FN Thomson Reuters Web of Science™
VR 1.0
PT J
AU Kuttiyiel, KA
Sasaki, K
Su, D
Vukmirovic, MB
Marinkovic, NS
Adzic, RR
AF Kuttiyiel, Kurian A.
Sasaki, Kotaro
Su, Dong
Vukmirovic, Miomir B.
Marinkovic, Nebojsa S.
Adzic, Radoslav R.
TI Pt monolayer on Au-stabilized PdNi core-shell nanoparticles for oxygen
reduction reaction
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Core-shell nanoparticles; Oxygen reduction; Pt monolayer; Pd-Ni;
Electrocatalysis
ID CATALYTIC-ACTIVITY; ELECTROCATALYSTS; PLATINUM; ELECTRODE; REMOVAL
AB Based on the unique catalytic properties of Pt by using its single layer on well-defined inexpensive nanosubstrates one can maximize its activity at the oxygen fuel cell cathode. This illustrates an efficient way of using Pt while overcoming its limited supply. We present a highly active and stable ORR catalyst, consisting of PdNi core-shell nanoparticles, which was protected against decomposition in acid by Au atoms and activated for oxygen reduction with a Pt monolayer. The roles of each component in the catalyst is investigated and in the best case the catalyst showed a Pt group metal mass activity that was approximately 3 times higher than that of the commercial Pt/C electrocatalyst. The Au protected PdNi core-shell nanoparticles were found to be stable support for Pt under high oxidizing conditions. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Kuttiyiel, Kurian A.; Sasaki, Kotaro; Vukmirovic, Miomir B.; Adzic, Radoslav R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Marinkovic, Nebojsa S.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA.
RP Adzic, RR (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM adzic@bnl.gov
RI Marinkovic, Nebojsa/A-1137-2016; Su, Dong/A-8233-2013
OI Marinkovic, Nebojsa/0000-0003-3579-3453; Su, Dong/0000-0002-1921-6683
FU US Department of Energy, Division of Chemical Sciences, Geosciences and
Biosciences Division [DE-AC02-98CH10886]; Synchrotron Catalysis
Consortium, US Department of Energy [DE-FG02-05ER15688]
FX This research was performed at Brookhaven National laboratory under
contract DE-AC02-98CH10886 with the US Department of Energy, Division of
Chemical Sciences, Geosciences and Biosciences Division. Beam lines X19A
and X18B at the NSLS are supported in part by the Synchrotron Catalysis
Consortium, US Department of Energy Grant No. DE-FG02-05ER15688.
NR 33
TC 32
Z9 32
U1 12
U2 100
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD NOV 1
PY 2013
VL 110
SI SI
BP 267
EP 272
DI 10.1016/j.electacta.2013.04.037
PG 6
WC Electrochemistry
SC Electrochemistry
GA 287GP
UT WOS:000329530300037
ER
PT J
AU Ferrandon, M
Wang, XP
Kropf, AJ
Myers, DJ
Wu, G
Johnston, CM
Zelenay, P
AF Ferrandon, Magali
Wang, Xiaoping
Kropf, A. Jeremy
Myers, Deborah J.
Wu, Gang
Johnston, Christina M.
Zelenay, Piotr
TI Stability of iron species in heat-treated polyaniline-iron-carbon
polymer electrolyte fuel cell cathode catalysts
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Non-precious metal catalyst; Oxygen reduction reaction (ORR); Stability;
Dissolution; X-ray absorption near edge spectroscopy (XANES)
ID OXYGEN REDUCTION REACTION; FE-BASED CATALYSTS; ACTIVE-SITES; AREA
CARBON; K-EDGE; PHTHALOCYANINE; SURFACE; ELECTROCATALYSTS;
ELECTROREDUCTION; DURABILITY
AB This paper describes the stability of Fe species in a heat-treated polyaniline-iron-carbon (PANI-Fe-C) oxygen reduction reaction (ORR) catalyst in an aqueous acidic electrolyte and in a membrane-electrode assembly (MEA) at various potentials. Linear combination fitting of ex situ and in situ X-ray absorption near-edge structure (XANES) spectra to the spectra for a suite of Fe standards was used to determine the catalyst iron speciation at various potentials, after potential cycling in an aqueous electrolyte, and after 200 h potentiostatic holds in MEAs. XANES edge-step analysis and inductively-coupled mass spectrometry were used to determine the amount of Fe lost from the catalyst into the aqueous electrolyte and from the MEA cathodes. Results showed that the Fe was lost from the catalyst in the electrochemical environment and the rate and extent of this loss were dependent on potential and on the type of electrolyte. The Fe specie primarily responsible for this loss was iron sulfide. Despite the large overall loss of Fe species from the catalyst that had been subjected to potentiostatic holds in an MM at either 0.4 V or 0.6 V for 200 h, H-2-air polarization curves showed only moderate loss of cathode kinetic performance while the performance in the mass transport region improved. Correlating the performance loss to the XANES speciation, the kinetic losses may be attributed to the oxidation of active site(s) and/or loss of pyrrolic-like and pyridinic-like coordination, as well as the mass transport improvement due to removal of inactive Fe species, predominantly sulfides. Species with porphyrazin-like coordination were stable in both the aqueous and MEA environments. It is speculated that the stability of the porphyrazin is responsible for the durability of this catalyst. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Ferrandon, Magali; Wang, Xiaoping; Kropf, A. Jeremy; Myers, Deborah J.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
[Wu, Gang; Johnston, Christina M.; Zelenay, Piotr] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
RP Ferrandon, M (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
EM ferrandon@anl.gov; zelenay@lanl.gov
RI Wu, Gang/E-8536-2010; BM, MRCAT/G-7576-2011; ID, MRCAT/G-7586-2011
OI Wu, Gang/0000-0003-4956-5208;
FU U.S. Department of Energy's Fuel Cell Technologies Program; U.S.
Department of Energy by University of Chicago Argonne, LLC
[DE-AC-02-06CH11357]; U.S. Department of Energy; MRCAT
FX Authors wish to thank Analytical Chemistry Laboratory at Argonne for the
elemental analyses. This work was supported by the U.S. Department of
Energy's Fuel Cell Technologies Program. Argonne National Laboratory is
managed for the U.S. Department of Energy by University of Chicago
Argonne, LLC, under contract DE-AC-02-06CH11357. Use of the Advanced
Photon Source was supported by the U.S. Department of Energy, Office of
Science, and Office of Basic Energy Sciences. MRCAT operations are
supported by the U.S. Department of Energy and the MRCAT member
institutions. The authors would like to thank their Department of Energy
Technology Development Manager, Nancy Garland, and the staff of sectors
10, 12, and 20 at the Advanced Photon Source, in particular Mahalingam
Balasubramanian and Nadia Leyarovska. The authors would also like to
thank James Gilbert for his assistance with the X-ray experiments.
NR 40
TC 31
Z9 31
U1 8
U2 99
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD NOV 1
PY 2013
VL 110
SI SI
BP 282
EP 291
DI 10.1016/j.electacta.2013.03.183
PG 10
WC Electrochemistry
SC Electrochemistry
GA 287GP
UT WOS:000329530300039
ER
PT J
AU Bowman, GR
Perez, AM
Ptacin, JL
Ighodaro, E
Folta-Stogniew, E
Comolli, LR
Shapiro, L
AF Bowman, Grant R.
Perez, Adam M.
Ptacin, Jerod L.
Ighodaro, Eseosa
Folta-Stogniew, Ewa
Comolli, Luis R.
Shapiro, Lucy
TI Oligomerization and higher-order assembly contribute to sub-cellular
localization of a bacterial scaffold
SO MOLECULAR MICROBIOLOGY
LA English
DT Article
ID DIVISION PROTEIN DIVIVA; CELL-DIVISION; CHROMOSOME SEGREGATION;
ESCHERICHIA-COLI; CAULOBACTER-CRESCENTUS; BINDING; CYCLE;
POLYDISPERSITY; MECHANISMS; DYNAMICS
AB In Caulobacter crescentus, the PopZ polar scaffold protein supports asymmetric cell division by recruiting distinct sets of binding partners to opposite cell poles. To understand how polar organizing centres are established by PopZ, we investigated a set of mutated PopZ proteins for defects in sub-cellular localization and recruitment activity. We identified a domain within the C-terminal 76 amino acids that is necessary and sufficient for accumulation as a single subcellular focus, a domain within the N-terminal 23 amino acids that is necessary for bipolar targeting, and a linker domain between these localization determinants that tolerates large variation. Mutations that inhibited dynamic PopZ localization inhibited the recruitment of other factors to cell poles. Mutations in the C-terminal domain also blocked discrete steps in the assembly of higher-order structures. Biophysical analysis of purified wild type and assembly defective mutant proteins indicates that PopZ self-associates into an elongated trimer, which readily forms a dimer of trimers through lateral contact. The final six amino acids of PopZ are necessary for connecting the hexamers into filaments, and these structures are important for sub-cellular localization. Thus, PopZ undergoes multiple orders of self-assembly, and the formation of an interconnected superstructure is a key feature of polar organization in Caulobacter.
C1 [Bowman, Grant R.; Perez, Adam M.; Ptacin, Jerod L.; Ighodaro, Eseosa; Shapiro, Lucy] Stanford Univ, Sch Med, Dept Dev Biol, Stanford, CA 94305 USA.
[Folta-Stogniew, Ewa] Yale Univ, Sch Med, WM Keck Biotechnol Resource Lab, New Haven, CT 06510 USA.
[Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
RP Bowman, GR (reprint author), Univ Wyoming, Dept Mol Biol, Laramie, WY 82071 USA.
EM grant.bowman@uwyo.edu
FU National Institute of Health [GM51426, GB32506]; Department of Energy
[DE-FG02-05ER64136]; Office of Basic Energy Sciences, Biological and
Environmental Research, of the US Department of Energy
[DE-AC02-05CH11231]; NIH [1S10RR023748-01]
FX We thank David Liberles for helpful advice. The work was supported by
National Institute of Health Grants GM51426 and GB32506, and Department
of Energy Grant DE-FG02-05ER64136 to L.S. L.R.C. was supported by Office
of Basic Energy Sciences, Biological and Environmental Research, of the
US Department of Energy under Contract No. DE-AC02-05CH11231. SEC-MALLS
instrumentation was supported by NIH Award Number 1S10RR023748-01.
NR 41
TC 10
Z9 10
U1 1
U2 11
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0950-382X
EI 1365-2958
J9 MOL MICROBIOL
JI Mol. Microbiol.
PD NOV
PY 2013
VL 90
IS 4
BP 776
EP 795
DI 10.1111/mmi.12398
PG 20
WC Biochemistry & Molecular Biology; Microbiology
SC Biochemistry & Molecular Biology; Microbiology
GA 295HU
UT WOS:000330108000008
PM 24102805
ER
PT J
AU Dawedeit, C
Kucheyev, SO
Shin, SJ
Willey, TM
Bagge-Hansen, M
Braun, T
Wang, YM
El-Dasher, BS
Teslich, NE
Biener, MM
Ye, JC
Kirste, L
Roehlig, CC
Wolfer, M
Woerner, E
van Buuren, AW
Hamza, AV
Wild, C
Biener, J
AF Dawedeit, Christoph
Kucheyev, Sergei O.
Shin, Swanee J.
Willey, Trevor M.
Bagge-Hansen, Michael
Braun, Tom
Wang, Y. Morris
El-Dasher, Bassem S.
Teslich, Nick E.
Biener, Monika M.
Ye, Jianchao
Kirste, Lutz
Roehlig, Claus-C.
Wolfer, Marco
Woerner, Eckhard
van Buuren, Anthony W.
Hamza, Alex V.
Wild, Christoph
Biener, Juergen
TI Grain size dependent physical and chemical properties of thick CVD
diamond films for high energy density physics experiments
SO DIAMOND AND RELATED MATERIALS
LA English
DT Article
DE Diamond film; Plasma CVD; Morphology; Texture; Grain size; Inertial
confinement fusion
ID NANOCRYSTALLINE DIAMOND; AMORPHOUS-CARBON; DEPOSITION; SIMULATION;
FUSION
AB We report on the grain size dependent morphological, physical and chemical properties of thick microwave-plasma assisted chemical vapor deposited (MPCVD) diamond films that are used as target materials for high energy density physics experiments at the Lawrence Livermore National Laboratory. Control over the grain size, ranging from several mu m to a few nm, was achieved by adjusting the CH4 content of the CH4/H-2 feed gas. The effect of grain size on surface roughness, morphology, texture, density, hydrogen and graphitic carbon content was systematically studied by a variety of techniques. For depositions performed at 35 to 45 mbar and 3000W microwave power (power density similar to 10W cm(-3)), an abrupt transition from micro-crystalline diamond to nanocrystalline diamond was observed at 3% CH4. This transition is accompanied by a dramatic decrease in surface roughness, a six percent drop in density and an increasing content in hydrogen and graphitic carbon impurities. Guided by these results, layered nano-microhybrid diamond samples were prepared by periodically changing the growth conditions from nano- to microcrystalline. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Dawedeit, Christoph; Kucheyev, Sergei O.; Shin, Swanee J.; Willey, Trevor M.; Bagge-Hansen, Michael; Braun, Tom; Wang, Y. Morris; El-Dasher, Bassem S.; Teslich, Nick E.; Biener, Monika M.; Ye, Jianchao; van Buuren, Anthony W.; Hamza, Alex V.; Biener, Juergen] Lawrence Livermore Natl Lab, Nanoscale Synth & Characterizat Lab, Livermore, CA 94550 USA.
[Kirste, Lutz; Roehlig, Claus-C.; Wolfer, Marco; Woerner, Eckhard; Wild, Christoph] Fraunhofer Inst Appl Solid State Phys, D-79108 Freiburg, Germany.
[Woerner, Eckhard; Wild, Christoph] Diamond Mat GmbH, D-79108 Freiburg, Germany.
RP Biener, J (reprint author), Lawrence Livermore Natl Lab, Nanoscale Synth & Characterizat Lab, Livermore, CA 94550 USA.
EM biener2@llnl.gov
RI Willey, Trevor/A-8778-2011; Wang, Yinmin (Morris)/F-2249-2010
OI Willey, Trevor/0000-0002-9667-8830; Wang, Yinmin
(Morris)/0000-0002-7161-2034
FU U.S. Department of Energy [DE-AC52-07NA27344]
FX This work was performed under the auspices of the U.S. Department of
Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344. CD gratefully acknowledges the support of the TUM
Faculty Graduate Center Mechanical Engineering at the Technische
Universitat Munchen.
NR 32
TC 7
Z9 7
U1 1
U2 39
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-9635
EI 1879-0062
J9 DIAM RELAT MATER
JI Diam. Relat. Mat.
PD NOV
PY 2013
VL 40
BP 75
EP 81
DI 10.1016/j.diamond.2013.10.001
PG 7
WC Materials Science, Multidisciplinary
SC Materials Science
GA 282DN
UT WOS:000329150600013
ER
PT J
AU Sullivan, JL
Wang, MQ
AF Sullivan, J. L.
Wang, M. Q.
TI Life cycle greenhouse gas emissions from geothermal electricity
production
SO JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY
LA English
DT Article
AB A life cycle analysis (LCA) is presented for greenhouse gas (GHG) emissions and fossil energy use associated with geothermal electricity production with a special focus on operational GHG emissions from hydrothermal flash and dry steam plants. The analysis includes results for both the plant and fuel cycle components of the total life cycle. The impact of recent changes to California's GHG reporting protocol for GHG emissions are discussed by comparing emission rate metrics derived from post and pre revision data sets. These metrics are running capacity weighted average GHG emission rates (g/kWh) and emission rate cumulative distribution functions. To complete our life cycle analysis, plant cycle results were extracted from our previous work and added to fuel cycle results. The resulting life cycle fossil energy and greenhouse gas emissions values are compared among a range of fossil, nuclear, and renewable power technologies, including geothermal. (C) 2013 AIP Publishing LLC.
C1 [Sullivan, J. L.; Wang, M. Q.] Argonne Natl Lab, Ctr Transportat Res, Div Energy Syst, Argonne, IL 60439 USA.
RP Sullivan, JL (reprint author), Argonne Natl Lab, Ctr Transportat Res, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA.
FU U.S. Department of Energy, Assistant Secretary for Energy Efficiency and
Renewable Energy, Office of Geothermal Technologies [DE-AC02-06CH11357];
Office of Geothermal Technologies, the Office of Energy Efficiency and
Renewable Energy, U.S. Department of Energy
FX Argonne National Laboratory's work was supported by the U.S. Department
of Energy, Assistant Secretary for Energy Efficiency and Renewable
Energy, Office of Geothermal Technologies, under contract
DE-AC02-06CH11357. We thank our sponsor, Arlene Anderson, of Office of
Geothermal Technologies, the Office of Energy Efficiency and Renewable
Energy, U.S. Department of Energy.
NR 18
TC 1
Z9 1
U1 3
U2 12
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1941-7012
J9 J RENEW SUSTAIN ENER
JI J. Renew. Sustain. Energy
PD NOV
PY 2013
VL 5
IS 6
AR 063122
DI 10.1063/1.4841235
PG 13
WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels
SC Science & Technology - Other Topics; Energy & Fuels
GA 282MO
UT WOS:000329176100022
ER
PT J
AU Campione, S
Sinclair, MB
Capolino, F
AF Campione, Salvatore
Sinclair, Michael B.
Capolino, Filippo
TI Effective medium representation and complex modes in 3D periodic
metamaterials made of cubic resonators with large permittivity at
mid-infrared frequencies
SO PHOTONICS AND NANOSTRUCTURES-FUNDAMENTALS AND APPLICATIONS
LA English
DT Article
DE Mode analysis; Metamaterials; Effective medium theory; Artificial
magnetism
ID METAL-NANOPARTICLE CHAINS; LINEAR-CHAINS; MICROWAVE-FREQUENCIES;
PLASMONIC NANOSPHERES; OPTICAL-PROPERTIES; REFRACTIVE-INDEX; WAVE-GUIDE;
ARRAYS; PARTICLES; SPHERES
AB We review some of the techniques that lead to the effective medium representation of a three-dimensional (3D) periodic metamaterial. We consider a 3D lattice of lead telluride cubic resonators at mid-infrared (MW) frequencies. Each cubic resonator is modeled with both an electric and a magnetic dipole, through a method called the dual dipole approximation. The electric and magnetic polarizabilities of a cubic resonator are computed via full-wave simulations by mapping the resonator's scattered field under electric/magnetic excitation only to the field radiated by an equivalent electric/magnetic dipole. We then analyze the allowed modes in the lattice, with transverse polarization and complex wavenumber, highlighting the attenuation that each mode experiences after one free space wavelength. We observe the presence of two modes with low attenuation constant, dominant in different frequency ranges, able to propagate inside the lattice: this allows the treatment of the metamaterial as a homogeneous material with effective parameters, evaluated by using various techniques. We then show that the metamaterial under analysis allows for the generation of artificial magnetism (i.e., relative effective permeability different than unity, including negative permeability with low losses) at MIR frequencies. (C) 2013 Elsevier BV. All rights reserved.
C1 [Campione, Salvatore; Capolino, Filippo] Univ Calif Irvine, Dept Elect Engn & Comp Sci, Irvine, CA 92697 USA.
[Sinclair, Michael B.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Capolino, F (reprint author), Univ Calif Irvine, Dept Elect Engn & Comp Sci, Irvine, CA 92697 USA.
EM mbsincl@sandia.gov; f.capolino@uci.edu
RI Campione, Salvatore/A-2349-2015
OI Campione, Salvatore/0000-0003-4655-5485
FU U.S. Department of Energy's National Nuclear Security Administration
[158883]; National Science Foundation [CMMI-1101074]
FX This work was performed, in part, at the Center for Integrated
Nanotechnologies, a U.S. Department of Energy, Office of Basic. Energy
Sciences user facility. Sandia National Laboratories is a multi-program
laboratory managed and operated by Sandia Corporation, a wholly owned
subsidiary of Lockheed Martin Corporation, for the U.S. Department of
Energy's National Nuclear Security Administration under contract
DE-AC04-94AL85000 #158883.; This material is also based upon work
supported by the National Science Foundation under Grant No.
CMMI-1101074. The authors also thank CST Inc. and Ansys Inc. for
providing CST Microwave Studio and HFSS, respectively, which were
instrumental in this work.
NR 92
TC 11
Z9 11
U1 0
U2 28
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1569-4410
EI 1569-4429
J9 PHOTONIC NANOSTRUCT
JI Photonics Nanostruct.
PD NOV
PY 2013
VL 11
IS 4
BP 423
EP 435
DI 10.1016/j.photonics.2013.07.013
PG 13
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Optics; Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Optics; Physics
GA 285US
UT WOS:000329421100013
ER
PT J
AU Denissen, NA
White, EB
AF Denissen, Nicholas A.
White, Edward B.
TI Secondary instability of roughness-induced transient growth
SO PHYSICS OF FLUIDS
LA English
DT Article
ID PLATE BOUNDARY-LAYER; BYPASS TRANSITION; OPTIMAL PERTURBATIONS; OPTIMAL
DISTURBANCES; ELEMENTS; FLOW; STREAKS; STABILITY; VORTICES; SURFACE
AB Calculations are performed to analyze the stability of steady roughness-induced transient growth to unsteady fluctuations. The basic states consist of an optimal transient growth model and a previously computed direct numerical simulation that fully resolves the three-dimensional roughness element. It is shown that sub-optimal transient growth produced by surface roughness is much more susceptible to destabilization than optimal perturbation predictions. The factors contributing to this behavior are analyzed in detail. Scaling properties from experiments allow computation of stability bounds for realistic surface roughness. These results are also used to explain the critical behavior seen in transition behind three-dimensional roughness elements. (C) 2013 AIP Publishing LLC.
C1 [Denissen, Nicholas A.] Los Alamos Natl Lab, X Computat Phys Div, Los Alamos, NM 87545 USA.
[White, Edward B.] Texas A&M Univ, Dept Aerosp Engn, College Stn, TX 77843 USA.
RP Denissen, NA (reprint author), Los Alamos Natl Lab, X Computat Phys Div, POB 1663, Los Alamos, NM 87545 USA.
FU NASA; AFOSR through AFOSR [FA9550-09-1-0341, FA9550-08-1-0093]; NSF
GRFP; Texas A&M Dwight Look College of Engineering; Los Alamos National
Laboratory
FX The authors would like to thank Dr. Donald Rizzetta for access to the
DNS results. The authors acknowledge the support of NASA and AFOSR
through AFOSR Grant Nos. FA9550-09-1-0341 and FA9550-08-1-0093. The
first author also acknowledges support from the NSF GRFP, the Texas A&M
Dwight Look College of Engineering, and Los Alamos National Laboratory.
NR 34
TC 8
Z9 8
U1 0
U2 18
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-6631
EI 1089-7666
J9 PHYS FLUIDS
JI Phys. Fluids
PD NOV
PY 2013
VL 25
IS 11
AR 114108
DI 10.1063/1.4829482
PG 18
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 282PK
UT WOS:000329184100053
ER
PT J
AU Mejia-Alvarez, R
Christensen, KT
AF Mejia-Alvarez, R.
Christensen, K. T.
TI Wall-parallel stereo particle-image velocimetry measurements in the
roughness sublayer of turbulent flow overlying highly irregular
roughness
SO PHYSICS OF FLUIDS
LA English
DT Article
ID REAL TURBINE ROUGHNESS; BOUNDARY-LAYERS; SURFACE-ROUGHNESS; EXPERIMENTAL
SUPPORT; VORTEX ORGANIZATION; PRESSURE-GRADIENT; REYNOLDS STRESS;
CHANNEL FLOW; STATISTICS; HYPOTHESIS
AB Stereo particle-image velocimetry measurements were conducted in a streamwise-spanwise (x - z) plane deep within the roughness sublayer (y = 0.047 delta; delta is the boundary-layer thickness) of a zero-pressure-gradient turbulent boundary layer overlying highly irregular surface roughness replicated from a turbine blade damaged by foreign-material deposition. The ensemble-averaged streamwise velocity defect revealed the tendency of the roughness to promote channeling of the flow in the form of low-momentum pathways (LMPs) and high-momentum pathways. Enhanced turbulent and vortical activity was observed both between and along the spanwise boundaries of these streamwise-elongated pathways. In particular, streamwise pathways of wall-normal vortex cores of opposing rotational sense were observed along the spanwise boundaries of the identified LMP in the rough-wall flow. Conditional averaging revealed that these counter-rotating vortical motions are associated with streamwise flow against the mean-flow direction and could perhaps be the origination mechanism of the LMPs. Two-point correlation coefficients of velocity and swirling strength reflected large-scale streamwise coherence of these quantities along and outboard of the identified LMP in the rough-wall flow, supporting the notion that the motions responsible for the LMP have large-scale, streamwise coherence. Finally, the influence of different topographical scales of the roughness on the flow in the roughness sublayer was explored using low-order models of the original, full surface as originally proposed by R. Mejia-Alvarez and K. T. Christensen [Phys. Fluids 22(1), 015106 (2010)]. While a model containing only the largest topographical scales qualitatively reproduced the features of the full-surface flow, additional intermediate topographical scales were required to quantitatively reproduce the statistical and structural nature of the full-surface flow in the roughness sublayer. (C) 2013 AIP Publishing LLC.
C1 [Mejia-Alvarez, R.; Christensen, K. T.] Univ Illinois, Dept Mech Sci & Engn, Urbana, IL 61801 USA.
[Christensen, K. T.] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Fukuoka 812, Japan.
RP Mejia-Alvarez, R (reprint author), Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA.
EM ktc@illinois.edu
RI Christensen, Kenneth/B-1123-2009
OI Christensen, Kenneth/0000-0003-1468-2455
FU Air Force Office of Scientific Research [FA9550-07-1-0129]
FX This work was supported by the Air Force Office of Scientific Research
under Grant No. FA9550-07-1-0129 (Dr. John Schmisseur, Program Manager).
NR 44
TC 15
Z9 15
U1 0
U2 10
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-6631
EI 1089-7666
J9 PHYS FLUIDS
JI Phys. Fluids
PD NOV
PY 2013
VL 25
IS 11
AR 115109
DI 10.1063/1.4832377
PG 24
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 282PK
UT WOS:000329184100063
ER
PT J
AU Olson, BJ
Lele, SK
AF Olson, Britton J.
Lele, Sanjiva K.
TI A mechanism for unsteady separation in over-expanded nozzle flow
SO PHYSICS OF FLUIDS
LA English
DT Article
ID LARGE-EDDY SIMULATION; DIRECT NUMERICAL-SIMULATION; BOUNDARY-LAYER
INTERACTION; DIFFUSERS; OSCILLATIONS; REGIME
AB Shock wave induced separation in an over-expanded planar nozzle is studied through numerical simulation. These Large-Eddy Simulations (LES) model previous experiments which have shown unsteady motion of the shock wave in flows with similar geometries but offered little insight into the underlying mechanism. Unsteady separation in nozzle flow leads to "side loads" in the rocket engine which can adversely affect the stability of the rocket. A mechanism for the low-frequency shock motion is identified and explained using the LES data. This mechanism is analyzed for a series of over-expanded planar nozzles of various area ratios and nozzle pressure ratios. The effect of grid resolution and Reynolds number on the instability is discussed. A simple reduced order model for the unsteady shock behavior is used to further validate the proposed mechanism. This model is derived from first principles and uses data from the LES calculations to capture the effects of the turbulent boundary layer and shear layer. (C) 2013 AIP Publishing LLC.
C1 [Olson, Britton J.; Lele, Sanjiva K.] Stanford Univ, Dept Aeronaut & Astronaut, Stanford, CA 94305 USA.
[Olson, Britton J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
RP Olson, BJ (reprint author), Stanford Univ, Dept Aeronaut & Astronaut, Stanford, CA 94305 USA.
EM olson45@llnl.gov
FU Stanford/CTR; Department of Energy SciDAC2 Grant [DE-FC02-06-ER25787];
DOE Computational Science Graduate Fellowship; U.S. Department of Energy
by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]
FX S.K.L. is deeply appreciative of Professor Parviz Moin's mentoring
during his early days at Stanford/CTR and his leadership in promoting
scholarship. We are pleased to offer this paper as a small token of our
appreciation on the occasion of his 60th birthday. This work is
supported by the Department of Energy SciDAC2 Grant (Grant No.
DE-FC02-06-ER25787) and the DOE Computational Science Graduate
Fellowship. The authors wish to thank Dr. Andrew Cook and Dr. William
Cabot for providing the Miranda code which was modified for the present
study. Furthermore, we are grateful to Dr. Papamoschou and Dr. Johnson
for generous sharing of their experimental data and for their valuable
insight. This work was performed under the auspices of the U.S.
Department of Energy by Lawrence Livermore National Laboratory under
Contract No. DE-AC52-07NA27344.
NR 40
TC 4
Z9 4
U1 3
U2 21
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-6631
EI 1089-7666
J9 PHYS FLUIDS
JI Phys. Fluids
PD NOV
PY 2013
VL 25
IS 11
AR 110809
DI 10.1063/1.4819349
PG 24
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 282PK
UT WOS:000329184100010
ER
PT J
AU Orlicz, GC
Balasubramanian, S
Prestridge, KP
AF Orlicz, G. C.
Balasubramanian, S.
Prestridge, K. P.
TI Incident shock Mach number effects on Richtmyer-Meshkov mixing in a
heavy gas layer
SO PHYSICS OF FLUIDS
LA English
DT Article
ID RAYLEIGH-TAYLOR INSTABILITY; NUMERICAL-SIMULATION; TRANSITION; FLUIDS;
FUSION; FLOW; PLIF
AB Experiments were performed at the horizontal shock tube facility at Los Alamos National Laboratory to study the effect of incident shock Mach number (M) on the development of Richtmyer-Meshkov instability after a shock wave impulsively accelerates a varicose-perturbed, heavy-gas curtain. Three cases of incident shock strength were experimentally investigated: M = 1.21, 1.36, and 1.50. We discuss the state of the mixing and the mechanisms that drive the mixing at both large and small scales by examining the time evolution of 2D density fields derived from quantitative planar laser-induced fluorescence measurements. Several differences in qualitative flow features are identified as a result of Mach number variation, and differences in vortex interaction, observed using particle image velocimetry, play a critical role in the development of the flow field. Several quantities, including mixing layer width, mixing layer area, interface length, instantaneous mixing rate, the density self-correlation parameter, probability density functions of the density field, and mixing progress variables are examined as a function of time. These quantities are also examined versus time scaled with the convection velocity of the mixing layer. A higher incident Mach number yields greater mixing uniformity at a given downstream location, while a lower Mach number produces a greater amount of total mixing between the two gases, suggesting possible implications for optimization in applications with confined geometries. (C) 2013 AIP Publishing LLC.
C1 [Orlicz, G. C.; Prestridge, K. P.] Los Alamos Natl Lab, Div Phys, Extreme Fluids Team, Los Alamos, NM 87545 USA.
[Balasubramanian, S.] Indian Inst Technol, Dept Mech Engn, Bombay 400076, Maharashtra, India.
RP Orlicz, GC (reprint author), Los Alamos Natl Lab, Div Phys, Extreme Fluids Team, P-23, Los Alamos, NM 87545 USA.
EM kpp@lanl.gov
RI Prestridge, Kathy/C-1137-2012
OI Prestridge, Kathy/0000-0003-2425-5086
NR 38
TC 12
Z9 13
U1 0
U2 21
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 1070-6631
EI 1089-7666
J9 PHYS FLUIDS
JI Phys. Fluids
PD NOV
PY 2013
VL 25
IS 11
AR 114101
DI 10.1063/1.4827435
PG 28
WC Mechanics; Physics, Fluids & Plasmas
SC Mechanics; Physics
GA 282PK
UT WOS:000329184100046
ER
PT J
AU Blaby, IK
Glaesener, AG
Mettler, T
Fitz-Gibbon, ST
Gallaher, SD
Liu, BS
Boyle, NR
Kropat, J
Stitt, M
Johnson, S
Benning, C
Pellegrini, M
Casero, D
Merchant, SS
AF Blaby, Ian K.
Glaesener, Anne G.
Mettler, Tabea
Fitz-Gibbon, Sorel T.
Gallaher, Sean D.
Liu, Bensheng
Boyle, Nanette R.
Kropat, Janette
Stitt, Mark
Johnson, Shannon
Benning, Christoph
Pellegrini, Matteo
Casero, David
Merchant, Sabeeha S.
TI Systems-Level Analysis of Nitrogen Starvation-Induced Modifications of
Carbon Metabolism in a Chlamydomonas reinhardtii Starchless Mutant
SO PLANT CELL
LA English
DT Article
ID ADP-GLUCOSE PYROPHOSPHORYLASE; DNA-SEQUENCING DATA; MATING-TYPE LOCUS;
FATTY-ACID; DIACYLGLYCEROL ACYLTRANSFERASE; TRIACYLGLYCEROL
ACCUMULATION; GENE-EXPRESSION; GAMETIC DIFFERENTIATION;
SKELETONEMA-COSTATUM; LIPID-METABOLISM
AB To understand the molecular basis underlying increased triacylglycerol (TAG) accumulation in starchless (sta) Chlamydomonas reinhardtii mutants, we undertook comparative time-course transcriptomics of strains CC-4348 (sta6 mutant), CC-4349, a cell wall-deficient (cw) strain purported to represent the parental STA6 strain, and three independent STA6 strains generated by complementation of sta6 (CC-4565/STA6-C2, CC-4566/STA6-C4, and CC-4567/STA6-C6) in the context of N deprivation. Despite N starvation-induced dramatic remodeling of the transcriptome, there were relatively few differences (5 x 10(2)) observed between sta6 and STA6, the most dramatic of which were increased abundance of transcripts encoding key regulated or rate-limiting steps in central carbon metabolism, specifically isocitrate lyase, malate synthase, transaldolase, fructose bisphosphatase and phosphoenolpyruvate carboxykinase (encoded by ICL1, MAS1, TAL1, FBP1, and PCK1 respectively), suggestive of increased carbon movement toward hexose-phosphate in sta6 by upregulation of the glyoxylate pathway and gluconeogenesis. Enzyme assays validated the increase in isocitrate lyase and malate synthase activities. Targeted metabolite analysis indicated increased succinate, malate, and Glc-6-P and decreased Fru-1,6-bisphosphate, illustrating the effect of these changes. Comparisons of independent data sets in multiple strains allowed the delineation of a sequence of events in the global N starvation response in C. reinhardtii, starting within minutes with the upregulation of alternative N assimilation routes and carbohydrate synthesis and subsequently a more gradual upregulation of genes encoding enzymes of TAG synthesis. Finally, genome resequencing analysis indicated that (1) the deletion in sta6 extends into the neighboring gene encoding respiratory burst oxidase, and (2) a commonly used STA6 strain (CC-4349) as well as the sequenced reference (CC-503) are not congenic with respect to sta6 (CC-4348), underscoring the importance of using complemented strains for more rigorous assignment of phenotype to genotype.
C1 [Blaby, Ian K.; Glaesener, Anne G.; Fitz-Gibbon, Sorel T.; Gallaher, Sean D.; Boyle, Nanette R.; Kropat, Janette; Merchant, Sabeeha S.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.
[Mettler, Tabea; Stitt, Mark] Max Planck Inst Mol Plant Physiol, D-14476 Potsdam, Germany.
[Fitz-Gibbon, Sorel T.; Pellegrini, Matteo; Casero, David] Univ Calif Los Angeles, Dept Mol Cell & Dev Biol, Los Angeles, CA 90095 USA.
[Liu, Bensheng; Benning, Christoph] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA.
[Johnson, Shannon] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Pellegrini, Matteo; Casero, David; Merchant, Sabeeha S.] Univ Calif Los Angeles, Inst Genom & Prote, Los Angeles, CA 90095 USA.
RP Merchant, SS (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.
EM merchant@chem.ucla.edu
RI Blaby, Ian/C-3292-2014;
OI Johnson, Shannon/0000-0002-3972-9208; Casero, David/0000-0002-7347-3330
FU Department of Energy (National Alliance for Advance Biofuels and
Bioproducts Consortium) [DE-EE0003046]; National Institutes of Health
[R24 GM092473, T32 ES015457]; U.S. Air Force Office of Scientific
Research [FA9550-11-10264]
FX This work was supported by Department of Energy Contract DE-EE0003046
(to S.S.M., M.P., and S.J. via the National Alliance for Advance
Biofuels and Bioproducts Consortium) and in part by the National
Institutes of Health R24 GM092473 to S.S.M. and the U.S. Air Force
Office of Scientific Research (FA9550-11-10264, to C.B.). I.K.B. is
supported by a training grant from the National Institutes of Health
(T32 ES015457). We thank Ursula Goodenough for forwarding us strains
cw15 (CC-4349), sta6 (CC-4348), STA6-C2 (CC-4565), STA6-C4 (CC-4566),
and STA6-C6 (CC-4567), David Dauvillee for an independent cw15
(CC-4568), and Anthony Huang for the MLDP1 antibody.
NR 88
TC 62
Z9 63
U1 8
U2 73
PU AMER SOC PLANT BIOLOGISTS
PI ROCKVILLE
PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA
SN 1040-4651
EI 1532-298X
J9 PLANT CELL
JI Plant Cell
PD NOV
PY 2013
VL 25
IS 11
BP 4305
EP 4323
DI 10.1105/tpc.113.117580
PG 19
WC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
SC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
GA 282LY
UT WOS:000329174400006
PM 24280389
ER
PT J
AU Shen, H
Mazarei, M
Hisano, H
Escamilla-Trevino, L
Fu, CX
Pu, YQ
Rudis, MR
Tang, YH
Xiao, XR
Jackson, L
Li, GF
Hernandez, T
Chen, F
Ragauskas, AJ
Stewart, CN
Wang, ZY
Dixon, RA
AF Shen, Hui
Mazarei, Mitra
Hisano, Hiroshi
Escamilla-Trevino, Luis
Fu, Chunxiang
Pu, Yunqiao
Rudis, Mary R.
Tang, Yuhong
Xiao, Xirong
Jackson, Lisa
Li, Guifen
Hernandez, Tim
Chen, Fang
Ragauskas, Arthur J.
Stewart, C. Neal, Jr.
Wang, Zeng-Yu
Dixon, Richard A.
TI A Genomics Approach to Deciphering Lignin Biosynthesis in Switchgrass
SO PLANT CELL
LA English
DT Article
ID PANICUM-VIRGATUM L.; CELL-SUSPENSION CULTURES; CAFFEIC ACID
3-O-METHYLTRANSFERASE; FERMENTABLE SUGAR YIELDS; EXPRESSED SEQUENCE
TAGS; FERULATE CROSS-LINKING; ARABIDOPSIS-THALIANA; BIOFUEL PRODUCTION;
CINNAMATE 4-HYDROXYLASE; O-METHYLTRANSFERASE
AB It is necessary to overcome recalcitrance of the biomass to saccharification (sugar release) to make switchgrass (Panicum virgatum) economically viable as a feedstock for liquid biofuels. Lignin content correlates negatively with sugar release efficiency in switchgrass, but selecting the right gene candidates for engineering lignin biosynthesis in this tetraploid outcrossing species is not straightforward. To assist this endeavor, we have used an inducible switchgrass cell suspension system for studying lignin biosynthesis in response to exogenous brassinolide. By applying a combination of protein sequence phylogeny with whole-genome microarray analyses of induced cell cultures and developing stem internode sections, we have generated a list of candidate monolignol biosynthetic genes for switchgrass. Several genes that were strongly supported through our bioinformatics analysis as involved in lignin biosynthesis were confirmed by gene silencing studies, in which lignin levels were reduced as a result of targeting a single gene. However, candidate genes encoding enzymes involved in the early steps of the currently accepted monolignol biosynthesis pathway in dicots may have functionally redundant paralogues in switchgrass and therefore require further evaluation. This work provides a blueprint and resources for the systematic genome-wide study of the monolignol pathway in switchgrass, as well as other C4 monocot species.
C1 [Shen, Hui; Escamilla-Trevino, Luis; Tang, Yuhong; Jackson, Lisa; Li, Guifen; Hernandez, Tim; Chen, Fang; Dixon, Richard A.] Samuel Roberts Noble Fdn Inc, Div Plant Biol, Ardmore, OK 73401 USA.
[Shen, Hui; Mazarei, Mitra; Hisano, Hiroshi; Escamilla-Trevino, Luis; Fu, Chunxiang; Pu, Yunqiao; Rudis, Mary R.; Tang, Yuhong; Xiao, Xirong; Jackson, Lisa; Li, Guifen; Hernandez, Tim; Chen, Fang; Ragauskas, Arthur J.; Stewart, C. Neal, Jr.; Wang, Zeng-Yu; Dixon, Richard A.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA.
[Mazarei, Mitra; Rudis, Mary R.; Stewart, C. Neal, Jr.] Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA.
[Hisano, Hiroshi; Fu, Chunxiang; Xiao, Xirong; Wang, Zeng-Yu] Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA.
[Pu, Yunqiao; Ragauskas, Arthur J.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA.
RP Dixon, RA (reprint author), Samuel Roberts Noble Fdn Inc, Div Plant Biol, Ardmore, OK 73401 USA.
EM Richard.Dixon@unt.edu
OI Pu, Yunqiao/0000-0003-2554-1447
FU BioEnergy Sciences Center, a U.S. Department of Energy Bioenergy
Research Center, through the Office of Biological and Environmental
Research in the Department of Energy Office of Science
FX This work was supported by the BioEnergy Sciences Center, a U.S.
Department of Energy Bioenergy Research Center, through the Office of
Biological and Environmental Research in the Department of Energy Office
of Science. We thank Yanbin Yin, Jiyi Zhang, Yinbin Ge, and Nick Krom
for excellent assistance with EST sequence annotation and
bioinformatics; Jin Nakashima for assistance with cell imaging; Mohamed
Bedair for assistance with GC-MS analysis; Tui Ray for technical support
with qRT-PCR analysis; Debra Mohnen and Ivana Gelineo-Albersheim for
helpful discussions concerning inducible cell cultures; and Mingyi Wang
and Xiaolan Rao for critical reading of the article.
NR 102
TC 30
Z9 31
U1 0
U2 45
PU AMER SOC PLANT BIOLOGISTS
PI ROCKVILLE
PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA
SN 1040-4651
EI 1532-298X
J9 PLANT CELL
JI Plant Cell
PD NOV
PY 2013
VL 25
IS 11
BP 4342
EP 4361
DI 10.1105/tpc.113.118828
PG 20
WC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
SC Biochemistry & Molecular Biology; Plant Sciences; Cell Biology
GA 282LY
UT WOS:000329174400008
PM 24285795
ER
PT J
AU Knowles, DW
Biggin, MD
AF Knowles, David W.
Biggin, Mark D.
TI Building quantitative, three-dimensional atlases of gene expression and
morphology at cellular resolution
SO WILEY INTERDISCIPLINARY REVIEWS-DEVELOPMENTAL BIOLOGY
LA English
DT Article
AB Animals comprise dynamic three-dimensional arrays of cells that express gene products in intricate spatial and temporal patterns that determine cellular differentiation and morphogenesis. A rigorous understanding of these developmental processes requires automated methods that quantitatively record and analyze complex morphologies and their associated patterns of gene expression at cellular resolution. Here we summarize light microscopy-based approaches to establish permanent, quantitative datasets-atlases-that record this information. We focus on experiments that capture data for whole embryos or large areas of tissue in three dimensions, often at multiple time points. We compare and contrast the advantages and limitations of different methods and highlight some of the discoveries made. We emphasize the need for interdisciplinary collaborations and integrated experimental pipelines that link sample preparation, image acquisition, image analysis, database design, visualization, and quantitative analysis. (C) 2013 Wiley Periodicals, Inc.
C1 [Knowles, David W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
RP Knowles, DW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
EM DWKnowles@lbl.gov
FU NIGMS NIH HHS [P01 GM099655, 1R01GM085298-01A1, R01 GM085298]
NR 0
TC 2
Z9 2
U1 0
U2 0
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1759-7684
EI 1759-7692
J9 WIRES DEV BIOL
JI Wiley Interdiscip. Rev.-Dev. Biol.
PD NOV-DEC
PY 2013
VL 2
IS 6
BP 767
EP 779
DI 10.1002/wdev.107
PG 13
WC Developmental Biology
SC Developmental Biology
GA 286HM
UT WOS:000329458400002
PM 24123936
ER
PT J
AU Kim, D
Croy, JR
Thackeray, MM
AF Kim, Donghan
Croy, Jason R.
Thackeray, Michael M.
TI Comments on stabilizing layered manganese oxide electrodes for Li
batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Layered manganese oxide; Li2MnO3; Cathode; Lithium battery
ID LITHIUM-ION BATTERIES; CATHODE MATERIALS; LOCAL-STRUCTURE; NMR; LI2MNO3;
VOLTAGE; LIMNO2; ELECTROCHEMISTRY; LINI0.5MN0.5O2; TRANSITION
AB An electrochemical study of structurally-integrated xLi(2)MnO(3)center dot(1-x)LiMn0.5Ni0.5O2 'composite' materials has been undertaken to investigate the stability of electrochemically-activated electrodes at the Li2MnO3-rich end of the Li2MnO3-LiMn0.5Ni0.5O2 tie-line, i.e., for 0.7 <= x <= 0.95. Excellent performance was observed for x = 0.7 in lithium half-cells; comparable to activated electrodes that have significantly lower values of x and are traditionally the preferred materials of choice. Electrodes with higher manganese content (x >= 0.8) showed significantly reduced performance. Implications for stabilizing low-cost manganese-rich, layered lithium-metaloxide electrode materials are discussed. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Kim, Donghan; Croy, Jason R.; Thackeray, Michael M.] Argonne Natl Lab, Electrochem Energy Storage Dept, Chem Sci & Engn Div, Lemont, IL 60439 USA.
RP Croy, JR (reprint author), Argonne Natl Lab, Electrochem Energy Storage Dept, Chem Sci & Engn Div, Lemont, IL 60439 USA.
EM croy@anl.gov
FU Office of Vehicle Technologies, Office of Energy Efficiency and
Renewable Energy of the U.S. Department of Energy; U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences
FX This work was supported by the Office of Vehicle Technologies, Office of
Energy Efficiency and Renewable Energy of the U.S. Department of Energy.
Bonil Koo and Soongu Kwon (CNM, Argonne National Laboratory) are thanked
for SEM data. Facilities at CNM are supported by the U.S. Department of
Energy, Office of Science, Office of Basic Energy Sciences.
NR 24
TC 26
Z9 26
U1 7
U2 88
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
EI 1873-1902
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD NOV
PY 2013
VL 36
BP 103
EP 106
DI 10.1016/j.elecom.2013.08.022
PG 4
WC Electrochemistry
SC Electrochemistry
GA 278ZE
UT WOS:000328927600026
ER
PT J
AU Logan, J
Lopez, A
Mai, T
Davidson, C
Bazilian, M
Arent, D
AF Logan, Jeffrey
Lopez, Anthony
Mai, Trieu
Davidson, Carolyn
Bazilian, Morgan
Arent, Douglas
TI Natural gas scenarios in the US power sector
SO ENERGY ECONOMICS
LA English
DT Article
DE Energy policy; Power sector modeling; Unconventional natural gas
ID SHALE GAS; PLAYS
AB The United States power sector is being transformed by the recent rise in the availability and use of unconventional natural gas, specifically shale gas. That transformation has already produced some of the most significant changes in the operation of the portfolio of electricity generation since WWII. Further implications are likely. To that end, we present results from numerical modeling of different United States (U.S.) power sector futures. These futures assess questions affecting today's natural gas and electric power markets, including the impacts of: forthcoming EPA rules on power plants, decarbonization options such as a clean energy standard (CES), potential improvements in key generation technologies, expanded use of natural gas outside of the power generation sector, and higher costs for natural gas production-assumed to arise from more robust environmental and safety practices in the field. The simulations were done using the ReEDS model looking out to the year 2050. ReEDS is a capacity expansion model that determines the least-cost combination of generation options that fulfill a variety of user-defined constraints such as projected load, capacity reserve margins, emissions limitations, and operating lifetimes. The baseline scenario shows strong growth in natural gas generation, leading to a roughly 2.5-fold increase in gas demand by 2050. Many other scenarios also see strong growth in gas-fired generation, highlighting questions about portfolio diversity, climate change, and research and development prioritization. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Logan, Jeffrey; Lopez, Anthony; Mai, Trieu; Davidson, Carolyn] Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Bazilian, Morgan; Arent, Douglas] Natl Renewable Energy Lab, Joint Inst Strateg Energy Anal, Golden, CO 80401 USA.
RP Logan, J (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.
EM jeffrey.logan@nrel.gov
NR 28
TC 18
Z9 18
U1 2
U2 22
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0140-9883
EI 1873-6181
J9 ENERG ECON
JI Energy Econ.
PD NOV
PY 2013
VL 40
BP 183
EP 195
DI 10.1016/j.eneco.2013.06.008
PG 13
WC Economics
SC Business & Economics
GA 281DX
UT WOS:000329081300018
ER
PT J
AU Schneider, E
Carlsen, B
Tavrides, E
van der Hoeven, C
Phathanapirom, U
AF Schneider, E.
Carlsen, B.
Tavrides, E.
van der Hoeven, C.
Phathanapirom, U.
TI Measures of the environmental footprint of the front end of the nuclear
fuel cycle
SO ENERGY ECONOMICS
LA English
DT Article
DE Nuclear fuel cycle; Environmental impacts
ID URANIUM ENRICHMENT; GENERATION; SYSTEMS
AB Previous estimates of environmental impacts associated with the front end of the nuclear fuel cycle (FEFC) have focused primarily on energy consumption and CO2 emissions. Results have varied widely. This work builds upon reports from operating facilities and other primary data sources to build a database of front end environmental impacts. This work also addresses land transformation and water withdrawals associated with the processes of the FEFC These processes include uranium extraction, conversion, enrichment, fuel fabrication, depleted uranium disposition, and transportation.
To allow summing the impacts across processes, all impacts were normalized per tonne of natural uranium mined as well as per MWh(e) of electricity produced, a more conventional unit for measuring environmental impacts that facilitates comparison with other studies. This conversion was based on mass balances and process efficiencies associated with the current once-through LWR fuel cycle.
Total energy input is calculated at 8.7 x 10(-3) GJ(e)/MWh(e) of electricity and 5.9 x 10(-3) GJ(t)/MWh(e) of thermal energy. It is dominated by the energy required for uranium extraction, conversion to fluoride compound for subsequent enrichment, and enrichment. An estimate of the carbon footprint is made from the direct energy consumption at 1.7 kg CO2/MWh(e). Water use is likewise dominated by requirements of uranium extraction, totaling 154 L/MWh(e). Land use is calculated at 8 x 10(-3) m(2)/MWh(e), over 90% of which is due to uranium extraction. Quantified impacts are limited to those resulting from activities performed within the FEFC process facilities (i.e. within the plant gates). Energy embodied in material inputs such as process chemicals and fuel cladding is identified but not explicitly quantified in this study. Inclusion of indirect energy associated with embodied energy as well as construction and decommissioning of facilities could increase the FEFC energy intensity estimate by a factor of up to 2. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Schneider, E.; Tavrides, E.; van der Hoeven, C.; Phathanapirom, U.] Univ Texas Austin, Nucl Engn Teaching Lab, Austin, TX 78758 USA.
[Carlsen, B.] Idaho Natl Lab, Idaho Falls, ID 83402 USA.
RP Schneider, E (reprint author), Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd,Bldg 159, Austin, TX 78758 USA.
EM eschneider@mail.utexas.edu
NR 55
TC 8
Z9 8
U1 2
U2 17
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0140-9883
EI 1873-6181
J9 ENERG ECON
JI Energy Econ.
PD NOV
PY 2013
VL 40
BP 898
EP 910
DI 10.1016/j.eneco.2013.01.002
PG 13
WC Economics
SC Business & Economics
GA 281DX
UT WOS:000329081300085
ER
PT J
AU Schneider, E
Carlsen, B
Tavrides, E
van der Hoeven, C
Phathanapirom, U
AF Schneider, E.
Carlsen, B.
Tavrides, E.
van der Hoeven, C.
Phathanapirom, U.
TI A top-down assessment of energy, water and land use in uranium mining,
milling, and refining
SO ENERGY ECONOMICS
LA English
DT Article
DE Uranium; Emissions; Environmental impacts
ID RESOURCES; SUSTAINABILITY
AB Land, water and energy use are key measures of the sustainability of uranium production into the future. As the most attractive, accessible deposits are mined out, future discoveries may prove to be significantly, perhaps unsustainably, more intensive consumers of environmental resources. A number of previous attempts have been made to provide empirical relationships connecting these environmental impact metrics to process variables such as stripping ratio and ore grade. These earlier attempts were often constrained by a lack of real world data and perform poorly when compared against data from modern operations. This paper conditions new empirical models of energy, water and land use in uranium mining, milling, and refining on contemporary data reported by operating mines. It shows that, at present, direct energy use from uranium production represents less than 1% of the electrical energy produced by the once-through fuel cycle. Projections of future energy intensity from uranium production are also possible by coupling the empirical models with estimates of uranium crustal abundance, characteristics of new discoveries, and demand. The projections show that even for the most pessimistic of scenarios considered, by 2100, the direct energy use from uranium production represents less than 3% of the electrical energy produced by the contemporary once-through fuel cycle. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Schneider, E.; Tavrides, E.; van der Hoeven, C.; Phathanapirom, U.] Univ Texas Austin, Nucl Engn Teaching Lab, Austin, TX 78758 USA.
[Carlsen, B.] Idaho Natl Lab, Idaho Falls, ID 83402 USA.
RP Schneider, E (reprint author), Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd,Bldg 159, Austin, TX 78758 USA.
EM eschneider@mail.utexas.edu
NR 38
TC 3
Z9 4
U1 2
U2 18
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0140-9883
EI 1873-6181
J9 ENERG ECON
JI Energy Econ.
PD NOV
PY 2013
VL 40
BP 911
EP 926
DI 10.1016/j.eneco.2013.08.006
PG 16
WC Economics
SC Business & Economics
GA 281DX
UT WOS:000329081300086
ER
PT J
AU Kaloni, TP
Balatsky, AV
Schwingenschlogl, U
AF Kaloni, T. P.
Balatsky, A. V.
Schwingenschloegl, U.
TI Substrate-enhanced superconductivity in Li-decorated graphene
SO EPL
LA English
DT Article
ID HEXAGONAL BORON-NITRIDE; STRONG-COUPLED SUPERCONDUCTORS;
TRANSITION-TEMPERATURE; ELECTRONIC-STRUCTURE; LAYER GRAPHENE; DENSITY;
DISPERSION; STATE
AB We investigate the role of the substrate for the strength of the electron-phonon coupling in Li-decorated graphene. We find that the interaction with a h-BN substrate leads to a significant enhancement from lambda(0) = 0.62 to lambda(1) = 0.67, which corresponds to a 25% increase of the transition temperature from T-c0 = 10.33K to T-c1 = 12.98 K. The superconducting gaps amount to 1.56 meV (suspended) and 1.98 meV (supported). These findings open up a new route to enhanced superconducting transition temperatures in graphene-based materials by substrate engineering. Copyright (C) EPLA, 2013
C1 [Kaloni, T. P.; Schwingenschloegl, U.] KAUST, PSE Div, Thuwal 239556900, Saudi Arabia.
[Balatsky, A. V.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Balatsky, A. V.] Los Alamos Natl Lab, Ctr Nanotechnol, Los Alamos, NM 87545 USA.
[Balatsky, A. V.] KTH Royal Inst Technol, NORDITA, SE-10691 Stockholm, Sweden.
[Balatsky, A. V.] Stockholm Univ, SE-10691 Stockholm, Sweden.
RP Kaloni, TP (reprint author), KAUST, PSE Div, Thuwal 239556900, Saudi Arabia.
EM udo.schwingenschlogl@kaust.edu.sa
OI Kaloni, Thaneshwor/0000-0001-9266-3482
FU US DOE; VR; [ERC-DM-321031]
FX We thank G. PROFETA for fruitful discussions. This work is supported by
US DOE, ERC-DM-321031, and VR.
NR 40
TC 21
Z9 21
U1 2
U2 30
PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY
PI MULHOUSE
PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE
SN 0295-5075
EI 1286-4854
J9 EPL-EUROPHYS LETT
JI EPL
PD NOV
PY 2013
VL 104
IS 4
AR 47013
DI 10.1209/0295-5075/104/47013
PG 6
WC Physics, Multidisciplinary
SC Physics
GA 278IL
UT WOS:000328882700027
ER
PT J
AU Udalov, OG
Glatz, A
Beloborodov, IS
AF Udalov, O. G.
Glatz, A.
Beloborodov, I. S.
TI Electron transport properties of composite ferroelectrics
SO EPL
LA English
DT Article
ID THIN-FILMS; NANOPARTICLES; CONDUCTIVITY; SYSTEMS; PHYSICS
AB We study electron transport in composite ferroelectrics -materials consisting of metallic grains embedded in a ferroelectric matrix. Due to its complex tunable morphology the thermodynamic properties of these materials can be essentially different from bulk or thin-film ferroelectrics. We calculate the conductivity of composite ferroelectrics by taking into account the interplay between charge localization, multiple grain boundaries, strong Coulomb repulsion, and ferroelectric order parameter. We show that the ferroelectricity plays a crucial role on the temperature behavior of the conductivity in the vicinity of the ferroelectric-paraelectric transition. Copyright (C) EPLA, 2013
C1 [Udalov, O. G.; Beloborodov, I. S.] Calif State Univ Northridge, Dept Phys & Astron, Northridge, CA 91330 USA.
[Udalov, O. G.] Russian Acad Sci, Inst Phys Microstruct, Nizhnii Novgorod 603950, Russia.
[Glatz, A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Glatz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.
RP Udalov, OG (reprint author), Calif State Univ Northridge, Dept Phys & Astron, Northridge, CA 91330 USA.
FU U.S. Department of Energy Office of Science [DE-AC02-06CH11357]; NSF
under Cooperative Agreement Award [EEC-1160504]; NSF PREM Award
[DMR-1234567]
FX We thank NIKOLAI CHTCHELKATCHEV and NICK KIOUSSIS for useful
discussions. AG was supported by the U.S. Department of Energy Office of
Science under the Contract No. DE-AC02-06CH11357. IB was supported by
NSF under Cooperative Agreement Award EEC-1160504 and NSF PREM Award
DMR-1234567.
NR 43
TC 4
Z9 4
U1 1
U2 12
PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY
PI MULHOUSE
PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE
SN 0295-5075
EI 1286-4854
J9 EPL-EUROPHYS LETT
JI EPL
PD NOV
PY 2013
VL 104
IS 4
AR 47004
DI 10.1209/0295-5075/104/47004
PG 6
WC Physics, Multidisciplinary
SC Physics
GA 278IL
UT WOS:000328882700018
ER
PT J
AU Smith, DP
Thrash, JC
Nicora, CD
Lipton, MS
Burnum-Johnson, KE
Carini, P
Smith, RD
Giovannoni, SJ
AF Smith, Daniel P.
Thrash, J. Cameron
Nicora, Carrie D.
Lipton, Mary S.
Burnum-Johnson, Kristin E.
Carini, Paul
Smith, Richard D.
Giovannoni, Stephen J.
TI Proteomic and Transcriptomic Analyses of "Candidatus Pelagibacter
ubique" Describe the First P-II-Independent Response to Nitrogen
Limitation in a Free-Living Alphaproteobacterium
SO MBIO
LA English
DT Article
ID EQUATORIAL PACIFIC-OCEAN; TROPICAL NORTH-ATLANTIC; AMMONIUM UPTAKE
SYSTEMS; ESCHERICHIA-COLI; NUTRIENT LIMITATION; GLUTAMINE-SYNTHETASE;
AZOSPIRILLUM-BRASILENSE; DESULFOVIBRIO-VULGARIS; ENRICHMENT EXPERIMENTS;
PHOSPHORUS LIMITATION
AB Nitrogen is one of the major nutrients limiting microbial productivity in the ocean, and as a result, most marine microorganisms have evolved systems for responding to nitrogen stress. The highly abundant alphaproteobacterium "Candidatus Pelagibacter ubique," a cultured member of the order Pelagibacterales (SAR11), lacks the canonical GlnB, GlnD, GlnK, and NtrB/NtrC genes for regulating nitrogen assimilation, raising questions about how these organisms respond to nitrogen limitation. A survey of 266 Alphaproteobacteria genomes found these five regulatory genes nearly universally conserved, absent only in intracellular parasites and members of the order Pelagibacterales, including "Ca. Pelagibacter ubique." Global differences in mRNA and protein expression between nitrogen-limited and nitrogen-replete cultures were measured to identify nitrogen stress responses in "Ca. Pelagibacter ubique" strain HTCC1062. Transporters for ammonium (AmtB), taurine (TauA), amino acids (YhdW), and opines (OccT) were all elevated in nitrogen-limited cells, indicating that they devote increased resources to the assimilation of nitrogenous organic compounds. Enzymes for assimilating amine into glutamine (GlnA), glutamate (GltBD), and glycine (AspC) were similarly upregulated. Differential regulation of the transcriptional regulator NtrX in the two-component signaling system NtrY/NtrX was also observed, implicating it in control of the nitrogen starvation response. Comparisons of the transcriptome and proteome supported previous observations of uncoupling between transcription and translation in nutrient-deprived "Ca. Pelagibacter ubique" cells. Overall, these data reveal a streamlined, P-II-independent response to nitrogen stress in "Ca. Pelagibacter ubique," and likely other Pelagibacterales, and show that they respond to nitrogen stress by allocating more resources to the assimilation of nitrogen-rich organic compounds.
IMPORTANCE Pelagibacterales are extraordinarily abundant and play a pivotal role in marine geochemical cycles, as one of the major recyclers of labile dissolved organic matter. They are also models for understanding how streamlining selection can reshape chemoheterotroph metabolism. Streamlining and its broad importance to environmental microbiology are emerging slowly from studies that reveal the complete genomes of uncultured organisms. Here, we report another remarkable example of streamlined metabolism in Pelagibacterales, this time in systems that control nitrogen assimilation. Pelagibacterales are major contributors to metatranscriptomes and metaproteomes from ocean systems, where patterns of gene expression are used to gain insight into ocean conditions and geochemical cycles. The data presented here supply background that is essential to interpreting data from field studies.
C1 [Smith, Daniel P.; Thrash, J. Cameron; Carini, Paul; Giovannoni, Stephen J.] Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA.
[Nicora, Carrie D.; Lipton, Mary S.; Burnum-Johnson, Kristin E.; Smith, Richard D.] Pacific NW Natl Lab, Biol & Computat Sci Div, Richland, WA 99352 USA.
RP Giovannoni, SJ (reprint author), Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA.
EM steve.giovannoni@oregonstate.edu
RI Smith, Richard/J-3664-2012; Burnum, Kristin/B-1308-2011; Carini,
Paul/H-8279-2014; Lipton, Mary/H-3913-2012;
OI Smith, Richard/0000-0002-2381-2349; Burnum, Kristin/0000-0002-2722-4149;
Carini, Paul/0000-0002-9653-7309; Thrash, Cameron/0000-0003-0896-9986
FU Gordon and Betty Moore Foundation; National Science Foundation
[DBI-1003269]; DOE [DE-AC05-76RL01830]
FX This study was supported by a Marine Microbiology Initiative
investigator award (S.J.G.) from the Gordon and Betty Moore Foundation.
The phylogenomics portions of this work (J.C.T.) were supported by the
National Science Foundation under award no. DBI-1003269. Proteomics
measurements were supported by the U.S. Department of Energy (DOE)
Office of Biological and Environmental Research (OBER) Pan-omics program
at Pacific Northwest National Laboratory (PNNL) and performed in the
Environmental Molecular Sciences Laboratory, a DOE OBER national
scientific user facility on the PNNL campus. PNNL is a multiprogram
national laboratory operated by Battelle for the DOE under contract
DE-AC05-76RL01830.
NR 107
TC 8
Z9 9
U1 2
U2 25
PU AMER SOC MICROBIOLOGY
PI WASHINGTON
PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA
SN 2150-7511
J9 MBIO
JI mBio
PD NOV-DEC
PY 2013
VL 4
IS 6
AR e00133-12
DI 10.1128/mBio.00133-12
PG 14
WC Microbiology
SC Microbiology
GA 282LZ
UT WOS:000329174500001
PM 24281717
ER
PT J
AU Iacovides, DC
Johnson, AB
Wang, N
Boddapati, S
Korkola, J
Gray, JW
AF Iacovides, Demetris C.
Johnson, Aimee B.
Wang, Nick
Boddapati, Shanta
Korkola, Jim
Gray, Joe W.
TI Identification and Quantification of AKT Isoforms and Phosphoforms in
Breast Cancer Using a Novel Nanofluidic Immunoassay
SO MOLECULAR & CELLULAR PROTEOMICS
LA English
DT Article
ID PROTEIN-KINASE B; CELL LUNG-CANCER; SIGNALING PATHWAY; PI3K PATHWAY;
ACTIVATION; AKT/PKB; PHOSPHORYLATION; OVEREXPRESSION; AMPLIFICATION;
INHIBITION
AB Breast cancer subtype-specific molecular variations can dramatically affect patient responses to existing therapies. It is thought that differentially phosphorylated protein isoforms might be a useful prognostic biomarker of drug response in the clinic. However, the accurate detection and quantitative analysis of cancer-related protein isoforms and phospho-isoforms in tumors are limited by current technologies. Using a novel, fully automated nanocapillary electrophoresis immunoassay (NanoPro(TM) 1000) designed to separate protein molecules based on their isoelectric point, we developed a reliable and highly sensitive assay for the detection and quantitation of AKT isoforms and phosphoforms in breast cancer. This assay enabled the measurement of activated AKT1/2/3 in breast cancer cells using protein produced from as few as 56 cells. Importantly, we were able to assign an identity for the phosphorylated S473 phosphoform of AKT1, the major form of activated AKT involved in multiple cancers, including breast, and a current focus in clinical trials for targeted intervention. The ability of our AKT assay to detect and measure AKT phosphorylation from very low amounts of total protein will allow the accurate evaluation of patient response to drugs targeting activated PI3K-AKT using scarce clinical specimens. Moreover, the capacity of this assay to detect and measure all three AKT isoforms using one single pan-specific antibody enables the study of the multiple and variable roles that these isoforms play in AKT tumorigenesis. Molecular & Cellular Proteomics 12: 10.1074/mcp.M112.023119, 3210-3220, 2013.
C1 [Iacovides, Demetris C.; Johnson, Aimee B.; Wang, Nick; Korkola, Jim; Gray, Joe W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
RP Gray, JW (reprint author), 3303 SW Bond Ave,Mail Code CH13B, Portland, OR 97239 USA.
EM grayjo@ohsu.edu
FU Office of Science, Office of Biological & Environmental Research, of the
U.S. Department of Energy [DE-AC02-05CH11231]; NCI, National Institutes
of Health [P50 CA 58207, U54 CA 112970, U24 CA 126477]; Susan G. Komen
Foundation [SAC110012]; SmithKline Beecham Corporation
FX This work was supported by the Director, Office of Science, Office of
Biological & Environmental Research, of the U.S. Department of Energy
under Contract No. DE-AC02-05CH11231; by the NCI, National Institutes of
Health (Grant Nos. P50 CA 58207, U54 CA 112970, and U24 CA 126477 to
J.W.G.); by the Susan G. Komen Foundation (SAC110012 to D. C. I. and
J.W.G.); and by a SmithKline Beecham Corporation grant to J.W.G.
NR 32
TC 14
Z9 14
U1 1
U2 16
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 1535-9476
EI 1535-9484
J9 MOL CELL PROTEOMICS
JI Mol. Cell. Proteomics
PD NOV
PY 2013
VL 12
IS 11
BP 3210
EP 3220
DI 10.1074/mcp.M112.023119
PG 11
WC Biochemical Research Methods
SC Biochemistry & Molecular Biology
GA 277JX
UT WOS:000328816000015
PM 23929892
ER
PT J
AU Nakayasu, ES
Tempel, R
Cambronne, XA
Petyuk, VA
Jones, MB
Gritsenko, MA
Monroe, ME
Yang, F
Smith, RD
Adkins, JN
Heffron, F
AF Nakayasu, Ernesto S.
Tempel, Rebecca
Cambronne, Xiaolu A.
Petyuk, Vladislav A.
Jones, Marcus B.
Gritsenko, Marina A.
Monroe, Matthew E.
Yang, Feng
Smith, Richard D.
Adkins, Joshua N.
Heffron, Fred
TI Comparative Phosphoproteomics Reveals Components of Host Cell Invasion
and Post-transcriptional Regulation During Francisella Infection
SO MOLECULAR & CELLULAR PROTEOMICS
LA English
DT Article
ID TANDEM MASS-SPECTRA; LIVE VACCINE STRAIN; TOLL-LIKE RECEPTORS; AIM2
INFLAMMASOME; MESSENGER-RNA; MURINE MACROPHAGES; IN-VITRO; TULARENSIS;
TRISTETRAPROLIN; APOPTOSIS
AB Francisella tularensis is a facultative intracellular bacterium that causes the deadly disease tularemia. Most evidence suggests that Francisella is not well recognized by the innate immune system that normally leads to cytokine expression and cell death. In previous work, we identified new bacterial factors that were hyper-cytotoxic to macrophages. Four of the identified hyper-cytotoxic strains (lpcC, manB, manC, and kdtA) had an impaired lipopolysaccharide (LPS) synthesis and produced an exposed lipid A lacking the O-antigen. These mutants were not only hyper-cytotoxic but also were phagocytosed at much higher rates compared with the wild type parent strain. To elucidate the cellular signaling underlying this enhanced phagocytosis and cell death, we performed a large-scale comparative phosphoproteomic analysis of cells infected with wild-type and delta-lpcC F. novicida. Our data suggest that not only actin but also intermediate filaments and microtubules are important for F. novicida entry into the host cells. In addition, we observed differential phosphorylation of tristetraprolin, a key component of the mRNA-degrading machinery that controls the expression of a variety of genes including many cytokines. Infection with the delta-lpcC mutant induced the hyper-phosphorylation and inhibition of tristetraprolin, leading to the production of cytokines such as IL-1beta and TNF-alpha that may kill the host cells by triggering apoptosis. Together, our data provide new insights for Francisella invasion and a post-transcriptional mechanism that prevents the expression of host immune response factors that control infection by this pathogen.
C1 [Nakayasu, Ernesto S.; Petyuk, Vladislav A.; Gritsenko, Marina A.; Monroe, Matthew E.; Yang, Feng; Smith, Richard D.; Adkins, Joshua N.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.
[Tempel, Rebecca; Heffron, Fred] Oregon Hlth & Sci Univ, Dept Mol Microbiol & Immunol, Portland, OR 97239 USA.
[Cambronne, Xiaolu A.] Oregon Hlth & Sci Univ, Vollum Inst, Portland, OR 97239 USA.
[Jones, Marcus B.] J Craig Venter Inst, Pathogen Funct Genom Resource Ctr, Rockville, MD USA.
RP Tempel, R (reprint author), Oregon Hlth & Sci Univ, Dept Mol Microbiol & Immunol, L220,3181 SW Sam Jackson Pk Rd, Portland, OR 97239 USA.
EM tempelr@ohsu.edu
RI Smith, Richard/J-3664-2012;
OI Smith, Richard/0000-0002-2381-2349; Cambronne, Lulu/0000-0002-3547-448X;
Petyuk, Vladislav/0000-0003-4076-151X
FU National Institute of Allergy and Infectious Diseases (NIH/DHHS)
[Y1-AI-4894-01]; National Institute for General Medicine [GM094623]; NIH
[5P41RR018522-10, NS076094]; National Institute of General Medical
Sciences [8 P41 GM103493-10]; U.S. Department of Energy Office of
Biological and Environmental Research (DOE/BER); DOE by Battelle
[DE-AC05-76RLO1830]
FX This work was supported by the National Institute of Allergy and
Infectious Diseases (NIH/DHHS through interagency agreement
Y1-AI-4894-01; project website www.SysBEP.org) and the National
Institute for General Medicine (GM094623). This work used
instrumentation and capabilities developed with support from the NIH
grant 5P41RR018522-10, the National Institute of General Medical
Sciences grant 8 P41 GM103493-10, and the U.S. Department of Energy
Office of Biological and Environmental Research (DOE/BER). Significant
portions of this work were performed in the EMSL, a DOE/BER national
scientific user facility located at Pacific Northwest National
Laboratory. The Pacific Northwest National Laboratory is operated for
the DOE by Battelle under Contract DE-AC05-76RLO1830. This work was also
supported by the NIH award NS076094 to X.A.C.
NR 63
TC 5
Z9 5
U1 1
U2 7
PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC
PI BETHESDA
PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA
SN 1535-9476
EI 1535-9484
J9 MOL CELL PROTEOMICS
JI Mol. Cell. Proteomics
PD NOV
PY 2013
VL 12
IS 11
BP 3297
EP 3309
DI 10.1074/mcp.M113.029850
PG 13
WC Biochemical Research Methods
SC Biochemistry & Molecular Biology
GA 277JX
UT WOS:000328816000021
PM 23970565
ER
PT J
AU Miller, MC
Vega, DA
AF Miller, M. C.
Vega, D. A.
TI US FUEL CYCLE TECHNOLOGIES R&D PROGRAM FOR NEXT GENERATION NUCLEAR
MATERIALS MANAGEMENT
SO NUCLEAR ENGINEERING AND TECHNOLOGY
LA English
DT Article
DE Nuclear Safeguards; Nuclear Material Control and Accountancy; Neutron
Detection; Gamma-ray Spectroscopy; Process Monitoring; Nuclear Material
Management
AB The U.S. Department of Energy's Fuel Cycle Technologies R&D program under the Office of Nuclear Energy is working to advance technologies to enhance both the existing and future fuel cycles. One thrust area is in developing enabling technologies for next generation nuclear materials management under the Materials Protection, Accounting and Control Technologies (MPACT) Campaign where advanced instrumentation, analysis and assessment methods, and security approaches are being developed under a framework of Safeguards and Security by Design. An overview of the MPACT campaign's activities and recent accomplishments is presented along with future plans.
C1 [Miller, M. C.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
[Vega, D. A.] US DOE, Off Nucl Energy, Germantown, MD 20874 USA.
RP Miller, MC (reprint author), Los Alamos Natl Lab, POB 1663 MS H816, Los Alamos, NM 87544 USA.
EM mmiller@lanl.gov
FU U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle
Technologies RD Program
FX The U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle
Technologies R&D Program supports the MPACT Campaign.
NR 24
TC 0
Z9 0
U1 1
U2 7
PU KOREAN NUCLEAR SOC
PI DAEJEON
PA NUTOPIA BLDG, 342-1 JANGDAE-DONG, DAEJEON, 305-308, SOUTH KOREA
SN 1738-5733
J9 NUCL ENG TECHNOL
JI Nucl. Eng. Technol.
PD NOV
PY 2013
VL 45
IS 6
SI SI
BP 803
EP 810
DI 10.5516/NET.02.2013.527
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 278XD
UT WOS:000328922300012
ER
PT J
AU Hughes, AM
Pozzi, ECC
Thorp, S
Garabalino, MA
Farias, RO
Gonzalez, SJ
Heber, EM
Itoiz, ME
Aromando, RF
Molinari, AJ
Miller, M
Nigg, DW
Curotto, P
Trivillin, VA
Schwint, AE
AF Monti Hughes, A.
Pozzi, E. C. C.
Thorp, S.
Garabalino, M. A.
Farias, R. O.
Gonzalez, S. J.
Heber, E. M.
Itoiz, M. E.
Aromando, R. F.
Molinari, A. J.
Miller, M.
Nigg, D. W.
Curotto, P.
Trivillin, V. A.
Schwint, A. E.
TI Boron neutron capture therapy for oral precancer: proof of principle in
an experimental animal model
SO ORAL DISEASES
LA English
DT Article
DE boron neutron capture therapy; hamster cheek pouch oral precancer model;
field cancerization; precancerous conditions; oral cancer
ID HAMSTER-CHEEK POUCH; RECURRENT HEAD; NECK-CANCER; CLINICAL-IMPLICATIONS;
FIELD CANCERIZATION; BNCT; MALIGNANCIES; TUMORS; BORONOPHENYLALANINE;
RADIOBIOLOGY
AB ObjectivesField-cancerized tissue can give rise to second primary tumours, causing therapeutic failure. Boron neutron capture therapy (BNCT) is based on biological targeting and would serve to treat undetectable foci of malignant transformation. The aim of this study was to optimize BNCT for the integral treatment for oral cancer, with particular emphasis on the inhibitory effect on tumour development originating in precancerous conditions, and radiotoxicity of different BNCT protocols in a hamster cheek pouch oral precancer model.
Materials and MethodsGroups of cancerized hamsters were locally exposed to single or double (2 or 4weeks apart) applications of BNCT at different dose levels, mediated by the boron compounds boronophenylalanine (BPA) or BPA and decahydrodecaborate (GB-10) administered jointly. Cancerized, sham-irradiated hamsters served as controls. Clinical status, tumour development from field-cancerized tissue and mucositis were followed for 8months.
ResultsA double application (4weeks apart) of BNCT mediated by GB-10+ BPA at a total dose of 10Gy in two 5-Gy doses rendered the best therapeutic advantage (63-100% inhibition of tumour development from field-cancerized tissue), minimizing dose-limiting mucositis.
ConclusionBNCT can be optimized for the integral treatment for head and neck cancer, considering the implications for field-cancerized tissue.
C1 [Monti Hughes, A.; Pozzi, E. C. C.; Garabalino, M. A.; Heber, E. M.; Itoiz, M. E.; Aromando, R. F.; Molinari, A. J.; Trivillin, V. A.; Schwint, A. E.] CNEA, Dept Radiobiol, San Martin, Argentina.
[Pozzi, E. C. C.; Curotto, P.] CNEA, Dept Res & Prod Reactors, Ezeiza, Argentina.
[Thorp, S.; Farias, R. O.; Gonzalez, S. J.; Miller, M.] CNEA, Dept Technol & Applicat Accelerators, Ezeiza, Argentina.
[Gonzalez, S. J.; Trivillin, V. A.; Schwint, A. E.] Consejo Nacl Invest Cient & Tecn, Natl Res Council, Caba, Argentina.
[Itoiz, M. E.; Aromando, R. F.] Univ Buenos Aires, Dept Oral Pathol, Fac Dent, Caba, Argentina.
[Nigg, D. W.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Schwint, AE (reprint author), CNEA, Radiat Pathol Div, Dept Radiobiol, Ave Gen Paz 1499,B1650KNA, Buenos Aires, DF, Argentina.
EM schwint@cnea.gov.ar
FU Agencia Nacional de Promocion Cientifica y Tecnologica (ANPCyT); Consejo
Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Argentina
FX The work was partially funded by grants from Agencia Nacional de
Promocion Cientifica y Tecnologica (ANPCyT) and Consejo Nacional de
Investigaciones Cientificas y Tecnicas (CONICET), Argentina, and
supported in-kind by Department of Energy (DOE) through Idaho National
Laboratory (INL), USA.
NR 46
TC 6
Z9 6
U1 0
U2 3
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1354-523X
EI 1601-0825
J9 ORAL DIS
JI Oral Dis.
PD NOV
PY 2013
VL 19
IS 8
BP 789
EP 795
DI 10.1111/odi.12077
PG 7
WC Dentistry, Oral Surgery & Medicine
SC Dentistry, Oral Surgery & Medicine
GA 283DH
UT WOS:000329224800006
ER
PT J
AU Chatrchyan, S
Khachatryan, V
Sirunyan, AM
Tumasyan, A
Adam, W
Bergauer, T
Dragicevic, M
Ero, J
Fabjan, C
Friedl, M
Fruhwirth, R
Ghete, VM
Hormann, N
Hrubec, J
Jeitler, M
Kiesenhofer, W
Knunz, V
Krammer, M
Kratschmer, I
Liko, D
Mikulec, I
Rabady, D
Rahbaran, B
Rohringer, C
Rohringer, H
Schofbeck, R
Strauss, J
Taurok, A
Treberer-Treberspurg, W
Waltenberger, W
Wulz, CE
Mossolov, V
Shumeiko, N
Gonzalez, JS
Alderweireldt, S
Bansal, M
Bansal, S
Cornelis, T
De Wolf, EA
Janssen, X
Knutsson, A
Luyckx, S
Mucibello, L
Ochesanu, S
Roland, B
Rougny, R
Staykova, Z
Van Haevermaet, H
Van Mechelen, R
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CA CMS Collaboration
TI Search for a new bottomonium state decaying to Upsilon(1S)pi(+)pi(-) in
pp collisions at root s=8 TeV
SO PHYSICS LETTERS B
LA English
DT Article
DE CMS; Physics; Exotic quarkonia
ID TETRAQUARKS; MODEL
AB The results of a search for the bottomonium counterpart, denoted as X-b, of the exotic charmonium state X(3872) is presented. The analysis is based on a sample of pp collisions at,root s = 8 TeV collected by the CMS experiment at the LHC, corresponding to an integrated luminosity of 20.7 fb(-1). The search looks for the exclusive decay channel X-b -> Upsilon(1S)pi(+)pi(-) followed by Upsilon(1S) -> mu(+)mu(-). No evidence for an X-b signal is observed. Upper limits are set at the 95% confidence level on the ratio of the inclusive production cross sections times the branching fractions to Upsilon(1S)pi(+)pi(-) of the X-b and the Upsilon(2S). The upper limits on the ratio are in the range 0.9-5.4% for X-b masses between 10 and 11 GeV. These are the first upper limits on the production of a possible X-b at a hadron collider. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved.
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[Blekman, F.; Blyweert, S.; D'Hondt, J.; Kalogeropoulos, A.; Keaveney, J.; Lowette, S.; Maes, M.; Olbrechts, A.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium.
[Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium.
[Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium.
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[Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Awad, A. M. Kuotb; Mahmoud, M. A.; Radi, A.] Egyptian Network High Energy Phys, Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt.
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[Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland.
[Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland.
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[Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany.
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[Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany.
[Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Kornmayer, A.; Pardo, P. Lobelle; Martschei, D.; Mozer, M. U.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Schilling, F. -R; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany.
[Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Topsis-giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece.
[Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece.
[Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece.
[Bencze, G.; Hajdu, C.; Hidas, R.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary.
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[Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India.
[Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India.
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[Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland.
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[Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy.
[Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy.
[Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, R.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy.
[Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, R.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy.
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[Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy.
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[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy.
[Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy.
[Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robtitti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy.
[Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy.
[Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, R.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy.
[Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, R.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy.
[Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy.
[De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy.
[Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy.
[Meola, S.] Univ G Marconi Roma, Naples, Italy.
[Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Fantinel, S.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Maron, G.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy.
[Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy.
[Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy.
[Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Pioppi, M.] INFN Sez Perugia, Perugia, Italy.
[Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy.
[Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, R.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy.
[Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy.
[Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy.
[Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Michell, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] INFN Sez Roma, Rome, Italy.
[Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Michell, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy.
[Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy.
[Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy.
[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy.
[Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy.
[Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy.
[Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea.
[Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea.
[Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea.
[Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea.
[Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea.
[Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea.
[Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania.
[Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico.
[Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico.
[Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico.
[Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico.
[Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand.
[Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand.
[Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan.
[Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland.
[Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland.
[Almeida, N.; Bargassa, R.; Beirao Da Cruz E Silva, C.; Faccioli, R.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, R.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal.
[Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia.
[Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia.
[Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Starodumov, A.; Nikitenko, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia.
[Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia.
[Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia.
[Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Penis, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Fernando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain.
[Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain.
[Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain.
[Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain.
[Rabady, D.; Genchev, V.; Iaydjiev, P.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Giordano, E.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Meola, S.; Paolucci, P.; Galanti, M.; D'Agnolo, R. T.; Pelliccioni, M.; Cossutti, F.; Seixas, J.; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stieger, B.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland.
[Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland.
[Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland.
[Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland.
[Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan.
[Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.; Chen, P. -H.; Tao, C. -Y.; Wang, T. -W.] NTU, Taipei, Taiwan.
[Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand.
[Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey.
[Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey.
[Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey.
[Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey.
[Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine.
[Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England.
[Worm, S. D.; Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Ilic, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England.
[Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England.
[Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA.
[Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA.
[Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA.
[Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA.
[Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA.
[Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA.
[Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA.
[Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA.
[Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA.
[Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA.
[Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA.
[Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA.
[Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA.
[Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA.
[Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA.
[Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA.
[Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA.
[Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA.
[Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, E.; Sen, S.; Tan, R.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA.
[Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA.
[Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA.
[Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA.
[Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA.
[Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA.
[Dahmes, B.; De Benedetti, A.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA.
[Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA.
[Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA.
[Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA.
[Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA.
[Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA.
[Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA.
[Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA.
[Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA.
[Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA.
[Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA.
[Parashar, N.] Purdue Univ Calumet, Hammond, LA USA.
[Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA.
[Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA.
[Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA.
[Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA.
[Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA.
[Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA.
[Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA.
[Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA.
[Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA.
[Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA.
[Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA.
[Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria.
[Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil.
[Dias, F. A.; Dubinin, M.] CALTECH, Pasadena, CA 91125 USA.
[Assran, Y.] Suez Canal Univ, Suez, Egypt.
[Elgammal, S.] Zewail City Sci & Technol, Zewail, Egypt.
[Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt.
[Awad, A. M. Kuotb; Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt.
[Radi, A.] British Univ Egypt, Cairo, Egypt.
[Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France.
[Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany.
[Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary.
[Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India.
[Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka.
[Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran.
[Fahim, A.] Sharif Univ Technol, Tehran, Iran.
[Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran.
[Gulmini, M.; Maron, G.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy.
[Androsov, K.; Grippo, M. T.; Martini, L.] Univ Siena, I-53100 Siena, Italy.
[Moon, C. S.] CNRS, IN2P3, Paris, France.
[Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico.
[Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy.
[Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy.
[Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland.
[Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey.
[Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey.
[Onengut, G.] Cag Univ, Mersin, Turkey.
[Sogut, K.] Mersin Univ, Mersin, Turkey.
[Karapinar, G.] Izmir Inst Technol, Izmir, Turkey.
[Isildak, B.] Ozyegin Univ, Istanbul, Turkey.
[Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey.
[Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey.
[Sonmez, N.] Ege Univ, Izmir, Turkey.
[Gunaydin, Y. O.] Mimar Sinan Univ, Istanbul, Turkey.
[Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, Kahramanmaras, Turkey.
[Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England.
[Wasserbaech, S.] Utah Valley Univ, Orem, UT USA.
[Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey.
[Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey.
[Bouhali, O.] Texas A&M Univ, Doha, Qatar.
[Kamon, T.] Kyungpook Natl Univ, Taegu 702701, South Korea.
RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia.
RI Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh,
Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni,
Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014;
Inst. of Physics, Gleb Wataghin/A-9780-2017; Tomei, Thiago/E-7091-2012;
Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan,
Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre
David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder,
Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim,
Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Codispoti,
Giuseppe/F-6574-2014; Bellan, Riccardo/G-2139-2014; Petrushanko,
Sergey/D-6880-2012; da Cruz e Silva, Cristovao/K-7229-2013; Marlow,
Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen,
Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini,
Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Ligabue,
Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko,
Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Montanari,
Alessandro/J-2420-2012; Moon, Chang-Seong/J-3619-2014; Gribushin,
Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Venturi,
Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; de la Cruz,
Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa,
Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat
Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini,
Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson,
Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014;
Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Dahms,
Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Chinellato, Jose
Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal,
Martti/F-4436-2012; Sen, Sercan/C-6473-2014; D'Alessandro,
Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl,
Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki,
Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; ciocci,
maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My,
Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Lo Vetere,
Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Rovelli,
Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani,
Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev,
Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae
Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012;
Della Ricca, Giuseppe/B-6826-2013
OI Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh,
Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni,
Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan,
Efe/0000-0001-5732-7950; Tomei, Thiago/0000-0002-1809-5226; Dubinin,
Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X;
Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre
David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626;
Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo
Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad,
Wael/0000-0003-1491-0446; Codispoti, Giuseppe/0000-0003-0217-7021; de
Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes,
Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz,
Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192;
Montanari, Alessandro/0000-0003-2748-6373; Moon,
Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691;
Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo,
Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787;
Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731;
Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155;
Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070;
Chinellato, Jose Augusto/0000-0002-3240-6270; Sen,
Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306;
Belyaev, Alexander/0000-0002-1733-4408; Stahl,
Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279;
Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose
Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462;
Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680;
Matorras, Francisco/0000-0003-4295-5668; Lo Vetere,
Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074;
Rovelli, Tiziano/0000-0002-9746-4842; TUVE',
Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix,
Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982
FU BMWF; FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP
(Brazil); MEYS (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS
(Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF
(Estonia); Academy of Finland; MEC; HIP (Finland); CEA; CNRS/IN2P3
(France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NKTH (Hungary);
DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU
(Republic of Korea); LAS (Lithuania); CINVESTAV; CONACYT; SEP; UASLP-FAI
(Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE; NSC (Poland); FCT
(Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON;
RosAtom; RAS; RFBR (Russia); MESTD (Serbia); SEIDI; CPAN (Spain); Swiss
Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter; IPST; NSTDA
(Thailand); TUBITAK; TAEK (Turkey); NASU (Ukraine); STFC (United
Kingdom); DOE; NSF (USA); Marie-Curie programme; European Research
Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan
Foundation; Alexander von Humboldt Foundation; Belgian Federal Science
Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie
et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door
Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth
and Sports (MEYS) of Czech Republic; Council of Science and Industrial
Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme
of Foundation for Polish Science; EU, Regional Development Fund; Thalis
and Aristeia programmes; EU-ESF; Greek NSRF
FX We congratulate our colleagues in the CERN accelerator departments for
the excellent performance of the LHC and thank the technical and
administrative staffs at CERN and at other CMS institutes for their
contributions to the success of the CMS effort. In addition, we
gratefully acknowledge the computing centres and personnel of the
Worldwide LHC Computing Grid for delivering so effectively the computing
infrastructure essential to our analyses. Finally, we acknowledge the
enduring support for the construction and operation of the LHC and the
CMS detector provided by the following funding agencies: BMWF and FWF
(Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP
(Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China);
COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09
and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and
CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA
and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN
(Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV,
CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC
(Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia,
Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR
(Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies
(Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand);
TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE
and NSF (USA).; Individuals have received support from the Marie-Curie
programme and the European Research Council and EPLANET (European
Union); the Leventis Foundation; the A.P. Sloan Foundation; the
Alexander von Humboldt Foundation; the Belgian Federal Science Policy
Office; the Fonds pour la Formation a la Recherche dans l'Industrie et
dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door
Wetenschap en Technologie (IWT-Belgium); the Ministry of Education,
Youth and Sports (MEYS) of Czech Republic; the Council of Science and
Industrial Research, India; the Compagnia di San Paolo (Torino); the
HOMING PLUS programme of Foundation for Polish Science, cofinanced by
EU, Regional Development Fund; and the Thalis and Aristeia programmes
cofinanced by EU-ESF and the Greek NSRF.
NR 33
TC 19
Z9 21
U1 5
U2 67
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 57
EP 76
DI 10.1016/j.physletb.2013.10.016
PG 20
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400009
ER
PT J
AU Chatrchyan, S
Khachatryan, V
Sirunyan, AM
Tumasyan, A
Adam, W
Bergauer, T
Dragicevic, M
Ero, J
Fabjan, C
Friedl, M
Fruhwirth, R
Ghete, VM
Hormann, N
Hrubec, J
Jeitler, M
Kiesenhofer, W
Kuinz, V
Krammer, M
Kratschmer, I
Liko, D
Mikulec, I
Rabady, D
Rahbaran, B
Rohringer, C
Rohringer, H
Schofbeck, R
Strauss, J
Taurok, A
Treberer-Treberspurg, W
Waltenberger, W
Wulz, CE
Mossolov, V
Shumeiko, N
Gonzalez, JS
Alderweireldt, S
Bansal, M
Bansal, S
Cornelis, T
De Wolf, EA
Janssen, X
Knutsson, A
Luyckx, S
Mucibello, L
Ochesanu, S
Roland, B
Rougny, R
Staykova, Z
Van Haevermaet, H
Van Mechelen, R
Van Remortel, N
Van Spilbeeck, A
Blekman, F
Blyweert, S
D'Hondt, J
Kalogeropoulos, A
Keaveney, J
Maes, M
Olbrechts, A
Tavernier, S
Van Doninck, W
Van Mulders, P
Van Onsem, GP
Villella, I
Caillol, C
Clerbaux, B
De Lentdecker, G
Favart, L
Gay, APR
Hreus, T
Leonard, A
Marage, PE
Mohammadi, A
Pernie, L
Reis, T
Seva, T
Thomas, L
Velde, CV
Vanlaer, R
Wang, J
Adler, V
Beernaert, K
Benucci, L
Cimmino, A
Costantini, S
Dildick, S
Garcia, G
Klein, B
Lellouch, J
Marinov, A
Mccartin, J
Rios, AAO
Ryckbosch, D
Sigamani, M
Strobbe, N
Thyssen, E
Tytgat, M
Walsh, S
Yazgan, E
Zaganidis, N
Basegmez, S
Beluffi, C
Bruno, G
Castello, R
Caudron, A
Ceard, L
Da Silveira, GG
Delaere, C
du Pree, T
Favart, D
Forthomme, L
Giammanco, A
Hollar, J
Jez, R
Lemaitre, V
Liao, J
Militaru, O
Nuttens, C
Pagano, D
Pin, A
Piotrzkowski, K
Popov, A
Selvaggi, M
Garcia, JMV
Beliy, N
Caebergs, T
Daubie, E
Hammad, GH
Alves, GA
Martins, MCM
Martins, T
Pol, ME
Souza, MHG
Alda, WL
Carvalho, W
Chinellato, J
Custodio, A
Da Costa, EM
Damiao, DD
Martins, CD
De Souza, SF
Malbouisson, H
Malek, M
Figueiredo, DM
Mundim, L
Nogima, H
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CA CMS Collaboration
TI Angular analysis and branching fraction measurement of the decay B-0 ->
K*(0)mu(+)mu(-)
SO PHYSICS LETTERS B
LA English
DT Article
DE CMS; Physics
ID PHYSICS; MODEL
AB The angular distributions and the differential branching fraction of the decay B-0 -> K*(892)(0)mu(+)mu(-) are studied using a data sample corresponding to an integrated luminosity of 5.2 fb(-1) collected with the CMS detector at the LHC in pp collisions at root s = 7 TeV. From more than 400 signal decays, the forward-backward asymmetry of the muons, the K*(892)(0) longitudinal polarization fraction, and the differential branching fraction are determined as a function of the square of the dimuon invariant mass. The measurements are in good agreement with standard model predictions. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved.
C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; CMS Collaboration] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Kueinz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria.
[Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus.
[Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Staykova, Z.; Van Haevermaet, H.; Van Mechelen, R.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium.
[Blekman, F.; Blyweert, S.; D'Hondt, J.; Kalogeropoulos, A.; Keaveney, J.; Maes, M.; Olbrechts, A.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium.
[Chatrchyan, S.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Pernie, L.; Reis, T.; Seva, T.; Thomas, L.; Velde, C. Vander; Vanlaer, R.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium.
[Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, E.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium.
[Chatrchyan, S.; Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jez, R.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Selvaggi, M.; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium.
[Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium.
[Chatrchyan, S.; Alves, G. A.; Correa Martins Junior, M.; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil.
[Alderweireldt, S.; Caudron, A.; Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil.
[Dias, F. A.; Fernandez Perez Tomei, T. R.; Lagana, C.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil.
[Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil.
[Genchev, V.; Iaydjiev, R.; Piperov, S.; Rodozov, M.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria.
[Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, R.] Univ Sofia, BU-1126 Sofia, Bulgaria.
[Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, X.; Wang, Z.; Xiao, H.] Inst High Energy Phys, Beijing 100039, Peoples R China.
[Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Teng, H.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.
[Avila, C.; Montoya, C. A. Carrillo; Sierra, L. F. Chaparro; Gomez, J. P.; Moreno, B. Gomez; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia.
[Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia.
[Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia.
[Brigljevic, V.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia.
[Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, E.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus.
[Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic.
[Abdelalim, A. A.; Assran, Y.; Elgammal, S.; Kamer, A. Ellithi; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt.
[Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia.
[Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland.
[Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland.
[Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland.
[Besancon, M.; Couderc, E.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, R.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France.
[Baffioni, S.; Beaudette, F.; Benhabib, L.; Bluj, M.; Busson, R.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France.
[Agram, J. -L.; Andrea, J.; Bloch, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, R.; Le Bihan, A. -C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France.
[Gadrat, S.] CNRS, IN2P3, Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France.
[Giammanco, A.; Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.] Univ Lyon 1, Univ Lyon, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France.
[Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Inform, GE-380086 Tbilisi, Rep of Georgia.
[Autermann, C.; Beranek, S.; Calpas, B.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, N.; Klein, K.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany.
[Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany.
[Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, E.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.; Gunnellini, P.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany.
[Attikis, A.; Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bell, A. J.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Grebenyuk, A.; Habib, S.; Hauk, J.; Hellwig, G.; Horton, D.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Lange, J.; Schmidt, A.] Deutsch Elektronen Synchroton, Hamburg, Germany.
[Attikis, A.; Martin, M. Aldaya; Blobel, V.; Enderle, H.; Erfle, J.; Garutti, E.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Marchesini, I.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany.
[Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hartmann, F.; Hauth, T.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Kornmayer, A.; Pardo, P. Lobelle; Martschei, D.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Inst Expt Kernphys, Karlsruhe, Germany.
[Attikis, A.; Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece.
[Gouskos, L.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece.
[Pardos, C. Diez; Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.] Univ Ioannina, GR-45110 Ioannina, Greece.
[Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary.
[Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary.
[Karancsi, J.; Raics, R.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary.
[Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India.
[Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India.
[Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India.
[Sharma, A.; Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Singh, A. P.; Dutta, D.] Saha Inst Nucl Phys, Kolkata, India.
[Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India.
[Abdulsalam, A.; Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India.
[Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India.
[Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran.
[Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland.
[Abbrescia, M.; Barbone, L.; Calabria, C.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Laselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, R.; Zito, G.] INFN Sez Bari, Bari, Italy.
[Selvaggi, M.; Abbrescia, M.; Barbone, L.; Calabria, C.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy.
[Creanza, D.; De Filippis, N.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy.
[Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, E.; Fanfani, A.; Fasanella, A.; Giacomelli, R.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanan, A.; Navarria, El.; Odorici, E.; Perrotta, A.; Primavera, E.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.; Cavallo, N.; Tosi, M.] INFN Sez Bologna, Bologna, Italy.
[Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, Er.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, A.; Guiducci, L.; Meneghelli, M.; Navarria, El.; Primavera, E.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.; Tosi, M.] Univ Bologna, Bologna, Italy.
[Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, E.; Potenza, R.; Tricomi, A.; Tuve, C.] 1NFN Sez Catania, Catania, Italy.
[Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, E.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy.
[Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschidi, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy.
[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy.
[Benussi, L.; Bianco, S.; Fabbri, E.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy.
[Fabbricatore, P.; Ferro, E.; Lo Vetere, M.; Musenich, R.; Tosi, S.] INFN Sez Genova, Genoa, Italy.
[Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy.
[Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; De Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy.
[Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; De Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy.
[Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, E.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy.
[De Cosa, A.; Iorio, A. O. M.] Univ Napoli Federico II, Naples, Italy.
[Cavallo, N.; Fabozzi, E.] Univ Basilicata Potenza, Naples, Italy.
[Meola, S.] Univ G Marconi Roma, Naples, Italy.
[Azzi, P.; Bacchetta, N.; Bellato, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, R.; Simonetto, E.; Torassa, E.; Tosi, M.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy.
[Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, R.; Simonetto, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy.
[Kanishchev, K.; Lazzizzera, I.] Univ Trent, Padua, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] INFN Sez Pavia, Pavia, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] Univ Pavia, I-27100 Pavia, Italy.
[Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, E.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy.
[Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, E.; Santocchia, A.; Spiezia, A.] Univ Pergia, Perugia, Italy.
[Androsov, K.; Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, E.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, E.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] 1NFN Sez Pisa, Pisa, Italy.
[Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy.
[D'Agnolo, R. T.; Foa, L.; Ligabue, E.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy.
[Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, R.; Michell, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] INFN Sez Roma, Rome, Italy.
[Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, R.; Michell, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.] Univ Roma, Rome, Italy.
[Da Costa, E. M.; Kargoll, B.; Bellato, M.; Amapane, N.; Arcidiacono, R.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Degano, A.; Demaria, N.; Mariotti, C.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Solano, A.] INFN Sez Torino, Turin, Italy.
[Masetti, G.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Solano, A.; Staiano, A.; Tamponi, U.] Univ Torino, Turin, Italy.
[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientate Novara, Turin, Italy.
[Montanan, A.; Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Penzo, A.; Schizzi, A.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy.
[Montanan, A.; Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Penzo, A.; Schizzi, A.] Univ Trieste, Trieste, Italy.
[Chang, S.; Nam, S. K.; Kim, D. H.] Kangwon Natl Univ, Chunchon, South Korea.
[Mohammadi, A.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Son, D. C.; Kim, H.; Park, C.; Lee, B.] Kyungpook Natl Univ, Taegu, South Korea.
[Kim, D. H.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea.
[Naranjo, I. N.; Gyun, D.; Hong, B.; Kim, T. J.; Lee, K. S.; Roh, Y.; Choi, M.; Park, C.] Korea Univ, Seoul, South Korea.
[Kim, D. H.; Choi, M.; Park, C.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea.
[Grebenyuk, A.; Kim, D. H.; Lee, S.; Lee, K. S.; Choi, M.; Choi, Y.; Goh, J.; Kwon, E.; Lee, B.; Seo, H.] Sungkyunkwan Univ, Suwon, South Korea.
[Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania.
[Vilela Pereira, A.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.] Ctr Invest Estudios & Avanzados IPN, Mexico City, DF, Mexico.
[Montoya, C. A. Carrillo; Valencia, E. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico.
[Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico.
[Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis, San Luis Potosi, Mexico.
[Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand.
[Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand.
[Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid i Azam Univ, Natl Ctr Phys, Islamabad, Pakistan.
[Fruehwirth, R.; Bialkowska, H.; Boimska, B.; Gorski, M.; Kazana, M.; Wrochna, G.; Zalewski, R.] Natl Ctr Nucl Res, Otwock, Poland.
[Fasanella, A.; Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland.
[Almeida, N.; Bargassa, R.; Beirao Da Cruz E Silva, C.; Faccioli, R.; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrument & Fis Expt Particulas, Lisbon, Portugal.
[Fasanella, A.; Afanasiev, S.; Bunin, R.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Malakhov, A.; Matveev, V.; Palichik, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia.
[Kim, D. H.; Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Levchenko, R.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, Russia.
[Dermenev, A.; Gninenko, S.; Golubev, N.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Kirakosyan, M.] Inst Nucl Res, Moscow, Russia.
[Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia.
[Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia.
[Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys & Vinca Inst Nucl Sci, Belgrade, Serbia.
[Garcia, G.; Cavallo, Er.; Santocchia, A.; Romero, A.; Aguilar-Benitez, M.; Maestre, J. Alcaraz; Battilana, C.; Chamizo-Llatas, M.; Colino, N.; De la Cruz, B.; Per, A. Delgado; Vazquez, D. Dominguez; Bedoya, C. Fernandez; Ramos, J. P. Fernandez; Flix, J.; Fouz, M. C.; Redondo, I.] CIEMAT, Madrid, Spain.
[Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain.
[Bruno, G.; Bedoya, C. Fernandez; Lopez, O. Gonzalez; Brun, H.; Cuevas, J.; Folgueras, S.; Gomez, Piedra] Univ Oviedo, Oviedo, Spain.
[Broccolo, G.; Lopez, O. Gonzalez; Menendez, J. Fernandez; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Campderros, J. Duarte; Graziano, A.; Jorda, C.; Marco, J.; Marco, R.; Rivero, C. Martinez; Sanchez, F. J. Munoz; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Vila, I.; Cortabitarte, R. Vilar; Bondu, O.] CSIC Univ Cantabria, ICFA, Santander, Spain.
[Moreno, B. Gomez; Bloch, D.; Cortabitarte, R. Vilar; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Visscher, S.; Dobson, M.; Giffels, M.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Gowdy, S.; Harris, P.; Hartl, C.; Hinzmann, A.; Janot, R.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Petrilli, A.; Pfeiffer, A.; Sakulin, H.; Santanastasio, E.; Schafer, C.; Schwick, C.; Segoni, I.; Veres, G. I.] CERN, European Org Nucl Res, Geneva, Switzerland.
[Dietz-Laursonn, E.; Dhingra, N.; Konstantinov, D.; Bertl, W.; Gabathuler, K.; Horisberger, R.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland.
[Bachmair, E.; Bani, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; Del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, E.; Nageli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland.
[Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland.
[Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan.
[Klein, B.; Chen, G. M.; Chang, S.; Lu, Y. J.; Bartalini, P.; Chang, P.; Chang, Y. W.; Chao, Y.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] NTU, Taipei, Taiwan.
[Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand.
[Fasanella, A.; Kodolova, O.; Lopez, O. Gonzalez; Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey.
[Kodolova, O.; Lopez, O. Gonzalez; Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle Tech Univ, Dept Phys, Ankara, Turkey.
[Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey.
[Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yuecel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey.
[Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine.
[Brooke, J. J.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England.
[Bell, A. J.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Abdulsalam, A.; Fasanella, A.; Kodolova, O.; Lopez, O. Gonzalez; Adiguzel, A.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England.
[Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England.
[Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA.
[Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA.
[Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA.
[Abdulsalam, A.; Fasanella, A.; Kodolova, O.; Lopez, O. Gonzalez; Buchmuller, O.; Charaf, O.; Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA.
[Breto, G.; Calderon De la Barca Sanchez, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA.
[Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA.
[Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Paramesvaran, S.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA.
[Simon, M.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, E.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA.
[Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magafia; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA.
[Giammanco, A.; Dias, F. A.; Chen, G. M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Di Marco, E.; Duarte, J.; Kcira, D.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA.
[Liu, H.; Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Jang, D. W.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA.
[Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA.
[Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA.
[Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA.
[Attikis, A.; Abdulsalam, A.; Fasanella, A.; Belyaev, A.; Adiguzel, A.; Belyaev, A.; Avetisyan, A.; Apresyan, A.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Abdulsalam, A.; Fasanella, A.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA.
[Martins, T.; Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA.
[Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.; Evdokimov, O.] Florida State Univ, Tallahassee, FL 32306 USA.
[Daskalakis, G.; Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA.
[Fasanella, A.; Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Canner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA.
[Abdulsalam, A.; Fasanella, A.; Adiguzel, A.; Apresyan, A.; Askew, A.; Evdokimov, O.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; One, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA.
[Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA.
[Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA.
[Marangelli, B.; Evdokimov, O.; Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA.
[Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Fasanella, A.; Evdokimov, O.; Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA.
[Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA.
[Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA.
[Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, OH USA.
[Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA.
[Dolen, J.; Godshalk, A.; Lashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA.
[Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA.
[Schmidt, A.; Stoye, M.; Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA.
[De Wolf, E. A.; Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Slaunwhite, J.; Valls, N.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA.
[Antonelli, L.; Bylsm, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA.
[Evdokimov, O.; Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.; Koybasi, O.] Princeton Univ, Princeton, NJ 08544 USA.
[Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA.
[Abdulsalam, A.; Fasanella, A.; Savoy-Navarro, A.; Evdokimov, O.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA.
Purdue Univ Calumet, Hammond, LA USA.
[Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA.
[Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, R.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA.
[Evdokimov, O.; Koybasi, O.; Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.; Bouhali, O.] Rutgers State Univ, Piscataway, NJ USA.
[Rose, A.; Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA.
[Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA.
[Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA.
[Mao, Y.; Sharan, M.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA.
[Wood, D.; Arenton, M. W.; Le, S. Bout; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.] Univ Virginia, Charlottesville, VA USA.
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[Rabady, D.; Genchev, V.; Iaydjiev, R.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland.
[Beluffi, C.] Univ Strasbourg, Univ Haute Alsace, CNRS IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France.
[Giammanco, A.] NICPB, Tallinn, Estonia.
[Popov, A.; Zhukov, V.; Katkov, I.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Chinellato, J.] Univ Estadual Campinas, Campinas, SP, Brazil.
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[Abdelalim, A. A.; Elgammal, S.] Zewail City Sci & Technol, Zewail, Egypt.
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[Kamer, A. Ellithi] Cairo Univ, Cairo, Egypt.
[Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt.
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[Radi, A.] Ain Shams Univ, Cairo, Egypt.
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[Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France.
[Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia.
[Bergholz, M.] Brandenburg Tech Univ Cottbus, Cottbus, Germany.
[Bergholz, M.] Univ Kansas, Lawrence, KS 66045 USA.
[Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary.
[Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary.
[Swain, S. K.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India.
[Guchait, M.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India.
[Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia.
[Maity, M.] Univ Visva Bharati, Santini Ketan, W Bengal, India.
[Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka.
[Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran.
[Fahim, A.] Sharif Univ Technol, Tehran, Iran.
[Safarzadeh, B.] Islam Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran.
[Martelli, A.; Androsov, K.] Univ Siena, I-53100 Siena, Italy.
[De La Cruz-Burelo, E.] Univ Michoacana, Morelia, Michoacan, Mexico.
[Adzic, P.; Krpic, D.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia.
[Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy.
[Rolandi, G.] Scuola Normale, Pisa, Italy.
[Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy.
[Sphicas, P.] Univ Athens, Athens, Greece.
[Worm, S. D.; Newbold, D. M.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Nageli, C.] Paul Scherrer Inst, Villigen, Switzerland.
[Starodumov, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland.
[Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey.
[Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey.
[Onengut, G.] Cag Univ, Mersin, Turkey.
[Sogut, K.] Mersin Univ, Mersin, Turkey.
[Karapinar, G.] Izmir Inst Technol, Izmir, Turkey.
[Isildak, B.] Ozyegin Univ, Istanbul, Turkey.
[Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey.
[Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey.
[Sonmez, N.] Ege Univ, Izmir, Turkey.
[Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey.
[Giinaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, Kahramanmaras, Turkey.
[Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England.
[Pioppi, M.] Univ Perugia, INFN Sez Perugia, I-06100 Perugia, Italy.
[Wasserbaech, S.] Utah Valley Univ, Orem, UT USA.
[Milenovic, P.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia.
[Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia.
[Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey.
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[Bouhali, O.] Texas A&M Univ, Doha, Qatar.
[Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea.
RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia.
RI Varela, Joao/K-4829-2016; Sguazzoni, Giacomo/J-4620-2015; Ligabue,
Franco/F-3432-2014; Menasce, Dario Livio/A-2168-2016; Bargassa,
Pedrame/O-2417-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Leonardo,
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Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Dubinin,
Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan,
Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre
David/D-4314-2011; Sznajder, Andre/L-1621-2016; Vilela Pereira,
Antonio/L-4142-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mundim,
Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016;
Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012;
Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini,
Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Wulz,
Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Codispoti,
Giuseppe/F-6574-2014; Bellan, Riccardo/G-2139-2014; Petrushanko,
Sergey/D-6880-2012; da Cruz e Silva, Cristovao/K-7229-2013; Lokhtin,
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Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel,
Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Ragazzi,
Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Russ,
James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar,
rocio/P-8480-2014; Dahms, Torsten/A-8453-2015; Grandi,
Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes,
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Ilkehan/B-6360-2013; Lazzizzera, Ignazio/E-9678-2015; Sen,
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Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi,
Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose
Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya,
Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras,
Francisco/I-4983-2015; Lo Vetere, Maurizio/J-5049-2012; Rovelli,
Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani,
Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev,
Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae
Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012;
Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012
OI Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli,
Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396;
Fiorendi, Sara/0000-0003-3273-9419; Martelli,
Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X;
Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146;
Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva,
Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964;
Ligabue, Franco/0000-0002-1549-7107; Abdelalim, Ahmed
Ali/0000-0002-2056-7894; Diemoz, Marcella/0000-0002-3810-8530; Tricomi,
Alessia Rita/0000-0002-5071-5501; Heredia De La Cruz,
Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco,
stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Longo,
Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735;
Baarmand, Marc/0000-0002-9792-8619; Boccali,
Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686;
Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud,
Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Lloret
Iglesias, Lara/0000-0002-0157-4765; Rolandi, Luigi
(Gigi)/0000-0002-0635-274X; Leonardo, Nuno/0000-0002-9746-4594; Goh,
Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni,
Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan,
Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro
Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Dubinin,
Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X;
Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre
David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela
Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo
Gil/0000-0003-3514-7056; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad,
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Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera,
Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087;
D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev,
Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506;
Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki,
Marcin/0000-0001-9482-4841; Hernandez Calama, Jose
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Flix, Josep/0000-0003-2688-8047; Della Ricca,
Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226
FU BMWF; FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP
(Brazil); MES (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS
(Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF
(Estonia); Academy of Finland; MEC; HIP (Finland); CEA; CNRS/IN2P3
(France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NKTH (Hungary);
DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU
(Republic of Korea); LAS (Lithuania); CINVESTAV; CONACYT; SEP; UASLP-FAI
(Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE; NSC (Poland); FCT
(Portugal); JINR (Dubna); MON; RAS; RFBR (Russia); MESTD (Serbia);
SEIDI; CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei);
ThEPCenter; IPST; STAR; NSTDA (Thailand); TUBITAK; TAEK (Turkey); NASU
(Ukraine); STFC (United Kingdom); DOE; NSF (USA); Marie-Curie programme;
European Research Council; EPLANET (European Union); Leventis
Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation;
Belgian Federal Science Policy Office; Fonds pour la Formation a la
Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium);
Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium);
Ministry of Education, Youth and Sports (MEYS) of Czech Republic;
Council of Science and Industrial Research, India; Compagnia di San
Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science;
EU, Regional Development Fund; Thalis and Aristeia programmes; EU-ESF;
Greek NSRF; RosAtom
FX We congratulate our colleagues in the CERN accelerator departments for
the excellent performance of the LHC and thank the technical and
administrative staffs at CERN and at other CMS institutes for their
contributions to the success of the CMS effort. In addition, we
gratefully acknowledge the computing centres and personnel of the
Worldwide LHC Computing Grid for delivering so effectively the computing
infrastructure essential to our analyses. Finally, we acknowledge the
enduring support for the construction and operation of the LHC and the
CMS detector provided by the following funding agencies: BMWF and FWF
(Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP
(Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS
(Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF
(Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and
CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA
and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN
(Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV,
CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC
(Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON,
RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain);
Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST,
STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine);
STFC (United Kingdom); DOE and NSF (USA).; Individuals have received
support from the Marie-Curie programme and the European Research Council
and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan
Foundation; the Alexander von Humboldt Foundation; the Belgian Federal
Science Policy Office; the Fonds pour la Formation a la Recherche dans
l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor
Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of
Education, Youth and Sports (MEYS) of Czech Republic; the Council of
Science and Industrial Research, India; the Compagnia di San Paolo
(Torino); the HOMING PLUS programme of Foundation for Polish Science,
cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia
programmes cofinanced by EU-ESF and the Greek NSRF.
NR 56
TC 32
Z9 32
U1 5
U2 68
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 77
EP 100
DI 10.1016/j.physletb.2013.10.017
PG 24
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400010
ER
PT J
AU Chatrchyan, S
Khachatryan, V
Sirunyan, AM
Tumasyan, A
Adam, W
Aguilo, E
Bergauer, T
Dragicevic, M
Ero, J
Fabjan, C
Friedl, M
Fruhwirth, R
Ghete, VM
Hormann, N
Hrubec, J
Jeitler, M
Kiesenhofer, W
Knunz, V
Krammer, M
Kratschmer, I
Liko, D
Mikulec, I
Pernicka, M
Rabady, D
Rahbaran, B
Rohringer, C
Rohringer, H
Schofbeck, R
Strauss, J
Taurok, A
Waltenberger, W
Wulz, CE
Mossolov, V
Shumeiko, N
Gonzalez, JS
Bansal, M
Bansal, S
Cornelis, T
De Wolf, EA
Janssen, X
Luyckx, S
Mucibello, L
Ochesanu, S
Roland, B
Rougny, R
Selvaggi, M
Van Haevermaet, H
Van Mechelen, P
Van Remortel, N
Van Spilbeeck, A
Blekman, F
Blyweert, S
D'Hondt, J
Suarez, RG
Kalogeropoulos, A
Maes, M
Olbrechts, A
Van Doninck, W
Van Mulders, R
Van Onsem, GP
Villella, I
Clerbaux, B
De Lentdecker, G
Dero, V
Gay, APR
Hreus, T
Leonard, A
Marage, PE
Mohammadi, A
Reis, T
Thomas, L
Velde, CV
Vanlaer, P
Wang, J
Adler, V
Beernaert, K
Cimmino, A
Costantini, S
Garcia, G
Grunewald, M
Klein, B
Lellouch, J
Marinov, A
Mccartin, J
Rios, AAO
Ryckbosch, D
Sigamani, M
Strobbe, N
Thyssen, F
Tytgat, M
Walsh, S
Yazgan, E
Zaganidis, N
Basegmez, S
Bruno, G
Castello, R
Ceard, L
Delaere, C
du Pree, T
Favart, D
Forthomme, L
Giammanco, A
Hollar, J
Lemaitre, V
Liao, J
Militaru, O
Nuttens, C
Pagano, D
Pin, A
Piotrzkowski, K
Garcia, JMV
Basegmez, S
Bruno, G
Castello, R
Ceard, L
Delaere, C
du Pree, T
Favart, D
Forthomme, L
Giammanco, A
Hollar, J
Lemaitre, V
Liao, J
Militaru, O
Nuttens, C
Pagano, D
Pin, A
Piotrzkowski, K
Garcia, JMV
Beliy, N
Caebergs, T
Daubie, E
Hammad, GH
Alves, GA
Martins, MC
Martins, T
Pol, ME
Souza, MHG
Alda, WL
Carvalho, W
Custodio, A
Da Costa, EM
Damiao, DD
Martins, CD
De Souza, SF
Malbouisson, H
Malek, M
Figueiredo, DM
Mundim, L
Nogima, H
Da Silva, WLP
Santoro, A
Jorge, LS
Sznajder, A
Pereira, AV
Anjos, TS
Bernardes, CA
Dias, FA
Tomei, TRFP
Gregores, EM
Lagana, C
Marinho, F
Mercadante, PG
Novaes, SF
Padula, SS
Genchev, V
Iaydjiev, R
Piperov, S
Rodozov, M
Stoykova, S
Sultanov, G
Tcholakov, V
Trayanov, R
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Hadjiiska, R
Kozhuharov, V
Litov, L
Pavlov, B
Petkov, P
Bian, JG
Chen, GM
Chen, HS
Jiang, CH
Liang, D
Liang, S
Meng, X
Tao, J
Wang, J
Wang, X
Wang, Z
Xiao, H
Xu, M
Zang, J
Zhang, Z
Asawatangtrakuldee, C
Ban, Y
Guo, Y
Li, W
Liu, S
Mao, Y
Qian, SJ
Teng, H
Wang, D
Zhang, L
Zou, W
Avila, C
Montoya, CAC
Gomez, JP
Moreno, BG
Oliveros, AFO
Sanabria, JC
Godinovic, N
Lelas, D
Plestina, R
Polic, D
Puljak, I
Antunovic, Z
Kovac, M
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Duric, S
Kadija, K
Luetic, J
Mekterovic, D
Morovic, S
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Galanti, M
Mavromanolakis, G
Mousa, J
Nicolaou, C
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Razis, PA
Finger, M
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Assran, Y
Elgammal, S
Kamel, AE
Mahmoud, MA
Mahrous, A
Radi, A
Kadastik, M
Muntel, M
Murumaa, M
Raidal, M
Rebane, L
Tiko, A
Eerola, P
Fedi, G
Voutilainen, M
Harkonen, J
Heikkinen, A
Karimaki, V
Kinnunen, R
Kortelainen, MJ
Lampen, T
Lassila-Perini, K
Lehti, S
Linden, T
Luukka, P
Maenpaa, T
Peltola, T
Tuominen, E
Tuominiemi, J
Tuovinen, E
Ungaro, D
Wendland, L
Banzuzi, K
Karjalainen, A
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TI Measurement of the Upsilon(1S), Upsilon(2S), and Upsilon(3S) cross
sections in pp collisions at root s=7 TeV
SO PHYSICS LETTERS B
LA English
DT Article
DE CMS; Physics; Quarkonia; Upsilon; Dimuons
ID QED RADIATIVE-CORRECTIONS; UNIVERSAL MONTE-CARLO; PHOTOS
AB The Upsilon(1S), Upsilon(2S), and Upsilon(3S) production cross sections are measured using a data sample corresponding to an integrated luminosity of 35.8 +/- 1.4 pb(-1) of proton-proton collisions at root s = 7 TeV, collected with the CMS detector at the LHC. The Upsilon resonances are identified through their decays to dimuons. Integrated over the Upsilon transverse momentum range p(T)(Upsilon) < 50 GeV/c and rapidity range vertical bar y(Upsilon)vertical bar < 2.4, and assuming unpolarized Upsilon production, the products of the Upsilon production cross sections and dimuon branching fractions are
sigma (pp -> Upsilon(1S)X) . B(Upsilon(1S) -> mu(+)mu(-)) = (8.55 +/- 0.05(-0.50)(+0.56) +/- 0.34) nb,
sigma (pp -> Upsilon(2S)X) . B(Upsilon(2S) -> mu(+)mu(-)) = (2.21 +/- 0.03(-0.14)(+0.16) +/- 0.09) nb,
sigma (pp -> Upsilon(3S)X) . B(Upsilon(3S) -> mu(+)mu(-)) = (1.11 +/- 0.02(-0.08)(+0.10) +/- 0.04) nb,
where the first uncertainty is statistical, the second is systematic, and the third is from the uncertainty in the integrated luminosity. The differential cross sections in bins of transverse momentum and rapidity, and the cross section ratios are presented. Cross section measurements performed within a restricted muon kinematic range and not corrected for acceptance are also provided. These latter measurements are independent of Upsilon polarization assumptions. The results are compared to theoretical predictions and previous measurements. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved.
C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia.
[Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Pernicka, M.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria.
[Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus.
[Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Selvaggi, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium.
[Blekman, F.; Blyweert, S.; D'Hondt, J.; Suarez, R. Gonzalez; Kalogeropoulos, A.; Maes, M.; Olbrechts, A.; Van Doninck, W.; Van Mulders, R.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium.
[Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Reis, T.; Thomas, L.; Velde, C. Vander; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium.
[Adler, V.; Beernaert, K.; Cimmino, A.; Costantini, S.; Garcia, G.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium.
[Basegmez, S.; Bruno, G.; Castello, R.; Ceard, L.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium.
[Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium.
[Alves, G. A.; Martins Junior, M. Correa; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil.
[Aida Junior, W. L.; Carvalho, W.; Custodio, A.; Da Costa, E. M.; Damiao, D. De Jesus; Martins, C. De Oliveira; De Souza, S. Fonseca; Malbouisson, H.; Malek, M.; Figueiredo, D. Matos; Mundim, L.; Nogima, H.; Da Silva, W. L. Prado; Santoro, A.; Jorge, L. Soares; Sznajder, A.; Pereira, A. Vilela] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil.
[Dias, F. A.; Fernandez Perez Tomei, T. R.; Lagana, C.; Marinho, F.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil.
[Anjos, T. S.; Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil.
[Genchev, V.; Iaydjiev, R.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria.
[Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria.
[Wang, J.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.; Zang, J.; Zhang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China.
[Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Teng, H.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.
[Avila, C.; Montoya, C. A. Carrillo; Gomez, J. P.; Moreno, B. Gomez; Oliveros, A. F. Osorio; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia.
[Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia.
[Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia.
[Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.] Rudjer Boskovic Inst, Zagreb, Croatia.
[Attikis, A.; Galanti, M.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus.
[Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic.
[Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt.
[Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia.
[Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland.
[Harkonen, J.; Heikkinen, A.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland.
[Banzuzi, K.; Karjalainen, A.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland.
[Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France.
[Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France.
[Agram, J. -L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J. -M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Strasbourg, CNRS, IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France.
[Fassi, F.; Mercier, D.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, CNRS, IN2P3, Villeurbanne, France.
[Beauceron, S.; Beaupere, N.; Bondu, O.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Tschudi, Y.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, Villeurbanne, France.
[Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informat, GE-380086 Tbilisi, Rep of Georgia.
[Autermann, C.; Beranek, S.; Calpas, B.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] RVVTH Aachen Univ, Inst Phys 1, Aachen, Germany.
[Weber, H.; Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany.
[Bontenackels, M.; Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Perchalla, L.; Pooth, O.; Sauerland, P.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany.
[Martin, M. Aldaya; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Castro, E.; Costanza, F.; Dammann, D.; Pardos, C. Diez; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Leonard, J.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Rosin, M.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Spiridonov, A.; Stein, M.; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany.
[Blobel, V.; Enderle, H.; Erfle, J.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Hermanns, T.; Hoeing, R. S.; Kaschube, K.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Lange, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany.
[Barth, C.; Berger, J.; Boeser, C.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hackstein, C.; Hartmann, F.; Hauth, T.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Pardo, P. Lobelle; Martschei, D.; Mueller, S.; Mueller, Th; Niegel, M.; Nuernberg, A.; Oberst, O.; Oehler, A.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany.
[Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Ntomari, E.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece.
[Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.] Univ Athens, Athens, Greece.
[Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.] Univ Ioannina, GR-45110 Ioannina, Greece.
[Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary.
[Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary.
[Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary.
[Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India.
[Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India.
[Banerjee, S.; Bhattacharya, S.; Dutta, S.; Gomber, B.; Jain, Sa; Jain, Sh; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India.
[Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India.
[Aziz, T.; Ganguly, S.; Guchait, M.; Gurtu, A.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] EHEP, Tata Inst Fundamental Res, Bombay, Maharashtra, India.
[Banerjee, S.; Dugad, S.] HECR, Tata Inst Fundamental Res, Bombay, Maharashtra, India.
[Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran.
[Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy.
[Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy.
[Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy.
[Abdulsalam, A.; Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy.
[Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy.
[Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy.
[Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy.
[Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, Florence, Italy.
[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Tropiano, A.] Univ Florence, Florence, Italy.
[Fabbri, F.; Benussi, L.; Bianco, S.; Colafranceschi, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy.
[Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy.
[Tosi, S.] Univ Genoa, Genoa, Italy.
[Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fats, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy.
[De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fats, T. Tabarelli] Univ Milano Bicocca, Milan, Italy.
[Buontempo, S.; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy.
[De Cosa, A.; Dogangun, O.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy.
[Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy.
[Meola, S.] Univ G Marconi Roma, Naples, Italy.
[Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy.
[Bisello, D.; Branca, A.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy.
[Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy.
[Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy.
[Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy.
[Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.] Univ Perugia, I-06100 Perugia, Italy.
[Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy.
[Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy.
[Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy.
[Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy.
[Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Roma, Rome, Italy.
[Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Mazza, G.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy.
[Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy.
[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.] Univ Piemonte Orientale Novara, Turin, Italy.
[Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy.
[Abdulsalam, A.; Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy.
[Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea.
[Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea.
[Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea.
[Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea.
[Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea.
[Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea.
[Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania.
[Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico.
[Carrillo Moreno, S.; Vazquez Valencia, F.] Univ lberoamer, Mexico City, DF, Mexico.
[Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico.
[Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico.
[Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand.
[Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand.
[Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan.
[Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland.
[Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland.
[Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal.
[Belotelov, I.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res Dubna, Dubna, Russia.
[Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia.
[Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia.
[Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Shreyber, I.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia.
[Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Fed, Protvino, Russia.
[Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia.
[Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Lopez, O. Gonzalez; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain.
[Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain.
[Bruno, G.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain.
[Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Cortabitarte, R. Vilar] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain.
[Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Govoni, P.; Goyvdy, S.; Guida, R.; Gundacker, S.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y. -J.; Lenzi, P.; Lourenco, C.; Magini, N.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C. .; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland.
[Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland.
[Weber, H.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; Del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland.
[Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland.
[Chang, Y. H.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan.
[Chang, Y. H.; Bartalini, P.; Chang, P.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan.
[Asavapibhop, B.; Srimanobhas, N.] Chulalongkorn Univ, Bangkok, Thailand.
[Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey.
[Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey.
[Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey.
[Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey.
[Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine.
[Godinovic, N.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England.
[Belyaev, A.; Basso, L.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England.
[Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England.
[Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA.
[Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA.
[Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.; Kropivnitskaya, A. .] Boston Univ, Boston, MA 02215 USA.
[Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA.
[Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA.
[Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA.
[Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA.
[Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA.
[Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA.
[Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA.
[Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA.
[Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA.
[Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA.
[Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA.
[Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A. .; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Park, M.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA.
[Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA.
[Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA.
[Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA.
[Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, E.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA.
[Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA.
[Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA.
[Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA.
[Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA.
[Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA.
[Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA.
[Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Krajczar, K.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA.
[Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA.
[Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, Oxford, MS 38677 USA.
[Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA.
[Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA.
[Kropivnitskaya, A. .; Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA.
[Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA.
[Antonelli, L.; Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA.
[Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA.
[Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA.
[Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA.
[Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA.
[Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA.
[Li, W.; Adair, A.; Akgun, B.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA.
[Kropivnitskaya, A. .; Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, R.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA.
[Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA.
[Park, M.; Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.; Gray, L.] Rutgers State Univ, Piscataway, NJ USA.
[Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA.
[Kropivnitskaya, A. .; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.] Texas A&M Univ, College Stn, TX USA.
[Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA.
[Appelt, E.; Delannoy, A. G.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA.
[Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA.
[Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA.
[Anderson, M.; Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA.
[Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria.
[Rabady, D.; Genchev, V.; Iaydjiev, R.; Puljak, I.; Chierici, R.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Calabria, C.; De Filippis, N.; Meneghelli, M.; Di Matteo, L.; Gennai, S.; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; D'Agnolo, R. T.; Fiori, F.; Squillacioti, P.; Grassi, M.; Meridiani, P.; Musich, M.; Marone, M.; Montanino, D.; Grishin, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland.
[Giammanco, A.] NICPB, Tallinn, Estonia.
[Dias, F. A.; Dubinin, M.] CALTECH, Pasadena, CA 91125 USA.
[Plestina, R.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France.
[Assran, Y.] Suez Canal Univ, Suez, Egypt.
[Elgammal, S.] Zewail City Sci & Technol, Zewail, Egypt.
[Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt.
[Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt.
[Mahrous, A.] Helwan Univ, Cairo, Egypt.
[Radi, A.] British Univ Egypt, Cairo, Egypt.
[Radi, A.] Ain Shams Univ, Cairo, Egypt.
[Bluj, M.] Natl Ctr Nucl Res, Otwock, Poland.
[Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France.
[Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia.
[Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia.
[Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, D-03044 Cottbus, Germany.
[Sibille, J.] Univ Kansas, Lawrence, KS 66045 USA.
[Horvath, D.] ATOMKI, Inst Nucl Res, Debrecen, Hungary.
[Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary.
[Guchait, M.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India.
[Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia.
[Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India.
[Arfaei, H.; Fahim, A.] Sharif Univ Technol, Tehran, Iran.
[Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran.
[Hashemi, M.] Shiraz Univ, Shiraz, Iran.
[Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran.
[Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy.
[Meola, S.] Univ Guglielmo Marconi, Rome, Italy.
[Martini, L.] Univ Siena, I-53100 Siena, Italy.
[Serban, A. T.] Univ Bucharest, Fac Phys, Bucharest, Romania.
[Adzic, P.; Krpic, D.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia.
[Felcini, M.] Univ Calif Los Angeles, Los Angeles, CA USA.
[Rolandi, G.] Scuola Normale, Pisa, Italy.
[Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy.
[Rovelli, C.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy.
[Sphicas, P.] Univ Athens, Athens, Greece.
[Worm, S. D.; Newbold, D. M.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England.
[Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland.
[Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia.
[Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland.
[Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey.
[Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey.
[Karapinar, G.] Izmir Inst Technol, Izmir, Turkey.
[Ozturk, S.] Univ Iowa, Iowa City, IA USA.
[Sogut, K.] Mersin Univ, Mersin, Turkey.
[Isildak, B.] Ozyegin Univ, Istanbul, Turkey.
[Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey.
[Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey.
[Sonmez, N.] Ege Univ, Izmir, Turkey.
[Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England.
[Pioppi, M.] Univ Perugia, Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy.
[Wasserbaech, S.] Utah Valley Univ, Orem, UT USA.
[Leonidopoulos, C.] Univ Edinburgh, Edinburgh, Midlothian, Scotland.
[Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia.
[Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia.
[Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia.
[Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey.
[Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey.
[Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey.
[Krajczar, K.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary.
[Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea.
RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia.
RI Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Leonidov,
Andrey/P-3197-2014; vilar, rocio/P-8480-2014; da Cruz e Silva,
Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Bernardes, Cesar
Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera,
Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro,
Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl,
Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Montanari,
Alessandro/J-2420-2012; Gribushin, Andrei/J-4225-2012; Cerrada,
Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon,
Alicia/K-3658-2014; Josa, Isabel/K-5184-2014; de la Cruz,
Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Arce,
Pedro/L-1268-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini,
Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Codispoti,
Giuseppe/F-6574-2014; Petrushanko, Sergey/D-6880-2012; Marlow,
Daniel/C-9132-2014; Janssen, Xavier/E-1915-2013; Novaes,
Sergio/D-3532-2012; Bellan, Riccardo/G-2139-2014; Lokhtin,
Igor/D-7004-2012; Tinti, Gemma/I-5886-2013; Bartalini,
Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Ligabue,
Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko,
Lev/D-7127-2012; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose
Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My,
Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi,
Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin,
Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov,
Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE',
Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin,
Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix,
Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei,
Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni,
Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez,
Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Sznajder,
Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Mundim,
Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Leonardo,
Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011;
Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan,
Efe/C-4521-2014;
OI Ferguson, Thomas/0000-0001-5822-3731; Benussi,
Luigi/0000-0002-2363-8889; Grandi, Claudio/0000-0001-5998-3070;
Lazzizzera, Ignazio/0000-0001-5092-7531; Sen,
Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306;
Belyaev, Alexander/0000-0002-1733-4408; Stahl,
Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279;
Montanari, Alessandro/0000-0003-2748-6373; Cerrada,
Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Arce,
Pedro/0000-0003-3009-0484; Calvo Alamillo, Enrique/0000-0002-1100-2963;
Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023;
Codispoti, Giuseppe/0000-0003-0217-7021; Novaes,
Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz,
Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192;
Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose
Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My,
Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668;
Ragazzi, Stefano/0000-0001-8219-2074; Rovelli,
Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM,
Tae Jeong/0000-0001-8336-2434; de Jesus Damiao,
Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della
Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226;
Dubinin, Mikhail/0000-0002-7766-7175; Paganoni,
Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco
Mendes, Andre David/0000-0001-5854-7699; Sznajder,
Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626;
Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446;
Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083;
Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301;
Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950;
Heath, Helen/0000-0001-6576-9740
FU BMWF; FWF (Austria); FNRS; FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP
(Brazil); MEYS (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS
(Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF
(Estonia); Academy of Finland; MEC; HIP (Finland); CEA; CNRS/IN2P3
(France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NKTH (Hungary);
DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU
(Republic of Korea); LAS (Lithuania); CINVESTAV; CONACYT; SEP; UASLP-FAI
(Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE; NSC (Poland); FCT
(Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON;
RosAtom; RAS; RFBR (Russia); MSTD (Serbia); SEIDI; CPAN (Spain); Swiss
Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter; IPST; NSTDA
(Thailand); TUBITAK; TAEK (Turkey); NASU (Ukraine); STFC (United
Kingdom); DOE; NSF (USA); Marie-Curie programme; European Research
Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan
Foundation; Alexander von Humboldt Foundation; Belgian Federal Science
Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie
et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door
Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth
and Sports (MEYS) of Czech Republic; Council of Science and Industrial
Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme
of Foundation for Polish Science; European Union, Regional Development
Fund
FX We congratulate our colleagues in the CERN accelerator departments for
the excellent performance of the LHC and thank the technical and
administrative staffs at CERN and at other CMS institutes for their
contributions to the success of the CMS effort. In addition, we
gratefully acknowledge the computing centres and personnel of the
Worldwide LHC Computing Grid for delivering so effectively the computing
infrastructure essential to our analyses. Finally, we acknowledge the
enduring support for the construction and operation of the LHC and the
CMS detector provided by the following funding agencies: BMWF and FWF
(Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP
(Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China);
COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09
and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and
CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA
and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN
(Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV,
CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC
(Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia,
Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR
(Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies
(Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand);
TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE
and NSF (USA). Individuals have received support from the Marie-Curie
programme and the European Research Council and EPLANET (European
Union); the Leventis Foundation; the A.P. Sloan Foundation; the
Alexander von Humboldt Foundation; the Belgian Federal Science Policy
Office; the Fonds pour la Formation a la Recherche dans l'Industrie et
dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door
Wetenschap en Technologie (IWT-Belgium); the Ministry of Education,
Youth and Sports (MEYS) of Czech Republic; the Council of Science and
Industrial Research, India; the Compagnia di San Paolo (Torino); and the
HOMING PLUS programme of Foundation for Polish Science, cofinanced from
European Union, Regional Development Fund.
NR 29
TC 24
Z9 24
U1 2
U2 63
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 101
EP 125
DI 10.1016/j.physletb.2013.10.033
PG 25
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400011
ER
PT J
AU Vecchi, L
AF Vecchi, Luca
TI A flavor sector for the composite Higgs
SO PHYSICS LETTERS B
LA English
DT Article
ID MODEL; BOSON; BREAKING; MASSES; LHC
AB We discuss flavor violation in large N Composite Higgs models. We focus on scenarios in which the masses of the Standard Model fermions are controlled by hierarchical mixing parameters, as in models of Partial Compositeness. We argue that a separation of scales between flavor and Higgs dynamics can be employed to parametrically suppress dipole and penguin operators, and thus effectively remove the experimental constraints arising from the lepton sector and the neutron EDM. The dominant source of flavor violation beyond the Standard Model is therefore controlled by 4-fermion operators, whose Wilson coefficients can be made compatible with data provided the Higgs dynamics approaches a "walking" regime in the IR. Models consistent with all flavor and electroweak data can be obtained with a new physics scale within the reach of the LHC. Explicit scenarios may be realized in a 5D framework, the new key ingredient being the introduction of flavor branes where the wave functions of the bulk fermions end. (C) 2013 Elsevier B.V. All rights reserved.
C1 Los Alamos Natl Lab, Div Theory T 2, Los Alamos, NM 87545 USA.
RP Vecchi, L (reprint author), Los Alamos Natl Lab, Div Theory T 2, POB 1663, Los Alamos, NM 87545 USA.
EM vecchi@lanl.gov
OI VECCHI, Luca/0000-0001-5254-8826
FU DOE Office of Science; LANL LDRD program
FX I thank Silvia for her patience, Marco Nardecchia and Ian Shoemaker for
discussions, and Kaustubh Agashe for comments, for suggesting a brief
discussion of the 5D realization, and for helping me in the
identification of the dual picture. This work was supported by the DOE
Office of Science and the LANL LDRD program.
NR 23
TC 1
Z9 1
U1 0
U2 1
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 130
EP 135
DI 10.1016/j.physletb.2013.08.006
PG 6
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400013
ER
PT J
AU Roberts, CD
Holt, RJ
Schmidt, SM
AF Roberts, Craig D.
Holt, Roy J.
Schmidt, Sebastian M.
TI Nucleon spin structure at very high x
SO PHYSICS LETTERS B
LA English
DT Article
DE Continuum strong QCD; Diquark correlations; Dynamical chiral symmetry
breaking; Dyson-Schwinger equations; Nucleon longitudinal spin
asymmetries; Parton distribution functions; Valence quarks at very high
x
ID QUARK-DIQUARK MODEL; QCD; DISTRIBUTIONS; SCATTERING; PROTON; PION
AB Dyson-Schwinger equation treatments of the strong interaction show that the presence and importance of nonpointlike diquark correlations within the nucleon are a natural consequence of dynamical chiral symmetry breaking. Using this foundation, we deduce a collection of simple formulae, expressed in terms of diquark appearance and mixing probabilities, from which one may compute ratios of longitudinal-spin-dependent u- and d-quark parton distribution functions on the domain x similar or equal to 1. A comparison with predictions from other approaches plus a consideration of extant and planned experiments shows that the measurement of nucleon longitudinal spin asymmetries on x similar or equal to 1 can add considerably to our capacity for discriminating between contemporary pictures of nucleon structure. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Roberts, Craig D.; Holt, Roy J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
[Schmidt, Sebastian M.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany.
[Schmidt, Sebastian M.] JARA, D-52425 Julich, Germany.
RP Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
FU Helmholtz Association International Fellow Award; Department of Energy,
Office of Nuclear Physics [DE-AC02-06CH11357]; Forschungszentrum Julich
GmbH
FX We are grateful for insightful comments from I.C. Cloet. C.D.R.
acknowledges support from an Helmholtz Association International Fellow
Award. Work otherwise funded by: Department of Energy, Office of Nuclear
Physics, contract No. DE-AC02-06CH11357; and Forschungszentrum Julich
GmbH.
NR 70
TC 19
Z9 19
U1 0
U2 5
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 249
EP 254
DI 10.1016/j.physletb.2013.09.038
PG 6
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400034
ER
PT J
AU Chang, L
Roberts, CD
Schmidt, SM
AF Chang, Lei
Roberts, Craig D.
Schmidt, Sebastian M.
TI Light front distribution of the chiral condensate
SO PHYSICS LETTERS B
LA English
DT Article
DE Quantum chromodynamics; Dynamical chiral symmetry breaking;
Dyson-Schwinger equations; Light-front quantum field theory
ID ENERGY-MOMENTUM-TENSOR; QUANTUM CHROMODYNAMICS; WAVE-FUNCTIONS; QCD;
CONSTANT; SYMMETRY; EQUATION; TRACE
AB The pseudoscalar projection of the pion's Poincare-covariant Bethe-Salpeter amplitude onto the light-front may be understood to provide the probability distribution of the chiral condensate within the pion. Unlike the parton distribution amplitudes usually considered and as befitting a collective effect, this condensate distribution receives contributions from all Fock space components of the pion's light-front wave function. We compute this condensate distribution using the Dyson-Schwinger equation (DSE) framework and show the result to be a model-independent feature of quantum chromodynamics (QCD). Our analysis establishes that this condensate is concentrated in the neighbourhood of the boundaries of the distribution's domain of support. It thereby confirms the dominant role played by many-particle Fock states within the pion's light-front wave function in generating the chiral condensate and verifies that light-front longitudinal zero modes do not play a material role in that process. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Chang, Lei] Forschungszentrum Julich, Inst Kernphys, D-52425 Julich, Germany.
[Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
[Schmidt, Sebastian M.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany.
[Schmidt, Sebastian M.] JARA, D-52425 Julich, Germany.
RP Schmidt, SM (reprint author), Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany.
FU Forschungszentrum Julich GmbH; Department of Energy, Office of Nuclear
Physics [DE-AC02-06CH11357]
FX We are grateful for insightful comments from S.J. Brodsky, I.C. Cloet
and P.C. Tandy. Work supported by: Forschungszentrum Julich GmbH; and
Department of Energy, Office of Nuclear Physics, contract No.
DE-AC02-06CH11357.
NR 59
TC 15
Z9 15
U1 0
U2 1
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0370-2693
EI 1873-2445
J9 PHYS LETT B
JI Phys. Lett. B
PD NOV
PY 2013
VL 727
IS 1-3
BP 255
EP 259
DI 10.1016/j.physletb.2013.09.040
PG 5
WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 273ES
UT WOS:000328518400035
ER
PT J
AU Brusseau, ML
Carroll, KC
Truex, MJ
Becker, DJ
AF Brusseau, Mark L.
Carroll, Kenneth C.
Truex, Michael J.
Becker, David J.
TI Characterization and Remediation of Chlorinated Volatile Organic
Contaminants in the Vadose Zone
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID SOIL-VAPOR EXTRACTION; UNSATURATED POROUS-MEDIA; NONAQUEOUS PHASE
LIQUID; PARTITIONING TRACER TESTS; 3-DIMENSIONAL NUMERICAL-MODEL;
EVAPORATIVE MASS-TRANSFER; LOW-PERMEABILITY SOILS; WATER-CONTENT;
IMMISCIBLE-LIQUID; HYDRAULIC TOMOGRAPHY
AB Contamination of vadose-zone systems by chlorinated solvents is widespread and poses significant potential risk to human health through impacts on groundwater quality and vapor intrusion. Soil vapor extraction (SVE) is the presumptive remedy for such contamination and has been used successfully for innumerable sites; however, SVE operations typically exhibit reduced mass-removal effectiveness at some point due to the impact of poorly accessible contaminant mass and associated mass-transfer limitations. Assessment of SVE performance and closure is currently based on characterizing contaminant mass discharge associated with the vadose-zone source and its impact on groundwater or vapor intrusion. These issues are addressed in this overview, with a focus on summarizing recent advances in our understanding of the transport, characterization, and remediation of chlorinated solvents in the vadose zone. The evolution of contaminant distribution with time and the associated impacts on remediation efficiency are discussed, as is potential impact of persistent sources on groundwater quality and vapor intrusion. In addition, alternative methods for site characterization and remediation are addressed.
C1 [Brusseau, Mark L.] Univ Arizona, Sch Earth & Environm Sci, Tucson, AZ 85721 USA.
[Carroll, Kenneth C.; Truex, Michael J.] Pacific NW Natl Lab, Richland, WA 99354 USA.
[Becker, David J.] US Army Corps Engineers, Environm & Munit Ctr Expertise, Omaha, NE 68102 USA.
RP Brusseau, ML (reprint author), Univ Arizona, Sch Earth & Environm Sci, Tucson, AZ 85721 USA.
EM Brusseau@email.arizona.edu
RI Carroll, Kenneth/H-5160-2011
OI Carroll, Kenneth/0000-0003-2097-9589
FU U.S. Department of Defense Environmental Security Technology
Certification Program [ER-201125]; USDOE Office of Environmental
Management, Office of Soil and Groundwater Remediation and Office of
Richland Operations; National Institute of Environmental Health Sciences
Superfund Research Program [ES04940]; USDOE [DE-AC05-76RL01830]
FX This research was supported by the U.S. Department of Defense
Environmental Security Technology Certification Program (ER-201125), the
USDOE Office of Environmental Management, Office of Soil and Groundwater
Remediation and Office of Richland Operations, and the National
Institute of Environmental Health Sciences Superfund Research Program
(ES04940). We thank Jim Hatton of AECOM, Inc., and Manfred Plaschke of
CRA, Inc., for graciously providing the SVE data sets for the AFP44 and
TAA sites, respectively. Assistance with graphics from Kyle Parker and
Jeff London is appreciated. The Pacific Northwest National Laboratory is
operated by Battelle Memorial Institute for the USDOE under Contract
DE-AC05-76RL01830.
NR 145
TC 10
Z9 10
U1 3
U2 33
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD NOV
PY 2013
VL 12
IS 4
DI 10.2136/vzj2012.0137
PG 17
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 274TF
UT WOS:000328628400002
ER
PT J
AU Dafflon, B
Hubbard, SS
Ulrich, C
Peterson, JE
AF Dafflon, Baptiste
Hubbard, Susan S.
Ulrich, Craig
Peterson, John E.
TI Electrical Conductivity Imaging of Active Layer and Permafrost in an
Arctic Ecosystem, through Advanced Inversion of Electromagnetic
Induction Data
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID LATERALLY CONSTRAINED INVERSION; GROUND-PENETRATING RADAR; THAW LAKE
BASINS; NEAR-SURFACE; RESISTIVITY TOMOGRAPHY; SOIL; ALASKA; ALGORITHM;
MODEL; CALIBRATION
AB Characterizing the spatial variability of active layer and permafrost properties is critical for parameterizing process-rich models that simulate feedbacks from Arctic ecosystem to a changing climate. Because of the sensitivity of electrical conductivity (EC) measurements to moisture content, salinity, and freeze state and the ease of collecting electromagnetic induction (EMI) data with portable tools (e. g., EM38, GEM2, or DUALEM) over large regions, EMI surveys hold great potential for Arctic ecosystem characterization. However, estimation of subsurface EC distribution from such data is challenging because of the insufficient amount of information such data provide towards finding a unique solution. The non-uniqueness problem is often approached by fixing inversion constraints and initial models without a clear understanding of their possible effects on the obtained results. Here we developed a direct search method, which involves a grid-based evaluation of one-dimensional layered model parameters, to estimate EC distribution from EMI data and evaluate the influence of prior constraints, data information content, and solution non-uniqueness. We applied the new method to EMI data acquired in Barrow, AK, as part of the Department of Energy Next-Generation Ecosystem Experiments (DOE NGEE-Arctic). Results demonstrate the success of the developed approach for estimating models that reproduce recorded data within a specified range of uncertainty at each measurement location, as well as the value of different types of constraints. Importantly, the method can be used to quickly investigate the need for and effects of different priors at numerous measurement locations, since the time-consuming simulation of the EMI signals from the multidimensional search grid is performed only once.
C1 [Dafflon, Baptiste; Hubbard, Susan S.; Ulrich, Craig; Peterson, John E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
RP Dafflon, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM bdafflon@lbl.gov
RI Dafflon, Baptiste/G-2441-2015; Hubbard, Susan/E-9508-2010
FU Office of Biological and Environmental Research in the DOE Office of
Science; [DE-AC02-05CH11231]
FX The Next-Generation Ecosystem Experiments (NGEE Arctic) project is
supported by the Office of Biological and Environmental Research in the
DOE Office of Science. This NGEE-Arctic research is supported through
contract number DE-AC02-05CH11231 to Lawrence Berkeley National
Laboratory. Logistical support in Barrow was provided by UMIAQ, LLC. The
authors thank Stan Wullschleger (NGEE-Arctic PI, ORNL) for facilitating
our field campaigns, Nigel Quinn (LBNL) for lending us EM38 tools, and
Jinsong Chen, Mike Commer (LBNL), and Roman Shekhtman (UBC) for
providing codes and guidance for using the EM forward modeling code from
LBNL and the University of British Columbia, respectively.
NR 56
TC 12
Z9 12
U1 0
U2 19
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD NOV
PY 2013
VL 12
IS 4
DI 10.2136/vzj2012.0161
PG 19
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 274TF
UT WOS:000328628400005
ER
PT J
AU Griffith, BC
Holt, RM
Glass, RJ
AF Griffith, B. Clark
Holt, Robert M.
Glass, Robert J.
TI Generating Reproducible Microscale Heterogeneity for Transmitted-Light
Flow Visualization Experiments
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID WETTING FRONT INSTABILITY; POROUS-MEDIA; LABORATORY EXPERIMENTS;
GRANULAR-MATERIALS; SIZE SEGREGATION; FINGERED FLOW; 2 DIMENSIONS;
SATURATION; DYNAMICS; SYSTEMS
AB We developed and evaluated a new approach for constructing reproducible, "geologically realistic" heterogeneity for near-two-dimensional transmitted-light experiments. By using an apparatus with a computer-controlled arm, mixtures of sand were deposited in an experimental chamber through a tube. Mechanical segregation processes within the tube and the chamber led to stratification that mimicked that produced by sedimentary processes. By varying the arm speed, stratum thickness and angle could be controlled. By using different sand mixtures, the grain size at the top and bottom of a stratum could be varied. Through the use of carefully designed computer programs, a variety of reproducible microheterogeneous and macroheterogeneous structures could be produced. A spectral evaluation of 10 sample chambers produced with a single program showed negligible differences between sample chambers.
C1 [Griffith, B. Clark] Intera Inc, Austin, TX 78754 USA.
[Holt, Robert M.] Univ Mississippi, Dept Geol & Geol Engn, University, MS 38655 USA.
[Glass, Robert J.] Sandia Natl Labs, Div Energy Nonproliferat & High Consequence Secur, Albuquerque, NM 87123 USA.
RP Holt, RM (reprint author), Univ Mississippi, Dept Geol & Geol Engn, 118 Carrier Hall, University, MS 38655 USA.
EM rmholt@olemiss.edu
FU U.S. Department of Energy's Office of Basic Energy Research Geoscience
Program [DE-AC04-94AL85000]
FX We are grateful for the efforts of four anonymous reviewers; their
comments greatly improved this manuscript. In addition, we wish to thank
Michael Young for his help with our manuscript. Our work was supported
by the U.S. Department of Energy's Office of Basic Energy Research
Geoscience Program under contract DE-AC04-94AL85000 to Sandia National
Laboratories. We also gratefully acknowledge Lee O'Rear and Will
Peplinski, whose help in the laboratory was invaluable.
NR 33
TC 0
Z9 0
U1 3
U2 8
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD NOV
PY 2013
VL 12
IS 4
DI 10.2136/vzj2011.0182
PG 8
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 274TF
UT WOS:000328628400001
ER
PT J
AU Salve, R
Rempe, D
AF Salve, Rohit
Rempe, Daniella
TI Backfill Impacts on Moisture Measurements in Fractured Rock
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID TIME-DOMAIN REFLECTOMETRY; SOIL-WATER CONTENT; DIELECTRIC-PROPERTIES;
PROBES; PERMITTIVITY; SUBSURFACE; DISCHARGE; HILLSLOPE; MODEL
AB As the scope of hillslope-hydrology investigations extend deeper, there will likely be an increase in the use of backfill to facilitate sensor installations, particularly in fractured rock. Because of the disparity in hydrologic properties of backfill and the native rock being monitored, discrepancies in measured values are imminent. In this study, we assessed the impact of different types of backfill that can be used to provide hydraulic continuity between sensors and the "measured" environment. During a period of 4 yr, the hydrologic response to seasonal wetting and drying was monitored with identical time domain reflectometry (TDR) sensors embedded in native rock, fracture infill, augured native rock, and silica powder. We found that while all backfills responded to wetting and drying events, there were differences in the response to individual rainfall events and in the amount of moisture measured. Our observations show that the use of any type of backfill for monitoring fractured rock hydrology will result in distorted measurements; however, our analysis suggests that simple calibrations between native rock and backfill measurements allow moisture content changes in the native rock to be quantified using backfill measurements. Backfill that is finer textured than native rock provides the best estimate of water content during long-term, uninterrupted drying events when the backfill measurements are calibrated to native rock conditions. Irrespective of calibration, backfill materials coarser than the native rock provide the best detection of the timing and duration of the hydrologic response to precipitation.
C1 [Salve, Rohit] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Rempe, Daniella] Univ Calif Berkeley, Berkeley, CA 94720 USA.
RP Salve, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
EM r_salve@lbl.gov
FU W.M. Keck Foundation; Laboratory Directed Research and Development
Program, USDOE; USDOE Office of Science Graduate Fellowship Program (DOE
SCGF); ORISE-ORAU [DE-AC05-06OR23100]
FX This study was supported by the W.M. Keck Foundation and the Laboratory
Directed Research and Development Program, USDOE. Daniella Rempe is
supported in part by the USDOE Office of Science Graduate Fellowship
Program (DOE SCGF), made possible in part by the American Recovery and
Reinvestment Act of 2009, administered by ORISE-ORAU under Contract no.
DE-AC05-06OR23100. We would like to thank Alessandro Uccelli for
assistance in the field.
NR 26
TC 0
Z9 0
U1 4
U2 10
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD NOV
PY 2013
VL 12
IS 4
DI 10.2136/vzj2013.04.0076
PG 9
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 274TF
UT WOS:000328628400046
ER
PT J
AU Wang, W
Kravchenko, AN
Johnson, T
Srinivasan, S
Ananyeva, KA
Smucker, AJM
Rose, JB
Rivers, ML
AF Wang, W.
Kravchenko, A. N.
Johnson, T.
Srinivasan, S.
Ananyeva, K. A.
Smucker, A. J. M.
Rose, J. B.
Rivers, M. L.
TI Intra-Aggregate Pore Structures and Escherichia coli Distribution by
Water Flow within and Movement Out of Soil Macroaggregates
SO VADOSE ZONE JOURNAL
LA English
DT Article
ID RAY COMPUTED MICROTOMOGRAPHY; SATURATED POROUS-MEDIA;
SPATIAL-DISTRIBUTION; ORGANIC-MATTER; TRANSPORT; MANURE; ATTACHMENT;
SURVIVAL; QUANTIFICATION; BACTERIA
AB Soil aggregates are an important structural component of the soil matrix that could harbor Escherichia coli and provide an environment for its survival and water flow reentering. Knowledge of the exact pore locations within soil aggregates obtained using X-ray computed microtomography opens new opportunities for understanding microorganism movement within the soil matrix. The first objective of this study was to assess E. coli spatial distribution within soil macroaggregates and its potential for leaving the aggregates with the saturated water flow. The second objective was to study the relationships between the distribution and movement of E. coli within soil aggregates and the aggregates' internal pore structures. We studied aggregates from the top (A) horizon of conventionally tilled (CT) and no-till (NT) corn-soybean-wheat rotations and native succession vegetation (NS) treatments at NSF Long-Term Ecological Research site, southwest Michigan. The results confirmed that E. coli movement in soil aggregates was mainly driven by water flow via capillary forces. E. coli redistribution was most pronounced in CT aggregates, followed by NT, and was almost negligible in NS aggregates. Pore characteristics that positively contributed to E. coli redistribution through the aggregates were the maximum flow in the aggregate centers and the ratio of the maximum flow and pore tortuosity. The E. coli retention in the aggregate's centers was positively related to porosity, percent of medium and large pores, and pore tortuosity.
C1 [Wang, W.] Palo Alto Med Fdn, Res Inst, Palo Alto, CA 94301 USA.
[Kravchenko, A. N.; Johnson, T.; Ananyeva, K. A.; Smucker, A. J. M.; Rose, J. B.] Michigan State Univ, Dep Plant Soil & Microbial Sci, E Lansing, MI 48824 USA.
[Srinivasan, S.] Millikin Univ, Dep Biol, Decatur, IL 62522 USA.
[Rivers, M. L.] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, Argonne, IL 60439 USA.
RP Kravchenko, AN (reprint author), Michigan State Univ, Dep Plant Soil & Microbial Sci, E Lansing, MI 48824 USA.
EM kravche1@msu.edu
FU National Research Initiative of the USDA Cooperative State Research,
Education and Extension Service [32008-35102-04567]; NSF Long-Term
Ecological Research Program at the Kellogg Biological Station; Michigan
State University AgBioResearch; Michigan State University High
Performance Computing Center; Institute for Cyber-Enabled Research
FX The project was supported in part by the National Research Initiative of
the USDA Cooperative State Research, Education and Extension Service,
grant number 32008-35102-04567. Support for this research was also
provided by the NSF Long-Term Ecological Research Program at the Kellogg
Biological Station and by Michigan State University AgBioResearch. The
authors acknowledge the support of the Michigan State University High
Performance Computing Center and the Institute for Cyber-Enabled
Research.
NR 71
TC 2
Z9 2
U1 5
U2 35
PU SOIL SCI SOC AMER
PI MADISON
PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA
SN 1539-1663
J9 VADOSE ZONE J
JI Vadose Zone J.
PD NOV
PY 2013
VL 12
IS 4
DI 10.2136/vzj2013.01.0012
PG 14
WC Environmental Sciences; Soil Science; Water Resources
SC Environmental Sciences & Ecology; Agriculture; Water Resources
GA 274TF
UT WOS:000328628400025
ER
PT J
AU Li, HJ
Gao, XD
DeMartini, JD
Kumar, R
Wyman, CE
AF Li, Hongjia
Gao, Xiadi
DeMartini, Jaclyn D.
Kumar, Rajeev
Wyman, Charles E.
TI Application of High Throughput Pretreatment and Co-Hydrolysis System to
Thermochemical Pretreatment. Part 2: Dilute Alkali
SO BIOTECHNOLOGY AND BIOENGINEERING
LA English
DT Article
DE high throughput pretreatment and co-hydrolysis; dilute alkali;
application; biomass recalcitrance
ID SODIUM-HYDROXIDE; LIGNOCELLULOSIC BIOMASS; ENZYMATIC-HYDROLYSIS; AQUEOUS
AMMONIA; PERACETIC-ACID; EXPLOSION AFEX; ETHANOL; SWITCHGRASS; STOVER;
SACCHARIFICATION
AB High throughput pretreatment (HTPH) and enzymatic hydrolysis systems are now vital for screening large numbers of biomass samples to investigate biomass recalcitrance over various pretreatment and enzymatic hydrolysis conditions. Although hydrothermal pretreatment is currently being employed in most high throughput applications, thermochemical pretreatment at low and high pH conditions can offer additional insights to better understand the roles of hemicellulose and lignin, respectively, in defining biomass recalcitrance. Thus, after successfully applying the HTPH approach to dilute acid pretreatment [Gao et al. (2012) Biotechnol. Bioeng. 110(3): 754-762], extension to dilute alkali pretreatment was also achieved using a similar single-step neutralization and buffering concept. In the latter approach, poplar and switchgrass were pretreated with 1wt% sodium hydroxide at 120 degrees C for different reaction times. Following pretreatment, an H(2)Cit(-)/HCit(2-) buffer with a pH of 4.5 was used to condition the pretreatment slurry to a pH range of 4.69-4.89, followed by enzymatic hydrolysis for 72h of the entire mixture. Sugar yields showed different trends for poplar and switchgrass with increases in pretreatment times, demonstrating the method provided a clearly discernible screening tool at alkali conditions. This method was then applied to selected Populus tremuloides samples to follow ring-by-ring sugar release patterns. Observed variations were compared to results from hydrothermal pretreatments, providing new insights in understanding the influence of biomass structural differences on recalcitrance. Biotechnol. Bioeng. 2013;110: 2894-2901. (c) 2013 Wiley Periodicals, Inc.
C1 [Li, Hongjia; Gao, Xiadi; DeMartini, Jaclyn D.; Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Dept Chem & Environm Engn, Bourns Coll Engn, Riverside, CA 92521 USA.
[Li, Hongjia; Gao, Xiadi; DeMartini, Jaclyn D.; Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol CE CERT, Riverside, CA 92521 USA.
[Li, Hongjia; Gao, Xiadi; DeMartini, Jaclyn D.; Kumar, Rajeev; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN USA.
RP Wyman, CE (reprint author), Univ Calif Riverside, Dept Chem & Environm Engn, Bourns Coll Engn, 446 Winston Chung Hall,900 Univ Ave, Riverside, CA 92521 USA.
EM charles.wyman@ucr.edu
OI Kumar, Rajeev/0000-0001-7523-0108
FU BioEnergy Science Center (BESC); Ford Motor Company
FX Contract grant sponsor: BioEnergy Science Center (BESC); Contract grant
sponsor: Ford Motor Company
NR 31
TC 2
Z9 2
U1 1
U2 24
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0006-3592
EI 1097-0290
J9 BIOTECHNOL BIOENG
JI Biotechnol. Bioeng.
PD NOV
PY 2013
VL 110
IS 11
BP 2894
EP 2901
DI 10.1002/bit.24951
PG 8
WC Biotechnology & Applied Microbiology
SC Biotechnology & Applied Microbiology
GA 264FY
UT WOS:000327863600010
PM 23637060
ER
PT J
AU Novichkov, PS
Kazakov, AE
Ravcheev, DA
Leyn, SA
Kovaleva, GY
Sutormin, RA
Kazanov, MD
Riehl, W
Arkin, AP
Dubchak, I
Rodionov, DA
AF Novichkov, Pavel S.
Kazakov, Alexey E.
Ravcheev, Dmitry A.
Leyn, Semen A.
Kovaleva, Galina Y.
Sutormin, Roman A.
Kazanov, Marat D.
Riehl, William
Arkin, Adam P.
Dubchak, Inna
Rodionov, Dmitry A.
TI RegPrecise 3.0-A resource for genome-scale exploration of
transcriptional regulation in bacteria
SO BMC GENOMICS
LA English
DT Article
DE Regulatory network; Regulon; Transcription factor; Riboswitch;
Comparative genomics; Bacteria
ID BACILLUS-SUBTILIS; FAMILIES DATABASE; NAD METABOLISM; CENTRAL CARBON;
RECONSTRUCTION; NETWORKS; REGULONS; INFERENCE; ACID; PROTEOBACTERIA
AB Background: Genome-scale prediction of gene regulation and reconstruction of transcriptional regulatory networks in prokaryotes is one of the critical tasks of modern genomics. Bacteria from different taxonomic groups, whose lifestyles and natural environments are substantially different, possess highly diverged transcriptional regulatory networks. The comparative genomics approaches are useful for in silico reconstruction of bacterial regulons and networks operated by both transcription factors (TFs) and RNA regulatory elements (riboswitches).
Description: RegPrecise (http://regprecise.lbl.gov) is a web resource for collection, visualization and analysis of transcriptional regulons reconstructed by comparative genomics. We significantly expanded a reference collection of manually curated regulons we introduced earlier. RegPrecise 3.0 provides access to inferred regulatory interactions organized by phylogenetic, structural and functional properties. Taxonomy-specific collections include 781 TF regulogs inferred in more than 160 genomes representing 14 taxonomic groups of Bacteria. TF-specific collections include regulogs for a selected subset of 40 TFs reconstructed across more than 30 taxonomic lineages. Novel collections of regulons operated by RNA regulatory elements (riboswitches) include near 400 regulogs inferred in 24 bacterial lineages. RegPrecise 3.0 provides four classifications of the reference regulons implemented as controlled vocabularies: 55 TF protein families; 43 RNA motif families; similar to 150 biological processes or metabolic pathways; and similar to 200 effectors or environmental signals. Genome-wide visualization of regulatory networks and metabolic pathways covered by the reference regulons are available for all studied genomes. A separate section of RegPrecise 3.0 contains draft regulatory networks in 640 genomes obtained by an conservative propagation of the reference regulons to closely related genomes.
Conclusions: RegPrecise 3.0 gives access to the transcriptional regulons reconstructed in bacterial genomes. Analytical capabilities include exploration of: regulon content, structure and function; TF binding site motifs; conservation and variations in genome-wide regulatory networks across all taxonomic groups of Bacteria. RegPrecise 3.0 was selected as a core resource on transcriptional regulation of the Department of Energy Systems Biology Knowledgebase, an emerging software and data environment designed to enable researchers to collaboratively generate, test and share new hypotheses about gene and protein functions, perform large-scale analyses, and model interactions in microbes, plants, and their communities.
C1 [Novichkov, Pavel S.; Kazakov, Alexey E.; Kovaleva, Galina Y.; Sutormin, Roman A.; Riehl, William; Arkin, Adam P.; Dubchak, Inna] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94710 USA.
[Ravcheev, Dmitry A.; Leyn, Semen A.; Kovaleva, Galina Y.; Kazanov, Marat D.; Rodionov, Dmitry A.] Russian Acad Sci, AA Kharkevich Inst Informat Transmiss Problems, Moscow 127994, Russia.
[Ravcheev, Dmitry A.; Rodionov, Dmitry A.] Sanford Burnham Med Res Inst, La Jolla, CA 92037 USA.
[Sutormin, Roman A.] Moscow MV Lomonosov State Univ, Dept Bioengn & Bioinformat, Moscow 119992, Russia.
RP Novichkov, PS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94710 USA.
EM PSNovichkov@lbl.gov; rodionov@burnham.org
RI Kazanov, Marat/D-6381-2013; Arkin, Adam/A-6751-2008; Ravcheev,
Dmitry/M-6877-2015;
OI Kazanov, Marat/0000-0002-2314-5507; Arkin, Adam/0000-0002-4999-2931;
Ravcheev, Dmitry/0000-0002-8435-5516; Rodionov,
Dmitry/0000-0002-0939-390X
FU Genomic Science Program (GSP), Office of Biological and Environmental
Research (OBER), U.S. Department of Energy (DOE) [DE-SC0004999];
Sanford-Burnham Medical Research Institute (SBMRI); Lawrence Berkeley
National Laboratory (LBNL); ENIGMA Science Focus Area (SFA) at LBNL
[DE-AC02-05CH11231]; GSP Foundational Science Focus Area (FSFA) of the
Pacific Northwest National Laboratory (PNNL); Russian Foundation for
Basic Research [12-04-33003, 12-04-32098, 12-04-31939]; [8135]
FX This research was supported by the Genomic Science Program (GSP), Office
of Biological and Environmental Research (OBER), U.S. Department of
Energy (DOE) under contract DE-SC0004999 with Sanford-Burnham Medical
Research Institute (SBMRI) and Lawrence Berkeley National Laboratory
(LBNL), the ENIGMA Science Focus Area (SFA) at LBNL (contract
DE-AC02-05CH11231), and by the GSP Foundational Science Focus Area
(FSFA) of the Pacific Northwest National Laboratory (PNNL). Additional
funding was provided by Russian Foundation for Basic Research
(12-04-33003, 12-04-32098 and 12-04-31939). MDK was supported by State
Contract#8135 (application 2012-1.2.2-12-000-1013-079).
NR 41
TC 65
Z9 66
U1 4
U2 20
PU BIOMED CENTRAL LTD
PI LONDON
PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND
SN 1471-2164
J9 BMC GENOMICS
JI BMC Genomics
PD NOV 1
PY 2013
VL 14
AR 745
DI 10.1186/1471-2164-14-745
PG 12
WC Biotechnology & Applied Microbiology; Genetics & Heredity
SC Biotechnology & Applied Microbiology; Genetics & Heredity
GA 274WF
UT WOS:000328636200001
PM 24175918
ER
PT J
AU Kramer, R
Bochev, P
Siefert, C
Voth, T
AF Kramer, Richard
Bochev, Pavel
Siefert, Christopher
Voth, Tom
TI An extended finite element method with algebraic constraints (XFEM-AC)
for problems with weak discontinuities
SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING
LA English
DT Article
DE Finite element; X-FEM; Dirichlet boundary condition; Constraints; Weak
discontinuity
ID DIRICHLET BOUNDARY-CONDITIONS; INTERFACE PROBLEMS; PARTITION
AB We present a new extended finite element method with algebraic constraints (XFEM-AC) for recovering weakly discontinuous solutions across internal element interfaces. If necessary, cut elements are further partitioned by a local secondary cut into body-fitting subelements. Each resulting subelement contributes an enrichment of the parent element. The enriched solutions are then tied using algebraic constraints, which enforce C continuity across both cuts. These constraints impose equivalence of the enriched and body-fitted finite element solutions, and are the key differentiating feature of the XFEM-AC. In so doing, a stable mixed formulation is obtained without having to explicitly construct a compatible Lagrange multiplier space and prove a formal inf-sup condition. Likewise, convergence of the XFEM-AC solution follows from its equivalence to the interface-fitted finite element solution. This relationship is further exploited to improve the numerical solution of the resulting XFEM-AC linear system. Examples are shown demonstrating the new approach for both steady-state and transient diffusion problems. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Kramer, Richard; Bochev, Pavel; Siefert, Christopher; Voth, Tom] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Kramer, R (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM rmkrame@sandia.gov
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX Sandia National Laboratories is a multi-program laboratory managed and
operated by Sandia Corporation, a wholly owned subsidiary of Lockheed
Martin Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000.
NR 21
TC 5
Z9 5
U1 0
U2 7
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0045-7825
EI 1879-2138
J9 COMPUT METHOD APPL M
JI Comput. Meth. Appl. Mech. Eng.
PD NOV 1
PY 2013
VL 266
BP 70
EP 80
DI 10.1016/j.cma.2013.07.013
PG 11
WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary
Applications; Mechanics
SC Engineering; Mathematics; Mechanics
GA 277EK
UT WOS:000328801600005
ER
PT J
AU Seleson, P
Gunzburger, M
Parks, ML
AF Seleson, Pablo
Gunzburger, Max
Parks, Michael L.
TI Interface problems in nonlocal diffusion and sharp transitions between
local and nonlocal domains
SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING
LA English
DT Article
DE Nonlocal diffusion; Interface problems; Interface conditions; Multiscale
modeling
ID FINITE-ELEMENT-METHOD; BOUNDARY-VALUE-PROBLEMS; PHASE-TRANSITIONS;
INTEGRODIFFERENTIAL MODEL; VECTOR CALCULUS; PERIDYNAMICS; ELASTICITY;
APPROXIMATION; PRINCIPLE; EQUATIONS
AB We investigate interface problems in nonlocal diffusion and demonstrate how to reformulate and generalize the classical treatment of interface problems in the presence of nonlocal interactions. Through formal derivations, we show that nonlocal diffusion interface problems converge to their classical local counterparts, in the limit of vanishing nonlocality. A central focus of this paper is local/nonlocal interface problems, or interface problems with sharp transitions between local and nonlocal domains. Such problems can be cast as instances of a nonlocal interface problem, with a finite horizon in certain regions and a vanishing horizon in other regions. We derive a local/nonlocal interface problem and utilize conservation principles to obtain local/nonlocal interface conditions. Comparisons between nonlocal, local, and local/nonlocal interface problems are presented, analytically and numerically, with a focus on multiscale aspects of nonlocal models induced by their inherent length scales. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Seleson, Pablo] Inst Computat Engn & Sci, Austin, TX 78712 USA.
[Gunzburger, Max] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA.
[Parks, Michael L.] Sandia Natl Labs, Ctr Res Comp, Albuquerque, NM 87185 USA.
RP Seleson, P (reprint author), Inst Computat Engn & Sci, 201 East 24th St,Stop C0200, Austin, TX 78712 USA.
EM seleson@ices.utexas.edu; gunzburg@fsu.edu; mlparks@sandia.gov
OI Seleson, Pablo/0000-0003-3279-4231
FU DOE at Florida State University [DE-SC0004970]; DOE at the University of
Texas [DE-FG02-05ER25701]; Laboratory Directed Research and Development
program at Sandia National Laboratories; United States Department of
Energy [DE-AC0494-AL85000]; ICES Postdoctoral Fellowship Program
FX This research was supported by DOE Grant DE-SC0004970 at Florida State
University, by DOE Grant DE-FG02-05ER25701 at the University of Texas,
and by the Laboratory Directed Research and Development program at
Sandia National Laboratories. Sandia is a multiprogram laboratory
operated by Sandia Corporation, a Lockheed Martin Company, for the
United States Department of Energy under contract DE-AC0494-AL85000. We
acknowledge helpful discussions with David Littlewood, Stewart Silling,
Jakob Ostien, and Qiang Du. Pablo Seleson acknowledges support from the
ICES Postdoctoral Fellowship Program and useful discussions with Serge
Prudhomme and Leszek Demkowicz.
NR 50
TC 13
Z9 13
U1 0
U2 9
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0045-7825
EI 1879-2138
J9 COMPUT METHOD APPL M
JI Comput. Meth. Appl. Mech. Eng.
PD NOV 1
PY 2013
VL 266
BP 185
EP 204
DI 10.1016/j.cma.2013.05.018
PG 20
WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary
Applications; Mechanics
SC Engineering; Mathematics; Mechanics
GA 277EK
UT WOS:000328801600012
ER
PT J
AU Kogge, P
Shalf, J
AF Kogge, Peter
Shalf, John
TI Exascale Computing Trends: Adjusting to the "New Normal" for Computer
Architecture
SO COMPUTING IN SCIENCE & ENGINEERING
LA English
DT Article
C1 [Kogge, Peter] Univ Notre Dame, Notre Dame, IN 46556 USA.
[Kogge, Peter] Univ Notre Dame, Coll Engn, Notre Dame, IN 46556 USA.
[Shalf, John] Lawrence Berkeley Natl Lab, Berkeley, CA USA.
RP Kogge, P (reprint author), Univ Notre Dame, Notre Dame, IN 46556 USA.
EM kogge@cse.nd.edu; jshalf@lbl.gov
NR 13
TC 12
Z9 12
U1 0
U2 8
PU IEEE COMPUTER SOC
PI LOS ALAMITOS
PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA
SN 1521-9615
EI 1558-366X
J9 COMPUT SCI ENG
JI Comput. Sci. Eng.
PD NOV-DEC
PY 2013
VL 15
IS 6
BP 16
EP 26
PG 11
WC Computer Science, Interdisciplinary Applications
SC Computer Science
GA 275XA
UT WOS:000328711500003
ER
PT J
AU Gropp, W
Snir, M
AF Gropp, William
Snir, Marc
TI Programming for Exascale Computers
SO COMPUTING IN SCIENCE & ENGINEERING
LA English
DT Article
ID HIGH-LEVEL; PARALLEL; MODEL
C1 [Gropp, William] Univ Illinois, Dept Comp Sci, Urbana, IL USA.
[Gropp, William] Univ Illinois, Inst Adv Comp Applicat & Technol, Urbana, IL USA.
[Gropp, William] Univ Illinois, Parallel Comp Inst, Urbana, IL USA.
[Snir, Marc] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA.
RP Gropp, W (reprint author), Univ Illinois, Dept Comp Sci, Urbana, IL USA.
EM wgropp@illinois.edu; snir@illinois.edu
OI Gropp, William/0000-0003-2905-3029
FU US Department of Energy, Office of Science, Advanced Scientific
Computing Research [DE-AC02-06CH11357, DESC0004131]
FX This work was supported by the US Department of Energy, Office of
Science, Advanced Scientific Computing Research, under contract
DE-AC02-06CH11357 and under award DESC0004131. We thank Gail Pieper for
her careful review of this article.
NR 42
TC 6
Z9 6
U1 1
U2 3
PU IEEE COMPUTER SOC
PI LOS ALAMITOS
PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA
SN 1521-9615
EI 1558-366X
J9 COMPUT SCI ENG
JI Comput. Sci. Eng.
PD NOV-DEC
PY 2013
VL 15
IS 6
BP 27
EP 35
PG 9
WC Computer Science, Interdisciplinary Applications
SC Computer Science
GA 275XA
UT WOS:000328711500004
ER
PT J
AU Cervini-Silva, J
Nieto-Camacho, A
Cornejo-Garrido, H
del Angel, P
Maya, N
Palacios, E
Montoya, JA
Gomez-Vidales, V
Ramirez-Apan, MT
AF Cervini-Silva, Javiera
Nieto-Camacho, Antonio
Cornejo-Garrido, Hilda
del Angel, Paz
Maya, Noel
Palacios, Eduardo
Ascencion Montoya, Jose
Gomez-Vidales, Virginia
Teresa Ramirez-Apan, Maria
TI Biological dissolution and activity of the Allende meteorite
SO GEOLOGICAL SOCIETY OF AMERICA BULLETIN
LA English
DT Article
ID EXPERIMENTAL AQUEOUS ALTERATION; LIPID-PEROXIDATION; OXIDATIVE STRESS;
CARBONACEOUS CHONDRITES; EARLY EARTH; MAGNETOTACTIC BACTERIA; OXIDIZING
CONDITIONS; ORGANIC-MOLECULES; HYDROGEN-PEROXIDE; PYRITE OXIDATION
AB This paper reports on the effect of the Allende meteorite on the integrity of biological material and addresses the question whether it can induce cell damage via oxidative stress and cell mortality. The reaction mechanisms addressed herein are studied using electronparamagnetic resonance spectroscopy (EPR), high-resolution transmission electron microscopy, scanning electron microscopy and energy dispersive spectroscopy, high-resolution X-ray diffraction, and the assays for thiobarbituric acid reactive substances (TBARS) and cell viability using 3-(4,5)-dimethylthiazol-2-yel-2, 5-diphenyltetrazolium bromide (MTT bromide). As determined by the TBARS assay, Allende specimens induced cell damage via oxidative stress. The contents of TBARS in suspensions containing 1000 ppm of Allende and Fe 1-x S were 6.8 +/- 0.7 and 5.8 +/- 0.6 nmol/ mg protein, respectively. EPR experiments conducted on reaction mixtures containing Allende, 5,5-dimethyl-1pyrroline- N-oxide (DMPO), and H-2 O-2 showed a quartet signal, a 1:2:2: 1 intensity, and hyperfi ne coupling constants corresponding to a N = 1.49 mT and a H = 1.49 mT, a signature of the DMPO-OH adduct. The intensity of the signal depended on the concentration of the solids in suspension, while the formation of DMPO-OH was limited by H-2 O-2.
Experiments were conducted to test for the production of the DMPO-OH adduct from ferric ions, and the plausible generation of HO_. The role of ethanol (CH3 CH2 OH) as scavenger of HO_ in Allende-DMPO suspensions was addressed. Results showed a six-line spectra, with hyperfi ne coupling constants a N = 15.8 G, a H =22.6 G, and g =2.0059, consistent with the formation of the DMPO-CH(OH)-CH 3 adduct, but not DMPO-OCH2 CH3. We explain these fi ndings as the result of formation of HO_ onto (or in proximity to) the mineral surface, with CH3 CH2 OH competing with DMPO for HO8, and ferric iron playing a lesser role in DMPO transformation. Our fi ndings are congruent with reported radical-scavenging experiments for pyrite under anoxic conditions, concluding the formation of HO8 at surface defect sites.
Experiments conducted in Allende-desferrioxamine B(DFO-B) suspensions showed the inhibition of the formation of HO_, by means of decreases in the DMPO-OH adduct signal, accounted for by the reaction between Fe(II) and HO_ to form Fe(III) and competing reaction mechanisms at the structural Fe centers, confi rming that the production of HO8 radicals is associated with iron centers and contributes to mineral dissolution. Small-sized magnetite domains present were recognized as catalytic sites for the production of HO8 radicals. The.-Fe-3 O-4 domains present in the Allende matrix exhibited a submicron range, an elongated-hexagonal habit, and a high degree of crystallinity, supporting the presence of biogenic.-Fe-3 O-4. Cell viability was found to be susceptible to the distribution and atomic environment of structural Fe.
C1 [Cervini-Silva, Javiera] Univ Autonoma Metropolitana, Unidad Cuajimalpa, Dept Proc & Tecnol, Mexico City, DF, Mexico.
[Cervini-Silva, Javiera] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
[Nieto-Camacho, Antonio; Teresa Ramirez-Apan, Maria] Univ Nacl Autonoma Mexico, Inst Quim, Lab Pruebas Biol, Mexico City 04510, DF, Mexico.
[Cornejo-Garrido, Hilda] Univ Nacl Autonoma Mexico, Mexico City 04510, DF, Mexico.
[del Angel, Paz; Maya, Noel; Palacios, Eduardo; Ascencion Montoya, Jose] Inst Mexicano Petr, Direcc Invest & Posgrad, Mexico City 07730, DF, Mexico.
[Gomez-Vidales, Virginia] Univ Nacl Autonoma Mexico, Inst Quim, Lab Resonancia Magnet Nucl, Mexico City 04510, DF, Mexico.
RP Cervini-Silva, J (reprint author), Univ Autonoma Metropolitana, Unidad Cuajimalpa, Dept Proc & Tecnol, Artificios 40, Mexico City, DF, Mexico.
EM jcervini@correo.cua.uam.mx
FU UAM-C; Instituto Mexicano del Petroleo
FX This work would have not been possible without the assistance of
librarians M. R. Galindo Ortega and M. I. Escalante Vargas (Universidad
Autonoma Metropolitana Unidad Cuajimalpa, UAM-C), and M. Sc. Claudia
Rivera Cerecedo and Hactor Malagon Rivero (Bioterio, Instituto de
Fisiolog a Celular, Universidad Nacional Autonoma de Mexico, UNAM). This
project was supported by a grant from UAM-C and the Instituto Mexicano
del Petroleo.
NR 82
TC 3
Z9 3
U1 2
U2 13
PU GEOLOGICAL SOC AMER, INC
PI BOULDER
PA PO BOX 9140, BOULDER, CO 80301-9140 USA
SN 0016-7606
EI 1943-2674
J9 GEOL SOC AM BULL
JI Geol. Soc. Am. Bull.
PD NOV-DEC
PY 2013
VL 125
IS 11-12
BP 1865
EP 1873
DI 10.1130/B30791.1
PG 9
WC Geosciences, Multidisciplinary
SC Geology
GA 273BI
UT WOS:000328507400011
ER
PT J
AU Hames, MC
McFeeters, H
Holloway, WB
Stanley, CB
Urban, VS
McFeeters, RL
AF Hames, Mary C.
McFeeters, Hana
Holloway, W. Blake
Stanley, Christopher B.
Urban, Volker S.
McFeeters, Robert L.
TI Small Molecule Binding, Docking, and Characterization of the Interaction
between Pth1 and Peptidyl-tRNA
SO INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
LA English
DT Article
DE peptidyl-tRNA hydrolase; small angle neutron scattering;
enzyme-substrate complex; docking; inhibition
ID ESCHERICHIA-COLI; MINIGENE EXPRESSION; ANGSTROM RESOLUTION;
CRYSTAL-STRUCTURE; STRUCTURAL BASIS; HYDROLASE; SITE; INHIBITION;
CRYSTALLIZATION; ACCUMULATION
AB Bacterial Pth1 is essential for viability. Pth1 cleaves the ester bond between the peptide and nucleotide of peptidyl-tRNA generated from aborted translation, expression of mini-genes, and short ORFs. We have determined the shape of the Pth1:peptidyl-tRNA complex using small angle neutron scattering. Binding of piperonylpiperazine, a small molecule constituent of a combinatorial synthetic library common to most compounds with inhibitory activity, was mapped to Pth1 via NMR spectroscopy. We also report computational docking results, modeling piperonylpiperazine binding based on chemical shift perturbation mapping. Overall these studies promote Pth1 as a novel antibiotic target, contribute to understanding how Pth1 interacts with its substrate, advance the current model for cleavage, and demonstrate feasibility of small molecule inhibition.
C1 [Hames, Mary C.; McFeeters, Hana; Holloway, W. Blake; McFeeters, Robert L.] Univ Alabama, Dept Chem, Huntsville, AL 35899 USA.
[Stanley, Christopher B.; Urban, Volker S.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.
RP McFeeters, RL (reprint author), Univ Alabama, Dept Chem, 301 Sparkman Dr, Huntsville, AL 35899 USA.
EM mcg0001@uah.edu; hk0003@uah.edu; beb0004@uah.edu; stanleycb@ornl.gov;
urbanvs@ornl.gov; robert.mcfeeters@uah.edu
RI Urban, Volker/N-5361-2015;
OI Urban, Volker/0000-0002-7962-3408; Hames, Mary/0000-0002-7727-6238;
Stanley, Christopher/0000-0002-4226-7710
FU U.S. Department of Energy for neutron scattering research at Oak Ridge
National Laboratory
FX Support from the U.S. Department of Energy for neutron scattering
research at Oak Ridge National Laboratory was provided to the Center for
Structural Molecular Biology (Office of Biological and Environmental
Research) and the High Flux Isotope Reactor (Scientific User Facilities
Division, Office of Basic Energy Sciences).
NR 43
TC 7
Z9 7
U1 0
U2 13
PU MDPI AG
PI BASEL
PA POSTFACH, CH-4005 BASEL, SWITZERLAND
SN 1422-0067
J9 INT J MOL SCI
JI Int. J. Mol. Sci.
PD NOV
PY 2013
VL 14
IS 11
BP 22741
EP 22752
DI 10.3390/ijms141122741
PG 12
WC Biochemistry & Molecular Biology; Chemistry, Multidisciplinary
SC Biochemistry & Molecular Biology; Chemistry
GA 274RR
UT WOS:000328624400090
PM 24256814
ER
PT J
AU Creminelli, P
Perko, A
Senatore, L
Simonovic, M
Trevisan, G
AF Creminelli, Paolo
Perko, Ashley
Senatore, Leonardo
Simonovic, Marko
Trevisan, Gabriele
TI The physical squeezed limit: consistency relations at order q(2)
SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS
LA English
DT Article
DE inflation; non-gaussianity; cosmological perturbation theory
ID NON-GAUSSIANITY; INFLATION; MODEL
AB In single-field models of inflation the effect of a long mode with momentum q reduces to a diffeomorphism at zeroth and first order in q. This gives the well-known consistency relations for the n-point functions. At order q(2) the long mode has a physical effect on the short ones, since it induces curvature, and we expect that this effect is the same as being in a curved FRW universe. In this paper we verify this intuition in various examples of the three-point function, whose behaviour at order q(2) can be written in terms of the power spectrum in a curved universe. This gives a simple alternative understanding of the level of non-Gaussianity in single-field models. Non-Gaussianity is always parametrically enhanced when modes freeze at a physical scale k(ph), (f) shorter than H: f(NL) similar to (k(ph), (f)/H)(2).
C1 [Creminelli, Paolo] Abdus Salam Int Ctr Theoret Phys, I-34151 Trieste, Italy.
[Perko, Ashley; Senatore, Leonardo] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94306 USA.
[Senatore, Leonardo] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA.
[Senatore, Leonardo] SLAC, Menlo Pk, CA 94025 USA.
[Senatore, Leonardo] CERN, Div Theory, CH-1211 Geneva 23, Switzerland.
[Simonovic, Marko; Trevisan, Gabriele] SISSA, I-34136 Trieste, Italy.
[Simonovic, Marko; Trevisan, Gabriele] Ist Nazl Fis Nucl, Sez Trieste, I-34136 Trieste, Italy.
RP Creminelli, P (reprint author), Abdus Salam Int Ctr Theoret Phys, Str Costiera 11, I-34151 Trieste, Italy.
EM creminel@ictp.it; perko@stanford.edu; senatore@stanford.edu;
msimonov@sissa.it; gtrevi@sissa.it
OI Simonovic, Marko/0000-0003-1627-4842
FU Gabilan Stanford Graduate Fellowship; DOE Early Career Award
[DE-FG02-12ER41854]; NSF [PHY-1068380]
FX It is a pleasure to thank D. Lopez Nacir and Matias Zaldarriaga for
useful comments. Ashley Perko is supported by a Gabilan Stanford
Graduate Fellowship. Leonardo Senatore is supported by DOE Early Career
Award DE-FG02-12ER41854 and by NSF grant PHY-1068380.
NR 19
TC 15
Z9 15
U1 0
U2 1
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1475-7516
J9 J COSMOL ASTROPART P
JI J. Cosmol. Astropart. Phys.
PD NOV
PY 2013
IS 11
AR 015
DI 10.1088/1475-7516/2013/11/015
PG 20
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 263YM
UT WOS:000327843900016
ER
PT J
AU Morrison, CB
Schneider, MD
AF Morrison, Christopher B.
Schneider, Michael D.
TI On estimating cosmology-dependent covariance matrices
SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS
LA English
DT Article
DE redshift surveys; cosmological simulations; cosmological parameters from
LSS; weak gravitational lensing
ID POWER SPECTRUM COVARIANCE; GALAXY FORMATION; MODEL; SIMULATIONS;
STATISTICS; IMPACT; SPACE
AB We describe a statistical model to estimate the covariance matrix of matter tracer two-point correlation functions with cosmological simulations. Assuming a fixed number of cosmological simulation runs, we describe how to build a 'statistical emulator' of the two-point function covariance over a specified range of input cosmological parameters. Because the simulation runs with different cosmological models help to constrain the form of the covariance, we predict that the cosmology-dependent covariance may be estimated with a comparable number of simulations as would be needed to estimate the covariance for fixed cosmology. Our framework is a necessary first step in planning a simulations campaign for analyzing the next generation of cosmological surveys.
C1 [Morrison, Christopher B.; Schneider, Michael D.] Univ Calif Davis, Davis, CA 95616 USA.
[Schneider, Michael D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
RP Morrison, CB (reprint author), Univ Calif Davis, 1 Shields Ave, Davis, CA 95616 USA.
EM cbmorrison@ucdavis.edu; schneider42@llnl.gov
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; NSF [AST-1009514]
FX Part of this work performed under the auspices of the U.S. Department of
Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344. Christopher Morrison acknowledges the support of NSF
Grant AST-1009514.
NR 32
TC 0
Z9 0
U1 1
U2 5
PU IOP PUBLISHING LTD
PI BRISTOL
PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND
SN 1475-7516
J9 J COSMOL ASTROPART P
JI J. Cosmol. Astropart. Phys.
PD NOV
PY 2013
IS 11
DI 10.1088/1475-7516/2013/11/009
PG 19
WC Astronomy & Astrophysics; Physics, Particles & Fields
SC Astronomy & Astrophysics; Physics
GA 263YM
UT WOS:000327843900010
ER
PT J
AU Beyerlein, IJ
Caro, A
Demkowicz, MJ
Mara, NA
Misra, A
Uberuaga, BP
AF Beyerlein, I. J.
Caro, A.
Demkowicz, M. J.
Mara, N. A.
Misra, A.
Uberuaga, B. P.
TI Radiation damage tolerant nanomaterials
SO MATERIALS TODAY
LA English
DT Article
ID NANOSTRUCTURED FERRITIC ALLOYS; AUSTENITIC STAINLESS-STEEL;
ION-IRRADIATION; NANOCRYSTALLINE ALLOYS; NANOLAYERED COMPOSITES;
PLASTIC-DEFORMATION; BIMETAL INTERFACES; THERMAL-STABILITY;
GRAIN-BOUNDARIES; NANOPOROUS GOLD
AB Designing a material from the atomic level to achieve a tailored response in extreme conditions is a grand challenge in materials research. Nanostructured metals and composites provide a path to this goal because they contain interfaces that attract, absorb and annihilate point and line defects. These interfaces recover and control defects produced in materials subjected to extremes of displacement damage, impurity implantation, stress and temperature. Controlling radiation-induced-defects via interfaces is shown to be the key factor in reducing the damage and imparting stability in certain nanomaterials under conditions where bulk materials exhibit void swelling and/or embrittlement. We review the recovery of radiation-induced point defects at free surfaces and grain boundaries and stabilization of helium bubbles at interphase boundaries and present an approach for processing bulk nanocomposites containing interfaces that are stable under irradiation.
C1 [Beyerlein, I. J.; Mara, N. A.; Misra, A.; Uberuaga, B. P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Demkowicz, M. J.] MIT, Cambridge, MA 02139 USA.
RP Mara, NA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM amisra@lanl.gov
RI Mara, Nathan/J-4509-2014; Beyerlein, Irene/A-4676-2011; Misra,
Amit/H-1087-2012
OI Mara, Nathan/0000-0002-9135-4693;
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences (DOE/BES) [2008LANL1026]; Center for Materials at Irradiation
and Mechanical Extremes, an Energy Frontier Research Center
FX This work was supported by the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences (DOE/BES) under Award No.
2008LANL1026 through the Center for Materials at Irradiation and
Mechanical Extremes, an Energy Frontier Research Center. Access to the
Center for Integrated Nanotechnologies, a DOE/BES sponsored user
facility is acknowledged. Work on nanoporous metal synthesis was
supported by LANL-LDRD program. Authors acknowledge discussions with
R.G. Hoagland, J.P. Hirth, W.D. Nix, G.R. Odette, M. Nastasi, M.I.
Baskes, A. Sutton, F. Williame, A.D. Rollett, R.S. Averback, P. Bellon,
and T.M. Pollock.
NR 81
TC 84
Z9 86
U1 24
U2 170
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 1369-7021
EI 1873-4103
J9 MATER TODAY
JI Mater. Today
PD NOV
PY 2013
VL 16
IS 11
BP 443
EP 449
DI 10.1016/j.mattod.2013.10.019
PG 7
WC Materials Science, Multidisciplinary
SC Materials Science
GA 274XO
UT WOS:000328639700018
ER
PT J
AU Ellern, I
Venkatasubramanian, A
Lee, JH
Hesketh, P
Stavila, V
Robinson, A
Allendorf, M
AF Ellern, Ilya
Venkatasubramanian, Anandram
Lee, Jin-Hwan
Hesketh, Peter
Stavila, Vitalie
Robinson, Alex
Allendorf, Mark
TI HKUST-1 coated piezoresistive microcantilever array for volatile organic
compound sensing
SO MICRO & NANO LETTERS
LA English
DT Article
DE adsorption; cantilevers; chemical sensors; copper compounds;
microsensors; organic compounds; piezoresistive devices; thin films;
transducers; microfabrication; temperature 293 K to 298 K; microporous
MOF coatings; low power operation; single chip sensing system;
reversible response; response time constants; characteristic response
features; methanol; water vapour; stress-induced piezoresistive
microcantilever array sensors; carrier gas; dry nitrogen; layer-by-layer
techniques; thin films; N-doped piezoresistive cantilever arrays;
electrical signals; surface strain; transduction mechanism; analyte
adsorption; mechanical strain; internal surface area; HKUST-1
metal-organic framework; volatile organic compound sensing; HKUST-1
coated piezoresistive microcantilever array
ID FRAMEWORK MATERIALS; CHEMICAL-DETECTION; SENSORS
AB The HKUST-1 metal-organic framework (MOF) was selected because of the large internal surface area, excellent stability and known properties. Mechanical strain is generated upon the adsorption of analytes into the MOF; it is proportional to concentration and is a function of adsorbed species. Piezoresistive microcantilevers serve as a transduction mechanism to convert surface strain into electrical signals. N-doped piezoresistive cantilever arrays were fabricated with ten structures per die. Thin films of HKUST-1 were grown at room temperature using layer-by-layer techniques. Dry nitrogen was used as a carrier gas to expose devices to varying concentrations of 12 different volatile organic compounds (VOCs). Results show that stress-induced piezoresistive microcantilever array sensors with MOF coatings can provide a highly sensitive and reversible sensing mechanism for water vapour and methanol. Characteristic response features allow discrimination based on shape, response time constants and magnitude of response for other VOCs. Devices provided reliable data and proved durable over 18 months of testing. The key advantages of this type of sensor are higher sensitivity with a microporous MOFs, reversible response, single chip sensing system and low power operation.
C1 [Ellern, Ilya; Venkatasubramanian, Anandram; Lee, Jin-Hwan; Hesketh, Peter] Georgia Inst Technol, Dept Mech Engn, Atlanta, GA 30332 USA.
[Lee, Jin-Hwan] Intel Corp, Rio Rancho, NM 87124 USA.
[Stavila, Vitalie; Allendorf, Mark] Sandia Natl Labs, Livermore, CA 94551 USA.
[Robinson, Alex] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Ellern, I (reprint author), Georgia Inst Technol, Dept Mech Engn, Atlanta, GA 30332 USA.
EM peter.hesketh@me.gatech.edu
FU Sandia Laboratory Directed Research and Development (LDRD) Program
FX This work was supported by the Sandia Laboratory Directed Research and
Development (LDRD) Program. The technical assistance of G. Spinner and
K. Martin at the Nanotechnology Research Centre is gratefully
acknowledged.
NR 21
TC 7
Z9 8
U1 7
U2 89
PU INST ENGINEERING TECHNOLOGY-IET
PI HERTFORD
PA MICHAEL FARADAY HOUSE SIX HILLS WAY STEVENAGE, HERTFORD SG1 2AY, ENGLAND
SN 1750-0443
J9 MICRO NANO LETT
JI Micro Nano Lett.
PD NOV
PY 2013
VL 8
IS 11
BP 766
EP 769
DI 10.1049/mnl.2013.0390
PG 4
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 257ZC
UT WOS:000327425500004
ER
PT J
AU Martin, MJ
AF Martin, M. J.
TI Nuclear Data Sheets for A=152
SO NUCLEAR DATA SHEETS
LA English
DT Article
ID RARE-EARTH NUCLEI; HIGH-SPIN STATES; CONTINUUM GAMMA-RAYS; INELASTIC
DEUTERON SCATTERING; EVEN SAMARIUM ISOTOPES; ELECTRON PARTICLE
PARAMETERS; THERMAL-NEUTRON CAPTURE; NEGATIVE-PARITY STATES; HIGH
ANGULAR-MOMENTUM; LOW-LYING STATES
AB Detailed level schemes, decay schemes, and the experimental data on which they are based are presented for all nuclei with mass number A=152. The experimental data are evaluated; inconsistencies and discrepancies are noted; and adopted values for level and gamma-ray energies, gamma intensities, as well as for other nuclear properties are given. This evaluation replaces the A=152 evaluation published by Agda Artna-Cohen in Nuclear Data Sheets 79, 1 (1996) and the evaluation for Dy-152 prepared by Balraj Singh and published in Nuclear Data Sheets 95, 995 (2002).
C1 Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Martin, MJ (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
FU Oak Ridge National Laboratory [DE-AC05-00OR22725]
FX Research sponsored by the Oak Ridge National Laboratory, managed by
UT-Battelle, LLC for the US Department of Energy under contract number
DE-AC05-00OR22725.
NR 622
TC 17
Z9 17
U1 0
U2 6
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0090-3752
EI 1095-9904
J9 NUCL DATA SHEETS
JI Nucl. Data Sheets
PD NOV
PY 2013
VL 114
IS 11
BP 1497
EP 1847
DI 10.1016/j.nds.2013.11.001
PG 351
WC Physics, Nuclear
SC Physics
GA 257VY
UT WOS:000327417100001
ER
PT J
AU Mullen, JC
Buric, MP
Chorpening, BT
Woodruff, SD
AF Mullen, Jessica C.
Buric, Michael P.
Chorpening, Benjamin T.
Woodruff, Steven D.
TI Azimuthal polarization for Raman enhancement in capillary waveguides
SO OPTICAL ENGINEERING
LA English
DT Article
DE hollow waveguide; Raman spectroscopy; azimuthal polarization; radial
polarization; gas sensing; spiral phase plate
ID GENERATION; LIGHT; LASER; BEAMS; MODE
AB Hollow, metal-lined capillary waveguides have recently been utilized in spontaneous gas-Raman spectroscopy to improve signal strength and response time. The hollow waveguide is used to contain the sample gases, efficiently propagate a pump beam, and efficiently collect Raman scattering from those gases. Transmission losses in the waveguide may be reduced by using an azimuthally polarized pump beam instead of a linearly or radially polarized pump. This will lead to improved Raman signal strength, accuracy, and response time in waveguide-based Raman gas-composition sensors. A linearly polarized laser beam is azimuthally polarized using passive components including a spiral phase plate and an azimuthal-type linear analyzer element. Half-wave plates are then used to switch between the azimuthally polarized beam and the radially polarized beam with no change in input pump power. The collected Raman signal strength and laser throughput are improved when the azimuthally polarized pump is used. Optimization of the hollow waveguide Raman gas sensor is discussed with respect to incident pump polarization. (C) 2013 Society of Photo-Optical Instrumentation Engineers (SPIE)
C1 [Mullen, Jessica C.; Buric, Michael P.; Chorpening, Benjamin T.; Woodruff, Steven D.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
RP Mullen, JC (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA.
EM Michael.Buric@netl.doe.gov
FU NETL-Strategic Center for Coal's Cross Cutting Research Program
FX This research was performed at the National Energy Technology Laboratory
(NETL) through the Innovative Process Technology Field Work Proposal and
supported by NETL-Strategic Center for Coal's Cross Cutting Research
Program with Patricia Rawls as Technical Program Monitor and Robert
Romanosky as Technology Manager. Author J. Mullen gratefully
acknowledges her appointment to NETL through the US Department of Energy
Oak Ridge Institute for Science and Education (ORISE) program.
NR 21
TC 2
Z9 2
U1 1
U2 14
PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS
PI BELLINGHAM
PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA
SN 0091-3286
EI 1560-2303
J9 OPT ENG
JI Opt. Eng.
PD NOV
PY 2013
VL 52
IS 11
AR 117103
DI 10.1117/1.OE.52.11.117103
PG 7
WC Optics
SC Optics
GA 278NY
UT WOS:000328898200044
ER
PT J
AU Hussain, H
Malik, SUR
Hameed, A
Khan, SU
Bickler, G
Min-Allah, N
Qureshi, MB
Zhang, LM
Wang, YJ
Ghani, N
Kolodziej, J
Zomaya, AY
Xu, CZ
Balaji, P
Vishnu, A
Pinel, F
Pecero, JE
Kliazovich, D
Bouvry, P
Li, HX
Wang, LZ
Chen, D
Rayes, A
AF Hussain, Hameed
Malik, Saif Ur Rehman
Hameed, Abdul
Khan, Samee Ullah
Bickler, Gage
Min-Allah, Nasro
Qureshi, Muhammad Bilal
Zhang, Limin
Wang Yongji
Ghani, Nasir
Kolodziej, Joanna
Zomaya, Albert Y.
Xu, Cheng-Zhong
Balaji, Pavan
Vishnu, Abhinav
Pinel, Fredric
Pecero, Johnatan E.
Kliazovich, Dzmitry
Bouvry, Pascal
Li, Hongxiang
Wang, Lizhe
Chen, Dan
Rayes, Ammar
TI A survey on resource allocation in high performance distributed
computing systems
SO PARALLEL COMPUTING
LA English
DT Review
DE Scheduling; Resource allocation; Resource management
ID MANAGEMENT SYSTEMS; GRID ENVIRONMENT; OPERATING SYSTEM; CLUSTER;
TAXONOMY; SERVICES; INFRASTRUCTURE; OPTIMIZATION; ARCHITECTURE;
DISCOVERY
AB An efficient resource allocation is a fundamental requirement in high performance computing (HPC) systems. Many projects are dedicated to large-scale distributed computing systems that have designed and developed resource allocation mechanisms with a variety of architectures and services. In our study, through analysis, a comprehensive survey for describing resource allocation in various HPCs is reported. The aim of the work is to aggregate under a joint framework, the existing solutions for HPC to provide a thorough analysis and characteristics of the resource management and allocation strategies. Resource allocation mechanisms and strategies play a vital role towards the performance improvement of all the HPCs classifications. Therefore, a comprehensive discussion of widely used resource allocation strategies deployed in HPC environment is required, which is one of the motivations of this survey. Moreover, we have classified the HPC systems into three broad categories, namely: (a) cluster, (b) grid, and (c) cloud systems and define the characteristics of each class by extracting sets of common attributes. All of the aforementioned systems are cataloged into pure software and hybrid/hardware solutions. The system classification is used to identify approaches followed by the implementation of existing resource allocation strategies that are widely presented in the literature. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Hussain, Hameed; Min-Allah, Nasro; Qureshi, Muhammad Bilal] COMSATS Inst Informat Technol, Islamabad 44000, Pakistan.
[Malik, Saif Ur Rehman; Hameed, Abdul; Khan, Samee Ullah; Bickler, Gage; Zhang, Limin] N Dakota State Univ, Fargo, ND 58108 USA.
[Wang Yongji] Chinese Acad Sci, Inst Software, Beijing, Peoples R China.
[Ghani, Nasir] Univ S Florida, Tampa, FL 33620 USA.
[Kolodziej, Joanna] Krakow Tech Univ, PL-31155 Krakow, Poland.
[Zomaya, Albert Y.] Univ Sydney, Sydney, NSW 2006, Australia.
[Xu, Cheng-Zhong] Wayne State Univ, Detroit, MI USA.
[Balaji, Pavan] Argonne Natl Lab, Argonne, IL 60439 USA.
[Vishnu, Abhinav] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Pinel, Fredric; Pecero, Johnatan E.; Kliazovich, Dzmitry; Bouvry, Pascal] Univ Luxembourg, L-1359 Luxembourg, Luxembourg.
[Li, Hongxiang] Univ Louisville, Louisville, KY 40292 USA.
[Wang, Lizhe] Chinese Acad Sci, Ctr Earth Observat & Digital Earth, Beijing, Peoples R China.
[Chen, Dan] China Univ Geosci, Wuhan 430074, Peoples R China.
[Rayes, Ammar] CISCO Syst, San Jose, CA USA.
RP Khan, SU (reprint author), N Dakota State Univ, Dept Elect & Comp Engn, Fargo, ND 58108 USA.
EM ham.hamdard@gmail.com; saif.rehmanmalik@ndsu.edu; abdul.hameed@ndsu.edu;
samee.khan@ndsu.edu; gage.n.bickler@ndsu.edu; nasar@comsats.edu.pk;
muhdbilal.qureshi@gmail.com; limin.zhang@ndsu.edu;
ywang@itechs.iscas.ac.cn; nghani@usf.edu; jkolodziej@uck.pk.edu.pl;
albert.zomaya@sydney.edu.au; czxu@wayne.edu; balaji@mcs.anl.gov;
abhinav.vishnu@pnl.gov; fredric.pinel@uni.lu; johnatan.pecero@uni.lu;
dzmitry.kliazovich@uni.lu; pascal.bouvry@uni.lu; h.li@louisville.edu;
lzwang@ceode.ac.cn; chendan@pmail.ntu.edu.sg; rayes@cisco.com
RI min-allah, nasro /A-3717-2015;
OI min-allah, nasro /0000-0002-3961-5956; Kolodziej,
Joanna/0000-0002-5181-8713; Bouvry, Pascal/0000-0001-9338-2834; Malik,
Saif Ur Rehman/0000-0001-8195-1630; Wang, Lizhe/0000-0003-2766-0845
NR 122
TC 25
Z9 26
U1 4
U2 40
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0167-8191
EI 1872-7336
J9 PARALLEL COMPUT
JI Parallel Comput.
PD NOV
PY 2013
VL 39
IS 11
BP 709
EP 736
DI 10.1016/j.parco.2013.09.009
PG 28
WC Computer Science, Theory & Methods
SC Computer Science
GA 275GB
UT WOS:000328663200004
ER
PT J
AU Nikiforov, MP
Darling, SB
AF Nikiforov, Maxim P.
Darling, Seth B.
TI Improved conductive atomic force microscopy measurements on organic
photovoltaic materials via mitigation of contact area uncertainty
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE organic photovoltaics; conductive AFM; charge transport; contact
mechanics
ID NANOSCALE CHARGE-TRANSPORT; NORMAL RANDOM-VARIABLES; SOLAR-CELLS;
BULK-HETEROJUNCTION; ACOUSTIC MICROSCOPY; CLAY NANOCOMPOSITES; FILMS;
MORPHOLOGY; POLYMERS; RATIO
AB Physical processes that lead to conversion of light into electrical energy inside photovoltaic devices happen at the nanoscale. Therefore, understanding of electrical properties of photovoltaic materials at this length scale is of paramount importance for improvement of device performance. In this paper, we describe and validate a new framework for high-resolution quantitative measurements of electrical and mechanical properties of compliant materials with sub-100-nm resolution. Previous approaches have generally suffered from uncertainty in the quantitative level of contact between the probe and the material being measured; the methodology presented here overcomes this obstacle. We use the broadly studied ITO/PEDOT:PSS/P3HT:PC61BM system as an example to illustrate variability of chemical composition and electrical properties of the active layer at hundred-nanometers and micrometer length scales. Copyright (c) 2012 John Wiley & Sons, Ltd.
C1 [Nikiforov, Maxim P.; Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Chicago, IL USA.
RP Nikiforov, MP (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, Chicago, IL USA.
EM maximnik@anl.gov
FU Director's Fellowship Program; U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX MPN is grateful to the Director's Fellowship Program for financial
support. MPN wants to thank Dr Yu-Chih Tseng for help with development
of the protocol for solar cell processing. Use of the Center for
Nanoscale Materials was supported by the U.S. Department of Energy,
Office of Science, Office of Basic Energy Sciences, under contract No.
DE-AC02-06CH11357.
NR 59
TC 9
Z9 9
U1 1
U2 30
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
EI 1099-159X
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD NOV
PY 2013
VL 21
IS 7
BP 1433
EP 1443
DI 10.1002/pip.2217
PG 11
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 270PH
UT WOS:000328330300001
ER
PT J
AU Hoff, TE
Perez, R
Kleissl, J
Renne, D
Stein, J
AF Hoff, Thomas E.
Perez, Richard
Kleissl, Jan
Renne, David
Stein, Joshua
TI Reporting of irradiance modeling relative prediction errors
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE irradiance; model; accuracy; percent error
AB Metrics used in assessing irradiance model accuracy, such as root mean square error and mean absolute error, are precisely defined. Their relative (%) counterpart, however, can be subject to interpretation and may cover a wide range of values for a given set of data depending on reporting practice. This note evaluates different approaches for the reporting of relative metrics quantifying the dispersion accuracy of a model and formulates recommendations for the most appropriate approach. Copyright (c) 2012 John Wiley & Sons, Ltd.
C1 [Hoff, Thomas E.] Clean Power Res, Napa, CA USA.
[Perez, Richard] SUNY Albany, ASRC, Albany, NY 12222 USA.
[Kleissl, Jan] Univ Calif San Diego, Jacob Sch Engn, San Diego, CA 92103 USA.
[Renne, David] NREL, Golden, CO USA.
[Stein, Joshua] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Perez, R (reprint author), SUNY Albany, ASRC, Albany, NY 12222 USA.
EM perez@asrc.cestm.albany.edu
NR 9
TC 13
Z9 13
U1 2
U2 9
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
EI 1099-159X
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD NOV
PY 2013
VL 21
IS 7
BP 1514
EP 1519
DI 10.1002/pip.2225
PG 6
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 270PH
UT WOS:000328330300008
ER
PT J
AU Hummon, M
Denholm, P
Margolis, R
AF Hummon, Marissa
Denholm, Paul
Margolis, Robert
TI Impact of photovoltaic orientation on its relative economic value in
wholesale energy markets
SO PROGRESS IN PHOTOVOLTAICS
LA English
DT Article
DE photovoltaic; wholesale electricity market; photovoltaic performance;
azimuth; PV economic value; PV orientation
ID SOLAR-RADIATION; SYSTEMS; PV; OPTIMIZATION; AZIMUTH; TILT
AB Most calculations of optimum photovoltaic (PV) performance focus on maximizing annual energy production. However, given the seasonally and daily time varying electricity demand and resulting variation in price, the PV orientation resulting in maximum energy yield may not yield the maximum economic benefit. With the use of historical solar irradiance and wholesale market prices for several locations in the USA, we evaluate the benefits of a variety of orientations for fixed and tracking PV arrays. We find that orienting fixed arrays slightly to the west of due south generally increases their economic value in the simulated systems because the reduced generation on an annual basis is more than offset by increased generation in high-value hours in late summer afternoons. However, this effect is small, typically providing an increase in value from 1% to 5%. The economic value of adjusting the orientation semi-annually (May 1st and September 1st) and monthly shows a modest increase in value from 3% to 5%. Several other implications of this analysis are also discussed. Copyright (c) 2012 John Wiley & Sons, Ltd.
C1 [Hummon, Marissa; Denholm, Paul; Margolis, Robert] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO USA.
RP Hummon, M (reprint author), Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO USA.
EM marissa.hummon@nrel.gov
NR 15
TC 13
Z9 13
U1 1
U2 13
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1062-7995
EI 1099-159X
J9 PROG PHOTOVOLTAICS
JI Prog. Photovoltaics
PD NOV
PY 2013
VL 21
IS 7
BP 1531
EP 1540
DI 10.1002/pip.2198
PG 10
WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied
SC Energy & Fuels; Materials Science; Physics
GA 270PH
UT WOS:000328330300010
ER
PT J
AU Geng, J
Navon, IM
Chen, X
AF Geng, Jian
Navon, I. Michael
Chen, Xiao
TI Non-parametric calibration of the local volatility surface for European
options using a second-order Tikhonov regularization (vol 14, pg 73,
2014)
SO QUANTITATIVE FINANCE
LA English
DT Correction
C1 [Geng, Jian] Florida State Univ, Dept Math, Tallahassee, FL 32306 USA.
[Navon, I. Michael] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA.
[Chen, Xiao] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA USA.
RP Geng, J (reprint author), Florida State Univ, Dept Math, Tallahassee, FL 32306 USA.
RI Navon, Ionel/A-5173-2008
OI Navon, Ionel/0000-0001-7830-7094
NR 1
TC 0
Z9 0
U1 0
U2 0
PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXFORDSHIRE, ENGLAND
SN 1469-7688
EI 1469-7696
J9 QUANT FINANC
JI Quant. Financ.
PD NOV 1
PY 2013
VL 13
IS 11
DI 10.1080/14697688.2013.844894
PG 1
WC Business, Finance; Economics; Mathematics, Interdisciplinary
Applications; Social Sciences, Mathematical Methods
SC Business & Economics; Mathematics; Mathematical Methods In Social
Sciences
GA 268XN
UT WOS:000328204100013
ER
PT J
AU Ginn, TR
Nassar, MK
Kamai, T
Klise, K
Tidwell, V
McKenna, S
AF Ginn, Timothy R.
Nassar, Mohamed K.
Kamai, Tamir
Klise, Katherine
Tidwell, Vince
McKenna, Sean
TI On a recent solute transport laboratory experiment involving sandstone
and its modeling
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE solute transport; anomalous dispersion; modeling
ID SCALES; SLAB
AB We analyze and simulate laboratory data on flow and solute transport in a submeter scale sample of Massillon sandstone and we re-evaluate studies that have stated that these data indicate a failure of the advection-dispersion, and that nonlocal modeling approaches are necessary. Our examination reveals experimental issues including artificial edge effects in the data, as well as inconsistency in the measured solute injection rates. When the edge effects are removed the data no longer exhibit power-law tailing. Our simulations show that failure of the advection-dispersion equation has not been demonstrated and that nonlocal approaches are not necessary.
C1 [Ginn, Timothy R.; Nassar, Mohamed K.; Kamai, Tamir] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA.
[Nassar, Mohamed K.] Univ Sadat City, Environm Studies & Res Inst, Sadat, Minufiya, Egypt.
[Klise, Katherine; Tidwell, Vince; McKenna, Sean] Sandia Natl Labs, Albuquerque, NM USA.
[McKenna, Sean] IBM Res, Smarter Cities Technol Ctr, Dublin, Ireland.
RP Ginn, TR (reprint author), Univ Calif Davis, Dept Civil & Environm Engn, 1 Shields Ave, Davis, CA 95616 USA.
EM trginn@ucdavis.edu
RI Kamai, Tamir/G-6591-2015
FU National Science Foundation [1114257, 1234367, 1215756]; U.S. Department
of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]
FX The assistance in data preparation and graphics by Andrew Benjamin and
Diego de la Torre is much appreciated. This material is based in part
upon work supported by the National Science Foundation under grant
1114257, 1234367, and 1215756. Sandia National Laboratories is a
multiprogram laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
Department of Energy's National Nuclear Security Administration under
contract DE-AC04-94AL85000.
NR 15
TC 2
Z9 2
U1 0
U2 5
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
EI 1944-7973
J9 WATER RESOUR RES
JI Water Resour. Res.
PD NOV
PY 2013
VL 49
IS 11
BP 7327
EP 7338
DI 10.1002/2013WR013729
PG 12
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 275NJ
UT WOS:000328683800011
ER
PT J
AU Visser, A
Broers, HP
Purtschert, R
Sultenfuss, J
de Jonge, M
AF Visser, Ate
Broers, Hans Peter
Purtschert, Roland
Sueltenfuss, Juergen
de Jonge, Martin
TI Groundwater age distributions at a public drinking water supply well
field derived from multiple age tracers (Kr-85, H-3/He-3, and Ar-39)
SO WATER RESOURCES RESEARCH
LA English
DT Article
DE public supply wells; groundwater age; transit times; noble gases;
tritium-helium; krypton-85; argon-39
ID HETEROGENEOUS UNCONFINED AQUIFERS; DATING YOUNG GROUNDWATER;
ENVIRONMENTAL TRACERS; CAPTURE ZONES; TRAVEL-TIME; HYDROLOGIC TRACERS;
PARTICLE-TRACKING; SCALE DISPERSION; MODELING FLOW; NOBLE-GASES
AB Groundwater age is a key aspect of production well vulnerability. Public drinking water supply wells typically have long screens and are expected to produce a mixture of groundwater ages. The groundwater age distributions of seven production wells of the Holten well field (Netherlands) were estimated from tritium-helium (H-3/He-3), krypton-85 (Kr-85), and argon-39 (Ar-39), using a new application of a discrete age distribution model and existing mathematical models, by minimizing the uncertainty-weighted squared differences of modeled and measured tracer concentrations. The observed tracer concentrations fitted well to a 4-bin discrete age distribution model or a dispersion model with a fraction of old groundwater. Our results show that more than 75% of the water pumped by four shallow production wells has a groundwater age of less than 20 years and these wells are very vulnerable to recent surface contamination. More than 50% of the water pumped by three deep production wells is older than 60 years. H-3/He-3 samples from short screened monitoring wells surrounding the well field constrained the age stratification in the aquifer. The discrepancy between the age stratification with depth and the groundwater age distribution of the production wells showed that the well field preferentially pumps from the shallow part of the aquifer. The discrete groundwater age distribution model appears to be a suitable approach in settings where the shape of the age distribution cannot be assumed to follow a simple mathematical model, such as a production well field where wells compete for capture area.
C1 [Visser, Ate] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Broers, Hans Peter] Deltares, Unit Soil & Groundwater Syst, Utrecht, Netherlands.
[Broers, Hans Peter] Geol Survey Netherlands, TNO, Utrecht, Netherlands.
[Broers, Hans Peter; de Jonge, Martin] Vrije Univ Amsterdam, Crit Zone Hydrol Grp, Amsterdam, Netherlands.
[Purtschert, Roland] Univ Bern, Bern, Switzerland.
[Sueltenfuss, Juergen] Univ Bremen, Inst Environm Phys, Dept Oceanog, D-28359 Bremen, Germany.
[de Jonge, Martin] Vitens Water, Zwolle, Netherlands.
RP Visser, A (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA.
EM visser3@llnl.gov
RI Visser, Ate/G-8826-2012; Purtschert, Roland/N-7108-2016
OI Purtschert, Roland/0000-0002-4734-7664
FU Department of Economic Affairs of the Netherlands; U. S. Department of
Energy; Lawrence Livermore National Laboratory [DE-AC52-07NA27344,
LLNL-JRNL-635812]
FX The authors are grateful for the permission, support, and funding (25%)
from Vitens Water, owner and operator of the Holten well field. This
study was cofunded by the Department of Economic Affairs of the
Netherlands. We appreciate the support of "Bundesamt fur Strahlenschutz
(Germany)'' that provided the measurements of the atmospheric
85Kr input activities. We thank Kip Solomon and Alan Rigby
for providing thoughtful discussion on the interpretation of the
diffusion sampler data. Elaborate comments from W. Aeschbach-Hertig, two
anonymous reviewers, and the Associate Editor enabled us to improve the
quality of the manuscript. Part of this work was performed under the
auspices of the U. S. Department of Energy by Lawrence Livermore
National Laboratory under contract DE-AC52-07NA27344. LLNL-JRNL-635812.
NR 94
TC 19
Z9 20
U1 6
U2 32
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 0043-1397
EI 1944-7973
J9 WATER RESOUR RES
JI Water Resour. Res.
PD NOV
PY 2013
VL 49
IS 11
BP 7778
EP 7796
AR 7778-7796
DI 10.1002/2013WR014012
PG 19
WC Environmental Sciences; Limnology; Water Resources
SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water
Resources
GA 275NJ
UT WOS:000328683800044
ER
PT J
AU Du, P
Luszczek, P
Tomov, S
Dongarra, J
AF Du, Peng
Luszczek, Piotr
Tomov, Stan
Dongarra, Jack
TI Soft error resilient QR factorization for hybrid system with GPGPU
SO JOURNAL OF COMPUTATIONAL SCIENCE
LA English
DT Article
DE Fault tolerance; Soft error; QR factorization; High performance
computing; Hybrid algorithm
ID MATRIX TRIANGULARIZATIONS; FAULT TOLERANCE; LINEAR ALGEBRA
AB The general purpose graphics processing units (GPGPUs) are increasingly deployed for scientific computing due to their performance advantages over CPUs. What followed is the fact that fault tolerance has become a more serious concern compared to the period when GPGPUs were used exclusively for graphics applications. Using CPUs and CPUs together in a hybrid computing system increases flexibility and performance but also increases the possibility of the computations being affected by soft errors, for example, in the form of bit flips. In this work, we propose a soft error resilient algorithm for QR factorization on such hybrid systems. Our contributions include: (1) a checkpointing and recovery mechanism for the left-factor Q whose performance is scalable on hybrid systems; (2) optimized Givens rotation utilities on GPGPUs to efficiently reduce an upper Hessenberg matrix to an upper triangular form for the protection of the right factor R; and (3) a recovery algorithm based on QR update on GPGPUs. Experimental results show that our fault tolerant QR factorization can successfully detect and recover from soft errors in the entire matrix with little overhead on hybrid systems with GPGPUs. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Du, Peng; Luszczek, Piotr; Tomov, Stan; Dongarra, Jack] Univ Tennessee, EECS, Knoxville, TN 37996 USA.
[Dongarra, Jack] Oak Ridge Natl Lab, Oak Ridge, TN USA.
[Dongarra, Jack] Univ Manchester, Manchester, Lancs, England.
RP Du, P (reprint author), Univ Tennessee, EECS, 1122 Volunteer Blvd, Knoxville, TN 37996 USA.
EM du@eecs.utk.edu; luszczek@eecs.utk.edu; tomov@eecs.utk.edu
RI Dongarra, Jack/E-3987-2014
NR 37
TC 4
Z9 4
U1 1
U2 4
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1877-7503
J9 J COMPUT SCI-NETH
JI J. Comput. Sci.
PD NOV
PY 2013
VL 4
IS 6
SI SI
BP 457
EP 464
DI 10.1016/j.jocs.2013.01.004
PG 8
WC Computer Science, Interdisciplinary Applications; Computer Science,
Theory & Methods
SC Computer Science
GA 268PZ
UT WOS:000328184300005
ER
PT J
AU He, J
Kowalkowski, J
Paterno, M
Holmgren, D
Simone, J
Sun, XH
AF He, Jun
Kowalkowski, Jim
Paterno, Marc
Holmgren, Don
Simone, James
Sun, Xian-He
TI Layout-aware scientific computing: A case study using the MILC code
SO JOURNAL OF COMPUTATIONAL SCIENCE
LA English
DT Article
DE Performance model; MILC; Communication
ID ALLOCATION; ALGORITHM
AB Nowadays, high performance computers have more cores and nodes than ever before. Computation is spread out among them, leading to more communication cost than before. For this reason, communication can easily become the bottleneck of a system and limit its scalability. The layout of an application on a computer is the key factor to preserve communication locality and reduce its cost. In this paper, we propose a straightforward model to optimize the layout for scientific applications by minimizing internode communication cost. The model takes into account the latency and bandwidth of the network and associates them with the dominant layout variables of the application. We take the MILC code as an example and analyze its communication patterns. According to our experimental results, the model developed for the MILC code achieved a satisfactory accuracy for predicting the performance, leading to up to 31% performance improvement. (C) 2013 Elsevier B.V. All rights reserved.
C1 [He, Jun; Sun, Xian-He] IIT, Dept Comp Sci, Chicago, IL 60616 USA.
[Kowalkowski, Jim; Paterno, Marc; Holmgren, Don; Simone, James] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.
[He, Jun] Univ Wisconsin Madison, Dept Comp Sci, Madison, WI USA.
[He, Jun] IIT, Chicago, IL 60616 USA.
RP He, J (reprint author), IIT, Dept Comp Sci, Chicago, IL 60616 USA.
EM jhe@cs.wisc.edu; jbk@fnal.gov; paterno@fnal.gov; djholm@fnal.gov;
simone@fnal.gov; sun@iit.edu
NR 16
TC 1
Z9 1
U1 0
U2 1
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1877-7503
J9 J COMPUT SCI-NETH
JI J. Comput. Sci.
PD NOV
PY 2013
VL 4
IS 6
SI SI
BP 496
EP 506
DI 10.1016/j.jocs.2013.05.007
PG 11
WC Computer Science, Interdisciplinary Applications; Computer Science,
Theory & Methods
SC Computer Science
GA 268PZ
UT WOS:000328184300010
ER
PT J
AU Yingst, RA
Kah, LC
Palucis, M
Williams, RME
Garvin, J
Bridges, JC
Bridges, N
Deen, RG
Farmer, J
Gasnault, O
Goetz, W
Hamilton, VE
Hipkin, V
Jensen, JK
King, PL
Koefoed, A
Le Mouelic, SP
Madsen, MB
Mangold, N
Martinez-Frias, J
Maurice, S
McCartney, EM
Newsom, H
Pariser, O
Sautter, VH
Wiens, RC
AF Yingst, R. A.
Kah, L. C.
Palucis, M.
Williams, R. M. E.
Garvin, J.
Bridges, J. C.
Bridges, N.
Deen, R. G.
Farmer, J.
Gasnault, O.
Goetz, W.
Hamilton, V. E.
Hipkin, V.
Jensen, J. K.
King, P. L.
Koefoed, A.
Le Mouelic, S. P.
Madsen, M. B.
Mangold, N.
Martinez-Frias, J.
Maurice, S.
McCartney, E. M.
Newsom, H.
Pariser, O.
Sautter, V. H.
Wiens, R. C.
TI Characteristics of pebble- and cobble-sized clasts along the Curiosity
rover traverse from Bradbury Landing to Rocknest
SO JOURNAL OF GEOPHYSICAL RESEARCH-PLANETS
LA English
DT Article
DE Mars; transport properties; fluvial processes; surface materials
ID GALE-CRATER; EARLY MARS; SITE; SURFACE; VENTIFACTS; ROCKS; VENUS; SHAPE
AB We have assessed the characteristics of clasts along Curiosity's traverse to shed light on the processes important in the genesis, modification, and transportation of surface materials. Pebble- to cobble-sized clasts at Bradbury Landing, and subsequently along Curiosity's traverse to Yellowknife Bay, reflect a mixing of two end-member transport mechanisms. The general clast population likely represents material deposited via impact processes, including meteorite fragments, ejecta from distant craters, and impactites consisting of shocked and shock-melted materials from within Gale Crater, which resulted predominantly in larger, angular clasts. A subset of rounded pebble-sized clasts has likely been modified by intermittent alluvial or fluvial processes. The morphology of this rounded clast population indicates that water was a more important transporting agent here than at other Mars sites that have been studied in situ. Finally, we identified populations of basalt clasts and porphyritic clasts of undetermined composition by their morphologic and textural characteristics; basalts are confirmed by geochemical data provided by ChemCam.
C1 [Yingst, R. A.; Williams, R. M. E.] Planetary Sci Inst, Tucson, AZ 85719 USA.
[Kah, L. C.] Univ Tennessee, Knoxville, TN USA.
[Palucis, M.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.
[Garvin, J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA.
[Bridges, J. C.] Univ Leicester, Dept Phys & Astron, Space Res Ctr, Leicester LE1 7RH, Leics, England.
[Bridges, N.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA.
[Deen, R. G.; Pariser, O.] CALTECH, Jet Prop Lab, Pasadena, CA USA.
[Farmer, J.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA.
[Gasnault, O.; Le Mouelic, S. P.; Mangold, N.; Maurice, S.] CNRS, UMR 6112, Lab Planetol & Geodynam Nantes, Nantes, France.
[Gasnault, O.; Le Mouelic, S. P.; Mangold, N.; Maurice, S.] Univ Nantes, Nantes, France.
[Goetz, W.] Max Planck Inst Sonnensyst Forsch, D-37191 Katlenburg Lindau, Germany.
[Hamilton, V. E.] SW Res Inst, Dept Space Studies, Boulder, CO USA.
[Hipkin, V.] Canadian Space Agcy, St Hubert, PQ, Canada.
[Jensen, J. K.; Koefoed, A.; Madsen, M. B.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark.
[King, P. L.] Australian Natl Univ, Res Sch Earth Sci, Coll Phys & Math Sci, Canberra, ACT, Australia.
[Martinez-Frias, J.] CSIC UCM, Inst Geosci, Fac Ciencias Geol, Madrid, Spain.
[McCartney, E. M.] Malin Space Sci Syst, San Diego, CA USA.
[Newsom, H.] Univ New Mexico, Inst Meteorit, Albuquerque, NM 87131 USA.
[Sautter, V. H.] MNHN, LMCM, Paris, France.
[Wiens, R. C.] Los Alamos Natl Lab, Los Alamos, NM USA.
RP Yingst, RA (reprint author), Planetary Sci Inst, 1700 E Ft Lowell,Ste 106, Tucson, AZ 85719 USA.
EM yingst@psi.edu
RI King, Penelope/A-1791-2011;
OI King, Penelope/0000-0002-8364-9168; Gasnault,
Olivier/0000-0002-6979-9012
FU Mars Science Laboratory Program through Malin Space Science Systems
[08-0315]; Danish Council for Independent Research/Natural Sciences
(FNU) [12-127126, 11-107019]; TICRA Foundation; Deutsche
Forschungsgemeinschaft (DFG) [GO 2288/1-1]; National Aeronautics and
Space Administration
FX We gratefully acknowledge the constructive reviews whose comments
improved this manuscript. This research was supported by the Mars
Science Laboratory Program through Malin Space Science Systems contract
08-0315 to R.A.Y. We thank Hallie E. Gengl, JPL's OPGS team, for
processing the standard clast survey images for stereo analysis by
generating the 3-D local-level maps. Work in Denmark was funded by the
Danish Council for Independent Research/Natural Sciences (FNU grants
12-127126 and 11-107019) and the TICRA Foundation. Work in Germany was
funded by the Deutsche Forschungsgemeinschaft (DFG grant GO 2288/1-1).
The work of R. Deen, O. Pariser, and Hallie Gengl was carried out at the
Jet Propulsion Laboratory, California Institute of Technology, under a
contract with the National Aeronautics and Space Administration.
NR 84
TC 16
Z9 16
U1 4
U2 20
PU AMER GEOPHYSICAL UNION
PI WASHINGTON
PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA
SN 2169-9097
EI 2169-9100
J9 J GEOPHYS RES-PLANET
JI J. Geophys. Res.-Planets
PD NOV
PY 2013
VL 118
IS 11
BP 2361
EP 2380
DI 10.1002/2013JE004435
PG 20
WC Geochemistry & Geophysics
SC Geochemistry & Geophysics
GA 270YJ
UT WOS:000328355300007
ER
PT J
AU Ho, CY
Tsai, SC
Lin, HT
Chen, FR
Kai, JJ
AF Ho, Chun-Yu
Tsai, Shuo-Cheng
Lin, Hua-Tay
Chen, Fu-Rong
Kai, Ji-Jung
TI Microstructural investigation of Si-ion-irradiated single crystal 3C-SiC
and SA-Tyrannohex SiC fiber-bonded composite at high temperatures
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID SILICON-CARBIDE; ELEVATED-TEMPERATURES; ELECTRON-MICROSCOPY;
HIGH-STRENGTH; DEGREES-C; DEFECTS; EVOLUTION; HELIUM
AB Silicon carbides (SiCs) are considered as one of the promising candidates for structural and core materials used in fusion reactor and high temperature gas-cooled reactor (HTGR) due to its high thermal stability, and good resistance to irradiation and chemical attack. Single crystal 3C-SiC with less intrinsic defects was used to precisely characterize the radiation-induced defects in 3C-SiC. In addition, there are limited discussions related to radiation effect of SA-Tyrannohex fiber-bonded composite at high temperatures. Therefore, in this study, single crystal 3C-SiC thin film and SA-Tyrannohex SiC fiber-bonded composite were irradiated at 1000-1350 degrees C with 7 MeV Si3+ ion to simulate the neutron irradiation in reactors. The microstructure of the irradiated SiC was examined by using high resolution transmission electron microscope (HRTEM). In irradiated single crystal 3C-SiC, high resolution images showed that the planar defects were extrinsic stacking faulted loop with changing atomic sequences and intrinsic stacking faulted loop, i.e. vacancy loop. In addition, dislocation loops, voids, and edge dislocations in SA-Tyrannohex SiC fiber-bonded composite after irradiation were investigated. Besides, larger voids (with diameter 10-40 nm) formed in alumina with preferred orientation after irradiation perhaps resulting in degradation of strength of the SA-Tyrannohex SiC fiber-bonded composite. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Ho, Chun-Yu; Kai, Ji-Jung] Natl Tsing Hua Univ, Inst Nucl Engn & Sci, Hsinchu 30013, Taiwan.
[Tsai, Shuo-Cheng; Chen, Fu-Rong; Kai, Ji-Jung] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan.
[Lin, Hua-Tay] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Kai, JJ (reprint author), Natl Tsing Hua Univ, Inst Nucl Engn & Sci, Hsinchu 30013, Taiwan.
EM ceer0001@gmail.com
OI KAI, Ji-jung/0000-0001-7848-8753
NR 26
TC 6
Z9 6
U1 2
U2 25
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 1
EP 7
DI 10.1016/j.jnucmat.2013.06.045
PG 7
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800001
ER
PT J
AU Yang, TF
Taylor, CA
Kong, SY
Wang, CX
Zhang, YW
Huang, XJ
Xue, JM
Yan, S
Wang, YG
AF Yang, Tengfei
Taylor, Caitlin A.
Kong, Shuyan
Wang, Chenxu
Zhang, Yanwen
Huang, Xuejun
Xue, Jianming
Yan, Sha
Wang, Yugang
TI The discrepancies in multistep damage evolution of yttria-stabilized
zirconia irradiated with different ions
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID CUBIC ZIRCONIA; RADIATION-DAMAGE; CERAMIC INSULATORS; DEFECT PRODUCTION;
METALS; REACTORS; OXIDES
AB This paper reports a comprehensive investigation of structural damage in yttria-stabilized zirconia irradiated with different ions over a wide fluence range. A similar multistep damage accumulation exists for the irradiations of different ions, but the critical doses for occurrence of second damage step, characterized by a faster increase in damage fraction, and the maximum elastic strain at the first damage step are varied and depend on ion mass. For irradiations of heavier ions, the second damage step occurs at a higher dose with a lower critical elastic strain. Furthermore, larger extended defects were observed in the irradiations of heavy ions at the second damage step. Associated with other experiment results and multistep damage accumulation model, the distinct discrepancies in the damage buildup under irradiations of different ions were interpreted by the effects of electronic excitation, energy of primary knock-on atom and chemistry contributions of deposited ions. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Yang, Tengfei; Kong, Shuyan; Wang, Chenxu; Huang, Xuejun; Xue, Jianming; Yan, Sha; Wang, Yugang] Peking Univ, State Key Lab Nucl Phys & Technol, Ctr Appl Phys & Technol, Beijing 100871, Peoples R China.
[Taylor, Caitlin A.; Zhang, Yanwen] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.
[Zhang, Yanwen] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
RP Wang, YG (reprint author), Peking Univ, State Key Lab Nucl Phys & Technol, Ctr Appl Phys & Technol, Beijing 100871, Peoples R China.
EM ygwang@pku.edu.cn
OI , /0000-0003-2655-0804
FU Ministry of Science and Technology of China [2010CB832904]; National
Natural Science Foundation of China [11075005, 91226202]
FX This work was financially supported by the Ministry of Science and
Technology of China (2010CB832904) and National Natural Science
Foundation of China (11075005) and (91226202).
NR 54
TC 6
Z9 6
U1 2
U2 20
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 40
EP 48
DI 10.1016/j.jnucmat.2013.06.033
PG 9
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800007
ER
PT J
AU Xu, HX
Stoller, RE
Osetsky, YN
AF Xu, Haixuan
Stoller, Roger E.
Osetsky, Yury N.
TI Cascade defect evolution processes: Comparison of atomistic methods
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID KINETIC MONTE-CARLO; FINDING SADDLE-POINTS; INFREQUENT EVENTS;
ALPHA-IRON; DAMAGE ACCUMULATION; RADIATION-DAMAGE; BCC IRON; SIMULATION;
DYNAMICS; IRRADIATION
AB Determining defect evolution beyond the molecular dynamics (MD) time scale is critical to bridging the gap between atomistic simulations and experiments. The recently developed self-evolving atomistic kinetic Monte Carlo (SEAKMC) method provides new opportunities to simulate long-term defect evolution with MD-like fidelity to the atomistic processes involved. To demonstrate this capability, three examples are presented in which SEAKMC has been used to investigate the evolution of typical radiation-induced defects in bcc iron. Depending on the particular example. SEAKMC results are compared with those obtained using two other on-the-fly KMC techniques, object KMC, and MD. The three examples are: (1) evolution of a vacancy-rich region similar to the core of a displacement cascade, (2) the stability of recently reported interstitial clusters with a structure similar to the 05 Laves phase, and (3) long-term aging of atomic displacement cascade debris. In the various examples, the SEAKMC approach provides better agreement with MD simulations, highlights the importance of the underlying atomistic processes, and provides new information on long-term defect evolution in iron. Published by Elsevier BV.
C1 [Xu, Haixuan; Stoller, Roger E.; Osetsky, Yury N.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
RP Xu, HX (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
EM xuh1@ornl.gov
RI Xu, Haixuan/C-9841-2009;
OI Osetskiy, Yury/0000-0002-8109-0030
FU Center for Defect Physics, an Energy Frontier Research Center; U.S.
Department of Energy, Office of Science [ERKCS99]; U.S. Department of
Energy Office of Basic Energy Sciences [ERKCS99]
FX Research at the Oak Ridge National Laboratory supported as part of the
Center for Defect Physics, an Energy Frontier Research Center funded by
the U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences under Award Number ERKCS99.
NR 33
TC 12
Z9 12
U1 4
U2 28
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 66
EP 70
DI 10.1016/j.jnucmat.2013.07.001
PG 5
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800010
ER
PT J
AU He, LF
Gupta, M
Yablinsky, CA
Gan, J
Kirk, MA
Bai, XM
Pakarinen, J
Allen, TR
AF He, Ling-Feng
Gupta, Mahima
Yablinsky, Clarissa A.
Gan, Jian
Kirk, Marquis A.
Bai, Xian-Ming
Pakarinen, Janne
Allen, Todd R.
TI In situ TEM observation of dislocation evolution in Kr-irradiated UO2
single crystal
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID URANIUM-DIOXIDE; DISPLACEMENT CASCADES; RADIATION-DAMAGE; DEFECTS;
BUBBLES; BURNUP; FUELS
AB In situ transmission electron microscopy(TEM) observation of UO2 single crystal irradiated with Kr ions at high temperatures was conducted to understand the dislocation evolution due to high-energy radiation. The dislocation evolution in UO2 single crystal is shown to occur as nucleation and growth of dislocation loops at low-irradiation doses, followed by transformation to extended dislocation segments and networks at high doses, as well as shrinkage and annihilation of some loops and dislocations due to high temperature annealing. Generally the trends of dislocation evolution in UO2 were similar under Kr irradiation at different ion energies and temperatures (150 keV at 600 degrees C and 1 MeV at 800 degrees C) used in this work. Interstitial-type dislocation loops with Burgers vector along (1 1 0) were observed in the Kr-irradiated UO2. The irradiated specimens were denuded of dislocation loops near the surface. Published by Elsevier B.V.
C1 [He, Ling-Feng; Gupta, Mahima; Yablinsky, Clarissa A.; Pakarinen, Janne; Allen, Todd R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA.
[Gan, Jian; Bai, Xian-Ming] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
[Kirk, Marquis A.] Argonne Natl Lab, Argonne, IL 60439 USA.
RP He, LF (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA.
EM lhe33@wisc.edu
RI He, Lingfeng/D-3534-2014; Bai, Xianming/E-2376-2017;
OI He, Lingfeng/0000-0003-2763-1462; Bai, Xianming/0000-0002-4609-6576;
Allen, Todd/0000-0002-2372-7259
FU Center for Materials Science of Nuclear Fuel, an Energy Frontier
Research Center; U.S. Department of Energy, Office of Science, Office of
Basic Energy Sciences; U.S. Department of Energy Office of Science
Laboratory [DE-AC02-06CH11357]
FX This work was supported as part of the Center for Materials Science of
Nuclear Fuel, an Energy Frontier Research Center funded by the U.S.
Department of Energy, Office of Science, Office of Basic Energy
Sciences. The electron microscopy was accomplished at the Electron
Microscopy Center for Materials Research at Argonne National Laboratory,
a U.S. Department of Energy Office of Science Laboratory operated under
Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC, and the Center
for Advanced Energy Studies located in Idaho Falls, Idaho. We thank
Peter M. Baldo of Argonne National Lab for his help in performing the
irradiations.
NR 34
TC 18
Z9 18
U1 0
U2 32
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 71
EP 77
DI 10.1016/j.jnucmat.2013.06.050
PG 7
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800011
ER
PT J
AU Taller, SA
Bai, XM
AF Taller, Stephen A.
Bai, Xian-Ming
TI Assessment of structures and stabilities of defect clusters and surface
energies predicted by nine interatomic potentials for UO2
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID STOICHIOMETRIC URANIUM-DIOXIDE; MOLECULAR-DYNAMICS SIMULATION;
THERMAL-CONDUCTIVITY; OXYGEN DIFFUSION; GRAIN-BOUNDARY; POINT-DEFECTS;
EQUILIBRIUM; HELIUM; OXIDES; DAMAGE
AB The irradiation in nuclear reactors creates many point defects and defect clusters in uranium dioxide (UO2) and their evolution severely degrades the thermal and mechanical properties of the nuclear fuels. Previously many empirical interatomic potentials have been developed for modeling defect production and evolution in UO2. However, the properties of defect clusters and extended defects are usually not fitted into these potentials. In this work nine interatomic potentials for UO2 are examined by using molecular statics and molecular dynamics to assess their applicability in predicting the properties of various types of defect clusters in UO2. The binding energies and structures for these defect clusters have been evaluated for each potential. In addition, the surface energies of voids of different radii and (1 1 0) flat surfaces predicted by these potentials are also evaluated. It is found that both good agreement and significant discrepancies exist for these potentials in predicting these properties. For oxygen interstitial clusters, these potentials predict significantly different defect cluster structures and stabilities; For defect clusters consisting of both uranium and oxygen defects, the prediction is in better agreement; The surface energies predicted by these potentials have significant discrepancies, and some of them are much higher than the experimentally measured values. The results from this work can provide insight on interpreting the outcome of atomistic modeling of defect production using these potentials and may provide guidelines for choosing appropriate potential models to study problems of interest in UO2. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Taller, Stephen A.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA.
[Bai, Xian-Ming] Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID 83415 USA.
RP Bai, XM (reprint author), Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID 83415 USA.
EM xianming.bai@inl.gov
RI Bai, Xianming/E-2376-2017
OI Bai, Xianming/0000-0002-4609-6576
FU U.S. Department of Energy, Office of Science [FWP 1356]; U.S. Department
of Energy Office of Science [FWP 1356]; U.S. Department of Energy
[DE-AC07-051D14517]
FX This work is conducted under the work scope of the Center for Materials
Science of Nuclear Fuel (CMSNF) at Idaho National Laboratory, an Energy
Frontier Research Center (EFRC) funded by the U.S. Department of Energy,
Office of Science, Office of Basic Energy Sciences under Award Number
FWP 1356. The authors acknowledge the High Performance Computing (HPC)
group at Idaho National Laboratory (INL) for allowing them to conduct
the calculations on INL's HPC clusters. S. A. T. would like to thank INL
for hosting his summer internship, and the Science Undergraduate
Laboratory Internship (SULI) program sponsored by the Department of
Energy's Office of Science for supporting his summer internship. This
manuscript has been coauthored by Battelle Energy Alliance, LLC under
Contract No. DE-AC07-051D14517 with the U.S. Department of Energy. The
United States Government retains and the publisher, by accepting the
article for publication, acknowledges that the United States Government
retains a nonexclusive, paid-up, irrevocable, world-wide license to
publish or reproduce the published form of this manuscript, or allow
others to do so, for United States Government purposes.
NR 54
TC 6
Z9 6
U1 1
U2 20
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 84
EP 98
DI 10.1016/j.jnucmat.2013.06.038
PG 15
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800013
ER
PT J
AU Men, D
Patel, MK
Usov, IO
Toiammou, M
Monnet, I
Pivin, JC
Porter, JR
Mecartney, ML
AF Men, Danju
Patel, Maulik K.
Usov, Igor O.
Toiammou, Moidi
Monnet, Isabelle
Pivin, Jean Claude
Porter, John R.
Mecartney, Martha L.
TI Radiation damage in multiphase ceramics
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID INDUCED PHASE-TRANSFORMATION; HEAVY-ION IRRADIATION; OXIDE FUELS;
INDUCED AMORPHIZATION; THERMAL-CONDUCTIVITY; MOLECULAR-DYNAMICS;
FISSION-PRODUCTS; URANIUM-DIOXIDE; MINOR ACTINIDES; PURE ZIRCONIA
AB Four-phase ceramic composites containing 3 mol% Y2O3 stabilized ZrO2 (3Y-TZP), Al2O3, MgAl2O4, and LaPO4 were synthesized as model materials representing inert matrix fuel with enhanced thermal conductivity and decreased radiation-induced microstructural damage with respect to single-phase UO2. This multi-phase concept, if successful, could be applied to design advanced nuclear fuels which could then be irradiated to higher burn-ups. 3Y-TZP in the composite represents a host (fuel) phase with the lowest thermal conductivity and Al2O3 is the high thermal conductivity phase. The role of MgAl2O4 and LaPO4 was to stabilize the structure under irradiation. The radiation response was evaluated by ion irradiation at 500 degrees C with 10 MeV Au ions and at 800 degrees C with 92 MeV Xe ions, to simulate damage due to primary knock-on atoms and fission fragments, respectively. Radiation damage and microstructural changes were characterized by X-ray diffraction, scanning electron microscopy and transmission electron microscopy and computational modeling. Al2O3. Y2O3 stabilized ZrO2 and MgAl2O4 phases exhibit high amorphization resistance and remain stable when irradiated with both Au and Xe ions. A monoclinic-to-tetragonal phase transformation, however, is promoted by Xe and Au ion irradiation in 3Y-TZP. The LaPO4 monazite phase appears to melt, dewet the other phases, and recrystallize under Au irradiation, but does not change under Xe irradiation. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Men, Danju; Mecartney, Martha L.] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA.
[Patel, Maulik K.; Usov, Igor O.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
[Toiammou, Moidi; Monnet, Isabelle] Univ Caen Basse Normandie, CEA, CNRS, CIMAP,ENSICAEN, F-14070 Caen 5, France.
[Pivin, Jean Claude] Univ Paris 11, CNRS, UMR 8609, Ctr Spectrometrie Nucl & Spectrometrie Masse,IN2P, F-91405 Orsay, France.
[Porter, John R.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA.
RP Mecartney, ML (reprint author), Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA.
EM martham@uci.edu
FU National Science Foundation [NSF DMR 0606063]; Office of Basic Energy
Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of
Science of the U.S. Department of Energy [DE-AC02-05CH11231]
FX This research was supported by the National Science Foundation, funding
under Grant NSF DMR 0606063. The opinions expressed are those of the
authors alone, and do not reflect any official endorsement by NSF. The
authors would like to thank Dr. Kurt E. Sickafus, while at Los Alamos
National Laboratory for his initial invitation to conduct research and
for input. The Xe beam-time was obtained at Grand Accelerateur National
d'Ions Lourds.; The TEM work on the FEI Tecnai, JEOL 3010. CM200,
assisted by Chengyu Song, was performed at Lawrence Berkeley Laboratory
National Center for Electron Microscopy, which is supported by the
Office of Science, Office of Basic Energy Sciences of the U.S.
Department of Energy under Contract No. DE-AC02-05CH11231.
NR 48
TC 5
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U1 5
U2 62
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 120
EP 127
DI 10.1016/j.jnucmat.2013.06.042
PG 8
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800017
ER
PT J
AU Dunn, AY
Capolungo, L
Martinez, E
Cherkaoui, M
AF Dunn, Aaron Y.
Capolungo, Laurent
Martinez, Enrique
Cherkaoui, Mohammed
TI Spatially resolved stochastic cluster dynamics for radiation damage
evolution in nanostructured metals
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID KINETIC MONTE-CARLO; ALPHA-FE; COMPUTER-SIMULATION; DEFECT PRODUCTION;
VACANCY CLUSTERS; HELIUM; CU; ACCUMULATION; DIFFUSION; MIGRATION
AB A spatially resolved stochastic cluster dynamics (SRSCD) model is introduced to describe radiation-induced defect evolution in metals. The stochastic nature of the method allows SRSCD to model more chemical species and more mobile defects than rate theory methods without loss of computational efficiency, while reaching larger timescales and simulating larger volumes than object-oriented kinetic Monte Carlo (OKMC) methods. To comprehend the capabilities of the method and access new understanding of defect evolution, SRSCD is used in three scenarios. In the first, the results of Frenkel pair implantation are found to match those of rate theory in both spatially homogeneous and spatially resolved media. Next, to study spatial resolution effects and correspondence to OKMC, the results of 20 key cascade implantation into copper is simulated and an acceptable match with OKMC is found. Finally the method is used to study the problem of helium desorption in thin iron foils. The model is compared with available experimental measures and is found to be in good agreement. The ability of SRSCD to include many mobile species of defects allows a detailed analysis of the mechanisms of helium release from the free surface of the iron foils. As a result new dominant mechanisms of helium release are discussed as well as their operating regimes. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Dunn, Aaron Y.; Capolungo, Laurent; Cherkaoui, Mohammed] CNRS, UMI Georgia Tech 2958, Georgia Inst Technol, George W Woodruff Sch Mech Engn, F-57070 Metz, France.
[Martinez, Enrique] Los Alamos Natl Lab, Los Alamos, NM USA.
RP Capolungo, L (reprint author), CNRS, UMI Georgia Tech 2958, Georgia Inst Technol, George W Woodruff Sch Mech Engn, F-57070 Metz, France.
EM laurent.capolungo@me.gatech.edu
OI Martinez Saez, Enrique/0000-0002-2690-2622
FU European Union; Center for Materials at Irradiation and Mechanical
Extremes, an Energy Frontier Research Center; US Department of Energy at
Los Alamos National Laboratory [2008LANL1026]
FX The authors gratefully acknowledge support from European Union, Project
RADINTERFACES. The authors thank I. Martin-Bragado and L Agudo for their
discussions and assistance on this work. The authors thank C. Ortiz and
M..). Caturla for their correspondence. A. Dunn would like to thank M.
McPhie for discussions on this work. E. Martinez gratefully acknowledges
support from thel funded by the US Department of Energy (Award Number
2008LANL1026) at Los Alamos National Laboratory.
NR 48
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 128
EP 139
DI 10.1016/j.jnucmat.2013.07.009
PG 12
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800018
ER
PT J
AU Crapps, J
DeCroix, DS
Galloway, JD
Korzekwa, DA
Aikin, R
Fielding, R
Kennedy, R
Unal, C
AF Crapps, J.
DeCroix, D. S.
Galloway, J. D.
Korzekwa, D. A.
Aikin, R.
Fielding, R.
Kennedy, R.
Unal, C.
TI Separate effects identification via casting process modeling for
experimental measurement of U-Pu-Zr alloys
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
AB Computational simulations of gravity casting processes for metallic U-Pu-Zr nuclear fuel rods have been performed using a design-of-experiments technique to determine the fluid flow, liquid heat transfer, and solid heat transfer parameters which most strongly influence the process solidification speed and fuel rod porosity. The results are used to make recommendations for the best investment of experimental time and effort to measure process parameters. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Crapps, J.; DeCroix, D. S.; Galloway, J. D.; Korzekwa, D. A.; Aikin, R.; Unal, C.] Los Alamos Natl Lab, Los Alamos, NM USA.
[Fielding, R.; Kennedy, R.] Idaho Natl Lab, Idaho Falls, ID USA.
[Crapps, J.] ExxonMobil Upstream Res Co, Houston, TX USA.
RP Crapps, J (reprint author), ExxonMobil Upstream Res Co, Houston, TX USA.
EM justin.crapps@gmail.com
FU Fuel Cycle Research and Development Project [FTLA11AF0207]
FX This work was funded through the Fuel Cycle Research and Development
Project. FTLA11AF0207.
NR 17
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U1 2
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 176
EP 184
DI 10.1016/j.jnucmat.2013.07.016
PG 9
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800024
ER
PT J
AU Pokorny, R
Rice, JA
Crum, JV
Schweiger, MJ
Hrma, P
AF Pokorny, Richard
Rice, Jarrett A.
Crum, Jarrod V.
Schweiger, Michael J.
Hrma, Pavel
TI Kinetic model for quartz and spinet dissolution during melting of
high-level-waste glass batch
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID BOROSILICATE GLASS; MOLTEN GLASS; COLD-CAP; CRYSTALLIZATION; CRYSTALS;
SILICA; TEMPERATURE; CONVERSION; PARTICLES; GROWTH
AB The dissolution of quartz particles and the growth and dissolution of crystalline phases during the conversion of batch to glass potentially affects both the glass melting process and product quality. Crystals of spinet exiting the cold cap to molten glass below can be troublesome during the vitrification of iron-containing high-level wastes. To estimate the distribution of quartz and spinel fractions within the cold cap, we used kinetic models that relate fractions of these phases to temperature and heating rate. Fitting the model equations to data showed that the heating rate, apart from affecting quartz and spinel behavior directly, also affects them indirectly via concurrent processes, such as the formation and motion of bubbles. Because of these indirect effects, it was necessary to allow one kinetic parameter (the pre-exponential factor) to vary with the heating rate. The resulting kinetic equations are sufficiently simple for the detailed modeling of batch-to-glass conversion as it occurs in glass melters. The estimated fractions and sizes of quartz and spinel particles as they leave the cold cap, determined in this study, will provide the source terms needed for modeling the behavior of these solid particles within the flow of molten glass in the melter. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Pokorny, Richard] Prague Inst Chem Technol, Dept Chem Engn, CR-16628 Prague 6, Czech Republic.
[Rice, Jarrett A.; Crum, Jarrod V.; Schweiger, Michael J.; Hrma, Pavel] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Hrma, Pavel] Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang, South Korea.
RP Hrma, P (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM pavel.hrma@pnnl.gov
FU Department of Energy's Waste Treatment & Immobilization Plant Federal
Project Office; WCU (World Class University) program through the
National Research Foundation of Korea; Ministry of Education, Science
and Technology [R31-30005]; specific university research (MSMT)
[20/2013]; Battelle [DE-AC05-76RL01830]
FX This work was supported by the Department of Energy's Waste Treatment &
Immobilization Plant Federal Project Office under the direction of Dr.
Albert A. Kruger and by the WCU (World Class University) program through
the National Research Foundation of Korea funded by the Ministry of
Education, Science and Technology (R31-30005). Richard Pokorny
acknowledges financial support from specific university research (MSMT
No. 20/2013). The authors are grateful to Jaehun Chun and Dong-Sang Kim
for insightful discussions and Derek R. Dixon for providing the scanning
electron micrograph image. Pacific Northwest National Laboratory is
operated for the U.S. Department of Energy by Battelle under Contract
DE-AC05-76RL01830.
NR 37
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U1 2
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 230
EP 235
DI 10.1016/j.jnucmat.2013.07.039
PG 6
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800032
ER
PT J
AU Allahar, KN
Burns, J
Jaques, B
Wu, YQ
Charit, I
Cole, J
Butt, DP
AF Allahar, Kerry N.
Burns, Jatuporn
Jaques, Brian
Wu, Y. Q.
Charit, Indrajit
Cole, James
Butt, Darryl P.
TI Ferritic oxide dispersion strengthened alloys by spark plasma sintering
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID FEAL ALLOY; STEELS; RECRYSTALLIZATION; MICROSTRUCTURE; STABILITY;
TITANIUM; REACTORS; TI
AB Spark plasma sintering (SPS) was used to consolidate a Fe-16Cr-3Al (wt.%) powder that was mechanically alloyed with Y2O3 and Ti powders to produce 0.5 Y2O3 and 0.5 Y2O3-1Ti powders. The effects of mechanical alloying and sintering conditions on the microstructure, relative density and hardness of the sintered oxide dispersion strengthened (ODS) alloys are presented. Scanning electron microscopy indicated a mixed fine-grain and coarse-grain microstructure that was attributed to recrystallization and grain growth during sintering. Analysis of the transmission electron microscopy (TEM) and atom probe tomography (APT) data identified Y-O and Y-O-Ti nanoclusters. Elemental ratios of these nanoclusters were consistent with that observed in hot-extruded ODS alloys. The influence of Ti was to refine the grains as well as the nanoclusters with there being greater number density and smaller sizes of the Y-O-Ti nanoclusters as compared to the Y-O nanoclusters. This resulted in the Ti-containing samples being harder than the Ti-free alloys. The hardness of the alloys with the Y-O-Ti nanoclusters was insensitive to sintering time while smaller hardness values were associated with longer sintering times for the alloys with the Y-O nanoclusters. Pressures greater than 80 MPa are recommended for improved densification as higher sintering temperatures and longer sintering times at 80 MPa did not improve the relative density beyond 97.5%. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Allahar, Kerry N.; Burns, Jatuporn; Jaques, Brian; Wu, Y. Q.; Butt, Darryl P.] Boise State Univ, Mat & Sci Engn Dept, Boise, ID 83725 USA.
[Charit, Indrajit] Univ Idaho, Dept Chem & Mat Engn, Moscow, ID 83844 USA.
[Cole, James] Idaho Natl Lab, Idaho Falls, ID 83401 USA.
[Allahar, Kerry N.; Burns, Jatuporn; Wu, Y. Q.; Butt, Darryl P.] Ctr Adv Energy Studies, Idaho Falls, ID 83401 USA.
RP Allahar, KN (reprint author), Ctr Adv Energy Studies, 995 Univ Blvd, Idaho Falls, ID 83401 USA.
EM KerryAllahar@boisestate.edu
OI Cole, James/0000-0003-1178-5846; Jaques, Brian/0000-0002-5324-555X
FU Battelle Energy Alliance through the Laboratory Directed Research and
Development program at the Idaho National Laboratory
FX Funding for this work was provided in part by Battelle Energy Alliance
through the Laboratory Directed Research and Development program at the
Idaho National Laboratory.
NR 30
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 256
EP 265
DI 10.1016/j.jnucmat.2013.07.019
PG 10
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800036
ER
PT J
AU White, JT
Nelson, AT
AF White, J. T.
Nelson, A. T.
TI Thermal conductivity of UO2+x and U4O9-y
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID NONSTOICHIOMETRIC U4O9-Y; ELECTRICAL-CONDUCTIVITY; UO2-BASED SIMFUEL;
URANIUM-DIOXIDE; DEFECTIVE FUEL; OXIDATION; TEMPERATURE; SCATTERING;
STEAM; HEAT
AB Stoichiometries of UO2 specimens ranging from 2.000 to 2.210 were prepared in situ at 1673 K within thermoanalytical equipment. Thermal conductivities were analyzed according to Klemens-Callaway defect model. Analysis of the data sets allows for extraction of the fundamental phonon-phonon and phonon-defect scattering contributions for the materials investigated. Low temperature thermal conductivity data was modeled using sigmoidal averaging to calculate the dual phase field UO2+x-U4O9-y. This allowed the thermal conductivity of U4O9-y to be calculated as a function of temperature up to 873 K. This fundamental dataset provides a key contribution to ongoing efforts in the modeling and simulation communities in the areas of both light water reactor fuel performance and accident evolution. (C) 2013 Elsevier B.V. All rights reserved.
C1 [White, J. T.; Nelson, A. T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP White, JT (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
EM jtwhite@lanl.gov; atnelson@lanl.gov
OI Nelson, Andrew/0000-0002-4071-3502
FU U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle Research
and Development program
FX The authors thank Mr. John Dunwoody and Mr. Darrin Byler of Los Alamos
National Laboratory for assistance in pellet fabrication and useful
discussions. The authors would like to extend their appreciation to D.R.
Clarke of Harvard University for his helpful advice on modeling the
thermal conductivity of this system, as well as to D.A. Andersson of Los
Alamos National Laboratory for insights into the defect structures of
hyperstoichiometric UO2. The support of the U.S. Department
of Energy, Office of Nuclear Energy Fuel Cycle Research and Development
program is gratefully acknowledged.
NR 38
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PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 342
EP 350
DI 10.1016/j.jnucmat.2013.07.063
PG 9
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800047
ER
PT J
AU Tan, L
Busby, JT
AF Tan, L.
Busby, J. T.
TI Alloying effect of Ni and Cr on irradiated microstructural evolution of
type 304 stainless steels
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
AB Life extension of the existing nuclear power plants imposes significant challenges to core structural materials that suffer increased fluences. This paper presents the microstructural evolution of a type 304 stainless steel and its variants alloyed with extra Ni and Cr under neutron irradiation at similar to 320 degrees C for up to 10.2 dpa. Similar to the reported data of type 304 variants, a large amount of Frank loops, ultrafine G-phase/M23C6 particles, and limited amount of cavities were observed in the irradiated samples. The irradiation promoted the growth of pre-existing M23C6 at grain boundaries and resulted in some phase transformation to CrC in the alloy with both extra Ni and Cr. A new type of ultrafine precipitates, possibly (Ti,Cr)N, was observed in all the samples, and its amount was increased by the irradiation. Additionally, alpha-ferrite was observed in the type 304 steel but not in the Ni or Ni + Cr alloyed variants. The effect of Ni and Cr alloying on the microstructural evolution is discussed. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Tan, L.; Busby, J. T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Tan, L (reprint author), 1 Bethel Valley Rd,POB 2008,MS-6151, Oak Ridge, TN 37831 USA.
EM tanl@ornl.gov
RI Tan, Lizhen/A-7886-2009
OI Tan, Lizhen/0000-0002-3418-2450
FU US Department of Energy (DOE), Office of Nuclear Energy, Light-Water
Reactor Sustainability Program [DE-AC05-00OR22725]; ORNL's Shared
Research Equipment (ShaRE) User Facility; Office of Basic Energy
Sciences, US DOE; UT-Battelle, LLC.
FX This research was sponsored by the US Department of Energy (DOE), Office
of Nuclear Energy, Light-Water Reactor Sustainability Program, under
contract DE-AC05-00OR22725 with UT-Battelle, LLC. Research supported in
part by ORNL's Shared Research Equipment (ShaRE) User Facility, which is
sponsored by the Office of Basic Energy Sciences, US DOE. The authors
thank Dr. M.N. Gussev for managing the irradiated materials, Dr. K.
Leonard assisting TEM characterization, Dr. K.G. Field helpful
discussion, and Ms. S.M. Curlin for preparation of the TEM specimens.
NR 22
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PU ELSEVIER SCIENCE BV
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SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 351
EP 358
DI 10.1016/j.jnucmat.2013.07.054
PG 8
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800048
ER
PT J
AU Gregg, DJ
Zhang, YJ
Middleburgh, SC
Conradson, SD
Triani, G
Lumpkin, GR
Vance, ER
AF Gregg, Daniel J.
Zhang, Yingjie
Middleburgh, Simon C.
Conradson, Steven D.
Triani, Gerry
Lumpkin, Gregory R.
Vance, Eric R.
TI The incorporation of plutonium in lanthanum zirconate pyrochlore
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID DIFFUSE-REFLECTANCE SPECTROSCOPY; BRANNERITE STRUCTURE; URANIUM-DIOXIDE;
OXIDES; SPECTRA; IONS; ZIRCONOLITE; DIFFRACTION; SPECIATION; LA2ZR2O7
AB The incorporation of plutonium (Pu) within lanthanum zirconate pyrochlore was investigated using air, argon, and N-2-3.5%H-2 sintering atmospheres together with Ca2+ and Sr2+ incorporation for charge compensation. The samples have been characterised in the first instance by X-ray diffraction (XRD), scanning electron microscopy (SEM) and diffuse reflectance spectroscopy (DRS). The results show Pu can be exchanged for La3+ on the A-site with and without charge compensation and for Zr4+ on the B-site. DRS measurements were made over the wavenumber range of 4000-19,000 cm(-1) and the Pu in all air- and argon-sintered samples was found to be present as Pu4+ while that in samples sintered in N-2-3.5%H-2 was present as Pu3+. The Pu valence was confirmed for three of the samples using X-ray near-edge absorption spectroscopy (XANES). Pu valences >4+ were not observed in any of the samples. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Gregg, Daniel J.; Zhang, Yingjie; Middleburgh, Simon C.; Triani, Gerry; Lumpkin, Gregory R.; Vance, Eric R.] Australian Nucl Sci & Technol Org, Inst Mat Engn, Kirrawee Dc, NSW 2232, Australia.
[Conradson, Steven D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Gregg, DJ (reprint author), Australian Nucl Sci & Technol Org, Inst Mat Engn, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia.
EM daniel.gregg@ansto.gov.au
RI Lumpkin, Gregory/A-7558-2008;
OI Middleburgh, Simon/0000-0001-6716-4200
NR 47
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U1 2
U2 28
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 444
EP 451
DI 10.1016/j.jnucmat.2013.07.030
PG 8
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800062
ER
PT J
AU Mosbrucker, PL
Brown, DW
Anderoglu, O
Balogh, L
Maloy, SA
Sisneros, TA
Almer, J
Tulk, EF
Morgenroth, W
Dippel, AC
AF Mosbrucker, P. L.
Brown, D. W.
Anderoglu, O.
Balogh, L.
Maloy, S. A.
Sisneros, T. A.
Almer, J.
Tulk, E. F.
Morgenroth, W.
Dippel, A. C.
TI Neutron and X-ray diffraction analysis of the effect of irradiation dose
and temperature on microstructure of irradiated HT-9 steel
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID LINE-PROFILE ANALYSIS; PLASTIC-DEFORMATION; DISLOCATION MODEL; STRAIN
ANISOTROPY; FERRITIC STEELS; CRYSTALS; STABILITY; EVOLUTION; STRENGTH;
PHASES
AB Material harvested from several positions within a nuclear fuel duct (the ACO-3 duct) used in a 6-year irradiation of a fuel assembly in the Fast Flux Test Reactor Facility (FFTF) was examined using neutron and high-energy X-ray diffraction. Samples with a wide range of irradiation dose and irradiation temperature history, reaching doses of up to 147 dpa and temperatures of up to 777 K, were examined. The response of various microstructural characteristics such as the weight fraction of M23C6 carbides, the dislocation density and character, and the crystallographic texture were determined using whole profile analysis of the diffraction data and related to the macroscopic mechanical behavior. For instance, the dislocation density was observed to be intimately linked with observed flow strength of the irradiated materials, following the Taylor law. In general, at the high doses studied in this work, the irradiation temperature is the predominant controlling factor of the dislocation density and, thus, the flow strength of the irradiated material. The results, representing some of the first diffraction work done on samples exposed to such a high received dose, demonstrate how non-destructive and stand-off diffraction techniques can be used to characterize irradiation induced microstructure and at least estimate mechanical properties in irradiated materials without exposing workers to radiation hazards. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Mosbrucker, P. L.; Tulk, E. F.] Kinectrics Inc, Toronto, ON M8Z 5G5, Canada.
[Brown, D. W.; Anderoglu, O.; Balogh, L.; Maloy, S. A.; Sisneros, T. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Almer, J.] Argonne Natl Lab, Argonne, IL 60439 USA.
[Morgenroth, W.] Goethe Univ Frankfurt, Abt Kristallog, Inst Geowissensch, D-60438 Frankfurt, Germany.
[Dippel, A. C.] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.
RP Brown, DW (reprint author), Los Alamos Natl Lab, MS-H805, Los Alamos, NM 87545 USA.
EM dbrown@lanl.gov
RI Maloy, Stuart/A-8672-2009; Balogh, Levente/S-1238-2016;
OI Maloy, Stuart/0000-0001-8037-1319; Mosbrucker,
Paula/0000-0003-0262-7117; Morgenroth, Wolfgang/0000-0001-8921-0052
FU LDRD program; LANL; U.S. DOE [DE-AC02-06CH1135]; U.S. DOE, Office of
Basic Energy Sciences; Los Alamos National Security LLC under DOE
[DE-AC52-06NA25396]
FX This work was supported by LDRD program funding at LANL. Use of the
Advanced Photon Source, an Office of Science User Facility operated for
the U.S. Department of Energy (DOE) Office of Science by Argonne
National Laboratory, was supported by the U.S. DOE under Contract No.
DE-AC02-06CH1135. The Lujan Center at the Los Alamos Neutron Science
Center at LANSCE is funded by the U.S. DOE, Office of Basic Energy
Sciences. Los Alamos National Laboratory is operated by Los Alamos
National Security LLC under DOE contract DE-AC52-06NA25396. Portions of
this research were carried out at the light source PETRA III at DESY, a
member of the Helmholtz Association (HGF). The authors acknowledge Tank
Saleh, John Balog and Toby Romero of LANL and Mychailo Toloczko of PNNL
for their help in preparing and shipping the samples.
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J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 522
EP 530
DI 10.1016/j.jnucmat.2013.07.065
PG 9
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800072
ER
PT J
AU Hales, JD
Williamson, RL
Novascone, SR
Perez, DM
Spencer, BW
Pastore, G
AF Hales, J. D.
Williamson, R. L.
Novascone, S. R.
Perez, D. M.
Spencer, B. W.
Pastore, G.
TI Multidimensional multiphysics simulation of TRISO particle fuel
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID HIGH-TEMPERATURE; FISSION-GAS; HTR FUEL; URANIUM-DIOXIDE; NUCLEAR-FUEL;
IRRADIATION; REACTORS; RELEASE
AB Multidimensional multiphysics analysis of TRISO-coated particle fuel using the BISON finite element nuclear fuels code is described. The governing equations and material models applicable to particle fuel and implemented in BISON are outlined. Code verification based on a recent IAEA benchmarking exercise is described, and excellent comparisons are reported. Multiple TRISO-coated particles of increasing geometric complexity are considered. The code's ability to use the same algorithms and models to solve problems of varying dimensionality from 1D through 3D is demonstrated. The code provides rapid solutions of 10 spherically symmetric and 2D axially symmetric models, and its scalable parallel processing capability allows for solutions of large, complex 3D models. Additionally, the flexibility to easily include new physical and material models and straightforward ability to couple to lower length scale simulations makes BISON a powerful tool for simulation of coated-particle fuel. Future code development activities and potential applications are identified. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Hales, J. D.; Williamson, R. L.; Novascone, S. R.; Perez, D. M.; Spencer, B. W.; Pastore, G.] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Williamson, RL (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA.
EM Jason.Hales@inl.gov; Richard.Williamson@inl.gov;
Stephen.Novascone@inl.gov; Danielle.Perez@inl.gov;
Benjamin.Spencer@inl.gov; Giovanni.Pastore@inl.gov
OI Hales, Jason/0000-0003-0836-0476; Williamson,
Richard/0000-0001-7734-3632; Pastore, Giovanni/0000-0003-2812-506X
FU U.S. Government [DE-AC07-05ID14517]
FX The submitted manuscript has been authored by a contractor of the U.S.
Government under Contract DE-AC07-05ID14517. Accordingly, the U.S.
Government retains a non-exclusive, royalty free license to publish or
reproduce the published form of this contribution, or allow others to do
so, for U.S. Government purposes.
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SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 531
EP 543
DI 10.1016/j.jnucmat.2013.07.070
PG 13
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800073
ER
PT J
AU Short, MP
Hussey, D
Kendrick, BK
Besmann, TM
Stanek, CR
Yip, S
AF Short, M. P.
Hussey, D.
Kendrick, B. K.
Besmann, T. M.
Stanek, C. R.
Yip, S.
TI Multiphysics modeling of porous CRUD deposits in nuclear reactors
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID THERMAL-CONDUCTIVITY; FUEL CRUD; TEMPERATURES; WATER; CONSTANTS; MEDIA
AB The formation of porous CRUD deposits on nuclear reactor fuel rods, a longstanding problem in the operation of pressurized water reactors (PWRs), is a significant challenge to science-based multiscale modeling and simulation. While existing, published studies have focused on individual or loosely coupled processes, such as heat transfer, fluid flow, and compound dissolution/precipitation, none have addressed their coupled effects sufficiently to enable a comprehensive, scientific understanding of CRUD. Here we present the formulation and results of a model, MAMBA-BDM, which begins to incorporate mechanistic details in describing CRUD in PWRs. CRUD is treated as a chemical deposition process in an environment of variable concentration, an arbitrary level of heating, and a complex fractal-based flow geometry. We present results on spatial distributions of temperature, pressure, velocity, and concentration that give insight into the interplay between these physical properties and geometrical parameters. We show the role of heat convection which has not been discussed previously. Furthermore, we suggest that the assumption of liquid saturation in the CRUD deserves scrutiny, as a result of our attempt to determine an effective CRUD thermal conductivity. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Short, M. P.; Yip, S.] MIT, Cambridge, MA 02139 USA.
[Hussey, D.] Elect Power Res Inst, Palo Alto, CA 94304 USA.
[Besmann, T. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Kendrick, B. K.; Stanek, C. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Short, MP (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA.
EM hereiam@mit.edu; dhussey@epri.com; bkendric@lanl.gov;
besmanntm@ornl.gov; stanek@lanl.gov; syip@mit.edu
OI Short, Michael/0000-0002-9216-2482
FU CASL, the Consortium for Advanced Simulation of LWRs
FX The authors wish to acknowledge CASL, the Consortium for Advanced
Simulation of LWRs, for generous funding of this work. The development
of MAMBA-BDM could not be realized without the consultation and support
of many members of the CASL/MPO team, as well as experts from industry.
Special recognition is due to David Andersson (LANL), Don Brenner
(NCSU), Jacopo Buongiorno (MIT), Jeff Deshon (EPRI), Avinash Dongare
(NCSU), Jacob Eapen (NCSU), Derek Gaston (INL), Jim Henshaw (NNL), Zeses
Karoutas (Westinghouse), John McGurk (NNL), Cody Permann (INL), and Jeff
Secker (Westinghouse). Special thanks is also due to Ittinop
Dumnernchanvanit (MIT), for his thorough reading of this manuscript.
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J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 579
EP 587
DI 10.1016/j.jnucmat.2013.08.014
PG 9
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800078
ER
PT J
AU McMurray, JW
Shin, D
Slone, BW
Besmann, TM
AF McMurray, J. W.
Shin, D.
Slone, B. W.
Besmann, T. M.
TI Thermochemical modeling of the U1-yGdyO2 +/- x phase
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SOLID-SOLUTIONS; OXYGEN
POTENTIALS; HIGH-TEMPERATURES; URANIA; SYSTEM; OXIDE; NONSTOICHIOMETRY;
SOLUBILITY
AB A thermodynamic model for the U1-yGdyO2 +/- x phase was developed using the compound energy formalism (CEF) with a three sublattice approach and is an extension of the already successful CEF representation of the fluorite UO2 +/- x phase. The Gibbs energies for the end-members created by the addition of Gd to the cation sublattice are estimated using the lattice stability of a fictive gadolinium oxide fluorite structure compound from density functional theory. The model interaction parameters are determined from reported oxygen potential-temperature-composition measurements. The calculated results are in good agreement with the experimental data and the trends are consistent. The CEF for the U1-yGdyO2 +/- x solid solution can be combined with other representations of actinide and fission product containing fluorite UO2 phases to develop multi-component models within the CEF framework. (C) 2013 Elsevier B.V. All rights reserved.
C1 [McMurray, J. W.; Shin, D.; Slone, B. W.; Besmann, T. M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
RP Besmann, TM (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
EM besmanntm@ornl.gov
RI Shin, Dongwon/C-6519-2008;
OI Shin, Dongwon/0000-0002-5797-3423; McMurray, Jacob/0000-0001-5111-3054
FU US Department of Energy, Office of Nuclear Energy Fuel Cycle Research
and Development Program
FX The authors would like to thank Stewart Voit and Dane Wilson for helpful
comments. The work was supported by the US Department of Energy, Office
of Nuclear Energy Fuel Cycle Research and Development Program.
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J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 588
EP 595
DI 10.1016/j.jnucmat.2013.08.005
PG 8
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800079
ER
PT J
AU Silva, CM
Lindemer, TB
Hunt, RD
Collins, JL
Terrani, KA
Snead, LL
AF Silva, Chinthaka M.
Lindemer, Terrence B.
Hunt, Rodney D.
Collins, Jack L.
Terrani, Kurt A.
Snead, Lance L.
TI Evaluation of sintering effects on SiC-incorporated UO2 kernels under Ar
and Ar-4%H-2 environments
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID SILICON-CARBIDE; FUEL; TEMPERATURE; IRRADIATION; OXIDATION
AB Silicon carbide (SiC) is suggested as an oxygen getter in UO2 kernels used for tristructural isotropic (TRISO) particle fuels and to prevent kernel migration during irradiation. Scanning electron microscopy and X-ray diffractometry analyses performed on sintered kernels verified that an internal gelation process can be used to incorporate SiC in UO2 fuel kernels. Even though the presence of UC in either argon (Ar) or Ar-4%H-2 sintered samples suggested a lowering of the SiC up to 3.5-1.4 mol%, respectively, the presence of other silicon-related chemical phases indicates the preservation of silicon in the kernels during sintering process. UC formation was presumed to occur by two reactions. The first was by the reaction of SiC with its protective SiO2 oxide layer on SiC grains to produce volatile SiO and free carbon that subsequently reacted with UO2 to form UC. The second process was direct UO2 reaction with SiC grains to form SiO, CO, and UC. A slightly higher density and UC content were observed in the sample sintered in Ar-4%H-2, but both atmospheres produced kernels with similar to 95% of theoretical density. It is suggested that incorporating CO in the sintering gas could prevent UC formation and preserve the initial SiC content. Published by Elsevier B.V.
C1 [Silva, Chinthaka M.; Lindemer, Terrence B.; Hunt, Rodney D.; Collins, Jack L.; Terrani, Kurt A.; Snead, Lance L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Silva, Chinthaka M.] Univ Tennessee, Knoxville, TN 37996 USA.
RP Silva, CM (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA.
EM silvagw@ornl.gov
FU US Department of Energy through the Office of Nuclear Energy, Science
and Technology [DE-AC05-00OR22725]; UT-Battelle, LLC; Fuel Cycle and
Isotopes Division; US Department of Energy [DE-AC05-00OR22725]
FX This research was sponsored by the US Department of Energy through the
Office of Nuclear Energy, Science and Technology's Deep-Burn Development
Project under Contract DE-AC05-00OR22725 with UT-Battelle, LLC. The work
was performed at the ORNL under the auspices of the Fuel Cycle and
Isotopes Division.; This manuscript has been authored by the Oak Ridge
National Laboratory, managed by UT-Battelle LLC under Contract No.
DE-AC05-00OR22725 with the US Department of Energy. The US Government
retains and the publisher, by accepting the article for publication,
acknowledges that the US Government retains a nonexclusive, paid-up,
irrevocable, worldwide license to publish or reproduce the published
form of this manuscript, or allow others to do so, for US Government
purposes.
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J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 443
IS 1-3
BP 596
EP 602
DI 10.1016/j.jnucmat.2013.08.007
PG 7
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 264UF
UT WOS:000327905800080
ER
PT J
AU Hill, MA
Schulze, RK
Bingert, JF
Field, RD
McCabe, RJ
Papin, PA
AF Hill, M. A.
Schulze, R. K.
Bingert, J. F.
Field, R. D.
McCabe, R. J.
Papin, P. A.
TI Filiform-mode hydride corrosion of uranium surfaces
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID ALPHA-URANIUM; ALUMINUM SHEET; HYDROGEN; GROWTH; NICKEL; MICROSTRUCTURE;
PRECIPITATION; NUCLEATION; MICROSCOPE; ZIRCALOY-4
AB Hydride nucleation and growth has previously been studied in uranium with an air-formed oxide. Preferred directional growth of uranium hydride has not been observed, presumably due to the constraint of the oxide layer and/or the presence of a surface layer distorted by mechanical grinding and polishing. Instead, hydrides typically first form as subsurface blisters that do not exhibit preferred growth directionality. By eliminating the strained surface layer through electropolishing, removing the natural oxide through ion sputtering, avoiding exposure of the uranium to air, and then exposing uranium to high purity hydrogen in an environmental cell, hydride growth patterns emerge that correspond to defect structures within the microstructure. These hydride growth patterns are similar to filiform corrosion, a type of corrosion that frequently forms under thin protective films. This work describes the first reported observation of filiform-like corrosion in uranium. The uranium hydride initiates at defects, but grows into filaments up to 20 pm wide, and tends to form in straight lines, largely propagating along twin boundaries. Propagation is driven by hydrogen reaction at the filament head, promoted by more efficient delivery of reactant. However, this phenomenon does not involve an electrochemical process associated with conventional filiform corrosion and is therefore described as filiform-like. Hydride growth was observed using optical microscopy for a period of nearly three years. Sample characterization included automated electron backscatter diffraction (EBSD) measurements to determine growth directions. Observation of this anomalous hydride growth provides clues as to the mechanisms operating in uranium hydriding for more conventionally prepared sample surfaces. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Hill, M. A.; Schulze, R. K.; Bingert, J. F.; Field, R. D.; McCabe, R. J.; Papin, P. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Hill, MA (reprint author), Los Alamos Natl Lab, MST-6,Mail Stop G770,POB 1663, Los Alamos, NM 87545 USA.
EM mahill@lanl.gov
OI McCabe, Rodney /0000-0002-6684-7410; Schulze, Roland/0000-0002-6601-817X
FU Enhanced Surveillance Campaign Office; National Nuclear Security
Administration of the U.S. Department of Energy [DE-AC52-06NA25396]
FX The authors acknowledge Rob Aikin for casting the uranium rods and
Robert Hanrahan for useful discussions. The authors also acknowledge the
funding support of the Enhanced Surveillance Campaign Office and its
Program Manager Tom Zocco. This work was performed at Los Alamos
National Laboratory, operated by Los Alamos National Security
Administration, LLC, for the National Nuclear Security Administration of
the U.S. Department of Energy under contract DE-AC52-06NA25396.
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J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 106
EP 115
DI 10.1016/j.jnucmat.2013.08.049
PG 10
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400014
ER
PT J
AU Hosemann, P
Martos, JN
Frazer, D
Vasudevamurthy, G
Byun, TS
Hunn, JD
Jolly, BC
Terrani, K
Okuniewski, M
AF Hosemann, P.
Martos, J. N.
Frazer, D.
Vasudevamurthy, G.
Byun, T. S.
Hunn, J. D.
Jolly, B. C.
Terrani, K.
Okuniewski, M.
TI Mechanical characteristics of SiC coating layer in TRISO fuel particles
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID MEASURING FRACTURE-TOUGHNESS; DEPOSITED SILICON-CARBIDE;
CHEMICAL-VAPOR-DEPOSITION; BRITTLE RING TEST; YOUNGS MODULUS;
SPHERICAL-PARTICLES; STRESS; MICROSTRUCTURE; INDENTATION; TEMPERATURE
AB Tristructural isotropic (TRISO) particles are considered as advanced fuel forms for a variety of fission platforms. While these fuel structures have been tested and deployed in reactors, the mechanical properties of these structures as a function of production parameters need to be investigated in order to ensure their reliability during service. Nanoindentation techniques, indentation crack testing, and half sphere crush testing were utilized in order to evaluate the integrity of the SiC coating layer that is meant to prevent fission product release in the coated particle fuel form. The results are complimented by scanning electron microscopy (SEM) of the grain structure that is subject to change as a function of processing parameters and can alter the mechanical properties such as hardness, elastic modulus, fracture toughness and fracture strength. Through utilization of these advanced techniques, subtle differences in mechanical properties that can be important for in-pile fuel performance can be distinguished and optimized in iteration with processing science of coated fuel particle production. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Hosemann, P.; Martos, J. N.; Frazer, D.] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Vasudevamurthy, G.] Virginia Commonwealth Univ, Richmond, VA 23284 USA.
[Byun, T. S.; Hunn, J. D.; Jolly, B. C.; Terrani, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Okuniewski, M.] Idaho Natl Lab, Idaho Falls, ID USA.
RP Hosemann, P (reprint author), 4169 Etcheverry Hall, Berkeley, CA 94720 USA.
EM peterh@berkeley.edu
OI Frazer, David/0000-0001-5139-858X; Hosemann, Peter/0000-0003-2281-2213
FU NRC [NRC-38-09-948]; US Department of Energy, Office of Nuclear Energy
under DOE Idaho Operations Office [DE-AC07-051D14517]
FX The authors want to thank the NRC for providing funding for this work,
through NRC faculty development grant number NRC-38-09-948. In addition,
we want to thank the DOE/AGR program at ORNL and the NRC safeguards
program for student support.; Instrument access at CAES was supported by
the ATR-NSUF user program at Idaho National Laboratory, which is
supported by the US Department of Energy, Office of Nuclear Energy under
DOE Idaho Operations Office Contract DE-AC07-051D14517.
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SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 133
EP 142
DI 10.1016/j.jnucmat.2013.08.041
PG 10
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400017
ER
PT J
AU Zhuo, MJ
Yan, L
Fu, EG
Wang, YQ
Misra, A
Nastasi, M
Uberuaga, BP
Jia, QX
AF Zhuo, M. J.
Yan, L.
Fu, E. G.
Wang, Y. Q.
Misra, A.
Nastasi, M.
Uberuaga, B. P.
Jia, Q. X.
TI Phase transformations and defect clusters in single crystal SrTiO3
irradiated at different temperatures
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID ION; RECRYSTALLIZATION; CRYSTALLIZATION; DISLOCATION; OXIDES; LOOPS
AB Radiation damage mechanisms in single crystal SrTiO3 irradiated with 250 key Ne ions to a fluence of 1.11 x 10(20) ions/m(2) at both room temperature and 773 K were systematically investigated. The irradiation-induced microstructural evolution was characterized using transmission electron microscopy. Ion irradiation at room temperature results in amorphization of crystalline SrTiO3 near the peak damage region at this fluence. On the other hand, ion irradiation at high temperature leads to less irradiation-induced damage in SrTiO3 due to the higher recovery rate of defects. Nevertheless, the formation of dislocation loops has been observed in the SrTiO3 crystals irradiated at high temperature. These dislocation loops were determined to be unfaulted loops with Burgers vector along < 0 1 1 >. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Zhuo, M. J.; Yan, L.; Fu, E. G.; Misra, A.; Nastasi, M.; Jia, Q. X.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
[Wang, Y. Q.; Uberuaga, B. P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
RP Uberuaga, BP (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
EM blas@lanl.gov; qxjia@lanl.gov
RI Jia, Q. X./C-5194-2008; Misra, Amit/H-1087-2012
FU Center for Materials at Irradiation and Mechanical Extremes, an Energy
Frontier Research Center; U.S. Department of Energy (DOE), Office of
Science, Office of Basic Energy Sciences [2008LANL1026]; National
Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396]
FX The authors wish to acknowledge K.E. Sickafus and T.E. Mitchell for
helpful discussions. This work was supported as part of the Center for
Materials at Irradiation and Mechanical Extremes, an Energy Frontier
Research Center funded by the U.S. Department of Energy (DOE), Office of
Science, Office of Basic Energy Sciences under Award Number
2008LANL1026. This work was performed, in part, at the Center for
Integrated Nanotechnologies, a U.S. DOE, Office of Basic Energy Sciences
user facility. Los Alamos National Laboratory operated by Los Alamos
National Security, LLC, for the National Nuclear Security Administration
of the U.S. DOE under contract DE-AC52-06NA25396
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SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 143
EP 147
DI 10.1016/j.jnucmat.2013.08.046
PG 5
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400018
ER
PT J
AU Nenoff, TM
Ferriera, SR
Huang, JY
Hanson, DJ
AF Nenoff, Tina M.
Ferriera, Summer R.
Huang, Jianyu
Hanson, Donald J.
TI Formation of uranium based nanoparticles via gamma-irradiation
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID COLLOIDAL SILVER; AQUEOUS-SOLUTION; CLUSTERS; NANOALLOYS; OXIDATION;
ALLOY
AB The ability to fabricate nuclear fuels at low temperatures allows for the production of complex Uranium metal and alloys with minimum volatility of alloy components in the process. Gamma irradiation is a valuable method for the synthesis of a wide range of metal-based nanoparticles. We report on the synthesis via room temperature radiolysis and characterization of uranium (depleted, d-U) metal and uranium-lathanide (d-ULn, Ln = lanthanide surrogates) alloy nanoparticles from aqueous acidic salt solutions. The lanthanide surrogates chosen include La and Eu due to their similarity in ionic size and charge in solution. Detailed characterization results including UV-vis, TEM/HR-TEM, and single particle EDX (elemental analyses) are presented for the room temperature formed nanoparticle products. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Nenoff, Tina M.; Ferriera, Summer R.] Sandia Natl Labs, Nanoscale Sci Dept, Albuquerque, NM 87185 USA.
[Huang, Jianyu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA.
[Hanson, Donald J.] Sandia Natl Labs, Dept Hot Cells & Gamma Facil, Albuquerque, NM 87185 USA.
RP Nenoff, TM (reprint author), Sandia Natl Labs, Nanoscale Sci Dept, POB 5800,MS-1415, Albuquerque, NM 87185 USA.
EM tmnenof@sandia.gov
FU Sandia's Laboratory Directed Research and Development (LDRD) program;
U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]
FX The authors acknowledge financial support from Sandia's Laboratory
Directed Research and Development (LDRD) program.; Sandia National
Laboratories is a multi-program laboratory managed and operated by
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000.
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SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 162
EP 167
DI 10.1016/j.jnucmat.2013.08.027
PG 6
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400020
ER
PT J
AU Barrow, L
Barrow, ATW
Almer, J
Daymond, MR
AF Barrow, L.
Barrow, A. T. W.
Almer, J.
Daymond, M. R.
TI The Zr20Nb-H phase diagram and the characterisation of hydrides in
beta-Zr
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID WT-PERCENT NB; ZIRCONIUM HYDRIDE; PRECIPITATION KINETICS;
NEUTRON-DIFFRACTION; ALLOYS; TRANSFORMATION; SOLUBILITY; NUCLEATION;
ZIRCALOY-4; STABILITY
AB In this work a combination of synchrotron X-ray diffraction, transmission electron microscopy and differential scanning calorimetry have been used to characterise the Zr20Nb-H phase diagram and hydrides in beta-Zr. A single hydride phase, termed gamma' was found to be present in beta-Zr over a wide range of H concentrations up to 1559 wppm. gamma'-hydride had an orthorhombic crystal structure with the composition ZrH0.4 +/- 0.2, and was found to be stable during heating to 450 degrees C; it can therefore be considered the equilibrium hydride in beta-Zr. Accompanying hydride nucleation is a volumetric strain of 10.4% that is accommodated elastically and plastically by the beta-Zr. The body-centre cubic to orthorhombic martensitic transformation is analogous to the Au-Cd system where the basal plane in the hydride is constructed from the (0 1 1)(beta) to give the Bain correspondence. There are strong similarities between the Zr20Nb-H and Nb-H phase diagrams with the former having a lower solubility for H at room temperature, similar to 130 wppm and similar to 290 wppm respectively. The room temperature solubility difference between body-centre cubic Nb and beta-Zr can be attributed to their electron configurations and the reduction in energy associated with the metallic Zr/Nb-H bonding. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Barrow, L.; Barrow, A. T. W.; Daymond, M. R.] Queens Univ, Dept Mech & Mat Engn, Nucl Mat Grp, Kingston, ON K7L 3N6, Canada.
[Almer, J.] Argonne Natl Lab, Argonne, IL 60439 USA.
RP Daymond, MR (reprint author), Queens Univ, Dept Mech & Mat Engn, Nucl Mat Grp, Kingston, ON K7L 3N6, Canada.
EM daymond@me.queensu.ca
FU NSERC; COG; OPG; Nu-Tech Precision Metals under the Industrial Research
Chair programme in Nuclear Materials at Queen's University; U.S.
Department of Energy, Office of Basic Energy Sciences
[DE-AC02-06CH11357]
FX This work was sponsored by NSERC, COG, OPG and Nu-Tech Precision Metals
under the Industrial Research Chair programme in Nuclear Materials at
Queen's University. Usage of the Advanced Photon Source (APS) was
supported by the U.S. Department of Energy, Office of Basic Energy
Sciences under contract number DE-AC02-06CH11357. The electron-energy
loss spectroscopy described in this paper was performed at the Canadian
Centre for Electron Microscopy at McMaster University, which is
supported by NSERC and other government agencies. The differential
scanning calorimetry work was carried by Patrick Wilson at Atomic Energy
Canada Ltd.
NR 43
TC 3
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U1 6
U2 11
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 292
EP 297
DI 10.1016/j.jnucmat.2013.08.031
PG 6
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400036
ER
PT J
AU Dinh, LN
Cairns, GA
Krueger, R
Mayer, BP
Maxwell, RS
AF Dinh, L. N.
Cairns, G. A.
Krueger, R.
Mayer, B. P.
Maxwell, R. S.
TI Aging aspects of DEB getters
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID CARBON-MONOXIDE; HYDROGEN UPTAKE; DESORPTION; PALLADIUM; KINETICS;
SURFACES; DPB
AB The changes in uptake capacity of 1,4-bis(phenylethynyl)benzene (DEB) blended with carbon-supported Pd (DEB-Pd/C) in the form of pellets as a function of temperature and time were investigated. Experimental results revealed a segregation and crystallization of DEB molecules toward the geometrical surfaces of the getter pellets, but very little or no diffusion-aggregation of Pd nano-catalysts even after long term storage at 75 degrees C in nitrogen. Despite the observation of surface segregation and crystallization of DEB molecules with increasing temperature and time, statistically there was no reduction in uptake capacity for the getter pellets stored at higher temperature. However, significant reversible reductions in uptake capacity was found among getter pellets exposed to air for extended time. The possible causes for these observations and their respective roles in the aging of getters are discussed. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Dinh, L. N.; Krueger, R.; Mayer, B. P.; Maxwell, R. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Cairns, G. A.] AWE plc, Reading, Berks, England.
RP Dinh, LN (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
EM dinh1@llnl.gov
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]
FX This work was performed under the auspices of the U.S. Department of
Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344. Furthermore the authors express their gratitude to
Dogan Ozkaya for the microscopy work, carried out under contract to AWE,
at Johnson Matthey.
NR 14
TC 2
Z9 2
U1 4
U2 10
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 298
EP 305
DI 10.1016/j.jnucmat.2013.09.018
PG 8
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400037
ER
PT J
AU Lepry, WC
Riley, BJ
Crum, JV
Rodriguez, CP
Pierce, DA
AF Lepry, William C.
Riley, Brian J.
Crum, Jarrod V.
Rodriguez, Carmen P.
Pierce, David A.
TI Solution-based approaches for making high-density sodalite waste forms
to immobilize spent electrochemical salts
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID ENCLATHRATED SODALITE; CRYSTAL-CHEMISTRY; DIFFRACTION; NEPHELINE;
MINERALS; FAMILY; CESIUM; PART; NAOH
AB Three different solution-based approaches were taken to make sodalite minerals as a host for a mixed salt simulating the waste in the electrochemical separations process of nuclear fuel reprocessing. The methods used an aqueous solution of mixed chlorides (simulated waste) but the other reactants varied: (1) Al(OH)(3) + NaOH + CS, (2) NaAlO2 + CS, and (3) Al2Si2O7 + NaOH, (CS = colloidal silica). The products were dried, ground, pressed into pellets, and fired at 650-950 degrees C. In some cases, either 5 or 10 mass% of a Si-Na-B oxide glass sintering aid was introduced at different stages in the process. Method (2) proved the most successful at producing high sodalite fractions (up to 100%) with minimal sintering aid additions and showed high consolidation potential (up to 91.4% of theoretical density) at reduced firing temperatures. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Lepry, William C.; Riley, Brian J.; Crum, Jarrod V.; Rodriguez, Carmen P.; Pierce, David A.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Riley, BJ (reprint author), Pacific NW Natl Lab, POB 999,MSIN K6-24, Richland, WA 99352 USA.
EM brian.riley@pnnl.gov
OI Riley, Brian/0000-0002-7745-6730
FU Battelle [DE-AC05-76RL01830]
FX The Pacific Northwest National Laboratory is operated by Battelle under
Contract Number DE-AC05-76RL01830. Authors thank Xiaohong (Shari) Li for
help with BET measurements, John McCloy for helpful review of this
document as well as Thomas Johnson and Steven Frank for project
oversight. Authors also thank the Southwest Research Institute for
analytical services of the PCT rinsates and leachates.
NR 48
TC 6
Z9 6
U1 1
U2 11
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 350
EP 359
DI 10.1016/j.jnucmat.2013.08.033
PG 10
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400044
ER
PT J
AU Kim, JH
Byun, TS
Hoelzer, DT
AF Kim, Jeoung Han
Byun, Thak Sang
Hoelzer, D. T.
TI High temperature deformation mechanisms of nano-structured ferritic
alloys in the context of internal variable theory of inelastic
deformation
SO JOURNAL OF NUCLEAR MATERIALS
LA English
DT Article
ID DISPERSION-STRENGTHENED-STEELS; CONSTITUTIVE ANALYSIS;
STRESS-RELAXATION; BEHAVIOR; TI-6AL-4V
AB The stress relaxation behavior of 14YWT and ODS-Eurofer97 was examined within the framework of an internal-variable theory of inelastic deformation. Stress versus strain rate curves obtained by stress relaxation tests for 14YWT were described well by the equations for grain-matrix deformation while those of ODS-Eurofer97 were fitted with the combined curves of grain matrix deformation and grain boundary sliding. The sudden drop of total elongation of 14YWT was discussed in light of fracture surface observations. Grain boundary decohesion at 900 degrees C was identified. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Kim, Jeoung Han] Korea Inst Mat Sci, Struct Mat Div, Chang Won 642831, Sangnamdong, South Korea.
[Byun, Thak Sang; Hoelzer, D. T.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA.
RP Kim, JH (reprint author), Korea Inst Mat Sci, Chang Won 642831, Sangnamdong, South Korea.
EM kjh1754@kims.re.kr
RI Hoelzer, David/L-1558-2016
NR 19
TC 1
Z9 1
U1 1
U2 11
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3115
EI 1873-4820
J9 J NUCL MATER
JI J. Nucl. Mater.
PD NOV
PY 2013
VL 442
IS 1-3
BP 458
EP 462
DI 10.1016/j.jnucmat.2013.02.048
PG 5
WC Materials Science, Multidisciplinary; Nuclear Science & Technology
SC Materials Science; Nuclear Science & Technology
GA 268MQ
UT WOS:000328175400060
ER
PT J
AU Wierer, JJ
Tsao, JY
Sizov, DS
AF Wierer, Jonathan J., Jr.
Tsao, Jeffrey Y.
Sizov, Dmitry S.
TI Comparison between blue lasers and light-emitting diodes for future
solid-state lighting
SO LASER & PHOTONICS REVIEWS
LA English
DT Article
DE Solid-state lighting; LEDs; LDs; light-emitting diodes; laser diodes;
semiconductor laser; blue lasers; III-nitride; InGaN; AlInGaN;
power-conversion efficiency; efficiency droop; quantum efficiency;
phosphor-converted LEDs; PC-LEDs; gain; semipolar GaN; Auger
recombination; cost of light; thermal management; heat management; heat
sink; areal chip cost
ID QUANTUM-WELL LASER; OPTICAL GAIN SPECTRA; HIGH-POWER; INGAN LASER;
DEGRADATION MECHANISMS; SEMICONDUCTOR-LASERS; LIFT-OFF; GAN; EFFICIENCY;
LEDS
AB Solid-state lighting (SSL) is now the most efficient source of high color quality white light ever created. Nevertheless, the blue InGaN light-emitting diodes (LEDs) that are the light engine of SSL still have significant performance limitations. Foremost among these is the decrease in efficiency at high input current densities widely known as efficiency droop. Efficiency droop limits input power densities, contrary to the desire to produce more photons per unit LED chip area and to make SSL more affordable. Pending a solution to efficiency droop, an alternative device could be a blue laser diode (LD). LDs, operated in stimulated emission, can have high efficiencies at much higher input power densities than LEDs can. In this article, LEDs and LDs for future SSL are explored by comparing: their current state-of-the-art input-power-density-dependent power-conversion efficiencies; potential improvements both in their peak power-conversion efficiencies and in the input power densities at which those efficiencies peak; and their economics for practical SSL.
C1 [Wierer, Jonathan J., Jr.; Tsao, Jeffrey Y.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Sizov, Dmitry S.] Corning Inc, Corning, NY 14831 USA.
RP Wierer, JJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.
EM jwierer@sandia.gov
RI Wierer, Jonathan/G-1594-2013
OI Wierer, Jonathan/0000-0001-6971-4835
FU Sandia's Solid-State-Lighting Science Energy Frontier Research Center;
U.S. Department of Energy, Office of Basic Energy Sciences. Sandia
National Laboratories; U.S. Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX The authors would like to thank Mike Coltrin, Weng Chow, Art Fischer,
and Nathan Young for their careful reading and useful suggestions for
the manuscript. Work at Sandia National Laboratories was supported by
Sandia's Solid-State-Lighting Science Energy Frontier Research Center,
funded by the U.S. Department of Energy, Office of Basic Energy
Sciences. Sandia National Laboratories is a multiprogram laboratory
managed and operated by Sandia Corporation, a wholly owned subsidiary of
Lockheed Martin Corporation, for the U.S. Department of Energy's
National Nuclear Security Administration under contract
DE-AC04-94AL85000.
NR 158
TC 66
Z9 67
U1 21
U2 127
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1863-8880
EI 1863-8899
J9 LASER PHOTONICS REV
JI Laser Photon. Rev.
PD NOV
PY 2013
VL 7
IS 6
BP 963
EP 993
DI 10.1002/lpor.201300048
PG 31
WC Optics; Physics, Applied; Physics, Condensed Matter
SC Optics; Physics
GA 268EA
UT WOS:000328150300016
ER
PT J
AU Jain, N
Buchner, J
Dorfman, S
Ji, HT
Sharma, AS
AF Jain, Neeraj
Buechner, Joerg
Dorfman, Seth
Ji, Hantao
Sharma, A. Surjalal
TI Current disruption and its spreading in collisionless magnetic
reconnection
SO PHYSICS OF PLASMAS
LA English
DT Article
ID THIN CURRENT SHEETS; ELECTRON MAGNETOHYDRODYNAMICS; 3-DIMENSIONAL
RECONNECTION; IMPULSIVE RECONNECTION; KINETIC SIMULATIONS;
MODE-INSTABILITY; X-LINE; SUBSTORMS; PLASMAS
AB Recent magnetic reconnection experiments (MRX) [Dorfman et al., Geophys. Res. Lett. 40, 233 (2013)] have disclosed current disruption in the absence of an externally imposed guide field. During current disruption in MRX, both the current density and the total observed out-of-reconnection-plane current drop simultaneous with a rise in out-of-reconnection-plane electric field. Here, we show that current disruption is an intrinsic property of the dynamic formation of an X-point configuration of magnetic field in magnetic reconnection, independent of the model used for plasma description and of the dimensionality (2D or 3D) of reconnection. An analytic expression for the current drop is derived from Ampere's Law. Its predictions are verified by 2D and 3D electron-magnetohydrodynamic (EMHD) simulations. Three dimensional EMHD simulations show that the current disruption due to localized magnetic reconnection spreads along the direction of the electron drift velocity with a speed which depends on the wave number of the perturbation. The implications of these results for MRX are discussed. (C) 2013 AIP Publishing LLC.
C1 [Jain, Neeraj; Buechner, Joerg; Ji, Hantao] Max Planck Princeton Ctr Plasma Phys, D-37191 Katlenburg Lindau, Germany.
[Jain, Neeraj; Buechner, Joerg] Max Planck Inst Solar Syst Res, D-37191 Katlenburg Lindau, Germany.
[Dorfman, Seth] Univ Calif Los Angeles, Los Angeles, CA 90095 USA.
[Ji, Hantao] Princeton Univ, Deparment Astrophys Sci, Princeton, NJ 08540 USA.
[Ji, Hantao] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA.
[Sharma, A. Surjalal] Univ Maryland, Dept Astron, College Pk, MD 20742 USA.
RP Jain, N (reprint author), Max Planck Princeton Ctr Plasma Phys, D-37191 Katlenburg Lindau, Germany.
FU Max-Planck/Princeton Center for Plasma Physics [M.MC.A.Aero8003 Max
Planck]; NSF [AGS 1027185]; DOS FES Fellowship; NDSEG Fellowship Program
[DE-AC02-09CH11466]
FX The work of N.J. was funded by the Max-Planck/Princeton Center for
Plasma Physics (Grant No. M.MC.A.Aero8003 Max Planck) and the NSF grant
(AGS 1027185) to the University of Maryland. The work of A.S. Sharma was
funded by the NSF grant (AGS 1027185) to the University of Maryland.
S.D. was supported by a DOS FES Fellowship and the NDSEG Fellowship
Program (Contract No. DE-AC02-09CH11466). The MPS authors (N.J. and
J.B.) thank Dr. Bernhardt Bandow for his help to numerically optimize
the EMHD code.
NR 38
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Z9 6
U1 3
U2 6
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD NOV
PY 2013
VL 20
IS 11
AR 112101
DI 10.1063/1.4827828
PG 11
WC Physics, Fluids & Plasmas
SC Physics
GA 270MY
UT WOS:000328323800003
ER
PT J
AU Schmit, PF
Molvig, K
Nakhleh, CW
AF Schmit, P. F.
Molvig, Kim
Nakhleh, C. W.
TI Tail-ion transport and Knudsen layer formation in the presence of
magnetic fields
SO PHYSICS OF PLASMAS
LA English
DT Article
ID CYLINDRICAL GEOMETRY; KINETIC SIMULATIONS; IGNITION CONDITIONS; TARGET
FUSION; ICF TARGETS; IMPLOSIONS; PLASMA; BURN
AB Knudsen layer losses of tail fuel ions could reduce significantly the fusion reactivity of highly compressed cylindrical and spherical targets in inertial confinement fusion (ICF). With the class of magnetized ICF targets in mind, the effect of embedded magnetic fields on Knudsen layer formation is investigated for the first time. The modified energy scaling of ion diffusivity in magnetized hot spots is found to suppress the preferential losses of tail-ions perpendicular to the magnetic field lines to a degree that the tail distribution can be at least partially, if not fully, restored. Two simple threshold conditions are identified leading to the restoration of fusion reactivity in magnetized hot spots. A kinetic equation for tail-ion transport in the presence of a magnetic field is derived, and solutions to the equation are obtained numerically in simulations. Numerical results confirm the validity of the threshold conditions for restored reactivity and identify two different asymptotic regimes of the fusion fuel. While Knudsen layer formation is shown to be suppressed entirely in strongly magnetized cylindrical hot spot cavities, uniformly magnetized spherical cavities demonstrate remnant, albeit reduced, levels of tail-ion depletion. (C) 2013 AIP Publishing LLC.
C1 [Schmit, P. F.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Molvig, Kim; Nakhleh, C. W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Schmit, PF (reprint author), Sandia Natl Labs, MS 1186,POB 5800, Albuquerque, NM 87185 USA.
FU Sandia National Laboratories Truman Fellowship in National Security
Science and Engineering; Sandia National Laboratories Truman Fellowship
in National Security Science and Engineering, which is part of the
Laboratory Directed Research and Development (LDRD) Program; Sandia
Corporation under its U.S. Department of Energy [DE-AC04-94AL85000]
FX The authors gratefully acknowledge Adam Sefkow, Dan Sinars, Patrick
Knapp, Evan Dodd, and Brian Albright for many useful discussions. This
research was supported in part by an appointment to the Sandia National
Laboratories Truman Fellowship in National Security Science and
Engineering, which is part of the Laboratory Directed Research and
Development (LDRD) Program, and sponsored by Sandia Corporation (a
wholly owned subsidiary of Lockheed Martin Corporation) as Operator of
Sandia National Laboratories under its U. S. Department of Energy
Contract No. DE-AC04-94AL85000.
NR 32
TC 14
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U1 0
U2 6
PU AMER INST PHYSICS
PI MELVILLE
PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD NOV
PY 2013
VL 20
IS 11
AR 112705
DI 10.1063/1.4831958
PG 15
WC Physics, Fluids & Plasmas
SC Physics
GA 270MY
UT WOS:000328323800036
ER
PT J
AU Sun, X
Intrator, TP
Liu, M
Sears, J
Weber, T
AF Sun, X.
Intrator, T. P.
Liu, M.
Sears, J.
Weber, T.
TI A phenomenological model on the kink mode threshold varying with the
inclination of sheath boundary
SO PHYSICS OF PLASMAS
LA English
DT Article
ID FLUX ROPES; PLASMA; INSTABILITY
AB In nature and many laboratory plasmas, a magnetic flux tube threaded by current or a flux rope has a footpoint at a boundary. The current driven kink mode is one of the fundamental ideal magnetohydrodynamic instabilities in plasmas. It has an instability threshold that has been found to strongly depend on boundary conditions (BCs). We provide a theoretical model to explain the transition of this threshold dependence between nonline tied and line tied boundary conditions. We evaluate model parameters using experimentally measured plasma data, explicitly verify several kink eigenfunctions, and validate the model predictions for boundary conditions BCs that span the range between NLT and LT BCs. Based on this model, one could estimate the kink threshold given knowledge of the displacement of a flux rope end, or conversely estimate flux rope end motion based on knowledge of it kink stability threshold. (C) 2013 AIP Publishing LLC.
C1 [Sun, X.; Liu, M.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China.
[Sun, X.; Intrator, T. P.; Sears, J.; Weber, T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Sun, X (reprint author), Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China.
FU DOE [DE-AC52-06NA25396]; DOE Office Fusion Energy Sciences; NASA
Geospace [NNHIOA044I]; NSF Center for Magnetic Self Organization; MOST
of China [2013GB112007]
FX T.P.I. acknowledges support from DOE DE-AC52-06NA25396; DOE Office
Fusion Energy Sciences; NASA Geospace NNHIOA044I; NSF Center for
Magnetic Self Organization. X.S. acknowledges support from MOST of
China, Contract number 2013GB112007.
NR 26
TC 2
Z9 2
U1 2
U2 4
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD NOV
PY 2013
VL 20
IS 11
AR 112106
DI 10.1063/1.4829431
PG 7
WC Physics, Fluids & Plasmas
SC Physics
GA 270MY
UT WOS:000328323800008
ER
PT J
AU Terry, PW
Pueschel, MJ
Carmody, D
Nevins, WM
AF Terry, P. W.
Pueschel, M. J.
Carmody, D.
Nevins, W. M.
TI The effect of magnetic flutter on residual flow
SO PHYSICS OF PLASMAS
LA English
DT Article
ID TURBULENCE; TOKAMAKS; DRIVEN
AB The hypothesis that stochastic magnetic fields disrupt zonal flows associated with ion temperature gradient turbulence saturation is investigated analytically with a residual flow calculation in the presence of magnetic flutter. The calculation starts from the time-asymptotic zero-beta residual flow of Rosenbluth and Hinton [Phys. Rev. Lett. 80, 724 (1998)] with the sudden application of an externally imposed, fixed magnetic field perturbation. The short-time electron response from radial charge loss due to magnetic flutter is calculated from the appropriate gyrokinetic equation. The potential evolution has quadratic behavior, with a zero crossing at finite time. The crossing time and its parametric dependencies are compared with numerical results from a gyrokinetic simulation of residual flow in the presence of magnetic flutter. The numerical and analytical results are in good agreement and support the hypothesis that the high-beta runaway of numerical simulations is a result of the disabling of zonal flows by finite-beta charge losses associated with magnetic flutter. (C) 2013 AIP Publishing LLC.
C1 [Terry, P. W.; Pueschel, M. J.; Carmody, D.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA.
[Nevins, W. M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA.
RP Terry, PW (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA.
FU US Department of Energy [DE-FG02-89ER53291]; Center for Momentum
Transport and Flow Organization
FX The authors acknowledge useful conversations with Frank Jenko, Chris
Hegna, and Felix Parra. This work was supported by US Department of
Energy (Grant No. DE-FG02-89ER53291) and the Center for Momentum
Transport and Flow Organization.
NR 18
TC 6
Z9 6
U1 1
U2 7
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 1070-664X
EI 1089-7674
J9 PHYS PLASMAS
JI Phys. Plasmas
PD NOV
PY 2013
VL 20
IS 11
AR 112502
DI 10.1063/1.4828396
PG 10
WC Physics, Fluids & Plasmas
SC Physics
GA 270MY
UT WOS:000328323800024
ER
PT J
AU Shehabi, A
DeForest, N
McNeil, A
Masanet, E
Greenblatt, J
Lee, ES
Masson, G
Helms, BA
Milliron, DJ
AF Shehabi, Arman
DeForest, Nicholas
McNeil, Andrew
Masanet, Eric
Greenblatt, Jeffery
Lee, Eleanor S.
Masson, Georgeta
Helms, Brett A.
Milliron, Delia J.
TI U.S. energy savings potential from dynamic daylighting control glazings
SO ENERGY AND BUILDINGS
LA English
DT Article
DE Indoor environmental quality; Energy efficiency; Day lighting; Radiance;
Glare; Dynamic prismatic optical elements (dPOE); Windows; Clerestories
ID PERFORMANCE
AB Daylighting controls have the potential to reduce the substantial amount of electricity consumed for lighting in commercial buildings. Material science research is now pursuing the development of a dynamic prismatic optical element (dPOE) window coating that can continuously readjust incoming light to maximize the performance and energy savings available from daylighting controls. This study estimates the technical potential for energy savings available from vertical daylighting strategies and explores additional savings that may be available if current dPOE research culminates in a successful market-ready product. Radiance daylight simulations are conducted with a multi-shape prismatic window coating. Simulated lighting energy savings are then applied to perimeter floorspace estimates generated from U.S. commercial building stock data. Results indicate that fully functional dPOE coatings, when paired with conventional vertical daylight strategies, have the potential to reduce energy use associated with U.S. commercial electric lighting demand by as much as 930TBtu. This reduction in electric lighting demand represents an approximately 85% increase in the energy savings estimated from implementing conventional vertical daylight strategies alone. Results presented in this study provide insight into energy and cost performance targets for dPOE coatings, which can help accelerate the development process and establish a successful new daylighting technology. Published by Elsevier B.V.
C1 [Shehabi, Arman; DeForest, Nicholas; McNeil, Andrew; Greenblatt, Jeffery; Lee, Eleanor S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Masanet, Eric] Northwestern Univ, McCormick Sch Engn, Evanston, IL 60208 USA.
[Masson, Georgeta; Helms, Brett A.; Milliron, Delia J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
RP Shehabi, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd,Bldg 90R2000, Berkeley, CA 94720 USA.
EM ashehabi@lbl.gov
RI Masanet, Eric /I-5649-2012; McNeil, Andrew/I-9530-2014; Milliron,
Delia/D-6002-2012; Foundry, Molecular/G-9968-2014;
OI McNeil, Andrew/0000-0001-9994-9002; Helms, Brett/0000-0003-3925-4174
FU Office of Science, Office of Basic Energy Sciences; DOE Early Career
Research Program Award; Laboratory Directed Research and Development
Program of Lawrence Berkeley National Laboratory; US DOE
[DE-AC02-05CH11231]
FX The authors thank William Morrow for his assistance with ArcGIS and
James O'Donnell for his work compiling ASHRAE 90.1 lighting schedules.
This work was conducted at Lawrence Berkeley National Laboratory.
Portions of this project were carried out at the Molecular Foundry,
Lawrence Berkeley National Laboratory, which is supported by the Office
of Science, Office of Basic Energy Sciences. D.J.M. was supported by a
DOE Early Career Research Program Award. Portions of this project were
supported by the Laboratory Directed Research and Development Program of
Lawrence Berkeley National Laboratory. All work was performed under the
US DOE Contract No. DE-AC02-05CH11231.
NR 23
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PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0378-7788
EI 1872-6178
J9 ENERG BUILDINGS
JI Energy Build.
PD NOV
PY 2013
VL 66
BP 415
EP 423
DI 10.1016/j.enbuild.2013.07.013
PG 9
WC Construction & Building Technology; Energy & Fuels; Engineering, Civil
SC Construction & Building Technology; Energy & Fuels; Engineering
GA 264TP
UT WOS:000327904200044
ER
PT J
AU Chan, WYR
Joh, J
Sherman, MH
AF Chan, Wanyu R.
Joh, Jeffrey
Sherman, Max H.
TI Analysis of air leakage measurements of US houses
SO ENERGY AND BUILDINGS
LA English
DT Article
DE Blower door; Fan pressurization test; Normalized leakage; Air
infiltration; Building envelope airtightness
ID RATES; MODEL
AB Building envelope airtightness is important for residential energy use, occupant health and comfort. We analyzed the air leakage measurements of 134,000 single-family detached homes in US, using normalized leakage (NL) as the metric. Weatherization assistance programs (WAPs) and residential energy efficiency programs contributed most of the data. We performed regression analyses to examine the relationship between NL and various house characteristics. Explanatory variables that are correlated with NL include year built, climate zone, floor area, house height, and whether homes participated in WAPs or if they are energy efficiency rated homes. Foundation type and whether ducts are located outside or inside the conditioned space are also found to be useful parameters for predicting NL. We developed a regression model that explains approximately 68% of the observed variability across US homes. Of these variables considered, year built and climate zone are the two that have the largest influence on NL. The regression model can be used to predict air leakage values for individual homes, and distributions for groups of homes, based on their characteristics. Using RECS 2009 data, the regression model predicts 90% of US houses have NL between 0.22 and 1.95, with a median of 0.67. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Chan, Wanyu R.; Joh, Jeffrey; Sherman, Max H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
RP Chan, WYR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd,Mailstop 90R3058, Berkeley, CA 94720 USA.
EM wrchan@lbl.gov
FU California Energy Commission Public Interest Energy Research Program
[CEC-500-07-006]; Assistant Secretary for Energy Efficiency and
Renewable Energy, Building Technologies Program [DE-AC02-05CH11231]
FX We greatly appreciate the organizations and individuals who shared their
blower door measurements and other diagnostic data with us. This work
was supported by the California Energy Commission Public Interest Energy
Research Program award number CEC-500-07-006 and the Assistant Secretary
for Energy Efficiency and Renewable Energy, Building Technologies
Program, of the US Department of Energy under contract No.
DE-AC02-05CH11231.
NR 27
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PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0378-7788
EI 1872-6178
J9 ENERG BUILDINGS
JI Energy Build.
PD NOV
PY 2013
VL 66
BP 616
EP 625
DI 10.1016/j.enbuild.2013.07.047
PG 10
WC Construction & Building Technology; Energy & Fuels; Engineering, Civil
SC Construction & Building Technology; Energy & Fuels; Engineering
GA 264TP
UT WOS:000327904200066
ER
PT J
AU Fox, EB
Liu, ZW
Liu, ZT
AF Fox, Elise B.
Liu, Zhong-Wen
Liu, Zhao-Tie
TI Ultraclean Fuels Production and Utilization for the Twenty-First
Century: Advances toward Sustainable Transportation Fuels
SO ENERGY & FUELS
LA English
DT Review
ID FISCHER-TROPSCH SYNTHESIS; CATALYSTS; HYDRODESULFURIZATION;
DESULFURIZATION; BIOMASS; STREAMS; SYNGAS; SULFUR
AB Ultraclean fuels production has become increasingly important as a method to help decrease emissions and allow for the introduction of alternative feedstocks for transportation fuels. Established methods, such as Fischer-Tropsch, have seen a resurgence of interest as natural gas prices drop and existing petroleum resources require more intensive cleanup and purification to meet stringent environmental standards. This review covers some of the advances in deep desulfurization and synthesis gas conversion into fuels and feedstocks that were presented at the 245th American Chemical Society (ACS) Spring Annual Meeting in New Orleans, LA, in the Division of Energy and Fuels symposium on "Ultraclean Fuels Production and Utilization".
C1 [Fox, Elise B.] Savannah River Natl Lab, Aiken, SC 29808 USA.
[Liu, Zhong-Wen; Liu, Zhao-Tie] Shaanxi Normal Univ, Sch Chem & Chem Engn, Key Lab Appl Surface & Colloid Chem, Xian 710062, Peoples R China.
RP Fox, EB (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA.
EM elise.fox@srnl.doe.gov
RI Fox, Elise/G-5438-2013;
OI Fox, Elise/0000-0002-4527-5820; LIU, ZHAO-TIE/0000-0002-8107-8234
FU ACS Division of Energy and Fuels; [DE-AC09-08SR22470]
FX The authors wish to thank the ACS Division of Energy and Fuels and
Program Chairs Yun Hang Hu and Todd H. Gardner for their support on this
effort. Dr. Elise Fox is an employee of Savannah River National
Laboratory, which is managed by Savannah River Nuclear Solutions. Her
portion of this work was prepared under Federal Contract
DE-AC09-08SR22470. The United States Government retains, and by
accepting the article for publication the publisher acknowledges that
the United States Government retains, a non-exclusive, paid-up,
irrevocable, worldwide license to publish or reproduce the published
form of this work, or allow others to do so, for United States
Government purposes.
NR 43
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD NOV
PY 2013
VL 27
IS 11
BP 6335
EP 6338
DI 10.1021/ef401094t
PG 4
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 259WU
UT WOS:000327557800001
ER
PT J
AU Fox, EB
Smith, LT
Williamson, TK
Kendrick, SE
AF Fox, Elise B.
Smith, L. Taylor
Williamson, Tyler K.
Kendrick, Sarah E.
TI Aging Effects on the Properties of Imidazolium-, Quaternary Ammonium-,
Pyridinium-, and Pyrrolidinium-Based Ionic Liquids Used in Fuel and
Energy Production
SO ENERGY & FUELS
LA English
DT Article
ID HEAT-TRANSFER FLUIDS; THERMAL-DEGRADATION; INFRARED-SPECTRA; WATER;
HEXAFLUOROPHOSPHATE; DESULFURIZATION; SOLVENTS; GASOLINE; SALTS; NEILS
AB Ionic liquids (ILs) are often cited for their excellent thermal stability, a key property for their use as solvents and in the chemical processing of biofuels. However, there has been little supporting data on the long-term aging effect of the temperature on these materials. Imizadolium-, quaternary ammonium-, pyridinium-, and pyrrolidnium-based ILs with the bis(trifluoromethylsulfonyl)imide and bis(perfluoroethylsulfonyl)imide anions were aged for 2520 h (15 weeks) at 200 C in air to determine the effects of an oxidizing environment on their chemical structure and thermal stability over time. It was found that the minor changes in the cation chemistry could greatly affect the properties of the ILs over time.
C1 [Fox, Elise B.; Smith, L. Taylor; Williamson, Tyler K.; Kendrick, Sarah E.] Savannah River Natl Lab, Aiken, SC 29808 USA.
RP Fox, EB (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA.
EM elise.fox@srnl.doe.gov
RI Fox, Elise/G-5438-2013
OI Fox, Elise/0000-0002-4527-5820
FU DOE-EERE Solar Energy Technology Program; Savannah River Nuclear
Solutions [DE-AC0908SR22470]; The Savannah River National Laboratory
FX The authors thank Ann E. Visser and Nicholas J. Bridges for helpful
discussions, insight, and IL structure drawings. The authors also thank
Erich Hansen for the use of his rheometer and his assistance. The
DOE-EERE Solar Energy Technology Program and the SunShot Initiative are
gratefully acknowledged for funding of this work. The Savannah River
National Laboratory is managed by Savannah River Nuclear Solutions. This
work was prepared under Federal Contract DE-AC0908SR22470.
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD NOV
PY 2013
VL 27
IS 11
BP 6355
EP 6361
DI 10.1021/ef401148j
PG 7
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 259WU
UT WOS:000327557800004
ER
PT J
AU Surasani, VK
Li, L
Ajo-Franklin, JB
Hubbard, C
Hubbard, SS
Wu, YX
AF Surasani, Vikranth K.
Li, Li
Ajo-Franklin, Jonathan B.
Hubbard, Chris
Hubbard, Susan S.
Wu, Yuxin
TI Bioclogging and Permeability Alteration by L-mesenteroides in a
Sandstone Reservoir: A Reactive Transport Modeling Study
SO ENERGY & FUELS
LA English
DT Article
ID SATURATED POROUS-MEDIA; BIOMASS PLUG DEVELOPMENT;
LEUCONOSTOC-MESENTEROIDES; MICROBIAL-GROWTH; HYDRAULIC CONDUCTIVITY;
PHYSICAL-PROPERTIES; BIOFILM GROWTH; OIL-RECOVERY; HYDROTHERMAL SYSTEMS;
SPATIAL-DISTRIBUTION
AB Selective bioclogging targets the biofilm growth in highly permeable zones of reservoirs or aquifers to divert water into low permeability zones. It alters the hydrodynamics of the subsurface flow systems to favorable performance conditions. Applications may include microbial-enhanced-hydrocarbon-recovery (MEHR) and bioremediation. Despite its success at the laboratory scale, application of bioclogging at the reservoir scale is hindered by the lack of understanding and advanced modeling and prediction tools. To understand controls of bioclogging processes at the reservoir scale, a Reactive Transport Model (RTM) has been developed in this work for in situ biostimulation of L. mesenteroides. This fermenting bacterium produces the biopolymer dextran in the presence of sucrose. As a first step, we considered the flow, transport, and bacterial growth and dextran production reactions in a single phase fluid (water) system, because most reactions occur either in the water phase or at the water-solid interface. Parameters for biomass growth and dextran production were obtained from column experimental data. The numerical experiments were carried out using the spatial distribution of porosity and permeability extracted from open-hole well logs collected at a characterization well near the King Island gas field in Southern Sacramento basin in California. The numerical experiments suggest that there exists an optimum range of injection rates (between 543 and 1,195 bbls/day). The volumetric injection rates need to be sufficiently fast to overcome microbial growth and clogging at the vicinity of the bore wells. They also need to be low enough to allow sufficiently long residence times for dextran production. Results show significant dextran formation and the associated porosity and permeability alterations to divert water into low permeability zones. The bioclogging effectiveness, measured by the percentage of the water diverted into the low permeability zones, varied between 10 to 75% depending on injection conditions. With the same total mass injection rates of sucrose, increasing flow rate is more effective in selectively bioclogging highly permeable zones than increasing sucrose concentration. Other processes, including the attachment of biomass to the solid surface without being washed out, are also important. The developed model offers a powerful tool to optimize injection conditions for effective bioclogging in naturally heterogeneous reservoirs.
C1 [Surasani, Vikranth K.; Li, Li] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA USA.
[Surasani, Vikranth K.] Birla Inst Sci & Technol, Dept Chem Engn, Hyderabad, Andhra Pradesh, India.
[Ajo-Franklin, Jonathan B.; Hubbard, Chris; Hubbard, Susan S.; Wu, Yuxin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Li, L (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA USA.
EM lili@eme.psu.edu
RI Hubbard, Christopher/J-6150-2014; Ajo-Franklin, Jonathan/G-7169-2015;
Hubbard, Susan/E-9508-2010; Wu, Yuxin/G-1630-2012; Li, Li/A-6077-2008;
OI Hubbard, Christopher/0000-0002-8217-8122; Wu, Yuxin/0000-0002-6953-0179;
Li, Li/0000-0002-1641-3710; Ajo-Franklin, Jonathan/0000-0002-6666-4702
FU Assistant Secretary for Fossil Energy; Office of Coal and Power Systems
through the National Energy Technology Laboratory; U.S. Department of
Energy [AC0205CH11231]
FX The project support from Energy Bioscience Institute (EBI), University
of California, Berkeley and the financial support from British Petroleum
are gratefully acknowledged. We would also like to thank John H. Beyer
and the WESTCARB partnership for allowing use of the Citizen Green #1
well logs for development of our synthetic reservoir model. WESTCARB
acquisition of the well logs was supported by the Assistant Secretary
for Fossil Energy, Office of Coal and Power Systems through the National
Energy Technology Laboratory, of the U.S. Department of Energy, under
contract number DE AC0205CH11231.
NR 70
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD NOV
PY 2013
VL 27
IS 11
BP 6538
EP 6551
DI 10.1021/ef401446f
PG 14
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 259WU
UT WOS:000327557800022
ER
PT J
AU Hammache, S
Hoffman, JS
Gray, ML
Fauth, DJ
Howard, BH
Pennline, HW
AF Hammache, Sonia
Hoffman, James S.
Gray, McMahan L.
Fauth, Daniel J.
Howard, Bret H.
Pennline, Henry W.
TI Comprehensive Study of the Impact of Steam on Polyethyleneimine on
Silica for CO2 Capture
SO ENERGY & FUELS
LA English
DT Article
ID CARBON-DIOXIDE CAPTURE; MESOPOROUS MOLECULAR-SIEVE; SOLID SORBENTS;
HIGH-CAPACITY; AMINE; ADSORPTION; ADSORBENT; PERFORMANCE; REMOVAL
AB An amine sorbent, prepared by impregnation of polyethyleneimine on silica, was tested for steam stability. The stability of the sorbent was investigated in a fixed bed reactor using multiple steam cycles of 90 vol % H2O/He at 105 degrees C, and the gas effluent was monitored with a mass spectrometer. CO2 uptake of sorbent was found to decrease with repeated exposure to steam. Characterization of the spent sorbent using N-2 physisorption, SEM, and thermogravimetric analysis (TGA) showed that the decrease in CO2 loading can possibly be attributed to a reagglomeration of the amine in the pores of the silica. No support effect was found in this study. The commercial SiO2 used, Cariact G10, was found to be stable under the conditions used. While it was found that subjecting the sorbent to several steam cycles decreased its CO2 uptake, a continuous exposure of the sorbent to steam did not have a significant performance impact. A silanated sorbent, consisting of a mixture of PEI and aminopropyltriethoxysilane on SiO2 support, was also investigated for steam stability. Similarly to the nonsilanated sorbent, the CO2 loading of this sorbent decreased upon steam exposure, although a mechanism for this change has not been postulated at this time.
C1 [Hammache, Sonia; Hoffman, James S.; Gray, McMahan L.; Fauth, Daniel J.; Howard, Bret H.; Pennline, Henry W.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
[Hammache, Sonia] URS Corp, South Pk, PA 15129 USA.
RP Hammache, S (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
EM Sonia.Hammache@contr.netl.doe.gov
FU National Energy Technology Laboratory's ongoing research under the RES
[DE-FE0004000]
FX This technical effort was performed in support of the National Energy
Technology Laboratory's ongoing research under the RES contract
DE-FE0004000. Reference in this work to any specific commercial product
is to facilitate understanding and does not necessarily imply
endorsement by the U.S. Department of Energy. S.H. would like to thank
Dr. Brian Kail for LCMS analysis.
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PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD NOV
PY 2013
VL 27
IS 11
BP 6899
EP 6905
DI 10.1021/ef401562w
PG 7
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 259WU
UT WOS:000327557800061
ER
PT J
AU Enick, RM
Koronaios, P
Stevenson, C
Warman, S
Morsi, B
Nulwala, H
Luebke, D
AF Enick, R. M.
Koronaios, P.
Stevenson, C.
Warman, S.
Morsi, B.
Nulwala, H.
Luebke, D.
TI Hydrophobic Polymeric Solvents for the Selective Absorption of CO2 from
Warm Gas Streams that also Contain H-2 and H2O
SO ENERGY & FUELS
LA English
DT Article
ID CARBON-DIOXIDE; SOLUBILITY; HYDROGEN; TEMPERATURES; PRESSURES; OIL
AB The hydrophobic polymers polydimethyl siloxane (PDMS) and polypropyleneglycol dimethylether (PPGDME) may provide an alternative to physical solvents based on the hydrophilic polymer polyethyleneglycol dimethylether (PEGDME) for the precombustion capture of CO2 from the warm, high pressure stream that also contains H2O and H-2. PPGDME can be made with a linear repeat unit (PPGDME(1), poly(1,3-propanediol) dimethylether) or a branched repeat unit (PPGDME(b), poly(1,2-propanediol) dimethylether). The solubility of CO2 and H-2 in each of the four solvents of specified average molecular weight (PEGDME 250, PDMS 550, PPGDME(1) 678 and PPGDME(b) 430) is determined between 25 and 120 degrees C at pressures to 10 MPa. CO2 is much more soluble in each solvent than H-2; however, the solubility of CO2 decreases as the solubility of H-2 increases with increasing temperature. PPGDME(1) 678 and PPGDME(b) 430 are comparable CO2 solvents. PPGDME(1) 678 absorbs less H-2 than all the other solvents, while PPGDME(b) 430 absorbs significantly more H-2. PDMS 550 is a very good CO2 solvent, absorbing more CO2 than all of the other solvents at all temperatures except for PEGDME 250 at 25 degrees C. PDMS 550 absorbs more H-2 than all of the other solvents.
C1 [Enick, R. M.; Morsi, B.; Nulwala, H.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.
[Enick, R. M.; Koronaios, P.; Stevenson, C.; Warman, S.] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA.
[Nulwala, H.] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA.
[Luebke, D.] US DOE NETL, Pittsburgh, PA 15236 USA.
RP Enick, RM (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd POB 10940, Pittsburgh, PA 15236 USA.
EM rme@pitt.edu
OI Nulwala, Hunaid/0000-0001-7481-3723
FU RES [DE-FE0004000]
FX As part of the National Energy Technology Laboratory's Regional
University Alliance (NETL-RUA), a collaboration initiative of the NETL,
this technical effort was performed under the RES contract DE-FE0004000.
NR 22
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0887-0624
EI 1520-5029
J9 ENERG FUEL
JI Energy Fuels
PD NOV
PY 2013
VL 27
IS 11
BP 6913
EP 6920
DI 10.1021/ef401740w
PG 8
WC Energy & Fuels; Engineering, Chemical
SC Energy & Fuels; Engineering
GA 259WU
UT WOS:000327557800063
ER
PT J
AU Teeguarden, JG
Fisher, JW
Doerge, DR
AF Teeguarden, Justin G.
Fisher, Jeffrey W.
Doerge, Daniel R.
TI Exposure Conditions and Pharmacokinetic Principles: Interpreting
Bisphenol A Absorption in the Canine Oral Cavity
SO ENVIRONMENTAL HEALTH PERSPECTIVES
LA English
DT Letter
C1 [Teeguarden, Justin G.] Pacific NW Natl Lab, Richland, WA 99352 USA.
[Fisher, Jeffrey W.; Doerge, Daniel R.] US FDA, Natl Ctr Toxicol Res, Jefferson, AR 72079 USA.
RP Teeguarden, JG (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM jt@pnl.gov
NR 7
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U1 0
U2 8
PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE
PI RES TRIANGLE PK
PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233,
RES TRIANGLE PK, NC 27709-2233 USA
SN 0091-6765
EI 1552-9924
J9 ENVIRON HEALTH PERSP
JI Environ. Health Perspect.
PD NOV-DEC
PY 2013
VL 121
IS 11-12
BP A323
EP A323
DI 10.1289/ehp.1307424
PG 1
WC Environmental Sciences; Public, Environmental & Occupational Health;
Toxicology
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Toxicology
GA 266ZA
UT WOS:000328061900003
PM 24284408
ER
PT J
AU Vesterinen, HM
Johnson, PI
Koustas, E
Lam, J
Sutton, P
Woodruff, TJ
AF Vesterinen, Hanna M.
Johnson, Paula I.
Koustas, Erica
Lam, Juleen
Sutton, Patrice
Woodruff, Tracey J.
TI In Support of EHP's Proposal to Adopt the ARRIVE Guidelines
SO ENVIRONMENTAL HEALTH PERSPECTIVES
LA English
DT Letter
ID SYSTEMATIC REVIEWS; QUALITY
C1 [Vesterinen, Hanna M.; Johnson, Paula I.; Sutton, Patrice; Woodruff, Tracey J.] Univ Calif San Francisco, Program Reprod Hlth & Environm, Oakland, CA USA.
[Koustas, Erica] Oak Ridge Inst Sci & Educ, Washington, DC USA.
[Lam, Juleen] Johns Hopkins Bloomberg Sch Publ Hlth, Dept Hlth Policy & Management, Baltimore, MD USA.
RP Vesterinen, HM (reprint author), Univ Calif San Francisco, Program Reprod Hlth & Environm, Oakland, CA USA.
EM VesterinenH@obgyn.ucsf.edu
FU NIEHS NIH HHS [P01 ES022841]
NR 15
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U1 0
U2 4
PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE
PI RES TRIANGLE PK
PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233,
RES TRIANGLE PK, NC 27709-2233 USA
SN 0091-6765
EI 1552-9924
J9 ENVIRON HEALTH PERSP
JI Environ. Health Perspect.
PD NOV-DEC
PY 2013
VL 121
IS 11-12
BP A325
EP A325
DI 10.1289/ehp.1307775
PG 1
WC Environmental Sciences; Public, Environmental & Occupational Health;
Toxicology
SC Environmental Sciences & Ecology; Public, Environmental & Occupational
Health; Toxicology
GA 266ZA
UT WOS:000328061900005
PM 24284027
ER
PT J
AU Kolemen, E
Ellis, R
La Haye, RJ
Humphreys, DA
Lohr, J
Noraky, S
Penaflor, BG
Welander, AS
AF Kolemen, E.
Ellis, R.
La Haye, R. J.
Humphreys, D. A.
Lohr, J.
Noraky, S.
Penaflor, B. G.
Welander, A. S.
TI Real-time mirror steering for improved closed loop neoclassical tearing
mode suppression by electron cyclotron current drive in DIII-D
SO FUSION ENGINEERING AND DESIGN
LA English
DT Article
DE NTM; Control; ECCD; DIII-D; Mirror; Steer
ID SYSTEM
AB The development and operation of the neoclassical tearing mode (NTM) avoidance and control system for DIII-D, which uses six sets of real-time steerable mirrors in order to move the electron cyclotron current drive (ECCD) deposition location in plasma, is described. The real-time DIII-D NTM control algorithm residing in the Plasma Control System (PCS) automatically detects an NTM by analysis of the Mirnov diagnostics, employs motional Stark effect (MSE) EFIT MHD equilibrium reconstruction to locate the rational q-surface where the NTM island can be found, then calculates the appropriate mirror position for alignment of the ECCD with the island using ray tracing. The control commands from PCS are sent to the electron cyclotron system to switch on and off or modulate the gyrotrons and to the steerable mirror system to move the steerable mirrors to the requested positions. Successful NTM suppression has been achieved in DIII-D using this control system to rapidly align the NTM island and the ECCD deposition location, and to actively maintain the alignment as plasma conditions change. (C) 2013 Published by Elsevier B.V.
C1 [Kolemen, E.; Ellis, R.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[La Haye, R. J.; Humphreys, D. A.; Lohr, J.; Noraky, S.; Penaflor, B. G.; Welander, A. S.] Gen Atom Co, San Diego, CA 92186 USA.
RP Kolemen, E (reprint author), Princeton Plasma Phys Lab, POB 45, Princeton, NJ 08543 USA.
EM ekolemen@pppl.gov
FU US Department of Energy [DE-AC02-09CH11466, DE-FC02-04ER54698]
FX This work was supported by the US Department of Energy under
DE-AC02-09CH11466 and DE-FC02-04ER54698.
NR 11
TC 7
Z9 7
U1 0
U2 8
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0920-3796
EI 1873-7196
J9 FUSION ENG DES
JI Fusion Eng. Des.
PD NOV
PY 2013
VL 88
IS 11
BP 2757
EP 2760
DI 10.1016/j.fusengdes.2013.02.168
PG 4
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 264VV
UT WOS:000327910000002
ER
PT J
AU Liu, HB
Abdou, MA
Greenwood, LR
AF Liu, Haibo
Abdou, Mohamed A.
Greenwood, Larry R.
TI Fe-55 effect on enhancing ferritic steel He/dpa ratio in fission reactor
irradiations to simulate fusion conditions
SO FUSION ENGINEERING AND DESIGN
LA English
DT Article
DE Fe-55 (n, a) cross section; He(appm)/dpa ratio; Isotopic tailoring;
Fusion material irradiation; Ferritic steel irradiation
ID HELIUM
AB This study evaluated methods for increasing the helium production rate in ferritic steel irradiation in a fission reactor neutron spectrum in order to increase the helium to atomic displacement ratio to values typical of fusion reactor first wall conditions. An early experiment showed that the accelerated He(appm)/dpa ratio of about 2.3 was achieved for 96% enriched Fe-54 in iron in the High Flux Isotope Reactor (HFIR), ORNL. In the current work, the ferritic steel He(appm)/dpa ratio was studied in the neutron spectrum of HFIR with the Fe-55 thermal neutron helium production taken into account. A benchmark calculation for the same sample, as used in the aforementioned experiment, was then used to adjust and evaluate the Fe-55 (n, a) cross section values in TALYS-based Evaluated Nuclear Data Library (TENDL). The analysis showed that a decrease of a factor of 6700 for the TENDL Fe-55 (n, a) cross section in the intermediate and low energy regions was required in order to fit the experimental results. The best fit to the cross section value at thermal neutron energy was about 27 mb. With the adjusted Fe-55 (n, a) cross sections, calculation showed that the Fe-54 and Fe-55 isotopes could be enriched by the isotopic tailoring technique in a ferritic steel sample irradiated in HFIR to significantly enhance the helium production rate. This new calculation can be used to guide future isotopic tailoring experiments designed to increase the He(appm)/dpa ratio in fission reactors. A benchmark experiment is suggested to be performed to evaluate the Fe-55 (n, a) cross section at thermal energy. Published by Elsevier B.V.
C1 [Liu, Haibo; Abdou, Mohamed A.] Univ Calif Los Angeles, Mech & Aerosp Engn Dept, Los Angeles, CA 90095 USA.
[Greenwood, Larry R.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Abdou, MA (reprint author), Univ Calif Los Angeles, Mech & Aerosp Engn Dept, Los Angeles, CA 90095 USA.
EM abdou@fusion.ucla.edu
RI Greenwood, Lawrence/H-9539-2016
OI Greenwood, Lawrence/0000-0001-6563-0650
FU US Department of Energy
FX Work supported by the US Department of Energy.
NR 19
TC 0
Z9 0
U1 1
U2 10
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0920-3796
EI 1873-7196
J9 FUSION ENG DES
JI Fusion Eng. Des.
PD NOV
PY 2013
VL 88
IS 11
BP 2860
EP 2864
DI 10.1016/j.fusengdes.2013.05.067
PG 5
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 264VV
UT WOS:000327910000018
ER
PT J
AU Youssef, M
Feder, R
Batistoni, P
Fischer, U
Jakhar, S
Konno, C
Loughlin, M
Villari, R
Wu, YC
AF Youssef, Mahmoud
Feder, Russell
Batistoni, Paola
Fischer, Ulrich
Jakhar, Shrichand
Konno, Chikara
Loughlin, Michael
Villari, Rosaria
Wu, Yican
TI Benchmarking of the 3-D CAD-based Discrete Ordinates code "ATTILA" for
dose rate calculations against experiments and Monte Carlo calculations
SO FUSION ENGINEERING AND DESIGN
LA English
DT Article
DE ATTILA 3-D Discrete Ordinates; ITER diagnostics ports; Shutdown dose
rates; 14-MeV integral experiments; Calculation benchmarking; FNG
facility
ID NEUTRONICS ANALYSIS; FUSION TECHNOLOGY; ITER; DIAGNOSTICS; PLUG;
VERIFICATION; VALIDATION; SHUT; JET
AB Shutdown dose rate (SDDR) inside and around the diagnostics ports of ITER is performed at PPPL/UCLA using the 3-D, FEM, Discrete Ordinates code, ATTILA, along with its updated FORNAX transmutation/decay gamma library. Other ITER partners assess SDDR using codes based on the Monte Carlo (MC) approach (e.g. MCNP code) for transport calculation and the radioactivity inventory code FISPACT or other equivalent decay data libraries for dose rate assessment. To reveal the range of discrepancies in the results obtained by various analysts, an extensive experimental and calculation benchmarking effort has been undertaken to validate the capability of ATTILA for dose rate assessment. On the experimental validation front, the comparison was performed using the measured data from two SDDR experiments performed at the FNG facility, Italy. Comparison was made to the experimental data and to MC results obtained by other analysts. On the calculation validation front, the ATTILA's predictions were compared to other results at key locations inside a calculation benchmark whose configuration duplicates an upper diagnostics port plug (UPP) in ITER. Both serial and parallel version of ATTILA-7.1.0 are used in the PPPL/UCLA analysis performed with FENDL-2.1/FORNAX databases. In the FNG 1st experimental, it was shown that ATTILA's dose rates are largely over estimated (by similar to 30-60%) with the ANSI/ANS-6.1.1 flux-to-dose factors whereas the ICRP-74 factors give better agreement (10-20%) with the experimental data and with the MC results at all cooling times. In the 2nd experiment, there is an under estimation in SDDR calculated by both MCNP and ATTILA based on ANSI/ANS-6.1.1 for cooling times up to similar to 4 days after irradiation. Thereafter, an over estimation is observed (similar to 5-10% with MCNP and similar to 10-15% with ATTILA). As for the calculation benchmark, the agreement is much better based on ICRP-74 1996 data. The divergence among all dose rate results at similar to 11 days cooling time is no more than 15% among all participants. Published by Elsevier B.V.
C1 [Youssef, Mahmoud] Univ Calif Los Angeles, Los Angeles, CA 90095 USA.
[Feder, Russell] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA.
[Batistoni, Paola] Culham Sci Ctr, EFDA JET, Abingdon, Oxon, England.
[Fischer, Ulrich] KIT, Karlsruhe, Germany.
[Jakhar, Shrichand] Inst Plasma Res, Bhat, Gandhinagar, India.
[Konno, Chikara] JAEA, Fus Neutron Grp, Div Fus Energy Technol, Tokai, Ibaraki, Japan.
[Loughlin, Michael] ITER Org, Project Engn & Integrat Div, St Paul Les Durance, France.
[Villari, Rosaria] ENEA Fus Tech Unit, I-00044 Frascati, Rome, Italy.
[Wu, Yican] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China.
RP Youssef, M (reprint author), Univ Calif Los Angeles, Los Angeles, CA 90095 USA.
EM youssef@fusion.ucla.edu; rfeder@pppl.gov
OI Jakhar, S./0000-0002-9656-5051
FU Princeton Plasma Physics Laboratory through US ITER Project [S006987-R];
Princeton Plasma Physics Laboratory through USITER [15300-PD0002-R00];
United States Department of Energy through PPPL Prime
[DE-AC02-09CH11466]
FX This work is funded by the Princeton Plasma Physics Laboratory under
contract # S006987-R through US ITER Project and USITER
15300-PD0002-R00. The work performed in support of this report was made
possible by the United States Department of Energy through PPPL Prime
Contract Number DE-AC02-09CH11466. All US ITER activities are managed by
the US ITER Project Office, hosted by Oak Ridge National Laboratory with
partner labs Princeton Plasma Physics Laboratory and Savannah River
National Laboratory. The project is being accomplished through a
collaboration of DOE Laboratories, Universities and industry.
NR 31
TC 3
Z9 3
U1 3
U2 14
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0920-3796
EI 1873-7196
J9 FUSION ENG DES
JI Fusion Eng. Des.
PD NOV
PY 2013
VL 88
IS 11
BP 3033
EP 3040
DI 10.1016/j.fusengdes.2013.07.010
PG 8
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 264VV
UT WOS:000327910000044
ER
PT J
AU Weng, QH
Zhou, YY
Quattrochi, DA
AF Weng, Qihao
Zhou, Yuyu
Quattrochi, Dale A.
TI Geographical applications of remote sensing
SO GEOCARTO INTERNATIONAL
LA English
DT Editorial Material
C1 [Weng, Qihao] Indiana State Univ, Ctr Urban & Environm Change, Dept Earth & Environm Syst, Terre Haute, IN 47809 USA.
[Zhou, Yuyu] Pacific NW Natl Lab, Joint Global Change Res Inst, Richland, WA 99352 USA.
[Quattrochi, Dale A.] NASA, Dept Earth Sci, George C Marshall Space Flight Ctr, Washington, DC 20546 USA.
RP Weng, QH (reprint author), Indiana State Univ, Ctr Urban & Environm Change, Dept Earth & Environm Syst, Terre Haute, IN 47809 USA.
EM qweng@indstate.edu; yuyu.zhou@pnnl.gov; dale.quattrochi@nasa.gov
OI Weng, Qihao/0000-0002-2498-0934
NR 0
TC 1
Z9 1
U1 0
U2 4
PU TAYLOR & FRANCIS LTD
PI ABINGDON
PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
SN 1010-6049
EI 1752-0762
J9 GEOCARTO INT
JI Geocarto Int.
PD NOV 1
PY 2013
VL 28
IS 7
SI SI
BP 561
EP 561
DI 10.1080/10106049.2013.856202
PG 1
WC Environmental Sciences; Geosciences, Multidisciplinary; Remote Sensing;
Imaging Science & Photographic Technology
SC Environmental Sciences & Ecology; Geology; Remote Sensing; Imaging
Science & Photographic Technology
GA 265CV
UT WOS:000327928200001
ER
PT J
AU Tomsia, AP
Lee, JS
Wegst, UGK
Saiz, E
AF Tomsia, Antoni P.
Lee, Janice S.
Wegst, Ulrike G. K.
Saiz, Eduardo
TI Nanotechnology for Dental Implants
SO INTERNATIONAL JOURNAL OF ORAL & MAXILLOFACIAL IMPLANTS
LA English
DT Article
DE bone formation; coatings; dental implants; hydroxyapatite;
nanotechnology; surface topography
ID BIOACTIVE GLASS COATINGS; PLASMA-SPRAYED COATINGS; TOTAL
HIP-ARTHROPLASTY; POROUS COATED IMPLANTS; OSTEOBLAST-LIKE CELLS;
METAL-ION RELEASE; TI-BASED IMPLANTS; IN-VITRO; ELECTROPHORETIC
DEPOSITION; MECHANICAL-PROPERTIES
AB With the advent of nanotechnology, an opportunity exists for the engineering of new dental implant materials. Metallic dental implants have been successfully used for decades, but they have shortcomings related to osseointegration and mechanical properties that do not match those of bone. Absent the development of an entirely new class of materials, faster osseointegration of currently available dental implants can be accomplished by various surface modifications. To date, there is no consensus regarding the preferred method(s) of implant surface modification, and further development will be required before the ideal implant surface can be created, let alone become available for clinical use. Current approaches can generally be categorized into three areas: ceramic coatings, surface functionalization, and patterning on the micro-to nanoscale. The distinctions among these are imprecise, as some or all of these approaches can be combined to improve in vivo implant performance. These surface improvements have resulted in durable implants with a high percentage of success and long-term function. Nanotechnology has provided another set of opportunities for the manipulation of implant surfaces in its capacity to mimic the surface topography formed by extracellular matrix components of natural tissue. The possibilities introduced by nanotechnology now permit the tailoring of implant chemistry and structure with an unprecedented degree of control. For the first time, tools are available that can be used to manipulate the physicochemical environment and monitor key cellular events at the molecular level. These new tools and capabilities will result in faster bone formation, reduced healing time, and rapid recovery to function.
C1 [Tomsia, Antoni P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Lee, Janice S.] Univ Calif San Francisco, Dept Oral & Maxillofacial Surg, San Francisco, CA USA.
[Wegst, Ulrike G. K.] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA.
[Saiz, Eduardo] Univ London Imperial Coll Sci Technol & Med, Ctr Adv Struct Ceram, Dept Mat, London SW7 2AZ, England.
RP Tomsia, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM aptomsia@lbl.gov
FU NIH National Institute of Dental and Craniofacial Research [5R01
DE015633]
FX This work was supported by the NIH National Institute of Dental and
Craniofacial Research under grant 5R01 DE015633 ("Complex nanocomposites
for bone regeneration"). The authors wish to thank Dr Alessandro Polini
for reading the manuscript and useful discussions.
NR 109
TC 11
Z9 11
U1 5
U2 25
PU QUINTESSENCE PUBLISHING CO INC
PI HANOVER PARK
PA 4350 CHANDLER DRIVE, HANOVER PARK, IL 60133 USA
SN 0882-2786
EI 1942-4434
J9 INT J ORAL MAX IMPL
JI Int. J. Oral Maxillofac. Implants
PD NOV-DEC
PY 2013
VL 28
IS 6
BP E535
EP E546
PG 12
WC Dentistry, Oral Surgery & Medicine
SC Dentistry, Oral Surgery & Medicine
GA 267VH
UT WOS:000328125900023
PM 24278949
ER
PT J
AU Zhong, DK
Zhao, SL
Polyansky, DE
Fujita, E
AF Zhong, Diane K.
Zhao, Shengliang
Polyansky, Dmitry E.
Fujita, Etsuko
TI Diminished photoisomerization of active ruthenium water oxidation
catalyst by anchoring to metal oxide electrodes
SO JOURNAL OF CATALYSIS
LA English
DT Article
DE Ruthenium catalyst; Water oxidation; Surface-binding; Photoisomerization
ID ARTIFICIAL PHOTOSYNTHESIS; POLYPYRIDYL COMPLEXES; REDOX PROPERTIES; RU
COMPLEXES; SINGLE-SITE; PHOSPHONATE; SURFACES; OXYGEN; PHOTOANODES;
HYDROGEN
AB Surface-binding of molecular water oxidation catalysts through phosphonated ligands offers a promising strategy for attaching homogeneous catalysts onto conductive or semiconductive oxide surfaces for heterogeneous catalysis. In this work, the highly active [Ru(tpy)(pynap)OH2](2+) (tpy = 2,2':6',2 ''-terpyridine; pynap = 2-(pyrid-2'-yl)-1,8-naphthyridine) water oxidation catalyst is attached onto metal oxide electrodes through a phosphate group. Electrochemical and photoelectrochemical results confirm that ruthenium oxidation chemistries and water oxidation proficiency remain largely unaffected by phosphonation. Surface-binding reveals minimal photoisomerization of the active d-form and allows us to evaluate photoelectrochemical and mechanistic properties of the catalyst. Spectroelectrochemical experiments support the evolution of multiple ruthenium oxidation states in agreement with Pourbaix diagrams. Although photoisomerization of d-[Ru(H2PO3-tpy)(pynap)OH2](2+) is considerably hindered when the catalyst is attached onto a rigid oxide electrode, surface desorption remains a major challenge. (C) 2013 Elsevier Inc. All rights reserved.
C1 [Zhong, Diane K.; Zhao, Shengliang; Polyansky, Dmitry E.; Fujita, Etsuko] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
RP Fujita, E (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM Fujita@bnl.gov
RI Polyansky, Dmitry/C-1993-2009
OI Polyansky, Dmitry/0000-0002-0824-2296
FU Brookhaven National Laboratory (BNL) [DE-AC02-98CH10886]; U.S.
Department of Energy; Division of Chemical Sciences, Geosciences, &
Biosciences, Office of Basic Energy Sciences; U.S. Department of Energy,
Office of Basic Energy Sciences
FX This work is carried out at Brookhaven National Laboratory (BNL) under
Contract DE-AC02-98CH10886 with the U.S. Department of Energy and
supported by its Division of Chemical Sciences, Geosciences, &
Biosciences, Office of Basic Energy Sciences. Part of the research is
carried out at the Center for Functional Nanomaterials (CFN) at BNL,
which is supported by the U.S. Department of Energy, Office of Basic
Energy Sciences. The authors thank Dr. Mingzhao Liu and Dr. Chang-Yong
Nam for their assistance with instrumentation at the CFN, Dr. Jonathan
F. Hull for providing us with nanoITO films and helpful advice on
spectroelectrochemistry, and Prof. Randolph Thummel and Dr. Ruifa Zong
for providing us with the pynap ligand.
NR 39
TC 15
Z9 15
U1 1
U2 34
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0021-9517
EI 1090-2694
J9 J CATAL
JI J. Catal.
PD NOV
PY 2013
VL 307
BP 140
EP 147
DI 10.1016/j.jcat.2013.07.018
PG 8
WC Chemistry, Physical; Engineering, Chemical
SC Chemistry; Engineering
GA 264TM
UT WOS:000327903900016
ER
PT J
AU Rodriguez, JA
Evans, J
Feria, L
Vidal, AB
Liu, P
Nakamura, K
Illas, F
AF Rodriguez, Jose A.
Evans, Jaime
Feria, Leticia
Vidal, Alba B.
Liu, Ping
Nakamura, Kenichi
Illas, Francesc
TI CO2 hydrogenation on Au/TiC, Cu/TiC, and Ni/TiC catalysts: Production of
CO, methanol, and methane
SO JOURNAL OF CATALYSIS
LA English
DT Article
DE CO2 activation; CO production; Methane synthesis; Metal carbides; Noble
metals
ID TRANSITION-METAL CARBIDES; DENSITY-FUNCTIONAL THEORY; AUGMENTED-WAVE
METHOD; GAS SHIFT KINETICS; CARBON-DIOXIDE; CHARGE POLARIZATION; CU
SURFACES; AU; NI(110); CU(110)
AB Small Au, Cu, and Ni particles in contact with TiC(001) display a very high activity for the catalytic hydrogenation of CO2. The major product over these catalysts is CO which is produced by the reverse water gas shift reaction (RWGS, CO2 + H-2 -> CO + H2O). In the cases of Au/TiC(001) and Cu/TiC(001), a substantial amount of methanol is also produced, but no methane is detected. Ni/TiC(001) produces a mixture of CO, methanol, and methane. The highest catalytic activity is found for small two-dimensional particles or clusters of the admetals in close contact with TiC(001). The catalytic activity of the supported metals can be orders of magnitude higher than those-of Au(100), Cu(100), or Ni(100). Density functional calculations point to HOCO as a key intermediate for the generation of CO through the RWGS, with the production of methanol probably involving the hydrogenation of a HCOO intermediate or the CO generated by the RWGS. (C) 2013 Elsevier Inc. All rights reserved.
C1 [Rodriguez, Jose A.; Vidal, Alba B.; Liu, Ping] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
[Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela.
[Feria, Leticia; Illas, Francesc] Univ Barcelona, Dept Quim Fis, E-08028 Barcelona, Spain.
[Feria, Leticia; Illas, Francesc] Univ Barcelona, Inst Quim Teor & Computac IQTCUB, E-08028 Barcelona, Spain.
[Vidal, Alba B.] IVIC, Ctr Quim, Caracas 1020A, Venezuela.
[Nakamura, Kenichi] Tokyo Inst Technol, Mat & Struct Lab, Yokohama, Kanagawa 2268503, Japan.
RP Rodriguez, JA (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
EM rodrigez@bnl.gov
RI Illas, Francesc /C-8578-2011
OI Illas, Francesc /0000-0003-2104-6123
FU US Department of Energy, Chemical Sciences Division [DE-AC02-98CH10886];
INTEVEP; IDB; Nippon Foundation for Materials Science; Spanish
MICINN/MINECO research grants [FIS2008-02238, CTQ2010-14872/BQU,
CTQ2012-30751]; Generalitat de Catalunya grants [2009SGR1041]; XRQTC;
ICREA Academia Award for excellence
FX The research carried out at BNL was supported by the US Department of
Energy, Chemical Sciences Division (DE-AC02-98CH10886). J.E. is grateful
to INTEVEP and IDB for support of the work carried out at the UCV. K.N.
is grateful to the Nippon Foundation for Materials Science for grants
that made possible part of this work. The research at UB was supported
support by Spanish MICINN/MINECO research grants FIS2008-02238,
CTQ2010-14872/BQU and CTQ2012-30751 and, in part, by Generalitat de
Catalunya grants 2009SGR1041 and XRQTC. FI acknowledges additional
support through the 2009 ICREA Academia Award for excellence in
research. Computational time on the Center for Functional Nanomaterials
at BNL and the Marenostrum supercomputer of the Barcelona Supercomputing
Center is gratefully acknowledged.
NR 58
TC 43
Z9 43
U1 19
U2 205
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0021-9517
EI 1090-2694
J9 J CATAL
JI J. Catal.
PD NOV
PY 2013
VL 307
BP 162
EP 169
DI 10.1016/j.jcat.2013.07.023
PG 8
WC Chemistry, Physical; Engineering, Chemical
SC Chemistry; Engineering
GA 264TM
UT WOS:000327903900019
ER
PT J
AU Saxena, A
Bhalla, AS
AF Saxena, A.
Bhalla, A. S.
TI Bioferroics and biomultiferroics: ferroic behaviour of biological
systems
SO MATERIALS RESEARCH INNOVATIONS
LA English
DT Article
DE Biomagnetism; Elastomechanics; Piezoelectric; Secondary ferroic;
Bioflexoelectric; Biosensory systems
ID BONE
AB The three primary ferroic properties, namely, ferromagnetism, ferroelectricity and ferroelasticity, have been observed in biological systems. The quest for the fourth primary ferroic, namely, ferrotoroidics, along with magnetoelectricity and multiferroic behaviour in biological systems is under way. Control of such bioferroic behaviour by small electric, magnetic and stress fields may lead to novel medical, therapeutic and diagnostic applications.
C1 [Saxena, A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Bhalla, A. S.] Univ Texas San Antonio, Dept Elect Engn, San Antonio, TX 78249 USA.
RP Saxena, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM avadh@lanl.gov
FU US Department of Energy National Science Foundation INAMM Program at
UTSA [0844081]
FX This work was supported in part by the US Department of Energy and in
part by the National Science Foundation INAMM Program at UTSA (grant no.
0844081).
NR 25
TC 1
Z9 1
U1 3
U2 39
PU MANEY PUBLISHING
PI LEEDS
PA STE 1C, JOSEPHS WELL, HANOVER WALK, LEEDS LS3 1AB, W YORKS, ENGLAND
SN 1432-8917
EI 1433-075X
J9 MATER RES INNOV
JI Mater. Res. Innov.
PD NOV
PY 2013
VL 17
IS 7
BP 440
EP 441
DI 10.1179/1433075X13Y.0000000177
PG 2
WC Materials Science, Multidisciplinary
SC Materials Science
GA 267CV
UT WOS:000328075200001
ER
PT J
AU Youngquist, JT
Schumacher, MH
Rose, JP
Raines, TC
Politz, MC
Copeland, MF
Pfleger, BF
AF Youngquist, J. Tyler
Schumacher, Martin H.
Rose, Joshua P.
Raines, Thomas C.
Politz, Mark C.
Copeland, Matthew F.
Pfleger, Brian F.
TI Production of medium chain length fatty alcohols in Escherichia coli
SO METABOLIC ENGINEERING
LA English
DT Article
DE Escherichia coli; Thioesterase; Acyl-CoA reductase; Fatty alcohol;
Dodecanol; Tetradecanol
ID ACYL-COA REDUCTASE; SYNTHETIC BIOLOGY; ACID PRODUCTION; EXPRESSION;
COENZYME; BIOSYNTHESIS; FUELS; MICROCOMPARTMENTS; OPTIMIZATION;
CONVERSION
AB Metabolic engineering offers the opportunity to produce a wide range of commodity chemicals that are currently derived from petroleum or other non-renewable resources. Microbial synthesis of fatty alcohols is an attractive process because it can control the distribution of chain lengths and utilize low cost fermentation substrates. Specifically, primary alcohols with chain lengths of 12 to 14 carbons have many uses in the production of detergents, surfactants, and personal care products. The current challenge is to produce these compounds at titers and yields that would make them economically competitive. Here, we demonstrate a metabolic engineering strategy for producing fatty alcohols from glucose. To produce a high level of 1-dodecanol and 1-tetradecanol, an acyl-ACP thioesterase (BTE), an acyl-CoA ligase (FadD), and an acyl-CoA/aldehyde reductase (MAACR) were overexpressecl in an engineered strain of Escherichia coli. Yields were improved by balancing expression levels of each gene, using a fed batch cultivation strategy, and adding a solvent to the culture for extracting the product from cells. Using these strategies, a Liter of over 1.6 g/L fatty alcohol with a yield of over 0.13 g fatty alcohol/g carbon source was achieved. These are the highest reported yield of fatty alcohols produced from glucose in E. coli. (C) 2013 Elsevier Inc. All tights reserved.
C1 [Youngquist, J. Tyler; Schumacher, Martin H.; Rose, Joshua P.; Raines, Thomas C.; Politz, Mark C.; Copeland, Matthew F.; Pfleger, Brian F.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA.
[Youngquist, J. Tyler; Pfleger, Brian F.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA.
RP Pfleger, BF (reprint author), 3629 Engn Hall,1415 Engn Dr, Madison, WI 53706 USA.
EM pfleger@engr.wisc.edu
FU DOE Great Lakes Bioenergy Research Center (GLBRC; DOE Office of Science
BER) [DE-FC02-07ER64494]; National Science Foundation [CBET-1149678];
National Institutes of Health [NHGRI HG002760, T32 GM08349]
FX This work was funded by the DOE Great Lakes Bioenergy Research Center
(GLBRC; DOE Office of Science BER DE-FC02-07ER64494) the National
Science Foundation (CBET-1149678) and the National Institutes of Health
(NHGRI HG002760 and T32 GM08349). The authors are grateful to Brett
Barney, Zachariah Harris, Mick McGee, and Daniel Mendez-Perez for their
contributions.
NR 47
TC 27
Z9 29
U1 5
U2 51
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 1096-7176
EI 1096-7184
J9 METAB ENG
JI Metab. Eng.
PD NOV
PY 2013
VL 20
BP 177
EP 186
DI 10.1016/j.ymben.2013.10.006
PG 10
WC Biotechnology & Applied Microbiology
SC Biotechnology & Applied Microbiology
GA 267ES
UT WOS:000328080100019
PM 24141053
ER
PT J
AU Hofmann, F
Abbey, B
Liu, WJ
Xu, RQ
Usher, BF
Balaur, E
Liu, YZ
AF Hofmann, Felix
Abbey, Brian
Liu, Wenjun
Xu, Ruqing
Usher, Brian F.
Balaur, Eugeniu
Liu, Yuzi
TI X-ray micro-beam characterization of lattice rotations and distortions
due to an individual dislocation
SO NATURE COMMUNICATIONS
LA English
DT Article
ID STRAIN FIELDS; LAUE MICRODIFFRACTION; EDGE DISLOCATION; WHITE-BEAM;
DIFFRACTION; DEFORMATION; RESOLUTION; GRADIENTS; DEFECTS; CRYSTAL
AB Understanding and controlling the behaviour of dislocations is crucial for a wide range of applications, from nano-electronics and solar cells to structural engineering alloys. Quantitative X-ray diffraction measurements of the strain fields due to individual dislocations, particularly in the bulk, however, have thus far remained elusive. Here we report the first characterization of a single dislocation in a freestanding GaAs/In0.2Ga0.8As/GaAs membrane by synchrotron X-ray micro-beam Laue diffraction. Our experimental X-ray data agrees closely with textbook anisotropic elasticity solutions for dislocations, providing one of few experimental validations of this fundamental theory. On the basis of the experimental uncertainty in our measurements, we predict the X-ray beam size required for three-dimensional measurements of lattice strains and rotations due to individual dislocations in the material bulk. These findings have important implications for the in situ study of dislocation structure formation, self-organization and evolution in the bulk.
C1 [Hofmann, Felix] Univ Oxford, Dept Engn Sci, Oxford OX1 3PJ, England.
[Abbey, Brian; Balaur, Eugeniu] La Trobe Univ, Dept Phys, ARC Ctr Excellence Coherent Xray Sci, Melbourne, Vic 3086, Australia.
[Abbey, Brian; Balaur, Eugeniu] Melbourne Ctr Nanofabricat, Melbourne, Vic 3168, Australia.
[Liu, Wenjun; Xu, Ruqing] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Usher, Brian F.] La Trobe Univ, Dept Elect Engn, Melbourne, Vic 3086, Australia.
[Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Hofmann, F (reprint author), Univ Oxford, Dept Engn Sci, Parks Rd, Oxford OX1 3PJ, England.
EM felix.hofmann@eng.ox.ac.uk
RI Abbey, Brian/D-3274-2011; Xu, Ruqing/K-3586-2012; Liu, Yuzi/C-6849-2011;
Balaur, Eugeniu/J-5865-2016
OI Abbey, Brian/0000-0001-6504-0503; Xu, Ruqing/0000-0003-1037-0059;
Balaur, Eugeniu/0000-0003-4029-2055
FU John Fell Oxford University Press (OUP) Research Fund; Australian
Research Council Centre of Excellence for Coherent X-ray Science;
Australian Synchrotron Research Program; U.S. DOE [DE-AC02-06CH11357];
U.S. Department of Energy, Office of Basic Energy Sciences
[DE-AC02-06CH11357]
FX F.H. acknowledges funding from the John Fell Oxford University Press
(OUP) Research Fund. B.A. acknowledges the support of the Australian
Research Council Centre of Excellence for Coherent X-ray Science and the
Australian Synchrotron Research Program. Use of the Advanced Photon
Source, an Office of Science User Facility operated for the U. S.
Department of Energy (DOE) Office of Science by Argonne National
Laboratory (ANL), was supported by the U.S. DOE under Contract No.
DE-AC02-06CH11357. Use of the Centre for Nanoscale Materials at ANL was
supported by the U.S. Department of Energy, Office of Basic Energy
Sciences, under Contract No. DE-AC02-06CH11357. The authors also
acknowledge the use of the facilities at the Melbourne Centre for
Nanofabrication.
NR 46
TC 6
Z9 6
U1 1
U2 39
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2774
DI 10.1038/ncomms3774
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266KY
UT WOS:000328023900012
PM 24216614
ER
PT J
AU Kim, K
Coh, S
Kisielowski, C
Crommie, MF
Louie, SG
Cohen, ML
Zettl, A
AF Kim, Kwanpyo
Coh, Sinisa
Kisielowski, C.
Crommie, M. F.
Louie, Steven G.
Cohen, Marvin L.
Zettl, A.
TI Atomically perfect torn graphene edges and their reversible
reconstruction
SO NATURE COMMUNICATIONS
LA English
DT Article
ID CARBON NANOTUBES; LAYER GRAPHENE; NANORIBBONS; NANOSTRUCTURES;
SPECTROSCOPY; STABILITY; DYNAMICS; ZIGZAG
AB The atomic structure of graphene edges is critical in determining the electrical, magnetic and chemical properties of truncated graphene structures, notably nanoribbons. Unfortunately, graphene edges are typically far from ideal and suffer from atomic-scale defects, structural distortion and unintended chemical functionalization, leading to unpredictable properties. Here we report that graphene edges fabricated by electron beam-initiated mechanical rupture or tearing in high vacuum are clean and largely atomically perfect, oriented in either the armchair or zigzag direction. We demonstrate, via aberration-corrected transmission electron microscopy, reversible and extended pentagon-heptagon (5-7) reconstruction at zigzag edges, and explore experimentally and theoretically the dynamics of the transitions between configuration states. Good theoretical-experimental agreement is found for the flipping rates between 5-7 and 6-6 zigzag edge states. Our study demonstrates that simple ripping is remarkably effective in producing atomically clean, ideal terminations, thus providing a valuable tool for realizing atomically tailored graphene and facilitating meaningful experimental study.
C1 [Kim, Kwanpyo; Coh, Sinisa; Crommie, M. F.; Louie, Steven G.; Cohen, Marvin L.; Zettl, A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Kim, Kwanpyo; Coh, Sinisa; Crommie, M. F.; Louie, Steven G.; Cohen, Marvin L.; Zettl, A.] Univ Calif Berkeley, Ctr Integrated Nanomech Syst, Berkeley, CA 94720 USA.
[Kim, Kwanpyo; Coh, Sinisa; Crommie, M. F.; Louie, Steven G.; Cohen, Marvin L.; Zettl, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Kisielowski, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA.
RP Zettl, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
EM azettl@berkeley.edu
RI Kim, Kwanpyo/D-9121-2011; Foundry, Molecular/G-9968-2014; Zettl,
Alex/O-4925-2016
OI Kim, Kwanpyo/0000-0001-8497-2330; Zettl, Alex/0000-0001-6330-136X
FU Office of Energy Research, Materials Sciences and Engineering Division,
of the US Department of Energy [DE-AC02-05CH11231]; Office of Naval
Research under MURI [N00014-09-1066]; National Science Foundation within
Center of Integrated Nanomechanical Systems [EEC-0832819]
FX This research was supported in part by the Director, Office of Energy
Research, Materials Sciences and Engineering Division, of the US
Department of Energy under Contract number DE-AC02-05CH11231, which
provided for TEM characterization, including that performed at the
National Center for Electron Microscopy, and theoretical modelling; by
the Office of Naval Research under MURI Grant N00014-09-1066, which
provided for graphene synthesis and suspension; and by the National
Science Foundation within the Center of Integrated Nanomechanical
Systems, under Grant EEC-0832819, which provided for additional sample
characterization and personnel support.
NR 38
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PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2723
DI 10.1038/ncomms3723
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266KD
UT WOS:000328021600004
PM 24177166
ER
PT J
AU Kiraly, B
Iski, EV
Mannix, AJ
Fisher, BL
Hersam, MC
Guisinger, NP
AF Kiraly, Brian
Iski, Erin V.
Mannix, Andrew J.
Fisher, Brandon L.
Hersam, Mark C.
Guisinger, Nathan P.
TI Solid-source growth and atomic-scale characterization of graphene on
Ag(111)
SO NATURE COMMUNICATIONS
LA English
DT Article
ID EPITAXIAL GRAPHENE; RAMAN-SPECTROSCOPY; GRAIN-BOUNDARIES; HIGH-QUALITY;
EDGE STATES; NANORIBBONS; SCATTERING; INTERFERENCE; DEFECTS
AB Silver is a desirable platform for graphene growth because of the potential for hybrid graphene plasmonics and its emerging role as a preferred growth substrate for other two-dimensional materials, such as silicene. Here we demonstrate the direct growth of monolayer graphene on a single-crystal Ag(111) substrate. The inert nature of Ag has made it difficult to use for graphene synthesis using standard chemical vapour deposition techniques, which we have overcome by using an elemental carbon source. Atomic-scale scanning tunnelling microscopy reveals that the atomically clean graphene-silver substrate is free of organic residue and other contaminants. The dendritic graphene possesses a variety of edge terminations, many of which give rise to quantum interferences previously seen only on insulating substrates. This scattering supports spectroscopic evidence that the graphene electronic structure is minimally perturbed by the underlying silver, providing a new system in which graphene is decoupled from its growth substrate.
C1 [Kiraly, Brian; Iski, Erin V.; Mannix, Andrew J.; Fisher, Brandon L.; Guisinger, Nathan P.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Kiraly, Brian; Mannix, Andrew J.; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.
[Hersam, Mark C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
RP Guisinger, NP (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave,Bldg 440, Argonne, IL 60439 USA.
EM nguisinger@anl.gov
RI Hersam, Mark/B-6739-2009
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]; National Science Foundation Graduate
Research Fellowship [DGE-0824162]; US Department of Energy SISGR
[DE-FG02-09ER16109]
FX We thank M. Koppen and C. Linsmeier for their help with the carbon
e-beam evaporation. Use of the Center for Nanoscale Materials was
supported by the U.S. Department of Energy, Office of Science, Office of
Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. B.K.
acknowledges support from a National Science Foundation Graduate
Research Fellowship (DGE-0824162). This work was also supported by the
US Department of Energy SISGR contract number DE-FG02-09ER16109.
NR 44
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Z9 39
U1 22
U2 176
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2804
DI 10.1038/ncomms3804
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LR
UT WOS:000328025800001
ER
PT J
AU Ma, T
Wang, JY
Zhou, GK
Yue, Z
Hu, QJ
Chen, Y
Liu, BB
Qiu, Q
Wang, Z
Zhang, J
Wang, K
Jiang, DC
Gou, CY
Yu, LL
Zhan, DL
Zhou, R
Luo, WC
Ma, H
Yang, YZ
Pan, SK
Fang, DM
Luo, YD
Wang, X
Wang, GN
Wang, J
Wang, Q
Lu, X
Chen, Z
Liu, JC
Lu, Y
Yin, Y
Yang, HM
Abbott, RJ
Wu, YX
Wan, DS
Li, J
Yin, TM
Lascoux, M
DiFazio, SP
Tuskan, GA
Wang, J
Liu, JQ
AF Ma, Tao
Wang, Junyi
Zhou, Gongke
Yue, Zhen
Hu, Quanjun
Chen, Yan
Liu, Bingbing
Qiu, Qiang
Wang, Zhuo
Zhang, Jian
Wang, Kun
Jiang, Dechun
Gou, Caiyun
Yu, Lili
Zhan, Dongliang
Zhou, Ran
Luo, Wenchun
Ma, Hui
Yang, Yongzhi
Pan, Shengkai
Fang, Dongming
Luo, Yadan
Wang, Xia
Wang, Gaini
Wang, Juan
Wang, Qian
Lu, Xu
Chen, Zhe
Liu, Jinchao
Lu, Yao
Yin, Ye
Yang, Huanming
Abbott, Richard J.
Wu, Yuxia
Wan, Dongshi
Li, Jia
Yin, Tongming
Lascoux, Martin
DiFazio, Stephen P.
Tuskan, Gerald A.
Wang, Jun
Liu Jianquan
TI Genomic insights into salt adaptation in a desert poplar
SO NATURE COMMUNICATIONS
LA English
DT Article
ID POPULUS-EUPHRATICA; RNA-SEQ; STRESS ACCLIMATION; GENE-EXPRESSION;
ARABIDOPSIS; TOLERANCE; TRANSPORT; DROUGHT; PLANTS; TRANSCRIPTOME
AB Despite the high economic and ecological importance of forests, our knowledge of the genomic evolution of trees under salt stress remains very limited. Here we report the genome sequence of the desert poplar, Populus euphratica, which exhibits high tolerance to salt stress. Its genome is very similar and collinear to that of the closely related mesophytic congener, P. trichocarpa. However, we find that several gene families likely to be involved in tolerance to salt stress contain significantly more gene copies within the P. euphratica lineage. Furthermore, genes showing evidence of positive selection are significantly enriched in functional categories related to salt stress. Some of these genes, and others within the same categories, are significantly upregulated under salt stress relative to their expression in another salt-sensitive poplar. Our results provide an important background for understanding tree adaptation to salt stress and facilitating the genetic improvement of cultivated poplars for saline soils.
C1 [Ma, Tao; Hu, Quanjun; Liu, Bingbing; Qiu, Qiang; Zhang, Jian; Wang, Kun; Jiang, Dechun; Zhou, Ran; Luo, Wenchun; Ma, Hui; Yang, Yongzhi; Wang, Xia; Wang, Gaini; Wang, Juan; Wang, Qian; Lu, Xu; Wu, Yuxia; Wan, Dongshi; Li, Jia; Liu Jianquan] Lanzhou Univ, Sch Life Sci, State Key Lab Grassland Agroecosyst, Lanzhou 730000, Peoples R China.
[Wang, Junyi; Yue, Zhen; Chen, Yan; Wang, Zhuo; Gou, Caiyun; Yu, Lili; Zhan, Dongliang; Pan, Shengkai; Fang, Dongming; Luo, Yadan; Chen, Zhe; Liu, Jinchao; Lu, Yao; Yin, Ye; Yang, Huanming; Wang, Jun] BGI Shenzhen, Shenzhen 518083, Peoples R China.
[Zhou, Gongke] Chinese Acad Sci, Key Lab Biofuels, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
[Zhou, Gongke] Chinese Acad Sci, Shandong Prov Key Lab Energy Genet, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
[Abbott, Richard J.] Univ St Andrews, Sch Biol, St Andrews KY16 9TH, Fife, Scotland.
[Yin, Tongming] Nanjing Forestry Univ, Key Lab Forest Genet & Gene Engn, Nanjing 210037, Jiangsu, Peoples R China.
[Lascoux, Martin] Uppsala Univ, Evolutionary Biol Ctr, Dept Ecol & Genet, S-75326 Uppsala, Sweden.
[DiFazio, Stephen P.] W Virginia Univ, Dept Biol, Morgantown, WV 26506 USA.
[Tuskan, Gerald A.] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA.
[Wang, Jun] Univ Copenhagen, Dept Biol, DK-1017 Copenhagen, Denmark.
RP Liu, JQ (reprint author), Lanzhou Univ, Sch Life Sci, State Key Lab Grassland Agroecosyst, Lanzhou 730000, Peoples R China.
EM wangj@genomics.org.cn; liujq@lzu.edu.cn
RI Wang, Jun/C-8434-2016; Tuskan, Gerald/A-6225-2011; Wang,
Jun/B-9503-2016;
OI Wang, Jun/0000-0002-8540-8931; Tuskan, Gerald/0000-0003-0106-1289; Hu,
Quanjun/0000-0001-6922-2144; Wang, Jun/0000-0002-2113-5874; Lascoux,
Martin/0000-0003-1699-9042
FU National Key Project for Basic Research [2012CB114504]; National High
Technology Research and Development Program of China (863 Program)
[2013AA100605]; National Science and Technology Support Program
[2013BAD22B01]; Fundamental Research Funds for the Central Universities
[lzujbky-2009-k05]; Shenzhen Municipal Government [ZYC200903240077A];
International Collaboration 111 Projects of China; 985 and 211 Projects
of Lanzhou University
FX Financial support was provided by the National Key Project for Basic
Research (2012CB114504), the National High Technology Research and
Development Program of China (863 Program, No. 2013AA100605), the
National Science and Technology Support Program (2013BAD22B01), the
Fundamental Research Funds for the Central Universities
(lzujbky-2009-k05), the International Collaboration 111 Projects of
China, the 985 and 211 Projects of Lanzhou University and the Shenzhen
Municipal Government (ZYC200903240077A).
NR 60
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U1 6
U2 80
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2797
DI 10.1038/ncomms3797
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LJ
UT WOS:000328025000012
PM 24256998
ER
PT J
AU Mann, IR
Lee, EA
Claudepierre, SG
Fennell, JF
Degeling, A
Rae, IJ
Baker, DN
Reeves, GD
Spence, HE
Ozeke, LG
Rankin, R
Milling, DK
Kale, A
Friedel, RHW
Honary, F
AF Mann, Ian R.
Lee, E. A.
Claudepierre, S. G.
Fennell, J. F.
Degeling, A.
Rae, I. J.
Baker, D. N.
Reeves, G. D.
Spence, H. E.
Ozeke, L. G.
Rankin, R.
Milling, D. K.
Kale, A.
Friedel, R. H. W.
Honary, F.
TI Discovery of the action of a geophysical synchrotron in the Earth's Van
Allen radiation belts
SO NATURE COMMUNICATIONS
LA English
DT Article
ID RELATIVISTIC ELECTRON FLUX; ULF WAVE POWER; INNER MAGNETOSPHERE;
GEOMAGNETIC STORMS; ACCELERATION; ENERGIZATION; DIFFUSION; PARTICLES;
DYNAMICS; FIELD
AB Although the Earth's Van Allen radiation belts were discovered over 50 years ago, the dominant processes responsible for relativistic electron acceleration, transport and loss remain poorly understood. Here we show evidence for the action of coherent acceleration due to resonance with ultra-low frequency waves on a planetary scale. Data from the CRRES probe, and from the recently launched multi-satellite NASA Van Allen Probes mission, with supporting modelling, collectively show coherent ultra-low frequency interactions which high energy resolution data reveals are far more common than either previously thought or observed. The observed modulations and energy-dependent spatial structure indicate a mode of action analogous to a geophysical synchrotron; this new mode of response represents a significant shift in known Van Allen radiation belt dynamics and structure. These periodic collisionless betatron acceleration processes also have applications in understanding the dynamics of, and periodic electromagnetic emissions from, distant plasma-astrophysical systems.
C1 [Mann, Ian R.; Lee, E. A.; Degeling, A.; Rae, I. J.; Ozeke, L. G.; Rankin, R.; Milling, D. K.; Kale, A.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada.
[Claudepierre, S. G.; Fennell, J. F.] Aerosp Corp, Los Angeles, CA 90009 USA.
[Rae, I. J.] Univ Coll London, Mullard Space Sci Lab, Dept Space & Climate Phys, Dorking RH5 6NT, Surrey, England.
[Baker, D. N.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA.
[Reeves, G. D.; Friedel, R. H. W.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA.
[Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA.
[Honary, F.] Univ Lancaster, Dept Phys, Lancaster LA1 4YB, England.
RP Mann, IR (reprint author), Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada.
EM imann@ualberta.ca
RI Friedel, Reiner/D-1410-2012; Degeling, Alexander/F-1091-2016;
OI Friedel, Reiner/0000-0002-5228-0281; Degeling,
Alexander/0000-0001-7338-9270; Reeves, Geoffrey/0000-0002-7985-8098
FU Canadian NSERC; RBSP-ECT; JHU/APL [967399]; NASA's Prime [NAS5-01072];
Canadian Array for Real-time Investigations of Magnetic Activity
(CARISMA); Canadian Space Agency; Facility for Data Analysis and
Modeling (FDAM); Canadian NSERC, Canada Foundation for Innovation,
WestGrid; Monitoring, Analyzing, and Assessing Radiation Belt Loss and
Energization (MAARBLE)
FX E.A.L. was supported by a Discovery Grant from Canadian NSERC awarded to
IRM. This work was supported by RBSP-ECT funding provided by JHU/APL
Contract No. 967399 under NASA's Prime Contract No. NAS5-01072. The
Canadian Array for Real-time Investigations of Magnetic Activity
(CARISMA; www.carisma.ca (2013)) array is operated by the University of
Alberta, funded by the Canadian Space Agency. The Sub-Auroral
Magnetometer Network data (SAMNET) is operated by the Space Plasma
Environment and Radio Science (SPEARS) group, Department of Physics,
Lancaster University. This work was supported by the Facility for Data
Analysis and Modeling (FDAM), with funding from Canadian NSERC, Canada
Foundation for Innovation, WestGrid, and the Canadian Space Agency. This
work was also supported by the Monitoring, Analyzing, and Assessing
Radiation Belt Loss and Energization (MAARBLE) project under the
European Commission (EC) FP7 framework (note that the work reflects the
authors views, and the EC is not liable for any use that may be made of
the information contained herein).
NR 31
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PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2795
DI 10.1038/ncomms3795
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LJ
UT WOS:000328025000010
ER
PT J
AU Petrovic, M
Rakic, IS
Runte, S
Busse, C
Sadowski, JT
Lazic, P
Pletikosic, I
Pan, ZH
Milun, M
Pervan, P
Atodiresei, N
Brako, R
Sokcevic, D
Valla, T
Michely, T
Kralj, M
AF Petrovic, M.
Rakic, I. Srut
Runte, S.
Busse, C.
Sadowski, J. T.
Lazic, P.
Pletikosic, I.
Pan, Z. -H.
Milun, M.
Pervan, P.
Atodiresei, N.
Brako, R.
Sokcevic, D.
Valla, T.
Michely, T.
Kralj, M.
TI The mechanism of caesium intercalation of graphene
SO NATURE COMMUNICATIONS
LA English
DT Article
ID METAL-SURFACES; GRAPHITE; SUPERCONDUCTIVITY; IR(111); IRIDIUM; CARBON;
FILMS
AB Properties of many layered materials, including copper- and iron-based superconductors, topological insulators, graphite and epitaxial graphene, can be manipulated by the inclusion of different atomic and molecular species between the layers via a process known as intercalation. For example, intercalation in graphite can lead to superconductivity and is crucial in the working cycle of modern batteries and supercapacitors. Intercalation involves complex diffusion processes along and across the layers; however, the microscopic mechanisms and dynamics of these processes are not well understood. Here we report on a novel mechanism for intercalation and entrapment of alkali atoms under epitaxial graphene. We find that the intercalation is adjusted by the van der Waals interaction, with the dynamics governed by defects anchored to graphene wrinkles. Our findings are relevant for the future design and application of graphene-based nano-structures. Similar mechanisms can also have a role for intercalation of layered materials.
C1 [Petrovic, M.; Rakic, I. Srut; Pletikosic, I.; Milun, M.; Pervan, P.; Kralj, M.] Inst Fiziku, Zagreb 10000, Croatia.
[Runte, S.; Busse, C.; Michely, T.] Univ Cologne, Inst Phys 2, D-50937 Cologne, Germany.
[Sadowski, J. T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Lazic, P.; Brako, R.; Sokcevic, D.] Rudjer Boskovic Inst, Zagreb 10000, Croatia.
[Pan, Z. -H.; Valla, T.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA.
[Atodiresei, N.] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany.
[Atodiresei, N.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany.
[Atodiresei, N.] JARA, D-52425 Julich, Germany.
RP Kralj, M (reprint author), Inst Fiziku, Bijenicka 46, Zagreb 10000, Croatia.
EM mkralj@ifs.hr
RI Lazic, Predrag/K-1908-2012; Busse, Carsten/A-7485-2008; Petrovic,
Marin/N-2473-2013; Kralj, Marko/A-8232-2008; Pletikosic,
Ivo/A-5683-2010; Pervan, Petar/F-8142-2010;
OI Busse, Carsten/0000-0001-5522-0578; Petrovic, Marin/0000-0002-2234-1207;
Kralj, Marko/0000-0002-9786-3130; Pletikosic, Ivo/0000-0003-4697-8912;
Pervan, Petar/0000-0002-0273-2737; Sadowski, Jerzy/0000-0002-4365-7796;
Atodiresei, Nicolae/0000-0002-8203-1227
FU Unity Through Knowledge Fund [66/10]; Deutsche Forschungsgemeinschaft
[Bu2197/2, INST 2156/514-1]; Ministry of Science and Technology of the
Republic of Croatia [098-0352828-2863]; German Academic Exchange Service
and Ministry of Science of the Republic of Croatia; U.S. Department of
Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]
FX We acknowledge experimental assistance by F. Craes and J. Klinkhammer.
This work was supported by the Unity Through Knowledge Fund (grant no.
66/10), the Deutsche Forschungsgemeinschaft (projects Bu2197/2 and INST
2156/514-1), the Ministry of Science and Technology of the Republic of
Croatia (contract no. 098-0352828-2863) and by the German Academic
Exchange Service and Ministry of Science of the Republic of Croatia via
the project 'Electrons in two dimensions'. Research carried out at the
Center for Functional Nanomaterials and National Synchrotron Light
Source, Brookhaven National Laboratory is supported by the U.S.
Department of Energy, Office of Basic Energy Sciences, under the
Contract No. DE-AC02-98CH10886.
NR 53
TC 57
Z9 57
U1 15
U2 193
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2772
DI 10.1038/ncomms3772
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266KY
UT WOS:000328023900010
PM 24212475
ER
PT J
AU Rasool, HI
Ophus, C
Klug, WS
Zettl, A
Gimzewski, JK
AF Rasool, Haider I.
Ophus, Colin
Klug, William S.
Zettl, A.
Gimzewski, James K.
TI Measurement of the intrinsic strength of crystalline and polycrystalline
graphene
SO NATURE COMMUNICATIONS
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; GRAIN-BOUNDARIES; DISLOCATION; NANOSCALE;
TRANSPORT; MEMBRANES; GROWTH; FILMS; MONOLAYER; SIZE
AB The mechanical properties of materials depend strongly on crystal structure and defect configuration. Here we measure the strength of suspended single-crystal and bicrystal graphene membranes prepared by chemical vapour deposition. Membranes of interest are first characterized by transmission electron microscopy and subsequently tested using atomic force microscopy. Single-crystal membranes prepared by chemical vapour deposition show strengths comparable to previous results of single-crystal membranes prepared by mechanical exfoliation. Grain boundaries with large mismatch angles in polycrystalline specimens have higher strengths than their low angle counterparts. Remarkably, these large angle grain boundaries show strength comparable to that of single-crystal graphene. To investigate this enhanced strength, we employ aberration-corrected high-resolution transmission electron microscopy to explicitly map the atomic-scale strain fields in suspended graphene. The high strength is attributed to the presence of low atomic-scale strain in the carbon-carbon bonds at the boundary.
C1 [Rasool, Haider I.; Zettl, A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Rasool, Haider I.; Zettl, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Rasool, Haider I.; Gimzewski, James K.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.
[Rasool, Haider I.; Klug, William S.; Gimzewski, James K.] Univ Calif Los Angeles, Calif NanoSyst Inst CNSI, Los Angeles, CA 90095 USA.
[Ophus, Colin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA.
[Klug, William S.] Univ Calif Los Angeles, Dept Mech & Aerosp Engn, Los Angeles, CA 90095 USA.
[Zettl, A.] Univ Calif Berkeley, COINS, Berkeley, CA 94720 USA.
[Gimzewski, James K.] Int Ctr Mat Nanoarchitecton MANA, Tsukuba, Ibaraki 3050044, Japan.
RP Rasool, HI (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
EM hrasool@berkeley.edu
RI Foundry, Molecular/G-9968-2014; Zettl, Alex/O-4925-2016;
OI Zettl, Alex/0000-0001-6330-136X; Ophus, Colin/0000-0003-2348-8558
FU MEXT WPI Program: International Center for Materials Nanoarchitectonics
(MANA) of Japan; Office of Energy Research, Office of Basic Energy
Sciences, Materials Sciences and Engineering Division, of the U.S.
Department of Energy (DOE) [DE-AC02-05CH11231]; Defense Threat Reduction
Agency (DTRA) [HDTRA1-13-1-0035]; National Science Foundation (NSF)
[DMR-1006128, CMMI-0748034]
FX H.I.R. and J.K.G. thank the MEXT WPI Program: International Center for
Materials Nanoarchitectonics (MANA) of Japan for financial support. This
work was supported in part by the Director, Office of Energy Research,
Office of Basic Energy Sciences, Materials Sciences and Engineering
Division, of the U.S. Department of Energy (DOE) under contract
DE-AC02-05CH11231, which provided for high-resolution TEM
characterization, including the work performed at the National Center of
Electron Microscopy (NCEM), and the Defense Threat Reduction Agency
(DTRA) under award HDTRA1-13-1-0035, which provided for graphene growth
and transfer. W.S.K. acknowledges support for this work from the
National Science Foundation (NSF) under Grant No. DMR-1006128 and
CMMI-0748034.
NR 45
TC 79
Z9 80
U1 14
U2 118
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2811
DI 10.1038/ncomms3811
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LV
UT WOS:000328026200001
ER
PT J
AU Yu, R
Goswami, P
Si, QM
Nikolic, P
Zhu, JX
AF Yu, Rong
Goswami, Pallab
Si, Qimiao
Nikolic, Predrag
Zhu, Jian-Xin
TI Superconductivity at the border of electron localization and itinerancy
SO NATURE COMMUNICATIONS
LA English
DT Article
ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; MAGNETIC EXCHANGE INTERACTIONS; IRON
PNICTIDES; SPIN-WAVES; INSULATOR; ORIGIN; FILMS; GAP
AB The superconducting state of iron pnictides and chalcogenides exists at the border of anti-ferromagnetic order. Consequently, these materials could provide clues about the relationship between magnetism and unconventional superconductivity. One explanation, motivated by the so-called bad metal behaviour of these materials proposes that magnetism and superconductivity develop out of quasi-localized magnetic moments that are generated by strong electron-electron correlations. Another suggests that these phenomena are the result of weakly interacting electron states that lie on nested Fermi surfaces. Here we address the issue by comparing the newly discovered alkaline iron selenide superconductors, which exhibit no Fermi-surface nesting, to their iron pnictide counterparts. We show that the strong-coupling approach leads to similar pairing amplitudes in these materials, despite their different Fermi surfaces. We also find that the pairing amplitudes are largest at the boundary between electronic localization and itinerancy, suggesting that new superconductors might be found in materials with similar characteristics.
C1 [Yu, Rong] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China.
[Yu, Rong; Goswami, Pallab; Si, Qimiao] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA.
[Nikolic, Predrag] George Mason Univ, Sch Phys Astron & Computat Sci, Fairfax, VA 22030 USA.
[Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM USA.
RP Si, QM (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA.
EM qmsi@rice.edu
RI Yu, Rong/H-3355-2016;
OI Zhu, Jianxin/0000-0001-7991-3918
FU NSF [DMR-1309531, DMR-0654118]; Robert A. Welch Foundation [C-1411];
National Science Foundation of China [11374361]; State of Florida; U. S.
Department of Energy through the National High Magnetic Field
Laboratory; Office of Naval Research [N00014-09-1-1025A]; National
Institute of Standards and Technology [70NANB7H6138, Am001]; U.S. DOE
[DE-AC52-06NA25396]; US DOE Office of Basic Energy Sciences; Center for
Integrated Nanotechnologies
FX This work was supported in part by the NSF Grant number DMR-1309531 and
the Robert A. Welch Foundation Grant number C-1411 (R.Y., P.G. and
Q.S.), the National Science Foundation of China Grant number 11374361
(R.Y.), the NSF Cooperative Agreement No. DMR-0654118, the State of
Florida, and the U. S. Department of Energy through the National High
Magnetic Field Laboratory (P.G.), the Office of Naval Research Grant
N00014-09-1-1025A and the National Institute of Standards and Technology
Grant 70NANB7H6138, Am001 (P.N.), and the U.S. DOE under Contract number
DE-AC52-06NA25396, the US DOE Office of Basic Energy Sciences and the
Center for Integrated Nanotechnologies-a US DOE user facility (J.-X.Z.).
NR 47
TC 24
Z9 24
U1 1
U2 41
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2783
DI 10.1038/ncomms3783
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LC
UT WOS:000328024300001
PM 24231858
ER
PT J
AU Zamadar, M
Asaoka, S
Grills, DC
Miller, JR
AF Zamadar, Matibur
Asaoka, Sadayuki
Grills, David C.
Miller, John R.
TI Giant infrared absorption bands of electrons and holes in conjugated
molecules
SO NATURE COMMUNICATIONS
LA English
DT Article
ID VIBRATIONAL-MODES; CHARGED SOLITONS; STRETCHING MODES; POLYMERS;
POLYACETYLENE; INTENSITIES; CARBONYL; POLARONS; STATE; DERIVATIVES
AB Infrared (IR) absorption bands often convey identifying information about molecules, but are usually weak, having molar absorption coefficients <200M(-1) cm(-1). Here we report observation of radical anions and cations of conjugated oligomers and polymers of fluorene and thiophene that possess intense mid-infrared absorption coefficients as large as 50,000M(-1) cm(-1), perhaps the largest known for molecular species. For anions of fluorene oligomers, F-n, n = 2-4, IR intensities increase almost linearly with n, but with a slope much larger than one, indicating that the absorptions are not extensive properties. Large intensities seem to arise from a mechanism known for charged solitons and polarons in conjugated polymers. In this mechanism, vibrations of ungerade symmetry drive substantial displacements of charge, creating the large dipole derivatives responsible for intense IR absorption. Both experiments and calculations find that pairing with counter-ions attenuates IR band intensities. The IR bands may be diagnostic for bound ion pairs and their escape to form free ions.
C1 [Zamadar, Matibur; Asaoka, Sadayuki; Grills, David C.; Miller, John R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
RP Miller, JR (reprint author), Brookhaven Natl Lab, Dept Chem, Bldg 555, Upton, NY 11973 USA.
EM jrmiller@bnl.gov
RI Grills, David/F-7196-2016
OI Grills, David/0000-0001-8349-9158
FU Brookhaven National Laboratory [DE-AC02-98CH10886]; US Department of
Energy; Division of Chemical Sciences, Geosciences & Biosciences, Office
of Basic Energy Sciences; Laboratory Directed Research at Brookhaven
National Laboratory [02544]
FX This research was carried out at Brookhaven National Laboratory under
contract DE-AC02-98CH10886 with the US Department of Energy and
supported by its Division of Chemical Sciences, Geosciences &
Biosciences, Office of Basic Energy Sciences, and to Laboratory Directed
Research Grant number 02544 at Brookhaven National Laboratory for
support to M.Z. and partial support to J.R.M. We thank Dr. Andrew Cook
for technical assistance and Larry Nafie for discussions.
NR 44
TC 5
Z9 5
U1 3
U2 41
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2818
DI 10.1038/ncomms3818
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266LY
UT WOS:000328026500001
ER
PT J
AU Zhang, JX
Ke, XX
Gou, GY
Seidel, J
Xiang, B
Yu, P
Liang, WI
Minor, AM
Chu, YH
Van Tendeloo, G
Ren, XB
Ramesh, R
AF Zhang, Jinxing
Ke, Xiaoxing
Gou, Gaoyang
Seidel, Jan
Xiang, Bin
Yu, Pu
Liang, Wen-I
Minor, Andrew M.
Chu, Ying-hao
Van Tendeloo, Gustaaf
Ren, Xiaobing
Ramesh, Ramamoorthy
TI A nanoscale shape memory oxide
SO NATURE COMMUNICATIONS
LA English
DT Article
ID FIELD-INDUCED STRAINS; BIFEO3 THIN-FILMS; ELECTROMECHANICAL RESPONSE;
PHASE-TRANSFORMATIONS; SINGLE-CRYSTALS; POLARIZATION; PSEUDOPOTENTIALS;
ALLOYS; TRANSITION; MECHANISM
AB Stimulus-responsive shape-memory materials have attracted tremendous research interests recently, with much effort focused on improving their mechanical actuation. Driven by the needs of nanoelectromechanical devices, materials with large mechanical strain, particularly at nanoscale level, are therefore desired. Here we report on the discovery of a large shape-memory effect in bismuth ferrite at the nanoscale. A maximum strain of up to similar to 14% and a large volumetric work density of similar to 600 +/- 90 J cm(-3) can be achieved in association with a martensitic-like phase transformation. With a single step, control of the phase transformation by thermal activation or electric field has been reversibly achieved without the assistance of external recovery stress. Although aspects such as hysteresis, microcracking and so on have to be taken into consideration for real devices, the large shape-memory effect in this oxide surpasses most alloys and, therefore, demonstrates itself as an extraordinary material for potential use in state-of-art nanosystems.
C1 [Zhang, Jinxing] Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China.
[Zhang, Jinxing; Seidel, Jan; Yu, Pu; Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Ke, Xiaoxing; Van Tendeloo, Gustaaf] Univ Antwerp, EMAT Electron Microscopy Mat Sci, B-2020 Antwerp, Belgium.
[Gou, Gaoyang; Ren, Xiaobing] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Multidisciplinary Mat Res Ctr, Xian 710049, Peoples R China.
[Seidel, Jan] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia.
[Xiang, Bin] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China.
[Yu, Pu] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China.
[Yu, Pu] Tsinghua Univ, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China.
[Liang, Wen-I; Chu, Ying-hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan.
[Xiang, Bin; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA.
[Minor, Andrew M.; Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
RP Zhang, JX (reprint author), Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China.
EM jxzhang@bnu.edu.cn; xiaoxing.ke@uantwerpen.be
RI Ying-Hao, Chu/A-4204-2008; Gou, Gaoyang/D-9289-2011; Yu, Pu/F-1594-2014;
Xiang, Bin/C-9192-2012; Ke, Xiaoxing/A-2723-2013; Foundry,
Molecular/G-9968-2014; Ren, Xiaobing/B-6072-2009
OI Ying-Hao, Chu/0000-0002-3435-9084; Ke, Xiaoxing/0000-0003-2004-6906;
Ren, Xiaobing/0000-0002-4973-2486
FU National Science Foundation of China [51322207, 51332001, 11274045];
European Research Council (ERC) [246791-COUNTATOMS]; National Basic
Research Program of China [2012CB619401]; Natural Science Foundation of
China [11204230]; National Super-conmputer Center in Tianjin (NSCC);
National Science Council, R.O.C [NSC-101-2119-M-009-003-MY2]; Ministry
of Education [MOE-ATU 101W961]; Center for Interdisciplinary Science of
National Chiao Tung University; Australian Research Council (ARC)
[FT110100523]; National Center for Electron Microscopy
[DE-AC02-05CH11231]
FX The work in Beijing Normal University is supported by the National
Science Foundation of China under contract numbers 51322207, 51332001
and 11274045. X.K. and G.V.T. are grateful to funding from the European
Research Council under the Seventh Framework Program (FP7), ERC Advanced
grant number 246791-COUNTATOMS. We thank Professor Dr Sandra Van Aert
for helpful discussions. G.Y.G. and X.B.R. were support by the National
Basic Research Program of China, under contract number 2012CB619401,
Natural Science Foundation of China (11204230) and National
Super-conmputer Center in Tianjin (NSCC). The work at National Chiao
Tung University is supported by the National Science Council, R.O.C
(NSC-101-2119-M-009-003-MY2), Ministry of Education (MOE-ATU 101W961)
and Center for Interdisciplinary Science of National Chiao Tung
University. J.S. acknowledges support by the Australian Research Council
(ARC) through a Future Fellowship (FT110100523). B.X. and A.M.M
acknowledge the support of National Center for Electron Microscopy,
under Contract #DE-AC02-05CH11231.
NR 60
TC 32
Z9 33
U1 17
U2 175
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2768
DI 10.1038/ncomms3768
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266KY
UT WOS:000328023900006
PM 24253399
ER
PT J
AU Wu, WM
Watson, DB
Luo, J
Carley, J
Mehlhorn, T
Kitanidis, PK
Jardine, PM
Criddle, CS
AF Wu, Wei-Min
Watson, David B.
Luo, Jian
Carley, Jack
Mehlhorn, Tonia
Kitanidis, Peter K.
Jardine, Phlip M.
Criddle, Craig S.
TI Surge block method for controlling well clogging and sampling sediment
during bioremediation
SO WATER RESEARCH
LA English
DT Article
DE Surge block; Bioremediation; Subsurface; Clogging; Well rehabilitation;
Sediment sampling
ID EMULSIFIED VEGETABLE-OIL; IN-SITU BIOREMEDIATION; MICROBIAL COMMUNITIES;
SUBMICROMOLAR LEVELS; ELECTRON-DONOR; URANIUM; BIOREDUCTION; REDUCTION;
SULFATE; AQUIFER
AB A surge block treatment method (i.e. inserting a solid rod plunger with a flat seal that closely fits the casing interior into a well and stocking it up and down) was performed for the rehabilitation of wells clogged with biomass and for the collection of time series sediment samples during in situ bioremediation tests for U(VI) immobilization at a the U.S. Department of Energy site in Oak Ridge, TN. The clogging caused by biomass growth had been controlled by using routine surge block treatment for18 times over a nearly four year test period. The treatment frequency was dependent of the dosage of electron donor injection and microbial community developed in the subsurface. Hydraulic tests showed that the apparent aquifer transmissivity at a clogged well with an inner diameter (ID) of 10.16 cm was increased by 8-13 times after the rehabilitation, indicating the effectiveness of the rehabilitation. Simultaneously with the rehabilitation, the surge block method was successfully used for collecting time series sediment samples composed of fine particles (clay and silt) from wells with ID 1.9-10.16 cm for the analysis of mineralogical and geochemical composition and microbial community during the same period. Our results demonstrated that the surge block method provided a cost-effective approach for both well rehabilitation and frequent solid sampling at the same location. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Wu, Wei-Min; Kitanidis, Peter K.; Criddle, Craig S.] Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA.
[Wu, Wei-Min] Stanford Univ, Ctr Sustainable Dev & Global Competitiveness, Stanford, CA 94305 USA.
[Watson, David B.; Carley, Jack; Mehlhorn, Tonia] Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37831 USA.
[Luo, Jian] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA.
[Jardine, Phlip M.] Univ Tennessee, Biosyst Engn & Soil Sci Dept, Knoxville, TN 37996 USA.
RP Wu, WM (reprint author), Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA.
EM wei-min.wu@stanford.edu; watsondb@ornl.gov
RI Watson, David/C-3256-2016
OI Watson, David/0000-0002-4972-4136
FU U.S. DOE Subsurface Biogeochemical Research Program [DOE-AC05-00OR22725,
DE-SC0006783]
FX This work was funded by the U.S. DOE Subsurface Biogeochemical Research
Program under grants DOE-AC05-00OR22725 and DE-SC0006783.
NR 23
TC 1
Z9 1
U1 2
U2 16
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0043-1354
J9 WATER RES
JI Water Res.
PD NOV 1
PY 2013
VL 47
IS 17
BP 6566
EP 6573
DI 10.1016/j.watres.2013.08.033
PG 8
WC Engineering, Environmental; Environmental Sciences; Water Resources
SC Engineering; Environmental Sciences & Ecology; Water Resources
GA 264WM
UT WOS:000327911700015
PM 24070865
ER
PT J
AU Cardiel, JJ
Tonggu, L
Dohnalkova, AC
de la Iglesia, P
Pozzo, DC
Wang, LG
Shen, AQ
AF Cardiel, Joshua J.
Tonggu, Lige
Dohnalkova, Alice C.
de la Iglesia, Pablo
Pozzo, Danilo C.
Wang, Liguo
Shen, Amy Q.
TI Worming Their Way into Shape: Toroidal Formations in Micellar Solutions
SO ACS NANO
LA English
DT Article
DE toroidal nanostructures; wormlike micelles; flow-induced structures;
microfluidics; sonication
ID DRYING-INDUCED ARTIFACTS; SURFACTANT DISPERSIONS; ELECTRON-MICROSCOPY;
ELASTIC PROPERTIES; WORMLIKE MICELLES; PHASE; SHEAR; VESICLES; FLOW;
ASSEMBLIES
AB We report the formation of nanostructured toroidal micellar bundles (nTMB) from a semidilute wormlike micellar solution, evidenced by both cryogenic-electron microscopy and transmission electron microscopy images. Our strategy for creating nTMB involves a two-step protocol consisting of a simple prestraining process followed by flow through a microfluidic device containing an array of microposts, producing strain rates in the wormlike micelles on the order of 10(5) s(-1). In combination with microfluidic confinement, these unusually large strain rates allow for the formation of stable nTMB. Electron microscopy images reveal a variety of nTMB morphologies and provide the size distribution of the nTMB. Small-angle neutron scattering indicates the underlying microstructural transition from wormlike micelles to nTMB. We also show that other flow-induced approaches such as sonication can induce and control the emergence of onion-like and nTMB structures, which may provide a useful tool for nanotemplating.
C1 [Cardiel, Joshua J.; Shen, Amy Q.] Univ Washington, Dept Mech Engn, Seattle, WA 98195 USA.
[Tonggu, Lige; Wang, Liguo] Univ Washington, Dept Biol Struct, Seattle, WA 98195 USA.
[Dohnalkova, Alice C.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA.
[de la Iglesia, Pablo; Pozzo, Danilo C.] Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA.
RP Shen, AQ (reprint author), Univ Washington, Dept Mech Engn, Seattle, WA 98195 USA.
EM amyshen@uw.edu
RI Shen, Amy/B-5981-2015
OI Shen, Amy/0000-0002-1222-6264
FU National Science Foundation [CBET 0852471, DMR 0907638, DMR 0944772];
Department of Energy's Office of Biological and Environmental Research
and located at Pacific Northwest National Laboratory [PNNL-EMSL-39946];
CONACYT-Ph.D. fellowship
FX We acknowledge support from the National Science Foundation (CBET
0852471 (A.Q.S.), DMR 0907638 (A.Q.S.), and DMR 0944772 (D.C.P.)). We
also thank NIST, U.S. Department of Commerce, in providing access to
neutron research facilities. A portion of the research was performed
using EMSL, a national scientific user facility sponsored by the
Department of Energy's Office of Biological and Environmental Research
and located at Pacific Northwest National Laboratory (PNNL-EMSL-39946).
J.J.C. is grateful for a CONACYT-Ph.D. fellowship.
NR 45
TC 3
Z9 3
U1 4
U2 52
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 9704
EP 9713
DI 10.1021/nn404191s
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200019
PM 24168354
ER
PT J
AU Meng, H
Zhao, Y
Dong, JY
Xue, M
Lin, YS
Ji, ZX
Mai, WX
Zhang, HY
Chang, CH
Brinker, CJ
Zink, JI
Nel, AE
AF Meng, Huan
Zhao, Yang
Dong, Juyao
Xue, Min
Lin, Yu-Shen
Ji, Zhaoxia
Mai, Wilson X.
Zhang, Haiyuan
Chang, Chong Hyun
Brinker, C. Jeffrey
Zink, Jeffrey I.
Nel, Andre E.
TI Two-Wave Nanotherapy To Target the Stroma and Optimize Gemcitabine
Delivery To a Human Pancreatic Cancer Model in Mice
SO ACS NANO
LA English
DT Article
DE nano-engineered approach; two-wave; pancreatic cancer; pericyte and
stroma; TGF-beta; gemcitabine; mesoporous silica nanoparticles; liposome
ID GROWTH-FACTOR-BETA; MESOPOROUS SILICA NANOPARTICLES; VIVO
ANTITUMOR-ACTIVITY; TGF-BETA; DUCTAL ADENOCARCINOMA; IN-VIVO; CYTIDINE
DEAMINASE; BREAST-CARCINOMA; PROSTATE-CANCER; NAB-PACLITAXEL
AB Pancreatic ductal adenocarcinoma (PDAC) elicits a dense stromal response that blocks vascular access because of pericyte coverage of vascular fenestrations. In this way, the PDAC stroma contributes to chemotherapy resistance in addition to causing other problems. In order to improve the delivery of gemcitabine, a first-line chemotherapeutic agent, a PEGylated drug-carrying liposome was developed, using a transmembrane ammonium sulfate gradient to encapsulate the protonated drug up to 20% w/w. However, because the liposome was precluded from entering the xenograft site due to the stromal interference, we developed a first-wave nanocarrier that decreases pericyte coverage of the vasculature through interference in the pericyte recruiting TGF-beta signaling pathway. This was accomplished using a polyethyleneimine (PEI)/polyethylene glycol (PEG)-coated mesoporous silica nanoparticle (MSNP) for molecular complexation to a small molecule TGF-beta inhibitor, LY364947. LY364947 contains a nitrogen atom that attaches, through H-bonding, to PEI amines with a high rate of efficiency. The copolymer coating also facilitates systemic biodistribution and retention at the tumor site. Because of the high loading capacity and pH-dependent LY364947 release from the MSNPs, we achieved rapid entry of IV-injected liposomes and MSNPs at the PDAC tumor site. This two-wave approach provided effective shrinkage of the tumor xenografts beyond 25 days, compared to the treatment with free drug or gemcitabine-loaded liposomes only. Not only does this approach overcome stromal resistance to drug delivery in PDAC, but it also introduces the concept of using a stepwise engineered approach to address a range of biological impediments that interfere in nanocancer therapy in a spectrum of cancers.
C1 [Meng, Huan; Zhao, Yang; Mai, Wilson X.; Zhang, Haiyuan; Nel, Andre E.] Univ Calif Los Angeles, Dept Med, Div NanoMed, Los Angeles, CA 90095 USA.
[Dong, Juyao; Xue, Min; Zink, Jeffrey I.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.
[Ji, Zhaoxia; Chang, Chong Hyun; Zink, Jeffrey I.; Nel, Andre E.] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA.
[Brinker, C. Jeffrey] Sandia Natl Labs, Selfassembled Mat Dept, Albuquerque, NM 87185 USA.
[Lin, Yu-Shen] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA.
[Brinker, C. Jeffrey] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA.
[Brinker, C. Jeffrey] Sandia Natl Labs, Albuquerque, NM 87106 USA.
RP Nel, AE (reprint author), Univ Calif Los Angeles, Dept Med, Div NanoMed, Los Angeles, CA 90095 USA.
EM hmeng@mednet.ucla.edu; anel@mednet.ucla.edu
RI Xue, Min/I-9276-2014; Meng, Huan/J-3428-2014; Zhao, Yang/J-2690-2014;
OI Xue, Min/0000-0002-8136-6551; Zhang, Haiyuan/0000-0003-4076-1771
FU U.S. Public Health Service [RO1 CA133697]; NCI [1U01CA151792-01]
FX This study was funded by the U.S. Public Health Service Grant RO1
CA133697. Y.-S.L. and C.J.B. are supported by NCI Cancer Nanotechnology
Platform Partnership Grant 1U01CA151792-01.
NR 64
TC 39
Z9 40
U1 9
U2 94
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10048
EP 10065
DI 10.1021/nn404083m
PG 18
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200053
PM 24143858
ER
PT J
AU Zhang, H
Son, JS
Jang, J
Lee, JS
Ong, WL
Malen, JA
Talapin, DV
AF Zhang, Hao
Son, Jae Sung
Jang, Jaeyoung
Lee, Jong-Soo
Ong, Wee-Liat
Malen, Jonathan A.
Talapin, Dmitri V.
TI Bi1-xSbx Alloy Nanocrystals: Colloidal Synthesis, Charge Transport, and
Thermoelectric Properties
SO ACS NANO
LA English
DT Article
DE Bi1-xSbx nanocrystals; electrical conductivity; Hall effect
measurements; grain boundaries; surface chemistry; thermoelectrics
ID BI-SB ALLOYS; CHALCOGENIDE SURFACE LIGANDS; BISMUTH NANOPARTICLES;
SEMICONDUCTING ALLOYS; ELECTRONIC-PROPERTIES; NANOWIRE ARRAYS;
THIN-FILMS; SOLIDS; INSB; TRISDIMETHYLAMINOANTIMONY
AB Nanostructured Bi1-xSbx alloys constitute a convenient system to study charge transport in a nanostructured narrow-gap semiconductor with promising thermoelectric properties. In this work, we developed the colloidal synthesis of monodisperse sub-10 nm Bi1-xSbx alloy nanocrystals (NCs) with controllable size and compositions. The surface chemistry of Bi1-xSbx NCs was tailored with inorganic ligands to improve the interparticle charge transport as well as to control the carrier concentration. Temperature-dependent (10-300 K) electrical measurements were performed on the Bi1-xSbx NC based pellets to investigate the effect of surface chemistry and grain size (similar to 10-40 nm) on their charge transport properties. The Hall effect measurements revealed that the temperature dependence of carrier mobility and concentration strongly depended on the grain size and the surface chemistry, which was different from the reported bulk behavior. At low temperatures, electron mobility in nanostructured Bi1-xSbx was directly proportional to the average grain size, while the concentration of free carriers was inversely proportional to the grain size. We propose a model explaining such behavior. Preliminary measurements of thermoelectric properties showed a ZT value comparable to those of bulk Bi1-xSbx alloys at 300 K, suggesting a potential of Bi1-xSbx NCs for low-temperature thermoelectric applications.
C1 [Zhang, Hao; Son, Jae Sung; Jang, Jaeyoung; Lee, Jong-Soo; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA.
[Zhang, Hao; Son, Jae Sung; Jang, Jaeyoung; Lee, Jong-Soo; Talapin, Dmitri V.] Univ Chicago, James Frank Inst, Chicago, IL 60637 USA.
[Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Malen, Jonathan A.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA.
[Ong, Wee-Liat; Malen, Jonathan A.] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA.
RP Talapin, DV (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA.
EM dvtalapin@uchicago.edu
RI Son, Jae Sung/C-2903-2014; Lee, Jong-Soo /F-7461-2010; Malen,
Jonathan/D-5954-2013
OI Lee, Jong-Soo /0000-0002-3045-2206; Malen, Jonathan/0000-0003-4560-4476
FU II-VI Foundation; NSF MRSEC Program [DMR-0213745]; AFOSR Young
Investigator Program [FA95501110030]; NSF CAREER [ENG1149374]
FX We thank W. Liu and M. Boles for the discussion on the synthesis of
Bi1-xSbx NCs and D. Dolzhnikov for the synthesis
of metal-free chalcogenide ligands. This work was supported by the II-VI
Foundation and the NSF MRSEC Program under Award Number DMR-0213745.
J.A.M. and W-L.O. acknowledge support from the AFOSR Young Investigator
Program (FA95501110030) and the NSF CAREER Award (ENG1149374).
NR 57
TC 15
Z9 15
U1 11
U2 91
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10296
EP 10306
DI 10.1021/nn404692s
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200078
PM 24134215
ER
PT J
AU Kaz, DM
Bischak, CG
Hetherington, CL
Howard, HH
Marti, X
Clarkson, JD
Adamo, C
Schlom, DG
Ramesh, R
Aloni, S
Ogletree, DF
Ginsberg, NS
AF Kaz, David M.
Bischak, Connor G.
Hetherington, Craig L.
Howard, Hannah H.
Marti, Xavier
Clarkson, James D.
Adamo, Carolina
Schlom, Darrell G.
Ramesh, Ramamoorthy
Aloni, Shaul
Ogletree, D. Frank
Ginsberg, Naomi S.
TI Bright Cathodoluminescent Thin Films for Scanning Nano-Optical
Excitation and Imaging
SO ACS NANO
LA English
DT Article
DE cathodoluminescence; thin-films; nano-optical; near-field; imaging;
nanopatterning
ID FIELD-EMISSION DISPLAY; ULTRA-HIGH-RESOLUTION; SCINTILLATION PROPERTIES;
SPATIAL-DISTRIBUTION; WAVE-GUIDES; MICROSCOPY; LUMINESCENCE;
FLUORESCENCE; SPECTROSCOPY; LIGHT
AB Demand for visualizing nanoscale dynamics in biological and advanced materials continues to drive the development of subdiffraction optical probes. While many strategies employ scanning tips for this purpose, we instead exploit a focused electron beam to create scannable nanoscale optical excitations in an epitaxially grown thin-film of cerium-doped yttrium aluminum perovskite, whose cathodoluminescence response is bright, robust, and spatially resolved to 18 nm. We also demonstrate lithographic patterning of the film's luminescence at the nanoscale. We anticipate that converting these films into free-standing membranes will yield a powerful near-field optical microscopy without the complication of mechanical scanning.
C1 [Kaz, David M.; Bischak, Connor G.; Hetherington, Craig L.; Howard, Hannah H.; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
[Ramesh, Ramamoorthy; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.
[Marti, Xavier; Clarkson, James D.; Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Kaz, David M.; Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.
[Ramesh, Ramamoorthy; Aloni, Shaul; Ogletree, D. Frank; Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Aloni, Shaul; Ogletree, D. Frank] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Adamo, Carolina; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA.
[Schlom, Darrell G.] Cornell Nanoscale Sci, Kavli Inst, Ithaca, NY 14853 USA.
[Ginsberg, Naomi S.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA.
RP Ginsberg, NS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
EM nsginsberg@berkeley.edu
RI Marti, Xavier/E-1103-2014; Foundry, Molecular/G-9968-2014; Ogletree, D
Frank/D-9833-2016
OI Marti, Xavier/0000-0003-1653-5619; Ogletree, D Frank/0000-0002-8159-0182
FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic
Energy Sciences, Office of Science, US. Department of Energy, FWP;
National Science Foundation [1152656]; Office of Science, Office of
Basic Energy Sciences, of the U.S. Department of Energy
[DE-AC02-05CH11231]; AFOSR [FA9550-10-1-0123]; NSF Graduate Research
Fellowship [DGE 1106400]
FX YAP:Ce film deposition was supported by the Chemical Sciences,
Geosciences and Biosciences Division, Office of Basic Energy Sciences,
Office of Science, US. Department of Energy, FWP number SISGRKN. CL
characterization and nano-fabrication were supported by the National
Science Foundation under Grant Number 1152656. CL, AFM and time-resolved
fluorescence at the LBL Molecular Foundry were supported by the Office
of Science, Office of Basic Energy Sciences, of the U.S. Department of
Energy under Contract No. DE-AC02-05CH11231. CA. and D.G.S. acknowledge
support under the AFOSR Grant No. FA9550-10-1-0123, C.G.B. acknowledges
an NSF Graduate Research Fellowship (DGE 1106400), and N.S.G.
acknowledges a David and Lucile Packard Fellowship for Science and
Engineering. We thank the P. Yang group for use of their XRD and the G.
R. Fleming group for use of their fluorimeter. N.S.G. also thanks T. G.
Ristroph for scintillating discussions.
NR 55
TC 10
Z9 10
U1 1
U2 35
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10397
EP 10404
DI 10.1021/nn404911a
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200089
PM 24156282
ER
PT J
AU Cox, PA
Waldow, DA
Dupper, TJ
Jesse, S
Ginger, DS
AF Cox, Phillip A.
Waldow, Dean A.
Dupper, Torin J.
Jesse, Stephen
Ginger, David S.
TI Mapping Nanoscale Variations in Photochemical Damage of
Polymer/Fullerene Solar Cells with Dissipation Imaging
SO ACS NANO
LA English
DT Article
DE atomic force microscopy; organic solar cells; photovoltaics; dissipation
imaging; photo-oxidation; photodegradation; PTB7
ID ATOMIC-FORCE MICROSCOPY; ORGANIC PHOTOVOLTAIC DEVICES;
ENERGY-DISSIPATION; TRAP FORMATION; DYNAMIC-MODE; ACTIVE LAYER;
DEGRADATION; MORPHOLOGY; EFFICIENCY; STABILITY
AB We use frequency-modulated electrostatic force microscopy to track changes in cantilever quality factor (Q) as a function of photochemical damage in a model organic photovoltaic system poly-[[4,8-bis[(2-ethylhexl)oxy]benzo[1,2-b:4,5-b']dithiophene-2,6-diy1]- [3-fluoro-2-[(2-ethylhexyl)carbonyl]thieno(3,4-b]thiophenediyl]] (PTB7) and 3'H-cyclopropa[8,25][5,6]fullerene-C71-D5h(6)-3'-butanoic acid, 3'-phenyl-, methyl ester (Pc71BM). We correlate local Q factor imaging with macroscopic device performance and show that, for this system, changes in cantilever Q correlate well with changes in external quantum efficiency and can thus be used to monitor local photochemical damage over the entire functional lifetime of a PTB7:PC71BM solar cell. We explore how Q imaging is affected by the choice of cantilever resonance frequency. Finally, we use Q imaging to elucidate the differences in the evolution of nanoscale structure in the photochemical damage occurring in PTB7:PC71BM solar cells processed with and without the solvent additive 1,8-diiodooctane (DIO). We show that processing with DIO not only yields a preferable morphology for uniform performance across the surface of the device but also enhances the stability of PTB7:PC71BM solar cells-an effect that can be predicted based on the local Q images.
C1 [Cox, Phillip A.; Dupper, Torin J.; Ginger, David S.] Univ Washington, Dept Chem, Seattle, WA 98195 USA.
[Waldow, Dean A.] Pacific Lutheran Univ, Dept Chem, Tacoma, WA 98447 USA.
[Jesse, Stephen] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
RP Ginger, DS (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA.
EM ginger@chem.washington.edu
RI Zhou, David/N-5367-2015; Jesse, Stephen/D-3975-2016; Ginger,
David/C-4866-2011;
OI Jesse, Stephen/0000-0002-1168-8483; Ginger, David/0000-0002-9759-5447;
Waldow, Dean/0000-0002-0588-4760
FU Scientific User Facilities Division, Office of Basic Energy Sciences,
U.S. Department of Energy
FX This work was initially seeded by the National Science Foundation (NSF)
DMR-1005504 and completed under NSF DMR-1306079. D.W. acknowledges NSF
for research instrumentation (MRI-0619826). Band excitation measurements
were conducted at the Center for Nanophase Materials Sciences, which is
sponsored at Oak Ridge National Laboratory by the Scientific User
Facilities Division, Office of Basic Energy Sciences, U.S. Department of
Energy.
NR 60
TC 11
Z9 11
U1 5
U2 67
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10405
EP 10413
DI 10.1021/nn404920t
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200090
PM 24138326
ER
PT J
AU Acharya, DP
Yoon, Y
Li, ZJ
Zhang, ZR
Lin, X
Mu, RT
Chen, L
Kay, BD
Rousseau, R
Dohnalek, Z
AF Acharya, Danda P.
Yoon, Yeohoon
Li, Zhenjun
Zhang, Zhenrong
Lin, Xiao
Mu, Rentao
Chen, Long
Kay, Bruce D.
Rousseau, Roger
Dohnalek, Zdenek
TI Site-Specific Imaging of Elemental Steps in Dehydration of Diols on
TiO2(110)
SO ACS NANO
LA English
DT Article
DE titanium dioxide; diols; scanning tunneling microscopy; adsorbate
dynamics; dehydration
ID DENSITY-FUNCTIONAL THEORY; ETHYLENE-GLYCOL; SINGLE-CRYSTAL; RUTILE
TIO2(110); O-H; DISSOCIATIVE ADSORPTION; ALIPHATIC-ALCOHOLS; SURFACE
SCIENCE; BOND SCISSION; TIO2
AB Scanning tunneling microscopy is employed to follow elemental steps in conversion of ethylene glycol and 1,3-propylene glycol on partially reduced TiO2(110) as a function of temperature. Mechanistic details about the observed processes are corroborated by density functional theory calculations. The use of these two diol reactants allows us to compare and contrast the chemistries of two functionally similar molecules with different steric constraints, thereby allowing us to understand how molecular geometry may influence the observed chemical reactivity. We find that both glycols initially adsorb on Ti sites, where a dynamic equilibrium between molecularly bound and deprotonated species is observed. As the diols start to diffuse along the Ti rows above 230 K, they irreversibly dissociate upon encountering bridging oxygen vacancies. Surprisingly, two dissociation pathways, one via O-H and the other via C-O bond scission, are observed. Theoretical calculations suggest that the differences in the C-O/O-H bond breaking processes are the result of steric factors enforced upon the diols by the second Ti-bound OH group. Above similar to 400 K, a new stable intermediate centered on the bridging oxygen (O-b) row is observed. Combined experimental and theoretical evidence shows that this intermediate is most likely a new dioxo species. Further annealing leads to sequential C-O-b bond cleavage and alkene desorption above similar to 500 K. Simulations demonstrate that the sequential C-O-b bond breaking process follows a homolytic diradical pathway, with the first C-O-b bond breaking event accompanied with a nonadiabatic electron transfer within the TiO2(110) substrate.
C1 [Acharya, Danda P.; Yoon, Yeohoon; Li, Zhenjun; Lin, Xiao; Mu, Rentao; Chen, Long; Kay, Bruce D.; Rousseau, Roger; Dohnalek, Zdenek] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
[Acharya, Danda P.; Yoon, Yeohoon; Li, Zhenjun; Lin, Xiao; Mu, Rentao; Chen, Long; Kay, Bruce D.; Rousseau, Roger; Dohnalek, Zdenek] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.
[Zhang, Zhenrong] Baylor Univ, Dept Phys, Waco, TX 76798 USA.
RP Rousseau, R (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, POB 999, Richland, WA 99352 USA.
EM Roger.Rousseau@pnnl.gov; Zdenek.Dohnalek@pnnl.gov
RI MU, RENTAO/A-1334-2014; Rousseau, Roger/C-3703-2014; Yoon,
Yeohoon/D-4934-2014; Mu, Rentao/H-1059-2011; Lin, Xiao/B-5055-2009;
OI Zhang, Zhenrong/0000-0003-3969-2326
FU Linus Pauling Distinguished Postdoctoral Fellowship Program; Laboratory
Directed Research and Development Program at Pacific Northwest National
Laboratory (PNNL); American Chemical Society Petroleum Research Fund;
U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Chemical Sciences, Geosciences Biosciences; Department of Energy's
Office of Biological and Environmental Research and located at Pacific
Northwest National Laboratory (PNNL)
FX X.L. is grateful for the support of the Linus Pauling Distinguished
Postdoctoral Fellowship Program funded by Laboratory Directed Research
and Development Program at Pacific Northwest National Laboratory (PNNL).
Z.Z. acknowledges the American Chemical Society Petroleum Research Fund
for the support of this research. Other authors were supported by the
U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Chemical Sciences, Geosciences & Biosciences, and the work was performed
in EMSL, a national scientific user facility sponsored by the Department
of Energy's Office of Biological and Environmental Research and located
at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram
national laboratory operated for the DOE by Battelle.
NR 62
TC 11
Z9 11
U1 2
U2 53
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10414
EP 10423
DI 10.1021/nn404934q
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200091
PM 24134162
ER
PT J
AU Choi, IC
Kim, YJ
Wang, YM
Ramamurty, U
Jang, JI
AF Choi, In-Chul
Kim, Yong-Jae
Wang, Y. Morris
Ramamurty, Upadrasta
Jang, Jae-il
TI Nanoindentation behavior of nanotwinned Cu: Influence of indenter angle
on hardness, strain rate sensitivity and activation volume
SO ACTA MATERIALIA
LA English
DT Article
DE Nanotwinned metals; Nanoindentation; Hardness; Strain-rate sensitivity;
Activation volume
ID NANO-SCALE TWINS; INDENTATION EXPERIMENTS; NANOCRYSTALLINE METALS;
NANOSCALE TWINS; ELASTIC-MODULUS; DEFORMATION; COPPER; STRESS; NICKEL;
CREEP
AB The influence of strain on the mechanical properties and deformation kinetic parameters of nanotwinned (at) copper is investigated by a series of nanoindentation experiments, which were performed by employing sharp indenters with five varying centerline-to-face angles (psi). Comparison experiments were also conducted on (1 1 0) single crystalline Cu. Experimental results indicate that, unlike coarsegrained materials, nt-Cu is prone to plastic flow softening with large material pile-up around the indentation impression at high levels of strains. Localized detwinning becomes more significant with decreasing psi, concomitant with reduced strain-rate sensitivity (m) and enhanced activation volume (V*). The m of nt-Cu is found to depend sensitively on psi with a variation of more than a factor of 3, whereas V* exhibits a much less sensitive trend. This paper discusses the validation of the experimental techniques and the implications of various deformation kinetic parameters on the underlying deformation mechanisms of nt-Ca. 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Choi, In-Chul; Kim, Yong-Jae; Jang, Jae-il] Hanyang Univ, Div Mat Sci & Engn, Seoul 133791, South Korea.
[Wang, Y. Morris] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
[Ramamurty, Upadrasta] Indian Inst Sci, Dept Mat Engn, Bangalore 560012, Karnataka, India.
[Ramamurty, Upadrasta] King Abdulaziz Univ, Ctr Excellence Adv Mat Res, Jeddah 21589, Saudi Arabia.
RP Jang, JI (reprint author), Hanyang Univ, Div Mat Sci & Engn, Seoul 133791, South Korea.
EM jijang@hanyang.ac.kr
RI Jang, Jae-il/A-3486-2011; Choi, In-Chul/E-1499-2014; Ramamurty,
Upadrasta/E-5623-2011; Wang, Yinmin (Morris)/F-2249-2010
OI Jang, Jae-il/0000-0003-4526-5355; Wang, Yinmin
(Morris)/0000-0002-7161-2034
FU Basic Science Research Program through the National Research Foundation
of Korea (NRF); Ministry of Education, Science and Technology
[2010-0025526]; Human Resources Development program of the Korea
Institute of Energy Technology Evaluation and Planning (KETEP) grant
[20114010203020]; Korea Government Ministry of Trade, Industry and
Energy; US Department of Energy by Lawrence Livermore National Security,
LLC [DE-AC52-07NA27344]
FX This research was supported by Basic Science Research Program through
the National Research Foundation of Korea (NRF) funded by the Ministry
of Education, Science and Technology (No. 2010-0025526), and in part by
the Human Resources Development program (No. 20114010203020) of the
Korea Institute of Energy Technology Evaluation and Planning (KETEP)
grant funded by the Korea Government Ministry of Trade, Industry and
Energy. The work at LLNL was performed under the auspices of the US
Department of Energy by Lawrence Livermore National Security, LLC under
Contract No. DE-AC52-07NA27344.
NR 60
TC 25
Z9 26
U1 5
U2 78
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
EI 1873-2453
J9 ACTA MATER
JI Acta Mater.
PD NOV
PY 2013
VL 61
IS 19
BP 7313
EP 7323
DI 10.1016/j.actamat.2013.08.037
PG 11
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 261SA
UT WOS:000327683700025
ER
PT J
AU Smith, HL
Hornbuckle, BC
Mauger, L
Fu, B
Tracy, SJ
Thompson, GB
Lucas, MS
Xiao, Y
Hu, MY
Zhao, J
Alp, EE
Fultz, B
AF Smith, Hillary L.
Hornbuckle, B. C.
Mauger, L.
Fu, B.
Tracy, S. J.
Thompson, G. B.
Lucas, M. S.
Xiao, Y.
Hu, M. Y.
Zhao, J.
Alp, E. Ercan
Fultz, B.
TI Changes in vibrational entropy during the early stages of chemical
unmixing in fcc Cu-6% Fe
SO ACTA MATERIALIA
LA English
DT Article
DE Nanocrystalline material; Microstructure formation; Vibrational entropy;
Atom probe tomography; Fe-Cu alloy
ID DENSITY-OF-STATES; NUCLEAR RESONANT SCATTERING; NANOCRYSTALLINE NI3FE;
SMALL PARTICLE; DYNAMICS; PHONONS; HEAT; IRON
AB A nanocrystalline face-centered cubic (fcc) solid solution of 6% Fe in Cu was prepared by high-energy ball milling, and annealed at temperatures from 200 to 360 degrees C to induce chemical unmixing. The chemical state of the material was characterized by three-dimensional atom probe microscopy, Mossbauer spectrometry and X-ray powder diffractometry. The unmixing was heterogeneous, with iron atoms forming iron-rich zones that thicken with further annealing. The phonon partial density of states (pDOS) of Fe-57 was measured by nuclear resonant inelastic X-ray scattering, showing the pDOS of the as-prepared material to be that of an fcc crystal. The features of this pDOS became broader in the early stages of unmixing, but only small changes in average phonon frequencies occurred until the body-centered cubic (bcc) phase began to form. The vibrational entropy calculated from the pDOS underwent little change during the early stage of annealing, but decreased rapidly when the bcc phase formed in the material. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Smith, Hillary L.; Mauger, L.; Tracy, S. J.; Fultz, B.] CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA.
[Hornbuckle, B. C.; Fu, B.; Thompson, G. B.] Univ Alabama, Dept Met & Mat Engn, Tuscaloosa, AL 35487 USA.
[Lucas, M. S.] Air Force Res Lab, Wright Patterson AFB, OH 45433 USA.
[Xiao, Y.] Carnegie Inst Sci, Geophys Lab, HPCAT, Argonne, IL 60439 USA.
[Hu, M. Y.; Zhao, J.; Alp, E. Ercan] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
RP Smith, HL (reprint author), CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA.
EM HLS@caltech.edu
OI Fu, Bianzhu/0000-0003-4085-0889
FU CIW through DOE-NNSA; CDAC through DOE-NNSA; UNLV through DOE-NNSA; LLNL
through DOE-NNSA; CIW through DOE-BES; CDAC through DOE-BES; UNLV
through DOE-BES; LLNL through DOE-BES; CIW through NSF; CDAC through
NSF; UNLV through NSF; LLNL through NSF; DOE-BES [DE-AC02-06CH11357,
DE-FG02-03ER46055]; NSF [DMR-0520547]
FX Portions of this work were performed at HPCAT (Sector 16), Advanced
Photon Source (APS), Argonne National Laboratory. HPCAT is supported by
CIW, CDAC, UNLV and LLNL through funding from DOE-NNSA, DOE-BES and NSF.
Use of the APS was supported by DOE-BES, under Contract No.
DE-AC02-06CH11357. This work benefited from DANSE software developed
under NSF Grant No. DMR-0520547. This work was supported by DOE-BES
under contract DE-FG02-03ER46055.
NR 40
TC 2
Z9 2
U1 2
U2 25
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
EI 1873-2453
J9 ACTA MATER
JI Acta Mater.
PD NOV
PY 2013
VL 61
IS 19
BP 7466
EP 7472
DI 10.1016/j.actamat.2013.08.057
PG 7
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 261SA
UT WOS:000327683700040
ER
PT J
AU Krcmar, M
Fu, CL
AF Krcmar, M.
Fu, C. L.
TI Effect of lattice anharmonicity in the structural phase transformation
of Laves phase HfV2 alloy: A first-principles investigation
SO ACTA MATERIALIA
LA English
DT Article
DE First-principles calculations; Mean-field analysis; Intermetallic Laves
phases; Phase transformations
ID AUGMENTED-WAVE METHOD; ELECTRONIC-STRUCTURE; TOTAL-ENERGY; ELASTIC
PROPERTIES; TRANSITIONS; NB; TA
AB First-principles theory was developed to study the structural phase transformations in the Laves phase HfV2 alloy. We explored the energy landscape and established the role of lattice anharmonicity underlying the structural phase transitions. Our approach is based on a phenomenological Landau theory for the structural phase transition and a mean-field approximation for the free energy. First-principles calculations were utilized to obtain the distortion energy as a function of relevant deformations, and to deduce parameters for constructing the free energy. Our result for the phase transition temperature of HfV2 is in good agreement with experiment. We find that the high-temperature cubic C15 phase is stabilized by the effect of lattice anharmonicity. The theory also predicts an anomalous increase in shear modulus with increasing temperature for systems where the anharmonicity is pronounced. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Krcmar, M.] Grand Valley State Univ, Dept Phys, Allendale, MI 49401 USA.
[Fu, C. L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.
RP Krcmar, M (reprint author), Grand Valley State Univ, Dept Phys, Allendale, MI 49401 USA.
EM krcmarm@gvsu.edu
FU Division of Materials Sciences and Engineering, Office of Basic Energy
Sciences, US Department of Energy; UT-Battelle, LLC.; National Science
Foundation [1228291]
FX This research is sponsored by the Division of Materials Sciences and
Engineering, Office of Basic Energy Sciences, US Department of Energy
under contract with UT-Battelle, LLC. Research at Grand Valley State
University (M.K.) is supported in part by National Science Foundation
grant 1228291.
NR 24
TC 1
Z9 1
U1 3
U2 17
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
EI 1873-2453
J9 ACTA MATER
JI Acta Mater.
PD NOV
PY 2013
VL 61
IS 19
BP 7473
EP 7480
DI 10.1016/j.actamat.2013.08.059
PG 8
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 261SA
UT WOS:000327683700041
ER
PT J
AU Beyerlein, IJ
Wang, J
Zhang, RF
AF Beyerlein, Irene J.
Wang, Jian
Zhang, Ruifeng
TI Mapping dislocation nucleation behavior from bimetal interfaces
SO ACTA MATERIALIA
LA English
DT Article
DE Interfaces; Nucleation; Dislocation; Nanocomposites
ID SEVERE PLASTIC-DEFORMATION; GRAIN-BOUNDARY LEDGES; CU-NB MULTILAYERS;
NANOLAMELLAR COMPOSITES; SCREW DISLOCATIONS; TWIN BOUNDARIES; PETCH
RELATION; HIGH-STRENGTH; METALS; SIMULATIONS
AB Interfaces between two dissimilar metals have been observed to exhibit a range of atomic structures, from atomically flat to atomically stepped. Using atomic-scale simulation and theory, we study the influence of the intrinsic bimetal interface structure on the nucleation of lattice dislocations. Interface structure is found to have a strong effect on which dislocations are nucleated and the type of nucleation site. We develop a theoretical model that provides criteria for predicting these effects based on key structural relationships between the interface and adjoining crystals. In recognition of these critical conditions, we construct a map that identifies the most likely nucleation site from a given interface. The theory and map developed here can guide efforts to tune interface structures for controlling the strength and deformation of heterogeneous materials. (C) 2013 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Beyerlein, Irene J.; Zhang, Ruifeng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
[Wang, Jian] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.
RP Beyerlein, IJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
EM Irene@lanl.gov
RI Beyerlein, Irene/A-4676-2011; Wang, Jian/F-2669-2012
OI Wang, Jian/0000-0001-5130-300X
FU Center for Materials at Irradiation and Mechanical Extremes; US
Department of Energy, Office of Science, Office of Basic Energy Sciences
[2008LANL1026]; National Nuclear Security Administration of the US
Department of Energy [DE-AC52-06NA25396]; Energy Frontier Research
Center
FX The authors gratefully acknowledge support by the Center for Materials
at Irradiation and Mechanical Extremes, an Energy Frontier Research
Center funded by the US Department of Energy, Office of Science, Office
of Basic Energy Sciences under Award Number 2008LANL1026. Los Alamos
National Laboratory, an affirmative action equal opportunity employer,
is operated by Los Alamos National Security, LLC, for the National
Nuclear Security Administration of the US Department of Energy under
Contract DE-AC52-06NA25396.
NR 62
TC 40
Z9 40
U1 4
U2 54
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6454
EI 1873-2453
J9 ACTA MATER
JI Acta Mater.
PD NOV
PY 2013
VL 61
IS 19
BP 7488
EP 7499
DI 10.1016/j.actamat.2013.08.061
PG 12
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering
SC Materials Science; Metallurgy & Metallurgical Engineering
GA 261SA
UT WOS:000327683700043
ER
PT J
AU Jeen, H
Bi, ZH
Choi, WS
Chisholm, MF
Bridges, CA
Paranthaman, MP
Lee, HN
AF Jeen, Hyoungjeen
Bi, Zhonghe
Choi, Woo Seok
Chisholm, Matthew F.
Bridges, Craig A.
Paranthaman, M. Parans
Lee, Ho Nyung
TI Orienting Oxygen Vacancies for Fast Catalytic Reaction
SO ADVANCED MATERIALS
LA English
DT Article
DE solid oxide fuel cells; oxygen reduction reaction; pulsed laser epitaxy;
brownmillerite; strontium cobaltite
ID FUEL-CELLS; ELECTRODES; EXCHANGE; SRCOO2.5; BROWNMILLERITE;
SPECTROSCOPY; PEROVSKITES; DIFFUSION; IMPEDANCE; DESIGN
C1 [Jeen, Hyoungjeen; Bi, Zhonghe; Choi, Woo Seok; Chisholm, Matthew F.; Bridges, Craig A.; Paranthaman, M. Parans; Lee, Ho Nyung] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Lee, HN (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
EM hnlee@ornl.gov
RI Choi, Woo Seok/G-8783-2014; Albe, Karsten/F-1139-2011; Paranthaman,
Mariappan/N-3866-2015; Lee, Ho Nyung/K-2820-2012
OI Paranthaman, Mariappan/0000-0003-3009-8531; Lee, Ho
Nyung/0000-0002-2180-3975
FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and
Engineering Division
FX The work was supported by the U.S. Department of Energy, Basic Energy
Sciences, Materials Sciences and Engineering Division.
NR 25
TC 19
Z9 19
U1 11
U2 96
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD NOV
PY 2013
VL 25
IS 44
BP 6459
EP 6463
DI 10.1002/adma.201302919
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 261VK
UT WOS:000327692500018
PM 24114810
ER
PT J
AU Baboly, MG
Su, MF
Reinke, CM
Alaie, S
Goettler, DF
El-Kady, I
Leseman, ZC
AF Baboly, M. Ghasemi
Su, M. F.
Reinke, C. M.
Alaie, S.
Goettler, D. F.
El-Kady, I.
Leseman, Z. C.
TI The effect of stiffness and mass on coupled oscillations in a phononic
crystal
SO AIP ADVANCES
LA English
DT Article
AB Insight into phononic bandgap formation is presented using a first principles-type approach where phononic lattices are treated as coupled oscillators connected via massless tethers. The stiffness of the tethers and the mass of the oscillator are varied and their influences on the bandgap formation are deduced. This analysis is reinforced by conducting numerical simulations to examine the modes bounding the bandgap and highlighting the effect of the above parameters. The analysis presented here not only sheds light on the origins of gap formation, but also allows one to define design rules for wide phononic gaps and maximum gap-to-midgap ratios. (c) 2013 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License.
C1 [Baboly, M. Ghasemi; Su, M. F.; Alaie, S.; Goettler, D. F.; Leseman, Z. C.] Univ New Mexico, Dept Mech Engn, Albuquerque, NM 87131 USA.
[Reinke, C. M.; El-Kady, I.] Sandia Natl Labs, Dept Adv Photon Microsyst, Albuquerque, NM 87185 USA.
RP Leseman, ZC (reprint author), Univ New Mexico, Dept Mech Engn, Albuquerque, NM 87131 USA.
EM zleseman@unm.edu
OI alaie, seyedhamidreza/0000-0001-6359-297X
FU National Science Foundation Division of CMMI [1056077]; U.S. Department
of Energy's National Nuclear Security Administration [AC04-94AL85000]
FX This work was supported by the National Science Foundation Division of
CMMI under Award 1056077. Sandia National Laboratories is a
multi-program laboratory managed and operated by Sandia Corporation, a
wholly owned subsidiary of Lockheed Martin Corporation, for the U.S.
Department of Energy's National Nuclear Security Administration under
contract DE-AC04-94AL85000.
NR 16
TC 3
Z9 3
U1 1
U2 11
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 2158-3226
J9 AIP ADV
JI AIP Adv.
PD NOV
PY 2013
VL 3
IS 11
AR 112121
DI 10.1063/1.4834335
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 261WJ
UT WOS:000327695000021
ER
PT J
AU Shell, SM
Hawkins, EK
Tsai, MS
Hlaing, AS
Rizzo, CJ
Chazin, WJ
AF Shell, Steven M.
Hawkins, Edward K.
Tsai, Miaw-Sheue
Hlaing, Aye Su
Rizzo, Carmelo J.
Chazin, Walter J.
TI Xeroderma pigmentosum complementation group C protein (XPC) serves as a
general sensor of damaged DNA
SO DNA REPAIR
LA English
DT Article
DE XPC; Nucleotide excision repair; Base excision repair; Lesion
recognition; DNA binding; High-throughput assay
ID NUCLEOTIDE EXCISION-REPAIR; SITE-SPECIFIC SYNTHESIS; IN-VITRO;
MOLECULAR-MECHANISMS; COMPLEX; RECOGNITION; ADDUCTS; OLIGONUCLEOTIDES;
BINDING; LESIONS
AB The Xeroderma pigmentosum complementation group C protein (XPC) serves as the primary initiating factor in the global genome nucleotide excision repair pathway (GG-NER). Recent reports suggest XPC also stimulates repair of oxidative lesions by base excision repair. However, whether XPC distinguishes among various types of DNA lesions remains unclear. Although the DNA binding properties of XPC have been studied by several groups, there is a lack of consensus over whether XPC discriminates between DNA damaged by lesions associated with NER activity versus those that are not. In this study we report a high-throughput fluorescence anisotropy assay used to measure the DNA binding affinity of XPC for a panel of DNA substrates containing a range of chemical lesions in a common sequence. Our results demonstrate that while XPC displays a preference for binding damaged DNA, the identity of the lesion has little effect on the binding affinity of XPC. Moreover, XPC was equally capable of binding to DNA substrates containing lesions not repaired by GG-NER. Our results suggest XPC may act as a general sensor of damaged DNA that is capable of recognizing DNA containing lesions not repaired by NER. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Shell, Steven M.; Chazin, Walter J.] Vanderbilt Univ, Ctr Mol Toxicol, Struct Biol Ctr, Dept Biochem, Nashville, TN 37232 USA.
[Shell, Steven M.; Hawkins, Edward K.; Rizzo, Carmelo J.; Chazin, Walter J.] Vanderbilt Univ, Vanderbilt Ingram Canc Ctr, Nashville, TN 37232 USA.
[Hawkins, Edward K.; Rizzo, Carmelo J.; Chazin, Walter J.] Vanderbilt Univ, Ctr Mol Toxicol, Dept Chem, Nashville, TN 37232 USA.
[Tsai, Miaw-Sheue; Hlaing, Aye Su] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
RP Chazin, WJ (reprint author), 465 21st Ave South,BIOSCI MRB 3,Suite 5140, Nashville, TN 37232 USA.
EM walter.j.chazin@vanderbilt.edu
FU NIH [R01 ES016561, P01 CA092584, P30 ES00267, P30 CA068485]; American
Cancer Society [119569-PF-11-271-01-DMC]; [T32 ES07028]
FX The authors wish to acknowledge Dan Dorset of the Vanderbilt University
High-throughput Screening Core Facility for his assistance with the
automated liquid handling system used in this study. This work was
supported by NIH grants R01 ES016561 (to CJR, WJC), P01 CA092584 (to
John A. Tainer), P30 ES00267 (to the Vanderbilt Center in Molecular
Toxicology), and P30 CA068485 (to the Vanderbilt-Ingram Cancer Center).
E.K.H. and S.M.S were provided pre- and post-doctoral support from
training grant T32 ES07028. S.M.S is supported by postdoctoral
fellowship 119569-PF-11-271-01-DMC from the American Cancer Society.
NR 52
TC 18
Z9 19
U1 1
U2 5
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1568-7864
EI 1568-7856
J9 DNA REPAIR
JI DNA Repair
PD NOV
PY 2013
VL 12
IS 11
BP 947
EP 953
DI 10.1016/j.dnarep.2013.08.013
PG 7
WC Genetics & Heredity; Toxicology
SC Genetics & Heredity; Toxicology
GA 260FA
UT WOS:000327579200010
PM 24051049
ER
PT J
AU Kroposki, B
Sen, PK
Malmedal, K
AF Kroposki, Benjamin
Sen, Pankaj K.
Malmedal, Keith
TI Optimum Sizing and Placement of Distributed and Renewable Energy Sources
in Electric Power Distribution Systems
SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS
LA English
DT Article; Proceedings Paper
CT 44th Annual Meeting of the IEEE-Industry-Applications-Society
CY OCT 04-08, 2009
CL Houston, TX
SP IEEE Ind Applicat Soc
DE Distributed energy resources (DERs); distributed generation;
distribution system; optimization; storage
AB Concerns with climate change, requirements for the renewable portfolio standards, government incentives, and lowering cost of renewable and distributed energy resources (DERs) are some of the driving forces for the steeper growth in DER installations. DERs are commonly connected near the load in electric power distribution systems and include renewable energy sources such as wind and solar, fossil-fuel-based generation such as microturbines, and other distributed energy storage elements. A novel methodology is developed in this paper that optimizes the sizing and placement of DER on electrical distribution feeders based on both technical and economic considerations and tested on the IEEE 34-bus system.
C1 [Kroposki, Benjamin] Natl Renewable Energy Lab, Distributed Energy Syst Integrat Grp, Golden, CO 80401 USA.
[Sen, Pankaj K.] Colorado Sch Mines, Power Syst Engn Res Ctr PSerc, Golden, CO 80401 USA.
[Malmedal, Keith] NEI Elect Power Engn Inc, Arvada, CO 80001 USA.
[Malmedal, Keith] Univ Colorado, Denver, CO 80217 USA.
RP Kroposki, B (reprint author), Natl Renewable Energy Lab, Distributed Energy Syst Integrat Grp, Golden, CO 80401 USA.
EM Benjamin.kroposki@nrel.gov; psen@mines.edu; kmalmedal@neiengineering.com
NR 16
TC 7
Z9 7
U1 4
U2 19
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0093-9994
EI 1939-9367
J9 IEEE T IND APPL
JI IEEE Trans. Ind. Appl.
PD NOV-DEC
PY 2013
VL 49
IS 6
BP 2741
EP 2752
DI 10.1109/TIA.2013.2262661
PG 12
WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic
SC Engineering
GA 259UT
UT WOS:000327552500042
ER
PT J
AU Kroposki, B
Sen, PK
Malmedal, K
AF Kroposki, Benjamin
Sen, Pankaj K.
Malmedal, Keith
TI Selection of Distribution Feeders for Implementing Distributed
Generation and Renewable Energy Applications
SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS
LA English
DT Article; Proceedings Paper
CT 53rd Annual IEEE Rural Electric Power Conference
CY APR 26-29, 2009
CL Fort Collins, CO
SP IEEE
DE Distributed energy resources (DERs); distributed generation; distributed
storage; distribution feeder; distribution system; optimization
ID INTEGRATING PHOTOVOLTAICS; DISTRIBUTION-SYSTEMS; UTILITY; LOSSES; IMPACT
AB Climate change concerns mandated renewable portfolio standards, lucrative government incentives, and accelerated cost reduction in renewables, and distributed energy applications are driving steep growth in system installations. Distributed energy resources (DERs) are not commonly connected to a bulk power transmission system but are interconnected near the load in the electric power distribution system. DER includes renewable energy such as wind and solar, fossil-fuel-based generation (micro-turbines and small gas turbines), and distributed energy storage. In this paper, a novel methodology is developed that ranks utility feeders for implementation of DER systems. This performance index is based on peak-load reduction, increased system capacity, load-generation correlation, and feeder load growth. This is based on a statistical measure that quantifies the relationship between loads and the stochastic nature of renewable resources. This allows the utility to gain insight into improved benefits from nondispatchable renewable resources such as solar and wind technologies as well as dispatchable DER technologies.
C1 [Kroposki, Benjamin] Natl Renewable Energy Lab, Distributed Energy Syst Integrat Grp, Golden, CO 80401 USA.
[Sen, Pankaj K.] Colorado Sch Mines, Div Engn, Golden, CO 80401 USA.
[Malmedal, Keith] NEI Elect Power Engn Inc, Arvada, CO 80001 USA.
RP Kroposki, B (reprint author), Natl Renewable Energy Lab, Distributed Energy Syst Integrat Grp, Golden, CO 80401 USA.
EM Benjamin.kroposki@nrel.gov; psen@mines.edu; kmalmedal@neiengineering.com
NR 26
TC 4
Z9 4
U1 0
U2 15
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0093-9994
EI 1939-9367
J9 IEEE T IND APPL
JI IEEE Trans. Ind. Appl.
PD NOV-DEC
PY 2013
VL 49
IS 6
BP 2825
EP 2834
DI 10.1109/TIA.2013.2262091
PG 10
WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic
SC Engineering
GA 259UT
UT WOS:000327552500051
ER
PT J
AU Ramani, S
Reiten, MT
Colestock, PL
Taylor, AJ
Azad, AK
O'Hara, JF
AF Ramani, Suchitra
Reiten, Matthew T.
Colestock, Patrick L.
Taylor, Antoinette J.
Azad, Abul K.
O'Hara, John F.
TI Electromagnetic Response of Finite Terahertz Metafilm Arrays Excited on
Total Internal Reflection Boundaries
SO IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY
LA English
DT Article
DE Attenuated total reflection (ATR); diffraction; metamaterials;
reflection; spectroscopy; surface wave; terahertz; time domain
ID SURFACE-PLASMONS; WAVES; METAMATERIALS; SPECTROSCOPY; PULSES; EDGE
AB Resonant excitation of planar terahertz metamaterials using attenuated total reflection is demonstrated. Experimental results reveal an anomalous increase in the resonance strength while the sample is illuminated near the edge of the metamaterial array with a finite-size terahertz beam. A re-radiation signal at the fundamental metamaterial resonance is observed on the transmission side of the total internal reflection interface where no signal was expected. Multiple theoretical approaches address the physical origins of this re-radiation signal and rich behavior has been simulated with numeric simulations. Although models indicate that surface waves could exist, radiation coupled across the total internal reflection surface appears predominately mediated by finite currents oscillating in resonators at the edge of the metafilm array. The observations could lead to a better understanding of boundary effects in finite, planar metamaterials and more accurate modeling of MM-mediated total reflection spectroscopy.
C1 [Ramani, Suchitra; O'Hara, John F.] Oklahoma State Univ, Dept Elect & Comp Engn, Stillwater, OK 74078 USA.
[Ramani, Suchitra; Azad, Abul K.] Los Alamos Natl Lab, MPA CINT, Los Alamos, NM 87545 USA.
[Reiten, Matthew T.] Los Alamos Natl Lab, AOT HPE, Los Alamos, NM 87545 USA.
[Colestock, Patrick L.] Los Alamos Natl Lab, ISR 2, Los Alamos, NM 87545 USA.
[Taylor, Antoinette J.] Los Alamos Natl Lab, MPA DO, Los Alamos, NM 87545 USA.
[O'Hara, John F.] Wavetech LLC, Perry, OK 73077 USA.
RP Ramani, S (reprint author), Oklahoma State Univ, Dept Elect & Comp Engn, Stillwater, OK 74078 USA.
EM s.ramani@okstate.edu; mtreiten@lanl.gov; colestoc@lanl.gov;
ttaylor@lanl.gov; aazad@lanl.gov; oharaj@okstate.edu
OI Azad, Abul/0000-0002-7784-7432
FU Los Alamos National Laboratory LDRD Program; National Nuclear Security
Administration of the U.S. Department of Energy [DE-AC52-06NA25396]
FX This work was supported by the Los Alamos National Laboratory LDRD
Program. This work was performed, in part, at the Center for Integrated
Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy
Sciences Nanoscale Science Research Center operated jointly by Los
Alamos and Sandia National Laboratories. Los Alamos National Laboratory,
an affirmative action/equal opportunity employer, is operated by Los
Alamos National Security, LLC, for the National Nuclear Security
Administration of the U.S. Department of Energy under Contract
DE-AC52-06NA25396.
NR 32
TC 0
Z9 0
U1 0
U2 7
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 2156-342X
J9 IEEE T THZ SCI TECHN
JI IEEE Trans. Terahertz Sci. Technol.
PD NOV
PY 2013
VL 3
IS 6
SI SI
BP 709
EP 720
DI 10.1109/TTHZ.2013.2284858
PG 12
WC Engineering, Electrical & Electronic; Optics; Physics, Applied
SC Engineering; Optics; Physics
GA 262GZ
UT WOS:000327723600008
ER
PT J
AU Chowdhury, DR
Azad, AK
Zhang, WL
Singh, R
AF Chowdhury, Dibakar Roy
Azad, Abul K.
Zhang, Weili
Singh, Ranjan
TI Near Field Coupling in Passive and Active Terahertz Metamaterial Devices
SO IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY
LA English
DT Article
DE Near fields; coupling; metamaterials; plasmonics; terahertz; ultrafast;
silicon
ID SPLIT-RING RESONATORS; NEGATIVE-INDEX; ARRAYS
AB A wide variety of optical phenomena rely on the near field manipulation and confinement of electromagnetic field in subwavelength metallic and dielectric resonators with applications ranging from the design of micro and nano scale photonic devices to super lenses and ultrasensitive sensors. In this invited paper, we present a discussion on controlling the metamaterial properties by active and passive manipulation of near field coupling in an array of split ring resonators. We show that near field coupling between the meta-atoms could lead to resonance tuning, mode splitting, and ultrafast switching in passive and active resonators. The near field coupling schemes discussed here demonstrate the application possibilities of such structures towards the design of active switches, amplitude modulators, frequency agile behaviors, and slow light devices, particularly for the terahertz frequency regime, which still suffers from the shortage of practical devices required to bridge the so called "THz gap."
C1 [Chowdhury, Dibakar Roy] Australian Natl Univ, Coll Engn & Comp Sci, Ctr Sustainable Energy Syst, Canberra, ACT 0200, Australia.
[Azad, Abul K.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
[Zhang, Weili] Oklahoma State Univ, Sch Elect & Comp Engn, Stillwater, OK 74078 USA.
[Singh, Ranjan] Nanyang Technol Univ, Ctr Disrupt Photon Technol, Singapore 639798, Singapore.
RP Chowdhury, DR (reprint author), Australian Natl Univ, Coll Engn & Comp Sci, Ctr Sustainable Energy Syst, Canberra, ACT 0200, Australia.
EM dibakarrc@gmail.com; ranjans@ntu.edu.sg
RI Singh, Ranjan/B-4091-2010; Zhang, Weili/C-5416-2011;
OI Singh, Ranjan/0000-0001-8068-7428; Zhang, Weili/0000-0002-8591-0200;
Azad, Abul/0000-0002-7784-7432
FU U.S. National Science Foundation (NSF)
FX This work was supported in part by the U.S. National Science Foundation
(NSF).
NR 51
TC 12
Z9 12
U1 5
U2 55
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 2156-342X
J9 IEEE T THZ SCI TECHN
JI IEEE Trans. Terahertz Sci. Technol.
PD NOV
PY 2013
VL 3
IS 6
SI SI
BP 783
EP 790
DI 10.1109/TTHZ.2013.2285569
PG 8
WC Engineering, Electrical & Electronic; Optics; Physics, Applied
SC Engineering; Optics; Physics
GA 262GZ
UT WOS:000327723600016
ER
PT J
AU Mitri, FG
AF Mitri, F. G.
TI Comment on "Effects of Multi-Scattering on the Performance of a
Single-Beam Acoustic Manipulation Device"
SO IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL
LA English
DT Editorial Material
ID RADIATION FORCE; RIGID SPHERE; BESSEL BEAM; FLUID
AB The concern addressed in the present commentary is to point out the omission of the azimuthal component F-phi of the axial acoustic radiation force provided in M. Az-arpeyvand, M. A. Alibakhshi, R. Self, "Effects of multi-scattering on the performance of a single-beam acoustic manipulation device,"IEEE Trans. Ultrason. Ferroelectr. Freq. Control, vol. 59, no. 8, pp. 1741-1749, 2012, which may suggest a miscalculation of the radiation force function Y-m and its related numerical computations.
C1 Los Alamos Natl Lab, Acoust & Sensors Technol Team, Los Alamos, NM 87545 USA.
RP Mitri, FG (reprint author), Los Alamos Natl Lab, Acoust & Sensors Technol Team, MPA 11,MS D429, Los Alamos, NM 87545 USA.
EM mitri@lanl.gov
NR 11
TC 0
Z9 0
U1 1
U2 10
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0885-3010
EI 1525-8955
J9 IEEE T ULTRASON FERR
JI IEEE Trans. Ultrason. Ferroelectr. Freq. Control
PD NOV
PY 2013
VL 60
IS 11
BP 2235
EP 2236
DI 10.1109/TUFFC.2013.2821
PG 2
WC Acoustics; Engineering, Electrical & Electronic
SC Acoustics; Engineering
GA 262JC
UT WOS:000327729700001
PM 24158280
ER
PT J
AU Caridade, M
Oliveira, VG
Agua-Doce, A
Graca, L
Ribeiro, RM
AF Caridade, Marta
Oliveira, Vanessa G.
Agua-Doce, Ana
Graca, Luis
Ribeiro, Ruy M.
TI The fate of CD4(+) T cells under tolerance-inducing stimulation: a
modeling perspective
SO IMMUNOLOGY AND CELL BIOLOGY
LA English
DT Article
DE anti-CD4; foxp3; immune tolerance; mathematical modeling; proliferation
kinetics
ID EXPERIMENTAL AUTOIMMUNE ENCEPHALOMYELITIS; INFECTIOUS TRANSPLANTATION
TOLERANCE; NONDEPLETING ANTI-CD4; CFSE DATA; LYMPHOCYTE DIVISION;
TRANSGENIC MICE; CLONAL DELETION; IN-VIVO; INDUCTION; ANTIBODIES
AB Non-depleting anti-CD4 monoclonal antibodies (MAbs) induce long-term dominant tolerance mediated by regulatory T cells in several animal models of transplantation, allergy and autoimmunity. However, despite many studies on tolerance induction following CD4 blockade, the consequences of this intervention on T-cell kinetics are still unknown. Mathematical models have been useful to understand lymphocyte dynamics, estimating rates of proliferation and cell death following an intervention. Using the same strategy, we found that CD4(+) T cells activated in vitro in the presence of non-depleting anti-CD4 MAbs are prevented from undergoing optimal proliferation and show a higher frequency of apoptosis. Although the changes are small, during the course of a proliferative response, they lead to very distinct final levels of cell numbers. The importance of these mechanisms, predicted by the mathematical model, was validated by showing that lck-driven Bcl-x(L) transgenic mice, bearing T cells resistant to apoptosis, fail to become tolerant to skin grafts following CD4-blockade. Our data show that, in addition to induction of regulatory T cells, CD4 blockade has a marked effect in the effector T-cell pool by the combined action of hindering proliferation while favoring apoptosis. It is, therefore, the combination of all those mechanisms that leads to stable tolerance.
C1 [Caridade, Marta; Oliveira, Vanessa G.; Agua-Doce, Ana; Graca, Luis; Ribeiro, Ruy M.] Univ Lisbon, Fac Med, Inst Mol Med, P-1649028 Lisbon, Portugal.
[Caridade, Marta; Oliveira, Vanessa G.; Agua-Doce, Ana; Graca, Luis] Gulbenkian Inst Sci, Oeiras, Portugal.
[Ribeiro, Ruy M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Graca, L (reprint author), Univ Lisbon, Fac Med, Inst Mol Med, Ave Prof Egas Moniz, P-1649028 Lisbon, Portugal.
EM lgraca@fm.ul.pt; ruy@lanl.gov
RI Graca, Luis/B-8887-2008; Caridade, Marta/L-5045-2013; Agua-Doce,
Ana/L-2997-2014;
OI Graca, Luis/0000-0001-6935-8500; Caridade, Marta/0000-0001-5294-1329;
Goncalves de Oliveira, Vanessa Alexandra/0000-0001-6884-2675; Agua-Doce,
Ana/0000-0002-0466-7297; Ribeiro, Ruy/0000-0002-3988-8241
FU Fundacao para a Ciencia e Tecnologia, Portugal [PIC/IC/82895/2007,
PTDC/SAU-TOX/114424/2009]; European Union [PCOFUND-GA-2009-246542];
Fundacao para a Ciencia e Tecnologia, Portugal
FX This work was funded by grants number PIC/IC/82895/2007 and
PTDC/SAU-TOX/114424/2009 from Fundacao para a Ciencia e Tecnologia,
Portugal (to Luis Graca). Ruy M Ribeiro has received funding from the
European Union 7th Framework Program under grant no
PCOFUND-GA-2009-246542 and from Fundacao para a Ciencia e Tecnologia,
Portugal.
NR 45
TC 1
Z9 1
U1 2
U2 6
PU NATURE PUBLISHING GROUP
PI NEW YORK
PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA
SN 0818-9641
EI 1440-1711
J9 IMMUNOL CELL BIOL
JI Immunol. Cell Biol.
PD NOV-DEC
PY 2013
VL 91
IS 10
BP 652
EP 660
DI 10.1038/icb.2013.63
PG 9
WC Cell Biology; Immunology
SC Cell Biology; Immunology
GA 260FT
UT WOS:000327581100010
PM 24145855
ER
PT J
AU Liu, J
Ru, P
Zhang, WN
Wong, CY
AF Liu, Jie
Ru, Peng
Zhang, Wei-Ning
Wong, Cheuk-Yin
TI CHAOTIC PARAMETER lambda IN HANBURY-BROWN-TWISS INTERFEROMETRY IN AN
ANISOTROPIC BOSON GAS MODEL
SO INTERNATIONAL JOURNAL OF MODERN PHYSICS E-NUCLEAR PHYSICS
LA English
DT Article
DE Chaotic parameter; Bose-Einstein condensation; two-pion interferometry;
high energy heavy-ion collisions
ID HEAVY-ION COLLISIONS
AB Using and two-body density matrices, we calculate the spatial and momentum distributions, two-particle Hanbury-Brown-Twiss (HBT) correlation functions, and the chaotic parameter lambda in HBT interferometry for the systems of boson gas within the harmonic oscillator potentials with anisotropic frequencies in transverse and longitudinal directions. The HBT chaotic parameter, which can be obtained by measuring the correlation functions at zero relative momentum of the particle pair, is related to the degree of Bose-Einstein condensation and thus the system environment. We investigate the effects of system temperature, particle number and the average momentum of the particle pair on the chaotic parameter. The value of lambda decreases with the condensed fraction, f(0). It is one for f(0) = 0 and zero for f(0) = 1. For a certain f(0) between 0 and 1, we find that lambda increases with the average momentum of the particle pair and decreases with the particle number of system. The results of lambda are sensitive to the ratio, nu = w(z)/w(rho), of the frequencies in longitudinal and transverse directions. They are smaller for larger nu when w(rho), is fixed. In the heavy-ion collisions at the Large Hadron Collider (LHC) energy the large identical pion multiplicity may possibly lead to a considerable Bose-Einstein condensation. Its effect on the chaotic parameter in two-pion interferometry is worth considering in earnest.
C1 [Liu, Jie; Ru, Peng; Zhang, Wei-Ning] Dalian Univ Technol, Sch Phys & Optoelect Technol, Dalian 116024, Liaoning, Peoples R China.
[Zhang, Wei-Ning] Harbin Inst Technol, Dept Phys, Harbin 150006, Heilongjiang, Peoples R China.
[Wong, Cheuk-Yin] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA.
RP Zhang, WN (reprint author), Dalian Univ Technol, Sch Phys & Optoelect Technol, Dalian 116024, Liaoning, Peoples R China.
EM wnzhang@dlut.edu.cn; wongc@ornl.gov
FU National Natural Science Foundation of China [11075027, 11275037]
FX This research was supported by the National Natural Science Foundation
of China under Grant Nos. 11075027 and 11275037.
NR 19
TC 2
Z9 2
U1 0
U2 1
PU WORLD SCIENTIFIC PUBL CO PTE LTD
PI SINGAPORE
PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE
SN 0218-3013
EI 1793-6608
J9 INT J MOD PHYS E
JI Int. J. Mod. Phys. E-Nucl. Phys.
PD NOV
PY 2013
VL 22
IS 11
AR 1350083
DI 10.1142/S0218301313500833
PG 25
WC Physics, Nuclear; Physics, Particles & Fields
SC Physics
GA 264BA
UT WOS:000327850700008
ER
PT J
AU Holden, NE
Coplen, TB
AF Holden, Norman E.
Coplen, Tyler B.
TI ConfChem Conference on A Virtual Colloquium to Sustain and Celebrate IYC
2011 Initiatives in Global Chemical Education: The IUPAC Periodic Table
of Isotopes for the Educational Community
SO JOURNAL OF CHEMICAL EDUCATION
LA English
DT Article
DE Continuing Education; General Public; Inorganic Chemistry; Public
Understanding/Outreach; Isotopes; Nuclear Radiochemistry;
Periodicity/Periodic Table
AB The IUPAC Periodic Table of the Isotopes (www.ciaaw.org) was prepared as an educational outreach effort to expose teachers, students, and the general public to the existence of both stable and radioactive isotopes of the chemical elements. This Table provides information on the isotopes of each element, including the mass number and fraction of each isotope in a stable or a long-lived radioactive chemical element. These data allow scientists to determine the atomic weight of each element, which connects the microscopic and the macroscopic worlds. For many elements, there is a variation in the fraction of an element's isotopes in naturally occurring substances. The atomic weight is variable beyond its measurement uncertainty and the upper and lower bounds of the standard atomic weight are presented as an interval, rather than as a value with uncertainty, for 10 elements. The Table provides examples of the importance of both the stable and radioactive isotopes in our everyday world because of the variability of the stable isotope ratios or the radioactive decay of the unstable isotopes. There are 440 examples of applications to our everyday life. Applications, such as medical, industrial, geo-chronological, earth and planetary science, biological and forensic science, and anthropological are shown. Readers of the conference paper responded with questions, and the answers to the questions are included. This communication summarizes one of the invited papers to the ConfChem online conference A Virtual Colloquium to Sustain and Celebrate IYC 2011 Initiates in Global Chemistry Education held from May 18 to June 28, 2012, and jointly hosted by the ACS DivCHED Committee on Computers in Chemical Education and the IUPAC Committee on Chemistry Education.
C1 [Holden, Norman E.] Brookhaven Natl Lab, Upton, NY 11973 USA.
[Coplen, Tyler B.] US Geol Survey, Reston, VA 20192 USA.
RP Holden, NE (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.
EM holden@bnl.gov
NR 0
TC 1
Z9 1
U1 0
U2 10
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0021-9584
EI 1938-1328
J9 J CHEM EDUC
JI J. Chem. Educ.
PD NOV
PY 2013
VL 90
IS 11
BP 1550
EP 1551
DI 10.1021/ed3008236
PG 2
WC Chemistry, Multidisciplinary; Education, Scientific Disciplines
SC Chemistry; Education & Educational Research
GA 262PE
UT WOS:000327747900033
ER
PT J
AU Kim, D
Schweiger, MJ
AF Kim, Dongsang
Schweiger, Michael J.
TI Incorporation and distribution of rhenium in a borosilicate glass melt
heat treated in a sealed ampoule
SO JOURNAL OF NON-CRYSTALLINE SOLIDS
LA English
DT Article
DE Rhenium; Technetium; Solubility; Low-activity waste; Borosilicate glass
AB We investigated a mass balance of rhenium (used as a surrogate for technetium-99) in a borosilicate glass that was mixed with excess Re source (KReO4) beyond its solubility and heat treated in a vacuum-sealed fused silica ampoule. Distribution of Re in the bulk of the glass, in a salt phase formed on the melt surface, and in condensate material deposited on the ampoule wall was evaluated to understand the Re migration into different phases during the reaction between the molten glass and KReO4. The information gained from this study will contribute to an effort to understand the mechanism of technetium retention in, or escape from, glass melt during early stages of glass batch melting, which is a goal of the present series of studies. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Kim, Dongsang; Schweiger, Michael J.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Kim, D (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA.
EM dongsang.kim@pnnl.gov
FU U.S. Department of Energy's Waste Treatment and Immobilization Plant
Federal Project Office; U.S. Department of Energy [DE-AC05-76RL01830]
FX This work was supported by the U.S. Department of Energy's Waste
Treatment and Immobilization Plant Federal Project Office under the
direction of Dr. Albert A. Kruger. The authors greatly appreciate Dr.
John McCloy for his helpful suggestions. Pacific Northwest National
Laboratory is operated by Battelle Memorial Institute for the U.S.
Department of Energy under contract DE-AC05-76RL01830.
NR 9
TC 2
Z9 2
U1 1
U2 7
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0022-3093
EI 1873-4812
J9 J NON-CRYST SOLIDS
JI J. Non-Cryst. Solids
PD NOV 1
PY 2013
VL 379
BP 123
EP 126
DI 10.1016/j.jnoncrysol.2013.07.031
PG 4
WC Materials Science, Ceramics; Materials Science, Multidisciplinary
SC Materials Science
GA 260DG
UT WOS:000327574600017
ER
PT J
AU Leggett, CJ
Jensen, MP
AF Leggett, Christina J.
Jensen, Mark P.
TI Studies of Size-Based Selectivity in Aqueous Ternary Complexes of
Americium(III) or Lanthanide(III) Cations
SO JOURNAL OF SOLUTION CHEMISTRY
LA English
DT Article
DE Ternary complexes; Thermodynamics; Americium; Lanthanides; Calorimetry
ID MIXED-LIGAND COMPLEXES; DICARBOXYLIC-ACIDS; STABILITY-CONSTANTS;
SINGLE-CRYSTAL; RARE-EARTHS; F-ELEMENTS; THERMODYNAMICS; LUMINESCENCE;
EDTA; AM3+
AB Spectrophotometric and calorimetric titrations were used to determine the equilibrium constants (log(10) K (111)) and enthalpies of formation (Delta H (111)) for aqueous ternary complexes of the form M(L-a)(L-b) (M = Nd3+, Sm3+, Tb3+, Ho3+, Er3+, or Am3+; L-a = DTPA(5-), DO3A(3-), or CDTA(4-); L-b = oxalate (Ox), malonate (Mal), or iminodiacetate (IDA)). Inner-sphere ternary complexes were readily formed with the septadentate DO3A (1,4,7,10-tetraazacyclododecane-1,4,7-triacetic acid) and hexadentate CDTA (trans-1,2-diaminocyclohexanetetraacetic acid) ligands, whose binary complexes have residual metal-coordinated water molecules that are readily displaced by the smaller secondary ligands. The stability constants for the formation of lanthanide-CDTA complexes with Ox, Mal, and IDA generally increase with decreasing ionic radius when steric hindrance is minimal, with the trend in the M(CDTA)(-) formation constants overshadowing any size-based reversal in the stepwise ternary complexation constants. Similar ternary complexes with DO3A showed little increase in thermodynamic stability compared to analogous CDTA complexes and no preference for larger Ln cations. The octadentate DTPA (diethylenetriaminepentaacetic acid) ligand proved too large to form ternary complexes to a measurable extent with any of the secondary ligands investigated, despite the presence of one residual inner sphere water molecule.
C1 [Leggett, Christina J.; Jensen, Mark P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
[Leggett, Christina J.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA.
RP Jensen, MP (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM mjensen@anl.gov
RI Jensen, Mark/G-9131-2012
OI Jensen, Mark/0000-0003-4494-6693
FU U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research
and Development Program [DE-AC0206CH11357]; U.S. DOE Office of Civilian
Radioactive Waste Management Fellowship
FX Work supported by the U.S. Department of Energy, Assistant Secretary of
the Office of Nuclear Energy, Fuel Cycle Research and Development
Program, under contract number DE-AC0206CH11357. C.J.L. acknowledges
support by a U.S. DOE Office of Civilian Radioactive Waste Management
Fellowship.
NR 38
TC 4
Z9 4
U1 1
U2 16
PU SPRINGER/PLENUM PUBLISHERS
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 0095-9782
EI 1572-8927
J9 J SOLUTION CHEM
JI J. Solut. Chem.
PD NOV
PY 2013
VL 42
IS 11
BP 2119
EP 2136
DI 10.1007/s10953-013-0098-3
PG 18
WC Chemistry, Physical
SC Chemistry
GA 264FD
UT WOS:000327861500004
ER
PT J
AU Benz, A
Campione, S
Liu, S
Montano, I
Klem, JF
Allerman, A
Wendt, JR
Sinclair, MB
Capolino, F
Brener, I
AF Benz, A.
Campione, S.
Liu, S.
Montano, I.
Klem, J. F.
Allerman, A.
Wendt, J. R.
Sinclair, M. B.
Capolino, F.
Brener, I.
TI Strong coupling in the sub-wavelength limit using metamaterial
nanocavities
SO NATURE COMMUNICATIONS
LA English
DT Article
ID SEMICONDUCTOR QUANTUM-WELLS; ELECTROMAGNETIC ENERGY; INTERSUBBAND;
REFRACTION; EMISSION; CRYSTAL
AB The interaction between cavity modes and optical transitions leads to new coupled light-matter states in which the energy is periodically exchanged between the matter states and the optical mode. Here we present experimental evidence of optical strong coupling between modes of individual sub-wavelength metamaterial nanocavities and engineered optical transitions in semiconductor heterostructures. We show that this behaviour is generic by extending the results from the mid-infrared (similar to 10 mu m) to the near-infrared (similar to 1.5 mu m). Using mid-infrared structures, we demonstrate that the light-matter coupling occurs at the single resonator level and with extremely small interaction volumes. We calculate a mode volume of 4.9 x 10(-4) (lambda/n)(3) from which we infer that only similar to 2,400 electrons per resonator participate in this energy exchange process.
C1 [Benz, A.; Liu, S.; Brener, I.] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA.
[Benz, A.; Liu, S.; Montano, I.; Klem, J. F.; Allerman, A.; Wendt, J. R.; Sinclair, M. B.; Brener, I.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Campione, S.; Capolino, F.] Univ Calif Irvine, Dept Elect Engn & Comp Sci, Irvine, CA 92697 USA.
RP Benz, A (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, POB 5800, Albuquerque, NM 87185 USA.
EM anbenz@sandia.gov; ibrener@sandia.gov
RI Liu, Sheng/P-6029-2014; Campione, Salvatore/A-2349-2015
OI Liu, Sheng/0000-0003-0967-4514; Campione, Salvatore/0000-0003-4655-5485
FU Laboratory Directed Research and Development program at Sandia National
Laboratories; US Department of Energy's National Nuclear Security
Administration [DE-AC04-94AL85000]
FX This work was performed, in part, at the Center for Integrated
Nanotechnologies, a US Department of Energy, Office of Basic Energy
Sciences user facility. Portions of this work were supported by the
Laboratory Directed Research and Development program at Sandia National
Laboratories. Sandia National Laboratories is a multi-program laboratory
managed and operated by Sandia Corporation, a wholly owned subsidiary of
Lockheed Martin Corporation, for the US Department of Energy's National
Nuclear Security Administration under contract DE-AC04-94AL85000.
NR 42
TC 39
Z9 39
U1 5
U2 48
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2882
DI 10.1038/ncomms3882
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266NI
UT WOS:000328030400001
PM 24287692
ER
PT J
AU Fang, L
Jia, Y
Mishra, V
Chaparro, C
Vlasko-Vlasov, VK
Koshelev, AE
Welp, U
Crabtree, GW
Zhu, S
Zhigadlo, ND
Katrych, S
Karpinski, J
Kwok, WK
AF Fang, L.
Jia, Y.
Mishra, V.
Chaparro, C.
Vlasko-Vlasov, V. K.
Koshelev, A. E.
Welp, U.
Crabtree, G. W.
Zhu, S.
Zhigadlo, N. D.
Katrych, S.
Karpinski, J.
Kwok, W. K.
TI Huge critical current density and tailored superconducting anisotropy in
SmFeAsO0.8F0.15 by low-density columnar-defect incorporation
SO NATURE COMMUNICATIONS
LA English
DT Article
ID PNICTIDE SUPERCONDUCTORS; MAGNETIZATION; CONDUCTORS; CRYSTALS
AB Iron-based superconductors could be useful for electricity distribution and superconducting magnet applications because of their relatively high critical current densities and upper critical fields. SmFeAsO0.8F0.15 is of particular interest as it has the highest transition temperature among these materials. Here we show that by introducing a low density of correlated nano-scale defects into this material by heavy-ion irradiation, we can increase its critical current density to up to 2 x 10(7) A cm(-2) at 5 K-the highest ever reported for an iron-based superconductor-without reducing its critical temperature of 50 K. We also observe a notable reduction in the thermodynamic superconducting anisotropy, from 8 to 4 upon irradiation. We develop a model based on anisotropic electron scattering that predicts that the superconducting anisotropy can be tailored via correlated defects in semimetallic, fully gapped type II superconductors.
C1 [Fang, L.; Jia, Y.; Mishra, V.; Chaparro, C.; Vlasko-Vlasov, V. K.; Koshelev, A. E.; Welp, U.; Crabtree, G. W.; Kwok, W. K.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.
[Zhigadlo, N. D.; Katrych, S.; Karpinski, J.] Swiss Fed Inst Technol, Solid State Phys Lab, CH-8093 Zurich, Switzerland.
[Katrych, S.; Karpinski, J.] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland.
RP Fang, L (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM lfang@anl.gov; wkwok@anl.gov
RI Koshelev, Alexei/K-3971-2013
OI Koshelev, Alexei/0000-0002-1167-5906
FU Department of Energy, Office of Basic Energy Sciences
[DE-AC02-06CH11357]; EC Research Council; Swiss National Science
Foundation; National Center of Competence in Research MaNEP (Materials
with Novel Electronic Properties); US Department of Energy, Office of
Science, Office of Basic Energy Sciences
FX Critical current measurements and theory were supported by the Center
for Emergent Superconductivity, an Energy Frontier Research Center
funded by the US Department of Energy, Office of Science, Office of
Basic Energy Sciences (L.F., Y.J., V.M., A.E.K., W.K.K., G.W.C.),
specific heat and magneto-optical measurements were supported by the
Department of Energy, Office of Basic Energy Sciences, under Contract
No. DE-AC02-06CH11357 (C.C., V.K. V.-V., U.W.). J.K. and S.K.
acknowledge support of the EC Research Council project SuperIron. N.D.Z.
acknowledges the support of the Swiss National Science Foundation and
the National Center of Competence in Research MaNEP (Materials with
Novel Electronic Properties).
NR 36
TC 24
Z9 24
U1 8
U2 43
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2655
DI 10.1038/ncomms3655
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266IS
UT WOS:000328017900001
PM 24189627
ER
PT J
AU Liu, J
Kargarian, M
Kareev, M
Gray, B
Ryan, PJ
Cruz, A
Tahir, N
Chuang, YD
Guo, JH
Rondinelli, JM
Freeland, JW
Fiete, GA
Chakhalian, J
AF Liu, Jian
Kargarian, Mehdi
Kareev, Mikhail
Gray, Ben
Ryan, Phil J.
Cruz, Alejandro
Tahir, Nadeem
Chuang, Yi-De
Guo, Jinghua
Rondinelli, James M.
Freeland, John W.
Fiete, Gregory A.
Chakhalian, Jak
TI Heterointerface engineered electronic and magnetic phases of NdNiO3 thin
films
SO NATURE COMMUNICATIONS
LA English
DT Article
ID METAL-INSULATOR-TRANSITION; RAY-ABSORPTION SPECTROSCOPY; AUGMENTED-WAVE
METHOD; EQUALS RARE-EARTH; RNIO3 PEROVSKITES; HUBBARD-MODEL; BAND-GAPS;
SPECTRA; SYSTEMS; OXIDE
AB Mott physics is characterized by an interaction-driven metal-to-insulator transition in a partially filled band. In the resulting insulating state, antiferromagnetic orders of the local moments typically develop, but in rare situations no long-range magnetic order appears, even at zero temperature, rendering the system a quantum spin liquid. A fundamental and technologically critical question is whether one can tune the underlying energetic landscape to control both metal-to-insulator and Neel transitions, and even stabilize latent metastable phases, ideally on a platform suitable for applications. Here we demonstrate how to achieve this in ultrathin films of NdNiO3 with various degrees of lattice mismatch, and report on the quantum critical behaviours not reported in the bulk by transport measurements and resonant X-ray spectroscopy/scattering. In particular, on the decay of the antiferromagnetic Mott insulating state into a non-Fermi liquid, we find evidence of a quantum metal-to-insulator transition that spans a non-magnetic insulating phase.
C1 [Liu, Jian; Kareev, Mikhail; Gray, Ben; Chakhalian, Jak] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA.
[Liu, Jian; Cruz, Alejandro; Tahir, Nadeem; Chuang, Yi-De; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.
[Liu, Jian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Kargarian, Mehdi; Fiete, Gregory A.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA.
[Ryan, Phil J.; Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.
[Rondinelli, James M.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA.
RP Liu, J (reprint author), Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA.
EM jian.liu@berkeley.edu
RI Rondinelli, James/A-2071-2009; Liu, Jian/I-6746-2013; Chakhalian,
Jak/F-2274-2015
OI Rondinelli, James/0000-0003-0508-2175; Liu, Jian/0000-0001-7962-2547;
FU DOD-ARO [0402-17291, W911NF-09-1-0527, W911NF-12-1-0573]; NSF
[DMR-0747808, DMR-0955778]; DARPA [D13AP00052, N66001-12-1-4224]; ALS
Doctoral Fellowship programme; US DOE, Office of Science, BES
[DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences
of the US Department of Energy [DE-AC02-05CH11231]; US Department of
Energy, Office of Science [DE-AC02-06CH11357]
FX We acknowledge numerous insightful discussions with D. I. Khomskii, A.J.
Millis, D. D. Sarma, S. Okamoto, G. A. Sawatzky, S. Papanikolaou, D.
Maslov and M. Lawler. We also acknowledge B. Dabrowski for providing the
bulk reference powders. J.C. was supported by DOD-ARO under the Grant
number 0402-17291 and NSF Grant number DMR-0747808, M. K. and G. A. F.
by DOD-ARO Grant number W911NF-09-1-0527, W911NF-12-1-0573, DARPA
D13AP00052 and NSF Grant number DMR-0955778. J.M.R. was supported by
DARPA under Award number N66001-12-1-4224. J.L. acknowledges the support
from the ALS Doctoral Fellowship programme. The density functional
studies made use of the CARBON cluster at the Center for Nanoscale
Materials (Argonne National Laboratory) supported by the US DOE, Office
of Science, BES, under Contract number DE-AC02-06CH11357. Work at ALS is
supported by the Director, Office of Science, Office of Basic Energy
Sciences, of the US Department of Energy under Contract number
DE-AC02-05CH11231. Work at the APS is supported by the US Department of
Energy, Office of Science under Grant number DE-AC02-06CH11357.
NR 57
TC 42
Z9 42
U1 9
U2 96
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2714
DI 10.1038/ncomms3714
PG 11
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266KB
UT WOS:000328021400003
PM 24193317
ER
PT J
AU Wen, H
Gomella, AA
Patel, A
Lynch, SK
Morgan, NY
Anderson, SA
Bennett, EE
Xiao, XH
Liu, C
Wolfe, DE
AF Wen, Han
Gomella, Andrew A.
Patel, Ajay
Lynch, Susanna K.
Morgan, Nicole Y.
Anderson, Stasia A.
Bennett, Eric E.
Xiao, Xianghui
Liu, Chian
Wolfe, Douglas E.
TI Subnanoradian X-ray phase-contrast imaging using a far-field
interferometer of nanometric phase gratings
SO NATURE COMMUNICATIONS
LA English
DT Article
ID FOURIER-TRANSFORM METHOD; UNWRAPPING ALGORITHM; DIFFRACTION; TOMOGRAPHY;
RETRIEVAL; MICROTOMOGRAPHY; RADIOGRAPHY; MICROSCOPY; RADIATION; RATIO
AB Hard X-ray phase-contrast imaging characterizes the electron density distribution in an object without the need for radiation absorption. The power of phase contrast to resolve subtle changes, such as those in soft tissue structures, lies in its ability to detect minute refractive bending of X-rays. Here we report a far-field, two-arm interferometer based on the new nanometric phase gratings, which can detect X-ray refraction with subnanoradian sensitivity, and at the same time overcomes the fundamental limitation of ultra-narrow bandwidths (Delta lambda/lambda similar to 10(-4)) of the current, most sensitive methods based on crystal interferometers. On a 1.5% bandwidth synchrotron source, we demonstrate clear visualization of blood vessels in unstained mouse organs in simple projection views, with over an order-of-magnitude higher phase contrast than current near-field grating interferometers.
C1 [Wen, Han; Gomella, Andrew A.; Patel, Ajay; Lynch, Susanna K.; Morgan, Nicole Y.; Anderson, Stasia A.; Bennett, Eric E.] NIH, Bethesda, MD 20892 USA.
[Xiao, Xianghui; Liu, Chian] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA.
[Wolfe, Douglas E.] Penn State Univ, State Coll, PA 16804 USA.
RP Wen, H (reprint author), NIH, Bldg 10, Bethesda, MD 20892 USA.
EM han.wen@nih.gov
FU US Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]
FX We thank the staff of the NanoFab facility of National Institute of
Standards and Technology, Gaithersburg, Maryland, for their assistance
with fabrication of the gratings; the Animal Surgery and Resources Core
and Dr. Alan Michelson of NHLBI, NIH, for their help with biological
specimens; Dr. Dumitru Mazilu for his help with mechanical design and
fabrication. Use of the Advanced Photon Source at Argonne National
Laboratory was supported by the US Department of Energy, Office of
Science, Office of Basic Energy Sciences, under contract no
DE-AC02-06CH11357.
NR 56
TC 11
Z9 11
U1 2
U2 19
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2013
VL 4
AR 2659
DI 10.1038/ncomms3659
PG 9
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 266IU
UT WOS:000328018100001
PM 24189696
ER
PT J
AU Becker-Weimann, S
Xiong, GF
Furuta, S
Han, J
Kuhn, I
Akavia, UD
Pe'er, D
Bissell, MJ
Xu, R
AF Becker-Weimann, Sabine
Xiong, Gaofeng
Furuta, Saori
Han, Ju
Kuhn, Irene
Akavia, Uri-David
Pe'er, Dana
Bissell, Mina J.
Xu, Ren
TI NFkB disrupts tissue polarity in 3D by preventing integration of
microenvironmental signals
SO ONCOTARGET
LA English
DT Article
DE Disorganization gene signature; p65; RelB; three-dimensional tissue
structure; tissue polarity
ID BREAST EPITHELIAL-CELLS; FACTOR-KAPPA-B; 3-DIMENSIONAL CULTURE;
EXTRACELLULAR-MATRIX; CANCER CELLS; ALPHA-6-BETA-4 INTEGRIN; RECIPROCAL
INTERACTIONS; GENE-EXPRESSION; IN-VIVO; GROWTH
AB The microenvironment of cells controls their phenotype, and thereby the architecture of the emerging multicellular structure or tissue. We have reported more than a dozen microenvironmental factors whose signaling must be integrated in order to effect an organized, functional tissue morphology. However, the factors that prevent integration of signaling pathways that merge form and function are still largely unknown. We have identified nuclear factor kappa B (NFkB) as a transcriptional regulator that disrupts important microenvironmental cues necessary for tissue organization. We compared the gene expression of organized and disorganized epithelial cells of the HMT-3522 breast cancer progression series: the non-malignant S1 cells that form polarized spheres ('acini'), the malignant T4-2 cells that form large tumor-like clusters, and the 'phenotypically reverted' T4-2 cells that polarize as a result of correction of the microenvironmental signaling. We identified 180 genes that display an increased expression in disorganized compared to polarized structures. Network, GSEA and transcription factor binding site analyses suggested that NFkB is a common activator for the 180 genes. NFkB was found to be activated in disorganized breast cancer cells, and inhibition of microenvironmental signaling via EGFR, beta1 integrin, MMPs, or their downstream signals suppressed its activation. The postulated role of NFkB was experimentally verified: Blocking the NFkB pathway with a specific chemical inhibitor or shRNA induced polarization and inhibited invasion of breast cancer cells in 3D cultures. These results may explain why NFkB holds promise as a target for therapeutic intervention: Its inhibition can reverse the oncogenic signaling involved in breast cancer progression and integrate the essential microenvironmental control of tissue architecture.
C1 [Becker-Weimann, Sabine; Furuta, Saori; Han, Ju; Kuhn, Irene; Bissell, Mina J.] Lawrence Berkeley Natl Lab 1, Div Life Sci, Berkeley, CA 94720 USA.
[Xiong, Gaofeng; Xu, Ren] Univ Kentucky, Markey Canc Ctr, Lexington, KY USA.
[Xu, Ren] Univ Kentucky, Dept Mol & Biomed Pharmacol, Lexington, KY USA.
[Akavia, Uri-David; Pe'er, Dana] Columbia Univ, Dept Biol Sci, New York, NY 10027 USA.
RP Bissell, MJ (reprint author), Lawrence Berkeley Natl Lab 1, Div Life Sci, Berkeley, CA 94720 USA.
EM mjbissell@lbl.gov; ren.xu2010@uky.edu
FU U.S. Department of Energy, the Office of Biological and Environmental
Research [DE-AC02-05CH1123, 03-76SF00098]; National Cancer Institute
[R01CA064786, U54CA143836, U54CA112970]; U.S. Department of Defense
Medical and Materiel Command [W81XWH0810736]; Breast Cancer Research
Foundation; AHA [12SDG8600000]; ACS [IRG 85-001-22]; Physical Sciences
Oncology Center
FX This work was supported by grants from the U.S. Department of Energy,
the Office of Biological and Environmental Research (contract no.
DE-AC02-05CH1123) and a Distinguished Fellow Award from the above
(contract no. 03-76SF00098), from the National Cancer Institute (awards
R01CA064786, U54CA143836 and U54CA112970) to MJB and SB, the U.S.
Department of Defense Medical and Materiel Command innovator awards
(contract no.W81XWH0810736) to MJB, in part by a grant from the Breast
Cancer Research Foundation to MJB, and in part by AHA (12SDG8600000) and
ACS grants (IRG 85-001-22) to R. X. R. X. thanks Dr. Catherine Anthony
for editorial assistance. We (MJB and SB) thank the Physical Sciences
Oncology Center for providing support for completion of this work.
NR 39
TC 14
Z9 15
U1 1
U2 6
PU IMPACT JOURNALS LLC
PI ALBANY
PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA
SN 1949-2553
J9 ONCOTARGET
JI Oncotarget
PD NOV
PY 2013
VL 4
IS 11
BP 2010
EP 2020
PG 11
WC Oncology; Cell Biology
SC Oncology; Cell Biology
GA 261KW
UT WOS:000327664900017
PM 24243820
ER
PT J
AU Cui, HY
Hanus, R
Kessler, MR
AF Cui, Hongyu
Hanus, Riley
Kessler, Michael R.
TI Degradation of ROMP-based bio-renewable polymers by UV radiation
SO POLYMER DEGRADATION AND STABILITY
LA English
DT Article
DE UV degradation; Photo-degradation; Bio-renewable; Auto-oxidation
ID TRANSFORM-INFRARED-SPECTROSCOPY; OPENING METATHESIS POLYMERIZATION;
POLYPROPYLENE; OXIDATION; OIL; POLYETHYLENE; MECHANISMS; BEHAVIOR;
PROFILE; FILMS
AB The degradation of a bio-renewable polymer under UV exposure was studied using various methods. Degradation of the bio-renewable polymer increased with increasing exposure time. Enhanced cross-link density in the early stage of degradation was confirmed by Soxhlet extraction. Tensile testing showed a transition from ductile failure to brittle fracture. Surface cracks and embrittlement were primary reasons for most reductions in mechanical properties, such as tensile strength and breaking strain. The effects of degradation were confined to the surface of thick bio-based polymer specimens, confirmed by both SEM and PAS-FTIR. Depth profile studies of degraded samples showed that the concentration of oxidation products, such as hydroxyl and carbonyl groups, varied with depth depending on the diffusion of oxygen. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Cui, Hongyu; Hanus, Riley; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA.
[Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA.
[Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA.
RP Kessler, MR (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA.
EM MichaelR.Kessler@wsu.edu
RI Kessler, Michael/C-3153-2008
OI Kessler, Michael/0000-0001-8436-3447
FU National Science Foundation (NSF) [0954314]; Consortium for Plant
Biotechnology Research (CPBR) through USEPA grant [EM-83438801]
FX Funding from the National Science Foundation (NSF) through Award
0954314, and the Consortium for Plant Biotechnology Research (CPBR)
through USEPA grant EM-83438801, is gratefully acknowledged. The
contents of the paper are solely the responsibility of the grantee and
do not necessarily represent the views of the USEPA. Further, USEPA does
not endorse the purchase of any commercial products or services
mentioned in this publication.
NR 23
TC 5
Z9 5
U1 3
U2 24
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0141-3910
EI 1873-2321
J9 POLYM DEGRAD STABIL
JI Polym. Degrad. Stabil.
PD NOV
PY 2013
VL 98
IS 11
BP 2357
EP 2365
DI 10.1016/j.polymdegradstab.2013.08.003
PG 9
WC Polymer Science
SC Polymer Science
GA 264VJ
UT WOS:000327908800030
ER
PT J
AU Anderson, BJ
AF Anderson, Benjamin J.
TI Thermal stability and lifetime estimates of a high temperature epoxy by
T-g reduction
SO POLYMER DEGRADATION AND STABILITY
LA English
DT Article
DE Epoxy; Degradation; Thermal aging; Lifetime
ID GLASS-TRANSITION TEMPERATURE; NON-ARRHENIUS BEHAVIOR; DEGRADATION;
PREDICTION; POLYMERS; KINETICS; RESINS; OXIDATION
AB Thermal degradation of a high temperature epoxy network is studied in terms glass transition temperature (T-g) reduction over a temperature window encompassing the T-g of the network. The T-g is shown to decrease as the network is thermally aged at elevated temperatures in air and in argon. The duration of the aging experiments is extended to long time such that the absolute T-g reduction approaches a long time reduction plateau. Degradation is dominated by non-oxidative pyrolysis with a small contribution from diffusion limited thermal oxidative degradation at the surface. A time-temperature superposition is constructed from the extent of T-g reduction of samples aged in air and the thermal shift factors are shown to have Arrhenius scaling behavior. An activation energy is extracted that agrees with previous activation energy measurements derived from other property measurements of the same network aged under similar conditions. The agreement of the activation energy with past results shows that T-g reduction is controlled by the same degradation mechanism and may be used as an observable for lifetime estimates when thermal degradation is pyrolytic in nature. The extent of T-g reduction is modeled with an autocatalytic rate expression and compared to previous property measurements to show the difference in sensitivity of observable material properties on degradation. (C) 2013 Elsevier Ltd. All rights reserved.
C1 Sandia Natl Labs, Mat Sci & Engn Ctr, Albuquerque, NM 87185 USA.
RP Anderson, BJ (reprint author), Sandia Natl Labs, Mat Sci & Engn Ctr, POB 5800, Albuquerque, NM 87185 USA.
EM bjander@sandia.gov
FU United States Department of Energy [DE-AC04-94AL85000]
FX The author thanks Joanetta Bruhn for material sample preparation,
thermal aging of samples, and DMA testing. The author also thanks Mat
Celina for helpful comments with regard to preparation of the
manuscript. Sandia is a multiprogram laboratory operated by Sandia
Corporation, a Lockheed Martin Company, for the United States Department
of Energy under contract DE-AC04-94AL85000.
NR 25
TC 3
Z9 3
U1 3
U2 19
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0141-3910
EI 1873-2321
J9 POLYM DEGRAD STABIL
JI Polym. Degrad. Stabil.
PD NOV
PY 2013
VL 98
IS 11
BP 2375
EP 2382
DI 10.1016/j.polymdegradstab.2013.08.001
PG 8
WC Polymer Science
SC Polymer Science
GA 264VJ
UT WOS:000327908800032
ER
PT J
AU Schmidt, MW
Gordon, MS
AF Schmidt, Michael W.
Gordon, Mark S.
TI The Decomposition of Hydrazine in the Gas Phase and over an Iridium
Catalyst
SO ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH
IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS
LA English
DT Article
DE Hydrazine; Gas Phase; Ir Catalyst; Quantum Chemistry
ID SUPPORTED METAL-CLUSTERS; REVERSE HYDROGEN SPILLOVER; MOLECULAR-ORBITAL
METHODS; PD AUTOMOTIVE CATALYSTS; GAMMA-ALUMINA SURFACES; OPEN-SHELL
SYSTEMS; TETRAIRIDIUM CLUSTERS; PERTURBATION-THEORY; BASIS-SETS;
AB-INITIO
AB Hydrazine is an important rocket fuel, used as both a monopropellant and a bipropellant. This paper presents theoretical results to complement the extensive experimental studies of the gas phase and Ir catalyzed decompositions involved in the monopropellant applications of hydrazine. Gas phase electronic structure theory calculations that include electron correlation predict that numerous molecular and free radical reactions occur within the same energy range as the basic free radical pathways: NN bond breaking around 65 kcal/mol and NH bond breaking around 81 kcal/mol. The data suggest that a revision to existing kinetics modeling is desirable, based on the energetics and the new elementary steps reported herein. A supported Ir-6 octahedron model for the Shell 405 Iridium catalyst used in thrusters was developed. Self-Consistent Field and electron correlation calculations (with core potentials and associated basis sets) find a rich chemistry for hydrazine on this catalyst model. The model catalyst provides dramatically lower NN and NH bond cleavage energies and an even smaller barrier to breaking the NH bond by NH2 abstractions. Thus, the low temperature decomposition over the catalyst is interpreted in terms of consecutive NH2 abstractions to produce ammonia and nitrogen. The higher temperature channel, which has hydrogen and nitrogen products, may be due to a mixture of two mechanisms. These two mechanisms are successive NH cleavages with surface H + H recombinations, and the same type of assisted H-2 eliminations found to occur in the gas phase part of this study.
C1 [Gordon, Mark S.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA.
Iowa State Univ, Ames Lab, Ames, IA 50011 USA.
RP Gordon, MS (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA.
EM mark@si.msg.chem.iastate.edu
FU Air Force Office of Scientific Research under AFOSR Award
[FA9550-09-1-0059]; Department of Defense
FX The research presented here is based upon work supported by the Air
Force Office of Scientific Research under AFOSR Award No.
FA9550-09-1-0059. The calculations were performed under the auspices of
a Department of Defense Grand Challenge grant of computer time, on a
computer cluster that was purchased in part by a DoD DURIP grant, and on
a GPU-based cluster that was provided in part by the Nvidia Corporation,
the Ames Laboratory, and Iowa State University. The authors are very
grateful to Dr. Spencer Pruitt for many helpful discussions.
NR 107
TC 4
Z9 4
U1 1
U2 25
PU WALTER DE GRUYTER GMBH
PI BERLIN
PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY
SN 0942-9352
J9 Z PHYS CHEM
JI Z. Phys. Chemie-Int. J. Res. Phys. Chem. Chem. Phys.
PD NOV
PY 2013
VL 227
IS 9-11
BP 1301
EP 1336
DI 10.1524/zpch.2013.0404
PG 36
WC Chemistry, Physical
SC Chemistry
GA 264EZ
UT WOS:000327861100009
ER
PT J
AU Di Gennaro, E
di Uccio, US
Aruta, C
Cantoni, C
Gadaleta, A
Lupini, AR
Maccariello, D
Marre, D
Pallecchi, I
Paparo, D
Perna, P
Riaz, M
Granozio, FM
AF Di Gennaro, Emiliano
di Uccio, Umberto Scotti
Aruta, Carmela
Cantoni, Claudia
Gadaleta, Alessandro
Lupini, Andrew R.
Maccariello, Davide
Marre, Daniele
Pallecchi, Ilaria
Paparo, Domenico
Perna, Paolo
Riaz, Muhammad
Granozio, Fabio Miletto
TI Persistent Photoconductivity in 2D Electron Gases at Different Oxide
Interfaces
SO ADVANCED OPTICAL MATERIALS
LA English
DT Article
ID LAALO3/SRTIO3 HETEROSTRUCTURES; HETEROINTERFACE; CONDUCTIVITY
AB The transport characterization in the dark and under light irradiation of three different interfaces-LaAlO3/SrTiO3, LaGaO3/SrTiO3, and the novel NdGaO3/ SrTiO3 heterostructure is reported. All of them share a perovskite structure, an insulating nature of the single building blocks, a polar/non-polar character, and a critical thickness of four unit cells for the onset of conductivity. The interface structure and charge confinement in NdGaO3/SrTiO3 are probed by atomic-scale-resolved electron energy loss spectroscopy showing that, similarly to LaAlO3/SrTiO3, extra electronic charge confined in a sheet of about 1.5 nm in thickness is present at the NdGaO3/SrTiO3 interface. Electric transport measurements performed in the dark and under radiation show remarkable similarities and provide evidence that the persistent perturbation induced by light is an intrinsic peculiar property of the three investigated oxide-based polar/non-polar interfaces. This sets a framework for understanding the previous contrasting results found in the literature about photoconductivity in LaAlO3/SrTiO3 and highlights the connection between the origin of persistent photoconductivity and the origin of conductivity itself. An improved understanding of the photoinduced metastable electron-hole pairs might allow light to be shed directly on the complex physics of this system and on the recently proposed perspectives of oxide interfaces for solar energy conversion.
C1 [Di Gennaro, Emiliano; di Uccio, Umberto Scotti; Aruta, Carmela; Maccariello, Davide; Paparo, Domenico; Perna, Paolo; Riaz, Muhammad; Granozio, Fabio Miletto] Univ Naples Federico II, CNR SPIN, I-80126 Naples, Italy.
[Di Gennaro, Emiliano; di Uccio, Umberto Scotti; Aruta, Carmela; Maccariello, Davide; Paparo, Domenico; Perna, Paolo; Riaz, Muhammad; Granozio, Fabio Miletto] Univ Naples Federico II, Dipartimento Fis, I-80126 Naples, Italy.
[Cantoni, Claudia; Lupini, Andrew R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
[Gadaleta, Alessandro; Marre, Daniele; Pallecchi, Ilaria] Univ Genoa, CNR SPIN, I-16146 Genoa, Italy.
[Gadaleta, Alessandro; Marre, Daniele; Pallecchi, Ilaria] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy.
RP Granozio, FM (reprint author), Univ Naples Federico II, CNR SPIN, Compl Univ Monte S Angelo,Via Cintia, I-80126 Naples, Italy.
EM fabio.miletto@spin.cnr
RI PERNA, PAOLO/C-3862-2012; Maccariello, Davide/J-8165-2013; Aruta,
Carmela/L-2957-2015; Paparo, Domenico/L-7766-2015; Marre,
Daniele/G-5965-2014; Di Gennaro, Emiliano/G-6311-2010; Cantoni,
Claudia/G-3031-2013
OI PERNA, PAOLO/0000-0001-8537-4834; Maccariello,
Davide/0000-0002-8681-2717; Aruta, Carmela/0000-0002-6917-6667; Paparo,
Domenico/0000-0002-7745-230X; Marre, Daniele/0000-0002-6230-761X; Di
Gennaro, Emiliano/0000-0003-4231-9776; Cantoni,
Claudia/0000-0002-9731-2021
FU EU; MIUR [264098]; US Department of Energy, Office of Science, Materials
Sciences and Engineering Division; ORNL's Shared Research Equipment
(ShaRE) User Program; Office of Basic Energy Sciences, U.S. Department
of Energy
FX Financial support by EU under the project OXIDES, by MIUR under Grant
Agreement PRIN 2008 - 2DEG FOXI, by European Union Seventh Framework
Program (FP7/2007-2013) under grant agreement N. 264098 - MAMA, and by
Compagnia di San Paolo is acknowledged. CC and ARL acknowledge funding
by the US Department of Energy, Office of Science, Materials Sciences
and Engineering Division. Part of this research was supported by ORNL's
Shared Research Equipment (ShaRE) User Program, which is sponsored by
the Office of Basic Energy Sciences, U.S. Department of Energy.
NR 56
TC 9
Z9 9
U1 6
U2 122
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 2195-1071
J9 ADV OPT MATER
JI Adv. Opt. Mater.
PD NOV
PY 2013
VL 1
IS 11
BP 834
EP 843
DI 10.1002/adom.201300150
PG 10
WC Materials Science, Multidisciplinary; Optics
SC Materials Science; Optics
GA 251KA
UT WOS:000326926100009
ER
PT J
AU Penton, CR
St Louis, D
Cole, JR
Luo, YQ
Wu, LY
Schuur, EAG
Zhou, JZ
Tiedje, JM
AF Penton, C. Ryan
St Louis, Derek
Cole, James R.
Luo, Yiqi
Wu, Liyou
Schuur, E. A. G.
Zhou, Jizhong
Tiedje, James M.
TI Fungal Diversity in Permafrost and Tallgrass Prairie Soils under
Experimental Warming Conditions
SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY
LA English
DT Article
ID COMMUNITY STRUCTURE; SEASONAL DYNAMICS; ARCTIC TUNDRA; MICROBIAL
COMMUNITIES; SEQUENCE DATABASES; ALASKAN TUNDRA; DNA-SEQUENCES; PH
GRADIENT; ROOTS; BACTERIAL
AB Soil fungi play a major role in terrestrial ecosystem functioning through interactions with soil structure, plants, micro- and mesofauna, and nutrient cycling through predation, pathogenesis, mutualistic, and saprotrophic roles. The diversity of soil fungi was assessed by sequencing their 28S rRNA gene in Alaskan permafrost and Oklahoma tallgrass prairie soils at experimental sites where the effect of climate warming is under investigation. A total of 226,695 reads were classified into 1,063 genera, covering 62% of the reference data set. Using the Bayesian Classifier offered by the Ribosomal Database Project (RDP) with 50% boot-strapping classification confidence, approximately 70% of sequences were returned as "unclassified" at the genus level, although the majority (similar to 65%) were classified at the class level, which provided insight into these lesser-known fungal lineages. Those unclassified at the genus level were subjected to BLAST analysis against the ARB-SILVA database, where similar to 50% most closely matched nonfungal taxa. Compared to the more abundant sequences, a higher proportion of rare operational taxonomic units (OTU) were successfully classified to genera at 50% bootstrap confidence, indicating that the fungal rare biosphere in these sites is not composed of sequencing artifacts. There was no significant effect after 1 year of warming on the fungal community structure at both sites, except perhaps for a few minor members, but there was a significant effect of sample depth in the permafrost soils. Despite overall significant community structure differences driven by variations in OTU dominance, the prairie and permafrost soils shared 90% and 63% of all fungal sequences, respectively, indicating a fungal "seed bank" common between both sites.
C1 [Penton, C. Ryan; St Louis, Derek; Cole, James R.; Tiedje, James M.] Michigan State Univ, Ctr Microbial Ecol, E Lansing, MI 48824 USA.
[Luo, Yiqi; Wu, Liyou] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA.
[Wu, Liyou; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.
[Schuur, E. A. G.] Univ Florida, Dept Biol, Gainesville, FL USA.
[Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China.
[Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.
RP Penton, CR (reprint author), Michigan State Univ, Ctr Microbial Ecol, E Lansing, MI 48824 USA.
EM pentonch@msu.edu
FU Department of Energy, Biological Systems Research on the Role of
Microbial Communities in Carbon Cycling Program [DE-SC0004601]
FX This work is supported by the Department of Energy, Biological Systems
Research on the Role of Microbial Communities in Carbon Cycling Program
(DE-SC0004601).
NR 81
TC 18
Z9 19
U1 6
U2 68
PU AMER SOC MICROBIOLOGY
PI WASHINGTON
PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA
SN 0099-2240
EI 1098-5336
J9 APPL ENVIRON MICROB
JI Appl. Environ. Microbiol.
PD NOV
PY 2013
VL 79
IS 22
BP 7063
EP 7072
DI 10.1128/AEM.01702-13
PG 10
WC Biotechnology & Applied Microbiology; Microbiology
SC Biotechnology & Applied Microbiology; Microbiology
GA 259CE
UT WOS:000327504200030
PM 24014534
ER
PT J
AU Ponoum, R
Rutbers, M
Boum, A
AF Ponoum, Ratcharit
Rutbers, Michael
Boum, Antonio
TI Energy Storage for PV Power
SO ASHRAE JOURNAL
LA English
DT Article
AB Photovoltaic (PV) power is one of the fastest growing renewable energy technologies today. Because of the intermittent nature of PV electrical output, energy storage will be an important enabler for its continued growth. Of the candidate storage technologies, electrochemical batteries hold the most promise for widespread deployment. Development of economical, scalable PV energy storage systems is being actively pursued across a range of battery technologies, from lead-acid to lithium-ion to redox flow batteries.
C1 [Rutbers, Michael] TIAX LLC, Mech Syst Grp, Lexington, MA USA.
[Boum, Antonio] US DOE, Washington, DC USA.
NR 11
TC 0
Z9 0
U1 0
U2 3
PU AMER SOC HEATING REFRIGERATING AIR-CONDITIONING ENG, INC,
PI ATLANTA
PA 1791 TULLIE CIRCLE NE, ATLANTA, GA 30329 USA
SN 0001-2491
EI 1943-6637
J9 ASHRAE J
JI ASHRAE J.
PD NOV
PY 2013
VL 55
IS 11
BP 80
EP 83
PG 4
WC Thermodynamics; Construction & Building Technology; Engineering,
Mechanical
SC Thermodynamics; Construction & Building Technology; Engineering
GA 252XP
UT WOS:000327046500018
ER
PT J
AU Janssen, R
Turhollow, AF
Rutz, D
Mergner, R
AF Janssen, Rainer
Turhollow, Anthony F.
Rutz, Dominik
Mergner, Rita
TI Production facilities for second-generation biofuels in the USA and the
EU - current status and future perspectives
SO BIOFUELS BIOPRODUCTS & BIOREFINING-BIOFPR
LA English
DT Article
DE second-generation biofuels; United States; Europe; demonstration plants;
ethanol; synthetic fuels
AB Second-generation biofuel production facilities have been slower to reach large-scale production than was anticipated a few years ago even though in Europe, the Renewable Energy Directive provides incentives; in the United States there are also financial incentives and the Energy Independence and Security Act of 2007 has targets for second-generation biofuels. But starting in 2013 it appears that significant quantities of second-generation biofuels will be produced. A variety of conversion processes, thermochemical and biological, as well as hybrids of the two is being utilized. There will be a variety of fuels - ethanol, drop-in fuels (e.g. gasoline, diesel), biodiesel, steam, electricity, bio-oil, sugars, and chemicals; and a variety of feedstocks - crop residues, wood, wood wastes, energy crops, waste oils and municipal solid waste (MSW). One approach to reducing the risk of moving from first- to second-generation biofuel production has been to take incremental steps such as converting the cellulosic part of grains into ethanol in addition to the starch portion. Many of the second-generation biofuel facilities are co-located with first-generation biofuel production facilities to share infrastructure as well as trade by-products (e.g. excess steam). One of the challenges has been financing, but both private and government sources are being utilized. Private sources include internal corporate funds and debt offerings, and venture capital. Government sources include the US federal government, the European Union, European national governments, and state and local governments. (c) 2013 Society of Chemical Industry and John Wiley & Sons, Ltd
C1 [Janssen, Rainer] WIP Renewable Energies, Biomass Dept, D-81369 Munich, Germany.
[Turhollow, Anthony F.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA.
[Rutz, Dominik; Mergner, Rita] WIP Renewable Energies, D-81369 Munich, Germany.
RP Janssen, R (reprint author), WIP Renewable Energies, Sylvensteinstr 2, D-81369 Munich, Germany.
EM rainer.janssen@wip-munich.de
FU Project BIOLYFE (Demonstrating large-scale bioethanol production from
lignocellulosic feedstocks); European Commission [FP7-239204,
FP7-227422]; Project SWEETFUEL (Sweet Sorghum: An alternative energy
crop); U.S. Department of Energy EERE Bioenergy Technologies Office; US
Department of Energy [DE-AC05-00OR22725]
FX This paper was supported by: Project BIOLYFE (Demonstrating large-scale
bioethanol production from lignocellulosic feedstocks) co-funded by the
European Commission in the 7th Framework Programme (Project No.
FP7-239204); Project SWEETFUEL (Sweet Sorghum: An alternative energy
crop) co-funded by the European Commission in the 7th Framework
Programme (Project No. FP7-227422); The U.S. Department of Energy EERE
Bioenergy Technologies Office and performed at Oak Ridge National
Laboratory (ORNL). ORNL is managed by UT-Battelle, LLC, for the US
Department of Energy under contract DE-AC05-00OR22725.
NR 39
TC 15
Z9 15
U1 5
U2 50
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1932-104X
EI 1932-1031
J9 BIOFUEL BIOPROD BIOR
JI Biofuels Bioprod. Biorefining
PD NOV
PY 2013
VL 7
IS 6
SI SI
BP 647
EP 665
DI 10.1002/bbb.1451
PG 19
WC Biotechnology & Applied Microbiology; Energy & Fuels
SC Biotechnology & Applied Microbiology; Energy & Fuels
GA 250YQ
UT WOS:000326893400014
ER
PT J
AU Stone, D
Auffhammer, M
Carey, M
Hansen, G
Huggel, C
Cramer, W
Lobell, D
Molau, U
Solow, A
Tibig, L
Yohe, G
AF Stone, Daithi
Auffhammer, Maximilian
Carey, Mark
Hansen, Gerrit
Huggel, Christian
Cramer, Wolfgang
Lobell, David
Molau, Ulf
Solow, Andrew
Tibig, Lourdes
Yohe, Gary
TI The challenge to detect and attribute effects of climate change on human
and natural systems
SO CLIMATIC CHANGE
LA English
DT Article
ID IMPACTS; VARIABILITY
AB Anthropogenic climate change has triggered impacts on natural and human systems world-wide, yet the formal scientific method of detection and attribution has been only insufficiently described. Detection and attribution of impacts of climate change is a fundamentally cross-disciplinary issue, involving concepts, terms, and standards spanning the varied requirements of the various disciplines. Key problems for current assessments include the limited availability of long-term observations, the limited knowledge on processes and mechanisms involved in changing environmental systems, and the widely different concepts applied in the scientific literature. In order to facilitate current and future assessments, this paper describes the current conceptual framework of the field and outlines a number of conceptual challenges. Based on this, it proposes workable cross-disciplinary definitions, concepts, and standards. The paper is specifically intended to serve as a baseline for continued development of a consistent cross-disciplinary framework that will facilitate integrated assessment of the detection and attribution of climate change impacts.
C1 [Stone, Daithi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Auffhammer, Maximilian] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Auffhammer, Maximilian] Natl Bur Econ Res, Cambridge, MA 02138 USA.
[Carey, Mark] Univ Oregon, Eugene, OR 97403 USA.
[Hansen, Gerrit] Potsdam Inst Climate Impact Res, Potsdam, Germany.
[Huggel, Christian] Univ Zurich, Zurich, Switzerland.
[Cramer, Wolfgang] Aix Marseille Univ CNRS IRD UAPV, IMBE, F-13545 Aix En Provence, France.
[Lobell, David] Stanford Univ, Stanford, CA 94305 USA.
[Molau, Ulf] Univ Gothenburg, Gothenburg, Sweden.
[Solow, Andrew] Woods Hole Oceanog Inst, Woods Hole, MA 02543 USA.
[Tibig, Lourdes] Manila Observ, Quezon City, Philippines.
[Yohe, Gary] Wesleyan Univ, Middletown, CT USA.
RP Stone, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS-50F1650, Berkeley, CA 94720 USA.
EM dstone@lbl.gov; wolfgang.cramer@imbe.fr
RI Cramer, Wolfgang/B-8221-2008;
OI Cramer, Wolfgang/0000-0002-9205-5812; Stone, Daithi/0000-0002-2518-100X
FU Regional and Global Climate Modeling Program of the Office of Biological
and Environmental Research in the Department of Energy Office of
Science; Earth System Modeling Program of the Office of Biological and
Environmental Research in the Department of Energy Office of Science
[DE-AC02-05CH11231]; German Ministry for Education and Research
FX We thank the Detection and Attribution Liaisons to IPCC AR5 WGII Chapter
18, Chris Field, and Mike Mastrandrea for many helpful discussions. We
are also grateful to Yuka Estrada and Monalisa Chatterjee for assistance
in graphic design. While the chapter authors are all members of the AR5
Chapter 18 author team, all opinions, findings, and errors are those of
the authors alone. Many of the discussions distilled here were conducted
during and around Lead Author Meetings of the IPCC assessment process,
supported by various national governments. DS was supported by the
Regional and Global Climate Modeling Program and the Earth System
Modeling Program of the Office of Biological and Environmental Research
in the Department of Energy Office of Science under contract number
DE-AC02-05CH11231. GH was supported by a grant from the German Ministry
for Education and Research.
NR 41
TC 27
Z9 28
U1 5
U2 35
PU SPRINGER
PI DORDRECHT
PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS
SN 0165-0009
EI 1573-1480
J9 CLIMATIC CHANGE
JI Clim. Change
PD NOV
PY 2013
VL 121
IS 2
BP 381
EP 395
DI 10.1007/s10584-013-0873-6
PG 15
WC Environmental Sciences; Meteorology & Atmospheric Sciences
SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences
GA 251QD
UT WOS:000326944000020
ER
PT J
AU Koch, A
McBratney, A
Adams, M
Field, D
Hill, R
Crawford, J
Minasny, B
Lal, R
Abbott, L
O'Donnell, A
Angers, D
Baldock, J
Barbier, E
Binkley, D
Parton, W
Wall, DH
Bird, M
Bouma, J
Chenu, C
Flora, CB
Goulding, K
Grunwald, S
Hempel, J
Jastrow, J
Lehmann, J
Lorenz, K
Morgan, CL
Rice, CW
Whitehead, D
Young, I
Zimmermann, M
AF Koch, Andrea
McBratney, Alex
Adams, Mark
Field, Damien
Hill, Robert
Crawford, John
Minasny, Budiman
Lal, Rattan
Abbott, Lynette
O'Donnell, Anthony
Angers, Denis
Baldock, Jeffrey
Barbier, Edward
Binkley, Dan
Parton, William
Wall, Diana H.
Bird, Michael
Bouma, Johan
Chenu, Claire
Flora, Cornelia Butler
Goulding, Keith
Grunwald, Sabine
Hempel, Jon
Jastrow, Julie
Lehmann, Johannes
Lorenz, Klaus
Morgan, Cristine L.
Rice, Charles W.
Whitehead, David
Young, Iain
Zimmermann, Michael
TI Soil Security: Solving the Global Soil Crisis
SO GLOBAL POLICY
LA English
DT Article
ID CARBON SEQUESTRATION; ORGANIC-CARBON; FOOD SECURITY; FRAMEWORK; WORLD
AB Soil degradation is a critical and growing global problem. As the world population increases, pressure on soil also increases and the natural capital of soil faces continuing decline. International policy makers have recognized this and a range of initiatives to address it have emerged over recent years. However, a gap remains between what the science tells us about soil and its role in underpinning ecological and human sustainable development, and existing policy instruments for sustainable development. Functioning soil is necessary for ecosystem service delivery, climate change abatement, food and fiber production and fresh water storage. Yet key policy instruments and initiatives for sustainable development have under-recognized the role of soil in addressing major challenges including food and water security, biodiversity loss, climate change and energy sustainability. Soil science has not been sufficiently translated to policy for sustainable development. Two underlying reasons for this are explored and the new concept of soil security is proposed to bridge the science-policy divide. Soil security is explored as a conceptual framework that could be used as the basis for a soil policy framework with soil carbon as an exemplar indicator.
C1 [Koch, Andrea; McBratney, Alex; Field, Damien; Hill, Robert; Crawford, John; Minasny, Budiman] Univ Sydney, Sydney, NSW 2006, Australia.
[Lal, Rattan] Ohio State Univ, Columbus, OH 43210 USA.
[Abbott, Lynette; O'Donnell, Anthony] Univ Western Australia, Nedlands, WA 6009, Australia.
[Barbier, Edward] Univ Wyoming, Laramie, WY 82071 USA.
[Binkley, Dan; Parton, William; Wall, Diana H.] Colorado State Univ, Ft Collins, CO 80523 USA.
[Bird, Michael] James Cook Univ, Townsville, Qld, Australia.
[Bouma, Johan] Wageningen Univ, NL-6700 AP Wageningen, Netherlands.
[Chenu, Claire] AgroParisTech, UMR Bioemco, Paris, France.
[Flora, Cornelia Butler] Iowa State Univ, Ames, IA 50011 USA.
[Grunwald, Sabine] Univ Florida, Gainesville, FL 32611 USA.
[Jastrow, Julie] Argonne Natl Lab, Argonne, IL 60439 USA.
[Lehmann, Johannes] Cornell Univ, Ithaca, NY 14853 USA.
[Morgan, Cristine L.] Texas A&M Univ, College Stn, TX 77843 USA.
[Rice, Charles W.] Kansas State Univ, Manhattan, KS 66506 USA.
[Young, Iain] Univ New England, Sch Environm & Rural Sci, Armidale, NSW 2351, Australia.
[Zimmermann, Michael] Univ Nat Resources & Life Sci Vienna, Vienna, Austria.
RP Koch, A (reprint author), Univ Sydney, Sydney, NSW 2006, Australia.
RI Morgan, Cristine`/A-1555-2013; James Cook University, TESS/B-8171-2012;
Abbott, Lynette/F-7489-2011; Baldock, Jeffrey/G-1362-2010; adams,
mark/H-1303-2012; Bird, Michael/G-5364-2010; Zimmermann,
Michael/F-7547-2010; Goulding, Keith/B-2635-2012;
OI Morgan, Cristine`/0000-0001-9836-0669; Abbott,
Lynette/0000-0001-8586-7858; Baldock, Jeffrey/0000-0002-6428-8555;
adams, mark/0000-0001-8989-508X; Minasny, Budiman/0000-0002-1182-2371;
Bird, Michael/0000-0003-1801-8703; Zimmermann,
Michael/0000-0002-5162-2008; Goulding, Keith/0000-0002-6465-1465; Field,
Damien/0000-0002-6877-8332
NR 48
TC 34
Z9 35
U1 16
U2 118
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1758-5880
EI 1758-5899
J9 GLOB POLICY
JI Glob. Policy
PD NOV
PY 2013
VL 4
IS 4
BP 434
EP 441
DI 10.1111/1758-5899.12096
PG 8
WC International Relations; Political Science
SC International Relations; Government & Law
GA 251AD
UT WOS:000326897700018
ER
PT J
AU Calyam, P
Dovrolis, C
Jorgenson, L
Kettimuthu, R
Tierney, B
Zurawski, J
AF Calyam, Prasad
Dovrolis, Constantine
Joergenson, Loki
Kettimuthu, Raj
Tierney, Brian
Zurawski, Jason
TI MONITORING AND TROUBLESHOOTING MULTI-DOMAIN NETWORKS USING MEASUREMENT
FEDERATIONS
SO IEEE COMMUNICATIONS MAGAZINE
LA English
DT Editorial Material
C1 [Calyam, Prasad] Univ Missouri, Dept Comp Sci, Columbia, MO 65211 USA.
[Dovrolis, Constantine] Georgia Inst Technol, Coll Comp, Atlanta, GA 30332 USA.
[Joergenson, Loki] Lionsgate Technol, Vancouver, BC, Canada.
[Joergenson, Loki] INETCO Syst, Burnaby, BC, Canada.
[Kettimuthu, Raj] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA.
[Kettimuthu, Raj] Univ Chicago, Computat Inst, Chicago, IL 60637 USA.
[Tierney, Brian] Lawrence Berkeley Natl Lab, ESnet Adv Network Technol Grp, Berkeley, CA USA.
[Zurawski, Jason] Lawrence Berkeley Natl Lab, Energy Sci Network ESnet, Sci Networking Div, Comp Sci Directorate, Berkeley, CA USA.
RP Calyam, P (reprint author), Univ Missouri, Dept Comp Sci, Columbia, MO 65211 USA.
EM calyamp@missouri.edu; dovrolis@cc.gatech.edu; ljorgenson@ACM.org;
kettimut@mcs.anl.gov; bltierney@es.net; zurawski@es.net
NR 0
TC 1
Z9 1
U1 0
U2 2
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 0163-6804
EI 1558-1896
J9 IEEE COMMUN MAG
JI IEEE Commun. Mag.
PD NOV
PY 2013
VL 51
IS 11
BP 53
EP 54
PG 2
WC Engineering, Electrical & Electronic; Telecommunications
SC Engineering; Telecommunications
GA 257ZM
UT WOS:000327426500007
ER
PT J
AU Cummings, AW
Varennes, J
Leonard, F
AF Cummings, Aron W.
Varennes, Julien
Leonard, Francois
TI Electrical Contacts to Three-Dimensional Arrays of Carbon Nanotubes
SO IEEE TRANSACTIONS ON NANOTECHNOLOGY
LA English
DT Article
DE Carbon nanotubes (CNTs); contact resistance; nanocontacts; nanotube
devices
ID FIELD-EFFECT TRANSISTORS; ELECTRONIC-STRUCTURE; PERFORMANCE; ROPES
AB We use numerical simulations to investigate the properties of metal contacts to three-dimensional arrays of carbon nanotubes (CNTs). For undoped arrays top-contacted with high or low work function metals, electrostatic screening is very strong, resulting in a small Schottky barrier for current injection in the top layer and large Schottky barriers for current injection in the deeper layers. As a consequence, the majority of the current flows through the top layer of the array. Our simulations show that doping of the CNT array can alleviate this problem, even without direct contact to each tube in the array; however, we find that the charge transfer length is unusually long in arrays and increases with the number of CNT layers under the contact. We also show that a bottom gate can modulate the contact resistance, but only very weakly. These results are important for the design of electronic and optoelectronic devices based on CNT arrays, because they suggest that increasing the thickness of the array does little to improve the device performance unless the film is strongly doped at the contacts and the contact is long, or unless each tube in the array is directly contacted by the metal.
C1 [Cummings, Aron W.; Varennes, Julien; Leonard, Francois] Sandia Natl Labs, Livermore, CA 94551 USA.
RP Cummings, AW (reprint author), ICN2, Campus UAB, Bellaterra 08193, Barcelona, Spain.
EM aron.cummings@icn.cat; julien.var@gmail.com; fleonar@sandia.gov
RI Cummings, Aron/A-1426-2014
OI Cummings, Aron/0000-0003-2307-497X
FU U.S. Department of Energy, Office of Science, through the National
Institute for Nano-Engineering (NINE) at Sandia National Laboratories;
Laboratory Directed Research and Development program at Sandia National
Laboratories; a multiprogram laboratory operated by Sandia Corporation;
a Lockheed Martin Co., for the United States Department of Energy
[DEAC01-94-AL85000]
FX This project was supported in part by the U.S. Department of Energy,
Office of Science, through the National Institute for Nano-Engineering
(NINE) at Sandia National Laboratories, and in part by the Laboratory
Directed Research and Development program at Sandia National
Laboratories, a multiprogram laboratory operated by Sandia Corporation,
a Lockheed Martin Co., for the United States Department of Energy under
Contract DEAC01-94-AL85000.
NR 32
TC 0
Z9 0
U1 3
U2 24
PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
PI PISCATAWAY
PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA
SN 1536-125X
EI 1941-0085
J9 IEEE T NANOTECHNOL
JI IEEE Trans. Nanotechnol.
PD NOV
PY 2013
VL 12
IS 6
BP 1166
EP 1172
DI 10.1109/TNANO.2013.2282902
PG 7
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Materials Science, Multidisciplinary; Physics, Applied
SC Engineering; Science & Technology - Other Topics; Materials Science;
Physics
GA 258AC
UT WOS:000327428600049
ER
PT J
AU Tafen, D
Gao, MC
AF Tafen, De Nyago
Gao, Michael C.
TI Oxygen Atom Adsorption on and Diffusion into Nb(110) and Nb(100) from
First Principles
SO JOM
LA English
DT Article
ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; NIOBIUM; SURFACE; OXIDATION;
STABILITY; METALS; AES; NB
AB To understand the dynamics of oxidation of Nb, we examine the adsorption, absorption, and diffusion of an oxygen atom on, in, and into Nb(110) and Nb(100) surfaces, respectively, using density functional theory. Our calculations predict that the oxygen atom adsorbs on the threefold site on Nb(110) and the fourfold hollow site on Nb(100), and the adsorption energy is -5.08 eV and -5.18 eV, respectively. We find the long and short bridge sites to be transition states for O diffusion on Nb(110), while the on-top site is a rank-2 saddle point. In the subsurface region, the oxygen atom prefers the octahedral site, as in bulk niobium. Our results show also that the O atom is more stable on Nb(110) subsurface than on Nb(100) subsurface. The diffusion of oxygen atoms into niobium surfaces passes through transition states where the oxygen atom is coordinated to four niobium atoms. The diffusion barriers of the oxygen atom into Nb(110) and Nb(100) are 1.81 eV and 2.05 eV, respectively. An analysis of the electronic density of states reveals the emergence of well-localized electronic states below the lowest states of clean Nb surfaces due to d-p orbital hybridization.
C1 [Tafen, De Nyago; Gao, Michael C.] Natl Energy Technol Lab, Albany, OR 97321 USA.
[Tafen, De Nyago; Gao, Michael C.] URS Corp, Albany, OR 97321 USA.
RP Tafen, D (reprint author), Natl Energy Technol Lab, 1450 Queen Ave SW, Albany, OR 97321 USA.
EM denyago.tafen@contr.netl.doe.gov
OI Tafen, De Nyago/0000-0002-4360-9508
FU National Energy Technology Laboratory's (NETL) ongoing research on
Turbines Materials Development for Oxy-combustion Environments under the
RES [DE-FE-0004000]; Texas Advanced Computing Center (TACC) [DMR120048];
National Science Foundation [OCI-1053575]
FX This technical effort was performed in support of the National Energy
Technology Laboratory's (NETL) ongoing research on Turbines Materials
Development for Oxy-combustion Environments under the RES Contract
DE-FE-0004000. This work used the computing facility at the Texas
Advanced Computing Center (TACC) through Award# DMR120048 by the Extreme
Science and Engineering Discovery Environment (XSEDE), which is
supported by National Science Foundation grant number OCI-1053575. "This
report was prepared as an account of work sponsored by an agency of the
United States Government. Neither the United States Government nor any
agency thereof, nor any of their employees, makes any warranty, express
or implied, or assumes any legal liability or responsibility for the
accuracy, completeness, or usefulness of any information, apparatus,
product, or process disclosed, or represents that its use would not
infringe privately owned rights. Reference herein to any specific
commercial product, process, or service by trade name, trademark,
manufacturer, or otherwise does not necessarily constitute or imply its
endorsement, recommendation, or favoring by the United States Government
or any agency thereof. The views and opinions of authors expressed
herein do not necessarily state or reflect those of the United States
Government or any agency thereof."
NR 31
TC 2
Z9 2
U1 2
U2 15
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1047-4838
EI 1543-1851
J9 JOM-US
JI JOM
PD NOV
PY 2013
VL 65
IS 11
BP 1473
EP 1481
DI 10.1007/s11837-013-0735-8
PG 9
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Mineralogy; Mining & Mineral Processing
SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy;
Mining & Mineral Processing
GA 258ZE
UT WOS:000327496400015
ER
PT J
AU Kim, S
Park, JS
AF Kim, Sungtae
Park, J. S.
TI Ab Initio Calculated Thermodynamic Properties of Mo5SiB2 Phase and
Nb5SiB2 Phase
SO JOM
LA English
DT Article
AB Due to their attractive high-temperature properties, multiphase Mo-Si-B alloys in the Mo-rich Mo-Si-B ternary system have been identified for high-temperature applications. The ternary intermetallic T-2 (Mo5SiB2) phase is a central feature of the phase equilibria within this ternary system. Experimental stability analyses of the T-2 phase shows its broad homogeneous composition ranges that can yield a constitutional defect structure such as vacancies for Mo-rich compositions and antisite defects for Mo-lean compositions. Previous thermodynamic model did not conform to the defect structures as reported in experiments, and thus subsequently a new sublattice thermodynamic model for the T-2 phase is initiated in this study. To support the new sublattice thermodynamic model, ab initio calculations were implemented to compute formation energy data. The calculated formation energy data explain a source for broad compositional homogeneity range of T-2 structure.
C1 [Kim, Sungtae] Sandia Natl Labs, Def Waste Management Programs, Carlsbad, NM 88220 USA.
[Park, J. S.] Hanbat Natl Univ, Dept Mat Sci & Engn, Taejon 305719, South Korea.
RP Kim, S (reprint author), Sandia Natl Labs, Def Waste Management Programs, 4100 Natl Pk Highway, Carlsbad, NM 88220 USA.
EM sunkim@sandia.gov
NR 10
TC 0
Z9 0
U1 2
U2 8
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1047-4838
EI 1543-1851
J9 JOM-US
JI JOM
PD NOV
PY 2013
VL 65
IS 11
BP 1482
EP 1486
DI 10.1007/s11837-013-0770-5
PG 5
WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical
Engineering; Mineralogy; Mining & Mineral Processing
SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy;
Mining & Mineral Processing
GA 258ZE
UT WOS:000327496400016
ER
PT J
AU Hu, HS
Kowalski, K
AF Hu, Han-Shi
Kowalski, Karol
TI Excitation Energies with Cost-Reduced Variant of the Active-Space
EOMCCSDT Method: The EOMCCSDt-(3)over-bar Approach
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID EQUATION-OF-MOTION; COUPLED-CLUSTER METHODS; EXCITED ELECTRONIC STATES;
SINGLE-REFERENCE FORMALISM; SYMMETRY-ADAPTED-CLUSTER;
CONFIGURATION-INTERACTION; TRANSITION-PROBABILITIES; RESPONSE FUNCTIONS;
BUILDING-BLOCKS; LINEAR-RESPONSE
AB In this paper, we discuss the performance of several simplified variants of equation-of-motion coupled cluster method (EOMCC) with iterative inclusion of singles, doubles, and active-space triples (EOMCCSDt). In particular, we explore simplified EOMCCSDt approaches that enable one to generate the triply excited amplitudes in an on-the-fly manner. The original EOMCCSDt formulation has already demonstrated great success in encapsulating the most important excited-state correlation effects due to triples. In analogy to the original EOMCCSDT-3 formulation, the proposed approach can bypass the typical bottlenecks associated with the need for storing triply excited amplitudes. In this paper, we illustrate the performance of several approximate EOMCCSDt methods, named EOMCCSDt-(3) over bar and energies close to the EOMCCSDt ones. The extrapolation of excitation energies for basis sets ranging from cc-pVDZ to cc-pV6Z for N-2 and C-2 shows very good convergence to the experimental results for states dominated by single excitations. The performance of the EOMCCSDt-(3) over barx approach is also compared with the results obtained with popular CCSDR(3) and CC3 approaches.
C1 [Hu, Han-Shi; Kowalski, Karol] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA.
RP Kowalski, K (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, K8-91,POB 999, Richland, WA 99352 USA.
EM karol.kowalski@pnl.gov
FU Extreme Scale Computing Initiative, a Laboratory Directed Research and
Development Program at Pacific Northwest National Laboratory; U.S.
Department of Energy by the Battelle Memorial Institute
[DE-AC06-76RLO-1830]; Department of Energy's Office of Biological and
Environmental Research
FX H.S.H. acknowledges Dr. Kiran Bhaskaran-Nair for helpful discussion and
Dr. Kenneth Lopata for helpful proof reading of the manuscript. This
work was supported by the Extreme Scale Computing Initiative (H.S.H.,
K.K.), a Laboratory Directed Research and Development Program at Pacific
Northwest National Laboratory. All calculations have been performed
using EMSL, a national scientific user facility sponsored by the
Department of Energy's Office of Biological and Environmental Research
and located at Pacific Northwest National Laboratory. The Pacific
Northwest National Laboratory is operated for the U.S. Department of
Energy by the Battelle Memorial Institute under Contract No.
DE-AC06-76RLO-1830.
NR 78
TC 2
Z9 2
U1 0
U2 9
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD NOV
PY 2013
VL 9
IS 11
BP 4761
EP 4768
DI 10.1021/ct400501z
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 252WV
UT WOS:000327044500010
PM 26583394
ER
PT J
AU Nicolai, A
Zhu, P
Sumpter, BG
Meunier, V
AF Nicolai, Adrien
Zhu, Pan
Sumpter, Bobby G.
Meunier, Vincent
TI Molecular Dynamics Simulations of Graphene Oxide Frameworks
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID BORONIC ACIDS; FREE-ENERGY; RESP MODEL; IMPLEMENTATION; MECHANICS;
ALKYL; AMBER; WELL
AB We use quantum mechanical calculations to develop a full set of force field parameters in order to perform molecular dynamics simulations to understand and optimize the molecular storage properties inside graphene oxide frameworks (GOFs). A set of boron-related parameters for commonly used empirical force fields is determined to describe the nonbonded and bonded interactions between linear boronic acid linkers and graphene sheets of GOF materials. The transferability of the parameters is discussed and their validity is quantified by comparing quantum mechanical and molecular mechanical structural and vibrational properties. The application of the model to the dynamics of water inside the GOFs reveals significant variations in structural flexibility depending on the linker density, which is shown to be usable as a tuning parameter for desired diffusion properties.
C1 [Nicolai, Adrien; Zhu, Pan; Meunier, Vincent] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA.
[Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
RP Meunier, V (reprint author), Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA.
EM meuniv@rpi.edu
RI Meunier, Vincent/F-9391-2010; Sumpter, Bobby/C-9459-2013
OI Meunier, Vincent/0000-0002-7013-179X; Sumpter, Bobby/0000-0001-6341-0355
FU Office of Naval Research; Center for Nanophase Materials Sciences;
Office of Science, U.S. Department of Energy
FX A.N. thanks Jingsong Huang (Oak Ridge National Laboratory) for helpful
discussions and Jonathan R. Owens for manuscript review. Work at RPI was
supported by the Office of Naval Research. Calculations were done on the
Computational Center for Nanotechnology Innovations (CCNI) cluster, at
Rensselaer Polytechnic Institute (RPI), and the Center for Nanophase
Materials Sciences (CNMS) cluster at Oak Ridge National Laboratory
(ORNL). B.G.S. was supported by the Center for Nanophase Materials
Sciences, which is sponsored at Oak Ridge National Laboratory by the
Office of Science, U.S. Department of Energy.
NR 26
TC 12
Z9 12
U1 9
U2 89
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD NOV
PY 2013
VL 9
IS 11
BP 4890
EP 4900
DI 10.1021/ct4006097
PG 11
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 252WV
UT WOS:000327044500024
PM 26583408
ER
PT J
AU Lopata, K
Govind, N
AF Lopata, Kenneth
Govind, Niranian
TI Near and Above Ionization Electronic Excitations with Non-Hermitian
Real-Time Time-Dependent Density Functional Theory
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID AB-INITIO; MOLECULES; ACETYLENE; STATES; PHOTOIONIZATION; DYNAMICS;
VALENCE; PHOTOABSORPTION; SPECTROSCOPY; CONTINUUM
AB We present a real-time time-dependent density functional theory (RT-TDDFT) prescription for capturing near and post-ionization excitations based on non-Hermitian von Neumann density matrix propagation with atom-centered basis sets, tuned range-separated DFT, and a phenomenological imaginary molecular orbital-based absorbing potential to mimic coupling to the continuum. The computed extreme ultraviolet absorption spectra for acetylene (C2H2), water (H2O), and Freon 12 (CF2Cl2) agree well with electron energy loss spectroscopy (EELS) data over the range of 0-50 eV. The absorbing potential removes spurious high-energy finite basis artifacts, yielding correct bound-to-bound transitions, metastable (autoionizing) resonance states, and consistent overall absorption shapes.
C1 [Lopata, Kenneth; Govind, Niranian] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA.
RP Lopata, K (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA.
EM klopata@lsu.edu; niri.govind@pnnl.gov
FU U.S. Department of Energy's Office of Biological and Environmental
Research; Department of Energy by the Battelle Memorial Institute
[DE-AC06-76RLO-1830]; EMSL; U.S. Department of Energy, Office of Basic
Energy Sciences under SciDAC program [DESC0008666]
FX The research was performed at the Environmental Molecular Sciences
Laboratory (EMSL), a national scientific user facility sponsored by the
U.S. Department of Energy's Office of Biological and Environmental
Research and located at the Pacific Northwest National Laboratory
(PNNL). PNNL is operated for the Department of Energy by the Battelle
Memorial Institute, under Contract DE-AC06-76RLO-1830. K.L. acknowledges
the William Wiley Postdoctoral Fellowship from EMSL. N.G. acknowledges
support from the U.S. Department of Energy, Office of Basic Energy
Sciences, under Grant No. DESC0008666 of the SciDAC program.
NR 61
TC 10
Z9 10
U1 1
U2 13
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD NOV
PY 2013
VL 9
IS 11
BP 4939
EP 4946
DI 10.1021/ct400569s
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 252WV
UT WOS:000327044500028
PM 26583412
ER
PT J
AU Akimov, AV
Prezhdo, OV
AF Akimov, Alexey V.
Prezhdo, Oleg V.
TI The PYXAID Program for Non-Adiabatic Molecular Dynamics in Condensed
Matter Systems
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID SENSITIZED SOLAR-CELLS; INITIO TIME-DOMAIN; CDSE QUANTUM DOTS;
BORN-OPPENHEIMER TRAJECTORIES; INTERFACIAL ELECTRON-TRANSFER; QUANTIZED
HAMILTON DYNAMICS; MULTIPLE EXCITON GENERATION; RETINAL CHROMOPHORE
MODEL; DENSITY-FUNCTIONAL THEORY; PROTON-TRANSFER REACTIONS
AB This work introduces the PYXAID program, developed for non-adiabatic molecular dynamics simulations in condensed matter systems. By applying the classical path approximation to the fewest switches surface hopping approach, we have developed an efficient computational tool that can be applied to study photoinduced dynamics at the air initio level in systems composed of hundreds of atoms and involving thousands of electronic states. The technique is used to study in detail the ultrafast relaxation of hot electrons in crystalline pentacene. The simulated relaxation occurs on a 500 fs time scale, in excellent agreement with experiment, and is driven by molecular lattice vibrations in the 200-250 cm(-1) frequency range. The PYXAID program is organized as a Python extension module and can be easily combined with other Python-driven modules, enhancing user-friendliness and flexibility of the software. The source code and additional information are available on the Web at the address http://gdriv.es/pyxaid. The program is released under the GNU General Public License.
C1 [Akimov, Alexey V.; Prezhdo, Oleg V.] Univ Rochester, Dept Chem, Rochester, NY 14627 USA.
[Akimov, Alexey V.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.
RP Prezhdo, OV (reprint author), Univ Rochester, Dept Chem, Rochester, NY 14627 USA.
EM oleg.prezhdo@rochester.edu
RI Akimov, Alexey/H-9547-2014
FU Computational Materials and Chemical Sciences Network (CMCSN) project at
Brookhaven National Laboratory [DE-AC02-98CH10886]; U.S. Department of
Energy [DE-SC0006527]; Division of Chemical Sciences, Geosciences &
Biosciences, Office of Basic Energy Sciences
FX The authors are grateful to Dhara Trivedi for comments on the
manuscript. A.V.A. was funded by the Computational Materials and
Chemical Sciences Network (CMCSN) project at Brookhaven National
Laboratory under contract DE-AC02-98CH10886 with the U.S. Department of
Energy and supported by its Division of Chemical Sciences, Geosciences &
Biosciences, Office of Basic Energy Sciences. O.V.P. acknowledges
financial support of the U.S. Department of Energy, grant DE-SC0006527.
NR 148
TC 71
Z9 71
U1 6
U2 65
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD NOV
PY 2013
VL 9
IS 11
BP 4959
EP 4972
DI 10.1021/ct400641n
PG 14
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 252WV
UT WOS:000327044500030
PM 26583414
ER
PT J
AU Nagarajan, A
Junghans, C
Matysiak, S
AF Nagarajan, Anu
Junghans, Christoph
Matysiak, Silvina
TI Multiscale Simulation of Liquid Water Using a Four-to-One Mapping for
Coarse-Graining
SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATIONS; IMPLICIT SOLVENT MODELS;
TEMPERATURE-DEPENDENCE; MAXIMUM DENSITY; RECENT PROGRESS; FREE-ENERGIES;
SOFT MATTER; PROTEINS; HYDRATION; ORDER
AB We present a multiresolution simulation scheme for the solvent environment where four atomistic water molecules are mapped onto one coarse-grained bead. Soft restraining potentials are used to allow a resolution exchange of four water molecules into a single coarse-grained site. We first study the effect of adding restraining potentials in liquid water using full all-atom simulations. The usage of very soft restraining potentials to bundle four nearest neighbor water molecules does not disrupt the hydrogen bonding patterns in the liquid water. The structural properties of the first solvation shell around hydrophobic, hydrophilic, and ionic solutes are well preserved when soft restraining potentials are added. By modeling a bundle of four water molecules as a single molecule, a smooth transition and free exchange between coarse-grained and all-atom resolution is possible by using the adaptive resolution scheme (AdResS).
C1 [Nagarajan, Anu; Matysiak, Silvina] Univ Maryland, Fischell Dept Bioengn, College Pk, MD 20742 USA.
[Junghans, Christoph] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.
RP Matysiak, S (reprint author), Univ Maryland, Fischell Dept Bioengn, College Pk, MD 20742 USA.
EM matysiak@umd.edu
RI Junghans, Christoph/G-4238-2010
OI Junghans, Christoph/0000-0003-0925-1458
FU National Science Foundation [TG-MCB110075, TG-MCB120045]; LANL
FX This research was supported in part by the National Science Foundation
through XSEDE resources provided by The Texas Advanced Computing Center
(TACC) under grant numbers [TG-MCB110075] and [TG-MCB120045]. We would
also like to thank Sebastian Fritsch for his help and support with
AdResS and the VOTCA package. Christoph Junghans thanks LANL for a
Director's fellowship.
NR 64
TC 7
Z9 7
U1 2
U2 18
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1549-9618
EI 1549-9626
J9 J CHEM THEORY COMPUT
JI J. Chem. Theory Comput.
PD NOV
PY 2013
VL 9
IS 11
BP 5168
EP 5175
DI 10.1021/ct400566j
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 252WV
UT WOS:000327044500046
PM 26583426
ER
PT J
AU Stickel, JJ
Knutsen, JS
Liberatore, MW
AF Stickel, Jonathan J.
Knutsen, Jeffrey S.
Liberatore, Matthew W.
TI Response of elastoviscoplastic materials to large amplitude oscillatory
shear flow in the parallel-plate and cylindrical-Couette geometries
SO JOURNAL OF RHEOLOGY
LA English
DT Article
ID YIELD-STRESS FLUIDS; FOURIER-TRANSFORM RHEOLOGY; ROTATIONAL VISCOMETER;
MODEL; LAOS; THIXOTROPY; RHEOMETRY; CURVES; GEL
AB Most investigations of large amplitude oscillatory shear (LAOS) rheometry to date have presumed uniform shear. The study of structured materials would especially benefit from LAOS rheometry but require the use of the larger gaps and roughened surfaces in parallel-plate and cylindrical-Couette geometries. However, in these geometries, the shear profiles are not homogeneous throughout the deformation field. For elastoviscoplastic materials undergoing LAOS in these geometries, both elastic and viscoplastic deformations may occur simultaneously, complicating the data analysis. By means of model simulations, we provide a comprehensive picture of a model elastoviscoplastic material undergoing oscillatory shear deformation in the parallel-plate and cylindrical-Couette geometries, and we compare the oscillatory signals to those obtained from a uniform-shear field. Both displacement-controlled and torque-controlled oscillatory flows were simulated. We show that using popular linear formulas for mapping displacement to strain and torque to stress results in strain and stress signals that deviate significantly from their uniform-shear counterparts. For some limited cases, specifically displacement-controlled parallel-plate and torque-controlled cylindrical-Couette oscillatory rheometry, the use of advanced mapping methods to improve the calculation of strain and stress signals was demonstrated. As an alternative, we suggest that analyzing LAOS signals via constitutive modeling provides a unifying approach. (C) 2013 The Society of Rheology.
C1 [Stickel, Jonathan J.] Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA.
[Knutsen, Jeffrey S.; Liberatore, Matthew W.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA.
RP Stickel, JJ (reprint author), Natl Bioenergy Ctr, Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA.
EM jonathan.stickel@nrel.gov
RI Liberatore, Matthew/B-6828-2008
FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable
Energy Laboratory; BioEnergy Technologies Office
FX This work was funded by the U.S. Department of Energy under Contract No.
DE-AC36-08-GO28308 with the National Renewable Energy Laboratory and
through the BioEnergy Technologies Office.
NR 46
TC 14
Z9 14
U1 2
U2 26
PU JOURNAL RHEOLOGY AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0148-6055
J9 J RHEOL
JI J. Rheol.
PD NOV
PY 2013
VL 57
IS 6
BP 1569
EP 1596
DI 10.1122/1.4820495
PG 28
WC Mechanics
SC Mechanics
GA 257BE
UT WOS:000327357100004
ER
PT J
AU Choudhary, K
Hill, LB
Kemper, TW
Sinnott, SB
AF Choudhary, Kamal
Hill, Leah B.
Kemper, Travis W.
Sinnott, Susan B.
TI Mechanisms for hyperthermal polyatomic hydrocarbon modification of PMMA
surfaces from molecular dynamics simulations
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; POLY(METHYL METHACRYLATE); POLYMER MELTS;
FILMS; ABLATION; HYDROGEN; CARBON; FLUOROCARBON; POLYSTYRENE; EROSION
AB Classical molecular dynamics simulations are performed to determine the mechanisms by which hyperthermal hydrocarbon polyatomics, which are present in low-energy plasmas, chemically modify polymer surfaces. In particular, C2H, CH3, and C3H5 are deposited on an amorphous poly (methyl methacrylate) (PMMA) substrate with kinetic energies of 4, 10, 25, and 50 eV and compared to the deposition of H at the same energies. The short-range forces on the atoms are determined using the second generation reactive empirical many-body potential, while the long-range forces are determined using a Lennard-Jones potential. The simulations predict that at all these incident energies, the chemical modification of the PMMA is limited to within a nanometer of the surface. Atoms, fragments, and incident polyatomics are further predicted to chemically attach to specific sites on the PMMA monomers at low energies and to attach to a wider range of sites at higher energies. However, no appreciable cross-linking between polymer chains is predicted to occur. Variation in the penetration depth of the deposited polyatomics or H is correlated to differences in their size and bond saturation. The greatest extent of chemical modification of the PMMA surface slab is achieved for C2H deposition with 50 eV of kinetic energy. (C) 2013 American Vacuum Society.
C1 [Choudhary, Kamal; Hill, Leah B.; Sinnott, Susan B.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA.
[Kemper, Travis W.] Natl Renewable Energy Lab, Golden, CO 80401 USA.
RP Choudhary, K (reprint author), Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA.
EM ssinn@mse.ufl.edu
RI Sinnott, Susan/P-8523-2014
OI Sinnott, Susan/0000-0002-3598-0403
FU National Science Foundation [CHE-0809376]
FX The authors gratefully acknowledge the support of the National Science
Foundation (CHE-0809376).
NR 48
TC 0
Z9 0
U1 2
U2 16
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0734-2101
J9 J VAC SCI TECHNOL A
JI J. Vac. Sci. Technol. A
PD NOV-DEC
PY 2013
VL 31
IS 6
AR 061403
DI 10.1116/1.4823477
PG 7
WC Materials Science, Coatings & Films; Physics, Applied
SC Materials Science; Physics
GA 255QC
UT WOS:000327253900023
ER
PT J
AU Jaffe, JE
Kaspar, TC
Droubay, TC
Varga, T
AF Jaffe, John E.
Kaspar, Tiffany C.
Droubay, Timothy C.
Varga, Tamas
TI Band offsets for mismatched interfaces: The special case of ZnO on CdTe
(001)
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A
LA English
DT Article
ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE
METHOD; SOLAR-CELL; ATOMIC-HYDROGEN; BASIS-SET; SEMICONDUCTORS;
ZINCBLENDE; METALS; TRANSITION
AB High-quality planar interfaces between ZnO and CdTe would be useful in optoelectronic applications. Although CdTe is zinc blende with cubic lattice constant a 6.482 angstrom while ZnO is hexagonal wurtzite with a = 3.253 angstrom and c = 5.213 angstrom, (001)-oriented cubic zinc blende ZnO films could be stabilized epitaxially on a CdTe (001) surface in an root 2 x root 2 R45 degrees configuration with a lattice mismatch of < 0.5%. Modeling such a configuration allows density-functional total-energy electronic-structure calculations to be performed on several interface arrangements (varying terminations and in-plane fractional translations) to identify the most likely form of the interface, and to predict valence-band offsets between CdTe and ZnO in each case. Growth of ZnO on Te-terminated CdTe(001) is predicted to produce small or even negative (CdTe below ZnO) valence band offsets, resulting in a Type I band alignment. Growth on Cd-terminated CdTe is predicted to produce large positive offsets for a Type II alignment as needed, for example, in solar cells. To corroborate some of these predictions, thin layers of ZnO were deposited on CdTe(001) by pulsed laser deposition, and the band alignments of the resulting heterojunctions were determined from x-ray photoelectron spectroscopy measurements. Although zinc blende ZnO could not be confirmed, the measured valence band offset (2.0-2.2 eV) matched well with the predicted value. (C) 2013 American Vacuum Society.
C1 [Jaffe, John E.; Kaspar, Tiffany C.; Droubay, Timothy C.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
[Varga, Tamas] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
RP Jaffe, JE (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, POB 999, Richland, WA 99352 USA.
EM Tiffany.Kaspar@pnnl.gov
RI Droubay, Tim/D-5395-2016
OI Droubay, Tim/0000-0002-8821-0322
FU U.S. Department of Energy's Office of Biological and Environmental
Research; Laboratory Directed Research and Development Program at PNNL
FX A portion of this research was performed using EMSL, a national
scientific user facility sponsored by the U.S. Department of Energy's
Office of Biological and Environmental Research and located at the
Pacific Northwest National Laboratory. This research was supported by
the Laboratory Directed Research and Development Program at PNNL.
NR 37
TC 0
Z9 0
U1 0
U2 16
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0734-2101
J9 J VAC SCI TECHNOL A
JI J. Vac. Sci. Technol. A
PD NOV-DEC
PY 2013
VL 31
IS 6
AR 061102
DI 10.1116/1.4816951
PG 9
WC Materials Science, Coatings & Films; Physics, Applied
SC Materials Science; Physics
GA 255QC
UT WOS:000327253900006
ER
PT J
AU Manandhar, K
Trenary, M
Otani, S
Zapol, P
AF Manandhar, Kedar
Trenary, Michael
Otani, Shigeki
Zapol, Peter
TI Dissociation of trimethylgallium on the ZrB2(0001) surface
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A
LA English
DT Article
ID PULSED-LASER DEPOSITION; MOLECULAR-BEAM EPITAXY; GROUP-III NITRIDES;
THREADING DISLOCATIONS; GALLIUM NITRIDE; GROWTH; GAN; DECOMPOSITION;
ADSORPTION; SI(100)
AB X-ray photoelectron spectroscopy and reflection absorption infrared spectroscopy (RAIRS) have been used to study the dissociative adsorption of trimethylgallium (TMG) on the ZrB2(0001) surface. Spectra were obtained as a function of annealing temperature following TMG exposure at temperatures of 95 and 300 K, and also as a function of TMG exposure for a surface temperature of 300 K. After annealing above 220 K, a significant decrease in the relative concentration of carbon and gallium occurred accompanied by a shift of similar to 0.2 eV in the Ga 2p(3/2) binding energy. The RAIR spectra show that after annealing to similar to 220 K, only one CH3 deformation band at 1196 cm(-1) remains, the intensity of which is considerably decreased indicating loss of at least one methyl group from TMG. Further annealing leads to the sequential loss of the other methyl groups. The first methyl desorbs while the last two dissociate to deposit two C atoms per TMG molecule onto the ZrB2 surface. (C) 2013 American Vacuum Society.
C1 [Manandhar, Kedar; Trenary, Michael] Univ Illinois, Dept Chem, Chicago, IL 60607 USA.
[Otani, Shigeki] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan.
[Zapol, Peter] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
RP Manandhar, K (reprint author), Univ Illinois, Dept Chem, 845W Taylor St, Chicago, IL 60607 USA.
EM mtrenary@uic.edu
RI Zapol, Peter/G-1810-2012
OI Zapol, Peter/0000-0003-0570-9169
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences-Materials Science [DE-AC02-06CH11357]; National Science
Foundation [CHE-1012201]
FX This work was supported by the U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences-Materials Science under
Contract No. DE-AC02-06CH11357. K. M. and M. T. also acknowledge partial
support from the National Science Foundation under grant CHE-1012201.
NR 55
TC 2
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U1 0
U2 9
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 0734-2101
J9 J VAC SCI TECHNOL A
JI J. Vac. Sci. Technol. A
PD NOV-DEC
PY 2013
VL 31
IS 6
AR UNSP 061405
DI 10.1116/1.4826881
PG 9
WC Materials Science, Coatings & Films; Physics, Applied
SC Materials Science; Physics
GA 255QC
UT WOS:000327253900025
ER
PT J
AU Anderson, EH
Chao, WL
Gullikson, EM
Rekawa, S
Andresen, N
Naulleau, P
AF Anderson, Erik H.
Chao, Weilun
Gullikson, Eric M.
Rekawa, Senajith
Andresen, Nord
Naulleau, Patrick
TI Silicon nitride zoneplates and packaging for extreme ultraviolet
instruments
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID GRATINGS
AB Diffractive optical elements such as Fresnel zoneplate lenses have many uses at extreme ultraviolet (EUV), particularly in short focal length, high-resolution applications. However, the diffraction efficiency of a pure absorption zoneplate is limited to about 10%, and it suffers additional loss through the membrane support material. To this end, the authors explored the possibility of silicon nitride (Si3N4) as a EUV phase shifting material. At an etched depth of 244 nm, they measured a diffraction efficiency of 18% in the first order and 18% in the zero order, which compares favorably to an amplitude grating of 10% and 25%, respectively. The measured efficiency as a function of etch depth matches the scalar theory quite well using a measured EUV index of refraction 0.9790 +0.0066i at the wavelength of 13.5 nm. To further increase the efficiency, zoneplates were made freestanding, with the support membrane completely removed, and a 15% absolute efficiency was obtained. Vector electromagnetic calculations showed that at normal incidence, these optics produce excellent wavefront and efficiency for outer zones of 50nm or larger. Zoneplates of narrower zones or those illuminated obliquely can suffer larger wavefront errors and low efficiency and would require careful design optimization. In the work, the authors also demonstrated a technique to package zoneplates and associated apertures for high precision insertion and removal from a EUV instrument. This technique has yielded alignment accuracy from a few microns to few 10s microns, depending on the exact design. (C) 2013 American Vacuum Society.
C1 [Anderson, Erik H.; Chao, Weilun; Gullikson, Eric M.; Rekawa, Senajith; Andresen, Nord; Naulleau, Patrick] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA.
RP Anderson, EH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Mail Stop 2-400,1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM wlchao@lbl.gov
FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials
Sciences and Engineering Division [DE-AC02-05CH11231]
FX This work was supported by the U.S. Department of Energy, Office of
Basic Energy Sciences, Materials Sciences and Engineering Division,
under Contract No. DE-AC02-05CH11231.
NR 9
TC 0
Z9 0
U1 3
U2 4
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06F606
DI 10.1116/1.4826695
PG 5
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300025
ER
PT J
AU Czaplewski, DA
Ocola, LE
AF Czaplewski, David A.
Ocola, Leonidas E.
TI Variation of backscatter electron intensity
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID PROXIMITY-EFFECT CORRECTION; BEAM LITHOGRAPHY; NANOMETER-SCALE;
PROTEINS; CRYSTAL; SILICON; QUBIT
AB The authors report experimental data on the dose contribution of backscattered electrons on a silicon substrate. The backscattered electron intensity, i.e., the relative dose contribution from backscattered electrons with respect to direct write dose, is not constant, but varies with the percentage of the total dose received by backscattered electrons. In order to measure the backscattered electron contribution, the position and number of electrons are controlled by electron beam lithography. The dose contribution is measured using a negative electron beam resist, which quantifies the electron interactions in a nanoscale volume on the surface of the substrate. The data presented here will lead to improvements in proximity effect correction algorithms and ultimately improve pattern creation using electron beam lithography. (C) 2013 American Vacuum Society.
C1 [Czaplewski, David A.; Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
RP Czaplewski, DA (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM dczaplewski@anl.gov
OI Ocola, Leonidas/0000-0003-4990-1064
FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of
Science, Office of Basic Energy Sciences User Facility
[DE-AC02-06CH11357]
FX This work was performed at the Center for Nanoscale Materials, a U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
User Facility under Contract No. DE-AC02-06CH11357.
NR 30
TC 0
Z9 0
U1 0
U2 2
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06F202
DI 10.1116/1.4818881
PG 5
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300004
ER
PT J
AU Divan, R
Rosenthal, D
Ogando, K
Ocola, LE
Rosenmann, D
Moldovan, N
AF Divan, Ralu
Rosenthal, Dan
Ogando, Karim
Ocola, Leonidas E.
Rosenmann, Daniel
Moldovan, Nicolaie
TI Metal-assisted etching of silicon molds for electroforming
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID ZONE PLATES; POROUS SILICON; NANOWIRES; FABRICATION; ARRAYS;
LITHOGRAPHY; NANOSTRUCTURES; DIAMETER
AB Ordered arrays of high-aspect-ratio micro/nanostructures in semiconductors stirred a huge scientific interest due to their unique one-dimensional physical morphology and the associated electrical, mechanical, chemical, optoelectronic, and thermal properties. Metal-assisted chemical etching enables fabrication of such high aspect ratio Si nanostructures with controlled diameter, shape, length, and packing density, but suffers from structure deformation and shape inconsistency due to uncontrolled migration of noble metal structures during etching. Hereby the authors prove that a Ti adhesion layer helps in stabilizing gold structures, preventing their migration on the wafer surface while not impeding the etching. Based on this finding, the authors demonstrate that the method can be used to fabricate linear Fresnel zone plates. (C) 2013 American Vacuum Society.
C1 [Divan, Ralu; Ocola, Leonidas E.; Rosenmann, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Rosenthal, Dan] Illinois Math & Sci Acad, Aurora, IL 60506 USA.
[Ogando, Karim] Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina.
[Ogando, Karim] Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina.
[Moldovan, Nicolaie] Adv Diamond Technol Inc, Romeoville, IL 60446 USA.
RP Divan, R (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM divan@anl.gov
OI Ocola, Leonidas/0000-0003-4990-1064
FU U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences [DE-AC02-06CH11357]; Argonne, a U.S. Department of Energy
Office of Science laboratory [DE-AC02-06CH11357]
FX Use of the Center for Nanoscale Materials, Argonne National Laboratory
was supported by the U.S. Department of Energy, Office of Science,
Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357.
The submitted manuscript has been created by UChicago Argonne, LLC,
Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S.
Department of Energy Office of Science laboratory, is operated under
Contract No. DE-AC02-06CH11357.
NR 36
TC 0
Z9 0
U1 2
U2 17
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06FF03
DI 10.1116/1.4821651
PG 6
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300053
ER
PT J
AU Li, LZ
Trusheim, M
Gaathon, O
Kisslinger, K
Cheng, CJ
Lu, M
Su, D
Yao, XW
Huang, HC
Bayn, I
Wolcott, A
Osgood, RM
Englund, D
AF Li, Luozhou
Trusheim, Matthew
Gaathon, Ophir
Kisslinger, Kim
Cheng, Ching-Jung
Lu, Ming
Su, Dong
Yao, Xinwen
Huang, Hsu-Cheng
Bayn, Igal
Wolcott, Abraham
Osgood, Richard M., Jr.
Englund, Dirk
TI Reactive ion etching: Optimized diamond membrane fabrication for
transmission electron microscopy
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID SINGLE-CRYSTAL-DIAMOND; NITROGEN-VACANCY CENTERS; CROSS-SECTION
SPECIMENS; VAPOR-DEPOSITED DIAMOND; RAMAN-SPECTROSCOPY; SAMPLE
PREPARATION; COLOR-CENTERS; BEAM; IMPLANTATION; DAMAGE
AB Commonly used preparation method for thin diamond membranes by focused ion beam (FIB) techniques results in surface damage. Here, the authors introduce an alternative method based on reactive ion etching (RIE). To compare these methods, cross-sectional samples are produced in single crystal diamond, a material that has generated growing interest for a variety of applications. The samples are examined by Raman spectroscopy and high-resolution transmission electron microscopy (TEM). Raman spectra indicate that the crystalline structure of the RIE-processed diamond is preserved, while the FIB-processed diamond membrane has a broad-background sp(2) feature. Atomic-resolution TEM imaging demonstrates that the RIE-based process produces no detectable damage, while the FIB-processed sample has an amorphous carbon layer of about 11 nm thick. These findings show that the RIE-based process allows the production of diamond TEM samples with reduced near-surface damage and can thus enable direct examination of growth defects and crystallographic damage induced by processes such as ion implantation and bombardment. (C) 2013 American Vacuum Society.
C1 [Li, Luozhou; Yao, Xinwen; Huang, Hsu-Cheng; Osgood, Richard M., Jr.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA.
[Trusheim, Matthew; Gaathon, Ophir; Osgood, Richard M., Jr.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA.
[Trusheim, Matthew; Gaathon, Ophir; Bayn, Igal; Englund, Dirk] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA.
[Kisslinger, Kim; Cheng, Ching-Jung; Lu, Ming; Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Wolcott, Abraham] Columbia Univ, Dept Chem, New York, NY 10027 USA.
RP Li, LZ (reprint author), Columbia Univ, Dept Elect Engn, New York, NY 10027 USA.
EM ll2670@columbia.edu; englund@mit.edu
RI Kisslinger, Kim/F-4485-2014; Su, Dong/A-8233-2013
OI Su, Dong/0000-0002-1921-6683
FU U.S. Air Force Office of Scientific Research Quantum Memories MURI,
PECASE, and Young Investigator Program (AFOSR) [FA9550-11-1-0014];
Defense Threat Reduction Agency [HDTRA1-11-1-0022]; U.S. Department of
Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]
FX This work was supported by the U.S. Air Force Office of Scientific
Research Quantum Memories MURI, PECASE, and Young Investigator Program
(AFOSR Grant No. FA9550-11-1-0014, supervised by Gernot Pomrenke), and
in part by the Defense Threat Reduction Agency, Basic Research Award
#HDTRA1-11-1-0022 to Columbia University. Research was carried out in
part at the Center for Functional Nanomaterials, Brookhaven National
Laboratory, which was supported by the U.S. Department of Energy, Office
of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The
authors would like to thank Mircea Cotlet, Aaron Stein, Fernando Camino,
Hsin-hui Huang, and Sergio Allegri for their assistance in this work.
NR 51
TC 7
Z9 7
U1 1
U2 26
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06FF01
DI 10.1116/1.4813559
PG 6
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300051
ER
PT J
AU Li, W
Esquiroz, VM
Urbanski, L
Patel, D
Menoni, CS
Marconi, MC
Stein, A
Chao, WL
Anderson, EH
AF Li, Wei
Esquiroz, Victor Martinez
Urbanski, Lukasz
Patel, Dinesh
Menoni, Carmen S.
Marconi, Mario C.
Stein, Aaron
Chao, Weilun
Anderson, Erik H.
TI Defect-free periodic structures using extreme ultraviolet Talbot
lithography in a table-top system
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID X-RAY LASER; ENHANCED RAMAN-SCATTERING; COHERENT DIFFRACTION
LITHOGRAPHY; INTERFEROMETRIC LITHOGRAPHY; INTERFERENCE LITHOGRAPHY;
WAVELENGTH RESOLUTION; PHOTONIC CRYSTALS; REPETITION RATE; LARGE-AREA;
FABRICATION
AB A compact nanofabrication system that combines Talbot lithography and a table-top extreme ultraviolet laser is presented. The lithographic method based on the Talbot effect provides a robust and simple experimental setup that is capable to print periodic structures over millimeter square areas free of defects. Test structures were printed and transferred into metal layers showing a complete coherent extreme ultraviolet lithographic process in a table-top system. (C) 2013 American Vacuum Society.
C1 [Li, Wei; Esquiroz, Victor Martinez; Urbanski, Lukasz; Patel, Dinesh; Menoni, Carmen S.; Marconi, Mario C.] Colorado State Univ, Engn Res Ctr Extreme Ultraviolet Sci & Technol, Ft Collins, CO 80523 USA.
[Li, Wei; Esquiroz, Victor Martinez; Urbanski, Lukasz; Patel, Dinesh; Menoni, Carmen S.; Marconi, Mario C.] Colorado State Univ, Elect & Comp Engn Dept, Ft Collins, CO 80523 USA.
[Stein, Aaron] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.
[Chao, Weilun; Anderson, Erik H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA.
RP Li, W (reprint author), Colorado State Univ, Engn Res Ctr Extreme Ultraviolet Sci & Technol, Ft Collins, CO 80523 USA.
EM Mario.marconi@colostate.edu
OI Stein, Aaron/0000-0003-4424-5416
FU National Science Foundation [ECCS 0901806]; NSF ERC for Extreme
Ultraviolet Science and Technology [EEC 0310717]; NSF SBIR program
[1248924]; U.S. Department of Energy, Office of Basic Energy Sciences
[DE-AC02-98CH10886]
FX This work was supported by the National Science Foundation, Award ECCS
0901806, and the NSF ERC for Extreme Ultraviolet Science and Technology,
Award EEC 0310717. Partial support from the NSF SBIR program through
Grant 1248924 is also acknowledged. The e-beam written mask research was
carried out at the Center for Functional Nanomaterials, Brookhaven
National Laboratory, which is supported by the U.S. Department of
Energy, Office of Basic Energy Sciences, under Contract No.
DE-AC02-98CH10886.
NR 40
TC 8
Z9 8
U1 1
U2 9
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06F604
DI 10.1116/1.4826344
PG 7
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300023
ER
PT J
AU Ocola, LE
Palacios, E
AF Ocola, Leonidas E.
Palacios, Edgar
TI Advances in ion beam micromachining for complex 3D microfluidics
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID MICROFABRICATION
AB In this paper, the authors present microfluidic mixers containing complex curvilinear and several tens of microns deep three-dimensional (3D) geometries used to decrease mixing lengths in passive microfluidic systems. In order to create these 3D geometries, the authors use ion beam micromachining (IB mu M) and address redeposition and exposure strategy effects that follow this type of fabrication. Results of this work clearly demonstrate that fabrication of 3D microfluidic mixers using IB mu M is achievable for real practical applications. In order to scale up to the tens of microns width and depth, and hundreds of microns in length fabrication, high current is required. This raises unique challenges of redeposition handling. This was achieved by realizing that redeposited silicon can be removed with an extended buffered oxide etch. In addition, data management and writing strategies not encountered in electron beam lithography have to be considered when designing the solid to be milled. Both designs, straight 3D and serpentine 3D mixers, were significantly faster mixers than the standard focusing mixer with no 3D texturing. This demonstrates that adding programmed depth variations to existing microfluidic devices can open new opportunities in microfluidic research and IB mu M. (C) 2013 American Vacuum Society.
C1 [Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA.
[Palacios, Edgar] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.
[Palacios, Edgar] Univ Illinois, Dept Civil & Mat Engn, Chicago, IL 60607 USA.
RP Ocola, LE (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM ocola@anl.gov
OI Ocola, Leonidas/0000-0003-4990-1064
FU Department of Energy [DE-AC02-06CH11357]; U.S. Department of Energy,
Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX This work was supported by the Department of Energy under Contract No.
DE-AC02-06CH11357. Use of the Center for Nanoscale Materials was
supported by the U.S. Department of Energy, Office of Basic Energy
Sciences, under Contract No. DE-AC02-06CH11357.
NR 21
TC 1
Z9 1
U1 4
U2 16
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 06F401
DI 10.1116/1.4819302
PG 7
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300008
ER
PT J
AU Voss, LF
Reinhardt, CE
Graff, RT
Conway, AM
Shao, QH
Nikolic, RJ
Dar, MA
Cheung, CL
AF Voss, Lars F.
Reinhardt, Cathy E.
Graff, Robert T.
Conway, Adam M.
Shao, Qinghui
Nikolic, Rebecca J.
Dar, Mushtaq A.
Cheung, Chin L.
TI Analysis of strain in dielectric coated three dimensional Si micropillar
arrays
SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B
LA English
DT Article
ID RAMAN MEASUREMENTS; SILICON; BORON; (10)BORON
AB Stress induced in [100] oriented Si circular micropillars by coatings of low pressure chemical vapor deposited B-10, SiyNx, and plasma enhanced chemical vapor deposited SiO2 were measured using micro-Raman spectroscopy. Both tensile and compressive strains in the Si micropillars were observed. Exceptionally large stresses were found to exist in some of the measured Si micropillars. The cross-sectional shapes of these structures were shown to be an important factor in correlating their strain concentrations which could fracture the micropillar. (C) 2013 American Vacuum Society.
C1 [Voss, Lars F.; Reinhardt, Cathy E.; Graff, Robert T.; Conway, Adam M.; Shao, Qinghui; Nikolic, Rebecca J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.
[Dar, Mushtaq A.; Cheung, Chin L.] Univ Nebraska, Dept Chem, Lincoln, NE 68588 USA.
[Dar, Mushtaq A.; Cheung, Chin L.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA.
RP Voss, LF (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA.
EM voss5@llnl.gov
RI Cheung, Chin Li/B-8270-2013
FU U.S. Department of Homeland Security, Domestic Nuclear Detection Office
[IAA HSHQDC-08-C-00874]; LLNL Laboratory Directed Research and
Development; U.S. DOE by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344, LLNL-JRNL-426150]
FX The authors acknowledge the assistance of Chris Orme with Raman
measurements. This work has been partially supported by the U.S.
Department of Homeland Security, Domestic Nuclear Detection Office,
under competitively awarded IAA HSHQDC-08-C-00874. This support does not
constitute an express or implied endorsement on the part of the
Government. This work has been partially supported by LLNL Laboratory
Directed Research and Development. This work was performed under the
auspices of the U.S. DOE by Lawrence Livermore National Laboratory under
Contract DE-AC52-07NA27344, LLNL-JRNL-426150.
NR 30
TC 2
Z9 2
U1 0
U2 4
PU A V S AMER INST PHYSICS
PI MELVILLE
PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA
SN 1071-1023
J9 J VAC SCI TECHNOL B
JI J. Vac. Sci. Technol. B
PD NOV
PY 2013
VL 31
IS 6
AR 060602
DI 10.1116/1.4826500
PG 5
WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology;
Physics, Applied
SC Engineering; Science & Technology - Other Topics; Physics
GA 262BE
UT WOS:000327708300061
ER
PT J
AU Almagro, JC
Gilliland, GL
Scott, J
Larrick, JW
Pluckthun, A
Veldman, T
Adams, GP
Parren, PWHI
Chester, KA
Bradbury, A
Reichert, JM
Huston, JS
AF Almagro, Juan Carlos
Gilliland, Gary L.
Scott, Jamie
Larrick, James W.
Plueckthun, Andreas
Veldman, Trudi
Adams, Gregory P.
Parren, Paul W. H. I.
Chester, Kerry A.
Bradbury, Andrew
Reichert, Janice M.
Huston, James S.
TI Antibody Engineering and Therapeutics Conference The Annual Meeting of
the Antibody Society, December 8-12, 2013, Huntington Beach, CA
SO MABS
LA English
DT Editorial Material
AB The Antibody Engineering and Therapeutics conference, which serves as the annual meeting of The Antibody Society, will be held in Huntington Beach, CA from Sunday December 8 through Thursday December 12, 2013. The scientific program will cover the full spectrum of challenges in antibody research and development, and provide updates on recent progress in areas from basic science through approval of antibody therapeutics. Keynote presentations will be given by Leroy Hood (Institute of System Biology), who will discuss a systems approach for studying disease that is enabled by emerging technology; Douglas Lauffenburger (Massachusetts Institute of Technology), who will discuss systems analysis of cell communication network dynamics for therapeutic biologics design; David Baker (University of Washington), who will describe computer-based design of smart protein therapeutics; and William Schief (The Scripps Research Institute), who will discuss epitope-focused immunogen design. In this preview of the conference, the workshop and session chairs share their thoughts on what conference participants may learn in sessions on: (1) three-dimensional structure antibody modeling; (2) identifying clonal lineages from next-generation data sets of expressed V-H gene sequences; (3) antibodies in cardiometabolic medicine; (4) the effects of antibody gene variation and usage on the antibody response; (5) directed evolution; (6) antibody pharmacokinetics, distribution and off-target toxicity; (7) use of knowledge-based design to guide development of complementarity-determining regions and epitopes to engineer or elicit the desired antibody; (8) optimizing antibody formats for immunotherapy; (9) antibodies in a complex environment; (10) polyclonal, oligoclonal and bispecific antibodies; (11) antibodies to watch in 2014; and (12) polyreactive antibodies and polyspecificity.
C1 [Almagro, Juan Carlos] Pfizer, Boston, MA USA.
[Gilliland, Gary L.] Janssen Res & Dev LLC, Spring House, PA USA.
[Scott, Jamie] Simon Fraser Univ, Burnaby, BC V5A 1S6, Canada.
[Larrick, James W.] Veloc Pharmaceut Dev, San Francisco, CA USA.
[Plueckthun, Andreas] Univ Zurich, Zurich, Switzerland.
[Veldman, Trudi] AbbVie Biores Ctr, Worcester, MA USA.
[Adams, Gregory P.] Fox Chase Canc Ctr, Philadelphia, PA 19111 USA.
[Parren, Paul W. H. I.] Genmab, Utrecht, Netherlands.
[Chester, Kerry A.] UCL, London, England.
[Bradbury, Andrew] Los Alamos Natl Lab, Los Alamos, NM USA.
[Reichert, Janice M.] Reichert Biotechnol Consulting LLC, Framingham, MA USA.
[Huston, James S.] Huston BioConsulting LLC, Boston, MA USA.
RP Reichert, JM (reprint author), Reichert Biotechnol Consulting LLC, Framingham, MA USA.
EM janice.reichert@landesbioscience.com
OI Bradbury, Andrew/0000-0002-5567-8172
NR 0
TC 2
Z9 2
U1 0
U2 10
PU LANDES BIOSCIENCE
PI AUSTIN
PA 1806 RIO GRANDE ST, AUSTIN, TX 78702 USA
SN 1942-0862
EI 1942-0870
J9 MABS-AUSTIN
JI mAbs
PD NOV 1
PY 2013
VL 5
IS 6
BP 817
EP 825
DI 10.4161/mabs.26545
PG 9
WC Medicine, Research & Experimental
SC Research & Experimental Medicine
GA 258CN
UT WOS:000327436700001
ER
PT J
AU Cheng, AX
Gou, JY
Yu, XH
Yang, HJ
Fang, X
Chen, XY
Liu, CJ
AF Cheng, Ai-Xia
Gou, Jin-Ying
Yu, Xiao-Hong
Yang, Huijun
Fang, Xin
Chen, Xiao-Ya
Liu, Chang-Jun
TI Characterization and Ectopic Expression of a Populus Hydroxyacid
Hydroxycinnamoyltransferase
SO MOLECULAR PLANT
LA English
DT Article
DE cutin; suberin; ferulate; BAHD; acyltransferase; Populus
ID ACID O-HYDROXYCINNAMOYLTRANSFERASE; ARABIDOPSIS-THALIANA; POTATO-TUBER;
TISSUE-CULTURES; CUTIN POLYESTER; LIPID POLYESTER; BRASSICA-NAPUS;
HIGHER-PLANTS; SUBERIN; BIOSYNTHESIS
AB A Populus BAHD/HXXXD acyltransferase was identified as hydroxyacid/fatty alcohol hydroxycinnamoyltransferase. When ectopically expressed in Arabidopsis, it increased the incorporation of ferulate in both suberin and cutin polyesters, which consequently enhanced the tolerance of transgenic plants to salt stress.Cutinized and suberized cell walls in plants constitute physiologically important environment interfaces. They act as barriers limiting the loss of water and nutrients and protecting against radiation and invasion of pathogens. The roles of cutin- and suberin polyesters are often attributed to their dominant aliphatic components, but the contribution of aromatic composition to their physiological function remains unclear. By functionally screening a subset of Populus trichocarpa BAHD/HXXXD acyltransferases, we identified a hydroxycinnamoyltransferase that shows specific transacylation activity on ?-hydroxyacids using both feruloyl- and p-coumaroyl- CoA as the acyl donors. We named this enzyme P. trichocarpa hydroxyacid/fatty alcohol hydroxycinnamoyltransferase 1 (PtFHT1). The ectopic expression of the PtFHT1 gene in Arabidopsis increased the incorporation of ferulate in root and seed suberins and in leaf cutin, but not that of p-coumarate, while the aliphatic load in both suberin and cutin polyesters essentially remained unaffected. The overaccumulation of ferulate in lipophilic polyester significantly increased the tolerance of transgenic plants to salt stress treatment; under sub-lethal conditions of salt stress, the ratios of their seed germination and seedling establishment were 50% higher than those of wild-type plants. Our study suggests that, although aromatics are the minor component of polyesters, they play important role in the sealing function of lipidic polymers in planta.
C1 [Cheng, Ai-Xia; Gou, Jin-Ying; Yu, Xiao-Hong; Yang, Huijun; Liu, Chang-Jun] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
[Cheng, Ai-Xia] Shandong Univ, Sch Pharmaceut Sci, Jinan 250012, Peoples R China.
[Fang, Xin; Chen, Xiao-Ya] Shanghai Inst Biol Sci, Inst Plant Physiol & Ecol, Shanghai 200032, Peoples R China.
RP Liu, CJ (reprint author), Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA.
EM cliu@bnl.gov
OI Chen, Xiaoya/0000-0002-2909-8414
FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of
Basic Energy Sciences of the US Department of Energy (DOE)
[DEAC0298CH10886]; National Science Foundation [MCB-1051675]; National
Science Foundation of China [31028003]
FX This work was supported by the Division of Chemical Sciences,
Geosciences, and Biosciences, Office of Basic Energy Sciences of the US
Department of Energy (DOE) (grant no. DEAC0298CH10886 to C.J.L.); the
transgenic Arabidopsis analyses were also partially supported by
National Science Foundation (grant no. MCB-1051675) and by the oversea
collaborative project of National Science Foundation of China (grant no.
31028003).
NR 55
TC 6
Z9 7
U1 0
U2 21
PU OXFORD UNIV PRESS
PI OXFORD
PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND
SN 1674-2052
EI 1752-9867
J9 MOL PLANT
JI Mol. Plant.
PD NOV
PY 2013
VL 6
IS 6
BP 1889
EP 1903
DI 10.1093/mp/sst085
PG 15
WC Biochemistry & Molecular Biology; Plant Sciences
SC Biochemistry & Molecular Biology; Plant Sciences
GA 259QK
UT WOS:000327541200013
PM 23709341
ER
PT J
AU Binder, M
Justo, A
Riley, R
Salamov, A
Lopez-Giraldez, F
Sjokvist, E
Copeland, A
Foster, B
Sun, H
Larsson, E
Larsson, KH
Townsend, J
Grigoriev, IV
Hibbett, DS
AF Binder, Manfred
Justo, Alfredo
Riley, Robert
Salamov, Asaf
Lopez-Giraldez, Francesc
Sjokvist, Elisabet
Copeland, Alex
Foster, Brian
Sun, Hui
Larsson, Ellen
Larsson, Karl-Henrik
Townsend, Jeffrey
Grigoriev, Igor V.
Hibbett, David S.
TI Phylogenetic and phylogenomic overview of the Polyporales
SO MYCOLOGIA
LA English
DT Article
DE genomics; new molecular markers; Polyporales; taxonomy
ID FUNGAL PHYLOGENETICS; SEQUENCE ALIGNMENTS; MAXIMUM-LIKELIHOOD;
DIVERGENCE TIMES; GENOME SEQUENCE; RIBOSOMAL DNA; PRIMER SETS;
BROWN-ROT; GENES; CLASSIFICATION
AB We present a phylogenetic and phylogenomic overview of the Polyporales. The newly sequenced genomes of Bjerkandera adusta, Ganoderma sp., and Phlebia brevispora are introduced and an overview of 10 currently available Polyporales genomes is provided. The new genomes are 39 500 000-49 900 00 bp and encode for 12 910 16 170 genes. We searched available genomes for single-copy genes and performed phylogenetic informativeness analyses to evaluate their potential for phylogenetic systematics of the Polyporales. Phylogenomic datasets (25, 71, 356 genes) were assembled for the 10 Polyporales species with genome data and compared with the most comprehensive dataset of Polyporales to date (six-gene dataset for 373 taxa, including taxa with missing data) Maximum likelihood and Bayesian phylogenetic analyses of genomic datasets yielded identical topologies, and the corresponding clades also were recovered in the 373-taxa dataset although with different support values in some datasets. Three previously recognized lineages of Polyporales, antrodia, core polyporoid and phlebioid clades, are supported in most datasets, while the status of the residual polyporoid clade remains uncertain and certain taxa (e.g. Gelatoporia, Grifola, Tyromyces) apparently do not belong to any of the major lineages of Polyporales. The most promising candidate single-copy genes are presented, and nodes in the Polyporales phylogeny critical for the suprageneric taxonomy of the order are identified and discussed.
C1 [Binder, Manfred; Justo, Alfredo; Hibbett, David S.] Clark Univ, Dept Biol, Worcester, MA 01610 USA.
[Binder, Manfred] CBS KNAW Fungal Biodivers Ctr, NL-3584 CT Utrecht, Netherlands.
[Riley, Robert; Salamov, Asaf; Copeland, Alex; Foster, Brian; Sun, Hui; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA.
[Lopez-Giraldez, Francesc; Townsend, Jeffrey] Yale Univ, Dept Ecol & Evolutionary Biol, Osborne Mem Labs 226, New Haven, CT 06520 USA.
[Sjokvist, Elisabet] Univ Gothenburg, Deptartment Biol & Environm Sci, SE-40530 Gothenburg, Sweden.
[Larsson, Ellen] Univ Gothenburg, Deptment Biol & Environm Sci, SE-40530 Gothenburg, Sweden.
[Larsson, Karl-Henrik] Univ Oslo, Nat Hist Museum, NO-0318 Oslo, Norway.
RP Grigoriev, IV (reprint author), US DOE, Joint Genome Inst, 2800 Michell Dr, Walnut Creek, CA 94598 USA.
EM ivgrigoriev@lbl.gov; dhibbett@clarku.edu
RI Binder, Manfred/C-8571-2013; Lopez-Giraldez, Francesc/A-5251-2011;
OI Lopez-Giraldez, Francesc/0000-0001-7476-9822; Sjokvist,
Elisabet/0000-0001-5890-8677
FU NSF through PolyPEET [DEB 0933081]; Office of Science of the US
Department of Energy [DE-ACO205CH11231]
FX We acknowledge the financial support of NSF through the PolyPEET grant
(DEB 0933081) to DSH. The work conducted by the US Department of Energy
Joint Genome Institute is supported by the Office of Science of the US
Department of Energy under contract No. DE-ACO205CH11231.
NR 64
TC 67
Z9 72
U1 4
U2 50
PU ALLEN PRESS INC
PI LAWRENCE
PA 810 E 10TH ST, LAWRENCE, KS 66044 USA
SN 0027-5514
EI 1557-2536
J9 MYCOLOGIA
JI Mycologia
PD NOV-DEC
PY 2013
VL 105
IS 6
BP 1350
EP 1373
DI 10.3852/13-003
PG 24
WC Mycology
SC Mycology
GA 260BJ
UT WOS:000327569700002
PM 23935031
ER
PT J
AU Syed, K
Nelson, DR
Riley, R
Yadav, JS
AF Syed, Khajamohiddin
Nelson, David R.
Riley, Robert
Yadav, Jagjit S.
TI Genomewide annotation and comparative genomics of cytochrome P450
monooxygenases (P450s) in the polypore species Bjerkandera adusta,
Ganoderma sp and Phlebia brevispora
SO MYCOLOGIA
LA English
DT Article
DE Bjerkandera adusta; Cytochrome P450 monooxygenases; Ganoderma sp.;
P450ome; Phanerochaete chrysosporium; Phlebia brevispora; Postia
placenta
ID PHANEROCHAETE-CHRYSOSPORIUM; HYDROXYLASE; SEQUENCE; ENZYMES
AB Genomewide annotation of cytochrome P450 monooxygenases (P450s) in three white-rot species of the fungal order Polyporales, namely Bjerkandera adusta, Ganoderma sp. and Phlebia brevispora, revealed a large contingent of P450 genes (P450ome) in their genomes. A total of 199 P450 genes in B. adusta and 209 P450 genes each in Ganoderma sp. and P. brevispora were identified. These P450omes were classified into families and subfamilies as follows: B. adusta (39 families, 86 subfamilies), Ganoderma sp. (41 families, 105 subfamilies) and P. brevispora (42 families, 111 subfamilies). Of note, the B. adusta genome lacked the CYP505 family (P450foxy), a group of P450-CPR fusion proteins. The three polypore species revealed differential enrichment of individual P450 families in their genomes. The largest GYP families in the three genomes were CYP5144 (67 P450s), CYP5359 (46 P450s) and CYP5344 (43 P450s) in B. adusta, Ganoderma sp. and P. brevispora, respectively. Our analyses showed that tandem gene duplications led to expansions in certain P450 families. An estimated 33% (72 P450s), 28% (55 P450s) and 23% (49 P450s) of P450ome genes were duplicated in P. brevispora, B. adusta and Ganoderma sp., respectively. Family-wise comparative analysis revealed that 22 GYP families are common across the three Polypore species. Comparative P450ome analysis with Ganoderma lucidum revealed the presence of 143 orthologs and 56 paralogs in Ganoderma sp. Multiple P450s were found near the characteristic biosynthetic genes for secondary metabolites, namely polyketide synthase (PKS), non-ribosomal peptide synthetase (NRPS), terpene cyclase and terpene synthase in the three genomes, suggesting a likely role of these P450s in secondary metabolism in these Polyporales. Overall, the three species had a richer P450 diversity both in terms of the P450 genes and P450 subfamilies as compared to the model white-rot and brown-rot polypore species Phanerochaete chrysosporium and Postia placenta.
C1 [Syed, Khajamohiddin; Yadav, Jagjit S.] Univ Cincinnati, Coll Med, Dept Environm Hlth, Environm Genet & Mol Toxicol Div, Cincinnati, OH 45267 USA.
[Nelson, David R.] Univ Tennessee, Ctr Hlth Sci, Dept Microbiol Immunol & Biochem, Memphis, TN 38163 USA.
[Riley, Robert] Dept Energy, Joint Genome Inst, Walnut Creek, CA 94598 USA.
RP Yadav, JS (reprint author), Univ Cincinnati, Coll Med, Dept Environm Hlth, Environm Genet & Mol Toxicol Div, Cincinnati, OH 45267 USA.
EM jagjit.yadav@uc.edu
OI Nelson, David/0000-0003-0583-5421
FU National Institute of Environmental Health Sciences (NIEHS)
[R01ES015543]
FX The work was supported primarily by the National Institute of
Environmental Health Sciences (NIEHS) grant R01ES015543 to JSY.
NR 24
TC 13
Z9 13
U1 1
U2 11
PU ALLEN PRESS INC
PI LAWRENCE
PA 810 E 10TH ST, LAWRENCE, KS 66044 USA
SN 0027-5514
EI 1557-2536
J9 MYCOLOGIA
JI Mycologia
PD NOV-DEC
PY 2013
VL 105
IS 6
BP 1445
EP 1455
DI 10.3852/13-002
PG 11
WC Mycology
SC Mycology
GA 260BJ
UT WOS:000327569700007
PM 23928414
ER
PT J
AU Howell, SL
Padalkar, S
Yoon, K
Li, QM
Koleske, DD
Wierer, JJ
'Wang, GT
Lauhon, LJ
AF Howell, Sarah L.
Padalkar, Sonal
Yoon, KunHo
Li, Qiming
Koleske, Daniel D.
Wierer, Jonathan J.
'Wang, George T.
Lauhon, Lincoln J.
TI Spatial Mapping of Efficiency of GaN/InGaN Nanowire Array Solar Cells
Using Scanning Photocurrent Microscopy
SO NANO LETTERS
LA English
DT Article
DE Nanowire; InGaN; SPCM; solar cell; photovoltaics
ID MULTIPLE-QUANTUM-WELLS; LIGHT-EMITTING-DIODES; RAMAN-SCATTERING;
PHOTOVOLTAICS; DEVICES; NANOROD
AB GaN-InGaN core shell nanowire array devices are characterized by spectrally resolved scanning photocurrent microscopy (SPCM). The spatially resolved external quantum efficiency is correlated with structure and composition inferred from atomic force microscope (AFM) topography, scanning transmission electron microscope (STEM) imaging, Raman microspectroscopy, and scanning photocurrent microscopy (SPCM) maps of the effective absorption edge. The experimental analyses are coupled with finite difference time domain simulations to provide mechanistic understanding of spatial variations in carrier generation and collection, which is essential to the development of heterogeneous novel architecture solar cell devices.
C1 [Howell, Sarah L.; Padalkar, Sonal; Yoon, KunHo; Lauhon, Lincoln J.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.
[Li, Qiming; Koleske, Daniel D.; Wierer, Jonathan J.; 'Wang, George T.] Sandia Natl Labs, Albuquerque, NM 87185 USA.
RP Lauhon, LJ (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA.
EM lauhon@northwestern.edu
RI Lauhon, Lincoln/B-7526-2009; Lauhon, Lincoln/H-2976-2015; Wierer,
Jonathan/G-1594-2013
OI Lauhon, Lincoln/0000-0001-6046-3304; Wierer,
Jonathan/0000-0001-6971-4835
FU DOE BES [DE-FG02-07ER46401]; NSF Graduate Research Fellowship
[DGE-1324585]; Sandia's Solid State Lighting Science Energy Frontier
Research Center; DOE BES; U.S. Department of Energy's National Nuclear
Security Administration [DE-AC04-94AL85000]
FX Nanowire SPCM and Raman studies in the group of L.J.L. were supported by
DOE BES grant DE-FG02-07ER46401. S.L.H. was supported in part by an NSF
Graduate Research Fellowship under DGE-1324585. The nanowire solar cell
growth, device fabrication, and STEM characterization were supported by
Sandia's Solid State Lighting Science Energy Frontier Research Center,
funded by DOE BES. Sandia National Laboratories is a multiprogram
laboratory managed and operated by Sandia Corporation, a wholly owned
subsidiary of Lockheed Martin Corporation, for the U.S. Department of
Energy's National Nuclear Security Administration under contract
DE-AC04-94AL85000.
NR 30
TC 40
Z9 40
U1 11
U2 108
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5123
EP 5128
DI 10.1021/nl402331u
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700021
PM 24099617
ER
PT J
AU Gu, M
Kushima, A
Shao, YY
Zhang, JG
Liu, J
Browning, ND
Li, J
Wang, CM
AF Gu, Meng
Kushima, Akihiro
Shao, Yuyan
Zhang, Ji-Guang
Liu, Jun
Browning, Nigel D.
Li, Ju
Wang, Chongmin
TI Probing the Failure Mechanism of SnO2 Nanowires for Sodium-Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Na-ion battery; SnO2 anode; in situ TEM; Na diffusion; DFT calculation;
failure mechanism
ID IN-SITU TEM; TRANSMISSION ELECTRON-MICROSCOPY; HIGH-CAPACITY;
HIGH-PERFORMANCE; SILICON NANOWIRES; ELECTROCHEMICAL LITHIATION;
NANOSTRUCTURED SILICON; ENERGY-STORAGE; LOW-COST; ANODE
AB Nonlithium metals such as sodium have attracted wide attention as a potential charge carrying ion for rechargeable batteries. Using in situ transmission electron microscopy in combination with density functional theory calculations, we probed the structural and chemical evolution of SnO2 nanowire anodes in Na-ion batteries and compared them quantitatively with results from Li-ion batteries (Huang, J. Y.; et al. Science 2010, 330, 1515-1520). Upon Na insertion into SnO2, a displacement reaction occurs, leading to the formation of amorphous NaxSn nanoparticles dispersed in Na2O matrix. With further Na insertion, the NaxSn crystallized into Na15Sn4 (x = 3.75). Upon extraction of Na (desodiation), the NaxSn transforms to Sn nanoparticles. Associated with the dealloying, pores are found to form, leading to a structure of Sn particles confined in a hollow matrix of Na2O. These pores greatly increase electrical impedance, therefore accounting for the poor cyclability of SnO2. DFT calculations indicate that Na+ diffuses 30 times slower than Li+ in SnO2, in agreement with in situ TEM measurement. Insertion of Na can chemomechanically soften the reaction product to a greater extent than in lithiation. Therefore, in contrast to the lithiation of SnO2 significantly less dislocation plasticity was seen ahead of the sodiation front. This direct comparison of the results from Na and Li highlights the critical role of ionic size and electronic structure of different ionic species on the charge/discharge rate and failure mechanisms in these batteries.
C1 [Gu, Meng; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.
[Kushima, Akihiro; Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA.
[Kushima, Akihiro; Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.
[Browning, Nigel D.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA.
[Shao, Yuyan; Zhang, Ji-Guang; Liu, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA.
RP Li, J (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA.
EM liju@mit.edu; Chongmin.wang@pnnl.gov
RI Kushima, Akihiro/H-2347-2011; Shao, Yuyan/A-9911-2008; Li,
Ju/A-2993-2008; Gu, Meng/B-8258-2013
OI Browning, Nigel/0000-0003-0491-251X; Shao, Yuyan/0000-0001-5735-2670;
Li, Ju/0000-0002-7841-8058;
FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation
Hub; U.S. Department of Energy, Office of Science, Basic Energy
Sciences; DOE's Office of Biological and Environmental Research;
Department of Energy [DE-AC05-76RLO1830]; NSF [DMR-1008104, DMR-1120901]
FX This work was supported as part of the Joint Center for Energy Storage
Research (JCESR), an Energy Innovation Hub funded by the U.S. Department
of Energy, Office of Science, Basic Energy Sciences. The work was
conducted in the William R. Wiley Environmental Molecular Sciences
Laboratory (EMSL), a national scientific user facility sponsored by
DOE's Office of Biological and Environmental Research and located at
PNNL. PNNL is operated by Battelle for the Department of Energy under
Contract DE-AC05-76RLO1830. A.K. and J.L. acknowledge support by NSF
DMR-1008104 and DMR-1120901.
NR 42
TC 76
Z9 78
U1 31
U2 332
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5203
EP 5211
DI 10.1021/nl402633n
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700034
PM 24079296
ER
PT J
AU Liang, WT
Hong, L
Yang, H
Fan, FF
Liu, Y
Li, H
Li, J
Huang, JY
Chen, LQ
Zhu, T
Zhang, SL
AF Liang, Wentao
Hong, Liang
Yang, Hui
Fan, FeiFei
Liu, Yang
Li, Hong
Li, Ju
Huang, Jian Yu
Chen, Long-Qing
Zhu, Ting
Zhang, Sulin
TI Nanovoid Formation and Annihilation in Gallium Nanodroplets under
Lithiation-Delithiation Cycling
SO NANO LETTERS
LA English
DT Article
DE Gallium nanodroplets; lithium ion battery; nanovoid; in situ TEM; phase
field
ID LITHIUM-ION BATTERIES; TRANSMISSION ELECTRON-MICROSCOPY; IN-SITU TEM;
SILICON NANOWIRES; ELECTROCHEMICAL LITHIATION; AMORPHOUS-SILICON; SNO2
NANOWIRE; CHALLENGES; FRACTURE; ALLOYS
AB The irreversible chemomechanical degradation is a critical issue in the development of high-capacity electrode materials for the next-generation lithium (Li)-ion batteries. Here we report the self-healing behavior of gallium nanodroplets (GaNDs) under electrochemical cycling at room temperature, observed with in situ transmission electron microscopy (TEM). During lithiation, the GaNDs underwent a liquid-to-solid phase transition, forming a crystalline phase (LixGa) with similar to 160% volume expansion. Owing to the uneven Li flow during lithiation, the fully lithiated GaNDs exhibited highly distorted morphologies. Upon delithiation, the reverse phase transition occurred, accompanied with the nucleation and growth of a nanosized void. After the GaNDs were fully delithiated, the nanovoid gradually annihilated. Our analysis, along with phase field modeling and experimental measurements of the void growth and annihilation, provides mechanistic insights into the void formation and annihilation mechanism. The GaNDs may function as an effective healing agent in durable composite electrodes for high-performance Li-ion batteries, wherein active components, such as Si, are susceptible to fracture.
C1 [Liang, Wentao; Yang, Hui; Zhang, Sulin] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16802 USA.
[Hong, Liang; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA.
[Fan, FeiFei; Zhu, Ting] Georgia Inst Technol, Woodruff Sch Mech Engn, Atlanta, GA 30332 USA.
[Liu, Yang; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA.
[Li, Hong] Chinese Acad Sci, Inst Phys, Renewable Energy Lab, Beijing 100190, Peoples R China.
[Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA.
[Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.
RP Zhang, SL (reprint author), Penn State Univ, Dept Engn Sci & Mech, 227 Hammond Bldg, University Pk, PA 16802 USA.
EM suz10@psu.edu
RI Hong, Liang/K-5673-2013; Li, Ju/A-2993-2008; Zhu, Ting/A-2206-2009; Li,
Hong/C-4643-2008; Zhang, Sulin /E-6457-2010; Chen, LongQing/I-7536-2012;
YANG, HUI/H-6996-2012; Liang, Wentao/J-8771-2015;
OI Li, Ju/0000-0002-7841-8058; Li, Hong/0000-0002-8659-086X; Chen,
LongQing/0000-0003-3359-3781; YANG, HUI/0000-0002-2628-4676; Fan,
Feifei/0000-0003-0455-4900
FU National Science Foundation [CMMI-1201058, CMMI-1100205, CMMI-1235092,
DMR-1240933, DMR-1120901]; Laboratory Directed Research and Development
(LDRD) project at Sandia National Laboratories (SNL); Nanostructures for
Electrical Energy Storage (NEES), an Energy Frontier Research Center
(EFRC); U.S. Department of Energy, Office of Science, Office of Basic
Energy Sciences [DESC0001160]; LDRD; NEES center; U.S. Department of
Energy's National Nuclear Security Administration [DE-AC04-94AL85000]
FX We acknowledge the support by National Science Foundation under the
grant numbers CMMI-1201058, CMMI-1100205, CMMI-1235092, DMR-1240933 and
DMR-1120901. Portions of this work were supported by a Laboratory
Directed Research and Development (LDRD) project at Sandia National
Laboratories (SNL) and partly by Nanostructures for Electrical Energy
Storage (NEES), an Energy Frontier Research Center (EFRC) funded by the
U.S. Department of Energy, Office of Science, Office of Basic Energy
Sciences under Award Number DESC0001160. The LDRD supported the
development and fabrication of platforms. The NEES center supported the
development of TEM techniques. CINT supported the TEM capability; in
addition, this work represents the efforts of several CINT users,
primarily those with affiliation external to Sandia National
Laboratories. In addition, this work was performed, in part, at the
Sandia-Los Alamos Center for Integrated Nanotechnologies (CINT), a U.S.
Department of Energy, Office of Basic Energy Sciences user facility.
Sandia National Laboratories is a multiprogram laboratory operated by
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under contract DE-AC04-94AL85000.
NR 47
TC 13
Z9 14
U1 17
U2 129
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5212
EP 5217
DI 10.1021/nl402644w
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700035
PM 24102207
ER
PT J
AU Xia, T
Zhang, W
Murowchick, J
Liu, G
Chen, XB
AF Xia, Ting
Zhang, Wei
Murowchick, James
Liu, Gao
Chen, Xiaobo
TI Built-in Electric Field-Assisted Surface-Amorphized Nanocrystals for
High-Rate Lithium-Ion Battery
SO NANO LETTERS
LA English
DT Article
DE Built-in electric field; surface-amorphized nanocsystals; titanium
dioxide; lithium-ion battery
ID ANATASE TIO2; TITANIUM-DIOXIDE; HIGH-CAPACITY; SILICON NANOWIRES;
PERFORMANCE; STORAGE; NANOTUBES; ANODES; NANOPARTICLES; NANOMATERIALS
AB High-power batteries require fast charge/discharge rates and high capacity besides safe operation. TiO2 has been investigated as a safer alternative candidate to the current graphite or incoming silicon anodes due to higher redox potentials in effectively preventing lithium deposition. However, its charge/discharge rates. are reluctant to improve due to poor ion diffusion coefficients, and its capacity fades quickly with rate as only thinner surface layers can be effectively used in faster charge/discharge processes. Here, we demonstrate that surface-amorphized TiO2 nanocrystals greatly improve lithium-ion rechargeable battery performance: 20 times rate and 340% capacity improvement over crystalline TiO2 nanocrystals. This improvement is benefited from the built-in electric field within the nanocrystals that induces much lower lithium-ion diffusion resistance and facilitates its transport in both insertion and extraction processes. This concept thus offers an innovative and general approach toward designing battery materials with better performance.
C1 [Xia, Ting; Chen, Xiaobo] Univ Missouri, Dept Chem, Kansas City, MO 64110 USA.
[Zhang, Wei; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Murowchick, James] Univ Missouri, Dept Geosci, Kansas City, MO 64110 USA.
RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM GLiu@lbl.gov; chenxiaobo@umkc.edu
OI Murowchick, James/0000-0003-2987-0352
FU College of Arts and Sciences, University of Missouri-Kansas City,
University of Missouri Research Board; University of Missouri Research
Board; Office of Vehicle Technologies of the United States Department of
Energy [DE-AC03-76SF00098]
FX X.C. thanks the support from College of Arts and Sciences, University of
Missouri-Kansas City, the University of Missouri Research Board, and the
generous gift from Dow Kokam. G.L. thanks the fund by the Assistant
Secretary for Energy Efficiency, Office of Vehicle Technologies of the
United States Department of Energy under Contract No. DE-AC03-76SF00098.
NR 39
TC 52
Z9 52
U1 4
U2 91
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5289
EP 5296
DI 10.1021/nl402810d
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700046
PM 24099557
ER
PT J
AU Jun, YC
Reno, J
Ribaudo, T
Shaner, E
Greffet, JJ
Vassant, S
Marquier, F
Sinclair, M
Brener, I
AF Jun, Young Chul
Reno, John
Ribaudo, Troy
Shaner, Eric
Greffet, Jean-Jacques
Vassant, Simon
Marquier, Francois
Sinclair, Mike
Brener, Igal
TI Epsilon-Near-Zero Strong Coupling in Metamaterial-Semiconductor Hybrid
Structures
SO NANO LETTERS
LA English
DT Article
DE Nano-optics; metamaterials; semiconductors; strong coupling;
optoelectronics; infrared
ID MOLECULES
AB We present a new type of electrically tunable strong coupling between planar metamaterials and epsilon-near-zero modes that exist in a doped semiconductor nanolayer. The use of doped semiconductors makes this strong coupling tunable over a wide range of wavelengths through the use of different doping densities. We also modulate this coupling by depleting the doped semiconductor layer electrically. Our hybrid approach incorporates strong optical interactions into a highly tunable, integrated device platform.
C1 [Jun, Young Chul; Reno, John; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA.
[Jun, Young Chul; Ribaudo, Troy; Shaner, Eric; Sinclair, Mike; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA.
[Jun, Young Chul] Inha Univ, Dept Phys, Inchon 402751, South Korea.
[Greffet, Jean-Jacques; Vassant, Simon; Marquier, Francois] Univ Paris 11, CNRS, Lab Charles Fabry, Inst Opt, F-91127 Palaiseau, France.
RP Jun, YC (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA.
EM youngchul.jun@inha.ac.kr; ibrener@sandia.gov
RI Jun, Young Chul/I-2274-2013; Marquier, Francois/A-2359-2015; Greffet,
Jean-Jacques/Q-2427-2015; Vassant, Simon/K-7787-2016
OI Jun, Young Chul/0000-0002-7578-8811; Marquier,
Francois/0000-0003-3118-1150; Greffet, Jean-Jacques/0000-0002-4048-2150;
Vassant, Simon/0000-0002-9896-6676
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]; MSIP (Ministry of Science, ICT&Future Planning),
Korea under the ITRC (Information Technology Research Center) support
program [NIPA-2013-H0301-13-1010]
FX This work was performed, in part, at the Center for Integrated
Nanotechnologies, an Office of Science User Facility operated for the
U.S. Department of Energy (DOE) Office of Science. Sandia National
Laboratories is a multiprogram laboratory managed and operated by Sandia
Corporation, a wholly owned subsidiary of Lockheed Martin Corporation,
for the U.S. Department of Energy's National Nuclear Security
Administration under contract DE-AC04-94AL85000. Y.C.J. acknowledges the
support from the MSIP (Ministry of Science, ICT&Future Planning), Korea,
under the ITRC (Information Technology Research Center) support program
(NIPA-2013-H0301-13-1010) supervised by the NIPA (National IT Industry
Promotion Agency).
NR 24
TC 37
Z9 37
U1 2
U2 47
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5391
EP 5396
DI 10.1021/nl402939t
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700062
PM 24124754
ER
PT J
AU Wu, MY
Sabisch, JEC
Song, XY
Minor, AM
Battaglia, VS
Liu, G
AF Wu, Mingyan
Sabisch, Julian E. C.
Song, Xiangyun
Minor, Andrew M.
Battaglia, Vincent S.
Liu, Gao
TI In Situ Formed Si Nanoparticle Network with Micron-Sized Si Particles
for Lithium-Ion Battery Anodes
SO NANO LETTERS
LA English
DT Article
DE Silicon; nanoparticle; lithium-ion battery; anode; conductive polymer
binder; additives
ID SOLID-ELECTROLYTE INTERPHASE; HIGH-CAPACITY; HIGH-PERFORMANCE;
RECHARGEABLE BATTERIES; SECONDARY BATTERIES; SILICON PARTICLES;
ENERGY-STORAGE; LI; NANOWIRES; CARBON
AB To address the significant challenges associated with large volume change of micrometer-sized Si particles as high-capacity anode materials for lithium-ion batteries, we demonstrated a simple but effective strategy: using Si nanoparticles as a structural and conductive additive, with micrometer-sized Si as the main lithium-ion storage material. The Si nanopartides connected into the network structure in situ during the charge process, to provide electronic connectivity and structure stability for the electrode. The resulting electrode showed a high specific capacity of 2500 mAh/g after 30 cycles with high initial Coulombic efficiency (73%) and good rate performance during electrochemical lithiation and delithiation: between 0.01 and 1 V vs Li/Li+.
C1 [Wu, Mingyan; Song, Xiangyun; Battaglia, Vincent S.; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
[Sabisch, Julian E. C.; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA.
[Sabisch, Julian E. C.; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94704 USA.
RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM gliu@lbl.gov
RI Foundry, Molecular/G-9968-2014
FU Office of Vehicle Technologies of the U.S. Department of Energy under
the Batteries for Advanced Transportation Technologies (BATT) Program;
University of California, Office of the President through the University
of California Discovery Grant; Office of Science, Office of Basic Energy
Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]
FX This work is funded by the Assistant Secretary for Energy Efficiency,
Office of Vehicle Technologies of the U.S. Department of Energy, under
the Batteries for Advanced Transportation Technologies (BATT) Program
and by University of California, Office of the President through the
University of California Discovery Grant. Electron microscopy
experiments were conducted at the National Center for Electron
Microscopy (NCEM), located at Lawrence Berkeley National Laboratory
(LBNL) and supported by the Director, Office of Science, Office of Basic
Energy Sciences, of the U.S. Department of Energy under contract no.
DE-AC02-05CH11231.
NR 51
TC 42
Z9 42
U1 20
U2 193
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5397
EP 5402
DI 10.1021/nl402953h
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700063
PM 24079331
ER
PT J
AU Marchuk, K
Fang, N
AF Marchuk, Kyle
Fang, Ning
TI Three-Dimensional Orientation Determination of Stationary Anisotropic
Nanoparticles with Sub-Degree Precision under Total Internal Reflection
Scattering Microscopy
SO NANO LETTERS
LA English
DT Article
DE Total internal reflection scattering (TIRS); single-particle;
orientation determination; microtubule cargo; localized surface plasmon
resonance
ID INTERFERENCE CONTRAST MICROSCOPY; ROTATIONAL-DYNAMICS; GOLD NANORODS;
TRACKING; SENSORS
AB Single-particle and single-molecule orientation determination plays a vital role in deciphering nanoscale motion in complex environments. Previous attempts to determine the absolute three-dimensional orientation of anisotropic particles rely on subjective pattern matching and are inherently plagued by high degrees of uncertainty. Herein, we describe a method utilizing total internal reflection scattering microscopy to determine the 3D orientation of gold nanorods with subdegree uncertainty. The method is then applied to the biologically relevant system of microtubule cargo loading. Finally, we demonstrate the method holds potential for identifying single particles versus proximate neighbors within the diffraction limited area.
C1 [Fang, Ning] US DOE, Ames Lab, Ames, IA 50011 USA.
Iowa State Univ, Dept Chem, Ames, IA 50011 USA.
RP Fang, N (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.
EM nfang@iastate.edu
FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of
Chemical Sciences, Geosciences, and Biosciences through the Ames
Laboratory; U.S. Department of Energy by Iowa State University [DE-AC02-
07CH11358]
FX The authors of this paper would like to thank Keith Fritzsching from
Iowa State University for his help regarding the home written MATLAB
codes. Keith provided valuable discussions concerning the design of the
programs along with help in the coding itself. This work was supported
by the U.S. Department of Energy, Office of Basic Energy Sciences,
Division of Chemical Sciences, Geosciences, and Biosciences through the
Ames Laboratory. The Ames Laboratory is operated for the U.S. Department
of Energy by Iowa State University under contract no. DE-AC02-
07CH11358.
NR 22
TC 12
Z9 12
U1 0
U2 25
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5414
EP 5419
DI 10.1021/nl4029818
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700066
PM 24144109
ER
PT J
AU Takahashi, T
Yu, ZB
Chen, K
Kiriya, D
Wang, C
Takei, K
Shiraki, H
Chen, T
Ma, BW
Javey, A
AF Takahashi, Toshitake
Yu, Zhibin
Chen, Kevin
Kiriya, Daisuke
Wang, Chuan
Takei, Kuniharu
Shiraki, Hiroshi
Chen, Teresa
Ma, Biwu
Javey, Ali
TI Carbon Nanotube Active-Matrix Backplanes for Mechanically Flexible
Visible Light and X-ray Imagers
SO NANO LETTERS
LA English
DT Article
DE Thin film transistors; single-walled carbon nanotubes; organic
photodiodes; electronic skin; bendable; imaging
ID DENSITY-GRADIENT ULTRACENTRIFUGATION; POLYMER PHOTOVOLTAIC CELLS;
ORGANIC PHOTODIODES; SOLAR-CELLS; ELECTRONIC SKIN; CIRCUITS; THIN;
EFFICIENCY; PRESSURE; VOLTAGE
AB We report visible light and X-ray imagers on lightweight and mechanically flexible plastic substrates. The process involves solution processing of organic photodetectors on top of an active-matrix backplane consisting of carbon nanotube thin-film transistors. The system takes advantage of the high mobility of nanotube transistors for low operating voltages and efficient light absorption of organic bulk-heterojunctions for high imaging sensitivity. With this highly scalable process scheme, 18 x 18 pixel-array flexible imagers (physical size of 2 cm x 1.5 cm) with high performance are successfully demonstrated. In addition, as the absorption peak of the adopted organic photodiodes covers the green band of the light spectrum, X-ray imaging is readily demonstrated by placing a scintillator film on top of the flexible imagers.
C1 [Takahashi, Toshitake; Yu, Zhibin; Chen, Kevin; Kiriya, Daisuke; Wang, Chuan; Takei, Kuniharu; Shiraki, Hiroshi; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94702 USA.
[Takahashi, Toshitake; Yu, Zhibin; Chen, Kevin; Kiriya, Daisuke; Wang, Chuan; Takei, Kuniharu; Shiraki, Hiroshi; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94702 USA.
[Takahashi, Toshitake; Yu, Zhibin; Chen, Kevin; Kiriya, Daisuke; Wang, Chuan; Takei, Kuniharu; Shiraki, Hiroshi; Ma, Biwu; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Ma, Biwu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
[Javey, Ali] King Abudulaziz Univ, Dept Chem, Fac Sci, Jeddah 21589, Saudi Arabia.
RP Javey, A (reprint author), Univ Calif Berkeley, Berkeley, CA 94702 USA.
EM ajavey@eecs.berkeley.edu
RI Wang, Chuan/B-3649-2011; Javey, Ali/B-4818-2013; Foundry,
Molecular/G-9968-2014
FU NSF NASCENT Center; Office of Science, Office of Basic Energy Sciences
of the U.S. Department of Energy [DE-AC02-05CH11231]
FX We thank Dr. R. Gupta of Harvard University for valuable discussions and
providing the GOS films. This work was supported by NSF NASCENT Center.
Work at the Molecular Foundry (photodiode fabrication) was supported by
the Office of Science, Office of Basic Energy Sciences, of the U.S.
Department of Energy under Contract No. DE-AC02-05CH11231. Measurements
of the photodiodes were performed in the Electronic Materials
laboratory, LBNL, which is supported by the Director, Office of Science,
Office Basic Energy Sciences, Division of Materials Sciences and
Engineering, of the U.S. Department of Energy.
NR 28
TC 29
Z9 29
U1 3
U2 31
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5425
EP 5430
DI 10.1021/nl403001r
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700068
PM 24143966
ER
PT J
AU Li, Z
Shao, S
Li, N
McCall, K
Wang, J
Zhang, SX
AF Li, Z.
Shao, S.
Li, N.
McCall, K.
Wang, J.
Zhang, S. X.
TI Single Crystalline Nanostructures of Topological Crystalline Insulator
SnTe with Distinct Facets and Morphologies
SO NANO LETTERS
LA English
DT Article
DE Topological crystalline insulators; tin telluride; nanowires; synthesis
ID SURFACE CONDUCTION; PHASE-TRANSITION; NANORIBBONS; NANOWIRES; STATES
AB Topological crystalline insulators (TCIs) are a new class of topological materials that possess unique metallic surface states protected by crystalline mirror symmetry. Their topological surface properties are expected to strongly depend on the surface orientation. By combining density functional theory (DFT) calculations and synthesis experiments, we demonstrate the controlled growth of single crystalline nanostructures of the prototypical TCI SnTe with distinct facets and morphologies. Our calculations suggest that the excess energy of the {111} surfaces can be either higher or lower than that of the {100} surfaces, depending on the stoichiometry, while the {110} is always higher than the {100}. In our synthesis experiment, we qualitatively controlled the stoichiometry by tailoring the growth temperature and obtained two types of single crystalline nanowires: smooth nanowires dominated by {100} facets at high temperatures and zigzag nanowires composed of both {100} and {111} surfaces at low temperatures. Notably, there is no {110} facet in our nanostructures, strongly supporting the DFT calculations. Our device fabrication and electrical characterizations suggest that both types of nanowires are suitable for transport studies of topological surface states.
C1 [Li, Z.; McCall, K.; Zhang, S. X.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA.
[Shao, S.; Wang, J.] Los Alamos Natl Lab, MST 8, Los Alamos, NM 87545 USA.
[Li, N.] Los Alamos Natl Lab, MPA CINT, Los Alamos, NM 87545 USA.
RP Wang, J (reprint author), Los Alamos Natl Lab, MST 8, Los Alamos, NM 87545 USA.
EM sxzhang@indiana.edu; wangj6@lanl.gov
RI Li, Nan /F-8459-2010; Shao, Shuai/B-2037-2014; Shao, Shuai/I-4108-2014;
Wang, Jian/F-2669-2012
OI Li, Nan /0000-0002-8248-9027; Shao, Shuai/0000-0002-4718-2783; Shao,
Shuai/0000-0002-4718-2783; Wang, Jian/0000-0001-5130-300X
FU Indiana University (IU); NSF REU program [PHY-1156540]; U.S. Department
of Energy, Office of Science, Office of Basic Energy Sciences; Los
Alamos National Laboratory Directed Research and Development
[LDRD-ER20140450]
FX S.X.Z. acknowledges startup fund from Indiana University (IU) and the
use of facility in the IU Nanoscience Center. KM. was supported by the
NSF REU program under Grant PHY-1156540. S.S., N.L., and J.W.
acknowledge the support provided by the U.S. Department of Energy,
Office of Science, Office of Basic Energy Sciences and also acknowledge
support provided by the Los Alamos National Laboratory Directed Research
and Development (LDRD-ER20140450).
NR 38
TC 30
Z9 30
U1 9
U2 98
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5443
EP 5448
DI 10.1021/nl4030193
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700071
PM 24138562
ER
PT J
AU Kang, J
Li, JB
Li, SS
Xia, JB
Wang, LW
AF Kang, Jun
Li, Jingbo
Li, Shu-Shen
Xia, Jian-Bai
Wang, Lin-Wang
TI Electronic Structural Moire Pattern Effects on MoS2/MoSe2 2D
Heterostructures
SO NANO LETTERS
LA English
DT Article
DE 2D heterostructure; lattice incommensurateness; Moire pattern; wave
function localization
ID HEXAGONAL BORON-NITRIDE; LAYERED MATERIALS; GRAPHENE; MOS2;
POLARIZATION; ENERGY
AB The structural and electronic properties of MoS2/MoSe2 bilayers are calculated using first-principles methods. It is found that the interlayer van der Waals interaction is not strong enough to form a lattice-matched coherent heterostructure. Instead, a nanometer-scale Moire pattern structure will be formed. By analyzing the electronic structures of different stacking configurations, we predict that the valence-band maximum (VBM) state will come from the Gamma point due to interlayer electronic coupling. This is confirmed by a direct calculation of a Moire pattern supercell containing 6630 atoms using the linear scaling three-dimensional fragment method. The VBM state is found to be strongly localized, while the conduction band minimum (CBM) state is only weakly localized, and it comes from the MoS2 layer at the K point. We predict such wave function localization can be a general feature for many two-dimensional (2D) van der Waals heterostructures and can have major impacts on the carrier mobility and other electronic and optical properties.
C1 [Kang, Jun; Li, Jingbo; Li, Shu-Shen; Xia, Jian-Bai] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China.
[Kang, Jun; Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Wang, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM lwwang@lbl.gov
RI Kang, Jun/F-7105-2011
OI Kang, Jun/0000-0003-4788-0028
FU Theory of Materials program; Office of Science (SC), Basic Energy
Science (BES)/Material Science and Engineering Division (MSED) of the
U.S. Department of Energy (DOE) [DE-AC02-05CH11231]
FX This work was supported by the Theory of Materials program, funded by
the Director, Office of Science (SC), Basic Energy Science
(BES)/Material Science and Engineering Division (MSED) of the U.S.
Department of Energy (DOE) under the contract no. DE-AC02-05CH11231. It
used resources of the National Energy Research Scientific Computing
Center (NERSC) and Oak Ridge Leadership Computing Facility (ORLCF) that
are supported by the Office of Science of the U.S. Department of Energy,
with the computational time allocated by the Innovative and Novel
Computational Impact on Theory and Experiment (INCITE) project.
NR 33
TC 84
Z9 84
U1 34
U2 300
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5485
EP 5490
DI 10.1021/nl4030648
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700078
PM 24079953
ER
PT J
AU Lin, YJ
Battaglia, C
Boccard, M
Hettick, M
Yu, ZB
Ballif, C
Ager, JW
Javey, A
AF Lin, Yongjing
Battaglia, Corsin
Boccard, Mathieu
Hettick, Mark
Yu, Zhibin
Ballif, Christophe
Ager, Joel W.
Javey, Ali
TI Amorphous Si Thin Film Based Photocathodes with High Photovoltage for
Efficient Hydrogen Production
SO NANO LETTERS
LA English
DT Article
DE Water splitting hydrogen production; photochemistry; high photovoltage;
a-Si photocathodes
ID VISIBLE-LIGHT; SOLAR; EVOLUTION; CELLS; SEMICONDUCTORS; ELECTROLYSIS;
CATALYST; DEVICE; NI
AB An amorphous Si thin film with TiO2 encapsulation layer is demonstrated as a highly promising and stable photocathode for solar hydrogen production. With platinum as prototypical cocatalyst, a photocurrent onset potential of 0.93 V vs RHE and saturation photocurrent of 11.6 mA/cm(2) are measured. Importantly, the a-Si photocathodes exhibit impressive photocurrent of similar to 6.1 mA/cm(2) at a large positive bias of 0.8 V vs RHE, which is the highest for all reported photocathodes at such positive potential. Ni-Mo alloy is demonstrated as an alternative low-cost catalyst with onset potential and saturation current similar to those obtained with platinum. This low-cost photocathode with high photovoltage and current is a highly promising photocathode for solar hydrogen production.
C1 [Lin, Yongjing; Battaglia, Corsin; Hettick, Mark; Yu, Zhibin; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94720 USA.
[Lin, Yongjing; Hettick, Mark; Ager, Joel W.; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.
[Lin, Yongjing; Battaglia, Corsin; Hettick, Mark; Yu, Zhibin; Ager, Joel W.; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Boccard, Mathieu; Ballif, Christophe] Ecole Polytech Fed Lausanne, Inst Microengn IMT, Photovolta & Thin Film Elect Lab, Lausanne, Switzerland.
RP Ager, JW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.
EM jwager@lbl.gov; ajavey@eecs.berkeley.edu
RI Battaglia, Corsin/B-2917-2010; Javey, Ali/B-4818-2013;
OI Ager, Joel/0000-0001-9334-9751
FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; WCU
program at Sunchon National University; Swiss Federal Office of Energy
FX The development and characterization of a-Si photocathodes were
supported through the Office of Science of the U.S. Department of Energy
under Award Number DE-SC0004993. A.J. acknowledges support from the WCU
program at Sunchon National University. Work at EPFL was supported by
the Swiss Federal Office of Energy.
NR 27
TC 61
Z9 65
U1 8
U2 104
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5615
EP 5618
DI 10.1021/nl403265k
PG 4
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700097
PM 24079390
ER
PT J
AU Niu, KY
Park, J
Zheng, HM
Aivisatos, AP
AF Niu, Kai-Yang
Park, Jungwon
Zheng, Haimei
Aivisatos, A. Paul
TI Revealing Bismuth Oxide Hollow Nanoparticle Formation by the Kirkendall
Effect
SO NANO LETTERS
LA English
DT Article
DE In situ TEM; liquid cell; Kirkendall effect; void formation; diffusion;
core-shell nanoparrcles
ID ELECTRON-MICROSCOPY; SHRINKING KINETICS; VACANCY DIFFUSION; GROWTH;
LIQUID; NANOSTRUCTURES; NANOSPHERES; TEMPERATURE; PARTICLES
AB We study the formation of bismuth oxide hollow nanoparticles by the Kirkendall effect using liquid cell transmission electron microscopy (TEM). Rich dynamics of bismuth diffusion through the bismuth oxide shell have been captured in situ. The diffusion coefficient of bismuth through bismuth oxide shell is 3-4 orders of magnitude higher than that of bulk. Observation reveals that defects, temperature, sizes of the particles, and so forth can affect the diffusion of reactive species and modify the kinetics of the hollowing process.
C1 [Niu, Kai-Yang; Zheng, Haimei; Aivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
[Park, Jungwon; Zheng, Haimei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.
[Aivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
EM hmzheng@lbl.gov; alivis@berkeley.edu
RI Foundry, Molecular/G-9968-2014; Alivisatos , Paul /N-8863-2015; Park,
Jungwon/O-1153-2016
OI Alivisatos , Paul /0000-0001-6895-9048; Park,
Jungwon/0000-0003-2927-4331
FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; DOE Office of
Science Early Career Research Program
FX The experiments were conducted using both MSD TEM facility and a
JEOL3010 microscope at National Center for Electron Microscopy (NCEM) of
the Lawrence Berkeley National Laboratory (LBNL), which is supported by
the U.S. Department of Energy (DOE) under contract no.
DE-AC02-05CH11231. H.Z. thanks the DOE Office of Science Early Career
Research Program for their support.
NR 33
TC 60
Z9 60
U1 14
U2 140
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5715
EP 5719
DI 10.1021/nl4035362
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700113
PM 24131312
ER
PT J
AU Cho, JH
Picraux, ST
AF Cho, Jeong-Hyun
Picraux, S. Tom
TI Enhanced Lithium Ion Battery Cycling of Silicon Nanowire Anodes by
Template Growth to Eliminate Silicon Underlayer Islands
SO NANO LETTERS
LA English
DT Article
DE Lithium-ion battery; anode; silicon nanowire; silicon island; anodic
aluminum oxide template
ID THIN-FILM ELECTRODES; PERFORMANCE; CAPACITY; LIFE; STABILITY; CELLS
AB It is well-known that one-dimensional nanostructures reduce pulverization of silicon (SO-based anode materials during Li ion cycling because they allow lateral relaxation. However, even with improved designs, Si nano-wirebased structures still exhibit limited cycling stability for extended numbers of cycles, with the specific capacity retention with cycling not showing significant improvements over commercial carbon-based anode materials. We have found that one important reason for the lack of long cycling stability can be the presence of milli- and microscale Si islands which typically form under nanowire arrays during their growth. Stress buildup in these Si island underlayers with cycling results in cracking, and the loss of specific capacity for Si nanowire anodes, due to progressive loss of contact with current collectors. We show that the formation of these parasitic Si islands for Si nanowires grown directly on metal current collectors can be avoided by growth through anodized aluminum oxide templates containing a high density of sub-100 nm nanopores. Using this template approach we demonstrate significantly enhanced cycling stability for Si nanowire-based lithium-ion battery anodes, with retentions of more than similar to 1000 rnA.h/g discharge capacity over 1100 cycles.
C1 [Cho, Jeong-Hyun; Picraux, S. Tom] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.
RP Cho, JH (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA.
EM jcho@umn.edu; picraux@lanl.gov
FU Nanostructures for Electrical Energy Storage, an Energy Frontier
Research Center; U.S. Department of Energy, Office of Science, Office of
Basic Energy Sciences [DESC0001160]; Los Alamos National Security, LLC,
for the National Nuclear Security Administration of the U.S. Department
of Energy [DE-AC52-06NA25396]
FX This work was supported as part of the Nanostructures for Electrical
Energy Storage, an Energy Frontier Research Center funded by the U.S.
Department of Energy, Office of Science, Office of Basic Energy Sciences
under Award Number DESC0001160. The work was performed, in part, at the
Center for Integrated Nanotechnologies, a U.S. Department of Energy,
Office of Science user facility. Los Alamos National Laboratory, an
affirmative action equal opportunity employer, is operated by Los Alamos
National Security, LLC, for the National Nuclear Security Administration
of the U.S. Department of Energy under contract DE-AC52-06NA25396.
NR 31
TC 36
Z9 36
U1 5
U2 110
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5740
EP 5747
DI 10.1021/nl4036498
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
Physics
GA 253TH
UT WOS:000327111700117
PM 24144166
ER
PT J
AU Gehin, JC
Maldonado, GI
AF Gehin, Jess C.
Maldonado, G. Ivan
TI Special Issue on the PHYSOR 2012 International Conference on the Physics
of Reactors Preface
SO NUCLEAR SCIENCE AND ENGINEERING
LA English
DT Editorial Material
C1 [Gehin, Jess C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
[Maldonado, G. Ivan] Univ Tennessee, Knoxville, TN 37996 USA.
RP Gehin, JC (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
NR 0
TC 0
Z9 0
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 0029-5639
EI 1943-748X
J9 NUCL SCI ENG
JI Nucl. Sci. Eng.
PD NOV
PY 2013
VL 175
IS 3
SI SI
BP VII
EP VII
PG 1
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 257DK
UT WOS:000327363600001
ER
PT J
AU Sanchez, R
Rabiti, C
Wang, YQ
AF Sanchez, Richard
Rabiti, Cristian
Wang, Yaqi
TI Nonlinear Acceleration of a Continuous Finite Element Discretization of
the Self-Adjoint Angular Flux Form of the Transport Equation
SO NUCLEAR SCIENCE AND ENGINEERING
LA English
DT Article; Proceedings Paper
CT American-Nuclear-Society (ANS) International Conference on the Physics
of Reactors (PHYSOR)
CY APR 15-20, 2012
CL Knoxville, TN
SP Amer Nucl Soc, Amer Nucl Soc, Reactor Phys Div, Amer Nucl Soc, Math & Computat Div
ID CONTINUOUS GALERKIN METHOD
AB Nonlinear acceleration of a continuous finite element (CFE) discretization of the transport equation requires a modification of the transport solution in order to achieve local conservation, a condition used in nonlinear acceleration to define the stopping criterion. In this work we implement a coarse-mesh finite difference acceleration for a CFE discretization of the second-order self-adjoint angular flux (SAAF) form of the transport equation and use a postprocessing to enforce local conservation. Numerical results are given for one-group source calculations of one-dimensional slabs. We also give a novel formal derivation of the boundary conditions for the SAAF.
C1 [Sanchez, Richard] Commissariat Energie Atom & Energies Alternat, Serv Etud Reacteurs & Math Appl, Ctr Saclay, DEN SERMA DM2S, Gif Sur Yvettes, France.
[Rabiti, Cristian; Wang, Yaqi] Idaho Natl Lab, Idaho Falls, ID 83415 USA.
RP Sanchez, R (reprint author), Commissariat Energie Atom & Energies Alternat, Serv Etud Reacteurs & Math Appl, Ctr Saclay, DEN SERMA DM2S, Gif Sur Yvettes, France.
EM richard.sanchez@cea.fr
NR 9
TC 1
Z9 1
U1 0
U2 2
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 0029-5639
EI 1943-748X
J9 NUCL SCI ENG
JI Nucl. Sci. Eng.
PD NOV
PY 2013
VL 175
IS 3
SI SI
BP 213
EP 226
PG 14
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 257DK
UT WOS:000327363600002
ER
PT J
AU Jarrell, JJ
Evans, TM
Davidson, GG
Godfrey, AT
AF Jarrell, Joshua J.
Evans, Thomas M.
Davidson, Gregory G.
Godfrey, Andrew T.
TI Full Core Reactor Analysis: Running Denovo on Jaguar
SO NUCLEAR SCIENCE AND ENGINEERING
LA English
DT Article; Proceedings Paper
CT American-Nuclear-Society (ANS) International Conference on the Physics
of Reactors (PHYSOR)
CY APR 15-20, 2012
CL Knoxville, TN
SP Amer Nucl Soc, Amer Nucl Soc, Reactor Phys Div, Amer Nucl Soc, Math & Computat Div
AB Fully consistent, full core, three-dimensional, deterministic neutron transport simulations using the orthogonal mesh code Denovo were run on the massively parallel computing architecture Jaguar XT5. Using energy and spatial parallelization schemes, Denovo was able to efficiently scale to more than 160000 processors. Cell-homogenized cross sections were used with step characteristics, linear discontinuous finite element, and trilinear discontinuous finite element spatial methods. It was determined that using the finite element methods gave considerably more accurate eigenvalue solutions for large aspect ratio meshes than using step characteristics.
C1 [Jarrell, Joshua J.; Evans, Thomas M.; Davidson, Gregory G.] Oak Ridge Natl Lab, Radiat Transport Grp, Oak Ridge, TN 37831 USA.
[Godfrey, Andrew T.] Oak Ridge Natl Lab, Reactor Phys Grp, Oak Ridge, TN 37831 USA.
RP Jarrell, JJ (reprint author), Oak Ridge Natl Lab, Radiat Transport Grp, POB 2008, Oak Ridge, TN 37831 USA.
EM jarrelljj@ornl.gov
OI Jarrell, Joshua/0000-0003-1041-8729
NR 12
TC 4
Z9 4
U1 0
U2 10
PU AMER NUCLEAR SOC
PI LA GRANGE PK
PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA
SN 0029-5639
EI 1943-748X
J9 NUCL SCI ENG
JI Nucl. Sci. Eng.
PD NOV
PY 2013
VL 175
IS 3
SI SI
BP 283
EP 291
PG 9
WC Nuclear Science & Technology
SC Nuclear Science & Technology
GA 257DK
UT WOS:000327363600008
ER
PT J
AU Neil, J
Hash, C
Brugh, A
Fisk, M
Storlie, CB
AF Neil, Joshua
Hash, Curtis
Brugh, Alexander
Fisk, Mike
Storlie, Curtis B.
TI Scan Statistics for the Online Detection of Locally Anomalous Subgraphs
SO TECHNOMETRICS
LA English
DT Article
DE Anomaly detection; Dynamic graph; Network intrusion detection; Path;
Star
ID INTRUSION DETECTION; APPROXIMATIONS; NETWORKS; MODELS; TIME
AB We introduce a computationally scalable method for detecting small anomalous areas in a large, time-dependent computer network, motivated by the challenge of identifying intruders operating inside enterprise-sized computer networks. Time-series of communications between computers are used to detect anomalies, and are modeled using Markov models that capture the bursty, often human-caused behavior that dominates a large subset of the time-series. Anomalies in these time-series are common, and the network intrusions we seek involve coincident anomalies over multiple connected pairs of computers. We show empirically that each time-series is nearly always independent of the time-series of other pairs of communicating computers. This independence is used to build models of normal activity in local areas from the models of the individual time-series, and these local areas are designed to detect the types of intrusions we are interested in. We define a locality statistic calculated by testing for deviations from historic behavior in each local area, and then define a scan statistic as the maximum deviation score over all local areas. We show that identifying these local anomalies is sufficient to correctly identify anomalies of various relevant shapes in the network. Supplementary material, including additional details and simulation code, are provided online.
C1 [Neil, Joshua; Hash, Curtis; Brugh, Alexander; Fisk, Mike] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
[Storlie, Curtis B.] Los Alamos Natl Lab, Stat Sci Grp CCS 6, Los Alamos, NM 87545 USA.
RP Neil, J (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM jneil@lanl.gov; chash@lanl.gov; abrugh@lanl.gov; mfisk@lanl.gov;
storlie@lanl.gov
NR 29
TC 12
Z9 12
U1 2
U2 4
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 403
EP 414
DI 10.1080/00401706.2013.822830
PG 12
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500004
ER
PT J
AU Lawrence, E
Wiel, SV
Bent, R
AF Lawrence, Earl
Wiel, Scott Vander
Bent, Russell
TI Model Bank State Estimation for Power Grids Using Importance Sampling
SO TECHNOMETRICS
LA English
DT Article
DE Electric power; Emulator; Network modeling; Simulator; Surrogate model
ID TOPOLOGY ERRORS; IDENTIFICATION; CALIBRATION; PREDICTION
AB Power grid operators decide where and how much power to generate based on the current topology and demands of the network. The topology can change as safety devices trigger (connecting or disconnecting parts of the network) or as lines go down. Often, the operator cannot observe these events directly, but instead has contemporary measurements and historical information about a subset of the line flows and bus (node) properties. This information can be used in conjunction with a computational model to infer the topology of the network. We present a Bayesian approach to topological inference that considers a bank of possible topologies. The solution provides a probability for each member in the model bank. The approach has two important features. First, we build a statistical approximation, or emulator, to the computational model, which is too computationally expensive to run a large number of times. Second, we use the emulator in an importance sampling scheme to estimate the probabilities. The resulting algorithm is fast enough to use in real time and very accurate. This article has online supplementary materials.
C1 [Lawrence, Earl; Wiel, Scott Vander; Bent, Russell] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Lawrence, E (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM earl@lanl.gov; scottv@lanl.gov; rbent@lanl.gov
OI Bent, Russell/0000-0002-7300-151X
FU LDRD program at Los Alamos National Laboratory
FX This work was supported by the LDRD program at Los Alamos National
Laboratory. Thanks to Kary Myers for organizing the Conference on Data
Analysis and for helpful comments on the article. Thanks also to the
reviewers, the associate editor, and, especially, the editor.
NR 23
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U1 1
U2 3
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 426
EP 435
DI 10.1080/00401706.2013.822424
PG 10
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500006
ER
PT J
AU Storlie, CB
Fugate, ML
Higdon, DM
Huzurbazar, AV
Francois, EG
McHugh, DC
AF Storlie, Curtis B.
Fugate, Michael L.
Higdon, David M.
Huzurbazar, Aparna V.
Francois, Elizabeth G.
McHugh, Douglas C.
TI Methods for Characterizing and Comparing Populations of Shock Wave
Curves
SO TECHNOMETRICS
LA English
DT Article
DE B-splines; Functional data analysis; Gaussian process; Hierarchical
modeling; Nonparametric regression; Onionskin
ID BAYES FACTORS; MODELS
AB At Los Alamos National Laboratory, engineers conduct experiments to evaluate how well detonators and high explosives work. The experimental unit, often called an "onionskin," is a hemisphere consisting of a detonator and a booster pellet surrounded by high explosive material. When the detonator explodes, a streak camera mounted above the pole of the hemisphere records when the shock wave arrives at the surface. The output from the camera is a two-dimensional image that is transformed into a curve that shows the arrival time as a function of polar angle. The statistical challenge is to characterize the population of arrival time curves and to compare the baseline population of onionskins to a new population. The engineering goal is to manufacture a new population of onionskins that generate arrival time curves with the same shape as the baseline. We present two statistical approaches that test for differences in mean curves and provide simultaneous confidence bands for the difference: (i) a B-Spline basis approach and (ii) a Bayesian hierarchical Gaussian process approach. In problems that involve complex modeling with modest sample sizes, it is important to apply multiple approaches with complementary strengths such as these to determine whether all approaches provide similar results. Solid performances of the two approaches are demonstrated on several simulations that were constructed to mimic the actual onionskin analysis. Finally, an analysis of onionskin data is presented. This article also has supplementary materials available online.
C1 [Storlie, Curtis B.; Fugate, Michael L.; Higdon, David M.; Huzurbazar, Aparna V.; Francois, Elizabeth G.; McHugh, Douglas C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Storlie, CB (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM storlie@lanl.gov; fugate@lanl.gov; dhigdon@lanl.gov; aparna@lanl.gov;
elizabethf@lanl.gov; dmchugh@lanl.gov
FU C-8 Enhanced Surveillance program of Los Alamos National Security, LLC
(LANS); U.S. Department of Energy [DE-AC52-06NA25396]
FX The authors' work was funded by the C-8 Enhanced Surveillance program of
Los Alamos National Security, LLC (LANS), operator of the Los Alamos
National Laboratory under Contract No. DE-AC52-06NA25396 with the U.S.
Department of Energy. This article is published under LA-UR-11-05417.
NR 30
TC 1
Z9 1
U1 1
U2 4
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 436
EP 449
DI 10.1080/00401706.2013.805662
PG 14
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500007
ER
PT J
AU Lennox, KP
Glascoe, LG
AF Lennox, Kristin P.
Glascoe, Lee G.
TI A Bayesian Measurement Error Model for Misaligned Radiographic Data
SO TECHNOMETRICS
LA English
DT Article
DE Bayesian nonparametrics; Berkson error; Curve registration;
Heteroscedasticity; Micro-computed tomography; p-splines
ID PENALIZED SPLINES; P-SPLINES; REGISTRATION; REGRESSION; PENALTIES
AB An understanding of the inherent variability in micro-computed tomography (micro-CT) data is essential to tasks such as statistical process control and the validation of radiographic simulation tools. These data present unique challenges to variability analysis due to the relatively low resolution of radiographs, and also due to minor variations from run to run which can result in misalignment or magnification changes between repeated measurements of a sample. Such positioning changes artificially inflate the variability of the data in ways that mask true physical phenomena. We present a novel Bayesian nonparametric regression model that incorporates both additive and multiplicative measurement error in addition to heteroscedasticity to address this problem. We use this model to assess the effects of sample thickness and sample position on measurement variability for an aluminum specimen. Supplementary materials for this article are available online.
C1 [Lennox, Kristin P.; Glascoe, Lee G.] Lawrence Livermore Natl Lab, Computat Engn Div, Livermore, CA 94550 USA.
RP Lennox, KP (reprint author), Lawrence Livermore Natl Lab, Computat Engn Div, 7000 East Ave, Livermore, CA 94550 USA.
EM lennox3@llnl.gov; glascoe1@llnl.gov
FU U.S. Department of Energy by Lawrence Livermore National Laboratory
[DE-AC52-07NA27344]; U.S. Department of Homeland Security, Science and
Technology Directorate
FX This work was performed under the auspices of the U.S. Department of
Energy by Lawrence Livermore National Laboratory under Contract
DE-AC52-07NA27344. The experimental data collection and analysis were
performed under sponsorship of the U.S. Department of Homeland Security,
Science and Technology Directorate. The authors also thank the Editor,
Associate Editor, and referees for their comments and suggestions.
NR 30
TC 0
Z9 0
U1 1
U2 4
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 450
EP 460
DI 10.1080/00401706.2013.838192
PG 11
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500008
ER
PT J
AU Lu, L
Chapman, JL
Anderson-Cook, CM
AF Lu, Lu
Chapman, Jessica L.
Anderson-Cook, Christine M.
TI A Case Study on Selecting a Best Allocation of New Data for Improving
the Estimation Precision of System and Subsystem Reliability Using
Pareto Fronts
SO TECHNOMETRICS
LA English
DT Article
DE Complex system reliability; Genetic algorithm; Multiple data sources;
Optimizing multiple objectives; Resource allocation; Sequential data
collection
ID RESPONSE-SURFACE DESIGN; BINOMIAL SUBSYSTEMS; MULTIPLE CRITERIA;
OPTIMIZATION; SERIES; COMPONENTS
AB This article demonstrates how the Pareto front multiple objective optimization approach can be used to select a best allocation of new data to collect from among many different possible data sources with the goal of maximally reducing the width of the credible intervals of system and two subsystem reliability estimates. The method provides a streamlined decision-making process by identifying a set of noninferior or admissible allocations either from a given set of candidate choices or through a global optimization search and then using graphical methods for selecting the best allocation from the set of contending choices based on the specific goals of the study. The approach allows for an easy assessment of the tradeoffs between criteria and the robustness of different choices to different prioritization of experiment objectives. This is important for decision makers to make a defensible choice of a best allocation that matches their priorities as well as to quantify the anticipated advantages of their choice relative to other options. The method is demonstrated on a small nonaging series system with two subsystems comprised of six components for a total of nine possible data sources. We first consider finding the Pareto front of superior allocations based on 60 logistically viable candidates that have been identified, and second, optimizing over all possible allocations within the allowable fixed budget and comparing how global solutions perform relative to the logistically viable choices. We develop a new search algorithm to populate the Pareto front while taking into account the different costs of the data sources. The method generalizes easily to other system structures and flexible objectives of interest. In addition, a new Fraction of Weight Space plot (FWS) is proposed to provide a simple comparison between different solution choices by summarizing individual performance over the entire weighting space. This article has supplementary materials and computer code available online.
C1 [Lu, Lu] Univ S Florida, Dept Math & Stat, Tampa, FL 33620 USA.
[Chapman, Jessica L.] St Lawrence Univ, Dept Math Comp Sci & Stat, Canton, NY 13617 USA.
[Anderson-Cook, Christine M.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA.
RP Lu, L (reprint author), Univ S Florida, Dept Math & Stat, Tampa, FL 33620 USA.
EM lulu1@usf.edu; jchapman@stlawu.edu; candcook@lanl.gov
FU NSF [0959713]
FX This work was funded in part by NSF Award # 0959713 awarded to St.
Lawrence University. In addition, the authors thank the editor, the
associate editor, and anonymous referees for their valuable comments and
suggestions that have substantially improved this article.
NR 22
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U1 2
U2 5
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 473
EP 487
DI 10.1080/00401706.2013.831776
PG 15
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500010
ER
PT J
AU Higdon, D
Gattiker, J
Lawrence, E
Pratola, M
Jackson, C
Tobis, M
Habib, S
Heitmann, K
Price, S
AF Higdon, Dave
Gattiker, Jim
Lawrence, Earl
Pratola, Matt
Jackson, Charles
Tobis, Michael
Habib, Salman
Heitmann, Katrin
Price, Steve
TI Computer Model Calibration Using the Ensemble Kalman Filter
SO TECHNOMETRICS
LA English
DT Article
DE Bayesian statistics; Computer experiments; Data assimilation; Gaussian
process; Model validation; Parameter estimation; Uncertainty
quantification
ID DIGITAL SKY SURVEY; DATA ASSIMILATION; PARAMETER-ESTIMATION; EFFICIENT
EMULATORS; INVERSE PROBLEMS; OUTPUT; STATE; VALIDATION; REDUCTION;
SYSTEMS
AB Computer model calibration is the process of determining input parameter settings to a computational model that are consistent with physical observations. This is often quite challenging due to the computational demands of running the model. In this article, we use the ensemble Kalman filter (EnKF) for computer model calibration. The EnKF has proven effective in quantifying uncertainty in data assimilation problems such as weather forecasting and ocean modeling. We find that the EnKF can be directly adapted to Bayesian computer model calibration. It is motivated by the mean and covariance relationship between the model inputs and outputs, producing an approximate posterior ensemble of the calibration parameters. While this approach may not fully capture effects due to nonlinearities in the computer model response, its computational efficiency makes it a viable choice for exploratory analyses, design problems, or problems with large numbers of model runs, inputs, and outputs.
C1 [Higdon, Dave; Gattiker, Jim; Lawrence, Earl] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA.
[Pratola, Matt] Ohio State Univ, Dept Stat, Columbus, OH 43210 USA.
[Jackson, Charles; Tobis, Michael] Univ Texas Austin, Inst Geophys, Austin, TX 78759 USA.
[Habib, Salman; Heitmann, Katrin] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.
[Price, Steve] Los Alamos Natl Lab, Fluid Dynam Grp, Los Alamos, NM 87545 USA.
RP Higdon, D (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663, Los Alamos, NM 87545 USA.
EM dhigdon@lanl.gov; gatt@lanl.gov; earl@lanl.gov; pratola@gmail.com;
charles@ig.utexas.edu; tobis@ig.utexas.edu; habib@anl.gov;
heitmann@hep.anl.gov; sprice@lanl.gov
RI Price, Stephen /E-1568-2013; Jackson, Charles/A-2202-2009
OI Price, Stephen /0000-0001-6878-2553; Jackson,
Charles/0000-0002-2870-4494
FU U.S. Department of Energy Office of Science; Office of Advanced
Scientific Computing Research; Scientific Discovery through Advanced
Computing (SciDAC) program
FX We thank the reviewers, Associate Editor, and Editor for many helpful
comments on earlier drafts. This work was supported in part by the U.S.
Department of Energy Office of Science, Office of Advanced Scientific
Computing Research, and Scientific Discovery through Advanced Computing
(SciDAC) program.
NR 50
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U1 2
U2 14
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 488
EP 500
DI 10.1080/00401706.2013.842936
PG 13
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500011
ER
PT J
AU Chen, WC
Ostrouchov, G
Pugmire, D
Prabhat
Wehner, M
AF Chen, Wei-Chen
Ostrouchov, George
Pugmire, David
Prabhat
Wehner, Michael
TI A Parallel EM Algorithm for Model-Based Clustering Applied to the
Exploration of Large Spatio-Temporal Data
SO TECHNOMETRICS
LA English
DT Article
DE Parallel computing; Parallel coordinate plot; Spatial time series;
Unsupervised learning
ID PRECIPITATION EXTREMES; DISCRIMINANT-ANALYSIS; MAXIMUM-LIKELIHOOD
AB We develop a parallel expectation-maximization (EM) algorithm for multivariate Gaussian mixture models and use it to perform model-based clustering of a large climate dataset. Three variants of the EM algorithm are reformulated in parallel and a new variant that is faster is presented. All are implemented using the single program, multiple data programming model, which is able to take advantage of the combined collective memory of large distributed computer architectures to process larger datasets. Displays of the estimated mixture model rather than the data allow us to explore multivariate relationships in a way that scales to arbitrary size data. We study the performance of our methodology on simulated data and apply our methodology to a high-resolution climate dataset produced by the community atmosphere model (CAM5). This article has supplementary material online.
C1 [Chen, Wei-Chen] Univ Tennessee, Dept Ecol & Evolutionary Biol, Knoxville, TN 37996 USA.
[Ostrouchov, George; Pugmire, David] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.
[Prabhat; Wehner, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA.
RP Chen, WC (reprint author), Univ Tennessee, Dept Ecol & Evolutionary Biol, Knoxville, TN 37996 USA.
EM wcchen@utk.edu; ostrouchovg@ornl.gov; pugmire@ornl.gov; prabhat@lbl.gov;
mfwehner@lbl.gov
FU Regional and Global Climate Modeling Program of the Office of Biological
and Environmental Research in the Department of Energy Office of Science
[DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy
[DE-AC05-00OR22725]
FX We sincerely thank the editor, an associate editor and two reviewers for
providing many insightful comments and suggestions which substantially
improved this article. Work at LBNL was supported by the Regional and
Global Climate Modeling Program of the Office of Biological and
Environmental Research in the Department of Energy Office of Science
under contract number DE-AC02-05CH11231. This research also used
resources of the Oak Ridge Leadership Computing Facility at the Oak
Ridge National Laboratory, which is supported by the Office of Science
of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725.
NR 31
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U1 1
U2 9
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 513
EP 523
DI 10.1080/00401706.2013.826146
PG 11
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500013
ER
PT J
AU Theiler, J
AF Theiler, James
TI Matched-Pair Machine Learning
SO TECHNOMETRICS
LA English
DT Article
DE Algorithms; Classification; Hyperspectral imagery; Hypothesis testing;
Signal detection; Structured data
ID PLUMES
AB Following an analogous distinction in statistical hypothesis testing and motivated by chemical plume detection in hyperspectral imagery, we investigate machine-learning algorithms where the training set is comprised of matched pairs. We find that even conventional classifiers exhibit improved performance when the input data have a matched-pair structure, and we develop an example of a "dipole" algorithm to directly exploit this structured input. In some scenarios, matched pairs can be generated from independent samples, with the effect of not only doubling the nominal size of the training set, but of providing the matched-pair structure that leads to better learning. The creation of matched pairs from a dataset of interest also permits a kind of transductive learning, which is found for the plume detection problem to exhibit improved performance. Supplementary materials for this article are available online.
C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA.
RP Theiler, J (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.
EM jt@lanl.gov
FU United States Department of Energy through the Los Alamos Laboratory
Directed Research and Development (LDRD) program
FX I am grateful to Bernard Foy for many valuable conversations about
chemical plumes in hyperspectral imagery, and to Don Hush and Reid
Porter for insightful discussions on transductive learning. I am very
pleased to acknowledge the reviewers and editors of Technometrics for
their careful reading of this article, and for their numerous and
thoughtful suggestions; thanks to them, this is a much better article.
This work was supported by the United States Department of Energy
through the Los Alamos Laboratory Directed Research and Development
(LDRD) program.
NR 18
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Z9 3
U1 1
U2 2
PU AMER STATISTICAL ASSOC
PI ALEXANDRIA
PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA
SN 0040-1706
EI 1537-2723
J9 TECHNOMETRICS
JI Technometrics
PD NOV
PY 2013
VL 55
IS 4
BP 536
EP 547
DI 10.1080/00401706.2013.838191
PG 12
WC Statistics & Probability
SC Mathematics
GA 257OO
UT WOS:000327394500015
ER
PT J
AU Wirth, M
Oh, H
Mormino, EC
Markley, C
Landau, SM
Jagust, WJ
AF Wirth, Miranka
Oh, Hwamee
Mormino, Elizabeth C.
Markley, Candace
Landau, Susan M.
Jagust, William J.
TI The effect of amyloid beta on cognitive decline is modulated by neural
integrity in cognitively normal elderly
SO ALZHEIMERS & DEMENTIA
LA English
DT Article
DE Alzheimer's disease; Cognitive aging; Memory; Preclinical decline;
Amyloid; PiB; Glucose metabolism; FDG; Gray matter structure
ID PRECLINICAL ALZHEIMERS-DISEASE; PITTSBURGH COMPOUND-B; A-BETA;
NONDEMENTED INDIVIDUALS; EPISODIC MEMORY; VOLUME LOSS; BRAIN;
DEPOSITION; IMPAIRMENT; DYSFUNCTION
AB Objective: Alzheimer's disease (AD) pathology of amyloid beta (A beta) accumulation and neurodegeneration may be relevant to preclinical cognitive decline. The objective of this study was to relate AD-sensitive biomarkers of A beta and neurodegeneration and their interaction to longitudinal cognitive change in cognitively normal elderly.
Methods: Thirty-eight older people completed at least three consecutive neuropsychological examinations. Using positron emission tomography (PET), A beta plaque burden was measured with [C-11] Pittsburgh compound B (PiB). PiB retention was dichotomized into a positive (n = 13) and negative (n = 25) PiB status. Neurodegenerative biomarkers were extracted within AD-vulnerable regions of interest (ROIs)-namely, the hippocampus and temporoparietal cortical areas. Within each ROT, metabolism was quantified with [F-18] fluorodeoxyglucose (FDG) PET, and the gray matter structure was evaluated using volume (hippocampus) or thickness (cortical regions). ROT-specific functional and structural biomarkers were combined further into cross-modality neurodegenerative composite measures. Using hierarchical regression models, PiB and the neurodegenerative biomarkers were related to cognitive trajectories.
Results: PiB positivity was associated with memory and nonmemory worsening. The neurodegenerative biomarkers modified these relationships. Longitudinal cognitive decline was accelerated in those individuals who exhibited both PiB positivity and lower neurodegenerative biomarker scores, although the two measures appeared to be independent. PiB retention interacted predominantly with the cortical neurodegenerative composite for nonmemory change. Memory decline was best explained by the interaction between PiB and the hippocampal neurodegenerative composite, suggesting regional specificity of the neurodegenerative modulations.
Conclusions: Our findings indicate that cognitive trajectories deteriorate at a faster rate in cognitively normal individuals expressing A beta burden and neurodegeneration within specific AD-sensitive regions. (C) 2013 The Alzheimer's Association. All rights reserved.
C1 [Wirth, Miranka; Oh, Hwamee; Mormino, Elizabeth C.; Markley, Candace; Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.
[Landau, Susan M.; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.
RP Wirth, M (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.
EM miranka.wirth@gmail.com
FU National Institutes of Health [AG034570]; Swiss National Science
Foundation [PA00P1_131515]
FX This work was supported by National Institutes of Health grant AG034570
and the Swiss National Science Foundation grant PAO0P1_131515. We
gratefully thank the following contributors: Martina Studer (University
of Bern, Switzerland, behavioral analysis), Cindee Madison (University
of California [UC] at Berkeley, neuroimaging analysis), Tad Haight (UC
at Berkeley, statistics support), Natalie Marchant (UC at Berkeley,
manuscript editing), Benedicte Rossi (UC at Berkeley, discussion).
NR 49
TC 18
Z9 18
U1 2
U2 8
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1552-5260
EI 1552-5279
J9 ALZHEIMERS DEMENT
JI Alzheimers. Dement.
PD NOV
PY 2013
VL 9
IS 6
BP 687
EP 698
DI 10.1016/j.jalz.2012.10.012
PG 12
WC Clinical Neurology
SC Neurosciences & Neurology
GA 254NP
UT WOS:000327172700009
PM 23474040
ER
PT J
AU Manghnani, MH
Hushur, A
Smyth, JR
Nestola, F
Dera, P
Sekar, M
Amulele, G
Frost, DJ
AF Manghnani, Murli H.
Hushur, Anwar
Smyth, Joseph R.
Nestola, Fabrizio
Dera, Przemyslaw
Sekar, Mariappan
Amulele, George
Frost, Daniel J.
TI Compressibility and structural stability of two variably hydrated
olivine samples (Fo(97)Fa(3)) to 34 GPa by X-ray diffraction and Raman
spectroscopy
SO AMERICAN MINERALOGIST
LA English
DT Article
DE Hydrous olivine; X-ray diffraction; Raman spectroscopy; hydration
mechanism; high pressure
ID SAN CARLOS OLIVINE; POSSIBLE HYDROGEN POSITIONS; HIGH-PRESSURE;
CRYSTAL-STRUCTURE; SILICA ACTIVITY; FORSTERITE MG2SIO4; ACCESSORY
MINERALS; THERMAL-EXPANSION; MANTLE PRESSURES; WATER
AB The content and transport of fluid phases such as water into the deep Earth is of great importance not only to correlate seismological models of the planet's interior with mineralogical models, but also for the understanding of the evolution of the solid Earth as well as the Earth's atmosphere. This study reports on the influence of water on the structural and physical properties of olivine, which is known to be the main constituent of the upper mantle.
Two hydrous olivines of composition Fo(97)Fa(3) with water content of 4883 parts per million by weight (ppmw) (SZ0407A) and 8000 ppmw (SZ0407B) were synthesized at 1250 degrees C and 12 GPa. Single-crystal X-ray diffraction was used to determine unit-cell parameters of SZ0407A and SZ0407B at pressures up to 7.1 GPa at room temperature. Synchrotron powder X-ray diffraction and Raman scattering experiments were performed on sample SZ0407A in a diamond-anvil cell to 34 GPa at room temperature. For both samples, the compressibility is the largest along the b-axis and smallest along the a-axis. Using the compression (V/V-o) vs. pressure data for sample SZ0407A to 29 GPa, in conjunction with the third-order Birch-Murnaghan equation of state, we calculate the isothermal bulk modulus and its pressure derivative as K-o = 119.2(12) GPa and K-o' = 6.6(4). Single-crystal compression data for sample SZ0407A to 7 GPa give K-o = 121.5(6) GPa and K-o' = 5.7(2); and for sample SZ0407B K-o = 122.2(12) GPa and K-o' = 6.2(4). High-pressure Raman spectra for SZ0407A up to 34 GPa show a continuous shift of all the observed bands to higher frequency with increasing pressure; there is no indication of any first-order phase transition. However, the Raman spectra indicate subtle discontinuous changes around 22 GPa, unobserved in previously reported studies on anhydrous olivines.
C1 [Manghnani, Murli H.; Hushur, Anwar; Amulele, George] Univ Hawaii, Hawaii Inst Geophys & Planetol, Honolulu, HI 96822 USA.
[Smyth, Joseph R.] Univ Colorado, Dept Geol Sci, Boulder, CO 80309 USA.
[Nestola, Fabrizio] Univ Padua, Dept Geosci, I-35131 Padua, Italy.
[Dera, Przemyslaw] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, Chicago, IL 60637 USA.
[Sekar, Mariappan] Indira Gandhi Ctr Atom Res, Kalpaakam 603102, Tamil Nadu, India.
[Frost, Daniel J.] Univ Bayreuth, Bayer Geoinst, D-95440 Bayreuth, Germany.
RP Manghnani, MH (reprint author), Univ Hawaii, Hawaii Inst Geophys & Planetol, Honolulu, HI 96822 USA.
EM murli@soest.hawaii.edu
RI nestola, fabrizio/K-2798-2015; Frost, Daniel/B-7526-2016
OI nestola, fabrizio/0000-0002-4875-5125; Frost, Daniel/0000-0002-4443-8149
FU U.S. National Science Foundation [EAR 0538884, 0957137, EAR 11-13369];
Alexander von Humboldt Foundation; National Science Foundation - Earth
Sciences [EAR-1128799]; Department of Energy, Geosciences
[DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science,
Office of Basic Energy Sciences [DE-AC02-06CH11357]
FX We thank the two reviewers, Quentin Williams, and Alexandra Friedrich
(Associate Editor) for their valuable comments and suggestions for
improving the manuscript. Thanks are due to John Balogh for maintaining
the Raman system in good working order. This work was supported by U.S.
National Science Foundation Grants EAR 0538884 and 0957137 to M.H.M.,
and EAR 11-13369 to J.R.S. Syntheses were performed at Bayerisches
Geoinstitut, Universitaet Bayreuth, Germany, and supported, in part, by
the Alexander von Humboldt Foundation to J.S. and F.N. Portions of this
work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon
Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is
supported by the National Science Foundation - Earth Sciences
(EAR-1128799) and Department of Energy, Geosciences (DE-FG02-94ER14466).
Use of the Advanced Photon Source was supported by the U.S. Department
of Energy, Office of Science, Office of Basic Energy Sciences, under
contract no. DE-AC02-06CH11357. The SOEST and HIGP contribution numbers
for this paper are 2013 and 8941.
NR 66
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U1 1
U2 40
PU MINERALOGICAL SOC AMER
PI CHANTILLY
PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA
SN 0003-004X
EI 1945-3027
J9 AM MINERAL
JI Am. Miner.
PD NOV-DEC
PY 2013
VL 98
IS 11-12
BP 1972
EP 1979
DI 10.2138/am.2013.4462
PG 8
WC Geochemistry & Geophysics; Mineralogy
SC Geochemistry & Geophysics; Mineralogy
GA 252YP
UT WOS:000327049100007
ER
PT J
AU Xiong, YL
Kirkes, L
Westfall, T
AF Xiong, Yongliang
Kirkes, Leslie
Westfall, Terry
TI Experimental determination of solubilities of sodium tetraborate (borax)
in NaCl solutions, and a thermodynamic model for the Na-B(OH)(3)-Cl-SO4
system to high-ionic strengths at 25 degrees C
SO AMERICAN MINERALOGIST
LA English
DT Article
DE Pitzer model; borate; actinide solubility; nuclear waste isolation;
geological repositories; Waste Isolation Pilot Plant (WIPP); performance
assessment (PA); concentrated brines
ID NUCLEAR-WASTE ISOLATION; ROOM-TEMPERATURE; NATURAL-WATERS;
HYDROMAGNESITE; DISSOCIATION; PREDICTION; EQUILIBRIA; STABILITY;
CONSTANTS; PAIRS
AB In this study, solubility experiments on sodium tetraborate (NaB4O7 center dot 10H(2)O, borax) are conducted in NaCl solutions up to 5.0 m at room temperature (22.5 +/- 1.5 degrees C). In combination with solubility data of sodium tetraborate in Na2SO4 solutions from the literature, the solubility constant (log K-sp) for sodium tetraborate for the following reaction
Na2B4O7 center dot 10H(2)O = 2Na(+) + 4B(OH)(4)(-) + 2H(+) + H2O (1) (1)
is determined as -24.80 +/- 0.10 based on the Pitzer model. In conjunction with the relevant Pitzer parameters, based on the above log K-sp for borax, and log beta(1) (0.25 +/- 0.01) evaluated from the literature for the following complex formation reaction
Na+ + B(OH)(4)(-) = NaB(OH)(4)(aq) (2)
a thermodynamic model with high precision is established for the Na+-B(OH)(3)-Cl--SO42- system at high-ionic strengths up to saturation of halite (NaCl), mirabilite (Na2SO4 center dot 10H(2)O), and thenardite (Na2SO4). The model is validated by comparison of model predicted equilibrium compositions for the assemblages of borax alone, borax + halite, borax + mirabilite, borax + halite + thenardite, and borax + mirabilite + thenardite in the mixtures of NaCl+Na2SO4 to ionic strengths of 8.0 m, with independent experimental values from the literature. The differences in concentrations of major ions, e.g., Na+, Cl-, and SO42-, between model predicted and experimental values are generally <0.5%. The difference for total boron concentrations is <0.05 m with an error <25%.
The revised thermodynamic model is applied to the potential recovery of borax from boron-enriched brines via evaporation at 25 degrees C, using the two brines from China as examples. The reaction path calculations suggest that the brine from the Zhabei Salt Lake in Xizang (Tibet) Autonomous Region, is suitable to recovery of borax via evaporation at 25 degrees C, whereas the brine from the western Sichuan Province, although it is enriched in boron, is not suitable to extraction of boron as borax, but is suitable to extraction of potassium as sylvite, via evaporation at 25 degrees C.
C1 [Xiong, Yongliang; Kirkes, Leslie; Westfall, Terry] Sandia Natl Labs, Carlsbad Programs Grp, Carlsbad, NM 88220 USA.
RP Xiong, YL (reprint author), Sandia Natl Labs, Carlsbad Programs Grp, 4100 Natl Pk Highway, Carlsbad, NM 88220 USA.
EM yxiong@sandia.gov
FU U.S. Department of Energy's National Nuclear Security Administration
[DE-AC04-94AL85000]; WIPP programs
FX Sandia National Laboratories is a multiprogram laboratory operated by
Sandia Corporation, a wholly owned subsidiary of Lockheed Martin
Corporation, for the U.S. Department of Energy's National Nuclear
Security Administration under Contract DE-AC04-94AL85000. This research
is funded by WIPP programs administered by the Office of Environmental
Management (EM) of the U.S. Department of Energy. We are grateful to
Shelly Nielsen, Taya Olivas, Tana Saul, Diana Goulding, Brittany Hoard,
Cassandra Marrs, Danelle Morrill, Mathew Stroble, and Kira Vincent, for
their laboratory assistance. We thank the journal reviewers for their
reviews, Rick Wilkin, the Associate Editor, and Keith Putirka, the
Editor, for their reviews and editorial efforts.
NR 31
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U1 2
U2 23
PU MINERALOGICAL SOC AMER
PI CHANTILLY
PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA
SN 0003-004X
EI 1945-3027
J9 AM MINERAL
JI Am. Miner.
PD NOV-DEC
PY 2013
VL 98
IS 11-12
BP 2030
EP 2036
DI 10.2138/am.2013.4398
PG 7
WC Geochemistry & Geophysics; Mineralogy
SC Geochemistry & Geophysics; Mineralogy
GA 252YP
UT WOS:000327049100012
ER
PT J
AU Pazmino, JH
Bai, CS
Miller, JT
Ribeiro, FH
Delgass, WN
AF Pazmino, Jorge H.
Bai, Chuansheng
Miller, Jeffrey T.
Ribeiro, Fabio H.
Delgass, W. Nicholas
TI Effects of Support on Sulfur Tolerance and Regeneration of Pt Catalysts
Measured by Ethylene Hydrogenation and EXAFS
SO CATALYSIS LETTERS
LA English
DT Article
DE Sulfur; Poisoning; Regeneration; Ethylene hydrogenation; EXAFS; SMSI;
Support effect
ID INFRARED-SPECTROSCOPY; REDUCTION CATALYST; PT/AL2O3 CATALYSTS; IRIDIUM
CATALYSTS; NOX STORAGE; PLATINUM; TIO2; CHEMISORPTION; PT(111); PT/TIO2
AB The effect of support on sulfur tolerance and regenerability under reducing environments was investigated by rate measurements for ethylene hydrogenation, hydrogen chemisorption, and extended X-ray absorption fine structure (EXAFS). Catalysts, 1 % Pt/Al2O3 and 1 % Pt/P25 (TiO2), were tested after sulfidation in H2S/H-2 at 250 A degrees C followed by regeneration treatments in H-2 at 250, 350 and 450 A degrees C. Our combined results showed a 20-27 times decrease in the rate of ethylene hydrogenation on both sulfided catalysts, accompanied by a 4-6 times drop in the Pt surface area. Regenerations up to 450 A degrees C were unable to remove all the sulfur, as evidenced by the presence of Pt-S bonds by EXAFS at about 2.25-2.33 , characteristic lengths for chemisorbed sulfur and bulk-type PtS. However, a partial recovery of the hydrogenation rate per mole of Pt was observed on sulfided Pt/Al2O3 after reduction at 450 A degrees C, while the induction of strong metal support interactions (SMSI) at reduction temperature above 350 A degrees C was observed on Pt/P25, regardless of the presence of sulfur. For Pt/P25, the reversal of the SMSI state together with sulfur removal by mild oxidation suggests that sequential reduction/oxidation treatments may be more effective in restoring the S-free state of TiO2-supported catalysts.
Pt/Al2O3 and Pt/TiO2 (P25) sulfur tolerance and regenerability were evaluated after reduction treatments in H-2. Both catalysts were equally poisoned by sulfur based on C2H4 hydrogenation. Reduction treatments up to 450 A degrees C were not able to remove sulfur on either catalyst. Sulfur on Pt may inhibit the formation of the SMSI state on Pt/TiO2, especially below 350 A degrees C.
C1 [Pazmino, Jorge H.; Ribeiro, Fabio H.; Delgass, W. Nicholas] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA.
[Bai, Chuansheng] ExxonMobil Res & Engn Co, Annandale, NJ 08801 USA.
[Miller, Jeffrey T.] Argonne Natl Lab, Div Chem Technol, Argonne, IL 60439 USA.
RP Delgass, WN (reprint author), Purdue Univ, Sch Chem Engn, 480 Stadium Mall Dr, W Lafayette, IN 47907 USA.
EM delgass@ecn.purdue.edu
RI ID, MRCAT/G-7586-2011;
OI Ribeiro, Fabio/0000-0001-7752-461X
FU ExxonMobil Research and Engineering Company
FX The authors would like to acknowledge Drs. Stuart Soled, Michael Daage,
Pallassana S. Vankataraman, Prasenjeet Ghosh and Yogesh V. Joshi for
useful discussions and active participation in this work and ExxonMobil
Research and Engineering Company for financial support.
NR 54
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U1 5
U2 46
PU SPRINGER
PI NEW YORK
PA 233 SPRING ST, NEW YORK, NY 10013 USA
SN 1011-372X
EI 1572-879X
J9 CATAL LETT
JI Catal. Lett.
PD NOV
PY 2013
VL 143
IS 11
BP 1098
EP 1107
DI 10.1007/s10562-013-1135-y
PG 10
WC Chemistry, Physical
SC Chemistry
GA 250YP
UT WOS:000326893300002
ER
PT J
AU Muller, MR
Muller, MB
Rao, P
AF Muller, Michael R.
Muller, Michael B.
Rao, Prakash
TI Optimize Energy Use in Industrial Cooling Systems
SO CHEMICAL ENGINEERING PROGRESS
LA English
DT Article
ID TOWERS
C1 [Muller, Michael R.; Muller, Michael B.] Rutgers State Univ, Piscataway, NJ 08855 USA.
[Rao, Prakash] Lawrence Berkeley Natl Lab, Berkeley, CA USA.
RP Muller, MR (reprint author), Rutgers State Univ, Piscataway, NJ 08855 USA.
EM mullerm@rci.rutgers.edu; mbmuller@caes.rutgers.edu; prao@lbl.gov
NR 12
TC 0
Z9 0
U1 1
U2 4
PU AMER INST CHEMICAL ENGINEERS
PI NEW YORK
PA 3 PARK AVE, NEW YORK, NY 10016-5901 USA
SN 0360-7275
EI 1945-0710
J9 CHEM ENG PROG
JI Chem. Eng. Prog.
PD NOV
PY 2013
VL 109
IS 11
BP 18
EP 23
PG 6
WC Engineering, Chemical
SC Engineering
GA 252XQ
UT WOS:000327046600009
ER
PT J
AU Caes, BR
Van Oosbree, TR
Lu, FC
Ralph, J
Maravelias, CT
Raines, RT
AF Caes, Benjamin R.
Van Oosbree, Thomas R.
Lu, Fachuang
Ralph, John
Maravelias, Christos T.
Raines, Ronald T.
TI Simulated Moving Bed Chromatography: Separation and Recovery of Sugars
and Ionic Liquid from Biomass Hydrolysates
SO CHEMSUSCHEM
LA English
DT Article
DE corn stover; ionic liquids; lignin; liquid chromatography;
oligosaccharides
ID LIGNOCELLULOSIC BIOMASS; BIOFUELS PRODUCTION; ESCHERICHIA-COLI; ARYL
ETHERS; CORN STOVER; CELLULOSE; LIGNIN; PRETREATMENT; DISSOLUTION;
HYDROLYZATE
C1 [Caes, Benjamin R.; Van Oosbree, Thomas R.; Lu, Fachuang; Ralph, John; Maravelias, Christos T.; Raines, Ronald T.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA.
[Caes, Benjamin R.; Raines, Ronald T.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA.
[Van Oosbree, Thomas R.; Lu, Fachuang; Ralph, John; Raines, Ronald T.] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA.
[Maravelias, Christos T.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA.
RP Caes, BR (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, 1550 Linden Dr, Madison, WI 53706 USA.
EM rtraines@wisc.edu
RI Maravelias, Christos/B-1376-2009
OI Maravelias, Christos/0000-0002-4929-1748
FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science)
[DE-FC02-07ER64494]; University of Wisconsin-Madison BACTER Institute
[DE-FG02-04ER25627]; NIH [P41 RR02301, P41 GM066326, RR02781, RR08438];
University of Wisconsin-Madison; NSF [DMB-8415048, OIA-9977486,
BIR-9214394]; USDA
FX This work was supported by the DOE Great Lakes Bioenergy Research Center
(DOE BER Office of Science DE-FC02-07ER64494) and the University of
Wisconsin-Madison BACTER Institute through grant DE-FG02-04ER25627. This
work made use of the National Magnetic Resonance Facility at Madison,
which is supported by NIH Grants P41 RR02301 and P41 GM066326.
Additional equipment was purchased with funds from the University of
Wisconsin-Madison, the NIH (RR02781, RR08438), the NSF (DMB-8415048,
OIA-9977486, BIR-9214394), and the USDA. We are grateful to Semba
Biosciences for the loan of an Octave 10 Chromatography System, Dr. A.
Grabski and Dr. R. Mierendorf for assistance with its use, Dr. N. de
Leon and Dr. B. E. Dale for corn stover samples, Dr. D. H. Keating for
E. coli KO11, Dr. M. T. Tremaine, S. Liu, and C. H. Eller for
experimental assistance, and Merck KGaA for [BMIM]Cl.
NR 63
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U1 3
U2 60
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1864-5631
EI 1864-564X
J9 CHEMSUSCHEM
JI ChemSusChem
PD NOV
PY 2013
VL 6
IS 11
BP 2083
EP 2089
DI 10.1002/cssc.201300267
PG 7
WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY
SC Chemistry; Science & Technology - Other Topics
GA 250HA
UT WOS:000326840000015
PM 23939991
ER
PT J
AU Chae, WS
Yu, H
Ham, SK
Lee, MJ
Jung, JS
Robinson, DB
AF Chae, Weon-Sik
Yu, Hyunung
Ham, Sung-Kyoung
Lee, Myung-Jin
Jung, Jin-Seung
Robinson, David B.
TI Bimodal porous gold opals for molecular sensing
SO ELECTRONIC MATERIALS LETTERS
LA English
DT Article
DE nanoporous; gold; bimodal; SERS; opal
ID ENHANCED RAMAN-SCATTERING; SURFACE-PLASMON; FILMS; FABRICATION;
ELECTRODES; SERS
AB We have fabricated bimodal porous gold skeletons by double-templating routes using poly(styrene) colloidal opals as templates. The fabricated gold skeletons show a bimodal pore-size distribution, with small pores within spheres and large pores between spheres. The templated bimodal porous gold skeletons were applied in Raman scattering experiments to study sensing efficiency for probe molecules. We found that the bimodal porous gold skeletons showed obvious enhancement of Raman scattering signals versus that of the unimodal porous gold which only has interstitial pores of several hundred nanometers.
C1 [Chae, Weon-Sik; Ham, Sung-Kyoung; Lee, Myung-Jin] Korea Basic Sci Inst, Gangneung Ctr, Kangnung 210702, South Korea.
[Yu, Hyunung] Korea Res Inst Stand & Sci, Taejon 305340, South Korea.
[Jung, Jin-Seung] Gangneung Wonju Nanot Univ, Dept Chem, Kangnung 210702, South Korea.
[Robinson, David B.] Sandia Natl Labs, Livermore, CA 94550 USA.
RP Chae, WS (reprint author), Korea Basic Sci Inst, Gangneung Ctr, Kangnung 210702, South Korea.
EM wschae@kbsi.re.kr
FU KBSI [F32603]; KRF [2011-0008671]; WISET grant [PGD046]
FX This work was supported by KBSI, International Joint Research Program
(F32603) and partly by a KRF grant (No. 2011-0008671) and a WISET grant
(PGD046).
NR 15
TC 7
Z9 7
U1 3
U2 16
PU KOREAN INST METALS MATERIALS
PI SEOUL
PA KIM BLDG 6TH FLOOR, SEOCHO-DAERO 56 GIL 38, SEOCHO-GU, SEOUL 137-881,
SOUTH KOREA
SN 1738-8090
EI 2093-6788
J9 ELECTRON MATER LETT
JI Electron. Mater. Lett.
PD NOV
PY 2013
VL 9
IS 6
BP 783
EP 786
DI 10.1007/s13391-013-6011-9
PG 4
WC Materials Science, Multidisciplinary
SC Materials Science
GA 253YQ
UT WOS:000327126500017
ER
PT J
AU Greene, DL
AF Greene, David L.
TI Energy policy: Where are the boundaries?
SO ENERGY POLICY
LA English
DT Editorial Material
C1 Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
RP Greene, DL (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.
NR 0
TC 2
Z9 2
U1 0
U2 14
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
EI 1873-6777
J9 ENERG POLICY
JI Energy Policy
PD NOV
PY 2013
VL 62
BP 1
EP 2
DI 10.1016/j.enpol.2013.08.042
PG 2
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 249IG
UT WOS:000326770300001
ER
PT J
AU Davidson, C
Steinberg, D
AF Davidson, Carolyn
Steinberg, Daniel
TI Evaluating the impact of third-party price reporting and other drivers
on residential photovoltaic price estimates
SO ENERGY POLICY
LA English
DT Article
DE Residential photovoltaic; Third-party ownership; Market tracking
AB Aim: Policy-makers typically track the rapidly evolving U.S. residential photovoltaic (PV) market by relying on price data reported by PV installers/integrators to incentive programs. Recent years have witnessed a shift toward third-party-owned (TPO) business models, in which the absence of a cash purchase price obscures data interpretation. Appraisals-often based on estimates of the average fair market value across a diverse fleet of systems-are one way TPO prices are reported.
Scope: This study investigates residential PV system price drivers to improve the accuracy, consistency, and relevance of PV price-tracking efforts. Our econometric approach evaluates system price drivers using California Solar Initiative data, controlling for system, installer, and geographic variables.
Conclusions: We find that reported prices for confirmed appraised systems are $1.13/W higher than non-appraised systems and do not respond to hypothesized price drivers. For non-appraised systems, we find preliminary evidence of market distortions based on the impact of the incentive level, module cost and household income on reported price. Further, unspecified installer heterogeneity-possibly due to differences in products, cost structure or reporting practices-is a substantial price driver. Using estimates, we develop a price model to approximate non-appraised system prices. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Davidson, Carolyn; Steinberg, Daniel] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO 80401 USA.
RP Davidson, C (reprint author), Natl Renewable Energy Lab, Strateg Energy Anal Ctr, 15013 Denver West Pkwy,RSF 300, Golden, CO 80401 USA.
EM Carolyn.Davidson@nrel.gov
OI Steinberg, Daniel/0000-0003-1769-2261
NR 23
TC 4
Z9 4
U1 1
U2 13
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
EI 1873-6777
J9 ENERG POLICY
JI Energy Policy
PD NOV
PY 2013
VL 62
BP 752
EP 761
DI 10.1016/j.enpol.2013.07.112
PG 10
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 249IG
UT WOS:000326770300076
ER
PT J
AU He, YX
Wang, B
Wang, JH
Xiong, W
Xia, T
AF He, Yongxiu
Wang, Bing
Wang, Jianhui
Xiong, Wei
Xia, Tian
TI Correlation between Chinese and international energy prices based on a
HP filter and time difference analysis
SO ENERGY POLICY
LA English
DT Article
DE Energy prices; HP filter; Time difference analysis
ID ELECTRICITY PRICE; GAS PRICES; OIL; CAUSALITY; DYNAMICS; MARKETS; COSTS;
COAL
AB To establish a reasonable system and mechanism for Chinese energy prices, we use the Granger causality test, Hodrick-Prescott (HP) filter and time difference analysis to research the pricing relationship between Chinese and international energy prices. We find that Chinese and international crude oil prices changed synchronously while Chinese refined oil prices follow the changes of international oil prices with the time difference being about 1 month to 2 months. Further, Australian coal prices Granger causes Chinese coal prices, and there is a high correlation between them. The U.S. electricity price is influenced by the WTI crude oil price, the U.S. gasoline price and the HenryHub gas price. Due to the unreasonable price-setting mechanism and regulation from the central government, China's terminal market prices for both electricity and natural gas do not reflect the real supply-demand situation. This paper provides quantitative results on the correlation between Chinese and international energy prices to better predict the impact of international energy price fluctuations on China's domestic energy supply and guide the design of more efficient energy pricing policies. Moreover, it provides references for developing countries to improve their energy market systems and trading, and to coordinate domestic and international energy markets. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [He, Yongxiu; Wang, Bing; Xiong, Wei; Xia, Tian] North China Elect Power Univ, Sch Econ & Management, Beijing 102206, Peoples R China.
[Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA.
[Wang, Jianhui] Shanghai Univ Elect Power, Sch Econ & Management, Shanghai, Peoples R China.
[Xia, Tian] Gansu Elect Power Corp, Lanzhou, Peoples R China.
RP He, YX (reprint author), North China Elect Power Univ, Sch Econ & Management, Bei Nong Rd 2, Beijing 102206, Peoples R China.
EM heyongxiu@ncepu.edu.cn
FU National Natural Science Foundation of China [71273089]; Beijing Natural
Science Foundation of China [9122022]; U.S. Department of Energy
[DE-AC02-06CH11357]
FX The work described in this paper was supported by the National Natural
Science Foundation of China (Grant No. 71273089) and Beijing Natural
Science Foundation of China (Grant No. 9122022). Argonne National
Laboratory's work was supported under U.S. Department of Energy contract
DE-AC02-06CH11357.
NR 24
TC 4
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U1 5
U2 27
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
EI 1873-6777
J9 ENERG POLICY
JI Energy Policy
PD NOV
PY 2013
VL 62
BP 898
EP 909
DI 10.1016/j.enpol.2013.07.136
PG 12
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 249IG
UT WOS:000326770300091
ER
PT J
AU Cappers, P
MacDonald, J
Goldman, C
Ma, O
AF Cappers, Peter
MacDonald, Jason
Goldman, Charles
Ma, Ookie
TI An assessment of market and policy barriers for demand response
providing ancillary services in US electricity markets
SO ENERGY POLICY
LA English
DT Article
DE Demand response; Renewable integration; Ancillary services
ID TECHNOLOGIES
AB An impact of increased variable renewable generation is the need for balancing authorities to procure more ancillary services. While demand response resources are technically capable of providing these services, current experience across the U.S. illustrates they are relatively minor players in most regions. Accessing demand response resources for ancillary services may require a number of changes to policies and common practices at multiple levels. Regional reliability councils must first define ancillary services such that demand response resources may provide them. Once the opportunity exists, balancing authorities define and promulgate rules that set the infrastructure investments and performance attributes of a resource wishing to provide such services. These rules also dictate expected revenue streams which reveal the cost effectiveness of these resources. The regulatory compact between utility and state regulators, along with other statutes and decisions by state policymakers, may impact the interest of demand response program providers to pursue these resources as ancillary service providers. This paper identifies within these broad categories specific market and policy barriers to demand response providing ancillary services in different wholesale and retail environments, with emphasis on smaller customers who must be aggregated through a program provider to meet minimum size requirements for wholesale transactions. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Cappers, Peter; MacDonald, Jason; Goldman, Charles] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Ma, Ookie] US DOE, Off Energy Efficiency & Renewable Energy, Washington, DC 20585 USA.
RP Cappers, P (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM PACappers@lbl.gov
RI MacDonald, Jason/C-8726-2013
OI MacDonald, Jason/0000-0003-0298-5387
NR 39
TC 26
Z9 27
U1 0
U2 11
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
EI 1873-6777
J9 ENERG POLICY
JI Energy Policy
PD NOV
PY 2013
VL 62
BP 1031
EP 1039
DI 10.1016/j.enpol.2013.08.003
PG 9
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 249IG
UT WOS:000326770300103
ER
PT J
AU Hong, LX
Zhou, N
Fridley, D
Raczkowski, C
AF Hong, Lixuan
Zhou, Nan
Fridley, David
Raczkowski, Chris
TI Assessment of China's renewable energy contribution during the 12th Five
Year Plan
SO ENERGY POLICY
LA English
DT Article
DE China; Renewable; 12th Five Year Plan
ID LARGE-SCALE INTEGRATION; SMALL CHP-PLANTS; WIND POWER; HIGH PENETRATION;
SYSTEM-ANALYSIS; ELECTRICITY; CHALLENGES; STRATEGIES; MARKET;
IMPLEMENTATION
AB In recent years, China has been ambitious in investing and developing renewable energy technologies, aiming to enhance its energy security, mitigate its energy-related CO2 emissions and develop renewable energy industry. The 12th Five Year Plan (2011-2015) has set clear targets on installed capacities of different renewable energy technologies. This study aimed to assess the possible contribution of 12th Five Year Plan for China's future energy system and identify factors that might influence its impacts. First, current status of renewable energy development in China has been reviewed. Then several energy scenarios have been developed in an hourly simulation using an energy system analysis tool EnergyPLAN. It was identified that existing grid bottleneck would greatly reduce the potential contribution of renewable installations in terms of share of renewable electricity generation, share of non-fossil fuels in primary energy and system CO2 emissions. In contrast, improving technical performance of renewable energy technologies and sectoral energy efficiency plays an important role in increasing the share of renewables and promoting China's energy system transition. Finally, some policy suggestions were drawn to facilitate a better implementation of the renewable energy plan. Published by Elsevier Ltd.
C1 [Hong, Lixuan; Zhou, Nan; Fridley, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Raczkowski, Chris] Azure Int, Beijing 100027, Peoples R China.
RP Hong, LX (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM lixuanhong@lbl.gov
NR 83
TC 20
Z9 22
U1 1
U2 36
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0301-4215
EI 1873-6777
J9 ENERG POLICY
JI Energy Policy
PD NOV
PY 2013
VL 62
BP 1533
EP 1543
DI 10.1016/j.enpol.2013.07.110
PG 11
WC Energy & Fuels; Environmental Sciences; Environmental Studies
SC Energy & Fuels; Environmental Sciences & Ecology
GA 249IG
UT WOS:000326770300157
ER
PT J
AU Wlodawer, A
Minor, W
Dauter, Z
Jaskolski, M
AF Wlodawer, Alexander
Minor, Wladek
Dauter, Zbigniew
Jaskolski, Mariusz
TI Protein crystallography for aspiring crystallographers or how to avoid
pitfalls and traps in macromolecular structure determination
SO FEBS JOURNAL
LA English
DT Review
DE data collection and processing; electron density maps; protein
crystallography; structure refinement; structure solution; structure
quality; structure validation
ID HIGH-RESOLUTION STRUCTURE; X-RAY-STRUCTURE; NATIVE BIOLOGICAL
MACROMOLECULES; PANCREATIC TRYPSIN-INHIBITOR; NERVE GROWTH-FACTOR;
CRYSTAL-STRUCTURE; ANOMALOUS DIFFRACTION; MOLECULAR-REPLACEMENT;
3-DIMENSIONAL STRUCTURE; SYNCHROTRON-RADIATION
AB The number of macromolecular structures deposited in the Protein Data Bank now approaches 100000, with the vast majority of them determined by crystallographic methods. Thousands of papers describing such structures have been published in the scientific literature, and 20 Nobel Prizes in chemistry or medicine have been awarded for discoveries based on macromolecular crystallography. New hardware and software tools have made crystallography appear to be an almost routine (but still far from being analytical) technique and many structures are now being determined by scientists with very limited experience in the practical aspects of the field. However, this apparent ease is sometimes illusory and proper procedures need to be followed to maintain high standards of structure quality. In addition, many noncrystallographers may have problems with the critical evaluation and interpretation of structural results published in the scientific literature. The present review provides an outline of the technical aspects of crystallography for less experienced practitioners, as well as information that might be useful for users of macromolecular structures, aiming to show them how to interpret (but not overinterpret) the information present in the coordinate files and in their description. A discussion of the extent of information that can be gleaned from the atomic coordinates of structures solved at different resolution is provided, as well as problems and pitfalls encountered in structure determination and interpretation.
C1 [Wlodawer, Alexander] NCI, Prot Struct Sect, Macromol Crystallog Lab, Frederick, MD 21702 USA.
[Minor, Wladek] Univ Virginia, Dept Mol Physiol & Biol Phys, Charlottesville, VA USA.
[Minor, Wladek] Midwest Ctr Struct Genom, Lemont, IL USA.
[Minor, Wladek] New York Struct Genom Consortium, New York, NY USA.
[Minor, Wladek] Ctr Struct Genom Infect Dis, Bethesda, MD USA.
[Dauter, Zbigniew] NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne Natl Lab, Chicago, IL USA.
[Jaskolski, Mariusz] Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, PL-60780 Poznan, Poland.
[Jaskolski, Mariusz] Polish Acad Sci, Inst Bioorgan Chem, Ctr Biocrystallog Res, Poznan, Poland.
RP Wlodawer, A (reprint author), NCI, Prot Struct Sect, Macromol Crystallog Lab, Frederick, MD 21702 USA.
EM wlodawer@nih.gov
RI Minor, Wladek/F-3096-2014;
OI Minor, Wladek/0000-0001-7075-7090
FU NIH, National Cancer Institute, Center for Cancer Research; Federal
funds from the National Institute of Allergy and Infectious Diseases,
National Institutes of Health, Department of Health and Human Services
[HHSN272201200026C]; [GM053163]; [GM094585]; [GM094662]; [GM093342]
FX We thank Dr Jerry Alexandratos for assistance with the preparation of
the figures and Milosz Ruszkowski for the photograph in Fig. 1A.
Original work in the laboratories of A. W. and Z.D. was supported by the
Intramural Research Program of the NIH, National Cancer Institute,
Center for Cancer Research. W. M. was supported by grants GM053163,
GM094585, GM094662 and GM093342, and was funded in part with Federal
funds from the National Institute of Allergy and Infectious Diseases,
National Institutes of Health, Department of Health and Human Services,
under Contract No. HHSN272201200026C.
NR 136
TC 27
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U1 3
U2 49
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 1742-464X
EI 1742-4658
J9 FEBS J
JI FEBS J.
PD NOV
PY 2013
VL 280
IS 22
BP 5705
EP 5736
DI 10.1111/febs.12495
PG 32
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 254AA
UT WOS:000327130900013
PM 24034303
ER
PT J
AU Rennie, E
Heazlewood, J
Stonebloom, S
Chiu, TY
Christiansen, K
Miles, G
Dupree, P
Scheller, H
AF Rennie, Emilie
Heazlewood, Joshua
Stonebloom, Solomon
Chiu, Tsan-Yu
Christiansen, Katy
Miles, Godfrey
Dupree, Paul
Scheller, Henrik
TI Identification of a GlcA transferase involved in biosynthesis of
glycosyl inositol phosphorylceramide sphingolipids in plants
SO GLYCOBIOLOGY
LA English
DT Meeting Abstract
CT Annual Conference of the Society-for-Glycobiology
CY NOV 17-20, 2013
CL St Petersburg, FL
SP Soc Glycobiol
C1 [Rennie, Emilie; Heazlewood, Joshua; Chiu, Tsan-Yu; Christiansen, Katy; Scheller, Henrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.
[Stonebloom, Solomon] Univ Copenhagen, DK-1168 Copenhagen, Denmark.
[Miles, Godfrey; Dupree, Paul] Univ Cambridge, Cambridge CB2 1TN, England.
RI Scheller, Henrik/A-8106-2008
OI Scheller, Henrik/0000-0002-6702-3560
NR 0
TC 0
Z9 0
U1 0
U2 3
PU OXFORD UNIV PRESS INC
PI CARY
PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA
SN 0959-6658
EI 1460-2423
J9 GLYCOBIOLOGY
JI Glycobiology
PD NOV
PY 2013
VL 23
IS 11
MA 11
BP 1333
EP 1333
PG 1
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 251YY
UT WOS:000326972400021
ER
PT J
AU Kronewitter, SR
Slysz, GW
LaMarche, BL
Hagler, CD
Harris, MY
Monroe, ME
Crowell, KL
Polyukh, CA
Zhao, R
Marginean, I
Fillmore, TL
Carlson, TS
Camp, DG
Payne, SH
Moore, RJ
Adkins, JN
Anderson, GA
Rodland, KD
Smith, RD
AF Kronewitter, Scott R.
Slysz, Gordon W.
LaMarche, Brian L.
Hagler, Clay D.
Harris, Myanna Y.
Monroe, Matthew E.
Crowell, Kevin L.
Polyukh, Christina A.
Zhao, Rui
Marginean, Ioan
Fillmore, Thomas L.
Carlson, Timothy S.
Camp, David G., II
Payne, Samuel H.
Moore, Ronald J.
Adkins, Joshua N.
Anderson, Gordon A.
Rodland, Karin D.
Smith, Richard D.
TI High-Throughput Human Serum N-Glycan Profiling with GlycoGrid 4D
Visualization and Automated Annotation Using GlyQ-IQ Multi-Core Software
and PNNL Institutional Computing
SO GLYCOBIOLOGY
LA English
DT Meeting Abstract
CT Annual Conference of the Society-for-Glycobiology
CY NOV 17-20, 2013
CL St Petersburg, FL
SP Soc Glycobiol
C1 [Kronewitter, Scott R.; Slysz, Gordon W.; LaMarche, Brian L.; Hagler, Clay D.; Harris, Myanna Y.; Monroe, Matthew E.; Crowell, Kevin L.; Polyukh, Christina A.; Zhao, Rui; Marginean, Ioan; Fillmore, Thomas L.; Carlson, Timothy S.; Camp, David G., II; Payne, Samuel H.; Moore, Ronald J.; Adkins, Joshua N.; Anderson, Gordon A.; Rodland, Karin D.; Smith, Richard D.] Pacific NW Natl Lab, Richland, WA 99352 USA.
RI Smith, Richard/J-3664-2012
OI Smith, Richard/0000-0002-2381-2349
NR 0
TC 0
Z9 0
U1 0
U2 4
PU OXFORD UNIV PRESS INC
PI CARY
PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA
SN 0959-6658
EI 1460-2423
J9 GLYCOBIOLOGY
JI Glycobiology
PD NOV
PY 2013
VL 23
IS 11
MA 74
BP 1356
EP 1356
PG 1
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 251YY
UT WOS:000326972400084
ER
PT J
AU Harvey, B
Rana, NA
Wang, T
Li, HL
Haltiwanger, RS
AF Harvey, Beth
Rana, Nadia A.
Wang, Tong
Li, Huilin
Haltiwanger, Robert S.
TI Investigating the Effects of Fringe Modification on Drosophila Notch
Structure and Function
SO GLYCOBIOLOGY
LA English
DT Meeting Abstract
CT Annual Conference of the Society-for-Glycobiology
CY NOV 17-20, 2013
CL St Petersburg, FL
SP Soc Glycobiol
C1 [Harvey, Beth; Rana, Nadia A.; Haltiwanger, Robert S.] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA.
[Wang, Tong; Li, Huilin] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.
NR 0
TC 0
Z9 0
U1 0
U2 2
PU OXFORD UNIV PRESS INC
PI CARY
PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA
SN 0959-6658
EI 1460-2423
J9 GLYCOBIOLOGY
JI Glycobiology
PD NOV
PY 2013
VL 23
IS 11
MA 132
BP 1375
EP 1375
PG 1
WC Biochemistry & Molecular Biology
SC Biochemistry & Molecular Biology
GA 251YY
UT WOS:000326972400142
ER
PT J
AU Jeanne, P
Guglielmi, Y
Cappa, F
AF Jeanne, Pierre
Guglielmi, Yves
Cappa, Frederic
TI Hydromechanical Heterogeneities of a Mature Fault Zone: Impacts on Fluid
Flow
SO GROUND WATER
LA English
DT Article
ID CARBONATE RESERVOIR; DAMAGE ZONE; SLIP; PERMEABILITY; DISPLACEMENT;
ROCKS; FIELD; ARCHITECTURE; EARTHQUAKE; PRESSURE
AB lec In this paper, fluid flow is examined for a mature strike-slip fault zone with anisotropic permeability and internal heterogeneity. The hydraulic properties of the fault zone were first characterized in situ by microgeophysical (V-P and sigma(c)) and rock-quality measurements (Q-value) performed along a 50-m long profile perpendicular to the fault zone. Then, the local hydrogeological context of the fault was modified to conduct a water-injection test. The resulting fluid pressures and flow rates through the different fault-zone compartments were then analyzed with a two-phase fluid-flow numerical simulation. Fault hydraulic properties estimated from the injection test signals were compa