stabilization SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID PARTICLE MESH EWALD; MOLECULAR-DYNAMICS; NEUTRON REFLECTOMETRY; HUMIC SUBSTANCES; LIPID BILAYERS; FATTY-ACIDS; ADSORPTION; SIMULATION; SEDIMENTS; CELLULOSE AB The complexity of the mineral-organic carbon interface may influence the extent of stabilization of Organic carbon compounds in soils, which is important for global climate futures. The nanoscale structure of a model interface was examined here by depositing films of organic carbon compounds of contrasting chemical character, hydrophilic glucose and amphiphilic stearic acid, onto a soil mineral analogue (Al2O3). Neutron reflectometry, a technique which provides depth-sensitive insight into the organization of the thin films, indicates that glucose molecules reside in a layer between Al2O3 and stearic acid, a result that was verified by water contact angle measurements. Molecular dynamics simulations reveal the thermodynamic driving force behind glucose partitioning on the mineral interface: The entropic penalty of confining the less mobile glucose on the mineral surface is lower than for stearic acid. The fundamental information obtained here helps rationalize how complex arrangements of organic carbon on soil mineral surfaces may arise. C1 [Petridis, Loukas] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. [Arnbaye, Haile] Oak Ridge Natl Lab, Res Accelerator Div, Oak Ridge, TN 37831 USA. [Jagadamma, Sindhu; Mayes, Melanie A.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Jagadamma, Sindhu; Mayes, Melanie A.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Kilbey, S. Michael, II; Lokitz, Bradley S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kilbey, S. Michael, II] Univ Tennessee, Dept Chem & Chem & Biomol Engn, Knoxville, TN 37996 USA. [Lauter, Valeria] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Petridis, L (reprint author), Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. EM petridisl@ornl.gov RI Lokitz, Bradley/Q-2430-2015; Ambaye, Haile/D-1503-2016; Petridis, Loukas/B-3457-2009 OI Lokitz, Bradley/0000-0002-1229-6078; Ambaye, Haile/0000-0002-8122-9952; Petridis, Loukas/0000-0001-8569-060X FU Oak Ridge National Laboratory (ORNL); Scientific User Facilities Division, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); Scientific User Facilities Division of BES at DOE; DOE [DE-AC05-00OR22725]; National Science Foundation [OCI-1053575] FX This project is funded by the Oak Ridge National Laboratory (ORNL) Director's Research and Development Program (LDRD). Research at the ORNL Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). A portion of this research was conducted at ORNL's Center for Nanophase Materials Sciences, which is sponsored by the Scientific User Facilities Division of BES at DOE. ORNL is managed by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the DOE. This work used the Extreme Science and Engineering Discovery Environment.(XSEDE), which is supported by National Science Foundation grant number OCI-1053575. NR 35 TC 3 Z9 3 U1 1 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 79 EP 84 DI 10.1021/es403430k PG 6 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800017 PM 24328330 ER PT J AU Kim, YH Yiacoumi, S Lee, I McFarlane, J Tsouris, C AF Kim, Yong-ha Yiacoumi, Sotira Lee, Ida McFarlane, Joanna Tsouris, Costas TI Influence of Radioactivity on Surface Charging and Aggregation Kinetics of Particles in the Atmosphere SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID POPULATION-BALANCE EQUATION; CHERNOBYL ACCIDENT; COLLOIDAL PARTICLES; ALPHA-PARTICLES; AEROSOLS; COAGULATION; FUKUSHIMA; IONIZATION; DEPOSITION; RADIONUCLIDES AB Radioactivity can influence surface interactions, but its effects on particle aggregation kinetics have not been included in transport modeling of radioactive particles. In this research, experimental and theoretical studies have been performed to investigate the influence of radioactivity on surface charging and aggregation kinetics of radioactive particles in the atmosphere. Radioactivity-induced charging mechanisms have been investigated at the microscopic level, and heterogeneous surface potential caused by radioactivity is reported. The radioactivity-induced surface charging is highly influenced by several parameters, such as rate and type of radioactive decay. A population balance model, including interparticle forces, has been employed to study the effects of radioactivity on particle aggregation kinetics in air. It has been found that radioactivity can hinder aggregation of particles because of similar surface charging caused by the decay process. Experimental and theoretical studies provide useful insights into the understanding of transport characteristics of radioactive particles emitted from severe nuclear events, such as the recent accident of Fukushima or deliberate explosions of radiological devices. C1 [Kim, Yong-ha; Yiacoumi, Sotira; Tsouris, Costas] Georgia Inst Technol, Atlanta, GA 30332 USA. [Lee, Ida] Univ Tennessee, Knoxville, TN 37996 USA. [McFarlane, Joanna; Tsouris, Costas] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tsouris, C (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA. EM tsourisc@ornl.gov RI Tsouris, Costas/C-2544-2016; McFarlane, Joanna/C-5998-2016 OI Tsouris, Costas/0000-0002-0522-1027; McFarlane, Joanna/0000-0002-4112-5104 FU Defense Threat Reduction Agency [DTRA1-08-10-BRCWMD-BAA]; U.S. Department of Energy [DEAC05-00OR22725] FX This work was supported by the Defense Threat Reduction Agency under Grant DTRA1-08-10-BRCWMD-BAA. The manuscript has been co-authored by UT-Battelle, LLC, under Contract DEAC05-00OR22725 with the U.S. Department of Energy. The authors are thankful to Laetitia H. Delmau and Ivan Dunbar for their technical assistance with aspects of radioactive substrate preparation. Amy Harkey edited the manuscript. NR 41 TC 2 Z9 2 U1 1 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 182 EP 189 DI 10.1021/es4047439 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800029 PM 24308778 ER PT J AU van Groos, PGK Esser, BK Williams, RW Hunt, JR AF van Groos, Paul G. Koster Esser, Bradley K. Williams, Ross W. Hunt, James R. TI Isotope Effect of Mercury Diffusion in Air SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID FIRED POWER-PLANTS; ELEMENTAL MERCURY; MASS-SPECTROMETRY; NUCLEAR VOLUME; GAS-PHASE; FLUE-GAS; FRACTIONATION; WATER; EQUILIBRIUM; EVAPORATION AB Identifying and reducing impacts from mercury sources in the environment remains a considerable challenge and requires process based models to quantify mercury stocks and flows. The stable isotope composition of mercury in environmental samples can help address this challenge by serving as a tracer of specific sources and processes. Mercury isotope variations are small and result only from isotope fractionation during transport, equilibrium, and transformation processes. Because these processes occur in both industrial and environmental settings, knowledge of their associated isotope effects is required to interpret mercury isotope data. To improve the mechanistic modeling of mercury isotope effects during gas phase diffusion, an experimental program tested the applicability of kinetic gas theory. Gas-phase elemental mercury diffusion through small bore needles from finite sources demonstrated mass dependent diffusivities leading to isotope fractionation described by a Rayleigh distillation model. The measured relative atomic diffusivities among mercury isotopes in air are large and in agreement with kinetic gas theory. Mercury diffusion in air offers a reasonable explanation of recent field results reported in the literature. C1 [van Groos, Paul G. Koster; Hunt, James R.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Esser, Bradley K.; Williams, Ross W.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94551 USA. RP van Groos, PGK (reprint author), Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. EM pkostervangroos@gmail.com FU United States Environmental Protection Agency (EPA) under the Science to Achieve Results (STAR) Graduate Fellowship Program; NIEHS [P42 ES04705] FX We thank V. Genetti at LLNL for technical assistance. We also thank two anonymous reviews for their helpful comments. The research described in this paper was funded in part by the United States Environmental Protection Agency (EPA) under the Science to Achieve Results (STAR) Graduate Fellowship Program. EPA has not officially endorsed this publication, and the views expressed herein may not reflect the views of the EPA. Additional funding provided by NIEHS Superfund Basic Research Program P42 ES04705. NR 38 TC 8 Z9 9 U1 2 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 227 EP 233 DI 10.1021/es4033666 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800034 ER PT J AU Hu, YD Li, QY Lee, B Jun, YS AF Hu, Yandi Li, Qingyun Lee, Byeongdu Jun, Young-Shin TI Aluminum Affects Heterogeneous Fe(III) (Hydr)oxide Nucleation, Growth, and Ostwald Ripening SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ACID-MINE DRAINAGE; X-RAY-SCATTERING; HYDROUS OXIDES; IRON-OXIDES; AL; COPRECIPITATION; FERRIHYDRITE; GOETHITE; KINETICS; COPPER AB Heterogeneous coprecipitation of iron and aluminum oxides is an important process for pollutant immobilization and removal in natural and engineered aqueous environments. Here, using a synchrotron-based small-angle X-ray scattering technique, we studied heterogeneous nucleation and growth of Fe(III) (hydr)oxide on quartz under conditions found in acid mine drainage (at pH = 3.7 +/- 0.2, [Fe3+] = 10(-4) M) with different initial aqueous Al/Fe ratios (0:1, 1:1, and 5:1). Interestingly, although the atomic ratios of Al/Fe in the newly formed Fe(III) (hydr)oxide precipitates were less than 1%, the in situ particle size and volume evolutions of the precipitates on quartz were significantly influenced by aqueous Al/Fe ratios. At the end of the 3 h experiments, with aqueous Al/Fe ratios of 0:1, 1:1, and 5:1, the average radii of gyration of particles on quartz were 5.7 +/- 0.3, 4.6 +/- 0.1, and 3.7 +/- 0.3 nm, respectively, and the ratio of total particle volumes on quartz was 1.7:3.4:1.0. The Fe(III) (hydr)oxide precipitates were poorly crystallized, and were positively charged in all solutions. In the presence of Al3+, Al3+ adsorption onto quartz changed the surface charge of quartz from negative to positive, which caused the slower heterogeneous growth of Fe(III) (hydr)oxide on quartz. Furthermore, Al affected the amount of water included in the Fe(III) (hydr)oxides, which can influence their adsorption capacity. This study yielded important information usable for pollutant removal not only in natural environments, but also in engineered water treatment processes. C1 [Hu, Yandi; Li, Qingyun; Jun, Young-Shin] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. [Hu, Yandi] Univ Houston, Dept Civil & Environm Engn, Houston, TX 77204 USA. [Lee, Byeongdu] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Jun, YS (reprint author), Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. EM ysjun@seas.wustl.edu RI Hu, Yandi/F-7968-2011; Foundry, Molecular/G-9968-2014; OI Hu, Yandi/0000-0002-8506-9335; Lee, Byeongdu/0000-0003-2514-8805 FU Washington University; NSF Environmental Chemical Science [ChE-1214090]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by a Washington University Faculty Start-up Grant and an NSF Environmental Chemical Science (ChE-1214090). We thank Dr. Debin Wang and Dr. Jim De Yoreo for XPS measurements at the Molecular Foundry, Lawrence Berkeley National Laboratory. We also thank Dr. Soenke Seifert for X-ray scattering experimental help, Dr. Alejandro Fernandez-Martinez for discussions about electron density, Dr. Matthew Suchomel for HR-XRD analysis of solid samples at APS Sector 11-BM, and Prof. James Ballard for valuable discussion. Use of the Advanced Photon Source (Sector 11-BM and 12ID-B) at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 35 TC 5 Z9 5 U1 4 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 299 EP 306 DI 10.1021/es403777w PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800042 PM 24289329 ER PT J AU Redden, G Fox, D Zhang, C Fujita, Y Guo, LJ Huang, H AF Redden, George Fox, Don Zhang, Chi Fujita, Yoshiko Guo, Luanjing Huang, Hai TI CaCO3 Precipitation, Transport and Sensing in Porous Media with In Situ Generation of Reactants SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CALCIUM-CARBONATE PRECIPITATION; UREA HYDROLYSIS; FLOW; REDUCTION; STRONTIUM; PH; COPRECIPITATION; PERMEABILITY; GROUNDWATER; DISSOLUTION AB Ureolytically driven calcite precipitation is a promising approach for inducing subsurface mineral precipitation, but engineered application requires the ability to control and predict precipitate distribution. To study the coupling between reactant transport and precipitate distribution, columns with defined zones of immobilized urease were used to examine the distribution of calcium carbonate precipitation along the flow path, at two different initial flow rates. As expected, with slower flow precipitate was concentrated toward the upstream end of the enzyme zone and with higher flow the solid was more uniformly distributed over the enzyme zone. Under constant hydraulic head conditions the flow rate decreased as precipitates decreased porosity and permeability. The hydrolysis/precipitation zone was expected to become compressed in the upstream direction. However, apparent reductions in the urea hydrolysis rate and changes in the distribution of enzyme activity, possibly due to CaCO3 precipitate hindering urea transport to the enzyme, or enzyme mobilization, mitigated reaction zone compression. Co-injected strontium was expected to be sequestered by coprecipitation with CaCO3, but the results suggested that coprecipitation was not an effective sequestration mechanism in this system. In addition, spectral induced polarization (SIP) was used to monitor the spatial and temporal evolution of the reaction zone. C1 [Redden, George] Montana State Univ, Bozeman, MT 59717 USA. [Fox, Don; Fujita, Yoshiko; Huang, Hai] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Zhang, Chi] Rutgers State Univ, Dept Earth & Environm Sci, Newark, NJ 07102 USA. [Guo, Luanjing] Univ Utah, Dept Chem Engn, Salt Lake City, UT 84112 USA. RP Redden, G (reprint author), Montana State Univ, Bozeman, MT 59717 USA. EM George.redden@coe.montana.edu RI Fujita, Yoshiko/S-2007-2016 OI Fujita, Yoshiko/0000-0002-4472-4102 FU Subsurface Biogeochemical Research Program; Office of Biological and Environmental Research; U.S. Department of Energy [DEAC07-051D14517] FX We thank James Henriksen for assistance with urease characterization, Joanna Taylor for assistance with analytical measurements, and Tammy Trowbridge for SEM imaging. This research was supported by the Subsurface Biogeochemical Research Program, Office of Biological and Environmental Research, U.S. Department of Energy, under contract DEAC07-051D14517. NR 39 TC 5 Z9 5 U1 3 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 542 EP 549 DI 10.1021/es4029777 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800070 PM 24289499 ER PT J AU Levine, JS Goldberg, DS Lackner, KS Matter, JM Supp, MG Ramakrishnan, TS AF Levine, Jonathan S. Goldberg, David S. Lackner, Klaus S. Matter, Juerg M. Supp, Michael G. Ramakrishnan, T. S. TI Relative Permeability Experiments of Carbon Dioxide Displacing Brine and Their Implications for Carbon Sequestration SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID IMMISCIBLE DISPLACEMENT; SUPERCRITICAL CO2; SILICA SURFACES; POROUS-MEDIA; FLOW; WETTABILITY; ROCKS AB To mitigate anthropogenically induced climate change and ocean acidification, net carbon dioxide emissions to the atmosphere must be reduced. One proposed option is underground CO2 disposal. Large-scale injection of CO2 into the Earth's crust requires an understanding of the multiphase flow properties of high-pressure CO2 displacing brine. We present laboratory-scale core flooding experiments designed to measure CO2 endpoint relative permeability for CO2 displacing brine at in situ pressures, salinities, and temperatures. Endpoint drainage CO2 relative permeabilities for liquid and supercritical CO2 were found to be clustered around 0.4 for both the synthetic and natural media studied. These values indicate that relative to CO2, water may not be strongly wetting the solid surface. Based on these results, CO2 injectivity will be reduced and pressure-limited reservoirs will have reduced disposal capacity, though area-limited reservoirs may have increased capacity. Future reservoir-scale modeling efforts should incorporate sensitivity to relative permeability. Assuming applicability of the experimental results to other lithologies and that the majority of reservoirs are pressure limited, geologic carbon sequestration would require approximately twice the number of wells for the same injectivity. C1 [Levine, Jonathan S.; Lackner, Klaus S.] Columbia Univ, Dept Earth & Environm Engn, New York, NY 10027 USA. [Goldberg, David S.] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY 10964 USA. [Levine, Jonathan S.; Supp, Michael G.; Ramakrishnan, T. S.] Schlumberger Doll Res Ctr, Cambridge, MA 02143 USA. RP Levine, JS (reprint author), Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM jonathan.levine@netl.doe.gov FU NYSERDA [NYSERDA-10113]; U.S. National Science Foundation FX J.L. acknowledges the entire CO2 research group at Schlumberger-Doll Research for help with experiments as well as helpful discussions. This work was supported by a NYSERDA grant (NYSERDA-10113), and J.L. acknowledges support from the U.S. National Science Foundation, through a Fellowship in the IGERT Joint Program in Applied Mathematics and Earth and Environmental Science at Columbia University. The manuscript was greatly improved thanks to the comments and feedback received from the reviewers. NR 52 TC 19 Z9 19 U1 1 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 7 PY 2014 VL 48 IS 1 BP 811 EP 818 DI 10.1021/es401549e PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 287NN UT WOS:000329548800103 PM 24274391 ER PT J AU Gilbert, JA van der Lelie, D Zarraonaindia, I AF Gilbert, Jack A. van der Lelie, Daniel Zarraonaindia, Iratxe TI Microbial terroir for wine grapes SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Editorial Material ID MICROORGANISMS; DIVERSITY; BERRIES C1 [Gilbert, Jack A.; Zarraonaindia, Iratxe] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [van der Lelie, Daniel] FMC Corp, Ctr Excellence Agr Biosolut, Res Triangle Pk, NC 27703 USA. [Zarraonaindia, Iratxe] Basque Fdn Sci, Ikerbasque, Bilbao 48011, Spain. RP Gilbert, JA (reprint author), Argonne Natl Lab, Inst Genom & Syst Biol, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gilbertjack@anl.gov NR 14 TC 24 Z9 24 U1 4 U2 50 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 5 EP 6 DI 10.1073/pnas.1320471110 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700028 PM 24309378 ER PT J AU Kim, S Stahlberg, J Sandgren, M Paton, RS Beckham, GT AF Kim, Seonah Stahlberg, Jerry Sandgren, Mats Paton, Robert S. Beckham, Gregg T. TI Quantum mechanical calculations suggest that lytic polysaccharide monooxygenases use a copper-oxyl, oxygen-rebound mechanism SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE C-H activation; copper monooxygenase; GH61; CBM33; biofuels ID ALPHA-HYDROXYLATING MONOOXYGENASE; DOPAMINE BETA-MONOOXYGENASE; GLYCOSIDE HYDROLASE FAMILY; ACTIVE-SITE; CATALYTIC MECHANISM; CELLOBIOSE DEHYDROGENASE; CELLULOSE; COMPLEXES; MONONUCLEAR; REACTIVITY AB Lytic polysaccharide monooxygenases (LPMOs) exhibit a mononuclear copper-containing active site and use dioxygen and a reducing agent to oxidatively cleave glycosidic linkages in polysaccharides. LPMOs represent a unique paradigm in carbohydrate turnover and exhibit synergy with hydrolytic enzymes in biomass depolymerization. To date, several features of copper binding to LPMOs have been elucidated, but the identity of the reactive oxygen species and the key steps in the oxidative mechanism have not been elucidated. Here, density functional theory calculations are used with an enzyme active site model to identify the reactive oxygen species and compare two hypothesized reaction pathways in LPMOs for hydrogen abstraction and polysaccharide hydroxylation; namely, a mechanism that employs a eta(1)-superoxo intermediate, which abstracts a substrate hydrogen and a hydroperoxo species is responsible for substrate hydroxylation, and a mechanism wherein a copper-oxyl radical abstracts a hydrogen and subsequently hydroxylates the substrate via an oxygen-rebound mechanism. The results predict that oxygen binds end-on (eta(1)) to copper, and that a copperoxyl-mediated, oxygen-rebound mechanism is energetically preferred. The N-terminal histidine methylation is also examined, which is thought to modify the structure and reactivity of the enzyme. Density functional theory calculations suggest that this posttranslational modification has only a minor effect on the LPMO active site structure or reactivity for the examined steps. Overall, this study suggests the steps in the LPMO mechanism for oxidative cleavage of glycosidic bonds. C1 [Kim, Seonah; Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80202 USA. [Stahlberg, Jerry; Sandgren, Mats] Swedish Univ Agr Sci, Dept Mol Biol, SE-75007 Uppsala, Sweden. [Stahlberg, Jerry] Norwegian Univ Life Sci, Dept Chem Biotechnol & Food Sci, NO-1432 As, Norway. [Paton, Robert S.] Univ Oxford, Chem Res Lab, Oxford OX1 3TA, England. RP Paton, RS (reprint author), Univ Oxford, Chem Res Lab, S Parks Rd, Oxford OX1 3TA, England. EM robert.paton@chem.ox.ac.uk; gregg.beckham@nrel.gov RI Paton, Robert/A-4564-2010; Stahlberg, Jerry/D-4163-2013 OI Paton, Robert/0000-0002-0104-4166; Stahlberg, Jerry/0000-0003-4059-8580 FU US Department of Energy BioEnergy Technologies Office; Faculty for Natural Resources and Agriculture at the Swedish University of Agricultural Sciences; Oxford University Press John Fell Fund; Royal Society [RG110617]; Texas Advanced Computing Center under the National Science Foundation Extreme Science and Engineering Discovery Environment Grant [MCB-090159] FX We thank Vincent Eijsink for a critical reading of the manuscript and for constructive comments; S. K. and G. T. B. thank the US Department of Energy BioEnergy Technologies Office for funding; J.S. and M. S. thank the Faculty for Natural Resources and Agriculture at the Swedish University of Agricultural Sciences through the research program MicroDrivE; and R. S. P. thanks the Oxford University Press John Fell Fund and the Royal Society (RG110617) for funding. Computer time was provided by the Texas Advanced Computing Center under the National Science Foundation Extreme Science and Engineering Discovery Environment Grant MCB-090159 and by the National Renewable Energy Laboratory Computational Sciences Center. NR 46 TC 61 Z9 61 U1 11 U2 88 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 149 EP 154 DI 10.1073/pnas.1316609111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700054 PM 24344312 ER PT J AU Li, D Furukawa, H Deng, HX Liu, C Yaghi, OM Eisenberg, DS AF Li, Dan Furukawa, Hiroyasu Deng, Hexiang Liu, Cong Yaghi, Omar M. Eisenberg, David S. TI Designed amyloid fibers as materials for selective carbon dioxide capture SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE amyloid materials; chemisorption; designed fibers ID METAL-ORGANIC FRAMEWORKS; CO2 ADSORPTION; FLUE-GAS; SEPARATION; PROTEINS; KINETICS; ENERGY; NANOFIBRILS; ADSORBENTS; FIBRILS AB New materials capable of binding carbon dioxide are essential for addressing climate change. Here, we demonstrate that amyloids, self-assembling protein fibers, are effective for selective carbon dioxide capture. Solid-state NMR proves that amyloid fibers containing alkylamine groups reversibly bind carbon dioxide via carbamate formation. Thermodynamic and kinetic capture-and-release tests show the carbamate formation rate is fast enough to capture carbon dioxide by dynamic separation, undiminished by the presence of water, in both a natural amyloid and designed amyloids having increased carbon dioxide capacity. Heating to 100 degrees C regenerates the material. These results demonstrate the potential of amyloid fibers for environmental carbon dioxide capture. C1 [Li, Dan; Furukawa, Hiroyasu; Deng, Hexiang; Liu, Cong; Yaghi, Omar M.; Eisenberg, David S.] Univ Calif Los Angeles, Dept Energy, Inst Genom & Prote, Los Angeles, CA 90095 USA. [Li, Dan; Furukawa, Hiroyasu; Deng, Hexiang; Liu, Cong; Yaghi, Omar M.; Eisenberg, David S.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Li, Dan; Liu, Cong; Eisenberg, David S.] Univ Calif Los Angeles, Inst Mol Biol, Los Angeles, CA 90095 USA. [Li, Dan; Liu, Cong; Eisenberg, David S.] Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. [Furukawa, Hiroyasu; Deng, Hexiang; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Furukawa, Hiroyasu; Deng, Hexiang; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Yaghi, OM (reprint author), Univ Calif Los Angeles, Dept Energy, Inst Genom & Prote, Los Angeles, CA 90095 USA. EM yaghi@berkeley.edu; david@mbi.ucla.edu RI Furukawa, Hiroyasu/C-5910-2008; Li, Dan/J-7581-2016; OI Furukawa, Hiroyasu/0000-0002-6082-1738; Yaghi, Omar/0000-0002-5611-3325 FU Department of Energy BER [DE-FC03-02ER63421]; National Science Foundation [MCB-0958111]; Howard Hughes Medical Institute FX We thank D. Anderson, University of California, Los Angeles (UCLA) for technical support and discussion, M. Sawaya (UCLA) for structure modeling, S. Das (UCLA) for his initial work, and C. Stevens (University of California, Berkeley) for her help in elemental analysis. This work was supported by Department of Energy BER Grant DE-FC03-02ER63421, National Science Foundation Grant MCB-0958111, and Howard Hughes Medical Institute. NR 41 TC 31 Z9 31 U1 11 U2 99 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 191 EP 196 DI 10.1073/pnas.1321797111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700061 PM 24367077 ER PT J AU Ivanova, MI Sievers, SA Guenther, EL Johnson, LM Winkler, DD Galaleldeen, A Sawaya, MR Hart, PJ Eisenberg, DS AF Ivanova, Magdalena I. Sievers, Stuart A. Guenther, Elizabeth L. Johnson, Lisa M. Winkler, Duane D. Galaleldeen, Ahmad Sawaya, Michael R. Hart, P. John Eisenberg, David S. TI Aggregation-triggering segments of SOD1 fibril formation support a common pathway for familial and sporadic ALS SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE protein aggregation; peptide structure; amyotrophic lateral sclerosis ID AMYOTROPHIC-LATERAL-SCLEROSIS; ZINC SUPEROXIDE-DISMUTASE; COPPER-BINDING-SITE; WILD-TYPE; TRANSGENIC MICE; MOLECULAR-BASIS; MUTATION; INCLUSIONS; INSIGHTS AB ALS is a terminal disease of motor neurons that is characterized by accumulation of proteinaceous deposits in affected cells. Pathological deposition of mutated Cu/Zn superoxide dismutase (SOD1) accounts for similar to 20% of the familial ALS (fALS) cases. However, understanding the molecular link between mutation and disease has been difficult, given that more than 140 different SOD1 mutants have been observed in fALS patients. In addition, the molecular origin of sporadic ALS (sALS) is unclear. By dissecting the amino acid sequence of SOD1, we identified four short segments with a high propensity for amyloid fibril formation. We find that fALS mutations in these segments do not reduce their propensity to form fibrils. The atomic structures of two fibril-forming segments from the C terminus, (DSVISLS107)-D-101 and (147)GVIGIAQ(153), reveal tightly packed beta-sheets with steric zipper interfaces characteristic of the amyloid state. Based on these structures, we conclude that both C-terminal segments are likely to form aggregates if available for interaction. Proline substitutions in (DSVISLS107)-D-101 and (147)GVIGIAQ(153) impaired nucleation and fibril growth of full-length protein, confirming that these segments participate in aggregate formation. Our hypothesis is that improper protein maturation and incompletely folded states that render these aggregation-prone segments available for interaction offer a common molecular pathway for sALS and fALS. C1 [Ivanova, Magdalena I.; Sievers, Stuart A.; Guenther, Elizabeth L.; Johnson, Lisa M.; Sawaya, Michael R.; Eisenberg, David S.] Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. [Ivanova, Magdalena I.; Sievers, Stuart A.; Guenther, Elizabeth L.; Johnson, Lisa M.; Sawaya, Michael R.; Eisenberg, David S.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Ivanova, Magdalena I.; Sievers, Stuart A.; Guenther, Elizabeth L.; Johnson, Lisa M.; Sawaya, Michael R.; Eisenberg, David S.] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA. [Ivanova, Magdalena I.] Univ Michigan, Dept Neurol, Sch Med, Ann Arbor, MI 48109 USA. [Sievers, Stuart A.] CALTECH, Div Biol, Pasadena, CA 91125 USA. [Winkler, Duane D.; Galaleldeen, Ahmad; Hart, P. John] Univ Texas Hlth Sci Ctr San Antonio, Dept Biochem, San Antonio, TX 78229 USA. [Winkler, Duane D.] Univ Texas Dallas, Dept Mol & Cell Biol, Richardson, TX 75080 USA. [Galaleldeen, Ahmad] St Marys Univ, Dept Biol Sci, San Antonio, TX 78228 USA. [Hart, P. John] South Texas Vet Hlth Care Syst, Dept Vet Affairs, Geriatr Res Educ & Clin Ctr, San Antonio, TX 78229 USA. RP Eisenberg, DS (reprint author), Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. EM david@mbi.ucla.edu FU Howard Hughes Medical Institute [P01 NS049134]; National Institutes of Health [AG029430]; NIH; Department of Energy; Department of Veterans Affairs [1I01BX000506]; Judith and Jean Pape Adams Charitable Foundation; NIH [R01 NS39112] FX We thank Dr. L. Goldschmidt, Dr. M. Chattopadhyay, Dr. R. Nelson, Dr. B. Chan, and Prof. J. S. Valentine for discussions; Dr. I. Kourinov, Dr. J. Schuermann, Dr. K. Rajashankar, Dr. N. Sukumar, and Dr. S. Banerjee at Advanced Photon Source beamline 24-ID-E and European Synchrotron Radiation Facility beamline ID13 for help with X-ray data collection; Howard Hughes Medical Institute, P01 NS049134, National Institutes of Health AG029430, NIH P01, and Department of Energy for support to the D.E. laboratory; and Department of Veterans Affairs 1I01BX000506, the Judith and Jean Pape Adams Charitable Foundation, and NIH R01 NS39112 for support to the P.J.H. laboratory. NR 27 TC 25 Z9 26 U1 1 U2 11 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 197 EP 201 DI 10.1073/pnas.1320786110 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700062 PM 24344300 ER PT J AU Chang, YC Bowie, JU AF Chang, Yu-Chu Bowie, James U. TI Measuring membrane protein stability under native conditions SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE membrane protein folding; steric trap ID BACTERIORHODOPSIN; STREPTAVIDIN; STATE; UREA AB The thermodynamic stability of proteins is typically measured at high denaturant concentrations and then extrapolated back to zero denaturant conditions to obtain unfolding free energies under native conditions. For membrane proteins, the extrapolations are fraught with considerable uncertainty as the denaturants may have complex effects on the membrane or micellar structure. We therefore sought to measure stability under native conditions, using a method that does not perturb the properties of the membrane or membrane mimetics. We use a technique called steric trapping to measure the thermodynamic stability of bacteriorhodopsin in bicelles and micelles. We find that bacteriorhodopsin has a high thermodynamic stability, with an unfolding free energy of similar to 11 kcal/mol in dimyristoyl phosphatidylcholine bicelles. Nevertheless, the stability is much lower than predicted by extrapolation of measurements made at high denaturant concentrations. We investigated the discrepancy and found that unfolding free energy is not linear with denaturant concentration. Apparently, long extrapolations of helical membrane protein unfolding free energies must be treated with caution. Steric trapping, however, provides a method for making these measurements. C1 [Chang, Yu-Chu; Bowie, James U.] Univ Calif Los Angeles, Dept Chem & Biochem, UCLA DOE Inst Genom & Prote, Inst Mol Biol, Los Angeles, CA 90095 USA. RP Bowie, JU (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, UCLA DOE Inst Genom & Prote, Inst Mol Biol, Los Angeles, CA 90095 USA. EM bowie@mbi.ucla.edu FU National Institutes of Health [R01 GM063919] FX We thank members of the J.U.B. laboratory for insightful discussion and critical reading of the manuscript. This work is supported by National Institutes of Health Grant R01 GM063919 (to J.U.B.). NR 23 TC 15 Z9 15 U1 1 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 219 EP 224 DI 10.1073/pnas.1318576111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700066 PM 24367094 ER PT J AU Lang, PT Holton, JM Fraser, JS Alber, T AF Lang, P. Therese Holton, James M. Fraser, James S. Alber, Tom TI Protein structural ensembles are revealed by redefining X-ray electron density noise SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE electron number density; refinement against perturbed input data; protein dynamics; molecular motions; Ringer ID CRYSTAL-STRUCTURES; MACROMOLECULAR MODELS; DIFFRACTION DATA; SPACE GROUP; KINASE-A; CRYSTALLOGRAPHY; REFINEMENT; CATALYSIS; VARIANCE; CAVITIES AB To increase the power of X-ray crystallography to determine not only the structures but also the motions of biomolecules, we developed methods to address two classic crystallographic problems: putting electron density maps on the absolute scale of e(-)/angstrom(3) and calculating the noise at every point in the map. We find that noise varies with position and is often six to eight times lower than thresholds currently used in model building. Analyzing the rescaled electron density maps from 485 representative proteins revealed unmodeled conformations above the estimated noise for 45% of side chains and a previously hidden, low-occupancy inhibitor of HIV capsid protein. Comparing the electron density maps in the free and nucleotide-bound structures of three human protein kinases suggested that substrate binding perturbs distinct intrinsic allosteric networks that link the active site to surfaces that recognize regulatory proteins. These results illustrate general approaches to identify and analyze alternative conformations, low-occupancy small molecules, solvent distributions, communication pathways, and protein motions. C1 [Lang, P. Therese; Fraser, James S.; Alber, Tom] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Holton, James M.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Holton, James M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Alber, T (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM tom@ucxray.berkeley.edu OI Fraser, James/0000-0002-5080-2859 FU National Science Foundation; National Science and Engineering Research Council of Canada; National Institutes of Health [R01 48958, DP5OD009180, GM073210, GM082250, GM094625]; US Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX We thank David Cerutti for providing access to molecular dynamics simulations. J.S.F. was supported by National Science Foundation and the National Science and Engineering Research Council of Canada fellowships. This work was supported by the National Institutes of Health Grants R01 48958 (to T.A.), DP5OD009180 (to J.S.F.), GM073210, GM082250, and GM094625 and the US Department of Energy under Contract DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. NR 34 TC 23 Z9 23 U1 1 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 7 PY 2014 VL 111 IS 1 BP 237 EP 242 DI 10.1073/pnas.1302823110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 284VY UT WOS:000329350700069 PM 24363322 ER PT J AU Stavola, M Bekisli, F Yin, WK Smithe, K Fowler, WB Boatner, LA AF Stavola, Michael Bekisli, Figen Yin, Weikai Smithe, Kirby Fowler, W. Beall Boatner, Lynn A. TI Contrasting the experimental properties of hydrogen in SnO2, In2O3, and TiO2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ELECTRICAL-ACTIVITY; OXIDE MUONICS; RUTILE TIO2; ZINC-OXIDE; CRYSTALS; DONOR AB IR spectroscopy has been used to investigate the properties of H and D in single crystals of the transparent conducting oxides, SnO2, and In2O3. H introduces several O-H stretching lines and also the broad absorption arising from free carriers. IR spectroscopy has been used to identify the sources of n-type conductivity, its thermal stability, and the reactions of H-containing defects. The properties of OH and OD centers in TiO2, while studied for decades, reveal new surprises and properties that are in sharp contrast to the shallow, H-related donors seen in SnO2 and In2O3. Recent theory and EPR experiments find that electrons in TiO2 become self-trapped at Ti sites to form small polarons. The OD center in TiO2 shows a multiline vibrational spectrum with an unusual temperature dependence that can be explained by a small polaron model with the donor electron self-trapped at different Ti sites near the OD oscillator. (C) 2014 AIP Publishing LLC. C1 [Stavola, Michael; Bekisli, Figen; Yin, Weikai; Smithe, Kirby; Fowler, W. Beall] Lehigh Univ, Dept Phys, Bethlehem, PA 18015 USA. [Stavola, Michael; Bekisli, Figen; Yin, Weikai; Smithe, Kirby; Fowler, W. Beall] Lehigh Univ, Sherman Fairchild Lab, Bethlehem, PA 18015 USA. [Boatner, Lynn A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Stavola, M (reprint author), Lehigh Univ, Dept Phys, Bldg 16, Bethlehem, PA 18015 USA. EM mjsa@Lehigh.edu RI Boatner, Lynn/I-6428-2013 OI Boatner, Lynn/0000-0002-0235-7594 FU NSF [DMR-1160756]; Humboldt Foundation; U.S. Department of Energy, Basic Energy Sciences, and Materials Sciences and Engineering Division FX The work at Lehigh University was supported by NSF Grant No. DMR-1160756. M.S. is grateful for an Award for Senior U.S. Scientists from the Humboldt Foundation that supports visits to TU Dresden. The research of L.A.B. at the Oak Ridge National Laboratory was sponsored by the U.S. Department of Energy, Basic Energy Sciences, and Materials Sciences and Engineering Division. NR 42 TC 7 Z9 7 U1 3 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 7 PY 2014 VL 115 IS 1 AR 012001 DI 10.1063/1.4837955 PG 5 WC Physics, Applied SC Physics GA 286GZ UT WOS:000329456300001 ER PT J AU Moussa, JE AF Moussa, Jonathan E. TI Cubic-scaling algorithm and self-consistent field for the random-phase approximation with second-order screened exchange SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL APPROXIMATIONS; PLESSET PERTURBATION-THEORY; ATOMIC ORBITAL BASIS; ELECTRON-GAS; CORRELATION ENERGY; LARGE MOLECULES; BASIS-SET; SYSTEMS; MODEL; CHEMISTRY AB The random-phase approximation with second-order screened exchange (RPA+SOSEX) is a model of electron correlation energy with two caveats: its accuracy depends on an arbitrary choice of mean field, and it scales as O(n(5)) operations and O(n(3)) memory for n electrons. We derive a new algorithm that reduces its scaling to O(n(3)) operations and O(n(2)) memory using controlled approximations and a new self-consistent field that approximates Brueckner coupled-cluster doubles theory with RPA+SOSEX, referred to as Brueckner RPA theory. The algorithm comparably reduces the scaling of second-order Moller-Plesset perturbation theory with smaller cost prefactors than RPA+SOSEX. Within a semiempirical model, we study H-2 dissociation to test accuracy and H-n rings to verify scaling. (C) 2014 AIP Publishing LLC. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Moussa, JE (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM godotalgorithm@gmail.com FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX I thank Jay Sau, Norm Tubman, Jeff Hammond, Andrew Baczewski, Rick Muller, and Toby Jacobson for discussions. I thank Andrew Baczewski for checking the mathematics and proofreading the manuscript. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 81 TC 13 Z9 13 U1 1 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 7 PY 2014 VL 140 IS 1 AR 014107 DI 10.1063/1.4855255 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 285PW UT WOS:000329407100011 PM 24410221 ER PT J AU Trimithioti, M Akimov, AV Prezhdo, OV Hayes, SC AF Trimithioti, Marilena Akimov, Alexey V. Prezhdo, Oleg V. Hayes, Sophia C. TI Analysis of depolarization ratios of ClNO2 dissolved in methanol SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RESONANCE RAMAN INTENSITIES; MOLECULAR-DYNAMICS SIMULATIONS; ELECTRONIC-STATE STRUCTURES; EXCITATION PROFILES; EXCITED-STATES; SOLVATION DYNAMICS; FERROCYTOCHROME-C; NITRYL CHLORIDE; 235 NM; PHOTODISSOCIATION AB A detailed analysis of the resonance Raman depolarization ratio dispersion curve for the N-O symmetric stretch of nitryl chloride in methanol at excitation wavelengths spanning the D absorption band is presented. The depolarization ratios are modeled using the time-dependent formalism for Raman scattering with contributions from two excited states (2(1)A1 and 3(1)B1), which are taken as linearly dissociative along the Cl-N coordinate. The analysis focuses on the interplay between different types of broadening revealing the importance of inhomogenous broadening in determining the relative contributions of the two electronic transitions. We find that the transition dipole moment (M) for 21A1 is greater than for 31B1, in agreement with gas phase calculations in the literature [A. Lesar, M. Hdoscek, M. Muhlhauser, and S. D. Peyerimhoff, Chem. Phys. Lett. 383, 84 (2004)]. However, we find that the polarity of the solvent influences the excited state energetics, leading to a reversal in the ordering of these two states with 31B1 shifting to lower energies. Molecular dynamics simulations along with linear response and ab initio calculations support the evidence extracted from resonance Raman intensity analysis, providing insights on ClNO2 electronic structure, solvation effects in methanol, and the source of broadening, emphasizing the importance of a contribution from inhomogeneous linewidth. (C) 2014 AIP Publishing LLC. C1 [Trimithioti, Marilena; Hayes, Sophia C.] Univ Cyprus, Dept Chem, CY-1678 Nicosia, Cyprus. [Akimov, Alexey V.; Prezhdo, Oleg V.] Univ Rochester, Dept Chem, Rochester, NY 14627 USA. [Akimov, Alexey V.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Hayes, SC (reprint author), Univ Cyprus, Dept Chem, POB 20537, CY-1678 Nicosia, Cyprus. EM shayes@ucy.ac.cy RI Akimov, Alexey/H-9547-2014 FU Cyprus Research Promotion Foundation [PENEK/ENISX/0508/19, KY-GA/0907/07]; Computational Materials and Chemical Sciences Network (CMCSN) project at Brookhaven National Laboratory [DE-AC02-98CH10886]; U.S. Department of Energy; Division of Chemical Sciences, Geosciences & Biosciences, Office of Basic Energy Sciences; U.S. Department of Energy [DE-SC0006527]; Republic of Cyprus; European fund for regional development of the European Union FX M.T. and S. C. H. gratefully acknowledge funding from the Cyprus Research Promotion Foundation, grant PENEK/ENISX/0508/19 and KY-GA/0907/07. The funds for the grant involve contributions from the Republic of Cyprus and the European fund for regional development of the European Union. A. V. A. was funded by the Computational Materials and Chemical Sciences Network (CMCSN) project at Brookhaven National Laboratory under contract DE-AC02-98CH10886 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Geosciences & Biosciences, Office of Basic Energy Sciences. O.V.P. acknowledges financial support from the U.S. Department of Energy, grant DE-SC0006527. The authors would like to acknowledge helpful discussions with Anne Myers Kelly and Soren Hassing, and would like to thank Antonjia Lesar for making available the results from electronic structure calculations for Fig. 3, as well as Christophe Jouvet for preliminary calculations. NR 72 TC 0 Z9 0 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 7 PY 2014 VL 140 IS 1 AR 014301 DI 10.1063/1.4854055 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 285PW UT WOS:000329407100013 PM 24410223 ER PT J AU Waters, SM Mccoy, JD Frischknecht, AL Brown, JR AF Waters, Sara M. McCoy, John D. Frischknecht, Amalie L. Brown, Jonathan R. TI Simulation of a small molecule analogue of a lithium ionomer in an external electric field SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SULFONATED POLYSTYRENE IONOMERS; ETHYLENE IONOMERS; PRECISE IONOMERS; CATION TYPE; DYNAMICS; MORPHOLOGY; RELAXATIONS; MODEL; MELTS AB We have investigated the ion dynamics in lithium-neutralized 2-pentylheptanoic acid, a small molecule analogue of a precise poly(ethylene-co-acrylic acid) lithium ionomer. Atomistic molecular dynamics simulations were performed in an external electric field. The electric field causes alignment of the ionic aggregates along the field direction. The energetic response of the system to an imposed oscillating electric field for a wide range of frequencies was tracked by monitoring the coulombic contribution to the energy. The susceptibility found in this manner is a component of the dielectric susceptibility typically measured experimentally. A dynamic transition is found and the frequency associated with this transition varies with temperature in an Arrhenius manner. The transition is observed to be associated with rearrangements of the ionic aggregates. (C) 2014 AIP Publishing LLC. C1 [Waters, Sara M.; McCoy, John D.; Brown, Jonathan R.] New Mexico Inst Min & Technol, Dept Mat Engn, Socorro, NM 87801 USA. [Frischknecht, Amalie L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mccoy, JD (reprint author), New Mexico Inst Min & Technol, Dept Mat Engn, Socorro, NM 87801 USA. EM mccoy@nmt.edu RI McCoy, John/B-3846-2010; Frischknecht, Amalie/N-1020-2014 OI McCoy, John/0000-0001-5404-1404; Frischknecht, Amalie/0000-0003-2112-2587 FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. We thank Dan Bolintineanu for assistance with the structure analysis, and Dan Bolintineanu and Mark Stevens for helpful discussions. NR 38 TC 6 Z9 6 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 7 PY 2014 VL 140 IS 1 AR 014902 DI 10.1063/1.4855715 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 285PW UT WOS:000329407100027 PM 24410237 ER PT J AU Huang, GY Kim, JJ Reger, AS Lorenz, R Moon, EW Zhao, C Casteel, DE Bertinetti, D VanSchouwen, B Selvaratnam, R Pflugrath, JW Sankaran, B Melacini, G Herberg, FW Kim, C AF Huang, Gilbert Y. Kim, Jeong Joo Reger, Albert S. Lorenz, Robin Moon, Eui-Whan Zhao, Chi Casteel, Darren E. Bertinetti, Daniela VanSchouwen, Bryan Selvaratnam, Rajeevan Pflugrath, James W. Sankaran, Banumathi Melacini, Giuseppe Herberg, Friedrich W. Kim, Choel TI Structural Basis for Cyclic-Nucleotide Selectivity and cGMP-Selective Activation of PKG I SO STRUCTURE LA English DT Article ID DEPENDENT PROTEIN-KINASE; NITRIC-OXIDE; REGULATORY SUBUNIT; CRYSTAL-STRUCTURE; CAMP; BINDING; BETA; REVEALS; DOMAIN; MODEL AB Cyclic guanosine monophosphate (cGMP) and cyclic AMP (cAMP)-dependent protein kinases (PKG and PKA) are closely related homologs, and the cyclic nucleotide specificity of each kinase is crucial for keeping the two signaling pathways segregated, but the molecular mechanism of cyclic nucleotide selectivity is unknown. Here, we report that the PKG I beta C-terminal cyclic nucleotide binding domain (CNB-B) is highly selective for cGMP binding, and we have solved crystal structures of CNB-B with and without bound cGMP. These structures, combined with a comprehensive mutagenic analysis, allowed us to identify Leu296 and Arg297 as key residues that mediate cGMP selectivity. In addition, by comparing the cGMP bound and unbound structures, we observed large conformational changes in the C-terminal helices in response to cGMP binding, which were stabilized by recruitment of Tyr351 as a "capping residue" for cGMP. The observed rearrangements of the C-terminal helices provide a mechanical insight into release of the catalytic domain and kinase activation. C1 [Huang, Gilbert Y.; Kim, Choel] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Kim, Jeong Joo; Reger, Albert S.; Moon, Eui-Whan; Kim, Choel] Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA. [Lorenz, Robin; Bertinetti, Daniela; Herberg, Friedrich W.] Univ Kassel, Dept Biochem, D-34132 Kassel, Germany. [Zhao, Chi] Rice Univ, Dept Chem, Houston, TX 77005 USA. [Casteel, Darren E.] Univ Calif San Diego, Dept Med, La Jolla, CA 92093 USA. [VanSchouwen, Bryan; Selvaratnam, Rajeevan; Melacini, Giuseppe] McMaster Univ, Dept Chem & Chem Biol, Hamilton, ON L8S 4M1, Canada. [Pflugrath, James W.] Rigaku Amer, The Woodlands, TX 77381 USA. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley tr Struct Biol, Berkeley, CA 94720 USA. RP Kim, C (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. EM ckim@bcm.edu RI Herberg, Friedrich/B-5572-2015; Bertinetti, Daniela/B-5655-2015 OI Herberg, Friedrich/0000-0001-7117-7653; FU National Institutes of Health (NIH) [RO1 GM090161]; BCM seed grant; Houston Area Molecular Biophysics Program, National Institute of General Medical Science [T32GM008280]; Canadian Institute of Health Research; European Union grant "Affinomics" [222635]; Federal Ministry of Education and Research Project "No Pain" [FKZ0316177F] FX We thank K. Sippel, M. Zhou, C. Peters, C.J. Lim, A. Koyfman, and S.S. Taylor for critical reading of the manuscript. We also thank E. Franz (University of Kassel) for expert technical assistance, S.R. Wasserman (Eli Lilly Beam line, APS) for his assistance with data collection, and S. Badal and F. Danesh (Baylor College of Medicine [BCMD for their assistance with HEK293T culture. C.K. is funded by National Institutes of Health (NIH) grant RO1 GM090161 and a BCM seed grant. G.Y.H. is supported by the Houston Area Molecular Biophysics Program, National Institute of General Medical Science grant no. T32GM008280. G.M. is funded by the Canadian Institute of Health Research. F.W.H. is supported in part by European Union grant "Affinomics" (Contract 222635) and the Federal Ministry of Education and Research Project "No Pain" (FKZ0316177F). The Berkeley Center for Structural Biology is supported in part by the NIH, the National Institute of General Medical Sciences, and the Howard Hughes Medical Institute. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-ACO2-05CH11231. NR 40 TC 13 Z9 13 U1 0 U2 6 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD JAN 7 PY 2014 VL 22 IS 1 BP 116 EP 124 DI 10.1016/j.str.2013.09.021 PG 9 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA 288DU UT WOS:000329593000013 PM 24239458 ER PT J AU Datskos, P Sharma, J AF Datskos, Panos Sharma, Jaswinder TI Synthesis of Segmented Silica Rods by Regulation of the Growth Temperature SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE colloids; growth regulation; segmented rods; silicates; temperature control ID REVERSE MICELLES; TRITON X-100; SHAPE; CYCLOHEXANE; PARTICLES; COMPLEX; WATER AB The control of the diameter of colloidal structures is of fundamental interest and practical importance. We synthesized segmented silica rods by regulating the reaction temperature while the rods were growing. With higher growth temperatures, the segment diameter became smaller. Longer incubation times gave longer segments at the same temperature. Similarly, high temperature for the same incubation time gave longer segments. It appears that the correlation between temperature and diameter results from the relation between temperature and the size of the emulsion droplet, that is, the higher the temperature, the smaller the emulsion droplet. C1 [Datskos, Panos; Sharma, Jaswinder] Oak Ridge Natl Lab, Nanosyst Separat & Mat Res Grp, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. Ctr Nanophase Mat Sci, Oak Ridge, TN USA. RP Sharma, J (reprint author), Oak Ridge Natl Lab, Nanosyst Separat & Mat Res Grp, Energy & Transportat Sci Div, 1 Bethel Valley Rd,MS 6054, Oak Ridge, TN 37831 USA. EM sharmajk@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX J. Sharma is a Eugene P. Wigner Fellow at the Oak Ridge National Laboratory managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract DE-AC05-00OR22725. The work was supported by the Laboratory Director's Research and Development Program of the Oak Ridge National Laboratory. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 18 TC 12 Z9 12 U1 7 U2 65 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 7 PY 2014 VL 53 IS 2 BP 451 EP 454 DI 10.1002/anie.201308140 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 282EH UT WOS:000329152600015 PM 24272918 ER PT J AU Vjunov, A Hu, MY Feng, J Camaioni, DM Mei, DH Hu, JZ Zhao, C Lercher, JA AF Vjunov, Aleksei Hu, Mary Y. Feng, Ju Camaioni, Donald M. Mei, Donghai Hu, Jian Z. Zhao, Chen Lercher, Johannes A. TI Following Solid-Acid-Catalyzed Reactions by MAS NMR Spectroscopy in Liquid Phase-Zeolite-Catalyzed Conversion of Cyclohexanol in Water SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE alcohol dehydration; heterogeneous catalysis; NMR spectroscopy; reaction mechanisms; zeolites ID NUCLEAR-MAGNETIC-RESONANCE; SPACE GAUSSIAN PSEUDOPOTENTIALS; IN-SITU; ALCOHOL DEHYDRATION; HIGH-TEMPERATURE; DIMETHYL ETHER; HYDRODEOXYGENATION; ADSORPTION; HYDROALKYLATION; METHANOL AB A microautoclave magic angle spinning NMR rotor is developed enabling insitu monitoring of solid-liquid-gas reactions at high temperatures and pressures. It is used in a kinetic and mechanistic study of the reactions of cyclohexanol on zeolite HBEA in 130 degrees C water. The (13)Cspectra show that dehydration of 1-C-13-cyclohexanol occurs with significant migration of the hydroxy group in cyclohexanol and the double bond in cyclohexene with respect to the C-13 label. A simplified kinetic model shows the E1-type elimination fully accounts for the initial rates of 1-C-13-cyclohexanol disappearance and the appearance of the differently labeled products, thus suggesting that the cyclohexyl cation undergoes a 1,2-hydride shift competitive with rehydration and deprotonation. Concurrent with the dehydration, trace amounts of dicyclohexyl ether are observed, and in approaching equilibrium, a secondary product, cyclohexyl-1-cyclohexene is formed. Compared to phosphoric acid, HBEA is shown to be a more active catalyst exhibiting a dehydration rate that is 100-fold faster per proton. C1 [Vjunov, Aleksei; Hu, Mary Y.; Feng, Ju; Camaioni, Donald M.; Mei, Donghai; Hu, Jian Z.; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Zhao, Chen; Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85748 Garching, Germany. [Zhao, Chen; Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Inst, D-85748 Garching, Germany. [Vjunov, Aleksei; Hu, Mary Y.; Feng, Ju; Camaioni, Donald M.; Mei, Donghai; Hu, Jian Z.; Zhao, Chen; Lercher, Johannes A.] Environm Mol Sci Lab, Richland, WA USA. RP Lercher, JA (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM johannes.lercher@pnnl.gov RI Mei, Donghai/A-2115-2012; Mei, Donghai/D-3251-2011; Hu, Jian Zhi/F-7126-2012 OI Mei, Donghai/0000-0002-0286-4182; FU U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; DOE by Battelle Memorial Institute [DE-AC06-76L0-1830] FX We thank Zizwe A. Chase and Junming Sun (both from Washington State University) for pretreating the catalyst. C. F. Peden is acknowledged for his support in developing the NMR capability. This work was supported by the U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. All experiments were performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for DOE by Battelle Memorial Institute under Contract no. DE-AC06-76L0-1830. NR 43 TC 21 Z9 21 U1 30 U2 172 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 7 PY 2014 VL 53 IS 2 BP 479 EP 482 DI 10.1002/anie.201306673 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 282EH UT WOS:000329152600021 PM 24282024 ER PT J AU Tian, J Ding, YD Zhou, TY Zhang, KD Zhao, X Wang, H Zhang, DW Liu, Y Li, ZT AF Tian, Jia Ding, Yu-Di Zhou, Tian-You Zhang, Kang-Da Zhao, Xin Wang, Hui Zhang, Dan-Wei Liu, Yi Li, Zhan-Ting TI Self-Assembly of Three-Dimensional Supramolecular Polymers through Cooperative Tetrathiafulvalene Radical Cation Dimerization SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE dimerization; radical cations; stacking interactions; supramolecular polymers; tetrathiafulvalene ID METAL-ORGANIC FRAMEWORKS; MIXED-VALENCE; ELECTRON-TRANSFER; ROOM-TEMPERATURE; CHARGE-TRANSFER; DONOR-ACCEPTOR; FUNCTIONAL MATERIALS; BLOCK-COPOLYMERS; DIMER STATES; PI-DIMERS AB The self-assembly of a new type of three-dimensional (3D) supramolecular polymers from tetrahedral monomers in both organic and aqueous media is described. We have designed and synthesized two tetraphenylmethane derivatives T1 and T2, both of which bear four tetrathiafulvalene (TTF) units. When the TTF units were oxidized to the radical cation TTF center dot+, their pre-organized tetrahedral arrangement remarkably enhanced their intermolecular dimerization, leading to the formation of new 3D spherical supramolecular polymers. The structure of the supramolecular polymers has been inferred on the basis of UV/Vis absorption, electron paramagnetic resonance, cyclic voltammetry, and dynamic light scattering (DLS) analysis, as well as by comparing these properties with those of the self-assembled structures of mono-, di-, and tritopic control compounds. DLS experiments revealed that the spherical supramolecular polymers had hydrodynamic diameters of 68 nm for T1 (75 mu m) in acetonitrile and 105 nm for T2 (75 mu m) in water/acetonitrile (1:1). The 3D spherical structures of the supramolecular polymers formed in different solvents were also supported by SEM and AFM experiments. C1 [Tian, Jia; Ding, Yu-Di; Wang, Hui; Zhang, Dan-Wei; Li, Zhan-Ting] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. [Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zhou, Tian-You; Zhang, Kang-Da; Zhao, Xin] Chinese Acad Sci, Shanghai Inst Organ Chem, Shanghai 200032, Peoples R China. RP Wang, H (reprint author), Fudan Univ, Dept Chem, 220 Handan Rd, Shanghai 200433, Peoples R China. EM wanghui@fudan.edu.cn; yliu@lbl.gov; ztli@fudan.edu.cn RI Zhang, Kang-Da/K-4546-2013; Liu, yi/A-3384-2008; Tian, Jia/O-2758-2014; Foundry, Molecular/G-9968-2014 OI Liu, yi/0000-0002-3954-6102; Tian, Jia/0000-0001-6793-2804; FU Ministry of Science and Technology [2013CB834501]; Ministry of Education [IRT1117]; Science and Technology Commission of Shanghai Municipality [13NM1400200]; National Natural Science Foundation of China [91227108, 21228203, J1103304] FX We thank the Ministry of Science and Technology (2013CB834501), the Ministry of Education (IRT1117), the Science and Technology Commission of Shanghai Municipality (13NM1400200), and the National Natural Science Foundation of China (91227108, 21228203, and J1103304) for financial support of this work. NR 99 TC 22 Z9 25 U1 6 U2 81 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JAN 7 PY 2014 VL 20 IS 2 BP 575 EP 584 DI 10.1002/chem.201302951 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 282TW UT WOS:000329197500031 PM 24302551 ER PT J AU Guttormsen, M Bernstein, LA Gorgen, A Jurado, B Siem, S Aiche, M Ducasse, Q Giacoppo, F Gunsing, F Hagen, TW Larsen, AC Lebois, M Leniau, B Renstrom, T Rose, SJ Tornyi, TG Tveten, GM Wiedeking, M Wilson, JN AF Guttormsen, M. Bernstein, L. A. Gorgen, A. Jurado, B. Siem, S. Aiche, M. Ducasse, Q. Giacoppo, F. Gunsing, F. Hagen, T. W. Larsen, A. C. Lebois, M. Leniau, B. Renstrom, T. Rose, S. J. Tornyi, T. G. Tveten, G. M. Wiedeking, M. Wilson, J. N. TI Scissors resonance in the quasicontinuum of Th, Pa, and U isotopes SO PHYSICAL REVIEW C LA English DT Article ID MAGNETIC DIPOLE STRENGTH; ACTINIDE NUCLEI; CROSS-SECTIONS; LEVEL DENSITY; SPECTRA; TH-232; U-238; MODEL; DEFORMATION; EXCITATIONS AB The gamma-ray strength function in the quasicontinuum has been measured for Th231-233, Pa-232,Pa-233, and U237-239 using the Oslo method. All eight nuclei show a pronounced increase in gamma strength at omega(SR) approximate to 2.4 MeV, which is interpreted as the low-energy M1 scissors resonance (SR). The total strength is found to be B-SR = 9-11 mu(2)(N) when integrated over the 1-4 MeV gamma-energy region. The SR displays a double-hump structure that is theoretically not understood. Our results are compared with data from (gamma, gamma') experiments and theoretical sum-rule estimates for a nuclear rigid-body moment of inertia. C1 [Guttormsen, M.; Gorgen, A.; Siem, S.; Giacoppo, F.; Hagen, T. W.; Larsen, A. C.; Renstrom, T.; Rose, S. J.; Tornyi, T. G.; Tveten, G. M.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Bernstein, L. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Jurado, B.; Aiche, M.; Ducasse, Q.] Univ Bordeaux, CENBG, CNRS IN2P3, F-33175 Gradignan, France. [Gunsing, F.] CEA Saclay, DSM Irfu SPhN, F-91191 Gif Sur Yvette, France. [Lebois, M.; Leniau, B.; Wilson, J. N.] Inst Phys Nucl Orsay, F-91406 Orsay, France. [Tornyi, T. G.] Hungarian Acad Sci, MTA Atomki, Inst Nucl Res, Debrecen, Hungary. [Wiedeking, M.] iThemba LABS, Somerset West, South Africa. RP Guttormsen, M (reprint author), Univ Oslo, Dept Phys, N-0316 Oslo, Norway. EM magne.guttormsen@fys.uio.no RI Larsen, Ann-Cecilie/C-8742-2014; OI Larsen, Ann-Cecilie/0000-0002-2188-3709; Tveten, Gry Merete/0000-0002-6942-8254; Gorgen, Andreas/0000-0003-1916-9941 FU Research Council of Norway (NFR); French national research programme GEDEPEON; U.S. Department of Energy [DE-AC52-07NA27344]; National Research Foundation of South Africa; European Commission [269499]; European Atomic Energy Community [FP7-249671] FX We would like to thank J. C. Muller, E. A. Olsen, A. Semchenkov and J. Wikne at the Oslo Cyclotron Laboratory for providing the stable and high-quality deuterium and 3He beams during the experiment, the Lawrence Livermore National Laboratory for providing the 232Th target and the GSI Target Laboratory for the production of the 238U target. We thank A. A. Kuliev, E. Guliyev and F. Ertugral for sharing details of their QRPA calculations. This work was supported by the Research Council of Norway (NFR), the French national research programme GEDEPEON, the U.S. Department of Energy under Contract No. DE-AC52-07NA27344, the National Research Foundation of South Africa, the European Commission within the 7th Framework Programme through Fission-2010-ERINDA (Project No. 269499) and by the European Atomic Energy Communitys 7th Framework Programme under Grant Agreement No. FP7-249671 (ANDES). NR 45 TC 16 Z9 16 U1 1 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 6 PY 2014 VL 89 IS 1 AR 014302 DI 10.1103/PhysRevC.89.014302 PG 11 WC Physics, Nuclear SC Physics GA AB9XL UT WOS:000332148900004 ER PT J AU Farago, O Gronbech-Jensen, N AF Farago, Oded Gronbech-Jensen, Niels TI Langevin dynamics in inhomogeneous media: Re- examining the Ito-Stratonovich dilemma SO PHYSICAL REVIEW E LA English DT Article ID FLUCTUATION-DISSIPATION THEOREM AB The diffusive dynamics of a particle in amedium with space-dependent friction coefficient is studied within the framework of the inertial Langevin equation. In this description, the ambiguous interpretation of the stochastic integral, known as the Ito-Stratonovich dilemma, is avoided since all interpretations converge to the same solution in the limit of small time steps. We use a newly developed method for Langevin simulations to measure the probability distribution of a particle diffusing in a flat potential. Our results reveal that both the Ito and Stratonovich interpretations converge very slowly to the uniform equilibrium distribution for vanishing time step sizes. Three other conventions exhibit significantly improved accuracy: (i) the "isothermal" (Hanggi) convention, (ii) the Stratonovich convention corrected by a drift term, and (iii) a newly proposed convention employing two different effective friction coefficients representing two different averages of the friction function during the time step. We argue that the most physically accurate dynamical description is provided by the third convention, in which the particle experiences a drift originating from the dissipation instead of the fluctuation term. This feature is directly related to the fact that the drift is a result of an inertial effect that cannot be well understood in the Brownian, overdamped limit of the Langevin equation. C1 [Farago, Oded; Gronbech-Jensen, Niels] Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. [Farago, Oded] Ben Gurion Univ Negev, Dept Biomed Engn, IL-84105 Beer Sheva, Israel. [Farago, Oded] Ben Gurion Univ Negev, Ilse Katz Inst Nanoscale Sci & Technol, IL-84105 Beer Sheva, Israel. [Gronbech-Jensen, Niels] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Gronbech-Jensen, Niels] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Farago, O (reprint author), Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. FU U.S. Department of Energy [DE-NE0000536000.] FX O.F. acknowledges Tamir Kamai for discussions on the Ito-Stratonovich dilemma. This project was supported in part by the U.S. Department of Energy Project No. DE-NE0000536000. NR 18 TC 13 Z9 13 U1 4 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 6 PY 2014 VL 89 IS 1 AR 013301 DI 10.1103/PhysRevE.89.013301 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AC0AA UT WOS:000332155800015 PM 24580354 ER PT J AU Jacob, RE Carson, JP AF Jacob, Richard E. Carson, James P. TI Automated measurement of heterogeneity in CT images of healthy and diseased rat lungs using variogram analysis of an octree decomposition SO BMC MEDICAL IMAGING LA English DT Article DE Lung imaging; Disease detection; COPD; Emphysema; Pulmonary; Octree; Variogram ID FRACTAL ANALYSIS; COMPUTED-TOMOGRAPHY; PULMONARY-EMPHYSEMA; QUANTIFICATION; ABNORMALITIES; DENSITOMETRY; FLOW; TOOL; MRI AB Background: Assessing heterogeneity in lung images can be an important diagnosis tool. We present a novel and objective method for assessing lung damage in a rat model of emphysema. We combined a three-dimensional (3D) computer graphics method-octree decomposition-with a geostatistics-based approach for assessing spatial relationships-the variogram-to evaluate disease in 3D computed tomography (CT) image volumes. Methods: Male, Sprague-Dawley rats were dosed intratracheally with saline (control), or with elastase dissolved in saline to either the whole lung (for mild, global disease) or a single lobe (for severe, local disease). Gated 3D micro-CT images were acquired on the lungs of all rats at end expiration. Images were masked, and octree decomposition was performed on the images to reduce the lungs to homogeneous blocks of 2 x 2 x 2, 4 x 4 x 4, and 8 x 8 x 8 voxels. To focus on lung parenchyma, small blocks were ignored because they primarily defined boundaries and vascular features, and the spatial variance between all pairs of the 8 x 8 x 8 blocks was calculated as the square of the difference of signal intensity. Variograms-graphs of distance vs. variance-were constructed, and results of a least-squares-fit were compared. The robustness of the approach was tested on images prepared with various filtering protocols. Statistical assessment of the similarity of the three control rats was made with a Kruskal-Wallis rank sum test. A Mann-Whitney-Wilcoxon rank sum test was used to measure statistical distinction between individuals. For comparison with the variogram results, the coefficient of variation and the emphysema index were also calculated for all rats. Results: Variogram analysis showed that the control rats were statistically indistinct (p = 0.12), but there were significant differences between control, mild global disease, and severe local disease groups (p < 0.0001). A heterogeneity index was calculated to describe the difference of an individual variogram from the control average. This metric also showed clear separation between dose groups. The coefficient of variation and the emphysema index, on the other hand, did not separate groups. Conclusion: These results suggest the octree decomposition and variogram analysis approach may be a rapid, non-subjective, and sensitive imaging-based biomarker for characterizing lung disease. C1 [Jacob, Richard E.; Carson, James P.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Jacob, RE (reprint author), Pacific NW Natl Lab, Div Biol Sci, 902 Battelle Blvd, Richland, WA 99352 USA. EM richard.jacob@pnnl.gov RI Zheng, Rong/F-1641-2016 FU National Heart, Lung, and Blood Institute [R01HL073598]; PNNL through internal Laboratory Directed Research and Development LDRD [DE-AC05-76RL01830] FX The authors would like to thank T. Curry of PNNL for assistance with animal handling and B. Amidan of PNNL for helpful discussions. This project was supported by Award Number R01HL073598 from the National Heart, Lung, and Blood Institute and by PNNL through internal Laboratory Directed Research and Development LDRD DE-AC05-76RL01830. There was no involvement on the part of the sponsors in study design; in the collection, analysis, and interpretation of data; in the writing of the report; or in the decision to submit the paper for publication. NR 38 TC 3 Z9 3 U1 1 U2 11 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2342 J9 BMC MED IMAGING JI BMC Med. Imag. PD JAN 6 PY 2014 VL 14 AR 1 DI 10.1186/1471-2342-14-1 PG 11 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA AB8ZK UT WOS:000332078500001 PM 24393332 ER PT J AU Ahmed, T Albers, RC Balatsky, AV Friedrich, C Zhu, JX AF Ahmed, Towfiq Albers, R. C. Balatsky, A. V. Friedrich, C. Zhu, Jian-Xin TI GW quasiparticle calculations with spin-orbit coupling for the light actinides SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-STRUCTURE; PLUTONIUM; SPECTRA; SYSTEMS AB We report on the importance of GW self-energy corrections for the electronic structure of light actinides in the weak-to-intermediate coupling regime. Our study is based on calculations of the band structure and total density of states of Np, U, and Pu using a one-shot GW approximation that includes spin-orbit coupling within a full potential LAPW framework. We also present RPA screened effective Coulomb interactions for the f-electron orbitals for different lattice constants, and show that there is an increased contribution from electron-electron correlation in these systems for expanded lattices. We find a significant amount of electronic correlation in these highly localized electronic systems. C1 [Ahmed, Towfiq; Albers, R. C.; Balatsky, A. V.; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Balatsky, A. V.; Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Balatsky, A. V.] KTH Royal Inst Technol, NORDITA, S-10691 Stockholm, Sweden. [Balatsky, A. V.] Stockholm Univ, S-10691 Stockholm, Sweden. [Friedrich, C.] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany. [Friedrich, C.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Friedrich, C.] JARA, D-52425 Julich, Germany. RP Zhu, JX (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jxzhu@lanl.gov RI Friedrich, Christoph/L-5029-2013 OI Friedrich, Christoph/0000-0002-3315-7536 FU U.S. DOE at LANL [DE-AC52-06NA25396]; LANL LDRD Program; Europe VR Program FX We thank A. Svane, N. E. Christensen, M. van Schilfgaarde, and A. N. Chantis for useful discussions and collaboration on related work. This work was supported by U.S. DOE at LANL under Contract No. DE-AC52-06NA25396, the LANL LDRD Program (T.A., R.C.A. & J.-X.Z.), and the Europe VR Program (A.V.B.). NR 39 TC 5 Z9 5 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 6 PY 2014 VL 89 IS 3 AR 035104 DI 10.1103/PhysRevB.89.035104 PG 6 WC Physics, Condensed Matter SC Physics GA AC0IE UT WOS:000332177200002 ER PT J AU Liu, XJ Wang, CZ Hupalo, M Lin, HQ Ho, KM Tringides, MC AF Liu, Xiaojie Wang, Cai-Zhuang Hupalo, Myron Lin, Hai-Qing Ho, Kai-Ming Tringides, Michael C. TI Quantum confinement induced oscillatory electric field on a stepped Pb(111) film and its influence on surface reactivity SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; WORK FUNCTION; METAL-FILMS AB When the thickness of ultrathin metal films approaches the nanometer scale comparable to the coherence length of the electrons, significant effects on the structure stability and the electronic properties of the metal films emerge due to electron confinement and quantization of the allowed electronic states in the direction perpendicular to the film. Using first-principles calculations, we showed that such quantum size effects can induce oscillatory electrostatic potential and thus alternating electric field on the surface of the wedge-shaped Pb(111) films. The alternating electric field has significant influence on surface reactivity, leading to selective even- or odd-layer adsorption preference depending on the charge state of the adatoms, consistent with the odd-layer preference of higher Mg coverage on wedge-shaped Pb(111) films, as observed in experiment. C1 [Liu, Xiaojie; Lin, Hai-Qing] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Liu, Xiaojie; Wang, Cai-Zhuang; Hupalo, Myron; Ho, Kai-Ming; Tringides, Michael C.] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Liu, Xiaojie; Wang, Cai-Zhuang; Hupalo, Myron; Ho, Kai-Ming; Tringides, Michael C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Liu, XJ (reprint author), Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. EM wangcz@ameslab.gov; haiqing0@csrc.ac.cn FU U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358] FX Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, including a grant of computer time at the National Energy Research Scientific Computing Center (NERSC) in Berkeley, CA under Contract No. DE-AC02-07CH11358. NR 22 TC 3 Z9 3 U1 1 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 6 PY 2014 VL 89 IS 4 AR 041401 DI 10.1103/PhysRevB.89.041401 PG 5 WC Physics, Condensed Matter SC Physics GA AC0IG UT WOS:000332177400002 ER PT J AU Rout, PK Pandey, H Wu, LJ Anupam Joshi, PC Hossain, Z Zhu, YM Budhani, RC AF Rout, P. K. Pandey, Himanshu Wu, Lijun Anupam Joshi, P. C. Hossain, Z. Zhu, Yimei Budhani, R. C. TI Two-dimensional electron-gas-like charge transport at the interface between a magnetic Heusler alloy and SrTiO3 SO PHYSICAL REVIEW B LA English DT Article ID LAALO3/SRTIO3 INTERFACES; OXIDE HETEROSTRUCTURES; INSULATOR INTERFACE; STRONTIUM-TITANATE; MOTT INSULATOR; BAND INSULATOR; SUPERCONDUCTIVITY AB We report remarkably low residual resistivity, giant residual resistivity ratio, free-electron-like Hall resistivity, and high mobility (approximate to 10(4) cm(2) V-1 s(-1)) charge transport in epitaxial films of Co2MnSi and Co2FeSi grown on (001) SrTiO3. This unusual behavior is not observed in films deposited on other cubic oxide substrates of comparable lattice parameters. The scaling of the resistivity with thickness of the films allows the extraction of interface conductance, which can be attributed to a layer of oxygen vacancies confined within 1.9 nm of the interface as revealed by atomically resolved electron microscopy and spectroscopy. The high mobility transport observed here at the interface of a fully spin polarized metal is potentially important for spintronics applications. C1 [Rout, P. K.; Pandey, Himanshu; Anupam; Joshi, P. C.; Hossain, Z.; Budhani, R. C.] Indian Inst Technol, Dept Phys, Condensed Matter Low Dimens Syst Lab, Kanpur 208016, Uttar Pradesh, India. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Upton, NY 11973 USA. [Budhani, R. C.] CSIR, Natl Phys Lab, New Delhi 110012, India. RP Rout, PK (reprint author), Indian Inst Technol, Dept Phys, Condensed Matter Low Dimens Syst Lab, Kanpur 208016, Uttar Pradesh, India. EM rcb@iitk.ac.in RI Pandey, Himanshu/A-5862-2012 OI Pandey, Himanshu/0000-0002-7380-366X FU CSIR, India; DST FX The authors thank Hari Kishan, V. P. S. Awana, M. Shivkumar, and Nanosciences Centre (IIT Kanpur) for help in various measurements. Our thanks are also due to S. S. P. Parkin and Michael Pepper for valuable discussions. P. K. R. and H. P. acknowledge financial support from the CSIR, India. R. C. B. acknowledges the J. C. Bose Fellowship of DST. NR 37 TC 5 Z9 5 U1 2 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 6 PY 2014 VL 89 IS 2 AR 020401 DI 10.1103/PhysRevB.89.020401 PG 5 WC Physics, Condensed Matter SC Physics GA AC0HZ UT WOS:000332176700001 ER PT J AU Song, YK Gao, JH Liang, ZT Wang, XN AF Song, Yu-kun Gao, Jian-hua Liang, Zuo-tang Wang, Xin-nian TI Azimuthal asymmetries in semi-inclusive deep inelastic scattering with polarized beam and/or target and their nuclear dependences SO PHYSICAL REVIEW D LA English DT Article ID FINAL-STATE INTERACTIONS; MUON PROTON-SCATTERING; POWER CORRECTIONS; PARTON DISTRIBUTIONS; HADRONIC SCATTERING; SPIN ASYMMETRY; LEPTOPRODUCTION; MODEL; GAUGE; PIONS AB Using the formalism obtained from collinear expansion, we calculate the differential cross section and azimuthal asymmetries in the semi-inclusive deeply inelastic lepton-nucleon (nucleus) scattering process e(-) + N(A) -> e(-) + q + X with both polarized beam and polarized target up to twist-3. We derive the azimuthal asymmetries in terms of twist-3 parton correlation functions. We simplify the results by using the QCD equation of motion that leads to a set of relationships between different twist-3 functions. We further study the nuclear dependence of azimuthal asymmetries and show that they have similar suppression factors as those in the unpolarized reactions. C1 [Song, Yu-kun; Liang, Zuo-tang] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Song, Yu-kun] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Song, Yu-kun; Gao, Jian-hua; Wang, Xin-nian] Cent China Normal Univ, Minist Educ, Key Lab Quark & Lepton Phys, Wuhan, Peoples R China. [Gao, Jian-hua] Shandong Univ Weihai, Sch Space Sci & Phys, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Peoples R China. [Wang, Xin-nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Wang, Xin-nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Song, YK (reprint author), Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. RI Gao, Jianhua/O-9550-2014; OI Wang, Xin-Nian/0000-0002-9734-9967; Song, Yu-kun/0000-0003-1854-5167 FU National Natural Science Foundation of China [11035003, 11105137, 11221504]; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; CCNU-QLPL Innovation Fund [QLPL2011P01] FX This work was supported in part by the National Natural Science Foundation of China under Grants No. 11035003, No. 11105137, and No. 11221504 and by the Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by CCNU-QLPL Innovation Fund (QLPL2011P01). NR 64 TC 10 Z9 10 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 6 PY 2014 VL 89 IS 1 AR 014005 DI 10.1103/PhysRevD.89.014005 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AB5OB UT WOS:000331837000004 ER PT J AU Law, S Roberts, C Kilpatrick, T Yu, L Ribaudo, T Shaner, EA Podolskiy, V Wasserman, D AF Law, S. Roberts, C. Kilpatrick, T. Yu, L. Ribaudo, T. Shaner, E. A. Podolskiy, V. Wasserman, D. TI All-Semiconductor Negative-Index Plasmonic Absorbers SO PHYSICAL REVIEW LETTERS LA English DT Article ID REFRACTION AB We demonstrate epitaxially grown all-semiconductor thin-film midinfrared plasmonic absorbers and show that absorption in these structures is linked to the excitation of highly confined negative-index surface plasmon polaritons. Strong (>98%) absorption is experimentally observed, and the spectral position and intensity of the absorption resonances are studied by reflection and transmission spectroscopy. Numerical models as well as an analytical description of the excited guided modes in our structures are presented, showing agreement with experiment. The structures investigated demonstrate a wavelength-flexible, all-semiconductor, plasmonic architecture with potential for both sensing applications and enhanced interaction of midinfrared radiation with integrated semiconductor optoelectronic elements. C1 [Law, S.; Kilpatrick, T.; Yu, L.; Wasserman, D.] Univ Illinois, Dept Elect & Comp Engn, Micro & Nanotechnol Lab, Urbana, IL 61801 USA. [Roberts, C.; Podolskiy, V.] Univ Massachusetts, Dept Phys & Appl Phys, Lowell, MA 01854 USA. [Ribaudo, T.; Shaner, E. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Law, S (reprint author), Univ Illinois, Dept Elect & Comp Engn, Micro & Nanotechnol Lab, Urbana, IL 61801 USA. FU AFOSR Young Investigator Program [FA9550-10-1-0226]; NSF MWN program [DMR-1209761, DMR-1210398]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the AFOSR Young Investigator Program (Grant No. FA9550-10-1-0226) and the NSF MWN program (Grants No. DMR-1209761 and No. DMR-1210398). Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 24 TC 18 Z9 18 U1 5 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 6 PY 2014 VL 112 IS 1 AR 017401 DI 10.1103/PhysRevLett.112.017401 PG 5 WC Physics, Multidisciplinary SC Physics GA AB6YT UT WOS:000331936900009 PM 24483930 ER PT J AU Chern, GW Reichhardt, C Nisoli, C AF Chern, Gia-Wei Reichhardt, Charles Nisoli, Cristiano TI Realizing three-dimensional artificial spin ice by stacking planar nano-arrays SO APPLIED PHYSICS LETTERS LA English DT Article AB Artificial spin ice is a frustrated magnetic two-dimensional nano-material, recently employed to study variety of tailor-designed unusual collective behaviours. Recently proposed extensions to three dimensions are based on self-assembly techniques and allow little control over geometry and disorder. We present a viable design for the realization of a three-dimensional artificial spin ice with the same level of precision and control allowed by lithographic nano-fabrication of the popular two-dimensional case. Our geometry is based on layering already available two-dimensional artificial spin ice and leads to an arrangement of ice-rule-frustrated units, which is topologically equivalent to that of the tetrahedra in a pyrochlore lattice. Consequently, we show, it exhibits a genuine ice phase and its excitations are, as in natural spin ice materials, magnetic monopoles interacting via Coulomb law. (C) 2014 AIP Publishing LLC. C1 [Chern, Gia-Wei; Reichhardt, Charles; Nisoli, Cristiano] Los Alamos Natl Lab, Ctr Nonlinear Studies & Theoret Div, Los Alamos, NM 87545 USA. RP Chern, GW (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies & Theoret Div, POB 1663, Los Alamos, NM 87545 USA. OI Nisoli, Cristiano/0000-0003-0053-1023 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX We are grateful to J. Hollingsworth and S. Ivanov (Center for Integrated Nanotechnologies, LANL and Sandia) for useful discussions on nano-fabrication techniques, and Cynthia Olson Reichhardt for a critical reading of the manuscript. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 40 TC 7 Z9 7 U1 4 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 013101 DI 10.1063/1.4861118 PG 4 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800066 ER PT J AU Ding, J Cheng, YQ Ma, E AF Ding, J. Cheng, Y. Q. Ma, E. TI On the origin of elastic strain limit of bulk metallic glasses SO APPLIED PHYSICS LETTERS LA English DT Article ID MECHANICAL-BEHAVIOR; ORDER AB All bulk metallic glasses exhibit a large and almost universal elastic strain limit. Here, we show that the magnitude of the yield strain of the glass state can be quantitatively derived from a characteristic property of the flow state typical in running shear bands (the root cause of yielding). The strain in the shear flow is mostly plastic, but associated with it there is an effective elastic atomic strain. The latter is almost identical for very different model systems in our molecular dynamics simulations, such that the corresponding yield strain is universal at any given homologous temperature. (C) 2014 AIP Publishing LLC. C1 [Ding, J.; Ma, E.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. [Cheng, Y. Q.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Ding, J (reprint author), Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. EM ding@jhu.edu; ema@jhu.edu RI Ma, En/A-3232-2010; Cheng, Yongqiang/F-6567-2010; Ding, Jun/K-1989-2012 OI Ding, Jun/0000-0002-4091-8663 FU US National Science Foundation, Division of Materials Research [NSF-DMR-0904188]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the US National Science Foundation, Division of Materials Research, under Contract No. NSF-DMR-0904188. Y.Q.C was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 31 TC 7 Z9 7 U1 2 U2 76 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 011912 DI 10.1063/1.4861606 PG 4 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800030 ER PT J AU Hopkins, PE Duda, JC Kaehr, B Zhou, XW Yang, CYP Jones, RE AF Hopkins, Patrick E. Duda, John C. Kaehr, Bryan Zhou, Xiao Wang Yang, C. -Y. Peter Jones, Reese E. TI Ultrafast and steady-state laser heating effects on electron relaxation and phonon coupling mechanisms in thin gold films (vol 103, 211910, 2013) SO APPLIED PHYSICS LETTERS LA English DT Correction C1 [Hopkins, Patrick E.; Duda, John C.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Duda, John C.] Seagate Technol, Bloomington, MN 55435 USA. [Kaehr, Bryan] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. [Kaehr, Bryan] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87106 USA. [Zhou, Xiao Wang; Yang, C. -Y. Peter; Jones, Reese E.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Hopkins, PE (reprint author), Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. EM phopkins@virginia.edu NR 1 TC 0 Z9 0 U1 1 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 019902 DI 10.1063/1.4860977 PG 1 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800109 ER PT J AU Kim, YS Kim, J Yoon, MJ Sohn, CH Lee, SB Lee, D Jeon, BC Yoo, HK Noh, TW Bostwick, A Rotenberg, E Yu, J Bu, SD Mun, BS AF Kim, Yong Su Kim, Jiyeon Yoon, Moon Jee Sohn, Chang Hee Lee, Shin Buhm Lee, Daesu Jeon, Byung Chul Yoo, Hyang Keun Noh, Tae Won Bostwick, Aaron Rotenberg, Eli Yu, Jaejun Bu, Sang Don Mun, Bongjin Simon TI Impact of vacancy clusters on characteristic resistance change of nonstoichiometric strontium titanate nano-film SO APPLIED PHYSICS LETTERS LA English DT Article ID RESISTIVE SWITCHING MEMORIES; DOPED SRTIO3; THIN-FILMS AB In practical applications to bipolar resistance switching (BRS) memory devices with enhanced performance and high-scalability, oxide materials are commonly fabricated to highly nonstoichiometric and nanometer scale films. In this study, we fabricated ultrathin strontium titanate film, which shows two types of BRS behavior. By using micro-beam X-ray photoemission spectroscopy, the changes of core-level spectra depending on the resistance states are spatially resolved. Experimental and calculated results demonstrated that the fundamental switching mechanism in the two types of BRS is originated from the migration of anion and cation vacancies and the formation of insulating vacancy clusters near vicinity of the interface. (C) 2014 AIP Publishing LLC. C1 [Kim, Yong Su; Yoon, Moon Jee; Sohn, Chang Hee; Lee, Shin Buhm; Lee, Daesu; Jeon, Byung Chul; Yoo, Hyang Keun; Noh, Tae Won] Seoul Natl Univ, IBS, CFI CES, Seoul 151747, South Korea. [Kim, Yong Su; Yoon, Moon Jee; Sohn, Chang Hee; Lee, Shin Buhm; Lee, Daesu; Jeon, Byung Chul; Yoo, Hyang Keun; Noh, Tae Won] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea. [Kim, Jiyeon; Yu, Jaejun] Seoul Natl Univ, Dept Phys & Astron, CSCMR, Seoul 151747, South Korea. [Bostwick, Aaron; Rotenberg, Eli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bu, Sang Don] Chonbuk Natl Univ, Dept Phys, Jeonju 561756, South Korea. [Mun, Bongjin Simon] Gwangju Inst Sci & Technol, Ertl Ctr Electrochem & Catalyst, Sch Phys & Chem, Dept Phys & Photon Sci, Kwangju 500712, South Korea. RP Kim, YS (reprint author), Seoul Natl Univ, IBS, CFI CES, Seoul 151747, South Korea. EM ysukim@phya.snu.ac.kr RI Lee, Daesu/G-6407-2011; Rotenberg, Eli/B-3700-2009; LEE, SHINBUHM/A-9494-2011; OI Rotenberg, Eli/0000-0002-3979-8844; LEE, SHINBUHM/0000-0002-4907-7362; Bu, Sang Don/0000-0003-4883-1308 FU Institute of Basic Science (IBS) [EM 1203]; Basic Science Research Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology (MEST [2012R1A1A2001745]; Accelerated Research Program [R17-2008-33-0100-0]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; PAL through the abroad beamtime program of Synchrotron Radiation Facility Project under MEST FX This research was supported by the Institute of Basic Science (IBS) (EM 1203). B.S.M. would like to thank the support by Basic Science Research Program through the National Research Foundation of Korea (NRF) by the Ministry of Education, Science and Technology (MEST) (2012R1A1A2001745) and Accelerated Research Program (R17-2008-33-0100-0). The Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was supported by PAL through the abroad beamtime program of Synchrotron Radiation Facility Project under MEST. NR 22 TC 8 Z9 8 U1 4 U2 46 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 013501 DI 10.1063/1.4860961 PG 5 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800088 ER PT J AU Li, DJ Hong, S Gu, SY Choi, Y Nakhmanson, S Heinonen, O Karpeev, D No, K AF Li, Dong Jun Hong, Seungbum Gu, Shiyuan Choi, YoonYoung Nakhmanson, Serge Heinonen, Olle Karpeev, Dmitry No, Kwangsoo TI Polymer piezoelectric energy harvesters for low wind speed SO APPLIED PHYSICS LETTERS LA English DT Article AB We fabricated polymer piezoelectric energy harvesters (PEHs) that can generate electric power at wind speed of less than 4.7m/s due to their high sensitivity to wind. In order to optimize their operating conditions, we evaluated three distinct PEH operation modes under the boundary conditions of single-side clamping. We found that a PEH connected to an external load of 120 k Omega shows the largest output power of 0.98 mu W at 3.9 m/s, with wind incident on its side (mode I). We attribute this result to large bending and torsion involved in this operation mode. (C) 2014 AIP Publishing LLC. C1 [Li, Dong Jun; Hong, Seungbum; No, Kwangsoo] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Hong, Seungbum; Choi, YoonYoung] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [Gu, Shiyuan; Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Nakhmanson, Serge] Univ Connecticut, Inst Mat Sci, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Karpeev, Dmitry] Argonne Natl Lab, Lemont, IL 60439 USA. RP Hong, S (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. EM hong@anl.gov; ksno@kaist.ac.kr RI Nakhmanson, Serge/A-6329-2014; Hong, Seungbum/B-7708-2009; No, Kwangsoo/C-1983-2011; OI Hong, Seungbum/0000-0002-2667-1983; Heinonen, Olle/0000-0002-3618-6092 FU National Research Foundation of Korea (NRF) [2010-0015063, 2011K000674]; Ministry of Education, Science and Technology (MEST); New & Renewable Energy of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant [20103020060010]; Ministry of Knowledge Economy, Korea; UChicago Argonne, a U.S. DOE Office of Science Laboratory [DE-AC02-06CH11357] FX This research was supported by the Mid-career Researcher Program (No. 2010-0015063) and Conversion Research Center Program (No. 2011K000674) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (MEST) and the New & Renewable Energy of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant (No. 20103020060010) funded by the Ministry of Knowledge Economy, Korea. Work at Argonne National Laboratory (S.H., S.G., Y.C., O.H., simulation, data analysis, and writing of manuscript) was supported by UChicago Argonne, a U.S. DOE Office of Science Laboratory, operated under Contract No. DE-AC02-06CH11357. NR 19 TC 7 Z9 7 U1 2 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 012902 DI 10.1063/1.4861187 PG 4 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800057 ER PT J AU Macfaden, AJ Reno, JL Brener, I Mitrofanov, O AF Macfaden, Alexander J. Reno, John L. Brener, Igal Mitrofanov, Oleg TI 3 mu m aperture probes for near-field terahertz transmission microscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID PULSES; TIME; SPECTROSCOPY; DIFFRACTION; GENERATION; ANTENNAS AB The transmission of electromagnetic waves through a sub-wavelength aperture is described by Bethe's theory. This imposes severe limitations on using apertures smaller than similar to 1/100 of the wavelength for near-field microscopy at terahertz (THz) frequencies. Experimentally, we observe that the transmitted evanescent field within 1 mu m of the aperture deviates significantly from the Bethe dependence of E alpha a(3). Using this effect, we realized THz near-field probes incorporating 3 mu m apertures and we demonstrate transmission mode THz time-domain near-field imaging with spatial resolution of 3 mu m, corresponding to k/100 (at 1 THz). (C) 2014 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Macfaden, Alexander J.; Mitrofanov, Oleg] UCL, Dept Elect & Elect Engn, London WC1E 7JE, England. [Reno, John L.; Brener, Igal; Mitrofanov, Oleg] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Reno, John L.; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mitrofanov, O (reprint author), UCL, Dept Elect & Elect Engn, London WC1E 7JE, England. EM o.mitrofanov@ucl.ac.uk RI Mitrofanov, Oleg/C-1938-2008 OI Mitrofanov, Oleg/0000-0003-3510-2675 FU Royal Society [UF080745]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to thank Professor Paul Planken for useful discussions of wave transmission through small apertures and gratefully acknowledge the support of the Royal Society [Grant No. UF080745]. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 22 TC 21 Z9 21 U1 4 U2 30 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 011110 DI 10.1063/1.4861621 PG 5 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800010 ER PT J AU Singh, DJ Xu, Q Ong, KP AF Singh, David J. Xu, Qiang Ong, Khuong P. TI Strain effects on the band gap and optical properties of perovskite SrSnO3 and BaSnO3 SO APPLIED PHYSICS LETTERS LA English DT Article ID CONDUCTING OXIDES; TRANSPARENT; STANNATE; SR AB We report calculations of the band gaps and optical spectra of perovskite BaSnO3 and SrSnO3 as a function of strain. We find that the behavior of these compounds is controlled almost entirely by the volumetric strain and in particular that unlike commonly studied transition metal based perovskites, there is little sensitivity to strains other than volumetric. The most effective tuning parameters for the gap and optical properties of stannate perovskites are composition (A-site alloying) and volumetric strain. (C) 2014 AIP Publishing LLC. C1 [Singh, David J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Xu, Qiang; Ong, Khuong P.] Agcy Sci Technol & Res, Inst High Performance Comp, Singapore 138632, Singapore. RP Singh, DJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. FU Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; A*STAR FX We thank Bharat Jalan for useful discussions. Work at ORNL was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Work at IHPC is supported by A*STAR. NR 32 TC 20 Z9 20 U1 16 U2 132 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 011910 DI 10.1063/1.4861838 PG 4 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800028 ER PT J AU Tongay, S Narang, DS Kang, J Fan, W Ko, CH Luce, AV Wang, KX Suh, J Patel, KD Pathak, VM Li, JB Wu, JQ AF Tongay, Sefaattin Narang, Deepa S. Kang, Jun Fan, Wen Ko, Changhyun Luce, Alexander V. Wang, Kevin X. Suh, Joonki Patel, K. D. Pathak, V. M. Li, Jingbo Wu, Junqiao TI Two-dimensional semiconductor alloys: Monolayer Mo1-xWxSe2 SO APPLIED PHYSICS LETTERS LA English DT Article ID METAL DICHALCOGENIDE ALLOYS; MOS2; PHOTOLUMINESCENCE; EXCITONS; DEFECTS; BANDGAP AB Monolayer Mo1-xWxSe2 (x = 0, 0.14, 0.75, and 1) alloys were experimentally realized from synthesized crystals. Mo1-xWxSe2 monolayers are direct bandgap semiconductors displaying high luminescence and are stable in ambient. The bandgap values can be tuned by varying the W composition. Interestingly, the bandgap values do not scale linearly with composition. Such non-linearity is attributed to localization of conduction band minimum states around Mo d orbitals, whereas the valence band maximum states are uniformly distributed among W and Mo d orbitals. Results introduce monolayer Mo1-xWxSe2 alloys with different gap values, and open a venue for broadening the materials library and applications of two-dimensional semiconductors. (C) 2014 AIP Publishing LLC. C1 [Tongay, Sefaattin; Fan, Wen; Ko, Changhyun; Luce, Alexander V.; Wang, Kevin X.; Suh, Joonki; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Tongay, Sefaattin; Kang, Jun; Suh, Joonki; Li, Jingbo; Wu, Junqiao] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Narang, Deepa S.] Alliance Univ, ACED, Dept Phys, Bangalore 562106, Karnataka, India. [Kang, Jun; Luce, Alexander V.; Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Patel, K. D.; Pathak, V. M.] Sardar Patel Univ, Dept Phys, Anand 388120, Gujarat, India. RP Tongay, S (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM tongay@berkeley.edu RI Kang, Jun/F-7105-2011; Wu, Junqiao/G-7840-2011; Foundry, Molecular/G-9968-2014; Ko, Changhyun/E-1686-2011 OI Kang, Jun/0000-0003-4788-0028; Wu, Junqiao/0000-0002-1498-0148; FU National Science Foundation [DMR-1306601]; Natural Science Foundation of China for Distinguished Young Scholar [60925016, 91233120]; Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation under Grant No. DMR-1306601. J.L. and the computational effort gratefully acknowledge support from the Natural Science Foundation of China for Distinguished Young Scholar (Grant Nos. 60925016 and 91233120). The nano-Auger and XPS part was a user project at the Molecular Foundry, which was supported by the Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231 NR 22 TC 46 Z9 48 U1 6 U2 84 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 6 PY 2014 VL 104 IS 1 AR 012101 DI 10.1063/1.4834358 PG 4 WC Physics, Applied SC Physics GA 291OT UT WOS:000329838800032 ER PT J AU Al-Rawashdeh, NAF Chatterjee, S Krause, JA Connick, WB AF Al-Rawashdeh, Nathir A. F. Chatterjee, Sayandev Krause, Jeanette A. Connick, William B. TI Ruthenium Bis-diimine Complexes with a Chelating Thioether Ligand: Delineating 1,10-Phenanthrolinyl and 2,2 '-Bipyridyl Ligand Substituent Effects SO INORGANIC CHEMISTRY LA English DT Article ID EXCITED-STATE PROPERTIES; CHARGE-TRANSFER TRANSITIONS; X-RAY STRUCTURE; METAL-COMPLEXES; 2,2-BIPYRIDINE COMPLEXES; PHOTOPHYSICAL PROPERTIES; REDOX POTENTIALS; ELECTROCHEMICAL POTENTIALS; POLYPYRIDINE COMPLEXES; ABSORPTION-SPECTRA AB Despite the high it-acidity of thioether donors, ruthenium(II) complexes with a bidentate 1,2-bis(phenylthio)ethane (dpte) ligand and two chelating diimine ligands (i.e., Ru(diimine)(2)(dpte)(2+)) exhibit room-temperature fluid solution emission originating from a lowest MLCT excited state (diimine = 2,2'-bipyridine, 5,5'-dimethyl-2,2'-bipyridine 4,4'-di-tert-butyl-2,2'-bipyridine, 1,10-phenanthroline, 5-methyl-1,10-phenanthroline, 5-chloro-1,10-phenanthroline, 5-bromo-1,10-phenanthroline, 5-nitro-1,10-phenanthroline, 4,7-diphenyl-1,10-phenanthroline, and 3,4,7,8-tetramethyl-1,10-phenanthroline). Crystal structures show that the complexes form 2 of the 12 possible conformational/configurational isomers, as well as nonstatistical distributions of geometric isomers; there also are short intramolecular pi-pi interactions between the diimine ligands and dpte phenyl groups. The photoinduced solvolysis product, [Ru(diimine)(2)(CH3CN)(2)](PF6)(2), for one complex in acetonitrile also was characterized by single-crystal X-ray diffraction. Variations in the MLCT energies and Ru(III/II) redox couple, E-o'(Ru3+/2+), can be understood in terms of the influence of the donor properties of the ligands on the mainly metal-based HOMO and mainly diimine ligand-based LUMO. E-o'(Ru3+/2+) also is quantitatively described using a summative Hammett parameter (sigma(T)), as well as using Lever's electrochemical parameters (E-L). Recommended parametrizations for substituted 2,2'-bipyridyl and 1,10-phenanthrolinyl ligands were derived from analysis of correlations of E-o'(Ru3+/2+) for 99 homo- and heteroleptic ruthenium(II) tris-diimine complexes. This analysis reveals that variations in E-o'(Ru3+/2+) due to substituents at the 4- and 4'-positions of bipyridyl ligands and 4- and 7-positions of phenanthrolinyl ligands are significantly more strongly correlated with sigma(+)(p) than either sigma(m) or sigma(p). Substituents at the 5- and 6-positions of phenanthrolinyl ligands are best described by sigma(m) and have effects comparable to those of substituents at the 3- and 8-positions. Correlations of E-L with sigma(T) for 1,10-phenanthrolinyl and 2,2'-bipyridyl ligands show similar results, except that sigma(p) and sigma(+)(p) are almost equally effective in describing the influence of substituents at the 4- and 4'-positions of bipyridyl ligands. MLCT energies and d(5)/d(6)-electron redox couples of the complexes with 5-substituted 1,10-phenanthroline exhibit correlations with values for other d(6)-electron metal complexes that can be rationalized in terms of the relative number of diimine ligands and substituents. C1 [Krause, Jeanette A.; Connick, William B.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. [Al-Rawashdeh, Nathir A. F.] Jordan Univ Sci & Technol, Dept Appl Chem Sci, Irbid 22110, Jordan. [Chatterjee, Sayandev] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Connick, WB (reprint author), Univ Cincinnati, Dept Chem, POB 210172, Cincinnati, OH 45221 USA. EM Bill.Connick@uc.edu OI Chatterjee, Sayandev/0000-0003-2218-5635 FU National Science Foundation [CHE-1152853, 0749790, 0134975]; Fulbright Scholar Program; Jordan University of Science and Technology; NSF-MM [CHE-0215950]; U.S. Department of Energy, Office of Energy Sciences [DE-AC02-05CH11231] FX This research was supported by the National Science Foundation (CHE-1152853, 0749790, 0134975). We thank Drs. Stephen Macha and Larry Sallans for expert technical assistance. N.A.F. Al-Rawashdeh thanks the Fulbright Scholar Program and the Jordan University of Science and Technology for financial support. Funding for the SMART6000 CCD diffractometer was through NSF-MM grant CHE-0215950. Synchrotron data were collected through the SCrALS (Service Crystallography at Advanced Light Source) project at Beam line 11.3.1 at the Advanced Light Source (ALS), Lawrence Berkeley National Laboratory. The ALS is supported by the U.S. Department of Energy, Office of Energy Sciences, under contract DE-AC02-05CH11231. NR 126 TC 7 Z9 7 U1 3 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JAN 6 PY 2014 VL 53 IS 1 BP 294 EP 307 DI 10.1021/ic4022454 PG 14 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 287GK UT WOS:000329529800038 PM 24325318 ER PT J AU Wilson, RE Schnaars, DD Andrews, MB Cahill, CL AF Wilson, Richard E. Schnaars, David D. Andrews, Michael B. Cahill, C. L. TI Supramolecular Interactions in PuO2Cl42- and PuCl62- Complexes with Protonated Pyridines: Synthesis, Crystal Structures, and Raman Spectroscopy SO INORGANIC CHEMISTRY LA English DT Article ID URANYL-ION; PLUTONIUM; NETWORKS; PHOSPHONATES; HYDROLYSIS; SPECIATION; AMERICIUM; CHEMISTRY; TRENDS AB The synthesis, crystal structures, and Raman spectra of seven plutonium chloride compounds are presented. The materials are based upon Pu(VI)O2Cl42- and Pu(IV)Cl-6(2-) anions that are charge balanced by protonated pyridinium cations. The single crystal X-ray structures show a variety of donor-acceptor interactions between the plutonium perhalo anions and the cationic pyridine groups. Complementary Raman spectra show that these interactions can be probed through the symmetric vibrational mode of the plutonyl moiety. Unlike previously reported studies in similar uranyl(VI) systems, the facile redox chemistry of plutonium, in aqueous, solution has demonstrated the feasibility of using not only the An(VI)O2Cl42- anion with approximate D-4h symmetry but also the approximately O-h An(IV)Cl-6(2-) anion in order to manipulate both the structure and dimensionality of such hybrid materials. C1 [Wilson, Richard E.; Schnaars, David D.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Andrews, Michael B.; Cahill, C. L.] George Washington Univ, Dept Chem, Washington, DC 20052 USA. RP Wilson, RE (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rewilson@anl.gov; cahill@gwu.edu RI Wilson, Richard/H-1763-2011; OI Wilson, Richard/0000-0001-8618-5680; Andrews, Michael/0000-0003-3762-8523 FU United States Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences [DE-AC02-06CH11357]; George Washington University [DE-FG02-05ER15736] FX This work was performed at Argonne National Laboratory, operated for the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences, under Contract Number DE-AC02-06CH11357. C.L.C. and M.B.A. were supported at The George Washington University by the same program, under Grant DE-FG02-05ER15736. NR 51 TC 6 Z9 6 U1 1 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JAN 6 PY 2014 VL 53 IS 1 BP 383 EP 392 DI 10.1021/ic4023294 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 287GK UT WOS:000329529800047 PM 24328217 ER PT J AU Bishop, JE AF Bishop, J. E. TI A displacement-based finite element formulation for general polyhedra using harmonic shape functions SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN ENGINEERING LA English DT Article DE finite element; polyhedra; polyhedron; harmonic function; barycentric coordinates ID LINEAR ELASTICITY; POLYTOPES; MESHES AB A displacement-based continuous-Galerkin finite element formulation for general polyhedra is presented for applications in nonlinear solid mechanics. The polyhedra can have an arbitrary number of vertices or faces. The faces of the polyhedra can have an arbitrary number of edges and can be nonplanar. The polyhedra can be nonconvex with only the mild restriction of star convexity with respect to the vertex-averaged centroid. Conforming shape functions are constructed using harmonic functions defined on the undeformed configuration, thus requiring the use of a total-Lagrangian finite element formulation in large deformation applications. For nonlinear applications with computationally intensive constitutive models, it is important to minimize the number of element quadrature points. For this reason, an integration scheme is adopted in which the number of quadrature points is equal to the number of vertices. As a first step toward verifying the element behavior in the general nonlinear setting, several linear verification examples are presented using both random Voronoi meshes and distorted hexahedral meshes. For the hexahedral meshes, results for the polyhedral formulation are compared to those of the standard trilinear hexahedral formulation. The element behavior in the nearly incompressible regime is also examined. Copyright (C) 2013 John Wiley & Sons, Ltd. C1 [Bishop, J. E.] Sandia Natl Labs, Computat Struct Mech Dept, Engn Sci Ctr, Albuquerque, NM 87185 USA. RP Bishop, JE (reprint author), Sandia Natl Labs, POB 5800,Mail Stop 0372, Albuquerque, NM 87185 USA. EM jebisho@sandia.gov FU Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; Defense Threat Reduction Agency [HDTRA1-09-0029, A12051]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001114. The initial research into the development of a polyhedral finite element was funded by the Defense Threat Reduction Agency (prime award HDTRA1-09-0029 to Rensselaer Polytechnic Institute, subcontract A12051 to Sandia National Laboratories) for applications in modeling pervasive fracture phenomena. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 37 TC 25 Z9 25 U1 2 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0029-5981 EI 1097-0207 J9 INT J NUMER METH ENG JI Int. J. Numer. Methods Eng. PD JAN 6 PY 2014 VL 97 IS 1 BP 1 EP 31 DI 10.1002/nme.4562 PG 31 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA CA0KD UT WOS:000348605800001 ER PT J AU Knox, KR Bozin, ES Malliakas, CD Kanatzidis, MG Billinge, SJL AF Knox, K. R. Bozin, E. S. Malliakas, C. D. Kanatzidis, M. G. Billinge, S. J. L. TI Local off-centering symmetry breaking in the high-temperature regime of SnTe SO PHYSICAL REVIEW B LA English DT Article ID STRUCTURAL PHASE-TRANSITIONS; MOSSBAUER-SPECTROSCOPY; LEAD CHALCOGENIDES; CRYSTAL-STRUCTURE; PHONON MODE; PBTE; SCATTERING; DISORDER; ORDER; MONOCHALCOGENIDES AB The local structure of SnTe has been studied using atomic pair distribution function analysis of x-ray and neutron data. Evidence is found for a locally distorted high-temperature state, which emerges on warming from an undistorted rocksalt structure. The structural distortion appears rapidly over a relatively narrow temperature range from 300 to 400 K. A similar effect has been reported in PbTe and PbS and dubbed emphanisis; here we report on emphanisis in a compound that does not contain Pb. The analysis suggests that this effect is unrelated to the low-temperature ferroelectric state in SnTe. C1 [Knox, K. R.; Bozin, E. S.; Billinge, S. J. L.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. [Malliakas, C. D.; Kanatzidis, M. G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Malliakas, C. D.; Kanatzidis, M. G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Billinge, S. J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Knox, KR (reprint author), Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. FU US DOE, Office of Science, Office of Basic Energy Sciences (DOE-BES) [DE-AC02-98CH10886]; DOE-BES [DE-AC02-06CH11357]; DOE BES; Los Alamos National Security LLC [DE-AC52-06NA25396] FX Data collection, analysis, and modeling were supported by US DOE, Office of Science, Office of Basic Energy Sciences (DOE-BES) under Contract No. DE-AC02-98CH10886. NSLS is operated by BNL under the same Contract No. Sample preparation and characterization were supported by DOE-BES under Contract No. DE-AC02-06CH11357. Neutron PDF experiments were carried out on NPDF at LANSCE, funded by DOE BES; Los Alamos National Laboratory is operated by Los Alamos National Security LLC under Contract No. DE-AC52-06NA25396. NR 51 TC 11 Z9 11 U1 5 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 3 PY 2014 VL 89 IS 1 AR 014102 DI 10.1103/PhysRevB.89.014102 PG 5 WC Physics, Condensed Matter SC Physics GA AC0FZ UT WOS:000332171500001 ER PT J AU Popovic, ZV Scepanovic, M Lazarevic, N Radonjic, MM Tanaskovic, D Lei, HC Petrovic, C AF Popovic, Z. V. Scepanovic, M. Lazarevic, N. Radonjic, M. M. Tanaskovic, D. Lei, Hechang Petrovic, C. TI Phonon and magnetic dimer excitations in Fe-based S = 2 spin-ladder compound BaFe2Se2O SO PHYSICAL REVIEW B LA English DT Article ID SCATTERING AB Raman scattering spectra of the new Fe-based S = 2 spin-ladder compound BaFe2Se2O are measured in a temperature range between 15 and 623 K. All six A(1g) and two B-1g Raman active modes of BaFe2Se2O, predicted by the factor-group analysis, have been experimentally observed at energies that are in a rather good agreement with the lattice dynamics calculation. The antiferromagnetic long-range spin ordering in BaFe2Se2O below T-N = 240 K leaves a fingerprint both in the A(1g) and B-1g phonon mode linewidth and energy. In the energy range between 400 and 650 cm(-1) we have observed a magnetic excitation related structure in the form of a magnon continuum, with the peaks corresponding to the singularities in the one-dimensional density of magnon states. The onset value of magnetic continuum (2 Delta(S)) is found at about 437 cm(-1) at 15 K. The magnetic continuum disappears at about 623 K, which led us to conclude that the short-range magnetic ordering in BaFe2Se2O exists apparently up to 2.6T(N). C1 [Popovic, Z. V.; Scepanovic, M.; Lazarevic, N.] Univ Belgrade, Inst Phys Belgrade, Ctr Solid State Phys & New Mat, Belgrade 11080, Serbia. [Radonjic, M. M.; Tanaskovic, D.] Univ Belgrade, Inst Phys Belgrade, Comp Sci Lab, Belgrade 11080, Serbia. [Lei, Hechang; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Popovic, ZV (reprint author), Univ Belgrade, Inst Phys Belgrade, Ctr Solid State Phys & New Mat, Pregrevica 118, Belgrade 11080, Serbia. RI Petrovic, Cedomir/A-8789-2009; Radonjic, Milos/M-1890-2015; LEI, Hechang/H-3278-2016 OI Petrovic, Cedomir/0000-0001-6063-1881; FU Serbian Ministry of Education, Science, and Technological Development [ON171032, ON171017, III45018]; U.S. DOE [DE-AC02-98CH10886]; Center for Emergent Superconductivity, an Energy Frontier Research Center; U.S. DOE, Office for Basic Energy Science; FP7 project EGI-InSPIRE; FP7 project PRACE-1IP; FP7 project HP-SEE FX This work was supported by the Serbian Ministry of Education, Science, and Technological Development under Projects ON171032, ON171017, and III45018. Work at Brookhaven was supported by the U.S. DOE under Contract No. DE-AC02-98CH10886 and in part by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. DOE, Office for Basic Energy Science (H.L. and C.P.). Numerical simulations were run on the AEGIS e-Infrastructure, supported in part by FP7 projects EGI-InSPIRE, PRACE-1IP, and HP-SEE. NR 23 TC 3 Z9 3 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 3 PY 2014 VL 89 IS 1 AR 014301 DI 10.1103/PhysRevB.89.014301 PG 5 WC Physics, Condensed Matter SC Physics GA AC0FZ UT WOS:000332171500002 ER PT J AU Shang, T Baumbach, RE Gofryk, K Ronning, F Weng, ZF Zhang, JL Lu, X Bauer, ED Thompson, JD Yuan, HQ AF Shang, T. Baumbach, R. E. Gofryk, K. Ronning, F. Weng, Z. F. Zhang, J. L. Lu, X. Bauer, E. D. Thompson, J. D. Yuan, H. Q. TI CeIrIn5: Superconductivity on a magnetic instability SO PHYSICAL REVIEW B LA English DT Article ID HEAVY; TEMPERATURE; PRESSURE; SYSTEMS; CE AB We report on the doping-induced antiferromagnetic state and Fermi-liquid state that are connected by a superconducting region in a series of CeIrIn5-xHgx, CeIrIn5-xSnx, and CeIr1-xPtxIn5 single crystals. Measurements of the specific heat C(T) and electrical resistivity rho(T) demonstrate that hole doping via Hg/In substitution gives rise to an antiferromagnetic ground state, but substitutions of In by Sn or Ir by Pt (electron doping) favor a paramagnetic Fermi-liquid state. A conelike non-Fermi-liquid region is observed near CeIrIn5, showing a diverging effective mass on the slightly Hg-doped side. The obtained temperature-doping phase diagram suggests that CeIrIn5 is in proximity to an antiferromagnetic quantum critical point, and heavy fermion superconductivity in this compound is mediated by magnetic quantum fluctuations rather than by valence fluctuations. C1 [Shang, T.; Weng, Z. F.; Zhang, J. L.; Lu, X.; Yuan, H. Q.] Zhejiang Univ, Ctr Correlated Matter, Hangzhou 310027, Zhejiang, Peoples R China. [Shang, T.; Weng, Z. F.; Zhang, J. L.; Lu, X.; Yuan, H. Q.] Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. [Shang, T.; Baumbach, R. E.; Gofryk, K.; Ronning, F.; Bauer, E. D.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Shang, T (reprint author), Zhejiang Univ, Ctr Correlated Matter, Hangzhou 310027, Zhejiang, Peoples R China. EM hqyuan@zju.edu.cn RI Lu, Xin/B-7358-2012; Gofryk, Krzysztof/F-8755-2014; OI Gofryk, Krzysztof/0000-0002-8681-6857; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU National Science Foundation of China [11174245, 10934005, 11374257]; National Basic Research Program of China (973 Program) [2009CB929104, 2011CBA00103]; Zhejiang Provincial Natural Science Foundation of China; Fundamental Research Funds for the Central Universities; Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering FX This work is partially supported by the National Science Foundation of China (Grants No. 11174245, No. 10934005, and No. 11374257), the National Basic Research Program of China (973 Program) (2009CB929104, 2011CBA00103), Zhejiang Provincial Natural Science Foundation of China, and the Fundamental Research Funds for the Central Universities. Work at LANL was performed under the auspices of the Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering. NR 39 TC 13 Z9 14 U1 0 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 3 PY 2014 VL 89 IS 4 AR 041101 DI 10.1103/PhysRevB.89.041101 PG 5 WC Physics, Condensed Matter SC Physics GA AC0HG UT WOS:000332174800001 ER PT J AU Poe, DP Veit, D Ranger, M Kaczmarski, K Tarafder, A Guiochon, G AF Poe, Donald P. Veit, Devon Ranger, Megan Kaczmarski, Krzysztof Tarafder, Abhijit Guiochon, Georges TI Pressure, temperature and density drops along supercritical fluid chromatography columns in different thermal environments. III. Mixtures of carbon dioxide and methanol as the mobile phase SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Supercritical fluid chromatography SFC; Pressure drop; Temperature drop; Density drop; Isenthalpic expansion ID DESIGNING OPERATIONS; ISOPYCNIC PLOTS; EFFICIENCY; RETENTION; PARTICLES; PROFILES; EQUATION; STATE AB The pressure, temperature and density drops along SFC columns eluted with a CO2/methanol mobile phase were measured and compared with theoretical values. For columns packed with 3- and 5-mu m particles the pressure and temperature drops were measured using a mobile phase of 95% CO2 and 5% methanol at a flow rate of 5 mL/min, at temperatures from 20 to 100 degrees C, and outlet pressures from 80 to 300 bar. The density drop was calculated based on the temperature and pressure at the column inlet and outlet. The columns were suspended in a circulating air bath, either bare or covered with foam insulation. The experimental measurements were compared to theoretical results obtained by numerical simulation. For the convective air condition at outlet pressures above 100 bar the average difference between the experimental and calculated temperature drops and pressure drops were 0.1 degrees C and 0.7% for the bare 3-mu m column, respectively, and were 0.6 degrees C and 4.1% for the insulated column. The observed temperature drops for the insulated columns are consistent with those predicted by the Joule Thomson coefficients for isenthalpic expansion. The dependence of the temperature and the pressure drops on the Joule Thomson coefficient and kinematic viscosity are described for carbon dioxide mobile phases containing up to 20% methanol. (C) 2013 Elsevier B.V. All rights reserved. C1 [Poe, Donald P.; Veit, Devon; Ranger, Megan] Univ Minnesota, Dept Chem & Biochem, Duluth, MN 55812 USA. [Kaczmarski, Krzysztof] Rzeszow Univ Technol, Dept Chem & Proc Engn, PL-35959 Rzeszow, Poland. [Tarafder, Abhijit] Waters Corp, Milford, MA USA. [Guiochon, Georges] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Guiochon, Georges] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. RP Poe, DP (reprint author), Univ Minnesota, Dept Chem & Biochem, Duluth, MN 55812 USA. EM dpoe@d.umn.edu FU American Chemical Society Petroleum Research Fund [51984-UR9]; Chancellor's Faculty Small Grant Program, University of Minnesota Duluth; Undergraduate Research Opportunities Program, University of Minnesota FX This work was supported by grants from the American Chemical Society Petroleum Research Fund grant #51984-UR9 and the Chancellor's Faculty Small Grant Program, University of Minnesota Duluth. D. Veit and M. Ranger are grateful for support from the Undergraduate Research Opportunities Program, University of Minnesota. NR 21 TC 9 Z9 9 U1 4 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD JAN 3 PY 2014 VL 1323 BP 143 EP 156 DI 10.1016/j.chroma.2013.11.012 PG 14 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA 293EI UT WOS:000329953800017 PM 24315126 ER PT J AU Van der Auwera, S Bulla, I Ziller, M Pohlmann, A Harder, T Stanke, M AF Van der Auwera, Sandra Bulla, Ingo Ziller, Mario Pohlmann, Anne Harder, Timm Stanke, Mario TI ClassyFlu: Classification of Influenza A Viruses with Discriminatively Trained Profile-HMMs SO PLOS ONE LA English DT Article ID MULTIPLE SEQUENCE ALIGNMENT; PANDEMIC INFLUENZA; MAXIMUM-LIKELIHOOD; THREAT AB Accurate and rapid characterization of influenza A virus (IAV) hemagglutinin (HA) and neuraminidase (NA) sequences with respect to subtype and clade is at the basis of extended diagnostic services and implicit to molecular epidemiologic studies. ClassyFlu is a new tool and web service for the classification of IAV sequences of the HA and NA gene into subtypes and phylogenetic clades using discriminatively trained profile hidden Markov models (HMMs), one for each subtype or clade. ClassyFlu merely requires as input unaligned, full-length or partial HA or NA DNA sequences. It enables rapid and highly accurate assignment of HA sequences to subtypes H1-H17 but particularly focusses on the finer grained assignment of sequences of highly pathogenic avian influenza viruses of subtype H5N1 according to the cladistics proposed by the H5N1 Evolution Working Group. NA sequences are classified into subtypes N1-N10. ClassyFlu was compared to semiautomatic classification approaches using BLAST and phylogenetics and additionally for H5 sequences to the new "Highly Pathogenic H5N1 Clade Classification Tool" (IRD-CT) proposed by the Influenza Research Database. Our results show that both web tools (ClassyFlu and IRD-CT), although based on different methods, are nearly equivalent in performance and both are more accurate and faster than semiautomatic classification. A retraining of ClassyFlu to altered cladistics as well as an extension of ClassyFlu to other IAV genome segments or fragments thereof is undemanding. This is exemplified by unambiguous assignment to a distinct cluster within subtype H7 of sequences of H7N9 viruses which emerged in China early in 2013 and caused more than 130 human infections. http://bioinf.uni-greifswald.de/ClassyFlu is a free web service. For local execution, the ClassyFlu source code in PERL is freely available. C1 [Van der Auwera, Sandra; Bulla, Ingo; Stanke, Mario] Ernst Moritz Arndt Univ Greifswald, Inst Math & Comp Sci, Greifswald, Germany. [Ziller, Mario; Pohlmann, Anne; Harder, Timm] Fed Res Inst Anim Hlth, Greifswald, Germany. [Bulla, Ingo] Los Alamos Natl Lab, Grp T6, Los Alamos, NM USA. RP Stanke, M (reprint author), Ernst Moritz Arndt Univ Greifswald, Inst Math & Comp Sci, Greifswald, Germany. EM mario.stanke@uni-greifswald.de FU Deutsche Forschungsgemeinschaft [STA 1009/5-1] FX Deutsche Forschungsgemeinschaft grant STA 1009/5-1. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 20 TC 0 Z9 0 U1 2 U2 14 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 3 PY 2014 VL 9 IS 1 AR e84558 DI 10.1371/journal.pone.0084558 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 286IH UT WOS:000329460800052 PM 24404173 ER PT J AU Vestrand, WT Wren, JA Panaitescu, A Wozniak, PR Davis, H Palmer, DM Vianello, G Omodei, N Xiong, S Briggs, MS Elphick, M Paciesas, W Rosing, W AF Vestrand, W. T. Wren, J. A. Panaitescu, A. Wozniak, P. R. Davis, H. Palmer, D. M. Vianello, G. Omodei, N. Xiong, S. Briggs, M. S. Elphick, M. Paciesas, W. Rosing, W. TI The Bright Optical Flash and Afterglow from the Gamma-Ray Burst GRB 130427A SO SCIENCE LA English DT Article ID LIGHT CURVES; EMISSION; 080319B; PROMPT AB The optical light generated simultaneously with x-rays and gamma rays during a gamma-ray burst (GRB) provides clues about the nature of the explosions that occur as massive stars collapse. We report on the bright optical flash and fading afterglow from powerful burst GRB 130427A. The optical and >100-megaelectron volt (MeV) gamma-ray flux show a close correlation during the first 7000 seconds, which is best explained by reverse shock emission cogenerated in the relativistic burst ejecta as it collides with surrounding material. At later times, optical observations show the emergence of emission generated by a forward shock traversing the circumburst environment. The link between optical afterglow and >100-MeV emission suggests that nearby early peaked afterglows will be the best candidates for studying gamma-ray emission at energies ranging from gigaelectron volts to teraelectron volts. C1 [Vestrand, W. T.; Wren, J. A.; Panaitescu, A.; Wozniak, P. R.; Davis, H.; Palmer, D. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Vianello, G.; Omodei, N.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Vianello, G.; Omodei, N.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Xiong, S.; Briggs, M. S.] Univ Alabama, Ctr Space Plasma & Aeron Res, Huntsville, AL 35899 USA. [Elphick, M.; Rosing, W.] Las Cumbres Observ Global Telescope Network, Santa Barbara, CA 93117 USA. [Paciesas, W.] Univ Space Res Assoc, Huntsville, AL 35899 USA. RP Vestrand, WT (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM vestrand@lanl.gov OI Wozniak, Przemyslaw/0000-0002-9919-3310; Omodei, Nicola/0000-0002-5448-7577 FU NASA; Laboratory Directed Research and Development program at Los Alamos National Laboratory FX This GRB research was supported by NASA and the Laboratory Directed Research and Development program at Los Alamos National Laboratory. The optical measurements reported in this paper are available online in the supplementary materials. NR 23 TC 29 Z9 31 U1 1 U2 7 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 3 PY 2014 VL 343 IS 6166 BP 38 EP 41 DI 10.1126/science.1242316 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282HR UT WOS:000329162000041 PM 24263131 ER PT J AU Ackermann, M Ajello, M Asano, K Atwood, WB Axelsson, M Baldini, L Ballet, J Barbiellini, G Baring, MG Bastieri, D Bechtol, K Bellazzini, R Bissaldi, E Bonamente, E Bregeon, J Brigida, M Bruel, P Buehler, R Burgess, JM Buson, S Caliandro, GA Cameron, RA Caraveo, PA Cecchi, C Chaplin, V Charles, E Chekhtman, A Cheung, CC Chiang, J Chiaro, G Ciprini, S Claus, R Cleveland, W Cohen-Tanugi, J Collazzi, A Cominsky, LR Connaughton, V Conrad, J Cutini, S D'Ammando, F de Angelis, A DeKlotz, M de Palma, F Dermer, CD Desiante, R Diekmann, A Di Venere, L Drell, PS Drlica-Wagner, A Favuzzi, C Fegan, SJ Ferrara, EC Finke, J Fitzpatrick, G Focke, WB Franckowiak, A Fukazawa, Y Funk, S Fusco, P Gargano, F Gehrels, N Germani, S Gibby, M Giglietto, N Giles, M Giordano, F Giroletti, M Godfrey, G Granot, J Grenier, IA Grove, JE Gruber, D Guiriec, S Hadasch, D Hanabata, Y Harding, AK Hayashida, M Hays, E Horan, D Hughes, RE Inoue, Y Jogler, T Johannesson, G Johnson, WN Kawano, T Knodlseder, J Kocevski, D Kuss, M Lande, J Larsson, S Latronico, L Longo, F Loparco, F Lovellette, MN Lubrano, P Mayer, M Mazziotta, MN McEnery, JE Michelson, PF Mizuno, T Moiseev, AA Monzani, ME Moretti, E Morselli, A Moskalenko, IV Murgia, S Nemmen, R Nuss, E Ohno, M Ohsugi, T Okumura, A Omodei, N Orienti, M Paneque, D Pelassa, V Perkins, JS Pesce-Rollins, M Petrosian, V Piron, F Pivato, G Porter, TA Racusin, JL Raino, S Rando, R Razzano, M Razzaque, S Reimer, A Reimer, O Ritz, S Roth, M Ryde, F Sartori, A Parkinson, PMS Scargle, JD Schulz, A Sgro, C Siskind, EJ Sonbas, E Spandre, G Spinelli, P Tajima, H Takahashi, H Thayer, JG Thayer, JB Thompson, DJ Tibaldo, L Tinivella, M Torres, DF Tosti, G Troja, E Usher, TL Vandenbroucke, J Vasileiou, V Vianello, G Vitale, V Winer, BL Wood, KS Yamazaki, R Younes, G Yu, HF Zhu, SJ Bhat, PN Briggs, MS Byrne, D Foley, S Goldstein, A Jenke, P Kippen, RM Kouveliotou, C McBreen, S Meegan, C Paciesas, WS Preece, R Rau, A Tierney, D van der Horst, AJ von Kienlin, A Wilson-Hodge, C Xiong, S Cusumano, G La Parola, V Cummings, JR AF Ackermann, M. Ajello, M. Asano, K. Atwood, W. B. Axelsson, M. Baldini, L. Ballet, J. Barbiellini, G. Baring, M. G. Bastieri, D. Bechtol, K. Bellazzini, R. Bissaldi, E. Bonamente, E. Bregeon, J. Brigida, M. Bruel, P. Buehler, R. Burgess, J. Michael Buson, S. Caliandro, G. A. Cameron, R. A. Caraveo, P. A. Cecchi, C. Chaplin, V. Charles, E. Chekhtman, A. Cheung, C. C. Chiang, J. Chiaro, G. Ciprini, S. Claus, R. Cleveland, W. Cohen-Tanugi, J. Collazzi, A. Cominsky, L. R. Connaughton, V. Conrad, J. Cutini, S. D'Ammando, F. de Angelis, A. DeKlotz, M. de Palma, F. Dermer, C. D. Desiante, R. Diekmann, A. Di Venere, L. Drell, P. S. Drlica-Wagner, A. Favuzzi, C. Fegan, S. J. Ferrara, E. C. Finke, J. Fitzpatrick, G. Focke, W. B. Franckowiak, A. Fukazawa, Y. Funk, S. Fusco, P. Gargano, F. Gehrels, N. Germani, S. Gibby, M. Giglietto, N. Giles, M. Giordano, F. Giroletti, M. Godfrey, G. Granot, J. Grenier, I. A. Grove, J. E. Gruber, D. Guiriec, S. Hadasch, D. Hanabata, Y. Harding, A. K. Hayashida, M. Hays, E. Horan, D. Hughes, R. E. Inoue, Y. Jogler, T. Johannesson, G. Johnson, W. N. Kawano, T. Knoedlseder, J. Kocevski, D. Kuss, M. Lande, J. Larsson, S. Latronico, L. Longo, F. Loparco, F. Lovellette, M. N. Lubrano, P. Mayer, M. Mazziotta, M. N. McEnery, J. E. Michelson, P. F. Mizuno, T. Moiseev, A. A. Monzani, M. E. Moretti, E. Morselli, A. Moskalenko, I. V. Murgia, S. Nemmen, R. Nuss, E. Ohno, M. Ohsugi, T. Okumura, A. Omodei, N. Orienti, M. Paneque, D. Pelassa, V. Perkins, J. S. Pesce-Rollins, M. Petrosian, V. Piron, F. Pivato, G. Porter, T. A. Racusin, J. L. Raino, S. Rando, R. Razzano, M. Razzaque, S. Reimer, A. Reimer, O. Ritz, S. Roth, M. Ryde, F. Sartori, A. Parkinson, P. M. Saz Scargle, J. D. Schulz, A. Sgro, C. Siskind, E. J. Sonbas, E. Spandre, G. Spinelli, P. Tajima, H. Takahashi, H. Thayer, J. G. Thayer, J. B. Thompson, D. J. Tibaldo, L. Tinivella, M. Torres, D. F. Tosti, G. Troja, E. Usher, T. L. Vandenbroucke, J. Vasileiou, V. Vianello, G. Vitale, V. Winer, B. L. Wood, K. S. Yamazaki, R. Younes, G. Yu, H. -F. Zhu, S. J. Bhat, P. N. Briggs, M. S. Byrne, D. Foley, S. Goldstein, A. Jenke, P. Kippen, R. M. Kouveliotou, C. McBreen, S. Meegan, C. Paciesas, W. S. Preece, R. Rau, A. Tierney, D. van der Horst, A. J. von Kienlin, A. Wilson-Hodge, C. Xiong, S. Cusumano, G. La Parola, V. Cummings, J. R. TI Fermi-LAT Observations of the Gamma-Ray Burst GRB 130427A SO SCIENCE LA English DT Article ID LARGE-AREA TELESCOPE; HIGH-ENERGY EMISSION; SPECTRAL COMPONENT; AFTERGLOW; PROMPT AB The observations of the exceptionally bright gamma-ray burst (GRB) 130427A by the Large Area Telescope aboard the Fermi Gamma-ray Space Telescope provide constraints on the nature of these unique astrophysical sources. GRB 130427A had the largest fluence, highest-energy photon (95 GeV), longest gamma-ray duration (20 hours), and one of the largest isotropic energy releases ever observed from a GRB. Temporal and spectral analyses of GRB 130427A challenge the widely accepted model that the nonthermal high-energy emission in the afterglow phase of GRBs is synchrotron emission radiated by electrons accelerated at an external shock. C1 [Ackermann, M.; Buehler, R.; Mayer, M.; Schulz, A.] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Ajello, M.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Asano, K.] Univ Tokyo, Inst Cosm Ray Res, Kashiwa, Chiba 2778582, Japan. [Atwood, W. B.; Razzano, M.; Ritz, S.; Parkinson, P. M. Saz] Univ Calif Santa Cruz, Dept Phys, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Atwood, W. B.; Razzano, M.; Ritz, S.; Parkinson, P. M. Saz] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Axelsson, M.; Larsson, S.] Stockholm Univ, Dept Astron, SE-10691 Stockholm, Sweden. [Axelsson, M.; Conrad, J.; Larsson, S.; Moretti, E.; Ryde, F.] AlbaNova, Oskar Klein Ctr Cosmoparticle Phys, SE-10691 Stockholm, Sweden. [Axelsson, M.; Moretti, E.; Ryde, F.] AlbaNova, Royal Inst Technol KTH, Dept Phys, SE-10691 Stockholm, Sweden. [Baldini, L.] Univ Pisa, I-56127 Pisa, Italy. [Baldini, L.; Bellazzini, R.; Bregeon, J.; Kuss, M.; Pesce-Rollins, M.; Razzano, M.; Sgro, C.; Spandre, G.; Tinivella, M.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Ballet, J.; Grenier, I. A.] Univ Paris Diderot, CEA Saclay, Serv Astrophys, Lab AIM,CEA IRFU CNRS, F-91191 Gif Sur Yvette, France. [Barbiellini, G.; Desiante, R.; Longo, F.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Barbiellini, G.; Longo, F.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Baring, M. G.] Rice Univ, Dept Phys & Astron, Houston, TX 77251 USA. [Bastieri, D.; Buson, S.; Rando, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bastieri, D.; Buson, S.; Chiaro, G.; Pivato, G.; Rando, R.] Univ Padua, Dipartimento Fis & Astron G Galilei, I-35131 Padua, Italy. [Bechtol, K.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Di Venere, L.; Drell, P. S.; Drlica-Wagner, A.; Focke, W. B.; Franckowiak, A.; Funk, S.; Godfrey, G.; Hayashida, M.; Inoue, Y.; Jogler, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Moskalenko, I. V.; Murgia, S.; Okumura, A.; Omodei, N.; Paneque, D.; Petrosian, V.; Porter, T. A.; Reimer, A.; Reimer, O.; Tajima, H.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Dept Phys, Stanford, CA 94305 USA. [Bechtol, K.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Di Venere, L.; Drell, P. S.; Drlica-Wagner, A.; Focke, W. B.; Franckowiak, A.; Funk, S.; Godfrey, G.; Hayashida, M.; Inoue, Y.; Jogler, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Moskalenko, I. V.; Murgia, S.; Okumura, A.; Omodei, N.; Paneque, D.; Petrosian, V.; Porter, T. A.; Reimer, A.; Reimer, O.; Tajima, H.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Bissaldi, E.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Bissaldi, E.] Univ Trieste, I-34127 Trieste, Italy. [Bonamente, E.; Cecchi, C.; Germani, S.; Lubrano, P.; Tosti, G.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Univ Bari, Dipartimento Fis M Merlin, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Politecn Bari, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Gargano, F.; Giglietto, N.; Giordano, F.; Loparco, F.; Mazziotta, M. 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[Okumura, A.; Tajima, H.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Paneque, D.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Perkins, J. S.] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. [Perkins, J. S.] Univ Maryland Baltimore Cty, Ctr Space Sci & Technol, Baltimore, MD 21250 USA. [Razzaque, S.] Univ Johannesburg, Dept Phys, ZA-2006 Auckland Pk, South Africa. [Reimer, A.; Reimer, O.] Leopold Franzens Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Reimer, A.; Reimer, O.] Leopold Franzens Univ Innsbruck, Inst Theoret Phys, A-6020 Innsbruck, Austria. [Roth, M.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Scargle, J. D.] NASA, Ames Res Ctr, Div Space Sci, Moffett Field, CA 94035 USA. [Siskind, E. J.] NYCB Real Time Comp Inc, Lattingtown, NY 11560 USA. [Sonbas, E.] Adyaman Univ, TR-02040 Adyaman, Turkey. [Torres, D. F.] ICREA, Barcelona, Spain. [Vianello, G.] CIFS, I-10133 Turin, Italy. [Vitale, V.] Univ Roma Tor Vergata, Dipartimento Fis, I-00133 Rome, Italy. [Yamazaki, R.] Aoyama Gakuin Univ, Dept Phys & Math, Sagamihara, Kanagawa 2525258, Japan. [Younes, G.; Kouveliotou, C.; Wilson-Hodge, C.] NASA, George C Marshall Space Flight Ctr, Huntsville, AL 35812 USA. [Kippen, R. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [van der Horst, A. J.] Univ Amsterdam, Astron Inst Anton Pannekoek, NL-1090 GE Amsterdam, Netherlands. [Cusumano, G.; La Parola, V.] INAF Ist Astrofis Spaziale & Fis Cosm, I-90146 Palermo, Italy. [Cummings, J. R.] Univ Maryland Baltimore Cty, Ctr Res & Explorat Space Sci & Technol, Baltimore, MD 21250 USA. RP Chiang, J (reprint author), Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Dept Phys, Stanford, CA 94305 USA. EM jchiang@slac.stanford.edu; charles.dermer@nrl.navy.mil; nicola.omodei@stanford.edu; giacomov@slac.stanford.edu; sjzhu@umd.edu; shaolin.xiong@uah.edu RI Johnson, Neil/G-3309-2014; Reimer, Olaf/A-3117-2013; Morselli, Aldo/G-6769-2011; Nemmen, Rodrigo/O-6841-2014; Funk, Stefan/B-7629-2015; Johannesson, Gudlaugur/O-8741-2015; Loparco, Francesco/O-8847-2015; Mazziotta, Mario /O-8867-2015; Gargano, Fabio/O-8934-2015; giglietto, nicola/I-8951-2012; Moskalenko, Igor/A-1301-2007; Sgro, Carmelo/K-3395-2016; Hays, Elizabeth/D-3257-2012; Bissaldi, Elisabetta/K-7911-2016; Torres, Diego/O-9422-2016; Di Venere, Leonardo/C-7619-2017; OI Reimer, Olaf/0000-0001-6953-1385; Morselli, Aldo/0000-0002-7704-9553; Funk, Stefan/0000-0002-2012-0080; Johannesson, Gudlaugur/0000-0003-1458-7036; Loparco, Francesco/0000-0002-1173-5673; Mazziotta, Mario /0000-0001-9325-4672; Gargano, Fabio/0000-0002-5055-6395; giglietto, nicola/0000-0002-9021-2888; Moskalenko, Igor/0000-0001-6141-458X; Bissaldi, Elisabetta/0000-0001-9935-8106; Torres, Diego/0000-0002-1522-9065; Di Venere, Leonardo/0000-0003-0703-824X; De Angelis, Alessandro/0000-0002-3288-2517; Cusumano, Giancarlo/0000-0002-8151-1990; Inoue, Yoshiyuki/0000-0002-7272-1136; Giordano, Francesco/0000-0002-8651-2394; La Parola, Valentina/0000-0002-8087-6488; Preece, Robert/0000-0003-1626-7335; Caraveo, Patrizia/0000-0003-2478-8018; Sgro', Carmelo/0000-0001-5676-6214; Burgess, James/0000-0003-3345-9515; Bastieri, Denis/0000-0002-6954-8862; Omodei, Nicola/0000-0002-5448-7577; Pesce-Rollins, Melissa/0000-0003-1790-8018; orienti, monica/0000-0003-4470-7094; Giroletti, Marcello/0000-0002-8657-8852; Moretti, Elena/0000-0001-5477-9097; Baldini, Luca/0000-0002-9785-7726; Larsson, Stefan/0000-0003-0716-107X NR 30 TC 65 Z9 67 U1 2 U2 43 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 3 PY 2014 VL 343 IS 6166 BP 42 EP 47 DI 10.1126/science.1242353 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282HR UT WOS:000329162000042 PM 24263133 ER PT J AU Preece, R Burgess, JM von Kienlin, A Bhat, PN Briggs, MS Byrne, D Chaplin, V Cleveland, W Collazzi, AC Connaughton, V Diekmann, A Fitzpatrick, G Foley, S Gibby, M Giles, M Goldstein, A Greiner, J Gruber, D Jenke, P Kippen, RM Kouveliotou, C McBreen, S Meegan, C Paciesas, WS Pelassa, V Tierney, D van der Horst, AJ Wilson-Hodge, C Xiong, S Younes, G Yu, HF Ackermann, M Ajello, M Axelsson, M Baldini, L Barbiellini, G Baring, MG Bastieri, D Bellazzini, R Bissaldi, E Bonamente, E Bregeon, J Brigida, M Bruel, P Buehler, R Buson, S Caliandro, GA Cameron, RA Caraveo, PA Cecchi, C Charles, E Chekhtman, A Chiang, J Chiaro, G Ciprini, S Claus, R Cohen-Tanugi, J Cominsky, LR Conrad, J D'Ammando, F de Angelis, A de Palma, F Dermer, CD Desiante, R Digel, SW Di Venere, L Drell, PS Drlica-Wagner, A Favuzzi, C Franckowiak, A Fukazawa, Y Fusco, P Gargano, F Gehrels, N Germani, S Giglietto, N Giordano, F Giroletti, M Godfrey, G Granot, J Grenier, IA Guiriec, S Hadasch, D Hanabata, Y Harding, AK Hayashida, M Iyyani, S Jogler, T Joannesson, G Kawano, T Knodlseder, J Kocevski, D Kuss, M Lande, J Larsson, J Larsson, S Latronico, L Longo, F Loparco, F Lovellette, MN Lubrano, P Mayer, M Mazziotta, MN Michelson, PF Mizuno, T Monzani, ME Moretti, E Morselli, A Murgia, S Nemmen, R Nuss, E Nymark, T Ohno, M Ohsugi, T Okumura, A Omodei, N Orienti, M Paneque, D Perkins, JS Pesce-Rollins, M Piron, F Pivato, G Porter, TA Racusin, JL Raino, S Rando, R Razzano, M Razzaque, S Reimer, A Reimer, O Ritz, S Roth, M Ryde, F Sartori, A Scargle, JD Schulz, A Sgro, C Siskind, EJ Spandre, G Spinelli, P Suson, DJ Tajima, H Takahashi, H Thayer, JG Thayer, JB Tibaldo, L Tinivella, M Torres, DF Tosti, G Troja, E Usher, TL Vandenbroucke, J Vasileiou, V Vianello, G Vitale, V Werner, M Winer, BL Wood, KS Zhu, S AF Preece, R. Burgess, J. Michael von Kienlin, A. Bhat, P. N. Briggs, M. S. Byrne, D. Chaplin, V. Cleveland, W. Collazzi, A. C. Connaughton, V. Diekmann, A. Fitzpatrick, G. Foley, S. Gibby, M. Giles, M. Goldstein, A. Greiner, J. Gruber, D. Jenke, P. Kippen, R. M. Kouveliotou, C. McBreen, S. Meegan, C. Paciesas, W. S. Pelassa, V. Tierney, D. van der Horst, A. J. Wilson-Hodge, C. Xiong, S. Younes, G. Yu, H. -F. Ackermann, M. Ajello, M. Axelsson, M. Baldini, L. Barbiellini, G. Baring, M. G. Bastieri, D. Bellazzini, R. Bissaldi, E. Bonamente, E. Bregeon, J. Brigida, M. Bruel, P. Buehler, R. Buson, S. Caliandro, G. A. Cameron, R. A. Caraveo, P. A. Cecchi, C. Charles, E. Chekhtman, A. Chiang, J. Chiaro, G. Ciprini, S. Claus, R. Cohen-Tanugi, J. Cominsky, L. R. Conrad, J. D'Ammando, F. de Angelis, A. de Palma, F. Dermer, C. D. Desiante, R. Digel, S. W. Di Venere, L. Drell, P. S. Drlica-Wagner, A. Favuzzi, C. Franckowiak, A. Fukazawa, Y. Fusco, P. Gargano, F. Gehrels, N. Germani, S. Giglietto, N. Giordano, F. Giroletti, M. Godfrey, G. Granot, J. Grenier, I. A. Guiriec, S. Hadasch, D. Hanabata, Y. Harding, A. K. Hayashida, M. Iyyani, S. Jogler, T. Joannesson, G. Kawano, T. Knoedlseder, J. Kocevski, D. Kuss, M. Lande, J. Larsson, J. Larsson, S. Latronico, L. Longo, F. Loparco, F. Lovellette, M. N. Lubrano, P. Mayer, M. Mazziotta, M. N. Michelson, P. F. Mizuno, T. Monzani, M. E. Moretti, E. Morselli, A. Murgia, S. Nemmen, R. Nuss, E. Nymark, T. Ohno, M. Ohsugi, T. Okumura, A. Omodei, N. Orienti, M. Paneque, D. Perkins, J. S. Pesce-Rollins, M. Piron, F. Pivato, G. Porter, T. A. Racusin, J. L. Raino, S. Rando, R. Razzano, M. Razzaque, S. Reimer, A. Reimer, O. Ritz, S. Roth, M. Ryde, F. Sartori, A. Scargle, J. D. Schulz, A. Sgro, C. Siskind, E. J. Spandre, G. Spinelli, P. Suson, D. J. Tajima, H. Takahashi, H. Thayer, J. G. Thayer, J. B. Tibaldo, L. Tinivella, M. Torres, D. F. Tosti, G. Troja, E. Usher, T. L. Vandenbroucke, J. Vasileiou, V. Vianello, G. Vitale, V. Werner, M. Winer, B. L. Wood, K. S. Zhu, S. TI The First Pulse of the Extremely Bright GRB 130427A: A Test Lab for Synchrotron Shocks SO SCIENCE LA English DT Article ID GAMMA-RAY BURSTS; BATSE OBSERVATIONS; PROMPT EMISSION; PEAK ENERGY; COMPONENT; SPECTRA AB Gamma-ray burst (GRB) 130427A is one of the most energetic GRBs ever observed. The initial pulse up to 2.5 seconds is possibly the brightest well-isolated pulse observed to date. A fine time resolution spectral analysis shows power-law decays of the peak energy from the onset of the pulse, consistent with models of internal synchrotron shock pulses. However, a strongly correlated power-law behavior is observed between the luminosity and the spectral peak energy that is inconsistent with curvature effects arising in the relativistic outflow. It is difficult for any of the existing models to account for all of the observed spectral and temporal behaviors simultaneously. C1 [Preece, R.] Univ Alabama, Dept Space Sci, Huntsville, AL 35899 USA. [Burgess, J. Michael; Bhat, P. N.; Briggs, M. S.; Chaplin, V.; Connaughton, V.; Jenke, P.; Meegan, C.; Pelassa, V.; Xiong, S.] Univ Alabama, CSPAR, Huntsville, AL 35899 USA. [von Kienlin, A.; Foley, S.; Greiner, J.; Gruber, D.; McBreen, S.; Yu, H. -F.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Byrne, D.; Fitzpatrick, G.; Foley, S.; McBreen, S.; Tierney, D.] Univ Coll Dublin, Dublin 4, Ireland. [Cleveland, W.; Paciesas, W. S.; Younes, G.] USRA, Columbia, MD 21044 USA. [Collazzi, A. C.; Goldstein, A.; Kouveliotou, C.; Wilson-Hodge, C.; Younes, G.] NASA, George C Marshall Space Flight Ctr, Huntsville, AL 35812 USA. [Diekmann, A.; Gibby, M.; Giles, M.] Jacobs Technol, Huntsville, AL 35806 USA. [Kippen, R. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [van der Horst, A. J.] Univ Amsterdam, Astron Inst Anton Pannekoek, NL-1090 GE Amsterdam, Netherlands. [Ackermann, M.; Buehler, R.; Mayer, M.; Schulz, A.] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Ajello, M.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Axelsson, M.; Larsson, S.] Stockholm Univ, Dept Astron, SE-10691 Stockholm, Sweden. [Axelsson, M.; Conrad, J.; Iyyani, S.; Larsson, J.; Larsson, S.; Moretti, E.; Nymark, T.] Oskar Klein Ctr Cosmoparticle Phys, SE-10691 Stockholm, Sweden. [Axelsson, M.; Iyyani, S.; Larsson, J.; Moretti, E.; Nymark, T.; Ryde, F.] AlbaNova, Royal Inst Technol KTH, Dept Phys, SE-10691 Stockholm, Sweden. [Baldini, L.] Univ Pisa, I-56127 Pisa, Italy. [Baldini, L.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Barbiellini, G.; Desiante, R.; Longo, F.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Barbiellini, G.; Longo, F.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Baring, M. G.] Rice Univ, Dept Phys & Astron, Houston, TX 77251 USA. [Bastieri, D.; Buson, S.; Rando, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bastieri, D.; Buson, S.; Chiaro, G.; Pivato, G.; Rando, R.] Univ Padua, Dipartimento Fis & Astron G Galilei, I-35131 Padua, Italy. [Bellazzini, R.; Bregeon, J.; Kuss, M.; Pesce-Rollins, M.; Razzano, M.; Sgro, C.; Spandre, G.; Tinivella, M.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Bissaldi, E.; Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Bissaldi, E.; Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Theoret Phys, A-6020 Innsbruck, Austria. [Bonamente, E.; Cecchi, C.; Germani, S.; Lubrano, P.; Tosti, G.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Bonamente, E.; Cecchi, C.; Germani, S.; Lubrano, P.; Tosti, G.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Univ Bari, Dipartimento Fis M Merlin, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Politecn Bari, I-70126 Bari, Italy. [Brigida, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Gargano, F.; Giglietto, N.; Giordano, F.; Loparco, F.; Mazziotta, M. N.; Raino, S.; Spinelli, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Bruel, P.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Caliandro, G. A.; Hadasch, D.; Torres, D. F.] CSIC, Inst CiEncies Espai IEEE, Barcelona 08193, Spain. [Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Digel, S. W.; Di Venere, L.; Drell, P. S.; Drlica-Wagner, A.; Franckowiak, A.; Godfrey, G.; Hayashida, M.; Jogler, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Murgia, S.; Okumura, A.; Omodei, N.; Paneque, D.; Porter, T. A.; Reimer, A.; Reimer, O.; Tajima, H.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Digel, S. W.; Di Venere, L.; Drell, P. S.; Drlica-Wagner, A.; Franckowiak, A.; Godfrey, G.; Hayashida, M.; Jogler, T.; Kocevski, D.; Lande, J.; Michelson, P. F.; Monzani, M. E.; Murgia, S.; Okumura, A.; Omodei, N.; Paneque, D.; Porter, T. A.; Reimer, A.; Reimer, O.; Tajima, H.; Thayer, J. G.; Thayer, J. B.; Tibaldo, L.; Usher, T. L.; Vandenbroucke, J.; Vianello, G.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Caraveo, P. A.; Sartori, A.] INAF Ist Astrofis Spaziale & Fis Cosm, I-20133 Milan, Italy. [Chekhtman, A.] George Mason Univ, Coll Sci, Ctr Earth Observing & Space Res, Fairfax, VA 22030 USA. [Chekhtman, A.] Naval Res Lab, Washington, DC 20375 USA. [Ciprini, S.] ASI Sci Data Ctr, I-00044 Frascati, Roma, Italy. [Ciprini, S.] Osserv Astron Roma, Ist Nazl Astrofis, I-00040 Monte Porzio Catone, Roma, Italy. [Cohen-Tanugi, J.; Nuss, E.; Piron, F.; Vasileiou, V.] Univ Montpellier 2, CNRS, IN2P3, Lab Univers & Particules Montpellier, Montpellier, France. [Cominsky, L. R.] Sonoma State Univ, Dept Phys & Astron, Rohnert Pk, CA 94928 USA. [Conrad, J.; Iyyani, S.; Larsson, S.] Stockholm Univ, AlbaNova, Dept Phys, SE-10691 Stockholm, Sweden. [D'Ammando, F.; Giroletti, M.; Orienti, M.] INAF Ist Radioastron, I-40129 Bologna, Italy. [de Angelis, A.] Univ Udine, Dipartimento Fis, I-33100 Udine, Italy. [de Angelis, A.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, I-33100 Udine, Italy. [Dermer, C. D.; Lovellette, M. N.; Wood, K. S.] Naval Res Lab, Div Space Sci, Washington, DC 20375 USA. [Fukazawa, Y.; Hanabata, Y.; Kawano, T.; Takahashi, H.] Hiroshima Univ, Dept Phys Sci, Hiroshima 7398526, Japan. [Gehrels, N.; Guiriec, S.; Harding, A. K.; Nemmen, R.; Perkins, J. S.; Racusin, J. L.; Troja, E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Granot, J.] Open Univ Israel, Dept Nat Sci, IL-43537 Raanana, Israel. [Grenier, I. A.] Univ Paris Diderot, CEA IRFU CNRS, Lab AIM, Serv Astrophys, F-91191 Gif Sur Yvette, France. [Hayashida, M.] Kyoto Univ, Grad Sch Sci, Dept Astron, Sakyo Ku, Kyoto 6068502, Japan. [Joannesson, G.] Univ Iceland, Inst Sci, IS-107 Reykjavik, Iceland. [Knoedlseder, J.] CNRS, IRAP, F-31028 Toulouse 4, France. [Knoedlseder, J.] Univ Toulouse, UPS OMP, IRAP, GAHEC, Toulouse, France. [Latronico, L.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Mizuno, T.; Ohsugi, T.] Hiroshima Univ, Hiroshima Astrophys Sci Ctr, Hiroshima 7398526, Japan. [Morselli, A.; Vitale, V.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Ohno, M.] Japan Aerosp Explorat Agcy JAXA, Inst Space & Astronaut Sci, Chuo Ku, Sagamihara, Kanagawa 2525210, Japan. [Okumura, A.; Tajima, H.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Paneque, D.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Perkins, J. S.] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. [Perkins, J. S.] Univ Maryland Baltimore Cty, Ctr Space Sci & Technol, Baltimore, MD 21250 USA. [Perkins, J. S.] CRESST, Greenbelt, MD 20771 USA. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Razzano, M.; Ritz, S.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Razzano, M.; Ritz, S.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Razzaque, S.] Univ Johannesburg, Dept Phys, ZA-2006 Auckland Pk, South Africa. [Roth, M.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Scargle, J. D.] NASA, Ames Res Ctr, Div Space Sci, Moffett Field, CA 94035 USA. [Siskind, E. J.] NYCB Real Time Comp Inc, Lattingtown, NY 11560 USA. [Suson, D. J.] Purdue Univ Calumet, Dept Chem & Phys, Hammond, IN 46323 USA. ICREA, Barcelona, Spain. [Troja, E.; Zhu, S.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Troja, E.; Zhu, S.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Vianello, G.] CIFS, I-10133 Turin, Italy. [Vitale, V.] Univ Roma Tor Vergata, Dipartimento Fis, I-00133 Rome, Italy. [Winer, B. L.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Dept Phys, Columbus, OH 43210 USA. RP Preece, R (reprint author), Univ Alabama, Dept Space Sci, Huntsville, AL 35899 USA. EM preecer@uah.edu; James.Burgess@uah.edu; azk@mpe.mpg.de; charles.dermer@nrl.navy.mil; nicola.omodei@stanford.edu RI Sgro, Carmelo/K-3395-2016; Reimer, Olaf/A-3117-2013; Morselli, Aldo/G-6769-2011; Bissaldi, Elisabetta/K-7911-2016; Torres, Diego/O-9422-2016; Di Venere, Leonardo/C-7619-2017; Iyyani, Shabnam/D-8736-2017; Nemmen, Rodrigo/O-6841-2014; Johannesson, Gudlaugur/O-8741-2015; Loparco, Francesco/O-8847-2015; Mazziotta, Mario /O-8867-2015; Gargano, Fabio/O-8934-2015; giglietto, nicola/I-8951-2012; OI Reimer, Olaf/0000-0001-6953-1385; Morselli, Aldo/0000-0002-7704-9553; Bissaldi, Elisabetta/0000-0001-9935-8106; Torres, Diego/0000-0002-1522-9065; Di Venere, Leonardo/0000-0003-0703-824X; Iyyani, Shabnam/0000-0002-2525-3464; Johannesson, Gudlaugur/0000-0003-1458-7036; Loparco, Francesco/0000-0002-1173-5673; Mazziotta, Mario /0000-0001-9325-4672; Gargano, Fabio/0000-0002-5055-6395; giglietto, nicola/0000-0002-9021-2888; Giordano, Francesco/0000-0002-8651-2394; Preece, Robert/0000-0003-1626-7335; Caraveo, Patrizia/0000-0003-2478-8018; Sgro', Carmelo/0000-0001-5676-6214; SPINELLI, Paolo/0000-0001-6688-8864; Burgess, James/0000-0003-3345-9515; Bastieri, Denis/0000-0002-6954-8862; Omodei, Nicola/0000-0002-5448-7577; /0000-0003-0065-2933; Pesce-Rollins, Melissa/0000-0003-1790-8018; Giroletti, Marcello/0000-0002-8657-8852; Moretti, Elena/0000-0001-5477-9097; Baldini, Luca/0000-0002-9785-7726; Larsson, Stefan/0000-0003-0716-107X NR 29 TC 28 Z9 29 U1 2 U2 30 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 3 PY 2014 VL 343 IS 6166 BP 51 EP 54 DI 10.1126/science.1242302 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282HR UT WOS:000329162000044 PM 24263132 ER PT J AU Talin, AA Centrone, A Ford, AC Foster, ME Stavila, V Haney, P Kinney, RA Szalai, V El Gabaly, F Yoon, HP Leonard, F Allendorf, MD AF Talin, A. Alec Centrone, Andrea Ford, Alexandra C. Foster, Michael E. Stavila, Vitalie Haney, Paul Kinney, R. Adam Szalai, Veronika El Gabaly, Farid Yoon, Heayoung P. Leonard, Francois Allendorf, Mark D. TI Tunable Electrical Conductivity in Metal-Organic Framework Thin-Film Devices SO SCIENCE LA English DT Article ID CHARGE-TRANSFER; CU-3(BTC)(2); SPECTROSCOPY; ELECTRODES; MECHANISM; ROUTE AB We report a strategy for realizing tunable electrical conductivity in metal-organic frameworks (MOFs) in which the nanopores are infiltrated with redox-active, conjugated guest molecules. This approach is demonstrated using thin-film devices of the MOF Cu-3(BTC)(2) (also known as HKUST-1; BTC, benzene-1,3,5-tricarboxylic acid) infiltrated with the molecule 7,7,8,8-tetracyanoquinododimethane (TCNQ). Tunable, air-stable electrical conductivity over six orders of magnitude is achieved, with values as high as 7 siemens per meter. Spectroscopic data and first-principles modeling suggest that the conductivity arises from TCNQ guest molecules bridging the binuclear copper paddlewheels in the framework, leading to strong electronic coupling between the dimeric Cu subunits. These ohmically conducting porous MOFs could have applications in conformal electronic devices, reconfigurable electronics, and sensors. C1 [Talin, A. Alec; Ford, Alexandra C.; Foster, Michael E.; Stavila, Vitalie; El Gabaly, Farid; Leonard, Francois; Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. [Talin, A. Alec; Centrone, Andrea; Haney, Paul; Kinney, R. Adam; Szalai, Veronika; Yoon, Heayoung P.] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. [Centrone, Andrea; Kinney, R. Adam; Yoon, Heayoung P.] Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA. RP Talin, AA (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM aatalin@sandia.gov; mdallen@sandia.gov FU Laboratory Directed Research and Development Program at Sandia National Laboratories; U.S. Department of Energy (DOE) SunShot Program; U.S. DOE National Nuclear Security Administration [DE-AC04-94AL85000]; Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DESC0001160]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. DOE [DE-AC04-94AL85000]; University of Maryland [70NANB10H193]; National Institute of Standards and Technology Center for Nanoscale Science and Technology through the University of Maryland [70NANB10H193] FX We thank S. T. Meek for organic synthesis in this work and D. Ruzmetov for help in fabrication. This work was supported by the Laboratory Directed Research and Development Program at Sandia National Laboratories and the U.S. Department of Energy (DOE) SunShot Program. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin company, for the U.S. DOE National Nuclear Security Administration under contract DE-AC04-94AL85000. A. A. T. was supported by the Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, Office of Basic Energy Sciences under award DESC0001160. F. E. G. was supported by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. DOE, under contract DE-AC04-94AL85000. A. C., R. A. K., and H.P.Y. acknowledge support under the Cooperative Research Agreement between the University of Maryland and the National Institute of Standards and Technology Center for Nanoscale Science and Technology, award 70NANB10H193, through the University of Maryland. NR 21 TC 250 Z9 251 U1 115 U2 849 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 3 PY 2014 VL 343 IS 6166 BP 66 EP 69 DI 10.1126/science.1246738 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282HR UT WOS:000329162000048 PM 24310609 ER PT J AU Lopez, I Ertem, MZ Maji, S Benet-Buchholz, J Keidel, A Kuhlmann, U Hildebrandt, P Cramer, CJ Batista, VS Llobet, A AF Lopez, Isidoro Ertem, Mehmed Z. Maji, Somnath Benet-Buchholz, Jordi Keidel, Anke Kuhlmann, Uwe Hildebrandt, Peter Cramer, Christopher J. Batista, Victor S. Llobet, Antoni TI A Self-Improved Water-Oxidation Catalyst: Is One Site Really Enough? SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE density functional calculations; reaction mechanisms; resonance Raman spectroscopy; ruthenium electrochemistry; water-oxidation catalysis ID RUTHENIUM OXO COMPLEXES; DENSITY FUNCTIONALS; BRIDGED COMPLEXES; MONONUCLEAR; REACTIVITIES; REDOX; 1,4,7-TRIMETHYL-1,4,7-TRIAZACYCLONONANE; EPOXIDATION; MECHANISM; KINETICS AB The homogeneous catalysis of water oxidation by transition-metal complexes has experienced spectacular development over the last five years. Practical energy-conversion schemes, however, require robust catalysts with large turnover frequencies. Herein we introduce a new oxidatively rugged and powerful dinuclear water-oxidation catalyst that is generated by self-assembly from a mononuclear catalyst during the catalytic process. Our kinetic and DFT computational analysis shows that two interconnected catalytic cycles coexist while the mononuclear system is slowly and irreversibly converted into the more stable dinuclear system: an extremely robust water-oxidation catalyst that does not decompose over extended periods of time. C1 [Lopez, Isidoro; Maji, Somnath; Benet-Buchholz, Jordi; Llobet, Antoni] Inst Chem Res Catalonia ICIQ, Tarragona 43007, Spain. [Keidel, Anke; Kuhlmann, Uwe; Hildebrandt, Peter] Tech Univ Berlin, Inst Chem, D-10623 Berlin, Germany. [Ertem, Mehmed Z.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Ertem, Mehmed Z.; Batista, Victor S.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Cramer, Christopher J.] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Cramer, Christopher J.] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. RP Cramer, CJ (reprint author), Univ Minnesota, Dept Chem, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM allobet@iciq.cat RI Hildebrandt, Peter/J-5658-2014; Benet-Buchholz, Jordi/L-1374-2014; Cramer, Christopher/B-6179-2011; Llobet, Antoni/C-3296-2016 OI Hildebrandt, Peter/0000-0003-1030-5900; Benet-Buchholz, Jordi/0000-0003-3984-3550; Cramer, Christopher/0000-0001-5048-1859; Llobet, Antoni/0000-0002-6176-5272 FU MINECO [CTQ2010-21497, PRI-PIBIN-2011-1278]; FPU; Torres Quevedo; Cluster of Excellence (UniCat); US Department of Energy (DOE) [DE-SC0001423]; Computational Materials and Chemical Sciences (CMCSN) project at Brookhaven National Laboratory with the US DOE [DE-AC02-98CH10886]; Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences; US National Science Foundation [CHE-0952054] FX Support from MINECO (CTQ2010-21497 and PRI-PIBIN-2011-1278), an FPU grant to I.L., and a Torres Quevedo contract to S.M. are gratefully acknowledged. Support has also been received from the Cluster of Excellence (UniCat) and the US Department of Energy (DOE) (Grant DE-SC0001423 to V.S.B.). M.Z.E. received funding from a Computational Materials and Chemical Sciences (CMCSN) project at Brookhaven National Laboratory under contract DE-AC02-98CH10886 with the US DOE and was supported by its Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences. C.J.C. acknowledges support from the US National Science Foundation (CHE-0952054). NR 46 TC 36 Z9 36 U1 5 U2 110 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 3 PY 2014 VL 53 IS 1 BP 205 EP 209 DI 10.1002/anie.201307509 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 275YI UT WOS:000328714900027 PM 24259487 ER PT J AU Hunault, M Robert, JL Newville, M Galoisy, L Calas, G AF Hunault, M. Robert, J-L. Newville, M. Galoisy, L. Calas, G. TI Spectroscopic properties of five-coordinated Co2+ in phosphates SO SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY LA English DT Article DE Cobalt(II); Phosphates; Five-coordination; XANES; UV-vis-NIR spectroscopy ID CRYSTAL-STRUCTURE; MAGNETIC-PROPERTIES; CERAMIC PIGMENTS; OPTICAL SPECTRA; COBALT; COMPLEXES; GLASSES; XANES; SITES; ORTHOPHOSPHATE AB Co-3(PO4)(2), SrCo2(PO4)(2), CO2P2O7, BaCoP2O7 and SrCoP2O7 present different geometries of five-coordinated Co2+ (Co-[5](2+)) sites, coexisting with Co-[6](2+) in Co-3(PO4)(2) and CO2P2O7, and Co-[4](2+) in SrCo2(PO4)(2). (CO)-C-[5] K-edge XANES spectra show that the intensity of the pre-edge and main-edge is intermediate between those of ([6])- and Co-[4]. Diffuse reflectance spectra show the contributions of Co2+ in (D-3h) symmetry for SrCo2(PO4)(2), and (C-4v) symmetry for BaCoP2O7 and SrCoP2O7. In Co-3(PO4)(2) and CO2P2O7 the multiple transitions observed arise from energy level splitting and may be labeled in (C-2v) symmetry. Spectroscopic data confirm that (D-3h) and (C-4v) symmetries may be distinguished upon the intensity of the optical absorption bands and crystal field splitting values. We discuss the influence of the geometrical distortion and of the nature of the next nearest neighbors. (C) 2013 Elsevier BM. All rights reserved. C1 [Hunault, M.; Robert, J-L.; Galoisy, L.; Calas, G.] Univ Paris 06, CNRS, IMPMC, UMR 7590, F-75252 Paris 05, France. [Newville, M.] Univ Chicago, Consortium Adv Radiat Sci, Adv Photon Source, GSECARS, Argonne, IL 60439 USA. RP Hunault, M (reprint author), Univ Paris 06, CNRS, IMPMC, UMR 7590, Case Courrier 115,4 Pl Jussieu, F-75252 Paris 05, France. EM myrtille.hunault@impmc.upmc.fr RI Calas, Georges/B-2445-2012; OI Calas, Georges/0000-0003-0525-5734; Hunault, Myrtille/0000-0002-3754-8630 FU National Science Foundation - Earth Sciences [EAR-1128799]; Department of Energy - Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX XANES spectroscopy was performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation - Earth Sciences (EAR-1128799) and Department of Energy - Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 38 TC 7 Z9 7 U1 7 U2 62 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1386-1425 J9 SPECTROCHIM ACTA A JI Spectroc. Acta Pt. A-Molec. Biomolec. Spectr. PD JAN 3 PY 2014 VL 117 BP 406 EP 412 DI 10.1016/j.saa.2013.08.021 PG 7 WC Spectroscopy SC Spectroscopy GA 268OH UT WOS:000328179900055 PM 24001982 ER PT J AU Dong, HN Dorfman, SM Holl, CM Meng, Y Prakapenka, VB He, DW Duffy, TS AF Dong, Haini Dorfman, Susannah M. Holl, Christopher M. Meng, Yue Prakapenka, Vitali B. He, Duanwei Duffy, Thomas S. TI Compression of lithium fluoride to 92GPa SO HIGH PRESSURE RESEARCH LA English DT Article DE equation of state; lithium fluoride; X-ray diffraction ID EQUATION-OF-STATE; HIGH-PRESSURES; ELASTIC-CONSTANTS; ALKALI-HALIDES; THERMAL EXPANSIVITY; NACL; LIF; TEMPERATURE; NAF; CRYSTALS AB The equation of state and compression behavior of lithium fluoride, LiF, have been determined to 92GPa by X-ray diffraction in a diamond anvil cell. A neon pressure-transmitting medium was used to minimize the effect of differential stress on the sample. Consistent results using multiple pressure standards were obtained. By fitting the pressure-volume data to a Birch-Murnaghan equation of state, the isothermal bulk modulus and its corresponding pressure derivative at zero pressure were determined to be K-0=70.1 +/- 0.7GPa, and K '(0)=4.3 +/- 0.1. If the bulk modulus is fixed at 66.2GPa, a value well constrained by independent elasticity measurements, we obtain K '(0)=4.6 +/- 0.1. The bulk modulus and its pressure derivative obtained from this work resolve the large discrepancy in previously reported values of K-0 and K '(0) for this material. Consequently, the equation of state of LiF is now sufficiently well constrained to allow its use as a pressure calibrant in high pressure experiments. C1 [Dong, Haini; Dorfman, Susannah M.; Holl, Christopher M.; Duffy, Thomas S.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Dong, Haini; He, Duanwei] Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China. [Meng, Yue] Carnegie Inst Sci, HPCAT, Argonne, IL 60439 USA. [Prakapenka, Vitali B.] Univ Chicago, Argonne Natl Lab, CARS, Argonne, IL 60439 USA. RP Dong, HN (reprint author), Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. EM hdong1229@gmail.com RI Duffy, Thomas/C-9140-2017; OI Duffy, Thomas/0000-0002-5357-1259; Dorfman, Susannah/0000-0002-3968-9592 FU NSF; Carnegie-DOE Alliance Center; COMPRES; GeoSoilEnviroCARS; NSF-Earth Sciences [EAR-1128799]; DOE-Geosciences [DE-FG02-94ER14466]; CIW; CDAC; UNLV; LLNL through DOE-NNSA; LLNL through DOE-BES; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the NSF and the Carnegie-DOE Alliance Center. We thank C. Stan and G. Finkelstein for their experimental assistance. High pressure gas loading was supported by COMPRES and GeoSoilEnviroCARS. Experiments were performed at GeoSoilEnviroCARS (Sector 13) and High Pressure Collaborative Access Team (HPCAT, Sector 16) at the APS. GeoSoilEnviroCARS is supported by the NSF-Earth Sciences (EAR-1128799) and DOE-Geosciences (DE-FG02-94ER14466). HPCAT is supported by CIW, CDAC, UNLV, and LLNL through funding from DOE-NNSA and DOE-BES, with partial instrumentation funding by NSF. The use of the APS was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 43 TC 3 Z9 3 U1 1 U2 15 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-7959 EI 1477-2299 J9 HIGH PRESSURE RES JI High Pressure Res. PD JAN 2 PY 2014 VL 34 IS 1 BP 39 EP 48 DI 10.1080/08957959.2013.878932 PG 10 WC Physics, Multidisciplinary SC Physics GA AE4XJ UT WOS:000333989600004 ER PT J AU Uhoya, W Cargill, D Gofryk, K Tsoi, GM Vohra, YK Sefat, AS Weir, ST AF Uhoya, Walter Cargill, Daniel Gofryk, Krzysztof Tsoi, Georgiy M. Vohra, Yogesh K. Sefat, Athena S. Weir, S. T. TI High pressure effects on the superconductivity in rare-earth-doped CaFe2As2 SO HIGH PRESSURE RESEARCH LA English DT Article DE electrical transport; X-ray diffraction; high pressure; iron based compounds; superconductivity ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; AMBIENT AB High pressure superconductivity in a rare-earth-doped Ca0.86Pr0.14Fe2As2 single-crystalline sample has been studied up to 12 GPa and temperatures down to 11 K using the designer diamond anvil cell under a quasi-hydrostatic pressure medium. The electrical resistance measurements were complemented by high pressure and low-temperature X-ray diffraction studies at a synchrotron source. The electrical resistance measurements show an intriguing observation of superconductivity under pressure, with T-c as high as similar to 51 K at 1.9 GPa, presenting the highest T-c reported in the intermetallic class of 122 iron-based superconductors. The resistive transition observed suggests a possible existence of two superconducting phases at low pressures of 0.5 GPa: one phase starting at T-c1 similar to 48 K and the other starts at T-c2 similar to 16 K. The two superconducting transitions show distinct variations with increasing pressure. High pressure and low-temperature structural studies indicate that the superconducting phase is a collapsed tetragonal ThCr2Si2-type (122) crystal structure. C1 [Uhoya, Walter; Cargill, Daniel; Tsoi, Georgiy M.; Vohra, Yogesh K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Cargill, Daniel] Hendrix Coll, Dept Phys, Conway, AR USA. [Gofryk, Krzysztof; Sefat, Athena S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Weir, S. T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Vohra, YK (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. EM ykvohra@uab.edu RI Gofryk, Krzysztof/F-8755-2014; Sefat, Athena/R-5457-2016; Uhoya, Walter/D-5476-2014 OI Sefat, Athena/0000-0002-5596-3504; Gofryk, Krzysztof/0000-0002-8681-6857; Uhoya, Walter/0000-0002-3197-7629 FU National Aeronautics and Space Administration (NASA) - Alabama Space Grant Consortium, Research Experiences for Undergraduates (REU) program [NNX10AJ80H]; Carnegie/Department of Energy (DOE) Alliance Center (CDAC) [DE-NA0002006]; Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX Daniel Cargill acknowledges support from the National Aeronautics and Space Administration (NASA) - Alabama Space Grant Consortium, Research Experiences for Undergraduates (REU) program under Award No. NNX10AJ80H. Walter Uhoya acknowledges support from the Carnegie/Department of Energy (DOE) Alliance Center (CDAC) under grant no. DE-NA0002006. The work at ORNL was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Portions of this work were performed in a synchrotron facility at HPCAT (Sector 16), Advanced Photon Source (APS) and Argonne National Laboratory. We are grateful to J. E. Mitchell for growing the single crystal of Ca0.86Pr0.14Fe2As2. NR 28 TC 3 Z9 3 U1 1 U2 33 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-7959 EI 1477-2299 J9 HIGH PRESSURE RES JI High Pressure Res. PD JAN 2 PY 2014 VL 34 IS 1 BP 49 EP 58 DI 10.1080/08957959.2013.879867 PG 10 WC Physics, Multidisciplinary SC Physics GA AE4XJ UT WOS:000333989600005 ER PT J AU Anderson, AJ Yan, H Mayanovic, RA Solferino, G Benmore, CJ AF Anderson, Alan J. Yan, Hao Mayanovic, Robert A. Solferino, Giulio Benmore, Chris J. TI High-energy X-ray diffraction of a hydrous silicate liquid under conditions of high pressure and temperature in a modified hydrothermal diamond anvil cell SO HIGH PRESSURE RESEARCH LA English DT Article DE hydrothermal diamond anvil cell; high-energy X-ray diffraction; hydrous silicate liquid; high pressure; high temperature ID GEOCHEMICAL IMPLICATIONS; NEUTRON-DIFFRACTION; WATER; MELTS; INTENSITIES; SOLUBILITY; SCATTERING; GLASSES; FLUIDS; KBAR AB In situ high-energy X-ray diffraction measurements were made for the first time on a water-saturated silicate melt at high pressure and temperature. A modified hydrothermal diamond anvil cell (HDAC), designed to minimize the path length of the X-ray beam within a diamond anvil and to increase the solid angle of the diffracted beam, was used to reduce high background contributions and extend X-ray diffraction data collection in Q space. Quantitative differential pair distribution function (PDF) analysis of X-ray diffraction data show that the first measurable (Si-O) peak is 0.095 angstrom greater in length in the hydrous melt than in the starting glass. Contributions from the H2O O-O correlations, as well as from the second nearest neighbor O-O correlations within the silicate melt, are evident within the second peak of the differential PDF. The procedure described opens new opportunities to directly investigate volatile-rich melts at high pressure and temperature. C1 [Anderson, Alan J.; Solferino, Giulio] St Francis Xavier Univ, Dept Earth Sci, Antigonish, NS B2G 2W5, Canada. [Yan, Hao; Mayanovic, Robert A.] Missouri State Univ, Dept Phys Astron & Mat Sci, Springfield, MO USA. [Benmore, Chris J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Anderson, AJ (reprint author), St Francis Xavier Univ, Dept Earth Sci, Antigonish, NS B2G 2W5, Canada. EM aanderso@stfx.ca OI Benmore, Chris/0000-0001-7007-7749 FU GEN-IV program; Natural Resources Canada through the Office of Energy Research and Development, Atomic Energy of Canada Limited; Natural Sciences and Engineering Research Council of Canada; EFree, an Energy Frontier Research Center; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SG0001057]; US DOE [DE-AC02-06CH11357] FX We thank Dr Jon Almer and Dr S. Shastri for their assistance with our experiments at sector 1-ID of the APS. We are grateful to Dr Richard Wirth of the GFZ, Potsdam for his TEM examination of the glass samples used in this study. A.J.A. acknowledges support from the GEN-IV program. Prof. Peter Ulmer (ETH Zurich) is acknowledged for assisting G. S. in the preparation of the glass used in this study. Funding to the Canada Gen-IV National Program was provided by Natural Resources Canada through the Office of Energy Research and Development, Atomic Energy of Canada Limited, and Natural Sciences and Engineering Research Council of Canada. R. A. M. and H.Y. were supported as part of the EFree, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SG0001057. Use of the APS, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 31 TC 1 Z9 1 U1 2 U2 18 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-7959 EI 1477-2299 J9 HIGH PRESSURE RES JI High Pressure Res. PD JAN 2 PY 2014 VL 34 IS 1 BP 100 EP 109 DI 10.1080/08957959.2013.870565 PG 10 WC Physics, Multidisciplinary SC Physics GA AE4XJ UT WOS:000333989600010 ER PT J AU Davisson, ML Rose, TP AF Davisson, M. Lee Rose, Tim P. TI Recharge and Flow in the Medicine Lake Volcano-Fall River Springs Groundwater Basin, California SO ENVIRONMENTAL FORENSICS LA English DT Article DE Medicine Lake; groundwater; Fall River; magmatic; isotopes ID NOBLE-GASES; NORTHERN CALIFORNIA; STABLE-ISOTOPES; CARBON-DIOXIDE; CASCADE RANGE; RADIOCARBON; ISLAND; AREA; PRECIPITATION; HYDROLOGY AB Isotopic measurements of the 34m(3)/s discharge from the Fall River Springs of northern California indicate recharge from 50km upgradient in high elevation regions of Medicine Lake Volcano. Age determinations suggest less than 20-year travel time. Data demonstrate Klamath Basin further north cannot be a recharge source. Mass balance calculations support that annual precipitation on the volcano supplies observed spring discharge, requiring 50%-75% recharge rates. Radiocarbon and delta C-13 of dissolved inorganic carbon indicate 30%-40% is derived from magmatic CO2. Measured excess He-3 is also consistent with the presence of magmatic gas derived from the Quaternary Age Medicine Lake Volcano. C1 [Davisson, M. Lee] ML Davisson & Associates Inc, Livermore, CA 94550 USA. [Rose, Tim P.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Davisson, ML (reprint author), ML Davisson & Associates Inc, 1228 Jessica Dr, Livermore, CA 94550 USA. EM mldavissonassoc@gmail.com FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 55 TC 0 Z9 0 U1 1 U2 9 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1527-5922 EI 1527-5930 J9 ENVIRON FORENSICS JI Environ. Forensics PD JAN 2 PY 2014 VL 15 IS 1 BP 66 EP 77 DI 10.1080/15275922.2013.873097 PG 12 WC Environmental Sciences SC Environmental Sciences & Ecology GA AD7YP UT WOS:000333483700008 ER PT J AU Li, W Wei, XY Zhu, JX Ting, CS Chen, Y AF Li, Wei Wei, Xin-Yuan Zhu, Jian-Xin Ting, C. S. Chen, Yan TI Pressure-induced topological quantum phase transition in Sb2Se3 SO PHYSICAL REVIEW B LA English DT Article ID SINGLE DIRAC CONE; INSULATOR; SURFACE; BI2TE3; SCHEMES; STATES; WELLS AB Based on the first-principles band structure calculations, we investigate the effects of hydrostatic pressure on the conventional insulator (CI) Sb2Se3 and predict that it undergoes a topological quantum phase transition from a CI to a nontrivial topological insulator at a critical pressure value. The pressure-induced topological quantum phase transition is confirmed by calculating the evolution of the bulk energy gap as a function of pressure, the inversion of energy band structure, and the Z(2) topological invariant, as well as the existence of the Dirac-like topological surface states. Our predictions can be tested by both spectroscopy and transport experiments. C1 [Li, Wei] Chinese Acad Sci, Shanghai Ctr Superconduct, Shanghai 200050, Peoples R China. [Li, Wei] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China. [Li, Wei; Wei, Xin-Yuan; Chen, Yan] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Li, Wei; Wei, Xin-Yuan; Chen, Yan] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Ting, C. S.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Ting, C. S.] Univ Houston, Dept Phys, Houston, TX 77204 USA. RP Li, W (reprint author), Chinese Acad Sci, Shanghai Ctr Superconduct, Shanghai 200050, Peoples R China. RI Chen, Yan/B-2158-2012 OI Chen, Yan/0000-0002-1906-1802 FU State Key Programs of China [2012CB921604, 2009CB929204]; National Natural Science Foundation of China [11074043, 11274069, 61171011, 11227902]; Robert A. Welch Foundation [E-1146]; National Nuclear Security Administration of the U.S. Department of Energy at LANL [DE-AC52-06NA25396]; U.S. Department of Energy Office of Basic Energy Sciences; Chinese Academy of Sciences [XDB04010600] FX We thank R. B. Tao, Z. Fang, X. M. Xie, Z. Liu, J.-H. She, B. Gao, D. W. Shen, G. Xu, and Q. S. Wu for helpful discussions. This work was supported by the State Key Programs of China (Grants No. 2012CB921604 and No. 2009CB929204) and the National Natural Science Foundation of China (Grants No. 11074043 and No. 11274069) (W. L. and Y.C.), the National Natural Science Foundation of China Grant No. 61171011 (X.-Y.W.), the Robert A. Welch Foundation under Grant No. E-1146 (C. S. T.), and the National Nuclear Security Administration of the U.S. Department of Energy at LANL under Contract No. DE-AC52-06NA25396 and the U.S. Department of Energy Office of Basic Energy Sciences (J.-X.Z.). W. L. also gratefully acknowledges financial support by the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No. XDB04010600) and the National Natural Science Foundation of China (Grant No. 11227902). NR 31 TC 16 Z9 16 U1 7 U2 58 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 2 PY 2014 VL 89 IS 3 AR 035101 DI 10.1103/PhysRevB.89.035101 PG 5 WC Physics, Condensed Matter SC Physics GA AC0EZ UT WOS:000332168900001 ER PT J AU Wu, CM Peng, R Dimitrijevic, NM Rajh, T Koodali, RT AF Wu, Chia-Ming Peng, Rui Dimitrijevic, Nada M. Rajh, Tijana Koodali, Ranjit T. TI Preparation of TiO2-SiO2 aperiodic mesoporous materials with controllable formation of tetrahedrally coordinated Ti4+ ions and their performance for photocatalytic hydrogen production SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Titanium dioxide; Silicon dioxide; Aperiodic mesoporous material; Hydrogen production; Tetrahedrally coordinated Ti4+ ion ID WATER DECOMPOSITION; LOCAL STRUCTURES; VISIBLE-LIGHT; SINGLE-SITE; UNDESIRABLE MOLECULES; CONTAINING MCM-41; ROOM-TEMPERATURE; MIXED-OXIDE; SILICA; REACTIVITY AB The efficiency of photocatalytic water splitting for TiO2 dispersed on four SiO2 aperiodic porous supports is discussed in this work. The four TiO2-SiO2 composite materials were prepared via a sol-gel method and then subjected to supercritical drying, natural drying, rotatory vapor drying, or hydrothermal synthesis and the materials were subsequently calcined under identical conditions. These synthetic strategies result in differences in textural properties (specific surface area, pore diameter etc.) and in the amount of tetrahedrally coordinated Ti4+ ions. The TiO2-SiO2 materials were thoroughly characterized by powder X-ray diffraction (XRD), UV-Vis diffuse reflectance spectra (DRS), nitrogen adsorption studies, FT-IR spectroscopy, transmission electron microscopic (TEM) studies, and electron paramagnetic resonance (EPR) studies. The photocatalytic activity for hydrogen production is maximum when the amount of tetrahedrally coordinated Ti4+ ions is high. Thus, this work provides guidance towards the preparation of photoactive materials for generating hydrogen from water. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Wu, Chia-Ming; Peng, Rui; Koodali, Ranjit T.] Univ S Dakota, Dept Chem, Vermillion, SD 57069 USA. [Dimitrijevic, Nada M.; Rajh, Tijana] Argonne Natl Lab, Argonne, IL 60439 USA. [Dimitrijevic, Nada M.; Rajh, Tijana] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Koodali, RT (reprint author), Univ S Dakota, Dept Chem, Vermillion, SD 57069 USA. EM Ranjit.Koodali@usd.edu RI Koodali, Ranjit/E-5595-2011; Peng, Rui/J-3781-2016 OI Koodali, Ranjit/0000-0002-2790-3053; Peng, Rui/0000-0002-1686-9574 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; [DE-EE 0000270]; [NSF-CHE 0722632]; [NSF-EPS 0903804] FX This work was supported by DE-EE 0000270, NSF-CHE 0722632, and NSF-EPS 0903804. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 35 TC 7 Z9 7 U1 3 U2 52 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 2 PY 2014 VL 39 IS 1 BP 127 EP 136 DI 10.1016/j.ijhydene.2013.10.079 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA AA2JV UT WOS:000330921800014 ER PT J AU Margevicius, KJ Generous, N Taylor-McCabe, KJ Brown, M Daniel, WB Castro, L Hengartner, A Deshpande, A AF Margevicius, Kristen J. Generous, Nicholas Taylor-McCabe, Kirsten J. Brown, Mac Daniel, W. Brent Castro, Lauren Hengartner, Andrea Deshpande, Alina TI Advancing a Framework to Enable Characterization and Evaluation of Data Streams Useful for Biosurveillance SO PLOS ONE LA English DT Article ID PUBLIC-HEALTH SURVEILLANCE; NEW-YORK-CITY; SYNDROMIC SURVEILLANCE; DISEASE DETECTION; SYSTEMS; TECHNOLOGIES AB In recent years, biosurveillance has become the buzzword under which a diverse set of ideas and activities regarding detecting and mitigating biological threats are incorporated depending on context and perspective. Increasingly, biosurveillance practice has become global and interdisciplinary, requiring information and resources across public health, One Health, and biothreat domains. Even within the scope of infectious disease surveillance, multiple systems, data sources, and tools are used with varying and often unknown effectiveness. Evaluating the impact and utility of state-of-the-art biosurveillance is, in part, confounded by the complexity of the systems and the information derived from them. We present a novel approach conceptualizing biosurveillance from the perspective of the fundamental data streams that have been or could be used for biosurveillance and to systematically structure a framework that can be universally applicable for use in evaluating and understanding a wide range of biosurveillance activities. Moreover, the Biosurveillance Data Stream Framework and associated definitions are proposed as a starting point to facilitate the development of a standardized lexicon for biosurveillance and characterization of currently used and newly emerging data streams. Criteria for building the data stream framework were developed from an examination of the literature, analysis of information on operational infectious disease biosurveillance systems, and consultation with experts in the area of biosurveillance. To demonstrate utility, the framework and definitions were used as the basis for a schema of a relational database for biosurveillance resources and in the development and use of a decision support tool for data stream evaluation. C1 [Margevicius, Kristen J.; Generous, Nicholas; Brown, Mac; Daniel, W. Brent; Castro, Lauren; Hengartner, Andrea; Deshpande, Alina] Los Alamos Natl Lab, Def Syst & Anal Div, Los Alamos, NM 87545 USA. [Taylor-McCabe, Kirsten J.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. RP Margevicius, KJ (reprint author), Los Alamos Natl Lab, Def Syst & Anal Div, Los Alamos, NM 87545 USA. EM kmargevicius@lanl.gov; deshpande_a@lanl.gov OI Generous, Nicholas/0000-0003-2238-428X; Margevicius, Kristen/0000-0002-4116-8307 FU Defense Threat Reduction Agency, Joint Science and Technology Office for Chemical and Biological Defense; U.S. Department of Energy [B114525l]; Los Alamos National Laboratory [B114525l] FX The Defense Threat Reduction Agency, Joint Science and Technology Office for Chemical and Biological Defense is acknowledged as the sponsor of this work, under a "work for others" arrangement, issued under the prime contract for research, development, test, and evaluation services between the U.S. Department of Energy and Los Alamos National Laboratory (#B114525l). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 59 TC 4 Z9 4 U1 2 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 2 PY 2014 VL 9 IS 1 AR e83730 DI 10.1371/journal.pone.0083730 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 286ID UT WOS:000329460100017 PM 24392093 ER PT J AU Shin, JW Buxboim, A Spinler, KR Swift, J Christian, DA Hunter, CA Leon, C Gachet, C Dingal, PCDP Ivanovska, IL Rehfeldt, F Chasis, JA Discher, DE AF Shin, Jae-Won Buxboim, Amnon Spinler, Kyle R. Swift, Joe Christian, David A. Hunter, Christopher A. Leon, Catherine Gachet, Christian Dingal, P. C. Dave P. Ivanovska, Irena L. Rehfeldt, Florian Chasis, Joel Anne Discher, Dennis E. TI Contractile Forces Sustain and Polarize Hematopoiesis from Stem and Progenitor Cells SO CELL STEM CELL LA English DT Article ID NONMUSCLE MYOSIN IIB; HUMAN CORD BLOOD; HEAVY-CHAIN; BONE-MARROW; ACTOMYOSIN CONTRACTILITY; DIVISION; DICTYOSTELIUM; SEGREGATION; EXPANSION; MEGAKARYOCYTES AB Self-renewal and differentiation of stem cells depend on asymmetric division and polarized motility processes that in other cell types are modulated by nonmuscle myosin-II (MII) forces and matrix mechanics. Here, mass spectrometry-calibrated intracellular flow cytometry of human hematopoiesis reveals MIIB to be a major isoform that is strongly polarized in hematopoietic stem cells and progenitors (HSC/Ps) and thereby downregulated in differentiated cells via asymmetric division. MIIA is constitutive and activated by dephosphorylation during cytokine-triggered differentiation of cells grown on stiff, endosteum-like matrix, but not soft, marrow-like matrix. In vivo, MIIB is required for generation of blood, while MIIA is required for sustained HSC/P engraftment. Reversible inhibition of both isoforms in culture with blebbistatin enriches for long-term hematopoietic multilineage reconstituting cells by 5-fold or more as assessed in vivo. Megakaryocytes also become more polyploid, producing 4-fold more platelets. MII is thus a multifunctional node in polarized division and niche sensing. C1 [Shin, Jae-Won; Buxboim, Amnon; Spinler, Kyle R.; Swift, Joe; Dingal, P. C. Dave P.; Ivanovska, Irena L.; Rehfeldt, Florian; Discher, Dennis E.] Univ Penn, Biophys Engn Lab, Philadelphia, PA 19104 USA. [Shin, Jae-Won; Discher, Dennis E.] Univ Penn, Cell & Mol Biol Grp, Philadelphia, PA 19104 USA. [Shin, Jae-Won; Discher, Dennis E.] Univ Penn, Pharmacol Grad Grp, Philadelphia, PA 19104 USA. [Christian, David A.; Hunter, Christopher A.] Univ Penn, Sch Vet Med, Dept Pathobiol, Philadelphia, PA 19104 USA. [Leon, Catherine; Gachet, Christian] Univ Strasbourg, INSERM, Etab Francais Sang, UMR S949, F-67000 Strasbourg, France. [Chasis, Joel Anne] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Chasis, Joel Anne] Univ Calif San Francisco, Div Hematol Oncol, San Francisco, CA 94143 USA. RP Discher, DE (reprint author), Univ Penn, Biophys Engn Lab, Philadelphia, PA 19104 USA. EM discher@seas.upenn.edu RI Swift, Joe/A-5149-2014; Rehfeldt, Florian/A-1078-2007; leon, catherine/G-6473-2015; Gachet, Christian/H-9156-2016 OI Swift, Joe/0000-0002-5039-9094; Rehfeldt, Florian/0000-0001-9086-3835; leon, catherine/0000-0002-8597-9929; FU National Institutes of Health [P01DK032094, R01HL062352, R01-EB007049, P30-DK090969, NCATS-8UL1TR000003]; Human Frontier Science Program; National Science Foundation; Nano Science and Engineering Center-Nano Bio Interface Center; American Heart Association FX We thank Dr. Robert Adelstein, Dr. Mary Anne Conti (NIH-NHLBI), and Dr. Leonard Zon (Harvard) for invaluable comments. We gratefully acknowledge Arielle Glatman Zaretsky for technical assistance in mouse BM transplantation and the Stem Cell Xenograft Core at the University of Pennsylvania, A. Secreto, J. Glover, and Dr. G. Danet-Desnoyers for cells and engraftment studies. This study was supported by the National Institutes of Health (P01DK032094; R01HL062352; R01-EB007049; P30-DK090969; NCATS-8UL1TR000003), the Human Frontier Science Program (I. I. and D. E. D.), the National Science Foundation (D. E. D.), the Nano Science and Engineering Center-Nano Bio Interface Center (D. E. D.), and the American Heart Association (J.-W.S.). NR 54 TC 39 Z9 39 U1 0 U2 33 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1934-5909 EI 1875-9777 J9 CELL STEM CELL JI Cell Stem Cell PD JAN 2 PY 2014 VL 14 IS 1 BP 81 EP 93 DI 10.1016/j.stem.2013.10.009 PG 13 WC Cell & Tissue Engineering; Cell Biology SC Cell Biology GA 287WB UT WOS:000329571900011 PM 24268694 ER PT J AU Paller, MH Sterrett, SC Tuberville, TD Fletcher, DE Grosse, AM AF Paller, Michael H. Sterrett, Sean C. Tuberville, Tracey D. Fletcher, Dean E. Grosse, Andrew M. TI Effects of disturbance at two spatial scales on macroinvertebrate and fish metrics of stream health SO JOURNAL OF FRESHWATER ECOLOGY LA English DT Article DE benthic macroinvertebrates; fish; metrics; streams; spatial scale; disturbance ID COASTAL-PLAIN STREAMS; ECOLOGICAL RELATIONSHIPS; FOREST ECOREGION; NORTHERN LAKES; SPECIES TRAITS; WATER-QUALITY; COMMUNITIES; ASSEMBLAGES; FRAMEWORK; RIVER AB We analyzed macroinvertebrate and fish assemblage data collected from the upper southeastern coastal plain of the USA to (1) assess the relative sensitivities of bioassessment metrics to in-stream habitat quality, catchment scale land disturbance, and the presence of a reservoir in the catchment and (2) determine whether fish differ from macroinvertebrates in their responses to these variables. Fish and macroinvertebrates responded differently to anthropogenic disturbance: macroinvertebrates were affected most strongly by in-stream habitat quality and fish by the presence of a reservoir in the catchment. Neither taxonomic group were significantly affected by the catchment scale disturbance, probably because the proportions of disturbed land in the study areas were low. Fish may be particularly sensitive to the presence of reservoirs because of their need to cover relatively large distances to complete life cycles and maintain viable populations and because of their sensitivity to the effects of invasive reservoir species, particularly predator fishes. Although not an important predictor in itself, disturbance at the watershed scale was significantly and positively related to in-stream habitat quality, indicating that watershed disturbance had an important indirect effect on aquatic organisms. Direct and indirect ordination showed that the metric data were more strongly related to the disturbance variables than the taxonomic data from which the metrics were derived, possibly because the metrics were less sensitive than the taxon-specific abundances to nondisturbance-related factors. Other factors that may have contributed to this result include greater statistical tractability of the metric data and the relatively high sensitivity of the collective properties represented by the metrics to disturbance-related environmental changes. C1 [Paller, Michael H.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Sterrett, Sean C.; Tuberville, Tracey D.; Fletcher, Dean E.; Grosse, Andrew M.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29808 USA. RP Paller, MH (reprint author), Savannah River Natl Lab, Savannah River Site, Aiken, SC 29808 USA. EM michael.paller@srnl.doe.gov FU DoD Strategic Environmental Research and Development Program (SERDP) [RC-1694]; DOE; EPA; U.S. DOE [DE-FC09-07SR22506] FX This research work was sponsored by the DoD Strategic Environmental Research and Development Program (SERDP) under project RC-1694, executed in partnership with DOE and EPA. This research was partially supported by the U.S. DOE award number DE-FC09-07SR22506 to the University of Georgia. NR 40 TC 3 Z9 5 U1 1 U2 33 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA SN 0270-5060 EI 2156-6941 J9 J FRESHWATER ECOL JI J. Freshw. Ecol. PD JAN 2 PY 2014 VL 29 IS 1 BP 83 EP 100 DI 10.1080/02705060.2013.832707 PG 18 WC Ecology; Limnology SC Environmental Sciences & Ecology; Marine & Freshwater Biology GA 290RQ UT WOS:000329776400007 ER PT J AU Comer, J Roux, B Chipot, C AF Comer, Jeffrey Roux, Benoit Chipot, Christophe TI Achieving ergodic sampling using replica-exchange free-energy calculations SO MOLECULAR SIMULATION LA English DT Article DE free-energy calculations; replica-exchange algorithms; multiple walkers; parallel tempering; entropy calculations ID MOLECULAR-DYNAMICS SIMULATIONS; MONTE-CARLO; THERMODYNAMIC DECOMPOSITION; FORCE-FIELDS; SYSTEMS; ALGORITHM; PROTEINS; SOLUTES; SOLVENT; VERSION AB Seamless combination of multiple-walker strategies with importance-sampling free-energy methods relying upon perturbation theory and the application of time-dependent biases on collective variables is explored as an alternate avenue to achieve ergodic sampling in molecular simulations. Free-energy perturbation is associated with a parallel-tempering scheme, wherein both temperatures and the Hamiltonians representative of the various strata of a stratification scheme are swapped sequentially. In addition, adaptive biasing force simulations are performed at different temperatures in a replica-exchange context, updating continuously across the different replicas the gradient of the free energy along the relevant collective variable. Performance of the proposed methodology is evaluated in two distinct applications, namely the computation of the entropy of hydration of ethanol, following either an alchemical or a geometrical route, and the entropy that underlies the reversible folding of a short peptide. C1 [Comer, Jeffrey; Chipot, Christophe] CNRS, Lab Int, F-54506 Vandoeuvre Les Nancy, France. [Comer, Jeffrey; Chipot, Christophe] Univ Lorraine, Univ Illinois Urbana Champaign, Unite Mixte Rech 7565, F-54506 Vandoeuvre Les Nancy, France. [Roux, Benoit] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Roux, Benoit] Univ Chicago, Dept Biochem & Mol Biol, Gordon Ctr Integrat Sci, Chicago, IL 60637 USA. [Chipot, Christophe] Univ Illinois, Beckman Inst Adv Sci & Engn, Theoret & Computat Biophys Grp, Urbana, IL USA. RP Chipot, C (reprint author), CNRS, Lab Int, BP 70239, F-54506 Vandoeuvre Les Nancy, France. EM chipot@ks.uiuc.edu FU France and Chicago Collaborating in the Sciences (FACCTS) Center; Direction Regionale a la Recherche et a la Technologie de Lorraine; National Science Foundation (NSF) [MCB-0920261] FX The authors are grateful to the France and Chicago Collaborating in the Sciences (FACCTS) Center and to the Direction Regionale a la Recherche et a la Technologie de Lorraine for their support. The research is funded by Grant No. MCB-0920261 from the National Science Foundation (NSF). The authors are indebted to the Grand Equipement National de Calcul Informatique (GENCI) and the Centre Informatique National de l'Enseignement Superieur for provision of generous amount of computer time. NR 47 TC 7 Z9 7 U1 4 U2 29 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0892-7022 EI 1029-0435 J9 MOL SIMULAT JI Mol. Simul. PD JAN 2 PY 2014 VL 40 IS 1-3 SI SI BP 218 EP 228 DI 10.1080/08927022.2013.841909 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 277IW UT WOS:000328813200025 ER PT J AU Campisi, J AF Campisi, Judith TI CELL BIOLOGY The beginning of the end SO NATURE LA English DT Editorial Material ID SENESCENCE C1 [Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Campisi, J (reprint author), Buck Inst Res Aging, Novato, CA 94945 USA. EM jcampisi@buckinstitute.org FU NIA NIH HHS [R37 AG009909, P01 AG041122, P01 AG017242] NR 8 TC 16 Z9 16 U1 2 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 2 PY 2014 VL 505 IS 7481 BP 35 EP 36 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282IB UT WOS:000329163300018 PM 24352243 ER PT J AU Schatz, H Gupta, S Moller, P Beard, M Brown, EF Deibel, AT Gasques, LR Hix, WR Keek, L Lau, R Steiner, AW Wiescher, M AF Schatz, H. Gupta, S. Moeller, P. Beard, M. Brown, E. F. Deibel, A. T. Gasques, L. R. Hix, W. R. Keek, L. Lau, R. Steiner, A. W. Wiescher, M. TI Strong neutrino cooling by cycles of electron capture and beta(-) decay in neutron star crusts SO NATURE LA English DT Article ID X-RAY-BURSTS; SUPERBURST IGNITION; INNER CRUST; MODELS; PHYSICS; INTERIORS; OCEAN AB The temperature in the crust of an accreting neutron star, which comprises its outermost kilometre, is set by heating from nuclear reactions at large densities(1-4), neutrino cooling(5,6) and heat transport from the interior(7-11). The heated crust has been thought to affect observable phenomena at shallower depths, such as thermonuclear bursts in the accreted envelope(10,11). Here we report that cycles of electron capture and its inverse, beta(-) decay, involving neutron-rich nuclei at a typical depth of about 150 metres, cool the outer neutron star crust by emitting neutrinos while also thermally decoupling the surface layers from the deeper crust. This 'Urca' mechanism(12) has been studied in the context of white dwarfs(13) and type Ia supernovae(14,15), but hitherto was not considered in neutron stars, because previous models(1,2) computed the crust reactions using a zero-temperature approximation and assumed that only a single nuclear species was present at any given depth. The thermal decoupling means that X-ray bursts and other surface phenomena are largely independent of the strength of deep crustal heating. The unexpectedly short recurrence times, of the order of years, observed for very energetic thermonuclear superbursts(16) are therefore not an indicator of a hot crust, but may point instead to an unknown local heating mechanism near the neutron star surface. C1 [Schatz, H.; Brown, E. F.; Keek, L.; Lau, R.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Schatz, H.; Moeller, P.; Beard, M.; Brown, E. F.; Deibel, A. T.; Keek, L.; Lau, R.; Steiner, A. W.; Wiescher, M.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Schatz, H.; Brown, E. F.; Deibel, A. T.; Keek, L.; Lau, R.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Gupta, S.] Indian Inst Technol Ropar, Rupnagar Ropar 140001, Punjab, India. [Moeller, P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Beard, M.; Wiescher, M.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Gasques, L. R.] Univ Sao Paulo, Inst Fis, Dept Fis Nucl, BR-05315970 Sao Paulo, Brazil. [Hix, W. R.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Hix, W. R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Steiner, A. W.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. RP Schatz, H (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, 640 South Shaw Lane, E Lansing, MI 48824 USA. EM schatz@nscl.msu.edu RI Gasques, Leandro Romero/E-2530-2012; Hix, William/E-7896-2011; OI Hix, William/0000-0002-9481-9126; Moller, Peter/0000-0002-5848-3565; Steiner, Andrew/0000-0003-2478-4017 FU NSF [PHY 08-22648, PHY 06-06007, AST 11-09176]; INT DOE [DE-FG02-00ER41132]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX This project was funded by NSF grants PHY 08-22648 (Joint Institute for Nuclear Astrophysics) and PHY 06-06007. A. W. S. was supported by INT DOE grant DE-FG02-00ER41132. E. F. B. was supported by NSF grant AST 11-09176. P.M. was supported by the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under contract no. DE-AC52-06NA25396. We thank D. M. Yakovlev, P. Shternin and S. Reddy for discussions and comments on the manuscript. NR 29 TC 26 Z9 26 U1 3 U2 15 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 2 PY 2014 VL 505 IS 7481 BP 62 EP + DI 10.1038/nature12757 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282IB UT WOS:000329163300023 PM 24291788 ER PT J AU Sherwood, OA Guilderson, TP Batista, FC Schiff, JT McCarthy, MD AF Sherwood, Owen A. Guilderson, Thomas P. Batista, Fabian C. Schiff, John T. McCarthy, Matthew D. TI Increasing subtropical North Pacific Ocean nitrogen fixation since the Little Ice Age SO NATURE LA English DT Article ID DEEP-SEA CORALS; AMINO-ACIDS; ISOTOPIC COMPOSITION; CLIMATE VARIABILITY; STATION ALOHA; PRODUCTIVITY; RADIOCARBON; CIRCULATION; PATTERNS; PLANKTON AB The North Pacific subtropical gyre (NPSG) plays a major part in the export of carbon and other nutrients to the deep ocean(1). Primary production in the NPSG has increased in recent decades despite a reduction in nutrient supply to surface waters(2,3). It is thought that this apparent paradox can be explained by a shift in plankton community structure from mostly eukaryotes to mostly nitrogen-fixing prokaryotes(2-4). It remains uncertain, however, whether the plankton community domain shift can be linked to cyclical climate variability or a long-term global warming trend(5). Here we analyse records of bulk and amino-acid-specific N-15/N-14 isotopic ratios (delta N-15) preserved in the skeletons of long-lived deep-sea proteinaceous corals collected from the Hawaiian archipelago; these isotopic records serve as a proxy for the source of nitrogen-supported export production through time. We find that the recent increase in nitrogen fixation is the continuation of a much larger, centennial-scale trend. After a millennium of relatively minor fluctuation, delta N-15 decreases between 1850 and the present. The total shift in delta N-15 of -2 per mil over this period is comparable to the total change in global mean sedimentary delta N-15 across the Pleistocene-Holocene transition, but it is happening an order of magnitude faster(6). We use a steady-state model and find that the isotopic mass balance between nitrate and nitrogen fixation implies a 17 to 27 per cent increase in nitrogen fixation over this time period. A comparison with independent records(7,8) suggests that the increase in nitrogen fixation might be linked to Northern Hemisphere climate change since the end of the Little Ice Age. C1 [Sherwood, Owen A.; Guilderson, Thomas P.; Batista, Fabian C.; Schiff, John T.; McCarthy, Matthew D.] Univ Calif Santa Cruz, Ocean Sci Dept, Santa Cruz, CA 95064 USA. [Guilderson, Thomas P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Guilderson, Thomas P.] Univ Calif Santa Cruz, Inst Marine Sci, Santa Cruz, CA 95064 USA. RP Sherwood, OA (reprint author), Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. EM owen.sherwood@colorado.edu FU NOAA/NURP; National Geographic Society [7717-04]; US Department of Energy [DE-AC52-07NA27344]; NSF [OCE 1061689] FX We thank the captain and crew of the RV Ka'imikai-o-Kanaloa and the pilots and engineers of the Hawaiian Undersea Research Laboratory's Pisces V submersible for their assistance in collecting the specimens presented here. Funding for sample collection was from NOAA/NURP and the National Geographic Society (grant number 7717-04). Radiocarbon analyses were performed under the auspices of the US Department of Energy (grant number DE-AC52-07NA27344). The bulk of the work presented here was funded by the NSF (grant number OCE 1061689). NR 47 TC 23 Z9 23 U1 5 U2 112 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 2 PY 2014 VL 505 IS 7481 BP 78 EP + DI 10.1038/nature12784 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 282IB UT WOS:000329163300027 PM 24336216 ER PT J AU Alleman, C Ghosh, S Luscher, DJ Bronkhorst, CA AF Alleman, Coleman Ghosh, Somnath Luscher, D. J. Bronkhorst, Curt A. TI Evaluating the effects of loading parameters on single-crystal slip in tantalum using molecular mechanics SO PHILOSOPHICAL MAGAZINE LA English DT Article DE crystal plasticity; molecular dynamics; tantalum; non-Schmid effects; strain rate; thermal activation; embedded atom method; finite element method; tension-compression asymmetry ID THERMALLY-ACTIVATED DEFORMATION; CENTERED CUBIC METALS; EMBEDDED-ATOM METHOD; HIGH-PURITY TANTALUM; PLASTIC-DEFORMATION; BCC METALS; SCREW DISLOCATIONS; ORIENTATION DEPENDENCE; TRANSITION-METALS; LOW TEMPERATURES AB This study is aimed at developing a physics-based crystal plasticity finite element model for body-centred cubic (BCC) metals, through the introduction of atomic-level deformation information from molecular dynamics (MD) investigations of dislocation motion at the onset of plastic flow. In this study, three critical variables governing crystal plasticity mediated by dislocation motion are considered. MD simulations are first performed across a range of finite temperatures up to 600K to quantify the temperature dependence of critical stress required for slip initiation. An important feature of slip in BCC metals is that it is not solely dependent on the Schmid law measure of resolved shear stress, commonly employed in crystal plasticity models. The configuration of a screw dislocation and its subsequent motion is studied under different load orientations to quantify these non-Schmid effects. Finally, the influence of strain rates on thermal activation is studied by inducing higher stresses during activation at higher applied strain rates. Functional dependence of the critical resolved shear stress on temperature, loading orientation and strain rate is determined from the MD simulation results. The functional forms are derived from the thermal activation mechanisms that govern the plastic behaviour and quantification of relevant deformation variables. The resulting physics-based rate-dependent crystal plasticity model is implemented in a crystal plasticity finite element code. Uniaxial simulations reveal orientation-dependent tension-compression asymmetry of yield that more accurately represents single-crystal experimental results than standard models. C1 [Alleman, Coleman; Ghosh, Somnath] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Luscher, D. J.; Bronkhorst, Curt A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ghosh, S (reprint author), Johns Hopkins Univ, Baltimore, MD 21218 USA. EM sghosh20@jhu.edu RI Bronkhorst, Curt/B-4280-2011; Ghosh, Somnath/A-2867-2012; Alleman, Coleman/N-1219-2016 OI Bronkhorst, Curt/0000-0002-2709-1964; Alleman, Coleman/0000-0002-6227-2314 FU Advanced Simulations and Computing Program at Los Alamos National Laboratory FX The authors gratefully acknowledge the Advanced Simulations and Computing Program at Los Alamos National Laboratory (Dr. M. Schraad, project leader) for support of this work. They also express appreciation for fruitful discussions with Dr. I. Beyerlein of Los Alamos National Laboratory and Professor V. Vitek of University of Pennsylvania. NR 60 TC 5 Z9 5 U1 2 U2 29 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD JAN 2 PY 2014 VL 94 IS 1 BP 92 EP 116 DI 10.1080/14786435.2013.843795 PG 25 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA 275JA UT WOS:000328670900007 ER PT J AU Nagle, NN Buttenfield, BP Leyk, S Spielman, S AF Nagle, Nicholas N. Buttenfield, Barbara P. Leyk, Stefan Spielman, Seth TI Dasymetric Modeling and Uncertainty SO ANNALS OF THE ASSOCIATION OF AMERICAN GEOGRAPHERS LA English DT Article DE dasymetric modeling; maximum entropy; small area estimation ID PROPORTIONAL FITTING PROCEDURE; AREAL INTERPOLATION; LAND-COVER; DENSITY-ESTIMATION; POPULATION; ACCURACY; FRAMEWORK; SURFACE; URBAN AB Dasymetric models increase the spatial resolution of population data by incorporating related ancillary data layers. The role of uncertainty in dasymetric modeling has not been fully addressed as of yet. Uncertainty is usually present because most population data are themselves uncertain, or the geographic processes that connect population and the ancillary data layers are not precisely known. A new dasymetric methodologythe penalized maximum entropy dasymetric model (P-MEDM)is presented that enables these sources of uncertainty to be represented and modeled. The P-MEDM propagates uncertainty through the model and yields fine-resolution population estimates with associated measures of uncertainty. This methodology contains a number of other benefits of theoretical and practical interest. In dasymetric modeling, researchers often struggle with identifying a relationship between population and ancillary data layers. The P-MEDM model simplifies this step by unifying how ancillary data are included. The P-MEDM also allows a rich array of data to be included, with disparate spatial resolutions, attribute resolutions, and uncertainties. Although the P-MEDM does not necessarily produce more precise estimates than do existing approaches, it does help to unify how data enter the dasymetric model, it increases the types of data that can be used, and it allows geographers to characterize the quality of their dasymetric estimates. We present an application of the P-MEDM that includes household-level survey data combined with higher spatial resolution data such as from census tracts, block groups, and land cover classifications. C1 [Nagle, Nicholas N.] Univ Tennessee, Dept Geog, Knoxville, TN 37996 USA. [Nagle, Nicholas N.] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN USA. [Buttenfield, Barbara P.; Leyk, Stefan; Spielman, Seth] Univ Colorado, Dept Geog, Boulder, CO 80309 USA. RP Nagle, NN (reprint author), Univ Tennessee, Dept Geog, Knoxville, TN 37996 USA. EM nnagle@utk.edu; babs@colorado.edu; stefan.leyk@colorado.edu; seth.spielman@colorado.edu RI Spielman, Seth/F-4023-2011 OI Spielman, Seth/0000-0002-5089-7632 FU NICHD NIH HHS [P2C HD066613, R24 HD066613] NR 46 TC 9 Z9 9 U1 0 U2 14 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXFORDSHIRE, ENGLAND SN 0004-5608 EI 1467-8306 J9 ANN ASSOC AM GEOGR JI Ann. Assoc. Am. Geogr. PD JAN 2 PY 2014 VL 104 IS 1 BP 80 EP 95 DI 10.1080/00045608.2013.843439 PG 16 WC Geography SC Geography GA 269NI UT WOS:000328247600005 PM 25067846 ER PT J AU Geng, J Navon, IM Chen, X AF Geng, Jian Navon, I. Michael Chen, Xiao TI Non-parametric calibration of the local volatility surface for European options using a second-order Tikhonov regularization SO QUANTITATIVE FINANCE LA English DT Article DE Local volatility surface; Second-order Tikhonov regularization; SVD; Large scale non-linear inverse problem; C61; C ID INVERSE PROBLEM; ALGORITHM; MODELS AB We calibrate the local volatility surface for European options across all strikes and maturities of the same underlying. There is no interpolation or extrapolation of either the option prices or the volatility surface. We do not make any assumption regarding the shape of the volatility surface except to assume that it is smooth. Due to the smoothness assumption, we apply a second-order Tikhonov regularization. We choose the Tikhonov regularization parameter as one of the singular values of the Jacobian matrix of the Dupire model. Finally we perform extensive numerical tests to assess and verify the aforementioned techniques for both volatility models with known analytical solutions of European option prices and real market option data. C1 [Geng, Jian] Florida State Univ, Dept Math, Tallahassee, FL 32306 USA. [Navon, I. Michael] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. [Chen, Xiao] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA USA. RP Navon, IM (reprint author), Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. EM inavon@fsu.edu RI Navon, Ionel/A-5173-2008; Chen, Xiao/K-3070-2014 OI Navon, Ionel/0000-0001-7830-7094; FU NSF [ATM-0931198]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors would like to thank Dr. Cristian Homescu from Wells Fargo for his helpful comments. The authors also owe their sincere gratitude to the two reviewers for patiently pointing out both some schematic deficiencies that we were able to make up during the revision process and also some typographical errors that make this paper much stronger. Prof. I. M. Navon would like to acknowledge support from NSF grant ATM-0931198. Dr. Xiao Chen would like to acknowledge support from the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 38 TC 2 Z9 2 U1 0 U2 6 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1469-7688 EI 1469-7696 J9 QUANT FINANC JI Quant. Financ. PD JAN 2 PY 2014 VL 14 IS 1 BP 73 EP 85 DI 10.1080/14697688.2013.819988 PG 13 WC Business, Finance; Economics; Mathematics, Interdisciplinary Applications; Social Sciences, Mathematical Methods SC Business & Economics; Mathematics; Mathematical Methods In Social Sciences GA 267YI UT WOS:000328133900006 ER PT J AU Park, Y Shankar, M Park, BH Ghosh, J AF Park, Yubin Shankar, Mallikarjun Park, Byung-Hoon Ghosh, Joydeep GP IEEE TI Graph Databases for Large-Scale Healthcare Systems: A Framework for Efficient Data Management and Data Services SO 2014 IEEE 30TH INTERNATIONAL CONFERENCE ON DATA ENGINEERING WORKSHOPS (ICDEW) LA English DT Proceedings Paper CT IEEE 30th International Conference on Data Engineering (ICDE) CY MAR 31-APR 04, 2014 CL Chicago, IL SP IEEE, Microsoft, Qatar Comp Res Inst, HERE Nokia, Purdue Univ, Cyber Ctr, NW Univ, McCormick Sch Engn, Google ID MODEL AB Designing a database system for both efficient data management and data services has been one of the enduring challenges in the healthcare domain. In many healthcare systems, data services and data management are often viewed as two orthogonal tasks; data services refer to retrieval and analytic queries such as search, joins, statistical data extraction, and simple data mining algorithms, while data management refers to building error-tolerant and non-redundant database systems. The gap between service and management has resulted in rigid database systems and schemas that do not support effective analytics. We compose a rich graph structure from an abstracted healthcare RDBMS to illustrate how we can fill this gap in practice. We show how a healthcare graph can be automatically constructed from a normalized relational database using the proposed "3NF Equivalent Graph" (3EG) transformation. We discuss a set of real world graph queries such as finding self-referrals, shared providers, and collaborative filtering, and evaluate their performance over a relational database and its 3EG-transformed graph. Experimental results show that the graph representation serves as multiple de-normalized tables, thus reducing complexity in a database and enhancing data accessibility of users. Based on this finding, we propose an ensemble framework of databases for healthcare applications. C1 [Park, Yubin; Ghosh, Joydeep] Univ Texas Austin, Austin, TX 78712 USA. [Shankar, Mallikarjun; Park, Byung-Hoon] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Park, Y (reprint author), Univ Texas Austin, Austin, TX 78712 USA. EM yubin.park@utexas.edu; shankarm@ornl.gov; parkbh@ornl.gov; ghosh@ece.utexas.edu OI Shankar, Mallikarjun/0000-0001-5289-7460 NR 32 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-3481-2 PY 2014 BP 12 EP 19 PG 8 WC Computer Science, Information Systems SC Computer Science GA BE0JN UT WOS:000366168000002 ER PT J AU Malik, T Chard, K Foster, I AF Malik, Tanu Chard, Kyle Foster, Ian GP IEEE TI Benchmarking Cloud-based Tagging Services SO 2014 IEEE 30TH INTERNATIONAL CONFERENCE ON DATA ENGINEERING WORKSHOPS (ICDEW) LA English DT Proceedings Paper CT IEEE 30th International Conference on Data Engineering (ICDE) CY MAR 31-APR 04, 2014 CL Chicago, IL SP IEEE, Microsoft, Qatar Comp Res Inst, HERE Nokia, Purdue Univ, Cyber Ctr, NW Univ, McCormick Sch Engn, Google AB Tagging services have emerged as a useful and popular way to organize data resources. Despite popular interest, an efficient implementation of tagging services is a challenge since highly dynamic schemas and sparse, heterogeneous attributes must be supported within a shared, openly writable database. NoSQL databases support dynamic schemas and sparse data but lack efficient native support for joins that are inherent to query and search functionality in tagging services. Relational databases provide sufficient support for joins, but offer a multitude of options to manifest dynamic schemas and tune sparse data models, making evaluation of a tagging service time consuming and painful. In this case-study paper, we describe a benchmark for tagging services, and propose benchmarking modules that can be used to evaluate the suitability of a database for workloads generated from tagging services. We have incorporated our modules as part of OLTP-Bench, a cloud-based benchmarking infrastructure, to understand performance characteristics of tagging systems on several relational DBMSs and cloud-based database-as-a-service (DBaaS) offerings. C1 [Malik, Tanu] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. Argonne Natl Lab, Chicago, IL 60637 USA. RP Malik, T (reprint author), Univ Chicago, Computat Inst, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM tanum@ci.uchicago.edu; kyle@ci.uchicago.edu; foster@anl.gov NR 8 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-3481-2 PY 2014 BP 231 EP 238 PG 8 WC Computer Science, Information Systems SC Computer Science GA BE0JN UT WOS:000366168000034 ER PT S AU Camp, D Bethel, EW Childs, H AF Camp, David Bethel, E. Wes Childs, Hank GP IEEE TI Transitioning Data Flow-Based Visualization Software to Multi-Core Hybrid Parallelism SO 2013 DATA-FLOW EXECUTION MODELS FOR EXTREME SCALE COMPUTING (DFM) SE Workshop on Data-Flow Execution Models for Extreme Scale Computing LA English DT Proceedings Paper CT 3rd Workshop on Data-Flow Execution Models for Extreme Scale Computing (DFM) CY SEP 08, 2013 CL Edinburgh, SCOTLAND AB Many of today's programs for supercomputers are designed for distributed-memory parallelism, but not for shared-memory parallelism. As architectural trends for supercomputers suggest an ever-increasing number of cores per node, these projects must evaluate whether they can benefit from hybrid parallelism - parallelism that blends distributed-and shared-memory approaches - and whether the costs for migrating to new architectures are prohibitive. With this research effort, we explore whether a data flow-based visualization tool could be easily migrated to a hybrid parallel setting, what the challenges are, and what benefits hybrid parallelism achieves. For results, we find that only a relatively small investment was required to transition the tool and it significantly improves performance and also reduces memory usage and communication costs. C1 [Camp, David; Bethel, E. Wes; Childs, Hank] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Childs, Hank] Univ Oregon, Eugene, OR 97403 USA. RP Camp, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM dcamp@lbl.gov; ewbethel@lbl.gov; hchilds@lbl.gov NR 20 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 2325-5579 BN 978-1-4799-5247-2 J9 WORKS DATA EXEC PY 2014 BP 59 EP 62 DI 10.1109/DFM.2013.12 PG 4 WC Computer Science, Hardware & Architecture; Computer Science, Theory & Methods SC Computer Science GA BD9ZC UT WOS:000365612300009 ER PT S AU Chen, GY Wu, B Li, D Shen, XP AF Chen, Guoyang Wu, Bo Li, Dong Shen, Xipeng GP IEEE TI PORPLE: An Extensible Optimizer for Portable Data Placement on GPU SO 2014 47TH ANNUAL IEEE/ACM INTERNATIONAL SYMPOSIUM ON MICROARCHITECTURE (MICRO) SE International Symposium on Microarchitecture Proceedings LA English DT Proceedings Paper CT 47th Annual IEEE/ACM International Symposium on Microarchitecture (MICRO) CY DEC 13-17, 2014 CL Cambridge, ENGLAND SP IEEE, ACM, IEEE Comp Soc DE GPU; cache; compiler; data placement; hardware specification language ID MEMORY AB GPU is often equipped with complex memory systems, including global memory, texture memory, shared memory, constant memory, and various levels of cache. Where to place the data is important for the performance of a GPU program. However, the decision is difficult for a programmer to make because of architecture complexity and the sensitivity of suitable data placements to input and architecture changes. This paper presents PORPLE, a portable data placement engine that enables a new way to solve the data placement problem. PORPLE consists of a mini specification language, a source-to-source compiler, and a runtime data placer. The language allows an easy description of a memory system; the compiler transforms a GPU program into a form amenable to runtime profiling and data placement; the placer, based on the memory description and data access patterns, identifies on the fly appropriate placement schemes for data and places them accordingly. PORPLE is distinctive in being adaptive to program inputs and architecture changes, being transparent to programmers (in most cases), and being extensible to new memory architectures. Our experiments on three types of GPU systems show that PORPLE is able to consistently find optimal or near-optimal placement despite the large differences among GPU architectures and program inputs, yielding up to 2.08X (1.59X on average) speedups on a set of regular and irregular GPU benchmarks. C1 [Chen, Guoyang; Shen, Xipeng] N Carolina State Univ, Dept Comp Sci, Raleigh, NC 27695 USA. [Wu, Bo] Colorado Sch Mines, Dept Elect Engn & Comp Sci, Golden, CO 80401 USA. [Li, Dong] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Chen, GY (reprint author), N Carolina State Univ, Dept Comp Sci, Raleigh, NC 27695 USA. EM gchen11@ncsu.edu; bwu@mines.edu; lid1@ornl.gov; xshen5@ncsu.edu NR 30 TC 12 Z9 12 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 1072-4451 BN 978-1-4799-6998-2 J9 INT SYMP MICROARCH PY 2014 BP 88 EP 100 DI 10.1109/MICRO.2014.20 PG 13 WC Computer Science, Hardware & Architecture SC Computer Science GA BD9XC UT WOS:000365531100008 ER PT J AU Saini, D Behlow, HW Serkiz, SM Skove, MJ Rao, AM AF Saini, Deepika Behlow, Herbert W. Serkiz, Steven. M. Skove, Malcolm. J. Rao, A. M. GP IEEE TI Harmonic Detection of Resonance Method SO 2014 IEEE 14TH INTERNATIONAL CONFERENCE ON NANOTECHNOLOGY (IEEE-NANO) LA English DT Proceedings Paper CT 14th IEEE International Conference on Nanotechnology (IEEE-NANO) CY AUG 14-21, 2014 CL Toronto, CANADA SP IEEE DE nanosensor; electrical actuation; electrical detection; capacitive detection; cantilever AB Electromechanical resonators in the micro (MEMS) and nano (NEMS) regimes have emerged as promising tools for use in diverse applications such as ultrasensitive physical, chemical, and biological sensors, with detection limits as low as a single molecule. The advent of state-of-the-art micro-fabrication techniques has enabled a high throughput platform for commercialization. However, the sensitivity and reliability of such devices are highly dependent on the employed detection technique. We present a highly useful yet simple electrical detection scheme: the Harmonic Detection of Resonance (HDR) method. The prominent HDR features will be discussed and applications ranging from the use of micro-cantilevers as sensors to probing mechanical properties in nano-cantilever systems will be presented. C1 [Saini, Deepika; Behlow, Herbert W.; Skove, Malcolm. J.; Rao, A. M.] Clemson Univ, Dept Phys & Astron, Clemson, SC 29634 USA. [Saini, Deepika; Behlow, Herbert W.; Skove, Malcolm. J.; Rao, A. M.] Clemson Nanomat Ctr, Clemson, SC 29634 USA. [Serkiz, Steven. M.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Saini, D (reprint author), Clemson Univ, Dept Phys & Astron, Clemson, SC 29634 USA. EM arao@clemson.edu NR 13 TC 1 Z9 1 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-5622-7 PY 2014 BP 188 EP 191 PG 4 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA BD9ZF UT WOS:000365620600043 ER PT J AU Moldovan, N Divan, R AF Moldovan, Nicolaie Divan, Ralu GP IEEE TI Si (100) and Si (311) - A Comparative Study for Nanofabrication SO 2014 IEEE 14TH INTERNATIONAL CONFERENCE ON NANOTECHNOLOGY (IEEE-NANO) LA English DT Proceedings Paper CT 14th IEEE International Conference on Nanotechnology (IEEE-NANO) CY AUG 14-21, 2014 CL Toronto, CANADA SP IEEE ID SILICON AB Bulk micromachining was mainly developed for Si (100) and Si (110) wafers and is based on crystallographic etching of silicon in KOH and other basic solutions, in order to obtain useful 3-dimensional structures. Recently, Si (311) joined the group of useful substrates for nanomanufacturing, but a thorough description of its capabilities was not yet reported. The hereby study investigates the particularities of crystal-orientation dependent etching of Si (311) wafers in comparison with Si (100) in some of the most popular solutions used for etching. By that, the experimental study adds to the base of knowledge of Si anisotropic etching and diversifies its capabilities. Of particular interest is Si (311)'s capability to form V-grooves of three-faceted pyramid shape, useful for forming wedge-free tips for subsequent molding, which can be exploited to form tips with sub-10 nm apex radii. C1 [Moldovan, Nicolaie] Adv Diamond Technol Inc, Romeoville, IL 60446 USA. [Divan, Ralu] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Moldovan, N (reprint author), Adv Diamond Technol Inc, Romeoville, IL 60446 USA. EM moldovan@thindiamond.com; divan@anl.gov NR 15 TC 0 Z9 0 U1 0 U2 1 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-5622-7 PY 2014 BP 215 EP 220 PG 6 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA BD9ZF UT WOS:000365620600049 ER PT J AU Poole, ZL Ohodnicki, P Chen, RZ Lin, YK Chen, KP AF Poole, Zsolt L. Ohodnicki, Paul Chen, Rongzhang Lin, Yuankun Chen, Kevin P. GP IEEE TI 3D Sub-Wavelength Refractive Index Adjusted Metal Oxides for Applications in Optical Sensing SO 2014 IEEE 14TH INTERNATIONAL CONFERENCE ON NANOTECHNOLOGY (IEEE-NANO) LA English DT Proceedings Paper CT 14th IEEE International Conference on Nanotechnology (IEEE-NANO) CY AUG 14-21, 2014 CL Toronto, CANADA SP IEEE ID THIN-FILMS; GAS SENSORS AB We present a refractive index engineering scheme for functional metal oxides (SnO2, ZnO, TiO2) by the method of sub-wavelength engineering on the 10-50nm scale for applications in optical sensing. The method employed is based on templating by a triblock copolymer Pluronic F-127 for the manufacture of controllable 3D sub-wavelength nanostructures. By this method we demonstrate that the refractive indices of functional metal oxides can be altered substantially from their nominal value of >= 2 to be as low as 1.25. C1 [Chen, Kevin P.] Univ Pittsburgh, Elect & Comp Engn Dept, Pittsburgh, PA 15261 USA. [Ohodnicki, Paul] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Lin, Yuankun] Univ N Texas, Dept Phys, Denton, TX 76203 USA. EM pec9@pitt.edu NR 21 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-5622-7 PY 2014 BP 439 EP 443 PG 5 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA BD9ZF UT WOS:000365620600099 ER PT J AU Behlow, HW Saini, D Elliott, B Serkiz, SM Skove, MJ Rao, AM AF Behlow, Herbert W. Saini, Deepika Elliott, Bevan Serkiz, Steven. M. Skove, Malcolm. J. Rao, A. M. GP IEEE TI Ringdown Sensing Method SO 2014 IEEE 14TH INTERNATIONAL CONFERENCE ON NANOTECHNOLOGY (IEEE-NANO) LA English DT Proceedings Paper CT 14th IEEE International Conference on Nanotechnology (IEEE-NANO) CY AUG 14-21, 2014 CL Toronto, CANADA SP IEEE DE electrical detection; ring-down; viscosity of gases; density of gases; cantilever; capacitive detection AB Miniaturization of devices into lab-on-chip designs is a dominating field of current scientific research. While the technology to build these devices is continuing to develop, the practical realization of such devices remain elusive, mainly due to lack of techniques that bridge the macroscopic world to the mechanical motion and/or the electronic signals generated on the micro-or nano-sized scale. Hence, there is an increasing need for sensitive detection techniques that can not only be implemented on such small scale systems but also be integrated with the current CMOS technology. In this regard, a fully electrical microcantilever-based ringdown method will be presented. We show that detection technique can be employed to precisely analyze the composition of gas mixtures. The viscosity and density can be measured simultaneously, which is illustrated for multiple gases yielding viscosities within +/- 2% and densities within +/- 6% of NIST values. C1 [Behlow, Herbert W.; Saini, Deepika; Elliott, Bevan; Skove, Malcolm. J.; Rao, A. M.] Clemson Nanomat Ctr, Dept Phys & Astron, Clemson, SC 29634 USA. [Serkiz, Steven. M.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Behlow, HW (reprint author), Clemson Nanomat Ctr, Dept Phys & Astron, Clemson, SC 29634 USA. EM arao@clemson.edu NR 11 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-5622-7 PY 2014 BP 456 EP 459 PG 4 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA BD9ZF UT WOS:000365620600103 ER PT J AU Cheng, JY Ng, PK Fisher, B Lilley, CM AF Cheng, Jian-Yih Ng, Poh-Keong Fisher, Brandon Lilley, Carmen M. GP IEEE TI Electric Field and Surface Step Assisted Cu3Si Nanowire Growth by Reactive Deposition Epitaxy SO 2014 IEEE 14TH INTERNATIONAL CONFERENCE ON NANOTECHNOLOGY (IEEE-NANO) LA English DT Proceedings Paper CT 14th IEEE International Conference on Nanotechnology (IEEE-NANO) CY AUG 14-21, 2014 CL Toronto, CANADA SP IEEE DE Copper; Silicide; Nanowire; Self-Assembly ID SILICIDE FORMATION; ROOM-TEMPERATURE; HEATING CURRENT; SI(001) AB Metal silicide nanowires such as copper silicide have been shown to self-assemble into nanowire and nanoisland structures on the surface of silicon substrates. The self-assembly of these nanostructures occurs during reactive deposition epitaxy (RDE). It was observed that varying the surface step orientation of a sample with respect to an applied electric field had a direct influence on the length of vicinal steps and the length of self-assembled nanowires grown using RDE. Si(110) substrates were diced so that the [110] surface step directions with respect to the applied electric field direction were parallel, perpendicular, and 45 degrees. All samples were prepared using the same preparation and Cu deposition parameters. Under the same growth parameters perpendicular orientation samples resulted in the longest thinnest nanowires, parallel orientation samples had short wider wires, whilst the 45 degrees orientation samples had wire dimensions slightly larger than those on the parallel orientation samples. C1 [Cheng, Jian-Yih; Lilley, Carmen M.] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA. [Ng, Poh-Keong; Lilley, Carmen M.] Univ Illinois, Dept Elect & Comp Engn, Chicago, IL 60607 USA. [Fisher, Brandon] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. RP Cheng, JY (reprint author), Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA. EM clilley@uic.edu NR 25 TC 0 Z9 0 U1 0 U2 1 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-5622-7 PY 2014 BP 478 EP 481 PG 4 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA BD9ZF UT WOS:000365620600108 ER PT B AU Steed, CA Swan, JE Fitzpatrick, PJ Jankun-Kelly, TJ AF Steed, Chad A. Swan, J. Edward, II Fitzpatrick, Patrick J. Jankun-Kelly, T. J. BA Huang, ML Huang, W BF Huang, ML Huang, W TI A Visual Analytics Approach for Correlation, Classification, and Regression Analysis SO INNOVATIVE APPROACHES OF DATA VISUALIZATION AND VISUAL ANALYTICS SE Advances in Data Mining and Database Management (ADMDM) Book Series LA English DT Article; Book Chapter ID PARALLEL; VISUALIZATION AB New approaches that combine the strengths of humans and machines are necessary to equip analysts with the proper tools for exploring today's increasingly complex, multivariate data sets. In this chapter, a visual data mining framework, called the Multidimensional Data eXplorer (MDX), is described that addresses the challenges of today's data by combining automated statistical analytics with a highly interactive parallel coordinates based canvas. In addition to several intuitive interaction capabilities, this framework offers a rich set of graphical statistical indicators, interactive regression analysis, visual correlation mining, automated axis arrangements and filtering, and data classification techniques. This chapter provides a detailed description of the system as well as a discussion of key design aspects and critical feedback from domain experts. C1 [Steed, Chad A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Swan, J. Edward, II; Jankun-Kelly, T. J.] Mississippi State Univ, Bagley Coll Engn, Mississippi State, MS USA. [Fitzpatrick, Patrick J.] Mississippi State Univ, Northern Gulf Inst, Mississippi State, MS USA. RP Steed, CA (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. OI Steed, Chad/0000-0002-3501-909X NR 31 TC 0 Z9 0 U1 0 U2 0 PU IGI GLOBAL PI HERSEY PA 701 E CHOCOLATE AVE, STE 200, HERSEY, PA 17033-1240 USA BN 978-1-4666-4310-9; 978-1-4666-4309-3 J9 ADV DATA MIN DATABAS PY 2014 BP 25 EP 45 DI 10.4018/978-1-4666-4309-3.ch002 D2 10.4018/978-1-4666-4309-3 PG 21 WC Computer Science, Artificial Intelligence; Computer Science, Information Systems SC Computer Science GA BD8PR UT WOS:000364181900003 ER PT S AU Aceti, F Liang, WH Oset, E Wu, JJ Zou, BS AF Aceti, F. Liang, W. H. Oset, E. Wu, J. J. Zou, B. S. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Isospin breaking and f(0)(980)-a(0)(980) mixing in the eta(1405) -> pi(0) f(0)(980) reaction SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN AB We make a theoretical study of the eta(1405) -> pi(0) f(0)(980) and eta(1405) -> pi(0) a(0)(980) reactions to determine the isospin violation and the mixing of the f(0)(980) and a(0)(980) resonances. We make use of the chiral unitary approach where these two resonances appear as dynamically generated by the meson-meson interaction provided by chiral Lagrangians. We obtain a very narrow shape for the f(0)(980) production in agreement with a BES experiment. As to the amount of isospin violation, assuming constant vertices for the primary eta(1405) -> pi(0) K (K) over bar and eta(1405) -> pi(0)pi(0)eta production, we find results which are much smaller than found in the experimental BES paper. The problem is solved by using the primary production driven by eta' -> K* (K) over bar followed by K* -> K pi. Thus, we can predict absolute values for the ratio Gamma(pi(0), pi(+) pi(-))/Gamma (pi(0), pi(0)eta) which are in fair agreement with experiment. C1 [Aceti, F.] Ctr Mixto Univ Valencia CSIC, Dept Fis Teor, Inst Invest Paterna, Valencia 46071, Spain. [Aceti, F.] Ctr Mixto Univ Valencia CSIC, IFIC, Valencia 46071, Spain. [Liang, W. H.; Oset, E.] Guangxi Normal Univ, Dept Phys, Guilin 541004, Peoples R China. [Wu, J. J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Zou, B. S.] Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, Beijing 100190, Peoples R China. [Zou, B. S.] Chinese Acad Sci, Inst High Energy Phys, Theoret Phys Ctr Sci Facil, Beijing 100049, Peoples R China. RP Aceti, F (reprint author), Ctr Mixto Univ Valencia CSIC, Dept Fis Teor, Inst Invest Paterna, Aptdo 22085, Valencia 46071, Spain. EM aceti@ifi.uv.es; oset@ific.uv.es NR 5 TC 0 Z9 0 U1 0 U2 3 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 03005 DI 10.1051/epjconf/20147303005 PG 5 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300043 ER PT S AU Dudek, J AF Dudek, Jozef CA Hadron Spectrum Collaboration BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Gluonic excitations in the hadronic spectrum SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN AB I describe progress made by the Hadron Spectrum Collaboration in understanding the role that excitations of the gluonic field play in determining the spectrum of hadrons. This is achieved through calculations of the hadron spectrum using lattice QCD techniques. Clear signals for the lightest set of hybrid mesons and baryons are presented, and a proposal that they correspond to the same chromomagnetic excitation is made. The prospects for studying the decay properties of excited hadrons are briefly discussed. C1 [Dudek, Jozef] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Dudek, Jozef] Old Dominion Univ, Norfolk, VA USA. RP Dudek, J (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM dudek@jlab.org NR 19 TC 0 Z9 0 U1 0 U2 0 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 01004 DI 10.1051/epjconf/20147301004 PG 6 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300004 ER PT S AU Fanelli, C Cisbani, E Hamilton, D Salme, G Wojtsekhowski, B AF Fanelli, C. Cisbani, E. Hamilton, D. Salme, G. Wojtsekhowski, B. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Investigating the proton structure through polarization transfers in real Compton scattering processes at JLAB SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN ID PARTON DISTRIBUTIONS; LIMIT AB In the present work, preliminary results of the analysis of polarization transfers in real Compton scattering (RCS) performed in Hall-C at JLAB are presented, for data collected at large scattering angle (theta(cm) = 70 degrees) in the experiment E07-002. A previous experiment, E99-114, has already demonstrated a complete inconsistence of its results with a pQCD mechanism at JLAB energy regime. This kind of experiment, therefore, is of crucial importance for understanding the nature of the reaction mechanism for such a simple process, involving a real photon. Furthermore, RCS experiments allow the extraction of Compton form factors and Generalized Parton Distributions (GPDs), the latter connected to the total angular momentum of the nucleon. C1 [Fanelli, C.; Salme, G.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Fanelli, C.; Salme, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Cisbani, E.] Ist Nazl Fis Nucl, Sez Roma, Grp Sanita, I-00161 Rome, Italy. [Cisbani, E.] Ist Super Sanita, I-00161 Rome, Italy. [Hamilton, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Wojtsekhowski, B.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Fanelli, C (reprint author), Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. EM cfanelli@iss.infn.it RI Cisbani, Evaristo/C-9249-2011; OI Cisbani, Evaristo/0000-0002-6774-8473; Salme', Giovanni/0000-0002-9209-3464 NR 17 TC 0 Z9 0 U1 0 U2 1 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 02015 DI 10.1051/epjconf/20147302015 PG 4 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300033 ER PT S AU Mack, DJ AF Mack, David J. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Physics and outlook for rare, all-neutral Eta decays SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN ID CP VIOLATION AB The eta meson provides a laboratory to study isospin violation and search for new flavor-conserving sources of C and CP violation with a sensitivity approaching 10(-6) of the isospin-conserving strong amplitude. Some of the most interesting rare eta decays are the neutral modes, yet the effective loss of photons from the relatively common decay eta -> 3 pi(0) -> 6 gamma (33%) has largely obscured rare decays producing 3-5 gamma's. Particularly important relevant branches include the highly suppressed eta -> pi(0)2 gamma -> 4 gamma, which provides a rare window on testing models of O(p(6)) contributions in ChPTh, and eta -> 3 gamma and eta -> 2 pi(0)gamma -> 5 gamma which provide direct constraints on C violation in flavor-conserving processes. The substitution of lead tungstate in the forward calorimeter of the GluEx setup in Jefferson Lab's new Hall D would allow dramatically improved measurements. The main niche of this facility, which we call the JLab Eta Factory (JEF), would be eta decay neutral modes. However, this could likely be expanded to rare eta' (958) decays for low energy QCD studies as well as eta decays involving muons for new physics searches. C1 [Mack, David J.] TJNAF, Newport News, VA 23606 USA. RP Mack, DJ (reprint author), TJNAF, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM mack@jlab.org NR 19 TC 0 Z9 0 U1 3 U2 3 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 03015 DI 10.1051/epjconf/20147303015 PG 4 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300053 ER PT S AU Pennington, MR AF Pennington, M. R. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI SPQR - Spectroscopy: Prospects, Questions & Results SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN ID PARTIAL-WAVE ANALYSIS; RESONANCES; BARYONS; DECAYS; STATES; MODEL AB Tremendous progress has been made in mapping out the spectrum of hadrons over the past decade with plans to make further advances in the decade ahead. Baryons and mesons, both expected and unexpected, have been found, the results of precision experiments often with polarized beams, polarized targets and sometimes polarization of the final states. All these hadrons generate poles in the complex energy plane that are consequences of the strong coupling regime of QCD. They reveal how this works. C1 [Pennington, M. R.] Thomas Jefferson Natl Accelerator Facil, Ctr Theory, Newport News, VA 23606 USA. RP Pennington, MR (reprint author), Thomas Jefferson Natl Accelerator Facil, Ctr Theory, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM michaelp@jlab.org NR 27 TC 2 Z9 2 U1 0 U2 0 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 01001 DI 10.1051/epjconf/20147301001 PG 6 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300001 ER PT S AU Roberts, CD AF Roberts, Craig D. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Images of the origin of mass SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN ID ELECTROMAGNETIC FORM-FACTORS; NUCLEON; QCD; EQUATIONS; THEOREM; SPIN AB Recent years have brought considerable progress with studies of the boundstate problem in continuum QCD. A small part of that made with Dyson Schwinger equations is highlighted herein. Topics covered include: opportunities provided by precision experimental studies of the (far) valence region; and capitalising upon new data on hadron elastic and transition form factors. C1 [Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM cdroberts@anl.gov NR 48 TC 0 Z9 0 U1 1 U2 1 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 01016 DI 10.1051/epjconf/20147301016 PG 7 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300016 ER PT S AU Smith, ES AF Smith, Elton S. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI The light meson spectroscopy program SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN AB Recent discoveries of a number of unexpected new charmomium-like meson states at the BaBar and Belle B-factories have demonstrated how little is still known about meson spectroscopy. In this talk we will review recent highlights of the light quark spectroscopy from collider and fixed target experiments. C1 [Smith, Elton S.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Smith, ES (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM elton@jlab.org NR 22 TC 0 Z9 0 U1 4 U2 4 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 01005 DI 10.1051/epjconf/20147301005 PG 6 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300005 ER PT S AU Szczepaniak, AP AF Szczepaniak, Adam P. BE Battaglieri, M DAngelo, A DeVita, R Pascolini, A Salme, G TI Low energy hadron phenomenology SO MENU 2013 - 13TH INTERNATIONAL CONFERENCE MESON-NUCLEON PHYSICS AND THE STRUCTURE OF THE NUCLEON SE EPJ Web of Conferences LA English DT Proceedings Paper CT 13th International Conference Meson-Nucleon Physics and the Structure of the Nucleon (MENU) CY SEP 30-OCT 04, 2013 CL Rome, ITALY SP Thomas Jefferson Natl Accelerator Facil, Jefferson Sci Associates, Univ William & Mary, Univ Rome Tor Vergata, CAEN ID HYBRID MESONS; MODEL; CONFINEMENT; SPECTRUM; LATTICE; STATES; FIELD; GEV/C AB This talk discusses some of latest theoretical, phenomenological and experimental results is hadron spectroscopy. C1 [Szczepaniak, Adam P.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Szczepaniak, Adam P.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47403 USA. [Szczepaniak, Adam P.] Jefferson Lab, Newport News, VA 23606 USA. RP Szczepaniak, AP (reprint author), Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. EM aszczepa@indiana.edu NR 49 TC 0 Z9 0 U1 1 U2 1 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 2100-014X J9 EPJ WEB CONF PY 2014 VL 73 AR 01015 DI 10.1051/epjconf/20147301015 PG 6 WC Physics, Multidisciplinary; Physics, Nuclear SC Physics GA BD9RB UT WOS:000365134300015 ER PT S AU Suzuki, A Williams, M Oono, Y Miura, R Hatakeyama, N Hori, M Miyamoto, A AF Suzuki, Ai Williams, Mark Oono, Yuka Miura, Ryuji Hatakeyama, Nozomu Hori, Michio Miyamoto, Akira BE Chu, D Narayan, SR Ryan, EM TI Influence of the Sintering of Electrocatalysts and Decrease of Proton Conductivity on the Current-Voltage Performance in the High-Temperature Proton Exchange Membrane Fuel Cells (HT-PEMFC) SO COMPUTATIONAL STUDIES ON BATTERY AND FUEL CELL MATERIALS SE ECS Transactions LA English DT Proceedings Paper CT Symposium on Computational Studies on Battery and Fuel Cell Materials held during the 225th Meeting of the Electrochemical-Society (ECS) CY MAY 11-15, 2014 CL Orlando, FL SP Electrochem Soc, Electrochem Soc, Energy Technol Div, Electrochem Soc, Battery Div, Electrochem Soc, High Temp Mat Div, Electrochem Soc, Phys & Analyt Electrochemistry Div ID PERCENT ORTHOPHOSPHORIC ACID; GAS-DIFFUSION ELECTRODES; DOPED POLYBENZIMIDAZOLE MEMBRANES; PHOSPHORIC-ACID; OXYGEN REDUCTION; CATALYST LAYER; LIFE TEST; OPERATING TEMPERATURE; NUMERICAL-SIMULATION; NONISOTHERMAL MODEL AB The influence of the sintering of electrocatalysts and decrease of the proton conductivity on the current-voltage performance in the HT-PEMFC was theoretically evaluated under the non-humid conditions at 150 degrees C, 170 degrees C and 190 degrees C. Decreasing rate of the proton conductivity was evaluated based on the tortuosity of the proton pass. The more the phosphoric acid was evaporated with a rise in temperature, the proton path found to become more tortuous and the proton conductivity was accordingly estimated to be decreased. A theoretical breakdown of the voltage drops indicated that the sintering of the electrocatalyst influenced on the voltage drop in earlier several hundreds of hours. The following voltage drop in the latter stage was caused mainly due to the decrease in the proton conductivity. C1 [Suzuki, Ai; Miura, Ryuji; Hatakeyama, Nozomu; Miyamoto, Akira] Tohoku Univ, New Ind Creat Hatchery Ctr, Sedani, Miyagi 9808579, Japan. [Williams, Mark] US DOE, NETL, Washington, DC 20585 USA. [Oono, Yuka; Hori, Michio] Daido Univ, Dept FC Ctr, Nagoya, Aichi 08901, Japan. RP Suzuki, A (reprint author), Tohoku Univ, New Ind Creat Hatchery Ctr, Sedani, Miyagi 9808579, Japan. NR 58 TC 0 Z9 0 U1 0 U2 1 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 S MAIN ST, PENNINGTON, NJ 08534-2839 USA SN 1938-5862 BN 978-1-60768-561-6 J9 ECS TRANSACTIONS PY 2014 VL 61 IS 13 BP 7 EP 22 DI 10.1149/06113.0007ecst PG 16 WC Electrochemistry; Energy & Fuels SC Electrochemistry; Energy & Fuels GA BD9SY UT WOS:000365225500002 ER PT S AU Gandomi, YA Zawodzinski, TA Mench, MM AF Gandomi, Yasser Ashraf Zawodzinski, T. A. Mench, M. M. BE Chu, D Narayan, SR Ryan, EM TI Concentrated Solution Model of Transport in All Vanadium Redox Flow Battery Membrane Separator SO COMPUTATIONAL STUDIES ON BATTERY AND FUEL CELL MATERIALS SE ECS Transactions LA English DT Proceedings Paper CT Symposium on Computational Studies on Battery and Fuel Cell Materials held during the 225th Meeting of the Electrochemical-Society (ECS) CY MAY 11-15, 2014 CL Orlando, FL SP Electrochem Soc, Electrochem Soc, Energy Technol Div, Electrochem Soc, Battery Div, Electrochem Soc, High Temp Mat Div, Electrochem Soc, Phys & Analyt Electrochemistry Div ID PERFORMANCE; CELL AB A model of transport across the ion-exchange membrane in allvanadium redox flow batteries has been proposed based on concentrated solution theory for species with high concentration. The model is based upon the Stefan-Maxwell multicomponent diffusion equation where the fluxes of the species including protons (H+), bisulfate (HSO4-), water (H2O) and the sulfonate functional groups (-SO3-) are fully coupled. The driving force for species transport has been modeled in terms of concentration and electrostatic potential gradients. The ionic transference numbers as well as water electro-osmosis drag coefficient has been calculated for different acid concentrations. C1 [Gandomi, Yasser Ashraf; Mench, M. M.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Electrochem Energy Storage & Convers Lab, Knoxville, TN 37996 USA. [Zawodzinski, T. A.] Univ Tennessee, Chem & Biomol Engn Dept, Knoxville, TN 37996 USA. [Zawodzinski, T. A.] Oak Ridge Natl Lab, Phys Chem Mat Grp, Oak Ridge, TN 37831 USA. [Mench, M. M.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Gandomi, YA (reprint author), Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Electrochem Energy Storage & Convers Lab, Knoxville, TN 37996 USA. NR 21 TC 4 Z9 4 U1 6 U2 12 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 S MAIN ST, PENNINGTON, NJ 08534-2839 USA SN 1938-5862 BN 978-1-60768-561-6 J9 ECS TRANSACTIONS PY 2014 VL 61 IS 13 BP 23 EP 32 DI 10.1149/06113.0023ecst PG 10 WC Electrochemistry; Energy & Fuels SC Electrochemistry; Energy & Fuels GA BD9SY UT WOS:000365225500003 ER PT S AU Matanovic, I Atanassov, P Garzon, FH Henson, NJ AF Matanovic, I. Atanassov, P. Garzon, F. H. Henson, N. J. BE Chu, D Narayan, SR Ryan, EM TI Density Functional Theory Study of the Alkali Metal Cation Adsorption on Pt(111), Pt(100), and Pt(110) Surfaces SO COMPUTATIONAL STUDIES ON BATTERY AND FUEL CELL MATERIALS SE ECS Transactions LA English DT Proceedings Paper CT Symposium on Computational Studies on Battery and Fuel Cell Materials held during the 225th Meeting of the Electrochemical-Society (ECS) CY MAY 11-15, 2014 CL Orlando, FL SP Electrochem Soc, Electrochem Soc, Energy Technol Div, Electrochem Soc, Battery Div, Electrochem Soc, High Temp Mat Div, Electrochem Soc, Phys & Analyt Electrochemistry Div ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; AB-INITIO; BASIS-SET; AU AB We used density functional theory to study the adsorption of hydrogen, lithium, sodium, and potassium cations on different surfaces of platinum, namely the Pt(111), Pt(110), and Pt(100) surfaces. It was found that at low H+ concentrations alkali metal cations can compete with hydrogen for adsorption on all the studied platinum surfaces leading to a site blocking effect during the electrochemical processes involving adsorption of hydrogen in alkaline media. The strongest site blocking effect is predicted to occur on the Pt(111) surface as hydrogen and alkali metal cations adsorb in the same fcc-hollow adsorption site. On the Pt(110) and Pt(100) surface hydrogen and alkali cations adsorb on different sites and can co-exist on the surface - the most favorable adsorption site for hydrogen is a bridge site, while the hollow site is favored for all the studied alkali metal cations. Based on the calculated adsorption Gibbs free energies and the number of available adsorption sites on different surfaces, the probability of the site blocking effect by alkali cations on different surfaces of platinum was determined as Pt(111)>Pt(110)>Pt(100). C1 [Matanovic, I.; Atanassov, P.] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. [Garzon, F. H.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Henson, N. J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Matanovic, I (reprint author), Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. EM igonzales@unm.edu OI Henson, Neil/0000-0002-1842-7884 NR 25 TC 8 Z9 8 U1 2 U2 5 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 S MAIN ST, PENNINGTON, NJ 08534-2839 USA SN 1938-5862 BN 978-1-60768-561-6 J9 ECS TRANSACTIONS PY 2014 VL 61 IS 13 BP 47 EP 53 DI 10.1149/06113.0047ecst PG 7 WC Electrochemistry; Energy & Fuels SC Electrochemistry; Energy & Fuels GA BD9SY UT WOS:000365225500005 ER PT J AU Linares, R Crassidis, JL Jah, MK AF Linares, Richard Crassidis, John L. Jah, Moriba K. GP IEEE TI Space Object Classification and Characterization Via Multiple Model Adaptive Estimation SO 2014 17TH INTERNATIONAL CONFERENCE ON INFORMATION FUSION (FUSION) LA English DT Proceedings Paper CT 17th International Conference on Information Fusion (FUSION) CY JUL 07-10, 2014 CL Salamanca, SPAIN SP ISIF, VNiVERSiDAD Salamanca, Univ Carlos Madrid, IBM, IEEE, Indra AB In recent years there has been an increase in the number of inactive and debris objects in space. The characterization of the uncertainty in the knowledge of these Space Objects (SOs) is very important in developing an understanding of the space debris fields and any present or future threat they may pose. This work examines classification based on Multiple Model Adaptive Estimation (MMAE) to extract SO characteristics from observations while estimating the probability the observations belong to a given class of objects. Recovering these characteristics and trajectories with sufficient accuracy is shown in this paper, where the characteristics are inherent in unique SO models used in the MMAE filter bank. A number of scenarios are shown to highlight the effectiveness of the proposed classification approach. The performance of this strategy is demonstrated via simulated scenarios. C1 [Linares, Richard] Los Alamos Natl Lab, ISR 1, Space Sci & Applicat, Los Alamos, NM 87545 USA. [Crassidis, John L.] SUNY Buffalo, Dept Mech & Aero Eng, Space Situat Awareness, Amherst, NY 14260 USA. [Jah, Moriba K.] Kirtland Air Force Base, US Air Force Res Lab, Space Situat Awareness, Albuquerque, NM 87117 USA. RP Linares, R (reprint author), Los Alamos Natl Lab, ISR 1, Space Sci & Applicat, Los Alamos, NM 87545 USA. EM linares@lanl.gov; johnc@buffalo.edu NR 15 TC 0 Z9 0 U1 0 U2 1 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA PY 2014 PG 7 WC Computer Science, Information Systems; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA BD8FB UT WOS:000363896100314 ER PT J AU Liu, Q Wang, X Rao, NSV AF Liu, Qiang Wang, Xin Rao, Nageswara S. V. GP IEEE TI Information Feedback for Estimation and Fusion in Long-Haul Sensor Networks SO 2014 17TH INTERNATIONAL CONFERENCE ON INFORMATION FUSION (FUSION) LA English DT Proceedings Paper CT 17th International Conference on Information Fusion (FUSION) CY JUL 07-10, 2014 CL Salamanca, SPAIN SP ISIF, VNiVERSiDAD Salamanca, Univ Carlos Madrid, IBM, IEEE, Indra DE Long-haul sensor networks; state estimate fusion; information feedback; estimation bias; root-mean-square-error (RMSE) performance; reporting deadline ID FADING CHANNELS; PERFORMANCE AB Long-haul sensor networks can be found in both civilian and military applications. In a typical long-haul sensor network, sensors are remotely deployed over a large geographical area to perform tracking and/or monitoring of one or more dynamic targets. A remote fusion center fuses the information provided by these sensors so that a final estimate of certain target characteristics - such as the position - is expected to possess much improved quality. However, imperfect communication conditions can become the bottleneck for desired estimation and fusion performance. The link-level loss and delay - such as that over a satellite channel - can easily reduce the chance that an estimate is successfully received by the fusion center, thereby limiting the potential information fusion gain and resulting in suboptimal accuracy performance of the underlying task. In this work, we explore the effect of information feedback in the context of state estimation and fusion in a communication-constrained long-haul sensor network. Different feedback configurations and schedules are proposed. In particular, the joint impact of communication delay/loss, information feedback, and computation constraints is explored by means of analytical and simulation studies. C1 [Liu, Qiang; Wang, Xin] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Rao, Nageswara S. V.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Liu, Q (reprint author), SUNY Stony Brook, Stony Brook, NY 11794 USA. EM qiangliu@ece.sunysb.edu; xwang@ece.sunysb.edu; raons@ornl.gov NR 20 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA PY 2014 PG 8 WC Computer Science, Information Systems; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA BD8FB UT WOS:000363896100306 ER PT J AU Rao, NSV Ma, CYT He, F Zhuang, J Yau, DKY AF Rao, Nageswara S. V. Ma, Chris Y. T. He, Fei Zhuang, Jun Yau, David K. Y. GP IEEE TI Cyber-Physical Correlations for Infrastructure Resilience: A Game-Theoretic Approach SO 2014 17TH INTERNATIONAL CONFERENCE ON INFORMATION FUSION (FUSION) LA English DT Proceedings Paper CT 17th International Conference on Information Fusion (FUSION) CY JUL 07-10, 2014 CL Salamanca, SPAIN SP ISIF, VNiVERSiDAD Salamanca, Univ Carlos Madrid, IBM, IEEE, Indra ID RESOURCE-ALLOCATION; ATTACKER; FACE AB In several critical infrastructures, the cyber and physical parts are correlated so that disruptions to one affect the other and hence the whole system. These correlations may be exploited to strategically launch components attacks, and hence must be accounted for ensuring the infrastructure resilience, specified by its survival probability. We characterize the cyber-physical interactions at two levels: (i) the failure correlation function specifies the conditional survival probability of cyber sub-infrastructure given the physical sub-infrastructure as a function of their marginal probabilities, and (ii) the individual survival probabilities of both sub-infrastructures are characterized by first-order differential conditions. We formulate a resilience problem for infrastructures composed of discrete components as a game between the provider and attacker, wherein their utility functions consist of an infrastructure survival probability term and a cost term expressed in terms of the number of components attacked and reinforced. We derive Nash Equilibrium conditions and sensitivity functions that highlight the dependence of infrastructure resilience on the cost term, correlation function and sub-infrastructure survival probabilities. These results generalize earlier ones based on linear failure correlation functions and independent component failures. We apply the results to models of cloud computing infrastructures and energy grids. C1 [Rao, Nageswara S. V.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [He, Fei; Zhuang, Jun] SUNY Buffalo, Buffalo, NY 14260 USA. [Yau, David K. Y.] Singapore Univ Technol & Design, Singapore, Singapore. RP Rao, NSV (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RI Zhuang, Jun/E-8081-2010 OI Zhuang, Jun/0000-0003-4830-6570 NR 20 TC 0 Z9 0 U1 2 U2 2 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA PY 2014 PG 8 WC Computer Science, Information Systems; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA BD8FB UT WOS:000363896100174 ER PT B AU Franks, LA James, RB Darken, LS AF Franks, Larry A. James, Ralph B. Darken, Larry S. BE Webster, JG Eren, H TI Radioactivity Detectors SO MEASUREMENT, INSTRUMENTATION, AND SENSORS HANDBOOK: SPATIAL, MECHANICAL, THERMAL, AND RADIATION MEASUREMENT, 2ND EDITION LA English DT Article; Book Chapter ID HIGH-PURITY GERMANIUM; RAY-DETECTORS; LOW-NOISE; DRIFT; RESOLUTION; FABRICATION; HGI2 C1 [Franks, Larry A.; James, Ralph B.] Sandia Natl Labs, Livermore, CA 94550 USA. [Darken, Larry S.] Oxford Instruments Inc, Oak Ridge, TN USA. RP Franks, LA (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. NR 49 TC 0 Z9 0 U1 0 U2 0 PU CRC PRESS-TAYLOR & FRANCIS GROUP PI BOCA RATON PA 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA BN 978-1-4398-4889-0; 978-1-4398-4888-3 PY 2014 PG 27 WC Engineering, Multidisciplinary; Remote Sensing SC Engineering; Remote Sensing GA BD7IZ UT WOS:000363202800082 ER PT B AU Auld, J Mohammadian, A AF Auld, Joshua Mohammadian, Abolfaz (Kouros) BA Rasouli, S Timmermans, H BF Rasouli, S Timmermans, H TI Collecting Activity-Travel and Planning Process Data Using GPS-Based Prompted Recall Surveys: Recent Experience and Future Directions SO MOBILE TECHNOLOGIES FOR ACTIVITY-TRAVEL DATA COLLECTION AND ANALYSIS SE Advances in Data Mining and Database Management (ADMDM) Book Series LA English DT Article; Book Chapter ID TRIPS AB This chapter details the design, implementation, and evaluation of an Intentet-based prompted recall survey that utilized GPS data collection. The design of the survey was unique in terms of prompted recall surveys using GPS with the use of instantaneous data processing, learning algorithms to reduce respondent burden, and the inclusion of questions relating to activity-planning behavior in a prompted recall survey. In the Urban Travel Route and Activity Choice Survey (UTRACS), data was collected on long-term activity-travel behavior and planning processes for 112 individuals over an average of 10 days. The results of the survey show that the planning data obtained from the survey respondents appear to be reliable, with minimal fatigue and conditioning effects. The documentation of the survey design process, coupled with the promising results, show how GPS-based prompted recall surveys using an Internet-based survey mode can collect useful activity processing data over long time frames. C1 [Auld, Joshua] Argonne Natl Lab, Argonne, IL 60439 USA. [Mohammadian, Abolfaz (Kouros)] Univ Illinois, Transportat Syst, Chicago, IL USA. RP Auld, J (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. NR 40 TC 0 Z9 0 U1 0 U2 0 PU IGI GLOBAL PI HERSEY PA 701 E CHOCOLATE AVE, STE 200, HERSEY, PA 17033-1240 USA BN 978-1-4666-6171-4; 978-1-4666-6170-7 J9 ADV DATA MIN DATABAS PY 2014 BP 53 EP 78 DI 10.4018/978-1-4666-6170-7.ch004 D2 10.4018/978-1-4666-6170-7 PG 26 WC Computer Science, Artificial Intelligence; Computer Science, Information Systems SC Computer Science GA BD7JK UT WOS:000363211700006 ER PT J AU Chen, J Waston, W Chen, MF AF Chen, Jie Waston, William, III Chen, Mayee F. GP IEEE TI Efficient GCD Computation for Big Integers on Xeon Phi Coprocessor SO 2014 9th IEEE International Conference on Networking, Architecture, and Storage (NAS) LA English DT Proceedings Paper CT 9th IEEE International Conference on Networking, Architecture, and Storage (NAS) CY AUG 06-08, 2014 CL Tianjin,, PEOPLES R CHINA SP IEEE, IEEE Comp Soc DE GCD; Xeon Phi; Vectorization; RSA; OpenMP AB Efficient calculation of the greatest common divisor (GCD) for big integers each whose number of bits is greater than or equal to 1024 has drawn a considerable amount of attention because it can be used to detect a weakness of the RSA security infrastructure. This paper presents a parallel binary GCD algorithm and its implementation for big integers on the Intel Xeon Phi coprocessor. This algorithm is capable of computing GCDs efficiently on many pairs of big integers in parallel by utilizing all cores on a Xeon Phi coprocessor as well as taking advantage of all vector processing units of the coprocessor to speed up critical integer operations within the algorithm. Using 240 threads on a Xeon Phi coprocessor to carry out GCD calculations for a large amount of 2048-bit integers, the implementation achieves the speedup of 30 times over a sequential binary GCD algorithm implementation on a single CPU core, and it delivers twice amount of performance in comparison to the same sequential binary GCD implementation running on 240 threads of the Xeon Phi. C1 [Chen, Jie; Waston, William, III] Jefferson Lab, Sci Comp Grp, Newport News, VA 23606 USA. [Chen, Mayee F.] Jamestown High Sch, Williamsburg, VA 23188 USA. RP Chen, J (reprint author), Jefferson Lab, Sci Comp Grp, Newport News, VA 23606 USA. EM chen@jlab.org; watson@jlab.org; mayeefchen@gmail.com NR 7 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-4087-5 PY 2014 BP 113 EP 117 DI 10.1109/NAS.2014.25 PG 5 WC Computer Science, Hardware & Architecture; Computer Science, Information Systems SC Computer Science GA BD8JB UT WOS:000363981700014 ER PT S AU Marra, JC Kim, DS AF Marra, James C. Kim, Dong-Sang BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Towards increased waste loading in high level waste glasses: developing a better understanding of crystallization behavior SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE DE vitrification; glass melter; nepheline; spinel; waste loading AB A number of waste components in US defense high level radioactive wastes (HLW) have proven challenging for current Joule heated ceramic melter (JCHM) operations and have limited the ability to increase waste loadings beyond already realized levels. Many of these "troublesome" waste species cause crystallization in the glass melt that can negatively impact product quality or have a deleterious effect on melter processing. Recent efforts at US Department of Energy laboratories have focused on understanding crystallization behavior within HLW glass melts and investigating approaches to mitigate the impacts of crystallization so that increases in waste loading can be realized. Advanced glass formulations have been developed to highlight the unique benefits of next-generation melter technologies such as the Cold Crucible Induction Melter (CCIM). Crystal-tolerant HLW glasses have been investigated to allow sparingly soluble components such as chromium to crystallize in the melter but pass out of the melter before accumulating. The Hanford site AZ-101 tank waste composition represents a waste group that is waste loading limited primarily due to high concentrations of Fe2O3 (with higher Al2O3). Systematic glass formulation development utilizing slightly higher process temperatures and higher tolerance to spinel crystals demonstrated that an increase in waste loading of more than 20% could be achieved for this waste composition, and by extension higher loadings for wastes in the same group. (C) 2014 Published by Elsevier Ltd. C1 [Marra, James C.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Kim, Dong-Sang] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Marra, JC (reprint author), Savannah River Natl Lab, POB 616, Aiken, SC 29808 USA. EM james.marra@srnl.doe.gov NR 13 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 87 EP 92 DI 10.1016/j.mspro.2014.10.012 PG 6 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100011 ER PT S AU Hrma, P AF Hrma, Pavel BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Conversion of nuclear waste into nuclear waste glass: Experimental investigation and mathematical modeling SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE ID COLD-CAP REACTIONS; MOLTEN GLASS; MELTER FEED; BATCH; VITRIFICATION; DISSOLUTION; PARTICLES; SILICA; QUARTZ AB The melter feed, slurry, or calcine charged on the top of a pool of molten glass forms a floating layer of reacting material called the cold cap. Between the cold-cap top, which is covered with boiling slurry, and its bottom, where bubbles separate it from molten glass, the temperature changes by up to 1000 K. The processes that occur over this temperature interval within the cold cap include liberation of gases, conduction and consumption of heat, dissolution of quartz particles, formation and dissolution of intermediate crystalline phases, and generation of foam and gas cavities. These processes have been investigated using thermal analyses, optical and electronic microscopies, x-ray diffraction, as well as other techniques. Properties of the reacting feed, such as heat conductivity and density, were measured as functions of temperature. Investigating the structure of quenched cold caps produced in a laboratory-scale melter complemented the crucible studies. The cold cap consists of two main layers. The top layer contains solid particles dissolving in the glass-forming melt and open pores through which gases are escaping. The bottom layer contains bubbly melt or foam where bubbles coalesce into larger cavities that move sideways and release the gas to the atmosphere. The feed-to-glass conversion became sufficiently understood for representing the cold-cap processes via mathematical models. These models, which comprise heat transfer, mass transfer, and reaction kinetics models, have been developed with the final goal to relate feed parameters to the rate of glass melting. (C) 2014 The Authors. Published by Elsevier C1 Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hrma, P (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM Pavel.Hrma@pnnl.gov NR 26 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 117 EP 123 DI 10.1016/j.mspro.2014.10.016 PG 7 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100015 ER PT S AU Vienna, JD AF Vienna, John D. BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Compositional Models of Glass/Melt Properties and their Use for Glass Formulation SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE DE Glass; Nuclear Waste; Property; Borosilicate; Melt; Formulation; Model ID MIXTURE; TEMPERATURE; LIQUIDUS AB Nuclear waste glasses must simultaneously meet a number of criteria related to their processability, product quality, and cost factors. The properties that must be controlled in glass formulation and waste vitrification plant operation tend to vary smoothly with composition allowing for glass property-composition models to be developed and used. Models have been fit to the key glass properties. The properties are transformed so that simple functions of composition (e.g., linear, polynomial, or component ratios) can be used as model forms. The model forms are fit to experimental data designed statistically to efficiently cover the composition space of interest. Examples of these models are found in literature. The glass property-composition models, their uncertainty definitions, property constraints, and optimality criteria are combined to formulate optimal glass compositions, control composition in vitrification plants, and to qualify waste glasses for disposal. An overview of current glass property-composition modeling techniques is summarized in this paper along with an example of how those models are applied to glass formulation and product qualification at the planned Hanford high-level waste vitrification plant. (C) 2014 The Authors. Published by Elsevier Ltd. C1 Pacific NW Natl Lab, Richland, WA 99352 USA. RP Vienna, JD (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.vienna@pnnl.gov NR 33 TC 1 Z9 1 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 148 EP 155 DI 10.1016/j.mspro.2014.10.020 PG 8 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100019 ER PT S AU Hopf, J Pierce, EM AF Hopf, Juliane Pierce, E. M. BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Topography and mechanical property mapping of International Simple Glass surfaces with atomic force microscopy SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE DE Quantitative Nanomechanical Peak Force (R) TappingMode (TM); atomic force microscopy; borosilicate glass; Young's modulus ID ELASTIC-MODULUS; CALCITE; ADHESION; BEHAVIOR; GROWTH; TERM AB Quantitative Nanomechanical Peak Force (R) (PF-QNM) TappingMode (TM) atomic force microscopy measurements are presented for the first time on polished glass surfaces. The PF-QNM technique allows for topography and mechanical property information to be measured simultaneously at each pixel. Results for the international simple glass-which represents a simplified version of SON68 glass-suggests the average Young's modulus of 78.8 +/- 15.1 GPa is within the experimental error of the modulus measured for SON68 glass (83.6 +/- 2 GPa) using conventional approaches. Application of the PF-QNM technique will be extended to in situ glass corrosion experiments with the goal of gaining atomic-scale insights into altered layer development by exploiting the mechanical property differences that exist between silica gel (e.g., altered layer) and pristine glass surface. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [Hopf, Juliane; Pierce, E. M.] Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37774 USA. RP Pierce, EM (reprint author), Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37774 USA. EM pierceem@ornl.gov RI Pierce, Eric/G-1615-2011 OI Pierce, Eric/0000-0002-4951-1931 NR 25 TC 3 Z9 3 U1 3 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 216 EP 222 DI 10.1016/j.mspro.2014.10.028 PG 7 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100028 ER PT S AU Weber, WJ AF Weber, William J. BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Radiation and Thermal Ageing of Nuclear Waste Glass SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE DE radiation effects; helium behavior; alpha decay; beta decay ID BOROSILICATE GLASS; IRRADIATION; PLUTONIUM; IMMOBILIZATION; FORMS AB The radioactive decay of fission products and actinides incorporated into nuclear waste glass leads to self-heating and self-radiation effects that may affect the stability, structure and performance of the glass in a closed system. Short-lived fission products cause significant self-heating for the first 600 years. Alpha decay of the actinides leads to self-radiation damage that can be significant after a few hundred years, and over the long time periods of geologic disposal, the accumulation of helium and radiation damage from alpha decay may lead to swelling, microstructural evolution and changes in mechanical properties. Four decades of research on the behavior of nuclear waste glass are reviewed. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Weber, WJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM wjweber@utk.edu RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 NR 25 TC 0 Z9 0 U1 4 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 237 EP 246 DI 10.1016/j.mspro.2014.10.031 PG 10 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100031 ER PT S AU Toulemonde, M Assmann, W Zhang, Y Backman, M Weber, WJ Dufour, C Wang, ZG AF Toulemonde, M. Assmann, W. Zhang, Y. Backman, M. Weber, W. J. Dufour, C. Wang, Z. G. BE Angeli, F Delaye, JM Schuller, S Pinet, O Rebiscoul, D Gin, S Peuget, S TI Material transformation: Interaction between nuclear and electronic energy losses SO 2ND INTERNATIONAL SUMMER SCHOOL ON NUCLEAR GLASS WASTEFORM: STRUCTURE, PROPERTIES AND LONG-TERM BEHAVIOR (SUMGLASS 2013) SE Procedia Materials Science LA English DT Proceedings Paper CT 2nd International Summer School on Nuclear Glass Wasteform - Structure, Properties and Long-Term Behavior (SumGLASS) CY SEP 23-27, 2013 CL FRANCE DE swift heavy ions; nuclear energy loss; electronic energy loss; interaction between nuclear and eelctronic; defects; sputtering; SiO2; Fe; Ti ID HEAVY-ION IRRADIATION; METALS; SIMULATIONS; DAMAGE; DEFECTS; SPIKES AB The interaction between nuclear and electronic energy losses induced by an individual ion are described and illustrated by four different experiments. Each experiment shows the different behaviors of the combined interactions. Defects created by nuclear energy loss are annealed by electronic energy loss in Fe by ions in the GeV energy regime, showing a competitive interaction (1+1<1). The sputtering of Ti is enhanced by electronic excitation induced by similar to 100 MeV ions supporting a synergetic interaction (1+1>2). Damage cross section in crystalline and amorphous SiO2 is enhanced by ions in the MeV regime, evidencing a cooperative interaction (1+1>1 and <2). Moreover Molecular Dynamic calculations show that defects created by nuclear and electronic collisions appear to be additive (1+1 = 2) in this same range of beam energy. (C) 2014 Published by Elsevier Ltd. C1 [Toulemonde, M.; Dufour, C.] Univ Caen, CIMAP, GANIL, CEA,CNRS,ENSICAEN, F-14070 Caen, France. [Assmann, W.] Univ Munich, D-85748 Garching, Germany. [Zhang, Y.; Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Tech Div, Oak Ridge, TN 37831 USA. [Zhang, Y.; Backman, M.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Wang, Z. G.] Chinese Acad Sci, IMP, Lanzhou 730000, Peoples R China. RP Toulemonde, M (reprint author), Univ Caen, CIMAP, GANIL, CEA,CNRS,ENSICAEN, Bd H Becquerel, F-14070 Caen, France. EM toulemonde@ganil.fr RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 NR 29 TC 0 Z9 0 U1 1 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-8128 J9 PROC MAT SCI PY 2014 VL 7 BP 272 EP 277 DI 10.1016/j.mspro.2014.10.035 PG 6 WC Engineering, Environmental; Materials Science, Multidisciplinary; Nuclear Science & Technology SC Engineering; Materials Science; Nuclear Science & Technology GA BD9FB UT WOS:000364543100035 ER PT S AU Brunecky, R Donohoe, BS Selig, MJ Wei, H Resch, M Himmel, ME AF Brunecky, Roman Donohoe, Bryon S. Selig, Michael J. Wei, Hui Resch, Michael Himmel, Michael E. BE Goldman, SL Kole, C TI Basic Biological Research Relevant to Feedstock Conversion SO COMPENDIUM OF BIOENERGY PLANTS: CORN SE Compendium of Bioenergy Plants LA English DT Article; Book Chapter DE Zea mays L. subspecies; Biofuels; Bioconversion; Thermophile; Termite; Cellulosome; CelA; CelE; Lignin; Cellulose; Xylan ID ENHANCE ENZYMATIC-HYDROLYSIS; DILUTE-ACID PRETREATMENT; MAIZE STEM TISSUES; CELLULOSE-I-BETA; CORN STOVER; LIGNOCELLULOSIC BIOMASS; MOLECULAR-CLONING; TOLERANT XYLANASE; CELL-WALLS; CALDICELLULOSIRUPTOR-BESCII AB Zea mays L. subspecies is an important feedstock for future bioconversion process of biomass to fuels and chemicals. However, conversion of this lignocellulosic material remains problematic due to the recalcitrant nature of corn stover. Here we examine some of the important considerations in the bioconversion of this feedstock, including a brief overview of the nature recalcitrance phenomenon, examining the anatomical as well as gross chemical factors of recalcitrance. Also examined herein are the major biopolymers and the role each one is thought to play in biomass recalcitrance. We then explore both current and future strategies employed to overcome natural plant cell wall recalcitrance, including an examination of pretreatment technologies and how these strategies inform the choice of enzymatic deconstruction systems. Finally we examine some potential future sources of biomass deconstructing enzymes, in particular the promise of extremozymes as well as cellulosomal and termite enzyme systems that may be used as future platforms for the conversion of lignocellulosic materials to their constitutative sugars. C1 [Brunecky, Roman; Donohoe, Bryon S.; Wei, Hui; Resch, Michael; Himmel, Michael E.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Selig, Michael J.] Univ Copenhagen, Dept Forest & Landscape, DK-1958 Frederiksberg C, Denmark. RP Brunecky, R (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM roman.brunecky@nrel.gov; bryon.donohoe@nrel.gov; michaeljselig@yahoo.com; hui.wei@nrel.gov; mchael.resch@nrel.gov; mike.himmel@nrel.gov NR 175 TC 1 Z9 1 U1 1 U2 1 PU CRC PRESS-TAYLOR & FRANCIS GROUP PI BOCA RATON PA 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA SN 2376-7073 BN 978-1-4822-1059-0 J9 COMPEND BIOENERG PLA PY 2014 BP 33 EP 77 PG 45 WC Agronomy; Biotechnology & Applied Microbiology; Plant Sciences; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Plant Sciences; Energy & Fuels GA BD9EM UT WOS:000364537700004 ER PT S AU Kwit, C Nageswara-Rao, M Stewart, CN AF Kwit, Charles Nageswara-Rao, Madhugiri Stewart, C. Neal, Jr. BE Luo, H Wu, Y Kole, C TI Switchgrass (Panicum virgatum L.) as a Bioenergy Crop: Advantages, Concerns, and Future Prospects SO COMPENDIUM OF BIOENERGY PLANTS: SWITCHGRASS SE Compendium of Bioenergy Plants LA English DT Article; Book Chapter ID MISCANTHUS X GIGANTEUS; SOIL CARBON SEQUESTRATION; UNITED-STATES; BIOFUEL PRODUCTION; BIOMASS PRODUCTION; ETHANOL-PRODUCTION; CLIMATE-CHANGE; USE EFFICIENCY; WATER-QUALITY; UPPER MIDWEST C1 [Kwit, Charles; Nageswara-Rao, Madhugiri; Stewart, C. Neal, Jr.] Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. [Stewart, C. Neal, Jr.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Kwit, C (reprint author), Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. EM ckwit@utk.edu; mnrao@utk.edu; nealstewart@utk.edu NR 101 TC 2 Z9 2 U1 5 U2 7 PU CRC PRESS-TAYLOR & FRANCIS GROUP PI BOCA RATON PA 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA SN 2376-7073 BN 978-1-4665-9637-5 J9 COMPEND BIOENERG PLA PY 2014 BP 403 EP 421 PG 19 WC Agronomy; Biotechnology & Applied Microbiology; Plant Sciences; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Plant Sciences; Energy & Fuels GA BD9EL UT WOS:000364537400016 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Section I: Food Security Policy Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 1 EP 5 PG 5 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900003 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Introduction to Food Security: Concepts and Measurement SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 7 EP 28 DI 10.1016/B978-0-12-405864-4.00001-6 PG 22 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900004 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Food Security, Poverty, and Nutrition Policy Analysis Statistical Methods and Applications Second Edition Preface SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP XVII EP + PG 28 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900001 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Food Security, Poverty, and Nutrition Policy Analysis Statistical Methods and Applications Second Edition Introduction SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP XXI EP XXXI PG 11 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900002 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Implications of Technological Change, Post-Harvest Technology, and Technology Adoption for Improved Food Security-Application of t-Statistic SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 29 EP 61 DI 10.1016/B978-0-12-405864-4.00002-8 PG 33 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900005 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Effects of Commercialization of Agriculture (Shift from Traditional Crop to Cash Crop) on Food Consumption and Nutrition-Application of Chi-Square Statistic SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 2 Z9 2 U1 1 U2 1 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 63 EP 91 DI 10.1016/B978-0-12-405864-4.00003-X PG 29 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900006 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Effects of Technology Adoption and Gender of Household Head: The Issue, Its Importance in Food Security-Application of Cramer's V and Phi Coefficient SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 93 EP 115 DI 10.1016/B978-0-12-405864-4.00004-1 PG 23 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900007 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Changes in Food Consumption Patterns: Its Importance to Food Security-Application of One-Way ANOVA SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 1 Z9 1 U1 0 U2 1 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 117 EP 138 DI 10.1016/B978-0-12-405864-4.00005-3 PG 22 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900008 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Impact of Market Access on Food Security - Application of Factor Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 139 EP 175 DI 10.1016/B978-0-12-405864-4.00006-5 PG 37 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900009 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Section II: Nutrition Policy Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 177 EP 184 PG 8 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900010 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Impact of Maternal Education and Care on Preschoolers' Nutrition - Application of Two-Way ANOVA SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 185 EP 213 DI 10.1016/B978-0-12-405864-4.00007-7 PG 29 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900011 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Indicators and Causal Factors of Nutrition - Application of Correlation Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 215 EP 241 DI 10.1016/B978-0-12-405864-4.00008-9 PG 27 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900012 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Effects of Individual, Household, and Community Indicators on Child's Nutritional Status - Application of Simple Linear Regression SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 243 EP 274 DI 10.1016/B978-0-12-405864-4.00009-0 PG 32 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900013 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Maternal Education and Community Characteristics as Indicators of Nutritional Status of Children - Application of Multivariate Regression SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 275 EP 311 DI 10.1016/B978-0-12-405864-4.00010-7 PG 37 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900014 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Section III: Special Topics on Poverty, Nutrition, and Food Policy Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 313 EP 315 PG 3 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900015 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Predicting Child Nutritional Status Using Related Socioeconomic Variables - Application of Discriminant Function Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 317 EP 359 DI 10.1016/B978-0-12-405864-4.00011-9 PG 43 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900016 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Measurement and Determinants of Poverty - Application of Logistic Regression Models SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 1 Z9 1 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 361 EP 415 DI 10.1016/B978-0-12-405864-4.00012-0 PG 55 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900017 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Classifying Households On Food Security and Poverty Dimensions - Application of K-Mean Cluster Analysis SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 417 EP 439 DI 10.1016/B978-0-12-405864-4.00003-2 PG 23 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900018 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Household Care as a Determinant of Nutritional Status-Application of Instrumental Variable Estimation SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 441 EP 460 DI 10.1016/B978-0-12-405864-4.00014-4 PG 20 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900019 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Achieving an Ideal Diet-Modeling with Linear Programming SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 1 Z9 1 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 461 EP 476 DI 10.1016/B978-0-12-405864-4.00015-6 PG 16 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900020 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Food and Nutrition Program Evaluation SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 477 EP 488 DI 10.1016/B978-0-12-405864-4.00016-8 PG 12 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900021 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Introduction to Software Access and Use SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Editorial Material; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 491 EP 491 DI 10.1016/B978-0-12-405864-4.00034-7 PG 1 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900022 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Software Information SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 493 EP 494 DI 10.1016/B978-0-12-405864-4.00025-9 PG 2 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900023 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI SPSS/PC plus Environment and Commands SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 495 EP 503 DI 10.1016/B978-0-12-405864-4.00026-0 PG 9 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900024 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Data Handling SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 505 EP 515 DI 10.1016/B978-0-12-405864-4.00027-2 PG 11 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900025 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI SPSS Programming Basics SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 517 EP 529 DI 10.1016/B978-0-12-405864-4.00028-4 PG 13 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900026 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI STATA-A Basic Tutorial SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 531 EP 536 DI 10.1016/B978-0-12-405864-4.00029-6 PG 6 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900027 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Anthropometric Indicators-Computation and Use SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 537 EP 542 DI 10.1016/B978-0-12-405864-4.00030-2 PG 6 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900028 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Elements of Matrix Algebra SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 543 EP 547 DI 10.1016/B978-0-12-405864-4.00031-4 PG 5 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900029 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Some Preliminary Statistical Concepts SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 549 EP 551 DI 10.1016/B978-0-12-405864-4.00032-6 PG 3 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900030 ER PT B AU Babu, SC Gajanan, SN Sanyal, P AF Babu, Suresh C. Gajanan, Shailendra N. Sanyal, Prabuddha BA Babu, SC Gajanan, SN Sanyal, P BF Babu, SC Gajanan, SN Sanyal, P TI Instrumental Variable Estimation SO Food Security, Poverty, and Nutrition Policy Analysis: Statistical Methods and Applications, 2nd Edition LA English DT Article; Book Chapter C1 [Babu, Suresh C.] Int Food Policy Res Inst, Washington, DC 20036 USA. [Gajanan, Shailendra N.] Univ Pittsburgh, Bradford, PA USA. [Sanyal, Prabuddha] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Babu, SC (reprint author), Int Food Policy Res Inst, Washington, DC 20036 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND BN 978-0-12-405909-2; 978-0-12-405864-4 PY 2014 BP 553 EP 558 DI 10.1016/B978-0-12-405864-4.00033-8 PG 6 WC Public, Environmental & Occupational Health; Social Sciences, Mathematical Methods; Planning & Development SC Public, Environmental & Occupational Health; Mathematical Methods In Social Sciences; Public Administration GA BD6EZ UT WOS:000362168900031 ER PT B AU Morris, DE de Bettencourt-Dias, A AF Morris, David E. de Bettencourt-Dias, Ana BE DeBettencourtDias, A TI Spectroscopic Techniques and Instrumentation SO Luminescence of Lanthanide Ions in Coordination Compounds and Nanomaterials LA English DT Article; Book Chapter ID METALLIC ION SOLVATION; QUANTUM YIELDS; LANTHANIDE LUMINESCENCE; INTEGRATING SPHERE; WATER-MOLECULES; RARE-EARTH; FT IR; COMPLEXES; EFFICIENCY; EUROPIUM C1 [Morris, David E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [de Bettencourt-Dias, Ana] Univ Nevada, Dept Chem, Reno, NV 89557 USA. RP Morris, DE (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. OI de Bettencourt-Dias, Ana/0000-0001-5162-2393 NR 57 TC 1 Z9 1 U1 0 U2 1 PU JOHN WILEY & SONS LTD PI CHICHESTER PA THE ATRIUM, SOUTHERN GATE, CHICHESTER PO19 8SQ, WEST SUSSEX, ENGLAND BN 978-1-118-68276-0; 978-1-119-95083-7 PY 2014 BP 49 EP 75 D2 10.1002/9781118682760 PG 27 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics SC Science & Technology - Other Topics; Materials Science; Optics GA BD6ZI UT WOS:000362774800003 ER PT J AU Shokri, A Deng, SHM Wang, XB Kass, SR AF Shokri, Alireza Deng, S. H. M. Wang, Xue-Bin Kass, Steven R. TI Molecular recognition: preparation and characterization of two tripodal anion receptors SO Organic Chemistry Frontiers LA English DT Article ID HYDROGEN-BONDING RECEPTORS; DENSITY FUNCTIONALS; BASIS-SETS; BINDING; TRANSPORTERS; ENERGETICS; THERMOCHEMISTRY; COORDINATION; DERIVATIVES; SCAFFOLDS AB Two new tripodal hydroxyl-based anion receptors (1 and 2) are reported and their 1 : 1 molecular complexes with Cl-, H2PO4-, and OAc- along with the (M - 1)(-) ion of 1 were characterized by negative ion photoelectron spectroscopy in the gas phase and by binding constant determinations in four solvents (i.e., CDCl3, CD2Cl2, CD3COCD3, and CD3CN). An intramolecular hydrogen bond network (HBN) in hexaol 1 was found to diminish its binding whereas the triol 2 is the strongest aliphatic hydroxyl-based receptor to date. C1 [Shokri, Alireza; Kass, Steven R.] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA. [Deng, S. H. M.; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Deng, S. H. M.; Wang, Xue-Bin] Washington State Univ, Dept Phys, Richland, WA 99354 USA. RP Shokri, A (reprint author), Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM xuebin.wang@pnnl.gov; kass@umn.edu FU DOE's Office of Biological and Environmental Research at Pacific Northwest National Laboratory; National Science Foundation; Minnesota Supercomputer Institute for Advanced Computational Research; U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX We thank Mr Masoud Samet for obtaining the 13C NMR spectrum of 1. Generous support from the National Science Foundation and the Minnesota Supercomputer Institute for Advanced Computational Research are gratefully acknowledged. The U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences supported the photoelectron spectra work (XBW), which was performed at the EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for DOE. NR 80 TC 10 Z9 10 U1 2 U2 6 PU CHINESE CHEMICAL SOC PI TAIPEI PA PO BOX 1-18, NANKANG, TAIPEI 115, TAIWAN SN 2052-4129 J9 ORG CHEM FRONT JI Org. Chem. Front. PY 2014 VL 1 IS 1 BP 54 EP 61 DI 10.1039/c3qo00009e PG 8 WC Chemistry, Organic SC Chemistry GA CV7AB UT WOS:000364422700008 ER PT J AU Targhetta, AD Owen, DE Gratz, PV AF Targhetta, Andrew D. Owen, Donald E., Jr. Gratz, Paul V. GP IEEE TI The Design Space of Ultra-low Energy Asymmetric Cryptography SO 2014 IEEE INTERNATIONAL SYMPOSIUM ON PERFORMANCE ANALYSIS OF SYSTEMS AND SOFTWARE (ISPASS) SE IEEE International Symposium on Performance Analysis of Systems and Software-ISPASS LA English DT Proceedings Paper CT IEEE International Symposium on Performance Analysis of Systems and Software (ISPASS) CY MAR 23-25, 2014 CL Monterey, CA SP IEEE, IEEE Comp Soc, IBM Res, ARM, Samsung Res America AB The energy cost of asymmetric cryptography, a vital component of modern secure communications, inhibits its wide spread adoption within the ultra-low energy regimes such as Implantable Medical Devices (IMDs), Wireless Sensor Networks (WSNs), and Radio Frequency Identification tags (RFIDs). Consequently, a gamut of hardware/software acceleration techniques exists to alleviate this energy burden. In this paper, we explore this design space, estimating the energy consumption for three levels of acceleration across the commercial security spectrum. First we examine an efficient baseline architecture centered around a pipelined RISC processor. We then include simple, yet beneficial instruction set extensions to our microarchitecture and evaluate the improvement in terms of energy per operation compared to baseline. Finally, we introduce a novel, dedicated accelerator to our microarchitecture and measure the energy per operation against the baseline and the ISA extensions. For ISA extensions, we show between 1.28 to 1.41 factor improvement in energy efficiency over baseline, while for full acceleration we demonstrate a 4.36 to 6.45 factor improvement. C1 [Targhetta, Andrew D.; Gratz, Paul V.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Owen, Donald E., Jr.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Targhetta, AD (reprint author), Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. EM atarghel@tamu.edu; deowen@sandia.gov; pgratz@gratzl.com NR 34 TC 3 Z9 3 U1 0 U2 4 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-3606-9 J9 INT SYM PERFORM ANAL PY 2014 BP 55 EP 65 PG 11 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA BD8LX UT WOS:000364102000007 ER PT J AU Widl, E Delinchantt, B Kubler, S Li, D Muller, W Norrefeldtl, V Nouidui, TS Stratbucker, S Wetter, M Wurtz, F Zuo, WD AF Widl, Edmund Delinchantt, Benoit Kuebler, Svea Li, Dan Mueller, Wolfgang Norrefeldtl, Victor Nouidui, Thierry Stephane Stratbuecker, Sebastian Wetter, Michael Wurtz, Frederic Zuo, Wangda GP IEEE TI Novel Simulation Concepts for Buildings and Community Energy Systems based on the Functional Mock-up Interface Specification SO 2014 WORKSHOP ON MODELING AND SIMULATION OF CYBER-PHYSICAL ENERGY SYSTEMS (MSCPES) LA English DT Proceedings Paper CT Workshop on Modeling and Simulation of Cyber-Physical Energy Systems (MSCPES) Held as Part of CPS Week CY APR 14-17, 2014 CL Berlin, GERMANY SP IEEE, IEEE Ind Elect Soc, Austrian Inst Technol, Berkeley Univ California DE buildings simulation; community energy system simulation; co-simulation; model exchange; Functional Mock-up Interface; FMI ID AIR-FLOW AB Research and development in the fields of building technologies and community energy systems have caused in recent years a transition away from stand-alone components towards dynamically interacting systems. However, the precise modeling and simulation of such complex cyber-physical systems proves challenging for the established simulation tools. This paper illustrates the applicability of co-simulation and model exchange concepts based on the Functional Mock-up Interface (FMI) specification for the simulation of buildings and community energy systems by comparing several state-of-the-art approaches. The presented applications thereby demonstrate the suitability and relevance of such modular and flexible simulation concepts for these fields. At the same time the importance of a common simulation interface is emphasized, which allows the reuse of individual components for a diverse range of applications. C1 [Widl, Edmund; Mueller, Wolfgang] AIT, Vienna, Austria. [Delinchantt, Benoit; Wurtz, Frederic] G2ELab, St Martin Dheres, France. [Kuebler, Svea; Norrefeldtl, Victor; Stratbuecker, Sebastian] Fraunhofer Inst Bldg Phys IBP, Holzkirchen Branch, Valley, Germany. [Li, Dan; Zuo, Wangda] Univ Miami, Coral Gables, FL 33124 USA. [Nouidui, Thierry Stephane; Wetter, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Widl, E (reprint author), AIT, Vienna, Austria. NR 27 TC 0 Z9 0 U1 2 U2 2 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-4702-7 PY 2014 PG 6 WC Computer Science, Interdisciplinary Applications; Energy & Fuels; Engineering, Electrical & Electronic SC Computer Science; Energy & Fuels; Engineering GA BD8RO UT WOS:000364221400003 ER PT J AU Pun, AB Gagnon, KJ Klivansky, LM Teat, SJ Li, ZT Liu, Y AF Pun, Andrew B. Gagnon, Kevin J. Klivansky, Liana M. Teat, Simon J. Li, Zhan-Ting Liu, Yi TI Solvent-driven selective pi-cation templating in dynamic assembly of interlocked molecules SO ORGANIC CHEMISTRY FRONTIERS LA English DT Article ID SELF-SORTING ORGANIZATION; METAL-ORGANIC FRAMEWORKS; 2 HETERODITOPIC MONOMERS; DIRECTED SYNTHESIS; SUPRAMOLECULAR POLYMER; COVALENT CHEMISTRY; BISTABLE ROTAXANES; SHAPE-PERSISTENT; BORROMEAN RINGS; ONE-POT AB Both bispyridinium (BPY) and trispyridinium (TPY) have been used to template the formation of linear or triply threaded [2]rotaxanes through imine-based dynamic clipping reactions. In this paper, we report contrasting solvent dependence between these two templated clipping reactions when two different solvents, namely CDCl3 and CD3CN, are used. The solvent dependence is elucidated based on H-1 NMR studies, and structural features are revealed by single crystal X-ray analyses of the respective linear and triply threaded interlocked molecules. We have shown that although both clipping reactions are affected by hydrogen-bonding and aromatic-aromatic interactions in general, the nature of the aromatic-aromatic interactions is quite different, which is responsible for the different solvent response. The BPY-based clipping reaction is driven by electrostatic interactions between aromatic surfaces, while the TPY-based reaction is mainly governed by the solvation/desolvation effect (solvophobic interactions). These findings led us to design a rare solvent switchable system. In competition clipping experiments employing both BPY and TPY as the templates, exclusive formation of the BPY-based linear [2]rotaxane can be achieved in pure CDCl3, while in pure CD3CN, a 6.7 : 1 selectivity is achieved in favor of the TPY-based triply threaded [2]rotaxane. The detailed structural analysis of the two [2] rotaxanes as well as the solvent-dependent selectivity, may encourage more integrated approaches for the design of complex molecular architectures. C1 [Pun, Andrew B.; Klivansky, Liana M.; Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Gagnon, Kevin J.; Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Li, Zhan-Ting] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. RP Pun, AB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd,MS 67R6110, Berkeley, CA 94720 USA. EM ztli@fudan.edu.cn; yliu@lbl.gov RI Foundry, Molecular/G-9968-2014; Liu, yi/A-3384-2008; OI Liu, yi/0000-0002-3954-6102; Pun, Andrew/0000-0002-3052-912X FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This study was performed at the Molecular Foundry and Advanced Light Source, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 94 TC 6 Z9 6 U1 5 U2 13 PU CHINESE CHEMICAL SOC PI TAIPEI PA PO BOX 1-18, NANKANG, TAIPEI 115, TAIWAN SN 2052-4129 J9 ORG CHEM FRONT JI Org. Chem. Front. PY 2014 VL 1 IS 2 BP 167 EP 175 DI 10.1039/c3qo00074e PG 9 WC Chemistry, Organic SC Chemistry GA CV7AF UT WOS:000364423200008 ER PT B AU Wielopolski, L AF Wielopolski, Lucian BE Bandyopadhyay, A TI GEOLOGICAL CARBON SEQUESTRATION: A NEW APPROACH FOR NEAR-SURFACE ASSURANCE MONITORING SO CARBON CAPTURE AND STORAGE: CO2 MANAGEMENT TECHNOLOGIES LA English DT Article; Book Chapter ID CO2 DETECTION TECHNIQUES; TRANSPORT MODELS; SOIL; EMISSIONS; RELEASE C1 Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. RP Wielopolski, L (reprint author), Brookhaven Natl Lab, Dept Environm Sci, Bldg 490, Upton, NY 11973 USA. NR 25 TC 0 Z9 0 U1 0 U2 1 PU CRC PRESS-TAYLOR & FRANCIS GROUP PI BOCA RATON PA 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA BN 978-1-4822-5061-9; 978-1-77188-021-3 PY 2014 BP 105 EP 120 DI 10.3390/ijerph8030818 D2 10.1201/b16845 PG 16 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA BD7HF UT WOS:000363064600005 ER PT B AU Carroll, SA McNab, WW Torres, SC AF Carroll, Susan A. McNab, Walt W. Torres, Sharon C. BE Bandyopadhyay, A TI EXPERIMENTAL STUDY OF CEMENT-SANDSTONE/SHALE-BRINE-CO2 INTERACTIONS SO CARBON CAPTURE AND STORAGE: CO2 MANAGEMENT TECHNOLOGIES LA English DT Article; Book Chapter ID WELL CEMENT; CO2 STORAGE; GEOLOGIC SEQUESTRATION; PORTLAND-CEMENT; CARBON-DIOXIDE; SIMULATION; ALGERIA; BRINE; DEGRADATION; INJECTION C1 [Carroll, Susan A.; McNab, Walt W.; Torres, Sharon C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Carroll, SA (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. NR 39 TC 0 Z9 0 U1 0 U2 0 PU CRC PRESS-TAYLOR & FRANCIS GROUP PI BOCA RATON PA 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA BN 978-1-4822-5061-9; 978-1-77188-021-3 PY 2014 BP 203 EP 235 DI 10.1186/1467-4866-12-9 D2 10.1201/b16845 PG 33 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA BD7HF UT WOS:000363064600008 ER PT J AU Boracchi, G Carrera, D Wohlberg, B AF Boracchi, Giacomo Carrera, Diego Wohlberg, Brendt GP IEEE TI Novelty Detection in Images by Sparse Representations SO 2014 IEEE SYMPOSIUM ON INTELLIGENT EMBEDDED SYSTEMS (IES) LA English DT Proceedings Paper CT IEEE Symposium on Intelligent Embedded Systems (IES) CY DEC 09-12, 2014 CL Orlando, FL SP IEEE, IEEE Computat Inelligence Soc ID SYSTEMS; SIGNALS AB We address the problem of automatically detecting anomalies in images, i. e., patterns that do not conform to those appearing in a reference training set. This is a very important feature for enabling an intelligent system to autonomously check the validity of acquired data, thus performing a preliminary, automatic, diagnosis. We approach this problem in a patch-wise manner, by learning a model to represent patches belonging to a training set of normal images. Here, we consider a model based on sparse representations, and we show that jointly monitoring the sparsity and the reconstruction error of such representation substantially improves the detection performance with respect to other approaches leveraging sparse models. As an illustrative application, we consider the detection of anomalies in scanning electron microscope (SEM) images, which is essential for supervising the production of nanofibrous materials. C1 [Boracchi, Giacomo; Carrera, Diego] Politecn Milan, Dipartimento Elettron Informaz & Bioingn, I-20133 Milan, Italy. [Wohlberg, Brendt] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Boracchi, G (reprint author), Politecn Milan, Dipartimento Elettron Informaz & Bioingn, I-20133 Milan, Italy. EM giacomo.boracchi@polimi.it; diego.carrera@polimi.it; brendt@lanl.gov OI Wohlberg, Brendt/0000-0002-4767-1843 NR 24 TC 3 Z9 3 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA BN 978-1-4799-4485-9 PY 2014 BP 47 EP 54 PG 8 WC Computer Science, Artificial Intelligence; Computer Science, Theory & Methods; Engineering, Electrical & Electronic SC Computer Science; Engineering GA BD8FP UT WOS:000363908600008 ER PT B AU Yu, BB Karr, DG Sirnivas, S AF Yu, Bingbin Karr, Dale G. Sirnivas, Senu GP ASME TI ICE NONSIMULTANEOUS FAILURE, BENDING AND FLOE IMPACT MODELING FOR SIMULATING WIND TURBINE DYNAMICS USING FAST SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 10: POLAR AND ARCTIC SCIENCE AND TECHNOLOGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div ID PART 1 AB Many promising locations for developing offshore wind energy are in cold regions. This type of environment introduces one important technological challenge for offshore wind turbine design: the impact of floating surface ice. Recent developments to add an ice-loading module to the wind turbine computer-aided-engineering tool FAST are described in this paper. These efforts enable FAST, developed and maintained by the National Renewable Energy Laboratory, to simulate the impact of ice on offshore wind turbines. The ice-loading module includes different ice mechanics models that address various ice properties, failure modes, and ice-structure interaction mechanisms. In a previous OMAE symposium paper, models for quasi-static crushing, transient dynamic ice breakage, and random forcing for the ice module were described. In this paper, three new models are presented. One model evaluates the ice-loading effective pressure reduction caused by ice nonsimultaneous failure in discrete local zones across the contact area. The second model generates time-dependent ice forces on conical structures caused by bending failure. The third model is used to simulate large ice floe interaction with wind turbine support systems. This third model describes ice forces that are limited by momentum or splitting failure of ice floes. These models are integrated in the FAST modularization framework and allow for the simulation of coupled ice force, ice floe motion, and wind turbine structure response. This paper also presents example numerical simulation results of wind turbine dynamics using FAST coupled with these three new models. C1 [Yu, Bingbin; Karr, Dale G.] Univ Michigan, Ann Arbor, MI 48105 USA. [Sirnivas, Senu] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yu, BB (reprint author), Univ Michigan, Ann Arbor, MI 48105 USA. EM ybingbin@umich.edu; dgkarr@umich.edu; Senu.Sirnivas@nrel.gov NR 33 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4556-1 PY 2014 AR UNSP V010T07A047 PG 18 WC Engineering, Marine; Engineering, Ocean; Engineering, Mechanical; Geosciences, Multidisciplinary SC Engineering; Geology GA BD7SE UT WOS:000363499200047 ER PT B AU Ahn, CH Dilmore, R Wang, JY AF Ahn, Chong Hyun Dilmore, Robert Wang, John Yilin GP ASME TI MODELING OF HYDRAULIC FRACTURE NETWORK PROPAGATION IN SHALE GAS RESERVOIRS SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 5 LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div ID INTERFACES AB The most effective method for stimulating shale gas reservoirs is horizontal drilling with successful multi-stage hydraulic fracture treatments. Recent fracture diagnostic technologies have shown that complex fracture networks are commonly created in the field. The interaction between preexisting natural fractures and the propagating hydraulic fracture is a critical factor affecting the complex fracture network. However, many existing numerical models simulate only planar hydraulic fractures without considering the pre-existing fractures in the formation. The shale formations already contain a large number of natural fractures, so an accurate fracture propagation model needs to be developed to optimize the fracturing process. In this paper, we first understood the interaction between hydraulic and natural fractures. We then developed a new, coupled numerical model that integrates dynamic fracture propagation, reservoir flow simulation, and the interactions between hydraulic fractures and pre-existing natural fractures. By using the developed model, we conducted parametric studies to quantify the effects of rock toughness, stress anisotropy, and natural fracture spacing on the geometry and conductivities of the hydraulic fracture network. Lastly, we introduced new parmeters Fracture Network Index (FNI) and Width Anistropy (W-ani) which may describe the characteristics of the fracture network in shale gas reservoirs. This new knowledge helps one understand and optimize the stimulation of shale gas reservoirs. C1 [Ahn, Chong Hyun; Wang, John Yilin] Penn State Univ, University Pk, PA 16802 USA. [Dilmore, Robert] US DOE, NETL, Pittsburgh, PA USA. RP Ahn, CH (reprint author), Penn State Univ, University Pk, PA 16802 USA. NR 23 TC 0 Z9 0 U1 0 U2 2 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4545-5 PY 2014 AR UNSP V005T11A021 PG 10 WC Engineering, Ocean; Engineering, Petroleum; Engineering, Mechanical SC Engineering GA BD7RW UT WOS:000363496900065 ER PT B AU Gueydon, S Duarte, T Jonkman, J AF Gueydon, Sebastien Duarte, Tiago Jonkman, Jason GP ASME TI COMPARISON OF SECOND-ORDER LOADS ON A SEMISUBMERSIBLE FLOATING WIND TURBINE SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9A: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB As offshore wind projects move to deeper waters, floating platforms become the most feasible solution for supporting the turbines. The oil and gas industry has gained experience with floating platforms that can be applied to offshore wind projects. This paper focuses on the analysis of second-order wave loading on semisubmersible platforms. Semisubmersibles, which are being chosen for different floating offshore wind concepts, are particularly prone to slow-drift motions. The slack catenary moorings usually result in large natural periods for surge and sway motions (more than 100 s), which are in the range of the second-order difference-frequency excitation force. Modeling these complex structures requires coupled design codes. Codes have been developed that include turbine aerodynamics, hydrodynamic forces on the platform, restoring forces from the mooring lines, flexibility of the turbine, and the influence of the turbine control system. In this paper two different codes are employed: FAST, which was developed by the National Renewable Energy Laboratory, and aNySIM, which was developed by the Maritime Research Institute Netherlands. The hydrodynamic loads are based on potential-flow theory, up to the second order. Hydrodynamic coefficients for wave excitation, radiation, and hydrostatic forces are obtained with two different panel codes, WAMIT (developed by the Massachusetts Institute of Technology) and DIFFRAC (developed by MARIN). The semisubmersible platform, developed for the International Energy Agency Wind Task 30 Offshore Code Comparison Collaboration Continuation project is used as a reference platform. Irregular waves are used to compare the behavior of this platform under slow-drift excitation loads. The results from this paper highlight the effects of these loads on semisubmersible-type platforms, which represent a promising solution for the commercial development of the offshore deepwater wind resource. C1 [Gueydon, Sebastien] MARIN, Wageningen, Netherlands. [Duarte, Tiago] Inst Super Tecn, EDP Inovacao, Lisbon, Portugal. [Jonkman, Jason] Natl Renewable Energy Lab, Golden, CO USA. RP Gueydon, S (reprint author), MARIN, Wageningen, Netherlands. NR 10 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4553-0 PY 2014 AR UNSP V09AT09A024 PG 12 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SC UT WOS:000363499000024 ER PT B AU Masciola, M Jonkman, J Robertson, A AF Masciola, Marco Jonkman, Jason Robertson, Amy GP ASME TI EXTENDING THE CAPABILITIES OF THE MOORING ANALYSIS PROGRAM: A SURVEY OF DYNAMIC MOORING LINE THEORIES FOR INTEGRATION INTO FAST SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9A: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div ID STEADY-STATE ANALYSIS; FINITE-ELEMENT; NUMERICAL-SIMULATION; UNDERWATER CABLES; SYSTEM; MODEL; FORMULATION; ALGORITHM; RODS AB Techniques to model dynamic mooring lines take various forms. The most widely used models include a heuristic representation of the physics (such as a lumped-mass system), a finite-element analysis discretization of the lines (discretized in space), or a finite-difference model (which is discretized in both space and time). In this paper, the authors explore the features of the various models, weigh the advantages of each, and propose a plan for implementing one dynamic mooring line model into the open-source Mooring Analysis Program (MAP). MAP is currently used as a module for the FAST offshore wind turbine computer-aided engineering (CAE) tool to model mooring systems quasi-statically, although dynamic mooring capabilities are desired. Based on the exploration in this paper, the lumped-mass representation is selected for implementation in MAP based on its simplicity, low computational cost, and ability to provide physics similar to those captured by higher-order models. To begin, the underlying theories defining the three classes of dynamic mooring line models are identified and explored. This leads to insight into the capabilities of each representation. These capabilities are weighed against the current needs of the FAST wind turbine CAE tool, to which MAP will be coupled. Based on the assessment, a plan for integrating the dynamic mooring line theory into the current MAP structure is developed. Common problems arising from the determination of the model static equilibrium and known issues with numerical stability are addressed. Because MAP is a module that FAST can call, a plan consistent with the FAST modularization framework principles is described. Adding dynamic mooring line capabilities extends the features in MAP and also allows uncoupled analysis to be performed through MAP's native Python bindings. C1 [Masciola, Marco; Jonkman, Jason; Robertson, Amy] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Masciola, M (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. NR 63 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4553-0 PY 2014 AR UNSP V09AT09A032 PG 13 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SC UT WOS:000363499000032 ER PT B AU Benitz, MA Schmidt, DP Lackner, MA Stewart, GM Jonkman, J Robertson, A AF Benitz, Maija A. Schmidt, David P. Lackner, Matthew A. Stewart, Gordon M. Jonkman, Jason Robertson, Amy GP ASME TI COMPARISON OF HYDRODYNAMIC LOAD PREDICTIONS BETWEEN REDUCED ORDER ENGINEERING MODELS AND COMPUTATIONAL FLUID DYNAMICS FOR THE OC4-DEEPCWIND SEMI-SUBMERSIBLE SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB Hydrodynamic loads on the platforms of floating offshore wind turbines are often predicted with computer-aided engineering tools that employ Morison's equation and/or potential-flow theory. This work compares results from one such tool, FAST, the National Renewable Energy Laboratory's wind turbine computer-aided engineering tool, and the high-fidelity computational fluid dynamics (CFD) package, OpenFOAM, for the OC4-DeepCwind semi-submersible analyzed in the International Energy Agency Wind Task 30 project. Load predictions from HydroDyn, the offshore hydrodynamics module of FAST, are compared with results from OpenFOAM. HydroDyn uses a combination of Morison's equation and potential-flow theory to predict the hydrodynamic forces on the structure, at a small computational cost compared to CFD. The implications of the assumptions in HydroDyn are evaluated based on this code-to-code comparison. C1 [Benitz, Maija A.; Schmidt, David P.; Lackner, Matthew A.; Stewart, Gordon M.] Univ Massachusetts, Dept Mech & Ind Engn, Amherst, MA 01003 USA. [Jonkman, Jason; Robertson, Amy] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Benitz, MA (reprint author), Univ Massachusetts, Dept Mech & Ind Engn, 160 Governors Dr, Amherst, MA 01003 USA. EM mbenitz@engin.umass.edu NR 20 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A006 PG 11 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100006 ER PT B AU Duarte, T Gueydon, S Jonkman, J Sarmento, A AF Duarte, Tiago Gueydon, Sebastien Jonkman, Jason Sarmento, Antonio GP ASME TI Computation of Wave Loads under Multidirectional Sea States for Floating Offshore Wind Turbines SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div DE Multidirectional Waves; Floating Wind Turbine; Synthesis of Multidirectional Seas AB This paper focuses on the analysis of a floating wind turbine under multidirectional wave loading. Special attention is given to the different methods used to synthesize the multidirectional sea state. This analysis includes the double-sum and single-sum methods, as well as an equal-energy discretization of the directional spectrum. These three methods are compared in detail, including the ergodicity of the solution obtained. From the analysis, the equal-energy method proved to be the most computationally efficient while still retaining the ergodicity of the solution. This method was chosen to be implemented in the numerical code FAST. Preliminary results on the influence of these wave loads on a floating wind turbine showed significant additional roll and sway motion of the platform. C1 [Duarte, Tiago] EDP Inovacao, Lisbon, Portugal. [Gueydon, Sebastien] MARIN, Wageningen, Netherlands. [Jonkman, Jason] Natl Renewable Energy Lab, Golden, CO USA. [Sarmento, Antonio] Univ Lisbon, IST, P-1699 Lisbon, Portugal. RP Duarte, T (reprint author), EDP Inovacao, Lisbon, Portugal. NR 14 TC 0 Z9 0 U1 1 U2 3 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A023 PG 8 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100023 ER PT B AU Fleming, PA Pineda, I Rossetti, M Wright, AD Arora, D AF Fleming, Paul A. Pineda, Isaac Rossetti, Michele Wright, Alan D. Arora, Dhiraj GP ASME TI EVALUATING METHODS FOR CONTROL OF AN OFFSHORE FLOATING TURBINE SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div ID WIND TURBINES AB Developing wind turbines on floating offshore platforms is a topic of growing interest. By using a floating platform, wind turbines can be located in areas with good resources and near to major load centers. However, there can be technical challenges with this approach, and one is the observed unstable interaction between the pitch speed controller and the platform motions. In this paper, we consider several controls-based methods for resolving this issue for a commercial-scale turbine on a tension-leg platform. The design of each method is reviewed and each is shown to resolve the unstable interaction. The methods are then compared through load suite analysis to assess the strengths and weaknesses of each approach. Finally, we present proposals for refining and combining these methods and further approaches for performance improvement that could be considered. C1 [Fleming, Paul A.; Wright, Alan D.] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO 80305 USA. [Pineda, Isaac; Rossetti, Michele] Alstom Wind, Barcelona, Spain. [Arora, Dhiraj] ALSTOM Power Inc, Richmond, VA USA. RP Fleming, PA (reprint author), Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO 80305 USA. EM paul.fleming@nrel.gov; isaac.pineda-amo@power.alstom.com; michele.rossetti@power.alstom.com; alan.wright@nrel.gov; dhiraj.arora@power.alstom.com NR 15 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A019 PG 9 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100019 ER PT B AU Fowler, MJ Owens, B Bull, D Goupee, AJ Hurtado, J Griffith, DT Alves, M AF Fowler, Matthew J. Owens, Brian Bull, Diana Goupee, Andrew J. Hurtado, John Griffith, D. Todd Alves, Marco GP ASME TI Hydrodynamic Module Coupling in the Offshore Wind Energy Simulation (OWENS) Tookit SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB When considering the future of offshore wind energy, developing cost effective methods of harnessing the offshore wind resource represents a significant challenge which must be overcome to make offshore wind a viable option. As the majority of the capital investment in offshore wind is in the form of infrastructure and operation and maintenance costs, reducing these expenditures could greatly reduce the cost of energy (COE) for an offshore wind project. Sandia National Laboratory and its partners (TU Delft, University of Maine, Iowa State, and TPI Composites) believe that vertical axis wind turbines (VAWTs) offer multiple advantages over other rotor configurations considering this new COE breakdown. The unique arrangement of a VAWT allows the heavy generator and related components to be located at the base of the tower as opposed to the top, as is typical of a horizontal axis wind turbine (HAWT). This configuration lowers the topside CG which reduces the platform stability requirements, leading to smaller and cheaper platforms. Additionally this locates high maintenance systems close to the ocean surface thus increasing maintainability. To support this project and the general wind research community, the Offshore Wind ENergy Simulation (OWENS) toolkit is being developed in conjunction with Texas A&M as an open source, modular aero-elastic analysis code with the capability to analyze floating VAWTS. The OWENS toolkit aims to establish a robust and flexible -finite element framework and VAWT mesh generation utility, coupled with a modular interface that allows users to integrate easily with existing codes, such as aerodynamic and hydrodynamic codes. Current efforts to include a hydrodynamic module are focused on coupling WavEC2Wire with OWENS. WavEC2Wire is a wave-to-wire numerical model developed by Marco Alves at the Insituto Superior Tecnico for the analysis of wave energy converter devices. It has been adapted from its original form and restructured for use as a hydrodynamic module capable of providing OWENS with necessary floating platform dynamics. Hence, WavEC2Wire functions as a rigid-body solver designed to calculate the platform motion due to wave loads, moorings, and the influence of the attached VAWT and tower. This paper presents the WavEC2Wire module and details the OWENS coupling method. Additionally, planned improvements in the WavEC2Wire module as well as future development in OWENS are presented. C1 [Fowler, Matthew J.; Goupee, Andrew J.] Univ Maine, Orono, ME 04469 USA. [Owens, Brian; Bull, Diana; Griffith, D. Todd] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Hurtado, John] Texas A&M Univ, College Stn, TX USA. [Alves, Marco] Wave Energy Ctr, Lisbon, Portugal. RP Fowler, MJ (reprint author), Univ Maine, Orono, ME 04469 USA. NR 15 TC 0 Z9 0 U1 1 U2 1 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A027 PG 10 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100027 ER PT B AU Lawson, M Yu, YH Nelessen, A Ruehl, K Michelen, C AF Lawson, Michael Yu, Yi-Hsiang Nelessen, Adam Ruehl, Kelley Michelen, Carlos GP ASME TI IMPLEMENTING NONLINEAR BUOYANCY AND EXCITATION FORCES IN THE WEC-SIM WAVE ENERGY CONVERTER MODELING TOOL SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB Wave energy converters (WECs) are commonly designed and analyzed using numerical models that combine multibody dynamics with hydrodynamic models based on the Cummins equation and linearized hydrodynamic coefficients. These modeling methods are attractive design tools because they are computationally inexpensive and do not require the use of high-performance computing resources necessitated by high-fidelity methods, such as Navier-Stokes computational fluid dynamics. Modeling hydrodynamics using linear coefficients assumes that the device undergoes small motions and that the wetted surface area of the devices is approximately constant. WEC devices, however, are typically designed to undergo large motions to maximize power extraction, calling into question the validity of assuming that linear hydrodynamic models accurately capture the relevant fluid-structure interactions. In this paper, we study how calculating buoyancy and Froude-Krylov forces from the instantaneous position of a WEC device changes WEC simulation results compared to simulations that use linear hydrodynamic coefficients. First, we describe the WEC-Sim tool used to perform simulations and how the ability to model instantaneous forces was incorporated into WEC-Sim. We then use a simplified one-body WEC device to validate the model and to demonstrate how accounting for these instantaneously calculated forces affects the accuracy of simulation results, such as device motions, hydrodynamic forces, and power generation. Other aspects of WEC-Sim code development and verification are presented in a companion paper [1] that is also being presented at OMAE2014. C1 [Lawson, Michael; Yu, Yi-Hsiang] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Nelessen, Adam] Georgia Tech, Atlanta, GA USA. [Ruehl, Kelley; Michelen, Carlos] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Lawson, M (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM michael.lawson@nrel.gov NR 6 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A043 PG 6 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100043 ER PT B AU Robertson, A Jonkman, J Vorpahl, F Popko, W Qvist, J Froyd, L Chen, XH Azcona, J Uzunoglu, E Soares, CG Luan, CY Huang, YT Fu, PC Yde, A Larsen, T Nichols, J Buils, R Lei, L Nygaard, TA Manolas, D Heege, A Vatne, SR Ormberg, H Duarte, T Godreau, C Hansen, HF Nielsen, AW Riber, H Le Cunff, C Beyer, F Yamaguchi, A Jung, KJ Shin, H Shi, W Park, H Alves, M Guerinel, M AF Robertson, Amy Jonkman, Jason Vorpahl, Fabian Popko, Wojciech Qvist, Jacob Froyd, Lars Chen, Xiaohong Azcona, Jose Uzunoglu, Emre Soares, Carlos Guedes Luan, Chenyu Huang Yutong Fu Pengcheng Yde, Anders Larsen, Torben Nichols, James Buils, Ricard Lei, Liu Nygaard, Tor Anders Manolas, Dimitris Heege, Andreas Vatne, Sigrid Ringdalen Ormberg, Harald Duarte, Tiago Godreau, Cyril Hansen, Hans Fabricius Nielsen, Anders Wedel Riber, Hans Le Cunff, Cedric Beyer, Friedemann Yamaguchi, Atsushi Jung, Kwang Jin Shin, Hyunkyoung Shi, Wei Park, Hyunchul Alves, Marco Guerinel, Matthieu GP ASME TI OFFSHORE CODE COMPARISON COLLABORATION CONTINUATION WITHIN IEA WIND TASK 30: PHASE II RESULTS REGARDING A FLOATING SEMISUBMERSIBLE WIND SYSTEM SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB Offshore wind turbines are designed and analyzed using comprehensive simulation tools (or codes) that account for the coupled dynamics of the wind inflow, aerodynamics, elasticity, and controls of the turbine, along with the incident waves, sea current, hydrodynamics, mooring dynamics, and foundation dynamics of the support structure. This paper describes the latest findings of the code-to-code verification activities of the Offshore Code Comparison Collaboration Continuation project, which operates under the International Energy Agency Wind Task 30. In the latest phase of the project, participants used an assortment of simulation codes to model the coupled dynamic response of a 5-MW wind turbine installed on a floating semisubmersible in 200 m of water. Code predictions were compared from load case simulations selected to test different model features. The comparisons have resulted in a greater understanding of offshore floating wind turbine dynamics and modeling techniques, and better knowledge of the validity of various approximations. The lessons learned from this exercise have improved the participants' codes, thus improving the standard of offshore wind turbine modeling. C1 [Robertson, Amy; Jonkman, Jason] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Vorpahl, Fabian; Popko, Wojciech] Fraunhofer Inst Wind Energy & Energy Syst Technol, Bremerhaven, Germany. [Qvist, Jacob; Froyd, Lars] 4subsea, Hvalstad, Norway. [Chen, Xiaohong] Amer Bur Shipping, Houston, TX USA. [Azcona, Jose] Natl Renewable Energy Ctr, Navarra, Spain. [Uzunoglu, Emre; Soares, Carlos Guedes] Univ Lisbon, CENTEC, Inst Super Tecn, Lisbon, Portugal. [Luan, Chenyu] CeSOS, Trondheim, Norway. [Luan, Chenyu] NOWITECH, Trondheim, Norway. [Huang Yutong; Fu Pengcheng] China Gen Certificat Ctr, Beijing, Peoples R China. [Yde, Anders; Larsen, Torben] Tech Univ Denmark, Roskilde, Denmark. [Nichols, James; Buils, Ricard] DNV GL, Hovik, Norway. [Lei, Liu] Goldwind, Beijing, Peoples R China. [Nygaard, Tor Anders] Inst Energy Technol, N-2007 Kjeller, Norway. [Manolas, Dimitris] Natl Tech Univ Athens, Athens, Greece. [Heege, Andreas] SAMTECH Sa, Barcelona, Spain. [Vatne, Sigrid Ringdalen; Ormberg, Harald] MARINTEK, Trondheim, Norway. [Duarte, Tiago; Godreau, Cyril] Univ Lisbon, Inst Super Tecn, P-1699 Lisbon, Portugal. [Hansen, Hans Fabricius; Nielsen, Anders Wedel] DHI, Horsholm, Denmark. [Riber, Hans; Le Cunff, Cedric] PRINCIPIA NORTH, Svendborg, Denmark. [Beyer, Friedemann] Univ Stuttgart, D-70174 Stuttgart, Germany. [Yamaguchi, Atsushi] Univ Tokyo, Tokyo, Japan. [Jung, Kwang Jin; Shin, Hyunkyoung] Univ Ulsan, Ulsan 680749, South Korea. [Shi, Wei; Park, Hyunchul] POSTECH, Pohang, South Korea. [Alves, Marco; Guerinel, Matthieu] WavEC Offshore Renewables, Lisbon, Portugal. RP Robertson, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. RI Guedes Soares, Carlos/H-1140-2012; Shi, Wei/H-8019-2015 OI Guedes Soares, Carlos/0000-0002-8570-4263; Shi, Wei/0000-0002-6312-0494 NR 5 TC 0 Z9 0 U1 0 U2 4 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A012 PG 15 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100012 ER PT B AU Ruehl, K Michelen, C Kanner, S Lawson, M Yu, YH AF Ruehl, Kelley Michelen, Carlos Kanner, Samuel Lawson, Michael Yu, Yi-Hsiang GP ASME TI PRELIMINARY VERIFICATION AND VALIDATION OF WEC-SIM, AN OPEN-SOURCE WAVE ENERGY CONVERTER DESIGN TOOL SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div AB To promote and support the wave energy industry, a wave energy converter (WEC) design tool, WEC-Sim, is being developed by Sandia National Laboratories and the National Renewable Energy Laboratory. In this paper, the WEC-Sim code is used to model a point absorber WEC designed by the U.S. Department of Energy's reference model project. Preliminary verification was performed by comparing results of the WEC-Sim simulation through a code-to-code comparison, utilizing the commercial codes ANSYS-AQWA, WaveDyn, and OrcaFlex. A preliminary validation of the code was also performed by comparing WEC-Sim simulation results to experimental wave tank tests. C1 [Ruehl, Kelley; Michelen, Carlos] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kanner, Samuel] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Lawson, Michael; Yu, Yi-Hsiang] Natl Renewable Energy Lab, Golden, CO USA. RP Ruehl, K (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. NR 19 TC 0 Z9 0 U1 1 U2 1 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A040 PG 7 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100040 ER PT B AU Yu, YH Li, Y Hallett, K Hotimsky, C AF Yu, Yi-Hsiang Li, Ye Hallett, Kathleen Hotimsky, Chad GP ASME TI DESIGN AND ANALYSIS FOR A FLOATING OSCILLATING SURGE WAVE ENERGY CONVERTER SO 33RD INTERNATIONAL CONFERENCE ON OCEAN, OFFSHORE AND ARCTIC ENGINEERING, 2014, VOL 9B: OCEAN RENEWABLE ENERGY LA English DT Proceedings Paper CT 33rd ASME International Conference on Ocean, Offshore and Arctic Engineering CY JUN 08-13, 2014 CL San Francisco, CA SP ASME, Ocean, Offshore & Arct Engn Div DE Wave energy; oscillating surge device; cost of energy AB This paper presents a recent study on the design and analysis of an oscillating surge wave energy converter (OSWEC). A successful wave energy conversion design requires balance between the design performance and cost. The cost of energy is often used as the metric to judge the design of the wave energy conversion (WEC) system, which is often determined based on the device's power performance; the cost of manufacturing, deployment, operation, and maintenance; and environmental compliance. The objective of this study is to demonstrate the importance of a cost-driven design strategy and how it can affect a WEC design. A set of three oscillating surge wave energy converter designs was analyzed and used as examples. The power generation performance of the design was modeled using a time-domain numerical simulation tool, and the mass properties of the design were determined based on a simple structure analysis. The results of those power performance simulations, the structure analysis, and a simple economic assessment were then used to determine the cost-efficiency of selected OSWEC designs. Finally, we present a discussion on the environmental barrier, integrated design strategy, and the key areas that need further investigation. C1 [Yu, Yi-Hsiang; Li, Ye; Hallett, Kathleen; Hotimsky, Chad] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yu, YH (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Yi-Hsiang.Yu@nrel.gov; Ye.Li@nrel.gov; Kathleen.Hallett@nrel.gov; Chad.Hotimsky@nrel.gov NR 19 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-4554-7 PY 2014 AR UNSP V09BT09A048 PG 10 WC Energy & Fuels; Engineering, Ocean; Engineering, Mechanical SC Energy & Fuels; Engineering GA BD7SD UT WOS:000363499100048 ER PT S AU Jeon, JH Chang, JT Pham, AV AF Jeon, Jae H. Chang, John T. Anh-Vu Pham GP IEEE TI Band-Notched UWB Equiangular Spiral Antenna SO 2014 IEEE ANTENNAS AND PROPAGATION SOCIETY INTERNATIONAL SYMPOSIUM (APSURSI) SE IEEE Antennas and Propagation Society International Symposium LA English DT Proceedings Paper CT IEEE Antennas-and-Propagation-Society International Symposium (APSURSI) CY JUL 06-11, 2014 CL Memphis, TN SP Inst Elect Elect Engineers, Inst Elect Elect Engineers Antennas & Propagat Soc AB A band-notched ultra-wideband equiangular spiral antenna is presented. With the spiral antenna on the top layer, bottom side is used for a secondary resonant structure to create a notch filter response. VSWR of 2:1 is achieved for the FCC UWB band, which is 3.1 to 10.6 GHz. Notch response is created over the IEEE 802.11a band, 5.15 to 5.85 GHz, VSWR reaching 12:1 at the center of the band at 5.5 GHz. Suppression of radiation in this band is evident in its gain profile over frequency and in current density plot around the resonant structure as well. C1 [Jeon, Jae H.; Chang, John T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Anh-Vu Pham] Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA. RP Jeon, JH (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM jeon2@llnl.gov; chang16@llnl.gov; pham@ece.ucdavis.edu NR 3 TC 1 Z9 1 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 1522-3965 BN 978-1-4799-3540-6 J9 IEEE ANTENNAS PROP PY 2014 BP 1323 EP 1324 PG 2 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA BD5LF UT WOS:000361554401220 ER PT S AU Yan, S Wang, CF Kotuiski, J Jin, JM AF Yan, Su Wang, Chao-Fu Kotuiski, Joseph Jin, Jian-Ming GP IEEE TI Time-Domain Finite Element Analysis of Ferromagnetic Hysteresis in Three Dimensions SO 2014 IEEE ANTENNAS AND PROPAGATION SOCIETY INTERNATIONAL SYMPOSIUM (APSURSI) SE IEEE Antennas and Propagation Society International Symposium LA English DT Proceedings Paper CT IEEE Antennas-and-Propagation-Society International Symposium (APSURSI) CY JUL 06-11, 2014 CL Memphis, TN SP Inst Elect Elect Engineers, Inst Elect Elect Engineers Antennas & Propagat Soc AB Nonlinear ferromagnetic hysteresis analysis is conducted using the three-dimensional time-domain finite element method combined with the inverse Jiles-Atherton (JA) vector hysteresis model. The second-order wave equation is formulated through the magnetic vector potential in the time domain. To incorporate the nonlinear JA model, the time-domain wave equation is discretized and solved by employing the polarization method and the Newmark-beta scheme. The capability of the proposed method is demonstrated by simulating the physical process of demagnetization, and the magnetic remanence in the ferromagnetic material is predicted. C1 [Yan, Su; Jin, Jian-Ming] Univ Illinois, Urbana, IL 61801 USA. [Yan, Su] Univ Elect Sci & Technol China, Chengdu 610054, Sichuan, Peoples R China. [Wang, Chao-Fu] Natl Univ Singapore, Singapore 117411, Singapore. [Kotuiski, Joseph] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Yan, S (reprint author), Univ Illinois, Urbana, IL 61801 USA. EM suyan@illinois.edu; cfwang@nus.edu.sg; jdkotul@sandia.gov; j-jin1@illinois.edu RI Yan, Su/G-8207-2016 OI Yan, Su/0000-0002-7376-3493 NR 6 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 1522-3965 BN 978-1-4799-3540-6 J9 IEEE ANTENNAS PROP PY 2014 BP 1889 EP 1890 PG 2 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA BD5LF UT WOS:000361554401494 ER PT S AU Yan, S Kotulski, J Wang, CF Jin, JM AF Yan, Su Kotulski, Joseph Wang, Chao-Fu Jin, Jian-Ming GP IEEE TI A Nonuniform Time-Stepping Scheme for Nonlinear Electromagnetic Analysis Using Time-Domain Finite Element Method SO 2014 IEEE ANTENNAS AND PROPAGATION SOCIETY INTERNATIONAL SYMPOSIUM (APSURSI) SE IEEE Antennas and Propagation Society International Symposium LA English DT Proceedings Paper CT IEEE Antennas-and-Propagation-Society International Symposium (APSURSI) CY JUL 06-11, 2014 CL Memphis, TN SP Inst Elect Elect Engineers, Inst Elect Elect Engineers Antennas & Propagat Soc AB In the time-domain finite element analysis of electromagnetic problems, the spatial discretization of the wave equation results in a second-order ordinary differential equation, which is usually discretized in the time domain with the Newmark-(3 method due to its second-order accuracy and unconditional stability. However, the commonly used uniform time-stepping scheme is not always the optimal choice. In this paper, a nonuniform time-stepping scheme is derived using the weighted residual approach. With the proposed method, the time-stepping sizes can be chosen according to the variation of the externally applied signal, which reduces the total number of time steps significantly. The nonlinear electromagnetic problem is analyzed with the proposed method, and its accuracy and efficiency are investigated and compared with the traditional uniform time-stepping scheme. C1 [Yan, Su; Jin, Jian-Ming] Univ Illinois, Urbana, IL 61801 USA. [Yan, Su] Univ Elect Sci & Technol China, Chengdu 610054, Sichuan, Peoples R China. [Kotulski, Joseph] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Wang, Chao-Fu] Natl Univ Singapore, Singapore 117411, Singapore. RP Yan, S (reprint author), Univ Illinois, Urbana, IL 61801 USA. EM suyan@illinois.edu; jdkotul@sandia.gov; cfwang@nus.edu.sg; j-jin1@illinois.edu RI Yan, Su/G-8207-2016 OI Yan, Su/0000-0002-7376-3493 NR 3 TC 0 Z9 0 U1 0 U2 0 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 1522-3965 BN 978-1-4799-3540-6 J9 IEEE ANTENNAS PROP PY 2014 BP 1895 EP 1896 PG 2 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA BD5LF UT WOS:000361554401497 ER PT S AU Hughey, S Shanker, B Baczewski, A AF Hughey, S. Shanker, B. Baczewski, A. GP IEEE TI Formulation of the Hardy Space Method in a Discontinuous Galerkin Framework SO 2014 IEEE ANTENNAS AND PROPAGATION SOCIETY INTERNATIONAL SYMPOSIUM (APSURSI) SE IEEE Antennas and Propagation Society International Symposium LA English DT Proceedings Paper CT IEEE Antennas-and-Propagation-Society International Symposium (APSURSI) CY JUL 06-11, 2014 CL Memphis, TN SP Inst Elect Elect Engineers, Inst Elect Elect Engineers Antennas & Propagat Soc ID INFINITE ELEMENTS AB Local transparent boundary conditions (TBCs) based upon the pole condition have shown a great deal of promise in recent years. Only recently has the pole condition been applied to the Maxwell Equations with the aid of vector Hardy space infinite elements [1]. In this work, we describe a variation on the conformal Finite Element formulation presented in [1] within an interior penalty Discontinuous Galerkin (DG) framework. Our primary reasons for doing so are the use of nonconformal meshing at the interior/exterior boundary and the use of locally-enriched function spaces to include desirable physics in numerical solutions. C1 [Hughey, S.; Shanker, B.] Michigan State Univ, Dept Elect & Comp Engn, E Lansing, MI 48825 USA. [Baczewski, A.] Sandia Natl Labs, Multiscale Sci, Albuquerque, NM 87185 USA. RP Hughey, S (reprint author), Michigan State Univ, Dept Elect & Comp Engn, E Lansing, MI 48825 USA. NR 3 TC 0 Z9 0 U1 0 U2 1 PU IEEE PI NEW YORK PA 345 E 47TH ST, NEW YORK, NY 10017 USA SN 1522-3965 BN 978-1-4799-3540-6 J9 IEEE ANTENNAS PROP PY 2014 BP 2244 EP 2245 PG 2 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA BD5LF UT WOS:000361554402164 ER PT S AU Walla, PJ Holleboom, CP Fleming, GR AF Walla, Peter Jomo Holleboom, Christoph-Peter Fleming, Graham R. BE DemmigAdams, B Garab, G Adams, W Govindjee TI Electronic Carotenoid-Chlorophyll Interactions Regulating Photosynthetic Light Harvesting of Higher Plants and Green Algae SO NON-PHOTOCHEMICAL QUENCHING AND ENERGY DISSIPATION IN PLANTS, ALGAE AND CYANOBACTERIA SE Advances in Photosynthesis and Respiration LA English DT Article; Book Chapter ID PHOTOPROTECTIVE ENERGY-DISSIPATION; TIME-RESOLVED FLUORESCENCE; EXCITED SINGLET-STATES; CHARGE-TRANSFER STATE; S-1 STATE; 2-PHOTON EXCITATION; PHOTOSYSTEM-II; COMPLEX-II; EXCITONIC INTERACTIONS; CATION FORMATION AB Electronic interactions between chlorophylls (Chl) and carotenoids (Car) play a major role in the regulation of photosynthetic light harvesting of higher plants and green algae. In this contribution, we discuss different electronic regulation models that are based on various Chl-Car interactions, leading to switching between efficient light harvesting and thermal dissipation of excess energy. Most regulation models are based on three types of electronic Chl-Car interactions: direct Chl -> Car S-1 energy transfer, quenching by Car radical cations and bidirectional quenching processes. We will give an overview of the observations that have been made in our as well as other laboratories supporting one or the other model and discuss possible scenarios that may provide a unified picture considering all three types of regulation models. C1 [Walla, Peter Jomo] Max Planck Inst Biophys Chem, Biomol Spect & Single Mol Detect Grp, D-37077 Gottingen, Germany. [Walla, Peter Jomo; Holleboom, Christoph-Peter] Tech Univ Carolo Wilhelmina Braunschweig, Inst Phys & Theoret Chem, Dept Biophys Chem, D-38106 Braunschweig, Germany. [Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Walla, PJ (reprint author), Max Planck Inst Biophys Chem, Biomol Spect & Single Mol Detect Grp, D-37077 Gottingen, Germany. EM pwalla@gwdg.de; fleming@cchem.berkeley.edu NR 56 TC 3 Z9 3 U1 0 U2 3 PU SPRINGER PI DORDRECHT PA PO BOX 17, 3300 AA DORDRECHT, NETHERLANDS SN 1572-0233 BN 978-94-017-9032-1; 978-94-017-9031-4 J9 ADV PHOTOSYNTH RESP JI Adv. Photo. Respirat. PY 2014 VL 40 BP 229 EP 243 DI 10.1007/978-94-017-9032-1_9 D2 10.1007/978-94-017-9032-1 PG 15 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA BD7IC UT WOS:000363120600010 ER PT S AU Brooks, MD Jansson, S Niyogi, KK AF Brooks, Matthew D. Jansson, Stefan Niyogi, Krishna K. BE DemmigAdams, B Garab, G Adams, W Govindjee TI PsbS-Dependent Non-Photochemical Quenching SO NON-PHOTOCHEMICAL QUENCHING AND ENERGY DISSIPATION IN PLANTS, ALGAE AND CYANOBACTERIA SE Advances in Photosynthesis and Respiration LA English DT Article; Book Chapter ID LIGHT-HARVESTING COMPLEX; PHOTOPROTECTIVE ENERGY-DISSIPATION; PHOTOSYSTEM-II ANTENNA; ABSORBED EXCITATION-ENERGY; XANTHOPHYLL-CYCLE ACTIVITY; HIGHER-PLANT CHLOROPLASTS; PIGMENT-BINDING PROTEIN; CHARGE-TRANSFER STATE; 22 KDA PROTEIN; DELTA-PH AB Much of the research on the thermal dissipation of excess absorbed light, measured as non-photochemical quenching (NPQ) of chlorophyll fluorescence, has been focused on a major, rapidly induced and rapidly reversible component of fluorescence quenching termed energy-dependent quenching, feedback de-excitation, or qE. A breakthrough in this field came with the discovery of the involvement of the photosystem II subunit S (PsbS) protein, a thylakoid membrane protein required for qE induction and relaxation. In this chapter, we discuss the history of how PsbS was first identified as a photosystem II subunit, the genetic characterization that defined its important role in qE, and the biochemical work describing how PsbS might regulate photosynthetic light harvesting. We emphasize how mutants affecting PsbS (i.e., npq4) have been invaluable tools in defining structural and spectroscopic changes associated with qE, and how these mutants have contributed to our current understanding of the physiological role of the thermal dissipation process accompanied by non-photochemical fluorescence quenching. C1 [Brooks, Matthew D.; Niyogi, Krishna K.] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Brooks, Matthew D.; Niyogi, Krishna K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Jansson, Stefan] Umea Univ, Dept Plant Physiol, Umea Plant Sci Ctr, S-90187 Umea, Sweden. RP Niyogi, KK (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM niyogi@berkeley.edu NR 119 TC 4 Z9 4 U1 1 U2 3 PU SPRINGER PI DORDRECHT PA PO BOX 17, 3300 AA DORDRECHT, NETHERLANDS SN 1572-0233 BN 978-94-017-9032-1; 978-94-017-9031-4 J9 ADV PHOTOSYNTH RESP JI Adv. Photo. Respirat. PY 2014 VL 40 BP 297 EP 314 DI 10.1007/978-94-017-9032-1_13 D2 10.1007/978-94-017-9032-1 PG 18 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA BD7IC UT WOS:000363120600014 ER PT S AU Strand, DD Kramer, DM AF Strand, Deserah D. Kramer, David M. BE DemmigAdams, B Garab, G Adams, W Govindjee TI Control of Non-Photochemical Exciton Quenching by the Proton Circuit of Photosynthesis SO NON-PHOTOCHEMICAL QUENCHING AND ENERGY DISSIPATION IN PLANTS, ALGAE AND CYANOBACTERIA SE Advances in Photosynthesis and Respiration LA English DT Article; Book Chapter ID CYCLIC ELECTRON FLOW; CHLOROPLAST ATP SYNTHASE; WATER-WATER CYCLE; PLASTID NDH GENES; EXCESS EXCITATION-ENERGY; COUPLING FACTOR ACTIVITY; RESPIRATORY COMPLEX I; TERMINAL OXIDASE PTOX; PHOTOSYSTEM-I; CHLAMYDOMONAS-REINHARDTII AB This chapter discusses our current understanding of the chloroplast proton circuit, i.e., those reactions that involve the storage and utilization of light energy in the transfer of protons, and its importance for regulating photosynthetic light-capture/electron-transfer reactions. The photosynthetic machinery of plants is finely tuned to balance the needs for efficient light capture with an avoidance of photodamage by regulating the capture of light energy, via thermal dissipation of excess excitation energy (assessed from non-photochemical quenching, NPQ, of chlorophyll fluorescence) by regulating light-driven electron transfer processes. In addition to driving ATP synthesis at the chloroplast ATP synthase, the thylakoid electrochemical gradient of protons or proton-motive force (pmf) plays a central role in regulating NPQ. The trans-thylakoid proton concentration gradient (Delta pH) component of pmf triggers the "energy-dependent", or qE component of NPQ, which protects photosystem II from photodamage and regulates electron transfer through the cytochrome b(6)f complex, thereby preventing damage to photosystem I. The extent and mode of storage in Delta pH and Delta psi of pmf are regulated by several processes that respond to the metabolic, or physiological, state of the organism. The extent of pmf is determined by proton influx (via linear and alternative electron flows) into the thylakoid lumen, and proton efflux through the chloroplast ATP synthase. Both processes are modulated by, or responsive to, environmental conditions and resulting metabolic fluctuations. Proton influx is controlled by linear electron flow and a series of alternative electron flow pathways, possibly including cyclic electron flow around photosystem I, the Mehler peroxidase reaction (or water-water cycle), and oxidation of plastoquinol by the plastid terminal oxidase. The fraction of pmf stored as Delta pH is also regulated by plastidic ionic strength or luminal buffering capacity, altering the sensitivity of pH-dependent processes to pmf. The integrated regulation of these processes is an open, active area of research. C1 [Strand, Deserah D.] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Strand, Deserah D.; Kramer, David M.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Kramer, David M.] Michigan State Univ, Dept Biochem & Mol Biol, Dept Plant Biol, E Lansing, MI 48824 USA. RP Kramer, DM (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, Dept Plant Biol, 612 Wilson Rd 106, E Lansing, MI 48824 USA. EM kramerd8@msu.edu NR 155 TC 4 Z9 4 U1 1 U2 2 PU SPRINGER PI DORDRECHT PA PO BOX 17, 3300 AA DORDRECHT, NETHERLANDS SN 1572-0233 BN 978-94-017-9032-1; 978-94-017-9031-4 J9 ADV PHOTOSYNTH RESP JI Adv. Photo. Respirat. PY 2014 VL 40 BP 387 EP 408 DI 10.1007/978-94-017-9032-1_18 D2 10.1007/978-94-017-9032-1 PG 22 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA BD7IC UT WOS:000363120600019 ER PT B AU Haroldsen, B Stofleth, J Yip, M Caplan, A AF Haroldsen, Brent Stofleth, Jerome Yip, Mien Caplan, Allan BE Stang, DL Hallman, RT Springer, W Kwon, Y Hafner, RS TI EXPERIENCE WITH USING CODE CASE 2564 TO DESIGN AND CERTIFY AN IMPULSIVELY LOADED VESSEL SO PROCEEDINGS OF THE ASME PRESSURE VESSELS AND PIPING CONFERENCE - 2013, VOL 5 LA English DT Proceedings Paper CT ASME Pressure Vessels and Piping Conference (PVP-2013) CY JUL 14-18, 2013 CL Paris, FRANCE SP ASME, Pressure Vessels & Pip Div AB Code Case 2564 for the design of impulsively loaded vessels was approved in January 2008. In 2010 the US Army Non-Stockpile Chemical Materiel Program, with support from Sandia National Laboratories, procured a vessel per this Code Case for use on the Explosive Destruction System (EDS). The vessel was delivered to the Army in August of 2010 and approved for use by the DoD Explosives Safety Board in 2012. Although others have used the methodology and design limits of the Code Case to analyze vessels, to our knowledge, this was the first vessel to receive an ASME explosive rating with a U3 stamp. This paper discusses lessons learned in the process. Of particular interest were issues related to defining the design basis in the User Design Specification and explosive qualification testing required for regulatory approval. Specifying and testing an impulsively loaded vessel is more complicated than a static pressure vessel because the loads depend on the size, shape, and location of the explosive charges in the vessel and on the kind of explosives used and the point of detonation. Historically the US Department of Defense and Department of Energy have required an explosive test. Currently the Code Case does not address testing requirements, but it would be beneficial if it did since having vetted, third party standards for explosive qualification testing would simplify the process for regulatory approval. C1 [Haroldsen, Brent; Yip, Mien] Sandia Natl Labs, Livermore, CA 94551 USA. [Stofleth, Jerome] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Caplan, Allan] US Army Project Manager Nonstockpile Chem Mat, Aberdeen Proving Ground, MD USA. RP Haroldsen, B (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM blharol@sandia.gov; jhstofl@sandia.gov; myip@sandia.gov; allan.p.caplan.civ@mail.mil NR 11 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-5569-0 PY 2014 AR V005T05A021 PG 7 WC Engineering, Industrial; Engineering, Mechanical SC Engineering GA BD7CC UT WOS:000362863900021 ER PT B AU Pritchard, PG Carroll, L Hassan, T AF Pritchard, P. G. Carroll, L. Hassan, T. BE Stang, DL Hallman, RT Springer, W Kwon, Y Hafner, RS TI Constitutive Modeling of High Temperature Uniaxial Creep-Fatigue and Creep-Ratcheting Responses of Alloy 617 SO PROCEEDINGS OF THE ASME PRESSURE VESSELS AND PIPING CONFERENCE - 2013, VOL 5 LA English DT Proceedings Paper CT ASME Pressure Vessels and Piping Conference (PVP-2013) CY JUL 14-18, 2013 CL Paris, FRANCE SP ASME, Pressure Vessels & Pip Div ID VISCOPLASTICITY; PLASTICITY AB Inconel Alloy 617 is a high temperature creep and corrosion resistant alloy and is a leading candidate for use in Intermediate Heat Exchangers (IHX) of the Next Generation Nuclear Plants (NGNP). The IHX of the NGNP is expected to experience operating temperatures in the range of 800 degrees-950 degrees C, which is in the creep regime of Alloy 617. A broad set of uniaxial, low-cycle fatigue, fatigue-creep, ratcheting, and ratcheting-creep experiments are conducted in order to study the fatigue and ratcheting responses, and their interactions with the creep response at high temperatures. A unified constitutive model developed at North Carolina State University is used to simulate these experimental responses. The model is developed based on the Chaboche viscoplastic model framework. It includes cyclic hardening/softening, strain rate dependence, strain range dependence, static and dynamic recovery modeling features. For simulation of the alloy 617 responses, new techniques of model parameter determination are developed for optimized simulations. This paper compares the experimental responses and model simulations for demonstrating the strengths and shortcomings of the model. C1 [Pritchard, P. G.; Hassan, T.] N Carolina State Univ, Raleigh, NC 27695 USA. [Carroll, L.] Idaho Natl Lab, Idaho Falls, ID USA. RP Pritchard, PG (reprint author), N Carolina State Univ, Raleigh, NC 27695 USA. NR 12 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-5569-0 PY 2014 AR V005T11A009 PG 11 WC Engineering, Industrial; Engineering, Mechanical SC Engineering GA BD7CC UT WOS:000362863900046 ER PT B AU Yip, M Haroldsen, B AF Yip, Mien Haroldsen, Brent BE Stang, DL Hallman, RT Springer, W Kwon, Y Hafner, RS TI DESIGN BASIS OF AN IMPULSIVELY LOADED VESSEL FOR SPECIFIC LOADING CONFIGURATIONS SO PROCEEDINGS OF THE ASME PRESSURE VESSELS AND PIPING CONFERENCE - 2013, VOL 5 LA English DT Proceedings Paper CT ASME Pressure Vessels and Piping Conference (PVP-2013) CY JUL 14-18, 2013 CL Paris, FRANCE SP ASME, Pressure Vessels & Pip Div AB For an impulsively loaded containment vessel, such as the Sandia Explosive Destruction System (EDS), the traditional notion of a single-value explosive rating may not be sufficient to qualify the vessel for many real-life loading situations, such as those involving multiple munitions placed in various geometric configurations. Other significant factors, including detonation timing, geometry of explosive(s), and standoff distances, need to be considered for a more accurate assessment of the vessel integrity. It is obvious that the vessel structural response from an explosive charge detonated at the geometric center of the vessel will be very different from the structural response from the same explosive charge detonated next to the vessel wall. It is, however, less obvious that the same explosive can produce vastly different vessel response if it is detonated at one end versus at the middle versus from both ends. The goal of this paper is to identify some of the effects that non-trivial loading situations have on the vessel structural integrity. The metric for determining vessel integrity is based on Code Case 2564 of the ASME Boiler and Pressure Vessel Code. Based on the findings of this work, it may be necessary to qualify impulsively loaded containment vessels for specific explosive configurations, which should include the quantity, geometry and location of the explosives, as well as the detonation points. C1 [Yip, Mien; Haroldsen, Brent] Sandia Natl Labs, Livermore, CA 94551 USA. RP Yip, M (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM myip@sandia.gov; blharol@sandia.gov NR 9 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC MECHANICAL ENGINEERS PI NEW YORK PA THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA BN 978-0-7918-5569-0 PY 2014 AR V005T05A022 PG 7 WC Engineering, Industrial; Engineering, Mechanical SC Engineering GA BD7CC UT WOS:000362863900022 ER EF